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Sample records for resonant soft x-ray

  1. Resonant Soft X-Ray Scattering - Combining Structural with Spectroscopic

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Refinement | Stanford Synchrotron Radiation Lightsource Resonant Soft X-Ray Scattering - Combining Structural with Spectroscopic Refinement Friday, September 28, 2012 - 10:00am SLAC, Bldg. 137, Room 322 SSRL Presents Kevin Stone X-ray absorption spectroscopy has become an important tool in understanding the electronic structure of materials. Resonant absorption edges in the soft x-ray regime are especially interesting as they allow the study of the lighter elements, such as in organic or

  2. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

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    Resonant Soft X-Ray Scattering of Tri-Block Copolymers Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print Wednesday, 30 May 2012 00:00 In principle, tri-block copolymers...

  3. Molecular orientation in soft matter thin films studied by resonant soft x-ray reflectivity

    SciTech Connect (OSTI)

    Mezger, Markus; Jerome, Blandine; Kortright, Jeffrey B; Valvidares, Manuel; Gullikson, Eric M; Giglia, Angelo; Mahne, Nicola; Nannarone, Stefano

    2011-04-05

    We present a technique to study depth profiles of molecular orientation in soft matter thin films with nanometer resolution. The method is based on dichroism in resonant soft x-ray reflectivity using linear s and p polarization. It combines the chemical sensitivity of near-edge x-ray absorption fine structure spectroscopy to specific molecular bonds and their orientation relative to the polarization of the incident beam with the precise depth profiling capability of x-ray reflectivity. We demonstrate these capabilities on side chain liquid crystalline polymer thin films with soft x-ray reflectivity data at the carbon K edge. Optical constants of the anisotropic refractive index ellipsoid were obtained from a quantitative analysis using the Berreman formalism. For films up to 50 nm thickness we find that the degree of orientation of the long axis exhibits no depth variation and is independent of the film thickness.

  4. Molecular orientation in soft matter thin films studied by resonant soft X-ray reflectivity

    SciTech Connect (OSTI)

    Mezger, Markus; Jerome, Blandine; Kortright, Jeffrey B.; Valvidares, Manuel; Gullikson, Eric; Giglia, Angelo; Mahne, Nicola; Nannarone, Stefano

    2011-01-12

    We present a technique to study depth profiles of molecular orientation in soft matter thin films with nanometer resolution. The method is based on dichroism in resonant soft X-ray reflectivity using linear s- and p-polarization. It combines the chemical sensitivity of Near-Edge X-ray Absorption Fine Structure spectroscopy to specific molecular bonds and their orientation relative to the polarization of the incident beam with the precise depth profiling capability of X-ray reflectivity. We demonstrate these capabilities on side chain liquid crystalline polymer thin films with soft X-ray reflectivity data at the carbon K edge. Optical constants of the anisotropic refractive index ellipsoid were obtained from a quantitative analysis using the Berreman formalism. For films up to 50 nm thickness we find that the degree of orientation of the long axis exhibits no depth variation and isindependent of the film thickness.

  5. Resonant elastic soft x-ray scattering in oxygen-ordered YBa2Cu3O6...

    Office of Scientific and Technical Information (OSTI)

    Resonant elastic soft x-ray scattering in oxygen-ordered YBa2Cu3O6+ Citation Details In-Document Search Title: Resonant elastic soft x-ray scattering in oxygen-ordered...

  6. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print In principle, tri-block copolymers (tri-BCPs), consisting of three chemically distinct polymers covalently joined...

  7. Combining THz laser excitation with resonant soft X-ray scattering at the

    Office of Scientific and Technical Information (OSTI)

    Linac Coherent Light Source (Journal Article) | SciTech Connect Combining THz laser excitation with resonant soft X-ray scattering at the Linac Coherent Light Source Citation Details In-Document Search Title: Combining THz laser excitation with resonant soft X-ray scattering at the Linac Coherent Light Source This paper describes the development of new instrumentation at the Linac Coherent Light Source for conducting THz excitation experiments in an ultra high vacuum environment probed by

  8. Resonant Soft X-Ray Scattering - Combining Structural with Spectroscop...

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    28, 2012 - 10:00am SLAC, Bldg. 137, Room 322 SSRL Presents Kevin Stone X-ray absorption spectroscopy has become an important tool in understanding the electronic structure...

  9. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Resonant Soft X-Ray Scattering of Tri-Block Copolymers Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print Wednesday, 30 May 2012 00:00 In principle, tri-block copolymers (tri-BCPs), consisting of three chemically distinct polymers covalently joined together at the ends of each polymer chain, can serve as scaffolds and templates for fabricating a vast number of nanostructures. While quantitatively understanding the details of the morphology and the manner in which the different blocks

  10. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print In principle, tri-block copolymers (tri-BCPs), consisting of three chemically distinct polymers covalently joined together at the ends of each polymer chain, can serve as scaffolds and templates for fabricating a vast number of nanostructures. While quantitatively understanding the details of the morphology and the manner in which the different blocks interact with surfaces and interfaces is critical to success, previous experiments

  11. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print In principle, tri-block copolymers (tri-BCPs), consisting of three chemically distinct polymers covalently joined together at the ends of each polymer chain, can serve as scaffolds and templates for fabricating a vast number of nanostructures. While quantitatively understanding the details of the morphology and the manner in which the different blocks interact with surfaces and interfaces is critical to success, previous experiments

  12. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print In principle, tri-block copolymers (tri-BCPs), consisting of three chemically distinct polymers covalently joined together at the ends of each polymer chain, can serve as scaffolds and templates for fabricating a vast number of nanostructures. While quantitatively understanding the details of the morphology and the manner in which the different blocks interact with surfaces and interfaces is critical to success, previous experiments

  13. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print In principle, tri-block copolymers (tri-BCPs), consisting of three chemically distinct polymers covalently joined together at the ends of each polymer chain, can serve as scaffolds and templates for fabricating a vast number of nanostructures. While quantitatively understanding the details of the morphology and the manner in which the different blocks interact with surfaces and interfaces is critical to success, previous experiments

  14. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print In principle, tri-block copolymers (tri-BCPs), consisting of three chemically distinct polymers covalently joined together at the ends of each polymer chain, can serve as scaffolds and templates for fabricating a vast number of nanostructures. While quantitatively understanding the details of the morphology and the manner in which the different blocks interact with surfaces and interfaces is critical to success, previous experiments

  15. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print In principle, tri-block copolymers (tri-BCPs), consisting of three chemically distinct polymers covalently joined together at the ends of each polymer chain, can serve as scaffolds and templates for fabricating a vast number of nanostructures. While quantitatively understanding the details of the morphology and the manner in which the different blocks interact with surfaces and interfaces is critical to success, previous experiments

  16. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Resonant Soft X-Ray Scattering of Tri-Block Copolymers Print In principle, tri-block copolymers (tri-BCPs), consisting of three chemically distinct polymers covalently joined together at the ends of each polymer chain, can serve as scaffolds and templates for fabricating a vast number of nanostructures. While quantitatively understanding the details of the morphology and the manner in which the different blocks interact with surfaces and interfaces is critical to success, previous experiments

  17. The simultaneous measurement of energy and linear polarization of the scattered radiation in resonant inelastic soft x-ray scattering

    SciTech Connect (OSTI)

    Braicovich, L. Minola, M.; Dellea, G.; Ghiringhelli, G.; Le Tacon, M.; Moretti Sala, M.; Morawe, C.; Peffen, J.-Ch.; Yakhou, F.; Brookes, N. B.; Supruangnet, R.

    2014-11-15

    Resonant Inelastic X-ray Scattering (RIXS) in the soft x-ray range is an element-specific energy-loss spectroscopy used to probe the electronic and magnetic excitations in strongly correlated solids. In the recent years, RIXS has been progressing very quickly in terms of energy resolution and understanding of the experimental results, but the interpretation of spectra could further improve, sometimes decisively, from a full knowledge of the polarization of incident and scattered photons. Here we present the first implementation, in a high resolution soft-RIXS spectrometer used to analyze the scattered radiation, of a device allowing the measurement of the degree of linear polarization. The system, based on a graded W/B{sub 4}C multilayer mirror installed in proximity of the CCD detector, has been installed on the AXES spectrometer at the ESRF (European Synchrotron Radiation Facility); it has been fully characterized and it has been used for a demonstration experiment at the Cu L{sub 3} edge on a high-T{sub c} superconducting cuprate. The loss in efficiency suffered by the spectrometer equipped with this test facility was a factor 17.5. We propose also a more advanced version, suitable for a routine use on the next generation of RIXS spectrometers and with an overall efficiency up to 10%.

  18. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

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    enormous parameter space for the creation of new morphologies. Illustration from F.S. Bates and G.H. Fredrickson, "Block copolymers-designer soft materials," Physics Today 52, 32...

  19. Combining THz laser excitation with resonant soft X-ray scattering at the Linac Coherent Light Source

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Turner, Joshua J.; Dakovski, Georgi L.; Hoffmann, Matthias C.; Hwang, Harold Y.; Zarem, Alex; Schlotter, William F.; Moeller, Stefan; Minitti, Michael P.; Staub, Urs; Johnson, Steven; et al

    2015-04-11

    This paper describes the development of new instrumentation at the Linac Coherent Light Source for conducting THz excitation experiments in an ultra high vacuum environment probed by soft X-ray diffraction. This consists of a cantilevered, fully motorized mirror system which can provide 600 kV cm⁻¹ electric field strengths across the sample and an X-ray detector that can span the full Ewald sphere with in-vacuum motion. The scientific applications motivated by this development, the details of the instrument, and spectra demonstrating the field strengths achieved using this newly developed system are discussed.

  20. Soft-x-ray spectroscopy study of nanoscale materials

    SciTech Connect (OSTI)

    Guo, J.-H.

    2005-07-30

    The ability to control the particle size and morphology of nanoparticles is of crucial importance nowadays both from a fundamental and industrial point of view considering the tremendous amount of high-tech applications. Controlling the crystallographic structure and the arrangement of atoms along the surface of nanostructured material will determine most of its physical properties. In general, electronic structure ultimately determines the properties of matter. Soft X-ray spectroscopy has some basic features that are important to consider. X-ray is originating from an electronic transition between a localized core state and a valence state. As a core state is involved, elemental selectivity is obtained because the core levels of different elements are well separated in energy, meaning that the involvement of the inner level makes this probe localized to one specific atomic site around which the electronic structure is reflected as a partial density-of-states contribution. The participation of valence electrons gives the method chemical state sensitivity and further, the dipole nature of the transitions gives particular symmetry information. The new generation synchrotron radiation sources producing intensive tunable monochromatized soft X-ray beams have opened up new possibilities for soft X-ray spectroscopy. The introduction of selectively excited soft X-ray emission has opened a new field of study by disclosing many new possibilities of soft X-ray resonant inelastic scattering. In this paper, some recent findings regarding soft X-ray absorption and emission studies of various nanostructured systems are presented.

  1. Biological Imaging by Soft X-Ray Diffraction Microscopy

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    Biological Imaging by Soft X-Ray Diffraction Microscopy Biological Imaging by Soft X-Ray Diffraction Microscopy Print Wednesday, 30 November 2005 00:00 Electron and x-ray...

  2. Reflection soft X-ray microscope and method

    DOE Patents [OSTI]

    Suckewer, Szymon (Princeton, NJ); Skinner, Charles H. (Lawrenceville, NJ); Rosser, Roy (Princeton, NJ)

    1993-01-01

    A reflection soft X-ray microscope is provided by generating soft X-ray beams, condensing the X-ray beams to strike a surface of an object at a predetermined angle, and focusing the X-ray beams reflected from the surface onto a detector, for recording an image of the surface or near surface features of the object under observation.

  3. Reflection soft X-ray microscope and method

    DOE Patents [OSTI]

    Suckewer, S.; Skinner, C.H.; Rosser, R.

    1993-01-05

    A reflection soft X-ray microscope is provided by generating soft X-ray beams, condensing the X-ray beams to strike a surface of an object at a predetermined angle, and focusing the X-ray beams reflected from the surface onto a detector, for recording an image of the surface or near surface features of the object under observation.

  4. Soft X-ray techniques to study mesoscale magnetism

    SciTech Connect (OSTI)

    Kortright, Jeffrey B.

    2003-06-26

    Heterogeneity in magnetization (M) is ubiquitous in modern systems. Even in nominally homogeneous materials, domains or pinning centers typically mediate magnetization reversal. Fundamental lengths determining M structure include the domain wall width and the exchange stiffness length, typically in the 4-400 nm range. Chemical heterogeneity (phase separation, polycrystalline microstructure, lithographic or other patterning, etc.) with length scales from nanometers to microns is often introduced to influence magnetic properties. With 1-2 nm wavelengths {lambda}, soft x-rays in principle can resolve structure down to {lambda}/2, and are well suited to study these mesoscopic length scales [1, 2]. This article highlights recent advances in resonant soft x-ray methods to resolve lateral magnetic structure [3], and discusses some of their relative merits and limitations. Only techniques detecting x-ray photons (rather than photo-electrons) are considered [4], since they are compatible with strong applied fields to probe relatively deeply into samples. The magneto-optical (MO) effects discovered by Faraday and Kerr were observed in the x-ray range over a century later, first at ''hard'' wavelengths in diffraction experiments probing interatomic magnetic structure [5]. In the soft x-ray range, magnetic linear [6] and circular [7] dichroism spectroscopies first developed that average over lateral magnetic structure. These large resonant MO effects enable different approaches to study magnetic structure or heterogeneity that can be categorized as microscopy or scattering [1]. Direct images of magnetic structure result from photo-emission electron microscopes [4, 8] and zone-plate microscopes [9, 10]. Scattering techniques extended into the soft x-ray include familiar specular reflection that laterally averages over structure but can provide depth-resolved information, and diffuse scattering and diffraction that provide direct information about lateral magnetic structure. Scattering techniques are further classified as partially for fully coherent according to the extent of transverse coherence of the incident beam.

  5. Reabsorption of Soft X-Ray Emission at High X-Ray Free-Electron Laser

    Office of Scientific and Technical Information (OSTI)

    Fluences (Journal Article) | SciTech Connect Journal Article: Reabsorption of Soft X-Ray Emission at High X-Ray Free-Electron Laser Fluences Citation Details In-Document Search Title: Reabsorption of Soft X-Ray Emission at High X-Ray Free-Electron Laser Fluences Authors: Schreck, Simon ; Beye, Martin ; Sellberg, Jonas A. ; McQueen, Trevor ; Laksmono, Hartawan ; Kennedy, Brian ; Eckert, Sebastian ; Schlesinger, Daniel ; Nordlund, Dennis ; Ogasawara, Hirohito ; Sierra, Raymond G. ; Segtnan,

  6. Electronic structure of titania aerogels: Soft x-ray absorption...

    Office of Scientific and Technical Information (OSTI)

    Journal Article: Electronic structure of titania aerogels: Soft x-ray absorption study Citation Details In-Document Search Title: Electronic structure of titania aerogels: Soft...

  7. Multiplet resonance lifetimes in resonant inelastic x-ray scattering...

    Office of Scientific and Technical Information (OSTI)

    Multiplet resonance lifetimes in resonant inelastic x-ray scattering involving shallow core levels Citation Details In-Document Search Title: Multiplet resonance lifetimes in ...

  8. Biological Imaging by Soft X-Ray Diffraction Microscopy

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    Biological Imaging by Soft X-Ray Diffraction Microscopy Print Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in...

  9. Ambient Pressure Photoelectron Spectroscopy Using Soft X-ray...

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    Ambient Pressure Photoelectron Spectroscopy Using Soft X-ray and Hard X-ray, and its applications in electrochemistry Friday, December 14, 2012 - 3:30pm SSRL, Bldg. 137, room 322...

  10. Biological Imaging by Soft X-Ray Diffraction Microscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Biological Imaging by Soft X-Ray Diffraction Microscopy Print Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in their ability to image with nanometer-scale resolution in three dimensions nonperiodic objects that are several microns in size. To fill this gap, the technique of coherent x-ray diffraction imaging now under development takes advantage of the penetrating power of x rays while simultaneously removing the limitations

  11. Biological Imaging by Soft X-Ray Diffraction Microscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Biological Imaging by Soft X-Ray Diffraction Microscopy Print Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in their ability to image with nanometer-scale resolution in three dimensions nonperiodic objects that are several microns in size. To fill this gap, the technique of coherent x-ray diffraction imaging now under development takes advantage of the penetrating power of x rays while simultaneously removing the limitations

  12. Biological Imaging by Soft X-Ray Diffraction Microscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Biological Imaging by Soft X-Ray Diffraction Microscopy Print Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in their ability to image with nanometer-scale resolution in three dimensions nonperiodic objects that are several microns in size. To fill this gap, the technique of coherent x-ray diffraction imaging now under development takes advantage of the penetrating power of x rays while simultaneously removing the limitations

  13. Biological Imaging by Soft X-Ray Diffraction Microscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Biological Imaging by Soft X-Ray Diffraction Microscopy Print Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in their ability to image with nanometer-scale resolution in three dimensions nonperiodic objects that are several microns in size. To fill this gap, the technique of coherent x-ray diffraction imaging now under development takes advantage of the penetrating power of x rays while simultaneously removing the limitations

  14. Biological Imaging by Soft X-Ray Diffraction Microscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Biological Imaging by Soft X-Ray Diffraction Microscopy Print Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in their ability to image with nanometer-scale resolution in three dimensions nonperiodic objects that are several microns in size. To fill this gap, the technique of coherent x-ray diffraction imaging now under development takes advantage of the penetrating power of x rays while simultaneously removing the limitations

  15. Biological Imaging by Soft X-Ray Diffraction Microscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Biological Imaging by Soft X-Ray Diffraction Microscopy Print Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in their ability to image with nanometer-scale resolution in three dimensions nonperiodic objects that are several microns in size. To fill this gap, the technique of coherent x-ray diffraction imaging now under development takes advantage of the penetrating power of x rays while simultaneously removing the limitations

  16. Biological Imaging by Soft X-Ray Diffraction Microscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Biological Imaging by Soft X-Ray Diffraction Microscopy Print Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in their ability to image with nanometer-scale resolution in three dimensions nonperiodic objects that are several microns in size. To fill this gap, the technique of coherent x-ray diffraction imaging now under development takes advantage of the penetrating power of x rays while simultaneously removing the limitations

  17. Biological Imaging by Soft X-Ray Diffraction Microscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Biological Imaging by Soft X-Ray Diffraction Microscopy Print Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in their ability to image with nanometer-scale resolution in three dimensions nonperiodic objects that are several microns in size. To fill this gap, the technique of coherent x-ray diffraction imaging now under development takes advantage of the penetrating power of x rays while simultaneously removing the limitations

  18. Biological Imaging by Soft X-Ray Diffraction Microscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Biological Imaging by Soft X-Ray Diffraction Microscopy Biological Imaging by Soft X-Ray Diffraction Microscopy Print Wednesday, 30 November 2005 00:00 Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in their ability to image with nanometer-scale resolution in three dimensions nonperiodic objects that are several microns in size. To fill this gap, the technique of coherent x-ray diffraction imaging now under development takes

  19. Multiplet resonance lifetimes in resonant inelastic x-ray scattering

    Office of Scientific and Technical Information (OSTI)

    involving shallow core levels (Journal Article) | SciTech Connect Multiplet resonance lifetimes in resonant inelastic x-ray scattering involving shallow core levels Citation Details In-Document Search Title: Multiplet resonance lifetimes in resonant inelastic x-ray scattering involving shallow core levels Authors: Wray, L. Andrew ; Yang, Wanli ; Eisaki, Hiroshi ; Hussain, Zahid ; Chuang, Yi-De Publication Date: 2012-11-19 OSTI Identifier: 1101794 Type: Publisher's Accepted Manuscript Journal

  20. Soft x-ray capabilities for investigating the strongly correlated...

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    Soft x-ray capabilities for investigating the strongly correlated electron materials Friday, September 14, 2012 - 1:00pm SLAC, Bldg. 137, Room 226 Jun-Sik Lee Seminar One of the...

  1. Inelastic X-ray and Nuclear Resonant Scattering | Advanced Photon...

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    XSD-IXN XSD-IXN Home Staff Inelastic X-ray and Nuclear Resonant Scattering The Inelastic X-ray and Nuclear Resonant Scattering group operates beamlines at APS Sectors 3, 9 and 30....

  2. Soft X-Ray and Vacuum Ultraviolet Based Spectroscopy of the Actinides...

    Office of Scientific and Technical Information (OSTI)

    spectroscopy, Synchrotron-radiation-based photoelectron spectroscopy, Soft x-ray absorption spectroscopy, Soft x-ray emission spectroscopy, Inverse photoelectron spectroscopy,...

  3. Soft x-ray reduction camera for submicron lithography

    DOE Patents [OSTI]

    Hawryluk, A.M.; Seppala, L.G.

    1991-03-26

    Soft x-ray projection lithography can be performed using x-ray optical components and spherical imaging lenses (mirrors), which form an x-ray reduction camera. The x-ray reduction is capable of projecting a 5x demagnified image of a mask onto a resist coated wafer using 4.5 nm radiation. The diffraction limited resolution of this design is about 135 nm with a depth of field of about 2.8 microns and a field of view of 0.2 cm[sup 2]. X-ray reflecting masks (patterned x-ray multilayer mirrors) which are fabricated on thick substrates and can be made relatively distortion free are used, with a laser produced plasma for the source. Higher resolution and/or larger areas are possible by varying the optic figures of the components and source characteristics. 9 figures.

  4. Soft x-ray reduction camera for submicron lithography

    DOE Patents [OSTI]

    Hawryluk, Andrew M. (2708 Rembrandt Pl., Modesto, CA 95356); Seppala, Lynn G. (7911 Mines Rd., Livermore, CA 94550)

    1991-01-01

    Soft x-ray projection lithography can be performed using x-ray optical components and spherical imaging lenses (mirrors), which form an x-ray reduction camera. The x-ray reduction is capable of projecting a 5x demagnified image of a mask onto a resist coated wafer using 4.5 nm radiation. The diffraction limited resolution of this design is about 135 nm with a depth of field of about 2.8 microns and a field of view of 0.2 cm.sup.2. X-ray reflecting masks (patterned x-ray multilayer mirrors) which are fabricated on thick substrates and can be made relatively distortion free are used, with a laser produced plasma for the source. Higher resolution and/or larger areas are possible by varying the optic figures of the components and source characteristics.

  5. X-ray imaging of Nonlinear Resonant Gyrotropic Magnetic Vortex...

    Office of Scientific and Technical Information (OSTI)

    X-ray imaging of Nonlinear Resonant Gyrotropic Magnetic Vortex Core Motion in Circular Permalloy Disks Citation Details In-Document Search Title: X-ray imaging of Nonlinear...

  6. Lensless imaging of nanoporous glass with soft X-rays

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Turner, Joshua J.; Nelson, Johanna; Huang, Xiaojing; Steinbrener, Jan; Jacobsen, Chris

    2013-06-01

    Coherent soft X-ray diffraction has been used to image nanoporous glass structure in two dimensions using different methods. The merit of the reconstructions was judged using a new method of Fourier phase correlation with a final, refined image. The porous structure was found to have a much larger average size then previously believed.

  7. Lasers, extreme UV and soft X-ray

    SciTech Connect (OSTI)

    Nilsen, Joseph

    2015-09-20

    Three decades ago, large ICF lasers that occupied entire buildings were used as the energy sources to drive the first X-ray lasers. Today X-ray lasers are tabletop, spatially coherent, high-repetition rate lasers that enable many of the standard optical techniques such as interferometry to be extended to the soft X-ray regime between wavelengths of 10 and 50 nm. Over the last decade X-ray laser performance has been improved by the use of the grazing incidence geometry, diode-pumped solid-state lasers, and seeding techniques. The dominant X-ray laser schemes are the monopole collisional excitation lasers either driven by chirped pulse amplification (CPA) laser systems or capillary discharge. The CPA systems drive lasing in neon-like or nickel-like ions, typically in the 10 – 30 nm range, while the capillary system works best for neon-like argon at 46.9 nm. Most researchers use nickel-like ion lasers near 14 nm because they are well matched to the Mo:Si multilayer mirrors that have peak reflectivity near 13 nm and are used in many applications. As a result, the last decade has seen the birth of the X-ray free electron laser (XFEL) that can reach wavelengths down to 0.15 nm and the inner-shell Ne laser at 1.46 nm.

  8. Lasers, extreme UV and soft X-ray

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Nilsen, Joseph

    2015-09-20

    Three decades ago, large ICF lasers that occupied entire buildings were used as the energy sources to drive the first X-ray lasers. Today X-ray lasers are tabletop, spatially coherent, high-repetition rate lasers that enable many of the standard optical techniques such as interferometry to be extended to the soft X-ray regime between wavelengths of 10 and 50 nm. Over the last decade X-ray laser performance has been improved by the use of the grazing incidence geometry, diode-pumped solid-state lasers, and seeding techniques. The dominant X-ray laser schemes are the monopole collisional excitation lasers either driven by chirped pulse amplification (CPA)more » laser systems or capillary discharge. The CPA systems drive lasing in neon-like or nickel-like ions, typically in the 10 – 30 nm range, while the capillary system works best for neon-like argon at 46.9 nm. Most researchers use nickel-like ion lasers near 14 nm because they are well matched to the Mo:Si multilayer mirrors that have peak reflectivity near 13 nm and are used in many applications. As a result, the last decade has seen the birth of the X-ray free electron laser (XFEL) that can reach wavelengths down to 0.15 nm and the inner-shell Ne laser at 1.46 nm.« less

  9. Soft x-ray diagnostics for pulsed power machines

    SciTech Connect (OSTI)

    Idzorek, G.C.; Coulter, W.L.; Walsh, P.J.; Montoya, R.R.

    1995-08-01

    A variety of soft x-ray diagnostics are being fielded on the Los Alamos National Laboratory Pegasus and Procyon pulsed power systems and also being fielded on joint US/Russian magnetized target fusion experiments known as MAGO (Magnitoye Obzhatiye). The authors have designed a low-cost modular photoemissive detector designated the XRD-96 that uses commercial 1100 series aluminum for the photocathode. In addition to photocathode detectors a number of designs using solid state silicon photodiodes have been designed and fielded. They also present a soft x-ray time-integrated pinhole camera system that uses standard type TMAX-400 photographic film that obviates the need for expensive and no longer produced zero-overcoat soft x-ray emulsion film. In a typical experiment the desired spectral energy cuts, signal intensity levels, and desired field of view will determine diagnostic geometry and x-ray filters selected. The authors have developed several computer codes to assist in the diagnostic design process and data deconvolution. Examples of the diagnostic design process and data analysis for a typical pulsed power experiment are presented.

  10. Magnetism studies using resonant, coherent, x-ray scattering | Stanford

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    Synchrotron Radiation Lightsource Magnetism studies using resonant, coherent, x-ray scattering Monday, September 10, 2012 - 10:00am SLAC, Bldg. 137, Room 226 Keoki Seu Seminar: With the advent of free electron lasers there has been interest in using coherent x-rays to probe condensed matter systems. Resonant scattering with x-rays allow elemental specificity with magnetic contrast, and coherent light leads to speckle in the scattered pattern due to interference from waves exiting the sample.

  11. Soft X-ray Shock Loading and Momentum Coupling in Meteorite and...

    Office of Scientific and Technical Information (OSTI)

    Journal Article: Soft X-ray Shock Loading and Momentum Coupling in Meteorite and Planetary Materials. Citation Details In-Document Search Title: Soft X-ray Shock Loading and ...

  12. Soft X-Ray and Vacuum Ultraviolet Based Spectroscopy of the Actinides...

    Office of Scientific and Technical Information (OSTI)

    Conference: Soft X-Ray and Vacuum Ultraviolet Based Spectroscopy of the Actinides Citation Details In-Document Search Title: Soft X-Ray and Vacuum Ultraviolet Based Spectroscopy of...

  13. In Operando Soft X-ray Spectroscopy of 3D Graphene Supercapacitor...

    Office of Scientific and Technical Information (OSTI)

    In Operando Soft X-ray Spectroscopy of 3D Graphene Supercapacitor Electrodes Citation Details In-Document Search Title: In Operando Soft X-ray Spectroscopy of 3D Graphene...

  14. Soft x-ray microscopy - a powerful analytical tool to image magnetism...

    Office of Scientific and Technical Information (OSTI)

    Soft x-ray microscopy - a powerful analytical tool to image magnetism down to fundamental length and times scales Citation Details In-Document Search Title: Soft x-ray microscopy -...

  15. Magnetic soft x-ray microscopy of the domain wall depinning process...

    Office of Scientific and Technical Information (OSTI)

    Magnetic soft x-ray microscopy of the domain wall depinning process in permalloy magnetic nanowires Citation Details In-Document Search Title: Magnetic soft x-ray microscopy of the...

  16. Standing-wave excited soft x-ray photoemission microscopy: application...

    Office of Scientific and Technical Information (OSTI)

    Standing-wave excited soft x-ray photoemission microscopy: application to Co microdot magnetic arrays Citation Details In-Document Search Title: Standing-wave excited soft x-ray...

  17. Femtosecond diffractive imaging with a soft-X-ray free-electron...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    diffractive imaging with a soft-X-ray free-electron laser We have demonstrated flash diffractive imaging of nanostructures using pulses from the first soft-X-ray free-electron...

  18. Resonant x-ray magnetic scattering in holmium

    SciTech Connect (OSTI)

    Gibbs, D.

    1991-01-01

    We review the results of resonant x-ray magnetic scattering experiments on the rare earth metal holmium. When the incident incident x-ray energy is tuned near the L{sub III} absorption edge, large resonant enhancements of the magnetic scattering and resonant integer harmonics are observed. These results are analyzed within the theory of x-ray resonance exchange scattering assuming electric dipole (2p {yields} 5d) and quadrupole (2p {yields} 4f) transitions among atomic orbitals. 30 refs., 5 figs.

