Microscopic characterization of the magnetic properties of the itinerant antiferromagnet La2Ni7 by La139 NMR/NQR measurements

Ding, Qing -Ping; Babu, Joyal; Rana, K.; Lee, Yongbin; Bud'ko, S. L.; Ribeiro, R. A.; Canfield, P. C.; Furukawa, Yuji

doi:10.1103/physrevb.108.064413

This content will become publicly available on Sat Aug 10 00:00:00 EDT 2024

Title: Microscopic characterization of the magnetic properties of the itinerant antiferromagnet La 2 Ni 7 by La 139 NMR/NQR measurements

Abstract

In this study, ¹³⁹La nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) measurements have been performed to investigate the magnetic properties of the itinerant magnet La₂Ni₇, which shows a series of antiferromagnetic (AFM) phase transitions at T_N1= 61 K, T_N2 = 56 K, and T_N3 = 42 K under zero magnetic field. Two distinct La NMR signals were observed due to the two crystallographically inequivalent La sites in La₂Ni₇ (La1 and La2 in the La₂ Ni₄ and the LaNi₅ subunits of the La₂Ni₇unit cell, respectively). From the ¹³⁹La NQR spectrum in the AFM state below T_N3, the AFM state was revealed to be a commensurate state where Ni-ordered moments align along the crystalline c axis. Owing to the two different La sites, we were able to estimate the average values of the Ni-ordered moments (0.09 – 0.10_μB/ Ni and 0.17_μB/ Ni around La1 and La2, respectively) from ¹³⁹La NMR spectrum measurements in the AFM state below T_N3, suggesting a nonuniform distribution of the Ni-ordered moments in the AFM state. In contrast, a more uniform distribution of the Ni-ordered moments in the saturated paramagnetic state induced by the application of high magnetic fields is observed. The temperature dependence ofmore »« less

Authors:

^[1];

^[2]; Rana, K. ^[1];

^[1]; Bud'ko, S. L. ^[2]; Ribeiro, R. A. ^[2]; Canfield, P. C. ^[2];

^[2]

Ames Laboratory (AMES), Ames, IA (United States)
Ames Laboratory (AMES), Ames, IA (United States); Iowa State Univ., Ames, IA (United States)

Publication Date:: Thu Aug 10 00:00:00 EDT 2023

Research Org.:: Ames Laboratory (AMES), Ames, IA (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)

OSTI Identifier:: 1994521

Report Number(s):: IS-J-11,130
Journal ID: ISSN 2469-9950; TRN: US2404973

Grant/Contract Number:: AC02-07CH11358

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review. B

Additional Journal Information:: Journal Volume: 108; Journal Issue: 6; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; magnetic order; magnetism; antiferromagnets; strongly correlated systems; nuclear magnetic resonance; nuclear quadrupole resonance

Citation Formats


                    Ding, Qing -Ping, Babu, Joyal, Rana, K., Lee, Yongbin, Bud'ko, S. L., Ribeiro, R. A., Canfield, P. C., and Furukawa, Yuji. Microscopic characterization of the magnetic properties of the itinerant antiferromagnet La2Ni7 by La139 NMR/NQR measurements.  United States: N. p., 2023. 
Web.  doi:10.1103/physrevb.108.064413.

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                    Ding, Qing -Ping, Babu, Joyal, Rana, K., Lee, Yongbin, Bud'ko, S. L., Ribeiro, R. A., Canfield, P. C., & Furukawa, Yuji. Microscopic characterization of the magnetic properties of the itinerant antiferromagnet La2Ni7 by La139 NMR/NQR measurements.  United States.  https://doi.org/10.1103/physrevb.108.064413

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                    Ding, Qing -Ping, Babu, Joyal, Rana, K., Lee, Yongbin, Bud'ko, S. L., Ribeiro, R. A., Canfield, P. C., and Furukawa, Yuji. Thu .  
"Microscopic characterization of the magnetic properties of the itinerant antiferromagnet La2Ni7 by La139 NMR/NQR measurements".  United States.  https://doi.org/10.1103/physrevb.108.064413.

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@article{osti_1994521,

  title        = {Microscopic characterization of the magnetic properties of the itinerant antiferromagnet La2Ni7 by La139 NMR/NQR measurements},

  author       = {Ding, Qing -Ping and Babu, Joyal and Rana, K. and Lee, Yongbin and Bud'ko, S. L. and Ribeiro, R. A. and Canfield, P. C. and Furukawa, Yuji},

