Surface engineering of hierarchical platinum-cobalt nanowires for efficient electrocatalysis
Abstract
Despite intense research in past decades, the lack of high-performance catalysts for fuel cell reactions remains a challenge in realizing fuel cell technologies for transportation applications. We report a facile strategy for synthesizing hierarchical platinum-cobalt nanowires with high-index, platinum-rich facets and ordered intermetallic structure. These structural features enable unprecedented performance for the oxygen reduction and alcohol oxidation reactions. The specific/mass activities of the platinum-cobalt nanowires for oxygen reduction reaction are 39.6/33.7 times higher than commercial Pt/C catalyst, respectively. Density functional theory simulations reveal that the active threefold hollow sites on the platinum-rich high-index facets provide an additional factor in enhancing oxygen reduction reaction activities. These nanowires are stable in the electrochemical conditions and also thermally stable. Our work may represent a key step towards scalable production of high-performance platinum-based nanowires for applications in catalysis and energy conversion.
- Authors:
-
- Soochow Univ., Jiangsu (China)
- Peking Univ., Beijing (China)
- California State Univ. (CalState), Northridge, CA (United States)
- Brookhaven National Lab. (BNL), Upton, NY (United States)
- Publication Date:
- Research Org.:
- Brookhaven Science Associates, LLC, Upton, NY (United States); Brookhaven National Laboratory (BNL), Upton, NY (United States). Center for Functional Nanomaterials (CFN)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1307420
- Alternate Identifier(s):
- OSTI ID: 1336135
- Report Number(s):
- BNL-112606-2016-JA
Journal ID: ISSN 2041-1723; ncomms11850
- Grant/Contract Number:
- SC0012704; SC00112704
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 7; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; Hierarchical Nanowires; STEM; Electrocatalysts; Center for Functional Nanomaterials
Citation Formats
Bu, Lingzheng, Guo, Shaojun, Zhang, Xu, Shen, Xuan, Su, Dong, Lu, Gang, Zhu, Xing, Yao, Jianlin, Guo, Jun, and Huang, Xiaoqing. Surface engineering of hierarchical platinum-cobalt nanowires for efficient electrocatalysis. United States: N. p., 2016.
Web. doi:10.1038/ncomms11850.
Bu, Lingzheng, Guo, Shaojun, Zhang, Xu, Shen, Xuan, Su, Dong, Lu, Gang, Zhu, Xing, Yao, Jianlin, Guo, Jun, & Huang, Xiaoqing. Surface engineering of hierarchical platinum-cobalt nanowires for efficient electrocatalysis. United States. https://doi.org/10.1038/ncomms11850
Bu, Lingzheng, Guo, Shaojun, Zhang, Xu, Shen, Xuan, Su, Dong, Lu, Gang, Zhu, Xing, Yao, Jianlin, Guo, Jun, and Huang, Xiaoqing. Wed .
"Surface engineering of hierarchical platinum-cobalt nanowires for efficient electrocatalysis". United States. https://doi.org/10.1038/ncomms11850. https://www.osti.gov/servlets/purl/1307420.
@article{osti_1307420,
title = {Surface engineering of hierarchical platinum-cobalt nanowires for efficient electrocatalysis},
author = {Bu, Lingzheng and Guo, Shaojun and Zhang, Xu and Shen, Xuan and Su, Dong and Lu, Gang and Zhu, Xing and Yao, Jianlin and Guo, Jun and Huang, Xiaoqing},
abstractNote = {Despite intense research in past decades, the lack of high-performance catalysts for fuel cell reactions remains a challenge in realizing fuel cell technologies for transportation applications. We report a facile strategy for synthesizing hierarchical platinum-cobalt nanowires with high-index, platinum-rich facets and ordered intermetallic structure. These structural features enable unprecedented performance for the oxygen reduction and alcohol oxidation reactions. The specific/mass activities of the platinum-cobalt nanowires for oxygen reduction reaction are 39.6/33.7 times higher than commercial Pt/C catalyst, respectively. Density functional theory simulations reveal that the active threefold hollow sites on the platinum-rich high-index facets provide an additional factor in enhancing oxygen reduction reaction activities. These nanowires are stable in the electrochemical conditions and also thermally stable. Our work may represent a key step towards scalable production of high-performance platinum-based nanowires for applications in catalysis and energy conversion.},
doi = {10.1038/ncomms11850},
journal = {Nature Communications},
number = ,
volume = 7,
place = {United States},
year = {Wed Jun 29 00:00:00 EDT 2016},
month = {Wed Jun 29 00:00:00 EDT 2016}
}
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journal, January 2016
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- Journal of Materials Chemistry A, Vol. 4, Issue 42
Well-defined PtNiCo core–shell nanodendrites with enhanced catalytic performance for methanol oxidation
journal, January 2016
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- Journal of Materials Chemistry A, Vol. 4, Issue 46
Facile construction of fascinating trimetallic PdAuAg nanocages with exceptional ethylene glycol and glycerol oxidation activity
journal, January 2017
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Deficient copper decorated platinum nanoparticles for selective hydrogenation of chloronitrobenzene
journal, January 2017
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Facile solvothermal synthesis of Pt 76 Co 24 nanomyriapods for efficient electrocatalysis
journal, January 2017
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- Journal of Materials Chemistry A, Vol. 5, Issue 21
Recent advances in cobalt phosphide based materials for energy-related applications
journal, January 2017
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Screw-like PdPt nanowires as highly efficient electrocatalysts for methanol and ethylene glycol oxidation
journal, January 2018
