Latent instabilities in metallic LaNiO₃ films by strain control of Fermi-surface topology
Abstract
Strain control is one of the most promising avenues to search for new emergent phenomena in transition metal-oxide films. Here, we investigate the strain-induced changes of electronic structures in strongly correlated LaNiO₃ (LNO) films, using angle-resolved photoemission spectroscopy and the dynamical mean-field theory. The strongly renormalized eg-orbital bands are systematically rearranged by misfit strain to change its fermiology. As tensile strain increases, the hole pocket centered at the A point elongates along the kz-axis and seems to become open, thus changing Fermi-surface (FS) topology from three- to quasi-two-dimensional. Concomitantly, the FS shape becomes flattened to enhance FS nesting. A FS superstructure withQ₁ = (1/2,1/2,1/2) appears in all LNO films, while a tensile-strained LNO film has an additional Q₂ = (1/4,1/4,1/4) modulation, indicating that some instabilities are present in metallic LNO films. Charge disproportionation and spin-density-wave fluctuations observed in other nickelates might be their most probable origins
- Authors:
-
- Institute for Basic Science, Seoul (Republic of Korea); Seoul National Univ., Seoul (Republic of Korea)
- Pohang Univ. of Science and Technology (POSTECH) (Korea, Republic of)
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Univ. of Seoul, Seoul (Republic of Korea)
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1191300
- Grant/Contract Number:
- AC02-05CH11231
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Scientific Reports
- Additional Journal Information:
- Journal Volume: 5; Journal Issue: 1; Journal ID: ISSN 2045-2322
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
Citation Formats
Yoo, Hyang Keun, Hyun, Seung Ill, Moreschini, Luca, Kim, Hyeong -Do, Chang, Young Jun, Sohn, Chang Hee, Jeong, Da Woon, Sinn, Soobin, Kim, Yong Su, Bostwick, Aaron, Rotenberg, Eli, Shim, Ji Hoon, and Noh, Tae Won. Latent instabilities in metallic LaNiO₃ films by strain control of Fermi-surface topology. United States: N. p., 2015.
Web. doi:10.1038/srep08746.
Yoo, Hyang Keun, Hyun, Seung Ill, Moreschini, Luca, Kim, Hyeong -Do, Chang, Young Jun, Sohn, Chang Hee, Jeong, Da Woon, Sinn, Soobin, Kim, Yong Su, Bostwick, Aaron, Rotenberg, Eli, Shim, Ji Hoon, & Noh, Tae Won. Latent instabilities in metallic LaNiO₃ films by strain control of Fermi-surface topology. United States. https://doi.org/10.1038/srep08746
Yoo, Hyang Keun, Hyun, Seung Ill, Moreschini, Luca, Kim, Hyeong -Do, Chang, Young Jun, Sohn, Chang Hee, Jeong, Da Woon, Sinn, Soobin, Kim, Yong Su, Bostwick, Aaron, Rotenberg, Eli, Shim, Ji Hoon, and Noh, Tae Won. Wed .
"Latent instabilities in metallic LaNiO₃ films by strain control of Fermi-surface topology". United States. https://doi.org/10.1038/srep08746. https://www.osti.gov/servlets/purl/1191300.
@article{osti_1191300,
title = {Latent instabilities in metallic LaNiO₃ films by strain control of Fermi-surface topology},
author = {Yoo, Hyang Keun and Hyun, Seung Ill and Moreschini, Luca and Kim, Hyeong -Do and Chang, Young Jun and Sohn, Chang Hee and Jeong, Da Woon and Sinn, Soobin and Kim, Yong Su and Bostwick, Aaron and Rotenberg, Eli and Shim, Ji Hoon and Noh, Tae Won},
abstractNote = {Strain control is one of the most promising avenues to search for new emergent phenomena in transition metal-oxide films. Here, we investigate the strain-induced changes of electronic structures in strongly correlated LaNiO₃ (LNO) films, using angle-resolved photoemission spectroscopy and the dynamical mean-field theory. The strongly renormalized eg-orbital bands are systematically rearranged by misfit strain to change its fermiology. As tensile strain increases, the hole pocket centered at the A point elongates along the kz-axis and seems to become open, thus changing Fermi-surface (FS) topology from three- to quasi-two-dimensional. Concomitantly, the FS shape becomes flattened to enhance FS nesting. A FS superstructure withQ₁ = (1/2,1/2,1/2) appears in all LNO films, while a tensile-strained LNO film has an additional Q₂ = (1/4,1/4,1/4) modulation, indicating that some instabilities are present in metallic LNO films. Charge disproportionation and spin-density-wave fluctuations observed in other nickelates might be their most probable origins},
doi = {10.1038/srep08746},
journal = {Scientific Reports},
number = 1,
volume = 5,
place = {United States},
year = {Wed Mar 04 00:00:00 EST 2015},
month = {Wed Mar 04 00:00:00 EST 2015}
}
Web of Science
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