  abstractNote = {In this study, 139La nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) measurements have been performed to investigate the magnetic properties of the itinerant magnet La2Ni7, which shows a series of antiferromagnetic (AFM) phase transitions at TN1= 61 K, TN2 = 56 K, and TN3 = 42 K under zero magnetic field. Two distinct La NMR signals were observed due to the two crystallographically inequivalent La sites in La2Ni7 (La1 and La2 in the La2 Ni4 and the LaNi5 subunits of the La2Ni7 unit cell, respectively). From the 139La NQR spectrum in the AFM state below TN3, the AFM state was revealed to be a commensurate state where Ni-ordered moments align along the crystalline c axis. Owing to the two different La sites, we were able to estimate the average values of the Ni-ordered moments (0.09 – 0.10μB/ Ni and 0.17μB/ Ni around La1 and La2, respectively) from 139La NMR spectrum measurements in the AFM state below TN3, suggesting a nonuniform distribution of the Ni-ordered moments in the AFM state. In contrast, a more uniform distribution of the Ni-ordered moments in the saturated paramagnetic state induced by the application of high magnetic fields is observed. The temperature dependence of the sublattice magnetization measured by the internal magnetic induction at the La2 site in the AFM state was reproduced by a local-moment model better than the self-consistent renormalization (SCR) theory for weak itinerant antiferromagnets. Given the small Ni-ordered moments in the magnetically ordered state, our results suggest that La2Ni7 has characteristics of both itinerant nature and localized nature in its magnetism. With this in mind, it is noteworthy that the temperature dependence of nuclear spin-relaxation rates (1/T1) in the paramagnetic state above TN1 measured at zero magnetic field can be explained qualitatively by both the SCR theory and the local-moment model.},

  doi          = {10.1103/physrevb.108.064413},

  journal      = {Physical Review. B},

  number       = 6,

  volume       = 108,

  place        = {United States},

  year         = {Thu Aug 10 00:00:00 EDT 2023},

  month        = {Thu Aug 10 00:00:00 EDT 2023}

}

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Title: Microscopic characterization of the magnetic properties of the itinerant antiferromagnet La 2 Ni 7 by La 139 NMR/NQR measurements

Abstract

Citation Formats

Generalized Gradient Approximation Made Simple journal, October 1996

Itinerant Electron Magnetism of Hexagonal La2Ni7 journal, January 2000

New materials physics journal, November 2019

Volovik effect and Fermi-liquid behavior in the s -wave superconductor CaPd 2 As 2 : As 75 NMR-NQR measurements journal, April 2016

Preserved entropy and fragile magnetism journal, July 2016

Magnetic fluctuations in the itinerant ferromagnet LaCrGe 3 studied by La 139 NMR journal, June 2019

Magnetic detwinning and biquadratic magnetic interaction in Eu Fe 2 As 2 revealed by Eu 153 NMR journal, November 2020

Electronic signatures of successive itinerant, antiferromagnetic transitions in hexagonal La2Ni7 journal, April 2023

NMR Investigations on the Spin Fluctuations in Itinerant Antiferromagnets III. CrB2 journal, August 1980

VESTA 3 for three-dimensional visualization of crystal, volumetric and morphology data journal, October 2011

Ferromagnetic Quantum Critical Point Avoided by the Appearance of Another Magnetic Phase in LaCrGe 3 under Pressure journal, July 2016

Nuclear Spin-Lattice Relaxation in Pure and Impure Indium. I. Normal State journal, July 1971

Magnetic properties of La2Ni7 journal, March 1983

Magnetic properties of La2Ni7 and its hydride journal, December 1983

Tricritical wings and modulated magnetic phases in LaCrGe3 under pressure journal, September 2017

Metamagnetic transitions in hexagonal La2Ni7 journal, April 2004

NMR Investigations on the Spin Fluctuations in Itinerant Antiferromagnets. II. V3S4 and V5S8 journal, June 1980

Magnetic properties of the itinerant ferromagnet LaCrGe3 under pressure studied by La139 NMR journal, May 2021

Nuclear magnetic relaxation in weakly ferro-and antiferromagnetic metals journal, July 1974

NMR determination of an incommensurate helical antiferromagnetic structure in EuCo 2 As 2 journal, May 2017

Effect of Spin Fluctuations on Itinerant Electron Antiferromagnetism journal, June 1974

Avoided ferromagnetic quantum critical point in pressurized La 5 Co 2 Ge 3 journal, February 2021

Successive Metamagnetic Transitions in Hexagonal La 2 Ni 7 journal, April 1999

Magnetism of R2Ni7 and RNi3 (R=Y, La, Ce) journal, May 1993

Hedgehog Spin-Vortex Crystal Antiferromagnetic Quantum Criticality in CaK ( Fe 1 − x Ni x ) 4 As 4 Revealed by NMR journal, September 2018

NMR study of itinerant antiferromagnet YMn12 journal, December 1990

The crystal structure of rare-earth nickel compounds of the type R2Ni7 journal, December 1970

