Induced Ti magnetization at La0.7Sr0.3MnO3 and BaTiO3 interfaces

Liu, Yaohua; Tornos, J.; te Velthuis, S. G.  E.; Freeland, J. W.; Zhou, H.; Steadman, P.; Bencok, P.; Leon, C.; Santamaria, J.

doi:10.1063/1.4946756

Title: Induced Ti magnetization at La_0.7Sr_0.3MnO₃ and BaTiO₃ interfaces

Abstract

In artificial multiferroics hybrids consisting of ferromagnetic La_0.7Sr_0.3MnO₃ (LSMO) and ferroelectric BaTiO₃ epitaxial layers, net Ti moments are found from polarized resonant soft x-ray reflectivity and absorption. The Ti dichroic reflectivity follows the Mn signal during the magnetization reversal, indicating exchange coupling between the Ti and Mn ions. However, the Ti dichroic reflectivity shows stronger temperature dependence than the Mn dichroic signal. Lastly, besides a reduced ferromagnetic exchange coupling in the interfacial LSMO layer, this may also be attributed to a weak Ti-Mn exchange coupling that is insufficient to overcome the thermal energy at elevated temperatures.

Authors:

^[1];

^[2]; te Velthuis, S. G. E. ^[3];

^[3]; Zhou, H. ^[3]; Steadman, P. ^[4]; Bencok, P. ^[4];

^[2]; Santamaria, J. ^[2]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Argonne National Lab. (ANL), Argonne, IL (United States)
Complutense University of Madrid (Spain)
Argonne National Lab. (ANL), Argonne, IL (United States)
Diamond Light Source, Didcot (United Kingdom)

Publication Date:: Fri Apr 01 00:00:00 EDT 2016

Research Org.:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1248790

Alternate Identifier(s):: OSTI ID: 1258773; OSTI ID: 1352669

Grant/Contract Number:: AC05-00OR22725; AC02-06CH11357

Resource Type:: Accepted Manuscript

Journal Name:: APL Materials

Additional Journal Information:: Journal Volume: 4; Journal Issue: 4; Journal ID: ISSN 2166-532X

Publisher:: American Institute of Physics (AIP)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; reflectivity; ferromagnetism; interfacial properties; magnetic resonance; X-ray absorption spectra

Citation Formats


                    Liu, Yaohua, Tornos, J., te Velthuis, S. G.  E., Freeland, J. W., Zhou, H., Steadman, P., Bencok, P., Leon, C., and Santamaria, J. Induced Ti magnetization at La0.7Sr0.3MnO3 and BaTiO3 interfaces.  United States: N. p., 2016. 
Web.  doi:10.1063/1.4946756.

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                    Liu, Yaohua, Tornos, J., te Velthuis, S. G.  E., Freeland, J. W., Zhou, H., Steadman, P., Bencok, P., Leon, C., & Santamaria, J. Induced Ti magnetization at La0.7Sr0.3MnO3 and BaTiO3 interfaces.  United States.  https://doi.org/10.1063/1.4946756

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                    Liu, Yaohua, Tornos, J., te Velthuis, S. G.  E., Freeland, J. W., Zhou, H., Steadman, P., Bencok, P., Leon, C., and Santamaria, J. Fri .  
"Induced Ti magnetization at La0.7Sr0.3MnO3 and BaTiO3 interfaces".  United States.  https://doi.org/10.1063/1.4946756.  https://www.osti.gov/servlets/purl/1248790.

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@article{osti_1248790,

  title        = {Induced Ti magnetization at La0.7Sr0.3MnO3 and BaTiO3 interfaces},

  author       = {Liu, Yaohua and Tornos, J. and te Velthuis, S. G.  E. and Freeland, J. W. and Zhou, H. and Steadman, P. and Bencok, P. and Leon, C. and Santamaria, J.},

  abstractNote = {In artificial multiferroics hybrids consisting of ferromagnetic La0.7Sr0.3MnO3 (LSMO) and ferroelectric BaTiO3 epitaxial layers, net Ti moments are found from polarized resonant soft x-ray reflectivity and absorption. The Ti dichroic reflectivity follows the Mn signal during the magnetization reversal, indicating exchange coupling between the Ti and Mn ions. However, the Ti dichroic reflectivity shows stronger temperature dependence than the Mn dichroic signal. Lastly, besides a reduced ferromagnetic exchange coupling in the interfacial LSMO layer, this may also be attributed to a weak Ti-Mn exchange coupling that is insufficient to overcome the thermal energy at elevated temperatures.},

  doi          = {10.1063/1.4946756},

  journal      = {APL Materials},

  number       = 4,

  volume       = 4,

  place        = {United States},

  year         = {Fri Apr 01 00:00:00 EDT 2016},

  month        = {Fri Apr 01 00:00:00 EDT 2016}

}

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Works referencing / citing this record:

Magneto-dynamic properties of complex oxide—La _0.7 Sr _0.3 MnO ₃ /SrTiO ₃ —heterostructure interface
journal, June 2019

Singh, Suraj; Bolstad, Torstein; Hallsteinsen, Ingrid
Applied Physics Letters, Vol. 114, Issue 22
DOI: 10.1063/1.5093324

Strain induced extrinsic magnetocaloric effects in La _0.67 Sr _0.33 MnO ₃ thin films, controlled by magnetic field
journal, February 2019

Giri, S. K.; MacManus-Driscoll, J. L.; Li, W.
Journal of Physics D: Applied Physics, Vol. 52, Issue 16
DOI: 10.1088/1361-6463/ab03be

Strain induced extrinsic magnetocaloric effects in La 0.67 Sr 0.33 MnO 3 thin films, controlled by magnetic field
text, January 2019

Giri, Sk; MacManus-Driscoll, Jl; Li, Weiwei
Apollo - University of Cambridge Repository
DOI: 10.17863/cam.38097

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Title: Induced Ti magnetization at La0.7Sr0.3MnO3 and BaTiO3 interfaces

Abstract

Citation Formats

Interface Physics in Complex Oxide Heterostructures journal, March 2011

Induced Magnetism at Oxide Interfaces journal, July 2013

Colloquium : Emergent properties in plane view: Strong correlations at oxide interfaces journal, October 2014

Interfacial magnetism in complex oxide heterostructures probed by neutrons and x-rays journal, September 2015

A high-mobility electron gas at the LaAlO3/SrTiO3 heterointerface journal, January 2004

Superconducting Interfaces Between Insulating Oxides journal, August 2007

Magnetic effects at the interface between non-magnetic oxides journal, June 2007

Emergent Spin Filter at the Interface between Ferromagnetic and Insulating Layered Oxides journal, December 2013

Magnetoelectric Devices for Spintronics journal, July 2014

Origin of the Magnetoelectric Coupling Effect in Pb ( Zr 0.2 Ti 0.8 ) O 3 / La 0.8 Sr 0.2 MnO 3 Multiferroic Heterostructures journal, March 2010

Electric modulation of magnetization at the BaTiO 3 /La 0.67 Sr 0.33 MnO 3 interfaces journal, June 2012

Tunnel junctions with multiferroic barriers journal, March 2007

Ferroelectric and multiferroic tunnel junctions journal, February 2012

Enhanced tunnelling electroresistance effect due to a ferroelectrically induced phase transition at a magnetic complex oxide interface journal, February 2013

Orbital Reconstruction and Covalent Bonding at an Oxide Interface journal, November 2007

Tunable Magnetic Interaction at the Atomic Scale in Oxide Heterostructures journal, October 2010

Correlating interfacial octahedral rotations with magnetism in (LaMnO3+δ)N/(SrTiO3)N superlattices journal, July 2014

Magnetic Oxide Heterostructures journal, July 2014

Reversible Control of Co Magnetism by Voltage-Induced Oxidation journal, December 2014

Ferromagnetic/superconducting proximity effect in La 0.7 Ca 0.3 MnO 3 / YBa 2 Cu 3 O 7 − δ superlattices journal, June 2003

Dichroic interference effects in circularly polarized soft-x-ray resonant magnetic scattering journal, October 1994

Suppressed magnetization at the surfaces and interfaces of ferromagnetic metallic manganites journal, July 2007

A unique polarized x-ray facility at the Advanced Photon Source journal, March 2002

Origin of Interface Magnetism in BiMnO 3 / SrTiO 3 and LaAlO 3 / SrTiO 3 Heterostructures journal, August 2013

Interface-induced room-temperature multiferroicity in BaTiO3 journal, August 2011

Electronic and Magnetic Reconstructions in La 0.7 Sr 0.3 MnO 3 / SrTiO 3 Heterostructures: A Case of Enhanced Interlayer Coupling Controlled by the Interface journal, April 2011

X-ray circular dichroism and local magnetic fields journal, February 1993

Magnetic Properties at Surface Boundary of a Half-Metallic Ferromagnet La 0.7 Sr 0.3 MnO 3 journal, August 1998

