Octave-spanning mid-infrared femtosecond OPA in a ZnGeP 2 pumped by a 2.4 μm Cr:ZnSe chirped-pulse amplifier
Abstract
We report on the highly efficient, octave-spanning mid-infrared (mid-IR) optical parametric amplification (OPA) in a ZnGeP 2 (ZGP) crystal, pumped by a 1 kHz, 2.4 μm, 250 fs Cr:ZnSe chirped-pulse amplifier. The full spectral coverage of 3−10 μm with the amplified signal and idler beams is demonstrated. The signal beam in the range of ∼3 − 5 μm is produced by either white light generation (WLG) in YAG or optical parametric generation (OPG) in ZGP using the common 2.4 μm pump laser. We demonstrate the pump to signal and idler combined conversion efficiency of 23% and the pulse energy of up to 130 μJ with ∼2 μJ OPG seeding, while we obtain the efficiency of 10% and the pulse energy of 55 μJ with ∼0.2 μJ WLG seeding. The OPA output energy is limited by the available pump pulse energy (0.55 mJ at ZGP crystal) and therefore further energy scaling is feasible with multi-stage OPA and higher pump pulse energy. The autocorrelation measurements based on random quasi-phase matching show that the signal pulse durations are ∼318 fs and ∼330 fs with WLG and OPG seeding, respectively. In addition, we show the spectrally filtered 30 μJ OPA output at 4.15 μm suitable for seeding a Fe:ZnSe amplifier. Ourmore »
- Authors:
- Publication Date:
- Research Org.:
- Univ. of Alabama, Birmingham, AL (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC); MIT Lincoln Laboratory; National Institute of Environmental Health Sciences; US Department of the Navy, Office of Naval Research (ONR)
- OSTI Identifier:
- 1671857
- Alternate Identifier(s):
- OSTI ID: 1852618
- Grant/Contract Number:
- SC0018378; IR10-773; P42 ES027723; N00014-17-1-2744
- Resource Type:
- Published Article
- Journal Name:
- Optics Express
- Additional Journal Information:
- Journal Name: Optics Express Journal Volume: 28 Journal Issue: 22; Journal ID: ISSN 1094-4087
- Publisher:
- Optical Society of America
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS
Citation Formats
Nam, Sang-Hoon, Fedorov, Vladimir, Mirov, Sergey, and Hong, Kyung-Han. Octave-spanning mid-infrared femtosecond OPA in a ZnGeP 2 pumped by a 2.4 μm Cr:ZnSe chirped-pulse amplifier. United States: N. p., 2020.
Web. doi:10.1364/OE.405648.
Nam, Sang-Hoon, Fedorov, Vladimir, Mirov, Sergey, & Hong, Kyung-Han. Octave-spanning mid-infrared femtosecond OPA in a ZnGeP 2 pumped by a 2.4 μm Cr:ZnSe chirped-pulse amplifier. United States. https://doi.org/10.1364/OE.405648
Nam, Sang-Hoon, Fedorov, Vladimir, Mirov, Sergey, and Hong, Kyung-Han. Mon .
"Octave-spanning mid-infrared femtosecond OPA in a ZnGeP 2 pumped by a 2.4 μm Cr:ZnSe chirped-pulse amplifier". United States. https://doi.org/10.1364/OE.405648.
