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Title: Coupling single giant nanocrystal quantum dots to the fundamental mode of patch nanoantennas through fringe field

Abstract

Through single dot spectroscopy and numerical simulation studies, we demonstrate that the fundamental mode of gold patch nanoantennas have fringe-field resonance capable of enhancing the nano-emitters coupled around the edge of the patch antenna. This fringe-field coupling is used to enhance the radiative rates of core/thick-shell nanocrystal quantum dots (g-NQDs) that cannot be embedded into the ultra-thin dielectric gap of patch nanoantennas due to their large sizes. We attain 14 and 3 times enhancements in single exciton radiative decay rate and bi-exciton emission efficiencies of g-NQDs respectively, with no detectable metal quenching. Our numerical studies confirmed our experimental results and further reveal that patch nanoantennas can provide strong emission enhancement for dipoles lying not only in radial direction of the circular patches but also in the direction normal to the antennas surface. Finally, this provides a distinct advantage over the parallel gap-bar antennas that can provide enhancement only for the dipoles oriented across the gap.

Authors:
 [1];  [1];  [1];  [1];  [1];  [1]
  1. Los Alamos National Lab. (LANL), Los Alamos, NM (United States). Center for Integrated Nanotechnologies (CINT)
Publication Date:
Research Org.:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1259295
Grant/Contract Number:  
2009LANL1096; U2013B0037
Resource Type:
Accepted Manuscript
Journal Name:
Scientific Reports
Additional Journal Information:
Journal Volume: 5; Journal ID: ISSN 2045-2322
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
77 NANOSCIENCE AND NANOTECHNOLOGY; nanocavities; quantum dots

Citation Formats

Wang, Feng, Karan, Niladri S., Minh Nguyen, Hue, Ghosh, Yagnaseni, Hollingsworth, Jennifer A., and Htoon, Han. Coupling single giant nanocrystal quantum dots to the fundamental mode of patch nanoantennas through fringe field. United States: N. p., 2015. Web. doi:10.1038/srep14313.
Wang, Feng, Karan, Niladri S., Minh Nguyen, Hue, Ghosh, Yagnaseni, Hollingsworth, Jennifer A., & Htoon, Han. Coupling single giant nanocrystal quantum dots to the fundamental mode of patch nanoantennas through fringe field. United States. https://doi.org/10.1038/srep14313
Wang, Feng, Karan, Niladri S., Minh Nguyen, Hue, Ghosh, Yagnaseni, Hollingsworth, Jennifer A., and Htoon, Han. Wed . "Coupling single giant nanocrystal quantum dots to the fundamental mode of patch nanoantennas through fringe field". United States. https://doi.org/10.1038/srep14313. https://www.osti.gov/servlets/purl/1259295.
@article{osti_1259295,
title = {Coupling single giant nanocrystal quantum dots to the fundamental mode of patch nanoantennas through fringe field},
author = {Wang, Feng and Karan, Niladri S. and Minh Nguyen, Hue and Ghosh, Yagnaseni and Hollingsworth, Jennifer A. and Htoon, Han},
abstractNote = {Through single dot spectroscopy and numerical simulation studies, we demonstrate that the fundamental mode of gold patch nanoantennas have fringe-field resonance capable of enhancing the nano-emitters coupled around the edge of the patch antenna. This fringe-field coupling is used to enhance the radiative rates of core/thick-shell nanocrystal quantum dots (g-NQDs) that cannot be embedded into the ultra-thin dielectric gap of patch nanoantennas due to their large sizes. We attain 14 and 3 times enhancements in single exciton radiative decay rate and bi-exciton emission efficiencies of g-NQDs respectively, with no detectable metal quenching. Our numerical studies confirmed our experimental results and further reveal that patch nanoantennas can provide strong emission enhancement for dipoles lying not only in radial direction of the circular patches but also in the direction normal to the antennas surface. Finally, this provides a distinct advantage over the parallel gap-bar antennas that can provide enhancement only for the dipoles oriented across the gap.},
doi = {10.1038/srep14313},
journal = {Scientific Reports},
number = ,
volume = 5,
place = {United States},
year = {Wed Sep 23 00:00:00 EDT 2015},
month = {Wed Sep 23 00:00:00 EDT 2015}
}

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Works referencing / citing this record:

Multiphoton Emission Enhancement from a Single Colloidal Quantum Dot Using SiO 2 -Coated Silver Nanoparticles
journal, February 2017