  19. High-order multilayer coated blazed gratings for high resolution soft x-ray spectroscopy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Voronov, Dmitriy L.; Goray, Leonid I.; Warwick, Tony; Yashchuk, Valeriy V.; Padmore, Howard A.

    2015-02-17

    A grand challenge in soft x-ray spectroscopy is to drive the resolving power of monochromators and spectrometers from the 104 achieved routinely today to well above 105. This need is driven mainly by the requirements of a new technique that is set to have enormous impact in condensed matter physics, Resonant Inelastic X-ray Scattering (RIXS). Unlike x-ray absorption spectroscopy, RIXS is not limited by an energy resolution dictated by the core-hole lifetime in the excitation process. Using much higher resolving power than used for normal x-ray absorption spectroscopy enables access to the energy scale of soft excitations in matter. Thesemoreexcitations such as magnons and phonons drive the collective phenomena seen in correlated electronic materials such as high temperature superconductors. RIXS opens a new path to study these excitations at a level of detail not formerly possible. However, as the process involves resonant excitation at an energy of around 1 keV, and the energy scale of the excitations one would like to see are at the meV level, to fully utilize the technique requires the development of monochromators and spectrometers with one to two orders of magnitude higher energy resolution than has been conventionally possible. Here we investigate the detailed diffraction characteristics of multilayer blazed gratings. These elements offer potentially revolutionary performance as the dispersive element in ultra-high resolution x-ray spectroscopy. In doing so, we have established a roadmap for the complete optimization of the grating design. Traditionally 1st order gratings are used in the soft x-ray region, but we show that as in the optical domain, one can work in very high spectral orders and thus dramatically improve resolution without significant loss in efficiency.less

  20. High-performance double-filter soft x-ray

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    performance double-filter soft x-ray diagnostic for measurement of electron temperature structure and dynamics M. B. McGarry, P. Franz, D. J. Den Hartog, J. A. Goetz, M. A. Thomas et al. Citation: Rev. Sci. Instrum. 83, 10E129 (2012); doi: 10.1063/1.4740274 View online: http://dx.doi.org/10.1063/1.4740274 View Table of Contents: http://rsi.aip.org/resource/1/RSINAK/v83/i10 Published by the American Institute of Physics. Additional information on Rev. Sci. Instrum. Journal Homepage:

  1. Lensless Imaging of Whole Biological Cells with Soft X-Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless Imaging of Whole Biological Cells with Soft X-Rays Print A team of scientists has used x-ray diffraction microscopy at ALS Beamline 9.0.1 to make images of whole yeast...

  2. Lensless Imaging of Whole Biological Cells with Soft X-Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    of Whole Biological Cells with Soft X-Rays Print A team of scientists has used x-ray diffraction microscopy at ALS Beamline 9.0.1 to make images of whole yeast cells, achieving the...

  3. Lensless Imaging of Whole Biological Cells with Soft X-Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Soft X-Rays Print Wednesday, 26 May 2010 00:00 A team of scientists has used x-ray diffraction microscopy at ALS Beamline 9.0.1 to make images of whole yeast cells, achieving the...

  4. Lensless Imaging of Whole Biological Cells with Soft X-Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Imaging of Whole Biological Cells with Soft X-Rays Print A team of scientists has used x-ray diffraction microscopy at ALS Beamline 9.0.1 to make images of whole yeast cells,...

  5. Soft x-ray undulator for the Siam Photon Source

    SciTech Connect (OSTI)

    Rugmai, S.; Dasri, T.; Prawanta, S.; Siriwattanapaitoon, S.; Kwankasem, A.; Sooksrimuang, V.; Chachai, W.; Suradet, N.; Juthong, N.; Tancharakorn, S.

    2007-01-19

    An undulator for production of intense soft x-rays has been designed for the Siam Photon Source. The construction of the undulator has been completed. It is now being characterized and prepared for installation. The device, named U60, is a pure permanent magnet planar undulator, consisting of 41 magnetic periods, with 60 mm period length. Utilization of the undulator radiation in the photon energy range of 30 - 900 eV is expected. The design studies of the magnetic structure, including investigation of perturbations arising from the magnetic field of the device, their effects on the SPS storage ring and compensation schemes are described. A magnetic measurement system has been constructed for magnetic characterization of the device. Partial results of magnetic measurements are presented.

  6. Experimental demonstration of a soft x-ray self-seeded free-electron laser

    Office of Scientific and Technical Information (OSTI)

    (Journal Article) | SciTech Connect Experimental demonstration of a soft x-ray self-seeded free-electron laser Citation Details In-Document Search Title: Experimental demonstration of a soft x-ray self-seeded free-electron laser The Linac Coherent Light Source has added self-seeding capability to the soft x-ray range using a grating monochromator system. We report demonstration of soft x-ray self-seeding with a measured resolving power of 2000-5000, wavelength stability of 10-4, and an

  7. Ambient Pressure Photoelectron Spectroscopy Using Soft X-ray and Hard

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-ray, and its applications in electrochemistry | Stanford Synchrotron Radiation Lightsource Ambient Pressure Photoelectron Spectroscopy Using Soft X-ray and Hard X-ray, and its applications in electrochemistry Friday, December 14, 2012 - 3:30pm SSRL, Bldg. 137, room 322 Zhi Liu The synchrotron based ambient pressure x-ray photoelectron spectroscopy (AP-XPS) endstation[1] pioneered at ALS based on differentially pumped electron energy analyzer has been recognized by scientific communities as

  8. Soft x-ray shock loading and momentum coupling in meteorite and planetary

    Office of Scientific and Technical Information (OSTI)

    materials. (Technical Report) | SciTech Connect Technical Report: Soft x-ray shock loading and momentum coupling in meteorite and planetary materials. Citation Details In-Document Search Title: Soft x-ray shock loading and momentum coupling in meteorite and planetary materials. X-ray momentum coupling coefficients, C{sub M}, were determined by measuring stress waveforms in planetary materials subjected to impulsive radiation loading from the Sandia National Laboratories Z-machine. Results

  9. Biological Imaging by Soft X-Ray Diffraction Microscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    methods (see previous highlight, "Demonstration of Coherent X-Ray Diffraction Imaging"). Experimental diffraction data used as input to the difference map algorithm....

  10. Linear Dichroism in Resonant Inelastic X-Ray Scattering to Molecular...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Linear Dichroism in Resonant Inelastic X-Ray Scattering to Molecular Spin-Orbit States Linear Dichroism in Resonant Inelastic X-Ray Scattering to Molecular Spin-Orbit States Print...

  11. Biological Imaging by Soft X-Ray Diffraction Microscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Microscopy Print Electron and x-ray microscopes are a valuable tool for both the life and materials sciences, but they are limited in their ability to image with...

  12. Biological Imaging by Soft X-Ray Diffraction Microscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    and angles of x rays scattered from the sample rather than transmitted through it). Shapiro et al. have now chimed in with the first lensless imaging of a sample as complex as a...

  13. New Zone Plate for Soft X-Ray Microscopy at 15-nm Spatial Resolution

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    New Zone Plate for Soft X-Ray Microscopy at 15-nm Spatial Resolution New Zone Plate for Soft X-Ray Microscopy at 15-nm Spatial Resolution Print Wednesday, 31 August 2005 00:00 Analytical tools that combine spatial resolution with elemental and chemical identification at the nanometer scale along with large penetration depth are indispensable for the life and physical sciences. The XM-1 soft x-ray microscope at the ALS produces images that not only reveal structures but can identify their

  14. Science Driver Requirements for Seeded Soft X-ray Free Electron...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Science Driver Requirements for Seeded Soft X-ray Free Electron Lasers Wednesday, December 2, 2015 - 2:00pm SLAC, Redtail Hawk Conference Room 108A Speaker: Fulvio Parmigiani,...

  15. Biological imaging by soft x-ray diffraction microscopy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Shapiro, D.; Thibault, P.; Beetz, T.; Elser, V.; Howells, M.; Jacobsen, C.; Kirz, J.; Lima, E.; Miao, H.; Neiman, A. M.; et al

    2005-10-25

    We have used the method of x-ray diffraction microscopy to image the complex-valued exit wave of an intact and unstained yeast cell. The images of the freeze-dried cell, obtained by using 750-eV x-rays from different angular orientations, portray several of the cell's major internal components to 30-nm resolution. The good agreement among the independently recovered structures demonstrates the accuracy of the imaging technique. To obtain the best possible reconstructions, we have implemented procedures for handling noisy and incomplete diffraction data, and we propose a method for determining the reconstructed resolution. This work represents a previously uncharacterized application of x-ray diffractionmore » microscopy to a specimen of this complexity and provides confidence in the feasibility of the ultimate goal of imaging biological specimens at 10-nm resolution in three dimensions.« less

  16. Science Driver Requirements for Seeded Soft X-ray Free Electron Lasers |

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Stanford Synchrotron Radiation Lightsource Science Driver Requirements for Seeded Soft X-ray Free Electron Lasers Wednesday, December 2, 2015 - 2:00pm SLAC, Redtail Hawk Conference Room 108A Speaker: Fulvio Parmigiani, Elettra-SincrotroneTrieste Program Description Starting from the archetypal FERMI externally seeded FEL, recent theoretical and experimental progress has shown the possibility of producing fully coherent, variable polarization and tunable, soft-X-ray, ultra-short pulses at

  17. New Zone Plate for Soft X-Ray Microscopy at 15-nm Spatial Resolution

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    New Zone Plate for Soft X-Ray Microscopy at 15-nm Spatial Resolution Print Analytical tools that combine spatial resolution with elemental and chemical identification at the nanometer scale along with large penetration depth are indispensable for the life and physical sciences. The XM-1 soft x-ray microscope at the ALS produces images that not only reveal structures but can identify their chemical elements and measure magnetic and other properties as well. Now a new method for creating optical

  18. New Zone Plate for Soft X-Ray Microscopy at 15-nm Spatial Resolution

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    New Zone Plate for Soft X-Ray Microscopy at 15-nm Spatial Resolution Print Analytical tools that combine spatial resolution with elemental and chemical identification at the nanometer scale along with large penetration depth are indispensable for the life and physical sciences. The XM-1 soft x-ray microscope at the ALS produces images that not only reveal structures but can identify their chemical elements and measure magnetic and other properties as well. Now a new method for creating optical

  19. New Zone Plate for Soft X-Ray Microscopy at 15-nm Spatial Resolution

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    New Zone Plate for Soft X-Ray Microscopy at 15-nm Spatial Resolution Print Analytical tools that combine spatial resolution with elemental and chemical identification at the nanometer scale along with large penetration depth are indispensable for the life and physical sciences. The XM-1 soft x-ray microscope at the ALS produces images that not only reveal structures but can identify their chemical elements and measure magnetic and other properties as well. Now a new method for creating optical

  20. New Zone Plate for Soft X-Ray Microscopy at 15-nm Spatial Resolution

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    New Zone Plate for Soft X-Ray Microscopy at 15-nm Spatial Resolution Print Analytical tools that combine spatial resolution with elemental and chemical identification at the nanometer scale along with large penetration depth are indispensable for the life and physical sciences. The XM-1 soft x-ray microscope at the ALS produces images that not only reveal structures but can identify their chemical elements and measure magnetic and other properties as well. Now a new method for creating optical

  1. Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography Print Wednesday, 24 February 2010 00:00 Humankind has benefitted from a long and productive relationship with yeast. For example, fermentation by yeast is an essential step in the production of bread, beer, wine, and even biofuels. However, not all yeast are beneficial. One strain of yeast, Candida albicans, grows unnoticed on most peoples' skin and in

  2. Soft X-ray Shock Loading and Momentum Coupling in Meteorite and Planetary

    Office of Scientific and Technical Information (OSTI)

    Materials. (Journal Article) | SciTech Connect Journal Article: Soft X-ray Shock Loading and Momentum Coupling in Meteorite and Planetary Materials. Citation Details In-Document Search Title: Soft X-ray Shock Loading and Momentum Coupling in Meteorite and Planetary Materials. Abstract not provided. Authors: Furnish, Michael David ; Remo, John L. ; Lawrence, R. Jeffery Publication Date: 2010-09-01 OSTI Identifier: 1122355 Report Number(s): SAND2010-6653J 491446 DOE Contract Number:

  3. Two-chicane compressed harmonic generation of soft x rays (Journal Article)

    Office of Scientific and Technical Information (OSTI)

    | SciTech Connect Two-chicane compressed harmonic generation of soft x rays Citation Details In-Document Search Title: Two-chicane compressed harmonic generation of soft x rays Authors: Ratner, Daniel ; Chao, Alex ; Huang, Zhirong Publication Date: 2011-02-07 OSTI Identifier: 1178293 Type: Published Article Journal Name: Physical Review Special Topics - Accelerators and Beams Additional Journal Information: Journal Volume: 14; Journal Issue: 2; Journal ID: ISSN 1098-4402 Publisher: American

  4. A table-top femtosecond time-resolved soft x-ray transient absorption spectrometer

    SciTech Connect (OSTI)

    Leone, Stephen; Loh, Zhi-Heng; Khalil, Munira; Correa, Raoul E.; Leone, Stephen R.

    2008-05-21

    A laser-based, table-top instrument is constructed to perform femtosecond soft x-ray transient absorption spectroscopy. Ultrashort soft x-ray pulses produced via high-order harmonic generation of the amplified output of a femtosecond Ti:sapphire laser system are used to probe atomic core-level transient absorptions in atoms and molecules. The results provide chemically specific, time-resolved dynamics with sub-50-fs time resolution. In this setup, high-order harmonics generated in a Ne-filled capillary waveguide are refocused by a gold-coated toroidal mirror into the sample gas cell, where the soft x-ray light intersects with an optical pump pulse. The transmitted high-order harmonics are spectrally dispersed with a home-built soft x-ray spectrometer, which consists of a gold-coated toroidal mirror, a uniform-line spaced plane grating, and a soft x-ray CCD camera. The optical layout of the instrument, design of the soft x-ray spectrometer, and spatial and temporal characterization of the high-order harmonics are described. Examples of static and time-resolved photoabsorption spectra collected on this apparatus are presented.

  5. Lensless Imaging of Whole Biological Cells with Soft X-Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless Imaging of Whole Biological Cells with Soft X-Rays Lensless Imaging of Whole Biological Cells with Soft X-Rays Print Wednesday, 26 May 2010 00:00 A team of scientists has used x-ray diffraction microscopy at ALS Beamline 9.0.1 to make images of whole yeast cells, achieving the highest resolution-11 to 13 nanometers (billionths of a meter)-ever obtained with this method for biological specimens. Their success indicates that full 3-D tomography of whole cells at equivalent resolution

  6. Synchrotron x-ray photoemission study of soft x-ray processed ultrathin glycine-water ice films

    SciTech Connect (OSTI)

    Tzvetkov, George; Netzer, Falko P.

    2011-05-28

    Ultrathin glycine-water ice films have been prepared in ultrahigh vacuum by condensation of H{sub 2}O and glycine at 90 K on single crystalline alumina surfaces and processed by soft x-ray (610 eV) exposure for up to 60 min. The physicochemical changes in the films were monitored using synchrotron x-ray photoemission spectroscopy. Two films with different amounts of H{sub 2}O have been considered in order to evaluate the influence of the water ice content on the radiation-induced effects. The analysis of C1s, N1s, and O1s spectral regions together with the changes in the valence band spectra indicates that amino acid degradation occurs fast mainly via decarboxylation and deamination of pristine molecules. Enrichment of the x-ray exposed surfaces with fragments with carbon atoms without strong electronegative substituents (C-C and C-H) is documented as well. In the thinner glycine-water ice film (six layers of glycine + six layers of water) the 3D ice suffers strongly from the x-rays and is largely removed from the sample. The rate of photodecomposition of glycine in this film is about 30% higher than for glycine in the thicker film (6 layers of glycine + 60 layers of water). The photoemission results suggest that the destruction of amino acid molecules is caused by the direct interaction with the radiation and that no chemical attack of glycine by the species released by water radiolysis is detected.

  7. SWIFT X-RAY OBSERVATIONS OF CLASSICAL NOVAE. II. THE SUPER SOFT SOURCE SAMPLE

    SciTech Connect (OSTI)

    Schwarz, Greg J.; Ness, Jan-Uwe; Osborne, J. P.; Page, K. L.; Evans, P. A.; Beardmore, A. P.; Walter, Frederick M.; Andrew Helton, L.; Woodward, Charles E.; Bode, Mike; Starrfield, Sumner; Drake, Jeremy J.

    2011-12-01

    The Swift gamma-ray burst satellite is an excellent facility for studying novae. Its rapid response time and sensitive X-ray detector provides an unparalleled opportunity to investigate the previously poorly sampled evolution of novae in the X-ray regime. This paper presents Swift observations of 52 Galactic/Magellanic Cloud novae. We included the X-Ray Telescope (0.3-10 keV) instrument count rates and the UltraViolet and Optical Telescope (1700-8000 A) filter photometry. Also included in the analysis are the publicly available pointed observations of 10 additional novae the X-ray archives. This is the largest X-ray sample of Galactic/Magellanic Cloud novae yet assembled and consists of 26 novae with Super Soft X-ray emission, 19 from Swift observations. The data set shows that the faster novae have an early hard X-ray phase that is usually missing in slower novae. The Super Soft X-ray phase occurs earlier and does not last as long in fast novae compared to slower novae. All the Swift novae with sufficient observations show that novae are highly variable with rapid variability and different periodicities. In the majority of cases, nuclear burning ceases less than three years after the outburst begins. Previous relationships, such as the nuclear burning duration versus t{sub 2} or the expansion velocity of the eject and nuclear burning duration versus the orbital period, are shown to be poorly correlated with the full sample indicating that additional factors beyond the white dwarf mass and binary separation play important roles in the evolution of a nova outburst. Finally, we confirm two optical phenomena that are correlated with strong, soft X-ray emission which can be used to further increase the efficiency of X-ray campaigns.

  8. Design and performance of AERHA, a high acceptance high resolution soft x-ray spectrometer

    SciTech Connect (OSTI)

    Chiuzbăian, Sorin G. Hague, Coryn F.; Brignolo, Stefania; Baumier, Cédric; Lüning, Jan; CNRS, UMR 7614, Laboratoire de Chimie Physique-Matière et Rayonnement, 11 rue Pierre et Marie Curie, F-75005 Paris; Synchrotron SOLEIL, L’Orme des Merisiers, Saint-Aubin, B.P. 48, F-91192 Gif-sur-Yvette ; Avila, Antoine; Delaunay, Renaud; Mariot, Jean-Michel; CNRS, UMR 7614, Laboratoire de Chimie Physique-Matière et Rayonnement, 11 rue Pierre et Marie Curie, F-75005 Paris ; Jaouen, Nicolas; Polack, François; Thomasset, Muriel; Lagarde, Bruno; Nicolaou, Alessandro; Sacchi, Maurizio; Sorbonne Universités, UPMC Univ Paris 06, UMR 7588, Institut des NanoSciences de Paris, 4 place Jussieu, F-75252 Paris Cedex 05; CNRS, UMR 7588, Institut des NanoSciences de Paris, 4 place Jussieu, F-75252 Paris Cedex 05

    2014-04-15

    A soft x-ray spectrometer based on the use of an elliptical focusing mirror and a plane varied line spacing grating is described. It achieves both high resolution and high overall efficiency while remaining relatively compact. The instrument is dedicated to resonant inelastic x-ray scattering studies. We set out how this optical arrangement was judged best able to guarantee performance for the 50 − 1000 eV range within achievable fabrication targets. The AERHA (adjustable energy resolution high acceptance) spectrometer operates with an effective angular acceptance between 100 and 250 μsr (energy dependent) and a resolving power well in excess of 5000 according to the Rayleigh criterion. The high angular acceptance is obtained by means of a collecting pre-mirror. Three scattering geometries are available to enable momentum dependent measurements with 135°, 90°, and 50° scattering angles. The instrument operates on the Synchrotron SOLEIL SEXTANTS beamline which serves as a high photon flux 2 × 200 μm{sup 2} focal spot source with full polarization control.

  9. Design and construction of a Fourier transform soft x-ray interferometer

    SciTech Connect (OSTI)

    Spring, John A.

    2000-05-10

    Helium, with its two electrons and one nucleus, is a three-body system. One of the models for investigating correlated electron motion in this system is autoionization, produced via double excitation of the electrons. Predictions about the autoionization spectrum of helium have differed from each other and from preliminary experimental data. However, previous experiments have not been able to distinguish among the theoretical predictions because their energy resolution is not high enough to resolve the narrow linewidths of quasi-forbidden peaks and the resonances that appear in the highest excited states. Consequently, a team of researchers at Lawrence Berkeley National Laboratory have embarked on a project for building a high-resolution Fourier-Transform Soft X-ray (or VUV) interferometer (FTSX) to provide definitive data to answer remaining questions about the autoionization spectrum of helium. The design and construction of this interferometer is described in detail below, including the use of a flexure stage to provide the large path length difference necessary for high resolution measurements, the manufacture of x-ray beamsplitters, a description of the software, and the solution to the problems of stick-slip, vibration, and alignment. Current progress of its development is also described, as well as future goals.

  10. The Soft X-ray research instrument at the Linac Coherent Light Source

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Dakovski, Georgi L.; Heimann, Philip; Holmes, Michael; Krupin, Oleg; European XFEL, Hamburg; Minitti, Michael P.; Mitra, Ankush; Moeller, Stefan; Rowen, Michael; Schlotter, William F.; et al

    2015-04-02

    The Soft X-ray Research instrument provides intense ultrashort X-ray pulses in the energy range 280–2000 eV. A diverse set of experimental stations may be installed to investigate a broad range of scientific topics such as ultrafast chemistry, highly correlated materials, magnetism, surface science, and matter under extreme conditions. A brief description of the main instrument components will be given, followed by some selected scientific highlights.

  11. Anti-contamination device for cryogenic soft X-ray diffraction microscopy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Huang, Xiaojing; Miao, Huijie; Nelson, Johanna; Turner, Joshua; Steinbrener, Jan; Shapiro, David; Kirz, Janos; Jacobsen, Chris

    2011-05-01

    Cryogenic microscopy allows one to view frozen hydrated biological and soft matter specimens with good structural preservation and a high degree of stability against radiation damage. We describe a liquid nitrogen-cooled anti-contamination device for cryogenic X-ray diffraction microscopy. The anti-contaminator greatly reduces the buildup of ice layers on the specimen due to condensation of residual water vapor in the experimental vacuum chamber. We show by coherent X-ray diffraction measurements that this leads to fivefold reduction of background scattering, which is important for far-field X-ray diffraction microscopy of biological specimens.

  12. Lensless Imaging of Whole Biological Cells with Soft X-Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless Imaging of Whole Biological Cells with Soft X-Rays Print A team of scientists has used x-ray diffraction microscopy at ALS Beamline 9.0.1 to make images of whole yeast cells, achieving the highest resolution-11 to 13 nanometers (billionths of a meter)-ever obtained with this method for biological specimens. Their success indicates that full 3-D tomography of whole cells at equivalent resolution should soon be possible. The National Center for X-Ray Tomography at ALS Beamline 2.1 images

  13. Lensless Imaging of Whole Biological Cells with Soft X-Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless Imaging of Whole Biological Cells with Soft X-Rays Print A team of scientists has used x-ray diffraction microscopy at ALS Beamline 9.0.1 to make images of whole yeast cells, achieving the highest resolution-11 to 13 nanometers (billionths of a meter)-ever obtained with this method for biological specimens. Their success indicates that full 3-D tomography of whole cells at equivalent resolution should soon be possible. The National Center for X-Ray Tomography at ALS Beamline 2.1 images

  14. Lensless Imaging of Whole Biological Cells with Soft X-Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless Imaging of Whole Biological Cells with Soft X-Rays Print A team of scientists has used x-ray diffraction microscopy at ALS Beamline 9.0.1 to make images of whole yeast cells, achieving the highest resolution-11 to 13 nanometers (billionths of a meter)-ever obtained with this method for biological specimens. Their success indicates that full 3-D tomography of whole cells at equivalent resolution should soon be possible. The National Center for X-Ray Tomography at ALS Beamline 2.1 images

  15. Lensless Imaging of Whole Biological Cells with Soft X-Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless Imaging of Whole Biological Cells with Soft X-Rays Print A team of scientists has used x-ray diffraction microscopy at ALS Beamline 9.0.1 to make images of whole yeast cells, achieving the highest resolution-11 to 13 nanometers (billionths of a meter)-ever obtained with this method for biological specimens. Their success indicates that full 3-D tomography of whole cells at equivalent resolution should soon be possible. The National Center for X-Ray Tomography at ALS Beamline 2.1 images

  16. Lensless Imaging of Whole Biological Cells with Soft X-Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless Imaging of Whole Biological Cells with Soft X-Rays Print A team of scientists has used x-ray diffraction microscopy at ALS Beamline 9.0.1 to make images of whole yeast cells, achieving the highest resolution-11 to 13 nanometers (billionths of a meter)-ever obtained with this method for biological specimens. Their success indicates that full 3-D tomography of whole cells at equivalent resolution should soon be possible. The National Center for X-Ray Tomography at ALS Beamline 2.1 images

  17. Lensless Imaging of Whole Biological Cells with Soft X-Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless Imaging of Whole Biological Cells with Soft X-Rays Print A team of scientists has used x-ray diffraction microscopy at ALS Beamline 9.0.1 to make images of whole yeast cells, achieving the highest resolution-11 to 13 nanometers (billionths of a meter)-ever obtained with this method for biological specimens. Their success indicates that full 3-D tomography of whole cells at equivalent resolution should soon be possible. The National Center for X-Ray Tomography at ALS Beamline 2.1 images

  18. Lensless Imaging of Whole Biological Cells with Soft X-Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless Imaging of Whole Biological Cells with Soft X-Rays Print A team of scientists has used x-ray diffraction microscopy at ALS Beamline 9.0.1 to make images of whole yeast cells, achieving the highest resolution-11 to 13 nanometers (billionths of a meter)-ever obtained with this method for biological specimens. Their success indicates that full 3-D tomography of whole cells at equivalent resolution should soon be possible. The National Center for X-Ray Tomography at ALS Beamline 2.1 images

  19. Lensless Imaging of Whole Biological Cells with Soft X-Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless Imaging of Whole Biological Cells with Soft X-Rays Print A team of scientists has used x-ray diffraction microscopy at ALS Beamline 9.0.1 to make images of whole yeast cells, achieving the highest resolution-11 to 13 nanometers (billionths of a meter)-ever obtained with this method for biological specimens. Their success indicates that full 3-D tomography of whole cells at equivalent resolution should soon be possible. The National Center for X-Ray Tomography at ALS Beamline 2.1 images

  20. Lensless Imaging of Whole Biological Cells with Soft X-Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless Imaging of Whole Biological Cells with Soft X-Rays Print A team of scientists has used x-ray diffraction microscopy at ALS Beamline 9.0.1 to make images of whole yeast cells, achieving the highest resolution-11 to 13 nanometers (billionths of a meter)-ever obtained with this method for biological specimens. Their success indicates that full 3-D tomography of whole cells at equivalent resolution should soon be possible. The National Center for X-Ray Tomography at ALS Beamline 2.1 images

  1. Soft x-ray ionization induced fragmentation of glycine

    SciTech Connect (OSTI)

    Itl, E.; Kooser, K.; Rachlew, E.; Huels, M. A.; Kukk, E.

    2014-06-21

    X-ray absorption commonly involves dissociative core ionization producing not only momentum correlated charged fragments but also low- and high-energy electrons capable of inducing damage in living tissue. This gives a natural motivation for studying the core ionization induced fragmentation processes in biologically important molecules such as amino acids. Here the fragmentation of amino acid glycine following carbon 1s core ionization has been studied. Using photoelectron-photoion-photoion coincidence technique, a detailed analysis on fragmentation of the sample molecule into pairs of momentum correlated cations has been carried out. The main characteristics of core ionization induced fragmentation of glycine were found to be the rupture of the CC{sub ?} bond and the presence of the CNH{sub 2}{sup +} fragment.

  2. ALP conversion and the soft X-ray excess in the outskirts of the Coma cluster

    SciTech Connect (OSTI)

    Kraljic, David; Rummel, Markus; Conlon, Joseph P. E-mail: Markus.Rummel@physics.ox.ac.uk

    2015-01-01

    It was recently found that the soft X-ray excess in the center of the Coma cluster can be fitted by conversion of axion-like-particles (ALPs) of a cosmic axion background (CAB) to photons. We extend this analysis to the outskirts of Coma, including regions up to 5 Mpc from the center of the cluster. We extract the excess soft X-ray flux from ROSAT All-Sky Survey data and compare it to the expected flux from ALP to photon conversion of a CAB. The soft X-ray excess both in the center and the outskirts of Coma can be simultaneously fitted by ALP to photon conversion of a CAB. Given the uncertainties of the cluster magnetic field in the outskirts we constrain the parameter space of the CAB. In particular, an upper limit on the CAB mean energy and a range of allowed ALP-photon couplings are derived.

