Low-temperature fabrication of efficient wide-bandgap organolead trihalide perovskite solar cells
Abstract
A mixed halide perovskite solar cell with a 1.72 eV bandgap is developed by incorporating Br into perovskite through a low-temperature solution process. A high efficiency of 13.1% is achieved by carefully tuning the thickness, morphology, and surface passivation of the perovskite layers. Furthermore, the fabrication techniques and conditions are compatible with future perovskite/Si tandem cell studies.
- Authors:
-
- Univ. of Nebraska, Lincoln, NE (United States)
- Publication Date:
- Research Org.:
- Univ. of Nebraska, Lincoln, NE (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1237998
- Grant/Contract Number:
- EE0006709
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Energy Materials
- Additional Journal Information:
- Journal Volume: 5; Journal Issue: 6; Journal ID: ISSN 1614-6832
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 14 SOLAR ENERGY; 36 MATERIALS SCIENCE
Citation Formats
Bi, Cheng, Yuan, Yongbo, Fang, Yanjun, and Huang, Jinsong. Low-temperature fabrication of efficient wide-bandgap organolead trihalide perovskite solar cells. United States: N. p., 2014.
Web. doi:10.1002/aenm.201401616.
Bi, Cheng, Yuan, Yongbo, Fang, Yanjun, & Huang, Jinsong. Low-temperature fabrication of efficient wide-bandgap organolead trihalide perovskite solar cells. United States. https://doi.org/10.1002/aenm.201401616
Bi, Cheng, Yuan, Yongbo, Fang, Yanjun, and Huang, Jinsong. Tue .
"Low-temperature fabrication of efficient wide-bandgap organolead trihalide perovskite solar cells". United States. https://doi.org/10.1002/aenm.201401616. https://www.osti.gov/servlets/purl/1237998.
@article{osti_1237998,
title = {Low-temperature fabrication of efficient wide-bandgap organolead trihalide perovskite solar cells},
author = {Bi, Cheng and Yuan, Yongbo and Fang, Yanjun and Huang, Jinsong},
abstractNote = {A mixed halide perovskite solar cell with a 1.72 eV bandgap is developed by incorporating Br into perovskite through a low-temperature solution process. A high efficiency of 13.1% is achieved by carefully tuning the thickness, morphology, and surface passivation of the perovskite layers. Furthermore, the fabrication techniques and conditions are compatible with future perovskite/Si tandem cell studies.},
doi = {10.1002/aenm.201401616},
journal = {Advanced Energy Materials},
number = 6,
volume = 5,
place = {United States},
year = {Tue Nov 25 00:00:00 EST 2014},
month = {Tue Nov 25 00:00:00 EST 2014}
}
Free Publicly Available Full Text
Publisher's Version of Record
Other availability
Search WorldCat to find libraries that may hold this journal
Cited by: 145 works
Citation information provided by
Web of Science
Web of Science
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.
Works referenced in this record:
High efficiency AlGaAs/Si monolithic tandem solar cell grown by metalorganic chemical vapor deposition
journal, September 1995
- Soga, T.; Kato, T.; Yang, M.
- Journal of Applied Physics, Vol. 78, Issue 6
Efficient planar heterojunction perovskite solar cells by vapour deposition
journal, September 2013
- Liu, Mingzhen; Johnston, Michael B.; Snaith, Henry J.
