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1

Note: Grazing incidence small and wide angle x-ray scattering combined with imaging ellipsometry  

SciTech Connect

The combination of grazing incidence small angle x-ray scattering (GISAXS) and grazing incidence wide angle x-ray scattering (GIWAXS) with optical imaging ellipsometry is presented as an upgrade of the available measurement techniques at the wiggler beamline BW4 of the Hamburger Synchrotronstrahlungslabor. The instrument is introduced with the description of the alignment procedure to assure the measurement of imaging ellipsometry and GISAXS/GIWAXS on the same sample spot. To demonstrate the possibilities of the new instrument examples of morphological investigation on films made of poly(3-hexylthiophene) and [6,6]-phenyl-C{sub 61} butyric acid methyl ester as well as textured poly(9,9-dioctylfluorene-alt-benzo-thia-diazole) are shown.

Koerstgens, V.; Meier, R.; Ruderer, M. A.; Guo, S.; Chiang, H.-Y.; Mueller-Buschbaum, P. [Technische Universitaet Muenchen, Physik-Department, Lehrstuhl fuer Funktionelle Materialien, James-Franck-Str. 1, 85748 Garching (Germany); Perlich, J.; Roth, S. V.; Gehrke, R. [HASYLAB, DESY, Notkestr. 85, 22607, Hamburg (Germany)

2012-07-15T23:59:59.000Z

2

Ray tracing flux calculation for the small and wide angle x-ray scattering diffraction station at the SESAME synchrotron radiation facility  

SciTech Connect

The calculation for the optics of the synchrotron radiation small and wide angle x-ray scattering beamline, currently under construction at SESAME is described. This beamline is based on a cylindrically bent germanium (111) single crystal with an asymmetric cut of 10.5 deg., followed by a 1.2 m long rhodium coated plane mirror bent into a cylindrical form. The focusing properties of bent asymmetrically cut crystals have not yet been studied in depth. The present paper is devoted to study of a particular application of a bent asymmetrically cut crystal using ray tracing simulations with the SHADOW code. These simulations show that photon fluxes of order of 1.09x10{sup 11} photons/s will be available at the experimental focus at 8.79 keV. The focused beam dimensions will be 2.2 mm horizontal full width at half maximum (FWHM) by 0.12 mm vertical (FWHM).

Salah, Wa'el [Synchrotron-light for Experimental Science and Application in the Middle East (SESAME), P.O. Box 7, Allan 19252 (Jordan); Department of Physics, The Hashemite University, Zarqa 13115 (Jordan); Sanchez del Rio, M. [European Synchrotron Radiation Facility, Bp 220, 38043 Grenoble Cedex (France); Hoorani, H. [Synchrotron-light for Experimental Science and Application in the Middle East (SESAME), P.O. Box 7, Allan 19252 (Jordan)

2009-09-15T23:59:59.000Z

3

Surface Area and Microporosity of Carbon Aerogels from Gas Adsorption and Small- and Wide-Angle X-ray Scattering Measurements  

E-Print Network (OSTI)

A carbon aerogel was obtained by carbonization of an organic aerogel prepared by sol-gel polymerization of resorcinol and formaldehyde in water. The carbon aerogel was then CO2 activated at 800 °C to increase its surface area and widen its microporosity. Evolution of these parameters was followed by gas adsorption and small- and wide-angle X-ray scattering (SAXS and WAXS, respectively) with contrast variation by using dry and wet (immersion in benzene and m-xylene) samples. For the original carbon aerogel, the surface area, SSAXS, obtained by SAXS, is larger than that obtained by gas adsorption (Sads). The values become nearly the same as the degree of activation of the carbon aerogel increases. This feature is due to the widening of the narrow microporosity in the carbon aerogel as the degree of activation is increased. In addition, WAXS results show that the short-range spatial correlations into the assemblies of hydrocarbon molecules confined inside the micropores are different from those existing in the liquid phase. 1.

David Fairén-jiménez; Francisco Carrasco-marín; David Djurado; Françoise Bley; Françoise Ehrburger-dolle; Carlos Moreno-castilla

2005-01-01T23:59:59.000Z

4

Fluctuation X-Ray Scattering  

SciTech Connect

The work supported by the grant was aimed at developing novel methods of finding the structures of biomolecules using x-rays from novel sources such as the x-ray free electron laser and modern synchrotrons

Saldin, PI: D. K.; Co-I's: J. C. H. Spence and P. Fromme

2013-01-25T23:59:59.000Z

5

Biomolecular solution X-ray scattering at the National Synchrotron Light Source  

E-Print Network (OSTI)

In recent years there has been a growing interest in the application of X-ray scattering techniques to biomolecules in solution. At NSLS, a new undulatorbased beamline, X9, has been constructed to address the oversubscribed user demand for X-ray scattering. Beamline X9 has the capability to perform small/wide-angle X-ray scattering (SAXS/WAXS) all in one single instrument. This is accomplished by utilizing a vacuum sample/detector chamber that is an integral part of the SAXS scattering flight path. This vacuum chamber allows a WAXS detector to be positioned at a close distance from the sample, while not interfering with scattered X-rays at small angles from reaching the SAXS detector. A regular training program, the X9 workbench, has also been established to allow users to become familiar with beamline X9 for solution X-ray scattering. Keywords: SAXS; WAXS; beamline; proteins; DNA/RNA. 1.

Marc Allaire; Lin Yang

2010-01-01T23:59:59.000Z

6

Inelastic X-ray and Nuclear Resonant Scattering  

NLE Websites -- All DOE Office Websites (Extended Search)

Beamlines Divisions Argonne Home > Advanced Photon Source > Inelastic X-ray and Nuclear Resonant Scattering The Inelastic X-ray and Nuclear Resonant Scattering group...

7

Small Angle X-Ray Scattering Detector  

DOE Patents (OSTI)

A detector for time-resolved small-angle x-ray scattering includes a nearly constant diameter, evacuated linear tube having an end plate detector with a first fluorescent screen and concentric rings of first fiber optic bundles for low angle scattering detection and an annular detector having a second fluorescent screen and second fiber optic bundles concentrically disposed about the tube for higher angle scattering detection. With the scattering source, i.e., the specimen under investigation, located outside of the evacuated tube on the tube's longitudinal axis, scattered x-rays are detected by the fiber optic bundles, to each of which is coupled a respective photodetector, to provide a measurement resolution, i.e., dq/q, where q is the momentum transferred from an incident x-ray to an x-ray scattering specimen, of 2% over two (2) orders of magnitude in reciprocal space, i.e., qmax/qmin approx=lO0.

Hessler, Jan P.

2004-06-15T23:59:59.000Z

8

Massively parallel X-ray scattering simulations  

Science Conference Proceedings (OSTI)

Although present X-ray scattering techniques can provide tremendous information on the nano-structural properties of materials that are valuable in the design and fabrication of energy-relevant nano-devices, a primary challenge remains in the analyses ...

Abhinav Sarje; Xiaoye S. Li; Slim Chourou; Elaine R. Chan; Alexander Hexemer

2012-11-01T23:59:59.000Z

9

X?ray Fluorescence (XRF) Assay Using Laser Compton Scattered (LCS) X?rays  

Science Conference Proceedings (OSTI)

Laser Compton Scattered (LCS) X?rays are produced as a result of the interaction between accelerated electrons and a laser beam. The yield of LCS X?rays is dependent on the laser power

Syed F. Naeem; Khalid Chouffani; Douglas P. Wells

2009-01-01T23:59:59.000Z

10

HIGH BRILLIANCE X-RAY SCATTERING FOR  

NLE Websites -- All DOE Office Websites (Extended Search)

BRILLIANCE X-RAY SCATTERING FOR BRILLIANCE X-RAY SCATTERING FOR LIFE SCIENCES (LIX) Group Leader: Lin Yang Proposal Team: O. Bilsel 1 , B. Hsiao 2 , H. Huang 3 , T. Irving 4 , A. Menzel 5 , L. Pollack 6 , C. Riekel 7 , J. Rubert 8 , H. Tsuruta 9 , L. Yang 10 1 University of Massachusetts, 2 Stony Brook University, 3 Rice University, 4 IIT, 5SLS, 6 Cornell University, 7 European Synchrotron Radiation Facility, 8 NEU, 9 Stanford Synchrotron Radiation Lightsource, 10 Brookhaven National Laboratory TECHNIQUES AND CAPABILITIES APPLICATIONS ADDITIONAL INFORMATION * Energy range 2-20keV using undulator source. Simultaneous SAXS/WAXS to cover 0.003-3Å -1 at 12keV with 1 micron spot size * Time-resolved solution scattering with resolution of (1) microseconds to milliseconds using continuous-flow mixing (5µm x 10µm spot size) and (2) milliseconds using stopped-

11

X-ray scattering intensities of water at extreme pressure and temperature  

DOE Green Energy (OSTI)

We have calculated the coherent x-ray scattering intensity of several phases of water at 1500 and 2000 K under high pressure, using ab initio Density Functional Theory (DFT). Our calculations span the molecular liquid, ice VII, and superionic solid phases, including the recently predicted symmetrically hydrogen bonded region of the superionic phase. We show that wide angle x-ray scattering intensity could be used to determine phase boundaries between these high pressure phases, and we compare the results for ice VII and superionic water. We compute simulated spectra and provide new atomic scattering form factors for water at extreme conditions, which take into account frequently neglected changes in ionic charge and electron delocalization. We show that our modifed atomic form factors allow for a nearly exact comaprison to the total x-ray scattering intensities calculated from DFT. Finally, we analyze the effect our new form factors have on determination of the oxygen-oxygen radial distribution function.

Goldman, N; Fried, L E

2007-01-03T23:59:59.000Z

12

Microstructural Mapping Using High-Energy X-Ray Scattering  

Science Conference Proceedings (OSTI)

Abstract Scope, Advanced characterization methods at the APS permit unique in- situ ... The combination of an undulator source, brilliance preserving optics and focusing .... Ultra-Small-Angle X-Ray Scattering—X-Ray Photon Correlation ...

13

Introduction to Neutron and X-Ray Scattering  

NLE Websites -- All DOE Office Websites (Extended Search)

Scattering Studies of Thin Scattering Studies of Thin Polymer Films Introduction to Neutron and X-Ray Scattering Sunil K. Sinha UCSD/LANL Acknowledgements: Prof. R.Pynn( Indiana U.) Prof. M.Tolan (U. Dortmund) Wilhelm Conrad Röntgen 1845-1923 1895: Discovery of X-Rays 1901 W. C. Röntgen in Physics for the discovery of x-rays. 1914 M. von Laue in Physics for x-ray diffraction from crystals. 1915 W. H. Bragg and W. L. Bragg in Physics for crystal structure determination. 1917 C. G. Barkla in Physics for characteristic radiation of elements. 1924 K. M. G. Siegbahn in Physics for x-ray spectroscopy. 1927 A. H. Compton in Physics for scattering of x-rays by electrons. 1936 P. Debye in Chemistry for diffraction of x-rays and electrons in gases.

14

X-Ray Scattering Group, Condensed Matter Physics & Materials...  

NLE Websites -- All DOE Office Websites (Extended Search)

Proceedings of the 12th International Clay Conference, Bahia Blanca, Argentina, July 22-28, 2001. Gibbs, D. X-ray magnetic scattering. Synchrotron Radiation News...

15

Inelastic X-ray Scattering Reveals Microscopic Transport Properties...  

NLE Websites -- All DOE Office Websites (Extended Search)

Inelastic X-ray Scattering Reveals Microscopic Transport Properties of Molten Aluminum Oxide The transport properties of high-temperature oxide melts are of considerable interest...

16

New Directions in X-ray Scattering - SSRL  

NLE Websites -- All DOE Office Websites (Extended Search)

associated with chemically and radioactively contaminated ground-water. Ability to probe weak scattering from single crystals as function of energy (resonance) and x-ray...

17

Photon Sciences | Beamlines | IXS: Inelastic X-ray Scattering  

NLE Websites -- All DOE Office Websites (Extended Search)

IXS: Inelastic X-ray Scattering IXS: Inelastic X-ray Scattering Poster | Fact Sheet | Preliminary Design Report Scientific Scope Many hot topics related to the high frequency dynamics of condensed matter require both a narrower and steeper resolution function and access to a broader dynamic range than what are currently available. This represents a sort of "no man's land" that falls right in the dynamic gap lying between the high frequency spectroscopies, such as inelastic x-ray scattering (IXS), and the low frequency ones. New IXS spectrometers with improved energy and momentum resolutions would be required to fill this gap. To achieve this goal, a new x-ray optics concept for both the monochromatization and energy analysis of x-rays will be implemented at the NSLS-II Inelastic X-ray Scattering beamline. This solution exploits the

18

Fast Lidar and Radar Multiple-Scattering Models. Part II: Wide-Angle Scattering Using the Time-Dependent Two-Stream Approximation  

Science Conference Proceedings (OSTI)

Spaceborne lidar returns from liquid water clouds contain significant contributions from photons that have experienced many wide-angle multiple-scattering events, resulting in returns appearing to originate from far beyond the end of the cloud. A ...

Robin J. Hogan; Alessandro Battaglia

2008-12-01T23:59:59.000Z

19

Probing Spatial, Electronic Structures with X-ray Scattering, Spectroscopic  

NLE Websites -- All DOE Office Websites (Extended Search)

Probing Spatial, Electronic Structures with X-ray Scattering, Spectroscopic Probing Spatial, Electronic Structures with X-ray Scattering, Spectroscopic Techniques Wednesday, September 5, 2012 - 10:45am SLAC, Bldg. 137, Room 226 Gang Chen Seminar: Structures at atomic scales are traditionally determined through X-ray crystallography that amplifies scattering intensities by introducing spatial periodicity. For amorphous materials and many macromolecules, such as viruses, proteins and biofilms, it is hard to determine structures due to their incapability to crystallize or change of configuration during crystallization. In this talk, I will present the application of X-ray reflectivity and a newly developed fluctuation X-ray scattering technique to study the structures of lipid membranes and randomly oriented nanoparticles. Three different types of domain registrations occurring with

20

ESRF HIGHLIGHTS 2005 X-RAY ABSORPTION AND MAGNETIC SCATTERING  

E-Print Network (OSTI)

96 ESRF HIGHLIGHTS 2005 X-RAY ABSORPTION AND MAGNETIC SCATTERING References [1] C. Antoniak, J to original phenomena. These effects are observed in charge-density wave (CDW) materials. Upon cooling of the screw like dislocation shown in Figure 121b. #12;97 HIGHLIGHTS 2005 ESRF X-RAY ABSORPTION AND MAGNETIC

Paris-Sud 11, Université de

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


21

Direct three-dimensional coherently scattered x-ray microtomography  

Science Conference Proceedings (OSTI)

Purpose: It has been shown that coherently scattered x rays can be used to discriminate and identify specific components in a mixture of low atomic weight materials. The authors demonstrated a new method of doing coherently scattered x-ray tomography with a thin sheet of x ray. Methods: A collimated x-ray fan-beam, a parallel polycapillary collimator, and a phantom consisting of several biocompatible materials of low attenuation-based contrast were used to investigate the feasibility of the method. Because of the particular experimental setup, only the phantom translation perpendicular to the x-ray beam is needed and, thus, there is no need of Radon-type tomographic reconstruction, except for the correction of the attenuation to the primary and scattered x rays, which was performed by using a conventional attenuation-based tomographic image data set. The coherent scatter image contrast changes with momentum transfer among component materials in the specimen were investigated with multiple x-ray sources with narrow bandwidth spectra generated with anode and filter combinations of Cu/Ni (8 keV), Mo/Zr (18 keV), and Ag/Pd (22 keV) and at multiple scatter angles by orienting the detector and polycapillary collimator at different angles to the illuminating x ray. Results: The contrast among different materials changes with the x-ray source energy and the angle at which the image was measured. The coherent scatter profiles obtained from the coherent scatter images are consistent with the published results. Conclusions: This method can be used to directly generate the three-dimensional coherent scatter images of small animal, biopsies, or other small objects with low atomic weight biological or similar synthetic materials with low attenuation contrast. With equipment optimized, submillimeter spatial resolution may be achieved.

Cui Congwu; Jorgensen, Steven M.; Eaker, Diane R.; Ritman, Erik L. [Department of Medical Physics, CancerCare Manitoba, 675 McDermot Avenue, Winnipeg, Manitoba R3E 0V9 (Canada); Department of Physiology and Biomedical Engineering, Mayo Clinic, 200 First Street Southwest, Alfred Building 2-409, Rochester, Minnesota 55905 (United States)

2010-12-15T23:59:59.000Z

22

Resonant Soft X-Ray Scattering - Combining Structural with Spectroscopic  

NLE Websites -- All DOE Office Websites (Extended Search)

Resonant Soft X-Ray Scattering - Combining Structural with Spectroscopic Resonant Soft X-Ray Scattering - Combining Structural with Spectroscopic Refinement Friday, September 28, 2012 - 10:00am SLAC, Bldg. 137, Room 322 SSRL Presents Kevin Stone X-ray absorption spectroscopy has become an important tool in understanding the electronic structure of materials. Resonant absorption edges in the soft x-ray regime are especially interesting as they allow the study of the lighter elements, such as in organic or organo-metallic substances, as well as important L-edges of the 3d transition metals important in magnetic and oxide systems. Measurements of soft x-ray absorption spectra are inherently surface sensitive, and are plagued by issues such as extinction (in electron yield measurements) or self absorption (in fluorescence yield

23

X-Ray Scattering Group, Condensed Matter Physics & Materials...  

NLE Websites -- All DOE Office Websites (Extended Search)

D.F. Inelastic x-ray scattering investigations of lattice dynamics in SmFeAsO1-xFy superconductors. Proceedings of The 9th International Conference on Spectroscopies in Novel...

24

Laser assisted Compton scattering of X-ray photons  

E-Print Network (OSTI)

The Compton scattering of X-ray photons, assisted by a short intense optical laser pulse is discussed. The differential scattering cross section reveals the interesting feature that the main Klein-Nishina line is accompanied by a series of side-lines forming a broad plateau where up to ${\\cal O} (10^3)$ laser photons participate simultaneously in a single scattering event. Due to the non-linear mixing of X-ray and laser photons a frequency dependent rotation of the polarization of the final state photons relative to the scattering plane emerges. A consistent description of the scattering process with short laser pulses requires to work with X-ray pulses. An experimental investigation can be accomplished, e.g., at LCLS or the European XFEL in the near future.

D. Seipt; B. Kampfer

2013-09-09T23:59:59.000Z

25

High performance x-ray anti-scatter grid  

DOE Patents (OSTI)

Disclosed are an x-ray anti-scatter grid for x-ray imaging, particularly for screening mammography, and method for fabricating same, x-rays incident along a direct path pass through a grid composed of a plurality of parallel or crossed openings, microchannels, grooves, or slots etched in a substrate, such as silicon, having the walls of the microchannels or slots coated with a high opacity material, such as gold, while x-rays incident at angels with respect to the slots of the grid, arising from scatter, are blocked. The thickness of the substrate is dependent on the specific application of the grid, whereby a substrate of the grid for mammography would be thinner than one for chest radiology. Instead of coating the walls of the slots, such could be filed with an appropriate liquid, such as mercury. 4 Figs.

Logan, C.M.

1995-05-23T23:59:59.000Z

26

High performance x-ray anti-scatter grid  

DOE Patents (OSTI)

An x-ray anti-scatter grid for x-ray imaging, particularly for screening mammography, and method for fabricating same, x-rays incident along a direct path pass through a grid composed of a plurality of parallel or crossed openings, microchannels, grooves, or slots etched in a substrate, such as silicon, having the walls of the microchannels or slots coated with a high opacity material, such as gold, while x-rays incident at angels with respect to the slots of the grid, arising from scatter, are blocked. The thickness of the substrate is dependent on the specific application of the grid, whereby a substrate of the grid for mammography would be thinner than one for chest radiology. Instead of coating the walls of the slots, such could be filed with an appropriate liquid, such as mercury.

Logan, Clinton M. (Pleasanton, CA)

1995-01-01T23:59:59.000Z

27

Active probing of cloud multiple scattering, optical depth, vertical thickness, and liquid water content using wide-angle imaging LIDAR.  

SciTech Connect

At most optical wavelengths, laser light in a cloud lidar experiment is not absorbed but merely scattered out of the beam, eventually escaping the cloud via multiple scattering. There is much information available in this light scattered far from the input beam, information ignored by traditional 'on-beam' lidar. Monitoring these off-beam returns in a fully space- and time-resolved manner is the essence of our unique instrument, Wide Angle Imaging Lidar (WAIL). In effect, WAIL produces wide-field (60-degree full-angle) 'movies' of the scattering process and records the cloud's radiative Green functions. A direct data product of WAIL is the distribution of photon path lengths resulting from multiple scattering in the cloud. Following insights from diffusion theory, we can use the measured Green functions to infer the physical thickness and optical depth of the cloud layer, and, from there, estimate the volume-averaged liquid water content. WAIL is notable in that it is applicable to optically thick clouds, a regime in which traditional lidar is reduced to ceilometry. Here we present recent WAIL data oti various clouds and discuss the extension of WAIL to full diurnal monitoring by means of an ultra-narrow magneto-optic atomic line filter for daytime measurements.

Love, Steven P.; Davis, A. B. (Anthony B.); Rohde, C. A. (Charles A.); Tellier, L. L. (Larry L.); Ho, Cheng,

2002-01-01T23:59:59.000Z

28

Imaging X-ray Thomson Scattering Spectrometer Design and Demonstration  

SciTech Connect

In many laboratory astrophysics experiments, intense laser irradiation creates novel material conditions with large, one-dimensional gradients in the temperature, density, and ionization state. X-ray Thomson scattering is a powerful technique for measuring these plasma parameters. However, the scattered signal has previously been measured with little or no spatial resolution, which limits the ability to diagnose inhomogeneous plasmas. We report on the development of a new imaging x-ray Thomson spectrometer (IXTS) for the Omega laser facility. The diffraction of x-rays from a toroidally-curved crystal creates high-resolution images that are spatially resolved along a one-dimensional profile while spectrally dispersing the radiation. This focusing geometry allows for high brightness while localizing noise sources and improving the linearity of the dispersion. Preliminary results are presented from a scattering experiment that used the IXTS to measure the temperature profile of a shocked carbon foam.

Gamboa, E.J. [University of Michigan; Huntington, C.M. [University of Michigan; Trantham, M.R. [University of Michigan; Keiter, P.A [University of Michigan; Drake, R.P. [University of Michigan; Montgomery, David [Los Alamos National Laboratory; Benage, John F. [Los Alamos National Laboratory; Letzring, Samuel A. [Los Alamos National Laboratory

2012-05-04T23:59:59.000Z

29

Electronic Structure of Dense Plasmas by X-Ray Scattering  

DOE Green Energy (OSTI)

We present an improved analytical expression for the x-ray dynamic structure factor from a dense plasma which includes the effects of weakly bound electrons. This result can be applied to describe scattering from low to moderate Z plasmas, and it covers the entire range of plasma conditions that can be found in inertial confinement fusion experiments, from ideal to degenerate up to moderately coupled systems. We use our theory to interpret x-ray scattering experiments from solid density carbon plasma and to extract accurate measurements of electron temperature, electron density and charge state. We use our experimental results to validate various equation-of-state models for carbon plasmas.

Gregori, G; Glenzer, S H; Rogers, F J; Pollaine, S M; Froula, D H; Blancard, C; Faussurier, G; Renaudin, P; Kuhlbrodt, S; Redmer, R; Landen, O L

2003-10-07T23:59:59.000Z

30

Neutron and X-Ray Scattering - Argonne National Laboratories, Materials  

NLE Websites -- All DOE Office Websites (Extended Search)

Home Home Neutron and X-Ray Scattering Neutron and X-ray Scattering Science Recent advances in neutron and x-ray scattering instrumentation at major DOE facilities such as the Spallation Neutron Source and Advanced Photon Source provide unprecedented insights into complex phenomena in bulk and interfacial materials. The vision of our group is to harness the complementarity of neutrons and x-rays to study how materials respond on a range of length and time scales to phase competition, so that we can learn to control emergent behavior and generate functional properties in energy-related materials. We use neutrons and x-rays to investigate the structure and dynamics of bulk and interfacial materials with properties that are useful for energy applications, such as superconductivity, magnetism and thermoelectricity. Phase competition can generate or enhance such properties, but it is extremely challenging to characterize fluctuations in the competing order, whether in bulk disordered materials, or artificial heterostructures. Our goal is to utilize efficient techniques that we have been developing for measuring nanoscale phase fluctuations, both static and dynamic, to enable the rational design of new materials for energy within MSD.

31

Neutron and Synchrotron X-Ray Scattering Studies of Superconductors  

Science Conference Proceedings (OSTI)

Superconductors hold the promise for a more stable and efficient electrical grid, but new isotropic, high-temperature superconductors are needed in order to reduce cable manufacturing costs. The effort to understand high-temperature superconductivity, especially in the layered cuprates, provides guidance to the search for new superconductors. Neutron scattering has long provided an important probe of the collective excitations that are involved in the pairing mechanism. For the cuprates, neutron and x-ray diffraction techniques also provide information on competing types of order, such as charge and spin stripes, that appear to be closely connected to the superconductivity. Recently, inelastic x-ray scattering has become competitive for studying phonons and may soon provide valuable information on electronic excitations. Examples of how these techniques contribute to our understanding of superconductivity are presented.

Tranquada,J.M.

2008-09-01T23:59:59.000Z

32

X-Ray Scattering Group, Condensed Matter Physics & Materials...  

NLE Websites -- All DOE Office Websites (Extended Search)

- Brookhaven National Laboratory, Upton, NY Beamline X1A2 - Soft x-ray diffraction and nano-imaging Beamline X17 - X-ray powder diffraction Beamline X22C - Resonant x-ray...

33

Air-core grid for scattered x-ray rejection  

DOE Patents (OSTI)

The invention is directed to a grid used in x-ray imaging applications to block scattered radiation while allowing the desired imaging radiation to pass through, and to process for making the grid. The grid is composed of glass containing lead oxide, and eliminates the spacer material used in prior known grids, and is therefore, an air-core grid. The glass is arranged in a pattern so that a large fraction of the area is open allowing the imaging radiation to pass through. A small pore size is used and the grid has a thickness chosen to provide high scatter rejection. For example, the grid may be produced with a 200 {micro}m pore size, 80% open area, and 4 mm thickness. 2 figs.

Logan, C.M.; Lane, S.M.

1995-10-03T23:59:59.000Z

34

Air-core grid for scattered x-ray rejection  

DOE Patents (OSTI)

The invention is directed to a grid used in x-ray imaging applications to block scattered radiation while allowing the desired imaging radiation to pass through, and to process for making the grid. The grid is composed of glass containing lead oxide, and eliminates the spacer material used in prior known grids, and is therefore, an air-core grid. The glass is arranged in a pattern so that a large fraction of the area is open allowing the imaging radiation to pass through. A small pore size is used and the grid has a thickness chosen to provide high scatter rejection. For example, the grid may be produced with a 200 .mu.m pore size, 80% open area, and 4 mm thickness.

Logan, Clinton M. (Pleasanton, CA); Lane, Stephen M. (Oakland, CA)

1995-01-01T23:59:59.000Z

35

Large-scale Nanostructure Simulations from X-ray Scattering Data On Graphics Processor Clusters  

E-Print Network (OSTI)

X-ray Scattering Data On Graphics Processor Clusters Abhinavaccelerators. General purpose graphics processors o?er ?nethe form factors on graphics processors. Form Factor Kernel

Sarje, Abhinav

2012-01-01T23:59:59.000Z

36

Anomalous Small-angle Scattering with Soft X-rays at Al and Si K ...  

Science Conference Proceedings (OSTI)

Anomalous Small-angle Scattering with Soft X-rays at Al and Si K Absorption ... and Cooling Cycles in a High Strength Quenched and Tempered Structural Steel.

37

K-alpha conversion efficiency measurments for x-ray scattering in inertial confinement fusion plasmas  

SciTech Connect

The conversion efficiency of ultra short-pulse laser radiation to K-{alpha} x-rays has been measured for various chlorine-containing targets to be used as x-ray scattering probes of dense plasmas. The spectral and temporal properties of these sources will allow spectrally-resolved x-ray scattering probing with picosecond temporal resolution required for measuring the plasma conditions in inertial confinement fusion experiments. Simulations of x-ray scattering spectra from these plasmas show that fuel capsule density, capsule ablator density, and shock timing information may be inferred.

Kritcher, A L; Neumayer, P; Urry, M K; Robey, H; Niemann, C; Landen, O L; Morse, E; Glenzer, S H

2006-11-21T23:59:59.000Z

38

Materials Small-angle X-ray Scattering (SAXS) | Stanford Synchrotron  

NLE Websites -- All DOE Office Websites (Extended Search)

Materials Small-angle X-ray Scattering (SAXS) Materials Small-angle X-ray Scattering (SAXS) Small Angle X-ray Scattering for Materials Science Small-angle X-ray scattering (SAXS) is a well-established characterization method for microstructure investigations in various materials. It probes electron density differences to give information about structural inhomogeneities from the near atomic scale (1 nm) to the micron scale (1 000 nm). The method involves measuring the scattered X-ray intensity as a function of (typically small) scattering angles and is generally performed in transmission. SAXS is used to characterize the size scale of inhomogeneities (e.g. pores, inclusions, second phase regions) in polymer blends, micro-emulsions, geological materials, bones, cements and ceramics. Instrumentation

39

Neutron and X-ray Scattering Investigations of Microscopic Energy ...  

Science Conference Proceedings (OSTI)

A Case Study in Future Energy Challenges: Towards In Situ Hard X-ray Microscopy of ... of Crystal Structure and Domain Character in Lead Free Piezoceramics.

40

Staff at sector 30, inelastic x-ray scattering  

NLE Websites -- All DOE Office Websites (Extended Search)

Status and Schedule Safety and Training Divisions APS Engineering Support Division AES Groups Accelerator Systems Division ASD Groups X-ray Science Division XSD Groups...

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


41

Direct and bulk-scattered forward-shock emissions: sources of X-ray afterglow diversity  

E-Print Network (OSTI)

I describe the modifications to the standard forward-shock model required to account for the X-ray light-curve features discovered by Swift in the early afterglow emission and propose that a delayed, pair-enriched, and highly relativistic outflow, which bulk-scatters the forward-shock synchrotron emission, yields sometimes a brighter X-ray emission, producing short-lived X-ray flares, X-ray light-curve plateaus ending with chromatic breaks, and fast post-plateau X-ray decays.

A. Panaitescu

2008-02-09T23:59:59.000Z

42

The Role of Surface X-ray Scattering in Electrocatalysis  

NLE Websites -- All DOE Office Websites (Extended Search)

3 3 N. M. Markovi , LBNL and C. A. Lucas, University of Liverpool Ecological and political realities have moved discussions of, and advances in, fuel cell technology into mainstream public awareness. Electrocatalysis, the science of modifying the overall rates of electrochemical reactions so that selectivity, yield and efficiency are maximized, is the work from which those advances spring. Studies in electrocatalysis have resulted in highly selective multicomponent gas mixture sensors, human blood component sensors, new electrocatalysts for oxidation/reduction of inorganic and organic pollutants in air and water, as well as better electrocatalysts for the fuel cell conversion of renewable and fossil fuels to electrical work. Studies of the mechanisms by which these catalysts operate have been advanced through development of in-situ surface x-ray scattering (SXS) techniques. SXS capabilities at SSRL were recently used to investigate the interface structure of an ultrathin COad (adsorbed carbon monoxide) overlayer on platinum. This work has elevated the macroscopic description of the COad state at the solid-liquid interface to a microscopic level and enabled the relation between the reactivity and the interfacial structure of COad/Pt to be understood.

43

Synchrotron X-ray Scattering Analysis of the Interaction Between Corn Starch and an Exogenous Lipid During Hydrothermal Treatment  

Science Conference Proceedings (OSTI)

Lipids have an important effect on starch physicochemical properties. There exist few reports about the effect of exogenous lipids on native corn starch structural properties. In this work, a study of the morphological, structural and thermal properties of native corn starch with L-alpha-lysophosphatidylcholine (LPC, the main phospholipid in corn) was performed under an excess of water. Synchrotron radiation, in the form of real-time small and wide-angle X-ray scattering (SAXS/WAXS), was used in order to track structural changes in corn starch, in the presence of LPC during a heating process from 30 to 85 C. When adding LCP, water absorption decreased within starch granule amorphous regions during gelatinization. This is explained by crystallization of the amylose-LPC inclusion complex during gelatinization, which promotes starch granule thermal stability at up to 95 C. Finally, a conceptual model is proposed for explaining the formation mechanism of the starch-LPC complex.

E Hernandez-Hernandez; C Avila-Orta; B Hsiao; j Castro-Rosas; J Gallegos-Infante; J Morales-Castro; L Ochoa-Martinez; C Gomez-Aldapa

2011-12-31T23:59:59.000Z

44

Magnetism studies using resonant, coherent, x-ray scattering...  

NLE Websites -- All DOE Office Websites (Extended Search)

10:00am SLAC, Bldg. 137, Room 226 Keoki Seu Seminar: With the advent of free electron lasers there has been interest in using coherent x-rays to probe condensed matter systems....

45

X-Ray Scattering Group, Condensed Matter Physics & Materials...  

NLE Websites -- All DOE Office Websites (Extended Search)

Ocko, B.M., Wen, K., Maoz, R., Cohen, H., and Sagiv, J. Non-destructive chemical modification of a preassembled silane multilayer: structural study by combined FTIR, x-ray...

46

Photon Sciences | Beamlines | CSX: Coherent Soft X-ray Scattering and  

NLE Websites -- All DOE Office Websites (Extended Search)

CSX: Coherent Soft X-ray Scattering and polarization CSX: Coherent Soft X-ray Scattering and polarization X-Ray 1 Poster | X-Ray 2 Poster | Fact Sheet | Preliminary Design Report Scientific Scope The Coherent Soft X-ray Scattering and Polarization (CSX) beamline design (source and optics) has been optimized to the NSLS-II parameters to provide the highest possible flux for experiments requiring either high coherence or full control of the polarization. Beamline Description The CSX beamline will be served by two identical EPU49 sources. Both EPUs are planned to operate in a canted geometry with opposite circular polarization for fast polarization switching experiments at the full polarization control (PC) branch. The EPUs will also be able to operate "phased" as a single device for high coherent flux experiments at the

47

X Ray Scattering | U.S. DOE Office of Science (SC)  

Office of Science (SC) Website

X Ray Scattering X Ray Scattering Materials Sciences and Engineering (MSE) Division MSE Home About Research Areas Energy Frontier Research Centers (EFRCs) DOE Energy Innovation Hubs BES Funding Opportunities The Computational Materials and Chemical Sciences Network (CMCSN) Theoretical Condensed Matter Physics Scientific Highlights Reports and Activities Principal Investigators' Meetings BES Home Research Areas X Ray Scattering Print Text Size: A A A RSS Feeds FeedbackShare Page This activity supports basic research on the fundamental interactions of photons with matter to achieve an understanding of atomic, electronic, and magnetic structures and excitations and their relationships to materials properties. The main emphasis is on x-ray scattering, spectroscopy, and imaging research, primarily at major BES-supported user facilities.

48

Resonant Soft X-Ray Scattering of Tri-Block Copolymers  

NLE Websites -- All DOE Office Websites (Extended Search)

previous experiments have been few. Now, an international team from the United States, Korea, and Japan has succeeded in combining resonant soft x-ray scattering (RSoXS) at ALS...

49

Electrochemical in-situ reaction cell for X-ray scattering, diffraction and spectroscopy  

DOE Green Energy (OSTI)

An electrochemical in-situ reaction cell for hard X-ray experiments with battery electrodes is described. Applications include the small angle scattering, diffraction, and near-edge spectroscopy of lithium manganese oxide electrodes.

Braun, Artur; Granlund, Eric; Cairns, Elton J.

2003-01-27T23:59:59.000Z

50

Entangled valence electron-hole dynamics revealed by stimulated attosecond x-ray Raman scattering  

SciTech Connect

We show that broadband x-ray pulses can create wavepackets of valence electrons and holes localized in the vicinity of a selected atom (nitrogen, oxygen or sulfur in cysteine) by resonant stimulated Raman scattering. The subsequent dynamics reveals highly correlated motions of entangled electrons and hole quasiparticles. This information goes beyond the time-dependent total charge density derived from x-ray diffraction.

Healion, Daniel; Zhang, Yu; Biggs, Jason D.; Govind, Niranjan; Mukamel, Shaul

2012-09-06T23:59:59.000Z

51

THE HARD X-RAY SPECTRUM OF NGC 1365: SCATTERED LIGHT, NOT BLACK HOLE SPIN  

SciTech Connect

Active galactic nuclei (AGNs) show excess X-ray emission above 10 keV compared with extrapolation of spectra from lower energies. Risaliti et al. have recently attempted to model the hard X-ray excess in the type 1.8 AGN NGC 1365, concluding that the hard excess most likely arises from Compton-scattered reflection of X-rays from an inner accretion disk close to the black hole. Their analysis disfavored a model in which the hard excess arises from a high column density of circumnuclear gas partially covering a primary X-ray source, despite such components being required in the NGC 1365 data below 10 keV. Using a Monte Carlo radiative transfer approach, we demonstrate that this conclusion is invalidated by (1) use of slab absorption models, which have unrealistic transmission spectra for partial covering gas, (2) neglect of the effect of Compton scattering on transmitted spectra, and (3) inadequate modeling of the spectrum of scattered X-rays. The scattered spectrum is geometry-dependent and, for high global covering factors, may dominate above 10 keV. We further show that, in models of circumnuclear gas, the suppression of the observed hard X-ray flux by reprocessing may be no larger than required by the ''light bending'' model invoked for inner disk reflection, and the expected emission line strengths lie within the observed range. We conclude that the time-invariant ''red wing'' in AGN X-ray spectra is probably caused by continuum transmitted through and scattered from circumnuclear gas, not by highly redshifted line emission, and that measurement of black hole spin is not possible.

Miller, L. [Department of Physics, Oxford University, Denys Wilkinson Building, Keble Road, Oxford OX1 3RH (United Kingdom); Turner, T. J. [Department of Physics, University of Maryland Baltimore County, Baltimore, MD 21250 (United States)

2013-08-10T23:59:59.000Z

52

Educational Programs - National School on Neutron & X-ray Scattering  

NLE Websites -- All DOE Office Websites (Extended Search)

and national laboratories, will include basic tutorials on the principles of scattering theory and the characteristics of the sources, as well as seminars on the application of...

53

X-ray Thomson scattering for partially ionized plasmas including the effect of bound levels  

E-Print Network (OSTI)

X-ray Thomson scattering is being developed as a method to measure the temperature, electron density, and ionization state of high energy density plasmas such as those used in inertial confinement fusion. Most experiments are currently done at large laser facilities that can create bright X-ray sources, however the advent of the X-ray free electron laser (X-FEL) provides a new bright source to use in these experiments. One challenge with X-ray Thomson scattering experiments is understanding how to model the scattering for partially ionized plasmas in order to include the contributions of the bound electrons in the scattered intensity. In this work we take the existing models of Thomson scattering that include elastic ion-ion scattering and the electron-electron plasmon scattering and add the contribution of the bound electrons in the partially ionized plasmas. We validated our model by analyzing existing beryllium experimental data. We then consider several higher Z materials such as Cr and predict the existe...

Nilsen, J; Cheng, K T

2013-01-01T23:59:59.000Z

54

SOFT INELASTIC X-RAY SCATTERING (SIX) Group Leader: Ignace Jarrige  

NLE Websites -- All DOE Office Websites (Extended Search)

INELASTIC X-RAY SCATTERING (SIX) INELASTIC X-RAY SCATTERING (SIX) Group Leader: Ignace Jarrige 1 Proposal Team: D. Arena 1 , A. Baron 2 , Y. Cai 1 , Y.-D. Chuang 3 , F. de Groot 4 , J. Guo 3 , J.P. Hill 1 , S. Hulbert 1 , C. McGuinness 5 , R. Reininger 9 , J.E. Rubenson 6 , C. Sanchez-Hanke 1 , T. Schmitt 7 , K. Smith 8 1 Brookhaven National Laboratory, 2 SPring-8, 3 Lawrence Berkeley Laboratory, 4 Utrecht University, 5 Trinity College Dublin, 6 Uppsala University, 7 Paul Scherrer Institute, 8 Boston University, 9 Argonne National Laboratory TECHNIQUE AND CAPABILITIES APPLICATIONS ADDITIONAL INFORMATION * Resonant inelastic x-ray scattering (RIXS) at unprecedented resolution (10 meV @ 1000 eV) to revolutionize study of low energy excitations in many important materials. * Continuously tunable momentum transfer (q) to study the

55

SSRL School 2007 on Hard X-ray Scattering Techniques in MES  

NLE Websites -- All DOE Office Websites (Extended Search)

May 15-17, 2007 SSRL School on Hard X-ray Scattering Techniques in Materials and Environmental Sciences Group photo taken at the SSRL School on Hard X-ray Scattering Techniques in Materials and Environmental Sciences. A large, printable version of this group image is available via clicking on the image. Overview: Modern synchrotron-based X-ray scattering (SR-XRS) techniques offer the ability to probe nano- and atomic-scale structures and order/disorder relationships that critically govern the properties of advanced technological and environmental materials. The high collimation, intensity, and tunability of SR allow the investigation of a wide range of materials, including thin films and interfaces, nanoparticles, amorphous materials, solutions, hydrated and disordered bacteriogenic minerals,

56

Electronic Structure Measurement of Solid Density Plasmas using X-Ray Scattering  

DOE Green Energy (OSTI)

We present an improved analytical expression for the x-ray dynamic structure factor from a dense plasma which includes the effects of weakly bound electrons. This result can be applied to describe scattering from low to moderate Z plasmas, and it covers the entire range of plasma conditions that can be found in inertial confinement fusion experiments, from ideal to degenerate up to moderately coupled systems. We use our theory to interpret x-ray scattering experiments from solid density carbon plasma and to extract accurate measurements of electron temperature, electron density and charge state. We use our experimental results to validate various equation-of-state models for carbon plasmas.

Gregori, G; Glenzer, S H; Rogers, F J; Landen, O L; Blancard, C; Faussurier, G; Renaudin, P; Kuhlbrodt, S; Redmer, R

2003-08-23T23:59:59.000Z

57

Investigation of the Electronic Structure of Solid Density Plasmas by X-Ray Scattering  

DOE Green Energy (OSTI)

We present an improved analytical expression for the x-ray dynamic structure factor from a dense plasma which includes the effects of weakly bound electrons. This result can be applied to describe scattering from low to moderate Z plasmas, and it covers the entire range of plasma conditions that can be found in inertial confinement fusion experiments, from ideal to degenerate up to moderately coupled systems. We use our theory to interpret x-ray scattering experiments from solid density carbon plasma and to extract accurate measurements of electron temperature, electron density and charge state. We use our experimental results to validate various equation-of-state models for carbon plasmas.

Gregori, G; Glenzer, S H; Forest, F J; Kuhlbrodt, S; Redmer, R; Faussurier, G; Blancard, C; Renaudin, P; Landen, O L

2003-05-19T23:59:59.000Z

58

Observations of non-collective x-ray scattering in warm dense carbon plasma  

Science Conference Proceedings (OSTI)

An experiment for observing the spectrally resolved non-collective x-ray scattering in warm dense carbon plasma is presented in this paper. The experiment used Ta M-band x-rays to heat a foamed carbon cylinder sample isochorically and measured the scattering spectrum with a HOPG crystal spectrometer. The spectrum was compared with the calculation results using a Born-Mermin-approximation model. The best fitting was found at an electron temperature of T{sub e}=34 eV and an electron density of n{sub e}=1.6 Multiplication-Sign 10{sup 23}cm{sup -3}.

Bao Lihua [Research Center of Laser Fusion, China Academy of Engineering Physics, P. O. Box 919-981, Mianyang 621900 (China); Department of Engineering Physics, Tsinghua University, Beijing 100084 (China); Zhang Jiyan; Zhao Yang; Ding Yongkun [Research Center of Laser Fusion, China Academy of Engineering Physics, P. O. Box 919-981, Mianyang 621900 (China); Zhang Xiaoding [Research Center of Laser Fusion, China Academy of Engineering Physics, P. O. Box 919-981, Mianyang 621900 (China); University of Science and Technology of China, Hefei 230026 (China)

2012-12-15T23:59:59.000Z

59

High energy resolution inelastic x-ray scattering at the SRI-CAT  

SciTech Connect

This report is a combination of vugraphs and two papers. The vugraphs give information on the beamline at the APS for IXS and the science addressable by IXS. They also cover the 10 milli-eV resolution spectrometer and the 200 milli-eV resolution spectrometer. The first paper covers the performance of the focusing Ge(444) backscattering analyzers for the inelastic x-ray scattering. The second paper discusses inelastic x-ray scattering from TiC and Ti single crystals.

Macrander, A.T.

1996-08-01T23:59:59.000Z

60

X-ray Scattering Reveals Unusual Growth of Lead on Silicon  

NLE Websites -- All DOE Office Websites (Extended Search)

X-ray Scattering Reveals Unusual Growth of Lead on Silicon X-ray Scattering Reveals Unusual Growth of Lead on Silicon Most thin films grow on substrates in only three ways: layer by layer, formation of atomic islands, or layers followed by islands. The particular growth mode that a given material will follow crucially depends on the relative magnitudes of the surface energy of the film versus the interfacial energy of the film on the substrate. Recently, a team of researchers from the University of Illinois, Academica Sinica in Taiwan, Georgia Tech, and the City University of Hong Kong has discovered a remarkable anomaly. By means of real-time x-ray scattering measurements, the researchers found that lead films grown on silicon adopt a completely novel pattern of growth. X-ray diffraction images taken with a CCD camera during growth of Pb films on Si(111). The interference fringes yield information about island height and layer thickness. Fig. 1. X-ray diffraction images taken with a CCD camera during growth of Pb films on Si(111). The interference fringes yield information about island height and layer thickness.

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61

2011 U.S. National School on Neutron and X-ray Scattering  

Science Conference Proceedings (OSTI)

The 13th annual U.S. National School on Neutron and X-ray Scattering was held June 11 to 25, 2011, at both Oak Ridge and Argonne National Laboratories. This school brought together 65 early career graduate students from 56 different universities in the US and provided them with a broad introduction to the techniques available at the major large-scale neutron and synchrotron x-ray facilities. This school is focused primarily on techniques relevant to the physical sciences, but also touches on cross-disciplinary bio-related scattering measurements. During the school, students received lectures by over 30 researchers from academia, industry, and national laboratories and participated in a number of short demonstration experiments at Argonne's Advanced Photon Source (APS) and Oak Ridge's Spallation neutron Source (SNS) and High Flux Isotope Reactor (HFIR) facilities to get hands-on experience in using neutron and synchrotron sources. The first week of this year's school was held at Oak Ridge National Lab, where Lab director Thom Mason welcomed the students and provided a shitorical perspective of the neutron and x-ray facilities both at Oak Ridge and Argonne. The first few days of the school were dedicated to lectures laying out the basics of scattering theory and the differences and complementarity between the neutron and x-ray probes given by Sunil Sinha. Jack Carpenter provided an introduction into how neutrons are generated and detected. After this basic introduction, the students received lectures each morning on specific techniques and conducted demonstration experiments each afternoon on one of 15 different instruments at either the SNS or HFIR. Some of the topics covered during this week of the school included inelastic neutron scattering by Bruce Gaulin, x-ray and neutron reflectivity by Chuck Majkrazak, small-angle scattering by Volker Urban, powder diffraction by Ashfia Huq and diffuse scattering by Gene Ice.

Lang, Jonathan [Argonne National Laboratory (ANL); te Vethuis, Suzanne [Argonne National Laboratory (ANL); Ekkebus, Allen E [ORNL; Chakoumakos, Bryan C [ORNL; Budai, John D [ORNL

2012-01-01T23:59:59.000Z

62

Uv Thomson scattering from x-ray laser plasmas  

SciTech Connect

Plasmas produced by irradiating massive carbon targets with a 1.064 {mu}m, 1.5 ns laser pulse at incident energies of {approximately}100 J have been investigated. UV thermal Thomson scattering was used to obtain the electron and ion temperatures, as well as drift velocities. The electron density was obtained by optical interferometry. The results are compared to hydrodynamic computer modeling. 6 refs., 6 figs.

La Fontaine, B.; Baldis, H.A.; Villeneuve, D.M.; Bernard, J.E.; Enright, G.D. (National Research Council of Canada, Ottawa, ON (Canada)); Rosen, M.D.; Young, P.E.; Matthews, D.L. (Lawrence Livermore National Lab., CA (USA))

1991-01-03T23:59:59.000Z

63

Resonant Soft X-Ray Scattering of Tri-Block Copolymers  

NLE Websites -- All DOE Office Websites (Extended Search)

Resonant Soft X-Ray Scattering Resonant Soft X-Ray Scattering of Tri-Block Copolymers Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print Wednesday, 30 May 2012 00:00 In principle, tri-block copolymers (tri-BCPs), consisting of three chemically distinct polymers covalently joined together at the ends of each polymer chain, can serve as scaffolds and templates for fabricating a vast number of nanostructures. While quantitatively understanding the details of the morphology and the manner in which the different blocks interact with surfaces and interfaces is critical to success, previous experiments have been few. Now, an international team from the United States, Korea, and Japan has succeeded in combining resonant soft x-ray scattering (RSoXS) at ALS Beamline 11.0.1 with transmission electron microscopy tomography (TEMT) and other techniques to unambiguously determine morphologies comprising two nested hexagonally packed arrays of nanoscopic, cylindrical microdomains in the bulk and a core-shell nanostructure in a thin film. Not only has this work revealed a new phase of ABC tri-block copolymer with complicated morphology, it has illustrated the importance of RSoXS as a unique, powerful tool for examining complex, multi-component systems that could not be characterized with conventional methods.