@article{osti_1671857,
title = {Octave-spanning mid-infrared femtosecond OPA in a ZnGeP 2 pumped by a 2.4 μm Cr:ZnSe chirped-pulse amplifier},
author = {Nam, Sang-Hoon and Fedorov, Vladimir and Mirov, Sergey and Hong, Kyung-Han},
abstractNote = {We report on the highly efficient, octave-spanning mid-infrared (mid-IR) optical parametric amplification (OPA) in a ZnGeP 2 (ZGP) crystal, pumped by a 1 kHz, 2.4 μm, 250 fs Cr:ZnSe chirped-pulse amplifier. The full spectral coverage of 3−10 μm with the amplified signal and idler beams is demonstrated. The signal beam in the range of ∼3 − 5 μm is produced by either white light generation (WLG) in YAG or optical parametric generation (OPG) in ZGP using the common 2.4 μm pump laser. We demonstrate the pump to signal and idler combined conversion efficiency of 23% and the pulse energy of up to 130 μJ with ∼2 μJ OPG seeding, while we obtain the efficiency of 10% and the pulse energy of 55 μJ with ∼0.2 μJ WLG seeding. The OPA output energy is limited by the available pump pulse energy (0.55 mJ at ZGP crystal) and therefore further energy scaling is feasible with multi-stage OPA and higher pump pulse energy. The autocorrelation measurements based on random quasi-phase matching show that the signal pulse durations are ∼318 fs and ∼330 fs with WLG and OPG seeding, respectively. In addition, we show the spectrally filtered 30 μJ OPA output at 4.15 μm suitable for seeding a Fe:ZnSe amplifier. Our ultrabroadband femtosecond mid-IR source is attractive for various applications, such as strong-field interactions, dielectric laser electron acceleration, molecular spectroscopy, and medical surgery.},
doi = {10.1364/OE.405648},
journal = {Optics Express},
number = 22,
volume = 28,
place = {United States},
year = {Mon Oct 12 00:00:00 EDT 2020},
month = {Mon Oct 12 00:00:00 EDT 2020}
}
https://doi.org/10.1364/OE.405648
Works referenced in this record:
Mid-Infrared Time-Resolved Frequency Comb Spectroscopy of Transient Free Radicals
journal, June 2014
- Fleisher, Adam J.; Bjork, Bryce J.; Bui, Thinh Q.
- The Journal of Physical Chemistry Letters, Vol. 5, Issue 13
Ultrafast Dynamics of Surface Plasmons in InAs by Time-Resolved Infrared Nanospectroscopy
journal, July 2014
- Wagner, Martin; McLeod, Alexander S.; Maddox, Scott J.
- Nano Letters, Vol. 14, Issue 8
Multi-mJ, kHz, 21 μm optical parametric chirped-pulse amplifier and high-flux soft x-ray high-harmonic generation
journal, January 2014
- Hong, Kyung-Han; Lai, Chien-Jen; Siqueira, Jonathas P.
- Optics Letters, Vol. 39, Issue 11
Random quasi-phase-matching in bulk polycrystalline isotropic nonlinear materials
journal, November 2004
- Baudrier-Raybaut, M.; Haïdar, R.; Kupecek, Ph.
- Nature, Vol. 432, Issue 7015
Frontiers of Mid-IR Lasers Based on Transition Metal Doped Chalcogenides
journal, September 2018
- Mirov, Sergey B.; Moskalev, Igor S.; Vasilyev, Sergey
- IEEE Journal of Selected Topics in Quantum Electronics, Vol. 24, Issue 5
Multi-octave supercontinuum generation from mid-infrared filamentation in a bulk crystal
journal, January 2012
- Silva, F.; Austin, D. R.; Thai, A.
- Nature Communications, Vol. 3, Issue 1
35-mJ 150-fs Fe:ZnSe hybrid mid-IR femtosecond laser at 44 μm for driving extreme nonlinear optics
journal, January 2019
- Migal, Ekaterina; Pushkin, Andrey; Bravy, Boris
- Optics Letters, Vol. 44, Issue 10
Multi-Watt mid-IR femtosecond polycrystalline Cr^2+:ZnS and Cr^2+:ZnSe laser amplifiers with the spectrum spanning 20–26 µm
journal, January 2016
- Vasilyev, Sergey; Moskalev, Igor; Mirov, Mike
- Optics Express, Vol. 24, Issue 2
Generation of 1 kHz, 23 mJ, 88 fs, 25 μm pulses from a Cr 2+ :ZnSe chirped pulse amplifier
journal, January 2018
- Ren, Xiaoming; Mach, Lam H.; Yin, Yanchun
- Optics Letters, Vol. 43, Issue 14
High-brightness table-top hard X-ray source driven by sub-100-femtosecond mid-infrared pulses
journal, November 2014
- Weisshaupt, Jannick; Juvé, Vincent; Holtz, Marcel
- Nature Photonics, Vol. 8, Issue 12
Multimicrojoule GaSe-based midinfrared optical parametric amplifier with an ultrabroad idler spectrum covering 42–16 μm
journal, January 2019
- Liu, Kun; Liang, Houkun; Wang, Lifeng
- Optics Letters, Vol. 44, Issue 4
7 μm, ultrafast, sub-millijoule-level mid-infrared optical parametric chirped pulse amplifier pumped at 2 μm
journal, January 2016
- Sanchez, D.; Hemmer, M.; Baudisch, M.
