Water Desalination Using Nanoporous Single-Layer Graphene with Tunable Pore Size
Abstract
Graphene has great potential to serve as a separation membrane due to its unique properties such as chemical and mechanical stability, flexibility and most importantly its one-atom thickness. In this study, we demonstrate first experimental evidence of the use of single-layer porous graphene as a desalination membrane. Nanometer-sized pores are introduced into single layer graphene using a convenient oxygen plasma etching process that permits tuning of the pore size. The resulting porous graphene membrane exhibited high rejection of salt ions and rapid water transport, thus functioning as an efficient water desalination membrane. Salt rejection selectivity of nearly 100% and exceptionally high water fluxes exceeding 105 g m-2 s-1 at 40 C were measured using saturated water vapor as a driving force.
- Authors:
-
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)
- Sponsoring Org.:
- USDOE Laboratory Directed Research and Development (LDRD) Program
- OSTI Identifier:
- 1185491
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Nanotechnology
- Additional Journal Information:
- Journal Volume: 10; Journal Issue: 5; Journal ID: ISSN 1748-3387
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 77 NANOSCIENCE AND NANOTECHNOLOGY
Citation Formats
Surwade, Sumedh P., Smirnov, Sergei N., Vlassiouk, Ivan V., Unocic, Raymond R., Veith, Gabriel M., Dai, Sheng, and Mahurin, Shannon Mark. Water Desalination Using Nanoporous Single-Layer Graphene with Tunable Pore Size. United States: N. p., 2015.
Web. doi:10.1038/nnano.2015.37.
Surwade, Sumedh P., Smirnov, Sergei N., Vlassiouk, Ivan V., Unocic, Raymond R., Veith, Gabriel M., Dai, Sheng, & Mahurin, Shannon Mark. Water Desalination Using Nanoporous Single-Layer Graphene with Tunable Pore Size. United States. https://doi.org/10.1038/nnano.2015.37
Surwade, Sumedh P., Smirnov, Sergei N., Vlassiouk, Ivan V., Unocic, Raymond R., Veith, Gabriel M., Dai, Sheng, and Mahurin, Shannon Mark. Mon .
"Water Desalination Using Nanoporous Single-Layer Graphene with Tunable Pore Size". United States. https://doi.org/10.1038/nnano.2015.37. https://www.osti.gov/servlets/purl/1185491.
@article{osti_1185491,
title = {Water Desalination Using Nanoporous Single-Layer Graphene with Tunable Pore Size},
author = {Surwade, Sumedh P. and Smirnov, Sergei N. and Vlassiouk, Ivan V. and Unocic, Raymond R. and Veith, Gabriel M. and Dai, Sheng and Mahurin, Shannon Mark},
abstractNote = {Graphene has great potential to serve as a separation membrane due to its unique properties such as chemical and mechanical stability, flexibility and most importantly its one-atom thickness. In this study, we demonstrate first experimental evidence of the use of single-layer porous graphene as a desalination membrane. Nanometer-sized pores are introduced into single layer graphene using a convenient oxygen plasma etching process that permits tuning of the pore size. The resulting porous graphene membrane exhibited high rejection of salt ions and rapid water transport, thus functioning as an efficient water desalination membrane. Salt rejection selectivity of nearly 100% and exceptionally high water fluxes exceeding 105 g m-2 s-1 at 40 C were measured using saturated water vapor as a driving force.},
doi = {10.1038/nnano.2015.37},
journal = {Nature Nanotechnology},
number = 5,
volume = 10,
place = {United States},
year = {Mon Mar 23 00:00:00 EDT 2015},
month = {Mon Mar 23 00:00:00 EDT 2015}
}
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- Sahu, Subin; Di Ventra, Massimiliano; Zwolak, Michael
- arXiv
Highly Efficient Ion Rejection by Graphene Oxide Membranes via Ion-controlling Interlayer Spacing
preprint, January 2016
- Chen, Liang; Shi, Guosheng; Shen, Jie
- arXiv
Perfect proton selectivity in ion transport through two-dimensional crystals
text, January 2019
- Mogg, L.; Zhang, S.; Hao, G. -P.
- arXiv
On-Surface Synthesis of a Nonplanar Porous Nanographene
text, January 2019
- Xu, Kun; Urgel, José I.; Eimre, Kristjan
- American Chemical Society