Ferromagnetism of Fe3Sn and alloys

Sales, Brian C.; Saparov, Bayrammurad; McGuire, Michael A.; Singh, David J.; Parker, David S.

doi:10.1038/srep07024

Title: Ferromagnetism of Fe₃Sn and alloys

Abstract

Hexagonal Fe₃Sn has many of the desirable properties for a new permanent magnet phase with a Curie temperature of 725 K, a saturation moment of 1.18 MA/m. and anisotropy energy, K₁ of 1.8 MJ/m³. However, contrary to earlier experimental reports, we found both experimentally and theoretically that the easy magnetic axis lies in the hexagonal plane, which is undesirable for a permanent magnet material. One possibility for changing the easy axis direction is through alloying. We used first principles calculations to investigate the effect of elemental substitutions. The calculations showed that substitution on the Sn site has the potential to switch the easy axis direction. Transition metal substitutions with Co or Mn do not have this effect. We attempted synthesis of a number of these alloys and found results in accord with the theoretical predictions for those that were formed. However, the alloys that could be readily made all showed an in-plane easy axis. The electronic structure of Fe₃Sn is reported, as are some are magnetic and structural properties for the Fe₃Sn₂, and Fe₅Sn₃ compounds, which could be prepared as mm-sized single crystals.

Authors:

Sales, Brian C. ^[1]; Saparov, Bayrammurad ^[1]; McGuire, Michael A. ^[1]; Singh, David J. ^[1]; Parker, David S. ^[1]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Publication Date:: Wed Nov 12 00:00:00 EST 2014

Research Org.:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:: USDOE Office of Energy Efficiency and Renewable Energy (EERE)

OSTI Identifier:: 1185566

Grant/Contract Number:: AC05-00OR22725

Resource Type:: Accepted Manuscript

Journal Name:: Scientific Reports

Additional Journal Information:: Journal Volume: 4; Journal ID: ISSN 2045-2322

Publisher:: Nature Publishing Group

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; condensed-matter physics; ferromagnetism; physics

Citation Formats


                    Sales, Brian C., Saparov, Bayrammurad, McGuire, Michael A., Singh, David J., and Parker, David S. Ferromagnetism of Fe3Sn and alloys.  United States: N. p., 2014. 
Web.  doi:10.1038/srep07024.

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                    Sales, Brian C., Saparov, Bayrammurad, McGuire, Michael A., Singh, David J., & Parker, David S. Ferromagnetism of Fe3Sn and alloys.  United States.  https://doi.org/10.1038/srep07024

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                    Sales, Brian C., Saparov, Bayrammurad, McGuire, Michael A., Singh, David J., and Parker, David S. Wed .  
"Ferromagnetism of Fe3Sn and alloys".  United States.  https://doi.org/10.1038/srep07024.  https://www.osti.gov/servlets/purl/1185566.

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@article{osti_1185566,

  title        = {Ferromagnetism of Fe3Sn and alloys},

  author       = {Sales, Brian C. and Saparov, Bayrammurad and McGuire, Michael A. and Singh, David J. and Parker, David S.},

  abstractNote = {Hexagonal Fe3Sn has many of the desirable properties for a new permanent magnet phase with a Curie temperature of 725 K, a saturation moment of 1.18 MA/m. and anisotropy energy, K1 of 1.8 MJ/m3. However, contrary to earlier experimental reports, we found both experimentally and theoretically that the easy magnetic axis lies in the hexagonal plane, which is undesirable for a permanent magnet material. One possibility for changing the easy axis direction is through alloying. We used first principles calculations to investigate the effect of elemental substitutions. The calculations showed that substitution on the Sn site has the potential to switch the easy axis direction. Transition metal substitutions with Co or Mn do not have this effect. We attempted synthesis of a number of these alloys and found results in accord with the theoretical predictions for those that were formed. However, the alloys that could be readily made all showed an in-plane easy axis. The electronic structure of Fe3Sn is reported, as are some are magnetic and structural properties for the Fe3Sn2, and Fe5Sn3 compounds, which could be prepared as mm-sized single crystals.},

  doi          = {10.1038/srep07024},

  journal      = {Scientific Reports},

  number       = ,

  volume       = 4,

  place        = {United States},

  year         = {Wed Nov 12 00:00:00 EST 2014},

  month        = {Wed Nov 12 00:00:00 EST 2014}

}

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https://doi.org/10.1038/srep07024

