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Title: Competition of branch-to-core exciton localization and interfacial electron transfer in CdSe tetrapods

Authors:
; ; ; ;
Publication Date:
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1255466
Grant/Contract Number:  
FG02-12ER16347; SC0008798
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Chemical Physics
Additional Journal Information:
Journal Name: Chemical Physics Journal Volume: 471 Journal Issue: C; Journal ID: ISSN 0301-0104
Publisher:
Elsevier
Country of Publication:
Netherlands
Language:
English

Citation Formats

Yang, Ye, Wu, Kaifeng, Chen, Zheyuan, Jeong, Ban-Seok, and Lian, Tianquan. Competition of branch-to-core exciton localization and interfacial electron transfer in CdSe tetrapods. Netherlands: N. p., 2016. Web. doi:10.1016/j.chemphys.2015.08.011.
Yang, Ye, Wu, Kaifeng, Chen, Zheyuan, Jeong, Ban-Seok, & Lian, Tianquan. Competition of branch-to-core exciton localization and interfacial electron transfer in CdSe tetrapods. Netherlands. https://doi.org/10.1016/j.chemphys.2015.08.011
Yang, Ye, Wu, Kaifeng, Chen, Zheyuan, Jeong, Ban-Seok, and Lian, Tianquan. Wed . "Competition of branch-to-core exciton localization and interfacial electron transfer in CdSe tetrapods". Netherlands. https://doi.org/10.1016/j.chemphys.2015.08.011.
@article{osti_1255466,
title = {Competition of branch-to-core exciton localization and interfacial electron transfer in CdSe tetrapods},
author = {Yang, Ye and Wu, Kaifeng and Chen, Zheyuan and Jeong, Ban-Seok and Lian, Tianquan},
abstractNote = {},
doi = {10.1016/j.chemphys.2015.08.011},
journal = {Chemical Physics},
number = C,
volume = 471,
place = {Netherlands},
year = {Wed Jun 01 00:00:00 EDT 2016},
month = {Wed Jun 01 00:00:00 EDT 2016}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1016/j.chemphys.2015.08.011

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Works referenced in this record:

Epitaxial Growth of Highly Luminescent CdSe/CdS Core/Shell Nanocrystals with Photostability and Electronic Accessibility
journal, July 1997

  • Peng, Xiaogang; Schlamp, Michael C.; Kadavanich, Andreas V.
  • Journal of the American Chemical Society, Vol. 119, Issue 30, p. 7019-7029
  • DOI: 10.1021/ja970754m

Hot-Electron Transfer from Semiconductor Nanocrystals
journal, June 2010


Comparison of Carrier Multiplication Yields in PbS and PbSe Nanocrystals: The Role of Competing Energy-Loss Processes
journal, January 2012

  • Stewart, John T.; Padilha, Lazaro A.; Qazilbash, M. Mumtaz
  • Nano Letters, Vol. 12, Issue 2
  • DOI: 10.1021/nl203367m

Identification of Optical Transitions in Colloidal CdSe Nanotetrapods
journal, November 2012

  • Nghia, Nguyen Xuan; Hai, Le Ba; Luyen, Nguyen Thi
  • The Journal of Physical Chemistry C, Vol. 116, Issue 48
  • DOI: 10.1021/jp304784w

Colloidal Semiconductor Quantum Dots with Tunable Surface Composition
journal, January 2012

  • Wei, Helen Hsiu-Ying; Evans, Christopher M.; Swartz, Brett D.
  • Nano Letters, Vol. 12, Issue 9
  • DOI: 10.1021/nl3012962

Seeded Growth of Highly Luminescent CdSe/CdS Nanoheterostructures with Rod and Tetrapod Morphologies
journal, October 2007

  • Talapin, Dmitri V.; Nelson, James H.; Shevchenko, Elena V.
  • Nano Letters, Vol. 7, Issue 10
  • DOI: 10.1021/nl072003g

Near Unity Quantum Yield of Light-Driven Redox Mediator Reduction and Efficient H 2 Generation Using Colloidal Nanorod Heterostructures
journal, July 2012

  • Zhu, Haiming; Song, Nianhui; Lv, Hongjin
  • Journal of the American Chemical Society, Vol. 134, Issue 28
  • DOI: 10.1021/ja303698e

Comparing Multiple Exciton Generation in Quantum Dots To Impact Ionization in Bulk Semiconductors: Implications for Enhancement of Solar Energy Conversion
journal, August 2010

  • Beard, Matthew C.; Midgett, Aaron G.; Hanna, Mark C.
  • Nano Letters, Vol. 10, Issue 8
  • DOI: 10.1021/nl101490z

Infrared-Active Heterostructured Nanocrystals with Ultralong Carrier Lifetimes
journal, July 2010