- Nature, Vol. 501, Issue 7467, p. 395-398
Sub-150 °C processed meso-superstructured perovskite solar cells with enhanced efficiency
journal, January 2014
- Wojciechowski, Konrad; Saliba, Michael; Leijtens, Tomas
- Energy Environ. Sci., Vol. 7, Issue 3
Solvent engineering for high-performance inorganic–organic hybrid perovskite solar cells
journal, July 2014
- Jeon, Nam Joong; Noh, Jun Hong; Kim, Young Chan
- Nature Materials, Vol. 13, Issue 9, p. 897-903
Sequential deposition as a route to high-performance perovskite-sensitized solar cells
journal, July 2013
- Burschka, Julian; Pellet, Norman; Moon, Soo-Jin
- Nature, Vol. 499, Issue 7458, p. 316-319
Chemical Management for Colorful, Efficient, and Stable Inorganic–Organic Hybrid Nanostructured Solar Cells
journal, March 2013
- Noh, Jun Hong; Im, Sang Hyuk; Heo, Jin Hyuck
- Nano Letters, Vol. 13, Issue 4, p. 1764-1769
Hybrid Lead Halide Iodide and Lead Halide Bromide in Efficient Hole Conductor Free Perovskite Solar Cell
journal, May 2014
- Aharon, Sigalit; Cohen, Bat El; Etgar, Lioz
- The Journal of Physical Chemistry C, Vol. 118, Issue 30
Recombination Study of Combined Halides (Cl, Br, I) Perovskite Solar Cells
journal, April 2014
- Suarez, Belen; Gonzalez-Pedro, Victoria; Ripolles, Teresa S.
- The Journal of Physical Chemistry Letters, Vol. 5, Issue 10
Voltage output of efficient perovskite solar cells with high open-circuit voltage and fill factor
journal, January 2014
- Ryu, Seungchan; Noh, Jun Hong; Jeon, Nam Joong
- Energy Environ. Sci., Vol. 7, Issue 8
CH 3 NH 3 Sn x Pb (1– x ) I 3 Perovskite Solar Cells Covering up to 1060 nm
journal, March 2014
- Ogomi, Yuhei; Morita, Atsushi; Tsukamoto, Syota
- The Journal of Physical Chemistry Letters, Vol. 5, Issue 6
Optical properties of CH3NH3PbX3 (X = halogen) and their mixed-halide crystals
journal, January 2002
- Kitazawa, N.; Watanabe, Y.; Nakamura, Y.
- Journal of Materials Science, Vol. 37, Issue 17, p. 3585-3587
All-solid-state hybrid solar cells based on a new organometal halide perovskite sensitizer and one-dimensional TiO2 nanowire arrays
journal, January 2013
- Qiu, Jianhang; Qiu, Yongcai; Yan, Keyou
- Nanoscale, Vol. 5, Issue 8
High performance hybrid solar cells sensitized by organolead halide perovskites
journal, January 2013
- Cai, Bing; Xing, Yedi; Yang, Zhou
- Energy & Environmental Science, Vol. 6, Issue 5
Efficient Planar Perovskite Solar Cells Based on 1.8 eV Band Gap CH 3 NH 3 PbI 2 Br Nanosheets via Thermal Decomposition
journal, August 2014
- Zhao, Yixin; Zhu, Kai
- Journal of the American Chemical Society, Vol. 136, Issue 35
High-Performance Planar-Heterojunction Solar Cells Based on Ternary Halide Large-Band-Gap Perovskites
journal, August 2014
- Liang, Po-Wei; Chueh, Chu-Chen; Xin, Xu-Kai
- Advanced Energy Materials, Vol. 5, Issue 1
The Role of Intrinsic Defects in Methylammonium Lead Iodide Perovskite
journal, March 2014
- Kim, Jongseob; Lee, Sung-Hoon; Lee, Jung Hoon
- The Journal of Physical Chemistry Letters, Vol. 5, Issue 8
Unusual defect physics in CH 3 NH 3 PbI 3 perovskite solar cell absorber
journal, February 2014
- Yin, Wan-Jian; Shi, Tingting; Yan, Yanfa
- Applied Physics Letters, Vol. 104, Issue 6
Unique Properties of Halide Perovskites as Possible Origins of the Superior Solar Cell Performance
journal, May 2014
- Yin, Wan-Jian; Shi, Tingting; Yan, Yanfa
- Advanced Materials, Vol. 26, Issue 27
Large fill-factor bilayer iodine perovskite solar cells fabricated by a low-temperature solution-process
journal, January 2014
- Wang, Qi; Shao, Yuchuan; Dong, Qingfeng
- Energy Environ. Sci., Vol. 7, Issue 7
Origin and elimination of photocurrent hysteresis by fullerene passivation in CH3NH3PbI3 planar heterojunction solar cells
journal, December 2014
- Shao, Yuchuan; Xiao, Zhengguo; Bi, Cheng
- Nature Communications, Vol. 5, Issue 1
Effect of Annealing Temperature on Film Morphology of Organic-Inorganic Hybrid Pervoskite Solid-State Solar Cells
journal, February 2014
- Dualeh, Amalie; Tétreault, Nicolas; Moehl, Thomas
- Advanced Functional Materials, Vol. 24, Issue 21, p. 3250-3258
Understanding the formation and evolution of interdiffusion grown organolead halide perovskite thin films by thermal annealing
journal, January 2014
- Bi, Cheng; Shao, Yuchuan; Yuan, Yongbo
- J. Mater. Chem. A, Vol. 2, Issue 43
Solvent Annealing of Perovskite-Induced Crystal Growth for Photovoltaic-Device Efficiency Enhancement
journal, August 2014
- Xiao, Zhengguo; Dong, Qingfeng; Bi, Cheng
- Advanced Materials, Vol. 26, Issue 37
Determination of defect distributions from admittance measurements and application to Cu(In,Ga)Se 2 based heterojunctions
journal, October 1996
- Walter, T.; Herberholz, R.; Müller, C.