  3. Multilayer films with sharp, stable interfaces for use in EUV and soft X-ray application

    DOE Patents [OSTI]

    Barbee, Jr., Troy W.; Bajt, Sasa

    2002-01-01

    The reflectivity and thermal stability of Mo/Si (molybdenum/silicon) multilayer films, used in soft x-ray and extreme ultraviolet region, is enhanced by deposition of a thin layer of boron carbide (e.g., B.sub.4 C) between alternating layers of Mo and Si. The invention is useful for reflective coatings for soft X-ray and extreme ultraviolet optics, multilayer for masks, coatings for other wavelengths and multilayers for masks that are more thermally stable than pure Mo/Si multilayers

  4. In Operando Soft X-ray Spectroscopy of 3D Graphene Supercapacitor

    Office of Scientific and Technical Information (OSTI)

    Electrodes (Journal Article) | SciTech Connect In Operando Soft X-ray Spectroscopy of 3D Graphene Supercapacitor Electrodes Citation Details In-Document Search Title: In Operando Soft X-ray Spectroscopy of 3D Graphene Supercapacitor Electrodes Authors: Bagge-Hansen, M ; Wood, B C ; Ogitsu, T ; Willey, T M ; Tran, I C ; Wittstock, A ; Biener, M M ; Merrill, M D ; Worsley, M A ; Otani, M ; Chuang, C H ; Prendergast, D ; Guo, J ; Baumann, T F ; van Buuren, T ; Biener, J ; Lee, J I Publication

  5. Electronic structure of titania aerogels: Soft x-ray absorption study

    Office of Scientific and Technical Information (OSTI)

    (Journal Article) | SciTech Connect Journal Article: Electronic structure of titania aerogels: Soft x-ray absorption study Citation Details In-Document Search Title: Electronic structure of titania aerogels: Soft x-ray absorption study Authors: Kucheyev, S O ; van Buuren, T ; Baumann, T F ; Satcher, Jr, J H ; Willey, T M ; Meulenberg, R W ; Felter, T E ; Poco, J F ; Gammon, S A ; Terminello, L J Publication Date: 2004-02-12 OSTI Identifier: 926419 Report Number(s): UCRL-JRNL-202402 DOE

  6. Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays Print Wednesday, 24 September 2008 00:00 The geometric structure of liquid water has been investigated in detail by many techniques, but many details are still under debate, such as the actual number of hydrogen bonds (at a given time) between the various water molecules. Even less is known about the electronic structure. Since it is the intermittent bonding

  7. Experimental demonstration of a soft x-ray self-seeded free-electron laser

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Ratner, D.; Abela, R.; Amann, J.; Behrens, C.; Bohler, D.; Bouchard, G.; Bostedt, C.; Boyes, M.; Chow, K.; Cocco, D.; et al

    2015-02-06

    The Linac Coherent Light Source has added self-seeding capability to the soft x-ray range using a grating monochromator system. We report demonstration of soft x-ray self-seeding with a measured resolving power of 2000-5000, wavelength stability of 10-4, and an increase in peak brightness by a factor of 2-5 across the photon energy range of 500-1000 eV. By avoiding the need for a monochromator at the experimental station, the self-seeded beam can deliver as much as 50 fold higher brightness to users.

  8. Gas cell for in situ soft X-ray transmission-absorption spectroscopy of

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    materials | Center for Gas SeparationsRelevant to Clean Energy Technologies | Blandine Jerome cell for in situ soft X-ray transmission-absorption spectroscopy of materials Previous Next List W. S. Drisdell and J. B. Kortright, Rev. Sci. Instrum. 85, 074103 (2014) DOI: 10.1063/1.4890816 1.4890816.figures.online.f1 Abstract: A simple gas cell design, constructed primarily from commercially available components, enables in situ soft X-ray transmission-absorption spectroscopy of materials in

  9. Soft x-ray ptychography studies of nanoscale magnetic and structural

    Office of Scientific and Technical Information (OSTI)

    correlations in thin SmCo5 films (Journal Article) | SciTech Connect Soft x-ray ptychography studies of nanoscale magnetic and structural correlations in thin SmCo5 films Citation Details In-Document Search This content will become publicly available on March 2, 2017 Title: Soft x-ray ptychography studies of nanoscale magnetic and structural correlations in thin SmCo5 films Authors: Shi, X. [1] ; Fischer, P. [2] ; Neu, V. [3] ; Elefant, D. [3] Search SciTech Connect for author "Elefant,

  10. Soft x-ray self-seeding simulation methods and their application for the

    Office of Scientific and Technical Information (OSTI)

    Linac Coherent Light Source (Journal Article) | SciTech Connect Soft x-ray self-seeding simulation methods and their application for the Linac Coherent Light Source Citation Details In-Document Search Title: Soft x-ray self-seeding simulation methods and their application for the Linac Coherent Light Source Authors: Serkez, Svitozar ; Krzywinski, Jacek ; Ding, Yuantao ; Huang, Zhirong Publication Date: 2015-03-13 OSTI Identifier: 1180929 Grant/Contract Number: AC02-76SF0051 Type: Published

  11. Method and apparatus for molecular imaging using X-rays at resonance wavelengths

    DOE Patents [OSTI]

    Chapline, Jr., George F. (Alamo, CA)

    1985-01-01

    Holographic X-ray images are produced representing the molecular structure of a microscopic object, such as a living cell, by directing a beam of coherent X-rays upon the object to produce scattering of the X-rays by the object, producing interference on a recording medium between the scattered X-rays from the object and unscattered coherent X-rays and thereby producing holograms on the recording surface, and establishing the wavelength of the coherent X-rays to correspond with a molecular resonance of a constituent of such object and thereby greatly improving the contrast, sensitivity and resolution of the holograms as representations of molecular structures involving such constituent. For example, the coherent X-rays may be adjusted to the molecular resonant absorption line of nitrogen at about 401.3 eV to produce holographic images featuring molecular structures involving nitrogen.

  12. High-performance soft x-ray spectromicroscopy beamline at SSRF

    SciTech Connect (OSTI)

    Xue Chaofan; Wang Yong; Guo Zhi; Wu Yanqing; Zhen Xiangjun; Chen Min; Chen Jiahua; Xue Song; Tai Renzhong; Peng Zhongqi; Lu Qipeng

    2010-10-15

    The Shanghai Synchrotron Radiation Facility (SSRF) is the first third-generation synchrotron facility in China and operated at an electron energy of 3.5 GeV. One of the seven beamlines in the first construction phase is devoted to soft x-ray spectromicroscopy and is equipped with an elliptically polarized undulator light source, a plane grating monochromator, and a scanning transmission x-ray microscope end station. Initial results reveal the high performance of this beamline, with an energy resolving power estimated to be over 10 000 at the argon L-edge and a spatial resolution better than 30 nm.

  13. Demonstration of 12 nm resolution Fresnel zone plate lens based soft x-ray microscopy

    SciTech Connect (OSTI)

    Chao, W.; Kim, J.; Rekawa, S.; Fischer, P.; Anderson, E. H.

    2009-06-05

    To extend soft x-ray microscopy to a resolution of order 10 nm or better, we developed a new nanofabrication process for Fresnel zone plate lenses. The new process, based on the double patterning technique, has enabled us to fabricate high quality gold zone plates with 12 nm outer zones. Testing of the zone plate with the full-field transmission x-ray microscope, XM-1, in Berkeley, showed that the lens clearly resolved 12 nm lines and spaces. This result represents a significant step towards 10 nm resolution and beyond.

  14. Soft X-ray irradiation of methanol ice: Formation of products as a function of photon energy

    SciTech Connect (OSTI)

    Chen, Y.-J.; Juang, K.-J.; Yih, T.-S.; Ciaravella, A.; Cecchi-Pestellini, C.; Muoz Caro, G. M.; Jimnez-Escobar, A.

    2013-12-01

    Pure methanol ices have been irradiated with monochromatic soft X-rays of 300 and 550 eV close to the 1s resonance edges of C and O, respectively, and with a broadband spectrum (250-1200 eV). The infrared (IR) spectra of the irradiated ices show several new products of astrophysical interest such as CH{sub 2}OH, H{sub 2}CO, CH{sub 4}, HCOOH, HCOCH{sub 2}OH, CH{sub 3}COOH, CH{sub 3}OCH{sub 3}, HCOOCH{sub 3}, and (CH{sub 2}OH){sub 2}, as well as HCO, CO, and CO{sub 2}. The effect of X-rays is the result of the combined interactions of photons and electrons with the ice. A significant contribution to the formation and growth of new species in the CH{sub 3}OH ice irradiated with X-rays is given by secondary electrons, whose energy distribution depends on the energy of X-ray photons. Within a single experiment, the abundances of the new products increase with the absorbed energy. Monochromatic experiments show that product abundances also increase with the photon energy. However, the abundances per unit energy of newly formed species show a marked decrease in the broadband experiment as compared to irradiations with monochromatic photons, suggesting a possible regulatory role of the energy deposition rate. The number of new molecules produced per absorbed eV in the X-ray experiments has been compared to those obtained with electron and ultraviolet (UV) irradiation experiments.

  15. Installation of soft X-ray array diagnostics and its application to tomography reconstruction using synthetic KSTAR X-ray images

    SciTech Connect (OSTI)

    Lee, Seung Hun; Jang, Juhyeok; Hong, Joohwan; Jang, Siwon; Choe, Wonho; Pacella, D.; Romano, A.; Gabellieri, L.; Kim, Junghee

    2014-11-15

    Four-array system of soft X-ray diagnostics was installed on KSTAR tokamak. Each array has 32 viewing chords of two photo-diode array detectors with spatial resolution of 2 cm. To estimate signals from the soft X-ray radiation power, typical n{sub e}, T{sub e}, and argon impurity line radiation profiles in KSTAR are chosen. The photo-diodes were absolutely calibrated as a function of the incident photon energy in 240 keV range with a portable X-ray tube. Two-dimensional T{sub e} image properties by multi-energy method were simulated and visualized with six combinations of beryllium filter sets within the dynamic range of signal ratio.

  16. The Ultraviolet Surprise. Efficient Soft X-Ray High Harmonic Generation in Multiply-Ionized Plasmas

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Popmintchev, Dimitar; Hernandez-Garcia, Carlos; Dollar, Franklin; Mancuso, Christopher; Perez-Hernandez, Jose A.; Chen, Ming-Chang; Hankla, Amelia; Gao, Xiaohui; Shim, Bonggu; Gaeta, Alexander L.; et al

    2015-12-04

    High-harmonic generation is a universal response of matter to strong femtosecond laser fields, coherently upconverting light to much shorter wavelengths. Optimizing the conversion of laser light into soft x-rays typically demands a trade-off between two competing factors. Reduced quantum diffusion of the radiating electron wave function results in emission from each species which is highest when a short-wavelength ultraviolet driving laser is used. But, phase matching—the constructive addition of x-ray waves from a large number of atoms—favors longer-wavelength mid-infrared lasers. We identified a regime of high-harmonic generation driven by 40-cycle ultraviolet lasers in waveguides that can generate bright beams inmore »the soft x-ray region of the spectrum, up to photon energies of 280 electron volts. Surprisingly, the high ultraviolet refractive indices of both neutral atoms and ions enabled effective phase matching, even in a multiply ionized plasma. We observed harmonics with very narrow linewidths, while calculations show that the x-rays emerge as nearly time-bandwidth–limited pulse trains of ~100 attoseconds.« less

  17. The Ultraviolet Surprise. Efficient Soft X-Ray High Harmonic Generation in Multiply-Ionized Plasmas

    SciTech Connect (OSTI)

    Popmintchev, Dimitar; Hernandez-Garcia, Carlos; Dollar, Franklin; Mancuso, Christopher; Perez-Hernandez, Jose A.; Chen, Ming-Chang; Hankla, Amelia; Gao, Xiaohui; Shim, Bonggu; Gaeta, Alexander L.; Tarazkar, Maryam; Romanov, Dmitri A.; Levis, Robert J.; Gaffney, Jim A.; Foord, Mark; Libby, Stephen B.; Jaron-Becker, Agnieskzka; Becker, Andreas; Plaja, Luis; Muranane, Margaret M.; Kapteyn, Henry C.; Popmintchev, Tenio

    2015-12-04

    High-harmonic generation is a universal response of matter to strong femtosecond laser fields, coherently upconverting light to much shorter wavelengths. Optimizing the conversion of laser light into soft x-rays typically demands a trade-off between two competing factors. Reduced quantum diffusion of the radiating electron wave function results in emission from each species which is highest when a short-wavelength ultraviolet driving laser is used. But, phase matching—the constructive addition of x-ray waves from a large number of atoms—favors longer-wavelength mid-infrared lasers. We identified a regime of high-harmonic generation driven by 40-cycle ultraviolet lasers in waveguides that can generate bright beams in the soft x-ray region of the spectrum, up to photon energies of 280 electron volts. Surprisingly, the high ultraviolet refractive indices of both neutral atoms and ions enabled effective phase matching, even in a multiply ionized plasma. We observed harmonics with very narrow linewidths, while calculations show that the x-rays emerge as nearly time-bandwidth–limited pulse trains of ~100 attoseconds.

  18. Soft X-ray Lithography Beamline at the Siam Photon Laboratory

    SciTech Connect (OSTI)

    Klysubun, P.; Chomnawang, N.; Songsiriritthigul, P.

    2007-01-19

    Construction of a soft x-ray lithography beamline utilizing synchrotron radiation generated by one of the bending magnets at the Siam Photon Laboratory is finished and the beamline is currently in a commissioning period. The beamline was modified from the existing monitoring beamline and is intended for soft x-ray lithographic processing and radiation biological research. The lithography exposure station with a compact one-dimensional scanning mechanism was constructed and assembled in-house. The front-end of the beamline has been modified to allow larger exposure area. The exposure station for studying radiation effects on biological samples will be set up in tandem with the lithography station, with a Mylar window for isolation. Several improvements to both the beamline and the exposure stations, such as improved scanning speed and the ability to adjust the exposure spectrum by means of low-Z filters, are planned and will be implemented in the near future.

  19. A multi-frame soft x-ray pinhole imaging diagnostic for single-shot applications

    SciTech Connect (OSTI)

    Wurden, G. A.; Coffey, S. K.

    2012-10-15

    For high energy density magnetized target fusion experiments at the Air Force Research Laboratory FRCHX machine, obtaining multi-frame soft x-ray images of the field reversed configuration (FRC) plasma as it is being compressed will provide useful dynamics and symmetry information. However, vacuum hardware will be destroyed during the implosion. We have designed a simple in-vacuum pinhole nosecone attachment, fitting onto a Conflat window, coated with 3.2 mg/cm{sup 2} of P-47 phosphor, and covered with a thin 50-nm aluminum reflective overcoat, lens-coupled to a multi-frame Hadland Ultra intensified digital camera. We compare visible and soft x-ray axial images of translating ({approx}200 eV) plasmas in the FRX-L and FRCHX machines in Los Alamos and Albuquerque.

  20. Soft x-ray capabilities for investigating the strongly correlated electron

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    materials | Stanford Synchrotron Radiation Lightsource Soft x-ray capabilities for investigating the strongly correlated electron materials Friday, September 14, 2012 - 1:00pm SLAC, Bldg. 137, Room 226 Jun-Sik Lee Seminar One of the most challenging extant issues in condensed matter physics and applied materials science is the search for post-silicon based electronics, and multi-functional complex oxides offer hopes that new classes of devices can be developed out of these intriguing

  1. Stereo soft x-ray microscopy and elemental mapping of hematite and clay suspensions

    SciTech Connect (OSTI)

    Gleber, S.-C.; Thieme, J.; Chao, W.; Fischer, P.

    2008-09-01

    The spatial arrangements of hematite particles within aqueous soil and clay samples are investigated with soft X-ray microscopy, taking advantage of the elemental contrast at the Fe-L edge around E = 707 eV. In combination with stereo microscopy, information about spatial arrangements are revealed and correlated to electrostatic interactions of the different mixtures. Manipulation of a sample mounted to the microscope is possible and particles added while imaging can be detected.

  2. Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography Print Humankind has benefitted from a long and productive relationship with yeast. For example, fermentation by yeast is an essential step in the production of bread, beer, wine, and even biofuels. However, not all yeast are beneficial. One strain of yeast, Candida albicans, grows unnoticed on most peoples' skin and in the intestines. In response to certain environmental conditions, C. albicans can switch to a pathogenic

  3. Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography Print Humankind has benefitted from a long and productive relationship with yeast. For example, fermentation by yeast is an essential step in the production of bread, beer, wine, and even biofuels. However, not all yeast are beneficial. One strain of yeast, Candida albicans, grows unnoticed on most peoples' skin and in the intestines. In response to certain environmental conditions, C. albicans can switch to a pathogenic

  4. Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography Print Humankind has benefitted from a long and productive relationship with yeast. For example, fermentation by yeast is an essential step in the production of bread, beer, wine, and even biofuels. However, not all yeast are beneficial. One strain of yeast, Candida albicans, grows unnoticed on most peoples' skin and in the intestines. In response to certain environmental conditions, C. albicans can switch to a pathogenic

  5. Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays Print The geometric structure of liquid water has been investigated in detail by many techniques, but many details are still under debate, such as the actual number of hydrogen bonds (at a given time) between the various water molecules. Even less is known about the electronic structure. Since it is the intermittent bonding between water molecules that gives liquid water its peculiar characteristics, the electronic structure

  6. Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays Print The geometric structure of liquid water has been investigated in detail by many techniques, but many details are still under debate, such as the actual number of hydrogen bonds (at a given time) between the various water molecules. Even less is known about the electronic structure. Since it is the intermittent bonding between water molecules that gives liquid water its peculiar characteristics, the electronic structure

  7. Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays Print The geometric structure of liquid water has been investigated in detail by many techniques, but many details are still under debate, such as the actual number of hydrogen bonds (at a given time) between the various water molecules. Even less is known about the electronic structure. Since it is the intermittent bonding between water molecules that gives liquid water its peculiar characteristics, the electronic structure

  8. Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays Print The geometric structure of liquid water has been investigated in detail by many techniques, but many details are still under debate, such as the actual number of hydrogen bonds (at a given time) between the various water molecules. Even less is known about the electronic structure. Since it is the intermittent bonding between water molecules that gives liquid water its peculiar characteristics, the electronic structure

  9. Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays Print The geometric structure of liquid water has been investigated in detail by many techniques, but many details are still under debate, such as the actual number of hydrogen bonds (at a given time) between the various water molecules. Even less is known about the electronic structure. Since it is the intermittent bonding between water molecules that gives liquid water its peculiar characteristics, the electronic structure

  10. Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays Print The geometric structure of liquid water has been investigated in detail by many techniques, but many details are still under debate, such as the actual number of hydrogen bonds (at a given time) between the various water molecules. Even less is known about the electronic structure. Since it is the intermittent bonding between water molecules that gives liquid water its peculiar characteristics, the electronic structure

  11. Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays Print The geometric structure of liquid water has been investigated in detail by many techniques, but many details are still under debate, such as the actual number of hydrogen bonds (at a given time) between the various water molecules. Even less is known about the electronic structure. Since it is the intermittent bonding between water molecules that gives liquid water its peculiar characteristics, the electronic structure

  12. Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays Print The geometric structure of liquid water has been investigated in detail by many techniques, but many details are still under debate, such as the actual number of hydrogen bonds (at a given time) between the various water molecules. Even less is known about the electronic structure. Since it is the intermittent bonding between water molecules that gives liquid water its peculiar characteristics, the electronic structure

  13. Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Isotope and Temperature Effects in Liquid Water Probed by Soft X Rays Print The geometric structure of liquid water has been investigated in detail by many techniques, but many details are still under debate, such as the actual number of hydrogen bonds (at a given time) between the various water molecules. Even less is known about the electronic structure. Since it is the intermittent bonding between water molecules that gives liquid water its peculiar characteristics, the electronic structure

  14. Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography Print Humankind has benefitted from a long and productive relationship with yeast. For example, fermentation by yeast is an essential step in the production of bread, beer, wine, and even biofuels. However, not all yeast are beneficial. One strain of yeast, Candida albicans, grows unnoticed on most peoples' skin and in the intestines. In response to certain environmental conditions, C. albicans can switch to a pathogenic

  15. Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography Print Humankind has benefitted from a long and productive relationship with yeast. For example, fermentation by yeast is an essential step in the production of bread, beer, wine, and even biofuels. However, not all yeast are beneficial. One strain of yeast, Candida albicans, grows unnoticed on most peoples' skin and in the intestines. In response to certain environmental conditions, C. albicans can switch to a pathogenic

  16. Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography Print Humankind has benefitted from a long and productive relationship with yeast. For example, fermentation by yeast is an essential step in the production of bread, beer, wine, and even biofuels. However, not all yeast are beneficial. One strain of yeast, Candida albicans, grows unnoticed on most peoples' skin and in the intestines. In response to certain environmental conditions, C. albicans can switch to a pathogenic

  17. Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography Print Humankind has benefitted from a long and productive relationship with yeast. For example, fermentation by yeast is an essential step in the production of bread, beer, wine, and even biofuels. However, not all yeast are beneficial. One strain of yeast, Candida albicans, grows unnoticed on most peoples' skin and in the intestines. In response to certain environmental conditions, C. albicans can switch to a pathogenic

  18. Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Imaging Antifungal Drug Molecules in Action using Soft X-Ray Tomography Print Humankind has benefitted from a long and productive relationship with yeast. For example, fermentation by yeast is an essential step in the production of bread, beer, wine, and even biofuels. However, not all yeast are beneficial. One strain of yeast, Candida albicans, grows unnoticed on most peoples' skin and in the intestines. In response to certain environmental conditions, C. albicans can switch to a pathogenic

  19. First Principles Calculations for X-ray Resonant Spectra and Elastic Properties

    SciTech Connect (OSTI)

    Yongbin Lee

    2006-05-01

    In this thesis, we discuss applications of first principles methods to x-ray resonant spectra and elastic properties calculation. We start with brief reviews about theoretical background of first principles methods, such as density functional theory, local density approximation (LDA), LDA+U, and the linear augmented plane wave (LAPW) method to solve Kohn-Sham equations. After that we discuss x-ray resonant scattering (XRMS), x-ray magnetic circular dichroism (XMCD) and the branching problem in the heavy rare earths Ledges. In the last chapter we discuss the elastic properties of the second hardest material AlMgB{sub 14}.

  20. Linear Dichroism in Resonant Inelastic X-Ray Scattering to Molecular

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Spin-Orbit States Linear Dichroism in Resonant Inelastic X-Ray Scattering to Molecular Spin-Orbit States Linear Dichroism in Resonant Inelastic X-Ray Scattering to Molecular Spin-Orbit States Print Thursday, 17 December 2009 13:47 Schematic representation of linear dichroism observed in KL x-ray emission. Coupling between the spin-orbit interaction and the molecular field, oriented along the chemical bond, leads to different spin-orbit ratios as a function of the angle between the incoming

  1. A soft x-ray transmission grating imaging-spectrometer for the National Ignition Facility

    SciTech Connect (OSTI)

    Moore, A S; Guymer, T M; Kline, J L; Morton, J; Taccetti, M; Lanier, N E; Bentley, C; Workman, J; Peterson, B; Mussack, K; Cowan, J; Prasad, R; Richardson, M; Burns, S; Kalantar, D H; Benedetti, L R; Bell, P; Bradley, D; Hsing, W; Stevenson, M

    2012-05-01

    A soft x-ray transmission grating spectrometer has been designed for use on high energy-density physics experiments at the National Ignition Facility (NIF); coupled to one of the NIF gated x-ray detectors (GXD) it records sixteen time-gated spectra between 250 and 1000eV with 100ps temporal resolution. The trade-off between spectral and spatial resolution leads to an optimized design for measurement of emission around the peak of a 100-300eV blackbody spectrum. Performance qualification results from the NIF, the Trident Laser Facility and VUV beamline at the National Synchrotron Light Source (NSLS), evidence a <100{micro}m spatial resolution in combination with a source-size limited spectral resolution that is <10eV at photon energies of 300eV.

  2. Influence of structural disorder on soft x-ray optical behavior of NbC thin films

    SciTech Connect (OSTI)

    Singh, Amol E-mail: rrcat.amol@gmail.com; Modi, Mohammed H.; Sinha, A. K.; Lodha, G. S.; Rajput, Parasmani

    2015-05-07

    Structural and chemical properties of compound materials are modified, when thin films are formed from bulk materials. To understand these changes, a study was pursued on niobium carbide (NbC) thin films of different thicknesses deposited on Si (100) substrate using ion beam sputtering technique. Optical response of the film was measured in 436?nm wavelength region using Indus-1 reflectivity beamline. A discrepancy in soft x-ray performance of NbC film was observed which could not be explained with Henke's tabulated data (see http://henke.lbl.gov/optical{sub c}onstants/ ). In order to understand this, detailed structural and chemical investigations were carried out using x-ray reflectivity, grazing incidence x-ray diffraction, x-ray absorption near edge structure, extended x-ray absorption fine structure, and x-ray photoelectron spectroscopy techniques. It was found that the presence of unreacted carbon and Nb deficiency due to reduced Nb-Nb coordination are responsible for lower soft x-ray reflectivity performance. NbC is an important material for soft x-ray optical devices, hence the structural disorder need to be controlled to achieve the best performances.

  3. Phase-matched generation of coherent soft and hard X-rays using IR lasers

    DOE Patents [OSTI]

    Popmintchev, Tenio V.; Chen, Ming-Chang; Bahabad, Alon; Murnane, Margaret M.; Kapteyn, Henry C.

    2013-06-11

    Phase-matched high-order harmonic generation of soft and hard X-rays is accomplished using infrared driving lasers in a high-pressure non-linear medium. The pressure of the non-linear medium is increased to multi-atmospheres and a mid-IR (or higher) laser device provides the driving pulse. Based on this scaling, also a general method for global optimization of the flux of phase-matched high-order harmonic generation at a desired wavelength is designed.

  4. Oxidation preventative capping layer for deep-ultra-violet and soft x-ray multilayers

    DOE Patents [OSTI]

    Prisbrey, Shon T.

    2004-07-06

    The invention uses iridium and iridium compounds as a protective capping layer on multilayers having reflectivity in the deep ultra-violet to soft x-ray regime. The iridium compounds can be formed in one of two ways: by direct deposition of the iridium compound from a prepared target or by depositing a thin layer (e.g., 5-50 angstroms) of iridium directly onto an element. The deposition energy of the incoming iridium is sufficient to activate the formation of the desired iridium compound. The compounds of most interest are iridium silicide (IrSi.sub.x) and iridium molybdenide (IrMo.sub.x).

  5. Enhancement of soft X-ray lasing action with thin blade radiators

    DOE Patents [OSTI]

    Suckewer, Szymon (Princeton Junction, NJ); Skinner, Charles H. (Kingston, NJ); Voorhees, David R. (Hopewell, NJ)

    1988-01-01

    An enhancement of approximately 100 of stimulated emission over spontaneous emission of the CVI 182 Angstrom line was obtained in a recombining magnetically confined plasma column. The plasma was formed by focusing a CO.sub.2 laser beam on a carbon disc. A magnetic solenoid produced a strong magnetic field which confined the plasma to the shape of a column. A single thin carbon blade extended parallel to the plasma column and served to make the column axially more uniform and also acted as a heat sink. Axial and transverse measurements of the soft X-ray lasing action were made from locations off-set from the central axis of the plasma column. Multiple carbon blades located at equal intervals around the plasma column were also found to produce acceptable results. According to another embodiment 10 a thin coating of aluminum or magnesium was placed on the carbon disc and blade. The Z of the coating should preferably be at least 5 greater than the Z of the target. Measurements of the soft X-rays generated at 182 Angstroms showed a significant increase in intensity enhancement.

  6. Regularization of soft-X-ray imaging in the DIII-D tokamak

    SciTech Connect (OSTI)

    Wingen, Andreas; Shafer, Morgan W; Unterberg, Ezekial A; Hill, Judith C; Hillis, Donald Lee

    2015-01-01

    An image inversion scheme for the soft X-ray imaging system (SXRIS) diagnostic at the DIII-D tokamak is developed to obtain the local soft X-ray emission at a poloidal cross-section from the spatially line-integrated image taken by the SXRIS camera. The scheme uses the Tikhonov regularization method since the inversion problem is generally ill-posed. The regularization technique uses the generalized singular value decomposition to determine a solution that depends on a free regularization parameter. The latter has to be chosen carefully, and the so called {\\it L-curve} method to find the optimum regularization parameter is outlined. A representative test image is used to study the properties of the inversion scheme with respect to inversion accuracy, amount/strength of regularization, image noise and image resolution. The optimum inversion parameters are identified, while the L-curve method successfully computes the optimum regularization parameter. Noise is found to be the most limiting issue, but sufficient regularization is still possible at noise to signal ratios up to 10%-15%. Finally, the inversion scheme is applied to measured SXRIS data and the line-integrated SXRIS image is successfully inverted.

  7. Electronic and magnetic properties of manganite thin films with different compositions and its correlation with transport properties: An X-ray resonant magnetic scattering study

    SciTech Connect (OSTI)

    Singh, Surendra; Freeland, J. W.; Fitzsimmons, M. R.; Jeen, H.; Biswas, A.

    2014-12-14

    Here, we present x-ray resonant magnetic dichroism and x-ray resonant magnetic scattering measurements of the temperature dependence of magnetism in Pr-doped La-Ca-Mn-O films grown on (110) NdGaO{sub 3} substrates. We observed thermal hysteresis of the ferromagnetism in one film that also showed large thermal hysteresis of ?18?K in transport measurements. While in a second film of a different nominal chemistry, which showed very small thermal hysteresis ?3?K in transport measurements, no thermal hysteresis of the ferromagnetism was observed. These macroscopic properties are correlated with evolution of surface magnetization across metal insulator transition for these films as observed by soft x-ray resonant magnetic scattering measurements.

  8. Design of Molecular Solar Cells via Feedback from Soft X-ray Spectroscopy

    SciTech Connect (OSTI)

    Himpsel, Franz J.

