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Title: Enhanced optical nonlinearities in the near-infrared using III-nitride heterostructures coupled to metamaterials

Abstract

We use planar metamaterial resonators to enhance, by more than two orders of magnitude, the optical second harmonic generation, in the near infrared, obtained from intersubband transitions in III-Nitride heterostructures. The improvement arises from two factors: employing an asymmetric double quantum well design and aligning the resonators’ cross-polarized resonances with the intersubband transition energies. The resulting nonlinear metamaterial operates at wavelengths where single photon detection is available, and represents a new class of sources for quantum photonics related phenomena.

Authors:
 [1];  [2];  [1];  [2];  [3];  [2];  [1]
  1. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States). Center for Integrated Nanotechnologies
  2. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
  3. Princeton Univ., NJ (United States). Electrical Engineering Dept.
Publication Date:
Research Org.:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA)
OSTI Identifier:
1257989
Alternate Identifier(s):
OSTI ID: 1420526
Report Number(s):
SAND-2015-6605J
Journal ID: ISSN 0003-6951; APPLAB; 641909
Grant/Contract Number:  
AC04-94AL85000
Resource Type:
Accepted Manuscript
Journal Name:
Applied Physics Letters
Additional Journal Information:
Journal Volume: 107; Journal Issue: 15; Journal ID: ISSN 0003-6951
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS

Citation Formats

Wolf, Omri, Allerman, Andrew A., Ma, Xuedan, Wendt, Joel R., Song, Alex Y., Shaner, Eric A., and Brener, Igal. Enhanced optical nonlinearities in the near-infrared using III-nitride heterostructures coupled to metamaterials. United States: N. p., 2015. Web. doi:10.1063/1.4933332.
Wolf, Omri, Allerman, Andrew A., Ma, Xuedan, Wendt, Joel R., Song, Alex Y., Shaner, Eric A., & Brener, Igal. Enhanced optical nonlinearities in the near-infrared using III-nitride heterostructures coupled to metamaterials. United States. https://doi.org/10.1063/1.4933332
Wolf, Omri, Allerman, Andrew A., Ma, Xuedan, Wendt, Joel R., Song, Alex Y., Shaner, Eric A., and Brener, Igal. Thu . "Enhanced optical nonlinearities in the near-infrared using III-nitride heterostructures coupled to metamaterials". United States. https://doi.org/10.1063/1.4933332. https://www.osti.gov/servlets/purl/1257989.
@article{osti_1257989,
title = {Enhanced optical nonlinearities in the near-infrared using III-nitride heterostructures coupled to metamaterials},
author = {Wolf, Omri and Allerman, Andrew A. and Ma, Xuedan and Wendt, Joel R. and Song, Alex Y. and Shaner, Eric A. and Brener, Igal},
abstractNote = {We use planar metamaterial resonators to enhance, by more than two orders of magnitude, the optical second harmonic generation, in the near infrared, obtained from intersubband transitions in III-Nitride heterostructures. The improvement arises from two factors: employing an asymmetric double quantum well design and aligning the resonators’ cross-polarized resonances with the intersubband transition energies. The resulting nonlinear metamaterial operates at wavelengths where single photon detection is available, and represents a new class of sources for quantum photonics related phenomena.},
doi = {10.1063/1.4933332},
journal = {Applied Physics Letters},
number = 15,
volume = 107,
place = {United States},
year = {Thu Oct 15 00:00:00 EDT 2015},
month = {Thu Oct 15 00:00:00 EDT 2015}
}

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Cited by: 24 works
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Works referenced in this record:

Coupled quantum well semiconductors with giant electric field tunable nonlinear optical properties in the infrared
journal, May 1994

  • Capasso, F.; Sirtori, C.; Cho, A. Y.
  • IEEE Journal of Quantum Electronics, Vol. 30, Issue 5
  • DOI: 10.1109/3.303697

Ultrastrong Light-Matter Coupling Regime with Polariton Dots
journal, November 2010


Quantum Vacuum Radiation Spectra from a Semiconductor Microcavity with a Time-Modulated Vacuum Rabi Frequency
journal, March 2007


Intersubband polaritons in the electrical dipole gauge
journal, January 2012


Microcavity Polariton Splitting of Intersubband Transitions
journal, March 2003


Ultrastrong Coupling of the Cyclotron Transition of a 2D Electron Gas to a THz Metamaterial
journal, March 2012


Second harmonic generation from metamaterials strongly coupled to intersubband transitions in quantum wells
journal, March 2014

  • Campione, Salvatore; Benz, Alexander; Sinclair, Michael B.
  • Applied Physics Letters, Vol. 104, Issue 13
  • DOI: 10.1063/1.4870072

Phased-array sources based on nonlinear metamaterial nanocavities
journal, July 2015

  • Wolf, Omri; Campione, Salvatore; Benz, Alexander
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms8667

Giant nonlinear response from plasmonic metasurfaces coupled to intersubband transitions
journal, July 2014

  • Lee, Jongwon; Tymchenko, Mykhailo; Argyropoulos, Christos
  • Nature, Vol. 511, Issue 7507
  • DOI: 10.1038/nature13455

