Atomic-scale electronic structure of the cuprate d-symmetry form factor density wave state
Abstract
Research on high-temperature superconducting cuprates is at present focused on identifying the relationship between the classic ‘pseudogap’ phenomenon1, 2 and the more recently investigated density wave state3–13. This state is generally characterized by a wavevector Q parallel to the planar Cu–O–Cu bonds 4–13 along with a predominantly d-symmetry form factor 14–17 (dFF-DW). To identify the microscopic mechanism giving rise to this state 18–30, one must identify the momentum-space states contributing to the dFF-DW spectral weight, determine their particle–hole phase relationship about the Fermi energy, establish whether they exhibit a characteristic energy gap, and understand the evolution of all these phenomena throughout the phase diagram. Here we use energy-resolved sublattice visualization14 of electronic structure and reveal that the characteristic energy of the dFF-DW modulations is actually the ‘pseudogap’ energy Δ1. Moreover, we demonstrate that the dFF-DW modulations at E = –Δ1 (filled states) occur with relative phase π compared to those at E = Δ1 (empty states). Lastly, we show that the conventionally defined dFF-DW Q corresponds to scattering between the ‘hot frontier’ regions of momentum-space beyond which Bogoliubov quasiparticles cease to exist30–32. These data indicate that the cuprate dFF-DW state involves particle–hole interactions focused at the pseudogap energy scale andmore »
- Authors:
-
- Brookhaven National Lab. (BNL), Upton, NY (United States)
- Cornell Univ., Ithaca, NY (United States); Univ. of St. Andrews, Scotland (United Kingdom)
- Cornell Univ., Ithaca, NY (United States); Univ. of St. Andrews, Scotland (United Kingdom); Brookhaven National Lab. (BNL), Upton, NY (United States)
- Univ. of St. Andrews, Scotland (United Kingdom); Max-Planck Institute for Chemical Physics of Solids, Dresden (Germany)
- Institute of Advanced Industrial Science and Technology, Ibaraki (Japan)
- Univ. of Tokyo, Tokyo (Japan)
- Cornell Univ., Ithaca, NY (United States); Binghamton Univ., Binghamton, NY (United States)
- Cornell Univ., Ithaca, NY (United States)
- Harvard Univ., Cambridge, MA (United States); Perimeter Institute for Theoretical Physics, Waterloo, ON (Canada)
- Publication Date:
- Research Org.:
- Brookhaven National Lab. (BNL), Upton, NY (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1246796
- Report Number(s):
- BNL-111972-2016-JA
Journal ID: ISSN 1745-2473; R&D Project: PO016; PM007; KC0202020; KC0201010
- Grant/Contract Number:
- SC00112704
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Physics
- Additional Journal Information:
- Journal Volume: 12; Journal Issue: 2; Journal ID: ISSN 1745-2473
- Publisher:
- Nature Publishing Group (NPG)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; electronic properties and materials; superconducting properties and materials
Citation Formats
M. H. Hamidian, Kim, Chung Koo, Edkins, S. D., Davis, J. C., Mackenzie, A. P., Eisaki, H., Uchida, S., Lawler, M. J., Kim, E. -A., Sachdev, S., and Fujita, K. Atomic-scale electronic structure of the cuprate d-symmetry form factor density wave state. United States: N. p., 2015.
Web. doi:10.1038/NPHYS3519.
M. H. Hamidian, Kim, Chung Koo, Edkins, S. D., Davis, J. C., Mackenzie, A. P., Eisaki, H., Uchida, S., Lawler, M. J., Kim, E. -A., Sachdev, S., & Fujita, K. Atomic-scale electronic structure of the cuprate d-symmetry form factor density wave state. United States. https://doi.org/10.1038/NPHYS3519
M. H. Hamidian, Kim, Chung Koo, Edkins, S. D., Davis, J. C., Mackenzie, A. P., Eisaki, H., Uchida, S., Lawler, M. J., Kim, E. -A., Sachdev, S., and Fujita, K. Mon .
"Atomic-scale electronic structure of the cuprate d-symmetry form factor density wave state". United States. https://doi.org/10.1038/NPHYS3519. https://www.osti.gov/servlets/purl/1246796.
@article{osti_1246796,
title = {Atomic-scale electronic structure of the cuprate d-symmetry form factor density wave state},
author = {M. H. Hamidian and Kim, Chung Koo and Edkins, S. D. and Davis, J. C. and Mackenzie, A. P. and Eisaki, H. and Uchida, S. and Lawler, M. J. and Kim, E. -A. and Sachdev, S. and Fujita, K.},
abstractNote = {Research on high-temperature superconducting cuprates is at present focused on identifying the relationship between the classic ‘pseudogap’ phenomenon1, 2 and the more recently investigated density wave state3–13. This state is generally characterized by a wavevector Q parallel to the planar Cu–O–Cu bonds 4–13 along with a predominantly d-symmetry form factor 14–17 (dFF-DW). To identify the microscopic mechanism giving rise to this state 18–30, one must identify the momentum-space states contributing to the dFF-DW spectral weight, determine their particle–hole phase relationship about the Fermi energy, establish whether they exhibit a characteristic energy gap, and understand the evolution of all these phenomena throughout the phase diagram. Here we use energy-resolved sublattice visualization14 of electronic structure and reveal that the characteristic energy of the dFF-DW modulations is actually the ‘pseudogap’ energy Δ1. Moreover, we demonstrate that the dFF-DW modulations at E = –Δ1 (filled states) occur with relative phase π compared to those at E = Δ1 (empty states). Lastly, we show that the conventionally defined dFF-DW Q corresponds to scattering between the ‘hot frontier’ regions of momentum-space beyond which Bogoliubov quasiparticles cease to exist30–32. These data indicate that the cuprate dFF-DW state involves particle–hole interactions focused at the pseudogap energy scale and between the four pairs of ‘hot frontier’ regions in momentum space where the pseudogap opens.},
doi = {10.1038/NPHYS3519},
journal = {Nature Physics},
number = 2,
volume = 12,
place = {United States},
year = {Mon Oct 26 00:00:00 EDT 2015},
month = {Mon Oct 26 00:00:00 EDT 2015}
}
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