Magnetochromic effect in multiferroic R In 1 ₋ x Mn x O 3 ( R = Tb , Dy)

Chen, P.; Holinsworth, B. S.; O'Neal, K. R.; Brinzari, T. V.; Mazumdar, D.; Topping, C. V.; Luo, X.; Cheong, S.-W.; Singleton, J.; McGill, S.; Musfeldt, J. L.

doi:10.1103/PhysRevB.91.205130

Title: Magnetochromic effect in multiferroic $R {In}_{1 ₋ x} {Mn}_{x} O_{3}$ ( $R = Tb$ , Dy)

Abstract

We combined high field magnetization and magneto-optical spectroscopy to investigate spin-charge coupling in Mn-substituted rare-earth indium oxides of chemical formula RIn₁₋_xMn_xO₃ (R=Tb, Dy). The edge states, on-site Mn³⁺d to d excitations, and rare-earth f-manifold excitations all track the magnetization energy due to dominant Zeeman interactions. The field-induced modifications to the rare-earth excitations are quite large because spin-orbit coupling naturally mixes spin and charge, suggesting that the next logical step in the design strategy should be to bring spin-orbit coupling onto the trigonal bipyramidal chromophore site with a 4 or 5d center.

Authors:: Chen, P.; Holinsworth, B. S.; O'Neal, K. R.; Brinzari, T. V.; Mazumdar, D.; Topping, C. V.; Luo, X.; Cheong, S.-W.; Singleton, J.; McGill, S.; Musfeldt, J. L.

Publication Date:: Tue May 26 00:00:00 EDT 2015

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1182831

Grant/Contract Number:: FG02-01ER45885; FG02-07ER46382

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Physical Review. B, Condensed Matter and Materials Physics

Additional Journal Information:: Journal Name: Physical Review. B, Condensed Matter and Materials Physics Journal Volume: 91 Journal Issue: 20; Journal ID: ISSN 1098-0121

Publisher:: American Physical Society

Country of Publication:: United States

Language:: English

Citation Formats


                    Chen, P., Holinsworth, B. S., O'Neal, K. R., Brinzari, T. V., Mazumdar, D., Topping, C. V., Luo, X., Cheong, S.-W., Singleton, J., McGill, S., and Musfeldt, J. L. Magnetochromic effect in multiferroic R In 1 ₋ x Mn x O 3 ( R = Tb , Dy).  United States: N. p., 2015. 
Web.  doi:10.1103/PhysRevB.91.205130.

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                    Chen, P., Holinsworth, B. S., O'Neal, K. R., Brinzari, T. V., Mazumdar, D., Topping, C. V., Luo, X., Cheong, S.-W., Singleton, J., McGill, S., & Musfeldt, J. L. Magnetochromic effect in multiferroic R In 1 ₋ x Mn x O 3 ( R = Tb , Dy).  United States.  https://doi.org/10.1103/PhysRevB.91.205130

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                    Chen, P., Holinsworth, B. S., O'Neal, K. R., Brinzari, T. V., Mazumdar, D., Topping, C. V., Luo, X., Cheong, S.-W., Singleton, J., McGill, S., and Musfeldt, J. L. Tue .  
"Magnetochromic effect in multiferroic R In 1 ₋ x Mn x O 3 ( R = Tb , Dy)".  United States.  https://doi.org/10.1103/PhysRevB.91.205130.

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@article{osti_1182831,

  title        = {Magnetochromic effect in multiferroic R In 1 ₋ x Mn x O 3 ( R = Tb , Dy)},

  author       = {Chen, P. and Holinsworth, B. S. and O'Neal, K. R. and Brinzari, T. V. and Mazumdar, D. and Topping, C. V. and Luo, X. and Cheong, S.-W. and Singleton, J. and McGill, S. and Musfeldt, J. L.},

  abstractNote = {We combined high field magnetization and magneto-optical spectroscopy to investigate spin-charge coupling in Mn-substituted rare-earth indium oxides of chemical formula RIn₁₋xMnxO₃ (R=Tb, Dy). The edge states, on-site Mn³⁺d to d excitations, and rare-earth f-manifold excitations all track the magnetization energy due to dominant Zeeman interactions. The field-induced modifications to the rare-earth excitations are quite large because spin-orbit coupling naturally mixes spin and charge, suggesting that the next logical step in the design strategy should be to bring spin-orbit coupling onto the trigonal bipyramidal chromophore site with a 4 or 5d center.},

  doi          = {10.1103/PhysRevB.91.205130},

  journal      = {Physical Review. B, Condensed Matter and Materials Physics},

  number       = 20,

  volume       = 91,

  place        = {United States},

  year         = {Tue May 26 00:00:00 EDT 2015},

  month        = {Tue May 26 00:00:00 EDT 2015}

}

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Title: Magnetochromic effect in multiferroic R In 1 ₋ x Mn x O 3 ( R = Tb , Dy)

Abstract

Citation Formats

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Title: Magnetochromic effect in multiferroic $R {In}_{1 ₋ x} {Mn}_{x} O_{3}$ ( $R = Tb$ , Dy)

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