64

Determination of phonon dispersion relations by X-ray thermal diffuse scattering  

SciTech Connect

Thermal diffuse scattering (TDS) of X-rays from crystals contains information on phonons. This paper reviews the general theory of TDS and some recent experiments aimed at further developing TDS into a useful and efficient method for studying phonon dispersion relations.

Xu, R.; Chiang, T.-C. (UIUC)

2010-07-20T23:59:59.000Z

65

Soft X-Ray Thomson Scattering in Warm Dense Hydrogen at FLASH  

DOE Green Energy (OSTI)

We present collective Thomson scattering with soft x-ray free electron laser radiation as a method to track the evolution of warm dense matter plasmas with {approx}200 fs time resolution. In a pump-probe scheme an 800 nm laser heats a 20 {micro}m hydrogen droplet to the plasma state. After a variable time delay in the order of ps the plasma is probed by an x-ray ultra violet (XUV) pulse which scatters from the target and is recorded spectrally. Alternatively, in a self-Thomson scattering experiment, a single XUV pulse heats the target while a portion of its photons are being scattered probing the target. From such inelastic x-ray scattering spectra free electron temperature and density can be inferred giving insight on relaxation time scales in plasmas as well as the equation of state. We prove the feasibility of this method in the XUV range utilizing the free electron laser facility in Hamburg, FLASH. We recorded Thomson scattering spectra for hydrogen plasma, both in the self-scattering and in the pump-probe mode using optical laser heating.

Faustlin, R R; Toleikis, S; Bornath, T; Doppner, T; Dusterer, S; Forster, E; Fortmann, C; Glenzer, S H; Gode, S; Gregori, G; Irsig, R; Laarmann, T; Lee, H J; Li, B; Meiwes-Broer, K; Mithen, J; Przystawik, A; Redlin, H; Redmer, R; Reinholz, H; Ropke, G; Tavella, F; Thiele, R; Tiggesbaumker, J; Uschmann, I; Zastrau, U; Tschentscher, T

2009-07-15T23:59:59.000Z

66

Electrochemically adsorbed Pb on Ag (111) studied with grazing- incidence x-ray scattering  

SciTech Connect

Grazing-incidence x-ray scattering studies of the evolution of electrochemically deposited layers of lead on silver (111) as a function of applied electrochemical potential are presented. Measurements were made with the adsorbed layers in contact with solution in a specially designed sample cell. The observed lead structures are a function of the applied potential and range from an incommensurate monolayer, resulting from underpotential deposition, to randomly oriented polycrystalline bulk lead, resulting from lower deposition potentials. These early experiments demonstrate the ability of in situ x-ray diffraction measurements to determine structures associated with electrochemical deposition. 6 refs., 4 figs.

Kortright, J.B.; Ross, P.N.; Melroy, O.R.; Toney, M.F.; Borges, G.L.; Samant, M.G.

1989-04-01T23:59:59.000Z

67

Soft x-ray scattering using FEL radiation for probing near-solid density plasmas at few electronvolt temperatures  

DOE Green Energy (OSTI)

We report on soft x-ray scattering experiments on cryogenic hydrogen and simple metal targets. As a source of intense and ultrashort soft x-ray pulses we have used free-electron laser radiation at 92 eV photon energy from FLASH at DESY, Hamburg. X-ray pulses with energies up to 100 {micro}J and durations below 50 fs provide interaction with the target leading simultaneously to plasma formation and scattering. Experiments exploiting both of these interactions have been carried out, using the same experimental setup. Firstly, recording of soft x-ray inelastic scattering from near-solid density hydrogen plasmas at few electronvolt temperatures confirms the feasibility of this diagnostics technique. Secondly, the soft x-ray excitation of few electronvolt solid-density plasmas in simple metals could be studied by recording soft x-ray line and continuum emission integrated over emission times from fs to ns.

Toleikis, S; Faustlin, R R; Cao, L; Doppner, T; Dusterer, S; Forster, E; Fortmann, C; Glenzer, S H; Gode, S; Gregori, G; Irsig, R; Laarmann, T; Lee, H J; Li, B; Meiwes-Broer, K; Przystawik, A; Radcliffe, P; Redmer, R; Tavella, F; Thiele, R; Tiggesbaumker, J; Truong, N X; Uschmann, I; Zastrau, U; Tschentscher, T

2009-03-03T23:59:59.000Z

68

Theme Article - Time-Resolved X-Ray Scattering from Coherent Excitations in Solids  

SciTech Connect

Recent advances in pulsed x-ray sources have opened up new opportunities to study the dynamics of matter directly in the time domain with picosecond to femtosecond resolution. In this article, we present recent results from a variety of ultrafast sources on time-resolved x-ray scattering from elementary excitations in periodic solids. A few representative examples are given on folded acoustic phonons, coherent optical phonons, squeezed phonons, and polaritons excited by femtosecond lasers. Next-generation light sources, such as the x-ray-free electron laser, will lead to improvements in coherence, flux, and pulse duration. These experiments demonstrate potential opportunities for studying matter far from equilibrium on the fastest time scales and shortest distances that will be available in the coming years.

Trigo, Mariano; Reis, David (SLAC)

2010-10-22T23:59:59.000Z

69

Theoretical Model and Interpretation of Dense Plasma X-Ray Thomson Scattering  

Science Conference Proceedings (OSTI)

The authors present analytical expressions for the dynamic structure factor, or form factor S(k,{omega}), which is the quantity describing the inelastic x-ray cross section from a dense plasma or a simple liquid. The results, based on the random phase approximation (RPA) for the treatment on the charged particle coupling, can be applied to describe scattering from either weakly coupled classical plasmas or degenerate electron liquids. The form factor correctly reproduces the Compton energy downshift and the usual Fermi-Dirac electron velocity distribution for S(k,{omega}) in the case of a cold degenerate plasma. the usual concept of scattering parameter is also reinterpreted for the degenerate case in order to include the effect of the Thomas-Fermi screening. The results shown in this work can be applied to interpreting x-ray scattering in warm dense plasmas occurring in inertial confinement fusion experiments or inside the interior of planets.

Gregori, G; Landen, O; Hicks, D; Pasley, J; Collins, G; Celliers, P; Bastea, M; Glenzer, S

2002-04-03T23:59:59.000Z

70

BIOISIS: Biological Macromolecules by Small Angle X-ray Scattering (SAXS)  

DOE Data Explorer (OSTI)

BIOISIS is an open access database dedicated to the study of biological macromolecules by small angle X-ray scattering (SAXS). BIOISIS aims to become the complete source for the deposition, distribution and maintenance of small angle X-ray scattering data and technologies. The database is designed around the concept of an ôexperimentö and relates a specific experiment to a set of genes, organisms, computational models and experimental data. As of May 2012, BIOSIS contains 7,118 genes covering four different organisms. Forty-two modeled structures are available. Clicking on a structures reveals scattering curves, experimental conditions, and experimental values. The data are collected at Beamline 12.3.1 of the Advanced Light Source (ALS).[Copied with editing from http://www.bioisis.net/about

Tainer, John (Scripps Research Institute); Hura, Greg (LBNL); Rambo, Robert P. (LBNL)

71

X-ray Thomson scattering measurements from shock-compressed deuterium  

Science Conference Proceedings (OSTI)

X-ray Thomson scattering has recently been shown to be an effective method of diagnosing a variety of high energy density plasma conditions. We apply this powerful technique to the widely studied problem of shock-compressed liquid deuterium. The behavior of deuterium under extreme conditions has received considerable attention due to its central role in models of giant planets and the importance of the high-pressure insulator-metal transition. We have used spectrally resolved x-ray scattering from electron-plasma waves to perform microscopic observations of ionization during compression. In these experiments, a single shock was launched in cryogenic deuterium reaching compressions of 3x. The 2 keV Ly-{alpha} line in silicon was used as an x-ray source in a forward scattering geometry. In addition to elastic scattering from tightly bound electrons, this low probe energy accessed the collective plasmon oscillations of delocalized electrons. Inelastic scattering from the plasmons allowed accurate measurements of the free electron density through the spectral position of the resonance and provided an estimate of the temperature through its ratio with the elastic feature. Combined with velocity interferometry from the reflective shock front, this lead to a direct determination of the ionization state. We compare the measured ionization conditions with computational models. Additionally, we discuss the possibility of using this technique to determine electrical conductivity and to directly observe pressure-induced molecular dissociation along the Hugoniot.

Davis, P.; Doeppner, T.; Rygg, J. R.; Fortmann, C.; Unites, W.; Salmonson, J.; Collins, G. W.; Landen, O. L.; Falcone, R. W.; Glenzer, S. H. [University of California, Berkeley. Berkeley, CA, 94720 (United States); Lawrence Livermore National Laboratory. Livermore, CA 94551 (United States); University of California, Berkeley. Berkeley, CA, 94720 (United States)

2012-05-25T23:59:59.000Z

72

Large-scale Nanostructure Simulations from X-ray Scattering Data On Graphics Processor Clusters  

Science Conference Proceedings (OSTI)

X-ray scattering is a valuable tool for measuring the structural properties of materialsused in the design and fabrication of energy-relevant nanodevices (e.g., photovoltaic, energy storage, battery, fuel, and carbon capture andsequestration devices) that are key to the reduction of carbon emissions. Although today's ultra-fast X-ray scattering detectors can provide tremendousinformation on the structural properties of materials, a primary challenge remains in the analyses of the resulting data. We are developing novelhigh-performance computing algorithms, codes, and software tools for the analyses of X-ray scattering data. In this paper we describe two such HPCalgorithm advances. Firstly, we have implemented a flexible and highly efficient Grazing Incidence Small Angle Scattering (GISAXS) simulation code based on theDistorted Wave Born Approximation (DWBA) theory with C++/CUDA/MPI on a cluster of GPUs. Our code can compute the scattered light intensity from any givensample in all directions of space; thus allowing full construction of the GISAXS pattern. Preliminary tests on a single GPU show speedups over 125x compared tothe sequential code, and almost linear speedup when executing across a GPU cluster with 42 nodes, resulting in an additional 40x speedup compared to usingone GPU node. Secondly, for the structural fitting problems in inverse modeling, we have implemented a Reverse Monte Carlo simulation algorithm with C++/CUDAusing one GPU. Since there are large numbers of parameters for fitting in the in X-ray scattering simulation model, the earlier single CPU code required weeks ofruntime. Deploying the AccelerEyes Jacket/Matlab wrapper to use GPU gave around 100x speedup over the pure CPU code. Our further C++/CUDA optimization deliveredan additional 9x speedup.

Sarje, Abhinav; Pien, Jack; Li, Xiaoye; Chan, Elaine; Chourou, Slim; Hexemer, Alexander; Scholz, Arthur; Kramer, Edward

2012-01-15T23:59:59.000Z

73

Resonant Soft X-Ray Scattering of Tri-Block Copolymers  

NLE Websites -- All DOE Office Websites (Extended Search)

Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print In principle, tri-block copolymers (tri-BCPs), consisting of three chemically distinct polymers covalently joined together at the ends of each polymer chain, can serve as scaffolds and templates for fabricating a vast number of nanostructures. While quantitatively understanding the details of the morphology and the manner in which the different blocks interact with surfaces and interfaces is critical to success, previous experiments have been few. Now, an international team from the United States, Korea, and Japan has succeeded in combining resonant soft x-ray scattering (RSoXS) at ALS Beamline 11.0.1 with transmission electron microscopy tomography (TEMT) and other techniques to unambiguously determine morphologies comprising two nested hexagonally packed arrays of nanoscopic, cylindrical microdomains in the bulk and a core-shell nanostructure in a thin film. Not only has this work revealed a new phase of ABC tri-block copolymer with complicated morphology, it has illustrated the importance of RSoXS as a unique, powerful tool for examining complex, multi-component systems that could not be characterized with conventional methods.

74

Resonant Soft X-Ray Scattering of Tri-Block Copolymers  

NLE Websites -- All DOE Office Websites (Extended Search)

Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print In principle, tri-block copolymers (tri-BCPs), consisting of three chemically distinct polymers covalently joined together at the ends of each polymer chain, can serve as scaffolds and templates for fabricating a vast number of nanostructures. While quantitatively understanding the details of the morphology and the manner in which the different blocks interact with surfaces and interfaces is critical to success, previous experiments have been few. Now, an international team from the United States, Korea, and Japan has succeeded in combining resonant soft x-ray scattering (RSoXS) at ALS Beamline 11.0.1 with transmission electron microscopy tomography (TEMT) and other techniques to unambiguously determine morphologies comprising two nested hexagonally packed arrays of nanoscopic, cylindrical microdomains in the bulk and a core-shell nanostructure in a thin film. Not only has this work revealed a new phase of ABC tri-block copolymer with complicated morphology, it has illustrated the importance of RSoXS as a unique, powerful tool for examining complex, multi-component systems that could not be characterized with conventional methods.

75

Resonant Soft X-Ray Scattering of Tri-Block Copolymers  

NLE Websites -- All DOE Office Websites (Extended Search)

Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print In principle, tri-block copolymers (tri-BCPs), consisting of three chemically distinct polymers covalently joined together at the ends of each polymer chain, can serve as scaffolds and templates for fabricating a vast number of nanostructures. While quantitatively understanding the details of the morphology and the manner in which the different blocks interact with surfaces and interfaces is critical to success, previous experiments have been few. Now, an international team from the United States, Korea, and Japan has succeeded in combining resonant soft x-ray scattering (RSoXS) at ALS Beamline 11.0.1 with transmission electron microscopy tomography (TEMT) and other techniques to unambiguously determine morphologies comprising two nested hexagonally packed arrays of nanoscopic, cylindrical microdomains in the bulk and a core-shell nanostructure in a thin film. Not only has this work revealed a new phase of ABC tri-block copolymer with complicated morphology, it has illustrated the importance of RSoXS as a unique, powerful tool for examining complex, multi-component systems that could not be characterized with conventional methods.

76

Resonant Soft X-Ray Scattering of Tri-Block Copolymers  

NLE Websites -- All DOE Office Websites (Extended Search)

Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print In principle, tri-block copolymers (tri-BCPs), consisting of three chemically distinct polymers covalently joined together at the ends of each polymer chain, can serve as scaffolds and templates for fabricating a vast number of nanostructures. While quantitatively understanding the details of the morphology and the manner in which the different blocks interact with surfaces and interfaces is critical to success, previous experiments have been few. Now, an international team from the United States, Korea, and Japan has succeeded in combining resonant soft x-ray scattering (RSoXS) at ALS Beamline 11.0.1 with transmission electron microscopy tomography (TEMT) and other techniques to unambiguously determine morphologies comprising two nested hexagonally packed arrays of nanoscopic, cylindrical microdomains in the bulk and a core-shell nanostructure in a thin film. Not only has this work revealed a new phase of ABC tri-block copolymer with complicated morphology, it has illustrated the importance of RSoXS as a unique, powerful tool for examining complex, multi-component systems that could not be characterized with conventional methods.

77

Resonant Soft X-Ray Scattering of Tri-Block Copolymers  

NLE Websites -- All DOE Office Websites (Extended Search)

Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print In principle, tri-block copolymers (tri-BCPs), consisting of three chemically distinct polymers covalently joined together at the ends of each polymer chain, can serve as scaffolds and templates for fabricating a vast number of nanostructures. While quantitatively understanding the details of the morphology and the manner in which the different blocks interact with surfaces and interfaces is critical to success, previous experiments have been few. Now, an international team from the United States, Korea, and Japan has succeeded in combining resonant soft x-ray scattering (RSoXS) at ALS Beamline 11.0.1 with transmission electron microscopy tomography (TEMT) and other techniques to unambiguously determine morphologies comprising two nested hexagonally packed arrays of nanoscopic, cylindrical microdomains in the bulk and a core-shell nanostructure in a thin film. Not only has this work revealed a new phase of ABC tri-block copolymer with complicated morphology, it has illustrated the importance of RSoXS as a unique, powerful tool for examining complex, multi-component systems that could not be characterized with conventional methods.

78

Physica B 283 (2000) 75}78 Phase-sensitive surface X-ray scattering study of a crystalline  

E-Print Network (OSTI)

Physica B 283 (2000) 75}78 Phase-sensitive surface X-ray scattering study of a crystalline organic}organic An X-ray study of a crystalline organic}organic heterostructure, consisting of a "lm of PTCDA (3 the determination of d with great sensitivity. 2000 Elsevier Science B.V. All rights reserved. PACS: 61.66.Hq; 68

Schreiber, Frank

79

A von Hamos x-ray spectrometer based on a segmented-type diffraction crystal for single-shot x-ray emission spectroscopy and time-resolved resonant inelastic x-ray scattering studies  

SciTech Connect

We report on the design and performance of a wavelength-dispersive type spectrometer based on the von Hamos geometry. The spectrometer is equipped with a segmented-type crystal for x-ray diffraction and provides an energy resolution in the order of 0.25 eV and 1 eV over an energy range of 8000 eV-9600 eV. The use of a segmented crystal results in a simple and straightforward crystal preparation that allows to preserve the spectrometer resolution and spectrometer efficiency. Application of the spectrometer for time-resolved resonant inelastic x-ray scattering and single-shot x-ray emission spectroscopy is demonstrated.

Szlachetko, J. [Paul Scherrer Institut, 5232 Villigen PSI (Switzerland); Institute of Physics, Jan Kochanowski University, 25-406 Kielce (Poland); Nachtegaal, M.; Boni, E. de; Willimann, M.; Safonova, O.; Sa, J.; Smolentsev, G.; Szlachetko, M.; Bergamaschi, A.; Schmitt, B.; David, C.; Luecke, A. [Paul Scherrer Institut, 5232 Villigen PSI (Switzerland); Bokhoven, J. A. van [Paul Scherrer Institut, 5232 Villigen PSI (Switzerland); Institute for Chemical and Bioengineering, ETH Zurich, 8093 Zuerich (Switzerland); Dousse, J.-Cl.; Hoszowska, J.; Kayser, Y. [Department of Physics, University of Fribourg, 1700 Fribourg (Switzerland); Jagodzinski, P. [University of Technology, Kielce (Poland)

2012-10-15T23:59:59.000Z

80

K-(alpha) X-ray Thomson Scattering From Dense Plasmas  

SciTech Connect

Spectrally resolved Thomson scattering using ultra-fast K-{alpha} x-rays has measured the compression and heating of shocked compressed matter. The evolution and coalescence of two shock waves traveling through a solid density LiH target were characterized by the elastic scattering component. The density and temperature at shock coalescence, 2.2 eV and 1.7 x 10{sup 23}cm{sup -3}, were determined from the plasmon frequency shift and the relative intensity of the elastic and inelastic scattering features in the collective scattering regime. The observation of plasmon scattering at coalescence indicates a transition to the dense metallic state in LiH. The density and temperature regimes accessed in these experiments are relevant for inertial confinement fusion experiments and for the study of planetary formation.

Kritcher, A L; Neumayer, P; Castor, J; Doppner, T; Falcone, R W; Landen, O L; Lee, H J; Lee, R W; Morse, E C; Ng, A; Pollaine, S; Price, D; Glenzer, S H

2009-05-07T23:59:59.000Z

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
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We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


81

Protein folding and protein metallocluster studies using synchrotron small angler X-ray scattering  

SciTech Connect

Proteins, biological macromolecules composed of amino-acid building blocks, possess unique three dimensional shapes or conformations which are intimately related to their biological function. All of the information necessary to determine this conformation is stored in a protein`s amino acid sequence. The problem of understanding the process by which nature maps protein amino-acid sequences to three-dimensional conformations is known as the protein folding problem, and is one of the central unsolved problems in biophysics today. The possible applications of a solution are broad, ranging from the elucidation of thousands of protein structures to the rational modification and design of protein-based drugs. The scattering of X-rays by matter has long been useful as a tool for the characterization of physical properties of materials, including biological samples. The high photon flux available at synchrotron X-ray sources allows for the measurement of scattering cross-sections of dilute and/or disordered samples. Such measurements do not yield the detailed geometrical information available from crystalline samples, but do allow for lower resolution studies of dynamical processes not observable in the crystalline state. The main focus of the work described here has been the study of the protein folding process using time-resolved small-angle x-ray scattering measurements. The original intention was to observe the decrease in overall size which must accompany the folding of a protein from an extended conformation to its compact native state. Although this process proved too fast for the current time-resolution of the technique, upper bounds were set on the probable compaction times of several small proteins. In addition, an interesting and unexpected process was detected, in which the folding protein passes through an intermediate state which shows a tendency to associate. This state is proposed to be a kinetic molten globule folding intermediate.

Eliezer, D.

1994-06-01T23:59:59.000Z

82

Epp: A C++ EGSnrc user code for x-ray imaging and scattering simulations  

Science Conference Proceedings (OSTI)

Purpose: Easy particle propagation (Epp) is a user code for the EGSnrc code package based on the C++ class library egspp. A main feature of egspp (and Epp) is the ability to use analytical objects to construct simulation geometries. The authors developed Epp to facilitate the simulation of x-ray imaging geometries, especially in the case of scatter studies. While direct use of egspp requires knowledge of C++, Epp requires no programming experience. Methods: Epp's features include calculation of dose deposited in a voxelized phantom and photon propagation to a user-defined imaging plane. Projection images of primary, single Rayleigh scattered, single Compton scattered, and multiple scattered photons may be generated. Epp input files can be nested, allowing for the construction of complex simulation geometries from more basic components. To demonstrate the imaging features of Epp, the authors simulate 38 keV x rays from a point source propagating through a water cylinder 12 cm in diameter, using both analytical and voxelized representations of the cylinder. The simulation generates projection images of primary and scattered photons at a user-defined imaging plane. The authors also simulate dose scoring in the voxelized version of the phantom in both Epp and DOSXYZnrc and examine the accuracy of Epp using the Kawrakow-Fippel test. Results: The results of the imaging simulations with Epp using voxelized and analytical descriptions of the water cylinder agree within 1%. The results of the Kawrakow-Fippel test suggest good agreement between Epp and DOSXYZnrc. Conclusions: Epp provides the user with useful features, including the ability to build complex geometries from simpler ones and the ability to generate images of scattered and primary photons. There is no inherent computational time saving arising from Epp, except for those arising from egspp's ability to use analytical representations of simulation geometries. Epp agrees with DOSXYZnrc in dose calculation, since they are both based on the well-validated standard EGSnrc radiation transport physics model.

Lippuner, Jonas; Elbakri, Idris A.; Cui Congwu; Ingleby, Harry R. [Department of Medical Physics, CancerCare Manitoba, 675 McDermot Avenue, Winnipeg, Manitoba R3E 0V9 (Canada) and Department of Physics and Astronomy, University of Manitoba, Winnipeg, Manitoba R3T 2N2 (Canada); Department of Medical Physics, CancerCare Manitoba, 675 McDermot Avenue, Winnipeg, Manitoba R3E 0V9 (Canada); Department of Physics and Astronomy, University of Manitoba, Winnipeg, Manitoba R3T 2N2 (Canada) and Department of Radiology, University of Manitoba, 820 Sherbrook Street, Winnipeg, Manitoba R3A 1R9 (Canada); Department of Medical Physics, CancerCare Manitoba, 675 McDermot Avenue, Winnipeg, Manitoba R3E 0V9 (Canada)

2011-03-15T23:59:59.000Z

83

Time-Resolved Small-Angle X-ray Scattering Studies Revealed Three Kinetic  

NLE Websites -- All DOE Office Websites (Extended Search)

June 2010 June 2010 Time-Resolved Small-Angle X-ray Scattering Studies Revealed Three Kinetic Stages of a T=4 Virus Maturation Most eukaryotic viruses, including HIV, influenza and herpes viruses, undergo maturation when transitioning from the noninfectious provirion to the infectious virion. Maturation processes involve reorganization of viral quaternary structure to defend viral gene from the cellular defense mechanism and lead to effective transfection. Nudaurelia capensis omega virus, NwV, is a T=4, non-enveloped, icosahedral, single strand RNA virus, where T is the triangulation number defining an icosahedral lattice of the virus capsid structure. Virus like particles (VLPs) of NwV exhibit large pH-dependent conformational changes (LCC) when the procapsid, purified at pH=7.6, (~480 Ã…) is exposed to pH=5.0, resulting in ~400 Ã… particles (Figure 1). In response to the LCC, an auto-proteolysis occurs in which each of 240 subunits is cleaved at Asn570-Phe571 (1). We investigated this pH-induced maturation by equilibrium and time-resolved small angle X-ray scattering (SAXS) at SSRL beam line 4-2.

84

Resonant Soft X-ray Scattering Studies of Multiferroic YMn2O5  

SciTech Connect

We performed soft x-ray resonant scattering at the MnL{sub 2,3}- and OK edges of YMn{sub 2}O{sub 5}. While the resonant intensity at the MnL{sub 2,3} edges represent the magnetic order parameter, the resonant scattering at the OK edge is found to be directly related to the macroscopic ferroelectric polarization. The latter observation reveals the important role of the spin-dependent Mn-O hybridization for the multiferroicity of YMn{sub 2}O{sub 5}. We present details about how to obtain correct energy dependent lineshapes and discuss the origin of the resonant intensity at the OK edge.

Partzsch, S.; Wilkins, S.B.; Schierle, E.; Soltwisch, V.; Hill, J.P.; Weschke, E.; Souptel, D.; Buchner, B.; Geck, J.

2011-06-17T23:59:59.000Z

85

Hydrogen bonding and coordination in normal and supercritical water from X-ray inelastic scattering  

E-Print Network (OSTI)

A direct measure of hydrogen bonding in water under conditions ranging from the normal state to the supercritical regime is derived from the Compton scattering of inelastically-scattered X-rays. First, we show that a measure of the number of electrons $n_e$ involved in hydrogen bonding at varying thermodynamic conditions can be directly obtained from Compton profile differences. Then, we use first-principles simulations to provide a connection between $n_e$ and the number of hydrogen bonds $n_{HB}$. Our study shows that over the broad range studied the relationship between $n_e$ and $n_{HB}$ is linear, allowing for a direct experimental measure of bonding and coordination in water. In particular, the transition to supercritical state is characterized by a sharp increase in the number of water monomers, but also displays a significant number of residual dimers and trimers.

Patrick H. -L. Sit; Christophe Bellin; Bernardo Barbiellini; D. Testemale; J. -L. Hazemann; T. Buslaps; Nicola Marzari; Abhay Shukla

2007-02-26T23:59:59.000Z

86

Defects and Polytypism in SiC: The Role of Diffuse X-Ray Scattering  

Science Conference Proceedings (OSTI)

Stacking faults (SFs) and the 3C-6H polytypic transition in thick (001)-oriented 3C-SiC crystals are studied by means of diffuse X-ray scattering. The presence of SFs lying in the {l_brace}111{r_brace} planes gives rise to streaked reciprocal lattice points with the streaks being parallel to the directions. In the case of low SF densities the defects are uncorrelated and the simulation of the diffuse intensity distribution allows to derive the SF density. In partially transformed crystals, the SFs are spatially correlated which gives rise to an intense and asymmetric diffuse scattering distribution. Its simulation allows to determine both the transformation mechanism and the transformation level.

Boulle, A.; Dompoint, D. [Science des Procedes Ceramiques et de Traitements de surface (SPCTS-CNRS UMR 6638), ENSCI 47 avenue Albert Thomas 87065 Limoges Cedex (France); Galben-Sandulache, I.; Chaussende, D. [Laboratoires des Materiaux et du Genie Physique (LMGP-CNRS UMR 5628), Grenoble INP, Minatec 3 parvis Louis Neel, BP 257, 38016 Grenoble Cedex 01 (France)

2010-11-01T23:59:59.000Z

87

Synchrotron X-ray scattering techniques for microelectronics-related materials studies  

Science Conference Proceedings (OSTI)

X-ray diffraction techniques using synchrotron radiation play a vital role in the understanding of structural behavior for a wide range of materials important in microelectronics. The extremely high flux of X-rays produced by synchrotron storage rings ...

J. L. Jordan-Sweet

2000-07-01T23:59:59.000Z

88

The phonon density of states of {alpha}- {delta}-plutonium by inelastic x-ray scattering.  

Science Conference Proceedings (OSTI)

Inelastic x-ray scattering measurements of the phonon density of states (DOS) were performed on polycrystalline samples of pure {alpha}-Pu and {delta}-Pu{sub 0.98}Ga{sub 0.02} at room temperature. The heat capacity of {alpha}-Pu is well reproduced by contributions calculated from the measured phonon DOS plus conventional thermal-expansion and electronic contributions, showing that {alpha}-Pu is a 'well-behaved' metal in this regard. A comparison of the phonon DOS of the two phases at room temperature showed that the vibrational entropy difference between them is only a quarter of the total entropy difference expected from known thermodynamic measurements. The missing entropy is too large to be accounted for by conventional electronic entropy and evidence from the literature rules out a contribution from spin fluctuations. Possible alternative sources for the missing entropy are discussed.

Manley, M. E.; Said, A.; Fluss, M. J.; Wall, M.; Lashley, J. C.; Alatas, A.; Moore, K. T.; LLNL; LANL

2009-02-01T23:59:59.000Z

89

Robust, high-throughput solution structural analyses by small angle X-ray scattering (SAXS)  

Science Conference Proceedings (OSTI)

We present an efficient pipeline enabling high-throughput analysis of protein structure in solution with small angle X-ray scattering (SAXS). Our SAXS pipeline combines automated sample handling of microliter volumes, temperature and anaerobic control, rapid data collection and data analysis, and couples structural analysis with automated archiving. We subjected 50 representative proteins, mostly from Pyrococcus furiosus, to this pipeline and found that 30 were multimeric structures in solution. SAXS analysis allowed us to distinguish aggregated and unfolded proteins, define global structural parameters and oligomeric states for most samples, identify shapes and similar structures for 25 unknown structures, and determine envelopes for 41 proteins. We believe that high-throughput SAXS is an enabling technology that may change the way that structural genomics research is done.

Hura, Greg L.; Menon, Angeli L.; Hammel, Michal; Rambo, Robert P.; Poole II, Farris L.; Tsutakawa, Susan E.; Jenney Jr, Francis E.; Classen, Scott; Frankel, Kenneth A.; Hopkins, Robert C.; Yang, Sungjae; Scott, Joseph W.; Dillard, Bret D.; Adams, Michael W. W.; Tainer, John A.

2009-07-20T23:59:59.000Z

90

Changes in the Atomic Structure through Glass Transition Observed by X-Ray Scattering  

SciTech Connect

The glass transition involves a minor change in the internal energy, and yet the physical and mechanical properties of a glass change dramatically. In order to determine the evolution of the atomic structure through the glass transition, we employed in-situ synchrotron X-ray scattering measurements as a function of temperature on a model material: Zr-Cu-Al metallic glass. We found that the thermal expansion at the atomic level is smaller than the macroscopic thermal expansion, and significantly increases above the glass transition temperature. The observed changes in the pair-distribution function (PDF) are explained in terms of the fluctuations in the local atomic volume and their change through the glass transition.

Egami, Takeshi [ORNL

2012-01-01T23:59:59.000Z

91

Small angle x-ray scattering studies of carbon anodes used in lithium rechargeable batteries.  

DOE Green Energy (OSTI)

In ANL laboratories, disordered carbons with predictable surface area and porosity properties have been prepared using inorganic templates containing well defined pore sizes. The carbons have been tested in electrochemical cells as anodes in lithium secondary batteries. They deliver high specific capacity and display excellent performance in terms of the number of cycles run. In situ small angle X-ray scattering (SAXS) during electrochemical cycling was carried out at the Advanced Photon Source, at ANL. In order to monitor the carbon electrode structural changes upon cycling, an electrochemical cell was specially designed to allow for the application of electrical current and the collection of SAXS data at the same time. Results show that upon cycling the structure of the carbon remains unchanged, which is desirable in reversible systems.

Sandi, G.; Carrado, K. A.; Winans, R. E.; Seifert, S.; Johnson, C. S.

1999-11-16T23:59:59.000Z

92

Observation of Laser Induced Magnetization Dynamics in Co/Pd Multilayers with Coherent X-ray Scattering  

SciTech Connect

We report on time-resolved coherent x-ray scattering experiments of laser induced magnetization dynamics in Co/Pd multilayers with a high repetition rate optical pump x-ray probe setup. Starting from a multi-domain ground state, the magnetization is uniformly reduced after excitation by an intense 50 fs laser pulse. Using the normalized time correlation, we study the magnetization recovery on a picosecond timescale. The dynamic scattering intensity is separated into an elastic portion at length scales above 65 nm which retains memory of the initial domain magnetization, and a fluctuating portion at smaller length scales corresponding to domain boundary motion during recovery.

Wu, Benny

2012-04-05T23:59:59.000Z

93

Single-shot Time-resolved X-ray Scattering Measurements in ...  

Science Conference Proceedings (OSTI)

We will describe detailed new measurement system and their results. ... Induced and Observed by Interaction with an Intense Femtosecond X-ray Laser Pulse.

94

A setup for resonant inelastic soft x-ray scattering on liquids at free electron laser light sources  

SciTech Connect

We present a flexible and compact experimental setup that combines an in vacuum liquid jet with an x-ray emission spectrometer to enable static and femtosecond time-resolved resonant inelastic soft x-ray scattering (RIXS) measurements from liquids at free electron laser (FEL) light sources. We demonstrate the feasibility of this type of experiments with the measurements performed at the Linac Coherent Light Source FEL facility. At the FEL we observed changes in the RIXS spectra at high peak fluences which currently sets a limit to maximum attainable count rate at FELs. The setup presented here opens up new possibilities to study the structure and dynamics in liquids.

Kunnus, Kristjan; Schreck, Simon; Foehlisch, Alexander [Institute for Methods and Instrumentation for Synchrotron Radiation Research, Helmholtz-Zentrum Berlin GmbH, Albert-Einstein-Strasse 15, 12489 Berlin (Germany); Institut fuer Physik und Astronomie, Universitaet Potsdam, Karl-Liebknecht-Strasse 24/25, 14476 Potsdam (Germany); Rajkovic, Ivan; Quevedo, Wilson; Gruebel, Sebastian; Scholz, Mirko [IFG Structural Dynamics of (Bio)chemical Systems, Max Planck Institute for Biophysical Chemistry, Am Fassberg 11, 37070 Goettingen (Germany); Eckert, Sebastian; Beye, Martin; Suljoti, Edlira; Weniger, Christian; Wernet, Philippe [Institute for Methods and Instrumentation for Synchrotron Radiation Research, Helmholtz-Zentrum Berlin GmbH, Albert-Einstein-Strasse 15, 12489 Berlin (Germany); Kalus, Christian [Abteilung Betrieb Beschleuniger BESSYII, Helmholtz-Zentrum Berlin GmbH, Albert-Einstein-Strasse 15, 12489 Berlin (Germany); Nordlund, Dennis [Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Zhang, Wenkai; Hartsock, Robert W.; Gaffney, Kelly J. [PULSE Institute, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Schlotter, William F.; Turner, Joshua J. [Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Kennedy, Brian [MAX-lab, PO Box 118, 221 00 Lund (Sweden); and others

2012-12-15T23:59:59.000Z

95

Resonant Inelastic X-ray Scattering of Rare-Earth and CopperSystems  

Science Conference Proceedings (OSTI)

Rare earths and copper systems were studied using X-ray absorption spectroscopy (XAS) and resonant inelastic X-ray scattering (RIXS). The use of monochromased synchotron radiation and improved energy resolution for RIXS made possible to obtain valuable information on the electronic structure in 4f, 5f and 3d systems. Experimental results for rare-earths (Ho, Gd, Cm, U, Np, Pu) were analyzed by atomic multiplet theory based on the Hartree-Fock calculations. The inelastic scattering structures in RIXS spectra at 5d edge of actinides found to be sensitive to actinide oxidation states in different systems. Comparison of experimental and calculated Cm 5d RIXS spectra gave direct information about valency of the 248-curium isotope in oxide. Scientific understanding of processes that control chemical changes of radioactive species from spent fuel is improved by studying interactions of actinide ions (U, Np, Pu) with corroded iron surfaces. RIXS measurements at the actinide 5d edge found to be sensitive to actinide oxidation states in different systems. Comparison of experimental and calculated Cm 5d RIXS spectra gave direct information about valency of the 248 curium isotope in oxide. Scientific understanding of processes that control chemical changes of radioactive species from spent fuel is improved by studying interactions of actinide ions (U, Np, Pu) with corroded iron surfaces. RIXS measurements at the actinide 5d edge indicate the reduction of U(VI), NP(V) and Pu(VI) to U(IV), Np(IV) and Pu(IV) by presence of iron ions. This thesis is also addressed to the study of changes in the electronic structure of copper films during interaction with synthetic groundwater solutions. The surface modifications induced by chemical reactions of oxidized 100 Angstrom Cu films with CL{sup -}, SO{sub 4}{sup 2-} and HCO{sub 3}{sup -} ions in aqueous solutions with various concentrations were studied in-situ using XAS. It was shown that the pH value, the concentration of Cl{sup -} ion and presence of HC{sub 3}{sup -} ion in the solutions strongly affect the speed of the corrosion reaction. The Cu 2p RIXS was used to distinguish between the species present on the copper surface while in contact with groundwater solution.

Kvashnina, Kristina

2007-07-11T23:59:59.000Z

96

A new method to derive electronegativity from resonant inelastic x-ray scattering  

SciTech Connect

Electronegativity is a well-known property of atoms and substituent groups. Because there is no direct way to measure it, establishing a useful scale for electronegativity often entails correlating it to another chemical parameter; a wide variety of methods have been proposed over the past 80 years to do just that. This work reports a new approach that connects electronegativity to a spectroscopic parameter derived from resonant inelastic x-ray scattering. The new method is demonstrated using a series of chlorine-containing compounds, focusing on the Cl 2p{sup -1}LUMO{sup 1} electronic states reached after Cl 1s{yields} LUMO core excitation and subsequent KL radiative decay. Based on an electron-density analysis of the LUMOs, the relative weights of the Cl 2p{sub z} atomic orbital contributing to the Cl 2p{sub 3/2} molecular spin-orbit components are shown to yield a linear electronegativity scale consistent with previous approaches.

Carniato, S.; Journel, L.; Guillemin, R.; Piancastelli, M. N.; Simon, M. [UPMC Univ Paris 06, UMR7614, Laboratoire de Chimie Physique-Matiere et Rayonnement, 11 rue Pierre et Marie Curie, 75231 Paris Cedex 05 (France); CNRS, LCPMR (UMR 7614), 11 rue Pierre et Marie Curie, 75231 Parix Cedex 05 (France); Stolte, W. C. [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Department of Chemistry, University of Nevada, Las Vegas, Nevada 89154-4009 (United States); Harry Reid Center for Environmental Studies, University of Nevada, Las Vegas, Nevada, 89154-4003 (United States); Lindle, D. W. [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Department of Chemistry, University of Nevada, Las Vegas, Nevada 89154-4009 (United States)

2012-10-14T23:59:59.000Z

97

Growth dynamics of pentacene thin films: Real-time synchrotron x-ray scattering study  

Science Conference Proceedings (OSTI)

Real-time synchrotron x-ray scattering in the anti-Bragg configuration was used to monitor the dynamics of pentacene film growth on inert substrates. A distributed-growth model, according to which pentacene molecules adsorbed on the nth layer can either nucleate and contribute to the growth of the (n+1)th layer or transfer downward and contribute to the growth of the nth layer, gave a good description of the data. For molecules adsorbed on the first and second layers, the probability of downward transfer was found to be dependent on the substrate, and independent of temperature within the range from 25 to 60 deg. C. For films grown on SiO{sub 2}, an Ehrlich-Schwoebel barrier of the order of 70 meV dominated downward transfer of pentacene molecules in layers away from the substrate. For films grown on an alkylated self-assembled monolayer, significant desorption of pentacene molecules from the substrate at elevated temperatures forced the growth mode toward the three-dimensional limit.

Mayer, Alex C.; Ruiz, Ricardo; Malliaras, George G. [Materials Science and Engineering, Cornell University, Ithaca, New York 14853 (United States); Zhou, Hua; Headrick, Randall L. [Department of Physics, University of Vermont, Burlington, Vermont 05405 (United States); Kazimirov, Alexander [Cornell High Energy Synchrotron Source, Ithaca, New York 14853 (United States)

2006-05-15T23:59:59.000Z

98

Synchrotron-based coherent scatter x-ray projection imaging using an array of monoenergetic pencil beams  

SciTech Connect

Traditional projection x-ray imaging utilizes only the information from the primary photons. Low-angle coherent scatter images can be acquired simultaneous to the primary images and provide additional information. In medical applications scatter imaging can improve x-ray contrast or reduce dose using information that is currently discarded in radiological images to augment the transmitted radiation information. Other applications include non-destructive testing and security. A system at the Canadian Light Source synchrotron was configured which utilizes multiple pencil beams (up to five) to create both primary and coherent scatter projection images, simultaneously. The sample was scanned through the beams using an automated step-and-shoot setup. Pixels were acquired in a hexagonal lattice to maximize packing efficiency. The typical pitch was between 1.0 and 1.6 mm. A Maximum Likelihood-Expectation Maximization-based iterative method was used to disentangle the overlapping information from the flat panel digital x-ray detector. The pixel value of the coherent scatter image was generated by integrating the radial profile (scatter intensity versus scattering angle) over an angular range. Different angular ranges maximize the contrast between different materials of interest. A five-beam primary and scatter image set (which had a pixel beam time of 990 ms and total scan time of 56 min) of a porcine phantom is included. For comparison a single-beam coherent scatter image of the same phantom is included. The muscle-fat contrast was 0.10 {+-} 0.01 and 1.16 {+-} 0.03 for the five-beam primary and scatter images, respectively. The air kerma was measured free in air using aluminum oxide optically stimulated luminescent dosimeters. The total area-averaged air kerma for the scan was measured to be 7.2 {+-} 0.4 cGy although due to difficulties in small-beam dosimetry this number could be inaccurate.

Landheer, Karl [Ottawa Medical Physics Institute and Ottawa-Carleton Institute for Physics, Department of Physics, Carleton University, 1125 Colonel By Drive, Ottawa K1S 5B6 (Canada); Johns, Paul C. [Ottawa Medical Physics Institute and Ottawa-Carleton Institute for Physics, Department of Physics, Carleton University, 1125 Colonel By Drive, Ottawa K1S 5B6 (Canada); Department of Radiology, University of Ottawa (Canada)

2012-09-15T23:59:59.000Z

99

X-ray resonant magnetic scattering study of magnetic stripe domains in a-GdFe thin films  

SciTech Connect

X-ray resonant magnetic scattering (XRMS) has been used to investigate the structure of magnetic stripe domain patterns in thin amorphous GdFe films. Under the influence of a perpendicular magnetic field, the scattered intensity displays a smooth transition from a structure factor of correlated stripes to the form factor of isolated domains. We derive a quite general expression that relates the total scattered intensity of XRMS to the absolute value of the magnetization. Furthermore, we compare our results for the domain period with domain theory. We obtain good agreement for prealigned stripes, but disorder tends to lead to an overestimation of the period measured with XRMS.

Miguel, J.; Peters, J. F.; Toulemonde, O. M.; Goedkoop, J. B. [Van der Waals-Zeeman Institute, University of Amsterdam, Valckenierstraat 65, 1018 XE, Amsterdam (Netherlands); Dhesi, S. S.; Brookes, N. B. [European Synchrotron Radiation Facility, ESRF, Boite Postale 220, F-38043 Grenoble Cedex (France)

2006-09-01T23:59:59.000Z

100

SSRL School 2008 on Hard X-ray Scattering Techniques in MES  

NLE Websites -- All DOE Office Websites (Extended Search)

May 20-22, 2008 SSRL School on Synchrotron X-ray Absorption Spectroscopy Techniques in Environmental and Materials Sciences: Theory and Application Group photo from the 2008 SSRL...

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


101

Soft x-ray scattering facility at the Advanced Light Source with real-time data processing and analysis  

Science Conference Proceedings (OSTI)

We present the development and characterization of a dedicated resonant soft x-ray scattering facility. Capable of operation over a wide energy range, the beamline and endstation are primarily used for scattering from soft matter systems around the carbon K-edge ({approx}285 eV). We describe the specialized design of the instrument and characteristics of the beamline. Operational characteristics of immediate interest to users such as polarization control, degree of higher harmonic spectral contamination, and detector noise are delineated. Of special interest is the development of a higher harmonic rejection system that improves the spectral purity of the x-ray beam. Special software and a user-friendly interface have been implemented to allow real-time data processing and preliminary data analysis simultaneous with data acquisition.

Gann, E.; Collins, B. A.; Ade, H. [Department of Physics, North Carolina State University, Raleigh, North Carolina 27695-8202 (United States); Young, A. T.; Nasiatka, J.; Padmore, H. A.; Hexemer, A.; Wang, C. [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Yan, H. [Department of Physics, North Carolina State University, Raleigh, North Carolina 27695-8202 (United States); Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States)

2012-04-15T23:59:59.000Z

102

In-situ Synchrotron Radiation X-ray Scattering Study On The Initial Structure Of Atomic Layer Deposition  

Science Conference Proceedings (OSTI)

Due to the excellent conformality of ALD, it is not only adopted thin film, but also has been adopted for the fabrication of nanostructures. The surface reaction of ALD process is dependent on the substrate condition, thus the study on initial stage of ALD process is crucial to achieve controllable film growth. By the way, because of quite low scattering intensity of initial ultra thin layer, the high flux Synchrotron Radiation is needed. Synchrotron radiation x-ray scattering measurements allow us to investigate the atomic structure evolution of a few nanometer thickness films at the initial growth stage, nondestructively. Ru and TaN ALD films were grown. The thickness, roughness, and electron density were estimated by X-Ray Reflectivity (XRR) analysis. The island structures and its coverage also were estimated.

Park, Y. J. [Pohang Accelerator Laboratory, POSTECH, Pohang, Gyeongbuk (Korea, Republic of); Department of MSE, POSTECH, Pohang, Gyeongbuk (Korea, Republic of); Lee, D. R. [Department of Physics, Soongsil univ., Seoul (Korea, Republic of); Baik, S. [Department of MSE, POSTECH, Pohang, Gyeongbuk (Korea, Republic of)

2011-12-23T23:59:59.000Z

103

Neutron and x-ray scattering studies of the metallurgical condition and residual stresses in Weldalite welds  

DOE Green Energy (OSTI)

Weldalite is a lithium-containing aluminum alloy which is being considered for aerospace applications because its favorable strength-to-weight ratio. Successful welding of this alloy depends on the control of the metallurgical condition and residual stresses in the heat affected zone. Neutron and x-ray scattering methods of residual stress measurement were applied to plasma arc welds made in aluminum-lithium alloy test panels as part of an evaluation of materials for use in welded structures. In the course of these studies discrepancies between x-ray and neutron results from the heat affected zone (HAZ) of the weld were found. Texture changes and recovery from the cold work, indicated in peak widths, were found in the HAZ as well. The consideration of x-ray and neutron results leads to the conclusion that there is a change in solute composition which modifies the d-spacings in the HAZ which affects the neutron diffraction determination of residual stresses. The composition changes give the appearance of significant compressive strains in the HAZ. This effect and sharp gradients in the texture give severe anomalies in the neutron measurement of residual stress. The use of combined x-ray and neutron techniques and the solution to the minimizing of the neutron diffraction anomalies are discussed.

Spooner, S. [Oak Ridge National Lab., TN (United States); Pardue, E.B.S. [Technology for Energy Corp., Knoxville, TN (United States)

1995-12-31T23:59:59.000Z

104

Polarization Dependence of L- and M-Edge Resonant Inelastic X-Ray Scattering in Transition-Metal Compounds  

SciTech Connect

The resonant inelastic x-ray scattering (RIXS) cross section at the L and M edges of transition-metal compounds is studied using an effective scattering operator. The intensities of the elastic peak and for spin-flip processes are derived. It is shown how the polarization dependence can be used to select transitions. Comparisons are made with experiment. A detailed analysis of the polarization and angular dependence of L- and M-edge RIXS for divalent copper compounds, such as the high-T{sub c} superconductors, is given.

van Veenendaal, Michel (ANL/NIU)

2010-12-03T23:59:59.000Z

105

Determining the electron-phonon coupling strength from Resonant Inelastic X-ray Scattering at transition metal L-edges  

SciTech Connect

We show that high-resolution Resonant Inelastic X-ray Scattering (RIXS) provides direct, element-specific and momentum-resolved information on the electron-phonon (e-p) coupling strength. Our theoretical analysis indicates how the e-p coupling can be extracted from RIXS spectra by determining the differential phonon scattering cross-section. An alternative manner to extract the coupling is to use the one- and two-phonon loss ratio, which is governed by the e-p coupling strength and the core-hole lifetime. This allows the determination of the e-p coupling on an absolute energy scale.