  • Lee, Doh C.; Robel, István; Pietryga, Jeffrey M.
  • Journal of the American Chemical Society, Vol. 132, Issue 29
  • DOI: 10.1021/ja102716p

Controlling Charge Separation and Recombination Rates in CdSe/ZnS Type I Core−Shell Quantum Dots by Shell Thicknesses
journal, October 2010

  • Zhu, Haiming; Song, Nianhui; Lian, Tianquan
  • Journal of the American Chemical Society, Vol. 132, Issue 42
  • DOI: 10.1021/ja106710m

Nearly Monodisperse and Shape-Controlled CdSe Nanocrystals via Alternative Routes:  Nucleation and Growth
journal, April 2002

  • Peng, Z. Adam; Peng, Xiaogang
  • Journal of the American Chemical Society, Vol. 124, Issue 13, p. 3343-3353
  • DOI: 10.1021/ja0173167

Ultrafast Electron−Hole Dynamics in Core/Shell CdSe/CdS Dot/Rod Nanocrystals
journal, December 2008

  • Lupo, Maria Grazia; Della Sala, Fabio; Carbone, Luigi
  • Nano Letters, Vol. 8, Issue 12
  • DOI: 10.1021/nl8028366

Trion, biexciton, and exciton dynamics in single self-assembled CdSe quantum dots
journal, September 2003


Ultrafast Electronic Delocalization in CdSe/CdS Quantum Rod Heterostructures
journal, November 2011

  • Smith, E. Ryan; Luther, Joseph M.; Johnson, Justin C.
  • Nano Letters, Vol. 11, Issue 11
  • DOI: 10.1021/nl202869z

Plasmon-Induced Hot Electron Transfer from the Au Tip to CdS Rod in CdS-Au Nanoheterostructures
journal, October 2013

  • Wu, Kaifeng; Rodríguez-Córdoba, William E.; Yang, Ye
  • Nano Letters, Vol. 13, Issue 11
  • DOI: 10.1021/nl402730m

Photodriven Charge Separation Dynamics in CdSe/ZnS Core/Shell Quantum Dot/Cobaloxime Hybrid for Efficient Hydrogen Production
journal, September 2012

  • Huang, Jier; Mulfort, Karen L.; Du, Pingwu
  • Journal of the American Chemical Society, Vol. 134, Issue 40
  • DOI: 10.1021/ja3062584

Ultrafast Exciton Dynamics and Light-Driven H 2 Evolution in Colloidal Semiconductor Nanorods and Pt-Tipped Nanorods
journal, February 2015

  • Wu, Kaifeng; Zhu, Haiming; Lian, Tianquan
  • Accounts of Chemical Research, Vol. 48, Issue 3
  • DOI: 10.1021/ar500398g

Shape Effects on Electronic States of Nanocrystals
journal, October 2003


Utilizing the Lability of Lead Selenide to Produce Heterostructured Nanocrystals with Bright, Stable Infrared Emission
journal, April 2008

  • Pietryga, Jeffrey M.; Werder, Donald J.; Williams, Darrick J.
  • Journal of the American Chemical Society, Vol. 130, Issue 14
  • DOI: 10.1021/ja710437r

Visible Light-Induced Charge Retention and Photocatalysis with Hybrid CdSe−Au Nanodumbbells
journal, February 2008

  • Costi, Ronny; Saunders, Aaron E.; Elmalem, Einat
  • Nano Letters, Vol. 8, Issue 2
  • DOI: 10.1021/nl0730514

Ultrafast Charge Separation and Long-Lived Charge Separated State in Photocatalytic CdS–Pt Nanorod Heterostructures
journal, June 2012

  • Wu, Kaifeng; Zhu, Haiming; Liu, Zheng
  • Journal of the American Chemical Society, Vol. 134, Issue 25
  • DOI: 10.1021/ja303306u

Artificial Atoms
journal, January 1993


Universal Length Dependence of Rod-to-Seed Exciton Localization Efficiency in Type I and Quasi-Type II CdSe@CdS Nanorods
journal, February 2015


Charge Carrier Resolved Relaxation of the First Excitonic State in CdSe Quantum Dots Probed with Near-Infrared Transient Absorption Spectroscopy
journal, November 2010

  • McArthur, Eric A.; Morris-Cohen, Adam J.; Knowles, Kathryn E.
  • The Journal of Physical Chemistry B, Vol. 114, Issue 45
  • DOI: 10.1021/jp102101f

Competition between Energy and Electron Transfer from CdSe QDs to Adsorbed Rhodamine B
journal, December 2009

  • Boulesbaa, Abdelaziz; Huang, Zhuangqun; Wu, David
  • The Journal of Physical Chemistry C, Vol. 114, Issue 2
  • DOI: 10.1021/jp909972b

