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Title: Big Data and Deep data in scanning and electron microscopies: functionality from multidimensional data sets

Abstract

The development of electron, and scanning probe microscopies in the second half of the twentieth century have produced spectacular images of internal structure and composition of matter with, at nanometer, molecular, and atomic resolution. Largely, this progress was enabled by computer-assisted methods of microscope operation, data acquisition and analysis. The progress in imaging technologies in the beginning of the twenty first century has opened the proverbial floodgates of high-veracity information on structure and functionality. High resolution imaging now allows information on atomic positions with picometer precision, allowing for quantitative measurements of individual bond length and angles. Functional imaging often leads to multidimensional data sets containing partial or full information on properties of interest, acquired as a function of multiple parameters (time, temperature, or other external stimuli). Here, we review several recent applications of the big and deep data analysis methods to visualize, compress, and translate this data into physically and chemically relevant information from imaging data.

Authors:
 [1];  [1];  [1];  [1];  [2];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1]
  1. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  2. Seoul National Univ. (Korea, Republic of)
Publication Date:
Research Org.:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1214489
Grant/Contract Number:  
AC05-00OR22725
Resource Type:
Accepted Manuscript
Journal Name:
Advanced Structural and Chemical Imaging
Additional Journal Information:
Journal Volume: 1; Journal Issue: 6; Journal ID: ISSN 2198-0926
Publisher:
Springer
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; 42 ENGINEERING

Citation Formats

Belianinov, Alex, Vasudevan, Rama K, Strelcov, Evgheni, Steed, Chad A, Yang, Sang Mo, Tselev, Alexander, Jesse, Stephen, Biegalski, Michael D, Shipman, Galen M, Symons, Christopher T, Borisevich, Albina Y, Archibald, Richard K, and Kalinin, Sergei. Big Data and Deep data in scanning and electron microscopies: functionality from multidimensional data sets. United States: N. p., 2015. Web. doi:10.1186/s40679-015-0006-6.
Belianinov, Alex, Vasudevan, Rama K, Strelcov, Evgheni, Steed, Chad A, Yang, Sang Mo, Tselev, Alexander, Jesse, Stephen, Biegalski, Michael D, Shipman, Galen M, Symons, Christopher T, Borisevich, Albina Y, Archibald, Richard K, & Kalinin, Sergei. Big Data and Deep data in scanning and electron microscopies: functionality from multidimensional data sets. United States. https://doi.org/10.1186/s40679-015-0006-6
Belianinov, Alex, Vasudevan, Rama K, Strelcov, Evgheni, Steed, Chad A, Yang, Sang Mo, Tselev, Alexander, Jesse, Stephen, Biegalski, Michael D, Shipman, Galen M, Symons, Christopher T, Borisevich, Albina Y, Archibald, Richard K, and Kalinin, Sergei. Wed . "Big Data and Deep data in scanning and electron microscopies: functionality from multidimensional data sets". United States. https://doi.org/10.1186/s40679-015-0006-6. https://www.osti.gov/servlets/purl/1214489.
@article{osti_1214489,
title = {Big Data and Deep data in scanning and electron microscopies: functionality from multidimensional data sets},
author = {Belianinov, Alex and Vasudevan, Rama K and Strelcov, Evgheni and Steed, Chad A and Yang, Sang Mo and Tselev, Alexander and Jesse, Stephen and Biegalski, Michael D and Shipman, Galen M and Symons, Christopher T and Borisevich, Albina Y and Archibald, Richard K and Kalinin, Sergei},
abstractNote = {The development of electron, and scanning probe microscopies in the second half of the twentieth century have produced spectacular images of internal structure and composition of matter with, at nanometer, molecular, and atomic resolution. Largely, this progress was enabled by computer-assisted methods of microscope operation, data acquisition and analysis. The progress in imaging technologies in the beginning of the twenty first century has opened the proverbial floodgates of high-veracity information on structure and functionality. High resolution imaging now allows information on atomic positions with picometer precision, allowing for quantitative measurements of individual bond length and angles. Functional imaging often leads to multidimensional data sets containing partial or full information on properties of interest, acquired as a function of multiple parameters (time, temperature, or other external stimuli). Here, we review several recent applications of the big and deep data analysis methods to visualize, compress, and translate this data into physically and chemically relevant information from imaging data.},
doi = {10.1186/s40679-015-0006-6},
journal = {Advanced Structural and Chemical Imaging},
number = 6,
volume = 1,
place = {United States},
year = {Wed May 13 00:00:00 EDT 2015},
month = {Wed May 13 00:00:00 EDT 2015}
}

Works referenced in this record:

A simple, combinatorial algorithm for solving SDD systems in nearly-linear time
conference, January 2013

  • Kelner, Jonathan A.; Orecchia, Lorenzo; Sidford, Aaron
  • Proceedings of the 45th annual ACM symposium on Symposium on theory of computing - STOC '13
  • DOI: 10.1145/2488608.2488724

Improved Nanotopography Sensing via Temperature Control of a Heated Atomic Force Microscope Cantilever
journal, November 2011


Chemistry and electronic structure of iron-based superconductors
journal, August 2011


Current imaging tunneling spectroscopy of metallic deposits on silicon
journal, July 1992


Spatially resolved mapping of disorder type and distribution in random systems using artificial neural network recognition
journal, July 2011


Local probing of relaxation time distributions in ferroelectric polymer nanomesas: Time-resolved piezoresponse force spectroscopy and spectroscopic imaging
journal, June 2008

  • Rodriguez, Brian J.; Jesse, Stephen; Kim, Jihee
  • Applied Physics Letters, Vol. 92, Issue 23
  • DOI: 10.1063/1.2942390

Distilling Free-Form Natural Laws from Experimental Data
journal, April 2009


Nanoscale Control of Phase Variants in Strain-Engineered BiFeO 3
journal, August 2011

