Nonlinear Fano-Resonant Dielectric Metasurfaces
Abstract
Strong nonlinear light matter interaction is highly sought-after for a variety of applications including lasing and all-optical light modulation. Recently, resonant plasmonic structures have been considered promising candidates for enhancing nonlinear optical processes due to their ability to greatly enhance the optical near-field; however, their small mode volumes prevent the inherently large nonlinear susceptibility of the metal from being efficiently exploited. We present an alternative approach that utilizes a Fano-resonant silicon metasurface. The metasurface results in strong near-field enhancement within the volume of the silicon resonator while minimizing two photon absorption. Here, we measure a third harmonic generation enhancement factor of 1.5 105 with respect to an unpatterned silicon film and an absolute conversion efficiency of 1.2 10 6 with a peak pump intensity of 3.2 GW cm 2. The enhanced nonlinearity, combined with a sharp linear transmittance spectrum, results in transmission modulation with a modulation depth of 36%. Finally, the modulation mechanism is studied by pump probe experiments
- Authors:
-
- Vanderbilt Univ., Nashville, TN (United States)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)
- Sponsoring Org.:
- USDOE Office of Science (SC); National Science Foundation (NSF)
- OSTI Identifier:
- 1265873
- Grant/Contract Number:
- AC05-00OR22725; ECCS-1351334; N00014-14-1-0475
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nano Letters
- Additional Journal Information:
- Journal Volume: 15; Journal Issue: 11; Journal ID: ISSN 1530-6984
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Yang, Yuanmu, Wang, Wenyi, Boulesbaa, Abdelaziz, Kravchenko, Ivan I., Briggs, Dayrl P., Puretzky, Alexander, Geohegan, David, and Valentine, Jason. Nonlinear Fano-Resonant Dielectric Metasurfaces. United States: N. p., 2015.
Web. doi:10.1021/acs.nanolett.5b02802.
Yang, Yuanmu, Wang, Wenyi, Boulesbaa, Abdelaziz, Kravchenko, Ivan I., Briggs, Dayrl P., Puretzky, Alexander, Geohegan, David, & Valentine, Jason. Nonlinear Fano-Resonant Dielectric Metasurfaces. United States. https://doi.org/10.1021/acs.nanolett.5b02802
Yang, Yuanmu, Wang, Wenyi, Boulesbaa, Abdelaziz, Kravchenko, Ivan I., Briggs, Dayrl P., Puretzky, Alexander, Geohegan, David, and Valentine, Jason. Mon .
"Nonlinear Fano-Resonant Dielectric Metasurfaces". United States. https://doi.org/10.1021/acs.nanolett.5b02802. https://www.osti.gov/servlets/purl/1265873.
@article{osti_1265873,
title = {Nonlinear Fano-Resonant Dielectric Metasurfaces},
author = {Yang, Yuanmu and Wang, Wenyi and Boulesbaa, Abdelaziz and Kravchenko, Ivan I. and Briggs, Dayrl P. and Puretzky, Alexander and Geohegan, David and Valentine, Jason},
abstractNote = {Strong nonlinear light matter interaction is highly sought-after for a variety of applications including lasing and all-optical light modulation. Recently, resonant plasmonic structures have been considered promising candidates for enhancing nonlinear optical processes due to their ability to greatly enhance the optical near-field; however, their small mode volumes prevent the inherently large nonlinear susceptibility of the metal from being efficiently exploited. We present an alternative approach that utilizes a Fano-resonant silicon metasurface. The metasurface results in strong near-field enhancement within the volume of the silicon resonator while minimizing two photon absorption. Here, we measure a third harmonic generation enhancement factor of 1.5 105 with respect to an unpatterned silicon film and an absolute conversion efficiency of 1.2 10 6 with a peak pump intensity of 3.2 GW cm 2. The enhanced nonlinearity, combined with a sharp linear transmittance spectrum, results in transmission modulation with a modulation depth of 36%. Finally, the modulation mechanism is studied by pump probe experiments},
doi = {10.1021/acs.nanolett.5b02802},
journal = {Nano Letters},
number = 11,
volume = 15,
place = {United States},
year = {Mon Oct 26 00:00:00 EDT 2015},
month = {Mon Oct 26 00:00:00 EDT 2015}
}
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Giant Electro-Optical Effect through Electrostriction in a Nanomechanical Metamaterial
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Generalized Optical Signal Processing Based on Multi-Operator Metasurfaces Synthesized by Susceptibility Tensors
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Enhanced Nonlinear Yield from Barium Titanate Metasurface Down to the Near Ultraviolet
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Fano Resonance in a Subwavelength Mie-based Metamolecule with Split Ring Resonator
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Thermal tuning capabilities of semiconductor metasurface resonators
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Accelerating Light with Metasurfaces
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All-dielectric metasurfaces with trapped modes: group-theoretical description
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Generating scattering dark states through the Fano interference between excitons and an individual silicon nanogroove
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Boosting third-harmonic generation by a mirror-enhanced anapole resonator
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Ultrafast control of third-order optical nonlinearities in fishnet metamaterials
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Giant field enhancement in high-index dielectric subwavelength particles
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Metasurface-assisted phase-matching-free second harmonic generation in lithium niobate waveguides
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Silicon metasurfaces for third harmonic geometric phase manipulation and multiplexed holography
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Tunable nanophotonics enabled by chalcogenide phase-change materials
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