Nanoscale suppression of magnetization at atomically assembled manganite interfaces: XMCD and XRMS measurements journal, July 2007

Visualizing short-range charge transfer at the interfaces between ferromagnetic and superconducting oxides journal, August 2013

Magneto-dynamic properties of complex oxide—La 0.7 Sr 0.3 MnO 3 /SrTiO 3 —heterostructure interface journal, June 2019

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Title: Induced Ti magnetization at La_0.7Sr_0.3MnO₃ and BaTiO₃ interfaces

Interface Physics in Complex Oxide Heterostructures
journal, March 2011

Induced Magnetism at Oxide Interfaces
journal, July 2013

Colloquium : Emergent properties in plane view: Strong correlations at oxide interfaces
journal, October 2014

Interfacial magnetism in complex oxide heterostructures probed by neutrons and x-rays
journal, September 2015

A high-mobility electron gas at the LaAlO3/SrTiO3 heterointerface
journal, January 2004

Superconducting Interfaces Between Insulating Oxides
journal, August 2007

Magnetic effects at the interface between non-magnetic oxides
journal, June 2007

Emergent Spin Filter at the Interface between Ferromagnetic and Insulating Layered Oxides
journal, December 2013

Magnetoelectric Devices for Spintronics
journal, July 2014

Origin of the Magnetoelectric Coupling Effect in $Pb ({Zr}_{0.2} {Ti}_{0.8}) O_{3} / {La}_{0.8} {Sr}_{0.2} {MnO}_{3}$ Multiferroic Heterostructures
journal, March 2010

Electric modulation of magnetization at the BaTiO ₃ /La _0.67 Sr _0.33 MnO ₃ interfaces
journal, June 2012

Tunnel junctions with multiferroic barriers
journal, March 2007

Ferroelectric and multiferroic tunnel junctions
journal, February 2012

Enhanced tunnelling electroresistance effect due to a ferroelectrically induced phase transition at a magnetic complex oxide interface
journal, February 2013

Orbital Reconstruction and Covalent Bonding at an Oxide Interface
journal, November 2007

Tunable Magnetic Interaction at the Atomic Scale in Oxide Heterostructures
journal, October 2010

Correlating interfacial octahedral rotations with magnetism in (LaMnO3+δ)N/(SrTiO3)N superlattices
journal, July 2014

Magnetic Oxide Heterostructures
journal, July 2014

Reversible Control of Co Magnetism by Voltage-Induced Oxidation
journal, December 2014

Ferromagnetic/superconducting proximity effect in ${La}_{0.7} {Ca}_{0.3} {MnO}_{3} / {YBa}_{2} {Cu}_{3} O_{7 - δ}$ superlattices
journal, June 2003

Dichroic interference effects in circularly polarized soft-x-ray resonant magnetic scattering
journal, October 1994

Suppressed magnetization at the surfaces and interfaces of ferromagnetic metallic manganites
journal, July 2007

A unique polarized x-ray facility at the Advanced Photon Source
journal, March 2002

Origin of Interface Magnetism in ${BiMnO}_{3} / {SrTiO}_{3}$ and ${LaAlO}_{3} / {SrTiO}_{3}$ Heterostructures
journal, August 2013

Interface-induced room-temperature multiferroicity in BaTiO3
journal, August 2011

Electronic and Magnetic Reconstructions in ${La}_{0.7} {Sr}_{0.3} {MnO}_{3} / {SrTiO}_{3}$ Heterostructures: A Case of Enhanced Interlayer Coupling Controlled by the Interface
journal, April 2011

X-ray circular dichroism and local magnetic fields
journal, February 1993

Magnetic Properties at Surface Boundary of a Half-Metallic Ferromagnet ${La}_{0.7} {Sr}_{0.3} {MnO}_{3}$
journal, August 1998

Nanoscale suppression of magnetization at atomically assembled manganite interfaces: XMCD and XRMS measurements
journal, July 2007

Visualizing short-range charge transfer at the interfaces between ferromagnetic and superconducting oxides
journal, August 2013

Magneto-dynamic properties of complex oxide—La _0.7 Sr _0.3 MnO ₃ /SrTiO ₃ —heterostructure interface
journal, June 2019

Strain induced extrinsic magnetocaloric effects in La _0.67 Sr _0.33 MnO ₃ thin films, controlled by magnetic field
journal, February 2019

Strain induced extrinsic magnetocaloric effects in La 0.67 Sr 0.33 MnO 3 thin films, controlled by magnetic field
text, January 2019