Wavefunction engineering in quantum confined semiconductor nanoheterostructures for efficient charge separation and solar energy conversion
journal, January 2012

  • Zhu, Haiming; Lian, Tianquan
  • Energy & Environmental Science, Vol. 5, Issue 11
  • DOI: 10.1039/c2ee22679k

Colloidal nanocrystal heterostructures with linear and branched topology
journal, July 2004

  • Milliron, Delia J.; Hughes, Steven M.; Cui, Yi
  • Nature, Vol. 430, Issue 6996, p. 190-195
  • DOI: 10.1038/nature02695

Multiple Exciton Generation and Dissociation in PbS Quantum Dot-Electron Acceptor Complexes
journal, July 2012

  • Yang, Ye; Rodríguez-Córdoba, William; Lian, Tianquan
  • Nano Letters, Vol. 12, Issue 8
  • DOI: 10.1021/nl301847r

Hole Removal Rate Limits Photodriven H 2 Generation Efficiency in CdS-Pt and CdSe/CdS-Pt Semiconductor Nanorod–Metal Tip Heterostructures
journal, May 2014

  • Wu, Kaifeng; Chen, Zheyuan; Lv, Hongjin
  • Journal of the American Chemical Society, Vol. 136, Issue 21
  • DOI: 10.1021/ja5023893

Heterogeneity of the Electron-Trapping Kinetics in CdSe Nanoparticles
journal, August 2011

  • Kern, Sean J.; Sahu, Kalyanasis; Berg, Mark A.
  • Nano Letters, Vol. 11, Issue 8
  • DOI: 10.1021/nl202086b

Tetrapod-Shaped Colloidal Nanocrystals of II−VI Semiconductors Prepared by Seeded Growth
journal, February 2009

  • Fiore, Angela; Mastria, Rosanna; Lupo, Maria Grazia
  • Journal of the American Chemical Society, Vol. 131, Issue 6
  • DOI: 10.1021/ja807874e

Synthesis of High Aspect Ratio Quantum-Size CdS Nanorods and Their Surface-Dependent Photoluminescence
journal, August 2008

  • Saunders, Aaron E.; Ghezelbash, Ali; Sood, Preeti
  • Langmuir, Vol. 24, Issue 16
  • DOI: 10.1021/la800964s

Hybrid Nanorod-Polymer Solar Cells
journal, March 2002

  • Huynh, W. U.; Dittmer, Janke J.; Alivisatos, A. Paul
  • Science, Vol. 295, Issue 5564, p. 2425-2427
  • DOI: 10.1126/science.1069156

Optical properties of tetrapod-shaped CdTe nanocrystals
journal, November 2005

  • Tarì, Davide; De Giorgi, Milena; Sala, Fabio Della
  • Applied Physics Letters, Vol. 87, Issue 22
  • DOI: 10.1063/1.2130727

Multiple exciton dissociation and hot electron extraction by ultrafast interfacial electron transfer from PbS QDs
journal, March 2014


Controlled growth of tetrapod-branched inorganic nanocrystals
journal, May 2003

  • Manna, Liberato; Milliron, Delia J.; Meisel, Andreas
  • Nature Materials, Vol. 2, Issue 6, p. 382-385
  • DOI: 10.1038/nmat902

Electron−Hole Dynamics in CdTe Tetrapods
journal, August 2006

  • Malkmus, Stephan; Kudera, Stefan; Manna, Liberato
  • The Journal of Physical Chemistry B, Vol. 110, Issue 35
  • DOI: 10.1021/jp0615306

Wave Function Engineering for Ultrafast Charge Separation and Slow Charge Recombination in Type II Core/Shell Quantum Dots
journal, June 2011

  • Zhu, Haiming; Song, Nianhui; Lian, Tianquan
  • Journal of the American Chemical Society, Vol. 133, Issue 22
  • DOI: 10.1021/ja202752s

Beyond Band Alignment: Hole Localization Driven Formation of Three Spatially Separated Long-Lived Exciton States in CdSe/CdS Nanorods
journal, July 2013

  • Wu, Kaifeng; Rodríguez-Córdoba, William E.; Liu, Zheng
  • ACS Nano, Vol. 7, Issue 8
  • DOI: 10.1021/nn402597p

Spatio-temporal dynamics of coupled electrons and holes in nanosize CdSe-CdS semiconductor tetrapods
journal, August 2010


Electrons in artificial atoms
journal, February 1996


Assessment of carrier-multiplication efficiency in bulk PbSe and PbS
journal, September 2009

  • Pijpers, J. J. H.; Ulbricht, R.; Tielrooij, K. J.
  • Nature Physics, Vol. 5, Issue 11
  • DOI: 10.1038/nphys1393

