Spin-liquid ground state in the frustrated J1-J2 zigzag chain system BaTb2O4

Aczel, A. A.; Li, L.; Garlea, V. O.; Yan, J. -Q.; Weickert, F.; Zapf, V. S.; Movshovich, R.; Jaime, M.; Baker, P. J.; Keppens, V.; Mandrus, D.

doi:10.1103/PhysRevB.92.041110

Title: Spin-liquid ground state in the frustrated $J_{1} - J_{2}$ zigzag chain system ${BaTb}_{2} O_{4}$

Abstract

We have investigated polycrystalline samples of the zigzag chain system BaTb₂O₄ with magnetic susceptibility, heat capacity, neutron powder diffraction, and muon spin relaxation measurements. No magnetic transitions are observed in the bulk measurements, while neutron diffraction reveals low-temperature, short-range, intrachain magnetic correlations between Tb³⁺ ions. Muon spin relaxation measurements indicate that these correlations are dynamic, as the technique detects no signatures of static magnetism down to 0.095 K. Altogether these findings provide strong evidence for a spin liquid ground state in BaTb₂O₄.

Authors:

Aczel, A. A. ^[1]; Li, L. ^[2]; Garlea, V. O. ^[1]; Yan, J. -Q. ^[3]; Weickert, F. ^[4]; Zapf, V. S. ^[4]; Movshovich, R. ^[4]; Jaime, M. ^[4]; Baker, P. J. ^[5]; Keppens, V. ^[2]; Mandrus, D. ^[3]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Univ. of Tennessee, Knoxville, TN (United States)
Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
STFC Rutherford Appleton Lab., Oxfordshire (United Kingdom)

Publication Date:: Mon Jul 13 00:00:00 EDT 2015

Research Org.:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1210136

Alternate Identifier(s):: OSTI ID: 1193915

Grant/Contract Number:: AC05-00OR22725

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review. B, Condensed Matter and Materials Physics

Additional Journal Information:: Journal Volume: 92; Journal Issue: 4; Journal ID: ISSN 1098-0121

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; spin liquid; frustration; neutron diffraction

Citation Formats


                    Aczel, A. A., Li, L., Garlea, V. O., Yan, J. -Q., Weickert, F., Zapf, V. S., Movshovich, R., Jaime, M., Baker, P. J., Keppens, V., and Mandrus, D. Spin-liquid ground state in the frustrated J1-J2 zigzag chain system BaTb2O4.  United States: N. p., 2015. 
Web.  doi:10.1103/PhysRevB.92.041110.

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                    Aczel, A. A., Li, L., Garlea, V. O., Yan, J. -Q., Weickert, F., Zapf, V. S., Movshovich, R., Jaime, M., Baker, P. J., Keppens, V., & Mandrus, D. Spin-liquid ground state in the frustrated J1-J2 zigzag chain system BaTb2O4.  United States.  https://doi.org/10.1103/PhysRevB.92.041110

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                    Aczel, A. A., Li, L., Garlea, V. O., Yan, J. -Q., Weickert, F., Zapf, V. S., Movshovich, R., Jaime, M., Baker, P. J., Keppens, V., and Mandrus, D. Mon .  
"Spin-liquid ground state in the frustrated J1-J2 zigzag chain system BaTb2O4".  United States.  https://doi.org/10.1103/PhysRevB.92.041110.  https://www.osti.gov/servlets/purl/1210136.