Ament, L.J.P.; van Veenendaal, M.; van den Brink, J. (Leiden); (NIU); (IFW Dresden)

2012-04-02T23:59:59.000Z

106

Exploring local atomic arrangements in amorphous and metastable phase change materials with x-ray and neutron total scattering  

SciTech Connect

Very little experimental work has conclusively explored the structural transformation between the amorphous and metastable crystalline phases of phase change chalcogenides. A recent flurry of theoretical work has supported likely mechanisms for the phase transition process in Ge-Sb-Te (GST) compositions and invigorated efforts at probing local atomic arrangements experimentally. The pair distribution function (PDF) formalism of total scattering data provides directly both local structure correlations at low real-space dimensions, and intermediate range order at higher length scales, a distinct advantage for following the relevant phase transition in phase change materials (PCM). A challenge facing the field is the difficulty in distinguishing separate peak contributions to pair correlation functions in amorphous and highly disordered samples. For example, various types of local order have been reported for Ge{sub x}Te{sub 1-x} phases, including both random mixtures and discrete structural units, and both 4-fold and 6-fold coordination around Ge. We describe our efforts in advancing capabilities for extracting and refining differential or partial pair distribution function data sets by combining neutron and x-ray total scattering, with extensions to isotopic substitution and anomalous x-ray scattering. Our results combining neutron and x-ray scattering for the Ge{sub x}Te{sub 1-x} series, for example, clearly distinguish Ge-Te and Te-Te contributions in nearest neighbor correlations. Presenting an additional challenge, phase change materials with fast switching speeds (those arguably of greatest technological interest) have stable bulk crystalline phases and do not readily form glasses until reduced to small dimensions. Thin film samples are inherently difficult to probe with conventional crystallographic methods. We demonstrate successful synchrotron x-ray total scattering experiments for PCM thin films with thicknesses between 100 nm and 1 um and describe how chemical short-range order and local bonding environments vary in amorphous, metastable and crystalline GeSb{sub 2}Te{sub 4} films. Total scattering methods for powders and thin films allow for a direct comparison of PCM properties (crystallization temperature, optical contrast between phases, phase change speed, etc.) with observed local structure and motivate further exploration into the atomic configurations enabling this fascinating class of materials.

Page, Katharine [Los Alamos National Laboratory; Daemen, Luc [Los Alamos National Laboratory; Proffen, Thomas [Los Alamos National Laboratory

2010-01-01T23:59:59.000Z

107

Inelastic x-ray scattering study of supercooled liquid and solid silicon.  

Science Conference Proceedings (OSTI)

Momentum-resolved inelastic x-ray scattering (IXS) technique is one of the powerful methods for the study of dynamical properties of a given system even in extreme conditions like high temperature and high pressure. At the same time, experimental studies of physical and structural properties of liquids have multiplied in recent years with the advent of containerless techniques. These methods reduce the possibility of contamination of specimens and remove external nucleation sites. Therefore, by combining the IXS method with the levitation method, the dynamical properties of stable liquids up to 3000 K and supercooled phase of liquids can be studied. Silicon is a basic material in the semiconductor industry and has been the subject of a large amount of experimental and theoretical studies over a long time. In the crystalline phase at ambient conditions, silicon is a diamond-structured semiconductor, but upon melting it undergoes a semiconductor-to-metal transition accompanied by significant changes in the structure and density. The coordination number increases from 4 in the solid to about 6.5 in the liquid, and liquid density is increased by about 10%. The principal purpose of the present study was to determine silicon's elastic modulus from the measurement of averaged sound speed determined from IXS. The experiments were carried out at the Advanced Photon Source (APS) beamline 3-ID with a high-resolution monochromator consisting of two nested channel-cut crystals and four backscattering analyzer setups in the horizontal scattering plane 6 m from the sample. The requirements for very high energy resolution and the basic principles of such instrumentation are discussed elsewhere as referenced. The levitation apparatus was enclosed in a bell jar specially designed for backscattering geometry with a separation of 10 cm between the sample and the detector. Silicon spheres of 2 to 3 mm in diameter were suspended in an argon gas jet and heated with a 270 W CO{sub 2} laser beam. Temperatures were measured during the experiment with a pyrometer whose operating wavelength was 0.65 {micro}m. The temperature gradient on the sample was estimated to be about +/- 20 K. The energy scans were taken for supercooled-liquid and hot-solid silicon at temperature T=1620 K. Sound velocities were determined from the initial slope of the excitation frequencies. Then, the longitudinal moduli for hotsolid and supercooled-liquid silicon were calculated from L = v{sub L}{sup 2}{rho} using measured velocities. In these calculations, density values were taken from Ohsaka et al. as referenced. Results are presented in Table 1. together with room-temperature, hot-solid single-crystal measurements, and stable-liquid values. Room-temperature longitudinal moduli were calculated from the values of the single-crystal elastic constants. They were measured between 300 K and 870 K. Since there was no phase transition up to temperature 1620 K for hot-solid silicon, it is reasonable to extrapolate these data to 1620 K in order to compare to our results for the hot solid. A significant difference (about 20%) is observed between our measurement and the extrapolated single-crystal value of the longitudinal modulus for solid silicon at temperature 1620K. This reduction of the longitudinal modulus may be an indication of the pre-melting. The factor of more than two change in the elastic modulus between supercooled liquid and hot solid at the same temperature can be attributed to the semiconductor-to-metal transition in silicon associated with melting. Also, the longitudinal modulus of the stable liquid is reported in Table 1. About a 10% difference is observed between the modulus of the supercooled and the stable liquid silicon. This can be interpreted as silicon still maintaining metallic properties with a significant increase in the degree of the directional bonding upon supercooling, as found in the x-ray diffraction and ab initio MD studies. All these results are discussed in reference.

Alatas, A.; Said, A.; Sinn, H.; Alp, E.E.; Kodituwakku, C.N.; Saboungi, M.L.; Price, D.L.; X-Ray Science Division; Western Michigan Univ.; Purdue Univ.; CRMD-CNRS; CRMHT-CNRS

2006-01-01T23:59:59.000Z

108

Tunable X-ray source  

DOE Patents (OSTI)

A method for the production of X-ray bunches tunable in both time and energy level by generating multiple photon, X-ray, beams through the use of Thomson scattering. The method of the present invention simultaneously produces two X-ray pulses that are tunable in energy and/or time.

Boyce, James R. (Williamsburg, VA)

2011-02-08T23:59:59.000Z

109

X-ray diffraction and scattering studies of coal constituents. Final technical report, January 1-December 31, 1983  

DOE Green Energy (OSTI)

The general objective of this work has been to use x-ray diffraction and scattering to examine whole coals, coal macerals and minerals in order to perform the following studies: (1) to identify and explain differences in vitrinites and framboids from various coals; (2) to correlate differences with basic coal compositions and properties; and (3) to determine the systematic variability in the micro compositional variation of macerals. The accomplishments have been: (a) the development of the Fourier transform technique to do proximate and ultimate analyses in a quick fashion; and (b) the investigation of the structure of pyrite framboids and preliminary studies of coal macerals. 3 figures, 12 tables.

Pavlovic, A. S.; Renton, J. T.

1984-03-15T23:59:59.000Z

110

The Lx-Yx Relation: Using Galaxy Cluster X-Ray Luminosity as a Robust, Low Scatter Mass Proxy  

E-Print Network (OSTI)

We use a sample of 115 galaxy clusters at 0.1scatter in the relation is dominated by cluster cores, and a tight LY relation (11% intrinsic scatter in Lx) is recovered if sufficiently large core regions (0.15R500) are excluded. The intrinsic scatter is well described by a lognormal distribution and the relations are consistent for relaxed and disturbed/merging clusters. We investigate the LY relation in low-quality data (e.g. for clusters detected in X-ray survey data) by estimating Lx from soft band count rates, and find that the scatter increases somewhat to 21%. We confirm the tight correlation between Yx and mass and the self-similar evolution of that scaling relation out to z=0.6 for a subset of clusters in our sample with mass estimates from the literature. This is used to estimate masses for the entire sample and hence measure the LM relation. We find that the scatter in the LM relation is much lower than previous estimates, due to the full removal of cluster cores and more robust mass estimates. For high-redshift clusters the scatter in the LM relation remains low if cluster cores are not excluded. These results suggest that cluster masses can be reliably estimated from simple luminosity measurements in low quality data where direct mass estimates, or measurements of Yx are not possible. This has important applications in the estimation of cosmological parameters from X-ray cluster surveys.

B. J. Maughan

2007-03-19T23:59:59.000Z

111

Fe K-edge X-ray resonant magnetic scattering from Ba(Fe1?xCox)2As2 superconductors  

SciTech Connect

We present an X-ray resonant magnetic scattering study at the Fe-K absorption edge of the BaFe2As2 compound. The energy spectrum of the resonant scattering, together with our calculation using the full-potential linear-augmented plane wave method with a local density functional suggests that the observed resonant scattering arises from electric dipole (E1) transitions. We discuss the role of Fe K-edge X-ray resonant magnetic scattering in understanding the relationship between the structure and the antiferromagnetic transition in the doped Ba(Fe1?xCox)2As2 superconductors.

Kim, Min Gyu; Kreyssig, Andreas; Lee, Yongbin; McQueeney, Robert J.; Harmon, Bruce N.; Goldman, Alan I.

2012-06-15T23:59:59.000Z

112

SSRL School 2007 on Hard X-ray Scattering: Techniques in MES  

NLE Websites -- All DOE Office Websites (Extended Search)

In-situ scattering, S. Webb Amorphous materials, T. Hufnagel Tuesday Afternoon, SurfaceThin Film Techniques Epitaxial thin film scattering, A. Vailionis Polycrystalline thin...

113

Global molecular structure and interfaces : refining an RNA : RNA complex structure using solution x-ray scattering data.  

SciTech Connect

Determining the global architecture of multicomponent systems is a central problem in understanding biomacromolecular machines. Defining interfaces among components and the global structure of multicomponent systems is a central problem in understanding the biological interactions on a molecular level. We demonstrate that solution X-ray scattering data can be used to precisely determine intermolecular interfaces from just the subunit structures, in the complete absence of intermolecular NMR restraints using an example of a 30 kDa RNA-RNA complex. The backbone root-mean-square deviation (rmsd) between structures that are determined using the scattering data and using intermolecular distance restraints is about 0.4 {angstrom}. Further, we refined the global structure of the complex using scattering data as a global restraint. The rmsd in backbone structures that are determined with and without the scattering data refinement is about 3.2 {angstrom}, suggesting the impact of the refinement to the overall structure. Information about the 'global correctness' of solution RNA structures could not be practically obtained otherwise, due to the molecular nature of the RNA molecules, but could only be defined by the scattering data together by residual dipolar couplings. This method provides a powerful new approach for refining global structures of macromolecular complexes whose subunits are elongated.

Zuo, X.; Wang, J.; Foster, T. R.; Schwieters, C. D.; Tiede, D. M.; Butcher, S. E.; Wang, Y.-X.; Chemical Sciences and Engineering Division; NCI-Frederick; Univ. of Wisconin at Madison; NIH

2008-03-19T23:59:59.000Z

114

Small-angle x-ray scattering measurements of the microstructure of liquid helium mixtures adsorbed in aerogel  

Science Conference Proceedings (OSTI)

Small-angle x-ray scattering (SAXS) was used to measure the microstructure of isotopic mixtures of {sup 3}He and {sup 4}He adsorbed into silica aerogels as a function of temperature and {sup 3}He concentration. The SAXS measurements could be well described by the formation of a nearly pure film of {sup 4}He which separates from the bulk mixture onto the aerogel strands and which thickens with decreasing temperature. Previous observations of a superfluid {sup 3}He-rich phase are consistent with superfluidity existing within this film phase. Observed differences between different density aerogels are explained in terms of the depletion of {sup 4}He from the bulk mixture due to film formation.

Lurio, L. B.; Mulders, N.; Paetkau, M.; Chan, M. H. W.; Mochrie, S. G. J. [Department of Physics, Northern Illinois University, DeKalb, Illinois 60115 (United States); Department of Physics, University of Delaware, Newark, Delaware 19716 (United States); Department of Physics and Astronomy, Okanagan College, British Columbia V1Y4X8 (Canada); Department of Physics, Pennsylvania State University, University Park, Pennsylvania 16802 (United States); Department of Physics, Yale University, New Haven, Connecticut 06511 (United States)

2007-07-15T23:59:59.000Z

115

Dynamic investigation of gold nanocrystal assembly using in situ grazing-incidence small angle x-ray scattering.  

SciTech Connect

Here we investigate the dynamic self-assembly pathway of ordered gold nanocrystal arrays during the self-assembly of gold nanocrystal micelles, with and without the presence of colloidal silica precursors, using grazing-incidence X-ray scattering performed at a synchrotron source. With silica precursors present, a lattice with rhombohedral symmetry is formed from the partial collapse of a face-centered cubic structure. In the absence of silica, a transient body-centered orthorhombic phase appears, which rapidly collapses into a glassy nanocrystal film. The appearance of face-centered and body-centered structures is consistent with a phase diagram for charged colloidal particles with assembly modulated via Coulomb screening.

Dunphy, D.; Fan, H.; Li, X.; Wang, J.; Brinker, C. J.; X-Ray Science Division; Univ. of New Mexico; SNL

2008-01-01T23:59:59.000Z

116

In-situ small-angle X-ray scattering study of the precipitation behavior in a Fe-25 at.%Co-9 at.%Mo alloy  

Science Conference Proceedings (OSTI)

Fe-Co-Mo alloys show extraordinary mechanical properties which make them potential candidates for various high-performance applications. In the present study, for the first time, the precipitation behavior in a Fe-25 at.%Co-9 at.%Mo alloy was studied by small-angle X-ray scattering using high-energy synchrotron radiation. The specimens were isothermally aged in an in-situ furnace. The small-angle X-ray scattering patterns showed scaling behavior and were evaluated by employing a model function from the literature. This approach provides information about the characteristic length scale and the volume fraction of the precipitates in the alloy.

Zickler, Gerald A. [Department of Physical Metallurgy and Materials Testing, Montanuniversitaet Leoben, Franz-Josef-Strasse 18, A-8700 Leoben (Austria); Christian Doppler Laboratory for Early Stages of Precipitation, Montanuniversitaet Leoben, Franz-Josef-Strasse 18, A-8700 Leoben (Austria)], E-mail: gerald.zickler@mu-leoben.at; Eidenberger, Elisabeth [Department of Physical Metallurgy and Materials Testing, Montanuniversitaet Leoben, Franz-Josef-Strasse 18, A-8700 Leoben (Austria); Leitner, Harald [Department of Physical Metallurgy and Materials Testing, Montanuniversitaet Leoben, Franz-Josef-Strasse 18, A-8700 Leoben (Austria); Christian Doppler Laboratory for Early Stages of Precipitation, Montanuniversitaet Leoben, Franz-Josef-Strasse 18, A-8700 Leoben (Austria); Stergar, Erich; Clemens, Helmut [Department of Physical Metallurgy and Materials Testing, Montanuniversitaet Leoben, Franz-Josef-Strasse 18, A-8700 Leoben (Austria); Staron, Peter; Lippmann, Thomas; Schreyer, Andreas [GKSS Research Center Geesthacht, Max-Planck-Strasse 1, D-21502 Geesthacht (Germany)

2008-12-15T23:59:59.000Z

117

THE ROLE OF INVERSE COMPTON SCATTERING IN SOLAR CORONAL HARD X-RAY AND {gamma}-RAY SOURCES  

SciTech Connect

Coronal hard X-ray (HXR) and continuum {gamma}-ray sources associated with the impulsive phase of solar flares have been the subject of renewed interest in recent years. They have been interpreted in terms of thin-target, non-thermal bremsstrahlung emission. This interpretation has led to rather extreme physical requirements in some cases. For example, in one case, essentially all of the electrons in the source must be accelerated to non-thermal energies to account for the coronal HXR source. In other cases, the extremely hard photon spectra of the coronal continuum {gamma}-ray emission suggest that the low-energy cutoff of the electron energy distribution lies in the MeV energy range. Here, we consider the role of inverse Compton scattering (ICS) as an alternate emission mechanism in both the ultra- and mildly relativistic regimes. It is known that relativistic electrons are produced during powerful flares; these are capable of upscattering soft photospheric photons to HXR and {gamma}-ray energies. Previously overlooked is the fact that mildly relativistic electrons, generally produced in much greater numbers in flares of all sizes, can upscatter extreme-ultraviolet/soft X-ray photons to HXR energies. We also explore ICS on anisotropic electron distributions and show that the resulting emission can be significantly enhanced over an isotropic electron distribution for favorable viewing geometries. We briefly review results from bremsstrahlung emission and reconsider circumstances under which non-thermal bremsstrahlung or ICS would be favored. Finally, we consider a selection of coronal HXR and {gamma}-ray events and find that in some cases the ICS is a viable alternative emission mechanism.

Chen Bin [Department of Astronomy, University of Virginia, Charlottesville, VA 22904 (United States); Bastian, T. S. [National Radio Astronomy Observatory, Charlottesville, VA 22903 (United States)

2012-05-01T23:59:59.000Z

118

Combined Use of Residual Dipolar Couplings and Solution X-ray Scattering To Rapidly Probe Rigid-Body Conformational Transitions in a Non-phosphorylatable Active-Site Mutant of the 128 kDa Enzyme I Dimer  

Science Conference Proceedings (OSTI)

The first component of the bacterial phosphotransferase system, enzyme I (EI), is a multidomain 128 kDa dimer that undergoes large rigid-body conformational transitions during the course of its catalytic cycle. Here we investigate the solution structure of a non-phosphorylatable active-site mutant in which the active-site histidine is substituted by glutamine. We show that perturbations in the relative orientations and positions of the domains and subdomains can be rapidly and reliably determined by conjoined rigid-body/torsion angle/Cartesian simulated annealing calculations driven by orientational restraints from residual dipolar couplings and shape and translation information afforded by small- and wide-angle X-ray scattering. Although histidine and glutamine are isosteric, the conformational space available to a Gln side chain is larger than that for the imidazole ring of His. An additional hydrogen bond between the side chain of Gln189 located on the EIN{sup {alpha}/{beta}} subdomain and an aspartate (Asp129) on the EIN{sup {alpha}} subdomain results in a small ({approx}9{sup o}) reorientation of the EIN{sup {alpha}} and EIN{sup {alpha}/{beta}} subdomains that is in turn propagated to a larger reorientation ({approx}26{sup o}) of the EIN domain relative to the EIC dimerization domain, illustrating the positional sensitivity of the EIN domain and its constituent subdomains to small structural perturbations.

Takayama, Yuki; Schwieters, Charles D.; Grishaev, Alexander; Ghirlando, Rodolfo; Clore, G. Marius (NIH)

2012-10-23T23:59:59.000Z

119

The Role of Inverse Compton Scattering in Solar Coronal Hard X-ray and Gamma-ray Sources  

E-Print Network (OSTI)

We consider the role of inverse Compton scattering (ICS) as a means of producing coronal hard X-ray (HXR) and continuum gamma-ray sources during solar flares. Coronal HXR and continuum gamma-ray emission observed during solar flares has been interpreted in terms of thin-target bremsstrahlung emission. In one case, this interpretation leads to the conclusion that the number of energetic electrons required to account for the coronal HXR source must be large, implying that essentially all electrons in the source must be accelerated to energies >~ 16 keV. In other cases, the spectral index of the photon spectrum of gamma-ray sources approaches the theoretical limit for bremsstrahlung emission (alpha ~ 1.5 - 2). Here we investigate ICS in both the fully relativistic and mildly relativistic regimes as an alternative to non-thermal bremsstrahlung. It is known that relativistic electrons are produced during powerful flares; these are capable of up-scattering soft photospheric photons to HXR energies. Previously overl...

Chen, Bin

2011-01-01T23:59:59.000Z

120

FINITE DIFFERENCE METHODS FOR THE WIDE-ANGLE `PARABOLIC' EQUATION  

E-Print Network (OSTI)

FINITE DIFFERENCE METHODS FOR THE WIDE-ANGLE `PARABOLIC' EQUATION GEORGIOS AKRIVIS Abstract. We consider a model initial and boundary value problem for the wide-angle `parabolic' equation Lur = icu, the wide-angle `parabolic'equation of underwater acoustics. Given R > 0, µ 0, > 0, , and q real

Akrivis, Georgios

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


121

Pressure and field tuning the magnetostructural phases of Mn3O4: Raman scattering and x-ray diffraction studies  

Science Conference Proceedings (OSTI)

We present temperature-, magnetic-field-, and pressure-dependent Raman scattering studies of single crystal Mn{sub 3}O{sub 4}, combined with temperature- and field-dependent x-ray diffraction studies, revealing the novel magnetostructural phases in Mn{sub 3}O{sub 4}. Our temperature-dependent studies showed that the commensurate magnetic transition at T{sub 2} = 33K in the binary spinel Mn{sub 3}O{sub 4} is associated with a structural transition from tetragonal to orthorhombic structures. Field-dependent studies showed that the onset and nature of this structural transition can be controlled with an applied magnetic field, and revealed evidence for a field-tuned quantum phase transition to a tetragonal spin-disordered phase for H {parallel} [1{bar 1}0]. Pressure-dependent Raman measurements showed that the magnetic easy axis direction in Mn{sub 3}O{sub 4} can be controlled - and the ferrimagnetic transition temperature increased - with applied pressure. Finally, combined pressure- and magnetic-field-tuned Raman measurements revealed a rich magnetostructural phase diagram - including a pressure- and field-induced magnetically frustrated tetragonal phase in the PH phase diagram - that can be generated in Mn{sub 3}O{sub 4} with applied pressure and magnetic field.

Kim, M.; Nelson, C.; Chen, X.M.; Wang, X.; Budakian, R.; Abbamonte, P. & Cooper, S.L.

2011-11-18T23:59:59.000Z

122

Dissolution dynamics of the calcite-water interface observed in situ by glancing-incidence X-ray scattering  

DOE Green Energy (OSTI)

Glancing-incidence X-ray scattering measurements made at the National Synchrotron Light Source were used to investigate dissolution dynamics in situ at the calcite-water interface. The relation between calcite saturation state and roughness of the calcite (1014) cleavage surface as a function of time was examined during pH titrations of an initially calcite-saturated solution. Systematic variations in roughness were observed as a function of saturation state as pH was titrated to values below that of calcite saturation. Different steady-state values of roughness were evident at fixed values of {Delta}G{sub r}, and these were correlated with the extent of undersaturation. A significant increase in roughness begins to occur with increasing undersaturation at a {Delta}G{sub r} value of approximately {minus}2.0 kcal/mol. The dissolution rate corresponding to this increase is about 1.5 x 10{sup 7} mmol/cm {center_dot} sec. This increase in roughness is attributed to a transition in the principal rate-determining dissolution mechanism, and is consistent with both powder-reaction studies of dissolution kinetics and single-crystal dissolution studies by atomic force microscopy. These data indicate some important potential applications of GIXS in the study of mineral-water interface geochemistry.

Sturchio, N.C.; Chiarello, R.P.

1995-06-02T23:59:59.000Z

123

Experimental and Theoretical Comparison of the O K-Edge Nonresonant Inelastic X-ray Scattering and X-ray Absorption Spectra of NaReO[subscript 4  

Science Conference Proceedings (OSTI)

Accurate X-ray absorption spectra (XAS) of first row atoms, e.g., O, are notoriously difficult to obtain due to the extreme sensitivity of the measurement to surface contamination, self-absorption, and saturation affects. Herein, we describe a comprehensive approach for determining reliable O K-edge XAS data for ReO{sub 4}{sup 1-} and provide methodology for obtaining trustworthy and quantitative data on nonconducting molecular systems, even in the presence of surface contamination. This involves comparing spectra measured by nonresonant inelastic X-ray scattering (NRIXS), a bulk-sensitive technique that is not prone to X-ray self-absorption and provides exact peak intensities, with XAS spectra obtained by three different detection modes, namely total electron yield (TEY), fluorescence yield (FY), and scanning transmission X-ray microscopy (STXM). For ReO{sub 4}{sup 1-}, TEY measurements were heavily influenced by surface contamination, while the FY and STXM data agree well with the bulk NRIXS analysis. These spectra all showed two intense pre-edge features indicative of the covalent interaction between the Re 5d and O 2p orbitals. Density functional theory calculations were used to assign these two peaks as O 1s excitations to the e and t{sub 2} molecular orbitals that result from Re 5d and O 2p covalent mixing in T{sub d} symmetry. Electronic structure calculations were used to determine the amount of O 2p character (%) in these molecular orbitals. Time dependent-density functional theory (TD-DFT) was also used to calculate the energies and intensities of the pre-edge transitions. Overall, under these experimental conditions, this analysis suggests that NRIXS, STXM, and FY operate cooperatively, providing a sound basis for validation of bulk-like excitation spectra and, in combination with electronic structure calculations, suggest that NaReO{sub 4} may serve as a well-defined O K-edge energy and intensity standard for future O K-edge XAS studies.

Bradley, Joseph A.; Yang, Ping; Batista, Enrique R.; Boland, Kevin S.; Burns, Carol J.; Clark, David L.; Conradson, Steven D.; Kozimor, Stosh A.; Martin, Richard L.; Seidler, Gerald T.; Scott, Brian L.; Shuh, David K.; Tyliszczak, Tolek; Wilkerson, Marianne P.; Wolfsberg, Laura E. (PNNL); (UWASH); (LBNL); (LANL)

2010-12-07T23:59:59.000Z

124

Experimental and Theoretical Comparison of the O K-Edge Non-Resonant Inelastic X-ray Scattering and X-ray Absorption Spectra of NaReO4  

Science Conference Proceedings (OSTI)

Accurate X-ray absorption spectra (XAS) of first row atoms, e.g. O, are notoriously difficult to obtain due to the extreme sensitivity of the measurement to surface contamination, self-absorption, and saturation effects. Herein, we describe a comprehensive approach for determining reliable O K-edge XAS data for ReO41- and provide methodology for obtaining trustworthy and quantitative data on non-conducting molecular systems, even in the presence of surface contamination. This involves comparing spectra measured by non-resonant inelastic X-ray scattering (NRIXS), a bulk-sensitive technique that is not prone to X-ray self-absorption and provides exact peak intensities, with XAS spectra obtained by three different detection modes, namely total electron yield (TEY), fluorescence yield (FY), and scanning transmission X-ray microscopy (STXM). For ReO41-, TEY measurements were heavily influenced by surface contamination, while the FY and STXM data agree well with the bulk NRIXS analysis. These spectra all showed two intense pre-edge features indicative of the covalent interaction between the Re 5d and O 2p orbitals. Time dependent density functional theory calculations were used to assign these two peaks as O 1s excitations to the e and t2 molecular orbitals that result from Re 5d and O 2p covalent mixing in Td symmetry. Electronic structure calculations were used to determine the amount of O 2p character (%) in these molecular orbitals. Time-dependent density functional theory (TD-DFT) was also used to calculate the energies and intensities of the pre-edge transitions. Overall, under these experimental conditions, this analysis suggests that NRIXS, STXM, and FY operate cooperatively, providing a sound basis for validation of bulk-like excitation spectra and, in combination with electronic structure calculations, suggest that NaReO4 may serve as a well-defined O K-edge energy and intensity standard for future O K edge XAS studies.

Bradley, Joseph A.; Yang, Ping; Batista, Enrique R.; Boland, Kevin S.; Burns, Carol J.; Clark, David L.; Conradson, Steven D.; Kozimor, Stosh A.; Martin, Richard L.; Seidler, Gerald T.; Scott, Brian L.; Shuh, David K.; Tyliszczak, T.; Wilkerson, Marianne P.; Wolfsberg, Laura E.

2010-09-14T23:59:59.000Z

125

Mass fractal characteristics of silica sonogels as determined by small-angle x-ray scattering and nitrogen adsorption  

SciTech Connect

A sample series of silica sonogels was prepared using different water-tetraethoxysilane molar ratio (r{sub w}) in the gelation step of the process in order to obtain aerogels with different bulk densities after the supercritical drying. The samples were analyzed by means of small-angle x-ray-scattering (SAXS) and nitrogen-adsorption techniques. Wet sonogels exhibit mass fractal structure with fractal dimension D increasing from {approx}2.1 to {approx}2.4 and mass-fractal correlation length {xi} diminishing from {approx}13 nm to {approx}2 nm, as r{sub w} is changed in the nominal range from 66 to 6. The process of obtaining aerogels from sonogels and heat treatment at 500 deg. C, in general, increases the mass-fractal dimension D, diminishes the characteristic length {xi} of the fractal structure, and shortens the fractal range at the micropore side for the formation of a secondary structured particle, apparently evolved from the original wet structure at a high resolution level. The overall mass-fractal dimension D of aerogels was evaluated as {approx}2.4 and {approx}2.5, as determined from SAXS and from pore-size distribution by nitrogen adsorption, respectively. The fine structure of the 'secondary particle' developed in the obtaining of aerogels could be described as a surface-mass fractal, with the correlated surface and mass-fractal dimensions decreasing from {approx}2.4 to {approx}2.0 and from {approx}2.7 to {approx}2.5, respectively, as the aerogel bulk density increases from 0.25 (r{sub w}=66) up to 0.91 g/cm{sup 3} (r{sub w}=6)

Donatti, D.A.; Vollet, D.R.; Ibanez Ruiz, A.; Mesquita, A.; Silva, T.F.P. [Unesp-Universidade Estadual Paulista, IGCE, Departamento de Fisica, P.O. Box 178 CEP, 13500-970 Rio Claro, Sao Paulo (Brazil)

2005-01-01T23:59:59.000Z

126

WAND: Wide-Angle Neutron Diffractometer at HFIR | ORNL Neutron Sciences  

NLE Websites -- All DOE Office Websites (Extended Search)

US/Japan Wide-Angle Neutron Diffractometer US/Japan Wide-Angle Neutron Diffractometer WAND Instrument scientist Jaime Fernandez-Baca (left) with a visiting researcher at WAND. The Wide-Angle Neutron Diffractometer (WAND) at the HFIR HB-2C beam tube was designed to provide two specialized data-collection capabilities: (1) fast measurements of medium-resolution powder-diffraction patterns and (2) measurements of diffuse scattering in single crystals using flat-cone geometry. For these purposes, this instrument is equipped with a curved, one-dimensional 3He position-sensitive detector covering 125º of the scattering angle with the focal distance of 71 cm. The sample and detector can be tilted in the flat-cone geometry mode. These features enable measurement of single-crystal diffraction patterns in a short time over a

127

Structural and magnetic properties of transition metal substituted BaFe{sub 2}As{sub 2} compounds studied by x-ray and neutron scattering  

Science Conference Proceedings (OSTI)

The purpose of my dissertation is to understand the structural and magnetic properties of the newly discovered FeAs-based superconductors and the interconnection between superconductivity, antiferromagnetism, and structure. X-ray and neutron scattering techniques are powerful tools to directly observe the structure and magnetism in this system. I used both xray and neutron scattering techniques on di#11;erent transition substituted BaFe2As2 compounds in order to investigate the substitution dependence of structural and magnetic transitions and try to understand the connections between them.

Kim, Min Gyu [Ames Laboratory

2012-08-28T23:59:59.000Z

128

Theoretical treatments of the bound-free contribution and experimental best practice in X-ray Thomson scattering from warm dense matter  

SciTech Connect

By comparison with high-resolution synchrotron x-ray experimental results, we assess several theoretical treatments for the bound-free (core-electron) contribution to x-ray Thomson scattering (i.e., also known as nonresonant inelastic x-ray scattering). We identify an often overlooked source of systematic error in the plane-wave form factor approximation (PWFFA) used in the inference of temperature, ionization state, and free electron density in some laser-driven compression studies of warm dense matter. This error is due to a direct violation of energy conservation in the PWFFA. We propose an improved practice for the bound-free term that will be particularly relevant for XRTS experiments performed with somewhat improved energy resolution at the National Ignition Facility or the Linac Coherent Light Source. Our results raise important questions about the accuracy of state variable determination in XRTS studies, given that the limited information content in low-resolution XRTS spectra does not strongly constrain the models of electronic structure being used to fit the spectra.

Mattern, Brian A.; Seidler, Gerald T. [Department of Physics, University of Washington, Seattle, Washington 98195-1560 (United States)

2013-02-15T23:59:59.000Z

129

A Survey of Students from the National School on Neutron and X-ray Scattering: Communication Habits and Preferences  

Science Conference Proceedings (OSTI)

Oak Ridge National Laboratory (ORNL) offers the scientific community unique access to two types of world-class neutron sources at a single site - the Spallation Neutron Source (SNS) and the High Flux Isotope Reactor (HFIR). The 85-MW HFIR provides one of the highest steady-state neutron fluxes of any research reactor in the world. And the SNS is one of the world's most intense pulse neutron beams. Management of these resources is the responsibility of the Neutron Sciences Directorate (NScD). NScD started conducting the National School on Neutron and X-ray Scattering (NXS) in conjunction with the Advanced Photon Source (APS) at Argonne National Laboratory in 2007. This survey was conducted to determine the most effective ways to reach students with information about what SNS and HFIR offer the scientific community, including content and communication vehicles. The emphasis is on gaining insights into compelling messages and the most effective channels, e.g., Web sites and social media, for communicating with students about neutron science The survey was conducted in two phases using a classic qualitative investigation to confirm language and content followed by a survey designed to quantify issues, assumptions, and working hypotheses. Phase I consisted of a focus group in late June 2010 with students attending NXS. The primary intent of the group was to inform development of an online survey. Phase two consisted of an online survey that was developed and pre-tested in July 2010 and launched on August 9, 2010 and remained in the field until September 9, 2010. The survey achieved an overall response rate of 48% for a total of 157 completions. The objective of this study is to determine the most effective ways to reach students with information about what SNS and HFIR offer the scientific community, including content and communication vehicles. The emphasis is on gaining insights into compelling messages and the most effective channels, e.g., Web sites, social media, for communicating with students about neutron science.

Bryant, Rebecca [Bryant Research, LLC

2010-12-01T23:59:59.000Z

130

In-line phase-contrast imaging of a biological specimen using a compact laser-Compton scattering-based x-ray source  

SciTech Connect

Laser-Compton scattering (LCS) x-ray sources have recently attracted much attention for their potential use at local medical facilities because they can produce ultrashort pulsed, high-brilliance, and quasimonochromatic hard x rays with a small source size. The feasibility of in-line phase-contrast imaging for a 'thick' biological specimens of rat lumbar vertebrae using the developed compact LCS-X in AIST was investigated for the promotion of clinical imaging. In the higher-quality images, anatomical details of the spinous processes of the vertebrae are more clearly observable than with conventional absorption radiography. The results demonstrate that phase-contrast radiography can be performed using LCS-X.

Ikeura-Sekiguchi, H.; Kuroda, R.; Yasumoto, M.; Toyokawa, H.; Koike, M.; Yamada, K. [National Institute of Advanced Industrial Science and Technology (AIST), Central 2-5, 1-1-1 Umezono, Tsukuba, Ibaraki 305-8568 (Japan); Sakai, F. [Sumitomo Heavy Industries, Ltd. (SHI), 2-1-1, Yatocho, Nishitokyo, Tokyo 188-8585 (Japan); Mori, K.; Maruyama, K. [Ibaraki Prefectural University of Health Sciences, 4669-2, Ami, Inashiki, Ibaraki 300-0394 (Japan); Oka, H.; Kimata, T. [St. Marianna University School of Medicine, 2-16-1, Sugao, Miyamae-ku, Kawasaki City 216-8512 (Japan)

2008-03-31T23:59:59.000Z

131

Chandra Observations and Monte Carlo Simulations of the Grain-Scattered Halo of the Binary X-Ray Pulsar 4U 1538-52  

E-Print Network (OSTI)

Properties of the X-ray halo of the eclipsing X-ray pulsar 4U 1538-52 are derived from a 25 ksec observation by the Chandra X-Ray Observatory. Profiles of the halo, compiled in two energy ranges, 2 to 4 keV and 4 to 6 keV, and three time intervals before and after an eclipse immersion, exhibit a three-peak shape. The observed profiles are fitted by the profiles of a simulated halo generated by a Monte Carlo ray-tracing code operating on a model of three discrete clouds and a spectrum of the photons emitted by the source over a period of time extending from 270 ksec before the observation began till it ended. The distances of the two nearer dust clouds are fixed at the distances of the peaks of atomic hydrogen derived from the 21-cm spectrum in the direction of the X-ray source, namely at 1.30 and 2.56 kpc. A good fit is achieved with the source at a distance 4.5 kpc, the distance of the third cloud at 4.05 kpc, the total scattering optical depth of the three clouds equal to 0.159 at 3 keV, and the column density of hydrogen set to 4.6x10^22 cm^-2. With Av=6.5 mag for the binary companion star, QV Nor, the ratio of the scattering optical depth at 3 keV to the visual extinction is 0.0234 mag^-1.

George W. Clark

2004-04-16T23:59:59.000Z

132

X-ray data booklet. Revision  

SciTech Connect

A compilation of data is presented. Included are properties of the elements, electron binding energies, characteristic x-ray energies, fluorescence yields for K and L shells, Auger energies, energy levels for hydrogen-, helium-, and neonlike ions, scattering factors and mass absorption coefficients, and transmission bands of selected filters. Also included are selected reprints on scattering processes, x-ray sources, optics, x-ray detectors, and synchrotron radiation facilities. (WRF)

Vaughan, D. (ed.)

1986-04-01T23:59:59.000Z

133

Soft x-ray circular dichroism and scattering using a modulated elliptically polarizing wiggler and double synchronous detection  

Science Conference Proceedings (OSTI)

We have constructed an experimental station (beamline) at the National Synchrotron Light Source to measure circular dichroism (CD) using soft x-rays (250 {le} hv {le} 900 eV) from a time modulated elliptically polarizing wiggler. The polarization of the soft x-ray beam switches periodically between two opposite polarizations, hence permitting the use of phase-sensitive (lock-in) detection. While the wiggler can be modulated at frequencies up to 100 Hz, switching transients limit the actual practical frequency to {approx}25 Hz. With analog detection, switching transients are blocked by a chopper synchronized to the frequency and phase of the wiggler. The CD is obtained from the ratio of the signal recovered at the frequency of polarization modulation, f, to the average beam intensity, which is recovered by synchronous detection at frequency 2f.

Sutherland, J.C.; Polewski, K.; Monteleone, D.C. [and others

1998-01-23T23:59:59.000Z

134

Study of the Stability of 3C-SiC Single Crystals Using High-Resolution Diffuse X-Ray Scattering  

SciTech Connect

The stability of (001)-oriented 3C silicon carbide crystals is studied by a method coupling high resolution x-ray diffraction and numerical simulations. The analysis of the diffuse scattering intensity distribution along selected directions in reciprocal space allows us to obtain qualitative and quantitative informations regarding the 3C-6H transition. Our latest results concerning the influence of the initial crystal quality (presence of defects) and of annealing time on the 3C-6H transition are presented in this article.

Dompoint, D.; Boulle, A. [Science des Procedes Ceramiques et de Traitements de Surface (SPCTS) CNRS UMR 6638, ENSCI, 47 avenue Albert Thomas 87065 Limoges Cedex (France); Galben-Sandulache, I. G.; Chaussende, D. [Laboratoire des Materiaux et du Genie Physique (LMGP) CNRS UMR 5628, Grenoble INP, Minatec, 3 parvis Louis Neel, BP 257, 38016 Grenoble Cedex 01 (France)

2010-11-01T23:59:59.000Z

135

An iterative three-dimensional electron density imaging algorithm using uncollimated Compton scattered x rays from a polyenergetic primary pencil beam  

Science Conference Proceedings (OSTI)

X-ray film-screen mammography is currently the gold standard for detecting breast cancer. However, one disadvantage is that it projects a three-dimensional (3D) object onto a two-dimensional (2D) image, reducing contrast between small lesions and layers of normal tissue. Another limitation is its reduced sensitivity in women with mammographically dense breasts. Computed tomography (CT) produces a 3D image yet has had a limited role in mammography due to its relatively high dose, low resolution, and low contrast. As a first step towards implementing quantitative 3D mammography, which may improve the ability to detect and specify breast tumors, we have developed an analytical technique that can use Compton scatter to obtain 3D information of an object from a single projection. Imaging material with a pencil beam of polychromatic x rays produces a characteristic scattered photon spectrum at each point on the detector plane. A comparable distribution may be calculated using a known incident x-ray energy spectrum, beam shape, and an initial estimate of the object's 3D mass attenuation and electron density. Our iterative minimization algorithm changes the initially arbitrary electron density voxel matrix to reduce regular differences between the analytically predicted and experimentally measured spectra at each point on the detector plane. The simulated electron density converges to that of the object as the differences are minimized. The reconstruction algorithm has been validated using simulated data produced by the EGSnrc Monte Carlo code system. We applied the imaging algorithm to a cylindrically symmetric breast tissue phantom containing multiple inhomogeneities. A preliminary ROC analysis scores greater than 0.96, which indicate that under the described simplifying conditions, this approach shows promise in identifying and localizing inhomogeneities which simulate 0.5 mm calcifications with an image voxel resolution of 0.25 cm and at a dose comparable to mammography.

Van Uytven, Eric; Pistorius, Stephen; Gordon, Richard [Department of Physics and Astronomy, University of Manitoba, Winnipeg, Manitoba R3T 2N2 (Canada) and Medical Physics, CancerCare Manitoba, 675 McDermot Ave., Winnipeg, Manitoba, R3A 1R9 (Canada); Department of Physics and Astronomy, University of Manitoba, Winnipeg, Manitoba R3T 2N2 (Canada); Medical Physics, CancerCare Manitoba, 675 McDermot Ave., Winnipeg, Manitoba R3A 1R9 (Canada) and Department of Radiology, University of Manitoba, HSC Room GA216, 820 Sherbrook Street, Winnipeg, Manitoba R3A 1R9 (Canada); Department of Radiology, University of Manitoba, HSC Room GA216, 820 Sherbrook Street, Winnipeg, Manitoba R3A 1R9 (Canada) and Department of Electrical and Computer Engineering, University of Manitoba, HSC Room GA216, 820 Sherbrook Street, Winnipeg, Manitoba R3A 1R9 (Canada)

2007-01-15T23:59:59.000Z

136

Sure, a textbook can tell you about Bragg's Law and the x-ray absorption energies for any element in the periodic table, but it can't tell you how to plan and carry out an x-ray scattering experiment at one of the 50 or so synchrotron radiation facilitie  

NLE Websites -- All DOE Office Websites (Extended Search)

Report Report SSRL 6 th Annual School on Synchrotron X-ray Scattering Techniques in Materials and Environmental Sciences: Theory and Application SSRL SR-XRS participants. Synchrotron-based X-ray scattering (SR-XRS) techniques offer the ability to probe nano- and atomic-scale structure that dictates the properties of advanced technological and environmental materials. Important materials studied at the Stanford Synchrotron Radiation Lightsource (SSRL) include organic and inorganic thin films and interfaces, nanoparticles, complex oxides, solutions, polymers, minerals and poorly crystalline materials. Good planning and a good working knowledge of beam lines and techniques are required to successfully conduct SR-XRS measurements. This sixth annual School at SSRL on Synchrotron X-ray

137

Place-exchange mechanism of Pt (111) oxidation/reduction as observed by synchrotron X-ray scattering  

DOE Green Energy (OSTI)

Structural changes in the Pt(111) single crystal surface associated with incipient electrochemical oxidation/reduction were studied by {ital in}{ital situ} synchrotron x-ray reflectivity. It was shown that lifting of Pt atoms of the surface layer occurs, substantiating the long-standing hypothesis of a place-exchange mechanism for solution/metal interface oxidation. It was also shown that, for a charge transfer of {approx_lt}1.7 e{sup -}/Pt atom, the initially flat surface structure could be recovered by electrochemical reduction. In constrast, the surface was irreversibly roughened for amounts of charge transfer exceeding {approx}1.7 e{sup -}/Pt, but the roughening involved only the atoms in the top layer of the original flat surface. A detailed mechanism is proposed for the place-exchange mechanism and the subsequent roughening of the electrode surface.

You, H.; Nagy, Z.; Zurawski, D.J.; Chiarello, R.P.

1996-07-01T23:59:59.000Z

138

Changes in Delta-Plutonium Due to Aging as Observed by Continuous in-situ X-ray Scattering  

Science Conference Proceedings (OSTI)

The aging in plutonium is predominantly caused by its internal self irradiation. The self-irradiation in Pu-239 is by the decay process of transmuting the Pu atom into uranium atom and emitting an {alpha}-particle. Most of the lattice damage comes from the uranium recoil resulting in Frenkel type defects consisting of vacancies and self-interstitial atoms, helium in growth and defect clusters and possibly even though it is not yet observed, the generation of voids. As part of the stockpile stewardship, it is important to understand the changes in the structure and microstructures and their correlations to the physical properties. Changes in the physical properties has direct relationship to the quality of the structure, in terms of formation of defects and defect clustering, accumulation of voids, grain boundaries, phase changes and etc. which can adversely affects the stability of the material. These changes are very difficult to monitor because of the high activity of the sample, high atomic number making x-ray and synchrotron probe into the bulk very difficult (neutron probe is not feasible) and the long life time which normally requires decades to measure. In this paper we describe the development of an in-situ in-house transmission X-ray diffraction (XRD) experimental technique used to monitor the structural changes in these materials. This technique calls for a very thin sample of less that 2 {mu}m and to accelerate the aging process due to self-irradiation, spiked alloy of 7.5 weight percent of Pu-238 is used. This is equivalent to roughly 17 times the normal rate of aging. Current results suggest that over a period of 2.8 equivalent years, an increase of 0.5% in unit cell parameter is observed. The increase appears to be an abrupt jump at about 1.1 equivalent years, brought about by the collapsing of the atoms from the interstitials to the lattice sites. Further data analysis is on the way. (authors)

Saw, Cheng K.; Wall, Mark A.; Chung, Brandon W. [MSTD-CMS, Lawrence Livermore National Laboratory, Livermore, California (United States)

2007-07-01T23:59:59.000Z

139

Kinetics of HEX-BCC Transition in a Triblock Copolymer in a Selective Solvent: Time Resolved Small Angle X-ray Scattering Measurements and Model Calculations  

E-Print Network (OSTI)

Time-resolved small angle x-ray scattering (SAXS) was used to examine the kinetics of the transition from HEX cylinders to BCC spheres at various temperatures in poly(styrene-b- ethylene-co-butylene-b-styrene) (SEBS) in mineral oil, a selective solvent for the middle EB block. Temperature-ramp SAXS and rheology measurements show the HEX to BCC order-order transition (OOT) at ~127 oC and order-disorder transition (ODT) at ~180 oC. We also observed the metastability limit of HEX in BCC with a spinodal temperature, Ts ~ 150 oC. The OOT exhibits 3 stages and occurs via a nucleation and growth mechanism when the final temperature Tf peak into two peaks when the cylinder spacing and modulation wavelength are incommensurate predicted by the model is confirmed by analysis of the SAXS data.

Minghai Li; Yongsheng Liu; Huifen Nie; Rama Bansil; Milos Steinhart

2007-10-24T23:59:59.000Z

140

On the absence of a positive sound dispersion in the THz dynamics of glycerol: an inelastic x-ray scattering study  

Science Conference Proceedings (OSTI)

The high frequency transport properties of glycerol are derived from inelastic x-ray scattering spectra measured at different pressures and compared with ultrasound absorption data. As a result, the presence of two distinct relaxation processes is inferred: a slow one, occurring in the GHz window and having an essentially structural character, and a fast one, related instead to microscopic degrees of freedom. While the former originates a neat increase of the apparent, i.e. frequency-dependent, sound velocity, the latter induces no visible dispersive effects on the acoustic propagation. The observed behavior is likely paradigmatic of all glass formers near or below the melting and it is here discussed and explained in some detail.

Cunsolo, Alessandro (BNL)

2012-10-23T23:59:59.000Z

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141

Direct detection of x-rays for protein crystallography  

DOE Patents (OSTI)

An apparatus and method for directly determining the crystalline structure of a protein crystal. The crystal is irradiated by a finely collimated x-ray beam. The interaction o f the x-ray beam with the crystal produces scattered x-rays. These scattered x-rays are detected by means of a large area, thick CCD which is capable of measuring a significant number of scattered x-rays which impact its surface. The CCD is capable of detecting the position of impact of the scattered x-ray on the surface of the CCD and the quantity of scattered x-rays which impact the same cell or pixel. This data is then processed in real-time and the processed data is outputted to produce an image of the structure of the crystal. If this crystal is a protein the molecular structure of the protein can be determined from the data received.

Atac, Muzaffer; McKay, Timothy

1997-12-01T23:59:59.000Z

142

X-Ray Topography  

Science Conference Proceedings (OSTI)

Sep 17, 2009 ... Stress Mapping Analysis by Ray Tracing (SMART): A New Technique ... technique of synchrotron X-ray topography, where a grid made out of ...

143

X-Ray Data from the X-Ray Data Booklet Online  

DOE Data Explorer (OSTI)

The original X-Ray Data Booklet, published in 1985, became a classic reference source. The online version has been significantly revised and updated to reflect today's science. Hundreds of pages of authoritative data provide the x-ray properties of elements, information on synchrotron radiation, scattering processes, optics and detectors, and other related calculations, formulas, and data tables.

Thompson, Albert C.; Attwood, David T.; Gullikson, Eric M.; Howells, Malcolm R.; Kortright, Jeffrey B.; Robinson, Arthur L.; Underwood, James H.; Kim, Kwang-Je; Kirz, Janos; Lindau, Ingolf; Pianetta, Piero; Winick, Herman; Williams, Gwyn P.; Scofield, James H.

144

Transient x-ray diffraction and its application to materials science and x-ray optics  

SciTech Connect

Time resolved x-ray diffraction and scattering have been applied to the measurement of a wide variety of physical phenomena from chemical reactions to shock wave physics. Interest in this method has heightened in recent years with the advent of versatile, high power, pulsed x-ray sources utilizing laser plasmas, electron beams and other methods. In this article, we will describe some of the fundamentals involved in time resolved x-ray diffraction, review some of the history of its development, and describe some recent progress in the field. In this article we will emphasize the use of laser-plasmas as the x-ray source for transient diffraction.

Hauer, A.A.; Kopp, R.; Cobble, J.; Kyrala, G.; Springer, R. [and others

1997-12-01T23:59:59.000Z

145

X-ray beamsplitter  

DOE Patents (OSTI)

An x-ray beamsplitter which splits an x-ray beam into two coherent parts by reflecting and transmitting some fraction of an incident beam has applications for x-ray interferometry, x-ray holography, x-ray beam manipulation, and x-ray laser cavity output couplers. The beamsplitter is formed of a wavelength selective multilayer thin film supported by a very thin x-ray transparent membrane. The beamsplitter resonantly transmits and reflects x-rays through thin film interference effects. A thin film is formed of 5-50 pairs of alternate Mo/Si layers with a period of 20-250 A. The support membrane is 10-200 nm of silicon nitride or boron nitride. The multilayer/support membrane structure is formed across a window in a substrate by first forming the structure on a solid substrate and then forming a window in the substrate to leave a free-standing structure over the window.

