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Title: GaMin’11 – an international inter-laboratory comparison for geochemical CO₂ - saline fluid - mineral interaction experiments

Abstract

Due to the strong interest in geochemical CO₂-fluid-rock interaction in the context of geological storage of CO₂ a growing number of research groups have used a variety of different experimental ways to identify important geochemical dissolution or precipitation reactions and – if possible – quantify the rates and extent of mineral or rock alteration. In this inter-laboratory comparison the gas-fluid-mineral reactions of three samples of rock-forming minerals have been investigated by 11 experimental labs. The reported results point to robust identification of the major processes in the experiments by most groups. The dissolution rates derived from the changes in composition of the aqueous phase are consistent overall, but the variation could be reduced by using similar corrections for changing parameters in the reaction cells over time. The comparison of experimental setups and procedures as well as of data corrections identified potential improvements for future gas-fluid-rock studies.

Authors:
 [1];  [1];  [2];  [2];  [3];  [3];  [3];  [4];  [4];  [5];  [6];  [6];  [6];  [6];  [7];  [7];  [8];  [8];  [8];  [9] more »;  [9];  [10];  [10];  [10];  [10];  [11];  [12];  [13];  [14] « less
  1. Federal Inst. for Geosciences and Natural Resesources (BGR), Hannover (Germany)
  2. United States Geological Survey, Menlo Park, CA (United States)
  3. British Geological Survey, Nottinghamshire (United Kingdom)
  4. Univ. of Leeds (United Kingdom)
  5. Carnegie Mellon Univ., Pittsburgh, PA (United States)
  6. National Energy Technology Lab., Pittsburgh, PA (United States)
  7. Univ. of Melbourne, (Austrialia)
  8. hGEOMAR Helmholtz Center for Ocean Research, Kiel (Germany)
  9. GFZ German Research Centre for Geosciences, Potsdam (Germany)
  10. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  11. Martin Luther Univ., Halle (Germany)
  12. Research Inst. of Innovative Tech. for the Earth (RITE), Kyoto (Japan)
  13. National Inst. of Advanced Science and Tech. (AIST) Tsukuba (Japan)
  14. GeoRessources, Universite de Lorraine, Nancy (France)
Publication Date:
Research Org.:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1196923
Grant/Contract Number:  
AC02-05CH11231
Resource Type:
Accepted Manuscript
Journal Name:
Energy Procedia
Additional Journal Information:
Journal Volume: 63; Journal Issue: C; Journal ID: ISSN 1876-6102
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
58 GEOSCIENCES; CCS; geochemical experiments; fluid-rock interaction; mineral dissolution; precipitation; method comparison

Citation Formats

Ostertag-Henning, C., Risse, A., Thomas, B., Rosenbauer, R., Rochelle, C., Purser, G., Kilpatrick, A., Rosenqvist, J., Yardley, B., Karamalidis, A., Griffith, C., Hedges, S., Dilmore, R., Goodman, A., Black, J., Haese, R., Deusner, C., Bigalke, N., Haeckel, M., Fischer, S., Liebscher, A., Icenhower, J. P., Daval, D., Saldi, G. D., Knauss, K. G., Schmidt, M., Mito, S., Sorai, M., and Truche, L. GaMin’11 – an international inter-laboratory comparison for geochemical CO₂ - saline fluid - mineral interaction experiments. United States: N. p., 2014. Web. doi:10.1016/j.egypro.2014.11.587.
Ostertag-Henning, C., Risse, A., Thomas, B., Rosenbauer, R., Rochelle, C., Purser, G., Kilpatrick, A., Rosenqvist, J., Yardley, B., Karamalidis, A., Griffith, C., Hedges, S., Dilmore, R., Goodman, A., Black, J., Haese, R., Deusner, C., Bigalke, N., Haeckel, M., Fischer, S., Liebscher, A., Icenhower, J. P., Daval, D., Saldi, G. D., Knauss, K. G., Schmidt, M., Mito, S., Sorai, M., & Truche, L. GaMin’11 – an international inter-laboratory comparison for geochemical CO₂ - saline fluid - mineral interaction experiments. United States. https://doi.org/10.1016/j.egypro.2014.11.587
Ostertag-Henning, C., Risse, A., Thomas, B., Rosenbauer, R., Rochelle, C., Purser, G., Kilpatrick, A., Rosenqvist, J., Yardley, B., Karamalidis, A., Griffith, C., Hedges, S., Dilmore, R., Goodman, A., Black, J., Haese, R., Deusner, C., Bigalke, N., Haeckel, M., Fischer, S., Liebscher, A., Icenhower, J. P., Daval, D., Saldi, G. D., Knauss, K. G., Schmidt, M., Mito, S., Sorai, M., and Truche, L. Wed . "GaMin’11 – an international inter-laboratory comparison for geochemical CO₂ - saline fluid - mineral interaction experiments". United States. https://doi.org/10.1016/j.egypro.2014.11.587. https://www.osti.gov/servlets/purl/1196923.
@article{osti_1196923,
title = {GaMin’11 – an international inter-laboratory comparison for geochemical CO₂ - saline fluid - mineral interaction experiments},
author = {Ostertag-Henning, C. and Risse, A. and Thomas, B. and Rosenbauer, R. and Rochelle, C. and Purser, G. and Kilpatrick, A. and Rosenqvist, J. and Yardley, B. and Karamalidis, A. and Griffith, C. and Hedges, S. and Dilmore, R. and Goodman, A. and Black, J. and Haese, R. and Deusner, C. and Bigalke, N. and Haeckel, M. and Fischer, S. and Liebscher, A. and Icenhower, J. P. and Daval, D. and Saldi, G. D. and Knauss, K. G. and Schmidt, M. and Mito, S. and Sorai, M. and Truche, L.},
abstractNote = {Due to the strong interest in geochemical CO₂-fluid-rock interaction in the context of geological storage of CO₂ a growing number of research groups have used a variety of different experimental ways to identify important geochemical dissolution or precipitation reactions and – if possible – quantify the rates and extent of mineral or rock alteration. In this inter-laboratory comparison the gas-fluid-mineral reactions of three samples of rock-forming minerals have been investigated by 11 experimental labs. The reported results point to robust identification of the major processes in the experiments by most groups. The dissolution rates derived from the changes in composition of the aqueous phase are consistent overall, but the variation could be reduced by using similar corrections for changing parameters in the reaction cells over time. The comparison of experimental setups and procedures as well as of data corrections identified potential improvements for future gas-fluid-rock studies.},
doi = {10.1016/j.egypro.2014.11.587},
journal = {Energy Procedia},
number = C,
volume = 63,
place = {United States},
year = {Wed Dec 31 00:00:00 EST 2014},
month = {Wed Dec 31 00:00:00 EST 2014}
}

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