Emergent ferromagnetism and T-linear scattering in USb2 at high pressure [Emergent ferromagnetism in USb2 under pressure]

Jeffries, Jason R.; Stillwell, Ryan L.; Weir, Samuel T.; Vohra, Yogesh K.; Butch, Nicholas P.

doi:10.1103/PhysRevB.93.184406

Title: Emergent ferromagnetism and $T$ -linear scattering in $USb_{2}$ at high pressure [Emergent ferromagnetism in USb₂ under pressure]

Abstract

The material USb₂ is a correlated, moderately heavy-electron compound within the uranium dipnictide (UX₂) series. It is antiferromagnetic with a relatively high transition temperature T_N = 204K and a large U-U separation. While the uranium atoms in the lighter dipnictides are considered to be localized, those of USb₂ exhibit hybridization and itineracy, promoting uncertainty as to the continuity of the magnetic order within the UX₂. We have explored the evolution of the magnetic order by employing magnetotransport measurements as a function of pressure and temperature. We find that the T_N in USb₂ is enhanced, moving towards that of its smaller sibling UAs₂. But, long before reaching a T_N as high as UAs₂, the antiferromagnetism of USb₂ is abruptly destroyed in favor of another magnetic ground state. We identify this pressure-induced ground state as being ferromagnetic based on the appearance of a strong anomalous Hall effect in the transverse resistance in magnetic field. At last with pressure, this emergent ferromagnetic state is suppressed and ultimately destroyed in favor of a non-Fermi-liquid ground state.

Authors:

Jeffries, Jason R. ^[1]; Stillwell, Ryan L. ^[1]; Weir, Samuel T. ^[1]; Vohra, Yogesh K. ^[2]; Butch, Nicholas P. ^[3]

Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Univ. of Alabama, Birmingham, AL (United States)
National Institute of Standards and Technology, Gaithersburg, MD (United States)

Publication Date:: Mon May 09 00:00:00 EDT 2016

Research Org.:: Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)

Sponsoring Org.:: USDOE National Nuclear Security Administration (NNSA)

OSTI Identifier:: 1342040

Alternate Identifier(s):: OSTI ID: 1252120

Report Number(s):: LLNL-JRNL-681439
Journal ID: ISSN 2469-9950; PRBMDO

Grant/Contract Number:: AC52-07NA27344; 14-ERD-041; NA0002014

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Volume: 93; Journal Issue: 18; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; 36 MATERIALS SCIENCE; 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Jeffries, Jason R., Stillwell, Ryan L., Weir, Samuel T., Vohra, Yogesh K., and Butch, Nicholas P. Emergent ferromagnetism and T-linear scattering in USb2 at high pressure [Emergent ferromagnetism in USb2 under pressure].  United States: N. p., 2016. 
Web.  doi:10.1103/PhysRevB.93.184406.

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                    Jeffries, Jason R., Stillwell, Ryan L., Weir, Samuel T., Vohra, Yogesh K., & Butch, Nicholas P. Emergent ferromagnetism and T-linear scattering in USb2 at high pressure [Emergent ferromagnetism in USb2 under pressure].  United States.  https://doi.org/10.1103/PhysRevB.93.184406

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                    Jeffries, Jason R., Stillwell, Ryan L., Weir, Samuel T., Vohra, Yogesh K., and Butch, Nicholas P. Mon .  
"Emergent ferromagnetism and T-linear scattering in USb2 at high pressure [Emergent ferromagnetism in USb2 under pressure]".  United States.  https://doi.org/10.1103/PhysRevB.93.184406.  https://www.osti.gov/servlets/purl/1342040.