  • Vasudevan, Rama K.; Liu, Yunya; Li, Jiangyu
  • Nano Letters, Vol. 11, Issue 8
  • DOI: 10.1021/nl201719w

Parameter Space Compression Underlies Emergent Theories and Predictive Models
journal, October 2013


Nano-chemistry and scanning probe nanolithographies
journal, January 2006

  • Garcia, Ricardo; Martinez, Ramses V.; Martinez, Javier
  • Chem. Soc. Rev., Vol. 35, Issue 1
  • DOI: 10.1039/B501599P

Bayes' Theorem in the 21st Century
journal, June 2013


Direct Mapping of Ion Diffusion Times on LiCoO2 Surfaces with Nanometer Resolution
journal, January 2011

  • Guo, S.; Jesse, S.; Kalnaus, S.
  • Journal of The Electrochemical Society, Vol. 158, Issue 8
  • DOI: 10.1149/1.3604759

7 × 7 Reconstruction on Si(111) Resolved in Real Space
journal, January 1983


Direct evidence of mesoscopic dynamic heterogeneities at the surfaces of ergodic ferroelectric relaxors
journal, February 2010


Unraveling Deterministic Mesoscopic Polarization Switching Mechanisms: Spatially Resolved Studies of a Tilt Grain Boundary in Bismuth Ferrite
journal, July 2009

  • Rodriguez, Brian J.; Choudhury, Samrat; Chu, Y. H.
  • Advanced Functional Materials, Vol. 19, Issue 13
  • DOI: 10.1002/adfm.200900100

Collective dynamics underpins Rayleigh behavior in disordered polycrystalline ferroelectrics
journal, April 2010

  • Bintachitt, P.; Jesse, S.; Damjanovic, D.
  • Proceedings of the National Academy of Sciences, Vol. 107, Issue 16
  • DOI: 10.1073/pnas.0913172107

Watching domains grow: In-situ studies of polarization switching by combined scanning probe and scanning transmission electron microscopy
journal, September 2011

  • Chang, Hyejung; Kalinin, Sergei V.; Yang, Seungyeul
  • Journal of Applied Physics, Vol. 110, Issue 5
  • DOI: 10.1063/1.3623779

Complete information acquisition in dynamic force microscopy
journal, March 2015

  • Belianinov, Alexei; Kalinin, Sergei V.; Jesse, Stephen
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms7550

Controlled mechnical modification of manganite surface with nanoscale resolution
journal, November 2014


Effect of Doping on Surface Reactivity and Conduction Mechanism in Samarium-Doped Ceria Thin Films
journal, November 2014

  • Yang, Nan; Belianinov, Alex; Strelcov, Evgheni
  • ACS Nano, Vol. 8, Issue 12
  • DOI: 10.1021/nn505345c

Current understanding and applications of the RHEED intensity oscillation technique
journal, February 1987


Mapping piezoelectric nonlinearity in the Rayleigh regime using band excitation piezoresponse force microscopy
journal, May 2011

  • Griggio, F.; Jesse, S.; Kumar, A.
  • Applied Physics Letters, Vol. 98, Issue 21
  • DOI: 10.1063/1.3593138

Joint Bayesian Endmember Extraction and Linear Unmixing for Hyperspectral Imagery
journal, November 2009

  • Dobigeon, N.; Moussaoui, S.; Coulon, M.
  • IEEE Transactions on Signal Processing, Vol. 57, Issue 11
  • DOI: 10.1109/TSP.2009.2025797

Theory of orientational glasses models, concepts, simulations
journal, December 1992


Real Space Mapping of Li-Ion Transport in Amorphous Si Anodes with Nanometer Resolution
journal, September 2010

  • Balke, Nina; Jesse, Stephen; Kim, Yoongu
  • Nano Letters, Vol. 10, Issue 9
  • DOI: 10.1021/nl101439x

Active centers, catalytic behavior, symbiosis and redox properties of MoV(Nb,Ta)TeO ammoxidation catalysts
journal, July 2006

  • Grasselli, Robert K.; Buttrey, Douglas J.; Burrington, James D.
  • Topics in Catalysis, Vol. 38, Issue 1-3
  • DOI: 10.1007/s11244-006-0066-x

Scanning force microscopy of domain structure in ferroelectric thin films: imaging and control
journal, September 1997


Domain Dynamics During Ferroelectric Switching
journal, November 2011


Nanoscale mapping of ion diffusion in a lithium-ion battery cathode
journal, August 2010


Double-Layer Mediated Electromechanical Response of Amyloid Fibrils in Liquid Environment
journal, January 2010

  • Nikiforov, M. P.; Thompson, G. L.; Reukov, V. V.
  • ACS Nano, Vol. 4, Issue 2
  • DOI: 10.1021/nn901127k

Quantifying the early stages of plasticity through nanoscale experiments and simulations
journal, March 2003


The band excitation method in scanning probe microscopy for rapid mapping of energy dissipation on the nanoscale
journal, September 2007


Spatially resolved probing of Preisach density in polycrystalline ferroelectric thin films
journal, October 2010

  • Guo, S.; Ovchinnikov, O. S.; Curtis, M. E.
  • Journal of Applied Physics, Vol. 108, Issue 8
  • DOI: 10.1063/1.3493738

A Preisach model with a temperature and time-dependent remanence maximum
journal, April 1997

  • Mitchler, P. D.; Roshko, R. M.; Dahlberg, E. Dan
  • Journal of Applied Physics, Vol. 81, Issue 8
  • DOI: 10.1063/1.364473

