Simultaneous observation of the quantization and the interference pattern of a plasmonic near-field
Abstract
Surface plasmon polaritons can confine electromagnetic fields in subwavelength spaces and are of interest for photonics, optical data storage devices and biosensing applications. In analogy to photons, they exhibit wave–particle duality, whose different aspects have recently been observed in separate tailored experiments. Here we demonstrate the ability of ultrafast transmission electron microscopy to simultaneously image both the spatial interference and the quantization of such confined plasmonic fields. Our experiments are accomplished by spatiotemporally overlapping electron and light pulses on a single nanowire suspended on a graphene film. The resulting energy exchange between single electrons and the quanta of the photoinduced near-field is imaged synchronously with its spatial interference pattern. In conclusion, this methodology enables the control and visualization of plasmonic fields at the nanoscale, providing a promising tool for understanding the fundamental properties of confined electromagnetic fields and the development of advanced photonic circuits.
- Authors:
-
- Ecole Polytechnique Federale Lausanne (Switzlerland). Lab. for Ultrafast Microscopy and Electron Scattering
- Trinity College, Hartford, CT (United States)
- Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States). Physical and Life Sciences Directorate
- Publication Date:
- Research Org.:
- Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1259503
- Grant/Contract Number:
- AC52-07NA27344; USED258697; 623982
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 6; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 70 PLASMA PHYSICS AND FUSION TECHNOLOGY
Citation Formats
Piazza, L., Lummen, T. T. A., Quiñonez, E., Murooka, Y., Reed, B. W., Barwick, B., and Carbone, F. Simultaneous observation of the quantization and the interference pattern of a plasmonic near-field. United States: N. p., 2015.
Web. doi:10.1038/ncomms7407.
Piazza, L., Lummen, T. T. A., Quiñonez, E., Murooka, Y., Reed, B. W., Barwick, B., & Carbone, F. Simultaneous observation of the quantization and the interference pattern of a plasmonic near-field. United States. https://doi.org/10.1038/ncomms7407
Piazza, L., Lummen, T. T. A., Quiñonez, E., Murooka, Y., Reed, B. W., Barwick, B., and Carbone, F. Mon .
"Simultaneous observation of the quantization and the interference pattern of a plasmonic near-field". United States. https://doi.org/10.1038/ncomms7407. https://www.osti.gov/servlets/purl/1259503.
@article{osti_1259503,
title = {Simultaneous observation of the quantization and the interference pattern of a plasmonic near-field},
author = {Piazza, L. and Lummen, T. T. A. and Quiñonez, E. and Murooka, Y. and Reed, B. W. and Barwick, B. and Carbone, F.},
abstractNote = {Surface plasmon polaritons can confine electromagnetic fields in subwavelength spaces and are of interest for photonics, optical data storage devices and biosensing applications. In analogy to photons, they exhibit wave–particle duality, whose different aspects have recently been observed in separate tailored experiments. Here we demonstrate the ability of ultrafast transmission electron microscopy to simultaneously image both the spatial interference and the quantization of such confined plasmonic fields. Our experiments are accomplished by spatiotemporally overlapping electron and light pulses on a single nanowire suspended on a graphene film. The resulting energy exchange between single electrons and the quanta of the photoinduced near-field is imaged synchronously with its spatial interference pattern. In conclusion, this methodology enables the control and visualization of plasmonic fields at the nanoscale, providing a promising tool for understanding the fundamental properties of confined electromagnetic fields and the development of advanced photonic circuits.},
doi = {10.1038/ncomms7407},
journal = {Nature Communications},
number = ,
volume = 6,
place = {United States},
year = {Mon Mar 02 00:00:00 EST 2015},
month = {Mon Mar 02 00:00:00 EST 2015}
}
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