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@article{osti_1210136,

  title        = {Spin-liquid ground state in the frustrated J1-J2 zigzag chain system BaTb2O4},

  author       = {Aczel, A. A. and Li, L. and Garlea, V. O. and Yan, J. -Q. and Weickert, F. and Zapf, V. S. and Movshovich, R. and Jaime, M. and Baker, P. J. and Keppens, V. and Mandrus, D.},

  abstractNote = {We have investigated polycrystalline samples of the zigzag chain system BaTb2O4 with magnetic susceptibility, heat capacity, neutron powder diffraction, and muon spin relaxation measurements. No magnetic transitions are observed in the bulk measurements, while neutron diffraction reveals low-temperature, short-range, intrachain magnetic correlations between Tb3+ ions. Muon spin relaxation measurements indicate that these correlations are dynamic, as the technique detects no signatures of static magnetism down to 0.095 K. Altogether these findings provide strong evidence for a spin liquid ground state in BaTb2O4.},

  doi          = {10.1103/PhysRevB.92.041110},

  journal      = {Physical Review. B, Condensed Matter and Materials Physics},

  number       = 4,

  volume       = 92,

  place        = {United States},

  year         = {Mon Jul 13 00:00:00 EDT 2015},

  month        = {Mon Jul 13 00:00:00 EDT 2015}

}

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Works referencing / citing this record:

Two-dimensional spin liquid behaviour in the triangular-honeycomb antiferromagnet TbInO3
journal, January 2019

Clark, Lucy; Sala, Gabriele; Maharaj, Dalini D.
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Two-dimensional spin liquid behaviour in the triangular-honeycomb antiferromagnet TbInO$_3$
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Clark, Lucy; Sala, Gabriele; Maharaj, Dalini D.
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Title: Spin-liquid ground state in the frustrated J 1 - J 2 zigzag chain system BaTb 2 O 4

Abstract

Citation Formats

Spin liquids in frustrated magnets journal, March 2010

The Resonating Valence Bond State in La2CuO4 and Superconductivity journal, March 1987

Spin Ice State in Frustrated Magnetic Pyrochlore Materials journal, November 2001

Quantum orders and symmetric spin liquids journal, April 2002

Spin Dynamics of the Spin- 1 / 2 Kagome Lattice Antiferromagnet ZnCu 3 ( OH ) 6 Cl 2 journal, March 2007

Fractionalized excitations in the spin-liquid state of a kagome-lattice antiferromagnet journal, December 2012

Vesignieite BaCu 3 V 2 O 8 (OH) 2 as a Candidate Spin-1/2 Kagome Antiferromagnet journal, March 2009

High-Pressure Sequence of Ba 3 NiSb 2 O 9 Structural Phases: New S = 1 Quantum Spin Liquids Based on Ni 2 + journal, November 2011

Geometrical Frustration in the Ferromagnetic Pyrochlore Ho 2 Ti 2 O 7 journal, September 1997

Zero-point entropy in ‘spin ice’ journal, May 1999

Absence of Ferromagnetism or Antiferromagnetism in One- or Two-Dimensional Isotropic Heisenberg Models journal, November 1966

Transition to long-range magnetic order in the highly frustrated insulating pyrochlore antiferromagnet Gd 2 Ti 2 O 7 journal, June 1999

Honeycombs of triangles and magnetic frustration in Sr L 2 O 4 ( L = Gd , Dy, Ho, Er, Tm, and Yb) journal, April 2005

Crystal structures and magnetic properties of magnetically frustrated systems BaLn 2 O 4 and Ba 3 Ln 4 O 9 (Ln = lanthanide) journal, December 2005

Single crystal synthesis and magnetism of the BaLn2O4 family (Ln = lanthanide) journal, September 2014

Coexistence of the long-range and short-range magnetic order components in SrEr 2 O 4 journal, November 2011

Evidence for SrHo 2 O 4 and SrDy 2 O 4 as model J 1 - J 2 zigzag chain materials journal, June 2014

Disorder from order among anisotropic next-nearest-neighbor Ising spin chains in SrHo 2 O 4 journal, February 2015

Universal emergence of the one-third plateau in the magnetization process of frustrated quantum spin chains journal, February 2007

Ground State Phase Diagram of Frustrated S = 1 X X Z chains: Chiral Ordered Phases journal, January 2000

Revised effective ionic radii and systematic studies of interatomic distances in halides and chalcogenides journal, September 1976