Angular brushing of extended parallel coordinates
conference, January 2002

  • Hauser, H.; Ledermann, F.; Doleisch, H.
  • InfoVis 2002. IEEE Symposium on Information Visualization, IEEE Symposium on Information Visualization, 2002. INFOVIS 2002.
  • DOI: 10.1109/INFVIS.2002.1173157

Picometre-precision analysis of scanning transmission electron microscopy images of platinum nanocatalysts
journal, June 2014

  • Yankovich, Andrew B.; Berkels, Benjamin; Dahmen, W.
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms5155

Learning Deep Architectures for AI
journal, January 2009

  • Bengio, Y.
  • Foundations and Trends® in Machine Learning, Vol. 2, Issue 1
  • DOI: 10.1561/2200000006

Large field-induced strains in a lead-free piezoelectric material
journal, January 2011

  • Zhang, J. X.; Xiang, B.; He, Q.
  • Nature Nanotechnology, Vol. 6, Issue 2, p. 98-102
  • DOI: 10.1038/nnano.2010.265

Factors Governing Oxygen Reduction in Solid Oxide Fuel Cell Cathodes
journal, October 2004


Resolution theory, and static and frequency-dependent cross-talk in piezoresponse force microscopy
journal, September 2010


Resonance enhancement in piezoresponse force microscopy: Mapping electromechanical activity, contact stiffness, and Q factor
journal, July 2006

  • Jesse, Stephen; Mirman, Boris; Kalinin, Sergei V.
  • Applied Physics Letters, Vol. 89, Issue 2
  • DOI: 10.1063/1.2221496

Deep Data Analysis of Conductive Phenomena on Complex Oxide Interfaces: Physics from Data Mining
journal, May 2014

  • Strelcov, Evgheni; Belianinov, Alexei; Hsieh, Ying-Hui
  • ACS Nano, Vol. 8, Issue 6
  • DOI: 10.1021/nn502029b

Ferroelastic domain wall dynamics in ferroelectric bilayers
journal, September 2010


Probing Local and Global Ferroelectric Phase Stability and Polarization Switching in Ordered Macroporous PZT
journal, February 2011

  • McLachlan, Martyn A.; McComb, David W.; Ryan, Mary P.
  • Advanced Functional Materials, Vol. 21, Issue 5
  • DOI: 10.1002/adfm.201002038

Diffuse phase transitions and random-field-induced domain states of the ‘‘relaxor’’ ferroelectric PbMg 1 / 3 Nb 2 / 3 O 3
journal, February 1992


Spin glasses: Experimental facts, theoretical concepts, and open questions
journal, October 1986


Differentiating 180° and 90° switching of ferroelectric domains with three-dimensional piezoresponse force microscopy
journal, November 2000

  • Roelofs, A.; Böttger, U.; Waser, R.
  • Applied Physics Letters, Vol. 77, Issue 21, p. 3444-3446
  • DOI: 10.1063/1.1328049

Big data in reciprocal space: Sliding fast Fourier transforms for determining periodicity
journal, March 2015

  • Vasudevan, Rama K.; Belianinov, Alex; Gianfrancesco, Anthony G.
  • Applied Physics Letters, Vol. 106, Issue 9
  • DOI: 10.1063/1.4914016

Generalized Preisach model of hysteresis
journal, January 1988

  • Mayergoyz, I. D.; Friedman, G.
  • IEEE Transactions on Magnetics, Vol. 24, Issue 1
  • DOI: 10.1109/20.43892

Subspace clustering for high dimensional data: a review
journal, June 2004

  • Parsons, Lance; Haque, Ehtesham; Liu, Huan
  • ACM SIGKDD Explorations Newsletter, Vol. 6, Issue 1
  • DOI: 10.1145/1007730.1007731

Electromechanical Imaging and Spectroscopy of Ferroelectric and Piezoelectric Materials: State of the Art and Prospects for the Future
journal, August 2009


Information foraging.
journal, October 1999


Searching for exotic particles in high-energy physics with deep learning
journal, July 2014

  • Baldi, P.; Sadowski, P.; Whiteson, D.
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms5308

Quantitative mapping of switching behavior in piezoresponse force microscopy
journal, July 2006

  • Jesse, Stephen; Lee, Ho Nyung; Kalinin, Sergei V.
  • Review of Scientific Instruments, Vol. 77, Issue 7
  • DOI: 10.1063/1.2214699

Real space mapping of polarization dynamics and hysteresis loop formation in relaxor-ferroelectric PbMg1/3Nb2/3O3–PbTiO3 solid solutions
journal, August 2010

  • Rodriguez, B. J.; Jesse, S.; Morozovska, A. N.
  • Journal of Applied Physics, Vol. 108, Issue 4
  • DOI: 10.1063/1.3474961

Separation of Non-Negative Mixture of Non-Negative Sources Using a Bayesian Approach and MCMC Sampling
journal, November 2006

  • Moussaoui, S.; Brie, D.; Mohammad-Djafari, A.
  • IEEE Transactions on Signal Processing, Vol. 54, Issue 11
  • DOI: 10.1109/TSP.2006.880310

Scanning Force Microscopy Studies of Domain Structure in B a T i O 3 Single Crystals
journal, April 1997

  • Gruverman, Alexei L.; Hatano, Jun; Tokumoto, Hiroshi
  • Japanese Journal of Applied Physics, Vol. 36, Issue Part 1, No. 4A
  • DOI: 10.1143/JJAP.36.2207

Riemannian Manifold Learning
journal, May 2008

  • Tong Lin,
  • IEEE Transactions on Pattern Analysis and Machine Intelligence, Vol. 30, Issue 5
  • DOI: 10.1109/TPAMI.2007.70735

Switching spectroscopy piezoresponse force microscopy of polycrystalline capacitor structures
journal, January 2009

  • Bintachitt, Patamas; Trolier-McKinstry, Susan; Seal, Katyayani
  • Applied Physics Letters, Vol. 94, Issue 4
  • DOI: 10.1063/1.3070543

