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Title: Lithium salts for advanced lithium batteries: Li-metal, Li-O2, and Li-S

Abstract

Presently lithium hexafluorophosphate (LiPF6) is the dominant Li-salt used in commercial rechargeable lithium-ion batteries (LIBs) based on a graphite anode and a 3-4 V cathode material. While LiPF6 is not the ideal Li-salt for every important electrolyte property, it has a uniquely suitable combination of properties (temperature range, passivation, conductivity, etc.) rendering it the overall best Li-salt for LIBs. However, this may not necessarily be true for other types of Li-based batteries. Indeed, next generation batteries, for example lithium-metal (Li-metal), lithium-oxygen (Li-O2), and lithium sulphur (Li-S), require a re-evaluation of Li-salts due to the different electrochemical and chemical reactions and conditions within such cells. Furthermore, this review explores the critical role Li-salts play in ensuring in these batteries viability.

Authors:
 [1];  [2];  [3];  [4];  [5]
+ Show Author Affiliations
  1. Univ. of Denmark, Roskilde (Denmark); Uppsala Univ., Uppsala (Sweden)
  2. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  3. Chalmers Univ. of Technology, Goteborg (Sweden); ALISTORE-ERI European Research Institute, Amiens (France)
  4. Uppsala Univ., Uppsala (Sweden); ALISTORE-ERI European Research Institute, Amiens (France)
  5. Technical University of Denmark
Publication Date:
Research Org.:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1195810
Grant/Contract Number:  
AC05-00OR22725
Resource Type:
Accepted Manuscript
Journal Name:
Energy & Environmental Science
Additional Journal Information:
Journal Volume: 8; Journal Issue: 7; Journal ID: ISSN 1754-5692
Publisher:
Royal Society of Chemistry
Country of Publication:
United States
Language:
English
Subject:
25 ENERGY STORAGE; 36 MATERIALS SCIENCE

Citation Formats

Younesi, Reza, Veith, Gabriel M., Johansson, Patrik, Edstrom, Kristina, and Vegge, Tejs. Lithium salts for advanced lithium batteries: Li-metal, Li-O2, and Li-S. United States: N. p., 2015. Web. doi:10.1039/C5EE01215E.
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Younesi, Reza, Veith, Gabriel M., Johansson, Patrik, Edstrom, Kristina, & Vegge, Tejs. Lithium salts for advanced lithium batteries: Li-metal, Li-O2, and Li-S. United States. https://doi.org/10.1039/C5EE01215E
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Younesi, Reza, Veith, Gabriel M., Johansson, Patrik, Edstrom, Kristina, and Vegge, Tejs. Mon . "Lithium salts for advanced lithium batteries: Li-metal, Li-O2, and Li-S". United States. https://doi.org/10.1039/C5EE01215E. https://www.osti.gov/servlets/purl/1195810.
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@article{osti_1195810,
title = {Lithium salts for advanced lithium batteries: Li-metal, Li-O2, and Li-S},
author = {Younesi, Reza and Veith, Gabriel M. and Johansson, Patrik and Edstrom, Kristina and Vegge, Tejs},
abstractNote = {Presently lithium hexafluorophosphate (LiPF6) is the dominant Li-salt used in commercial rechargeable lithium-ion batteries (LIBs) based on a graphite anode and a 3-4 V cathode material. While LiPF6 is not the ideal Li-salt for every important electrolyte property, it has a uniquely suitable combination of properties (temperature range, passivation, conductivity, etc.) rendering it the overall best Li-salt for LIBs. However, this may not necessarily be true for other types of Li-based batteries. Indeed, next generation batteries, for example lithium-metal (Li-metal), lithium-oxygen (Li-O2), and lithium sulphur (Li-S), require a re-evaluation of Li-salts due to the different electrochemical and chemical reactions and conditions within such cells. Furthermore, this review explores the critical role Li-salts play in ensuring in these batteries viability.},
doi = {10.1039/C5EE01215E},
journal = {Energy & Environmental Science},
number = 7,
volume = 8,
place = {United States},
year = {Mon Jun 01 00:00:00 EDT 2015},
month = {Mon Jun 01 00:00:00 EDT 2015}
}
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