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@article{osti_1342040,

  title        = {Emergent ferromagnetism and T-linear scattering in USb2 at high pressure [Emergent ferromagnetism in USb2 under pressure]},

  author       = {Jeffries, Jason R. and Stillwell, Ryan L. and Weir, Samuel T. and Vohra, Yogesh K. and Butch, Nicholas P.},

  abstractNote = {The material USb2 is a correlated, moderately heavy-electron compound within the uranium dipnictide (UX2) series. It is antiferromagnetic with a relatively high transition temperature TN = 204K and a large U-U separation. While the uranium atoms in the lighter dipnictides are considered to be localized, those of USb2 exhibit hybridization and itineracy, promoting uncertainty as to the continuity of the magnetic order within the UX2. We have explored the evolution of the magnetic order by employing magnetotransport measurements as a function of pressure and temperature. We find that the TN in USb2 is enhanced, moving towards that of its smaller sibling UAs2. But, long before reaching a TN as high as UAs2, the antiferromagnetism of USb2 is abruptly destroyed in favor of another magnetic ground state. We identify this pressure-induced ground state as being ferromagnetic based on the appearance of a strong anomalous Hall effect in the transverse resistance in magnetic field. At last with pressure, this emergent ferromagnetic state is suppressed and ultimately destroyed in favor of a non-Fermi-liquid ground state.},

  doi          = {10.1103/PhysRevB.93.184406},

  journal      = {Physical Review B},

  number       = 18,

  volume       = 93,

  place        = {United States},

  year         = {Mon May 09 00:00:00 EDT 2016},

  month        = {Mon May 09 00:00:00 EDT 2016}

}

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Works referencing / citing this record:

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Nature Communications, Vol. 10, Issue 1
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Microscopic mechanism for the unusual antiferromagnetic order and the pressure-induced transition to ferromagnetism in ${USb}_{2}$
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Wysokiński, Marcin M.
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Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion
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Giannakis, Ioannis; Leshen, Justin; Kavai, Mariam
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Magnetotransport as a probe of phase transformations in metallic antiferromagnets: The case of $UIrS i_{3}$
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Physical Review B, Vol. 100, Issue 1
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Orbital-selective Kondo-lattice and enigmatic f-electrons emerging from inside the antiferromagnetic phase of a heavy fermion
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Giannakis, Ioannis; Leshen, Justin; Kavai, Mariam
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High temperature singlet-based magnetism from Hund's rule correlations
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Title: Emergent ferromagnetism and T -linear scattering in USb 2 at high pressure [Emergent ferromagnetism in USb2 under pressure]

Abstract

Citation Formats

On the temperature correction to the ruby pressure scale journal, May 1991

Cylindrical Fermi surfaces formed by a fiat magnetic Brillouin zone in uranium dipnictides journal, August 2000

Antiferromagnetic Structure of Uranium Diphosphide journal, January 1966

Actinoid pnictides—II journal, January 1978

Non-Fermi liquids journal, March 1999

Quantum critical scaling at the edge of Fermi liquid stability in a cuprate superconductor journal, May 2012

Emergence of non-Fermi-liquid behavior due to Fermi surface reconstruction in the underdoped cuprate superconductors journal, May 2010

Neutron-Diffraction Study of Antiferromagnetism in USb2 and UBi2 journal, January 1967

Unusual strong spin-fluctuation effects around the critical pressure of the itinerant Ising-type ferromagnet URhAl journal, March 2015

Ab initio study of the electronic properties and Fermi surface of the uranium dipnictides journal, January 2006

Quantum criticality journal, January 2005

Link between spin fluctuations and electron pairing in copper oxide superconductors journal, August 2011

Unusual quasiparticle renormalizations from angle resolved photoemission on USb 2 journal, August 2009

Hyperfine interactions in the antiferromagnetic states of U X 2 ( X = P , A s , S b , B i ) journal, February 2004

Crystal field interpretation of the magnetic properties of UX2 compounds (X = P, As, Sb, Bi) journal, March 1984

Incoherent non-Fermi-liquid scattering in a Kondo lattice journal, September 2007

Magnetic and transport properties of UBi 2 and USb 2 single crystals journal, April 2006

Epitaxial diamond encapsulation of metal microprobes for high pressure experiments journal, November 2000