Ionic field effect and memristive phenomena in single-point ferroelectric domain switching
journal, July 2014

  • Ievlev, Anton V.; Morozovska, Anna N.; Eliseev, Eugene A.
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms5545

Defect-induced asymmetry of local hysteresis loops on BiFeO3 surfaces
journal, October 2009

  • Maksymovych, Peter; Balke, Nina; Jesse, Stephen
  • Journal of Materials Science, Vol. 44, Issue 19
  • DOI: 10.1007/s10853-009-3697-z

Nonlinear Phenomena in Multiferroic Nanocapacitors: Joule Heating and Electromechanical Effects
journal, October 2011

  • Kim, Yunseok; Kumar, Amit; Tselev, Alexander
  • ACS Nano, Vol. 5, Issue 11
  • DOI: 10.1021/nn203342v

Research Update: Spatially resolved mapping of electronic structure on atomic level by multivariate statistical analysis
journal, December 2014

  • Belianinov, Alex; Ganesh, Panchapakesan; Lin, Wenzhi
  • APL Materials, Vol. 2, Issue 12
  • DOI: 10.1063/1.4902996

Mapping bias-induced phase stability and random fields in relaxor ferroelectrics
journal, August 2009

  • Rodriguez, B. J.; Jesse, S.; Bokov, A. A.
  • Applied Physics Letters, Vol. 95, Issue 9
  • DOI: 10.1063/1.3222868

Principal component and spatial correlation analysis of spectroscopic-imaging data in scanning probe microscopy
journal, February 2009


A Global Geometric Framework for Nonlinear Dimensionality Reduction
journal, December 2000


Mapping internal structure of coal by confocal micro-Raman spectroscopy and scanning microwave microscopy
journal, June 2014


Local bias-induced phase transitions
journal, November 2008


Piezoelectric response of nanoscale PbTiO3 in composite PbTiO3−CoFe2O4 epitaxial films
journal, August 2008

  • Tan, Zhuopeng; Roytburd, Alexander L.; Levin, Igor
  • Applied Physics Letters, Vol. 93, Issue 7
  • DOI: 10.1063/1.2969038

Mechanically-Induced Resistive Switching in Ferroelectric Tunnel Junctions
journal, February 2012

  • Lu, H.; Kim, D. J.; Bark, C. -W.
  • Nano Letters, Vol. 12, Issue 12
  • DOI: 10.1021/nl303396n

Insertion Electrode Materials for Rechargeable Lithium Batteries
journal, July 1998


Atomic force microscope cantilevers for combined thermomechanical data writing and reading
journal, February 2001

  • King, William P.; Kenny, Thomas W.; Goodson, Kenneth E.
  • Applied Physics Letters, Vol. 78, Issue 9
  • DOI: 10.1063/1.1351846

Local thermomechanical characterization of phase transitions using band excitation atomic force acoustic microscopy with heated probe
journal, August 2008

  • Jesse, S.; Nikiforov, M. P.; Germinario, L. T.
  • Applied Physics Letters, Vol. 93, Issue 7
  • DOI: 10.1063/1.2965470

A visual analytics agenda
journal, January 2006

  • Thomas, J. J.; Cook, K. A.
  • IEEE Computer Graphics and Applications, Vol. 26, Issue 1
  • DOI: 10.1109/MCG.2006.5

Measuring oxygen reduction/evolution reactions on the nanoscale
journal, August 2011

  • Kumar, Amit; Ciucci, Francesco; Morozovska, Anna N.
  • Nature Chemistry, Vol. 3, Issue 9
  • DOI: 10.1038/nchem.1112

Dual-frequency resonance-tracking atomic force microscopy
journal, October 2007


Nanometer-scale flow of molten polyethylene from a heated atomic force microscope tip
journal, May 2012


Domain pinning near a single-grain boundary in tetragonal and rhombohedral lead zirconate titanate films
journal, April 2015


Mapping Irreversible Electrochemical Processes on the Nanoscale: Ionic Phenomena in Li Ion Conductive Glass Ceramics
journal, October 2011

  • Arruda, Thomas M.; Kumar, Amit; Kalinin, Sergei V.
  • Nano Letters, Vol. 11, Issue 10
  • DOI: 10.1021/nl202039v

Silicon Nanowire Transistors with a Channel Width of 4 nm Fabricated by Atomic Force Microscope Nanolithography
journal, November 2008

  • Martinez, J.; Martínez, R. V.; Garcia, R.
  • Nano Letters, Vol. 8, Issue 11
  • DOI: 10.1021/nl801599k

Local measurements of Preisach density in polycrystalline ferroelectric capacitors using piezoresponse force spectroscopy
journal, March 2010

  • Ovchinnikov, O.; Jesse, S.; Guo, S.
  • Applied Physics Letters, Vol. 96, Issue 11
  • DOI: 10.1063/1.3360220

Correlative Multimodal Probing of Ionically-Mediated Electromechanical Phenomena in Simple Oxides
journal, October 2013

  • Kim, Yunseok; Strelcov, Evgheni; Hwang, In Rok
  • Scientific Reports, Vol. 3, Issue 1
  • DOI: 10.1038/srep02924

Disorder Identification in Hysteresis Data: Recognition Analysis of the Random-Bond–Random-Field Ising Model
journal, October 2009


Multidimensional Spectral Hashing
book, January 2012


Direct imaging of the spatial and energy distribution of nucleation centres in ferroelectric materials
journal, February 2008

  • Jesse, Stephen; Rodriguez, Brian J.; Choudhury, Samrat
  • Nature Materials, Vol. 7, Issue 3
  • DOI: 10.1038/nmat2114