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Cited by: 47 works

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Figures / Tables:

Figure 1: The calculated densities-of-states of Fe₃Sn in the non-magnetic state (a) and in the ferromagnetic state (b).

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Works referenced in this record:

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Works referencing / citing this record:

Structurally Ordered Intermetallic Cobalt Stannide Nanocrystals for High‐Performance Electrocatalytic Overall Water‐Splitting
journal, October 2018

Menezes, Prashanth W.; Panda, Chakadola; Garai, Somenath
Angewandte Chemie, Vol. 130, Issue 46
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Structurally Ordered Intermetallic Cobalt Stannide Nanocrystals for High‐Performance Electrocatalytic Overall Water‐Splitting
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Angewandte Chemie International Edition, Vol. 57, Issue 46
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Massive Dirac fermions in a ferromagnetic kagome metal
journal, March 2018

Ye, Linda; Kang, Mingu; Liu, Junwei
Nature, Vol. 555, Issue 7698
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Tuning magnetocrystalline anisotropy by cobalt alloying in hexagonal Fe3Ge1
journal, September 2018

McGuire, Michael A.; Shanavas, K. V.; Kesler, Michael S.
Scientific Reports, Vol. 8, Issue 1
DOI: 10.1038/s41598-018-32577-x

Fe-Sn nanocrystalline films for flexible magnetic sensors with high thermal stability
journal, March 2019

Satake, Y.; Fujiwara, K.; Shiogai, J.
Scientific Reports, Vol. 9, Issue 1
DOI: 10.1038/s41598-019-39817-8

Tuning the Magnetic Properties and Structural Stabilities of the 2-17-3 Magnets ${Sm}_{2} {Fe}_{17} X_{3}$ ( $X = C$ , N) by Substituting La or Ce for Sm
journal, March 2018

Pandey, Tribhuwan; Du, Mao-Hua; Parker, David S.
Physical Review Applied, Vol. 9, Issue 3
DOI: 10.1103/physrevapplied.9.034002

Reorientation of antiferromagnetism in cobalt doped FeSn
journal, November 2019

Meier, William R.; Yan, Jiaqiang; McGuire, Michael A.
Physical Review B, Vol. 100, Issue 18
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Tuning the magnetocrystalline anisotropy of ${Fe}_{3} Sn$ by alloying
journal, January 2019

Vekilova, Olga Yu.; Fayyazi, Bahar; Skokov, Konstantin P.
Physical Review B, Vol. 99, Issue 2
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Electronic, magnetic, and thermodynamic properties of the kagome layer compound FeSn
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Sales, Brian C.; Yan, Jiaqiang; Meier, William R.
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Tartrate-Based Electrolyte for Electrodeposition of Fe–Sn Alloys
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Mrkonjić Zajkoska, Simona; Dobročka, Edmund; Hansal, Selma
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Fe-Sn nanocrystalline films for flexible magnetic sensors with high thermal stability
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Structural, electronic and magnetic properties of the ordered binary FePt, MnPt, and CrPt3 alloys
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Title: Ferromagnetism of Fe3Sn and alloys

Abstract

Citation Formats

Figures / Tables:

Generalized Gradient Approximation Made Simple journal, October 1996

High pressure X-ray diffraction study of all Fe–Sn intermetallic compounds and one Fe–Sn solid solution journal, September 2006

