Effects of strain and quantum confinement in optically pumped nuclear magnetic resonance in GaAs: Interpretation guided by spin-dependent band structure calculations
Abstract
A combined experimental-theoretical study of optically pumped NMR (OPNMR) has been performed in a GaAs/Al0.1Ga0.9As quantum well film with thermally induced biaxial strain. The photon energy dependence of the Ga-71 OPNMR signal was recorded at magnetic fields of 4.9 and 9.4 T at a temperature of 4.8-5.4 K. The data were compared to the nuclear spin polarization calculated from differential absorption to spin-up and spin-down states of the conduction band using a modified Pidgeon Brown model. Reasonable agreement between theory and experiment is obtained, facilitating assignment of features in the OPNMR energy dependence to specific interband transitions. Despite the approximations made in the quantum-mechanical model and the inexact correspondence between the experimental and calculated observables, the results provide insight into how effects of strain and quantum confinement are manifested in OPNMR signals
- Authors:
-
- Univ. of Florida, Gainesville, FL (United States)
- National High Magnetic Field Lab., Tallahassee, FL (United States)
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Publication Date:
- Research Org.:
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Sponsoring Org.:
- USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1226082
- Alternate Identifier(s):
- OSTI ID: 1181332
- Report Number(s):
- SAND-2014-17522J
Journal ID: ISSN 1098-0121; PRBMDO; 537386
- Grant/Contract Number:
- AC04-94AL85000; AC04–94AL85000
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review. B, Condensed Matter and Materials Physics
- Additional Journal Information:
- Journal Volume: 90; Journal Issue: 15; Journal ID: ISSN 1098-0121
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Citation Formats
Wood, R. M., Saha, D., McCarthy, L. A., Tokarski, III, J. T., Sanders, G. D., Kuhns, P. L., McGill, S. A., Reyes, A. P., Reno, J. L., Stanton, C. J., and Bowers, C. R. Effects of strain and quantum confinement in optically pumped nuclear magnetic resonance in GaAs: Interpretation guided by spin-dependent band structure calculations. United States: N. p., 2014.
Web. doi:10.1103/PhysRevB.90.155317.
Wood, R. M., Saha, D., McCarthy, L. A., Tokarski, III, J. T., Sanders, G. D., Kuhns, P. L., McGill, S. A., Reyes, A. P., Reno, J. L., Stanton, C. J., & Bowers, C. R. Effects of strain and quantum confinement in optically pumped nuclear magnetic resonance in GaAs: Interpretation guided by spin-dependent band structure calculations. United States. https://doi.org/10.1103/PhysRevB.90.155317
Wood, R. M., Saha, D., McCarthy, L. A., Tokarski, III, J. T., Sanders, G. D., Kuhns, P. L., McGill, S. A., Reyes, A. P., Reno, J. L., Stanton, C. J., and Bowers, C. R. Wed .
"Effects of strain and quantum confinement in optically pumped nuclear magnetic resonance in GaAs: Interpretation guided by spin-dependent band structure calculations". United States. https://doi.org/10.1103/PhysRevB.90.155317. https://www.osti.gov/servlets/purl/1226082.
@article{osti_1226082,
title = {Effects of strain and quantum confinement in optically pumped nuclear magnetic resonance in GaAs: Interpretation guided by spin-dependent band structure calculations},
author = {Wood, R. M. and Saha, D. and McCarthy, L. A. and Tokarski, III, J. T. and Sanders, G. D. and Kuhns, P. L. and McGill, S. A. and Reyes, A. P. and Reno, J. L. and Stanton, C. J. and Bowers, C. R.},
abstractNote = {A combined experimental-theoretical study of optically pumped NMR (OPNMR) has been performed in a GaAs/Al0.1Ga0.9As quantum well film with thermally induced biaxial strain. The photon energy dependence of the Ga-71 OPNMR signal was recorded at magnetic fields of 4.9 and 9.4 T at a temperature of 4.8-5.4 K. The data were compared to the nuclear spin polarization calculated from differential absorption to spin-up and spin-down states of the conduction band using a modified Pidgeon Brown model. Reasonable agreement between theory and experiment is obtained, facilitating assignment of features in the OPNMR energy dependence to specific interband transitions. Despite the approximations made in the quantum-mechanical model and the inexact correspondence between the experimental and calculated observables, the results provide insight into how effects of strain and quantum confinement are manifested in OPNMR signals},
doi = {10.1103/PhysRevB.90.155317},
journal = {Physical Review. B, Condensed Matter and Materials Physics},
number = 15,
volume = 90,
place = {United States},
year = {Wed Oct 29 00:00:00 EDT 2014},
month = {Wed Oct 29 00:00:00 EDT 2014}
}
Web of Science
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