    2015-06-12

    Spectroscopy with soft X-rays was used to develop new materials and novel designs for solar cells and artificial photosynthesis. In order to go beyond the widely-used trial-and-error approach of gradually improving a particular design, we started from the most general layout of a solar cell (or a photo-electrochemical device) and asked which classes of materials are promising for best performance. For example, the most general design of a solar cell consists of a light absorber, an electron donor, and an electron acceptor. These are characterized by four energy levels, which were measured by a combination of spectroscopic X-ray techniques. Tuning synchrotron radiation to the absorption edges of specific elements provided element- and bond-selectivity. The spectroscopic results were complemented by state-of-the-art calculations of the electronic states. These helped explaining the observed energy levels and the orbitals associated with them. The calculations were extended to a large class of materials (for example thousands of porphyrin dye complexes) in order to survey trends in the energy level structure. A few highlights serve as examples: 1) Organic molecules combining absorber, donor, and acceptor with atomic precision. 2) Exploration of highly p-doped diamond films as inert, transparent electron donors. 3) Surface-sensitive characterization of nanorod arrays used as photoanodes in water splitting. 4) Computational design of molecular complexes for efficient solar cells using two photons.

  9. Analysis of soft x-ray/VUV transmission characteristics of Si and Al filters

    SciTech Connect (OSTI)

    Joseph, Aby; Modi, Mohammed H.; Singh, Amol; Gupta, R. K.; Lodha, G. S.

    2013-02-05

    Ultrathin filters of Al (1500A) and Si (1200A) should exhibit more than 65% transmission above their Labsorption edges in the soft x-ray/vacuum ultra violet region(Si L-edge: 124 A and Al L-edge: 170 A). However, the measured transmission characteristics of these filters showed {approx}40% transmission. The transmission measurements of these filters were carried at the reflectivity beamline of Indus-1 synchrotron source out over a large wavelength range of 120-360A. In order to understand the measured transmission performance a detailed model fitting is performed using the Paratt formalism. It is found that the oxidation of the surface region of the filters is responsible for the reduced transmission performance. Effects of higher harmonics of the toroidal grating monochromator are also considered in the data analysis.

  10. New Soft X-ray Beamline (BL10) at the SAGA Light Source

    SciTech Connect (OSTI)

    Yoshimura, D.; Setoyama, H.; Okajima, T.

    2010-06-23

    A new soft X-ray beamline (BL10) at the SAGA Light Source (SAGA-LS) was constructed at the end of 2008. Commissioning of this new beamline started at the beginning of 2009. Synchrotron radiation from a variably polarizing undulator (APPLE-II) can be used in this beamline. The obtained light is monochromatized by a varied-line-spacing plane grating monochromator with the variable included angle mechanism. Its designed resolving power and photon flux are 3,000-10,000 and 10{sup 12}-10{sup 9} photons/s at 300 mA, respectively. The performance test results were generally satisfactory. An overview of the optical design of the beamline and the current status of commissioning are reported.

  11. Investigation on the properties of a laminar grating as a soft x-ray beam splitter

    SciTech Connect (OSTI)

    Liu Ying; Fuchs, Hans-Joerg; Liu Zhengkun; Chen Huoyao; He Shengnan; Fu Shaojun; Kley, Ernst-Bernhard; Tuennermann, Andreas

    2010-08-10

    Laminar-type gratings as soft x-ray beam splitters for interferometry are presented. Gold-coated grating beam splitters with 1000 lines/mm are designed for grazing incidence operation at 13.9nm. They are routinely fabricated using electron beam lithography and ion etching techniques. The laminar grating is measured to have almost equal absolute efficiencies of about 20% in the zeroth and -1st orders, which enables a fringe visibility up to 0.99 in the interferometer. The discrepancy of the grating profiles between the optimized theoretical and the experimental results is analyzed according to the comparison of the optimized simulation results and the measurement realization of the grating efficiencies. By a precise control of the grating profile, the grating efficiency in the -1st order and the fringe visibility could be improved to 25% and 1, respectively.

  12. Cluster beam targets for laser plasma extreme ultraviolet and soft x-ray sources

    DOE Patents [OSTI]

    Kublak, Glenn D. (124 Turquoise Way, Livermore, Alameda County, CA 94550); Richardson, Martin C. (CREOL

    1996-01-01

    Method and apparatus for producing extreme ultra violet (EUV) and soft x-ray radiation from an ultra-low debris plasma source are disclosed. Targets are produced by the free jet expansion of various gases through a temperature controlled nozzle to form molecular clusters. These target clusters are subsequently irradiated with commercially available lasers of moderate intensity (10.sup.11 -10.sup.12 watts/cm.sup.2) to produce a plasma radiating in the region of 0.5 to 100 nanometers. By appropriate adjustment of the experimental conditions the laser focus can be moved 10-30 mm from the nozzle thereby eliminating debris produced by plasma erosion of the nozzle.

  13. Cluster beam targets for laser plasma extreme ultraviolet and soft x-ray sources

    DOE Patents [OSTI]

    Kublak, G.D.; Richardson, M.C.

    1996-11-19

    Method and apparatus for producing extreme ultraviolet (EUV) and soft x-ray radiation from an ultra-low debris plasma source are disclosed. Targets are produced by the free jet expansion of various gases through a temperature controlled nozzle to form molecular clusters. These target clusters are subsequently irradiated with commercially available lasers of moderate intensity (10{sup 11}--10{sup 12} watts/cm{sup 2}) to produce a plasma radiating in the region of 0.5 to 100 nanometers. By appropriate adjustment of the experimental conditions the laser focus can be moved 10--30 mm from the nozzle thereby eliminating debris produced by plasma erosion of the nozzle. 5 figs.

  14. Resonantly photo-pumped nickel-like erbium X-ray laser

    DOE Patents [OSTI]

    Nilsen, Joseph (Livermore, CA)

    1990-01-01

    A resonantly photo-pumped X-ray laser (10) that enhances the gain of seve laser lines that also lase because of collisional excitations and recombination processes, is described. The laser comprises an aluminum (12) and erbium (14) foil combination (16) that is driven by two beams (18, 20) of intense line focused (22, 24) optical laser radiation. Ground state nickel-like erbium ions (34) are resonantly photo-pumped by line emission from hydrogen-like aluminum ions (32).

  15. Imaging Antifungal Drug Molecules in Action using Soft X-Ray...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    development. Cell CAT Scans: 3-D Cell Imaging Routine medical x rays, such as chest x rays, can be used to identify a number of diseases. But this technique only produces...

  16. Molecular orientation in soft matter thin films studied by resonant soft

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    x-ray reflectivity | Center for Gas SeparationsRelevant to Clean Energy Technologies | Blandine Jerome orientation in soft matter thin films studied by resonant soft x-ray reflectivity Previous Next List Markus Mezger, Blandine Jérôme, Jeffrey B. Kortright, Manuel Valvidares, Eric M. Gullikson, Angelo Giglia, Nicola Mahne, and Stefano Nannarone, Phys. Rev. B 83, 155406 (2011) DOI: 10.1103/PhysRevB.83.155406 Abstract: We present a technique to study depth profiles of molecular orientation

  17. Vacuum space charge effects in sub-picosecond soft X-ray photoemission on a molecular adsorbate layer

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Dell'Angela, M.; Anniyev, T.; Beye, M.; Coffee, R.; Föhlisch, A.; Gladh, J.; Kaya, S.; Katayama, T.; Krupin, O.; Nilsson, A.; et al

    2015-03-01

    Vacuum space charge-induced kinetic energy shifts of O 1s and Ru 3d core levels in femtosecond soft X-ray photoemission spectra (PES) have been studied at a free electron laser (FEL) for an oxygen layer on Ru(0001). We fully reproduced the measurements by simulating the in-vacuum expansion of the photoelectrons and demonstrate the space charge contribution of the high-order harmonics in the FEL beam. Employing the same analysis for 400 nm pump-X-ray probe PES, we can disentangle the delay dependent Ru 3d energy shifts into effects induced by space charge and by lattice heating from the femtosecond pump pulse.

  18. R&D for a Soft X-Ray Free Electron Laser Facility

    SciTech Connect (OSTI)

    Corlett, John; Attwood, David; Byrd, John; Denes, Peter; Falcone, Roger; Heimann, Phil; Leemans, Wim; Padmore, Howard; Prestemon, Soren; Sannibale, Fernando; Schlueter, Ross; Schroeder, Carl; Staples, John; Venturini, Marco; Warwick, Tony; Wells, Russell; Wilcox, Russell; Zholent, Alexander; Adolphsen, Chris; Arthur, John; Bergmann, Uwe; Cai, Yunhai; Colby, Eric; Dowell, David; Emma, Paul; Fox, John; Frisch, Josef; Galayda, John; Hettel, Robert; Huang, Zhirong; Phinney, Nan; Rabedeau, Tom; Raubenheimer, Tor; Reis, David; Schmerge, John; Stöhr, Joachim; Stupakov, Gennady; White, Bill; Xiang, Dao

    2009-06-08

    Several recent reports have identified the scientific requirements for a future soft x-ray light source, and a high-repetition-rate free-electron laser (FEL) facility that is responsive to these requirements is now on the horizon. R&D in some critical areas is needed, however, to demonstrate technical performance, thus reducing technical risks and construction costs. Such a facility most likely will be based on a CW superconducting linear accelerator with beam supplied by a high-brightness, high-repetition-rate photocathode electron gun operating in CW mode, and on an array of FELs to which the accelerated beam is distributed, each operating at high repetition rate and with even pulse spacing. Dependent on experimental requirements, the individual FELs can be configured for either self-amplified spontaneous emission (SASE), seeded, or oscillator mode of operation, including the use of high-gain harmonic generation (HGHG), echo-enhanced harmonic generation (EEHG), harmonic cascade, or other configurations. In this White Paper we identify the overall accelerator R&D needs, and highlight the most important pre-construction R&D tasks required to value-engineer the design configuration and deliverables for such a facility. In Section 1.4 we identify the comprehensive R&D ultimately needed. We identify below the highest-priority requirements for understanding machine performance and reduce risk and costs at this pre-conceptual design stage. Details of implementing the required tasks will be the subject of future evaluation. Our highest-priority R&D program is the injector, which must be capable of delivering a beam with bunches up to a nanocoulomb at MHz repetition rate and with normalized emittance {le} 1 mm {center_dot} mrad. This will require integrated accelerating structure, cathode, and laser systems development. Cathode materials will impact the choice of laser technology in wavelength and energy per pulse, as well as vacuum requirements in the accelerating structure. Demonstration experiments in advanced seeding techniques, such as EEHG, and other optical manipulations to enhance the FEL process are required to reduce technical risk in producing temporally coherent and ultrashort x-ray output using optical seed lasers. Success of EEHG in particular would result in reduced development and cost of laser systems and accelerator hardware for seeded FELs. With a 1.5-2.5 GeV linac, FELs could operate in the VUV-soft x-ray range, where the actual beam energy will be determined by undulator technology; for example, to use the lower energy would require the use of advanced designs for which undulator R&D is needed. Significant reductions in both unit costs and accelerator costs resulting from the lower electron beam energy required to achieve lasing at a particular wavelength could be obtained with undulator development. Characterization of the wakefields of the vacuum chambers in narrow-gap undulators will be needed to minimize risk in ability to deliver close to transform limited pulses. CW superconducting RF technology for an FEL facility with short bunches at MHz rate and up to mA average current will require selection of design choices in cavity frequency and geometry, higher order mode suppression and power dissipation, RF power supply and distribution, accelerating gradient, and cryogenics systems. R&D is needed to define a cost and performance optimum. Developments in laser technology are proceeding at rapid pace, and progress in high-power lasers, harmonic generation, and tunable sources will need to be tracked.

  19. High-resolution Bent-crystal Spectrometer for the Ultra-soft X-ray Region

    DOE R&D Accomplishments [OSTI]

    Beiersdorfer, P.; von Goeler, S.; Bitter, M.; Hill, K. W.; Hulse, R. A.; Walling, R. S.

    1988-10-01

    A multichannel vacuum Brag-crystal spectrometer has been developed for high-resolution measurements of the line emission from tokamak plasmas in the wavelength region between 4 and 25 angstrom. The spectrometer employs a bent crystal in Johann geometry and a microchannel-plate intensified photodiode array. The instrument is capable of measuring high-resolution spectra (lambda/..delta..lambda approx. 3000) with fast time resolution (4 msec per spectrum) and good spatial resolution (3 cm). The spectral bandwidth is ..delta..lambda/lambda{sub 0} = 8 angstrom. A simple tilt mechanism allows access to different wavelength intervals. In order to illustrate the utility of the new spectrometer, time- and space-resolved measurements of the n = 3 to n = 2 spectrum of selenium from the Princeton Large Torus tokamak plasmas are presented. The data are used to determine the plasma transport parameters and to infer the radial distribution of fluorinelike, neonlike, and sodiumlike ions of selenium in the plasma. The new ultra-soft x-ray spectrometer has thus enabled us to demonstrate the utility of high-resolution L-shell spectroscopy of neonlike ions as a fusion diagnostic.

  20. Soft X-Ray Diffraction Microscopy of a Frozen Hydrated Yeast Cell

    SciTech Connect (OSTI)

    Huang Xiaojing; Nelson, Johanna; Lima, Enju; Miao, Huijie; Steinbrener, Jan; Stewart, Andrew; Turner, Joshua J.; Jacobsen, Chris; Kirz, Janos; Marchesini, Stefano; Shapiro, David; Neiman, Aaron M.

    2009-11-06

    We report the first image of an intact, frozen hydrated eukaryotic cell using x-ray diffraction microscopy, or coherent x-ray diffraction imaging. By plunge freezing the specimen in liquid ethane and maintaining it below -170 deg. C, artifacts due to dehydration, ice crystallization, and radiation damage are greatly reduced. In this example, coherent diffraction data using 520 eV x rays were recorded and reconstructed to reveal a budding yeast cell at a resolution better than 25 nm. This demonstration represents an important step towards high resolution imaging of cells in their natural, hydrated state, without limitations imposed by x-ray optics.

  1. Absolute timing measurements of the Ni-like Pd and Sn soft-x-ray lasers

    SciTech Connect (OSTI)

    Staub, F.; Braud, M.; Balmer, J.E.; Nilsen, J.

    2005-10-15

    The absolute time of emission of the x-ray laser output with respect to the arrival of a 100-ps pump pulse has been measured with the aid of a calibrated timing fiducial. The results show the x-ray laser to appear up to 60 ps (80 ps) before the peak of the pump pulse in the case of the Sn (Pd) x-ray laser, which is in good agreement with simulations obtained from the LASNEX and CRETIN codes. The pulse duration was found to be {approx}45 ps for both the Sn and the Pd x-ray lasers.

  2. Soft X-Ray Diffraction Microscopy of a Frozen Hydrated Yeast Cell

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Huang, Xiaojing; Nelson, Johanna; Kirz, Janos; Lima, Enju; Marchesini, Stefano; Miao, Huijie; Neiman, Aaron M.; Shapiro, David; Steinbrener, Jan; Stewart, Andrew; et al

    2009-11-01

    We report the first image of an intact, frozen hydrated eukaryotic cell using x-ray diffraction microscopy, or coherent x-ray diffraction imaging. By plunge freezing the specimen in liquid ethane and maintaining it below -170 °C, artifacts due to dehydration, ice crystallization, and radiation damage are greatly reduced. In this example, coherent diffraction data using 520 eV x rays were recorded and reconstructed to reveal a budding yeast cell at a resolution better than 25 nm. This demonstration represents an important step towards high resolution imaging of cells in their natural, hydrated state, without limitations imposed by x-ray optics.

  3. Polarization periodicity in the B1 columnar phase determined by resonant x-ray scattering

    SciTech Connect (OSTI)

    Folcia, C.L.; Pindak, R.; Ortega, J.; Etxebarria, J.; Pan, L.; Wang, S.; Huang, C.C.; Ponsinet, V.; Barois, P. and Gimeno, N.

    2011-07-14

    We report structural results that evidence the polarization distribution of the blocks in the columnar phase of an achiral bent-core liquid crystal. The study was performed using resonant x-ray diffraction at the sulfur K edge on oriented samples aligned on substrates. The extra periodicity is revealed through the violation of the systematic extinction rule of the structural symmetry group along the experimentally accessible diffraction direction. Further data obtained from the polarization analysis of a resonant reflection give information concerning the transition mechanism between B{sub 1} and B{sub 2} phases.

  4. Polarization Periodicity in the B(1) Columnar Phase Determined by Resonant X-ray Scattering

    SciTech Connect (OSTI)

    C Folcia; J Ortega; J Etxebarria; L Pan; S Wang; C Huang; V Ponsinet; P Barois; R Pindak; N Gimeno

    2011-12-31

    We report structural results that evidence the polarization distribution of the blocks in the columnar phase of an achiral bent-core liquid crystal. The study was performed using resonant x-ray diffraction at the sulfur K edge on oriented samples aligned on substrates. The extra periodicity is revealed through the violation of the systematic extinction rule of the structural symmetry group along the experimentally accessible diffraction direction. Further data obtained from the polarization analysis of a resonant reflection give information concerning the transition mechanism between B{sub 1} and B{sub 2} phases.

  5. Soft x-ray free-electron laser induced damage to inorganic scintillators

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Burian, Tomáš; Hájková, Věra; Chalupský, Jaromír; Vyšín, Luděk; Boháček, Pavel; Přeček, Martin; Wild, Jan; Özkan, Cigdem; Coppola, Nicola; Farahani, Shafagh Dastjani; et al

    2015-01-07

    An irreversible response of inorganic scintillators to intense soft x-ray laser radiation was investigated at the FLASH (Free-electron LASer in Hamburg) facility. Three ionic crystals, namely, Ce:YAG (cerium-doped yttrium aluminum garnet), PbWO4 (lead tungstate), and ZnO (zinc oxide), were exposed to single 4.6 nm ultra-short laser pulses of variable pulse energy (up to 12 μJ) under normal incidence conditions with tight focus. Damaged areas produced with various levels of pulse fluences, were analyzed on the surface of irradiated samples using differential interference contrast (DIC) and atomic force microscopy (AFM). The effective beam area of 22.2 ± 2.2 μm2 was determinedmore » by means of the ablation imprints method with the use of poly(methyl methacrylate) - PMMA. Applied to the three inorganic materials, this procedure gave almost the same values of an effective area. The single-shot damage threshold fluence was determined for each of these inorganic materials. The Ce:YAG sample seems to be the most radiation resistant under the given irradiation conditions, its damage threshold was determined to be as high as 660.8 ± 71.2 mJ/cm2. Contrary to that, the PbWO4 sample exhibited the lowest radiation resistance with a threshold fluence of 62.6 ± 11.9 mJ/cm2. The threshold for ZnO was found to be 167.8 ± 30.8 mJ/cm2. Both interaction and material characteristics responsible for the damage threshold difference are discussed in the article.« less

  6. Viewing spin structures with soft x-ray microscopy (Journal Article...

    Office of Scientific and Technical Information (OSTI)

    effects as contrast mechanism, high spatial resolution provided by state-of-the-art X-ray optics and fast time resolution limited by the inherent time structure of current...

  7. Soft x-ray spectromicroscopy development for materials science at the Advanced Light Source

    SciTech Connect (OSTI)

    Warwick, T.; Padmore, H.; Ade, H.; Hitchcock, A.P.; Rightor, E.G.; Tonner, B.P.

    1996-08-01

    Several third generation synchrotron radiation facilities are now operational and the high brightness of these photon sources offers new opportunities for x-ray microscopy. Well developed synchrotron radiation spectroscopy techniques are being applied in new instruments capable of imaging the surface of a material with a spatial resolution smaller than one micron. There are two aspects to this. One is to further the field of surface science by exploring the effects of spatial variations across a surface on a scale not previously accessible to x-ray measurements. The other is to open up new analytical techniques in materials science using x-rays, on a spatial scale comparable to that of the processes or devices to be studied. The development of the spectromicroscopy program at the Advanced Light Source will employ a variety of instruments, some are already operational. Their development and use will be discussed, and recent results will be presented to illustrate their capabilities.

  8. Soft X-Ray Spectroscopic Study of Dense Strontium-Doped Lanthanum Manganite Cathodes for Solid Oxide Fuel Cell Applications

    SciTech Connect (OSTI)

    L Piper; A Preston; S Cho; A DeMasi; J Laverock; K Smith; L Miara; J Davis; S Basu; et al.

    2011-12-31

    The evolution of the Mn charge state, chemical composition, and electronic structure of La{sub 0.8}Sr{sub 0.2}MnO{sub 3} (LSMO) cathodes during the catalytic activation of solid oxide fuel cell (SOFC) has been studies using X-ray spectroscopy of as-processed, exposed, and activated dense thin LSMO films. Comparison of O K-edge and Mn L{sub 3,2}-edge X-ray absorption spectra from the different stages of LSMO cathodes revealed that the largest change after the activation occurred in the Mn charge state with little change in the oxygen environment. Core-level X-ray photoemission spectroscopy and Mn L{sub 3} resonant photoemission spectroscopy studies of exposed and as-processed LSMO determined that the SOFC environment (800 C ambient pressure of O{sub 2}) alone results in La deficiency (severest near the surface with Sr doping >0.55) and a stronger Mn{sup 4+} contribution, leading to the increased insulating character of the cathode prior to activation. Meanwhile, O K-edge X-ray absorption measurements support Sr/La enrichment nearer the surface, along with the formation of mixed Sr{sub x}Mn{sub y}O{sub z} and/or passive MnO{sub x} and SrO species.

  9. Commissioning of a Soft X-ray Beamline PF-BL-16A with a Variable-Included-Angle Varied-Line-Spacing Grating Monochromator

    SciTech Connect (OSTI)

    Amemiya, Kenta; Toyoshima, Akio; Kikuchi, Takashi; Kosuge, Takashi; Nigorikawa, Kazuyuki; Sumii, Ryohei; Ito, Kenji

    2010-06-23

    The design and commissioning of a new soft X-ray beamline, BL-16A, at the Photon Factory is presented. The beamline consists of a pre-focusing mirror, an entrance slit, a variable-included-angle varied-line-spacing plane grating monochromator, and a post-focusing system as usual, and provides circularly and linearly polarized soft X rays in the energy range 200-1500 eV with an APPLE-II type undulator. The commissioning procedure for the beamline optics is described in detail, especially the check of the focal position for the zero-th order and diffracted X rays.

  10. Inverse Compton Origin of the Hard X-ray and Soft gamma-ray Emission from the Galactic Ridge

    SciTech Connect (OSTI)

    Porter, Troy A.; Moskalenko, Igor V.; Strong, Andrew W.; Orlando, Elena; Bouchet, Laurent

    2008-09-30

    A recent re-determination of the non-thermal component of the hard X-ray to soft {gamma}-ray emission from the Galactic ridge, using the SPI instrument on the INTErnational Gamma-Ray Astrophysics Laboratory (INTEGRAL) Observatory, is shown to be well reproduced as inverse-Compton emission from the interstellar medium. Both cosmic-ray primary electrons and secondary electrons and positrons contribute to the emission. The prediction uses the GALPROP model and includes a new calculation of the interstellar radiation field. This may solve a long-standing mystery of the origin of this emission, and potentially opens a new window on Galactic cosmic rays.

  11. Nematicity in stripe ordered cuprates probed via resonant x-ray scattering

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Achkar, A. J.; Zwiebler, M.; McMahon, Christopher; He, F.; Sutarto, R.; Dijianto, Isaiah; Hao, Zhihao; Gingras, Michael J.P.; Hucker, M.; Gu, G. D.; et al

    2016-02-05

    We found that in underdoped cuprate superconductors, a rich competition occurs between superconductivity and charge density wave (CDW) order. Whether rotational symmetry-breaking (nematicity) occurs intrinsically and generically or as a consequence of other orders is under debate. Here, we employ resonant x-ray scattering in stripe-ordered superconductors (La,M)2CuO4 to probe the relationship between electronic nematicity of the Cu 3d orbitals, structure of the (La,M)2O2 layers, and CDW order. We find distinct temperature dependences for the structure of the (La,M)2O2 layers and the electronic nematicity of the CuO2 planes, with only the latter being enhanced by the onset of CDW order. Ourmore » results identify electronic nematicity as an order parameter that is distinct from a purely structural order parameter in underdoped striped cuprates.« less

  12. Damage Threshold of Platinum Coating used for Optics for Self-Seeding of Soft X-ray Free Electron Laser

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Krzywinski, Jacek; Cocco, Daniele; Moeller, Stefan; Ratner, Daniel

    2015-02-23

    We investigated the experimental damage threshold of platinum coating on a silicon substrate illuminated by soft x-ray radiation at grazing incidence angle of 2.1 deg. The coating was the same as the blazed grating used for the soft X-ray self-seeding optics of the Linac Coherent Light Source free electron laser. The irradiation condition was chosen such that the absorbed dose was similar to the maximum dose expected for the grating. The expected dose was simulated by solving the Helmholtz equation in non-homogenous media. The experiment was performed at 900 eV photon energy for both single pulse and multi-shot conditions. Wemorehave not observed single shot damage. This corresponds to a single shot damage threshold being higher than 3 J/cm2. The multiple shot damage threshold measured for 10 shots and about 600 shots was determined to be 0.95 J/cm2 and 0.75 J/cm2 respectively. The damage threshold occurred at an instantaneous dose which is higher that the melt dose of platinum.less

  13. Calculated Performance Of The Variable-Polarization Undulator Upgrade To The Daresbury SRS Soft X-Ray Undulator Beamline

    SciTech Connect (OSTI)

    Roper, Mark D.; Bird, Daniel T.

    2004-05-12

    The soft x-ray beamline 5U1 on the Daresbury Laboratory SRS currently uses a planar undulator, producing linearly polarized radiation in the range 100 to 1000 eV. The undulator is soon to be replaced by a variable-polarization device of the Apple II design. The aim is to produce circularly polarized light in the energy range 265 to 1000 eV, covering the K-edges of C, N and O, and the first row transition element L-edges. This will greatly enhance the provision of circularly polarized soft-x-rays on the SRS and open up new opportunities for experimenters. The device will also produce linear polarization with a selectable angle of polarization with respect to the orbit plane, which is currently unavailable on the SRS. In order to provide the coverage over this energy range, we are exploiting the relatively large emittance of the SRS to allow us to use the second and third harmonics even in circular polarization mode. This paper presents the expected beamline output in various polarization modes and the predicted degree of polarization.

  14. Intense {ital J}=0{endash}1 soft-x-ray lasing at 28.5 nm in neonlike chromium

    SciTech Connect (OSTI)

    Praeg, A.R.; Loewenthal, F.; Balmer, J.E.

    1996-11-01

    Intense 3{ital p}-3{ital s}, {ital J}=0{endash}1 soft-x-ray lasing at 28.5 nm in neonlike chromium has been observed experimentally using a compact Nd:glass laser as the driver. 2.4-cm-long polished chromium slab targets were irradiated with up to 100-J/500-ps pulses at the fundamental wavelength of 1.054 {mu}m. The prepulse technique was applied using a defined prepulse 5 ns before the main pulse and with a prepulse-to-main pulse energy ratio of 0.7{percent}. It is demonstrated that a pump energy of {approximately}80 J, corresponding to a pump irradiance of approximately 9 TW/cm{sup 2} is sufficient to observe soft-x-ray lasing at 28.5 nm. At a drive laser energy of {approximately}90 J a gain coefficient of (2.2{plus_minus}0.5) cm{sup {minus}1} was measured. The one-dimensional space-resolved measurements show that the 28.5-nm laser line is emitted from a 60-{mu}m-wide (full width at half maximum) plasma region. {copyright} {ital 1996 The American Physical Society.}

  15. The Soft X-Ray Cosmos: ROSAT Science Symposium and Data Analysis Workshop

    SciTech Connect (OSTI)

    Schlegel, E.M.

    1994-12-31

    These proceedings represent papers presented at the ROSAT Science Symposium and Data Analysis Workshop held in College Park, Maryland. The aim was to showcase the results obtained thus far using ROSAT, the Roentgen Satellite, and to provide a forum for discussion regarding the means for extracting the maximum amount of information from ROSAT data. The cosmic x-ray sources discussed, included the cataclysmic variables, the Algol binary systems, the dark matter, galactic clusters, blazars, and many others. Star formation by galaxy interactions was also discussed. There were ninety one papers presented at the conference and none of these have been abstracted for the Energy Science and Technology database. (AIP)

  16. Soft x-ray backlighting of cryogenic implosions using a narrowband crystal imaging system (invited)

    SciTech Connect (OSTI)

    Stoeckl, C. Bedzyk, M.; Brent, G.; Epstein, R.; Fiksel, G.; Guy, D.; Goncharov, V. N.; Hu, S. X.; Ingraham, S.; Jacobs-Perkins, D. W.; Jungquist, R. K.; Marshall, F. J.; Mileham, C.; Nilson, P. M.; Sangster, T. C.; Shoup, M. J.; Theobald, W.

    2014-11-15

    A high-performance cryogenic DT inertial confinement fusion implosion experiment is an especially challenging backlighting configuration because of the high self-emission of the core at stagnation and the low opacity of the DT shell. High-energy petawatt lasers such as OMEGA EP promise significantly improved backlighting capabilities by generating high x-ray intensities and short emission times. A narrowband x-ray imager with an astigmatism-corrected bent quartz crystal for the Si He{sub ?} line at ?1.86 keV was developed to record backlit images of cryogenic direct-drive implosions. A time-gated recording system minimized the self-emission of the imploding target. A fast target-insertion system capable of moving the backlighter target ?7 cm in ?100 ms was developed to avoid interference with the cryogenic shroud system. With backlighter laser energies of ?1.25 kJ at a 10-ps pulse duration, the radiographic images show a high signal-to-background ratio of >100:1 and a spatial resolution of the order of 10 ?m. The backlit images can be used to assess the symmetry of the implosions close to stagnation and the mix of ablator material into the dense shell.