- Journal of Applied Physics, Vol. 80, Issue 8
Hole Transport in Poly(phenylene vinylene)/Methanofullerene Bulk-Heterojunction Solar Cells
journal, September 2004
- Melzer, C.; Koop, E. J.; Mihailetchi, V. D.
- Advanced Functional Materials, Vol. 14, Issue 9
Efficient Hybrid Solar Cells Based on Meso-Superstructured Organometal Halide Perovskites
journal, October 2012
- Lee, M. M.; Teuscher, J.; Miyasaka, T.
- Science, Vol. 338, Issue 6107, p. 643-647
Works referencing / citing this record:
Bright Light-Emitting Diodes Based on Organometal Halide Perovskite Nanoplatelets
journal, November 2015
- Ling, Yichuan; Yuan, Zhao; Tian, Yu
- Advanced Materials, Vol. 28, Issue 2
Efficient Flexible Solar Cell based on Composition-Tailored Hybrid Perovskite
journal, June 2017
- Bi, Cheng; Chen, Bo; Wei, Haotong
- Advanced Materials, Vol. 29, Issue 30
Matching Charge Extraction Contact for Wide-Bandgap Perovskite Solar Cells
journal, May 2017
- Lin, Yuze; Chen, Bo; Zhao, Fuwen
- Advanced Materials, Vol. 29, Issue 26
Nonradiative Recombination in Perovskite Solar Cells: The Role of Interfaces
journal, October 2019
- Wolff, Christian M.; Caprioglio, Pietro; Stolterfoht, Martin
- Advanced Materials, Vol. 31, Issue 52
Structure and Growth Control of Organic-Inorganic Halide Perovskites for Optoelectronics: From Polycrystalline Films to Single Crystals
journal, March 2016
- Chen, Yani; He, Minhong; Peng, Jiajun
- Advanced Science, Vol. 3, Issue 4
Solid‐State Ligand‐Exchange Fabrication of CH 3 NH 3 PbI 3 Capped PbS Quantum Dot Solar Cells
journal, February 2016
- Peng, Jiajun; Chen, Yani; Zhang, Xianfeng
- Advanced Science, Vol. 3, Issue 6
TiO 2 Phase Junction Electron Transport Layer Boosts Efficiency of Planar Perovskite Solar Cells
journal, January 2018
- Zhu, Yayun; Deng, Kaimo; Sun, Haoxuan
- Advanced Science, Vol. 5, Issue 3
Improving Film Formation and Photovoltage of Highly Efficient Inverted-Type Perovskite Solar Cells through the Incorporation of New Polymeric Hole Selective Layers
journal, December 2015
- Xue, Qifan; Chen, Guiting; Liu, Meiyue
- Advanced Energy Materials, Vol. 6, Issue 5
Solvent-Mediated Dimension Tuning of Semiconducting Oxide Nanostructures as Efficient Charge Extraction Thin Films for Perovskite Solar Cells with Efficiency Exceeding 16%
journal, January 2016
- Wu, Wu-Qiang; Huang, Fuzhi; Chen, Dehong
- Advanced Energy Materials, Vol. 6, Issue 7
Inverted Perovskite Solar Cells: Progresses and Perspectives
journal, May 2016
- Liu, Tanghao; Chen, Ke; Hu, Qin
- Advanced Energy Materials, Vol. 6, Issue 17
Progress in Tandem Solar Cells Based on Hybrid Organic-Inorganic Perovskites
journal, March 2017
- Chen, Bo; Zheng, Xiaopeng; Bai, Yang
- Advanced Energy Materials, Vol. 7, Issue 14
Improving the Performance and Stability of Inverted Planar Flexible Perovskite Solar Cells Employing a Novel NDI-Based Polymer as the Electron Transport Layer