Ceglio, Natale M. (Livermore, CA); Stearns, Daniel S. (Mountain View, CA); Hawryluk, Andrew M. (Modesto, CA); Barbee, Jr., Troy W. (Palo Alto, CA)

1989-01-01T23:59:59.000Z

146

Investigations of the R5(SixGe1-x)4 Intermetallic Compounds by X-Ray Resonant Magnetic Scattering  

SciTech Connect

The XRMS experiment on the Gd{sub 5}Ge{sub 4} system has shown that, below the Neel temperature, T{sub N} = 127 K, the magnetic unit cells is the same as the chemical unit cell. From azimuth scans and the Q dependence of the magnetic scattering, all three Gd sites in the structure were determined to be in the same magnetic space group Pnma. The magnetic moments are aligned along the c-axis and the c-components of the magnetic moments at the three different sites are equal. The ferromagnetic slabs are stacked antiferromagnetically along the b-direction. They found an unusual order parameter curve in Gd{sub 5}Ge{sub 4}. A spin-reorientation transition is a possibility in Gd{sub 5}Ge{sub 4}, which is similar to the Tb{sub 5}Ge{sub 4} case. Tb{sub 5}Ge{sub 4} possesses the same Sm{sub 5}Ge{sub 4}-type crystallographic structure and the same magnetic space group as Gd{sub 5}Ge{sub 4} does. The difference in magnetic structure is that Tb{sub 5}Ge{sub 4} has a canted one but Gd{sub 5}Ge{sub 4} has nearly a collinear one in the low temperature antiferromagnetic phase. The competition between the magneto-crystalline anisotropy and the nearest-neighbor magnetic exchange interactions may allow a 3-dimensional canted antiferromagnetic structure in Tb{sub 5}Ge{sub 4}. The spin-reorientation transition in both Gd{sub 5}Ge{sub 4} and Tb{sub 5}Ge{sub 4} may arise from the competition between the magnetic anisotropy from the spin-orbit coupling of the conduction electrons and the dipolar interactions anisotropy.

Lizhi Tan

2008-08-18T23:59:59.000Z

147

Characterization of nanostructured zirconia prepared by hydrolysis and reverse micelle synthesis by small-angle neutron and X-ray scattering  

DOE Green Energy (OSTI)

Low temperature techniques such as hydrolysis and reverse micelle syntheses provide the opportunity to determine the relationship between the structural properties and preparation conditions of zirconia powders as well as to tailor their physicochemical properties. The authors have performed small-angle neutron and synchrotron X-ray scattering (SANS and SAXS) experiments to study the nucleation and organization of zirconia nanoparticles via different preparation routes. First, the formation of reverse micelles in individual and mixed solutions of (ZrOCl{sub 2}+D{sub 2}O)/AOT/C{sub 6}D{sub 5}CD{sub 3}, and (NH{sub 4}OH+H{sub 2}O)/AOT/C{sub 6}D{sub 5}CD{sub 3} systems at water/AOT molar ratio of 20 was characterized. Second, the aggregation of zirconia gels obtained from the reaction of the reverse micelle solutions after heat treatments was studied. Third, the nanostructure of zirconia powders prepared by the reverse micelle method is compared with the corresponding powders prepared by hydrolysis after different heat treatments.

Thiyagarajan, P.; Li, X.; Littrell, K.; Seifert, S.; Csencsits, R.; Loong, C.

1999-12-07T23:59:59.000Z

148

Small-angle x-ray scattering studies of microvoids in amorphous silicon-based semiconductors. Annual subcontract report, 1 February 1992--31 January 1993  

DOE Green Energy (OSTI)

This report describes work to provide now details of the microstructure for the size scale from about 1 nm to 30 nm in high-quality a-Si:H and related alloys prepared by current state-of-the-art deposition methods as well as by now and emerging deposition technologies to help determine the role of microvoids and other density fluctuations in controlling the opto-electronic properties. The objectives are to determine whether the presence of microstructure as detected by small-angle X-ray scattering (SAXS) (1) limits the photovoltaic (PV) properties of device-quality a-Si:H; (2) plays a role in determine the photostability of a-Si:H; and (3) is responsible for degradation of the PV properties due to alloying with Ge, C, and other constituents. We collaborated with several groups that can supply relevant systematic sets of samples and the associated opto-electronic data to help address these issues. The project also included developing a method to standardize the procedures, minimize substrate influences, and implement improved data reduction and modeling methodology.

Williamson, D.L.; Jones, S.J.; Chen, Y. [Colorado School of Mines, Golden, CO (United States)

1994-06-01T23:59:59.000Z

149

X-ray generator  

DOE Patents (OSTI)

Apparatus and method for producing coherent secondary x-rays that are controlled as to direction by illuminating a mixture of high z and low z gases with an intense burst of primary x-rays. The primary x-rays are produced with a laser activated plasma, and these x-rays strip off the electrons of the high z atoms in the lasing medium, while the low z atoms retain their electrons. The neutral atoms transfer electrons to highly excited states of the highly striped high z ions giving an inverted population which produces the desired coherent x-rays. In one embodiment, a laser, light beam provides a laser spark that produces the intense burst of coherent x-rays that illuminates the mixture of high z and low z gases, whereby the high z atoms are stripped while the low z ones are not, giving the desired mixture of highly ionized and neutral atoms. To this end, the laser spark is produced by injecting a laser light beam, or a plurality of beams, into a first gas in a cylindrical container having an adjacent second gas layer co-axial therewith, the laser producing a plasma and the intense primary x-rays in the first gas, and the second gas containing the high and low atomic number elements for receiving the primary x-rays, whereupon the secondary x-rays are produced therein by stripping desired ions in a neutral gas and transfer of electrons to highly excited states of the stripped ions from the unionized atoms. Means for magnetically confining and stabilizing the plasma are disclosed for controlling the direction of the x-rays.

Dawson, John M. (Los Angeles, CA)

1976-01-01T23:59:59.000Z

150

X-Ray Interactions with Matter  

DOE Data Explorer (OSTI)

The primary interactions of low-energy x-rays within condensed matter, viz. photoabsorption and coherent scattering, are described for photon energies outside the absorption threshold regions by using atomic scattering factors. The atomic scattering factors may be accurately determined from the atomic photoabsorption cross sections using modified Kramers-Kronig dispersion relations. From a synthesis of the currently available experimental data and recent theoretical calculations for photoabsorption, the angle-independent, forward-scattering components of the atomic scattering factors have been thus semiempirically determined and tabulated here for 92 elements and for the region 50-30,000 eV. Atomic scattering factors for all angles of coherent scattering and at the higher photon energies are obtained from these tabulated forward-scattering values by adding a simple angle-dependent form-factor correction. The incoherent scattering contributions that become significant for the light elements at the higher photon energies are similarly determined. The basic x-ray interaction relations that are used in applied x-ray physics are presented here in terms of the atomic scattering factors. The bulk optical constants are also related to the atomic scattering factors. These atomic and optical relations are applied to the detailed calculation of the reflectivity characteristics of a series of practical x-ray mirror, multilayer, and crystal monochromators. Comparisons of the results of this semiempirical,"atom-like", description of x-ray interactions for the low-energy region with those of experiment and ab initio theory are presented. (Taken from the abstract in OSTI Record 6131765) (Specialized Interface)

Henke, B.L.; Gullikson, E.M.; Davis, J.C.

151

Gamma Radiation & X-Rays  

NLE Websites -- All DOE Office Websites (Extended Search)

Gamma Radiation and X-Rays 1. Gamma radiation and X-rays are electromagnetic radiation like visible light, radio waves, and ultraviolet light. These electromagnetic radiations...

152

Reply to Comment on X-ray resonant scattering studies of orbital and charge ordering in Pr[sub 1-x]Ca[sub x]MnO[sub 3].  

SciTech Connect

The interpretation given in our recent x-ray scattering study of Pr{sub 1-x}Ca{sub x}MnO{sub 3} in terms of charge and orbital ordering is questioned in the preceding Comment by Garcia and Subias. They argue that anisotropy of the charge distribution induced by local distortions gives rise to the so-called charge order reflections. In this Reply we suggest that the two different pictures are reconcilable.

Zimmermann, M. V.; Grenier, S.; Nelson, C. S.; Hill, J. P.; Gibbs, D.; Blume, M.; Casa, D.; Keimer, B.; Murakami, Y.; Kao, C.-C.; Venkataraman, C.; Gog, T.; Tomioka, Y.; Tokura, Y.; HASYLAB, DESY; BNL; Rutgers Univ.; Max-Planck-Institut; Tohoku Univ.; NSLS; JRCAT; Univ. of Tokyo

2003-09-01T23:59:59.000Z

153

Scattering  

NLE Websites -- All DOE Office Websites (Extended Search)

Scattering Print Scattering Print When a crystalline sample is illuminated with x-rays, the x-rays are scattered (diffracted) into very specific directions with various intensities. Detectors are used to measure this "diffraction pattern," which is then processed by computers to deduce the arrangement of atoms within the crystal. Hard x-rays have wavelengths comparable to the distance between atoms. Essentially everything we know about the atomic structure of materials is based on results from x-ray and neutron diffraction. From advanced ceramics to catalysts, from semiconductor technology to the frontiers of medicine, and from new magnetic materials and devices to framework compounds used to sequester radioactive waste, crystallography using hard x-ray diffraction techniques at synchrotron radiation facilities plays a crucial role in our ability to understand and control the world in which we live.

154

Scattering  

NLE Websites -- All DOE Office Websites (Extended Search)

Scattering Print Scattering Print When a crystalline sample is illuminated with x-rays, the x-rays are scattered (diffracted) into very specific directions with various intensities. Detectors are used to measure this "diffraction pattern," which is then processed by computers to deduce the arrangement of atoms within the crystal. Hard x-rays have wavelengths comparable to the distance between atoms. Essentially everything we know about the atomic structure of materials is based on results from x-ray and neutron diffraction. From advanced ceramics to catalysts, from semiconductor technology to the frontiers of medicine, and from new magnetic materials and devices to framework compounds used to sequester radioactive waste, crystallography using hard x-ray diffraction techniques at synchrotron radiation facilities plays a crucial role in our ability to understand and control the world in which we live.

155

Lensless X-Ray Imaging in Reflection  

NLE Websites -- All DOE Office Websites (Extended Search)

Lensless X-Ray Imaging in Lensless X-Ray Imaging in Reflection Lensless X-Ray Imaging in Reflection Print Wednesday, 26 October 2011 00:00 The advent of x-ray free-electron laser (XFEL) light sources has led to an outburst of research activities in the field of lensless imaging. XFELs combine the advantages of sychrotron light sources (high brightness and x-ray wavelengths relevant to atomic and molecular phenomena) with the advantages of visible-light lasers (highly coherent beams). All of these characteristics are important for coherent x-ray diffraction imaging-lensless imaging techniques that are proving to be integral to single-shot, high-resolution imaging of both complex materials and biological samples. Existing techniques are typically designed for transmission geometry, however, and use isolated objects, requiring special sample fabrication and restricting the type of samples under investigation. Recently, researchers from the ALS and the University of Oregon have shown at ALS Beamline 12.0.2 that it is possible to form x-ray holograms in reflection geometry by using the light scattered from a sample, opening the door to lensless imaging of a wealth of new material samples.

156

Hydrogen absorption in epitaxial W/Nb(001) and polycrystalline Fe/Nb(110) multilayers studied in-situ by X-ray/neutron scattering techniques and X-ray absorption spectroscopy  

DOE Green Energy (OSTI)

Hydrogen can be absorbed in large quantities by 100 {angstrom} thin Nb layers embedded in epitaxial W/Nb and polycrystalline Fe/Nb multilayers. The solubility and the hydrogen-induced structural changes of the host lattice are explored in-situ by small-angle neutron/X-ray reflectometry and high-angle diffraction. These measurements reveal for both systems that the relative out-of-plane expansion of the Nb layers is considerably larger than the relative increase of the Nb interplanar spacing indicating two distinctly different mechanisms of hydrogen absorption. In Fe/Nb multilayers, hydrogen expands the Nb interplanar spacing in a continuous way as function of the external pressure. In contrast, the Nb lattice expansion is discontinuous in epitaxial W/Nb multilayers: A jump in the Nb(002) Bragg reflection position occurs at a critical hydrogen pressure of 1 mbar. In-situ EXAFS spectroscopy also exhibits an irreversible expansion of the Nb lattice in the film plane for p{sub H{sub 2}}> 1 mbar. This can be regarded as a structural phase transition from an exclusively out-of-plane to a three-dimensionally expanded state at low and high hydrogen pressures, respectively.

Klose, F.; Rehm, C.; Fieber-Erdmann, M.; Holub-Krappe, E.; Bleif, H. J.; Sowers, H.; Goyette, R.; Troger, L.; Maletta, H.

1999-11-02T23:59:59.000Z

157

ERROR ESTIMATES FOR FINITE DIFFERENCE METHODS FOR A WIDE-ANGLE `PARABOLIC' EQUATION  

E-Print Network (OSTI)

ERROR ESTIMATES FOR FINITE DIFFERENCE METHODS FOR A WIDE-ANGLE `PARABOLIC' EQUATION G. D. AKRIVIS-value problem for a third-order p.d.e., a wide-angle `parabolic' equation frequently used in underwater. wide-angle `parabolic' equation, Underwater Acoustics, finite difference error esti- mates, interface

Akrivis, Georgios

158

X-ray microtomography  

SciTech Connect

In this tutorial, we describe X-ray microtomography as a technique to nondestructively characterize material microstructure in three dimensions at a micron level spatial resolution. While commercially available laboratory scale instrumentation is available, we focus our attention on synchrotron-based systems, where we can exploit a high flux, monochromatic X-ray beam to produce high fidelity three-dimensional images. A brief description of the physics and the mathematical analysis behind the technique is followed by example applications to specific materials characterization problems, with a particular focus on the utilization of three-dimensional image processing that can be used to extract a wide range of useful information.

Landis, Eric N., E-mail: landis@maine.edu [Department of Civil and Environmental Engineering, University of Maine, 5711 Boardman Hall, Orono, Maine 04469 (United States); Keane, Denis T., E-mail: dtkeane@northwestern.edu [Department of Materials Science and Engineering, Northwestern University (United States); DND-CAT, Advanced Photon Source, Argonne National Laboratory, Bldg. 432/A002, 9700 S. Cass Ave, Argonne, Illinois 60439 (United States)

2010-12-15T23:59:59.000Z

159

Nanostructure of a-Si:H and related alloys by small-angle scattering of neutrons and X-rays: Annual technical progress report: May 22, 1998 -- May 21, 1999  

DOE Green Energy (OSTI)

This report describes work being performed to provide details of the microstructure in high-quality hydrogenated amorphous silicon and related alloys on the nanometer scale. The materials under study are being prepared by state-of-the-art deposition methods, as well as by new and emerging deposition techniques. The purpose is to establish the role of nanostructural features in controlling opto-electronic and photovoltaic properties. The approach centers around the use of the uncommon technique of small-angle scattering of both X-rays (SAXS) and neutrons (SANS). SAXS has already been established as highly sensitive to microvoids and columnar-like microstructure. A major goal of this research is to establish the sensitivity of SANS to the hydrogen nanostructure. Conventional X-ray diffraction techniques are being used to examine medium-range order and microcrystallinity, particularly near the boundary between amorphous and microcrystalline material.

Williamson, D. L.

1999-12-21T23:59:59.000Z

160

Lensless X-Ray Imaging in Reflection  

NLE Websites -- All DOE Office Websites (Extended Search)

Lensless X-Ray Imaging in Reflection Print Lensless X-Ray Imaging in Reflection Print The advent of x-ray free-electron laser (XFEL) light sources has led to an outburst of research activities in the field of lensless imaging. XFELs combine the advantages of sychrotron light sources (high brightness and x-ray wavelengths relevant to atomic and molecular phenomena) with the advantages of visible-light lasers (highly coherent beams). All of these characteristics are important for coherent x-ray diffraction imaging-lensless imaging techniques that are proving to be integral to single-shot, high-resolution imaging of both complex materials and biological samples. Existing techniques are typically designed for transmission geometry, however, and use isolated objects, requiring special sample fabrication and restricting the type of samples under investigation. Recently, researchers from the ALS and the University of Oregon have shown at ALS Beamline 12.0.2 that it is possible to form x-ray holograms in reflection geometry by using the light scattered from a sample, opening the door to lensless imaging of a wealth of new material samples.

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161

Lensless X-Ray Imaging in Reflection  

NLE Websites -- All DOE Office Websites (Extended Search)

Lensless X-Ray Imaging in Reflection Print Lensless X-Ray Imaging in Reflection Print The advent of x-ray free-electron laser (XFEL) light sources has led to an outburst of research activities in the field of lensless imaging. XFELs combine the advantages of sychrotron light sources (high brightness and x-ray wavelengths relevant to atomic and molecular phenomena) with the advantages of visible-light lasers (highly coherent beams). All of these characteristics are important for coherent x-ray diffraction imaging-lensless imaging techniques that are proving to be integral to single-shot, high-resolution imaging of both complex materials and biological samples. Existing techniques are typically designed for transmission geometry, however, and use isolated objects, requiring special sample fabrication and restricting the type of samples under investigation. Recently, researchers from the ALS and the University of Oregon have shown at ALS Beamline 12.0.2 that it is possible to form x-ray holograms in reflection geometry by using the light scattered from a sample, opening the door to lensless imaging of a wealth of new material samples.

162

Lensless X-Ray Imaging in Reflection  

NLE Websites -- All DOE Office Websites (Extended Search)

X-Ray Imaging in Reflection Print X-Ray Imaging in Reflection Print The advent of x-ray free-electron laser (XFEL) light sources has led to an outburst of research activities in the field of lensless imaging. XFELs combine the advantages of sychrotron light sources (high brightness and x-ray wavelengths relevant to atomic and molecular phenomena) with the advantages of visible-light lasers (highly coherent beams). All of these characteristics are important for coherent x-ray diffraction imaging-lensless imaging techniques that are proving to be integral to single-shot, high-resolution imaging of both complex materials and biological samples. Existing techniques are typically designed for transmission geometry, however, and use isolated objects, requiring special sample fabrication and restricting the type of samples under investigation. Recently, researchers from the ALS and the University of Oregon have shown at ALS Beamline 12.0.2 that it is possible to form x-ray holograms in reflection geometry by using the light scattered from a sample, opening the door to lensless imaging of a wealth of new material samples.

163

Lensless X-Ray Imaging in Reflection  

NLE Websites -- All DOE Office Websites (Extended Search)

X-Ray Imaging in Reflection Print X-Ray Imaging in Reflection Print The advent of x-ray free-electron laser (XFEL) light sources has led to an outburst of research activities in the field of lensless imaging. XFELs combine the advantages of sychrotron light sources (high brightness and x-ray wavelengths relevant to atomic and molecular phenomena) with the advantages of visible-light lasers (highly coherent beams). All of these characteristics are important for coherent x-ray diffraction imaging-lensless imaging techniques that are proving to be integral to single-shot, high-resolution imaging of both complex materials and biological samples. Existing techniques are typically designed for transmission geometry, however, and use isolated objects, requiring special sample fabrication and restricting the type of samples under investigation. Recently, researchers from the ALS and the University of Oregon have shown at ALS Beamline 12.0.2 that it is possible to form x-ray holograms in reflection geometry by using the light scattered from a sample, opening the door to lensless imaging of a wealth of new material samples.

164

Compton backscattered collimated x-ray source  

SciTech Connect

A high-intensity, inexpensive and collimated x-ray source for applications such as x-ray lithography is disclosed. An intense pulse from a high power laser, stored in a high-finesse resonator, repetitively collides nearly head-on with and Compton backscatters off a bunched electron beam, having relatively low energy and circulating in a compact storage ring. Both the laser and the electron beams are tightly focused and matched at the interaction region inside the optical resonator. The laser-electron interaction not only gives rise to x-rays at the desired wavelength, but also cools and stabilizes the electrons against intrabeam scattering and Coulomb repulsion with each other in the storage ring. This cooling provides a compact, intense bunch of electrons suitable for many applications. In particular, a sufficient amount of x-rays can be generated by this device to make it an excellent and flexible Compton backscattered x-ray (CBX) source for high throughput x-ray lithography and many other applications.

Ruth, Ronald D. (Woodside, CA); Huang, Zhirong (Stanford, CA)

1998-01-01T23:59:59.000Z

165

Compton backscattered collmated X-ray source  

SciTech Connect

A high-intensity, inexpensive and collimated x-ray source for applications such as x-ray lithography is disclosed. An intense pulse from a high power laser, stored in a high-finesse resonator, repetitively collides nearly head-on with and Compton backscatters off a bunched electron beam, having relatively low energy and circulating in a compact storage ring. Both the laser and the electron beams are tightly focused and matched at the interaction region inside the optical resonator. The laser-electron interaction not only gives rise to x-rays at the desired wavelength, but also cools and stabilizes the electrons against intrabeam scattering and Coulomb repulsion with each other in the storage ring. This cooling provides a compact, intense bunch of electrons suitable for many applications. In particular, a sufficient amount of x-rays can be generated by this device to make it an excellent and flexible Compton backscattered x-ray (CBX) source for high throughput x-ray lithography and many other applications.

Ruth, Ronald D. (Woodside, CA); Huang, Zhirong (Stanford, CA)

2000-01-01T23:59:59.000Z

166

APS 7-BM Beamline: X-Ray Resources  

NLE Websites -- All DOE Office Websites (Extended Search)

Useful Websites Useful Websites X-Ray Interactions with Matter from CRXO at LBNL. Intuitive interface for x-ray transmission and reflectivity for a wide range of materials. X-Ray Data Booklet from LBNL. Slightly outdated in places, but many useful tables of edge energies, fluorescence lines, and crystal lattice spacings. NIST XCOM Database. Powerful database of photoelectric absorption, elastic scattering, and Compton scattering cross-sections for a wide range of materials. X-Ray Server. Maintained by Sergey Stepanov at GMCA at the APS, this website has several powerful calculators for simulating x-ray reflection and diffraction. Software X-Ray Oriented Programs (XOP). This program, written by scientists at the ESRF and APS, is widely used in the synchrotron research community.

167

X-Ray and Neutron Diffraction  

Science Conference Proceedings (OSTI)

Oct 20, 2010 ... Advanced X-Ray Scattering Techniques for Multi-Length Scale ... ?-Ti using the 3DXRD station 34-ID-E at the Advanced Photon Source, Argonne National Laboratory. ... Research at APS 34-ID-E, partly funded by BES/DOE.

168

X-ray Science Division: Groups  

NLE Websites -- All DOE Office Websites (Extended Search)

Division: Groups Division: Groups Atomic, Molecular and Optical Physics (AMO) Primary Contact: Stephen Southworth Work focuses on understanding how strong optical and x-ray fields interact with matter, with an emphasis on photonic control of electronic, atomic and molecular motion. Chemical and Materials Science (CMS) Primary Contact: Randy Winans Research Disciplines: Chemistry, Materials Science Detectors (DET) Primary Contact: Antonino Miceli GMCA Structural Biology Facility (MX) Primary Contact: Robert Fischetti Research Disciplines: Biology, Life Sciences Imaging (IMG) Primary Contact: Francesco DeCarlo Research Disciplines: Materials Science, Biology, Physics, Life Sciences Inelastic X-ray & Nuclear Resonant Scattering (IXN) Primary Contact: Thomas Gog Research Disciplines: Condensed Matter Physics, Geophysics, Materials

169

X-ray Security Screening  

Science Conference Proceedings (OSTI)

National and International Standards for X-ray Security Screening Applications. Summary: The primary objective of this ...

2013-03-13T23:59:59.000Z

170

X-Ray Diffraction Microscopy of Magnetic Structures  

NLE Websites -- All DOE Office Websites (Extended Search)

X-Ray Diffraction Microscopy of Magnetic Structures Print X-Ray Diffraction Microscopy of Magnetic Structures Print science brief icon Scientists working at ALS Beamline 12.0.2.2 have demonstrated a new x-ray technique for producing short-exposure nanoscale images of the magnetic structure of materials. The new method combines aspects of coherent x-ray diffraction, which can determine 3-D charge distributions, and resonant magnetic scattering, which is sensitive to magnetic structures. Physicists have used coherent x-ray diffraction to measure the electron density of complicated molecules. The formula used to make these calculations contains terms that relate to the electron spin of magnetic atoms, but these terms are traditionally ignored since coherent x-ray diffraction has not been used to retrieve magnetic information. Using the full formula allows for the determination of not only the electron density, but also the magnetic spin distribution and its orientation.

171

X-Ray Diffraction Microscopy of Magnetic Structures  

NLE Websites -- All DOE Office Websites (Extended Search)

X-Ray Diffraction Microscopy of Magnetic Structures Print X-Ray Diffraction Microscopy of Magnetic Structures Print science brief icon Scientists working at ALS Beamline 12.0.2.2 have demonstrated a new x-ray technique for producing short-exposure nanoscale images of the magnetic structure of materials. The new method combines aspects of coherent x-ray diffraction, which can determine 3-D charge distributions, and resonant magnetic scattering, which is sensitive to magnetic structures. Physicists have used coherent x-ray diffraction to measure the electron density of complicated molecules. The formula used to make these calculations contains terms that relate to the electron spin of magnetic atoms, but these terms are traditionally ignored since coherent x-ray diffraction has not been used to retrieve magnetic information. Using the full formula allows for the determination of not only the electron density, but also the magnetic spin distribution and its orientation.

172

X-Ray Diffraction Microscopy of Magnetic Structures  

NLE Websites -- All DOE Office Websites (Extended Search)

X-Ray Diffraction Microscopy of Magnetic Structures Print X-Ray Diffraction Microscopy of Magnetic Structures Print science brief icon Scientists working at ALS Beamline 12.0.2.2 have demonstrated a new x-ray technique for producing short-exposure nanoscale images of the magnetic structure of materials. The new method combines aspects of coherent x-ray diffraction, which can determine 3-D charge distributions, and resonant magnetic scattering, which is sensitive to magnetic structures. Physicists have used coherent x-ray diffraction to measure the electron density of complicated molecules. The formula used to make these calculations contains terms that relate to the electron spin of magnetic atoms, but these terms are traditionally ignored since coherent x-ray diffraction has not been used to retrieve magnetic information. Using the full formula allows for the determination of not only the electron density, but also the magnetic spin distribution and its orientation.

173

Scanning x-ray microscope  

Science Conference Proceedings (OSTI)

A scanning x-ray microscope is described including: an x-ray source capable of emitting a beam of x-rays; a collimator positioned to receive the beam of x-rays and to collimate this beam, a focusing cone means to focus the beam of x-rays, directed by the collimator, onto a focal plane, a specimen mount for supporting a specimen in the focal plane to receive the focused beam of x-rays, and x-ray beam scanning means to relatively move the specimen and the focusing cone means and collimator to scan the focused x-ray beam across the specimen. A detector is disposed adjacent the specimen to detect flourescent photons emitted by the specimen upon exposure to the focused beam of x-rays to provide an electrical output representative of this detection. Means are included for displaying and/or recording the information provided by the output from the detector, as are means for providing information to the recording and/or display means representative of the scan rate and position of the focused x-ray beam relative to the specimen whereby the recording and/or display means can correlate the information received to record and/or display quantitive and distributive information as to the quantity and distribution of elements detected in the specimen. Preferably there is provided an x-ray beam modulation means upstream, relative to the direction of emission of the xray beam, of the focusing cone means.

Wang, C.

1982-02-23T23:59:59.000Z

174

X-ray lithography source  

SciTech Connect

A high-intensity, inexpensive X-ray source for X-ray lithography for the production of integrated circuits. Foil stacks are bombarded with a high-energy electron beam of 25 to 250 MeV to produce a flux of soft X-rays of 500 eV to 3 keV. Methods of increasing the total X-ray power and making the cross section of the X-ray beam uniform are described. Methods of obtaining the desired X-ray-beam field size, optimum frequency spectrum and elminating the neutron flux are all described. A method of obtaining a plurality of station operation is also described which makes the process more efficient and economical. The satisfying of these issues makes transition radiation an exellent moderate-priced X-ray source for lithography.

Piestrup, Melvin A. (Woodside, CA); Boyers, David G. (Mountain View, CA); Pincus, Cary (Sunnyvale, CA)

1991-01-01T23:59:59.000Z

175

X-ray lithography source  

DOE Patents (OSTI)

A high-intensity, inexpensive X-ray source for X-ray lithography for the production of integrated circuits is disclosed. Foil stacks are bombarded with a high-energy electron beam of 25 to 250 MeV to produce a flux of soft X-rays of 500 eV to 3 keV. Methods of increasing the total X-ray power and making the cross section of the X-ray beam uniform are described. Methods of obtaining the desired X-ray-beam field size, optimum frequency spectrum and eliminating the neutron flux are all described. A method of obtaining a plurality of station operation is also described which makes the process more efficient and economical. The satisfying of these issues makes transition radiation an excellent moderate-priced X-ray source for lithography. 26 figures.

Piestrup, M.A.; Boyers, D.G.; Pincus, C.

1991-12-31T23:59:59.000Z

176

Miniature x-ray source  

DOE Patents (OSTI)

A miniature x-ray source capable of producing broad spectrum x-ray emission over a wide range of x-ray energies. The miniature x-ray source comprises a compact vacuum tube assembly containing a cathode, an anode, a high voltage feedthru for delivering high voltage to the anode, a getter for maintaining high vacuum, a connection for an initial vacuum pump down and crimp-off, and a high voltage connection for attaching a compact high voltage cable to the high voltage feedthru. At least a portion of the vacuum tube wall is highly x-ray transparent and made, for example, from boron nitride. The compact size and potential for remote operation allows the x-ray source, for example, to be placed adjacent to a material sample undergoing analysis or in proximity to the region to be treated for medical applications.

Trebes, James E. (Livermore, CA); Stone, Gary F. (Livermore, CA); Bell, Perry M. (Tracy, CA); Robinson, Ronald B. (Modesto, CA); Chornenky, Victor I. (Minnetonka, MN)

2002-01-01T23:59:59.000Z

177

Synchrotron X-ray Measurements  

Science Conference Proceedings (OSTI)

... fine structure (EXAFS) spectroscopy; (3) variable kinetic energy X-ray ... advanced materials is critical to the development and optimization of products ...

2012-10-04T23:59:59.000Z

178

X-ray Absorption Spectroscopy  

SciTech Connect

This review gives a brief description of the theory and application of X-ray absorption spectroscopy, both X-ray absorption near edge structure (XANES) and extended X-ray absorption fine structure (EXAFS), especially, pertaining to photosynthesis. The advantages and limitations of the methods are discussed. Recent advances in extended EXAFS and polarized EXAFS using oriented membranes and single crystals are explained. Developments in theory in understanding the XANES spectra are described. The application of X-ray absorption spectroscopy to the study of the Mn4Ca cluster in Photosystem II is presented.

Yano, Junko; Yachandra, Vittal K.

2009-07-09T23:59:59.000Z

179

Synchrotron x-ray sources and new opportunities in the soil and environmental sciences  

Science Conference Proceedings (OSTI)

This report contains the following papers: characteristics of the advanced photon source and comparison with existing synchrotron facilities; x-ray absorption spectroscopy: EXAFS and XANES -- A versatile tool to study the atomic and electronic structure of materials; applications of x-ray spectroscopy and anomalous scattering experiments in the soil and environmental sciences; X-ray fluorescence microprobe and microtomography.

Schulze, D. (Purdue Univ., Lafayette, IN (USA)); Anderson, S. (Michigan State Univ., East Lansing, MI (USA)); Mattigod, S. (Pacific Northwest Lab., Richland, WA (USA))

1990-07-01T23:59:59.000Z

180

Changes in delta-Plutonium due to self-irradiation aging observed by Continuous in-situ X-ray Scattering  

Science Conference Proceedings (OSTI)

The aging in plutonium is predominantly caused by its internal self-irradiation. The self-irradiation in Pu-239 is by the decay process of transmuting the Pu atom into uranium atom and emitting an {alpha}-particle. Most of the lattice damage comes from the uranium recoil resulting in Frenkel-type defects consisting of vacancies and self-interstitial atoms, helium in-growth and defect clusters and possibly even though it is not yet observed, the generation of voids. As part of the stockpile stewardship, it is important to understand the changes in the structure and microstructures and their correlations to the physical properties. Changes in the physical properties have a direct relationship to the quality of the structure, in terms of formation of defects and defect clustering, accumulation of voids, grain boundaries, phase changes and etc. which can adversely affect the stability of the material. These changes are very difficult to monitor because of the high activity of the sample, high atomic number making x-ray and synchrotron probe into the bulk very difficult (neutron probe is not feasible) and the long life time which normally requires decades to measure. In this paper we describe the development of an in-situ in-house transmission x-ray diffraction (XRD) experimental technique used to monitor the structural changes in these materials. This technique calls for a very thin sample of less that 2 mm and to accelerate the aging process due to self-irradiation, spiked alloy of 7.5 weight percent of Pu-238 is used. This is equivalent to roughly 17 times the normal rate of aging. Current results suggest that over a period of 2.8 equivalent years, an increase of 0.5% in unit cell parameter is observed. The increase appears to be an abrupt jump at about 1.1 equivalent years, brought about by the collapsing of the atoms from the interstitials to the lattice sites. Further data analysis is on the way.

Saw, C K; Chung, B W; Wall, M A

2007-01-05T23:59:59.000Z

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


181

DISCRETE TRANSPARENT BOUNDARY CONDITIONS FOR WIDE ANGLE PARABOLIC EQUATIONS IN UNDERWATER  

E-Print Network (OSTI)

DISCRETE TRANSPARENT BOUNDARY CONDITIONS FOR WIDE ANGLE PARABOLIC EQUATIONS IN UNDERWATER ACOUSTICS "parabolic" equations (WAPEs) in underwater acoustics (assuming cylindrical symmetry). Existing the discretization of transparent bottom boundary conditions. In oceanography one wants to calculate the underwater

Ehrhardt, Matthias

182

Grazing Incidence Small-Angle X-Ray Scattering Studies of the Synthesis and Growth of CdS Quantum Dots from Constituent Atoms in SiO2 Matrix  

Science Conference Proceedings (OSTI)

Grazing incidence small angle X-ray scattering was applied to study the synthesis and growth of CdS quantum dots (QDs) from Cd and S atoms implanted in SiO{sub 2}. For a dose of 10{sup 17}/cm{sup 2}, the partial synthesis of CdS QDs occurred already during implantation, with only moderate size increase upon subsequent annealing up to T{sub a} = 1073 K. The dynamics of QD synthesis and growth were considerably different for just two times lower dose, where synthesis started only if the implanted samples were annealed at T{sub a} = 773 K or higher, with a strong increase of the size of QDs upon annealing at higher T{sub a}. The results suggest that high-dose implantation followed by low-temperature annealing could lead to better defined sizes and narrower size distributions of QDs.

Desnica, U. V. [R. Boskovic Institute, Zagreb, Croatia; Dubcek, P. [R. Boskovic Institute, Zagreb, Croatia; Desnica-Frankovic, I. D. [R. Boskovic Institute, Zagreb, Croatia; Buljan, M. [R. Boskovic Institute, Zagreb, Croatia; Bernstorff, S. [Sincrotrone Trieste, Basovizza, Italy; White, Clark W [ORNL

2003-01-01T23:59:59.000Z

183

X-ray diffuse scattering measurements of chemical short-range order and lattice strains in a highly magnetostrictive Fe0.813Ga0.187 alloy in an applied magnetic field  

SciTech Connect

The rapid growth of the magnetostriction coefficient of ferromagnetic Fe1?xGax alloys that occurs at a composition range from 0X-ray diffuse scattering measurements sensitive to the atomic short-range ordering and lattice strain were performed on a quenched 18.7 at. % Ga alloy and show no dependence on the application of a magnetic field. This negative result sets limits on the role of nanoscale precipitates in magnetostriction.

Du, Yingzhou; Lograsso, Thomas A.; McQueeney, Robert J.

2012-06-28T23:59:59.000Z

184

Structural characterization of Green River oil-shale at high-pressure using pair distribution function analysis and small angle x-ray scattering.  

Science Conference Proceedings (OSTI)

The compression behavior of a silicate-rich oil shale from the Green River formation in the pressure range 0.0-2.4 GPa was studied using in situ high pressure X-ray pair distribution function (PDF) measurements for the sample contained within a Paris-Edinburgh cell. The real-space local structural information in the PDF, G(r), was used to evaluate the compressibility of the oil shale. Specifically, the pressure-induced reduction in the medium- to long-range atom distances (6-20 {angstrom}) yielded an average sample compressibility corresponding to a bulk modulus of ca. 61-67 GPa. A structural model consisting of a three phase mixture of the principal crystalline oil shale components (quartz, albite and Illite) provided a good fit to the ambient pressure PDF data (R 30.7%). Indeed the features in the PDF beyond 6 {angstrom}, were similarly well fit by a single phase model of the highest symmetry, highly crystalline quartz component.

Locke, D. R.; Chupas, P. J.; Chapman, K. W.; Pugmire, R. J.; Winans, R. E.; Univ. of Utah

2008-01-01T23:59:59.000Z

185

A highly modular beamline electrostatic levitation facility, optimized for in situ high-energy x-ray scattering studies of equilibrium and supercooled liquids  

Science Conference Proceedings (OSTI)

High-energy x-ray diffraction studies of metallic liquids provide valuable information about structural evolution on the atomic length scale, leading to insights into the origin of the nucleation barrier and the processes of supercooling and glass formation. The containerless processing of the beamline electrostatic levitation (BESL) facility allows coordinated thermophysical and structural studies of equilibrium and supercooled liquids to be made in a contamination-free, high-vacuum ({approx}10{sup -8} Torr) environment. To date, the incorporation of electrostatic levitation facilities into synchrotron beamlines has been difficult due to the large footprint of the apparatus and the difficulties associated with its transportation and implementation. Here, we describe a modular levitation facility that is optimized for diffraction studies of high-temperature liquids at high-energy synchrotron beamlines. The modular approach used in the apparatus design allows it to be easily transported and quickly setup. Unlike most previous electrostatic levitation facilities, BESL can be operated by a single user instead of a user team.

Mauro, N.A.; Kelton, K.F. (WU)

2011-10-27T23:59:59.000Z

186

High-Energy X-ray Studies of Real Materials Under Real Conditions and in Real Time  

SciTech Connect

High-energy x-rays from 3rd generation synchrotron sources, including the APS, possess a unique combination of high penetration power and high spatial, reciprocal space, and temporal resolution. These characteristics can be exploited to non-destructively measure phase, texture and strain distributions under extreme environments including thermo-mechanical loading, high-pressure, irradiation and supercritical environments. Over the past several years, the 1-ID beamline has developed a number of programs for these purposes, namely (i) high-energy diffraction microscopy, in which grain and sub-grain volumes are mapped in polycrystalline aggregates, and (ii) combined small-and wide-angle x-ray scattering which permits information over a broad range of length scales to be collected from the same (micron-level) volume. These programs have been increasingly used to test and extend predictive simulations of materials behavior over size scales ranging from nm to mm. Select studies will be presented including nucleation and growth of nanomaterials, void and structural evolution in complex composites under thermo-mechanical and irradiated environments, and microstructural changes in layered systems including thermal-barrier coatings, batteries and fuel cells. Finally, extension of these programs, through the planned APS upgrade, to higher spatio-temporal resolution will be described.

Almer, Jonathan (ANL)

2011-05-11T23:59:59.000Z

187

X-ray Imaging Workshop  

NLE Websites -- All DOE Office Websites (Extended Search)

Imaging and Spectro-microscopy: Imaging and Spectro-microscopy: the Present and the Future Stanford Synchrotron Radiation Laboratory October 8-9, 2002 Organizers: John Miao & Keith Hodgson A workshop on "X-ray Imaging and Spectro-microscopy: the Present and the Future" was held on October 8-9, 2002. This workshop, organized by John Miao (SSRL) and Keith Hodgson (SSRL) provided a forum to discuss the scientific applications of a variety of imaging and spectro-microscopic techniques, including photoemission electron microscopy (PEEM), angle resolved photoemission spectroscopy (ARPES), coherent diffraction imaging, x-ray microscopy, micro-tomography, holographic imaging, and x-ray micro-probe. Twelve invited speakers discussed the important scientific applications of these techniques, and also predicted the future scientific directions with the advance of instrumentation and x-ray sources. The workshop was well attended with over fifty registered attendees.

188

Miniature x-ray source  

DOE Patents (OSTI)

A miniature x-ray source utilizing a hot filament cathode. The source has a millimeter scale size and is capable of producing broad spectrum x-ray emission over a wide range of x-ray energies. The miniature source consists of a compact vacuum tube assembly containing the hot filament cathode, an anode, a high voltage feedthru for delivering high voltage to the cathode, a getter for maintaining high vacuum, a connector for initial vacuum pump down and crimp-off, and a high voltage connection for attaching a compact high voltage cable to the high voltage feedthru. At least a portion of the vacuum tube wall is fabricated from highly x-ray transparent materials, such as sapphire, diamond, or boron nitride.

Trebes, James E. (Livermore, CA); Bell, Perry M. (Tracy, CA); Robinson, Ronald B. (Modesto, CA)

2000-01-01T23:59:59.000Z

189

Method and apparatus for molecular imaging using X-rays at resonance wavelengths  

DOE Patents (OSTI)

Holographic X-ray images are produced representing the molecular structure of a microscopic object, such as a living cell, by directing a beam of coherent X-rays upon the object to produce scattering of the X-rays by the object, producing interference on a recording medium between the scattered X-rays from the object and unscattered coherent X-rays and thereby producing holograms on the recording surface, and establishing the wavelength of the coherent X-rays to correspond with a molecular resonance of a constituent of such object and thereby greatly improving the contrast, sensitivity and resolution of the holograms as representations of molecular structures involving such constituent. For example, the coherent X-rays may be adjusted to the molecular resonant absorption line of nitrogen at about 401.3 eV to produce holographic images featuring molecular structures involving nitrogen.

Chapline, Jr., George F. (Alamo, CA)

1985-01-01T23:59:59.000Z

190

Tokamak x ray diagnostic instrumentation  

SciTech Connect

Three classes of x-ray diagnostic instruments enable measurement of a variety of tokamak physics parameters from different features of the x-ray emission spectrum. (1) The soft x-ray (1 to 50 keV) pulse-height-analysis (PHA) diagnostic measures impurity concentrations from characteristic line intensities and the continuum enhancement, and measures the electron temperature from the continuum slope. (2) The Bragg x-ray crystal spectrometer (XCS) measures the ion temperature and neutral-beam-induced toroidal rotation velocity from the Doppler broadening and wavelength shift, respectively, of spectral lines of medium-Z impurity ions. Impurity charge state distributions, precise wavelengths, and inner-shell excitation and recombination rates can also be studied. X rays are diffracted and focused by a bent crystal onto a position-sensitive detector. The spectral resolving power E/..delta..E is greater than 10/sup 4/ and time resolution is 10 ms. (3) The x-ray imaging system (XIS) measures the spatial structure of rapid fluctuations (0.1 to 100 kHZ) providing information on MHD phenomena, impurity transport rates, toroidal rotation velocity, plasma position, and the electron temperature profile. It uses an array of silicon surface-barrier diodes which view different chords of the plasma through a common slot aperture and operate in current (as opposed to counting) mode. The effectiveness of shields to protect detectors from fusion-neutron radiation effects has been studied both theoretically and experimentally.

Hill, K.W.; Beiersdorfer, P.; Bitter, M.; Fredrickson, E.; Von Goeler, S.; Hsuan, H.; Johnson, L.C.; Liew, S.L.; McGuire, K.; Pare, V.

1987-01-01T23:59:59.000Z

191

X-ray Transition Energies Search Form  

Science Conference Proceedings (OSTI)

[skip navigation] X-ray Transition Energies Database Main Page Search for X-ray transition energies by element(s), transition ...

192

Femtosecond Time-Delay X-ray Holography  

NLE Websites -- All DOE Office Websites (Extended Search)

Time-Delay X-ray Holography Time-Delay X-ray Holography X-ray free-electron lasers (XFELs) will produce photon pulses with a unique and desirable combination of properties. Their short X-ray wavelengths allow penetration into materials and the ability to probe structure at and below the nanometer scale. Their ultra-short duration gives information about this structure at the fundamental time-scales of atoms and molecules. The extreme intensity of the pulses will allow this information to be acquired in a single shot, so that these studies can be carried out on non-repeatable processes or on weakly-scattering objects that will be modified by the pulse. A fourth property of XFEL pulses is their high transverse coherence, which brings the promise of decades of innovation in visible optics to the X-ray regime, such as holography, interferometry, and laser-based imaging. Making an effective use of XFEL pulses, however, will benefit from innovations that are new to both X-ray science and coherent optics. One such innovation is the new method of time-delay X-ray holography [i], recently demonstrated at the FLASH FEL at DESY in Hamburg, to measure the evolution of objects irradiated by intense pulses.

193

Compact x-ray source and panel  

SciTech Connect

A compact, self-contained x-ray source, and a compact x-ray source panel having a plurality of such x-ray sources arranged in a preferably broad-area pixelized array. Each x-ray source includes an electron source for producing an electron beam, an x-ray conversion target, and a multilayer insulator separating the electron source and the x-ray conversion target from each other. The multi-layer insulator preferably has a cylindrical configuration with a plurality of alternating insulator and conductor layers surrounding an acceleration channel leading from the electron source to the x-ray conversion target. A power source is connected to each x-ray source of the array to produce an accelerating gradient between the electron source and x-ray conversion target in any one or more of the x-ray sources independent of other x-ray sources in the array, so as to accelerate an electron beam towards the x-ray conversion target. The multilayer insulator enables relatively short separation distances between the electron source and the x-ray conversion target so that a thin panel is possible for compactness. This is due to the ability of the plurality of alternating insulator and conductor layers of the multilayer insulators to resist surface flashover when sufficiently high acceleration energies necessary for x-ray generation are supplied by the power source to the x-ray sources.

Sampayon, Stephen E. (Manteca, CA)

2008-02-12T23:59:59.000Z

194

X-ray emission from colliding laser plasmas  

SciTech Connect

Colliding Au, CD and Ti-Cr plasmas have been generated by illuminating two opposing foils each with a {approximately} 100J, 0.5 nsec, 2{omega} Nd-glass laser beam from the Trident laser facility at Los Alamos. The plasmas are being used to study plasma interactions which span the parameter regime from interpenetrating to collisional stagnation. X-ray emission during the laser target interaction and the subsequent collision is used to diagnose the initial plasma conditions and the colliding plasma properties. X-ray instrumentation consists of a 100 ps gated x-ray pinhole imager, a time-integratcd bremsstrahlung x-ray spectrograph and a gated x-ray spectrograph used to record isoelectronic spectra from the Ti-Cr plasmas. The imager has obtained multi-frame images of the collision and therefore, a measure of the stagnation length which is a function of the ion charge state and density and a strong function of the electron temperature. Other instrumentation includes a Thomson scattering spectrometer with probe beam, neutron detectors used to monitor the CD coated foil collisions and an ion spectrometer. We will describe the current status of the experiments and current results with emphasis on the x-ray emission diagnostics. We will also briefly describe the modeling using Lasnex and ISIS, a particle-in-cell code with massless fluid electrons and inter particle (classical) collisions.

Wilke, M.; Obst, A.W.; Winske, D. [and others

1995-09-01T23:59:59.000Z

195

A multi-crystal wavelength dispersive x-ray spectrometer  

Science Conference Proceedings (OSTI)

A multi-crystal wavelength dispersive hard x-ray spectrometer with high-energy resolution and large solid angle collection is described. The instrument is specifically designed for time-resolved applications of x-ray emission spectroscopy (XES) and x-ray Raman scattering (XRS) at X-ray Free Electron Lasers (XFEL) and synchrotron radiation facilities. It also simplifies resonant inelastic x-ray scattering (RIXS) studies of the whole 2d RIXS plane. The spectrometer is based on the Von Hamos geometry. This dispersive setup enables an XES or XRS spectrum to be measured in a single-shot mode, overcoming the scanning needs of the Rowland circle spectrometers. In conjunction with the XFEL temporal profile and high-flux, it is a powerful tool for studying the dynamics of time-dependent systems. Photo-induced processes and fast catalytic reaction kinetics, ranging from femtoseconds to milliseconds, will be resolvable in a wide array of systems circumventing radiation damage.

Alonso-Mori, Roberto; Montanez, Paul; Delor, James; Bergmann, Uwe [LCLS, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Kern, Jan [LCLS, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Physical Biosciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720-8099 (United States); Sokaras, Dimosthenis; Weng, Tsu-Chien; Nordlund, Dennis [SSRL, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Tran, Rosalie; Yachandra, Vittal K.; Yano, Junko [Physical Biosciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720-8099 (United States)

2012-07-15T23:59:59.000Z

196

Microgap x-ray detector  

DOE Patents (OSTI)

An x-ray detector which provides for the conversion of x-ray photons into photoelectrons and subsequent amplification of these photoelectrons through the generation of electron avalanches in a thin gas-filled region subject to a high electric potential. The detector comprises a cathode (photocathode) and an anode separated by the thin, gas-filled region. The cathode may comprise a substrate, such a beryllium, coated with a layer of high atomic number material, such as gold, while the anode can be a single conducting plane of material, such as gold, or a plane of resistive material, such as chromium/silicon monoxide, or multiple areas of conductive or resistive material, mounted on a substrate composed of glass, plastic or ceramic. The charge collected from each electron avalanche by the anode is passed through processing electronics to a point of use, such as an oscilloscope.