  17. Soft x-ray intensity profile measurements of electron cyclotron heated plasmas using semiconductor detector arrays in GAMMA 10 tandem mirror

    SciTech Connect (OSTI)

    Minami, R., E-mail: minami@prc.tsukuba.ac.jp; Imai, T.; Kariya, T.; Numakura, T.; Eguchi, T.; Kawarasaki, R.; Nakazawa, K.; Kato, T.; Sato, F.; Nanzai, H.; Uehara, M.; Endo, Y.; Ichimura, M. [Plasma Research Center, University of Tsukuba, Tsukuba, Ibaraki 305-8577 (Japan)

    2014-11-15

    Temporally and spatially resolved soft x-ray analyses of electron cyclotron heated plasmas are carried out by using semiconductor detector arrays in the GAMMA 10 tandem mirror. The detector array has 16-channel for the measurements of plasma x-ray profiles so as to make x-ray tomographic reconstructions. The characteristics of the detector array make it possible to obtain spatially resolved plasma electron temperatures down to a few tens eV and investigate various magnetohydrodynamic activities. High power electron cyclotron heating experiment for the central-cell region in GAMMA 10 has been started in order to reduce the electron drag by increasing the electron temperature.

  18. Surface layering and melting in an ionic liquid studied by resonant soft

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-ray reflectivity | Center for Gas SeparationsRelevant to Clean Energy Technologies | Blandine Jerome Surface layering and melting in an ionic liquid studied by resonant soft X-ray reflectivity Previous Next List Markus Mezger, Benjamin M. Ocko, Harald Reichert, and Moshe Deutsche, PNAS, 110, 3733-3737, 2013, DOI: 10.1073/pnas.1211749110 Abstract: The molecular-scale structure of the ionic liquid [C18mim]+[FAP]- near its free surface was studied by complementary methods. X-ray absorption

  19. Experimental comparison of grating- and propagation-based hard X-ray phase tomography of soft tissue

    SciTech Connect (OSTI)

    Lang, S.; Schulz, G.; Müller, B.; Zanette, I.; Dominietto, M.; Langer, M.; Rack, A.; Le Duc, G.; David, C.; Mohr, J.; Pfeiffer, F.; Weitkamp, T.

    2014-10-21

    When imaging soft tissues with hard X-rays, phase contrast is often preferred over conventional attenuation contrast due its superior sensitivity. However, it is unclear which of the numerous phase tomography methods yields the optimized results at given experimental conditions. Therefore, we quantitatively compared the three phase tomography methods implemented at the beamline ID19 of the European Synchrotron Radiation Facility: X-ray grating interferometry (XGI), and propagation-based phase tomography, i.e., single-distance phase retrieval (SDPR) and holotomography (HT), using cancerous tissue from a mouse model and an entire heart of a rat. We show that for both specimens, the spatial resolution derived from the characteristic morphological features is about a factor of two better for HT and SDPR compared to XGI, whereas the XGI data generally exhibit much better contrast-to-noise ratios for the anatomical features. Moreover, XGI excels in fidelity of the density measurements, and is also more robust against low-frequency artifacts than HT, but it might suffer from phase-wrapping artifacts. Thus, we can regard the three phase tomography methods discussed as complementary. The application will decide which spatial and density resolutions are desired, for the imaging task and dose requirements, and, in addition, the applicant must choose between the complexity of the experimental setup and the one of data processing.

  20. Growth kinetics and compositional analysis of silicon rich a-SiN{sub x}:H film: A soft x-ray reflectivity study

    SciTech Connect (OSTI)

    Singh, Sarab Preet; Srivastava, P.; Modi, Mohammed H.

    2010-10-11

    We report soft x-ray reflectivity measurements near the Si L{sub 2,3} absorption edge for Si-rich silicon nitride thin film obtained by Hg-sensitized photochemical vapor deposition. We demonstrate that the precise analysis of optical index profile derived over extended energy region gives compositional details of the film. This nondestructive approach is used in Si-rich silicon nitride film to reveal buried Si-rich interfacial layer. Further, the combined study of soft x-ray reflectivity and optical density obtained from the reflectivity fitting at various photon energies provide a qualitative estimation of the film composition and its growth.

  1. Raman and fluorescence characteristics of resonant inelastic X-ray scattering from doped superconducting cuprates

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Huang, H. Y.; Jia, C. J.; Chen, Z. Y.; Wohlfeld, K.; Moritz, B.; Devereaux, T. P.; Wu, W. B.; Okamoto, J.; Lee, W. S.; Hashimoto, M.; et al

    2016-01-22

    Measurements of spin excitations are essential for an understanding of spin-mediated pairing for superconductivity; and resonant inelastic X-ray scattering (RIXS) provides a considerable opportunity to probe high-energy spin excitations. However, whether RIXS correctly measures the collective spin excitations of doped superconducting cuprates remains under debate. Here we demonstrate distinct Raman- and fluorescence-like RIXS excitations of Bi1.5Pb0.6Sr1.54CaCu2O8+δ. Combining photon-energy and momentum dependent RIXS measurements with theoretical calculations using exact diagonalization provides conclusive evidence that the Raman-like RIXS excitations correspond to collective spin excitations, which are magnons in the undoped Mott insulators and evolve into paramagnons in doped superconducting compounds. In contrast,more » the fluorescence-like shifts are due primarily to the continuum of particle-hole excitations in the charge channel. Our results show that under the proper experimental conditions RIXS indeed can be used to probe paramagnons in doped high-Tc cuprate superconductors.« less

  2. Plasma dynamics above solar flare soft x-ray loop tops

    SciTech Connect (OSTI)

    Doschek, G. A.; Warren, H. P.; McKenzie, D. E.

    2014-06-10

    We measure non-thermal motions in flare loop tops and above the loop tops using profiles of highly ionized spectral lines of Fe XXIV and Fe XXIII formed at multimillion-degree temperatures. Non-thermal motions that may be due to turbulence or multiple flow regions along the line of sight are extracted from the line profiles. The non-thermal motions are measured for four flares seen at or close to the solar limb. The profile data are obtained using the Extreme-ultraviolet Imaging Spectrometer on the Hinode spacecraft. The multimillion-degree non-thermal motions are between 20 and 60 km s{sup 1} and appear to increase with height above the loop tops. Motions determined from coronal lines (i.e., lines formed at about 1.5 MK) tend to be smaller. The multimillion-degree temperatures in the loop tops and above range from about 11 MK to 15 MK and also tend to increase with height above the bright X-ray-emitting loop tops. The non-thermal motions measured along the line of sight, as well as their apparent increase with height, are supported by Solar Dynamics Observatory Atmospheric Imaging Assembly measurements of turbulent velocities in the plane of the sky.

  3. An experimental apparatus for diffraction-limites soft x-ray nanofocusing

    SciTech Connect (OSTI)

    Merthe, Daniel; Goldberg, Kenneth; Yashchuk, Valeriy; Yuan, Sheng; McKinney, Wayne; Celestre, Richard; Mochi, Iacopo; Macdougall, James; Morrison, Gregory; Rakawa, Senajith; Anderson, Erik; Smith, Brian; Domning, Edward; Warwick, Tony; Padmore, Howard

    2011-10-21

    Realizing the experimental potential of high-brightness, next generation synchrotron and free-electron laser light sources requires the development of reflecting x-ray optics capable of wavefront preservation and high-resolution nano-focusing. At the Advanced Light Source (ALS) beamline 5.3.1, we are developing broadly applicable, high-accuracy, in situ, at-wavelength wavefront measurement techniques to surpass 100-nrad slope measurement accuracy for diffraction-limited Kirkpatrick-Baez (KB) mirrors. The at-wavelength methodology we are developing relies on a series of wavefront-sensing tests with increasing accuracy and sensitivity, including scanning-slit Hartmann tests, grating-based lateral shearing interferometry, and quantitative knife-edge testing. We describe the original experimental techniques and alignment methodology that have enabled us to optimally set a bendable KB mirror to achieve a focused, FWHM spot size of 150 nm, with 1 nm (1.24 keV) photons at 3.7 mrad numerical aperture. The predictions of wavefront measurement are confirmed by the knife-edge testing.The side-profiled elliptically bent mirror used in these one-dimensional focusing experiments was originally designed for a much different glancing angle and conjugate distances. This work demonstrates that high-accuracy, at-wavelength wavefront-slope feedback can be used to optimize the pitch, roll, and mirror-bending forces in situ, using procedures that are deterministic and repeatable.

  4. Extraordinary luminous soft X-ray transient MAXI J0158744 as an ignition of a nova on a very massive O-Ne white dwarf

    SciTech Connect (OSTI)

    Morii, M.; Serino, M.; Mihara, T.; Sugizaki, M.; Tomida, H.; Kimura, M.; Nakahira, S.; Suwa, F.; Negoro, H.; Kennea, J. A.; Pritchard, T.; Page, K. L.; Osborne, J. P.; Curran, P. A.; Walter, F. M.; Kuin, N. P. M.; Hiroi, K.; Usui, R.; Kawai, N.; Gehrels, N.; and others

    2013-12-20

    We present the observation of an extraordinary luminous soft X-ray transient, MAXI J0158744, by the Monitor of All-sky X-ray Image (MAXI) on 2011 November 11. This transient is characterized by a soft X-ray spectrum, a short duration (1.3 10{sup 3} s < ?T{sub d} < 1.10 10{sup 4} s), a rapid rise (<5.5 10{sup 3} s), and a huge peak luminosity of 2 10{sup 40} erg s{sup 1} in 0.7-7.0 keV band. With Swift observations and optical spectroscopy from the Small and Moderate Aperture Research Telescope System, we confirmed that the transient is a nova explosion, on a white dwarf in a binary with a Be star, located near the Small Magellanic Cloud. An early turn-on of the super-soft X-ray source (SSS) phase (<0.44 days), the short SSS phase duration of about one month, and a 0.92 keV neon emission line found in the third MAXI scan, 1296 s after the first detection, suggest that the explosion involves a small amount of ejecta and is produced on an unusually massive O-Ne white dwarf close to, or possibly over, the Chandrasekhar limit. We propose that the huge luminosity detected with MAXI was due to the fireball phase, a direct manifestation of the ignition of the thermonuclear runaway process in a nova explosion.

  5. Final Scientific/Technical Report: Electronics for Large Superconducting Tunnel Junction Detector Arrays for Synchrotron Soft X-ray Research

    SciTech Connect (OSTI)

    Warburton, William K

    2009-03-06

    Superconducting tunnel junction (STJ) detectors offer a an approach to detecting soft x-rays with energy resolutions 4-5 times better and at rates 10 faster than traditions semiconductor detectors. To make such detectors feasible, however, then need to be deployed in large arrays of order 1000 detectors, which in turn implies that their processing electronics must be compact, fully computer controlled, and low cost per channel while still delivering ultra-low noise performance so as to not degrade the STJ's performance. We report on our progress in designing a compact, low cost preamplifier intended for this application. In particular, we were able to produce a prototype preamplifier of 2 sq-cm area and a parts cost of less than $30 that matched the energy resolution of the best conventional system to date and demonstrated its ability to acquire an STJ I-V curve under computer control, the critical step for determining and setting the detectors' operating points under software control.

  6. IMPULSIVE ACCELERATION OF CORONAL MASS EJECTIONS. II. RELATION TO SOFT X-RAY FLARES AND FILAMENT ERUPTIONS

    SciTech Connect (OSTI)

    Bein, B. M.; Berkebile-Stoiser, S.; Veronig, A. M.; Temmer, M.; Vrsnak, B.

    2012-08-10

    Using high time cadence images from the STEREO EUVI, COR1, and COR2 instruments, we derived detailed kinematics of the main acceleration stage for a sample of 95 coronal mass ejections (CMEs) in comparison with associated flares and filament eruptions. We found that CMEs associated with flares reveal on average significantly higher peak accelerations and lower acceleration phase durations, initiation heights, and heights, at which they reach their peak velocities and peak accelerations. This means that CMEs that are associated with flares are characterized by higher and more impulsive accelerations and originate from lower in the corona where the magnetic field is stronger. For CMEs that are associated with filament eruptions we found only for the CME peak acceleration significantly lower values than for events that were not associated with filament eruptions. The flare rise time was found to be positively correlated with the CME acceleration duration and negatively correlated with the CME peak acceleration. For the majority of the events the CME acceleration starts before the flare onset (for 75% of the events) and the CME acceleration ends after the soft X-ray (SXR) peak time (for 77% of the events). In {approx}60% of the events, the time difference between the peak time of the flare SXR flux derivative and the peak time of the CME acceleration is smaller than {+-}5 minutes, which hints at a feedback relationship between the CME acceleration and the energy release in the associated flare due to magnetic reconnection.

  7. Induced magnetic anisotropy in Si-free nanocrystalline soft magnetic materials: A transmission x-ray diffraction study

    SciTech Connect (OSTI)

    Parsons, R. Suzuki, K.; Yanai, T.; Kishimoto, H.; Kato, A.; Ohnuma, M.

    2015-05-07

    In order to better understand the origin of field-induced anisotropy (K{sub u}) in Si-free nanocrystalline soft magnetic alloys, the lattice spacing of the bcc-Fe phase in nanocrystalline Fe{sub 94?x}Nb{sub 6}B{sub x} (x?=?10, 12, 14) alloys annealed under an applied magnetic field has been investigated by X-ray diffraction in transmission geometry (t-XRD) with the diffraction vector parallel and perpendicular to the field direction. The saturation magnetostriction (?{sub s}) of nanocrystalline Fe{sub 94?x}Nb{sub 6}B{sub x} was found to increase linearly with the volume fraction of the residual amorphous phase and is well described by taking into account the volume-weighted average of two local ?{sub s} values for the bcc-Fe nanocrystallites (?5??2?ppm) and the residual amorphous matrix (+8??2?ppm). The lattice distortion required to produce the measured K{sub u} values (?100?J/m{sup 3}) was estimated via the inverse magnetostrictive effect using the measured ?{sub s} values and was compared to the lattice spacing estimations made by t-XRD. The lattice strain required to produce K{sub u} under the magnetoelastic model was not observed by the t-XRD experiments and so the findings of this study suggest that the origin of magnetic field induced K{sub u} cannot be explained through the magnetoelastic effect.

  8. Probing single magnon excitations in Sr₂IrO₄ using O K-edge resonant inelastic x-ray scattering

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Liu, X.; Dean, M. P. M.; Liu, J.; Chiuzbaian, S. G.; Jaouen, N.; Nicolaou, A.; Yin, W. G.; Rayan Serrao, C.; Ramesh, R.; Ding, H.; et al

    2015-04-28

    Resonant inelastic X-ray scattering (RIXS) at the L-edge of transition metal elements is now commonly used to probe single magnon excitations. Here we show that single magnon excitations can also be measured with RIXS at the K-edge of the surrounding ligand atoms when the center heavy metal elements have strong spin-orbit coupling. This is demonstrated with oxygen K-edge RIXS experiments on the perovskite Sr₂IrO₄, where low energy peaks from single magnon excitations were observed. This new application of RIXS has excellent potential to be applied to a wide range of magnetic systems based on heavy elements, for which the L-edgemore » RIXS energy resolutions in the hard X-ray region is usually poor.« less

  9. X-ray beamsplitter

    DOE Patents [OSTI]

    Ceglio, Natale M. (Livermore, CA); Stearns, Daniel S. (Mountain View, CA); Hawryluk, Andrew M. (Modesto, CA); Barbee, Jr., Troy W. (Palo Alto, CA)

    1989-01-01

    An x-ray beamsplitter which splits an x-ray beam into two coherent parts by reflecting and transmitting some fraction of an incident beam has applications for x-ray interferometry, x-ray holography, x-ray beam manipulation, and x-ray laser cavity output couplers. The beamsplitter is formed of a wavelength selective multilayer thin film supported by a very thin x-ray transparent membrane. The beamsplitter resonantly transmits and reflects x-rays through thin film interference effects. A thin film is formed of 5-50 pairs of alternate Mo/Si layers with a period of 20-250 A. The support membrane is 10-200 nm of silicon nitride or boron nitride. The multilayer/support membrane structure is formed across a window in a substrate by first forming the structure on a solid substrate and then forming a window in the substrate to leave a free-standing structure over the window.

  10. X-ray beamsplitter

    DOE Patents [OSTI]

    Ceglio, N.M.; Stearns, D.G.; Hawryluk, A.M.; Barbee, T.W. Jr.

    1987-08-07

    An x-ray beamsplitter which splits an x-ray beam into two coherent parts by reflecting and transmitting some fraction of an incident beam has applications for x-ray interferometry, x-ray holography, x-ray beam manipulation, and x-ray laser cavity output couplers. The beamsplitter is formed of a wavelength selective multilayer thin film supported by a very thin x-ray transparent membrane. The beamsplitter resonantly transmits and reflects x-rays through thin film interference effects. A thin film is formed of 5--50 pairs of alternate Mo/Si layers with a period of 20--250 A. The support membrane is 10--200 nm of silicon nitride or boron nitride. The multilayer/support membrane structure is formed across a window in a substrate by first forming the structure on a solid substrate and then forming a window in the substrate to leave a free-standing structure over the window. 6 figs.

  11. Soft-x-ray

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    RFX-Associazione EURATOM ENEA Sulla Fusione, Italy and Istituto Nazionale di Fisica della Materia, Unita' di Ricerca di Padova, Italy B. E. Chapman and D. Craig Department of ...

  12. Tunable coherent soft X-ray source based on the generation of high-order harmonic of femtosecond laser radiation in gas-filled capillaries

    SciTech Connect (OSTI)

    Malkov, Yu A; Yashunin, D A; Kiselev, A M; Stepanov, A N; Andreev, N E

    2014-05-30

    We have carried out experimental and theoretical investigations of a tunable coherent soft X-ray radiation source in the 30 – 52 nm wavelength range based on the generation of high-order harmonics of femtosecond laser radiation propagating in a dielectric xenon-filled capillary. The long path of laser pulse propagation through the capillary permits tuning the generated harmonic wavelengths to almost completely span the range under consideration. (interaction of radiation with matter)

  13. X-ray laser

    DOE Patents [OSTI]

    Nilsen, Joseph (Livermore, CA)

    1991-01-01

    An X-ray laser (10) that lases between the K edges of carbon and oxygen, i.e. between 44 and 23 Angstroms, is provided. The laser comprises a silicon (12) and dysprosium (14) foil combination (16) that is driven by two beams (18, 20) of intense line focused (22, 24) optical laser radiation. Ground state nickel-like dysprosium ions (34) are resonantly photo-pumped to their upper X-ray laser state by line emission from hydrogen-like silicon ions (32). The novel X-ray laser should prove especially useful for the microscopy of biological specimens.

  14. X-ray lithography source

    DOE Patents [OSTI]

    Piestrup, M.A.; Boyers, D.G.; Pincus, C.

    1991-12-31

    A high-intensity, inexpensive X-ray source for X-ray lithography for the production of integrated circuits is disclosed. Foil stacks are bombarded with a high-energy electron beam of 25 to 250 MeV to produce a flux of soft X-rays of 500 eV to 3 keV. Methods of increasing the total X-ray power and making the cross section of the X-ray beam uniform are described. Methods of obtaining the desired X-ray-beam field size, optimum frequency spectrum and eliminating the neutron flux are all described. A method of obtaining a plurality of station operation is also described which makes the process more efficient and economical. The satisfying of these issues makes transition radiation an excellent moderate-priced X-ray source for lithography. 26 figures.

  15. X-ray lithography source

    DOE Patents [OSTI]

    Piestrup, Melvin A. (Woodside, CA); Boyers, David G. (Mountain View, CA); Pincus, Cary (Sunnyvale, CA)

    1991-01-01

    A high-intensity, inexpensive X-ray source for X-ray lithography for the production of integrated circuits. Foil stacks are bombarded with a high-energy electron beam of 25 to 250 MeV to produce a flux of soft X-rays of 500 eV to 3 keV. Methods of increasing the total X-ray power and making the cross section of the X-ray beam uniform are described. Methods of obtaining the desired X-ray-beam field size, optimum frequency spectrum and elminating the neutron flux are all described. A method of obtaining a plurality of station operation is also described which makes the process more efficient and economical. The satisfying of these issues makes transition radiation an exellent moderate-priced X-ray source for lithography.

  16. Melatonin Protects Human Cells from Clustered DNA Damages, Killing and Acquisition of Soft Agar Growth Induced by X-rays or 970 MeV/n Fe ions

    SciTech Connect (OSTI)

    Das, B.; Sutherland, B.; Bennett, P. V.; Cutter, N. C.; Sutherland, J. C.

    2011-06-01

    We tested the ability of melatonin (N-acetyl-5 methoxytryptamine), a highly effective radical scavenger and human hormone, to protect DNA in solution and in human cells against induction of complex DNA clusters and biological damage induced by low or high linear energy transfer radiation (100 kVp X-rays, 970 MeV/nucleon Fe ions). Plasmid DNA in solution was treated with increasing concentrations of melatonin (0.0-3.5 mM) and were irradiated with X-rays. Human cells (28SC monocytes) were also irradiated with X-rays and Fe ions with and without 2 mM melatonin. Agarose plugs containing genomic DNA were subjected to Contour Clamped Homogeneous Electrophoretic Field (CHEF) followed by imaging and clustered DNA damages were measured by using Number Average length analysis. Transformation experiments on human primary fibroblast cells using soft agar colony assay were carried out which were irradiated with Fe ions with or without 2 mM melatonin. In plasmid DNA in solution, melatonin reduced the induction of single- and double-strand breaks. Pretreatment of human 28SC cells for 24 h before irradiation with 2 mM melatonin reduced the level of X-ray induced double-strand breaks by {approx}50%, of abasic clustered damages about 40%, and of Fe ion-induced double-strand breaks (41% reduction) and abasic clusters (34% reduction). It decreased transformation to soft agar growth of human primary cells by a factor of 10, but reduced killing by Fe ions only by 20-40%. Melatonin's effective reduction of radiation-induced critical DNA damages, cell killing, and striking decrease of transformation suggest that it is an excellent candidate as a countermeasure against radiation exposure, including radiation exposure to astronaut crews in space travel.

  17. Soft X-ray extended emissions of short gamma-ray bursts as electromagnetic counterparts of compact binary mergers: possible origin and detectability

    SciTech Connect (OSTI)

    Nakamura, Takashi; Nakauchi, Daisuke [Department of Physics, Kyoto University, Oiwake-cho, Kitashirakawa, Sakyo-ku, Kyoto 606-8502 (Japan); Kashiyama, Kazumi [Department of Astronomy and Astrophysics, Department of Physics, Center for Particle and Gravitational Astrophysics, Pennsylvania State University, University Park, PA 16802 (United States); Suwa, Yudai [Yukawa Institute for Theoretical Physics, Kyoto University, Oiwake-cho, Kitashirakawa, Sakyo-ku, Kyoto 606-8502 (Japan); Sakamoto, Takanori [Department of Physics and Mathematics, College of Science and Engineering, Aoyama Gakuin University, 5-10-1 Fuchinobe, Chuo-ku, Sagamihara-shi, Kanagawa 252-5258 (Japan); Kawai, Nobuyuki [Department of Physics, Tokyo Insititute of Technology, 2-12-1 Ookayama, Meguro-ku, Tokyo 152-8551 (Japan)

    2014-11-20

    We investigate the possible origin of extended emissions (EEs) of short gamma-ray bursts with an isotropic energy of ?10{sup 50-51} erg and a duration of a few 10 s to ?100 s, based on a compact binary (neutron star (NS)-NS or NS-black hole (BH)) merger scenario. We analyze the evolution of magnetized neutrino-dominated accretion disks of mass ?0.1 M {sub ?} around BHs formed after the mergers and estimate the power of relativistic outflows via the Blandford-Znajek (BZ) process. We show that a rotation energy of the BH up to ? 10{sup 52} erg can be extracted with an observed timescale of ? 30(1 + z) s with a relatively small disk viscosity parameter of ? < 0.01. Such a BZ power dissipates by clashing with non-relativistic pre-ejected matter of mass M ? 10{sup (2-4)} M {sub ?}, and forms a mildly relativistic fireball. We show that the dissipative photospheric emissions from such fireballs are likely in the soft X-ray band (1-10 keV) for M ? 10{sup 2} M {sub ?}, possibly in NS-NS mergers, and in the BAT band (15-150 keV) for M ? 10{sup 4} M {sub ?}, possibly in NS-BH mergers. In the former case, such soft EEs can provide a good chance of ?6 yr{sup ?1} (??{sub softEE}/4?) (R{sub GW}/40 yr{sup ?1}) for simultaneous detections of the gravitational waves with a ?0.1 angular resolution by soft X-ray survey facilities like the Wide-Field MAXI. Here, ??{sub softEE} is the beaming factor of the soft EEs and R{sub GW} is the NS-NS merger rate detectable by the advanced LIGO, the advanced Virgo, and KAGRA.

  18. Resonant inelastic x-ray scattering study of charge excitations in superconducting and nonsuperconducting PrFeAsO??y

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Jarrige, I.; Nomura, T.; Ishii, K.; Gretarsson, H.; Kim, Y.-J.; Kim, J.; Upton, M.; Casa, D.; Gog, T.; Ishikado, M.; et al

    2012-09-05

    We report the first observation by momentum-resolved resonant inelastic x-ray scattering of charge excitations in an iron-based superconductor and its parent compound, PrFeAsO?.? and PrFeAsO, respectively, with two main results. First, using calculations based on a 16-band dp model, we show that the energy of the lowest-lying excitations, identified as dd interband transitions of dominant xz,yz orbital character, exhibits a dramatic dependence on electron correlation. This enables us to estimate the Coulomb repulsion U and Hund's coupling J, and to highlight the role played by J in these peculiar orbital-dependent electron correlation effects. Second, we show that short-range antiferromagnetic correlations,morewhich are a prerequisite to the occurrence of these excitations at the ? point, are still present in the superconducting state.less

  19. In situ soft X-ray absorption spectroscopy investigation of electrochemical corrosion of copper in aqueous NaHCO3 solution

    SciTech Connect (OSTI)

    Jiang, Peng; Chen, Jeng-Lung; Borondics, Ferenc; Glans, Per-Anders; West, Mark W.; Chang, Ching-Lin; Salmeron, Miquel; Guo, Jinghua

    2010-03-31

    A novel electrochemical setup has been developed for soft x-ray absorption studies of the electronic structure of electrode materials during electrochemical cycling. In this communication we illustrate the operation of the cell with a study of the corrosion behavior of copper in aqueous NaHCO3 solution via the electrochemically induced changes of its electronic structure. This development opens the way for in situ investigations of electrochemical processes, photovoltaics, batteries, fuel cells, water splitting, corrosion, electrodeposition, and a variety of important biological processes.

  20. Observation of coupled vortex gyrations by 70-ps-time and 20-nm-space- resolved full-field magnetic transmission soft x-ray microscopy

    SciTech Connect (OSTI)

    Jung, Hyunsung; Yu, Young-Sang; Lee, Ki-Suk; Im, Mi-Young; Fischer, Peter; Bocklage, Lars; Vogel, Andreas; Bolte, Markus; Meier, Guido; Kim, Sang-Koog

    2010-09-01

    We employed time-and space-resolved full-field magnetic transmission soft x-ray microscopy to observe vortex-core gyrations in a pair of dipolar-coupled vortex-state Permalloy (Ni{sub 80}Fe{sub 20}) disks. The 70 ps temporal and 20 nm spatial resolution of the microscope enabled us to simultaneously measure vortex gyrations in both disks and to resolve the phases and amplitudes of both vortex-core positions. We observed their correlation for a specific vortex-state configuration. This work provides a robust and direct method of studying vortex gyrations in dipolar-coupled vortex oscillators.

  1. Method based on atomic photoionization for spot-size measurement on focused soft x-ray free-electron laser beams

    SciTech Connect (OSTI)

    Sorokin, A. A.; Gottwald, A.; Hoehl, A.; Kroth, U.; Schoeppe, H.; Ulm, G.; Richter, M.; Bobashev, S. V.; Domracheva, I. V.; Smirnov, D. N.; Tiedtke, K.; Duesterer, S.; Feldhaus, J.; Hahn, U.; Jastrow, U.; Kuhlmann, M.; Nunez, T.; Ploenjes, E.; Treusch, R.

    2006-11-27

    A method has been developed and applied to measure the beam waist and spot size of a focused soft x-ray beam at the free-electron laser FLASH of the Deutsches Elektronen-Synchrotron in Hamburg. The method is based on a saturation effect upon atomic photoionization and represents an indestructible tool for the characterization of powerful beams of ionizing electromagnetic radiation. At the microfocus beamline BL2 at FLASH, a full width at half maximum focus diameter of (15{+-}2) {mu}m was determined.

  2. Plasma Interactions in Laser Irradiated Semi-Cylindrical Cavities Studied with Soft X-Ray Interferometry Using a Capillary Discharge Laser

    SciTech Connect (OSTI)

    Purvis, M A; Grava, J; Filevich, J; Marconi, M; Rocca, J J; Moon, S J; Dunn, J; Nilsen, J; Shlyaptsev, V N; Jankowska, E

    2007-09-19

    Soft x-ray interferometry was used to measure the evolution of dense converging plasmas created by laser irradiation of 500 {micro}m diameter semi-cylindrical carbon targets. Optical laser pulses with an intensity of {approx} 1 x 10{sup 12} W cm{sup -2} and 120 ps duration were used to heat the surface of the cavities. The dense plasma formed expands from the walls converging slightly off the semi-cylinder's axis, giving rise to a bright localized high density plasma region. A sequence of electron density maps were measured using a 46.9 nm wavelength tabletop capillary discharge soft x-ray laser probe and a amplitude division interferometer based on diffraction gratings. The measured density profiles are compared with simulations conducted using the multi-dimensional hydrodynamic code HYDRA. The benchmarked model was then used to simulate particle trajectories which reveal that the increase in electron density near the axis is mainly the result of the convergence of plasma that originated at the bottom of the groove during laser irradiation.