Semi-Supervised Linear Spectral Unmixing Using a Hierarchical Bayesian Model for Hyperspectral Imagery
journal, July 2008

  • Dobigeon, Nicolas; Tourneret, Jean-Yves; Chang, Chein-I
  • IEEE Transactions on Signal Processing, Vol. 56, Issue 7
  • DOI: 10.1109/TSP.2008.917851

Extracting physics through deep data analysis
journal, November 2014


Probing Local Ionic Dynamics in Functional Oxides at the Nanoscale
journal, July 2013

  • Strelcov, Evgheni; Kim, Yunseok; Jesse, Stephen
  • Nano Letters, Vol. 13, Issue 8
  • DOI: 10.1021/nl400780d

Consequences of High Adatom Energy during Pulsed Laser Deposition of La 0.7 Sr 0.3 MnO 3
journal, January 2012

  • Boschker, Jos E.; Folven, Erik; Monsen, Åsmund F.
  • Crystal Growth & Design, Vol. 12, Issue 2
  • DOI: 10.1021/cg201461a

Nonlinear Dimensionality Reduction by Locally Linear Embedding
journal, December 2000


Switching spectroscopy piezoresponse force microscopy of ferroelectric materials
journal, February 2006

  • Jesse, Stephen; Baddorf, Arthur P.; Kalinin, Sergei V.
  • Applied Physics Letters, Vol. 88, Issue 6
  • DOI: 10.1063/1.2172216

The International Exascale Software Project roadmap
journal, January 2011

  • Dongarra, Jack; Beckman, Pete; Moore, Terry
  • The International Journal of High Performance Computing Applications, Vol. 25, Issue 1
  • DOI: 10.1177/1094342010391989

Spatial distribution of relaxation behavior on the surface of a ferroelectric relaxor in the ergodic phase
journal, October 2009

  • Kalinin, S. V.; Rodriguez, B. J.; Jesse, S.
  • Applied Physics Letters, Vol. 95, Issue 14
  • DOI: 10.1063/1.3242011

The plane with parallel coordinates
journal, August 1985


Temperature-dependent phase transitions in zeptoliter volumes of a complex biological membrane
journal, December 2010


Does freezing in PbMg1/3Nb2/3O3 relaxor manifest itself in nonlinear dielectric susceptibility?
journal, March 1999

  • Tagantsev, A. K.; Glazounov, A. E.
  • Applied Physics Letters, Vol. 74, Issue 13
  • DOI: 10.1063/1.123710

Band excitation in scanning probe microscopy: sines of change
journal, November 2011


Real-space mapping of dynamic phenomena during hysteresis loop measurements: Dynamic switching spectroscopy piezoresponse force microscopy
journal, May 2011

  • Kumar, A.; Ovchinnikov, O. S.; Funakubo, H.
  • Applied Physics Letters, Vol. 98, Issue 20
  • DOI: 10.1063/1.3590919

Big data visual analytics for exploratory earth system simulation analysis
journal, December 2013


Mechanical Control of Electroresistive Switching
journal, August 2013

  • Kim, Yunseok; Kelly, Simon J.; Morozovska, Anna
  • Nano Letters, Vol. 13, Issue 9
  • DOI: 10.1021/nl401411r

N-FINDR: an algorithm for fast autonomous spectral end-member determination in hyperspectral data
conference, October 1999

  • Winter, Michael E.
  • SPIE's International Symposium on Optical Science, Engineering, and Instrumentation, SPIE Proceedings
  • DOI: 10.1117/12.366289

Laplacian Eigenmaps for Dimensionality Reduction and Data Representation
journal, June 2003


Guided analysis of hurricane trends using statistical processes integrated with interactive parallel coordinates
conference, October 2009

  • Steed, Chad A.; Swan, J. Edward; Jankun-Kelly, T. J.
  • 2009 IEEE Symposium on Visual Analytics Science and Technology
  • DOI: 10.1109/VAST.2009.5332586

Local Conduction at the BiFeO3-CoFe2O4 Tubular Oxide Interface
journal, July 2012

  • Hsieh, Ying-Hui; Liou, Jia-Ming; Huang, Bo-Chao
  • Advanced Materials, Vol. 24, Issue 33, p. 4564-4568
  • DOI: 10.1002/adma.201201929

Mapping chemical and bonding information using multivariate analysis of electron energy-loss spectrum images
journal, October 2006


Rapid multidimensional data acquisition in scanning probe microscopy applied to local polarization dynamics and voltage dependent contact mechanics
journal, September 2008

  • Jesse, Stephen; Maksymovych, Peter; Kalinin, Sergei V.
  • Applied Physics Letters, Vol. 93, Issue 11
  • DOI: 10.1063/1.2980031

Computational modeling of the forward and reverse problems in instrumented sharp indentation
journal, November 2001


Band Excitation in Scanning Probe Microscopy: Recognition and Functional Imaging
journal, April 2014


Decoupling Electrochemical Reaction and Diffusion Processes in Ionically-Conductive Solids on the Nanometer Scale
journal, November 2010

  • Balke, Nina; Jesse, Stephen; Kim, Yoongu
  • ACS Nano, Vol. 4, Issue 12
  • DOI: 10.1021/nn101502x

The future lies in uncertainty
journal, July 2014


Scented Widgets: Improving Navigation Cues with Embedded Visualizations
journal, November 2007

  • Willett, Wesley; Heer, Jeffrey; Agrawala, Maneesh
  • IEEE Transactions on Visualization and Computer Graphics, Vol. 13, Issue 6
  • DOI: 10.1109/TVCG.2007.70589

Nanoscale ferroelectrics: processing, characterization and future trends
journal, July 2006


Morphology Mapping of Phase-Separated Polymer Films Using Nanothermal Analysis
journal, August 2010