Nanostructure Absorption: A Comparative Study of Nanowire and Colloidal Quantum Dot Absorption Cross Sections
journal, November 2010

  • Giblin, Jay; Kuno, Masaru
  • The Journal of Physical Chemistry Letters, Vol. 1, Issue 23
  • DOI: 10.1021/jz1013104

State-resolved studies of biexcitons and surface trapping dynamics in semiconductor quantum dots
journal, August 2008

  • Sewall, Samuel L.; Cooney, Ryan R.; Anderson, Kevin E. H.
  • The Journal of Chemical Physics, Vol. 129, Issue 8
  • DOI: 10.1063/1.2971181

The Role of Hole Localization in Sacrificial Hydrogen Production by Semiconductor–Metal Heterostructured Nanocrystals
journal, July 2011

  • Acharya, Krishna P.; Khnayzer, Rony S.; O’Connor, Timothy
  • Nano Letters, Vol. 11, Issue 7
  • DOI: 10.1021/nl201388c

Strong Electronic Coupling and Ultrafast Electron Transfer between PbS Quantum Dots and TiO 2 Nanocrystalline Films
journal, December 2011

  • Yang, Ye; Rodríguez-Córdoba, William; Xiang, Xu
  • Nano Letters, Vol. 12, Issue 1
  • DOI: 10.1021/nl2035783

Synthesis and Micrometer-Scale Assembly of Colloidal CdSe/CdS Nanorods Prepared by a Seeded Growth Approach
journal, October 2007

  • Carbone, Luigi; Nobile, Concetta; De Giorgi, Milena
  • Nano Letters, Vol. 7, Issue 10
  • DOI: 10.1021/nl0717661

A Multi-Timescale Map of Radiative and Nonradiative Decay Pathways for Excitons in CdSe Quantum Dots
journal, February 2011

  • Knowles, Kathryn E.; McArthur, Eric A.; Weiss, Emily A.
  • ACS Nano, Vol. 5, Issue 3
  • DOI: 10.1021/nn2002689

Synthesis and Characterization of Strongly Luminescing ZnS-Capped CdSe Nanocrystals
journal, January 1996

  • Hines, Margaret A.; Guyot-Sionnest, Philippe
  • The Journal of Physical Chemistry, Vol. 100, Issue 2, p. 468-471
  • DOI: 10.1021/jp9530562

Wave Function Engineering for Efficient Extraction of up to Nineteen Electrons from One CdSe/CdS Quasi-Type II Quantum Dot
journal, February 2012

  • Zhu, Haiming; Song, Nianhui; Rodríguez-Córdoba, William
  • Journal of the American Chemical Society, Vol. 134, Issue 9
  • DOI: 10.1021/ja210312s

Multiple Exciton Dissociation in CdSe Quantum Dots by Ultrafast Electron Transfer to Adsorbed Methylene Blue
journal, April 2010

  • Huang, Jier; Huang, Zhuangqun; Yang, Ye
  • Journal of the American Chemical Society, Vol. 132, Issue 13
  • DOI: 10.1021/ja100106z

Type-II Quantum Dots: CdTe/CdSe(Core/Shell) and CdSe/ZnTe(Core/Shell) Heterostructures
journal, September 2003

  • Kim, Sungjee; Fisher, Brent; Eisler, Hans-Jürgen
  • Journal of the American Chemical Society, Vol. 125, Issue 38, p. 11466-11467
  • DOI: 10.1021/ja0361749

Multiexciton Annihilation and Dissociation in Quantum Confined Semiconductor Nanocrystals
journal, November 2012

  • Zhu, Haiming; Yang, Ye; Lian, Tianquan
  • Accounts of Chemical Research, Vol. 46, Issue 6
  • DOI: 10.1021/ar300202d

Biexciton effects in femtosecond nonlinear transmission of semiconductor quantum dots
journal, September 1994


Slow Electron Cooling in Colloidal Quantum Dots
journal, November 2008


Photocatalytic Hydrogen Production with Tunable Nanorod Heterostructures
journal, March 2010

  • Amirav, Lilac; Alivisatos, A. Paul
  • The Journal of Physical Chemistry Letters, Vol. 1, Issue 7
  • DOI: 10.1021/jz100075c

Structure stability and carrier localization in Cd X ( X = S , S e , Te ) semiconductors
journal, September 2000


Hole Surface Trapping in CdSe Nanocrystals: Dynamics, Rate Fluctuations, and Implications for Blinking
journal, January 2012

  • Gómez-Campos, Francisco M.; Califano, Marco
  • Nano Letters, Vol. 12, Issue 9
  • DOI: 10.1021/nl3016279

Quantum dot solar cells
journal, April 2002