Does the Use of Diamond-Like Carbon Coating and Organophosphate Lubricant Additive Together Cause Excessive Tribochemical Material Removal?
Abstract
We observe unexpected wear increase on a steel surface that rubbed against diamond-like carbon (DLC) coatings only when lubricated by phosphate-based antiwear additives. Contrary to the literature hypothesis of a competition between zinc dialkyldithiophosphate produced tribofilms and DLC-induced carbon transfer, here a new wear mechanism based on carbon-catalyzed tribochemical interactions supported by surface characterization is proposed
- Authors:
-
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science and Technology Div.
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE)
- OSTI Identifier:
- 1213333
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Materials Interfaces
- Additional Journal Information:
- Journal Volume: 2; Journal Issue: 15; Journal ID: ISSN 2196-7350
- Publisher:
- Wiley-VCH
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; diamond-like carbon (DLC); ionic liquids; lubricants; tribochemical; ZDDP
Citation Formats
Zhou, Yan, Leonard, Donovan N., Meyer, Harry M., Luo, Huimin, and Qu, Jun. Does the Use of Diamond-Like Carbon Coating and Organophosphate Lubricant Additive Together Cause Excessive Tribochemical Material Removal?. United States: N. p., 2015.
Web. doi:10.1002/admi.201500213.
Zhou, Yan, Leonard, Donovan N., Meyer, Harry M., Luo, Huimin, & Qu, Jun. Does the Use of Diamond-Like Carbon Coating and Organophosphate Lubricant Additive Together Cause Excessive Tribochemical Material Removal?. United States. https://doi.org/10.1002/admi.201500213
Zhou, Yan, Leonard, Donovan N., Meyer, Harry M., Luo, Huimin, and Qu, Jun. Sat .
"Does the Use of Diamond-Like Carbon Coating and Organophosphate Lubricant Additive Together Cause Excessive Tribochemical Material Removal?". United States. https://doi.org/10.1002/admi.201500213. https://www.osti.gov/servlets/purl/1213333.
@article{osti_1213333,
title = {Does the Use of Diamond-Like Carbon Coating and Organophosphate Lubricant Additive Together Cause Excessive Tribochemical Material Removal?},
author = {Zhou, Yan and Leonard, Donovan N. and Meyer, Harry M. and Luo, Huimin and Qu, Jun},
abstractNote = {We observe unexpected wear increase on a steel surface that rubbed against diamond-like carbon (DLC) coatings only when lubricated by phosphate-based antiwear additives. Contrary to the literature hypothesis of a competition between zinc dialkyldithiophosphate produced tribofilms and DLC-induced carbon transfer, here a new wear mechanism based on carbon-catalyzed tribochemical interactions supported by surface characterization is proposed},
doi = {10.1002/admi.201500213},
journal = {Advanced Materials Interfaces},
number = 15,
volume = 2,
place = {United States},
year = {Sat Aug 22 00:00:00 EDT 2015},
month = {Sat Aug 22 00:00:00 EDT 2015}
}
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Works referencing / citing this record:
Unusual Competitive and Synergistic Effects of Graphite Nanoplates in Engine Oil on the Tribofilm Formation
journal, August 2019
- Pham, Sang T.; Wan, Shanhong; Tieu, Kiet A.
- Advanced Materials Interfaces, Vol. 6, Issue 19
Understanding Tribofilm Formation Mechanisms in Ionic Liquid Lubrication
journal, August 2017
- Zhou, Yan; Leonard, Donovan N.; Guo, Wei
- Scientific Reports, Vol. 7, Issue 1