Anisotropy of the physical properties of uniaxial antiferromagnetic USb2 journal, April 1992

Dependence of ordering temperature on pressure, carrier density and U-U distance in uranium pnictides; pressure and hall effects examinations of UP2 and USb2 journal, September 1991

Electrical and Mechanical Properties of C 70 Fullerene and Graphite under High Pressures Studied Using Designer Diamond Anvils journal, December 2000

Suppression of magnetism and development of superconductivity within the collapsed tetragonal phase of Ca 0 . 67 Sr 0 . 33 Fe 2 As 2 under pressure journal, May 2012

Calibration of the ruby pressure gauge to 800 kbar under quasi-hydrostatic conditions journal, January 1986

Magnetism and structural distortions in uranium sulfide under pressure journal, June 2013

H − T phase diagram of URu 2 Si 2 in high magnetic fields journal, July 2003

Magnetic and magnetoelastic properties of UCo 2 Si 2 as studied by high-field magnetization and ultrasound measurements journal, June 2013

Anomalous Hall effect journal, May 2010

Strongly coupled electronic, magnetic, and lattice degrees of freedom in LaC o 5 under pressure journal, November 2015

Robust ferromagnetism in the compressed permanent magnet Sm 2 Co 17 journal, September 2014

X-ray circular dichroism as a probe of orbital magnetization journal, March 1992

X-ray circular dichroism and local magnetic fields journal, February 1993

Tricritical Point and Wing Structure in the Itinerant Ferromagnet UGe 2 journal, November 2010

Ferromagnetic Quantum Critical Endpoint in UCoAl journal, September 2011

Heavy-fermion systems journal, October 1984

Non-Fermi-liquid behavior in d - and f -electron metals journal, October 2001

Quantum order-by-disorder driven phase reconstruction in the vicinity of ferromagnetic quantum critical points journal, April 2012

Heavy-fermion systems journal, November 2000

Twisting the thermoelectric potential journal, January 2021

Quantum criticality journal, February 2011

Antiferromagnetic Structure of Uranium Diphosphide book, December 1966

Emergence of non-Fermi-liquid behavior due to Fermi surface reconstruction in the underdoped cuprate superconductors text, January 2010

Quantum order-by-disorder driven phase reconstruction in the vicinity of ferromagnetic quantum critical points text, January 2012

Strongly Coupled Electronic, Magnetic, and Lattice Degrees of Freedom in LaCo5 under Pressure text, January 2015

High temperature singlet-based magnetism from Hund’s rule correlations journal, February 2019

Microscopic mechanism for the unusual antiferromagnetic order and the pressure-induced transition to ferromagnetism in USb 2 journal, January 2018

Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion journal, October 2019

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Title: Emergent ferromagnetism and $T$ -linear scattering in $USb_{2}$ at high pressure [Emergent ferromagnetism in USb₂ under pressure]

On the temperature correction to the ruby pressure scale
journal, May 1991

Cylindrical Fermi surfaces formed by a fiat magnetic Brillouin zone in uranium dipnictides
journal, August 2000

Antiferromagnetic Structure of Uranium Diphosphide
journal, January 1966

Actinoid pnictides—II
journal, January 1978

Non-Fermi liquids
journal, March 1999

Quantum critical scaling at the edge of Fermi liquid stability in a cuprate superconductor
journal, May 2012

Emergence of non-Fermi-liquid behavior due to Fermi surface reconstruction in the underdoped cuprate superconductors
journal, May 2010

Neutron-Diffraction Study of Antiferromagnetism in USb2 and UBi2
journal, January 1967

Unusual strong spin-fluctuation effects around the critical pressure of the itinerant Ising-type ferromagnet URhAl
journal, March 2015

Ab initio study of the electronic properties and Fermi surface of the uranium dipnictides
journal, January 2006

Quantum criticality
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Link between spin fluctuations and electron pairing in copper oxide superconductors
journal, August 2011

Unusual quasiparticle renormalizations from angle resolved photoemission on USb ₂
journal, August 2009