- Optica, Vol. 3, Issue 2
Broadband mid-infrared pulses from potassium titanyl arsenate/zinc germanium phosphate optical parametric amplifier pumped by Tm, Ho-fiber-seeded Ho:YAG chirped-pulse amplifier
journal, January 2016
- Malevich, Pavel; Kanai, Tsuneto; Hoogland, Heinar
- Optics Letters, Vol. 41, Issue 5
Refractive-index measurements and Sellmeier coefficients for zinc germanium phosphide from 2 to 9 µm with implications for phase matching in optical frequency-conversion devices
journal, January 2001
- Zelmon, David E.; Hanning, Elizabeth A.; Schunemann, Peter G.
- Journal of the Optical Society of America B, Vol. 18, Issue 9
Parametric generation of energetic short mid-infrared pulses for dielectric laser acceleration
journal, November 2014
- Wandel, S.; Xu, G.; Yin, Y.
- Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 47, Issue 23
Progress in Cr 2+ and Fe 2+ doped mid-IR laser materials
journal, January 2010
- Mirov, S.; Fedorov, V.; Moskalev, I.
- Laser & Photonics Reviews, Vol. 4, Issue 1
High-energy mid-infrared sub-cycle pulse synthesis from a parametric amplifier
journal, July 2017
- Liang, Houkun; Krogen, Peter; Wang, Zhou
- Nature Communications, Vol. 8, Issue 1
Progress in Mid-IR Lasers Based on Cr and Fe-Doped II–VI Chalcogenides
journal, January 2015
- Mirov, Sergey B.; Fedorov, Vladimir V.; Martyshkin, Dmitry
- IEEE Journal of Selected Topics in Quantum Electronics, Vol. 21, Issue 1
Carrier-to-envelope phase-stable, mid-infrared, ultrashort pulses from a hybrid parametric generator: Cr:ZnSe laser amplifier system
journal, January 2019
- Komm, Pavel; Sheintop, Uzziel; Noach, Salman
- Optics Express, Vol. 27, Issue 13
Design criteria for ultrafast optical parametric amplifiers
journal, August 2016
- Manzoni, C.; Cerullo, G.
- Journal of Optics, Vol. 18, Issue 10
High-energy, kHz-rate, picosecond, 2-μm laser pump source for mid-IR nonlinear optical devices
conference, March 2013
- Dergachev, Alex
- SPIE LASE, SPIE Proceedings
Ultrafast middle-IR lasers and amplifiers based on polycrystalline Cr:ZnS and Cr:ZnSe
journal, January 2017
- Vasilyev, Sergey; Moskalev, Igor; Mirov, Mike
- Optical Materials Express, Vol. 7, Issue 7
Super-octave longwave mid-infrared coherent transients produced by optical rectification of few-cycle 25-μm pulses
journal, January 2019
- Vasilyev, Sergey; Moskalev, Igor S.; Smolski, Viktor O.
- Optica, Vol. 6, Issue 1
Directly diode-pumped, Kerr-lens mode-locked, few-cycle Cr:ZnSe oscillator
journal, January 2019
- Nagl, Nathalie; Gröbmeyer, Sebastian; Pervak, Vladimir
- Optics Express, Vol. 27, Issue 17