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Strain engineering of metal-based nanomaterials for energy electrocatalysis
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Hierarchical branched platinum–copper tripods as highly active and stable catalysts
journal, January 2018
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1D alloy ultrafine Pt–Fe nanowires as efficient electrocatalysts for alcohol electrooxidation in alkaline media
journal, January 2018
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Core@shell structured Co–CoO@NC nanoparticles supported on nitrogen doped carbon with high catalytic activity for oxygen reduction reaction
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Synergistically enhanced hydrogen evolution electrocatalysis by in situ exsolution of metallic nanoparticles on perovskites
journal, January 2018
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Hyperbranched PdRu nanospine assemblies: an efficient electrocatalyst for formic acid oxidation
journal, January 2018
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Solvent-mediated length tuning of ultrathin platinum–cobalt nanowires for efficient electrocatalysis
journal, January 2018
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Atomic (single, double, and triple atoms) catalysis: frontiers, opportunities, and challenges
journal, January 2019
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Localized surface plasmon enhanced electrocatalytic methanol oxidation of AgPt bimetallic nanoparticles with an ultra-thin shell
journal, January 2019
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Synthesis of ammonia via electrochemical nitrogen reduction on high-index faceted Au nanoparticles with a high faradaic efficiency
journal, January 2019
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Regulating locations of active sites: a novel strategy to greatly improve the stability of PtAu electrocatalysts
journal, January 2019
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Concave PtCo nanooctahedra with high-energy {110} facets for the oxygen reduction reaction
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Ultra-small intermetallic NiZn nanoparticles: a non-precious metal catalyst for efficient electrocatalysis
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One-pot synthesis of PtIn/3D-GNs composites with high alloying degree for electro-photo synergistic catalysis
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In situ high-potential-driven surface restructuring of ternary AgPd–Pt dilute aerogels with record-high performance improvement for formate oxidation electrocatalysis
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Facile synthesis of ultrathin Pt–Pd nanosheets for enhanced formic acid oxidation and oxygen reduction reaction
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One-step solid-phase boronation to fabricate self-supported porous FeNiB/FeNi foam for efficient electrocatalytic oxygen evolution and overall water splitting
journal, January 2019
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Advanced engineering of core/shell nanostructures for electrochemical carbon dioxide reduction
journal, January 2019
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Interfacial synergy of ultralong jagged Pt 85 Mo 15 –S nanowires with abundant active sites on enhanced hydrogen evolution in an alkaline solution
journal, January 2019
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SnO 2 patched ultrathin PtRh nanowires as efficient catalysts for ethanol electrooxidation
journal, January 2019
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Asymmetric PdPtCu mesoporous hemispheres on nitrogen-functionalized graphene for methanol oxidation electrocatalysis
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Cobalt-platinum nanomotors for local gas generation
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Monatomic Co, , and nanowires on Ir(100) and Pt(100) surfaces: Formation, structure, and energetics
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Surface-modulated palladium-nickel icosahedra as high-performance non-platinum oxygen reduction electrocatalysts
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Annealing Behaviour of Pt and PtNi Nanowires for Proton Exchange Membrane Fuel Cells
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Stability of High-Performance Pt-Based Catalysts for Oxygen Reduction Reactions
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Ultrathin PtPd-Based Nanorings with Abundant Step Atoms Enhance Oxygen Catalysis
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Alloy Nanocatalysts for the Electrochemical Oxygen Reduction (ORR) and the Direct Electrochemical Carbon Dioxide Reduction Reaction (CO 2 RR)
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Pt‐Based Nanocrystal for Electrocatalytic Oxygen Reduction
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Intermetallic PtBi Nanoplates Boost Oxygen Reduction Catalysis with Superior Tolerance over Chemical Fuels
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A Comprehensive Review on Controlling Surface Composition of Pt-Based Bimetallic Electrocatalysts
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Crystallinity-Modulated Electrocatalytic Activity of a Nickel(II) Borate Thin Layer on Ni 3 B for Efficient Water Oxidation
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Facile Solvothermal Synthesis of Pt 4 Co Multi-dendrites: An Effective Electrocatalyst for Oxygen Reduction and Glycerol Oxidation
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In Situ Incorporation Strategy for Bimetallic FeCo-Doped Carbon as Highly Efficient Bifunctional Oxygen Electrocatalysts
