Revisited reaction-diffusion model of thermal desorption spectroscopy experiments on hydrogen retention in material

Guterl, Jerome; Smirnov, R. D.; Krasheninnikov, S. I.

doi:10.1063/1.4926546

Title: Revisited reaction-diffusion model of thermal desorption spectroscopy experiments on hydrogen retention in material

Authors:

^[1]; Smirnov, R. D. ^[1]; Krasheninnikov, S. I. ^[1]

University of California San Diego, La Jolla, California 92093, USA

Publication Date:: Tue Jul 28 00:00:00 EDT 2015

Sponsoring Org.:: USDOE

OSTI Identifier:: 1228709

Grant/Contract Number:: FG02-04ER54739; SC0001999

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Journal of Applied Physics

Additional Journal Information:: Journal Name: Journal of Applied Physics Journal Volume: 118 Journal Issue: 4; Journal ID: ISSN 0021-8979

Publisher:: American Institute of Physics

Country of Publication:: United States

Language:: English

Citation Formats


                    Guterl, Jerome, Smirnov, R. D., and Krasheninnikov, S. I. Revisited reaction-diffusion model of thermal desorption spectroscopy experiments on hydrogen retention in material.  United States: N. p., 2015. 
Web.  doi:10.1063/1.4926546.

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                    Guterl, Jerome, Smirnov, R. D., & Krasheninnikov, S. I. Revisited reaction-diffusion model of thermal desorption spectroscopy experiments on hydrogen retention in material.  United States.  https://doi.org/10.1063/1.4926546

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                    Guterl, Jerome, Smirnov, R. D., and Krasheninnikov, S. I. Tue .  
"Revisited reaction-diffusion model of thermal desorption spectroscopy experiments on hydrogen retention in material".  United States.  https://doi.org/10.1063/1.4926546.

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@article{osti_1228709,

  title        = {Revisited reaction-diffusion model of thermal desorption spectroscopy experiments on hydrogen retention in material},

  author       = {Guterl, Jerome and Smirnov, R. D. and Krasheninnikov, S. I.},

  abstractNote = {},

  doi          = {10.1063/1.4926546},

  journal      = {Journal of Applied Physics},

  number       = 4,

  volume       = 118,

  place        = {United States},

  year         = {Tue Jul 28 00:00:00 EDT 2015},

  month        = {Tue Jul 28 00:00:00 EDT 2015}

}

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Works referenced in this record:

Hydrogen diffusion and vacancies formation in tungsten: Density Functional Theory calculations and statistical models
journal, August 2015

Fernandez, N.; Ferro, Y.; Kato, D.
Acta Materialia, Vol. 94
DOI: 10.1016/j.actamat.2015.04.052

Towards a better understanding of hydrogen measurements obtained by thermal desorption spectroscopy using FEM modeling
journal, February 2015

Legrand, E.; Oudriss, A.; Savall, C.
International Journal of Hydrogen Energy, Vol. 40, Issue 6
DOI: 10.1016/j.ijhydene.2014.12.069

Thermal desorption from metal surfaces: A review
journal, January 1975

King, David A.
Surface Science, Vol. 47, Issue 1
DOI: 10.1016/0039-6028(75)90302-7

Surface morphology and deuterium retention of tungsten after low- and high-flux deuterium plasma exposure
journal, June 2014

't Hoen, M. H. J.; Balden, M.; Manhard, A.
Nuclear Fusion, Vol. 54, Issue 8
DOI: 10.1088/0029-5515/54/8/083014

Recent analysis of key plasma wall interactions issues for ITER
journal, June 2009

Roth, Joachim; Tsitrone, E.; Loarte, A.
Journal of Nuclear Materials, Vol. 390-391
DOI: 10.1016/j.jnucmat.2009.01.037

Depth distribution of deuterium in single- and polycrystalline tungsten up to depths of several micrometers
journal, March 2005

Alimov, V. Kh.; Roth, J.; Mayer, M.
Journal of Nuclear Materials, Vol. 337-339
DOI: 10.1016/j.jnucmat.2004.10.082

Deuterium release from implanted beryllium and beryllium oxide
journal, August 2011

Oberkofler, M.; Linsmeier, Ch.
Journal of Nuclear Materials, Vol. 415, Issue 1
DOI: 10.1016/j.jnucmat.2010.11.015

Hydrogen Storage Material Composed of Polyacetylene and LiH and Investigation of Its Mechanisms
journal, July 2014

Yoshida, Akihiro; Okuyama, Takashi; Mori, Yoshinori
Chemistry of Materials, Vol. 26, Issue 14
DOI: 10.1021/cm500042c