  3. Comparison of the Radially Produced Electric-Field Shear Effects Analyzed from End-Loss Current and Central-Cell Soft X-Ray Data

    SciTech Connect (OSTI)

    Hirata, M. [Plasma Research Centre, University of Tsukuba (Japan); Cho, T. [Plasma Research Centre, University of Tsukuba (Japan); Yoshida, M. [Plasma Research Centre, University of Tsukuba (Japan); Kohagura, J. [Plasma Research Centre, University of Tsukuba (Japan); Numakura, T. [Plasma Research Centre, University of Tsukuba (Japan); Yokoyama, N. [Plasma Research Centre, University of Tsukuba (Japan); Tokioka, S. [Plasma Research Centre, University of Tsukuba (Japan); Fukai, T. [Plasma Research Centre, University of Tsukuba (Japan); Tomii, Y. [Plasma Research Centre, University of Tsukuba (Japan); Miyake, Y. [Plasma Research Centre, University of Tsukuba (Japan); Shimizu, K. [Plasma Research Centre, University of Tsukuba (Japan); Kiminami, S. [Plasma Research Centre, University of Tsukuba (Japan); Kondoh, T. [Japan Atomic Energy Research Institute (Japan); Miyoshi, S. [Plasma Research Centre, University of Tsukuba (Japan)

    2005-01-15

    Significant effects of sheared transverse electric fields in plasmas on both turbulent fluctuations and drift waves are experimentally demonstrated with improvement in plasma confinement for the first time in the tandem mirror GAMMA 10. Here, electron-cyclotron heatings (ECH) for ion-confining potential formation are applied in association with a significant rise in the absolute value of the central-cell potential and the resulting formation of a strong shear of electric fields of the order of 10 kV/m2 in the radial direction of the plasma column (dEr/dr). The central-cell line density increases during ECH in association with decreasing fluctuations. Various fluctuation diagnostics, in particular, the frequency analyses of end-loss ion currents and central soft x-ray brightness, show the consistent features. This encourages the usefulness of potentials and radial electric-field shear for confinement improvements.

  4. Development of extreme ultraviolet and soft x-ray multilayer optics for scientific studies with femtosecond/attosecond sources

    SciTech Connect (OSTI)

    Aquila, Andrew Lee

    2009-05-21

    The development of multilayer optics for extreme ultraviolet (EUV) radiation has led to advancements in many areas of science and technology, including materials studies, EUV lithography, water window microscopy, plasma imaging, and orbiting solar physics imaging. Recent developments in femtosecond and attosecond EUV pulse generation from sources such as high harmonic generation lasers, combined with the elemental and chemical specificity provided by EUV radiation, are opening new opportunities to study fundamental dynamic processes in materials. Critical to these efforts is the design and fabrication of multilayer optics to transport, focus, shape and image these ultra-fast pulses This thesis describes the design, fabrication, characterization, and application of multilayer optics for EUV femtosecond and attosecond scientific studies. Multilayer mirrors for bandwidth control, pulse shaping and compression, tri-material multilayers, and multilayers for polarization control are described. Characterization of multilayer optics, including measurement of material optical constants, reflectivity of multilayer mirrors, and metrology of reflected phases of the multilayer, which is critical to maintaining pulse size and shape, were performed. Two applications of these multilayer mirrors are detailed in the thesis. In the first application, broad bandwidth multilayers were used to characterize and measure sub-100 attosecond pulses from a high harmonic generation source and was performed in collaboration with the Max-Planck institute for Quantum Optics and Ludwig- Maximilians University in Garching, Germany, with Professors Krausz and Kleineberg. In the second application, multilayer mirrors with polarization control are useful to study femtosecond spin dynamics in an ongoing collaboration with the T-REX group of Professor Parmigiani at Elettra in Trieste, Italy. As new ultrafast x-ray sources become available, for example free electron lasers, the multilayer designs described in this thesis can be extended to higher photon energies, and such designs can be used with those sources to enable new scientific studies, such as molecular bonding, phonon, and spin dynamics.

  5. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    vast number of nanostructures. While quantitatively understanding the details of the morphology and the manner in which the different blocks interact with surfaces and interfaces...

  6. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    thermoelectrics and separations media, to name a few. Yet, by simply attaching one more polymer that is chemically distinct from the other blocks to the end of the di-BCP and by...

  7. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    conducted by: C. Wang and A. Hexemer (ALS), D.H. Lee (Dankook University, Korea), M.I. Kim (University of California, Berkeley), W. Zhao and T.P. Russell (University of...

  8. Combining THz laser excitation with resonant soft X-ray scattering...

    Office of Scientific and Technical Information (OSTI)

    for photosynthesis at room temperature (Kern et al., 2013). ... One area, however, which has shown increased potential is in ... Recent work has even utilized pulsed pumping schemes at ...

  9. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    array of morphologies and properties that make them candidates for applications in biomaterials, fuel cells and batteries, magnetic storage, and more. So far, so good, but the...

  10. Combining THz laser excitation with resonant soft X-ray scattering...

    Office of Scientific and Technical Information (OSTI)

    Authors: Turner, Joshua J. 1 ; Dakovski, Georgi L. 1 ; Hoffmann, Matthias C. 1 ; Hwang, Harold Y. 2 ; Zarem, Alex 1 ; Schlotter, William F. 1 ; Moeller, Stefan 1 ; ...

  11. Direct observation of ferromagnetism in grain boundary phase of Nd-Fe-B sintered magnet using soft x-ray magnetic circular dichroism

    SciTech Connect (OSTI)

    Nakamura, T.; Yasui, A.; Kotani, Y.; Iwai, H.; Akiya, T.; Ohkubo, T.; Hono, K.; Hirosawa, S.; Gohda, Y.

    2014-11-17

    We have investigated the magnetism of the grain boundary (GB) phase in a Nd{sub 14.0}Fe{sub 79.7}Cu{sub 0.1}B{sub 6.2} sintered magnet using soft x-ray magnetic circular dichroism (XMCD) at the Fe L{sub 2,3}-edges. Soft XMCD spectra were measured from the fractured surface that was confirmed to be covered with a thin GB phase by Auger electron spectroscopy. The magnetic moment of Fe in the GB phase was estimated to be m{sub GB}=1.4??{sub B} at 30?C using the sum rule analysis for XMCD spectra, which is 60% of that of Fe in the Nd{sub 2}Fe{sub 14}B compound. The temperature dependence of m{sub GB} evaluated with reference to Fe in the Nd{sub 2}Fe{sub 14}B phase indicated that the Curie temperature of the GB phase is more than 50?C lower compared to that of Nd{sub 2}Fe{sub 14}B.

  12. Absolute radiant power measurement for the Au M lines of laser-plasma using a calibrated broadband soft X-ray spectrometer with flat-spectral response

    SciTech Connect (OSTI)

    Troussel, Ph.; Villette, B.; Oudot, G.; Tassin, V.; Bridou, F.; Delmotte, F.; Krumrey, M.

    2014-01-15

    CEA implemented an absolutely calibrated broadband soft X-ray spectrometer called DMX on the Omega laser facility at the Laboratory for Laser Energetics (LLE) in 1999 to measure radiant power and spectral distribution of the radiation of the Au plasma. The DMX spectrometer is composed of 20 channels covering the spectral range from 50 eV to 20 keV. The channels for energies below 1.5 keV combine a mirror and a filter with a coaxial photo-emissive detector. For the channels above 5 keV the photoemissive detector is replaced by a conductive detector. The intermediate energy channels (1.5 keV < photon energy < 5 keV) use only a filter and a coaxial detector. A further improvement of DMX consists in flat-response X-ray channels for a precise absolute measurement of the photon flux in the photon energy range from 0.1 keV to 6 keV. Such channels are equipped with a filter, a Multilayer Mirror (MLM), and a coaxial detector. We present as an example the development of channel for the gold M emission lines in the photon energy range from 2 keV to 4 keV which has been successfully used on the OMEGA laser facility. The results of the radiant power measurements with the new MLM channel and with the usual channel composed of a thin titanium filter and a coaxial detector (without mirror) are compared. All elements of the channel have been calibrated in the laboratory of the Physikalisch-Technische Bundesanstalt, Germany's National Metrology Institute, at the synchrotron radiation facility BESSY II in Berlin using dedicated well established and validated methods.

  13. SU-E-T-537: Comparison of Intra-Operative Soft X-Rays to Low Energy Electron Beams for Treatment of Superficial Lesions

    SciTech Connect (OSTI)

    Chinsky, B; Diak, A; Gros, S; Sethi

    2014-06-01

    Purpose: Superficial soft x-ray applicators have recently been designed for use with existing intra-operative radiotherapy systems. These applicators may be used in treating superficial lesions which are conventionally treated with electron beams. The purpose of this abstract is to compare dose distributions of an intra-operative 50kV x-ray unit with low energy electrons for the treatment of superficial lesions. Methods: Dosimetric parameters for 1 and 3-cm diameter Intrabeam superficial x-ray applicators were measured with EBT3 Gafchromic film in a solid water phantom. Depth dose distributions and profiles (d=2, 5, 10 and 15mm) were obtained by prescribing a dose of 400cGy at 5mm depth below the phantom surface. Corresponding dose profiles for 6-MeV electrons were acquired from a Varian Clinac 21EX at 100 SSD. H and D calibration curves were generated for each modality for 0-800cGy. Results: Dose coverage, penumbra, dose uniformity, surface dose, and dose fall-off were examined. Compared to electrons, Intrabeam lateral dose coverage at 5mm depth was 70% larger with a much sharper (1/4) penumbra. Electron isodose levels bulged with depth, whereas Intrabeam isodose levels exhibited a convex cone shape. The Intrabeam dose profiles demonstrated horns in the dose distribution up to a 5mm depth and an exponential dose fall-off. Relative surface dose was higher for the Intrabeam applicators. Treatment times were comparable for both modalities. Conclusions: The very small penumbra of Intrabeam at shallow depths could be useful in treating superficial lesions adjacent to critical structures. The exponential dose fall-off of Intrabeam makes it appealing in the sparing of structures beyond the lesion. However, for lesions past a depth of 5mm, electrons would be desirable as they penetrate farther and provide skin sparing. Intrabeam may be preferable for sites that are difficult to treat with electrons due to mechanical and physical limitations.

  14. X-ray laser microscope apparatus

    DOE Patents [OSTI]

    Suckewer, Szymon (Princeton, NJ); DiCicco, Darrell S. (Plainsboro, NJ); Hirschberg, Joseph G. (Coral Gables, FL); Meixler, Lewis D. (East Windsor, NJ); Sathre, Robert (Princeton, NJ); Skinner, Charles H. (Lawrenceville, NJ)

    1990-01-01

    A microscope consisting of an x-ray contact microscope and an optical microscope. The optical, phase contrast, microscope is used to align a target with respect to a source of soft x-rays. The source of soft x-rays preferably comprises an x-ray laser but could comprise a synchrotron or other pulse source of x-rays. Transparent resist material is used to support the target. The optical microscope is located on the opposite side of the transparent resist material from the target and is employed to align the target with respect to the anticipated soft x-ray laser beam. After alignment with the use of the optical microscope, the target is exposed to the soft x-ray laser beam. The x-ray sensitive transparent resist material whose chemical bonds are altered by the x-ray beam passing through the target mater GOVERNMENT LICENSE RIGHTS This invention was made with government support under Contract No. De-FG02-86ER13609 awarded by the Department of Energy. The Government has certain rights in this invention.

  15. BURST FLUENCE DISTRIBUTIONS OF SOFT GAMMA REPEATERS 1806-20 AND 1900+14 IN THE ROSSI X-RAY TIMING EXPLORER PCA ERA

    SciTech Connect (OSTI)

    Prieskorn, Zachary; Kaaret, Philip, E-mail: prieskorn@psu.edu [Department of Physics and Astronomy, University of Iowa, Iowa City, IA 52242 (United States)

    2012-08-10

    We study the fluence distributions of over 3040 bursts from SGR 1806-20 and over 1963 bursts from SGR 1900+14 using the complete set of observations available from the Rossi X-Ray Timing Explorer/Proportional Counter Array through 2011 March. Cumulative event distributions are presented for both sources and are fitted with single and broken power laws as well as an exponential cutoff. The distributions are best fitted by a broken power law with exponential cutoff; however the statistical significance of the cutoff is not high and the upper portion of the broken power law can be explained as the expected number of false bursts due to random noise fluctuations. Event distributions are also examined in high and low burst rate regimes and power-law indices are found to be consistent, independent of the burst rate. The contribution function of the event fluence is calculated. This distribution shows that the energy released in the soft gamma repeater (SGR) bursts is dominated by the most powerful events for both sources. The power-law nature of these distributions combined with the dominant energy dissipation of the system occurring in the large, less frequent bursts is indicative of a self-organized critical system, as suggested by Gogus et al. in 1999.

  16. INTEGRAL SPI observations of Cygnus X-1 in the soft state: What about the jet contribution in hard X-rays?

    SciTech Connect (OSTI)

    Jourdain, E.; Roques, J. P.; Chauvin, M.

    2014-07-01

    During the first 7 yr of the INTEGRAL mission (2003-2009), Cyg X-1 has essentially been detected in its hard state (HS), with some incursions in intermediate HSs. This long, spectrally stable period allowed in particular the measurement of the polarization of the high-energy component that has long been observed above 200 keV in this peculiar object. This result strongly suggests that here we see the contribution of the jet, known to emit a strong synchrotron radio emission. In 2010 June, Cyg X-1 underwent a completed transition toward a soft state (SS). It gave us the unique opportunity to study in detail the corona emission in this spectral state, and to investigate in particular the behavior of the jet contribution. Indeed, during the SS, the hard X-ray emission decreases drastically, with its maximum energy shifted toward lower energy and its flux divided by a factor of ?5-10. Interestingly, the radio emission follows a similar drop, supporting the correlation between the jet emission and the hard component, even though the flux is too low to quantify the polarization characteristics.

  17. Simultaneous near-field and far-field imaging of the 11.9-nm Ni-like Sn soft-x-ray laser

    SciTech Connect (OSTI)

    Staub, F.; Braud, M.; Balmer, J.E.; Nilsen, J.; Bajt, S.

    2004-07-01

    We report on two-dimensional near-field imaging experiments of the 11.9-nm Sn x-ray laser that were performed with a set of Mo/Y multilayer mirrors having reflectivities of up to {approx}45% at normal and at 45 deg. incidence. Second-moment analysis of the x-ray laser emission was used to determine values of the x-ray beam propagation factor M{sup 2} for a range of irradiation parameters. The results reveal a reduction of M{sup 2} with increasing prepulse amplitude. The spatial size of the output is a factor of {approx}2 smaller than previously measured for the 14.7-nm Pd x-ray laser, while the distance of the x-ray emission with respect to the target surface remains roughly the same.

  18. X-Ray Diagnostics

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    including film developing and scanning, and image plate scanning. Related images X-ray framing camera being loaded into the TIM in the Trident North Target Area. X-ray framing...

  19. Performances of a bent-crystal spectrometer adapted to resonant x-ray emission measurements on gas-phase samples

    SciTech Connect (OSTI)

    Journel, Loiec; El Khoury, Lara; Marin, Thierry; Guillemin, Renaud; Carniato, Stephane; Avila, Antoine; Delaunay, Renaud; Hague, Coryn F.; Simon, Marc

    2009-09-15

    We describe a bent-crystal spectrometer adapted to measure x-ray emission resulting from core-level excitation of gas-phase molecules in the 0.8-8 keV energy range. The spectrometer is based on the Johann principle, and uses a microfocused photon beam to provide high-resolution (resolving power of {approx}7500). A gas cell was designed to hold a high-pressure (300 mbar) sample of gas while maintaining a high vacuum (10{sup -9} mbar) in the chamber. The cell was designed to optimize the counting rate (2000 cts/s at the maximum of the Cl K{alpha} emission line), while minimizing self-absorption. Example of the K{alpha} emission lines of CH{sub 3}Cl molecules is presented to illustrate the capabilities of this new instrument.

  20. X-Ray Diagnostics

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-Ray Diagnostics X-Ray Diagnostics Maintenance of existing devices and development of advanced concepts Contact John Oertel (505) 665-3246 Email Hot, dense matter produced by intense laser interaction with a solid target often produces x-rays with energies from 100 eV to those exceeding 100 keV. A suite of diagnostics and methods have been deployed at Trident to diagnose the x-ray emission from laser-matter interaction experiments, or to use the x-rays as a probe of dense matter. These

  1. Ultrafast dynamics of strong-field dissociative ionization ofCH2Br2 probed by femtosecond soft x-ray transient absorptionspectroscopy

    SciTech Connect (OSTI)

    Loh, Zhi-Heng; Leone, Stephen R.

    2008-01-15

    Femtosecond time-resolved soft x-ray transient absorption spectroscopy based on a high-order harmonic generation source is used to investigate the dissociative ionization of CH{sub 2}Br{sub 2} induced by 800 nm strong-field irradiation. At moderate peak intensities (2.0 x 10{sup 14} W/cm{sup 2}), strong-field ionization is accompanied by ultrafast C-Br bond dissociation, producing both neutral Br ({sup 2}P{sub 3/2}) and Br* ({sup 2}P{sub 1/2}) atoms together with the CH{sub 2}Br{sup +} fragment ion. The measured rise times for Br and Br* are 130 {+-} 22 fs and 74 {+-} 10 fs, respectively. The atomic bromine quantum state distribution shows that the Br/Br* population ratio is 8.1 {+-} 3.8 and that the Br {sup 2}P{sub 3/2} state is not aligned. The observed product distribution and the timescales of the photofragment appearances suggest that multiple field-dressed potential energy surfaces are involved in the dissociative ionization process. In addition, the transient absorption spectrum of CH{sub 2}Br{sub 2}{sup +} suggests that the alignment of the molecule relative to the polarization axis of the strong-field ionizing pulse determines the electronic symmetry of the resulting ion; alignment of the Br-Br, H-H, and C{sub 2} axis of the molecule along the polarization axis results in the production of the ion {tilde X}({sup 2}B{sub 2}), {tilde B}({sup 2}B{sub 1}) and {tilde C}({sup 2}A{sub 1}) states, respectively. At higher peak intensities (6.2 x 10{sup 14} W/cm{sup 2}), CH{sub 2}Br{sub 2}{sup +} undergoes sequential ionization to form the metastable CH{sub 2}Br{sub 2}{sup 2+} dication. These results demonstrate the potential of core-level probing with high-order harmonic transient absorption spectroscopy for studying ultrafast molecular dynamics.

  2. Characterization of a chiral phase in an achiral bent-core liquid crystal by polarization studies of resonant x-ray forbidden reflections

    SciTech Connect (OSTI)

    Ponsinet, V.; Pindak, R.; Barois, P.; Pan, L.; Wang, S.; Huang, C.C.; Wang, S.T.; Baumeister, U. and Weissflog, W.

    2011-07-15

    The chiral antiferroelectric structure of an achiral bent-core liquid crystal is characterized by resonant x-ray scattering at chlorine K edge. The 'forbidden' reflections resulting from the glide or screw symmetry elements are restored by the anisotropy of the tensor structure factor, which we calculate for two possible structural models. A careful analysis of the polarization states of the restored 'forbidden' reflections enables an unambiguous identification of a chiral structure (i.e., the so-called anticlinic, antiferroelectric smectic-C or Sm-C{sub A}P{sub A}) coexisting with the achiral synclinic antiferroelectric smectic-C or Sm-C{sub S}P{sub A}. The method proves to be quite powerful as it identifies the chiral structure within coexisting phases despite an imperfect orientation of the sample. The volume fraction of the chiral phase and the distribution of alignment are extracted from the data.

  3. Soft X-ray absorption spectroscopy of La{sub 0.7}Ca{sub 0.3}Mn{sub 1?X}Al{sub X}O{sub 3} thin films

    SciTech Connect (OSTI)

    Kumar, Manish Choudhary, R. J. Phase, D. M.

    2014-04-24

    Epitaxial thin films of rare earth manganites have generated much attention recently due to their rich phase diagram. The electronic structure of these films is playing a very crucial role and demands a fundamental understanding prior to device fabrication. We have investigated the electronic structure of La{sub 0.7}Ca{sub 0.3}Mn{sub 1?X}Al{sub X}O{sub 3} (X=0, 0.15) epitaxial thin films by soft X-ray absorption spectroscopy technique using the surface sensitive total electron yield (TEY) mode.

  4. High-energy magnetic excitations in overdoped La 2 - x Sr x CuO 4 studied by neutron and resonant inelastic x-ray scattering

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Wakimoto, S.; Ishii, K.; Kimura, H.; Fujita, M.; Dellea, G.; Kummer, K.; Braicovich, L.; Ghiringhelli, G.; Debeer-Schmitt, L. M.; Granroth, G. E.

    2015-05-21

    We have performed neutron inelastic scattering and resonant inelastic x-ray scattering (RIXS) at the Cu-L₃ edge to study high-energy magnetic excitations at energy transfers of more than 100 meV for overdoped La2-xSrxCuO₄ with x=0.25 (Tc=15 K) and x=0.30 (nonsuperconducting) using identical single-crystal samples for the two techniques. From constant-energy slices of neutron-scattering cross sections, we have identified magnetic excitations up to ~250 meV for x=0.25. Although the width in the momentum direction is large, the peak positions along the (π,π) direction agree with the dispersion relation of the spin wave in the nondoped La₂CuO₄ (LCO), which is consistent with themore » previous RIXS results of cuprate superconductors. Using RIXS at the Cu-L₃ edge, we have measured the dispersion relations of the so-called paramagnon mode along both (π,π) and (π,0) directions. Although in both directions the neutron and RIXS data connect with each other and the paramagnon along (π,0) agrees well with the LCO spin-wave dispersion, the paramagnon in the (π,π) direction probed by RIXS appears to be less dispersive and the excitation energy is lower than the spin wave of LCO near (π/2,π/2). Thus, our results indicate consistency between neutron inelastic scattering and RIXS, and elucidate the entire magnetic excitation in the (π,π) direction by the complementary use of two probes. The polarization dependence of the RIXS profiles indicates that appreciable charge excitations exist in the same energy range of magnetic excitations, reflecting the itinerant character of the overdoped sample. A possible anisotropy in the charge excitation intensity might explain the apparent differences in the paramagnon dispersion in the (π,π) direction as detected by the x-ray scattering.« less

  5. Chest x-Rays

    Broader source: Energy.gov [DOE]

    The B-reading is a special reading of a standard chest x-ray film performed by a physician certified by the National Institute for Occupational Safety and Health (NIOSH). The reading looks for changes on the chest x-ray that may indicate exposure and disease caused by agents such as asbestos or silica.

  6. Soft X-ray laser using pumping of 3P and 4P levels of He-like and H-like ions

    DOE Patents [OSTI]

    Hagelstein, Peter L. (Livermore, CA)

    1987-01-01

    X-ray laser method and apparatus for producing coherent radiation at, for example, energies of at least 40 eV, using Be-like Cr, N-like Ni, He-like Na, B-like Cr, Be-like Mn or similar multiply ionized species to pump appropriate high energy transitions in He-like or H-like N, O, F, C or rare gases, with associated laser transition gains of 4-50 cm.sup.-1.

  7. Soft x-ray laser using pumping of 3p and 4p levels of He-like and H-like ions

    DOE Patents [OSTI]

    Hagelstein, P.L.

    1985-07-05

    X-ray laser method and apparatus for producing coherent radiation at, for example, energies of at least 40 eV, using Be-like Cr, N-like Ni, He-like Na, B-like Cr, Be-like Mn or similar multiply ionized species to pump appropriate high energy transitions in He-like or H-like N, O, F, C or rare gases, with associated laser transition gains of 4 to 50 cm/sup -1/.

  8. X-Ray Diffraction Microscopy of Magnetic Structures

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-Ray Diffraction Microscopy of Magnetic Structures Print science brief icon Scientists working at ALS Beamline 12.0.2.2 have demonstrated a new x-ray technique for producing short-exposure nanoscale images of the magnetic structure of materials. The new method combines aspects of coherent x-ray diffraction, which can determine 3-D charge distributions, and resonant magnetic scattering, which is sensitive to magnetic structures. Physicists have used coherent x-ray diffraction to measure the

  9. X-Ray Diffraction Microscopy of Magnetic Structures

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-Ray Diffraction Microscopy of Magnetic Structures Print science brief icon Scientists working at ALS Beamline 12.0.2.2 have demonstrated a new x-ray technique for producing short-exposure nanoscale images of the magnetic structure of materials. The new method combines aspects of coherent x-ray diffraction, which can determine 3-D charge distributions, and resonant magnetic scattering, which is sensitive to magnetic structures. Physicists have used coherent x-ray diffraction to measure the

  10. X-Ray Diffraction Microscopy of Magnetic Structures

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-Ray Diffraction Microscopy of Magnetic Structures Print science brief icon Scientists working at ALS Beamline 12.0.2.2 have demonstrated a new x-ray technique for producing short-exposure nanoscale images of the magnetic structure of materials. The new method combines aspects of coherent x-ray diffraction, which can determine 3-D charge distributions, and resonant magnetic scattering, which is sensitive to magnetic structures. Physicists have used coherent x-ray diffraction to measure the

  11. X-Ray Diffraction Microscopy of Magnetic Structures

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-Ray Diffraction Microscopy of Magnetic Structures Print science brief icon Scientists working at ALS Beamline 12.0.2.2 have demonstrated a new x-ray technique for producing short-exposure nanoscale images of the magnetic structure of materials. The new method combines aspects of coherent x-ray diffraction, which can determine 3-D charge distributions, and resonant magnetic scattering, which is sensitive to magnetic structures. Physicists have used coherent x-ray diffraction to measure the

  12. Soft X-ray laser using pumping of 3P and 4P levels of He-like and H-like ions

    DOE Patents [OSTI]

    Hagelstein, P.L.

    1987-04-21

    X-ray laser method and apparatus are disclosed for producing coherent radiation at, for example, energies of at least 40 eV, using Be-like Cr, N-like Ni, He-like Na, B-like Cr, Be-like Mn or similar multiply ionized species to pump appropriate high energy transitions in He-like or H-like N, O, F, C or rare gases, with associated laser transition gains of 4-50 cm[sup [minus]1]. 8 figs.

  13. Soft x-ray laser using pumping of 3P and 4P levels of He-like and H-like ions

    DOE Patents [OSTI]

    Hagelstein, P.

    1982-03-26

    X-ray laser method and apparatus for producing coherent radiation at, for example, energies of 40 to 189 eV, using Be-like Cr, N-like Ni, He-like Na, B-like Cr, Be-like Mn or similar multiply ionized species to pump appropriate high energy transitions in He-like or H-like rare gases or N, O, F, or C gases, with associated laser transition gains of 20 to 50 cm/sup -1/.

  14. X-Ray Detection

    Office of Scientific and Technical Information (OSTI)

    ratio, I I on I off , recorded with plus (+, blue) and minus (-, red) x-ray helicities. This measurement was taken at -5 mA, which corresponds to a current...

  15. Probing the f-state configuration of URu2Si2 with U LIII-edge resonant x-ray absorption spectroscopy

    SciTech Connect (OSTI)

    Medling, S. A.; Booth, C. H.; Tobin, J. G.; Baumbach, R. E.; Bauer, E. D.; Sokaras, D.; Nordlund, D.; Weng, T. C.

    2015-09-05

    It has often been said that the most interesting ph- syics occurs when competing interactions are of nearly the same magnitude. Such a situation is surely oc- curing at URu2Si2’s so-called “hidden-order transition”, which garners its name from the missing entropy at a 17.5 K phase transition relative to that expected for a conventional antiferromagnetic phase transition, de- spite the presence of only a very small ordered mag- netic moment.? Despite this discrepancy being identi- fied in 1985, the identification of the order parameter remains elusive, although progress toward understand- ing this transition has been steady since that time, and URu2Si2 remains an important research subject today.? The work described below provides measures of the 5f orbital occupancy and itinerancy using resonant x-ray emission spectroscopy (RXES) at the U LIII absorption edge and measuring U L 1 emission that potentially acts as a dividing line between different classes of “hidden- order” theories.

  16. X-ray fluorescence mapping

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-Ray Microscopy and Imaging: X-ray Fluorescence Mapping Of increasing scientific interest is the detection, quantification and mapping of elemental content of samples, often down...

  17. X-ray Imaging Workshop

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    microscopy (PEEM), angle resolved photoemission spectroscopy (ARPES), coherent diffraction imaging, x-ray microscopy, micro-tomography, holographic imaging, and x-ray...

  18. Gamma Radiation & X-Rays

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Gamma Radiation and X-Rays 1. Gamma radiation and X-rays are electromagnetic radiation like visible light, radio waves, and ultraviolet light. These electromagnetic radiations...

  19. Compton backscattered collimated x-ray source

    DOE Patents [OSTI]

    Ruth, R.D.; Huang, Z.

    1998-10-20

    A high-intensity, inexpensive and collimated x-ray source is disclosed for applications such as x-ray lithography is disclosed. An intense pulse from a high power laser, stored in a high-finesse resonator, repetitively collides nearly head-on with and Compton backscatters off a bunched electron beam, having relatively low energy and circulating in a compact storage ring. Both the laser and the electron beams are tightly focused and matched at the interaction region inside the optical resonator. The laser-electron interaction not only gives rise to x-rays at the desired wavelength, but also cools and stabilizes the electrons against intrabeam scattering and Coulomb repulsion with each other in the storage ring. This cooling provides a compact, intense bunch of electrons suitable for many applications. In particular, a sufficient amount of x-rays can be generated by this device to make it an excellent and flexible Compton backscattered x-ray (CBX) source for high throughput x-ray lithography and many other applications. 4 figs.