Band parameters for III–V compound semiconductors and their alloys
journal, June 2001

  • Vurgaftman, I.; Meyer, J. R.; Ram-Mohan, L. R.
  • Journal of Applied Physics, Vol. 89, Issue 11, p. 5815-5875
  • DOI: 10.1063/1.1368156

Band structure engineering of a nonlinear optical response in semiconductor superlattices
journal, June 1990


Nonlinear optics with intersubband transitions in high-band offset heterostructures
conference, February 2007

  • Xie, Feng; Chaganti, V. R.; Belyanin, Alexey
  • Integrated Optoelectronic Devices 2007, SPIE Proceedings
  • DOI: 10.1117/12.714273

Intersubband resonant enhancement of second-harmonic generation in GaN∕AlN quantum wells
journal, October 2006

  • Nevou, L.; Tchernycheva, M.; Julien, F.
  • Applied Physics Letters, Vol. 89, Issue 15
  • DOI: 10.1063/1.2358118

Strong coupling in the sub-wavelength limit using metamaterial nanocavities
journal, November 2013

  • Benz, A.; Campione, S.; Liu, S.
  • Nature Communications, Vol. 4, Article No. 2882
  • DOI: 10.1038/ncomms3882

Electrodynamic modeling of strong coupling between a metasurface and intersubband transitions in quantum wells
journal, April 2014


Optical Strong Coupling between near-Infrared Metamaterials and Intersubband Transitions in III-Nitride Heterostructures
journal, September 2014

  • Benz, Alexander; Campione, Salvatore; Moseley, Michael W.
  • ACS Photonics, Vol. 1, Issue 10
  • DOI: 10.1021/ph500192v

Silicon impurity-induced layer disordering of AlGaN/AlN superlattices
journal, August 2010

  • Wierer, J. J.; Allerman, A. A.; Li, Q.
  • Applied Physics Letters, Vol. 97, Issue 5
  • DOI: 10.1063/1.3478002

Nonequilibrium Green’s function theory for transport and gain properties of quantum cascade structures
journal, December 2002


Quantum transport theory of electrons in solids: A single-particle approach
journal, October 1991


Resonant nonlinear optics in coherently prepared media: Full analytic solutions
journal, September 2002


Model system for optical nonlinearities: Asymmetric quantum wells
journal, November 1991


Double-resonance enhanced intersubband second-order nonlinear optical susceptibilities in GaN/AlGaN step quantum wells
journal, January 2014


Systematic experimental and theoretical investigation of intersubband absorption in Ga N Al N quantum wells
journal, March 2006


Comparative study of intersubband absorption in AlGaN/GaN and AlInN/GaN superlattices: Impact of material inhomogeneities
journal, December 2013


Controlling light with metamaterial-based nonlinear photonic crystals
journal, February 2015


Observation of large second order susceptibility via intersubband transitions at λ∼10 μm in asymmetric coupled AlInAs/GaInAs quantum wells
journal, October 1991

  • Sirtori, Carlo; Capasso, Federico; Sivco, Deborah L.
  • Applied Physics Letters, Vol. 59, Issue 18
  • DOI: 10.1063/1.106050

Nonlinear optical susceptibilities of AlN film
journal, December 1977

  • Fujii, Y.; Yoshida, S.; Misawa, S.
  • Applied Physics Letters, Vol. 31, Issue 12
  • DOI: 10.1063/1.89550

Study of nonlinear optical effects in GaN:Mg epitaxial film
journal, November 1996

  • Zhang, H. Y.; He, X. H.; Shih, Y. H.
  • Applied Physics Letters, Vol. 69, Issue 20
  • DOI: 10.1063/1.117741

Optically nonlinear effects in intersubband transitions of GaN∕AlN-based superlattice structures
journal, September 2007

  • Hofstetter, Daniel; Baumann, Esther; Giorgetta, Fabrizio R.
  • Applied Physics Letters, Vol. 91, Issue 13
  • DOI: 10.1063/1.2793190

Characterization of a planar artificial magnetic metamaterial surface
journal, September 2006


Determination of effective permittivity and permeability of metamaterials from reflection and transmission coefficients
journal, April 2002


Characterizing Metasurfaces/Metafilms: The Connection Between Surface Susceptibilities and Effective Material Properties
journal, January 2011

  • Holloway, Christopher L.; Kuester, Edward F.; Dienstfrey, Andrew
  • IEEE Antennas and Wireless Propagation Letters, Vol. 10
  • DOI: 10.1109/LAWP.2011.2182591

Works referencing / citing this record:

Mid-infrared second-harmonic generation in ultra-thin plasmonic metasurfaces without a full-metal backplane
journal, June 2018


Giant Efficiency of Visible Second-Harmonic Light by an All-Dielectric Multiple-Quantum-Well Metasurface
journal, December 2019


Inverse-designed photonic fibers and metasurfaces for nonlinear frequency conversion [Invited]
journal, January 2018

  • Sitawarin, Chawin; Jin, Weiliang; Lin, Zin
  • Photonics Research, Vol. 6, Issue 5
  • DOI: 10.1364/prj.6.000b82

Multipolar second harmonic generation in a symmetric nonlinear metamaterial
journal, August 2017