Wuest, Craig R. (Danville, CA); Bionta, Richard M. (Livermore, CA); Ables, Elden (Livermore, CA)

1994-01-01T23:59:59.000Z

197

Chest x-Rays | Department of Energy  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

Chest x-Rays Chest x-Rays Chest x-Rays Chest X-ray B-Reading The B-reading is a special reading of a standard chest x-ray film performed by a physician certified by the National Institute for Occupational Safety and Health (NIOSH). The reading looks for changes on the chest x-ray that may indicate exposure and disease caused by agents such as asbestos or silica. The B-reading is considered a special reading because doctors who are certified by NIOSH to perform B-readings use a specific protocol to read and record the findings as developed by the International Labour Organization (ILO). The ILO's protocol provides rules for systematically examining the x-ray in a step-by-step method and recording certain abnormalities or changes on the chest x-ray that can be attributable to

198

Spectral analysis of X-ray binaries  

E-Print Network (OSTI)

In this thesis, I present work from three separate research projects associated with observations of X-ray binaries. Two of those revolve around spectral characteristics of neutron star low-mass X-ray binaries (NS-LMXBs), ...

Fridriksson, Joel Karl

2011-01-01T23:59:59.000Z

199

Cryotomography x-ray microscopy state  

Science Conference Proceedings (OSTI)

An x-ray microscope stage enables alignment of a sample about a rotation axis to enable three dimensional tomographic imaging of the sample using an x-ray microscope. A heat exchanger assembly provides cooled gas to a sample during x-ray microscopic imaging.

Le Gros, Mark (Berkeley, CA); Larabell, Carolyn A. (Berkeley, CA)

2010-10-26T23:59:59.000Z

200

Concept development for the ITER equatorial port visible/infrared wide angle viewing system  

Science Conference Proceedings (OSTI)

The ITER equatorial port visible/infrared wide angle viewing system concept is developed from the measurement requirements. The proposed solution situates 4 viewing systems in the equatorial ports 3, 9, 12, and 17 with 4 views each (looking at the upper target, the inner divertor, and tangentially left and right). This gives sufficient coverage. The spatial resolution of the divertor system is 2 times higher than the other views. For compensation of vacuum-vessel movements, an optical hinge concept is proposed. Compactness and low neutron streaming is achieved by orienting port plug doglegs horizontally. Calibration methods, risks, and R and D topics are outlined.

Reichle, R.; Beaumont, B.; Boilson, D.; Bouhamou, R.; Direz, M.-F.; Encheva, A.; Henderson, M.; Kazarian, F.; Lamalle, Ph.; Lisgo, S.; Mitteau, R.; Patel, K. M.; Pitcher, C. S.; Pitts, R. A.; Prakash, A.; Raffray, R.; Schunke, B.; Snipes, J.; Diaz, A. Suarez; Udintsev, V. S. [ITER Organization, Route de Vinon-sur-Verdon, 13115 St Paul-lez-Durance (France); and others

2012-10-15T23:59:59.000Z

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


201

X-ray transmissive debris shield  

DOE Patents (OSTI)

An X-ray debris shield for use in X-ray lithography that is comprised of an X-ray window having a layer of low density foam exhibits increased longevity without a substantial increase in exposure time. The low density foam layer serves to absorb the debris emitted from the X-ray source and attenuate the shock to the window so as to reduce the chance of breakage. Because the foam is low density, the X-rays are hardly attenuated by the foam and thus the exposure time is not substantially increased.

Spielman, R.B.

1996-05-21T23:59:59.000Z

202

X-ray transmissive debris shield  

DOE Patents (OSTI)

An X-ray debris shield for use in X-ray lithography that is comprised of an X-ray window having a layer of low density foam exhibits increased longevity without a substantial increase in exposure time. The low density foam layer serves to absorb the debris emitted from the X-ray source and attenuate the shock to the window so as to reduce the chance of breakage. Because the foam is low density, the X-rays are hardly attenuated by the foam and thus the exposure time is not substantially increased.

Spielman, Rick B. (Albuquerque, NM)

1996-01-01T23:59:59.000Z

203

Graded index and randomly oriented core-shell silicon nanowires with broadband and wide angle antireflection for photovoltaic cell applications  

E-Print Network (OSTI)

Antireflection with broadband and wide angle properties is important for a wide range of applications on photovoltaic cells and display. The SiOx shell layer provides a natural antireflection from air to the Si core absorption layer. In this work, we have demonstrated the random core-shell silicon nanowires with both broadband (from 400nm to 900nm) and wide angle (from normal incidence to 60\\degree) antireflection characteristics within AM1.5 solar spectrum. The graded index structure from the randomly oriented core-shell (Air/SiOx/Si) nanowires may provide a potential avenue to realize a broadband and wide angle antireflection layer.

Pignalosa, P; Qiao, L; Tseng, M; Yi, Yasha

2011-01-01T23:59:59.000Z

204

Directional x-ray dark-field imaging of strongly ordered systems  

Science Conference Proceedings (OSTI)

Recently a novel grating based x-ray imaging approach called directional x-ray dark-field imaging was introduced. Directional x-ray dark-field imaging yields information about the local texture of structures smaller than the pixel size of the imaging system. In this work we extend the theoretical description and data processing schemes for directional dark-field imaging to strongly scattering systems, which could not be described previously. We develop a simple scattering model to account for these recent observations and subsequently demonstrate the model using experimental data. The experimental data includes directional dark-field images of polypropylene fibers and a human tooth slice.

Jensen, Torben Haugaard; Feidenhans'l, Robert [Niels Bohr Institute, University of Copenhagen, 2100 Copenhagen (Denmark); Bech, Martin; Pfeiffer, Franz [Department of Physics, Technical University of Munich, 85747 Garching (Germany); Zanette, Irene; Weitkamp, Timm [European Synchrotron Radiation Facility, 38043 Grenoble (France); David, Christian; Rutishauser, Simon [Paul Scherrer Institut, 5232 Villigen PSI (Switzerland); Deyhle, Hans [Biomaterials Science Center, University of Basel, 4031 Basel (Switzerland); Institute for Materials Science, School of Dental Medicine, University of Basel, 4031 Basel (Switzerland); Reznikova, Elena; Mohr, Juergen [Karlsruhe Institute of Technology, Institute for Microstructure Technology, 76021 Karlsruhe (Germany)

2010-12-01T23:59:59.000Z

205

Modeling of the ITER-like wide-angle infrared thermography view of JET  

SciTech Connect

Infrared (IR) thermography systems are mandatory to ensure safe plasma operation in fusion devices. However, IR measurements are made much more complicated in metallic environment because of the spurious contributions of the reflected fluxes. This paper presents a full predictive photonic simulation able to assess accurately the surface temperature measurement with classical IR thermography from a given plasma scenario and by taking into account the optical properties of PFCs materials. This simulation has been carried out the ITER-like wide angle infrared camera view of JET in comparing with experimental data. The consequences and the effects of the low emissivity and the bidirectional reflectivity distribution function used in the model for the metallic PFCs on the contribution of the reflected flux in the analysis are discussed.

Aumeunier, M.-H. [CEA, IRFM, F-13108 Saint-Paul-Lez-Durance (France); OPTIS, ZE de La Farlede, F-83078 Toulon Cedex 9 (France); Firdaouss, M.; Travere, J.-M.; Loarer, T.; Gauthier, E.; Martin, V. [CEA, IRFM, F-13108 Saint-Paul-Lez-Durance (France); Chabaud, D.; Humbert, E. [OPTIS, ZE de La Farlede, F-83078 Toulon Cedex 9 (France); Collaboration: JET-EFDA Contributors

2012-10-15T23:59:59.000Z

206

Diffuse Scattering  

NLE Websites -- All DOE Office Websites (Extended Search)

Diffuse Scattering Diffuse Scattering * Anticipatory (trick) question: If you have an x-ray or neutron detector looking at a small sample volume, which will scatter more x- rays or neutrons into the detector 1 atom 100 atoms or 1000 atoms? X-ray or neutron beam Answer: Depends! Diffuse Scattering Gene E. Ice Materials Science and Technology Division Oak Ridge National Laboratory, USA National School on Neutron and X-ray Scattering ORNL/SNS June 2011 Presentation concentrates year graduate-level course into 1 hour * Skip mathematical complexities * Expose to range of applications * Develop intuition for length scales * Talk like x-ray/neutron scattering guru - Reciprocal space - Debye Temperature - Laue monotonic - Krivoglaz defects of 1st/2nd kinds! Great for cocktail parties or impressing attractive strangers-

207

X-ray transmissive debris shield  

DOE Patents (OSTI)

A composite window structure is described for transmitting x-ray radiation and for shielding radiation generated debris. In particular, separate layers of different x-ray transmissive materials are laminated together to form a high strength, x-ray transmissive debris shield which is particularly suited for use in high energy fluences. In one embodiment, the composite window comprises alternating layers of beryllium and a thermoset polymer.

Spielman, Rick B. (Albuquerque, NM)

1994-01-01T23:59:59.000Z

208

NIST X-Ray Transition Energies  

Science Conference Proceedings (OSTI)

... with the International System of measurement ... titled "X-ray transition energies: new approach ... and by NIST's Systems Integration for Manufacturing ...

2011-12-09T23:59:59.000Z

209

X-ray Line Profile Analysis  

Science Conference Proceedings (OSTI)

... Magnetic Composite Materials · X-Ray Studies of Structural Effects Induced by Pulsed (30 Tesla), High Magnetic Fields at the Advanced Photon Source ...

210

NIST: X-Ray Mass Attenuation Coefficients  

Science Conference Proceedings (OSTI)

... NIST reserves the right to charge for these data in the ... ?/? and the mass energy-absorption coefficient ... The tables cover energies of the photon (x-ray ...

2011-12-09T23:59:59.000Z

211

Lensless X-Ray Imaging in Reflection  

NLE Websites -- All DOE Office Websites (Extended Search)

relevant to atomic and molecular phenomena) with the advantages of visible-light lasers (highly coherent beams). All of these characteristics are important for coherent x-ray...

212

Hard X-Ray Quad Collimator  

Technology Development and Commercialization Division One of the best ways to obtain small?size x?ray beams for structural biology research is to ...

213

X-ray spectroscopy of neutron star low-mass X-ray binaries  

E-Print Network (OSTI)

In this thesis, I present work spanning a variety of topics relating to neutron star lowmass X-ray binaries (LMXBs) and utilize spectral information from X-ray observations to further our understanding of these sources. ...

Krauss, Miriam Ilana

2007-01-01T23:59:59.000Z

214

X-Ray Multilayer Database from the LBL Center for X-Ray Optics (CXRO)  

DOE Data Explorer (OSTI)

An important activity of the Center for X-ray Optics (CXRO) is research on x-ray mirrors and their use in optical devices to focus and deflect x-ray beams. The two kinds of mirrors most widely used are glancing incidence reflectors and multilayer coatings. The X-Ray Multilayer Database is based on the results of surveys taken at the biennial Physics of X-Ray Multilayer Structures conferences. It contains measured x-ray reflectances reported for various multilayers. The database is provided as a service to the x-ray and multilayer research communities and is intended to reflect the state-of-the-art in multilayer x-ray mirrors. (Specialized Interface)

215

Materials Analysis by Soft x-ray Scanning Transmission X-ray ...  

Science Conference Proceedings (OSTI)

About this Abstract. Meeting, Materials Science & Technology 2013. Symposium, Optical and X-ray Imaging Techniques for Material Characterization.

216

P-wave velocity structure of the southern Ryukyu margin east of Taiwan: Results from the ACTS wide-angle seismic experiment  

E-Print Network (OSTI)

Okinawa trough over the Ryukyu arc and forearc. Wide angle seismic data were recorded by the OBS array

Demouchy, Sylvie

217

Mode-Locked Multichromatic X-Rays in a Seeded Free-Electron Laser for Single-Shot X-Ray Spectroscopy  

SciTech Connect

We present the promise of generating gigawatt mode-locked multichromatic x rays in a seeded free-electron laser (FEL). We show that, by using a laser to imprint periodic modulation in electron beam phase space, a single-frequency coherent seed can be amplified and further translated to a mode-locked multichromatic output in an FEL. With this configuration the FEL output consists of a train of mode-locked ultrashort pulses which span a wide frequency gap with a series of equally spaced sharp lines. These gigawatt multichromatic x rays may potentially allow one to explore the structure and dynamics of a large number of atomic states simultaneously. The feasibility of generating mode-locked x rays ranging from carbon K edge ({approx}284 eV) to copper L{sub 3} edge ({approx}931 eV) is confirmed with numerical simulation using the realistic parameters of the linac coherent light source (LCLS) and LCLS-II. We anticipate that the mode-locked multichromatic x rays in FELs may open up new opportunities in x-ray spectroscopy (i.e. resonant inelastic x-ray scattering, time-resolved scattering and spectroscopy, etc.).

Xiang, Dao; Ding, Yuantao; Raubenheimer, Tor; Wu, Juhao; /SLAC

2012-05-10T23:59:59.000Z

218

Fiber fed x-ray/gamma ray imaging apparatus  

SciTech Connect

X-ray/gamma ray imaging apparatus is disclosed for detecting the position, energy, and intensity of x-ray/gamma ray radiation comprising scintillation means disposed in the path of such radiation and capable of generating photons in response to such radiation; first photodetection means optically bonded to the scintillation means and capable of generating an electrical signal indicative of the intensity, and energy of the radiation detected by the scintillation means; second photodetection means capable of generating an electrical signal indicative of the position of the radiation in the radiation pattern; and means for optically coupling the scintillation means to the second photodetection means. The photodetection means are electrically connected to control and storage means which may also be used to screen out noise by rejecting a signal from one photodetection means not synchronized to a signal from the other photodetection means; and also to screen out signals from scattered radiation.

Hailey, Charles J. (San Francisco, CA); Ziock, Klaus-Peter (Livermore, CA)

1992-01-01T23:59:59.000Z

219

Wide-Angle Imaging Lidar Deployment at the ARM Southern Great Plains Site: Intercomparison of Cloud Property Retrievals  

Science Conference Proceedings (OSTI)

The Wide-Angle Imaging Lidar (WAIL), a new instrument that measures cloud optical and geometrical properties by means of off-beam lidar returns, was deployed as part of a multi-instrument campaign to probe a cloud field at the Atmospheric ...

Igor N. Polonsky; Steven P. Love; Anthony B. Davis

2005-06-01T23:59:59.000Z

220

APS Bending Magnet X-rays and  

NLE Websites -- All DOE Office Websites (Extended Search)

Irradiation of Nd-Fe-B Permanent Magnets with Irradiation of Nd-Fe-B Permanent Magnets with APS Bending Magnet X-rays and 60 Co γ-rays J. Alderman and P.K. Job APS Operations Division Advanced Photon Source J. Puhl Ionizing Radiation Division National Institute of Standards and Technology June 2000 Table of Contents Introduction Radiation-Induced Demagnetization of Permanent Magnets Resources Required γ-ray Irradiation Results and Analysis of γ-ray Irradiation X-ray Irradiation Results and Analysis of X-ray Irradiation Summary and Conclusions Acknowledgements References Tables and Figures Introduction The Advanced Photon Source (APS), as well as other third-generation synchrotron light sources, uses permanent magnets in the insertion devices to produce x-rays for scientific

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


221

High-Resolution X-ray Spectroscopy  

Science Conference Proceedings (OSTI)

... In support of these efforts, we also maintain laboratory x-ray sources from 1 keV to 300 keV, energy and intensity calibration facilities, and a vacuum ...

2013-02-26T23:59:59.000Z

222

X-ray image intensifier phosphor  

DOE Patents (OSTI)

Y/sub 1-x/Gd/sub x/.PO$sub 4$:Tb$sup 3+$ is an effective phosphor for use in X-ray intensifier screens and in nuclear radiation detection systems.

D' Silva, A.P.; Fassel, V.A.

1975-12-01T23:59:59.000Z

223

Kaonic Atom X?ray Spectra  

Science Conference Proceedings (OSTI)

In kaonic atoms energy displacement and broadening of states result from the strong interaction. The most simple kaonic atoms like kaonic hydrogen and deuterium open the possibility to measure this strong interaction induced shift and width by x?ray spectroscopy. In the SIDDHARTA experiment al LNF (Frascati) the DA?NE electron?positron collider delivers nearly mono?energetic negatively charged kaons from ? meson decay. This unique kaon source is used to form kaonic atoms. New high performance x?ray detectors (silicon drift detectors) arranged in an array allow x?ray spectroscopy with high energy resolution combined with timing capability. High precision x?ray measurements like SIDDHARTA at LNF will open the way to study the low energy regime of the strong force in the antikaon?nucleon interaction. The experiment and its current status is presented in this talk.

J. Marton; on behalf of the SIDDHARTA Collaboration

2009-01-01T23:59:59.000Z

224

World's First Hard X-ray Laser  

NLE Websites -- All DOE Office Websites (Extended Search)

LCLS is the world's most powerful X-ray laser. Its highly focused beam, which arrives in staccato bursts a few quadrillionths of a second long, allows researchers to probe complex,...

225

X-ray grid-detector apparatus  

DOE Patents (OSTI)

A hybrid grid-detector apparatus for x-ray systems wherein a microchannel plate structure has an air-interspaced grid portion and a phosphor/optical fluid-filled grid portion. The grids are defined by multiple adjacent channels separated by lead-glass septa. X-rays entering the air-interspaced grid portion at an angle of impingement upon the septa are attenuated, while non-impinging x-rays pass through to the phosphor/fluid filled portion. X-ray energy is converted to luminescent energy in the phosphor/fluid filled portion and the resultant beams of light are directed out of the phosphor/optical fluid filled portion to an imaging device.

Boone, John M. (Folsom, CA); Lane, Stephen M. (Oakland, CA)

1998-01-27T23:59:59.000Z

226

X-Ray Nanoimaging: Instruments and Methods  

NLE Websites -- All DOE Office Websites (Extended Search)

X-Ray Nanoimaging: Instruments and Methods To be held as part of SPIE. http:spie.orgOP318 August 28-29, 2013; San Diego, California, USA...

227

X-Ray Emission from Compact Sources  

SciTech Connect

This paper presents a review of the physical parameters of neutron stars and black holes that have been derived from X-ray observations. I then explain how these physical parameters can be used to learn about the extreme conditions occurring in regions of strong gravity, and present some recent evidence for relativistic effects seen in these systems. A glossary of commonly used terms and a short tutorial on the names of X-ray sources are also included.

Cominsky, L

2004-03-23T23:59:59.000Z

228

Argonne CNM: X-Ray Microscopy Capabilities  

NLE Websites -- All DOE Office Websites (Extended Search)

X-Ray Microscopy Facilities X-Ray Microscopy Facilities The Hard X-Ray Nanoprobe (HXN) facility provides scanning fluorescence, scanning diffraction, and full-field transmission and tomographic imaging capabilities with a spatial resolution of 30 nm over a spectral range of 6-12 keV. Modes of Operation Full-Field Transmission Imaging and Nanotomography X-ray transmission imaging uses both the absorption and phase shift of the X-ray beam by the sample as contrast mechanisms. Absorption contrast is used to map the sample density. Elemental constituents can be located by using differential edge contrast in this mode. Phase contrast can be highly sensitive to edges and interfaces even when the X-ray absorption is weak. These contrast mechanisms are exploited to image samples rapidly in full-field transmission mode under various environmental conditions, or combined with nanotomography methods to study the three-dimensional structure of complex and amorphous nanomaterials with the HXN.

229

Kinematics of Compton backscattering x-ray source for angiography  

SciTech Connect

Calculations of X-Ray production rates, energy spread, and spectrum of Compton-backscattered photons from a Free Electron Laser on an electron beam in a low energy (136-MeV) compact (8.5-m circumference) storage ring indicate that an X-Ray intensity of 34.6 10{sup 7} X-Ray photons per 0.5-mm {times} 0.5-mm pixel for Coronary Angiography near the 33.169-keV iodine K-absorption edge can be achieved in a 4-msec pulse within a scattering cone of 1-mrad half angle. This intensity, at 10-m from the photon-electron interaction point to the patient is about a factor of 10 larger than presently achieved from a 4.5-T superconducting wiggler source in the NSLS 2.5-GeV storage ring and over an area about 5 times larger. The 2.2-keV energy spread of the Compton-backscattered beam is, however, much larger than the 70-eV spread presently attained form the wiggler source and use of a monochromator. The beam spot at the 10-m interaction point-to-patient distance is 20-mm diameter; larger spots are attainable at larger distances but with a corresponding reduction in X-Ray flux. Such a facility could be an inexpensive clinical alternative to present methods of non-invasive Digital Subtraction Angiography (DSA), small enough to be deployed in an urban medical center, and could have other medical, industrial and aerospace applications. Problems with the Compton backscattering source include laser beam heating of the mirror in the FEL oscillator optical cavity, achieving a large enough X-Ray beam spot at the patient, and obtaining radiation damping of the transverse oscillations and longitudinal emittance dilution of the storage ring electron beam resulting from photon-electron collisions without going to higher electron energy where the X-Ray energy spread becomes excessive for DSA. 38 refs.

Blumberg, L.N.

1992-05-01T23:59:59.000Z

230

Copper Ridges Nearly Double X-ray Sensor Performance  

Science Conference Proceedings (OSTI)

... Physics Letters,* can measure X-ray energies with an ... X-rays and measure the energy based on ... by NASA and the NIST Office of Microelectronics ...

2011-10-03T23:59:59.000Z

231

Sandia National Laboratories X-ray Tube with Magnetic Electron ...  

... for the U.S. Department of Energy’s National ... high average power large area X-ray tube provides increased X-ray generation efficiency through ...

232

XIPE: the X-ray Imaging Polarimetry Explorer  

E-Print Network (OSTI)

X-ray polarimetry, sometimes alone, and sometimes coupled to spectral and temporal variability measurements and to imaging, allows a wealth of physical phenomena in astrophysics to be studied. X-ray polarimetry investigates the acceleration process, for example, including those typical of magnetic reconnection in solar flares, but also emission in the strong magnetic fields of neutron stars and white dwarfs. It detects scattering in asymmetric structures such as accretion disks and columns, and in the so-called molecular torus and ionization cones. In addition, it allows fundamental physics in regimes of gravity and of magnetic field intensity not accessible to experiments on the Earth to be probed. Finally, models that describe fundamental interactions (e.g. quantum gravity and the extension of the Standard Model) can be tested. We describe in this paper the X-ray Imaging Polarimetry Explorer (XIPE), proposed in June 2012 to the first ESA call for a small mission with a launch in 2017 but not selected. XIPE ...

Soffitta, Paolo; Bellazzini, Ronaldo; Braga, João; Costa, Enrico; Fraser, George W; Gburek, Szymon; Huovelin, Juhani; Matt, Giorgio; Pearce, Mark; Poutanen, Juri; Reglero, Victor; Santangelo, Andrea; Sunyaev, Rashid A; Tagliaferri, Gianpiero; Weisskopf, Martin; Aloisio, Roberto; Amato, Elena; Attiná, Primo; Axelsson, Magnus; Baldini, Luca; Basso, Stefano; Bianchi, Stefano; Blasi, Pasquale; Bregeon, Johan; Brez, Alessandro; Bucciantini, Niccoló; Burderi, Luciano; Burwitz, Vadim; Casella, Piergiorgio; Churazov, Eugene; Civitani, Marta; Covino, Stefano; da Silva, Rui Miguel Curado; Cusumano, Giancarlo; Dadina, Mauro; D'Amico, Flavio; De Rosa, Alessandra; Di Cosimo, Sergio; Di Persio, Giuseppe; Di Salvo, Tiziana; Dovciak, Michal; Elsner, Ronald; Eyles, Chris J; Fabian, Andrew C; Fabiani, Sergio; Feng, Hua; Giarrusso, Salvatore; Goosmann, René W; Grandi, Paola; Grosso, Nicolas; Israel, Gianluca; Jackson, Miranda; Kaaret, Philip; Karas, Vladimir; Kuss, Michael; Lai, Dong; La Rosa, Giovanni; Larsson, Josefin; Larsson, Stefan; Latronico, Luca; Maggio, Antonio; Maia, Jorge; Marin, Frédéric; Massai, Marco Maria; Mineo, Teresa; Minuti, Massimo; Moretti, Elena; Muleri, Fabio; O'Dell, Stephen L; Pareschi, Giovanni; Peres, Giovanni; Pesce, Melissa; Petrucci, Pierre-Olivier; Pinchera, Michele; Porquet, Delphine; Ramsey, Brian; Rea, Nanda; Reale, Fabio; Rodrigo, Juana Maria; Ró?a?ska, Agata; Rubini, Alda; Rudawy, Pawel; Ryde, Felix; Salvati, Marco; Júnior, Valdivino Alexandre de Santiago; Sazonov, Sergey; Sgró, Carmelo; Silver, Eric; Spandre, Gloria; Spiga, Daniele; Stella, Luigi; Tamagawa, Toru; Tamborra, Francesco; Tavecchio, Fabrizio; Dias, Teresa Teixeira; van Adelsberg, Matthew; Wu, Kinwah; Zane, Silvia

2013-01-01T23:59:59.000Z

233

X-Ray Light Sources | U.S. DOE Office of Science (SC)  

Office of Science (SC) Website

X-Ray Light Sources X-Ray Light Sources Scientific User Facilities (SUF) Division SUF Home About User Facilities X-Ray Light Sources Neutron Scattering Facilities Nanoscale Science Research Centers Electron-Beam Microcharacterization Centers Accelerator & Detector Research & Development Principal Investigators' Meetings Scientific Highlights Construction Projects BES Home User Facilities X-Ray Light Sources Print Text Size: A A A RSS Feeds FeedbackShare Page This activity supports the operation of five DOE light sources. The unique properties of synchrotron radiation include its continuous spectrum, high flux and brightness, and in the case of the Linac Coherent Light Source, high coherence, which makes it an indispensable tool in the exploration of matter. The wavelengths of the emitted photons span a range of dimensions

234

Radiographic X-Ray Pulse Jitter  

Science Conference Proceedings (OSTI)

The Dual Beam Radiographic Facility consists of two identical radiographic sources. Major components of the machines are: Marx generator, water-filled pulse-forming line (PFL), water-filled coaxial transmission line, three-cell inductive voltage adder, and rod-pinch diode. The diode pulse has the following electrical specifications: 2.25-MV, 60-kA, 60-ns. Each source has the following x-ray parameters: 1-mm-diameter spot size, 4-rad at 1 m, 50-ns full width half max. The x-ray pulse is measured with PIN diode detectors. The sources were developed to produce high resolution images on single-shot, high-value experiments. For this application it is desirable to maintain a high level of reproducibility in source output. X-ray pulse jitter is a key metric for analysis of reproducibility. We will give measurements of x-ray jitter for each machine. It is expected that x-ray pulse jitter is predominantly due to PFL switch jitter, and therefore a correlation of the two will be discussed.

Mitton, C. V., Good, D. E., Henderson, D. J., Hogge, K. W.

2011-01-15T23:59:59.000Z

235

Frontiers in X-Ray Science  

Science Conference Proceedings (OSTI)

The year 2010 marked the fiftieth anniversary of the optical laser and the first anniversary of the world's first hard x-ray free-electron laser, the Linac Coherent Light Source (LCLS) at SLAC. This exciting, new accelerator-based source of x-rays provides peak brilliances roughly a billion times greater than currently available from synchrotron sources such as the Advanced Photon Source at Argonne, and thus explores a qualitatively different parameter space. This talk will describe the first experiments at the LCLS aimed at understanding the nature of high intensity x-ray interactions, related applications in ultrafast imaging on the atomic scale and sketch nascent plans for the extension of both linac and storage-ring based photon sources.

Linda Young

2011-02-23T23:59:59.000Z

236

Radiobiological studies using gamma and x rays.  

Science Conference Proceedings (OSTI)

There are approximately 500 self-shielded research irradiators used in various facilities throughout the U.S. These facilities use radioactive sources containing either 137Cs or 60Co for a variety of biological investigations. A report from the National Academy of Sciences[1] described the issues with security of particular radiation sources and the desire for their replacement. The participants in this effort prepared two peer-reviewed publications to document the results of radiobiological studies performed using photons from 320-kV x rays and 137Cs on cell cultures and mice. The effectiveness of X rays was shown to vary with cell type.

Potter, Charles Augustus; Longley, Susan W.; Scott, Bobby R. [Lovelace Respiratory Research Institute, Albuquerque, NM; Lin, Yong [Lovelace Respiratory Research Institute, Albuquerque, NM; Wilder, Julie [Lovelace Respiratory Research Institute, Albuquerque, NM; Hutt, Julie A. [Lovelace Respiratory Research Institute, Albuquerque, NM; Padilla, Mabel T. [Lovelace Respiratory Research Institute, Albuquerque, NM; Gott, Katherine M. [Lovelace Respiratory Research Institute, Albuquerque, NM

2013-02-01T23:59:59.000Z

237

Non-Invasive Early Detection and Molecular Analysis of Low X-ray Dose  

NLE Websites -- All DOE Office Websites (Extended Search)

Invasive Early Detection & Molecular Analysis of Low X-ray Dose Effects Invasive Early Detection & Molecular Analysis of Low X-ray Dose Effects in the Lens Lee Goldstein Boston University School of Medicine Abstract Purpose: The lens is a highly-ordered tissue with unique optical properties and exquisite radiosensitivity. The focus of this project is to evaluate radiation cataract dose response and mechanisms associated with low-linear energy transfer (LET) X-rays. We aim to investigate the natural history of Rayleigh light scattering changes in pre-cataractous lenses of mice exposed to radiations using a fully-validated, performance-tested quasi-elastic light scattering (QLS) instrument developed by Dr. Goldstein and colleagues at Boston University. This innovative laser-based technology quantitatively assays pre-cataractous molecular pathology in the lenses of living mice

238

The Soft-X-Ray Spectral Shape of X-Ray-Weak Seyferts  

E-Print Network (OSTI)

(I) We observed eight Seyfert~2s and two X--ray--weak Seyfert~1/QSOs with the ROSAT PSPC, and one Seyfert~2 with the ROSAT HRI. These targets were selected from the Extended 12\\um\\ Galaxy Sample. (II) Both Seyfert~1/QSOs vary by factors of 1.5---2. The photon indices steepen in the more luminous state, consistent with the variability being mainly due to the softest X--rays, which are confined to a size of less than a parsec. (III) Both the Seyfert~2s and Seyfert~1/QSOs are best fit with a photon index of $\\Gamma\\sim3$, which is steeper than the canonical value of $\\Gamma\\sim1.7$ measured for X--ray--strong Seyferts by ROSAT and at higher energies. Several physical explanations are suggested for the steeper slopes of X--ray--weak objects. (IV) We observed one Seyfert~2, NGC~5005, with the ROSAT HRI, finding about 13\\% of the soft X--rays to come from an extended component. This and other observations suggest that different components to the soft X--ray spectrum of some, if not all, X--ray--weak Seyferts may come from spatially distinct regions.

Brian Rush; Matthew A. Malkan

1995-07-27T23:59:59.000Z

239

Sharper Focusing of Hard X-rays  

NLE Websites -- All DOE Office Websites (Extended Search)

Sharper Focusing of Hard X-rays FROM: Physics News Update Number 773 #1, April 12, 2006, by Phil Schewe and Ben Stein Note: This text has been slightly modified from the original. Sharper focusing of hard x-rays has been achieved with a device developed at Argonne National Lab. Because of their high energy, x-rays are hard to focus: they can be reflected from a surface but only at a glancing angle (less than a tenth of a degree); they can be refracted but the index of refraction is very close to 1, so that making efficient lenses becomes a problem; and they can be diffracted, but the relatively thick, variable pitch grating required for focusing is tricky to achieve. The Argonne device is of the diffraction type, and it consists of a stack of alternating layers of metal and silicon, made by depositing progressively thicker layers. When the x-rays fall on such a structure, nearly edge-on, what they see is a grating (called a linear zone plate) consisting of a sort of bar-code pattern.

240

Multiple wavelength x-ray monochromators  

DOE Patents (OSTI)

An apparatus and method is provided for separating input x-ray radiation containing first and second x-ray wavelengths into spatially separate first and second output radiation which contain the first and second x-ray wavelengths, respectively. The apparatus includes a crystalline diffractor which includes a first set of parallel crystal planes, where each of the planes is spaced a predetermined second distance from one another. The crystalline diffractor also includes a second set of parallel crystal planes inclined at an angle with respect to the first set of crystal planes where each of the planes of the second set of parallel crystal planes is spaced a predetermined second distance from one another. In one embodiment, the crystalline diffractor is comprised of a single crystal. In a second embodiment, the crystalline diffractor is comprised of a stack of two crystals. In a third embodiment, the crystalline diffractor includes a single crystal that is bent for focussing the separate first and second output x-ray radiation wavelengths into separate focal points.

Steinmeyer, P.A.

1991-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


241

Multiple wavelength x-ray monochromators  

DOE Patents (OSTI)

An apparatus and method is provided for separating input x-ray radiation containing first and second x-ray wavelengths into spatially separate first and second output radiation which contain the first and second x-ray wavelengths, respectively. The apparatus includes a crystalline diffractor which includes a first set of parallel crystal planes, where each of the planes is spaced a predetermined second distance from one another. The crystalline diffractor also includes a second set of parallel crystal planes inclined at an angle with respect to the first set of crystal planes where each of the planes of the second set of parallel crystal planes is spaced a predetermined second distance from one another. In one embodiment, the crystalline diffractor is comprised of a single crystal. In a second embodiment, the crystalline diffractor is comprised of a stack of two crystals. In a third embodiment, the crystalline diffractor includes a single crystal that is bent for focussing the separate first and second output x-ray radiation wavelengths into separate focal points.

Steinmeyer, P.A.

1991-12-31T23:59:59.000Z

242

Soft x-ray laser microscope  

Science Conference Proceedings (OSTI)

The program consisted of two phases (Phase I and Phase II). The goal of the Phase I (first year program) was to design and construct the Soft X-ray Laser Contact Microscope. Such microscope was constructed and adapted to PPL's 18.2nm soft X-ray Laser (SXL), which in turn was modified and prepared for microscopy experiments. Investigation of the photoresist response to 18.2nm laser radiation and transmissivity of 0.1m thick silicion-nitride (Si[sub 3]N[sub 4]) windows were important initial works. The goal of the first year of Phase II was to construct X-ray contact microscope in combination with existing optical phase microscope, already used by biologists. In the second year of Phase II study of dehydrated Horeseshoe Crab and Hela cancer cells were performed with COXRALM. Also during Phase II, the Imaging X-Ray Laser Microscope (IXRALM) was designed and constructed. This paper describes the development of each of the microscopes and their application for research.

Suckewer, P.I.

1990-10-01T23:59:59.000Z

243

Rise time measurement for ultrafast X-ray pulses  

Science Conference Proceedings (OSTI)

A pump-probe scheme measures the rise time of ultrafast x-ray pulses. Conventional high speed x-ray diagnostics (x-ray streak cameras, PIN diodes, diamond PCD devices) do not provide sufficient time resolution to resolve rise times of x-ray pulses on the order of 50 fs or less as they are being produced by modern fast x-ray sources. Here, we are describing a pump-probe technique that can be employed to measure events where detector resolution is insufficient to resolve the event. The scheme utilizes a diamond plate as an x-ray transducer and a p-polarized probe beam.

Celliers, Peter M. (Berkeley, CA); Weber, Franz A. (Oakland, CA); Moon, Stephen J. (Tracy, CA)

2005-04-05T23:59:59.000Z

244

Rise Time Measurement for Ultrafast X-Ray Pulses  

DOE Patents (OSTI)

A pump-probe scheme measures the rise time of ultrafast x-ray pulses. Conventional high speed x-ray diagnostics (x-ray streak cameras, PIN diodes, diamond PCD devices) do not provide sufficient time resolution to resolve rise times of x-ray pulses on the order of 50 fs or less as they are being produced by modern fast x-ray sources. Here, we are describing a pump-probe technique that can be employed to measure events where detector resolution is insufficient to resolve the event. The scheme utilizes a diamond plate as an x-ray transducer and a p-polarized probe beam.

Celliers, Peter M.; Weber, Franz A.; Moon, Stephen J.

2005-04-05T23:59:59.000Z

245

X-ray flashes and X-ray rich gamma ray bursts. Memorie della Societa’ Astronomica Italiana  

E-Print Network (OSTI)

Abstract. X-ray flashes are detected in the Wide Field Cameras on BeppoSAX in the energy range 2-25 keV as bright X-ray sources lasting of the order of minutes, but remaining undetected in the Gamma Ray Bursts Monitor on BeppoSAX. They have properties very similar to the x-ray counterparts of GRBs and account for some of the Fast X-ray Transient events seen in almost every x-ray satellite. We review their X-ray properties and show that x-ray flashes are in fact very soft, x-ray rich, untriggered gamma ray bursts, in which the peak energy in 2-10 keV x-rays could be up to a factor of 100 larger than the peak energy in the 50-300 keV gamma ray range. The frequency is ? 100 yr ?1. 1 Fast X-ray Transients/High-latitude X-ray Transients Fast X-ray Transients have been observed with many x-ray satellites. In particular they are seen with x-ray instruments that scan the entire sky on a regular basis. Such events are detected in one sky scan and disappeared in the next, typically limiting the duration to be longer than a minute and shorter than a few hours. For this reason they are called Fast Transients. The first transients

John Heise; Jean In ’t Z; Peter M. Woods

2001-01-01T23:59:59.000Z

246

X-Ray Absorption and X-Ray Raman Scattering Studies of Battery ...  

Science Conference Proceedings (OSTI)

Knowledge of the redox chemistry and changes in the structure during electrochemical cycling is of paramount importance in designing new battery materials ...

247

Electronic Properties of Hydrogen Storage Materials with Photon-in/Photon-out Soft-X-Ray Spectroscopy  

DOE Green Energy (OSTI)

The applications of resonant soft X-ray emission spectroscopy on a variety of carbon systems have yielded characteristic fingerprints. With high-resolution monochromatized synchrotron radiation excitation, resonant inelastic X-ray scattering has emerged as a new source of information about electronic structure and excitation dynamics. Photon-in/photon-out soft-X-ray spectroscopy is used to study the electronic properties of fundamental materials, nanostructure, and complex hydrides and will offer potential in-depth understanding of chemisorption and/or physisorption mechanisms of hydrogen adsorption/desorption capacity and kinetics.

Guo, Jinghua

2008-09-22T23:59:59.000Z

248

Core and Valence Excitations in Resonant X-ray Spectroscopy using Restricted Excitation Window Time-dependent Density Functional Theory  

Science Conference Proceedings (OSTI)

We report simulations of X-ray absorption near edge structure (XANES), resonant inelastic X-ray scattering (RIXS) and 1D stimulated X-ray Raman spectroscopy (SXRS) signals of cysteine at the oxygen, nitrogen and sulfur K and L2,3 edges. The simulated XANES signals from the restricted window time-dependent density functional theory (REW-TDDFT) and the static exchange (STEX) method are compared with experiments, showing that REW-TDDFT is more accurate and computationally less expensive than STEX. Simulated RIXS and 1D SXRS signals from REW-TDDFT give some insights on the correlation of different excitations in the molecule.

Zhang, Yu; Biggs, Jason D.; Healion, Daniel; Govind, Niranjan; Mukamel, Shaul

2012-11-21T23:59:59.000Z

249

X-rays Illuminate Ancient Archimedes Text  

NLE Websites -- All DOE Office Websites (Extended Search)

Related Links: Related Links: May 2005 Headlines TIP Article Press Release Walters Art Museum SSRL Home Page SLAC Home Page Stanford Home Page Tuesday, 31 May 2005 X-rays Illuminate Ancient Archimedes Text (contact: Uwe Bergmann, bergmann@slac.stanford.edu) Archimedes Figure Image provided by Will Noel, The Walters Art Museum An early transcription of Archimedes' mathematical theories has been brought to light through the probing of high-intensity x-rays at SSRL's BL6-2. The text contains part of the Method of Mechanical Theorems, one of Archimedes' most important works, which was probably copied out by a scribe in the tenth century. The parchment on which it was written was later scraped down and reused as pages in a twelfth century prayer book, producing a document known as a palimpsest (which comes from the Greek,

250

High resolution x-ray microscope  

Science Conference Proceedings (OSTI)

The authors present x-ray images of grid meshes and biological material obtained using a microspot x-ray tube with a multilayer optic and a 92-element parabolic compound refractive lens (CRL) made of a plastic containing only hydrogen and carbon. Images obtained using this apparatus are compared with those using an area source with a spherical lens and a spherical lens with multilayer condenser. The authors found the best image quality using the multilayer condenser with a parabolic lens, compared to images with a spherical lens and without the multilayer optics. The resolution was measured using a 155-element parabolic CRL and a multilayer condenser with the microspot tube. The experiment demonstrates about 1.1 {mu}m resolution.

Gary, C. K.; Park, H.; Lombardo, L. W.; Piestrup, M. A.; Cremer, J. T.; Pantell, R. H.; Dudchik, Y. I. [Adelphi Technology, Inc. 981-B Industrial Road, San Carlos, California 94070 (United States); Department of Electrical Engineering, Stanford University, Stanford, California 94305 (United States); Institute of Applied Physics Problems, Kurchatova 7, Minsk 220064 (Belarus)

2007-04-30T23:59:59.000Z

251

Sample holder for x-ray diffractometry  

DOE Patents (OSTI)

A sample holder for use with x-ray diffractometers with the capability to rotate the sample, as well as to adjust the position of the sample in the x, y, and z directions. Adjustment in the x direction is accomplished through loosening set screws, moving a platform, and retightening the set screws. Motion translators are used for adjustment in the y and z directions. An electric motor rotates the sample, and receives power from the diffractometer.

Hesch, V.L.

1991-12-31T23:59:59.000Z

252

TENDER ENERGY X-RAY ABSORPTION  

NLE Websites -- All DOE Office Websites (Extended Search)

TENDER ENERGY X-RAY ABSORPTION TENDER ENERGY X-RAY ABSORPTION SPECTROSCOPY (TES) Project Team: S. Bare 1,2 , J. Brandes 3 , T. Buonassisi 4 , J. Chen 5,2 , M. Croft 6 , E. DiMasi 7 , A. Frenkel 8,2 , D. Hesterberg 9 , S. Hulbert 7,2 , S. Khalid 7 , S. Myneni 10 , P. Northrup 7,11 , E.T. Rasbury 11 , B. Ravel 12 , R. Reeder 11 , J. Rodriguez 7,2 , D. Sparks 5,13 , V. Stojanoff 7 , G. Waychunas 14 1 UOP LLC, 2 Synchrotron Catalysis Consortium, 3 Skidaway Inst. of Oceanography, 4 MIT Laboratory for Photovoltaics Research, 5 Univ. of Delaware, 6 Rutgers Univ., 7 Brookhaven National Lab, 8 Yeshiva Univ., 9 North Carolina State Univ., 10 Princeton Univ., 11 Stony Brook Univ., 12 NIST, 13 Delaware Environmental Inst., 14 Lawrence Berkeley National Lab TECHNIQUES: High performance and in-situ X-ray absorption spectroscopy and spatially-resolved XAS of

253

Hard X-ray Variability of AGN  

E-Print Network (OSTI)

Aims: Active Galactic Nuclei are known to be variable throughout the electromagnetic spectrum. An energy domain poorly studied in this respect is the hard X-ray range above 20 keV. Methods: The first 9 months of the Swift/BAT all-sky survey are used to study the 14 - 195 keV variability of the 44 brightest AGN. The sources have been selected due to their detection significance of >10 sigma. We tested the variability using a maximum likelihood estimator and by analysing the structure function. Results: Probing different time scales, it appears that the absorbed AGN are more variable than the unabsorbed ones. The same applies for the comparison of Seyfert 2 and Seyfert 1 objects. As expected the blazars show stronger variability. 15% of the non-blazar AGN show variability of >20% compared to the average flux on time scales of 20 days, and 30% show at least 10% flux variation. All the non-blazar AGN which show strong variability are low-luminosity objects with L(14-195 keV) < 1E44 erg/sec. Conclusions: Concerning the variability pattern, there is a tendency of unabsorbed or type 1 galaxies being less variable than the absorbed or type 2 objects at hardest X-rays. A more solid anti-correlation is found between variability and luminosity, which has been previously observed in soft X-rays, in the UV, and in the optical domain.

V. Beckmann; S. D. Barthelmy; T. J. -L. Courvoisier; N. Gehrels; S. Soldi; J. Tueller; G. Wendt

2007-09-14T23:59:59.000Z

254

Local structure of Rb{sub 2}Li{sub 4}(SeO{sub 4}){sub 3}{center_dot}2H{sub 2}O by the modeling of X-ray diffuse scattering - from average-structure to microdomain model  

Science Conference Proceedings (OSTI)

Local structure of dirubidium tetralithium tris(selenate(VI)) dihydrate - Rb{sub 2}Li{sub 4}(SeO{sub 4}){sub 3}{center_dot} 2H{sub 2}O has been determined basing on the modeling of X-ray diffuse scattering. The origin of observed structured diffuse streaks is SeO{sub 4} tetrahedra switching between two alternative positions in two quasi-planar layers existing in each unit cell and formation of domains with specific SeO{sub 4} tetrahedra configuration locally fulfilling condition for C-centering in the 2a Multiplication-Sign 2b Multiplication-Sign c superstructure cell. The local structure solution is characterized by a uniform distribution of rather large domains (ca. thousand of unit cells) in two layers, but also monodomains can be taken into account. Inside a single domain SeO{sub 4} tetrahedra are ordered along ab-diagonal forming two-string ribbons. Inside the ribbons SeO{sub 4} and LiO{sub 4} tetrahedra share the oxygen corners, whereas ribbons are bound to each other by a net of hydrogen bonds and fastened by corner sharing SeO{sub 4} tetrahedra of the neighboring layers. - Graphical abstract: Experimental sections of the reciprocal space showing diffraction effects observed for RLSO. Bragg spots are visible on sections with integer indices (1 kl section - on the left), streaks - on sections with fractional ones (1.5 kl section - on the right). At the center: resulting local structure of the A package modeled as a microdomain: two-string ribbons of ordered oxygen-corners-sharing SeO{sub 4} and LiO{sub 4} terahedra extended along ab-diagonal are seen; ribbons are bound by hydrogen bonds (shown in pink); the multiplied 2a Multiplication-Sign 2b unit cell is shown. Highlights: Black-Right-Pointing-Pointer X-ray diffuse scattering in RLSO was registered and modeled. Black-Right-Pointing-Pointer The origin of diffuse streaks is SeO{sub 4} tetrahedra switching in two structure layers. Black-Right-Pointing-Pointer The local structure is characterized by a uniform distribution of microdomains. Black-Right-Pointing-Pointer Inside a single domain SeO{sub 4} tetrahedra are ordered along ab-diagonal forming ribbons. Black-Right-Pointing-Pointer The ribbons are bound to each other by a net of hydrogen bonds.

Komornicka, Dorota [Institute of Low Temperature and Structure Research, Polish Academy of Sciences, ul. Okolna 2, 50-420 Wroclaw (Poland); Wolcyrz, Marek, E-mail: m.wolcyrz@int.pan.wroc.pl [Institute of Low Temperature and Structure Research, Polish Academy of Sciences, ul. Okolna 2, 50-420 Wroclaw (Poland); Pietraszko, Adam [Institute of Low Temperature and Structure Research, Polish Academy of Sciences, ul. Okolna 2, 50-420 Wroclaw (Poland)

2012-08-15T23:59:59.000Z

255

Anomalous X-ray Diffraction Studies for Photovoltaic Applications  

DOE Green Energy (OSTI)

Anomalous X-ray Diffraction (AXRD) has become a useful technique in characterizing bulk and nanomaterials as it provides specific information about the crystal structure of materials. In this project we present the results of AXRD applied to materials for photovoltaic applications: ZnO loaded with Ga and ZnCo{sub 2}O{sub 4} spinel. The X-ray diffraction data collected for various energies were plotted in Origin software. The peaks were fitted using different functions including Pseudo Voigt, Gaussian, and Lorentzian. This fitting provided the integrated intensity data (peaks area values), which when plotted as a function of X-ray energies determined the material structure. For the first analyzed sample, Ga was not incorporated into the ZnO crystal structure. For the ZnCo{sub 2}O{sub 4} spinel Co was found in one or both tetrahedral and octahedral sites. The use of anomalous X-ray diffraction (AXRD) provides element and site specific information for the crystal structure of a material. This technique lets us correlate the structure to the electronic properties of the materials as it allows us to probe precise locations of cations in the spinel structure. What makes it possible is that in AXRD the diffraction pattern is measured at a number of energies near an X-ray absorption edge of an element of interest. The atomic scattering strength of an element varies near its absorption edge and hence the total intensity of the diffraction peak changes by changing the X-ray energy. Thus AXRD provides element specific structural information. This method can be applied to both crystalline and liquid materials. One of the advantages of AXRD in crystallography experiments is its sensitivity to neighboring elements in the periodic tables. This method is also sensitive to specific crystallographic phases and to a specific site in a phase. The main use of AXRD in this study is for transparent conductors (TCs) analysis. TCs are considered to be important materials because of their efficiency and low risk of environmental pollution. These materials are important to solar cells as a result of their remarkable combination of optical and electrical properties, including high electrical conductivity and high optical transparency in the spectrum of visible light. TCs provide a transparent window, which allows sunlight to pass through while also allowing electricity to conduct out of the cell. Spinel materials have the chemical form AB{sub 2}O{sub 4}, and are made of a face-centered cubic (FCC) lattice of oxygen anions and cations in specific interstitial sites. A normal spinel has all A cations on tetrahedral sites and B cations on octahedral sites. In contrast; an inverse spinel has the A and half of the B cations on octahedral sites and the other half of the B cations on tetrahedral sites; a mixed spinel lies between. In the spinel structure, 8 of 64 possible tetrahedral sites and 16 of 32 possible octahedral sites are filled. Normal spinels have particularly high conduction as the linear octahedral chains of B cations likely serve as conduction paths. In this paper we present how the data obtained with AXRD is used to analyze TCs properties as they apply to photovoltaic applications. One of the materials used for this analysis is zinc oxide. It has been loaded with 5% and 10% of Ga, which has an absorption edge of 10367 eV. The peak (100) was measured for the zinc oxide loaded with 10% Ga. In the case of 5% Ga, we measured peaks (100) and (101). With the information provided by the AXRD we can identify if Ga is being incorporated in the ZnO crystal structure. The analysis of 311 plane in the ZnCo{sub 2}O{sub 4} spinel shows if Co is in tetrahedral or octahedral site.

