Itinerant Antiferromagnetism in FeMnP0.8Si0.2

Sales, Brian C.; Susner, Michael A.; Conner, Benjamin S.; Yan, Jiaqiang Q.; May, Andrew F.

doi:10.1103/PhysRevB.92.104429

Title: Itinerant Antiferromagnetism in FeMnP_0.8Si_0.2

Abstract

Compounds based on the Fe₂P structure have continued to attract interest because of the interplay between itinerant and localized magnetism in a noncentrosymmetric crystal structure, and because of the recent developments of these materials for magnetocaloric applications. We report the growth and characterization of millimeter-sized single crystals of FeMnP_0.8Si_0.2 with the Fe₂P structure. Single-crystal x-ray diffraction, magnetization, resistivity, and Hall and heat capacity data are reported. The crystals exhibit itinerant antiferromagnetic order below 158 K with no hint of ferromagnetic behavior in the magnetization curves and with the spins ordered primarily in the ab plane. The room-temperature resistivity is close to the Ioffe-Regel limit for a metal. Single-crystal x-ray diffraction indicates a strong preference for Mn to occupy the larger pyramidal 3g site. The cation site preference in the as-grown crystals and the antiferromagnetism were not changed after high-temperature anneals and a rapid quench to room temperature

Authors:

Sales, Brian C. ^[1]; Susner, Michael A. ^[1]; Conner, Benjamin S. ^[1]; Yan, Jiaqiang Q. ^[2]; May, Andrew F. ^[1]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)

Publication Date:: Fri Sep 25 00:00:00 EDT 2015

Research Org.:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Critical Materials Institute (CMI)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Energy Efficiency and Renewable Energy (EERE)

OSTI Identifier:: 1224171

Alternate Identifier(s):: OSTI ID: 1224637

Grant/Contract Number:: AC05-00OR22725

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review. B, Condensed Matter and Materials Physics

Additional Journal Information:: Journal Volume: 92; Journal Issue: 10; Journal ID: ISSN 1098-0121

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE

Citation Formats


                    Sales, Brian C., Susner, Michael A., Conner, Benjamin S., Yan, Jiaqiang Q., and May, Andrew F. Itinerant Antiferromagnetism in FeMnP0.8Si0.2.  United States: N. p., 2015. 
Web.  doi:10.1103/PhysRevB.92.104429.

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                    Sales, Brian C., Susner, Michael A., Conner, Benjamin S., Yan, Jiaqiang Q., & May, Andrew F. Itinerant Antiferromagnetism in FeMnP0.8Si0.2.  United States.  https://doi.org/10.1103/PhysRevB.92.104429

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                    Sales, Brian C., Susner, Michael A., Conner, Benjamin S., Yan, Jiaqiang Q., and May, Andrew F. Fri .  
"Itinerant Antiferromagnetism in FeMnP0.8Si0.2".  United States.  https://doi.org/10.1103/PhysRevB.92.104429.  https://www.osti.gov/servlets/purl/1224171.

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@article{osti_1224171,

  title        = {Itinerant Antiferromagnetism in FeMnP0.8Si0.2},

  author       = {Sales, Brian C. and Susner, Michael A. and Conner, Benjamin S. and Yan, Jiaqiang Q. and May, Andrew F.},

  abstractNote = {Compounds based on the Fe2P structure have continued to attract interest because of the interplay between itinerant and localized magnetism in a noncentrosymmetric crystal structure, and because of the recent developments of these materials for magnetocaloric applications. We report the growth and characterization of millimeter-sized single crystals of FeMnP0.8Si0.2 with the Fe2P structure. Single-crystal x-ray diffraction, magnetization, resistivity, and Hall and heat capacity data are reported. The crystals exhibit itinerant antiferromagnetic order below 158 K with no hint of ferromagnetic behavior in the magnetization curves and with the spins ordered primarily in the ab plane. The room-temperature resistivity is close to the Ioffe-Regel limit for a metal. Single-crystal x-ray diffraction indicates a strong preference for Mn to occupy the larger pyramidal 3g site. The cation site preference in the as-grown crystals and the antiferromagnetism were not changed after high-temperature anneals and a rapid quench to room temperature},

  doi          = {10.1103/PhysRevB.92.104429},

  journal      = {Physical Review. B, Condensed Matter and Materials Physics},

  number       = 10,

  volume       = 92,

  place        = {United States},

  year         = {Fri Sep 25 00:00:00 EDT 2015},

  month        = {Fri Sep 25 00:00:00 EDT 2015}

}

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https://doi.org/10.1103/PhysRevB.92.104429

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Cited by: 4 works

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Figures / Tables:

FIG. 1: Crystal structure of FeMnP_0.8Si_0.2. View along the (001) direction (a), and view along (110) direction (b) The small P (Si) atoms are blue, the medium Fe atoms are red and the largest Mn atoms are yellow. The structure is drawn with Mn fully occupying the pyramidal (3g )more »

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Similar Records

Title: Itinerant Antiferromagnetism in FeMnP0.8Si0.2

Abstract

Citation Formats

Figures / Tables:

Magnetic Properties of Single Crystals of the System (Fe 1- x Ni x ) 2 P journal, January 1978

Magnetic Properties of (Fe1-xMnx)2P Compounds journal, February 1982

Determination of the homogeneity range and refinement of the crystal structure of Fe2P journal, September 1973

Crystallographic and Magnetic Properties of Solid Solutions of the Phosphides M 2 P, M = Cr, Mn, Fe, Co, and Ni journal, March 1969

Neutron Scattering Investigation of Itinerant Electron System Fe 2 P journal, June 1988

Itinerant ferromagnetism in Fe2P journal, October 1988

Spin Fluctuations in Ferromagnetic Metals –Temperature Variation of Local Moment and Short Range Order journal, February 1982

