Analogy Between the “Hidden Order” and the Orbital Antiferromagnetism in URu2-xFexSi2

Kung, H.-H.; Ran, S.; Kanchanavatee, N.; Krapivin, V.; Lee, A.; Mydosh, J. A.; Haule, K.; Maple, M. B.; Blumberg, G.

doi:10.1103/PhysRevLett.117.227601

Title: Analogy Between the “Hidden Order” and the Orbital Antiferromagnetism in ${URu}_{2 - x} {Fe}_{x} {Si}_{2}$

Abstract

We study URu_2-xFe_xSi₂, in which two types of staggered phases compete at low temperature as the iron concentration x is varied: the nonmagnetic \hidden order" (HO) phase below the critical concentration x_c, and unconventional antiferromagnetic (AF) phase above x_c. By using polarization resolved Raman spectroscopy, we detect a collective mode of pseudovector-like A_{2_g} symmetry whose energy continuously evolves with increasing x; it monotonically decreases in the HO phase until it vanishes at x = x_c, and then reappears with increasing energy in the AF phase. The mode's evolution provides direct evidence for unified order parameter for both nonmagnetic and magnetic phases arising from the orbital degrees-of-freedom of the uranium-5f electrons.

Authors:

Kung, H.-H. ^[1]; Ran, S. ^[2]; Kanchanavatee, N. ^[2]; Krapivin, V. ^[1]; Lee, A. ^[1]; Mydosh, J. A. ^[3]; Haule, K. ^[1]; Maple, M. B. ^[2]; Blumberg, G. ^[4]

Rutgers Univ., Piscataway, NJ (United States). Dept. of Physics & Astronomy
Univ. of California, San Diego, CA (United States). Dept. of Physics; Univ. of California, San Diego, CA (United States). Center for Advanced Nanoscience
Leiden Univ. (Netherlands). Kamerlingh Onnes Lab.
Rutgers Univ., Piscataway, NJ (United States). Dept. of Physics & Astronomy; National Inst. of Chemical Physics and Biophysics,Tallinn (Estonia)

Publication Date:: Tue Nov 22 00:00:00 EST 2016

Research Org.:: Rutgers Univ., New Brunswick, NJ (United States)

Sponsoring Org.:: National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1418620

Alternate Identifier(s):: OSTI ID: 1333315

Grant/Contract Number:: SC0005463; DMR-1104884; DMR-1405303; FG02-04ER46105; DMR-1206553

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review Letters

Additional Journal Information:: Journal Volume: 117; Journal Issue: 22; Journal ID: ISSN 0031-9007

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Kung, H.-H., Ran, S., Kanchanavatee, N., Krapivin, V., Lee, A., Mydosh, J. A., Haule, K., Maple, M. B., and Blumberg, G. Analogy Between the “Hidden Order” and the Orbital Antiferromagnetism in URu2-xFexSi2.  United States: N. p., 2016. 
Web.  doi:10.1103/PhysRevLett.117.227601.

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                    Kung, H.-H., Ran, S., Kanchanavatee, N., Krapivin, V., Lee, A., Mydosh, J. A., Haule, K., Maple, M. B., & Blumberg, G. Analogy Between the “Hidden Order” and the Orbital Antiferromagnetism in URu2-xFexSi2.  United States.  https://doi.org/10.1103/PhysRevLett.117.227601

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                    Kung, H.-H., Ran, S., Kanchanavatee, N., Krapivin, V., Lee, A., Mydosh, J. A., Haule, K., Maple, M. B., and Blumberg, G. Tue .  
"Analogy Between the “Hidden Order” and the Orbital Antiferromagnetism in URu2-xFexSi2".  United States.  https://doi.org/10.1103/PhysRevLett.117.227601.  https://www.osti.gov/servlets/purl/1418620.