Spin Fluctuations in Itinerant Electron Magnetism book, January 1985

Formation of short-range magnetic order and avoided ferromagnetic quantum criticality in pressurized LaCrGe 3 journal, February 2021

Small-moment antiferromagnetic ordering in single-crystalline La 2 Ni 7 journal, January 2022

Correlations between stacked structures and weak itinerant magnetic properties of La2 − x Y x Ni7 compounds journal, July 2020

Principles of Magnetic Resonance book, January 1990

NMR Investigations on the Spin Fluctuations in Itinerant Antiferromagnets. I. V 3 Se 4 and V 5 Se 8 journal, May 1980

Ferromagnetic Quantum Critical Point in Noncentrosymmetric Systems journal, April 2020

Crystal structures of AB3 and A2B7 rare earth-nickel phases journal, May 1969

Weak itinerant magnetic phases of La2Ni7 journal, August 2022

Generalized Gradient Approximation Made Simple
journal, October 1996

Itinerant Electron Magnetism of Hexagonal La₂Ni₇
journal, January 2000

New materials physics
journal, November 2019

Volovik effect and Fermi-liquid behavior in the $s$ -wave superconductor ${CaPd}_{2} {As}_{2} : {}^{75}{As}$ NMR-NQR measurements
journal, April 2016

Preserved entropy and fragile magnetism
journal, July 2016

Magnetic fluctuations in the itinerant ferromagnet ${LaCrGe}_{3}$ studied by ${}^{139}{La}$ NMR
journal, June 2019

Magnetic detwinning and biquadratic magnetic interaction in $Eu {Fe}_{2} {As}_{2}$ revealed by ${}^{153}{Eu}$ NMR
journal, November 2020

Electronic signatures of successive itinerant, antiferromagnetic transitions in hexagonal La₂Ni₇
journal, April 2023

NMR Investigations on the Spin Fluctuations in Itinerant Antiferromagnets III. CrB₂
journal, August 1980

VESTA 3 for three-dimensional visualization of crystal, volumetric and morphology data
journal, October 2011

Ferromagnetic Quantum Critical Point Avoided by the Appearance of Another Magnetic Phase in ${LaCrGe}_{3}$ under Pressure
journal, July 2016

Nuclear Spin-Lattice Relaxation in Pure and Impure Indium. I. Normal State
journal, July 1971

Magnetic properties of La2Ni7
journal, March 1983

Magnetic properties of La2Ni7 and its hydride
journal, December 1983

Tricritical wings and modulated magnetic phases in LaCrGe3 under pressure
journal, September 2017

Metamagnetic transitions in hexagonal La2Ni7
journal, April 2004

NMR Investigations on the Spin Fluctuations in Itinerant Antiferromagnets. II. V₃S₄ and V₅S₈
journal, June 1980

Magnetic properties of the itinerant ferromagnet LaCrGe3 under pressure studied by La139 NMR
journal, May 2021

Nuclear magnetic relaxation in weakly ferro-and antiferromagnetic metals
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NMR determination of an incommensurate helical antiferromagnetic structure in ${EuCo}_{2} {As}_{2}$
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Effect of Spin Fluctuations on Itinerant Electron Antiferromagnetism
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Avoided ferromagnetic quantum critical point in pressurized ${La}_{5} {Co}_{2} {Ge}_{3}$
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Successive Metamagnetic Transitions in Hexagonal La ₂ Ni ₇
journal, April 1999

Magnetism of R2Ni7 and RNi3 (R=Y, La, Ce)
journal, May 1993

Hedgehog Spin-Vortex Crystal Antiferromagnetic Quantum Criticality in $CaK ({Fe}_{1 - x} {Ni}_{x})_{4} {As}_{4}$ Revealed by NMR
journal, September 2018

NMR study of itinerant antiferromagnet YMn12
journal, December 1990

The crystal structure of rare-earth nickel compounds of the type R2Ni7
journal, December 1970

Spin Fluctuations in Itinerant Electron Magnetism
book, January 1985

Formation of short-range magnetic order and avoided ferromagnetic quantum criticality in pressurized ${LaCrGe}_{3}$
journal, February 2021

Small-moment antiferromagnetic ordering in single-crystalline ${La}_{2} {Ni}_{7}$
journal, January 2022

Correlations between stacked structures and weak itinerant magnetic properties of La₂ ₋ _xY_xNi₇ compounds
journal, July 2020

Principles of Magnetic Resonance
book, January 1990

NMR Investigations on the Spin Fluctuations in Itinerant Antiferromagnets. I. V ₃ Se ₄ and V ₅ Se ₈
journal, May 1980

Ferromagnetic Quantum Critical Point in Noncentrosymmetric Systems
journal, April 2020

Crystal structures of AB3 and A2B7 rare earth-nickel phases
journal, May 1969

Weak itinerant magnetic phases of La2Ni7
journal, August 2022