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Gold-Copper Aerogels with Intriguing Surface Electronic Modulation as Highly Active and Stable Electrocatalysts for Oxygen Reduction and Borohydride Oxidation
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Nanocatalysts for Electrocatalytic Oxidation of Ethanol
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Highly Efficient Carbon Dioxide Hydrogenation to Methanol Catalyzed by Zigzag Platinum-Cobalt Nanowires
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Highly active zigzag-like Pt-Zn alloy nanowires with high-index facets for alcohol electrooxidation
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Rational Design and Synthesis of Low-Temperature Fuel Cell Electrocatalysts
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Electrode Materials for Rechargeable Zinc-Ion and Zinc-Air Batteries: Current Status and Future Perspectives
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Fabrication and enhanced hydrogen evolution reaction performance of a Cu 3 BiS 3 nanorods/TiO 2 heterojunction film
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One-step green synthesis of composition-tunable Pt–Cu alloy nanowire networks with high catalytic activity for 4-nitrophenol reduction
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Ternary PtVCo dendrites for the hydrogen evolution reaction, oxygen evolution reaction, overall water splitting and rechargeable Zn–air batteries
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Size-dependent synthesis and catalytic activities of trimetallic PdAgCu mesoporous nanospheres in ethanol electrooxidation
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Ligand-mediated bifunctional catalysis for enhanced oxygen reduction and methanol oxidation tolerance in fuel cells
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The OH − -driven synthesis of Pt–Ni nanocatalysts with atomic segregation for alkaline hydrogen evolution reaction
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Multidimensional nanostructured membrane electrode assemblies for proton exchange membrane fuel cell applications
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Atomically dispersed metal catalysts for the oxygen reduction reaction: synthesis, characterization, reaction mechanisms and electrochemical energy applications
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Cyanogel auto-reduction induced synthesis of PdCo nanocubes on carbon nanobowls: a highly active electrocatalyst for ethanol electrooxidation
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Nanoscale engineering of porous Fe-doped Pd nanosheet assemblies for efficient methanol and ethanol electrocatalyses
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Shaping well-defined noble-metal-based nanostructures for fabricating high-performance electrocatalysts: advances and perspectives
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Understanding the roles of amorphous domains and oxygen-containing groups of nitrogen-doped carbon in oxygen reduction catalysis: toward superior activity
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Transition metal-doped ultrathin RuO 2 networked nanowires for efficient overall water splitting across a broad pH range
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Morphology controllable synthesis of PtNi concave nanocubes enclosed by high-index facets supported on porous graphene for enhanced hydrogen evolution reaction
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Design of ultrathin Pt-Mo-Ni nanowire catalysts for ethanol electrooxidation
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Highly Durable and Active Pt-Based Nanoscale Design for Fuel-Cell Oxygen-Reduction Electrocatalysts
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Tungsten‐Doped L1 0 ‐PtCo Ultrasmall Nanoparticles as a High‐Performance Fuel Cell Cathode
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Noble metal-free catalysts for oxygen reduction reaction
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1-Naphthol induced Pt3Ag nanocorals as bifunctional cathode and anode catalysts of direct formic acid fuel cells
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Highly crystalline PtCu nanotubes with three dimensional molecular accessible and restructured surface for efficient catalysis
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Kinetically controlled synthesis of AuPt bi-metallic aerogels and their enhanced electrocatalytic performances
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Preparation of Ni@Pt core@shell conformal nanofibre oxygen reduction electrocatalysts via microwave-assisted galvanic displacement
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Semiconductor nanowire plasmonic lasers
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Ternary PtPdCu Multicubes as a Highly Active and Durable Catalyst toward the Oxygen Reduction Reaction
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Uniformly dispersed platinum-cobalt alloy nanoparticles with stable compositions on carbon substrates for methanol oxidation reaction
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Wire-like Pt on mesoporous Ti0.7W0.3O2 Nanomaterial with Compelling Electro-Activity for Effective Alcohol Electro-Oxidation
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Size-dependent synthesis and catalytic activities of trimetallic PdAgCu mesoporous nanospheres in ethanol electrooxidation
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Design of ultrathin Pt-Mo-Ni nanowire catalysts for ethanol electrooxidation
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Nanostructure Optimization of Platinum-Based Nanomaterials for Catalytic Applications
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