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@article{osti_1418620,

  title        = {Analogy Between the “Hidden Order” and the Orbital Antiferromagnetism in URu2-xFexSi2},

  author       = {Kung, H.-H. and Ran, S. and Kanchanavatee, N. and Krapivin, V. and Lee, A. and Mydosh, J. A. and Haule, K. and Maple, M. B. and Blumberg, G.},

  abstractNote = {We study URu2-xFexSi2, in which two types of staggered phases compete at low temperature as the iron concentration x is varied: the nonmagnetic \hidden order" (HO) phase below the critical concentration xc, and unconventional antiferromagnetic (AF) phase above xc. By using polarization resolved Raman spectroscopy, we detect a collective mode of pseudovector-like A2g symmetry whose energy continuously evolves with increasing x; it monotonically decreases in the HO phase until it vanishes at x = xc, and then reappears with increasing energy in the AF phase. The mode's evolution provides direct evidence for unified order parameter for both nonmagnetic and magnetic phases arising from the orbital degrees-of-freedom of the uranium-5f electrons.},

  doi          = {10.1103/PhysRevLett.117.227601},

  journal      = {Physical Review Letters},

  number       = 22,

  volume       = 117,

  place        = {United States},

  year         = {Tue Nov 22 00:00:00 EST 2016},

  month        = {Tue Nov 22 00:00:00 EST 2016}

}

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https://doi.org/10.1103/PhysRevLett.117.227601

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Cited by: 22 works

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Figures / Tables:

FIG. 1. : (a) The upper panel shows the phase diagram of URu₂Si₂ system, where the black lines show the phase boundaries. The measurements on the iron substituted URu_2−xFe_xSi₂ crystals from neutron diffraction [18] (blue triangle), electrical resistivity [2] (green square), magnetic susceptibility [2] (purple triangle), and heat capacity [3]more »

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Works referenced in this record:

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Works referencing / citing this record:

Hidden order and beyond: an experimental—theoretical overview of the multifaceted behavior of URu ₂ Si ₂
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Similar Records

Title: Analogy Between the “Hidden Order” and the Orbital Antiferromagnetism in URu 2 - x Fe x Si 2

Abstract

Citation Formats

Figures / Tables:

Parasitic Small-Moment Antiferromagnetism and Nonlinear Coupling of Hidden Order and Antiferromagnetism in URu 2 Si 2 Observed by Larmor Diffraction journal, March 2010

Optical conductivity of URu 2 Si 2 in the Kondo liquid and hidden-order phases journal, July 2015

Electrodynamics of the antiferromagnetic phase in URu 2 Si 2 journal, November 2015

Antiferromagnetism and hidden order in isoelectronic doping of URu 2 Si 2 journal, February 2016

Chemical pressure tuning of URu 2 Si 2 via isoelectronic substitution of Ru with Fe journal, February 2015

High Magnetic Field Studies of the Hidden Order Transition in U R u 2 S i 2 journal, December 2002

Competition between hidden order and antiferromagnetism in URu 2 Si 2 under uniaxial stress studied by neutron scattering journal, December 2005

Magnetic excitations and phonon anomalies in U Ru 2 Si 2 journal, October 1987

Excitons and Plasmons in Superconductors journal, February 1961

Magnetic excitations and ordering in the heavy-electron superconductor URu 2 Si 2 journal, April 1987

Partially gapped Fermi surface in the heavy-electron superconductor URu 2 Si 2 journal, January 1986

Raman scattering and anomalous current algebra in Mott insulators journal, July 1994

Imaging the Fano lattice to ‘hidden order’ transition in URu2Si2 journal, June 2010

Complex Landau-Ginzburg theory of the hidden order in URu 2 Si 2 journal, March 2010

Role of commensurate and incommensurate low-energy excitations in the paramagnetic to hidden-order transition of URu 2 Si 2 journal, September 2015

Temperature-pressure phase diagram of U Ru 2 Si 2 from resistivity measurements and ac calorimetry: Hidden order and Fermi-surface nesting journal, March 2008

Antiferromagnetic critical pressure in URu 2 Si 2 under hydrostatic conditions journal, August 2010

Spatially Inhomogeneous Development of Antiferromagnetism in URu 2 Si 2 : Evidence from S 29 i NMR under Pressure journal, August 2001

Arrested Kondo effect and hidden order in URu2Si2 journal, September 2009

Superconductivity and magnetic order in a strongly interacting fermi-system: URu2Si2 journal, June 1986

Observation of multiple-gap structure in hidden order state of URu 2 Si 2 from optical conductivity journal, July 2012

Visualizing the formation of the Kondo lattice and the hidden order in URu2Si2 journal, May 2010

Superconducting and Magnetic Transitions in the Heavy-Fermion System U Ru 2 Si 2 journal, December 1985