  • Nikiforov, M. P.; Gam, S.; Jesse, S.
  • Macromolecules, Vol. 43, Issue 16
  • DOI: 10.1021/ma1011254

Big-Data Reflection High Energy Electron Diffraction Analysis for Understanding Epitaxial Film Growth Processes
journal, October 2014

  • Vasudevan, Rama K.; Tselev, Alexander; Baddorf, Arthur P.
  • ACS Nano, Vol. 8, Issue 10
  • DOI: 10.1021/nn504730n

Recent developments in catalysis using nanostructured materials
journal, March 2009


Robust non-linear dimensionality reduction using successive 1-dimensional Laplacian Eigenmaps
conference, January 2007

  • Gerber, Samuel; Tasdizen, Tolga; Whitaker, Ross
  • Proceedings of the 24th international conference on Machine learning - ICML '07
  • DOI: 10.1145/1273496.1273532

Bulk superconductivity at 14 K in single crystals of Fe 1 + y Te x Se 1 x
journal, March 2009


Spatially Resolved Mapping of Polarization Switching Behavior in Nanoscale Ferroelectrics
journal, January 2008


Machine learning identifies a strong association between warming and reduced primary productivity in an oligotrophic ocean gyre
journal, February 2020

  • D’Alelio, Domenico; Rampone, Salvatore; Cusano, Luigi Maria
  • Scientific Reports, Vol. 10, Issue 1
  • DOI: 10.1038/s41598-020-59989-y

Parallel Coordinates
book, April 2021


Parallel Coordinates
reference-book, January 2016


Probing Local and Global Ferroelectric Phase Stability and Polarization Switching in Ordered Macroporous PZT
journal, February 2011

  • McLachlan, Martyn A.; McComb, David W.; Ryan, Mary P.
  • Advanced Functional Materials, Vol. 21, Issue 5
  • DOI: 10.1002/adfm.201002038

Spatially Resolved Mapping of Polarization Switching Behavior in Nanoscale Ferroelectrics
journal, January 2008


Visual Analytics
book, January 2016


Active centers, catalytic behavior, symbiosis and redox properties of MoV(Nb,Ta)TeO ammoxidation catalysts
journal, July 2006

  • Grasselli, Robert K.; Buttrey, Douglas J.; Burrington, James D.
  • Topics in Catalysis, Vol. 38, Issue 1-3
  • DOI: 10.1007/s11244-006-0066-x

Current understanding and applications of the RHEED intensity oscillation technique
journal, February 1987


Ferroelastic domain wall dynamics in ferroelectric bilayers
journal, September 2010


Extracting physics through deep data analysis
journal, November 2014


GX-Means: A model-based divide and merge algorithm for geospatial image clustering
journal, January 2011


Mapping chemical and bonding information using multivariate analysis of electron energy-loss spectrum images
journal, October 2006


Consequences of High Adatom Energy during Pulsed Laser Deposition of La 0.7 Sr 0.3 MnO 3
journal, January 2012

  • Boschker, Jos E.; Folven, Erik; Monsen, Åsmund F.
  • Crystal Growth & Design, Vol. 12, Issue 2
  • DOI: 10.1021/cg201461a

Factors Governing Oxygen Reduction in Solid Oxide Fuel Cell Cathodes
journal, October 2004


Morphology Mapping of Phase-Separated Polymer Films Using Nanothermal Analysis
journal, August 2010

  • Nikiforov, M. P.; Gam, S.; Jesse, S.
  • Macromolecules, Vol. 43, Issue 16
  • DOI: 10.1021/ma1011254

Real Space Mapping of Li-Ion Transport in Amorphous Si Anodes with Nanometer Resolution
journal, September 2010

  • Balke, Nina; Jesse, Stephen; Kim, Yoongu
  • Nano Letters, Vol. 10, Issue 9
  • DOI: 10.1021/nl101439x

Mapping Irreversible Electrochemical Processes on the Nanoscale: Ionic Phenomena in Li Ion Conductive Glass Ceramics
journal, October 2011

  • Arruda, Thomas M.; Kumar, Amit; Kalinin, Sergei V.
  • Nano Letters, Vol. 11, Issue 10
  • DOI: 10.1021/nl202039v

Mechanically-Induced Resistive Switching in Ferroelectric Tunnel Junctions
journal, February 2012

  • Lu, H.; Kim, D. J.; Bark, C. -W.
  • Nano Letters, Vol. 12, Issue 12
  • DOI: 10.1021/nl303396n

Probing Local Ionic Dynamics in Functional Oxides at the Nanoscale
journal, July 2013

  • Strelcov, Evgheni; Kim, Yunseok; Jesse, Stephen
  • Nano Letters, Vol. 13, Issue 8
  • DOI: 10.1021/nl400780d

Mechanical Control of Electroresistive Switching
journal, August 2013

  • Kim, Yunseok; Kelly, Simon J.; Morozovska, Anna
  • Nano Letters, Vol. 13, Issue 9
  • DOI: 10.1021/nl401411r

Silicon Nanowire Transistors with a Channel Width of 4 nm Fabricated by Atomic Force Microscope Nanolithography
journal, November 2008

  • Martinez, J.; Martínez, R. V.; Garcia, R.
  • Nano Letters, Vol. 8, Issue 11
  • DOI: 10.1021/nl801599k

Double-Layer Mediated Electromechanical Response of Amyloid Fibrils in Liquid Environment
journal, January 2010

  • Nikiforov, M. P.; Thompson, G. L.; Reukov, V. V.
  • ACS Nano, Vol. 4, Issue 2
  • DOI: 10.1021/nn901127k

Measuring oxygen reduction/evolution reactions on the nanoscale
journal, August 2011

  • Kumar, Amit; Ciucci, Francesco; Morozovska, Anna N.
  • Nature Chemistry, Vol. 3, Issue 9
  • DOI: 10.1038/nchem.1112