  20. Compton backscattered collimated x-ray source

    DOE Patents [OSTI]

    Ruth, Ronald D. (Woodside, CA); Huang, Zhirong (Stanford, CA)

    1998-01-01

    A high-intensity, inexpensive and collimated x-ray source for applications such as x-ray lithography is disclosed. An intense pulse from a high power laser, stored in a high-finesse resonator, repetitively collides nearly head-on with and Compton backscatters off a bunched electron beam, having relatively low energy and circulating in a compact storage ring. Both the laser and the electron beams are tightly focused and matched at the interaction region inside the optical resonator. The laser-electron interaction not only gives rise to x-rays at the desired wavelength, but also cools and stabilizes the electrons against intrabeam scattering and Coulomb repulsion with each other in the storage ring. This cooling provides a compact, intense bunch of electrons suitable for many applications. In particular, a sufficient amount of x-rays can be generated by this device to make it an excellent and flexible Compton backscattered x-ray (CBX) source for high throughput x-ray lithography and many other applications.

  1. Compton backscattered collmated X-ray source

    DOE Patents [OSTI]

    Ruth, Ronald D. (Woodside, CA); Huang, Zhirong (Stanford, CA)

    2000-01-01

    A high-intensity, inexpensive and collimated x-ray source for applications such as x-ray lithography is disclosed. An intense pulse from a high power laser, stored in a high-finesse resonator, repetitively collides nearly head-on with and Compton backscatters off a bunched electron beam, having relatively low energy and circulating in a compact storage ring. Both the laser and the electron beams are tightly focused and matched at the interaction region inside the optical resonator. The laser-electron interaction not only gives rise to x-rays at the desired wavelength, but also cools and stabilizes the electrons against intrabeam scattering and Coulomb repulsion with each other in the storage ring. This cooling provides a compact, intense bunch of electrons suitable for many applications. In particular, a sufficient amount of x-rays can be generated by this device to make it an excellent and flexible Compton backscattered x-ray (CBX) source for high throughput x-ray lithography and many other applications.

  2. X-ray microtomography

    SciTech Connect (OSTI)

    Landis, Eric N.; Keane, Denis T.

    2010-12-15

    In this tutorial, we describe X-ray microtomography as a technique to nondestructively characterize material microstructure in three dimensions at a micron level spatial resolution. While commercially available laboratory scale instrumentation is available, we focus our attention on synchrotron-based systems, where we can exploit a high flux, monochromatic X-ray beam to produce high fidelity three-dimensional images. A brief description of the physics and the mathematical analysis behind the technique is followed by example applications to specific materials characterization problems, with a particular focus on the utilization of three-dimensional image processing that can be used to extract a wide range of useful information.

  3. X-ray beam finder

    DOE Patents [OSTI]

    Gilbert, H.W.

    1983-06-16

    An X-ray beam finder for locating a focal spot of an X-ray tube includes a mass of X-ray opaque material having first and second axially-aligned, parallel-opposed faces connected by a plurality of substantially identical parallel holes perpendicular to the faces and a film holder for holding X-ray sensitive film tightly against one face while the other face is placed in contact with the window of an X-ray head.

  4. Full multiple scattering analysis of XANES at the Cd L3 and O K edges in CdO films combined with a soft-x-ray emission investigation

    SciTech Connect (OSTI)

    Demchenko, I. N.; Denlinger, J. D.; Chernyshova, M.; Yu, K. M.; Speaks, D. T.; Olalde-Velasco, P.; Hemmers, O.; Walukiewicz, W.; Derkachova, A.; Lawniczak-Jablonska, K.

    2010-07-05

    X-ray absorption near edge structure (XANES) at the cadmium L3 and oxygen K edges for CdO thin films grown by pulsed laser deposition method, is interpreted within the real-space multiple scattering formalism, FEFF code. The features in the experimental spectra are well reproduced by calculations for a cluster of about six and ten coordination shells around the absorber for L3 edge of Cd and K edge of O, respectively. The calculated projected electronic density of states is found to be in good agreement with unoccupied electronic states in experimental data and allows to conclude that the orbital character of the lowest energy of the conductive band is Cd-5s-O-2p. The charge transfer has been quantified and not purely ionic bonding has been found. Combined XANES and resonant inelastic x-ray scattering measurements allow us to determine the direct and indirect band gap of investigated CdO films to be {approx}2.4-eV and {approx}0.9-eV, respectively.

  5. Fabrication process for a gradient index x-ray lens

    DOE Patents [OSTI]

    Bionta, R.M.; Makowiecki, D.M.; Skulina, K.M.

    1995-01-17

    A process is disclosed for fabricating high efficiency x-ray lenses that operate in the 0.5-4.0 keV region suitable for use in biological imaging, surface science, and x-ray lithography of integrated circuits. The gradient index x-ray optics fabrication process broadly involves co-sputtering multi-layers of film on a wire, followed by slicing and mounting on block, and then ion beam thinning to a thickness determined by periodic testing for efficiency. The process enables the fabrication of transmissive gradient index x-ray optics for the 0.5-4.0 keV energy range. This process allows the fabrication of optical elements for the next generation of imaging and x-ray lithography instruments in the soft x-ray region. 13 figures.

  6. Fabrication process for a gradient index x-ray lens

    DOE Patents [OSTI]

    Bionta, Richard M. (Livermore, CA); Makowiecki, Daniel M. (Livermore, CA); Skulina, Kenneth M. (Livermore, CA)

    1995-01-01

    A process for fabricating high efficiency x-ray lenses that operate in the 0.5-4.0 keV region suitable for use in biological imaging, surface science, and x-ray lithography of integrated circuits. The gradient index x-ray optics fabrication process broadly involves co-sputtering multi-layers of film on a wire, followed by slicing and mounting on block, and then ion beam thinning to a thickness determined by periodic testing for efficiency. The process enables the fabrication of transmissive gradient index x-ray optics for the 0.5-4.0 keV energy range. This process allows the fabrication of optical elements for the next generation of imaging and x-ray lithography instruments m the soft x-ray region.

  7. X-RAY POINT-SOURCE POPULATIONS CONSTITUTING THE GALACTIC RIDGE X-RAY EMISSION

    SciTech Connect (OSTI)

    Morihana, Kumiko [Institute of Physical and Chemical Research (RIKEN), 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan)] [Institute of Physical and Chemical Research (RIKEN), 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Tsujimoto, Masahiro; Ebisawa, Ken [Japan Aerospace Exploration Agency, Institute of Space and Astronautical Science, 3-1-1 Yoshino-dai, Chuo-ku, Sagamihara, Kanagawa 252-5210 (Japan)] [Japan Aerospace Exploration Agency, Institute of Space and Astronautical Science, 3-1-1 Yoshino-dai, Chuo-ku, Sagamihara, Kanagawa 252-5210 (Japan); Yoshida, Tessei, E-mail: morihana@crab.riken.jp [National Astronomical Observatory of Japan, 2-21-1, Osawa, Mitaka, Tokyo 181-8588 (Japan)] [National Astronomical Observatory of Japan, 2-21-1, Osawa, Mitaka, Tokyo 181-8588 (Japan)

    2013-03-20

    Apparently diffuse X-ray emission has been known to exist along the central quarter of the Galactic Plane since the beginning of X-ray astronomy; this is referred to as the Galactic Ridge X-ray emission (GRXE). Recent deep X-ray observations have shown that numerous X-ray point sources account for a large fraction of the GRXE in the hard band (2-8 keV). However, the nature of these sources is poorly understood. Using the deepest X-ray observations made in the Chandra bulge field, we present the result of a coherent photometric and spectroscopic analysis of individual X-ray point sources for the purpose of constraining their nature and deriving their fractional contributions to the hard-band continuum and Fe K line emission of the GRXE. Based on the X-ray color-color diagram, we divided the point sources into three groups: A (hard), B (soft and broad spectrum), and C (soft and peaked spectrum). The group A sources are further decomposed spectrally into thermal and non-thermal sources with different fractions in different flux ranges. From their X-ray properties, we speculate that the group A non-thermal sources are mostly active galactic nuclei and the thermal sources are mostly white dwarf (WD) binaries such as magnetic and non-magnetic cataclysmic variables (CVs), pre-CVs, and symbiotic stars, whereas the group B and C sources are X-ray active stars in flares and quiescence, respectively. In the log N-log S curve of the 2-8 keV band, the group A non-thermal sources are dominant above Almost-Equal-To 10{sup -14} erg cm{sup -2} s{sup -1}, which is gradually taken over by Galactic sources in the fainter flux ranges. The Fe K{alpha} emission is mostly from the group A thermal (WD binaries) and the group B (X-ray active stars) sources.

  8. Tunable X-ray source

    DOE Patents [OSTI]

    Boyce, James R. (Williamsburg, VA)

    2011-02-08

    A method for the production of X-ray bunches tunable in both time and energy level by generating multiple photon, X-ray, beams through the use of Thomson scattering. The method of the present invention simultaneously produces two X-ray pulses that are tunable in energy and/or time.

  9. Miniature x-ray source

    DOE Patents [OSTI]

    Trebes, James E. (Livermore, CA); Stone, Gary F. (Livermore, CA); Bell, Perry M. (Tracy, CA); Robinson, Ronald B. (Modesto, CA); Chornenky, Victor I. (Minnetonka, MN)

    2002-01-01

    A miniature x-ray source capable of producing broad spectrum x-ray emission over a wide range of x-ray energies. The miniature x-ray source comprises a compact vacuum tube assembly containing a cathode, an anode, a high voltage feedthru for delivering high voltage to the anode, a getter for maintaining high vacuum, a connection for an initial vacuum pump down and crimp-off, and a high voltage connection for attaching a compact high voltage cable to the high voltage feedthru. At least a portion of the vacuum tube wall is highly x-ray transparent and made, for example, from boron nitride. The compact size and potential for remote operation allows the x-ray source, for example, to be placed adjacent to a material sample undergoing analysis or in proximity to the region to be treated for medical applications.

  10. X-Ray Science Education

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    TV Network external link DNA Interactive external link Reciprocal Net external link X-ray Science Courses and Programs Various educational efforts are closely related to the...

  11. X-ray shearing interferometer

    DOE Patents [OSTI]

    Koch, Jeffrey A. (Livermore, CA)

    2003-07-08

    An x-ray interferometer for analyzing high density plasmas and optically opaque materials includes a point-like x-ray source for providing a broadband x-ray source. The x-rays are directed through a target material and then are reflected by a high-quality ellipsoidally-bent imaging crystal to a diffraction grating disposed at 1.times. magnification. A spherically-bent imaging crystal is employed when the x-rays that are incident on the crystal surface are normal to that surface. The diffraction grating produces multiple beams which interfere with one another to produce an interference pattern which contains information about the target. A detector is disposed at the position of the image of the target produced by the interfering beams.

  12. Cryogenic, high-resolution x-ray detector with high count rate capability

    DOE Patents [OSTI]

    Frank, Matthias (Oakland, CA); Mears, Carl A. (Windsor, CA); Labov, Simon E. (Berkeley, CA); Hiller, Larry J. (Livermore, CA); Barfknecht, Andrew T. (Menlo Park, CA)

    2003-03-04

    A cryogenic, high-resolution X-ray detector with high count rate capability has been invented. The new X-ray detector is based on superconducting tunnel junctions (STJs), and operates without thermal stabilization at or below 500 mK. The X-ray detector exhibits good resolution (.about.5-20 eV FWHM) for soft X-rays in the keV region, and is capable of counting at count rates of more than 20,000 counts per second (cps). Simple, FET-based charge amplifiers, current amplifiers, or conventional spectroscopy shaping amplifiers can provide the electronic readout of this X-ray detector.

  13. Miniature x-ray source

    DOE Patents [OSTI]

    Trebes, James E. (Livermore, CA); Bell, Perry M. (Tracy, CA); Robinson, Ronald B. (Modesto, CA)

    2000-01-01

    A miniature x-ray source utilizing a hot filament cathode. The source has a millimeter scale size and is capable of producing broad spectrum x-ray emission over a wide range of x-ray energies. The miniature source consists of a compact vacuum tube assembly containing the hot filament cathode, an anode, a high voltage feedthru for delivering high voltage to the cathode, a getter for maintaining high vacuum, a connector for initial vacuum pump down and crimp-off, and a high voltage connection for attaching a compact high voltage cable to the high voltage feedthru. At least a portion of the vacuum tube wall is fabricated from highly x-ray transparent materials, such as sapphire, diamond, or boron nitride.

  14. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless X-Ray Imaging in Reflection Lensless X-Ray Imaging in Reflection Print Wednesday, 26 October 2011 00:00 The advent of x-ray free-electron laser (XFEL) light sources has...

  15. SMB, X-ray Absorption Spectroscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Absorption Spectroscopy X-ray Absorption Spectroscopy X-ray absorption spectroscopy (XAS) is a well-established technique for simultaneous local geometric and electronic structure...

  16. Vanadium-pumped titanium x-ray laser

    DOE Patents [OSTI]

    Nilsen, Joseph (Livermore, CA)

    1992-01-01

    A resonantly photo-pumped x-ray laser (10) is formed of a vanadium (12) and titanium (14) foil combination (16) that is driven by two beams (18, 20) of intense line focused (22, 24) optical laser radiation. Ground state neon-like titanium ions (34) are resonantly photo-pumped by line emission from fluorine-like vanadium ions (32).

  17. Vanadium-pumped titanium x-ray laser

    DOE Patents [OSTI]

    Nilsen, J.

    1992-05-26

    A resonantly photo-pumped x-ray laser is formed of a vanadium and titanium foil combination that is driven by two beams of intense line focused optical laser radiation. Ground state neon-like titanium ions are resonantly photo-pumped by line emission from fluorine-like vanadium ions. 4 figs.

  18. Compact x-ray source and panel

    DOE Patents [OSTI]

    Sampayon, Stephen E. (Manteca, CA)

    2008-02-12

    A compact, self-contained x-ray source, and a compact x-ray source panel having a plurality of such x-ray sources arranged in a preferably broad-area pixelized array. Each x-ray source includes an electron source for producing an electron beam, an x-ray conversion target, and a multilayer insulator separating the electron source and the x-ray conversion target from each other. The multi-layer insulator preferably has a cylindrical configuration with a plurality of alternating insulator and conductor layers surrounding an acceleration channel leading from the electron source to the x-ray conversion target. A power source is connected to each x-ray source of the array to produce an accelerating gradient between the electron source and x-ray conversion target in any one or more of the x-ray sources independent of other x-ray sources in the array, so as to accelerate an electron beam towards the x-ray conversion target. The multilayer insulator enables relatively short separation distances between the electron source and the x-ray conversion target so that a thin panel is possible for compactness. This is due to the ability of the plurality of alternating insulator and conductor layers of the multilayer insulators to resist surface flashover when sufficiently high acceleration energies necessary for x-ray generation are supplied by the power source to the x-ray sources.

  19. Focused X-ray source

    DOE Patents [OSTI]

    Piestrup, M.A.; Boyers, D.G.; Pincus, C.I.; Maccagno, P.

    1990-08-21

    Disclosed is an intense, relatively inexpensive X-ray source (as compared to a synchrotron emitter) for technological, scientific, and spectroscopic purposes. A conical radiation pattern produced by a single foil or stack of foils is focused by optics to increase the intensity of the radiation at a distance from the conical radiator. 8 figs.

  20. Focused X-ray source

    DOE Patents [OSTI]

    Piestrup, Melvin A. (Woodside, CA); Boyers, David G. (Mountain View, CA); Pincus, Cary I. (Sunnyvale, CA); Maccagno, Pierre (Stanford, CA)

    1990-01-01

    An intense, relatively inexpensive X-ray source (as compared to a synchrotron emitter) for technological, scientific, and spectroscopic purposes. A conical radiation pattern produced by a single foil or stack of foils is focused by optics to increase the intensity of the radiation at a distance from the conical radiator.

  1. Magnetic structures of FeTiO{sub 3}-Fe{sub 2}O{sub 3} solid solution thin films studied by soft X-ray magnetic circular dichroism and ab initio multiplet calculations

    SciTech Connect (OSTI)

    Hojo, H. E-mail: fujita@dipole7.kuic.kyoto-u.ac.jp; Fujita, K. E-mail: fujita@dipole7.kuic.kyoto-u.ac.jp; Matoba, T.; Tanaka, K.; Ikeno, H.; Mizoguchi, T.; Tanaka, I.; Nakamura, T.; Takeda, Y.; Okane, T.

    2014-03-17

    The solid solutions between ilmenite (FeTiO{sub 3}) and hematite (α-Fe{sub 2}O{sub 3}) have recently attracted considerable attention as a spintronic material due to their interesting magnetic and electrical properties. In this study, the electronic and magnetic structures of epitaxially grown 0.6FeTiO{sub 3}·0.4Fe{sub 2}O{sub 3} solid solution thin films were investigated by combining x-ray absorption near-edge structure (XANES), x-ray magnetic circular dichroism (XMCD) for two different crystallographic projections, and first-principles theoretical calculations. The Fe L-edge XANES and XMCD spectra reveal that Fe is in the mixed-valent Fe{sup 2+}–Fe{sup 3+} states while Fe{sup 2+} ions are mainly responsible for the magnetization. Moreover, the experimental Fe L-edge XANES and XMCD spectra change depending on the incident x-ray directions, and the theoretical spectra explain such spectral features. We also find a large orbital magnetic moment, which can originate the magnetic anisotropy of this system. On the other hand, although the valence state of Ti was interpreted to be 4+ from the Ti L-edge XANES, XMCD signals indicate that some electrons are present in the Ti-3d orbital, which are coupled antiparallel to the magnetic moment of Fe{sup 2+} ions.

  2. Hard x-ray delay line for x-ray photon correlation spectroscopy...

    Office of Scientific and Technical Information (OSTI)

    Hard x-ray delay line for x-ray photon correlation spectroscopy and jitter-free pump-probe experiments at LCLS Citation Details In-Document Search Title: Hard x-ray delay line for...

  3. A computational study of x-ray emission from high-Z x-ray sources...

    Office of Scientific and Technical Information (OSTI)

    study of x-ray emission from high-Z x-ray sources on the National Ignition Facility laser Citation Details In-Document Search Title: A computational study of x-ray emission...

  4. Femtosecond X-ray Absorption Spectroscopy at a Hard X-ray Free...

    Office of Scientific and Technical Information (OSTI)

    Femtosecond X-ray Absorption Spectroscopy at a Hard X-ray Free Electron Laser: Application to Spin Crossover Dynamics Citation Details In-Document Search Title: Femtosecond X-ray...

  5. Microgap x-ray detector

    DOE Patents [OSTI]

    Wuest, C.R.; Bionta, R.M.; Ables, E.

    1994-05-03

    An x-ray detector is disclosed which provides for the conversion of x-ray photons into photoelectrons and subsequent amplification of these photoelectrons through the generation of electron avalanches in a thin gas-filled region subject to a high electric potential. The detector comprises a cathode (photocathode) and an anode separated by the thin, gas-filled region. The cathode may comprise a substrate, such a beryllium, coated with a layer of high atomic number material, such as gold, while the anode can be a single conducting plane of material, such as gold, or a plane of resistive material, such as chromium/silicon monoxide, or multiple areas of conductive or resistive material, mounted on a substrate composed of glass, plastic or ceramic. The charge collected from each electron avalanche by the anode is passed through processing electronics to a point of use, such as an oscilloscope. 3 figures.

  6. Microgap x-ray detector

    DOE Patents [OSTI]

    Wuest, Craig R.; Bionta, Richard M.; Ables, Elden

    1994-01-01

    An x-ray detector which provides for the conversion of x-ray photons into photoelectrons and subsequent amplification of these photoelectrons through the generation of electron avalanches in a thin gas-filled region subject to a high electric potential. The detector comprises a cathode (photocathode) and an anode separated by the thin, gas-filled region. The cathode may comprise a substrate, such a beryllium, coated with a layer of high atomic number material, such as gold, while the anode can be a single conducting plane of material, such as gold, or a plane of resistive material, such as chromium/silicon monoxide, or multiple areas of conductive or resistive material, mounted on a substrate composed of glass, plastic or ceramic. The charge collected from each electron avalanche by the anode is passed through processing electronics to a point of use, such as an oscilloscope.

  7. EVIDENCE OF NON-THERMAL X-RAY EMISSION FROM HH 80

    SciTech Connect (OSTI)

    Lpez-Santiago, J.; Peri, C. S.; Benaglia, P.; Bonito, R.; Miceli, M.; Albacete-Colombo, J. F.; De Castro, E.

    2013-10-20

    Protostellar jets appear at all stages of star formation when the accretion process is still at work. Jets travel at velocities of hundreds of km s{sup 1}, creating strong shocks when interacting with the interstellar medium. Several cases of jets have been detected in X-rays, typically showing soft emission. For the first time, we report evidence of hard X-ray emission possibly related to non-thermal processes not explained by previous models of the post-shock emission predicted in the jet/ambient interaction scenario. HH 80 is located at the south head of the jet associated with the massive protostar IRAS 18162-2048. It shows soft and hard X-ray emission in regions that are spatially separated, with the soft X-ray emission region situated behind the region of hard X-ray emission. We propose a scenario for HH 80 where soft X-ray emission is associated with thermal processes from the interaction of the jet with denser ambient matter and hard X-ray emission is produced by synchrotron radiation at the front shock.

  8. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-Ray Imaging in Reflection Print The advent of x-ray free-electron laser (XFEL) light sources has led to an outburst of research activities in the field of lensless imaging. XFELs...

  9. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless X-Ray Imaging in Reflection Print The advent of x-ray free-electron laser (XFEL) light sources has led to an outburst of research activities in the field of lensless...

  10. X-Ray Nanoimaging: Instruments and Methods

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-Ray Nanoimaging: Instruments and Methods X-Ray Nanoimaging: Instruments and Methods Print To be held as part of SPIE. http://spie.org/OP318 August 28-29, 2013; San Diego, California, USA

  11. Producing X-rays at the APS

    ScienceCinema (OSTI)

    None

    2013-04-19

    An introduction and overview of the Advanced Photon Source at Argonne National Laboratory, the technology that produces the brightest X-ray beams in the Western Hemisphere, and the research carried out by scientists using those X-rays.

  12. Neutron and X-ray Scattering

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Neutron and X-ray Scattering Neutron and X-ray Scattering When used together, neutrons and high-energy x-rays provide a supremely powerful scientific tool for mining details about the structure of materials. Combining neutrons and high-energy x-rays to explore the frontiers of materials in extreme environments. Illuminating previously inaccessible time and spatial scales. Enabling in situ research to design, discover, and control materials. Get Expertise Donald Brown Email Pushing the limits of

  13. Phase-sensitive X-ray imager

    DOE Patents [OSTI]

    Baker, Kevin Louis

    2013-01-08

    X-ray phase sensitive wave-front sensor techniques are detailed that are capable of measuring the entire two-dimensional x-ray electric field, both the amplitude and phase, with a single measurement. These Hartmann sensing and 2-D Shear interferometry wave-front sensors do not require a temporally coherent source and are therefore compatible with x-ray tubes and also with laser-produced or x-pinch x-ray sources.

  14. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless X-Ray Imaging in Reflection Print The advent of x-ray free-electron laser (XFEL) light sources has led to an outburst of research activities in the field of lensless imaging. XFELs combine the advantages of sychrotron light sources (high brightness and x-ray wavelengths relevant to atomic and molecular phenomena) with the advantages of visible-light lasers (highly coherent beams). All of these characteristics are important for coherent x-ray diffraction imaging-lensless imaging

  15. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless X-Ray Imaging in Reflection Print The advent of x-ray free-electron laser (XFEL) light sources has led to an outburst of research activities in the field of lensless imaging. XFELs combine the advantages of sychrotron light sources (high brightness and x-ray wavelengths relevant to atomic and molecular phenomena) with the advantages of visible-light lasers (highly coherent beams). All of these characteristics are important for coherent x-ray diffraction imaging-lensless imaging

  16. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless X-Ray Imaging in Reflection Print The advent of x-ray free-electron laser (XFEL) light sources has led to an outburst of research activities in the field of lensless imaging. XFELs combine the advantages of sychrotron light sources (high brightness and x-ray wavelengths relevant to atomic and molecular phenomena) with the advantages of visible-light lasers (highly coherent beams). All of these characteristics are important for coherent x-ray diffraction imaging-lensless imaging

  17. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless X-Ray Imaging in Reflection Print The advent of x-ray free-electron laser (XFEL) light sources has led to an outburst of research activities in the field of lensless imaging. XFELs combine the advantages of sychrotron light sources (high brightness and x-ray wavelengths relevant to atomic and molecular phenomena) with the advantages of visible-light lasers (highly coherent beams). All of these characteristics are important for coherent x-ray diffraction imaging-lensless imaging

  18. Cryotomography x-ray microscopy state

    DOE Patents [OSTI]

    Le Gros, Mark (Berkeley, CA); Larabell, Carolyn A. (Berkeley, CA)

    2010-10-26

    An x-ray microscope stage enables alignment of a sample about a rotation axis to enable three dimensional tomographic imaging of the sample using an x-ray microscope. A heat exchanger assembly provides cooled gas to a sample during x-ray microscopic imaging.

  19. X-ray transmissive debris shield

    DOE Patents [OSTI]

    Spielman, R.B.

    1996-05-21

    An X-ray debris shield for use in X-ray lithography that is comprised of an X-ray window having a layer of low density foam exhibits increased longevity without a substantial increase in exposure time. The low density foam layer serves to absorb the debris emitted from the X-ray source and attenuate the shock to the window so as to reduce the chance of breakage. Because the foam is low density, the X-rays are hardly attenuated by the foam and thus the exposure time is not substantially increased.

  20. X-ray transmissive debris shield

    DOE Patents [OSTI]

    Spielman, Rick B. (Albuquerque, NM)

    1996-01-01

    An X-ray debris shield for use in X-ray lithography that is comprised of an X-ray window having a layer of low density foam exhibits increased longevity without a substantial increase in exposure time. The low density foam layer serves to absorb the debris emitted from the X-ray source and attenuate the shock to the window so as to reduce the chance of breakage. Because the foam is low density, the X-rays are hardly attenuated by the foam and thus the exposure time is not substantially increased.

  1. X-Ray Microscopy | Argonne National Laboratory

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-Ray Microscopy X-Ray Microscopy This group exploits the unique capabilities of hard X-ray microscopy to visualize and understand the structure and behavior of hybrid, energy-related, and tailored nanomaterials The Hard X-Ray Nanoprobe, located at Sector 26 of the Advanced Photon Source (APS) and operated by our group and APS, is the only dedicated X-ray microscopy beamline within the portfolios of the nation's Nanoscale Science Research Centers. Our scientific program seeks to understand

  2. X-ray lithography using holographic images

    DOE Patents [OSTI]

    Howells, Malcolm R. (Berkeley, CA); Jacobsen, Chris (Sound Beach, NY)

    1995-01-01

    A non-contact X-ray projection lithography method for producing a desired X-ray image on a selected surface of an X-ray-sensitive material, such as photoresist material on a wafer, the desired X-ray image having image minimum linewidths as small as 0.063 .mu.m, or even smaller. A hologram and its position are determined that will produce the desired image on the selected surface when the hologram is irradiated with X-rays from a suitably monochromatic X-ray source of a selected wavelength .lambda.. On-axis X-ray transmission through, or off-axis X-ray reflection from, a hologram may be used here, with very different requirements for monochromaticity, flux and brightness of the X-ray source. For reasonable penetration of photoresist materials by X-rays produced by the X-ray source, the wavelength X, is preferably chosen to be no more than 13.5 nm in one embodiment and more preferably is chosen in the range 1-5 nm in the other embodiment. A lower limit on linewidth is set by the linewidth of available microstructure writing devices, such as an electron beam.

  3. Controlling X-rays With Light

    SciTech Connect (OSTI)

    Glover, Ernie; Hertlein, Marcus; Southworth, Steve; Allison, Tom; van Tilborg, Jeroen; Kanter, Elliot; Krassig, B.; Varma, H.; Rude, Bruce; Santra, Robin; Belkacem, Ali; Young, Linda

    2010-08-02

    Ultrafast x-ray science is an exciting frontier that promises the visualization of electronic, atomic and molecular dynamics on atomic time and length scales. A largelyunexplored area of ultrafast x-ray science is the use of light to control how x-rays interact with matter. In order to extend control concepts established for long wavelengthprobes to the x-ray regime, the optical control field must drive a coherent electronic response on a timescale comparable to femtosecond core-hole lifetimes. An intense field is required to achieve this rapid response. Here an intense optical control pulse isobserved to efficiently modulate photoelectric absorption for x-rays and to create an ultrafast transparency window. We demonstrate an application of x-ray transparencyrelevant to ultrafast x-ray sources: an all-photonic temporal cross-correlation measurement of a femtosecond x-ray pulse. The ability to control x-ray/matterinteractions with light will create new opportunities at current and next-generation x-ray light sources.

  4. Some new schemes for producing high-accuracy elliptical X-ray mirrors by elastic bending

    SciTech Connect (OSTI)

    Padmore, H.A.; Howells, M.R.; Irick, S.; Renner, T.; Sandler, R.; Koo, Y.-M.

    1996-08-01

    Although x-ray micro-foci can be produced by a variety of diffractive methods, grazing incidence mirrors are the only route to an achromatic focus. In this paper we describe our efforts to produce elliptically shaped mirrors with the very high figure accuracy necessary for producing a micro-focus. The motivation for this work is provided by the need to produce achromatic foci for a range of applications ranging from tunable micro-focus x-ray photoelectron spectroscopy ({mu}-XPS) at soft x-ray energies to micro-focus white beam x-ray diffraction ({mu}-XRD) at hard x-ray energies. We describe the methodology of beam bending, a practical example of a system we have produced for {mu}-XRD, and results demonstrating the production of a surface with micro-radian figure accuracy.