Hybridization gap versus hidden-order gap in URu 2 Si 2 as revealed by optical spectroscopy journal, May 2012

Pressure dependence of the magnetization of U Ru 2 Si 2 journal, September 2006

Evidence for broken time-reversal symmetry in the superconducting phase of URu 2 Si 2 journal, April 2015

Symmetry of the Excitations in the Hidden Order State of URu 2 Si 2 journal, December 2014

Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of URu 2 Si 2 journal, November 2011

Field-Induced Fermi Surface Reconstruction and Adiabatic Continuity between Antiferromagnetism and the Hidden-Order State in URu 2 Si 2 journal, April 2007

Hybridization gap and anisotropic far-infrared optical conductivity of URu 2 Si 2 journal, November 2011

Field Reentrance of the Hidden Order State of URu 2 Si 2 under Pressure journal, May 2009

Twofold enhancement of the hidden-order/large-moment antiferromagnetic phase boundary in the URu 2 − x Fe x Si 2 system journal, December 2011

Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2 journal, January 2011

Chirality density wave of the "hidden order" phase in URu2Si2 journal, February 2015

Evidence for a nematic component to the hidden-order parameter in URu2Si2 from differential elastoresistance measurements journal, March 2015

Field Reentrance of the Hidden Order State of URu2Si2 under Pressure text, January 2009

Arrested Kondo effect and hidden order in URu_2Si_2 text, January 2009

Visualizing the Formation of the Kondo Lattice and the Hidden Order in URu2Si2 text, January 2010

Imaging the Fano Lattice to 'Hidden Order' Transition in URu2Si2 text, January 2010

Hybridization gap and anisotropic far-infrared optical conductivity of URu2Si2 text, January 2010

Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2 text, January 2011

Role of commensurate and incommensurate low-energy excitations in the paramagnetic to hidden-order transition of URu$_2$Si$_2$ text, January 2011

Evidence for a nematic component to the Hidden Order parameter in URu2Si2 from differential elastoresistance measurements text, January 2014

Chirality density wave of the 'hidden order' phase in URu$_2$Si$_2$ text, January 2014

Electrodynamics of the antiferromagnetic phase in URu$_2$Si$_2$ text, January 2015

Optical conductivity of URu$_2$Si$_2$ in the Kondo Liquid and Hidden-Order Phases text, January 2015

Pressure dependence of the magnetization of URu2Si2 text, January 2006

Hidden order and beyond: an experimental—theoretical overview of the multifaceted behavior of URu 2 Si 2 journal, January 2020

Octupolar order in d-orbital Mott insulators text, January 2019

Title: Analogy Between the “Hidden Order” and the Orbital Antiferromagnetism in ${URu}_{2 - x} {Fe}_{x} {Si}_{2}$

Parasitic Small-Moment Antiferromagnetism and Nonlinear Coupling of Hidden Order and Antiferromagnetism in ${URu}_{2} {Si}_{2}$ Observed by Larmor Diffraction
journal, March 2010

Optical conductivity of ${URu}_{2} {Si}_{2}$ in the Kondo liquid and hidden-order phases
journal, July 2015

Electrodynamics of the antiferromagnetic phase in ${URu}_{2} {Si}_{2}$
journal, November 2015

Antiferromagnetism and hidden order in isoelectronic doping of ${URu}_{2} {Si}_{2}$
journal, February 2016

Chemical pressure tuning of ${URu}_{2} {Si}_{2}$ via isoelectronic substitution of Ru with Fe
journal, February 2015

High Magnetic Field Studies of the Hidden Order Transition in ${U R u}_{2} {S i}_{2}$
journal, December 2002

Competition between hidden order and antiferromagnetism in ${URu}_{2} {Si}_{2}$ under uniaxial stress studied by neutron scattering
journal, December 2005

Magnetic excitations and phonon anomalies in U ${Ru}_{2}$ ${Si}_{2}$
journal, October 1987

Excitons and Plasmons in Superconductors
journal, February 1961

Magnetic excitations and ordering in the heavy-electron superconductor ${URu}_{2}$ ${Si}_{2}$
journal, April 1987

Partially gapped Fermi surface in the heavy-electron superconductor ${URu}_{2}$ ${Si}_{2}$
journal, January 1986

Raman scattering and anomalous current algebra in Mott insulators
journal, July 1994