Not Available

2011-06-22T23:59:59.000Z

256

Energy Determination of X-Ray Transition Energies Using the ...  

Science Conference Proceedings (OSTI)

... We chose to measure x-ray transition energies from NIST ... This resulted in the production of x-ray emission ... would yield not only an energy scale for ...

2012-10-02T23:59:59.000Z

257

SLAC National Accelerator Laboratory - SLAC's X-ray Laser Explores...  

NLE Websites -- All DOE Office Websites (Extended Search)

X-ray Laser Explores Big Data Frontier By Glenn Roberts Jr. June 12, 2013 It's no surprise that the data systems for SLAC's Linac Coherent Light Source X-ray laser have drawn...

258

Biological Imaging by Soft X-Ray Diffraction Microscopy  

NLE Websites -- All DOE Office Websites (Extended Search)

Biological Imaging by Soft X-Ray Diffraction Microscopy Print Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in...

259

SLAC National Accelerator Laboratory - SLAC X-rays Help Discover...  

NLE Websites -- All DOE Office Websites (Extended Search)

which pulses 120 times a second. In the instant before the intense X-rays destroy a nanocrystal, detectors record a flash of X-ray diffraction information. Finally, scientists use...

260

Using Light to Control How X Rays Interact with Matter  

NLE Websites -- All DOE Office Websites (Extended Search)

Using Light to Control How X Rays Interact with Matter Using Light to Control How X Rays Interact with Matter Print Wednesday, 27 January 2010 00:00 Schemes that use one light...

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


261

Nuclear resonant X-ray spectroscopy of (Mg,Fe)SiO3 orthoenstatites JENNIFER M. JACKSON1,*, EMILY A. HAMECHER1  

E-Print Network (OSTI)

Nuclear resonant X-ray spectroscopy of (Mg,Fe)SiO3 orthoenstatites JENNIFER M. JACKSON1,*, EMILY A, 9700 S. Cass Ave., Argonne, IL 60439, USA Abstract: We present nuclear resonant inelastic X-ray scattering (NRIXS) and synchrotron Mo¨ssbauer spectroscopy (SMS) measurements, both nuclear resonant X

Jackson, Jennifer M.

262

Strengthened lithium for x-ray blast windows  

Science Conference Proceedings (OSTI)

Lithium's high x-ray transparency makes it an attractive material for windows intended to protect soft x-ray diagnostics in high energy density experiments. Pure lithium is soft and weak, but lithium mixed with lithium hydride powder becomes harder and stronger, in principle without any additional x-ray absorption. A comparison with the standard material for x-ray windows, beryllium, suggests that lithium or lithium strengthened by lithium hydride may well be an excellent option for such windows.

Pereira, N. R. [Ecopulse Inc., P.O. Box 528, Springfield, Virginia 22150 (United States); Imam, M. A. [Materials Science and Technology Division, Naval Research Laboratory, Washington, DC 20375 (United States)

2008-05-15T23:59:59.000Z

263

Electron and X-Ray Microscopy: Structural Characterization of ...  

Science Conference Proceedings (OSTI)

Oct 28, 2009 ... Recent Advances in Structural Characterization of Materials: Electron and X-Ray Microscopy: Structural Characterization of Nanoscale ...

264

X-ray Microscopy and Imaging: 2-BM  

NLE Websites -- All DOE Office Websites (Extended Search)

BM BM Introduction The 2-BM beamline offers measurement capabilities for x-ray microtomography, x-ray topography and x-ray microdiffraction. X-ray microtomography and x-ray diffraction instruments are installed on separate optical tables for independent operation with fast switch over time. Optically-coupled high-resolution CCD system is used for microtomography and topography with up to 1 micron spatial resolution. X-ray microdiffraction setup consists of KB microfocussing mirrors (~3 micron minimum spot), four-circle Huber diffractometer, high-precision translation sample stage, two orthogonally-mounted video cameras for viewing sample, fluorescence detector (Si-drift diode) and diffraction detector (a scintillation detector or a CCD). Three different levels of monochromaticity are available. Conventional monochromatic x-rays from a double-bounced Si (111) crystal monochromator (DCM, D E/E=1E-4), wide band-pass monochromatic x-rays from a double multilayer monochromator (DMM, D E/E=1~4E-2) and pink beam. The available x-ray range is from 5 keV to 30 keV. The lower limit is due to the x-ray windows and the upper limit is due to the critical angle of the x-ray mirror. Two different coatings (Cr and Pt) for the x-ray mirror allow either 20 keV or 30 keV energy cutoff.

265

Phase Contrast Microscopy with Soft and Hard X-rays  

E-Print Network (OSTI)

Calibration ­ Uses up part of dynamic range · Solution: ­ Soft x-rays: Back side Illumination ­ Hard xPhase Contrast Microscopy with Soft and Hard X-rays Using a Segmented Detector Benjamin Hornberger ­ Phase Contrast 101 · A Segmented Detector for Hard X-ray Microprobes ­ Segmented Silicon Chip ­ Charge

Homes, Christopher C.

266

A bright point source of ultrashort hard x-rays from laser bioplasmas  

E-Print Network (OSTI)

Micro and nano structures scatter light and amplify local electric fields very effectively. Energy incident as intense ultrashort laser pulses can be converted to x-rays and hot electrons more efficiently with a substrate that suitably modifies the local fields. Here we demonstrate that coating a plain glass surface with a few micron thick layer of an ubiquitous microbe, {\\it Escherichia coli}, catapults the brightness of hard x-ray bremsstrahlung emission (up to 300 keV) by more than two orders of magnitude at an incident laser intensity of 10$^{16}$ W cm$^{-2}$. This increased yield is attributed to the local enhancement of electric fields around individual {\\it E. coli} cells and is reproduced by detailed particle-in-cell (PIC) simulations. This combination of laser plasmas and biological targets can lead to turnkey, multi-kilohertz and environmentally safe sources of hard x-rays.

Krishnamurthy, M; Lad, Amit D; Ahmad, Saima; Narayanan, V; Rajeev, R; Kundu, M; Kumar, G Ravindra; Ray, Krishanu

2010-01-01T23:59:59.000Z

267

In Situ X-Ray Probing Reveals Fingerprints of Surface Platinum Oxide  

DOE Green Energy (OSTI)

In situ x-ray absorption spectroscopy (XAS) at the Pt L{sub 3} edge is a useful probe for Pt-O interactions at polymer electrolyte membrane fuel cell (PEMFC) cathodes. We show that XAS using the high energy resolution fluorescence detection (HERFD) mode, applied to a well-defined monolayer Pt/Rh(111) sample where the bulk penetrating hard x-rays probe only surface Pt atoms, provides a unique sensitivity to structure and chemical bonding at the Pt-electrolyte interface. Ab initio multiple-scattering calculations using the FEFF8 code and complementary extended x-ray absorption fine structure (EXAFS) results indicate that the commonly observed large increase of the white-line at high electrochemical potentials on PEMFC cathodes originates from platinum oxide formation, whereas previously proposed chemisorbed oxygen-containing species merely give rise to subtle spectral changes.

Friebel, Daniel

2011-08-24T23:59:59.000Z

268

X-Ray Shines Light on Water Mystery  

DOE Green Energy (OSTI)

Water is the key compound for our existence on this planet and it is involved in many important physical, chemical, biological and geological processes. Although water is the most common molecular substance it is also most unusual with many anomalies in its thermodynamic properties such as compressibility, density variation and heat capacity. The question of the structure of the hydrogen bonding network in water has been discussed intensively for over 100 years and has not yet been resolved. This talk will describe recent x-ray spectroscopy and scattering measurements showing that the liquid can be described as fluctuations between two types of local hydrogen bonded structures driven by in commensurate requirements for minimizing enthalpy and maximizing entropy.

Nilsson, Anders (SLAC)

2010-11-17T23:59:59.000Z

269

Quantitative Analysis of Mt. St. Helens Ash by X-Ray Diffraction and X-Ray Fluorescence Spectrometry  

Science Conference Proceedings (OSTI)

A quantitative study by x-ray diffraction, optical polarizing microscopy, and x-ray fluorescence spectrometry of fallout and ambient ash from three Mt. St. Helens eruptions has revealed a consistent picture of the mineralogical and elemental ...

Briant L. Davis; L. Ronald Johnson; Dana T. Griffen; William Revell Phillips; Robert K. Stevens; David Maughan

1981-08-01T23:59:59.000Z

270

X-Ray Imaging Crystal Spectrometer for Extended X-Ray Sources  

DOE Patents (OSTI)

Spherically or toroidally curved, double focusing crystals are used in a spectrometer for X-ray diagnostics of an extended X-ray source such as a hot plasma produced in a tokamak fusion experiment to provide spatially and temporally resolved data on plasma parameters such as ion temperature, toroidal and poloidal rotation, electron temperature, impurity ion charge-state distributions, and impurity transport. The imaging properties of these spherically or toroidally curved crystals provide both spectrally and spatially resolved X-ray data from the plasma using only one small spherically or toroidally curved crystal, thus eliminating the requirement for a large array of crystal spectrometers and the need to cross-calibrate the various crystals.

Bitter, Manfred L.; Fraekel, Benjamin; Gorman, James L.; Hill, Kenneth W.; Roquemore, Lane A.; Stodiek, Wolfgang; Goeler, Schweickhard von

1999-05-01T23:59:59.000Z

271

Calibrating X-ray Imaging Devices for Accurate Intensity Measurement  

SciTech Connect

The purpose of the project presented is to develop methods to accurately calibrate X-ray imaging devices. The approach was to develop X-ray source systems suitable for this endeavor and to develop methods to calibrate solid state detectors to measure source intensity. NSTec X-ray sources used for the absolute calibration of cameras are described, as well as the method of calibrating the source by calibrating the detectors. The work resulted in calibration measurements for several types of X-ray cameras. X-ray camera calibration measured efficiency and efficiency variation over the CCD. Camera types calibrated include: CCD, CID, back thinned (back illuminated), front illuminated.

Haugh, M. J.

2011-07-28T23:59:59.000Z

272

Apparatus for monitoring x-ray beam alignment  

DOE Patents (OSTI)

A self-contained, hand-held apparatus is provided for monitoring alignment of an x-ray beam in an instrument employing an x-ray source. The apparatus includes a transducer assembly containing a photoresistor for providing a range of electrical signals responsive to a range of x-ray beam intensities from the x-ray beam being aligned. A circuit, powered by a 7.5 VDC power supply and containing an audio frequency pulse generator whose frequency varies with the resistance of the photoresistor, is provided for generating a range of audible sounds. A portion of the audible range corresponds to low x-ray beam intensity. Another portion of the audible range corresponds to high x-ray beam intensity. The transducer assembly may include an a photoresistor, a thin layer of x-ray fluorescent material, and a filter layer transparent to x-rays but opaque to visible light. X-rays from the beam undergoing alignment penetrate the filter layer and excite the layer of fluorescent material. The light emitted from the fluorescent material alters the resistance of the photoresistor which is in the electrical circuit including the audio pulse generator and a speaker. In employing the apparatus, the x-ray beam is aligned to a complete alignment by adjusting the x-ray beam to produce an audible sound of the maximum frequency.

Steinmeyer, P.A.

1989-09-12T23:59:59.000Z

273

Photon Sciences | Beamlines | HXN: Hard X-ray Nanoprobe  

NLE Websites -- All DOE Office Websites (Extended Search)

HXN: Hard X-ray Nanoprobe HXN: Hard X-ray Nanoprobe Poster | Fact Sheet | Preliminary Design Report Scientific Scope The Hard X-ray Nanoprobe beamline and endstation instruments (HXN) will be designed and constructed to explore new frontiers of hard x-ray microscopy applications with the highest achievable spatial resolution. Currently the available spatial resolution for scientific applications, provided by scanning x-ray microscopes in the hard x-ray regime, is limited to ~50nm, which is still insufficient for probing the nanoscale interfacial structures critical in determining properties and functionalities of material and biological systems. The HXN beamline aims to enable x-ray experiments at spatial resolutions ranging from 10 to 30 nm with an ultimate goal of ~1 nm. Beamline Description

274

X-ray chemistry in envelopes around young stellar objects  

E-Print Network (OSTI)

We present chemical models of the envelope of a young stellar object (YSO) exposed to a central X-ray source. The models are applied to the massive star-forming region AFGL 2591 for different X-ray fluxes. The total X-ray ionization rate is dominated by the `secondary' ionization rate of H2 resulting from fast electrons. The carbon, sulphur and nitrogen chemistries are discussed. It is found that He+ and H3+ are enhanced and trigger a peculiar chemistry. Several molecular X-ray tracers are found and compared to tracers of the far ultraviolet (FUV) field. Like ultraviolet radiation fields, X-rays enhance simple hydrides, ions and radicals. In contrast to ultraviolet photons, X-rays can penetrate deep into the envelope and affect the chemistry even at large distances from the source. Whereas the FUV enhanced species cover a region of 200-300 AU, the region enhanced by X-rays is >1000 AU. Best-fit models for AFGL 2591 predict an X-ray luminosity LX > 1e+31 ergs/s with a hard X-ray spectrum TX > 3e+07 K. Furthermore, we find LX/Lbol ~ 1e-6. The chemistry of the bulk of the envelope mass is dominated by cosmic-ray induced reactions rather than by X-ray induced ionization for X-ray luminosities LX < 1e+33 ergs/s. The calculated line intensities of HCO+ and HCS+ show that high-J lines are more affected than lower J lines by the presence of X-rays due to their higher critical densities, and that such differences are detectable even with large aperture single-dish telescopes. Future instruments such as Herschel-HIFI or SOFIA will be able to observe X-ray enhanced hydrides whereas the sensitivity and spatial resolution of ALMA is well-suited to measure the size and geometry of the region affected by X-rays.

P. Staeuber; S. D. Doty; E. F. van Dishoeck; A. O. Benz

2005-06-14T23:59:59.000Z

275

ASCA Observation of an X-Ray-Luminous Active Nucleus in Markarian 231  

E-Print Network (OSTI)

We have obtained a moderately long (100 kilosecond) ASCA observation of the Seyfert 1 galaxy Markarian 231, the most luminous of the local ultraluminous infrared galaxy (ULIRG) population. In the best-fitting model we do not see the X-ray source directly; the spectrum consists of a scattered power-law component and a reflection component, both of which have been absorbed by a column N_H \\approx 3 X 10^(22)/cm^2. About 3/4 of the observed hard X-rays arise from the scattered component, reducing the equivalent width of the iron K alpha line. The implied ratio of 1-10 keV X-ray luminosity to bolometric luminosity, L_x/L_bol \\sim 2%, is typical of Sy 1 galaxies and radio-quiet QSOs of comparable bolometric luminosities, and indicates that the bolometric luminosity is dominated by the AGN. Our estimate of the X-ray luminosity also moves Mrk 231 in line with the correlations found for AGN with extremely strong Fe II emission. A second source separated by about 2 arcminutes is also clearly detected, and contributes ...

Maloney, P R; Maloney, Philip R.; Reynolds, Christopher S

2000-01-01T23:59:59.000Z

276

X-Ray Diffraction on NIF  

SciTech Connect

The National Ignition Facility (NIF) is currently a 192 beam, 1.6 MJ laser. NIF Ramp-Compression Experiments have already made the relevant exo-planet pressure range from 1 to 50 Mbar accessible. We Proposed to Study Carbon Phases by X-Ray Diffraction on NIF. Just a few years ago, ultra-high pressure phase diagrams for materials were very 'simple'. New experiments and theories point out surprising and decidedly complex behavior at the highest pressures considered. High pressures phases of aluminum are also predicted to be complex. Recent metadynamics survey of carbon proposed a dynamic pathway among multiple phases. We need to develop diagnostics and techniques to explore this new regime of highly compressed matter science. X-Ray Diffraction - Understand the phase diagram/EOS/strength/texture of materials to 10's of Mbar. Strategy and physics goals: (1) Powder diffraction; (2) Begin with diamond; (3) Continue with metals etc.; (4) Explore phase diagrams; (5) Develop liquid diffraction; and (6) Reduce background/improve resolution.

Eggert, J H; Wark, J

2012-02-15T23:59:59.000Z

277

Proton induced quasi-monochromatic x-ray beams for soft x-ray spectroscopy studies and selective x-ray fluorescence analysis  

Science Conference Proceedings (OSTI)

We present the analytical features and performance of an x-ray spectroscopy end station of moderate energy resolution operating with proton-induced quasi-monochromatic x-ray beams. The apparatus was designed, installed and operated at the 5.5 MV Tandem VdG Accelerator Laboratory of the Institute of Nuclear Physics, N.C.S.R. 'Demokritos,' Athens. The setup includes a two-level ultrahigh vacuum chamber that hosts in the lower level up to six primary targets in a rotatable holder; there, the irradiation of pure element materials-used as primary targets-with few-MeV high current ({approx}{mu}A) proton beams produces intense quasi-monochromatic x-ray beams of selectable energy. In the chamber's upper level, a six-position rotatable sample holder hosts the targets considered for x-ray spectroscopy studies. The proton-induced x-ray beam, after proper collimation, is guided to the sample position whereas various filters can be also inserted along the beam's path to eliminate the backscattered protons or/and to absorb selectively components of the x-ray beam. The apparatus incorporates an ultrathin window Si(Li) spectrometer (FWHM 136 eV at 5.89 keV) coupled with low-noise electronics capable of efficiently detecting photons down to carbon K{alpha}. Exemplary soft x-ray spectroscopy studies and results of selective x-ray fluorescence analysis are presented.

Sokaras, D. [Institute of Nuclear Physics, N.C.S.R. Demokritos, Aghia Paraskevi, 15310 Athens (Greece); Zarkadas, Ch. [PANalytical B.V., 7600 AA Almelo (Netherlands); Fliegauf, R.; Beckhoff, B. [Physikalisch-Technische Bundesanstalt, Abbestrasse 2-12, 10587 Berlin (Germany); Karydas, A. G. [Institute of Nuclear Physics, N.C.S.R. Demokritos, Aghia Paraskevi, 15310 Athens (Greece); Nuclear Spectrometry and Applications Laboratory, IAEA Laboratories, A-2444 Seibersdorf (Austria)

2012-12-15T23:59:59.000Z

278

2011 X-Ray Science Gordon Research Conference (August 7-12, 2011, Colby, College. Waterville, ME)  

SciTech Connect

The 2011 Gordon Research Conference on X-ray Science will feature forefront x-ray-based science enabled by the rapid improvements in synchrotron and x-ray laser sources. Across the world, x-ray sources are playing an increasingly important role in physics, materials, chemistry, and biology, expanding into ever broadening areas of science and engineering. With the first hard x-ray free electron laser source beginning operation and with other advanced x-ray sources operational and planned, it is a very exciting and pivotal time for exchange ideas about the future of x-ray science and applications. The Conference will provide the forum for this interaction. An international cast of speakers will illuminate sessions on ultrafast science, coherence, imaging, in situ studies, extreme conditions, new developments in optics, sources, and detectors, inelastic scattering, nanoscience, life science, and energy sciences. The Conference will bring together investigators at the forefront of these areas, and will provide a venue for young scientists entering a career in x-ray research to present their research in poster format, hold discussions in a friendly setting, and exchange ideas with leaders in the field. Some poster presenters will be selected for short talks. The collegial atmosphere of this Conference, with ample time for discussion as well as opportunities for informal gatherings in the afternoons and evenings, will provide an avenue for scientists from different disciplines to exchange ideas about forefront x-ray techniques and will promote cross-fertilization between the various research areas represented.

Gregory Stephenson

2011-08-12T23:59:59.000Z

279

Absolute x-ray energy calibration over a wide energy range using a diffraction-based iterative method  

SciTech Connect

In this paper, we report a method of precise and fast absolute x-ray energy calibration over a wide energy range using an iterative x-ray diffraction based method. Although accurate x-ray energy calibration is indispensable for x-ray energy-sensitive scattering and diffraction experiments, there is still a lack of effective methods to precisely calibrate energy over a wide range, especially when normal transmission monitoring is not an option and complicated micro-focusing optics are fixed in place. It is found that by using an iterative algorithm the x-ray energy is only tied to the relative offset of sample-to-detector distance, which can be readily varied with high precision of the order of 10{sup -5}-10{sup -6} spatial resolution using gauge blocks. Even starting with arbitrary initial values of 0.1 A, 0.3 A, and 0.4 A, the iteration process converges to a value within 3.5 eV for 31.122 keV x-rays after three iterations. Different common diffraction standards CeO{sub 2}, Au, and Si show an energy deviation of 14 eV. As an application, the proposed method has been applied to determine the energy-sensitive first sharp diffraction peak of network forming GeO{sub 2} glass at high pressure, exhibiting a distinct behavior in the pressure range of 2-4 GPa. Another application presented is pair distribution function measurement using calibrated high-energy x-rays at 82.273 keV. Unlike the traditional x-ray absorption-based calibration method, the proposed approach does not rely on any edges of specific elements, and is applicable to the hard x-ray region where no appropriate absorption edge is available.

Hong Xinguo; Chen Zhiqiang [Mineral Physics Institute, Stony Brook University, Stony Brook, New York 11794 (United States); Duffy, Thomas S. [Department of Geosciences, Princeton University, Princeton, New Jersey 08544 (United States)

2012-06-15T23:59:59.000Z

280

The Supergiant Fast X-ray Transient with the shortest orbital period: Suzaku observes one orbit in IGRJ16479-4514  

E-Print Network (OSTI)

The eclipsing hard X-ray source IGR J16479-4514 is the Supergiant Fast X-ray Transient (SFXT) with the shortest orbital period (3.32 days). This allowed us to perform a 250 ks long X-ray observation with Suzaku in 2012 February, covering most of its orbit, including the eclipse egress. Outside the eclipse, the source luminosity is around a few 1E34erg/s. The X-ray spectrum can be fit with an absorbed power law together with a neutral iron emission line at 6.4 keV. The column density is constant at 1E23 cm-2 outside the X-ray eclipse. During the eclipse it is lower, consistent with a scattering origin for the low X-ray emission during the eclipse by the supergiant companion wind. The scattered X-ray emission during the X-ray eclipse is used to directly probe the density of the companion wind at the orbital separation, resulting in 7E-14 g/cm3, which translates into a ratio Mdot_w/v_terminal = 7E-17 solar masses/km of the wind mass loss rate to the wind terminal velocity. This ratio, assuming reasonable termina...

Sidoli, L; Sguera, V; Bodaghee, A; Tomsick, J A; Pottschmidt, K; Rodriguez, J; Romano, P; Wilms, J

2013-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
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281

Gray scale x-ray mask  

DOE Patents (OSTI)

The present invention describes a method for fabricating an embossing tool or an x-ray mask tool, providing microstructures that smoothly vary in height from point-to-point in etched substrates, i.e., structure which can vary in all three dimensions. The process uses a lithographic technique to transfer an image pattern in the surface of a silicon wafer by exposing and developing the resist and then etching the silicon substrate. Importantly, the photoresist is variably exposed so that when developed some of the resist layer remains. The remaining undeveloped resist acts as an etchant barrier to the reactive plasma used to etch the silicon substrate and therefore provides the ability etch structures of variable depths.

Morales, Alfredo M. (Livermore, CA); Gonzales, Marcela (Seattle, WA)

2006-03-07T23:59:59.000Z

282

The ITER VIS/IR wide angle viewing system: Challenges and on-going R and D  

SciTech Connect

The ITER tokamak is the next generation fusion device which will allow studying burning plasma obtained by a Deuterium-Tritium (D-T) fusion reaction during hundreds of seconds. ITER vacuum vessel real-time protection will be mandatory during plasma operation to avoid water leaks and critical plasma facing components degradation. The protection system will be based on a wide angle viewing system (WAVS) composed with 18 visible (VIS) and 18 infrared (IR) cameras covering 80 % of the vacuum vessel which will be one of the major imaging systems of ITER. Compared to protection systems routinely used on current tokamaks and based on imaging (VIS and/or IR), new constraints must be taken into account because of their influence on the system performance: the harsh environment (high neutron flux) and the metallic plasma facing components (both first wall and divertor). In this new demanding context, we have achieved three mandatory R and D studies starting from the understanding of the source of signals by using realistic photonic simulation up to real-time processing strategy taken into account first order optical design constraints to define what type of performance could be reached for ITER vacuum vessel protection. (authors)

Travere, J. M.; Aumeunier, M. H.; Joanny, M.; Jouve, M.; Martin, V.; Moncada, V.; Salasca, S. [CEA DSM, IRFM, F-13018 Saint Paul-Lez-Durance (France); Marot, L. [Univ. of Basel, Dept. of Physics, CH-4056 Basel (Switzerland); Chabaud, D. [OPTIS, ZE de la Farlede, F-83078 Toulon Cedex 9 (France); Ferme, J. J. [SESO, Pole d'Activite d'Aix en Provence, 305 Rue Louis Armand, F-13792 Aix en Provence Cedex 3 (France); Bremond, F.; Thonnat, M. [INRIA, 2004 route des Lucioles, F-06902 Sophia Antipolis Cedex (France)

2011-07-01T23:59:59.000Z

283

Extending synchrotron-based atomic physics experiments into the hard X-ray region  

Science Conference Proceedings (OSTI)

The high-brightness, hard x-ray beams available from third-generation synchrotron sources are opening new opportunities to study the deepest inner shells of atoms, an area where little work has been done and phenomena not observed in less tightly bound inner-shells are manifested. In addition scattering processes which are weak at lower energies become important, providing another tool to investigate atomic structure as well as an opportunity to study photon/atom interactions beyond photoabsorption. In this contribution the authors discuss some of the issues related to extending synchrotron-based atomic physics experiments into the hard x-ray region from the physical and the experimental point of view. They close with a discussion of a technique, resonant Raman scattering, that may prove invaluable in determining the spectra of the very highly-excited states resulting from the excitation of deep inner shells.

LeBrun, T. [Argonne National Lab., IL (United States). Physics Div.

1996-12-31T23:59:59.000Z

284

Biological Imaging by Soft X-Ray Diffraction Microscopy  

NLE Websites -- All DOE Office Websites (Extended Search)

Biological Imaging by Soft X-Ray Diffraction Microscopy Print Biological Imaging by Soft X-Ray Diffraction Microscopy Print Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in their ability to image with nanometer-scale resolution in three dimensions nonperiodic objects that are several microns in size. To fill this gap, the technique of coherent x-ray diffraction imaging now under development takes advantage of the penetrating power of x rays while simultaneously removing the limitations imposed by lens-based optical systems. Researchers from Stony Brook University, in collaboration with scientists at the ALS and Cornell University, have taken a large step in this direction by using a lensless x-ray diffraction microscope to image a freeze-dried yeast cell to better than 30-nm resolution. Images were made at several angular orientations of the cell.

285

Definition: X-Ray Diffraction (XRD) | Open Energy Information  

Open Energy Info (EERE)

X-Ray Diffraction (XRD) X-Ray Diffraction (XRD) Jump to: navigation, search Dictionary.png X-Ray Diffraction (XRD) X-Ray Diffraction (XRD) is a laboratory-based technique commonly used for identification of crystalline materials and analysis of unit cell dimensions. One of two primary types of XRD analysis (X-ray powder diffraction and single-crystal XRD) is commonly applied to samples to obtain specific information about the crystalline material under investigation. X-ray powder diffraction is widely used in geology, environmental science, material science, and engineering to rapidly identify unknown crystalline substances (typically in less than 20 minutes). A pure, finely ground, and homogenized sample is required for determination of the bulk composition. Additional uses include detailed

286

X-Ray Diffraction (XRD) | Open Energy Information  

Open Energy Info (EERE)

X-Ray Diffraction (XRD) X-Ray Diffraction (XRD) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Technique: X-Ray Diffraction (XRD) Details Activities (0) Areas (0) Regions (0) NEPA(0) Exploration Technique Information Exploration Group: Lab Analysis Techniques Exploration Sub Group: Rock Lab Analysis Parent Exploration Technique: Rock Lab Analysis Information Provided by Technique Lithology: Rapid and unambiguous identification of unknown minerals.[1] Stratigraphic/Structural: Hydrological: Thermal: Dictionary.png X-Ray Diffraction (XRD): X-Ray Diffraction (XRD) is a laboratory-based technique commonly used for identification of crystalline materials and analysis of unit cell dimensions. One of two primary types of XRD analysis (X-ray powder diffraction and single-crystal XRD) is commonly applied to samples to

287

Portable X-Ray Diffraction (XRD) | Open Energy Information  

Open Energy Info (EERE)

Portable X-Ray Diffraction (XRD) Portable X-Ray Diffraction (XRD) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Technique: Portable X-Ray Diffraction (XRD) Details Activities (0) Areas (0) Regions (0) NEPA(0) Exploration Technique Information Exploration Group: Field Techniques Exploration Sub Group: Data Collection and Mapping Parent Exploration Technique: Data Collection and Mapping Information Provided by Technique Lithology: Rapid and unambiguous identification of unknown minerals.[1] Stratigraphic/Structural: Hydrological: Thermal: Dictionary.png Portable X-Ray Diffraction (XRD): Portable X-Ray Diffraction (XRD) is a field-based technique that can be used for identification of crystalline materials and analysis of unit cell dimensions. Portable XRD analysis is similar to X-ray powder diffraction,

288

Biological Imaging by Soft X-Ray Diffraction Microscopy  

NLE Websites -- All DOE Office Websites (Extended Search)

Biological Imaging by Soft X-Ray Diffraction Microscopy Print Biological Imaging by Soft X-Ray Diffraction Microscopy Print Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in their ability to image with nanometer-scale resolution in three dimensions nonperiodic objects that are several microns in size. To fill this gap, the technique of coherent x-ray diffraction imaging now under development takes advantage of the penetrating power of x rays while simultaneously removing the limitations imposed by lens-based optical systems. Researchers from Stony Brook University, in collaboration with scientists at the ALS and Cornell University, have taken a large step in this direction by using a lensless x-ray diffraction microscope to image a freeze-dried yeast cell to better than 30-nm resolution. Images were made at several angular orientations of the cell.

289

X-Ray Fluorescence (XRF) | Open Energy Information  

Open Energy Info (EERE)

X-Ray Fluorescence (XRF) X-Ray Fluorescence (XRF) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Technique: X-Ray Fluorescence (XRF) Details Activities (0) Areas (0) Regions (0) NEPA(0) Exploration Technique Information Exploration Group: Lab Analysis Techniques Exploration Sub Group: Rock Lab Analysis Parent Exploration Technique: Rock Lab Analysis Information Provided by Technique Lithology: Bulk and trace element analysis of rocks, minerals, and sediments. Stratigraphic/Structural: Hydrological: Thermal: Dictionary.png X-Ray Fluorescence (XRF): X-Ray Fluorescence is a lab-based technique used for bulk chemical analysis of rock, mineral, sediment, and fluid samples. The technique depends on the fundamental principles of x-ray interactions with solid materials, similar

290

Biological Imaging by Soft X-Ray Diffraction Microscopy  

NLE Websites -- All DOE Office Websites (Extended Search)

Biological Imaging by Soft X-Ray Diffraction Microscopy Print Biological Imaging by Soft X-Ray Diffraction Microscopy Print Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in their ability to image with nanometer-scale resolution in three dimensions nonperiodic objects that are several microns in size. To fill this gap, the technique of coherent x-ray diffraction imaging now under development takes advantage of the penetrating power of x rays while simultaneously removing the limitations imposed by lens-based optical systems. Researchers from Stony Brook University, in collaboration with scientists at the ALS and Cornell University, have taken a large step in this direction by using a lensless x-ray diffraction microscope to image a freeze-dried yeast cell to better than 30-nm resolution. Images were made at several angular orientations of the cell.

291

Biological Imaging by Soft X-Ray Diffraction Microscopy  

NLE Websites -- All DOE Office Websites (Extended Search)

Biological Imaging by Soft X-Ray Diffraction Microscopy Print Biological Imaging by Soft X-Ray Diffraction Microscopy Print Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in their ability to image with nanometer-scale resolution in three dimensions nonperiodic objects that are several microns in size. To fill this gap, the technique of coherent x-ray diffraction imaging now under development takes advantage of the penetrating power of x rays while simultaneously removing the limitations imposed by lens-based optical systems. Researchers from Stony Brook University, in collaboration with scientists at the ALS and Cornell University, have taken a large step in this direction by using a lensless x-ray diffraction microscope to image a freeze-dried yeast cell to better than 30-nm resolution. Images were made at several angular orientations of the cell.

292

Density gradient free electron collisionally excited x-ray laser  

DOE Patents (OSTI)

An operational x-ray laser is provided that amplifies 3p-3s transition x-ray radiation along an approximately linear path. The x-ray laser is driven by a high power optical laser. The driving line focused optical laser beam illuminates a free-standing thin foil that may be associated with a substrate for improved structural integrity. This illumination produces a generally cylindrically shaped plasma having an essentially uniform electron density and temperature, that exists over a long period of time, and provides the x-ray laser gain medium. The x-ray laser may be driven by more than one optical laser beam. The x-ray laser has been successfully demonstrated to function in a series of experimental tests.

Campbell, E.M.; Rosen, M.D.

1984-11-29T23:59:59.000Z

293

Fabrication process for a gradient index x-ray lens  

DOE Patents (OSTI)

A process for fabricating high efficiency x-ray lenses that operate in the 0.5-4.0 keV region suitable for use in biological imaging, surface science, and x-ray lithography of integrated circuits. The gradient index x-ray optics fabrication process broadly involves co-sputtering multi-layers of film on a wire, followed by slicing and mounting on block, and then ion beam thinning to a thickness determined by periodic testing for efficiency. The process enables the fabrication of transmissive gradient index x-ray optics for the 0.5-4.0 keV energy range. This process allows the fabrication of optical elements for the next generation of imaging and x-ray lithography instruments m the soft x-ray region.

Bionta, Richard M. (Livermore, CA); Makowiecki, Daniel M. (Livermore, CA); Skulina, Kenneth M. (Livermore, CA)

1995-01-01T23:59:59.000Z

294

Fabrication process for a gradient index x-ray lens  

DOE Patents (OSTI)

A process is disclosed for fabricating high efficiency x-ray lenses that operate in the 0.5-4.0 keV region suitable for use in biological imaging, surface science, and x-ray lithography of integrated circuits. The gradient index x-ray optics fabrication process broadly involves co-sputtering multi-layers of film on a wire, followed by slicing and mounting on block, and then ion beam thinning to a thickness determined by periodic testing for efficiency. The process enables the fabrication of transmissive gradient index x-ray optics for the 0.5-4.0 keV energy range. This process allows the fabrication of optical elements for the next generation of imaging and x-ray lithography instruments in the soft x-ray region. 13 figures.

Bionta, R.M.; Makowiecki, D.M.; Skulina, K.M.

1995-01-17T23:59:59.000Z

295

Multilayers for next generation x-ray sources  

Science Conference Proceedings (OSTI)

Multilayers are artificially layered structures that can be used to create optics and optical elements for a broad range of x-ray wavelengths, or can be optimized for other applications. The development of next generation x-ray sources (synchrotrons and x-ray free electron lasers) requires advances in x-ray optics. Newly developed multilayer-based mirrors and optical elements enabled efficient band-pass filtering, focusing and time resolved measurements in recent FLASH (Free Electron LASer in Hamburg) experiments. These experiments are providing invaluable feedback on the response of the multilayer structures to high intensity, short pulsed x-ray sources. This information is crucial to design optics for future x-ray free electron lasers and to benchmark computer codes that simulate damage processes.

Bajt, S; Chapman, H N; Spiller, E; Hau-Riege, S; Alameda, J; Nelson, A J; Walton, C C; Kjornrattanawanich, B; Aquila, A; Dollar, F; Gullikson, E; Tarrio, C

2007-05-04T23:59:59.000Z

296

Rigorous Simulation of X-Ray Thermal Diffuse Scattering  

Science Conference Proceedings (OSTI)

In-Situ Neutron Diffraction and Crystal Plasticity Modeling of a-Uranium · In-Situ Studies of the ... Thermal Residual Stresses and Strains in Depleted Uranium.

297

X-ray Diffuse Scattering Measurements of Nucleation Dynamics...  

NLE Websites -- All DOE Office Websites (Extended Search)

high pressure conditions which relax into the liquid-vapor coexistence region of the phase diagram, leading to a rapid phase-explosion-driven boiling process within the...

298

NIST X-Ray Form Factor, Atten., and Scattering Database  

Science Conference Proceedings (OSTI)

... regard to extrapolation to energies outside tabulated ... K , as functions of energy and wavelength ... and by NIST's Systems Integration for Manufacturing ...

2011-12-09T23:59:59.000Z

299

National School on Neutron and X-ray Scattering  

NLE Websites -- All DOE Office Websites (Extended Search)

B See "Experiments Schedule" Experiment Time C See "Experiments Schedule" ReceptionBanquet Argonne Guest House Building 460 6:00 pm - Reception 7:00 pm - Dinner 7:00 pm Dinner...

300

X-Ray Scattering Group, Condensed Matter Physics & Materials...  

NLE Websites -- All DOE Office Websites (Extended Search)

Symposium on Optics and Photonics, San Diego, California, July 31-August 4, 2005. Proc. SPIE, Vol. 5932, 59322A, Sept. 19, 2005. Turgeman, R., Gershevitz, O., Deutsch, M., Ocko,...

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


301

X-Ray Scattering Group, Condensed Matter Physics & Materials...  

NLE Websites -- All DOE Office Websites (Extended Search)

S.-W. Magnetic-field-induced collapse of charge-ordered nanoclusters and the colossal magnetoresistance effect in Nd0.7Sr0.3MnO3. Phys. Rev. B 64, 220405(R), 1-5 (2001)....

302

X-Ray Scattering Group, Condensed Matter Physics & Materials...  

NLE Websites -- All DOE Office Websites (Extended Search)

G., Balicas, L., Xin, Y., Dagotto, E., Crow, J., Nelson, C., and Agterberg, D. Tunneling magnetoresistance and quantum oscillations in bilayered Ca3Ru2O7. Phys. Rev. B 67, 060406...

303

X-Ray Scattering Group, Condensed Matter Physics & Materials...  

NLE Websites -- All DOE Office Websites (Extended Search)

Group Photos August 2013: John with the Beamline Advisory Team for the SIX project at NSLS-II. The preparations for the external building for SIX can be seen in the background....

304

Photon Sciences | Beamlines | CHX: Coherent Hard X-ray Scattering...  

NLE Websites -- All DOE Office Websites (Extended Search)

exceeding, for a photon energy near E8 keV, 1021 phsmrad2mm20.1 % bw (more than one order of magnitude higher than that of the Advanced Photon Source), the CHX beamline will...

305

X-Ray Scattering Group, Condensed Matter Physics & Materials...  

NLE Websites -- All DOE Office Websites (Extended Search)

highlights Quantum Persistence of Magnetic Excitations in Overdoped High Temperature Superconductors Novel Magnetic Dispersions by Mixing Ir and Cu Materials Today Popular...

306

X-Ray Scattering Group, Condensed Matter Physics & Materials...  

NLE Websites -- All DOE Office Websites (Extended Search)

T., and Billinge, S. Local structural investigation of SmFeAsO1-xFx high temperature superconductors. J. Phys.: Condens. Matter 23, 272201 (2011). Partzsch, S., Wilkins,...

307

Femtosecond X-Rays from 90{degree} Thomson Scattering  

E-Print Network (OSTI)

system allows single bunch measurement of beam emittance, energy, charge and bunch length. The main laser

Leemans, W.

2008-01-01T23:59:59.000Z

308

NIST X-Ray Form Factor, Atten., and Scattering Database ...  

Science Conference Proceedings (OSTI)

... and Liberman while much of the experimental data was synthesised by ... for the range of Z and energy of general ... the range of Z and energies, and in ...

2010-10-05T23:59:59.000Z

309

Time-resolved x-ray scattering instrumentation  

DOE Patents (OSTI)

An apparatus and method for increased speed and efficiency of data compilation and analysis in real time is presented in this disclosure. Data is sensed and grouped in combinations in accordance with predetermined logic. The combinations are grouped so that a simplified reduced signal results, such as pairwise summing of data values having offsetting algebraic signs, thereby reducing the magnitude of the net pair sum. Bit storage requirements are reduced and speed of data compilation and analysis is increased by manipulation of shorter bit length data values, making real time evaluation possible.

Borso, C.S.

1985-11-21T23:59:59.000Z

310

Fourteenth National School on Neutron and X-ray Scattering  

E-Print Network (OSTI)

either nuclear physics parameters such as the effective delayed neutron fraction, or the so- called several new features in the physics of the ADS that require further development of the theory of neutron / q 3.784= #12;Neutron Fluctuations in Reactors R111 The physical reason for the above

Pennycook, Steve

311

Thirteenth National School on Neutron and X-ray Scattering  

E-Print Network (OSTI)

Spallation-Driven Cold Neutron Sources Dr. Bradley J. Micklich Senior Physicist, Physics Division physics research Want neutron wavelengths about the dimensions of interest, or neutron energies that can using an intense source of longerwavelength neutrons ­ fundamental nuclear physics (neutron halflife

312

National School on Neutron and X-ray Scattering  

E-Print Network (OSTI)

Cooling of isolated neutron stars as a probe of superdense matter physics Alexander Kaminker physics Alexander Kaminker 1. Introduction Microscopic theories of superdense matter in neutron star cores #12;Cooling of isolated neutron stars as a probe of superdense matter physics Alexander Kaminker

313

X-Ray Scattering Group, Condensed Matter Physics & Materials...  

NLE Websites -- All DOE Office Websites (Extended Search)

of Groningen Josh Turner LCLS Mary Upton Argonne National Lab Julian Baumert Yuguang Cai University of Kentucky Antonio Checco Soft Matter Group, BNL Scott Coburn NSLSII, BNL...

314

Probing warm dense lithium by inelastic X-ray scattering  

E-Print Network (OSTI)

-26000, NWFP, Pakistan 9 Institut f¨ur Kernphysik, Technische Universit¨at Darmstadt, Schlo�gartenstr. 9-temperature superconductors and nuclear matter1 . Warm dense matter, defined by temperatures of a few electron volts

Loss, Daniel

315

NUMERICAL SIMULATIONS OF CHROMOSPHERIC HARD X-RAY SOURCE SIZES IN SOLAR FLARES  

Science Conference Proceedings (OSTI)

X-ray observations are a powerful diagnostic tool for transport, acceleration, and heating of electrons in solar flares. Height and size measurements of X-ray footpoint sources can be used to determine the chromospheric density and constrain the parameters of magnetic field convergence and electron pitch-angle evolution. We investigate the influence of the chromospheric density, magnetic mirroring, and collisional pitch-angle scattering on the size of X-ray sources. The time-independent Fokker-Planck equation for electron transport is solved numerically and analytically to find the electron distribution as a function of height above the photosphere. From this distribution, the expected X-ray flux as a function of height, its peak height, and full width at half-maximum are calculated and compared with RHESSI observations. A purely instrumental explanation for the observed source size was ruled out by using simulated RHESSI images. We find that magnetic mirroring and collisional pitch-angle scattering tend to change the electron flux such that electrons are stopped higher in the atmosphere compared with the simple case with collisional energy loss only. However, the resulting X-ray flux is dominated by the density structure in the chromosphere and only marginal increases in source width are found. Very high loop densities (>10{sup 11} cm{sup -3}) could explain the observed sizes at higher energies, but are unrealistic and would result in no footpoint emission below about 40 keV, contrary to observations. We conclude that within a monolithic density model the vertical sizes are given mostly by the density scale height and are predicted smaller than the RHESSI results show.

Battaglia, M.; Kontar, E. P.; Fletcher, L.; MacKinnon, A. L., E-mail: marina.battaglia@fhnw.ch [SUPA, School of Physics and Astronomy, University of Glasgow, Glasgow G12 8QQ (United Kingdom)

2012-06-10T23:59:59.000Z

316

Ultra-short wavelength x-ray system  

DOE Patents (OSTI)

A method and apparatus to generate a beam of coherent light including x-rays or XUV by colliding a high-intensity laser pulse with an electron beam that is accelerated by a synchronized laser pulse. Applications include x-ray and EUV lithography, protein structural analysis, plasma diagnostics, x-ray diffraction, crack analysis, non-destructive testing, surface science and ultrafast science.

Umstadter, Donald (Ann Arbor, MI); He, Fei (Ann Arbor, MI); Lau, Yue-Ying (Potomac, MD)

2008-01-22T23:59:59.000Z

317

Comparison of heavy charged particles and x-rays for axial tomograpic scanning  

SciTech Connect

Heavy charged particles are applicable to the problem of 3- dimensional reconstruction of electron density distributions of biological samples. The transverse uncertainty in the path of a heavy charged particle due to multiple scattering can be reduced by measuring the entrance and exit positions and angles of the particle. Patient doses for He ions and 80 keV x rays are compared under conditions suitable for imaging the human head. (auth)

Huesman, R.H.; Rosenfeld, A.H.; Solmitz, F.T.

1975-09-01T23:59:59.000Z

318

NIST X-Ray Mass Attenuation Coefficients - Version History  

Science Conference Proceedings (OSTI)

... year, month day with database access date.) Hubbell, JH and Seltzer, SM (2004), Tables of X-Ray Mass Attenuation Coefficients and Mass Energy- ...

2010-10-05T23:59:59.000Z

319

4D Functional Materials Science with X-ray Microscopy  

Science Conference Proceedings (OSTI)

Ultrafast Electron Diffraction Studies of Lattice Dynamics in Thin Bismuth Films · Understanding Fatigue and Corrosion-Fatigue Behavior by In Situ 3D X-ray ...

320

Optical and X-ray Imaging Techniques for Material Characterization ...  

Science Conference Proceedings (OSTI)

Ultrafast X-ray and 2-dimensional UV Spectroscopy of TiO2 Nanoparticles: Majed Chergui1; 1Ecole Polytechnique Fédérale de Lausanne Mesoporous titanium ...

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


321

X-Ray and Neutron Diffraction - Programmaster.org  

Science Conference Proceedings (OSTI)

Oct 20, 2010 ... Strain Determination in Nanoscale Microelectronic Materials Using X-Ray Diffraction: Conal Murray1; 1IBM T.J. Watson Research Center

322

High Temperature X-ray Diffraction Characterization of Thermal ...  

Science Conference Proceedings (OSTI)

Application of Conical Beam X-Ray Tomography to Multi-Phase Materials ... Digital Construction and Characterization of Reticulated Porous Microstructures ...

323

dosimetry of x-rays, gamma rays and electrons  

Science Conference Proceedings (OSTI)

... NIST and BIPM Standards for Air Kerma in Medium-Energy X-rays ... of the codes are available from the Government Printing Office, Washington, DC ...

2013-06-28T23:59:59.000Z

324

APS X-ray Optics Fabrication and Characterization Facility  

SciTech Connect

The APS is in the process of assembling an X-ray Optics Fabrication and characterization Facility. This report will describe its current (as of February 1993) design.

Davey, S.

1993-02-01T23:59:59.000Z

325

X-ray compass for determining device orientation  

DOE Patents (OSTI)

An apparatus and method for determining the orientation of a device with respect to an x-ray source are disclosed. In one embodiment, the present invention is coupled to a medical device in order to determine the rotational orientation of the medical device with respect to the x-ray source. In such an embodiment, the present invention is comprised of a scintillator portion which is adapted to emit photons upon the absorption of x-rays emitted from the x-ray source. An x-ray blocking portion is coupled to the scintillator portion. The x-ray blocking portion is disposed so as to vary the quantity of x-rays which penetrate the scintillator portion based upon the particular rotational orientation of the medical device with respect to the x-ray source. A photon transport mechanism is also coupled to the scintillator portion. The photon transport mechanism is adapted to pass the photons emitted from the scintillator portion to an electronics portion. By analyzing the quantity of the photons, the electronics portion determines the rotational orientation of the medical device with respect to the x-ray source. 25 figs.

Da Silva, L.B.; Matthews, D.L.; Fitch, J.P.; Everett, M.J.; Colston, B.W.; Stone, G.F.

1999-06-15T23:59:59.000Z

326

Synchrotron X-ray Studies of Supercritical Carbon Dioxide/ Reservoir...  

Open Energy Info (EERE)

Edit with form History Facebook icon Twitter icon Synchrotron X-ray Studies of Supercritical Carbon Dioxide Reservoir Rock Interfaces Geothermal Lab Call Project Jump to:...

327

Phase Sensitive X-ray Imager for More Accurate Digital ...  

Livermore Lab Report. News Archive. News ... use of higher energy X-rays which would result in a lower amount of absorbed radiation to the ... testing ...

328

Neutron and X-Ray Studies of Advanced Materials IV  

Science Conference Proceedings (OSTI)

We propose to organize a seven-session Symposium on Neutron and X-Ray ... the advent of new powerful neutron sources such as the Spallation Neutron ...

329

Available Technologies: High Temperature Strain Cell for X-ray ...  

High Temperature Strain Cell for X-ray ... Six hexapole infrared lamps focus inside the sample chamber onto a ceramic material sample with a spherical ...