Hyperfine interactions in the antiferromagnetic states of $U X_{2}$ $(X = P, A s, S b, B i)$
journal, February 2004

Crystal field interpretation of the magnetic properties of UX2 compounds (X = P, As, Sb, Bi)
journal, March 1984

Incoherent non-Fermi-liquid scattering in a Kondo lattice
journal, September 2007

Magnetic and transport properties of UBi ₂ and USb ₂ single crystals
journal, April 2006

Epitaxial diamond encapsulation of metal microprobes for high pressure experiments
journal, November 2000

Anisotropy of the physical properties of uniaxial antiferromagnetic USb2
journal, April 1992

Dependence of ordering temperature on pressure, carrier density and U-U distance in uranium pnictides; pressure and hall effects examinations of UP2 and USb2
journal, September 1991

Electrical and Mechanical Properties of $C_{70}$ Fullerene and Graphite under High Pressures Studied Using Designer Diamond Anvils
journal, December 2000

Suppression of magnetism and development of superconductivity within the collapsed tetragonal phase of ${Ca}_{0.67} {Sr}_{0.33} {Fe}_{2} {As}_{2}$ under pressure
journal, May 2012

Calibration of the ruby pressure gauge to 800 kbar under quasi-hydrostatic conditions
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Magnetism and structural distortions in uranium sulfide under pressure
journal, June 2013

$H - T$ phase diagram of ${URu}_{2} {Si}_{2}$ in high magnetic fields
journal, July 2003

Magnetic and magnetoelastic properties of UCo $_{2}$ Si $_{2}$ as studied by high-field magnetization and ultrasound measurements
journal, June 2013

Anomalous Hall effect
journal, May 2010

Strongly coupled electronic, magnetic, and lattice degrees of freedom in $LaC o_{5}$ under pressure
journal, November 2015

Robust ferromagnetism in the compressed permanent magnet ${Sm}_{2} {Co}_{17}$
journal, September 2014

X-ray circular dichroism as a probe of orbital magnetization
journal, March 1992

X-ray circular dichroism and local magnetic fields
journal, February 1993

Tricritical Point and Wing Structure in the Itinerant Ferromagnet ${UGe}_{2}$
journal, November 2010

Ferromagnetic Quantum Critical Endpoint in UCoAl
journal, September 2011

Heavy-fermion systems
journal, October 1984

Non-Fermi-liquid behavior in $d$ - and $f$ -electron metals
journal, October 2001

Quantum order-by-disorder driven phase reconstruction in the vicinity of ferromagnetic quantum critical points
journal, April 2012

Heavy-fermion systems
journal, November 2000

Twisting the thermoelectric potential
journal, January 2021

Quantum criticality
journal, February 2011

Antiferromagnetic Structure of Uranium Diphosphide
book, December 1966

Emergence of non-Fermi-liquid behavior due to Fermi surface reconstruction in the underdoped cuprate superconductors
text, January 2010

Quantum order-by-disorder driven phase reconstruction in the vicinity of ferromagnetic quantum critical points
text, January 2012

Strongly Coupled Electronic, Magnetic, and Lattice Degrees of Freedom in LaCo5 under Pressure
text, January 2015

High temperature singlet-based magnetism from Hund’s rule correlations
journal, February 2019

Microscopic mechanism for the unusual antiferromagnetic order and the pressure-induced transition to ferromagnetism in ${USb}_{2}$
journal, January 2018

Orbital-selective Kondo lattice and enigmatic f electrons emerging from inside the antiferromagnetic phase of a heavy fermion
journal, October 2019

Magnetotransport as a probe of phase transformations in metallic antiferromagnets: The case of $UIrS i_{3}$
journal, July 2019

Orbital-selective Kondo-lattice and enigmatic f-electrons emerging from inside the antiferromagnetic phase of a heavy fermion
text, January 2019

High temperature singlet-based magnetism from Hund's rule correlations
text, January 2019