Imaging the Fano lattice to ‘hidden order’ transition in URu2Si2
journal, June 2010

Complex Landau-Ginzburg theory of the hidden order in URu ₂ Si ₂
journal, March 2010

Role of commensurate and incommensurate low-energy excitations in the paramagnetic to hidden-order transition of ${URu}_{2} {Si}_{2}$
journal, September 2015

Temperature-pressure phase diagram of $U {Ru}_{2} {Si}_{2}$ from resistivity measurements and ac calorimetry: Hidden order and Fermi-surface nesting
journal, March 2008

Antiferromagnetic critical pressure in ${URu}_{2} {Si}_{2}$ under hydrostatic conditions
journal, August 2010

Spatially Inhomogeneous Development of Antiferromagnetism in ${URu}_{2} {Si}_{2}$ : Evidence from ${}^{29}S i$ NMR under Pressure
journal, August 2001

Arrested Kondo effect and hidden order in URu2Si2
journal, September 2009

Superconductivity and magnetic order in a strongly interacting fermi-system: URu2Si2
journal, June 1986

Observation of multiple-gap structure in hidden order state of URu $_{2}$ Si $_{2}$ from optical conductivity
journal, July 2012

Visualizing the formation of the Kondo lattice and the hidden order in URu2Si2
journal, May 2010

Superconducting and Magnetic Transitions in the Heavy-Fermion System U ${Ru}_{2}$ ${Si}_{2}$
journal, December 1985

Hybridization gap versus hidden-order gap in URu $_{2}$ Si $_{2}$ as revealed by optical spectroscopy
journal, May 2012

Pressure dependence of the magnetization of $U {Ru}_{2} {Si}_{2}$
journal, September 2006

Evidence for broken time-reversal symmetry in the superconducting phase of ${URu}_{2} {Si}_{2}$
journal, April 2015

Symmetry of the Excitations in the Hidden Order State of ${URu}_{2} {Si}_{2}$
journal, December 2014

Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of ${URu}_{2} {Si}_{2}$
journal, November 2011

Field-Induced Fermi Surface Reconstruction and Adiabatic Continuity between Antiferromagnetism and the Hidden-Order State in ${URu}_{2} {Si}_{2}$
journal, April 2007

Hybridization gap and anisotropic far-infrared optical conductivity of URu $_{2}$ Si $_{2}$
journal, November 2011

Field Reentrance of the Hidden Order State of URu ₂ Si ₂ under Pressure
journal, May 2009

Twofold enhancement of the hidden-order/large-moment antiferromagnetic phase boundary in the URu $_{2 - x}$ Fe $_{x}$ Si $_{2}$ system
journal, December 2011

Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2
journal, January 2011

Chirality density wave of the "hidden order" phase in URu2Si2
journal, February 2015

Evidence for a nematic component to the hidden-order parameter in URu2Si2 from differential elastoresistance measurements
journal, March 2015

Field Reentrance of the Hidden Order State of URu2Si2 under Pressure
text, January 2009

Arrested Kondo effect and hidden order in URu_2Si_2
text, January 2009

Visualizing the Formation of the Kondo Lattice and the Hidden Order in URu2Si2
text, January 2010

Imaging the Fano Lattice to 'Hidden Order' Transition in URu2Si2
text, January 2010

Hybridization gap and anisotropic far-infrared optical conductivity of URu2Si2
text, January 2010

Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2
text, January 2011

Role of commensurate and incommensurate low-energy excitations in the paramagnetic to hidden-order transition of URu$_2$Si$_2$
text, January 2011

Evidence for a nematic component to the Hidden Order parameter in URu2Si2 from differential elastoresistance measurements
text, January 2014

Chirality density wave of the 'hidden order' phase in URu$_2$Si$_2$
text, January 2014

Electrodynamics of the antiferromagnetic phase in URu$_2$Si$_2$
text, January 2015

Optical conductivity of URu$_2$Si$_2$ in the Kondo Liquid and Hidden-Order Phases
text, January 2015

Pressure dependence of the magnetization of URu2Si2
text, January 2006

Hidden order and beyond: an experimental—theoretical overview of the multifaceted behavior of URu ₂ Si ₂
journal, January 2020

Octupolar order in d-orbital Mott insulators
text, January 2019