Polarized Neutron Diffraction Study of Fe 2 P Single Crystal journal, May 1979

Pressure-Induced Antiferromagnetism of Fe 2 P journal, July 1985

A Mössbauer study of Fe2P1−xSix (x ≤ 0.35) journal, July 1984

A Mössbauer and X-ray study of Fe2P1−xBx compounds (x < 0.15) journal, October 1980

Mixed Magnetism for Refrigeration and Energy Conversion journal, September 2011

Real-space observation of a two-dimensional skyrmion crystal journal, June 2010

Spin Transfer Torques in MnSi at Ultralow Current Densities journal, December 2010

A thermodynamic theory of “weak” ferromagnetism of antiferromagnetics journal, January 1958

Anisotropic Superexchange Interaction and Weak Ferromagnetism journal, October 1960

Recent developments in magnetocaloric materials journal, May 2005

Transition-metal-based magnetic refrigerants for room-temperature applications journal, January 2002

Taming the First-Order Transition in Giant Magnetocaloric Materials journal, February 2014

Phase diagram, structures and magnetism of the FeMnP 1−x Si x -system journal, January 2015

Structure, magnetism, and magnetocaloric properties of MnFeP1−xSix compounds journal, April 2008

Local Observation of the Site Occupancy of Mn in a MnFePSi Compound journal, March 2015

Orientation dependence of the anomalous Hall resistivity in single crystals of Yb 14 Mn Sb 11 journal, January 2008

Effect of boron substitution on the ferromagnetic transition of MnFe0.95P2/3Si1/3 journal, May 2015

Order-disorder induced magnetic structures of FeMnP 0 . 75 Si 0 . 25 journal, April 2011

Microscopic theory of magnetism in the magnetocaloric material Fe 2 P 1 − x T x ( T = B and Si) journal, July 2012

Detailed study of the magnetic ordering in FeMnP0.75Si0.25 journal, January 2015

Magnetic, thermodynamic, and transport characterization ofNa0.75CoO2single crystals journal, November 2004

The dynamics of spin-density waves journal, January 1994

Specific Heat of the Ferromagnet Fe2P journal, June 1982

Anomalous Hall effect in three ferromagnetic compounds: Eu Fe 4 Sb 12 , Yb 14 Mn Sb 11 , and Eu 8 Ga 16 Ge 30 journal, June 2006

Ioffe-Regel criterion and resistivity of metals journal, December 1981

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Title: Itinerant Antiferromagnetism in FeMnP_0.8Si_0.2

Magnetic Properties of Single Crystals of the System (Fe _{1- x} Ni _x ) ₂ P
journal, January 1978

Magnetic Properties of (Fe_1-xMn_x)₂P Compounds
journal, February 1982

Determination of the homogeneity range and refinement of the crystal structure of Fe2P
journal, September 1973

Crystallographic and Magnetic Properties of Solid Solutions of the Phosphides M ₂ P, M = Cr, Mn, Fe, Co, and Ni
journal, March 1969

Neutron Scattering Investigation of Itinerant Electron System Fe ₂ P
journal, June 1988

Itinerant ferromagnetism in Fe2P
journal, October 1988

Spin Fluctuations in Ferromagnetic Metals –Temperature Variation of Local Moment and Short Range Order
journal, February 1982

Polarized Neutron Diffraction Study of Fe ₂ P Single Crystal
journal, May 1979

Pressure-Induced Antiferromagnetism of Fe ₂ P
journal, July 1985

A Mössbauer study of Fe2P1−xSix (x ≤ 0.35)
journal, July 1984

A Mössbauer and X-ray study of Fe2P1−xBx compounds (x < 0.15)
journal, October 1980

Mixed Magnetism for Refrigeration and Energy Conversion
journal, September 2011

Real-space observation of a two-dimensional skyrmion crystal
journal, June 2010

Spin Transfer Torques in MnSi at Ultralow Current Densities
journal, December 2010

A thermodynamic theory of “weak” ferromagnetism of antiferromagnetics
journal, January 1958

Anisotropic Superexchange Interaction and Weak Ferromagnetism
journal, October 1960

Recent developments in magnetocaloric materials
journal, May 2005

Transition-metal-based magnetic refrigerants for room-temperature applications
journal, January 2002

Taming the First-Order Transition in Giant Magnetocaloric Materials
journal, February 2014

Phase diagram, structures and magnetism of the FeMnP _1−x Si _x -system
journal, January 2015

Structure, magnetism, and magnetocaloric properties of MnFeP1−xSix compounds
journal, April 2008

Local Observation of the Site Occupancy of Mn in a MnFePSi Compound
journal, March 2015

Orientation dependence of the anomalous Hall resistivity in single crystals of ${Yb}_{14} Mn {Sb}_{11}$
journal, January 2008

Effect of boron substitution on the ferromagnetic transition of MnFe0.95P2/3Si1/3
journal, May 2015

Order-disorder induced magnetic structures of FeMnP $_{0.75}$ Si $_{0.25}$
journal, April 2011

Microscopic theory of magnetism in the magnetocaloric material ${Fe}_{2}$ P $_{1 - x}$ T $_{x}$ ( $T = B$ and Si)
journal, July 2012

Detailed study of the magnetic ordering in FeMnP0.75Si0.25
journal, January 2015

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journal, January 1994

Specific Heat of the Ferromagnet Fe₂P
journal, June 1982

Anomalous Hall effect in three ferromagnetic compounds: $Eu {Fe}_{4} {Sb}_{12}$ , ${Yb}_{14} Mn {Sb}_{11}$ , and ${Eu}_{8} {Ga}_{16} {Ge}_{30}$
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