Modelling deuterium release during thermal desorption of D+-irradiated tungsten
journal, March 2008

Poon, M.; Haasz, A. A.; Davis, J. W.
Journal of Nuclear Materials, Vol. 374, Issue 3
DOI: 10.1016/j.jnucmat.2007.09.028

Solution and Diffusion of Hydrogen in Tungsten
journal, May 1969

Frauenfelder, R.
Journal of Vacuum Science and Technology, Vol. 6, Issue 3
DOI: 10.1116/1.1492699

Numerical modeling of thermal desorption mass spectroscopy (TDS) for the study of hydrogen diffusion and trapping interactions in metals
journal, March 2015

Hurley, Caitlin; Martin, Frantz; Marchetti, Loïc
International Journal of Hydrogen Energy, Vol. 40, Issue 8
DOI: 10.1016/j.ijhydene.2015.01.001

Experiments on the release of tritium from the first wall of JET
journal, September 1993

Andrew, P.; Coad, J. P.; Ehrenberg, J.
Nuclear Fusion, Vol. 33, Issue 9
DOI: 10.1088/0029-5515/33/9/I11

Comparison of hydrogen retention in W and W/Ta alloys
journal, July 2012

Schmid, K.; Rieger, V.; Manhard, A.
Journal of Nuclear Materials, Vol. 426, Issue 1-3
DOI: 10.1016/j.jnucmat.2012.04.003

Modelling of monovacancy diffusion in W over wide temperature range
journal, March 2014

Bukonte, L.; Ahlgren, T.; Heinola, K.
Journal of Applied Physics, Vol. 115, Issue 12
DOI: 10.1063/1.4869497

Modeling of Hydrogen Retention and Outgassing from Co-Deposits with Distributed Energy States: Modeling of Hydrogen Retention and Outgassing from Co-Deposits with Distributed Energy States
journal, June 2014

Smirnov, R. D.; Krasheninnikov, S. I.; Guterl, J.
Contributions to Plasma Physics, Vol. 54, Issue 4-6
DOI: 10.1002/ctpp.201410033

Long-Term Hydrogen Outgassing from Plasma Facing Components: Long-Term Hydrogen Outgassing from Plasma Facing Components
journal, June 2014

Guterl, J.; Smirnov, R. D.; Krasheninnikov, S. I.
Contributions to Plasma Physics, Vol. 54, Issue 4-6
DOI: 10.1002/ctpp.201410034

Hydrogen isotope retention and recycling in fusion reactor plasma-facing components
journal, February 2002

Causey, Rion A.
Journal of Nuclear Materials, Vol. 300, Issue 2-3
DOI: 10.1016/S0022-3115(01)00732-2

Hydrogen interaction with point defects in tungsten
journal, September 2010

Heinola, K.; Ahlgren, T.; Nordlund, K.
Physical Review B, Vol. 82, Issue 9
DOI: 10.1103/PhysRevB.82.094102

Hydrogen transport in solids with traps in the case of continuum distribution of detrapping energies
journal, April 2014

Krasheninnikov, S. I.; Marenkov, E. D.; Smirnov, R. D.
Physica Scripta, Vol. T159
DOI: 10.1088/0031-8949/2014/T159/014060

A full tungsten divertor for ITER: Physics issues and design status
journal, July 2013

Pitts, R. A.; Carpentier, S.; Escourbiac, F.
Journal of Nuclear Materials, Vol. 438
DOI: 10.1016/j.jnucmat.2013.01.008

Hydrogen in metals studied by Thermal Desorption Spectroscopy (TDS)
journal, April 2015

Hultquist, G.; Graham, M. J.; Smialek, J. L.
Corrosion Science, Vol. 93
DOI: 10.1016/j.corsci.2015.01.003

An analysis of thermal desorption mass spectra. I.
journal, May 1978

Chan, C. -M.; Aris, R.; Weinberg, W. H.
Applications of Surface Science, Vol. 1, Issue 3
DOI: 10.1016/0378-5963(78)90038-7

Defects in tungsten responsible for molecular hydrogen isotope retention after exposure to low energy plasmas
journal, June 2009

Causey, R. A.; Doerner, R.; Fraser, H.
Journal of Nuclear Materials, Vol. 390-391
DOI: 10.1016/j.jnucmat.2009.01.300

Review of hydrogen retention in tungsten
journal, April 2014

Tanabe, T.
Physica Scripta, Vol. T159
DOI: 10.1088/0031-8949/2014/T159/014044

Influence of the microstructure on the deuterium retention in tungsten
journal, August 2011