journal, February 2018
- Kim, Hong Il; Kim, Myeong-Jong; Choi, Kyoungwon
- Advanced Energy Materials, Vol. 8, Issue 16
Interface Modification by Ionic Liquid: A Promising Candidate for Indoor Light Harvesting and Stability Improvement of Planar Perovskite Solar Cells
journal, July 2018
- Li, Meng; Zhao, Chao; Wang, Zhao-Kui
- Advanced Energy Materials, Vol. 8, Issue 24
Effect of Halide Composition on the Photochemical Stability of Perovskite Photovoltaic Materials
journal, August 2016
- Misra, Ravi K.; Ciammaruchi, Laura; Aharon, Sigalit
- ChemSusChem, Vol. 9, Issue 18
Recent Progress in Organic Electron Transport Materials in Inverted Perovskite Solar Cells
journal, April 2019
- Said, Ahmed Ali; Xie, Jian; Zhang, Qichun
- Small, Vol. 15, Issue 27
Perovskite Solar Cells: Optoelectronic Simulation and Optimization
journal, July 2018
- An, Yidan; Shang, Aixue; Cao, Guoyang
- Solar RRL, Vol. 2, Issue 11
An efficient, flexible perovskite solar module exceeding 8% prepared with an ultrafast PbI2 deposition rate
journal, January 2018
- Li, Kunpeng; Xiao, Junyan; Yu, Xinxin
- Scientific Reports, Vol. 8, Issue 1
Room-temperature solution-processed and metal oxide-free nano-composite for the flexible transparent bottom electrode of perovskite solar cells
journal, January 2016
- Lu, Haifei; Sun, Jingsong; Zhang, Hong
- Nanoscale, Vol. 8, Issue 11
MAPbI 3−x Br x mixed halide perovskites for fully printable mesoscopic solar cells with enhanced efficiency and less hysteresis
journal, January 2016
- Cao, Kun; Li, Hao; Liu, ShuangShuang
- Nanoscale, Vol. 8, Issue 16
Effect of BCP buffer layer on eliminating charge accumulation for high performance of inverted perovskite solar cells
journal, January 2017
- Chen, Chuanliang; Zhang, Shasha; Wu, Shaohang
- RSC Advances, Vol. 7, Issue 57
The synergistic effect of cooperating solvent vapor annealing for high-efficiency planar inverted perovskite solar cells
journal, January 2019
- Yi, Ahra; Chae, Sangmin; Lee, Hanbin
- Journal of Materials Chemistry A, Vol. 7, Issue 48
Wide-bandgap, low-bandgap, and tandem perovskite solar cells
journal, July 2019
- Song, Zhaoning; Chen, Cong; Li, Chongwen
- Semiconductor Science and Technology, Vol. 34, Issue 9
Matching Charge Extraction Contact for Wide-Bandgap Perovskite Solar Cells
text, January 2017
- B., Chen,; Y., Shao,; J., Huang,
- The University of North Carolina at Chapel Hill University Libraries
Nonradiative Recombination in Perovskite Solar Cells: The Role of Interfaces
text, January 2019
- Wolff, Christian M.; Caprioglio, Pietro; Stolterfoht, Martin
- FID GEO
Effect of Halide Composition on the Photochemical Stability of Perovskite Photovoltaic Materials
text, January 2016
- Misra, Ravi K.; Ciammaruchi, Laura; Aharon, Sigalit
- arXiv