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Title: Current progress and future challenges in thermoelectric power generation: From materials to devices

Abstract

Thermoelectric power generation (TEG) represents one of the cleanest methods of energy conversion available today. It can be used in applications ranging from the harvesting of waste heat to conversion of solar energy into useful electricity. Remarkable advances have been achieved in recent years for various thermoelectric (TE) material systems. The introduction of nanostructures is used to tune the transport of phonons, while band structure engineering allows for the tailoring of electron transport. In this overview, top-down approaches to phonon engineering, such as atomic construction of new materials, will be reviewed. Bottom-up approaches to electron engineering, such as the formation of ordered nanostructures, will also be discussed. The assembly of TEG devices is still particularly challenging, and consequently, thermal-to-electric conversion utilizing these devices has been realized only in niche applications. In this review paper, we will discuss some of the challenges that must be overcome to enable widespread use of TE devices. These include thermal stability at the material level, and reliable contact at the device level.

Authors:
 [1];  [1];  [1];  [1]
  1. Univ. of Houston, TX (United States). Texas Center for Superconductivity (TcSUH)
Publication Date:
Research Org.:
Energy Frontier Research Centers (EFRC) (United States). Solid-State Solar-Thermal Energy Conversion Center (S3TEC)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1387171
Alternate Identifier(s):
OSTI ID: 1250972
Grant/Contract Number:  
SC0001299; FG02-09ER46577; SC0010831; FG02-13ER46917; DOE DE-SC0010831; EE0005806
Resource Type:
Accepted Manuscript
Journal Name:
Acta Materialia
Additional Journal Information:
Journal Volume: 87; Journal Issue: C; Related Information: S3TEC partners with Massachusetts Institute of Technology (lead); Boston College; Oak Ridge National Laboratory; Rensselaer Polytechnic Institute; Journal ID: ISSN 1359-6454
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
30 DIRECT ENERGY CONVERSION; solar (photovoltaic); solar (thermal); solid state lighting; phonons; thermal conductivity; thermoelectric; defects; mechanical behavior; charge transport; spin dynamics; materials and chemistry by design; optics; synthesis (novel materials); synthesis (self-assembly); synthesis (scalable processing)

Citation Formats

Liu, Weishu, Jie, Qing, Kim, Hee Seok, and Ren, Zhifeng. Current progress and future challenges in thermoelectric power generation: From materials to devices. United States: N. p., 2015. Web. doi:10.1016/j.actamat.2014.12.042.
Liu, Weishu, Jie, Qing, Kim, Hee Seok, & Ren, Zhifeng. Current progress and future challenges in thermoelectric power generation: From materials to devices. United States. https://doi.org/10.1016/j.actamat.2014.12.042
Liu, Weishu, Jie, Qing, Kim, Hee Seok, and Ren, Zhifeng. Sat . "Current progress and future challenges in thermoelectric power generation: From materials to devices". United States. https://doi.org/10.1016/j.actamat.2014.12.042. https://www.osti.gov/servlets/purl/1387171.
@article{osti_1387171,
title = {Current progress and future challenges in thermoelectric power generation: From materials to devices},
author = {Liu, Weishu and Jie, Qing and Kim, Hee Seok and Ren, Zhifeng},
abstractNote = {Thermoelectric power generation (TEG) represents one of the cleanest methods of energy conversion available today. It can be used in applications ranging from the harvesting of waste heat to conversion of solar energy into useful electricity. Remarkable advances have been achieved in recent years for various thermoelectric (TE) material systems. The introduction of nanostructures is used to tune the transport of phonons, while band structure engineering allows for the tailoring of electron transport. In this overview, top-down approaches to phonon engineering, such as atomic construction of new materials, will be reviewed. Bottom-up approaches to electron engineering, such as the formation of ordered nanostructures, will also be discussed. The assembly of TEG devices is still particularly challenging, and consequently, thermal-to-electric conversion utilizing these devices has been realized only in niche applications. In this review paper, we will discuss some of the challenges that must be overcome to enable widespread use of TE devices. These include thermal stability at the material level, and reliable contact at the device level.},
doi = {10.1016/j.actamat.2014.12.042},
journal = {Acta Materialia},
number = C,
volume = 87,
place = {United States},
year = {Sat Jan 31 00:00:00 EST 2015},
month = {Sat Jan 31 00:00:00 EST 2015}
}

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Cited by: 392 works
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