Coexistence of long- and short-range magnetic order in the frustrated magnet SrYb 2 O 4 journal, August 2012

Magnetic ordering in the frustrated J 1 − J 2 Ising chain candidate BaNd 2 O 4 journal, October 2014

Low-temperature magnetic ordering in SrEr 2 O 4 journal, November 2008

Low temperature magnetic structure of geometrically frustrated SrHo 2 O 4 journal, December 2012

Highly frustrated magnetism in SrHo 2 O 4 : Coexistence of two types of short-range order journal, July 2013

Incommensurate antiferromagnetic order in the manifoldly-frustrated SrTb2O4 with transition temperature up to 4.28 K journal, July 2014

Magnetic field-induced ordering in SrDy 2 O 4 journal, May 2013

Magnetic and Thermal Properties of Tb ( OH ) 3 journal, November 1973

Heat-capacity measurements on rare-earth double oxides R2M2O7 journal, September 1969

Lack of evidence for a singlet crystal-field ground state in the magnetic pyrochlore Tb 2 Ti 2 O 7 journal, October 2011

Recent advances in magnetic structure determination by neutron powder diffraction journal, October 1993

Lifting of the ground-state degeneracy by crystal-field interactions in the pyrochlore journal, January 1996

Neutron-diffraction study of magnetic ordering in the pyrochlore series R 2 Mo 2 O 7 ( R =Nd,Tb,Y) journal, March 1991

Cooperative Paramagnetism in the Geometrically Frustrated Pyrochlore Antiferromagnet Tb 2 Ti 2 O 7 journal, February 1999

Spin-liquid behavior in a kagomé antiferromagnet: Deuteronium jarosite journal, November 2007

Absence of long-range magnetic ordering in the pyrochlore compound Er 2 Sn 2 O 7 journal, September 2011

Short-range magnetic correlations in the highly correlated electron compound CeCu 4 Ga journal, September 2014

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Title: Spin-liquid ground state in the frustrated $J_{1} - J_{2}$ zigzag chain system ${BaTb}_{2} O_{4}$

Spin liquids in frustrated magnets
journal, March 2010

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journal, March 1987

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journal, November 2001

Quantum orders and symmetric spin liquids
journal, April 2002

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Vesignieite BaCu ₃ V ₂ O ₈ (OH) ₂ as a Candidate Spin-1/2 Kagome Antiferromagnet
journal, March 2009

High-Pressure Sequence of ${Ba}_{3} {NiSb}_{2} O_{9}$ Structural Phases: New $S = 1$ Quantum Spin Liquids Based on ${Ni}^{2 +}$
journal, November 2011

Geometrical Frustration in the Ferromagnetic Pyrochlore ${Ho}_{2} {Ti}_{2} O_{7}$
journal, September 1997

Zero-point entropy in ‘spin ice’
journal, May 1999

Absence of Ferromagnetism or Antiferromagnetism in One- or Two-Dimensional Isotropic Heisenberg Models
journal, November 1966

Transition to long-range magnetic order in the highly frustrated insulating pyrochlore antiferromagnet ${Gd}_{2} {Ti}_{2} O_{7}$
journal, June 1999

Honeycombs of triangles and magnetic frustration in $Sr L_{2} O_{4}$ ( $L = Gd$ , Dy, Ho, Er, Tm, and Yb)
journal, April 2005

Crystal structures and magnetic properties of magnetically frustrated systems BaLn ₂ O ₄ and Ba ₃ Ln ₄ O ₉ (Ln = lanthanide)
journal, December 2005

Single crystal synthesis and magnetism of the BaLn2O4 family (Ln = lanthanide)
journal, September 2014

Coexistence of the long-range and short-range magnetic order components in SrEr $_{2}$ O $_{4}$
journal, November 2011

Evidence for ${SrHo}_{2} O_{4}$ and ${SrDy}_{2} O_{4}$ as model $J_{1}$ - $J_{2}$ zigzag chain materials
journal, June 2014