The Metal Flux: A Preparative Tool for the Exploration of Intermetallic Compounds journal, November 2005

Magnetic properties of Y2Fe14B and Nd2Fe14B single crystals journal, September 1984

New developments in hard magnetic materials journal, September 1991

Hard Magnetic Materials: A Perspective journal, December 2011

Growth of single crystals from metallic fluxes journal, June 1992

Exchange Anisotropy and Long‐Range Magnetic Order in the Mixed Intermetallic Compounds, (Mn, Fe) 3 Sn journal, March 1965

Mossbauer effect study of Fe 3 Sn 2 journal, February 1978

Magnetic properties of Fe 3 Sn 2 . II. Neutron diffraction study (and Mossbauer effect) journal, November 1978

Mössbauer-Effect Studies of Iron-Tin Alloys journal, November 1970

R 2 Fe 14 B materials: Intrinsic properties and technological aspects journal, October 1991

Aligned crystallite powder of NdFeAsO 0.86 F 0.14 : Magnetic hysteresis and penetration depth journal, June 2009

Magnetic properties of Y2Fe14B and Nd2Fe14B single crystals journal, December 1993

The Metal Flux: A Preparative Tool for the Exploration of Intermetallic Compounds journal, January 2006

The Metal Flux: A Preparative Tool for the Exploration of Intermetallic Compounds journal, January 2006

Magnetic properties of Y2Fe14B and Nd2Fe14B single crystals journal, December 1993

High pressure X-ray diffraction study of all Fe–Sn intermetallic compounds and one Fe–Sn solid solution journal, September 2006

Structurally Ordered Intermetallic Cobalt Stannide Nanocrystals for High‐Performance Electrocatalytic Overall Water‐Splitting journal, October 2018

Structurally Ordered Intermetallic Cobalt Stannide Nanocrystals for High‐Performance Electrocatalytic Overall Water‐Splitting journal, November 2018

Massive Dirac fermions in a ferromagnetic kagome metal journal, March 2018

Tuning magnetocrystalline anisotropy by cobalt alloying in hexagonal Fe3Ge1 journal, September 2018

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Tuning the magnetocrystalline anisotropy of Fe 3 Sn by alloying journal, January 2019

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Title: Ferromagnetism of Fe₃Sn and alloys

Generalized Gradient Approximation Made Simple
journal, October 1996

High pressure X-ray diffraction study of all Fe–Sn intermetallic compounds and one Fe–Sn solid solution
journal, September 2006

The Metal Flux: A Preparative Tool for the Exploration of Intermetallic Compounds
journal, November 2005

Magnetic properties of Y2Fe14B and Nd2Fe14B single crystals
journal, September 1984

New developments in hard magnetic materials
journal, September 1991

Hard Magnetic Materials: A Perspective
journal, December 2011

Growth of single crystals from metallic fluxes
journal, June 1992

Exchange Anisotropy and Long‐Range Magnetic Order in the Mixed Intermetallic Compounds, (Mn, Fe) ₃ Sn
journal, March 1965

Mossbauer effect study of Fe ₃ Sn ₂
journal, February 1978

Magnetic properties of Fe ₃ Sn ₂ . II. Neutron diffraction study (and Mossbauer effect)
journal, November 1978

Mössbauer-Effect Studies of Iron-Tin Alloys
journal, November 1970

$R_{2}$ ${Fe}_{14}$ B materials: Intrinsic properties and technological aspects
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Aligned crystallite powder of ${NdFeAsO}_{0.86} F_{0.14}$ : Magnetic hysteresis and penetration depth
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Magnetic properties of Y2Fe14B and Nd2Fe14B single crystals
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The Metal Flux: A Preparative Tool for the Exploration of Intermetallic Compounds
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The Metal Flux: A Preparative Tool for the Exploration of Intermetallic Compounds
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High pressure X-ray diffraction study of all Fe–Sn intermetallic compounds and one Fe–Sn solid solution
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