Nanoscale mapping of ion diffusion in a lithium-ion battery cathode
journal, August 2010


Large field-induced strains in a lead-free piezoelectric material
journal, January 2011

  • Zhang, J. X.; Xiang, B.; He, Q.
  • Nature Nanotechnology, Vol. 6, Issue 2, p. 98-102
  • DOI: 10.1038/nnano.2010.265

Does freezing in PbMg1/3Nb2/3O3 relaxor manifest itself in nonlinear dielectric susceptibility?
journal, March 1999

  • Tagantsev, A. K.; Glazounov, A. E.
  • Applied Physics Letters, Vol. 74, Issue 13
  • DOI: 10.1063/1.123710

Differentiating 180° and 90° switching of ferroelectric domains with three-dimensional piezoresponse force microscopy
journal, November 2000

  • Roelofs, A.; Böttger, U.; Waser, R.
  • Applied Physics Letters, Vol. 77, Issue 21, p. 3444-3446
  • DOI: 10.1063/1.1328049

Atomic force microscope cantilevers for combined thermomechanical data writing and reading
journal, February 2001

  • King, William P.; Kenny, Thomas W.; Goodson, Kenneth E.
  • Applied Physics Letters, Vol. 78, Issue 9
  • DOI: 10.1063/1.1351846

Switching spectroscopy piezoresponse force microscopy of ferroelectric materials
journal, February 2006

  • Jesse, Stephen; Baddorf, Arthur P.; Kalinin, Sergei V.
  • Applied Physics Letters, Vol. 88, Issue 6
  • DOI: 10.1063/1.2172216

Quantitative mapping of switching behavior in piezoresponse force microscopy
journal, July 2006

  • Jesse, Stephen; Lee, Ho Nyung; Kalinin, Sergei V.
  • Review of Scientific Instruments, Vol. 77, Issue 7
  • DOI: 10.1063/1.2214699

Local probing of relaxation time distributions in ferroelectric polymer nanomesas: Time-resolved piezoresponse force spectroscopy and spectroscopic imaging
journal, June 2008

  • Rodriguez, Brian J.; Jesse, Stephen; Kim, Jihee
  • Applied Physics Letters, Vol. 92, Issue 23
  • DOI: 10.1063/1.2942390

Piezoelectric response of nanoscale PbTiO3 in composite PbTiO3−CoFe2O4 epitaxial films
journal, August 2008

  • Tan, Zhuopeng; Roytburd, Alexander L.; Levin, Igor
  • Applied Physics Letters, Vol. 93, Issue 7
  • DOI: 10.1063/1.2969038

Rapid multidimensional data acquisition in scanning probe microscopy applied to local polarization dynamics and voltage dependent contact mechanics
journal, September 2008

  • Jesse, Stephen; Maksymovych, Peter; Kalinin, Sergei V.
  • Applied Physics Letters, Vol. 93, Issue 11
  • DOI: 10.1063/1.2980031

Switching spectroscopy piezoresponse force microscopy of polycrystalline capacitor structures
journal, January 2009

  • Bintachitt, Patamas; Trolier-McKinstry, Susan; Seal, Katyayani
  • Applied Physics Letters, Vol. 94, Issue 4
  • DOI: 10.1063/1.3070543

Spatial distribution of relaxation behavior on the surface of a ferroelectric relaxor in the ergodic phase
journal, October 2009

  • Kalinin, S. V.; Rodriguez, B. J.; Jesse, S.
  • Applied Physics Letters, Vol. 95, Issue 14
  • DOI: 10.1063/1.3242011

Local measurements of Preisach density in polycrystalline ferroelectric capacitors using piezoresponse force spectroscopy
journal, March 2010

  • Ovchinnikov, O.; Jesse, S.; Guo, S.
  • Applied Physics Letters, Vol. 96, Issue 11
  • DOI: 10.1063/1.3360220

Real space mapping of polarization dynamics and hysteresis loop formation in relaxor-ferroelectric PbMg1/3Nb2/3O3–PbTiO3 solid solutions
journal, August 2010

  • Rodriguez, B. J.; Jesse, S.; Morozovska, A. N.
  • Journal of Applied Physics, Vol. 108, Issue 4
  • DOI: 10.1063/1.3474961

Watching domains grow: In-situ studies of polarization switching by combined scanning probe and scanning transmission electron microscopy
journal, September 2011

  • Chang, Hyejung; Kalinin, Sergei V.; Yang, Seungyeul
  • Journal of Applied Physics, Vol. 110, Issue 5
  • DOI: 10.1063/1.3623779

A Preisach model with a temperature and time-dependent remanence maximum
journal, April 1997

  • Mitchler, P. D.; Roshko, R. M.; Dahlberg, E. Dan
  • Journal of Applied Physics, Vol. 81, Issue 8
  • DOI: 10.1063/1.364473

Collective dynamics underpins Rayleigh behavior in disordered polycrystalline ferroelectrics
journal, April 2010

  • Bintachitt, P.; Jesse, S.; Damjanovic, D.
  • Proceedings of the National Academy of Sciences, Vol. 107, Issue 16
  • DOI: 10.1073/pnas.0913172107

Theory of orientational glasses models, concepts, simulations
journal, December 1992


Band excitation in scanning probe microscopy: sines of change
journal, November 2011


Dual-frequency resonance-tracking atomic force microscopy
journal, October 2007


Temperature-dependent phase transitions in zeptoliter volumes of a complex biological membrane
journal, December 2010


Nanometer-scale flow of molten polyethylene from a heated atomic force microscope tip
journal, May 2012


Oscillation of the lattice relaxation in layer-by-layer epitaxial growth of highly strained materials
journal, August 1993