Disorder from order among anisotropic next-nearest-neighbor Ising spin chains in ${SrHo}_{2} O_{4}$
journal, February 2015

Universal emergence of the one-third plateau in the magnetization process of frustrated quantum spin chains
journal, February 2007

Ground State Phase Diagram of Frustrated S = 1 X X Z chains: Chiral Ordered Phases
journal, January 2000

Revised effective ionic radii and systematic studies of interatomic distances in halides and chalcogenides
journal, September 1976

Coexistence of long- and short-range magnetic order in the frustrated magnet SrYb $_{2}$ O $_{4}$
journal, August 2012

Magnetic ordering in the frustrated $J_{1} - J_{2}$ Ising chain candidate ${BaNd}_{2} O_{4}$
journal, October 2014

Low-temperature magnetic ordering in ${SrEr}_{2} O_{4}$
journal, November 2008

Low temperature magnetic structure of geometrically frustrated SrHo ₂ O ₄
journal, December 2012

Highly frustrated magnetism in SrHo $_{2}$ O $_{4}$ : Coexistence of two types of short-range order
journal, July 2013

Incommensurate antiferromagnetic order in the manifoldly-frustrated SrTb2O4 with transition temperature up to 4.28 K
journal, July 2014

Magnetic field-induced ordering in SrDy ₂ O ₄
journal, May 2013

Magnetic and Thermal Properties of Tb ${(OH)}_{3}$
journal, November 1973

Heat-capacity measurements on rare-earth double oxides R2M2O7
journal, September 1969

Lack of evidence for a singlet crystal-field ground state in the magnetic pyrochlore Tb $_{2}$ Ti $_{2}$ O $_{7}$
journal, October 2011

Recent advances in magnetic structure determination by neutron powder diffraction
journal, October 1993

Lifting of the ground-state degeneracy by crystal-field interactions in the pyrochlore
journal, January 1996

Neutron-diffraction study of magnetic ordering in the pyrochlore series $R_{2}$ ${Mo}_{2}$ $O_{7}$ ( R =Nd,Tb,Y)
journal, March 1991

Cooperative Paramagnetism in the Geometrically Frustrated Pyrochlore Antiferromagnet ${Tb}_{2} {Ti}_{2} O_{7}$
journal, February 1999

Spin-liquid behavior in a kagomé antiferromagnet: Deuteronium jarosite
journal, November 2007

Absence of long-range magnetic ordering in the pyrochlore compound Er ₂ Sn ₂ O ₇
journal, September 2011

Short-range magnetic correlations in the highly correlated electron compound ${CeCu}_{4} Ga$
journal, September 2014

Coexisting magnetic order and cooperative paramagnetism in the stuffed pyrochlore ${Tb}_{2 + x} {Ti}_{2 - 2 x} {Nb}_{x} O_{7}$
journal, February 2010

Neutron scattering studies of the cooperative paramagnet pyrochlore ${Tb}_{2} {Ti}_{2} O_{7}$
journal, November 2001

Spin freezing in the geometrically frustrated pyrochlore antiferromagnet ${Tb}_{2}$ ${Mo}_{2}$ $O_{7}$
journal, November 1992

Quantum spin ice: a search for gapless quantum spin liquids in pyrochlore magnets
journal, May 2014

Muon spin rotation and relaxation in magnetic materials
journal, October 1997

Muon spin relaxation investigation of the spin dynamics of geometrically frustrated antiferromagnets $Y_{2}$ ${Mo}_{2}$ $O_{7}$ and ${Tb}_{2}$ ${Mo}_{2}$ $O_{7}$
journal, October 1996

Two-dimensional spin liquid behaviour in the triangular-honeycomb antiferromagnet TbInO3
journal, January 2019

Two-dimensional spin liquid behaviour in the triangular-honeycomb antiferromagnet TbInO$_3$
text, January 2018