Manhard, A.; Schmid, K.; Balden, M.
Journal of Nuclear Materials, Vol. 415, Issue 1
DOI: 10.1016/j.jnucmat.2010.10.045

Transport of hydrogen in metals with occupancy dependent trap energies
journal, October 2014

Schmid, K.; von Toussaint, U.; Schwarz-Selinger, T.
Journal of Applied Physics, Vol. 116, Issue 13
DOI: 10.1063/1.4896580

Temperature dependence of deuterium retention mechanisms in tungsten
journal, October 2012

Roszell, J. P.; Davis, J. W.; Haasz, A. A.
Journal of Nuclear Materials, Vol. 429, Issue 1-3
DOI: 10.1016/j.jnucmat.2012.05.018

Binding States of Hydrogen on Tungsten
journal, June 1971

Tamm, P. W.; Schmidt, L. D.
The Journal of Chemical Physics, Vol. 54, Issue 11
DOI: 10.1063/1.1674753

Deuterium retention in tungsten after heavy ion damage and hydrogen isotope exchange in PISCES
journal, August 2014

Barton, J. L.; Wang, Y. Q.; Dittmar, T.
Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 332
DOI: 10.1016/j.nimb.2014.02.077

Simulation of irradiation induced deuterium trapping in tungsten
journal, August 2012

Ahlgren, T.; Heinola, K.; Vörtler, K.
Journal of Nuclear Materials, Vol. 427, Issue 1-3
DOI: 10.1016/j.jnucmat.2012.04.031

The dissociation of hydrogen by tungsten
journal, December 1936

Bryce, G.
Mathematical Proceedings of the Cambridge Philosophical Society, Vol. 32, Issue 4
DOI: 10.1017/S0305004100019381

Interaction of Hydrogen with Tungsten
journal, March 1960

Hickmott, T. W.
The Journal of Chemical Physics, Vol. 32, Issue 3
DOI: 10.1063/1.1730802

Hydrogen trapping models in steel
journal, December 2000

Krom, Alfons H. M.; Bakker, Ad
Metallurgical and Materials Transactions B, Vol. 31, Issue 6
DOI: 10.1007/s11663-000-0032-0

Ion-driven deuterium retention in tungsten
journal, February 2008

Ogorodnikova, O. V.; Roth, J.; Mayer, M.
Journal of Applied Physics, Vol. 103, Issue 3
DOI: 10.1063/1.2828139

Hydrogen in tungsten: Absorption, diffusion, vacancy trapping, and decohesion
journal, February 2010

Johnson, Donald F.; Carter, Emily A.
Journal of Materials Research, Vol. 25, Issue 2
DOI: 10.1557/JMR.2010.0036

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Title: Revisited reaction-diffusion model of thermal desorption spectroscopy experiments on hydrogen retention in material

Citation Formats

Hydrogen diffusion and vacancies formation in tungsten: Density Functional Theory calculations and statistical models journal, August 2015

Towards a better understanding of hydrogen measurements obtained by thermal desorption spectroscopy using FEM modeling journal, February 2015

Thermal desorption from metal surfaces: A review journal, January 1975

Surface morphology and deuterium retention of tungsten after low- and high-flux deuterium plasma exposure journal, June 2014

Recent analysis of key plasma wall interactions issues for ITER journal, June 2009

Depth distribution of deuterium in single- and polycrystalline tungsten up to depths of several micrometers journal, March 2005

Deuterium release from implanted beryllium and beryllium oxide journal, August 2011

Hydrogen Storage Material Composed of Polyacetylene and LiH and Investigation of Its Mechanisms journal, July 2014

Modelling deuterium release during thermal desorption of D+-irradiated tungsten journal, March 2008

Solution and Diffusion of Hydrogen in Tungsten journal, May 1969

Numerical modeling of thermal desorption mass spectroscopy (TDS) for the study of hydrogen diffusion and trapping interactions in metals journal, March 2015

Experiments on the release of tritium from the first wall of JET journal, September 1993

Comparison of hydrogen retention in W and W/Ta alloys journal, July 2012

Modelling of monovacancy diffusion in W over wide temperature range journal, March 2014

Modeling of Hydrogen Retention and Outgassing from Co-Deposits with Distributed Energy States: Modeling of Hydrogen Retention and Outgassing from Co-Deposits with Distributed Energy States journal, June 2014

Long-Term Hydrogen Outgassing from Plasma Facing Components: Long-Term Hydrogen Outgassing from Plasma Facing Components journal, June 2014

Hydrogen isotope retention and recycling in fusion reactor plasma-facing components journal, February 2002

Hydrogen interaction with point defects in tungsten journal, September 2010

Hydrogen transport in solids with traps in the case of continuum distribution of detrapping energies journal, April 2014