330

X-ray compass for determining device orientation  

DOE Patents (OSTI)

An apparatus and method for determining the orientation of a device with respect to an x-ray source. In one embodiment, the present invention is coupled to a medical device in order to determine the rotational orientation of the medical device with respect to the x-ray source. In such an embodiment, the present invention is comprised of a scintillator portion which is adapted to emit photons upon the absorption of x-rays emitted from the x-ray source. An x-ray blocking portion is coupled to the scintillator portion. The x-ray blocking portion is disposed so as to vary the quantity of x-rays which penetrate the scintillator portion based upon the particular rotational orientation of the medical device with respect to the x-ray source. A photon transport mechanism is also coupled to the scintillator portion. The photon transport mechanism is adapted to pass the photons emitted from the scintillator portion to an electronics portion. By analyzing the quantity of the photons, the electronics portion determines the rotational orientation of the medical device with respect to the x-ray source.

Da Silva, Luiz B. (Danville, CA); Matthews, Dennis L. (Moss Beach, CA); Fitch, Joseph P. (Livermore, CA); Everett, Matthew J. (Pleasanton, CA); Colston, Billy W. (Livermore, CA); Stone, Gary F. (Livermore, CA)

1999-01-01T23:59:59.000Z

331

SLAC National Accelerator Laboratory - X-ray Laser Pulses in...  

NLE Websites -- All DOE Office Websites (Extended Search)

SLAC researchers have demonstrated for the first time how to produce pairs of X-ray laser pulses in slightly different wavelengths, or colors, with finely adjustable intervals...

332

NIST X-Ray Transition Energies Version History  

Science Conference Proceedings (OSTI)

... Jr., P. Indelicato, L. de Billy, E. Lindroth, and J. Anton, "X-ray transition energies: new approach to a ... [Type of medium] Available: URL [Access date]. ...

2010-10-05T23:59:59.000Z

333

Optical and X-ray Imaging Techniques for Material Characterization  

Science Conference Proceedings (OSTI)

Hyperspectral CARS Microscopy in the Fingerprint Region · In Situ X-ray ... Opportunities for Multimodal CARS Microscopy in Materials Science · Photoemission ...

334

Particle Accelerator & X-Ray Optics | Argonne National Laboratory  

NLE Websites -- All DOE Office Websites (Extended Search)

Hard X-Ray Quad Collimator Facilitates Microcrystallography Experiments Isotopic Abundance in Atom Trap Trace Analysis Nanomaterials Analysis using a Scanning Electron Microscope...

335

X RAY TU E WITH MAGNETI ELE TRON STEERING  

Sandia National Laboratories has created an improved efficiency compact X-ray source to address a wide range ... escape the anode and cause electron h ...

336

Temporal multiplexing radiography for dynamic x-ray imaging  

Science Conference Proceedings (OSTI)

All current x-ray imaging devices acquire images sequentially, one at a time. Using a spatially distributed multibeam x-ray source we recently demonstrated the feasibility for multiplexing x-ray imaging, which can significantly increase the data collection speed. Here we present a general methodology for dynamic x-ray imaging of an object in cyclic motion with temporal multiplexing. Compared to the conventional sequential imaging technique, where 2N-1 phase images are required and N exposures are needed for a single phase image, a temporal multiplexing of dimension 2N-1 can reduce the imaging time by a factor of N while maintaining the temporal resolution.

Cao Guohua [Department of Physics and Astronomy, University of North Carolina, Chapel Hill, North Carolina 27599 (United States); Zhang Jian [Department of Radiation Oncology and Department of Physics and Astronomy, University of North Carolina, Chapel Hill, North Carolina 27599 (United States); Zhou, Otto; Lu Jianping [Department of Physics and Astronomy and Curriculum in Applied Sciences and Engineering, University of North Carolina, Chapel Hill, North Carolina, 27599 (United States)

2009-09-15T23:59:59.000Z

337

Refractive Optics for Hard X-ray Transmission Microscopy  

Science Conference Proceedings (OSTI)

For hard x-ray transmission microscopy at photon energies higher than 15 keV we design refractive condenser and imaging elements to be used with synchrotron light sources as well as with x-ray tube sources. The condenser lenses are optimized for low x-ray attenuation--resulting in apertures greater than 1 mm--and homogeneous intensity distribution on the detector plane, whereas the imaging enables high-resolution (condenser and imaging lenses are being developed. The imaging lenses (compound refractive lenses, CRLs) are made of SU-8 negative resist by deep x-ray lithography. SU-8 shows high radiation stability. The fabrication technique enables high-quality lens structures regarding surface roughness and arrangement precision with arbitrary 2D geometry. To provide point foci, crossed pairs of lenses are used. Condenser lenses have been made utilizing deep x-ray lithographic patterning of thick SU-8 layers, too, whereas in this case, the aperture is limited due to process restrictions. Thus, in terms of large apertures, condenser lenses made of structured and rolled polyimide film are more attractive. Both condenser types, x-ray mosaic lenses and rolled x-ray prism lenses (RXPLs), are considered to be implemented into a microscope setup. The x-ray optical elements mentioned above are characterized with synchrotron radiation and x-ray laboratory sources, respectively.

Simon, M.; Last, A.; Mohr, J.; Nazmov, V.; Reznikova, E. [Institute for Microstructure Technology, Karlsruhe Institute of Technology Kaiserstrasse 12, 76131 Karlsruhe (Germany); Ahrens, G.; Voigt, A. [Microresist Technology, Koepenikerstrasse 325, 12555 Berlin (Germany)

2011-09-09T23:59:59.000Z

338

SLAC National Accelerator Laboratory - X-ray Science  

NLE Websites -- All DOE Office Websites (Extended Search)

energy technologies. SLAC's unique X-ray facilities - the Linac Coherent Light Source (LCLS) and the Stanford Synchrotron Radiation Lightsource (SSRL) - attract thousands of...

339

Bibliography of NRL Works on X-Ray Fluorescence Authored ...  

Science Conference Proceedings (OSTI)

... LS Birks, and EJ Brooks, "Grain-Boundary Diffusion of Zinc in Copper ... 111 J. Gilfrich, "X-Ray Diffraction Studies on the Titanium-Nickel System," in ...

2012-10-05T23:59:59.000Z

340

In situ X-ray Characterization of Energy Storage Materials |...  

NLE Websites -- All DOE Office Websites (Extended Search)

to accurately characterize the dynamic electrochemical processes at the nanometer and atomic level, we have employed a set of complementary, in situ X-ray characterization...

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


341

For Prospective Users: Learn about x-ray research  

NLE Websites -- All DOE Office Websites (Extended Search)

research in the fields of materials science; biological science; physics; chemistry; environmental, geophysical, and planetary science; and innovative x-ray instrumentation....

342

Improved Treatment of X-ray Resistant & Inoperable Cancers ...  

If the electron beam can be transported to the internal cancer without exposure to tissue, ... This figure shows a comparison of X-ray radiation ...

343

Spatially-Resolved X-Ray Microdiffraction Studies Inside Individual ...  

Science Conference Proceedings (OSTI)

This talk will describe recent advances including increased scanning speed, and will describe the use of this x-ray microscope to study mesoscale structural ...

344

Development of Coherent X-Ray Diffraction Microscopy and Its ...  

Science Conference Proceedings (OSTI)

About this Abstract. Meeting, 2010 TMS Annual Meeting & Exhibition. Symposium , Neutron and X-Ray Studies of Advanced Materials III. Presentation Title, 2010 ...

345

Background X-ray Spectrum of Radioactive Samples  

Science Conference Proceedings (OSTI)

An energy-dispersive X-ray spectrometer (EDS) is commonly used with a scanning electron microscope (SEM) to analyze the elemental compositions and microstructures of a variety of samples. For example, the microstructures of nuclear fuels are commonly investigated with this technique. However, the radioactivity of some materials introduces additional X-rays that contribute to the EDS background spectrum. These X-rays are generally not accounted for in spectral analysis software, and can cause misleading results. X-rays from internal conversion [1], Bremsstrahlung [2] radiation associated with alpha ionizations and beta particle interactions [3], and gamma rays from radioactive decay can all elevate the background of radioactive materials.

Shannon Yee; Dawn E. Janney

2008-02-01T23:59:59.000Z

346

Grain Boundary Deformation Analyzed Via X-Ray Diffraction ...  

Science Conference Proceedings (OSTI)

Modeling the Influence of the Second Phase Particle Spatial Distribution on Recrystallization of AA 7050 · Near-Field High Energy X-ray Diffraction Microscopy ...

347

Applications of High Resolution X-ray Computed Tomography in ...  

Science Conference Proceedings (OSTI)

... data, including concentration profiles from x-ray absorption measurements during ... Dynamic Evolution of Liquid-liquid Phase Separation While Cooling in a

348

Determining the Uncertainty of X-Ray Absorption ...  

Science Conference Proceedings (OSTI)

... The apparatus uses a tungsten filament and a tungsten target to generate x rays and the detector contains a CZT crystal. ...

2005-01-28T23:59:59.000Z

349

X-ray Detection with Large Area Avalanche Photodiodes for ...  

Science Conference Proceedings (OSTI)

... The primary photon detector was a 12-element ... The overall energy range for the experiment was ... to directly detect X-rays with energies between 0.3 ...

2013-07-23T23:59:59.000Z

350

Spectrometry of X-Ray Beams Used for Calibrations  

Science Conference Proceedings (OSTI)

... and used to calibrate a wavelength-dispersive crystal x-ray spectrograph used by Lawrence Livermore National Laboratory (LLNL) to diagnose ...

2012-06-26T23:59:59.000Z

351

X-ray Tube with Magnetic Electron Steering - Energy ...  

The high average power large area X-ray tube provides ... Solar Photovoltaic; Solar ... Description This invention consists of a cathode and anode ...

352

X-Ray Microdiffraction for VLSI  

Science Conference Proceedings (OSTI)

Energy windows, with resolutions Ehkl(2 )/Ehkl(2 )=0.03, were then opened in the multichannel analyzer (MCA), and the scattered intensities Ihkl were ...

353

X-ray Methods in High-Intensity Discharges and Metal-Halide Lamps: X-ray Induced Fluorescence  

SciTech Connect

We describe the use of x-ray induced fluorescence to study metal-halide high-intensity discharge lamps and to measure equilibrium vapor pressures of metal-halide salts. The physical principles of metal-halide lamps, relevant aspects of x-ray-atom interactions, the experimental method using synchrotron radiation, and x-ray induced fluorescence measurements relevant to metal-halide lamps are covered.

Curry, John J.; Lapatovich, Walter P.; Henins, Albert (NIST)

2011-12-09T23:59:59.000Z

354

Discovery of Two Types of X-ray Dips in Cyg X-1  

E-Print Network (OSTI)

We observed Cyg X-1 with {\\em RXTE} contiguously over its 5.6-day binary orbit. The source was found to be in the hard state throughout the observation. Many intensity dips were detected in the X-ray light curves. We found that the dips fell into two distinct categories based on their spectral properties. One type exhibits strong energy-dependent attenuation of X-ray emission at low energies during a dip, which is characteristic of photoelectric absorption, but the other type shows nearly energy-independent attenuation. While the first type of dips are likely caused by density enhancement in an inhomogeneous wind of the companion star, as previous studies have indicated, the second type might be due to partial obscuration of an extended X-ray emitting region by optically thick ``clumps'' in the accretion flow. It is also possible that the latter are caused by a momentary decrease in the X-ray luminosity of the source, due, for instance, to a decrease in the mass accretion rate, or by Thomson scattering in highly ionized ``clumps''. We discuss the implications of these scenarios.

Y. X. Feng; Wei Cui

2001-12-06T23:59:59.000Z

355

COSMIC-RAY AND X-RAY HEATING OF INTERSTELLAR CLOUDS AND PROTOPLANETARY DISKS  

SciTech Connect

Cosmic-ray and X-ray heating are derived from the electron energy-loss calculations of Dalgarno, Yan, and Liu for hydrogen-helium gas mixtures. These authors treated the heating from elastic scattering and collisional de-excitation of rotationally excited hydrogen molecules. Here we consider the heating that can arise from all ionization and excitation processes, with particular emphasis on the reactions of cosmic-ray and X-ray generated ions with the heavy neutral species, which we refer to as chemical heating. In molecular regions, chemical heating dominates and can account for 50% of the energy expended in the creation of an ion pair. The heating per ion pair ranges in the limit of negligible electron fraction from {approx}4.3 eV for diffuse atomic gas to {approx}13 eV for the moderately dense regions of molecular clouds and to {approx}18 eV for the very dense regions of protoplanetary disks. An important general conclusion of this study is that cosmic-ray and X-ray heating depends on the physical properties of the medium, i.e., on the molecular and electron fractions, the total density of hydrogen nuclei, and, to a lesser extent, on the temperature. It is also noted that chemical heating, the dominant process for cosmic-ray and X-ray heating, plays a role in UV irradiated molecular gas.

Glassgold, Alfred E. [Astronomy Department, University of California, Berkeley, CA 94720-3411 (United States); Galli, Daniele [INAF-Osservatorio Astrofisico di Arcetri, Largo E. Fermi 5, I-50125 (Italy); Padovani, Marco, E-mail: aglassgold@berkeley.edu, E-mail: galli@arcetri.astro.it, E-mail: marco.padovani@lra.ens.fr [Laboratoire de Radioastronomie Millimetrique, UMR 8112 du CNRS, Ecole Normale Superieure et Observatoire de Paris, 24 rue Lhomond, F-75231 Paris Cedex 05 (France)

2012-09-10T23:59:59.000Z

356

Angular Correlations of the X-Ray Background and Clustering of Extragalactic X-Ray Sources  

E-Print Network (OSTI)

The information content of the autocorrelation function (ACF) of intensity fluctuations of the X-ray background (XRB) is analyzed. The tight upper limits set by ROSAT deep survey data on the ACF at arcmin scales imply strong constraints on clustering properties of X-ray sources at cosmological distances and on their contribution to the soft XRB. If quasars have a clustering radius r_0=12-20 Mpc (H_0=50), and their two point correlation function, is constant in comoving coordinates as indicated by optical data, they cannot make up more 40-50% of the soft XRB (the maximum contribution may reach 80% in the case of stable clustering, epsilon=0). Active Star-forming (ASF) galaxies clustered like normal galaxies, with r_0=10-12 Mpc can yield up to 20% or up to 40% of the soft XRB for epsilon=-1.2 or epsilon=0, respectively. The ACF on degree scales essentially reflects the clustering properties of local sources and is proportional to their volume emissivity. The upper limits on scales of a few degrees imply that hard X-ray selected AGNs have r_06 deg, if real, may be due to AGNs with r_0=20 Mpc; the contribution from clusters of galaxies with r_0~50 Mpc is a factor 2 lower.

L. Danese; L. Toffolatti; A. Franceschini; J. M. Martin-Mirones; G. De Zotti

1993-02-24T23:59:59.000Z

357

Energy distribution measurement of narrow-band ultrashort x-ray beams via K-edge filters subtraction  

Science Conference Proceedings (OSTI)

The characterization of novel x-ray sources includes the measurement of the photon flux and the energy distribution of the produced beam. The aim of BEATS2 experiment at the SPARC-LAB facility of the INFN National Laboratories of Frascati (Rome, Italy) is to investigate possible medical applications of an x-ray source based on Thomson relativistic back-scattering. This source is expected to produce a pulsed quasi-monochromatic x-ray beam with an instantaneous flux of 10{sup 20} ph/s in pulses 10 ps long and with an average energy of about 20 keV. A direct measurement of energy distribution of this beam is very difficult with traditional detectors because of the extremely high photon flux. In this paper, we present a method for the evaluation of the energy distribution of quasi-monochromatic x-ray beams based on beam filtration with K-edge absorbing foils in the energy range of interest (16-22 keV). The technique was tested measuring the energy distribution of an x-ray beam having a spectrum similar to the expected one (SPARC-LAB Thomson source) by using a tungsten anode x-ray tube properly filtered and powered. The energy distribution obtained has been compared with the one measured with a HPGe detector showing very good agreement.

Cardarelli, Paolo; Di Domenico, Giovanni; Marziani, Michele; Mucollari, Irena; Pupillo, Gaia; Sisini, Francesco; Taibi, Angelo; Gambaccini, Mauro [Dipartimento di Fisica, Universita di Ferrara and INFN - Ferrara, via Saragat 1, I-44122 Ferrara (Italy)

2012-10-01T23:59:59.000Z

358

GRB 071112C: A CASE STUDY OF DIFFERENT MECHANISMS IN X-RAY AND OPTICAL TEMPORAL EVOLUTION  

SciTech Connect

We present a study on GRB 071112C X-ray and optical light curves. In these two wavelength ranges, we have found different temporal properties. The R-band light curve showed an initial rise followed by a single power-law decay, while the X-ray light curve was described by a single power-law decay plus a flare-like feature. Our analysis shows that the observed temporal evolution cannot be described by the external shock model in which the X-ray and optical emission are produced by the same emission mechanism. No significant color changes in multi-band light curves and a reasonable value of the initial Lorentz factor ({Gamma}{sub 0} = 275 {+-} 20) in a uniform interstellar medium support the afterglow onset scenario as the correct interpretation for the early R band rise. The result suggests that the optical flux is dominated by afterglow. Our further investigations show that the X-ray flux could be created by an additional feature related to energy injection and X-ray afterglow. Different theoretical interpretations indicate the additional feature in X-ray can be explained by either late internal dissipation or local inverse-Compton scattering in the external shock.

Huang, K. Y.; Tung, Y. H.; Lin, H. M.; Wang, S. Y.; Lehner, M. J.; Wang, J. H.; Wen, C. Y. [Institute of Astronomy and Astrophysics, Academia Sinica, P.O. Box 23-141, Taipei 106, Taiwan (China); Urata, Y.; Ip, W. H. [Institute of Astronomy, National Central University, Chung-Li 32054, Taiwan (China); Xin, L. P.; Qiu, Y.; Wei, J. [National Astronomical Observatories, Chinese Academy of Sciences, Beijing 100012 (China); Yoshida, M. [Hiroshima Astrophysical Science Center, Hiroshima University, 1-3-1 Kagamiyama, Higashi-Hiroshima, Hiroshima 739-8526 (Japan); Zheng, W.; Akerlof, C. [Department of Physics, University of Michigan, Ann Arbor, MI 48109 (United States); Bianco, F. B. [Department of Physics, University of California Santa Barbara, Mail Code 9530, Santa Barbara, CA 93106-9530 (United States); Kawai, N. [Department of Physics, Tokyo Institute of Technology, 2-21-1 Ookayama, Meguro-ku, Tokyo 152-8551 (Japan); Kuroda, D. [Okayama Astrophysical Observatory, National Astronomical Observatory of Japan, Kamogata, Asakuchi, Okayama 719-0232 (Japan); Marshall, S. L. [Kavli Institute for Particle Astrophysics and Cosmology, 2575 Sand Hill Road, MS 29, Menlo Park, CA 94025 (United States); Schwamb, M. E. [Department of Physics, Yale University, P.O. Box 208121, New Haven, CT 06520-8121 (United States); and others

2012-03-20T23:59:59.000Z

359

X-RAY SUBSTRUCTURE STUDIES OF FOUR GALAXY CLUSTERS USING XMM-NEWTON DATA  

SciTech Connect

Mahdavi et al. find that the degree of agreement between weak lensing and X-ray mass measurements is a function of cluster radius. Numerical simulations also point out that X-ray mass proxies do not work equally well at all radii. The origin of the effect is thought to be associated with cluster mergers. Recent work presenting the cluster maps showed an ability of X-ray maps to reveal and study cluster mergers in detail. Here, we present a first attempt to use the study of substructure in assessing the systematics of the hydrostatic mass measurements using two-dimensional (2D) X-ray diagnostics. The temperature map is uniquely able to identify the substructure in an almost relaxed cluster which would be unnoticed in the intracluster medium electron number density and pressure maps. We describe the radial fluctuations in the 2D maps by a cumulative/differential scatter profile relative to the mean profile within/at a given radius. The amplitude indicates {approx}10% fluctuations in the temperature, electron number density, and entropy maps, and {approx}15% fluctuations in the pressure map. The amplitude of and the discontinuity in the scatter complement 2D substructure diagnostics, e.g., indicating the most disturbed radial range. There is a tantalizing link between the substructure identified using the scatter of the entropy and pressure fluctuations and the hydrostatic mass bias relative to the expected mass based on the M-Y{sub X} and M-M{sub gas} relations particularly at r{sub 500}. XMM-Newton observations with {approx}120,000 source photons from the cluster are sufficient to apply our substructure diagnostics via the spectrally measured 2D temperature, electron number density, entropy, and pressure maps.

Zhang Yuying; Reiprich, Thomas H.; Hudson, Daniel S. [Argelander Institut fuer Astronomie, Universitaet Bonn, Auf dem Huegel 71, 53121 Bonn (Germany); Finoguenov, Alexis [Max-Planck-Institut fuer extraterrestrische Physik, Giessenbachstrasse, 85748 Garching (Germany); Sarazin, Craig L. [Department of Astronomy, University of Virginia, P.O. Box 400325, Charlottesville, VA 22904 (United States)

2009-07-10T23:59:59.000Z

360

X-ray spectral states of microquasars  

E-Print Network (OSTI)

We discuss the origin of the dramatically different X-ray spectral shapes observed in the Low Hard State (LHS: dominated by thermal comptonisation) and the High Soft State (HSS: dominated by the accretion disc thermal emission and non-thermal comptonisation in the corona). We present numerical simulations using a new code accounting for the so-called synchrotron boiler effect. These numerical simulations when compared to the data allow us to constrain the magnetic field and temperature of the hot protons in the corona. For the hard state of Cygnus X-1 we find a magnetic field below equipartition with radiation, suggesting that the corona is not powered through magnetic field dissipation (as assumed in most accretion disc corona models). On the other hand, our results also point toward proton temperatures that are substantially lower than typical temperatures of the ADAF models. Finally, we show that in both spectral states Comptonising plasma could be powered essentially through power-law acceleration of non-thermal electrons, which are then partly thermalised by the synchrotron and Coulomb boiler. This suggests that, contrary to current beliefs, the corona of the HSS and that of the LHS could be of very similar nature. The differences between the LHS and HSS coronal spectra would then be predominantly caused by the strong disc soft cooling emission which is present in the HSS and absent in the LHS.

Julien Malzac; Renaud Belmont

2008-10-25T23:59:59.000Z

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


361

X-ray attenuation properties of stainless steel (u)  

SciTech Connect

Stainless steel vessels are used to enclose solid materials for studying x-ray radiolysis that involves gas release from the materials. Commercially available stainless steel components are easily adapted to form a static or a dynamic condition to monitor the gas evolved from the solid materials during and after the x-ray irradiation. Experimental data published on the x-ray attenuation properties of stainless steel, however, are very scarce, especially over a wide range of x-ray energies. The objective of this work was to obtain experimental data that will be used to determine how a poly-energetic x-ray beam is attenuated by the stainless steel container wall. The data will also be used in conjunction with MCNP (Monte Carlos Nuclear Particle) modeling to develop an accurate method for determining energy absorbed in known solid samples contained in stainless steel vessels. In this study, experiments to measure the attenuation properties of stainless steel were performed for a range of bremsstrahlung x-ray beams with a maximum energy ranging from 150 keV to 10 MeV. Bremsstrahlung x-ray beams of these energies are commonly used in radiography of engineering and weapon components. The weapon surveillance community has a great interest in understanding how the x-rays in radiography affect short-term and long-term properties of weapon materials.

Wang, Lily L [Los Alamos National Laboratory; Berry, Phillip C [Los Alamos National Laboratory

2009-01-01T23:59:59.000Z

362

Hard X-ray Phase Contrast -Techniques and Applications -  

E-Print Network (OSTI)

Hard X-ray Phase Contrast Microscopy - Techniques and Applications - A Dissertation Presented of the Graduate School ii #12;Abstract of the Dissertation Hard X-ray Phase Contrast Microscopy - Techniques . . . . . . . . . . . . . . . . . . 58 3.2.4 Reconstruction Example for Integration Method . . . . 59 3.2.5 The Imaginary Part

363

High-energy x-ray production with pyroelectric crystals  

Science Conference Proceedings (OSTI)

The invention of pyroelectric x-ray generator technology has enabled researchers to develop ultraportable, low-power x-ray sources for use in imaging, materials analysis, and other applications. For many applications, the usefulness of an x-ray source is determined by its yield and endpoint energy. In x-ray fluorescence, for example, high-energy sources enable the excitation of the K-shell x-ray peaks for high-Z materials as well as the lower-energy L-shell peaks, allowing more positive sample identification. This report shows how a paired-crystal pyroelectric source can be used to approximately double the endpoint x-ray energy, in addition to doubling the x-ray yield, versus a single-crystal source. As an example of the advantage of a paired-crystal system, we present a spectrum showing the fluorescence of the K shell of thorium using a pyroelectric source, as well as a spectrum showing the fluorescence of the K shell of lead. Also shown is an x-ray spectrum with an endpoint energy of 215 keV.

Geuther, Jeffrey A.; Danon, Yaron [Department of Mechanical, Aerospace, and Nuclear Engineering, Rensselaer Polytechnic Institute, Troy, New York 12180 (United States)

2005-05-15T23:59:59.000Z

364

Improved Anti-Scatter Grids and Collimators  

Office of Technology Transfer Improved Anti-Scatter Grids and Collimators New Fabrication Method Enhances X-Ray, Nuclear Imaging to Save Lives, Reduce ...

365

New Morphological Paradigm Uncovered in Organic Solar Cells  

NLE Websites -- All DOE Office Websites (Extended Search)

studied using grazing-incidence wide-angle x-ray scattering (GIWAXS). Thermodynamic phase diagram for the P3HT (polymer) - PCBM (fullerene) system where the polymer...

366

Flat Quartz-Crystal X-ray Spectrometer for Nuclear Forensics Applications  

E-Print Network (OSTI)

The ability to quickly and accurately quantify the plutonium (Pu) content in pressurized water reactor (PWR) spent nuclear fuel (SNF) is critical for nuclear forensics purposes. One non-destructive assay (NDA) technique being investigated to detect bulk Pu in SNF is measuring the self-induced x-ray fluorescence (XRF). Previous XRF measurements of Three Mile Island (TMI) PWR SNF taken in July 2008 and January 2009 at Oak Ridge National Laboratory (ORNL) successfully illustrated the ability to detect the 103.7 keV x ray from Pu using a planar high-purity germanium (HPGe) detector. This allows for a direct measurement of Pu in SNF. Additional gamma ray and XRF measurements were performed on TMI SNF at ORNL in October 2011 to measure the signal-to-noise ratio for the 103.7 keV peak. Previous work had shown that the Pu/U peak ratio was directly proportional to the Pu/U content and increased linearly with burnup. However, the underlying Compton background significantly reduced the signal-to-noise ratio for the x-ray peaks of interest thereby requiring a prolonged count time. Comprehensive SNF simulations by Stafford et al showed the contributions to the Compton continuum were due to high-energy gamma rays scattering in the fuel, shipping tube, cladding, collimator and detector1. The background radiation was primarily due to the incoherent scattering of the 137Cs 661.7 keV gamma. In this work methods to reduce the Compton background and thereby increase the signal-to-noise ratio were investigated. To reduce the debilitating effects of the Compton background, a crystal x-ray spectrometer system was designed. This wavelength-dispersive spectroscopy technique isolated the Pu and U x rays according to Bragg's law by x-ray diffraction through a crystal structure. The higher energy background radiation was blocked from reaching the detector using a customized collimator and shielding system. A flat quartz-crystal x-ray spectrometer system was designed specifically to fit the constraints and requirements of detecting XRF from SNF. Simulations were performed to design and optimize the collimator design and to quantify the improved signal-to-noise ratio of the Pu and U x-ray peaks. The proposed crystal spectrometer system successfully diffracted the photon energies of interest while blocking the high-energy radiation from reaching the detector and contributing to background counts. The spectrometer system provided a higher signal-to-noise ratio and lower percent error for the XRF peaks of interest from Pu and U. Using the flat quartz-crystal x-ray spectrometer and customized collimation system, the Monte Carlo N-Particle (MCNP) simulations showed the 103.7 keV Pu x-ray peak signal-to-noise ratio improved by a factor of 13 and decreased the percent error by a factor of 3.3.

Goodsell, Alison

2012-08-01T23:59:59.000Z

367

Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism  

NLE Websites -- All DOE Office Websites (Extended Search)

Unexpected Angular Dependence of Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism Print Wednesday, 29 August 2007 00:00 Using spectroscopic information for magnetometry and magnetic microscopy obviously requires detailed theoretical understanding of spectral shape and magnitude of dichroism signals. A research team at ALS Beamline 4.0.2 has now shown unambiguously that, contrary to common belief, spectral shape and magnitude of x-ray magnetic linear dichroism (XMLD) are not only determined by the relative orientation of magnetic moments and x-ray polarization, but their orientation relative to the crystallographic axes must be taken into account for accurate interpretation of XMLD data. Magnetism and X Rays

368

Broadband high resolution X-ray spectral analyzer  

DOE Patents (OSTI)

A broad bandwidth high resolution x-ray fluorescence spectrometer has a performance that is superior in many ways to those currently available. It consists of an array of 4 large area microcalorimeters with 95% quantum efficiency at 6 keV and it produces x-ray spectra between 0.2 keV and 7 keV with an energy resolution of 7 to 10 eV. The resolution is obtained at input count rates per array element of 10 to 50 Hz in real-time, with analog pulse processing and thermal pile-up rejection. This performance cannot be matched by currently available x-ray spectrometers. The detectors are incorporated into a compact and portable cryogenic refrigerator system that is ready for use in many analytical spectroscopy applications as a tool for x-ray microanalysis or in research applications such as laboratory and astrophysical x-ray and particle spectroscopy.

Silver, Eric H. (Berkeley, CA); Legros, Mark (Berkeley, CA); Madden, Norm W. (Livermore, CA); Goulding, Fred (Lafayette, CA); Landis, Don (Pinole, CA)

1998-01-01T23:59:59.000Z

369

X-Ray Observations of Gamma-Ray Burst Afterglows  

E-Print Network (OSTI)

The discovery by the BeppoSAX satellite of X-ray afterglow emission from the gamma-ray burst which occurred on 28 February 1997 produced a revolution in our knowledge of the gamma-ray burst phenomenon. Along with the discovery of X-ray afterglows, the optical afterglows of gamma-ray bursts were discovered and the distance issue was settled, at least for long $\\gamma$-ray bursts. The 30 year mystery of the gamma-ray burst phenomenon is now on the way to solution. Here I rewiew the observational status of the X-ray afterglow emission, its mean properties (detection rate, continuum spectra, line features, and light curves), and the X-ray constraints on theoretical models of gamma-ray bursters and their progenitors. I also discuss the early onset afterglow emission, the remaining questions, and the role of future X-ray afterglow observations.

Filippo Frontera

2004-06-25T23:59:59.000Z

370

Broadband high resolution X-ray spectral analyzer  

DOE Patents (OSTI)

A broad bandwidth high resolution X-ray fluorescence spectrometer has a performance that is superior in many ways to those currently available. It consists of an array of 4 large area microcalorimeters with 95% quantum efficiency at 6 keV and it produces X-ray spectra between 0.2 keV and 7 keV with an energy resolution of 7 to 10 eV. The resolution is obtained at input count rates per array element of 10 to 50 Hz in real-time, with analog pulse processing and thermal pile-up rejection. This performance cannot be matched by currently available X-ray spectrometers. The detectors are incorporated into a compact and portable cryogenic refrigerator system that is ready for use in many analytical spectroscopy applications as a tool for X-ray microanalysis or in research applications such as laboratory and astrophysical X-ray and particle spectroscopy. 6 figs.

Silver, E.H.; Legros, M.; Madden, N.W.; Goulding, F.; Landis, D.

1998-07-07T23:59:59.000Z

371

USING THE X-RAY EMISSION LINES OF SEYFERT 2 AGN TO MEASURE ABUNDANCE RATIOS  

E-Print Network (OSTI)

We measure the metal abundance ratios in the X-ray photoionized gas located near the narrow line region of a sample of Seyfert 2 AGN. The high-resolution X-ray spectra observed with the Chandra high- and low-energy transmission grating spectrometers are compared with models of the resonant scattering and recombination emission from a plasma in thermal balance, and with multiple temperature zones. The abundance ratios in the sample are close to the Solar values, with slight over-abundances of N in NGC 1068, and of Ne in NGC 4151. Our X-ray spectral models use fewer degrees of freedom than previous works. Motivation. Our goal is to use X-ray abundance measurements to cross-calibrate with the optical spectra of quasars. These optical spectra are used to measure the star formation history of the early Universe. 1 To Determine the Abundance Ratios, we fit the Seyfert 2 spectra with models of photoionized plasmas, and then search for deviations in the data from Solar abundances, as shown in Fig. 1. The fluxes of radiative recombination continuum (RRC) features and the radiative recombination (RR) forbidden lines depend little on radiation transfer effects, so they are the most reliable abundance indicators. At low continuum optical depths, the recombination emission flux scales linearly with abundances. Our model allows us to fit the RRC and RR fluxes by accounting for the broad ionization distribution in the plasma. X-ray Emission Line Model. We model a photoionized plasma in ionization equilibrium and thermal balance with a grid of zones, each with ionization parameter log ? = 1.0, 1.5,...4.5 (in c.g.s. units). The XSTAR plasma code yields the charge state distribution of each zone. 2 In order to calculate the recombination emission, we use the photoelectric cross sections

Mario A. Jimenez-garate; Toan Khu

2004-01-01T23:59:59.000Z

372

Enhancement of Terrestrial Diffuse X-ray Emission Associated With Coronal Mass Ejection and Geomagnetic Storm  

E-Print Network (OSTI)

We present an analysis of a Suzaku observation taken during the geomagnetic storm of 2005 August 23-24. We found time variation of diffuse soft X-ray emission when a coronal mass ejection hit Earth and caused a geomagnetic storm. The diffuse emission consists of fluorescent scattering of solar X-rays and exospheric solarwind charge exchange. The former is characterized by a neutral oxygen emission line due to strong heating of the upper atmosphere during the storm time, while the latter is dominated by a sum of C V, C VI, N VI, N VII, O VII, and O VIII emission lines due to the enhanced solar wind flux in the vicinity of the exosphere. Using the solar wind data taken with the ACE and WIND satellites,a time correlation between the solar wind and the strong O VII line flux were investigated. We estimated necessary column densities for the solar X-ray scattering and exospheric SWCX. From these results, we argue that a part of the solar wind ions enter inside the magnetosphere and cause the SWCX reaction.

Ezoe, Yuichiro; Yoshitake, Hiroshi; Mitsuda, Kazuhisa; Terada, Naoki; Oishi, Shihoko; Ohashi, Takaya

2011-01-01T23:59:59.000Z

373

Crosscheck of different techniques for two dimensional power spectral density measurements of x-ray optics  

Science Conference Proceedings (OSTI)

The consistency of different instruments and methods for measuring two-dimensional (2D) power spectral density (PSD) distributions are investigated. The instruments are an interferometric microscope, an atomic force microscope (AFM) and the X-ray Reflectivity and Scattering experimental facility, all available at Lawrence Berkeley National Laboratory. The measurements were performed with a gold-coated mirror with a highly polished stainless steel substrate. It was shown that these three techniques provide essentially consistent results. For the stainless steel mirror, an envelope over all measured PSD distributions can be described with an inverse power-law PSD function. It is also shown that the measurements can be corrected for the specific spatial frequency dependent systematic errors of the instruments. The AFM and the X-ray scattering measurements were used to determine the modulation transfer function of the interferometric microscope. The corresponding correction procedure is discussed in detail. Lower frequency investigation of the 2D PSD distribution was also performed with a long trace profiler and a ZYGO GPI interferometer. These measurements are in some contradiction, suggesting that the reliability of the measurements has to be confirmed with additional investigation. Based on the crosscheck of the performance of all used methods, we discuss the ways for improving the 2D PSD characterization of X-ray optics.

Yashchuk, Valeriy V.; Irick, Steve C.; Gullikson, Eric M.; Howells, Malcolm R.; MacDowell, Alastair A.; McKinney, Wayne R.; Salmassi, Farhad; Warwick, Tony

2005-07-12T23:59:59.000Z

374

Fast-switching elliptically polarized soft X-ray beam X13A at NSLS  

SciTech Connect

The X13A beamline at NSLS is dedicated to the generation and uses of fast-switching elliptically polarized soft X-ray radiation in the energy range from 250 to {approx}1600 eV. The source for this beamline is an elliptically polarized wiggler (EPW) that delivers linearly elliptically polarized soft X-rays at a switching rate, between right- and left-handed polarization, up to 100 Hz. The optical design is a spherical grating monochromator (SGM) that focuses and diffracts in plane orthogonal to the polarization switching direction. The X13A beamline scientific program is dedicated to spectroscopy and scattering studies of magnetism and magnetic materials. The fast-switching capability of the EPW enables the use of lock-in techniques, thereby greatly enhancing the detection sensitivity for small polarization-dependent signals.

Sanchez-Hanke, C.; Kao, C.; Hulbert, S.

2009-07-21T23:59:59.000Z

375

Structure determination of thin CoFe films by anomalous x-ray diffraction  

Science Conference Proceedings (OSTI)

This work reports on the investigation of structure-property relationships in thin CoFe films grown on MgO. Because of the very similar scattering factors of Fe and Co, it is not possible to distinguish the random A2 (W-type) structure from the ordered B2 (CsCl-type) structure with commonly used x-ray sources. Synchrotron radiation based anomalous x-ray diffraction overcomes this problem. It is shown that as grown thin films and 300 K post annealed films exhibit the A2 structure with a random distribution of Co and Fe. In contrast, films annealed at 400 K adopt the ordered B2 structure.

Gloskovskii, Andrei; Stryganyuk, Gregory; Ouardi, Siham [Institut fuer Anorganische und Analytische Chemie, Johannes Gutenberg-Universitaet, 55099 Mainz (Germany); Fecher, Gerhard H.; Felser, Claudia [Institut fuer Anorganische und Analytische Chemie, Johannes Gutenberg-Universitaet, 55099 Mainz (Germany); Max Planck Institute for Chemical Physics of Solids, D-01187 Dresden (Germany); Hamrle, Jaroslav; Pistora, Jaromir [Department of Physics and Nanotechnology Centre, VSB-Technical University of Ostrava, 70833 Ostrava (Czech Republic); Bosu, Subrojati; Saito, Kesami; Sakuraba, Yuya; Takanashi, Koki [Institute for Materials Research (IMR), Tohoku University, Sendai 980-8577 (Japan)

2012-10-01T23:59:59.000Z

376

Biological Imaging by Soft X-Ray Diffraction Microscopy  

NLE Websites -- All DOE Office Websites (Extended Search)

Biological Imaging by Soft X-Ray Biological Imaging by Soft X-Ray Diffraction Microscopy Biological Imaging by Soft X-Ray Diffraction Microscopy Print Wednesday, 30 November 2005 00:00 Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in their ability to image with nanometer-scale resolution in three dimensions nonperiodic objects that are several microns in size. To fill this gap, the technique of coherent x-ray diffraction imaging now under development takes advantage of the penetrating power of x rays while simultaneously removing the limitations imposed by lens-based optical systems. Researchers from Stony Brook University, in collaboration with scientists at the ALS and Cornell University, have taken a large step in this direction by using a lensless x-ray diffraction microscope to image a freeze-dried yeast cell to better than 30-nm resolution. Images were made at several angular orientations of the cell.

377

Resonant Auger Effect at High X-Ray Intensity  

SciTech Connect

The resonant Auger effect of atomic neon exposed to high-intensity x-ray radiation in resonance with the 1s {yields} 3p transition is discussed. High intensity here means that the x-ray peak intensity is sufficient ({approx} 10{sup 18} W/cm{sup 2}) to induce Rabi oscillations between the neon ground state and the 1s{sup -1}3p ({sup 1}P) state within the relaxation lifetime of the inner-shell vacancy. For the numerical analysis presented, an effective two-level model, including a description of the resonant Auger decay process, is employed. Both coherent and chaotic x-ray pulses are treated. The latter are used to simulate radiation from x-ray free-electron lasers based on the principle of self-amplified spontaneous emission. Observing x-ray-driven atomic population dynamics in the time domain is challenging for chaotic pulse ensembles. A more practical option for experiments using x-ray free-electron lasers is to measure the line profiles in the kinetic energy distribution of the resonant Auger electron. This provides information on both atomic population dynamics and x-ray pulse properties.

Rohringer, N; Santra, R

2008-03-27T23:59:59.000Z

378

X-ray emission from laser-produced plasmas  

SciTech Connect

The intensity and spectral characteristics of x-ray emitted from laser-produced plasmas have been investigated computatinoally and experimentally. a two-dimensional implosi code was used successfully to calculate laser-plasma radiation characteristics and to aid in the design of laser targets for high-yield x-ray production. Other computer codes, in use or under development predict lime strengths and energies for laser-plasma x-ray emission. An experimental effort is aimed at reliable measurements of x-ray yields and spectra. a wide variety of x-ray detection methods have been evaluated, and x-ray yields have been measured from plasmas produced with two dissimilar laser systems. The high energy x-ray spectrum, from about 10 to 140 keV, has been studied using high-gain scintillatino detectors and thick K-edge filters. Various supplementary measurements have provided information concerning characteristics of the target-reflected laser light, the ion energies, and the laser intensity patterns.

Violet, C.E. [ed.

1974-07-01T23:59:59.000Z

379

Optical systems for synchrotron radiation: lecture 4. Soft x-ray imaging systems  

Science Conference Proceedings (OSTI)

The history and present techniques of soft x-ray imaging are reviewed briefly. The physics of x-ray imaging is described, including the temporal and spatial coherence of x-ray sources. Particular technologies described are: contact x-ray microscopy, zone plate imaging, scanned image zone plate microscopy, scanned image reflection microscopy, and soft x-ray holography and diffraction. (LEW)

Howells, M.R.

1986-04-01T23:59:59.000Z

380

X-ray afterglows from gamma-ray bursts  

E-Print Network (OSTI)

We consider possible interpretations of the recently detected X- ray afterglow from the gamma-ray burst source GRB 970228. Cosmological and Galactic models of gamma-ray bursts predict different flux and spectral evolution of X-ray afterglows. We show that models based on adiabatic expansion of relativistic forward shocks require very efficient particle energization or post-burst re-acceleration during the expansion. Cooling neutron star models predict a very distinctive spectral and flux evolution that can be tested in current X-ray data.

M. Tavani

1997-03-24T23:59:59.000Z

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


381

Ten years of Vela x-ray observations  

SciTech Connect

The Vela spacecraft, particularly Vela 5B, produced all-sky X-ray data of unprecedented length and completeness. The data led to the discovery of X-ray bursts and numerous transient outbursts. Recent re-analysis has put the data in the form of 10-day skymaps covering a 7-year period, which have led to the discovery or confirmation of a number of long-term periodicities, and have made possible a time-lapse movie of the X-ray sky.

Terrell, J.; Priedhorsky, W.C.

1983-01-01T23:59:59.000Z

382

Sixth International Conference on X-ray Microscopy  

SciTech Connect

More than 180 participants from around the world crowded the Clark Kerr Campus of the University of California, Berkeley, from August 1-6, 1999 for the Sixth International Conference on X-Ray Microscopy (XRM99). Held every three years since 1983, the XRM conferences have become the primary international forum for the presentation and discussion of advances in high-spatial-resolution x-ray imaging and applications (including the use of x-ray spectroscopic and analytical techniques) in biological and medical sciences, environmental and soil sciences, and materials and surface sciences.

Robinson, Arthur L.

1999-08-23T23:59:59.000Z

383

Chandra X-ray Observatory Detection of Extended X-ray Emission from the Planetary Nebula BD+303639  

E-Print Network (OSTI)

We report the detection of well resolved, extended X-ray emission from the young planetary nebula BD+303639 using the Advanced CCD Imaging Spectrometer (ACIS) aboard the Chandra X-ray Observatory. The X-ray emission from BD+303639 appears to lie within, but is concentrated to one side of, the interior of the shell of ionized gas seen in high-resolution optical and IR images. The relatively low X-ray temperature (Tx ~ 3x10^6 K) and asymmetric morphology of the X-ray emission suggests that conduction fronts are present and/or mixing of shock-heated and photoionized gas has occurred and, furthermore, hints at the presence of magnetic fields. The ACIS spectrum suggests that the X-ray emitting region is enriched in the products of helium burning. Our detection of extended X-ray emission from BD+303639 demonstrates the power and utility of Chandra imaging as applied to the study of planetary nebulae.

Kästner, J H; Vrtilek, S D; Dgani, R; Kastner, Joel H.; Soker, Noam; Vrtilek, Saeqa; Dgani, Ruth

2000-01-01T23:59:59.000Z

384

Chandra X-ray Observatory Detection of Extended X-ray Emission from the Planetary Nebula BD+303639  

E-Print Network (OSTI)

We report the detection of well resolved, extended X-ray emission from the young planetary nebula BD+303639 using the Advanced CCD Imaging Spectrometer (ACIS) aboard the Chandra X-ray Observatory. The X-ray emission from BD+303639 appears to lie within, but is concentrated to one side of, the interior of the shell of ionized gas seen in high-resolution optical and IR images. The relatively low X-ray temperature (Tx ~ 3x10^6 K) and asymmetric morphology of the X-ray emission suggests that conduction fronts are present and/or mixing of shock-heated and photoionized gas has occurred and, furthermore, hints at the presence of magnetic fields. The ACIS spectrum suggests that the X-ray emitting region is enriched in the products of helium burning. Our detection of extended X-ray emission from BD+303639 demonstrates the power and utility of Chandra imaging as applied to the study of planetary nebulae.

Joel H. Kastner; Noam Soker; Saeqa Vrtilek; Ruth Dgani

2000-10-09T23:59:59.000Z

385

A Chandra/ACIS Study of 30 Doradus II. X-ray Point Sources in the Massive Star Cluster R136 and Beyond  

E-Print Network (OSTI)

We have studied the X-ray point source population of the 30 Doradus star-forming complex in the Large Magellanic Cloud using high-spatial-resolution X-ray images and spatially-resolved spectra obtained with the Advanced CCD Imaging Spectrometer (ACIS) aboard the Chandra X-ray Observatory. Here we describe the X-ray sources in a 17 ? × 17 ? field centered on R136, the massive star cluster at the center of the main 30 Dor nebula. We detect 20 of the 32 Wolf-Rayet stars in the ACIS field. R136 is resolved at the subarcsecond level into almost 100 X-ray sources, including many typical O3–O5 stars as well as a few bright X-ray sources previously reported. Over two orders of magnitude of scatter in LX is seen among R136 O stars, suggesting that X-ray emission in the most massive stars depends critically on the details of wind properties and binarity of each system, rather than reflecting the widely-reported characteristic value LX/Lbol ? 10 ?7. Such a canonical ratio may exist for single massive stars in R136, but our data are too shallow to confirm this relationship. Through this and future X-ray studies of 30 Doradus, the complete life cycle of a massive stellar cluster can be revealed. Subject headings: HII regions ? Magellanic Clouds ? open clusters and associations: individual (R 136) ? X-rays: individual (30 Doradus) ?stars: Wolf-Rayet ? X-rays: stars 1.

Leisa K. Townsley; Patrick S. Broos; Eric D. Feigelson; Gordon P. Garmire; Konstantin V

2006-01-01T23:59:59.000Z

386

Scanning Transmission X-ray Microscopy: Applications in Atmospheric Aerosol Research  

E-Print Network (OSTI)

G. R. et al. Scanning transmission X-ray microscopy: A newwith the scanning transmission X-ray microscope at BESSY II.T. et al. Scanning transmission X-ray microscopy imaging of

Moffet, Ryan C.

2011-01-01T23:59:59.000Z

387

Argonne CNM Highlight: World?s Most Precise ?Hard X-Ray?  

NLE Websites -- All DOE Office Websites (Extended Search)

World's Most Precise "Hard X-Ray" Nanoprobe Activated X-rays from an APS undulator exiting the front end window of the nanoprobe beamline. X-rays from an APS undulator exiting the...

388

X-ray Science Division: Mission and Goals | Advanced Photon Source  

NLE Websites -- All DOE Office Websites (Extended Search)

X-ray Science Division: Mission and Goals The mission of the X-ray Science Division (XSD) is to enable and perform world class research using x-rays. This mission is accomplished...

389

Active pixel sensors for X-ray astronomy  

E-Print Network (OSTI)

An active pixel sensor array, APS-1, has been fabricated for the purpose of scientific x-ray detection. This thesis presents the results of testing the device. Alternate design architectures are explored. Recommendations ...

Cohen, Matthew (Matthew L.)

2005-01-01T23:59:59.000Z

390

Photon Sciences | Beamlines | SRX: Submicron Resolution X-ray Spectroscopy  

NLE Websites -- All DOE Office Websites (Extended Search)

SRX: Submicron Resolution X-ray Spectroscopy SRX: Submicron Resolution X-ray Spectroscopy Poster | Fact Sheet | Preliminary Design Report Scientific Scope Scientific communities such as environmental sciences, life sciences, and material sciences have identified the need to develop analytical resources to advance the understanding of complex natural and engineered systems that are heterogeneous on the micron to nanometer scale. These needs for high intensity x-ray nanoprobes resulted in the commitment of the NSLS-II Project to build the Submicron Resolution X-ray (SRX) Spectroscopy beamline showing a unique combination of high spectral resolution over a very broad energy range and very high beam intensity in a sub-micrometer spot. NSLS-II will provide one of the best sources in the world for such an instrument.

391

Definition: Portable X-Ray Diffraction (XRD) | Open Energy Information  

Open Energy Info (EERE)

Definition Definition Edit with form History Facebook icon Twitter icon » Definition: Portable X-Ray Diffraction (XRD) Jump to: navigation, search Dictionary.png Portable X-Ray Diffraction (XRD) Portable X-Ray Diffraction (XRD) is a field-based technique that can be used for identification of crystalline materials and analysis of unit cell dimensions. Portable XRD analysis is similar to X-ray powder diffraction, which has traditionally been used in geology, environmental science, material science, and engineering to rapidly identify unknown crystalline substances. Portable XRD analysis allows for simpler sample preparation, faster analytical times than traditional methods (less than 2 minutes), and can be performed at the sampling site in the field. A pure, finely ground

392

SLAC National Accelerator Laboratory - Fifth X-ray Instrument...  

