Autoignition response of n-butanol and its blend with primary reference fuel constituents of gasoline.
Abstract
We study the influence of blending n-butanol on the ignition delay times of n-heptane and iso-octane, the primary reference fuels for gasoline. The ignition delay times are measured using a rapid compression machine, with an emphasis on the low-to-intermediate temperature conditions. The experiments are conducted at equivalence ratios of 0.4 and 1.0, for a compressed pressure of 20 bar, with the temperatures at the end of compression ranging from 613 K to 979 K. The effect of n-butanol addition on the development of the two-stage ignition characteristics for the two primary reference fuels is also examined. The experimental results are compared to predictions obtained using a detailed chemical kinetic mechanism, which has been obtained by a systematic merger of previously reported base models for the combustion of the individual fuel constituents. In conclusion, a sensitivity analysis on the base, and the merged models, is also performed to understand the dependence of autoignition delay times on the model parameters.
- Authors:
-
- Univ. of Connecticut, Storrs, CT (United States)
- Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
- Publication Date:
- Research Org.:
- Energy Frontier Research Centers (EFRC) (United States). Combustion Energy Frontier Research Center (CEFRC); Lawrence Livermore National Lab., Livermore, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1281683
- Alternate Identifier(s):
- OSTI ID: 1246735
- Report Number(s):
- LLNL-JRNL-591474
Journal ID: ISSN 0010-2180
- Grant/Contract Number:
- AC52-07NA27344; SC0001198
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Combustion and Flame
- Additional Journal Information:
- Journal Volume: 162; Journal Issue: 6; Journal ID: ISSN 0010-2180
- Publisher:
- Elsevier
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 30 DIRECT ENERGY CONVERSION; 37 INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY; n-butanol; iso-octane; n-heptane; autoignition; fuel blend combustion
Citation Formats
Kumar, Kamal, Zhang, Yu, Sung, Chi -Jen, and Pitz, William J. Autoignition response of n-butanol and its blend with primary reference fuel constituents of gasoline.. United States: N. p., 2015.
Web. doi:10.1016/j.combustflame.2015.02.014.
Kumar, Kamal, Zhang, Yu, Sung, Chi -Jen, & Pitz, William J. Autoignition response of n-butanol and its blend with primary reference fuel constituents of gasoline.. United States. https://doi.org/10.1016/j.combustflame.2015.02.014
Kumar, Kamal, Zhang, Yu, Sung, Chi -Jen, and Pitz, William J. Mon .
"Autoignition response of n-butanol and its blend with primary reference fuel constituents of gasoline.". United States. https://doi.org/10.1016/j.combustflame.2015.02.014. https://www.osti.gov/servlets/purl/1281683.
@article{osti_1281683,
title = {Autoignition response of n-butanol and its blend with primary reference fuel constituents of gasoline.},
author = {Kumar, Kamal and Zhang, Yu and Sung, Chi -Jen and Pitz, William J.},
abstractNote = {We study the influence of blending n-butanol on the ignition delay times of n-heptane and iso-octane, the primary reference fuels for gasoline. The ignition delay times are measured using a rapid compression machine, with an emphasis on the low-to-intermediate temperature conditions. The experiments are conducted at equivalence ratios of 0.4 and 1.0, for a compressed pressure of 20 bar, with the temperatures at the end of compression ranging from 613 K to 979 K. The effect of n-butanol addition on the development of the two-stage ignition characteristics for the two primary reference fuels is also examined. The experimental results are compared to predictions obtained using a detailed chemical kinetic mechanism, which has been obtained by a systematic merger of previously reported base models for the combustion of the individual fuel constituents. In conclusion, a sensitivity analysis on the base, and the merged models, is also performed to understand the dependence of autoignition delay times on the model parameters.},
doi = {10.1016/j.combustflame.2015.02.014},
journal = {Combustion and Flame},
number = 6,
volume = 162,
place = {United States},
year = {Mon Apr 13 00:00:00 EDT 2015},
month = {Mon Apr 13 00:00:00 EDT 2015}
}
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Works referencing / citing this record:
Influences of isomeric butanol addition on anti-knock tendency of primary reference fuel and toluene primary reference fuel gasoline surrogates
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- International Journal of Engine Research