A full tungsten divertor for ITER: Physics issues and design status journal, July 2013

Hydrogen in metals studied by Thermal Desorption Spectroscopy (TDS) journal, April 2015

An analysis of thermal desorption mass spectra. I. journal, May 1978

Defects in tungsten responsible for molecular hydrogen isotope retention after exposure to low energy plasmas journal, June 2009

Review of hydrogen retention in tungsten journal, April 2014

Influence of the microstructure on the deuterium retention in tungsten journal, August 2011

Transport of hydrogen in metals with occupancy dependent trap energies journal, October 2014

Temperature dependence of deuterium retention mechanisms in tungsten journal, October 2012

Binding States of Hydrogen on Tungsten journal, June 1971

Deuterium retention in tungsten after heavy ion damage and hydrogen isotope exchange in PISCES journal, August 2014

Simulation of irradiation induced deuterium trapping in tungsten journal, August 2012

The dissociation of hydrogen by tungsten journal, December 1936

Interaction of Hydrogen with Tungsten journal, March 1960

Hydrogen trapping models in steel journal, December 2000

Ion-driven deuterium retention in tungsten journal, February 2008

Hydrogen in tungsten: Absorption, diffusion, vacancy trapping, and decohesion journal, February 2010

Hydrogen diffusion and vacancies formation in tungsten: Density Functional Theory calculations and statistical models
journal, August 2015

Towards a better understanding of hydrogen measurements obtained by thermal desorption spectroscopy using FEM modeling
journal, February 2015

Thermal desorption from metal surfaces: A review
journal, January 1975

Surface morphology and deuterium retention of tungsten after low- and high-flux deuterium plasma exposure
journal, June 2014

Recent analysis of key plasma wall interactions issues for ITER
journal, June 2009

Depth distribution of deuterium in single- and polycrystalline tungsten up to depths of several micrometers
journal, March 2005

Deuterium release from implanted beryllium and beryllium oxide
journal, August 2011

Hydrogen Storage Material Composed of Polyacetylene and LiH and Investigation of Its Mechanisms
journal, July 2014

Modelling deuterium release during thermal desorption of D+-irradiated tungsten
journal, March 2008

Solution and Diffusion of Hydrogen in Tungsten
journal, May 1969

Numerical modeling of thermal desorption mass spectroscopy (TDS) for the study of hydrogen diffusion and trapping interactions in metals
journal, March 2015

Experiments on the release of tritium from the first wall of JET
journal, September 1993

Comparison of hydrogen retention in W and W/Ta alloys
journal, July 2012

Modelling of monovacancy diffusion in W over wide temperature range
journal, March 2014

Modeling of Hydrogen Retention and Outgassing from Co-Deposits with Distributed Energy States: Modeling of Hydrogen Retention and Outgassing from Co-Deposits with Distributed Energy States
journal, June 2014

Long-Term Hydrogen Outgassing from Plasma Facing Components: Long-Term Hydrogen Outgassing from Plasma Facing Components
journal, June 2014

Hydrogen isotope retention and recycling in fusion reactor plasma-facing components
journal, February 2002

Hydrogen interaction with point defects in tungsten
journal, September 2010

Hydrogen transport in solids with traps in the case of continuum distribution of detrapping energies
journal, April 2014

A full tungsten divertor for ITER: Physics issues and design status
journal, July 2013

Hydrogen in metals studied by Thermal Desorption Spectroscopy (TDS)
journal, April 2015

An analysis of thermal desorption mass spectra. I.
journal, May 1978

Defects in tungsten responsible for molecular hydrogen isotope retention after exposure to low energy plasmas
journal, June 2009

Review of hydrogen retention in tungsten
journal, April 2014

Influence of the microstructure on the deuterium retention in tungsten
journal, August 2011

Transport of hydrogen in metals with occupancy dependent trap energies
journal, October 2014

Temperature dependence of deuterium retention mechanisms in tungsten
journal, October 2012

Binding States of Hydrogen on Tungsten
journal, June 1971

Deuterium retention in tungsten after heavy ion damage and hydrogen isotope exchange in PISCES
journal, August 2014

Simulation of irradiation induced deuterium trapping in tungsten
journal, August 2012

The dissociation of hydrogen by tungsten
journal, December 1936

Interaction of Hydrogen with Tungsten
journal, March 1960

Hydrogen trapping models in steel
journal, December 2000

Ion-driven deuterium retention in tungsten
journal, February 2008

Hydrogen in tungsten: Absorption, diffusion, vacancy trapping, and decohesion
journal, February 2010