Generalized Preisach model of hysteresis
journal, January 1988

  • Mayergoyz, I. D.; Friedman, G.
  • IEEE Transactions on Magnetics, Vol. 24, Issue 1
  • DOI: 10.1109/20.43892

Blind Unmixing of Linear Mixtures using a Hierarchical Bayesian Model. Application to Spectroscopic Signal Analysis
conference, August 2007

  • Dobigeon, Nicolas; Tourneret, Jean-Yves; Moussaoui, Said
  • 2007 IEEE/SP 14th Workshop on Statistical Signal Processing
  • DOI: 10.1109/ssp.2007.4301222

Electromechanical Imaging and Spectroscopy of Ferroelectric and Piezoelectric Materials: State of the Art and Prospects for the Future
journal, August 2009


Distilling Free-Form Natural Laws from Experimental Data
journal, April 2009


Domain Dynamics During Ferroelectric Switching
journal, November 2011


The future lies in uncertainty
journal, July 2014


Nonlinear Dimensionality Reduction by Locally Linear Embedding
journal, December 2000


Subspace clustering for high dimensional data: a review
journal, June 2004

  • Parsons, Lance; Haque, Ehtesham; Liu, Huan
  • ACM SIGKDD Explorations Newsletter, Vol. 6, Issue 1
  • DOI: 10.1145/1007730.1007731

Laplacian Eigenmaps for Dimensionality Reduction and Data Representation
journal, June 2003


The International Exascale Software Project roadmap
journal, January 2011

  • Dongarra, Jack; Beckman, Pete; Moore, Terry
  • The International Journal of High Performance Computing Applications, Vol. 25, Issue 1
  • DOI: 10.1177/1094342010391989

Chemistry and electronic structure of iron-based superconductors
journal, August 2011


Learning Deep Architectures for AI
journal, January 2009

  • Bengio, Y.
  • Foundations and Trends® in Machine Learning, Vol. 2, Issue 1
  • DOI: 10.1561/2200000006

Algorithm AS 136: A K-Means Clustering Algorithm
journal, January 1979

  • Hartigan, J. A.; Wong, M. A.
  • Applied Statistics, Vol. 28, Issue 1
  • DOI: 10.2307/2346830

Joint Bayesian endmember extraction and linear unmixing for hyperspectral imagery
text, January 2009


Parameter Space Compression Underlies Emergent Theories and Predictive Models
text, January 2013


Works referencing / citing this record:

LiberTEM/LiberTEM: 0.5.1
software, August 2020


LiberTEM/LiberTEM: 0.2.0
software, October 2019


LiberTEM/LiberTEM: 0.3.0
software, December 2019


LiberTEM/LiberTEM-blobfinder: 0.4.0
software, February 2020


LiberTEM/LiberTEM: 0.4.0
software, February 2020


LiberTEM/LiberTEM: 0.4.1
software, February 2020


Identification of phases, symmetries and defects through local crystallography
journal, July 2015

  • Belianinov, Alex; He, Qian; Kravchenko, Mikhail
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms8801

Understanding and designing magnetoelectric heterostructures guided by computation: progresses, remaining questions, and perspectives
journal, May 2017


Automated defect analysis in electron microscopic images
journal, July 2018


Application of pan-sharpening algorithm for correlative multimodal imaging using AFM-IR
journal, April 2019

  • Borodinov, Nikolay; Bilkey, Natasha; Foston, Marcus
  • npj Computational Materials, Vol. 5, Issue 1
  • DOI: 10.1038/s41524-019-0186-z

Machine learning-based multidomain processing for texture-based image segmentation and analysis
journal, January 2020

  • Borodinov, Nikolay; Tsai, Wan-Yu; Korolkov, Vladimir V.
  • Applied Physics Letters, Vol. 116, Issue 4
  • DOI: 10.1063/1.5135328

Multifrequency spectrum analysis using fully digital G Mode-Kelvin probe force microscopy
journal, February 2016


Decoding crystallography from high-resolution electron imaging and diffraction datasets with deep learning
journal, October 2019


LiberTEM/LiberTEM: 0.2.2
software, October 2019


LiberTEM/LiberTEM-blobfinder: 0.4.0
software, February 2020


Research Update: Towards designed functionalities in oxide-based electronic materials
journal, August 2015

  • Rondinelli, James M.; Poeppelmeier, Kenneth R.; Zunger, Alex
  • APL Materials, Vol. 3, Issue 8
  • DOI: 10.1063/1.4928289

Direct atomic fabrication and dopant positioning in Si using electron beams with active real-time image-based feedback
journal, April 2018


Adjustable general line coordinates for visual knowledge discovery in n-D data
journal, July 2017


LiberTEM/LiberTEM: 0.5.0
software, April 2020


Machine Detection of Enhanced Electromechanical Energy Conversion in PbZr 0.2 Ti 0.8 O 3 Thin Films
journal, May 2018


Smart machine learning or discovering meaningful physical and chemical contributions through dimensional stacking
journal, August 2019

  • Griffin, Lee A.; Gaponenko, Iaroslav; Zhang, Shujun
  • npj Computational Materials, Vol. 5, Issue 1
  • DOI: 10.1038/s41524-019-0222-z

LiberTEM/LiberTEM: 0.2.1
software, October 2019


Atomic-scale observation of structural and electronic orders in the layered compound α-RuCl3
journal, December 2016

  • Ziatdinov, M.; Banerjee, A.; Maksov, A.
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms13774

Decoding crystallography from high-resolution electron imaging and diffraction datasets with deep learning
journal, October 2019


Theory-Guided Machine Learning in Materials Science
journal, June 2016


Detecting Nematic Order in STM/STS Data with Artificial Intelligence
text, January 2019


Next-Generation Information Technology Systems for Fast Detectors in Electron Microscop
text, January 2020