NLE Websites -- All DOE Office Websites (Extended Search)

and more.) The technique has been used for years to probe materials with visible-light lasers, and more recently with X-ray light from synchrotrons. But the LCLS is the first...

393

SLAC National Accelerator Laboratory - X-ray Vision Exposes Aerosol...  

NLE Websites -- All DOE Office Websites (Extended Search)

up exciting possibilities in the study of aerosol dynamics using highly focused X-ray lasers, such as SLAC's Linac Coherent Light Source (LCLS). "Our study shows that LCLS can...

394

Lensless Imaging of Magnetic Nanostructures by X-ray Spectro...  

NLE Websites -- All DOE Office Websites (Extended Search)

F. Schlotter and J. Sthr (SSRL) The unprecedented properties of X-ray free electron lasers (X-FELs) under development world wide will open the door for entirely new classes of...

395

The Ulysses Catalog of Solar Hard X-Ray Flares  

E-Print Network (OSTI)

rupted full-Sun coverage of major solar X-ray ?are activity.of Ulysses from the Sun in AU, and its solar longitude andof the solar disk shows the view of the Sun from Earth,

Tranquille, C.; Hurley, K.; Hudson, H. S.

2009-01-01T23:59:59.000Z

396

Linda Young Named to Head X-ray Science Division  

NLE Websites -- All DOE Office Websites (Extended Search)

to the APS Hard X-ray Nanoprobe Earns an R&D 100 Award Winans of XSD Elected to ACS Fellowship Gluskin of Photon Sciences named Argonne Distinguished Fellow UChicago...

397

Radiological Safety Training for Radiation-Producing (X-Ray)...  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

for General Radiation Safety Installations Using Non-Medical X-Ray and Sealed Gamma-Ray Sources, Energies up to 10 MEV, ANSI Standard N43.3, American National Standards...

398

Low Dose Radiation Research Program: Comparison of Soft X Rays...  

NLE Websites -- All DOE Office Websites (Extended Search)

Comparison of Soft X-Rays and Ions Irradiation in a Model of V79 Mammalian Cell Authors: B. Ginovska, J.H. Miller, D. J. Lynch and W. E. Wilson Institutions: School of Electrical...

399

SLAC National Accelerator Laboratory - X-rays Reveal How Soil...  

NLE Websites -- All DOE Office Websites (Extended Search)

2012 Menlo Park, Calif. - Researchers working at the U.S. Department of Energy's (DOE) SLAC National Accelerator Laboratory have used powerful X-rays to help decipher how certain...

400

Argonne TDC: Large Area CCD X-Ray Detector  

Large-Area CCD X-Ray Detector Opening Up New Horizons in the Study of Cellular and Metabolic Processes, Genetics, and Drug Development 2000 R&D 100 Award Winner!

Note: This page contains sample records for the topic "wide-angle x-ray scattering" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


401

Vitreous carbon mask substrate for X-ray lithography  

DOE Patents (OSTI)

The present invention is directed to the use of vitreous carbon as a substrate material for providing masks for X-ray lithography. The new substrate also enables a small thickness of the mask absorber used to pattern the resist, and this enables improved mask accuracy. An alternative embodiment comprised the use of vitreous carbon as a LIGA substrate wherein the VC wafer blank is etched in a reactive ion plasma after which an X-ray resist is bonded. This surface treatment provides a surface enabling good adhesion of the X-ray photoresist and subsequent nucleation and adhesion of the electrodeposited metal for LIGA mold-making while the VC substrate practically eliminates secondary radiation effects that lead to delamination of the X-ray resist form the substrate, the loss of isolated resist features, and the formation of a resist layer adjacent to the substrate that is insoluble in the developer.

Aigeldinger, Georg (Livermore, CA); Skala, Dawn M. (Fremont, CA); Griffiths, Stewart K. (Livermore, CA); Talin, Albert Alec (Livermore, CA); Losey, Matthew W. (Livermore, CA); Yang, Chu-Yeu Peter (Dublin, CA)

2009-10-27T23:59:59.000Z

402

SLAC National Accelerator Laboratory - X-ray Laser Takes Aim...  

NLE Websites -- All DOE Office Websites (Extended Search)

Laser Takes Aim at Cosmic Mystery December 12, 2012 Menlo Park, Calif. - Scientists have used powerful X-rays from the Linac Coherent Light Source (LCLS) at the U.S. Department of...

403

SLAC National Accelerator Laboratory - X-ray Laser Sees Photosynthesis...  

NLE Websites -- All DOE Office Websites (Extended Search)

new window on the way plants generate the oxygen we breathe, researchers used an X-ray laser at the Department of Energy's (DOE) SLAC National Accelerator Laboratory to...

404

SLAC National Accelerator Laboratory - X-ray Laser Brings Cellular...  

NLE Websites -- All DOE Office Websites (Extended Search)

a March experiment indicates it has, for the first time, used an X-ray free-electron laser - SLAC's Linac Coherent Light Source - to reconstitute the structure of a G...

405

Material Characterization with X-ray and Optical Techniques I  

Science Conference Proceedings (OSTI)

In Situ X-ray Nanocharacterization of Defects in Solar Cells: Mariana Bertoni1; ... a strong modeling tool for predicting and optimizing solar cell efficiency. ... levels (11 steps up to 55%) in order to understand the sequential damage process.

406

SLAC National Accelerator Laboratory - X-rays Capture Electron...  

NLE Websites -- All DOE Office Websites (Extended Search)

X-rays Capture Electron 'Dance' By Glenn Roberts Jr. January 30, 2013 The way electrons move within and between molecules, transferring energy as they go, plays an important role...

407

Using Light to Control How X Rays Interact with Matter  

NLE Websites -- All DOE Office Websites (Extended Search)

Using Light to Control How X Rays Interact with Matter Print Schemes that use one light pulse to manipulate interactions of another with matter are well developed in the...

408

Heat conduction in X-ray clusters: Spitzer over 3  

E-Print Network (OSTI)

Effective heat conduction in a random variable magnetic field should be equal to one third of the Spitzer's value. Recent observations indicate that this heat conduction is sufficient to account for the bremsstrahlung in cooling X-ray clusters.

Andrei Gruzinov

2002-03-04T23:59:59.000Z

409

The Ulysses Catalog of Solar Hard X-Ray Flares  

E-Print Network (OSTI)

its Solar X-ray/Cosmic Gamma-Ray Burst Experiment (GRB) hasInstrument The Ulysses Gamma-Ray Burst (GRB) instrument, hasrate due to a cosmic gamma-ray burst or a solar ?are, but we

Tranquille, C.; Hurley, K.; Hudson, H. S.

2009-01-01T23:59:59.000Z

410

Towards hard x-ray imaging at GHz frame rate  

SciTech Connect

Gigahertz (GHz) imaging using hard x-rays ( Greater-Than-Or-Equivalent-To 10 keV) can be useful to high-temperature plasma experiments, as well as research and applications using coherent photons from synchrotron radiation and x-ray free electron lasers. GHz framing rate can be achieved by using multiple cameras through multiplexing. The advantages and trade-offs of single-photon detection mode, when no more than one x-ray photon is detected per pixel, are given. Two possible paths towards x-ray imaging at GHz frame rates using a single camera are: (a) avalanche photodiode arrays of high-Z materials and (b) microchannel plate photomultipliers in conjunction with materials with large indices of refraction.

Wang Zhehui; Morris, C. L.; Kapustinsky, J. S.; Kwiatkowski, K.; Luo, S.-N. [Los Alamos National Laboratory, Los Alamos, New Mexico 87545 (United States)

2012-10-15T23:59:59.000Z

411

Towards hard X-ray imaging at GHz frame rate  

Science Conference Proceedings (OSTI)

Gigahertz (GHz) imaging using hard X-rays ({approx}> 10 keV) can be useful to high-temperature plasma experiments, as well as research using coherent photons from synchrotron radiation and X-ray free electron lasers. GHz framing rate can be achieved by using multiple cameras through multiplexing. The advantages and trade-offs of single-photon detection mode, when no more than one X-ray photon is detected per pixel, are given. Two possible paths towards X-ray imaging at GHz frame rates using a single camera are (a) Avalanche photodiode arrays of high-Z materials and (b) Microchannel plate photomultipliers in conjunction with materials with large indices of refraction.

Wang, Zhehui [Los Alamos National Laboratory; Morris, Christopher [Los Alamos National Laboratory; Luo, Shengnian [Los Alamos National Laboratory; Kwiatkowski, Kris K. [Los Alamos National Laboratory; Kapustinsky, Jon S. [Los Alamos National Laboratory

2012-05-02T23:59:59.000Z

412

Science Challenges & Opportunities for an Advanced X-ray Free...  

NLE Websites -- All DOE Office Websites (Extended Search)

Science Challenges & Opportunities for an Advanced X-ray Free-electron Laser Wednesday, October 2, 2013 - 3:00pm SLAC, Kavli 3rd Floor Conference Room Robert Schoenlein, Lawrence...

413

SLAC National Accelerator Laboratory - X-ray Laser Research Ranks...  

NLE Websites -- All DOE Office Websites (Extended Search)

selected science "Breakthrough of the Year": the discovery of what appears to be the Higgs boson. Scientists aimed the Linac Coherent Light Source X-ray laser at thousands of tiny...

414

Calibration of High-Resolution X-Ray Tomography With ...  

Science Conference Proceedings (OSTI)

... The x-ray attenuation of the sample at this energy was close to the ... J. Coal Geol. ... G. Xu, DE Eastman, I. McNulty, SP Frigo, Y. Wang, CC Retsch, IC ...

2001-04-11T23:59:59.000Z

415

X-ray streak and framing camera techniques  

SciTech Connect

This paper reviews recent developments and applications of ultrafast diagnostic techniques for x-ray measurements. These techniques, based on applications of image converter devices, are already capable of significantly important resolution capabilities. Techniques capable of time resolution in the sub-nanosecond regime are being considered. Mechanical cameras are excluded from considerations as are devices using phosphors or fluors as x-ray converters.

Coleman, L.W.; Attwood, D.T.

1975-12-23T23:59:59.000Z

416

The complex soft X-ray spectrum of NGC 4151  

E-Print Network (OSTI)

We present a detailed analysis of the complex soft X-ray spectrum of NGC 4151 measured by the RGS instruments aboard XMM-Newton. The XMM-Newton RGS spectra demonstrate that the soft X-ray emission is extremely rich in X-ray emission lines and radiative recombination continua (RRC), with no clear evidence for any underlying continuum emission. Line emission, and the associated RRC, are clearly detected from hydrogen-like and helium-like ionization states of neon, oxygen, nitrogen and carbon. The measured lines are blueshifted with a velocity of between ~100-1000 km/s, with respect to the systemic velocity of NGC 4151, approximately consistent with the outflow velocities of the absorption lines observed in the UV, suggestive of an origin for the UV and soft X-ray emission in the same material. Plasma diagnostics imply a range of electron temperatures of ~1-5x10^4 K and electron densities of between 10^8-10^10 cm^-3. The soft X-ray spectrum of NGC 4151 is extremely similar to that of NGC 1068, suggesting that the soft X-ray excesses observed in many Seyfert galaxies may be composed of similar emission features. Modelling the RGS spectra in terms of emission from photoionized and photoexcited gas in an ionization cone reproduces all of the hydrogen-like and helium-like emission features observed in the soft X-ray spectrum of NGC 4151 in detail and confirms the correspondence between the soft X-ray emission in NGC 4151 and NGC 1068.

N. J. Schurch; R. S. Warwick; R. E. Griffiths; S. M. Kahn

2004-01-26T23:59:59.000Z

417

Apparatus for obtaining an X-ray image  

DOE Patents (OSTI)

A computed tomography apparatus in which a fan-shaped X-ray beam is caused to pass through a section of an object, enabling absorption detection on the opposite side of the object by a detector comprising a plurality of discrete detector elements. An electron beam generating the X-ray beam by impacting upon a target is caused to rotate over the target.

Watanabe, Eiji (Tokyo, JP)

1979-01-01T23:59:59.000Z

418

Kinoform optics applied to X-ray photon correlation specroscopy  

Science Conference Proceedings (OSTI)

Moderate-demagnification higher-order silicon kinoform focusing lenses have been fabricated to facilitate small-angle X-ray photon correlation spectroscopy (XPCS) experiments. The geometric properties of such lenses, their focusing performance and their applicability for XPCS measurements are described. It is concluded that one-dimensional vertical X-ray focusing via silicon kinoform lenses significantly increases the usable coherent flux from third-generation storage-ring light sources for small-angle XPCS experiments.

Sandy, A.R.; Evans-Lutterodt, K.; Narayanan, S.; Sprung, M.; Su, J.D; Isakovic, A.F.; Stein, A.

2010-03-01T23:59:59.000Z

419

Using Light to Control How X Rays Interact with Matter  

NLE Websites -- All DOE Office Websites (Extended Search)

Using Light to Control How X Rays Interact with Matter Print Using Light to Control How X Rays Interact with Matter Print Schemes that use one light pulse to manipulate interactions of another with matter are well developed in the visible-light regime where an optical control pulse influences how an optical probe pulse interacts with a medium. This approach has opened new research directions in fields like quantum computing and nonlinear optics, while also spawning entirely new research areas, such as electromagnetically induced transparency and slow light. However, it has been unclear whether similar optical control schemes could be used to modify how x rays interact with matter. In a dramatic breakthrough demonstration at the ALS, a Berkeley Lab-Argonne National Laboratory group has now used powerful visible-light lasers to render a nominally opaque material transparent to x rays. While x-ray transparency will have immediate applications at x-ray light sources, the important result is that the findings lay a foundation for a broader spectrum of applications.

420

Using Light to Control How X Rays Interact with Matter  

NLE Websites -- All DOE Office Websites (Extended Search)

Using Light to Control How X Rays Interact with Matter Print Using Light to Control How X Rays Interact with Matter Print Schemes that use one light pulse to manipulate interactions of another with matter are well developed in the visible-light regime where an optical control pulse influences how an optical probe pulse interacts with a medium. This approach has opened new research directions in fields like quantum computing and nonlinear optics, while also spawning entirely new research areas, such as electromagnetically induced transparency and slow light. However, it has been unclear whether similar optical control schemes could be used to modify how x rays interact with matter. In a dramatic breakthrough demonstration at the ALS, a Berkeley Lab-Argonne National Laboratory group has now used powerful visible-light lasers to render a nominally opaque material transparent to x rays. While x-ray transparency will have immediate applications at x-ray light sources, the important result is that the findings lay a foundation for a broader spectrum of applications.

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421

Using Light to Control How X Rays Interact with Matter  

NLE Websites -- All DOE Office Websites (Extended Search)

Using Light to Control How X Using Light to Control How X Rays Interact with Matter Using Light to Control How X Rays Interact with Matter Print Wednesday, 27 January 2010 00:00 Schemes that use one light pulse to manipulate interactions of another with matter are well developed in the visible-light regime where an optical control pulse influences how an optical probe pulse interacts with a medium. This approach has opened new research directions in fields like quantum computing and nonlinear optics, while also spawning entirely new research areas, such as electromagnetically induced transparency and slow light. However, it has been unclear whether similar optical control schemes could be used to modify how x rays interact with matter. In a dramatic breakthrough demonstration at the ALS, a Berkeley Lab-Argonne National Laboratory group has now used powerful visible-light lasers to render a nominally opaque material transparent to x rays. While x-ray transparency will have immediate applications at x-ray light sources, the important result is that the findings lay a foundation for a broader spectrum of applications.

422

Quiet Sun X-rays as Signature for New Particles  

E-Print Network (OSTI)

We have studied published data from the Yohkoh solar X-ray mission, with the purpose of searching for signals from radiative decays of new, as yet undiscovered massive neutral particles. This search is based on the prediction that solar axions of the Kaluza-Klein type should result in the emission of X-rays from the Sun direction beyond the limb with a characteristic radial distribution. These X-rays should be observed more easily during periods of quiet Sun. An additional signature is the observed emission of hard X-rays by SMM, NEAR and RHESSI. The recent observation made by RHESSI of a continuous emission from the non-flaring Sun of X-rays in the 3 to ~15 keV range fits the generic axion scenario. This work also suggests new analyses of existing data, in order to exclude instrumental effects; it provides the rationale for targeted observations with present and upcoming (solar) X-ray telescopes, which can provide the final answer on the nature of the signals considered here. Such measurements become more promising during the forthcoming solar cycle minimum with an increased number of quiet Sun periods.

K. Zioutas; K. Dennerl; L. DiLella; D. H. H. Hoffmann; J. Jacoby; Th. Papaevangelou

2004-03-08T23:59:59.000Z

423

Understanding Water Uptake and Transport in Nafion Using X-ray...  

NLE Websites -- All DOE Office Websites (Extended Search)

Understanding Water Uptake and Transport in Nafion Using X-ray Microtomography Title Understanding Water Uptake and Transport in Nafion Using X-ray Microtomography Publication Type...

424

Dilation x-ray imager a new/faster gated x-ray imager for the NIF  

SciTech Connect

As the yield on implosion shots increases it is expected that the peak x-ray emission reduces to a duration with a FWHM as short as 20 ps for {approx}7 Multiplication-Sign 10{sup 18} neutron yield. However, the temporal resolution of currently used gated x-ray imagers on the NIF is 40-100 ps. We discuss the benefits of the higher temporal resolution for the NIF and present performance measurements for dilation x-ray imager, which utilizes pulse-dilation technology [T. J. Hilsabeck et al., Rev. Sci. Instrum. 81, 10E317 (2010)] to achieve x-ray imaging with temporal gate times below 10 ps. The measurements were conducted using the COMET laser, which is part of the Jupiter Laser Facility at the Lawrence Livermore National Laboratory.

Nagel, S. R.; Bell, P. M.; Bradley, D. K.; Ayers, M. J.; Barrios, M. A.; Felker, B.; Smith, R. F.; Collins, G. W.; Jones, O. S.; Piston, K.; Raman, K. S. [Lawrence Livermore National Laboratory, 7000 East Avenue, Livermore, California 94550 (United States); Hilsabeck, T. J.; Kilkenny, J. D.; Chung, T.; Sammuli, B. [General Atomics, P.O. Box 85608, San Diego, California 92186-5608 (United States); Hares, J. D.; Dymoke-Bradshaw, A. K. L. [Kentech Instruments Ltd., Wallingford, Oxfordshire OX10 (United Kingdom)

2012-10-15T23:59:59.000Z

425

HSQ double patterning process for 12 nm resolution x-ray zone plates  

DOE Green Energy (OSTI)

Soft x-ray zone plate microscopy is a powerful nano-analytic technique used for a wide variety of scientific and technological studies. Pushing its spatial resolution to 10 nm and below is highly desired and feasible due to the short wavelength of soft x-rays. Instruments using Fresnel zone plate lenses achieve a spatial resolution approximately equal to the smallest, outer most zone width. We developed a double patterning zone plate fabrication process based on a high-resolution resist, hydrogen silsesquioxane (HSQ), to bypass the limitations of conventional single exposure fabrication to pattern density, such as finite beam size, scattering in resist and modest intrinsic resist contrast. To fabricate HSQ structures with zone widths in the order of 10 nm on gold plating base, a surface conditioning process with (3-mercaptopropyl) trimethoxysilane, 3-MPT, is used, which forms a homogeneous hydroxylation surface on gold surface and provides good anchoring for the desired HSQ structures. Using the new HSQ double patterning process, coupled with an internally developed, sub-pixel alignment algorithm, we have successfully fabricated in-house gold zone plates of 12 nm outer zones. Promising results for 10 nm zone plates have also been obtained. With the 12 nm zone plates, we have achieved a resolution of 12 nm using the full-field soft x-ray microscope, XM-1.

Chao, Weilun; Kim, Jihoon; Rekawa, Senajith; Fischer, Peter; Anderson, Erik H.

2009-06-16T23:59:59.000Z

426

Dynamics and rheology under continuous shear flow studied by X-ray photon correlation spectroscopy  

E-Print Network (OSTI)

X-ray Photon Correlation Spectroscopy (XPCS) has emerged as a unique technique allowing the measurement of dynamics in materials on mesoscopic lengthscales. In particular, applications in soft matter physics cover a broad range of topics which include, but are not limited to, nanostructured materials such as colloidal suspensions or polymers, dynamics at liquid surfaces, membranes and interfaces, and the glass or gel transition. One of the most common problems associated with the use of bright X-ray beams with soft materials is beam induced radiation damage, and this is likely to become an even more limiting factor at future synchrotron and free electron laser sources. Flowing the sample during data acquisition is one of the simplest method allowing to limit the radiation damage. In addition to distributing the dose over many different scatterers, the method also enables new functionalities such as time-resolved studies in mixing cells. Here, we further develop an experimental technique that was recently proposed combining XPCS and continuously flowing samples. More specifically, we use a model system to show how the macroscopic advective response to flow and the microscopic dissipative dynamics (diffusion) can be quantified from the X-ray data. The method has many potential applications, e.g. dynamics of glasses and gels under continuous shear/flow, protein aggregations processes, the interplay between dynamics and rheology in complex fluids.

Andrei Fluerasu; Pawel Kwasniewski; Chiara Caronna; Fanny Destremaut; Jean-Baptiste Salmon; Anders Madsen

2010-01-10T23:59:59.000Z

427

SPEAR3 Beam Line Availability  

NLE Websites -- All DOE Office Websites (Extended Search)

Beam Line Support | Floor Support | Administrative Support SPEAR3 Beam Line Availability Beam Line BL Type Technique(s) Status 1-4 X-ray Small and Wide Angle X-ray Scattering Open...

428

NEUTRON AND SYNCHROTRON X-RAY FIBER DIFFRACTION STUDIES OF CELLULOSE POLYMORPHS.  

DOE Green Energy (OSTI)

Although the crystalline nature of cellulose has been one of most studied structural problems in polymer science there remain many open questions. Cellulose is a polymer formed by (1-4)-linked {beta}-D-glucosyl residues that are alternately rotated by 180o along the polymer axis to form flat ribbon-like chains. Each glucosyl unit bears three hydroxyl groups, one an hydroxymethyl group. It has been long recognized that these hydroxyl groups and their ability to bond via hydrogen bonding not only play a major role in directing how the crystal structure of cellulose forms but also in governing important physical properties of cellulose materials. Through the development of new techniques we have been able to prepare fiber samples of cellulose with exceptionally high order. The quality of these samples is allowing us to exploit the unique properties of synchrotron X-ray and neutron sources in order to collect diffraction data to near atomic resolution. Synchrotron X-rays are used to provide accurate crystallographic parameters for C and O atoms. However, because of the relatively weak scattering power of H atoms for X-rays, neutrons are used to determine H atom parameters. We have developed methods for replacing labile H atoms with D, without any loss in crystalline perfection. Deuterated fibers can diffract neutrons with intensities that are substantially different from the intensities diffracted from hydrogenated fibers. These differences, along with the phases calculated from the C and O positions determined in our X-ray studies, are used to calculate Fourier difference syntheses in which density associated with labile hydrogen atoms is imaged. The unprecedented high resolution of these data is revealing new information on cellulose structure and hydrogen bonding.

Los Alamos National Laboratory

2001-01-01T23:59:59.000Z

429

Electronic State Interferences in Resonant X-Ray Emission after K-Shell Excitation in HCl  

SciTech Connect

We have measured a series of high-resolution x-ray spectra emitted upon resonant photoexcitation of HCl. The photon energy was tuned across the dissociative 1s{yields}6{sigma}* resonance and the Rydberg states converging to the Cl 1s{sup -1} threshold, and inelastic photon scattering was observed in the region of KL emission lines. Excellent agreement is found between fully ab initio calculated and measured spectra if interferences between different excitation-emission paths are taken into account. The effect of electronic state interferences is enhanced due to dynamical broadening of the 6{sigma}* resonance in HCl.

Kavcic, M.; Zitnik, M.; Bucar, K.; Mihelic, A.; Carniato, S.; Journel, L.; Guillemin, R.; Simon, M. [Jozef Stefan Institute, Post Office Box 3000, SI-1001 Ljubljana (Slovenia); UPMC Univ Paris 06, UMR 7614, Laboratoire de Chimie Physique Matiere et Rayonnement, F-75005 Paris (France); CNRS, UMR 7614, Laboratoire de Chimie Physique Matiere et Rayonnement, F-75005 Paris (France)

2010-09-10T23:59:59.000Z

430

Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism  

NLE Websites -- All DOE Office Websites (Extended Search)

Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism Print Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism Print Using spectroscopic information for magnetometry and magnetic microscopy obviously requires detailed theoretical understanding of spectral shape and magnitude of dichroism signals. A research team at ALS Beamline 4.0.2 has now shown unambiguously that, contrary to common belief, spectral shape and magnitude of x-ray magnetic linear dichroism (XMLD) are not only determined by the relative orientation of magnetic moments and x-ray polarization, but their orientation relative to the crystallographic axes must be taken into account for accurate interpretation of XMLD data. Magnetism and X Rays The ancient Greeks and also the Chinese knew about strange and rare stones with the power to attract iron. Moreover, when freely suspended these objects pointed north-south. Throughout the past, we have used this phenomenon-magnetism-for navigation and more recently for power production and digital information storage, all while trying to explore and understand its origins. In 1986 researchers at a facility similar to the ALS observed for the first time that the absorption of x rays depends not only on the composition of a material-that is, if it contains iron, nickel, or other elements-but also on its magnetism. The effect is unique in that it allows us to distinguish which atomic species magnetism originates from and provides information about their local atomic environment-for example, whether a magnetic species is surrounded by 4 or 6 oxygen atoms. A research team at the ALS has now shown that the relationship between magnetic order and absorption of x rays is even more complex and exciting than has been assumed for the past 20 years, leading to a reassessment of previous results.

431

Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism  

NLE Websites -- All DOE Office Websites (Extended Search)

Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism Print Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism Print Using spectroscopic information for magnetometry and magnetic microscopy obviously requires detailed theoretical understanding of spectral shape and magnitude of dichroism signals. A research team at ALS Beamline 4.0.2 has now shown unambiguously that, contrary to common belief, spectral shape and magnitude of x-ray magnetic linear dichroism (XMLD) are not only determined by the relative orientation of magnetic moments and x-ray polarization, but their orientation relative to the crystallographic axes must be taken into account for accurate interpretation of XMLD data. Magnetism and X Rays The ancient Greeks and also the Chinese knew about strange and rare stones with the power to attract iron. Moreover, when freely suspended these objects pointed north-south. Throughout the past, we have used this phenomenon-magnetism-for navigation and more recently for power production and digital information storage, all while trying to explore and understand its origins. In 1986 researchers at a facility similar to the ALS observed for the first time that the absorption of x rays depends not only on the composition of a material-that is, if it contains iron, nickel, or other elements-but also on its magnetism. The effect is unique in that it allows us to distinguish which atomic species magnetism originates from and provides information about their local atomic environment-for example, whether a magnetic species is surrounded by 4 or 6 oxygen atoms. A research team at the ALS has now shown that the relationship between magnetic order and absorption of x rays is even more complex and exciting than has been assumed for the past 20 years, leading to a reassessment of previous results.

432

Tokamak physics studies using x-ray diagnostic methods  

SciTech Connect

X-ray diagnostic measurements have been used in a number of experiments to improve our understanding of important tokamak physics issues. The impurity content in TFTR plasmas, its sources and control have been clarified through soft x-ray pulse-height analysis (PHA) measurements. The dependence of intrinsic impurity concentrations and Z/sub eff/ on electron density, plasma current, limiter material and conditioning, and neutral-beam power have shown that the limiter is an important source of metal impurities. Neoclassical-like impurity peaking following hydrogen pellet injection into Alcator C and a strong effect of impurities on sawtooth behavior were demonstrated by x-ray imaging (XIS) measurements. Rapid inward motion of impurities and continuation of m = 1 activity following an internal disruption were demonstrated with XIS measurements on PLT using injected aluminum to enhance the signals. Ion temperatures up to 12 keV and a toroidal plasma rotation velocity up to 6 x 10/sup 5/ m/s have been measured by an x-ray crystal spectrometer (XCS) with up to 13 MW of 85-keV neutral-beam injection in TFTR. Precise wavelengths and relative intensities of x-ray lines in several helium-like ions and neon-like ions of silver have been measured in TFTR and PLT by the XCS. The data help to identify the important excitation processes predicted in atomic physics. Wavelengths of n = 3 to 2 silver lines of interest for x-ray lasers were measured, and precise instrument calibration techniques were developed. Electron thermal conductivity and sawtooth dynamics have been studied through XIS measurements on TFTR of heat-pulse propagation and compound sawteeth. A non-Maxwellian electron distribution function has been measured, and evidence of the Parail-Pogutse instability identified by hard x-ray PHA measurements on PLT during lower-hybrid current-drive experiments.

Hill, K.W.; Bitter, M.; von Goeler, S.; Beiersdorfer, P.; Fredrickson, E.; Hsuan, H.; McGuire, K.; Sauthoff, N.R.; Sesnic, S.; Stevens, J.E.

1987-03-01T23:59:59.000Z

433

Water destruction by X-rays in young stellar objects  

E-Print Network (OSTI)

We study the H2O chemistry in star-forming environments under the influence of a central X-ray source and a central far ultraviolet (FUV) radiation field. The gas-phase water chemistry is modeled as a function of time, hydrogen density and X-ray flux. To cover a wide range of physical environments, densities between n_H = 10^4-10^9 cm^-3 and temperatures between T = 10-1000 K are studied. Three different regimes are found: For T water abundance is of order 10^-7-10^-6 and can be somewhat enhanced or reduced due to X-rays, depending on time and density. For 100 K 10^-3 ergs s-1 cm^-2 (t = 10^4 yrs) and for F_X > 10^-4 ergs s^-1 cm^-2 (t = 10^5 yrs). At higher temperatures (T > 250 K) and hydrogen densities, water can persist with x(H2O) ~ 10^-4 even for high X-ray fluxes. The X-ray and FUV models are applied to envelopes around low-mass Class 0 and I young stellar objects (YSOs). Water is destroyed in both Class 0 and I envelopes on relatively short timescales (t ~ 5000 yrs) for realistic X-ray fluxes, although the effect is less prominent in Class 0 envelopes due to the higher X-ray absorbing densities there. FUV photons from the central source are not effective in destroying water. The average water abundance in Class I sources for L_X > 10^27 ergs s^-1 is predicted to be x(H2O) < 10^-6.

P. Stauber; J. K. Jorgensen; E. F. van Dishoeck; S. D. Doty; A. O. Benz

2006-02-06T23:59:59.000Z

434

Formation and destruction of jets in X-ray binaries  

E-Print Network (OSTI)

Neutron-star and black-hole X-ray binaries (XRBs) exhibit radio jets, whose properties depend on the X-ray spectral state and history of the source. In particular, black-hole XRBs emit compact, steady radio jets when they are in the so-called hard state, the jets become eruptive as the sources move toward the soft state, disappear in the soft state, and re-appear when the sources return to the hard state. On the other hand, jets from neutron-star X-ray binaries are typically weaker radio emitters than the black-hole ones at the same X-ray luminosity and in some cases radio emission is detected in the soft state. Significant phenomenology has been accumulated so far regarding the spectral states of neutron-star and black-hole XRBs, and there is general agreement about the type of the accretion disk around the compact object in the various spectral states. Our aim is to investigate whether the phenomenology regarding the X-ray emission on one hand and the jet appearance and disappearance on the other can be put...

Kylafis, N D; Kazanas, D; Christodoulou, D M

2011-01-01T23:59:59.000Z

435

Viewing spin structures with soft x-ray microscopy  

SciTech Connect

The spin of the electron and its associated magnetic moment marks the basic unit for magnetic properties of matter. Magnetism, in particular ferromagnetism and antiferromagnetism is described by a collective order of these spins, where the interaction between individual spins reflects a competition between exchange, anisotropy and dipolar energy terms. As a result the energetically favored ground state of a ferromagnetic system is a rather complex spin configuration, the magnetic domain structure. Magnetism is one of the eldest scientific phenomena, yet it is one of the most powerful and versatile utilized physical effects in modern technologies, such as in magnetic storage and sensor devices. To achieve highest storage density, the relevant length scales, such as the bit size in disk drives is now approaching the nanoscale and as such further developments have to deal with nanoscience phenomena. Advanced characterization tools are required to fully understand the underlying physical principles. Magnetic microscopes using polarized soft X-rays offer a close-up view into magnetism with unique features, these include elemental sensitivity due to X-ray magnetic dichroism effects as contrast mechanism, high spatial resolution provided by state-of-the-art X-ray optics and fast time resolution limited by the inherent time structure of current X-ray sources, which will be overcome with the introduction of ultrafast and high brilliant X-ray sources.

Fischer, Peter

2010-06-01T23:59:59.000Z

436

YOHKOH remnants: partially occulted flares in hard X-rays  

E-Print Network (OSTI)

Flares being partially occulted by the solar limb, are the best reservoir of our knowledge about hard X-ray loop-top sources. Recently, the survey of partially occulted flares observed by the RHESSI has been published (Krucker & Lin 2008). The extensive YOHKOH database still awaits such activities. This work is an attempt to fill this gap. Among from 1286 flares in the YOHKOH Hard X-ray Telescope Flare Catalogue, for which the hard X-ray images had been enclosed, we identified 98 events that occurred behind the solar limb. We investigated their hard X-ray spectra and spatial structure. We found that in most cases the hard X-ray spectrum of partially occulted flares consists of two components, non-thermal and thermal, which are co-spatial. The photon energy spectra of the partially occulted flares are systematically steeper than spectra of the non-occulted flares. Such a difference we explain as a consequence of intrinsically dissimilar conditions ruling in coronal parts of flares, in comparison with the f...

Tomczak, M

2009-01-01T23:59:59.000Z

437

Method and apparatus for micromachining using hard X-rays  

DOE Patents (OSTI)

An X-ray source such as a synchrotron which provides a significant spectral content of hard X-rays is used to expose relatively thick photoresist such that the portions of the photoresist at an exit surface receive at least a threshold dose sufficient to render the photoresist susceptible to a developer, while the entrance surface of the photoresist receives an exposure which does not exceed a power limit at which destructive disruption of the photoresist would occur. The X-ray beam is spectrally shaped to substantially eliminate lower energy photons while allowing a substantial flux of higher energy photons to pass through to the photoresist target. Filters and the substrate of the X-ray mask may be used to spectrally shape the X-ray beam. Machining of photoresists such as polymethylmethacrylate to micron tolerances may be obtained to depths of several centimeters, and multiple targets may be exposed simultaneously. The photoresist target may be rotated and/or translated in the beam to form solids of rotation and other complex three-dimensional structures.

Siddons, David Peter (Shoreham, NY); Johnson, Erik D. (Ridge, NY); Guckel, Henry (Madison, WI); Klein, Jonathan L. (Madison, WI)

1997-10-21T23:59:59.000Z

438

Method and apparatus for micromachining using hard X-rays  

DOE Patents (OSTI)

An X-ray source such as a synchrotron which provides a significant spectral content of hard X-rays is used to expose relatively thick photoresist such that the portions of the photoresist at an exit surface receive at least a threshold dose sufficient to render the photoresist susceptible to a developer, while the entrance surface of the photoresist receives an exposure which does not exceed a power limit at which destructive disruption of the photoresist would occur. The X-ray beam is spectrally shaped to substantially eliminate lower energy photons while allowing a substantial flux of higher energy photons to pass through to the photoresist target. Filters and the substrate of the X-ray mask may be used to spectrally shape the X-ray beam. Machining of photoresists such as polymethylmethacrylate to micron tolerances may be obtained to depths of several centimeters, and multiple targets may be exposed simultaneously. The photoresist target may be rotated and/or translated in the beam to form solids of rotation and other complex three-dimensional structures. 21 figs.

Siddons, D.P.; Johnson, E.D.; Guckel, H.; Klein, J.L.

1997-10-21T23:59:59.000Z

439

Ultrafast x-ray diagnostics for laser fusion experiments  

SciTech Connect

Temporally, spectrally, and spatially resolved x-ray emission diagnostics are important tools in the study of the heating and compression of laser fusion targets by sub-nanosecond laser pulses. The use of the Livermore 15 psec resolution x-ray streak camera to make such measurements is reviewed. Temporal histories of spectrally resolved x-ray emission in the 1 to 10 keV range have been obtained. These data have served to further define the x-ray streak camera as a quantative diagnostic tool and have also provided data relating to the absorption and compression phases of laser heating. The x-ray streak camera has been used in conjunction with a specially designed pinhole imaging system to temporally record images of laser compressed targets with a spatial resolution of approximately 6 ..mu..m. Implosion characteristics are presented for experiments with glass microshell targets. The concept, development, and testing of an ultrafast framing camera for full two-dimensional time resolved imaging is discussed. A prototype camera, based on the image dissection-restoration concept, has achieved an approximately 200 psec frame period with a resolution of 50 ..mu..m.

Coleman, L.W.

1976-08-16T23:59:59.000Z

440

The complex soft X-ray spectrum of NGC 4151  

E-Print Network (OSTI)

We present a detailed analysis of the complex soft X-ray spectrum of NGC 4151 measured by the RGS instruments aboard XMM-Newton. The XMM-Newton RGS spectra demonstrate that the soft X-ray emission is extremely rich in X-ray emission lines and radiative recombination continua (RRC), with no clear evidence for any underlying continuum emission. Line emission, and the associated RRC, are clearly detected from hydrogen-like and helium-like ionization states of neon, oxygen, nitrogen and carbon. The measured lines are blueshifted with a velocity of between ?100-1000 km s ?1, with respect to the systemic velocity of NGC 4151, approximately consistent with the outflow velocities of the absorption lines observed in the UV spectrum of NGC 4151 (Kriss et al. 1995), suggestive of an origin for the UV and soft X-ray emission in the same material. Plasma diagnostics from the observed helium-like triplets, imply a range of electron temperatures of ?1-5×10 4 K and electron densities of between 10 8-10 10 cm ?3. The soft X-ray spectrum of NGC 4151 is extremely similar to that of NGC 1068, both in terms of the atomic species present and in terms of the relative strengths

N. J. Schurch; R. S. Warwick; R. E. Griffiths; S. M. Kahn

2004-01-01T23:59:59.000Z

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441

The complex soft X-ray spectrum of NGC 4151  

E-Print Network (OSTI)

We present a detailed analysis of the complex soft X-ray spectrum of NGC 4151 measured by the RGS instruments aboard XMM-Newton. The XMM-Newton RGS spectra demonstrate that the soft X-ray emission is extremely rich in X-ray emission lines and radiative recombination continua (RRC), with no clear evidence for any underlying continuum emission. Line emission, and the associated RRC, are clearly detected from hydrogen-like and helium-like ionization states of neon, oxygen, nitrogen and carbon. The measured lines are blueshifted with a velocity of between ~100-1000 km/s, with respect to the systemic velocity of NGC 4151, approximately consistent with the outflow velocities of the absorption lines observed in the UV, suggestive of an origin for the UV and soft X-ray emission in the same material. Plasma diagnostics imply a range of electron temperatures of ~1-5x10^4 K and electron densities of between 10^8-10^10 cm^-3. The soft X-ray spectrum of NGC 4151 is extremely similar to that of NGC 1068, suggesting that th...

Schurch, N J; Griffiths, R E; Kahn, S M

2004-01-01T23:59:59.000Z

442

The History of X-ray Free-Electron Lasers  

Science Conference Proceedings (OSTI)

The successful lasing at the SLAC National Accelerator Laboratory of the Linear Coherent Light Source (LCLS), the first X-ray free-electron laser (X-ray FEL), in the wavelength range 1.5 to 15 {angstrom}, pulse duration of 60 to few femtoseconds, number of coherent photons per pulse from 10{sup 13} to 10{sup 11}, is a landmark event in the development of coherent electromagnetic radiation sources. Until now electrons traversing an undulator magnet in a synchrotron radiation storage ring provided the best X-ray sources. The LCLS has set a new standard, with a peak X-ray brightness higher by ten orders of magnitudes and pulse duration shorter by three orders of magnitudes. LCLS opens a new window in the exploration of matter at the atomic and molecular scales of length and time. Taking a motion picture of chemical processes in a few femtoseconds or less, unraveling the structure and dynamics of complex molecular systems, like proteins, are some of the exciting experiments made possible by LCLS and the other X-ray FELs now being built in Europe and Asia. In this paper, we describe the history of the many theoretical, experimental and technological discoveries and innovations, starting from the 1960s and 1970s, leading to the development of LCLS.

Pellegrini, C.; /UCLA /SLAC

2012-06-28T23:59:59.000Z

443

Flat Field Anomalies in an X-ray CCD Camera Measured Using a Manson X-ray Source  

SciTech Connect

The Static X-ray Imager (SXI) is a diagnostic used at the National Ignition Facility (NIF) to measure the position of the X-rays produced by lasers hitting a gold foil target. The intensity distribution taken by the SXI camera during a NIF shot is used to determine how accurately NIF can aim laser beams. This is critical to proper NIF operation. Imagers are located at the top and the bottom of the NIF target chamber. The CCD chip is an X-ray sensitive silicon sensor, with a large format array (2k x 2k), 24 ?m square pixels, and 15 ?m thick. A multi-anode Manson X-ray source, operating up to 10kV and 10W, was used to characterize and calibrate the imagers. The output beam is heavily filtered to narrow the spectral beam width, giving a typical resolution E/?E?10. The X-ray beam intensity was measured using an absolute photodiode that has accuracy better than 1% up to the Si K edge and better than 5% at higher energies. The X-ray beam provides full CCD illumination and is flat, within ±1% maximum to minimum. The spectral efficiency was measured at 10 energy bands ranging from 930 eV to 8470 eV. We observed an energy dependent pixel sensitivity variation that showed continuous change over a large portion of the CCD. The maximum sensitivity variation occurred at 8470 eV. The geometric pattern did not change at lower energies, but the maximum contrast decreased and was not observable below 4 keV. We were also able to observe debris, damage, and surface defects on the CCD chip. The Manson source is a powerful tool for characterizing the imaging errors of an X-ray CCD imager. These errors are quite different from those found in a visible CCD imager.

M. J. Haugh and M. B. Schneider

2008-10-31T23:59:59.000Z

444

ON THE X-RAY OUTBURSTS OF TRANSIENT ANOMALOUS X-RAY PULSARS AND SOFT GAMMA-RAY REPEATERS  

SciTech Connect

We show that the X-ray outburst light curves of four transient anomalous X-ray pulsars (AXPs) and soft gamma-ray repeaters (SGRs), namely, XTE J1810-197, SGR 0501+4516, SGR 1627-41, and CXOU J164710.2-455216, can be produced by the fallback disk model that was also applied to the outburst light curves of persistent AXPs and SGRs in our earlier work. The model solves the diffusion equation for the relaxation of a disk that has been pushed back by a soft gamma-ray burst. The sets of main disk parameters used for these transient sources are very similar to each other and to those employed in our earlier models of persistent AXPs and SGRs. There is a characteristic difference between the X-ray outburst light curves of transient and persistent sources. This can be explained by the differences in the disk surface density profiles of the transient and persistent sources in quiescence indicated by their quiescent X-ray luminosities. Our results imply that a viscous disk instability operating at a critical temperature in the range of {approx}1300-2800 K is a common property of all fallback disks around AXPs and SGRs. The effect of the instability is more pronounced and starts earlier for the sources with lower quiescent luminosities, which leads to the observable differences in the X-ray enhancement light curves of transient and persistent sources. A single active disk model with the same basic disk parameters can account for the enhancement phases of both transient and persistent AXPs and SGRs. We also present a detailed parameter study to show the effects of disk parameters on the evolution of the X-ray luminosity of AXPs and SGRs in the X-ray enhancement phases.

Cal Latin-Small-Letter-Dotless-I skan, Sirin; Ertan, Uenal [Sabanc Latin-Small-Letter-Dotless-I University, Orhanl Latin-Small-Letter-Dotless-I -Tuzla, Istanbul, 34956 (Turkey)

2012-10-20T23:59:59.000Z

445

New Homogeneous Standards by Atomic Layer Deposition for Synchrotron X-ray Fluorescence and Absorption Spectroscopies.  

SciTech Connect

Quantification of synchrotron XRF analyses is typically done through comparisons with measurements on the NIST SRM 1832/1833 thin film standards. Unfortunately, these standards are inhomogeneous on small scales at the tens of percent level. We are synthesizing new homogeneous multilayer standards using the Atomic Layer Deposition technique and characterizing them using multiple analytical methods, including ellipsometry, Rutherford Back Scattering at Evans Analytical, Synchrotron X-ray Fluorescence (SXRF) at Advanced Photon Source (APS) Beamline 13-ID, Synchrotron X-ray Absorption Spectroscopy (XAS) at Advanced Light Source (ALS) Beamlines 11.0.2 and 5.3.2.1 and by electron microscopy techniques. Our motivation for developing much-needed cross-calibration of synchrotron techniques is borne from coordinated analyses of particles captured in the aerogel of the NASA Stardust Interstellar Dust Collector (SIDC). The Stardust Interstellar Dust Preliminary Examination (ISPE) team have characterized three sub-nanogram, {approx}1{micro}m-sized fragments considered as candidates to be the first contemporary interstellar dust ever collected, based on their chemistries and trajectories. The candidates were analyzed in small wedges of aerogel in which they were extracted from the larger collector, using high sensitivity, high spatial resolution >3 keV synchrotron x-ray fluorescence spectroscopy (SXRF) and <2 keV synchrotron x-ray transmission microscopy (STXM) during Stardust ISPE. The ISPE synchrotron techniques have complementary capabilities. Hard X-ray SXRF is sensitive to sub-fg mass of elements Z {ge} 20 (calcium) and has a spatial resolution as low as 90nm. X-ray Diffraction data were collected simultaneously with SXRF data. Soft X-ray STXM at ALS beamline 11.0.2 can detect fg-mass of most elements, including cosmochemically important oxygen, magnesium, aluminum and silicon, which are invisible to SXRF in this application. ALS beamline 11.0.2 has spatial resolution better than 25 nm. Limiting factors for Stardust STXM analyses were self-imposed limits of photon dose due to radiation damage concerns, and significant attenuation of <1500 eV X-rays by {approx}80{micro}m thick, {approx}25 mg/cm{sup 3} density silica aerogel capture medium. In practice, the ISPE team characterized the major, light elements using STXM (O, Mg, Al, Si) and the heavier minor and trace elements using SXRF. The two data sets overlapped only with minor Fe and Ni ({approx}1% mass abundance), providing few quantitative cross-checks. New improved standards for cross calibration are essential for consortium-based analyses of Stardust interstellar and cometary particles, IDPs. Indeed, they have far reaching application across the whole synchrotron-based analytical community. We have synthesized three ALD multilayers simultaneously on silicon nitride membranes and silicon and characterized them using RBS (on Si), XRF (on Si{sub 3}N{sub 4}) and STXM/XAS (holey Si{sub 3}N{sub 4}). The systems we have started to work with are Al-Zn-Fe and Y-Mg-Er. We have found these ALD multi-layers to be uniform at {micro}m- to nm scales, and have found excellent consistency between four analytical techniques so far. The ALD films can also be used as a standard for e-beam instruments, eg., TEM EELS or EDX. After some early issues with the consistency of coatings to the back-side of the membrane windows, we are confident to be able to show multi-analytical agreement to within 10%. As the precision improves, we can use the new standards to verify or improve the tabulated cross-sections.

Butterworth, A.L.; Becker, N.; Gainsforth, Z.; Lanzirotti, A.; Newville, M.; Proslier, T.; Stodolna, J.; Sutton, S.; Tyliszczak, T.; Westphal, A.J.; Zasadzinski, J. (UCB)

2012-03-13T23:59:59.000Z

446

Phase Contrast Microscopy with Soft and Hard X-rays Using a Segmented  

E-Print Network (OSTI)

Phase Contrast Microscopy with Soft and Hard X-rays Using a Segmented Detector A Dissertation Contrast Microscopy with Soft and Hard X-rays Using a Segmented Detector by Benjamin Hornberger Doctor. In the hard x-ray range (multi-keV), the main focus lies on trace ele- ment mapping by x-ray fluorescence

447

HARD X-RAY AND MICROWAVE OBSERVATIONS OF MICROFLARES Jiong Qiu,1, 2  

E-Print Network (OSTI)

HARD X-RAY AND MICROWAVE OBSERVATIONS OF MICROFLARES Jiong Qiu,1, 2 Chang Liu,2 Dale E. Gary,2 Gelu, we study solar microflares using the coordinated hard X-ray and microwave observations obtained the time derivative of soft X-rays and 14­20 keV hard X-rays, i.e., the Neupert effect, in about one

448

Exploring nanomagnetism with soft x-ray microscopy  

SciTech Connect

Magnetic soft X-ray microscopy images magnetism in nanoscale systems with a spatial resolution down to 15nm provided by state-of-the-art Fresnel zone plate optics. X-ray magnetic circular dichroism (X-MCD) is used as element-specific magnetic contrast mechanism similar to photoemission electron microscopy (PEEM), however, with volume sensitivity and the ability to record the images in varying applied magnetic fields which allows to study magnetization reversal processes at fundamental length scales. Utilizing a stroboscopic pump-probe scheme one can investigate fast spin dynamics with a time resolution down to 70 ps which gives access to precessional and relaxation phenomena as well as spin torque driven domain wall dynamics in nanoscale systems. Current developments in zone plate optics aim for a spatial resolution towards 10nm and at next generation X-ray sources a time resolution in the fsec regime can be envisioned.

Fischer, P.; Kim, D.-H.; Mesler, B.L.; Chao, W.; Sakdinawat,A.E.; Anderson, E.H.