  5. X-ray transmissive debris shield

    DOE Patents [OSTI]

    Spielman, Rick B. (Albuquerque, NM)

    1994-01-01

    A composite window structure is described for transmitting x-ray radiation and for shielding radiation generated debris. In particular, separate layers of different x-ray transmissive materials are laminated together to form a high strength, x-ray transmissive debris shield which is particularly suited for use in high energy fluences. In one embodiment, the composite window comprises alternating layers of beryllium and a thermoset polymer.

  6. High speed x-ray beam chopper

    DOE Patents [OSTI]

    McPherson, Armon (Oswego, IL); Mills, Dennis M. (Naperville, IL)

    2002-01-01

    A fast, economical, and compact x-ray beam chopper with a small mass and a small moment of inertia whose rotation can be synchronized and phase locked to an electronic signal from an x-ray source and be monitored by a light beam is disclosed. X-ray bursts shorter than 2.5 microseconds have been produced with a jitter time of less than 3 ns.

  7. X-ray microscopy. Beyond ensemble averages

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Ice, Gene E.; Budai, John D.

    2015-06-23

    This work exemplifies emerging tools to characterize local materials structure and dynamics, made possible by powerful X-ray synchrotron and transmission electron microscopy methods.

  8. Compound refractive X-ray lens

    DOE Patents [OSTI]

    Nygren, David R. (Berkeley, CA); Cahn, Robert (Walnut Creek, CA); Cederstrom, Bjorn (Traellborg, SE); Danielsson, Mats (Stocksund, SE); Vestlund, Jonas (Stockholm, SE)

    2000-01-01

    An apparatus and method for focusing X-rays. In one embodiment, his invention is a commercial-grade compound refractive X-ray lens. The commercial-grade compound refractive X-ray lens includes a volume of low-Z material. The volume of low-Z material has a first surface which is adapted to receive X-rays of commercially-applicable power emitted from a commercial-grade X-ray source. The volume of low-Z material also has a second surface from which emerge the X-rays of commercially-applicable power which were received at the first surface. Additionally, the commercial-grade compound refractive X-ray lens includes a plurality of openings which are disposed between the first surface and the second surface. The plurality of openings are oriented such that the X-rays of commercially-applicable power which are received at the first surface, pass through the volume of low-Z material and through the plurality openings. In so doing, the X-rays which emerge from the second surface are refracted to a focal point.

  9. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-Ray Imaging in Reflection Print The advent of x-ray free-electron laser (XFEL) light sources has led to an outburst of research activities in the field of lensless imaging. XFELs combine the advantages of sychrotron light sources (high brightness and x-ray wavelengths relevant to atomic and molecular phenomena) with the advantages of visible-light lasers (highly coherent beams). All of these characteristics are important for coherent x-ray diffraction imaging-lensless imaging techniques that

  10. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-Ray Imaging in Reflection Print The advent of x-ray free-electron laser (XFEL) light sources has led to an outburst of research activities in the field of lensless imaging. XFELs combine the advantages of sychrotron light sources (high brightness and x-ray wavelengths relevant to atomic and molecular phenomena) with the advantages of visible-light lasers (highly coherent beams). All of these characteristics are important for coherent x-ray diffraction imaging-lensless imaging techniques that

  11. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless X-Ray Imaging in Reflection Lensless X-Ray Imaging in Reflection Print Wednesday, 26 October 2011 00:00 The advent of x-ray free-electron laser (XFEL) light sources has led to an outburst of research activities in the field of lensless imaging. XFELs combine the advantages of sychrotron light sources (high brightness and x-ray wavelengths relevant to atomic and molecular phenomena) with the advantages of visible-light lasers (highly coherent beams). All of these characteristics are

  12. X-ray enhancement and long-term evolution of swift J1822.31606

    SciTech Connect (OSTI)

    Benli, Onur; al??kan, ?.; Ertan, .; Alpar, M. A. [Sabanc? University, Orhanl?-Tuzla, ?stanbul 34956 (Turkey); Trmper, J. E. [Max-Planck-Institut fr extraterrestrische Physik, Geissenbachstrasse, 85740 Garching bei Mnchen (Germany); Kylafis, N. D., E-mail: onurbenli@sabanciuniv.edu [Physics Department and Institute of Theoretical and Computational Physics, University of Crete, 71003 Heraklion, Crete (Greece)

    2013-12-01

    We investigate the X-ray enhancement and the long-term evolution of the recently discovered second 'low-B magnetar' Swift J1822.3-1606 in the frame of the fallback disk model. During a soft gamma burst episode, the inner disk matter is pushed back to larger radii, forming a density gradient at the inner disk. Subsequent relaxation of the inner disk could account for the observed X-ray enhancement light curve of Swift J1822.3-1606. We obtain model fits to the X-ray data with basic disk parameters similar to those employed to explain the X-ray outburst light curves of other anomalous X-ray pulsars and soft gamma repeaters. The long period (8.4 s) of the neutron star can be reached by the effect of the disk torques in the long-term accretion phase ((1-3) 10{sup 5} yr). The currently ongoing X-ray enhancement could be due to a transient accretion epoch, or the source could still be in the accretion phase in quiescence. Considering these different possibilities, we determine the model curves that could represent the long-term rotational and the X-ray luminosity evolution of Swift J1822.3-1606, which constrain the strength of the magnetic dipole field to the range of (1-2) 10{sup 12} G on the surface of the neutron star.

  13. Photoionization-pumped, Ne II, x-ray laser studies project. Final report

    SciTech Connect (OSTI)

    Richardson, M.C.; Hagelstein, P.L.; Eckart, M.J.; Forsyth, J.M.; Gerrassimenko, M.; Soures, J.M.

    1984-01-01

    The energetics of this pumping scheme are shown. Short-pulse (50 to 100 ps) laser irradiation of an appropriate x-ray flashlamp medium generates broad-band emission in the range of 300 to 800 eV which preferentially photoionizes Ne to the /sup 2/S state of Ne II creating an inversion at approximately 27 eV. Although this approach does not depend on precise spectral overlap between the x-ray pump radiation and the medium to be pumped, it does require that the x-ray medium remain un-ionized prior to photoionization by the soft x-ray emission. Well-controlled focus conditions are required to ensure that the x-ray medium is not subjected to electron or x-ray preheat prior to irradiation by the soft x-ray source. The magnitude of the population inversion is predicted to be critically dependent upon rapid photoionization of the two states; therefore, ultra-short pulse irradiation of the laser flashlamps is required.

  14. Background-reducing X-ray multilayer mirror

    DOE Patents [OSTI]

    Bloch, Jeffrey J. (Los Alamos, NM); Roussel-Dupre', Diane (Los Alamos, NM); Smith, Barham W. (Los Alamos, NM)

    1992-01-01

    Background-reducing x-ray multilayer mirror. A multiple-layer "wavetrap" deposited over the surface of a layered, synthetic-microstructure soft x-ray mirror optimized for reflectivity at chosen wavelengths is disclosed for reducing the reflectivity of undesired, longer wavelength incident radiation incident thereon. In three separate mirror designs employing an alternating molybdenum and silicon layered, mirrored structure overlaid by two layers of a molybdenum/silicon pair anti-reflection coating, reflectivities of near normal incidence 133, 171, and 186 .ANG. wavelengths have been optimized, while that at 304 .ANG. has been minimized. The optimization process involves the choice of materials, the composition of the layer/pairs as well as the number thereof, and the distance therebetween for the mirror, and the simultaneous choice of materials, the composition of the layer/pairs, and their number and distance for the "wavetrap."

  15. A compact x-ray free electron laser

    SciTech Connect (OSTI)

    Barletta, W.A. . Center for Advanced Accelerators Physics Lawrence Livermore National Lab., CA ); Atac, M.; Cline, D.B.; Kolonko, J. . Center for Advanced Accelerators Physics); Bhowmik, A.; Bobbs, B.; Cover, R.A.; Dixon, F.P.; Rakowsky, G. . Rocketdyne Div.); Gallardo

    1988-01-01

    We present a design concept and simulation of the performance of a compact x-ray, free electron laser driven by ultra-high gradient rf-linacs. The accelerator design is based on recent advances in high gradient technology by a LLNL/SLAC/LBL collaboration and on the development of bright, high current electron sources by BNL and LANL. The GeV electron beams generated with such accelerators can be converted to soft x-rays in the range from 2--10 nm by passage through short period, high field strength wigglers as are being designed at Rocketdyne Linear light sources of this type can produce trains of picosecond (or shorter) pulses of extremely high spectral brilliance suitablee for flash holography of biological specimens in vivo and for studies of fast chemical reactions. 12 refs., 8 figs., 4 tabs.

  16. Phased Contrast X-Ray Imaging

    ScienceCinema (OSTI)

    Erin Miller

    2012-12-31

    The Pacific Northwest National Laboratory is developing a range of technologies to broaden the field of explosives detection. Phased contrast X-ray imaging, which uses silicon gratings to detect distortions in the X-ray wave front, may be applicable to mail or luggage scanning for explosives; it can also be used in detecting other contraband, small-parts inspection, or materials characterization.

  17. PROBING THE COSMIC X-RAY AND MeV GAMMA-RAY BACKGROUND RADIATION THROUGH THE

    Office of Scientific and Technical Information (OSTI)

    ANISOTROPY (Journal Article) | SciTech Connect PROBING THE COSMIC X-RAY AND MeV GAMMA-RAY BACKGROUND RADIATION THROUGH THE ANISOTROPY Citation Details In-Document Search Title: PROBING THE COSMIC X-RAY AND MeV GAMMA-RAY BACKGROUND RADIATION THROUGH THE ANISOTROPY While the cosmic soft X-ray background is very likely to originate from individual Seyfert galaxies, the origin of the cosmic hard X-ray and MeV gamma-ray background is not fully understood. It is expected that Seyferts including

  18. High-resolution Soft-RIXS: Scientific Goals and Technical Challenges |

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Stanford Synchrotron Radiation Lightsource High-resolution Soft-RIXS: Scientific Goals and Technical Challenges Tuesday, November 22, 2011 - 3:30pm SSRL Conference Room 137-322 Giacomo Ghiringhelli, CNR/SPIN and Dipartimento di Fisica, Politecnico di Milano, Italy Visiting scholar at SIMES-Department of physics, Stanford University The interest in resonant inelastic soft x-ray scattering has been recently boosted mainly by results on high Tc superconductors and other cuprates, where orbital

  19. Femtosecond x-rays link melting of charge density wave correlations and light-enhanced coherent transport in YBa?Cu?O?.?

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Forst, M.; Hill, J. P.; Frano, A.; Kaiser, S.; Mankowsky, R.; Hunt, C. R.; Turner, J. J.; Dakovski, G. L.; Minitti, M. P.; Robinson, J.; et al

    2014-11-17

    We use femtosecond resonant soft x-ray diffraction to measure the optically stimulated ultrafast changes of charge density wave correlations in underdoped YBa?Cu?O?.?. We find that when coherent interlayer transport is enhanced by optical excitation of the apical oxygen distortions, at least 50% of the in-plane charge density wave order is melted. These results indicate that charge ordering and superconductivity may be competing up to the charge ordering transition temperature, with the latter becoming a hidden phase that is accessible only by nonlinear phonon excitation.

  20. Femtosecond x rays link melting of charge-density wave correlations and light-enhanced coherent transport in YBa2Cu3O6.6

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Först, M.; Frano, A.; Kaiser, S.; Mankowsky, R.; Hunt, C. R.; Turner, J. J.; Dakovski, G. L.; Minitti, M. P.; Robinson, J.; Loew, T.; et al

    2014-11-17

    In this study, we use femtosecond resonant soft x-ray diffraction to measure the optically stimulated ultrafast changes of charge density wave correlations in underdoped YBa₂Cu₃O₆.₆. We find that when coherent interlayer transport is enhanced by optical excitation of the apical oxygen distortions, at least 50% of the in-plane charge density wave order is melted. These results indicate that charge ordering and superconductivity may be competing up to the charge ordering transition temperature, with the latter becoming a hidden phase that is accessible only by nonlinear phonon excitation.

  1. Reabsorption of Soft X-Ray Emission at High X-Ray Free-Electron...

    Office of Scientific and Technical Information (OSTI)

    Publication Date: 2014-10-06 OSTI Identifier: 1180829 Type: Publisher's Accepted Manuscript Journal Name: Physical Review Letters Additional Journal Information: Journal Volume: ...

  2. SIMULTANEOUS X-RAY AND ULTRAVIOLET OBSERVATIONS OF THE SW SEXTANTIS STAR DW URSAE MAJORIS

    SciTech Connect (OSTI)

    Hoard, D. W.; Wachter, S. [Spitzer Science Center, California Institute of Technology, MS 220-6, 1200 E. California Blvd., Pasadena, CA 91125 (United States); Lu, Ting-Ni [Institute of Astronomy, National Tsing Hua University, Hsinchu 30013, Taiwan (China); Knigge, Christian [School of Physics and Astronomy, University of Southampton, Highfield, Southampton SO17 1BJ (United Kingdom); Homer, Lee; Szkody, Paula [Department of Astronomy, University of Washington, Box 351580, Seattle, WA 98195-1580 (United States); Still, M. [NASA Ames Research Center, Moffett Field, CA 94035 (United States); Long, Knox S. [Space Telescope Science Institute, 3700 San Martin Drive, Baltimore, MD 21218 (United States); Dhillon, V. S., E-mail: hoard@ipac.caltech.ed [Department of Physics and Astronomy, University of Sheffield, Sheffield S3 7RH (United Kingdom)

    2010-11-15

    We present the first pointed X-ray observation of DW Ursae Majoris, a novalike cataclysmic variable (CV) and one of the archetype members of the SW Sextantis class, obtained with the XMM-Newton satellite. These data provide the first detailed look at an SW Sex star in the X-ray regime (with previous X-ray knowledge of the SW Sex stars limited primarily to weak or non-detections in the ROSAT All Sky Survey). It is also one of only a few XMM-Newton observations (to date) of any high mass transfer rate novalike CV, and the only one in the evolutionarily important 3-4 hr orbital period range. The observed X-ray spectrum of DW UMa is very soft, with {approx}95% of the detected X-ray photons at energies <2 keV. The spectrum can be fit equally well by a one-component cooling flow model, with a temperature range of 0.2-3.5 keV, or a two-component, two-temperature thermal plasma model, containing hard ({approx}5-6 keV) and soft ({approx}0.8 keV) components. The X-ray light curve of DW UMa shows a likely partial eclipse, implying X-ray reprocessing in a vertically extended region, and an orbital modulation, implying a structural asymmetry in the X-ray reprocessing site (e.g., it cannot be a uniform corona). We also obtained a simultaneous near-ultraviolet light curve of DW UMa using the Optical Monitor on XMM-Newton. This light curve is similar in appearance to published optical-UV light curves of DW UMa and shows a prominent deep eclipse. Regardless of the exact nature of the X-ray reprocessing site in DW UMa, the lack of a prominent hard X-ray total eclipse and very low fraction of high energy X-rays point to the presence of an optically and geometrically thick accretion disk that obscures the boundary layer and modifies the X-ray spectrum emitted near the white dwarf.

  3. Laser plasma x-ray source for ultrafast time-resolved x-ray absorption spectroscopy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Miaja-Avila, L.; O'Neil, G. C.; Uhlig, J.; Cromer, C. L.; Dowell, M. L.; Jimenez, R.; Hoover, A. S.; Silverman, K. L.; Ullom, J. N.

    2015-03-02

    We describe a laser-driven x-ray plasma source designed for ultrafast x-ray absorption spectroscopy. The source is comprised of a 1 kHz, 20 W, femtosecond pulsed infrared laser and a water target. We present the x-ray spectra as a function of laser energy and pulse duration. Additionally, we investigate the plasma temperature and photon flux as we vary the laser energy. We obtain a 75 μm FWHM x-ray spot size, containing ~106 photons/s, by focusing the produced x-rays with a polycapillary optic. Since the acquisition of x-ray absorption spectra requires the averaging of measurements from >107 laser pulses, we also presentmore » data on the source stability, including single pulse measurements of the x-ray yield and the x-ray spectral shape. In single pulse measurements, the x-ray flux has a measured standard deviation of 8%, where the laser pointing is the main cause of variability. Further, we show that the variability in x-ray spectral shape from single pulses is low, thus justifying the combining of x-rays obtained from different laser pulses into a single spectrum. Finally, we show a static x-ray absorption spectrum of a ferrioxalate solution as detected by a microcalorimeter array. Altogether, our results demonstrate that this water-jet based plasma source is a suitable candidate for laboratory-based time-resolved x-ray absorption spectroscopy experiments.« less

  4. Femtosecond all-optical synchronization of an X-ray free-electron laser

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Schulz, S.; Grguraš, I.; Behrens, C.; Bromberger, H.; Costello, J. T.; Czwalinna, M. K.; Felber, M.; Hoffmann, M. C.; Ilchen, M.; Liu, H. Y.; et al

    2015-01-20

    Many advanced applications of X-ray free-electron lasers require pulse durations and time resolutions of only a few femtoseconds. To generate these pulses and to apply them in time-resolved experiments, synchronization techniques that can simultaneously lock all independent components, including all accelerator modules and all external optical lasers, to better than the delivered free-electron laser pulse duration, are needed. Here we achieve all-optical synchronization at the soft X-ray free-electron laser FLASH and demonstrate facility-wide timing to better than 30 fs r.m.s. for 90 fs X-ray photon pulses. Crucially, our analysis indicates that the performance of this optical synchronization is limited primarilymore » by the free-electron laser pulse duration, and should naturally scale to the sub-10 femtosecond level with shorter X-ray pulses.« less

  5. Femtosecond all-optical synchronization of an X-ray free-electron laser

    SciTech Connect (OSTI)

    Schulz, S.; Grguraš, I.; Behrens, C.; Bromberger, H.; Costello, J. T.; Czwalinna, M. K.; Felber, M.; Hoffmann, M. C.; Ilchen, M.; Liu, H. Y.; Mazza, T.; Meyer, M.; Pfeiffer, S.; Prędki, P.; Schefer, S.; Schmidt, C.; Wegner, U.; Schlarb, H.; Cavalieri, A. L.

    2015-01-20

    Many advanced applications of X-ray free-electron lasers require pulse durations and time resolutions of only a few femtoseconds. To generate these pulses and to apply them in time-resolved experiments, synchronization techniques that can simultaneously lock all independent components, including all accelerator modules and all external optical lasers, to better than the delivered free-electron laser pulse duration, are needed. Here we achieve all-optical synchronization at the soft X-ray free-electron laser FLASH and demonstrate facility-wide timing to better than 30 fs r.m.s. for 90 fs X-ray photon pulses. Crucially, our analysis indicates that the performance of this optical synchronization is limited primarily by the free-electron laser pulse duration, and should naturally scale to the sub-10 femtosecond level with shorter X-ray pulses.

  6. X-ray source for mammography

    DOE Patents [OSTI]

    Logan, C.M.

    1994-12-20

    An x-ray source is described utilizing anode material which shifts the output spectrum to higher energy and thereby obtains higher penetrating ability for screening mammography application, than the currently utilized anode material. The currently used anode material (molybdenum) produces an energy x-ray spectrum of 17.5/19.6 keV, which using the anode material of this invention (e.g. silver, rhodium, and tungsten) the x-ray spectrum would be in the 20-35 keV region. Thus, the anode material of this invention provides for imaging of breasts with higher than average x-ray opacity without increase of the radiation dose, and thus reduces the risk of induced breast cancer due to the radiation dose administered for mammograms. 6 figures.

  7. X-Ray Nanoimaging: Instruments and Methods

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-Ray Nanoimaging: Instruments and Methods To be held as part of SPIE. http://spie.org/OP318 August 28-29, 2013; San Diego, California, USA

  8. Small Angle X-Ray Scattering Detector

    DOE Patents [OSTI]

    Hessler, Jan P.

    2004-06-15

    A detector for time-resolved small-angle x-ray scattering includes a nearly constant diameter, evacuated linear tube having an end plate detector with a first fluorescent screen and concentric rings of first fiber optic bundles for low angle scattering detection and an annular detector having a second fluorescent screen and second fiber optic bundles concentrically disposed about the tube for higher angle scattering detection. With the scattering source, i.e., the specimen under investigation, located outside of the evacuated tube on the tube's longitudinal axis, scattered x-rays are detected by the fiber optic bundles, to each of which is coupled a respective photodetector, to provide a measurement resolution, i.e., dq/q, where q is the momentum transferred from an incident x-ray to an x-ray scattering specimen, of 2% over two (2) orders of magnitude in reciprocal space, i.e., qmax/qmin approx=lO0.

  9. X-Ray Nanoimaging: Instruments and Methods

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-Ray Nanoimaging: Instruments and Methods To be held as part of SPIE. http:spie.orgOP318 August 28-29, 2013; San Diego, California, USA...

  10. X-ray source for mammography

    DOE Patents [OSTI]

    Logan, Clinton M.

    1994-01-01

    An x-ray source utilizing anode material which shifts the output spectrum to higher energy and thereby obtains higher penetrating ability for screening mammography application, than the currently utilized anode material. The currently used anode material (molybdenum) produces an energy x-ray spectrum of 17.5/19.6 keV, which using the anode material of this invention (e.g. silver, rhodium, and tungsten) the x-ray spectrum would be in the 20-35 keV region. Thus, the anode material of this invention provides for imaging of breasts with higher than average x-ray opacity without increase of the radiation dose, and thus reduces the risk of induced breast cancer due to the radiation dose administered for mammograms.

  11. X-ray grid-detector apparatus

    DOE Patents [OSTI]

    Boone, John M. (Folsom, CA); Lane, Stephen M. (Oakland, CA)

    1998-01-27

    A hybrid grid-detector apparatus for x-ray systems wherein a microchannel plate structure has an air-interspaced grid portion and a phosphor/optical fluid-filled grid portion. The grids are defined by multiple adjacent channels separated by lead-glass septa. X-rays entering the air-interspaced grid portion at an angle of impingement upon the septa are attenuated, while non-impinging x-rays pass through to the phosphor/fluid filled portion. X-ray energy is converted to luminescent energy in the phosphor/fluid filled portion and the resultant beams of light are directed out of the phosphor/optical fluid filled portion to an imaging device.

  12. Femtosecond X-ray protein nanocrystallography

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Femtosecond X-ray protein nanocrystallography Authors: Chapman, H.N., Fromme, P., Barty, A., White, T.A., Kirian, R.A., Aquila, A., Hunter, M.S., Schulz, J., DePonte, D.P.,...

  13. Subject: Ames Blue Alert - X-ray Shutter Maintenance

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ames Blue Alert - X-ray Shutter Maintenance Statement: This lesson learned involves an Ames Laboratory x-ray system. Prior to starting x- ray experiments checking the operability...

  14. Femtosecond Time-Delay X-ray Holography

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Time-Delay X-ray Holography X-ray free-electron lasers (XFELs) will produce photon pulses with a unique and desirable combination of properties. Their short X-ray wavelengths allow...

  15. X-ray Tube with Magnetic Electron Steering - Energy Innovation...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Increases the proportion of electrons emitted from the cathode that contribute to X-ray production in a compact geometry Provides increased X-ray generation efficiency by...

  16. X-Ray Microcomputed Tomography for the Durability Characterization...

    Office of Scientific and Technical Information (OSTI)

    Conference: X-Ray Microcomputed Tomography for the Durability Characterization of Limestone Aggregate Citation Details In-Document Search Title: X-Ray Microcomputed Tomography for...

  17. X-ray transient absorption and picosecond IR spectroscopy of...

    Office of Scientific and Technical Information (OSTI)

    X-ray transient absorption and picosecond IR spectroscopy of fulvalene(tetracarbonyl)diruthenium on photoexcitation Citation Details In-Document Search Title: X-ray transient ...

  18. Generation of Coherent X-Ray Radiation through Modulation Compression...

    Office of Scientific and Technical Information (OSTI)

    Journal Article: Generation of Coherent X-Ray Radiation through Modulation Compression Citation Details In-Document Search Title: Generation of Coherent X-Ray Radiation through...

  19. Category:X-Ray Diffraction (XRD) | Open Energy Information

    Open Energy Info (EERE)

    X-Ray Diffraction (XRD) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Geothermalpower.jpg Looking for the X-Ray Diffraction (XRD) page? For detailed information on...

  20. Exotic X-ray back-diffraction: a path toward a softinelastic X-ray

    Office of Scientific and Technical Information (OSTI)

    scattering spectrometer (Journal Article) | SciTech Connect Exotic X-ray back-diffraction: a path toward a softinelastic X-ray scattering spectrometer Citation Details In-Document Search Title: Exotic X-ray back-diffraction: a path toward a softinelastic X-ray scattering spectrometer Authors: Hoennicke M. ; Zhou J. ; Conley,R. ; Cusatis,C. ; Kakuno,E.M. ; Bouet,N. ; Marques,J.B. ; Vicentin,F.C. Publication Date: 2014-09-20 OSTI Identifier: 1165974 Report Number(s): BNL--107230-2014-JA

  1. Transient x-ray diffraction and its application to materials science and x-ray optics

    SciTech Connect (OSTI)

    Hauer, A.A.; Kopp, R.; Cobble, J.; Kyrala, G.; Springer, R.

    1997-12-01

    Time resolved x-ray diffraction and scattering have been applied to the measurement of a wide variety of physical phenomena from chemical reactions to shock wave physics. Interest in this method has heightened in recent years with the advent of versatile, high power, pulsed x-ray sources utilizing laser plasmas, electron beams and other methods. In this article, we will describe some of the fundamentals involved in time resolved x-ray diffraction, review some of the history of its development, and describe some recent progress in the field. In this article we will emphasize the use of laser-plasmas as the x-ray source for transient diffraction.

  2. Signal-to-noise and radiation exposure considerations in conventional and diffraction x-ray microscopy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Huang, Xiaojing; Miao, Huijie; Steinbrener, Jan; Nelson, Johanna; Shapiro, David; Stewart, Andrew; Turner, Joshua; Jacobsen, Chris

    2009-01-01

    Using a signal-to-noise ratio estimation based on correlations between multiple simulated images, we compare the dose efficiency of two soft x-ray imaging systems: incoherent brightfield imaging using zone plate optics in a transmission x-ray microscope (TXM), and x-ray diffraction microscopy (XDM) where an image is reconstructed from the far-field coherent diffraction pattern. In XDM one must computationally phase weak diffraction signals; in TXM one suffers signal losses due to the finite numerical aperture and efficiency of the optics. In simulations with objects representing isolated cells such as yeast, we find that XDM has the potential for delivering equivalent resolution imagesmore » using fewer photons. As a result, this can be an important advantage for studying radiation-sensitive biological and soft matter specimens.« less

  3. Dimensionality and noise in energy selective x-ray imaging

    SciTech Connect (OSTI)

    Alvarez, Robert E.

    2013-11-15

    Purpose: To develop and test a method to quantify the effect of dimensionality on the noise in energy selective x-ray imaging.Methods: The Cramr-Rao lower bound (CRLB), a universal lower limit of the covariance of any unbiased estimator, is used to quantify the noise. It is shown that increasing dimensionality always increases, or at best leaves the same, the variance. An analytic formula for the increase in variance in an energy selective x-ray system is derived. The formula is used to gain insight into the dependence of the increase in variance on the properties of the additional basis functions, the measurement noise covariance, and the source spectrum. The formula is also used with computer simulations to quantify the dependence of the additional variance on these factors. Simulated images of an object with three materials are used to demonstrate the trade-off of increased information with dimensionality and noise. The images are computed from energy selective data with a maximum likelihood estimator.Results: The increase in variance depends most importantly on the dimension and on the properties of the additional basis functions. With the attenuation coefficients of cortical bone, soft tissue, and adipose tissue as the basis functions, the increase in variance of the bone component from two to three dimensions is 1.4 10{sup 3}. With the soft tissue component, it is 2.7 10{sup 4}. If the attenuation coefficient of a high atomic number contrast agent is used as the third basis function, there is only a slight increase in the variance from two to three basis functions, 1.03 and 7.4 for the bone and soft tissue components, respectively. The changes in spectrum shape with beam hardening also have a substantial effect. They increase the variance by a factor of approximately 200 for the bone component and 220 for the soft tissue component as the soft tissue object thickness increases from 1 to 30 cm. Decreasing the energy resolution of the detectors increases the variance of the bone component markedly with three dimension processing, approximately a factor of 25 as the resolution decreases from 100 to 3 bins. The increase with two dimension processing for adipose tissue is a factor of two and with the contrast agent as the third material for two or three dimensions is also a factor of two for both components. The simulated images show that a maximum likelihood estimator can be used to process energy selective x-ray data to produce images with noise close to the CRLB.Conclusions: The method presented can be used to compute the effects of the object attenuation coefficients and the x-ray system properties on the relationship of dimensionality and noise in energy selective x-ray imaging systems.

  4. X-ray lithography using holographic images

    DOE Patents [OSTI]

    Howells, Malcolm S. (Berkeley, CA); Jacobsen, Chris (Sound Beach, NY)

    1997-01-01

    Methods for forming X-ray images having 0.25 .mu.m minimum line widths on X-ray sensitive material are presented. A holgraphic image of a desired circuit pattern is projected onto a wafer or other image-receiving substrate to allow recording of the desired image in photoresist material. In one embodiment, the method uses on-axis transmission and provides a high flux X-ray source having modest monochromaticity and coherence requirements. A layer of light-sensitive photoresist material on a wafer with a selected surface is provided to receive the image(s). The hologram has variable optical thickness and variable associated optical phase angle and amplitude attenuation for transmission of the X-rays. A second embodiment uses off-axis holography. The wafer receives the holographic image by grazing incidence reflection from a hologram printed on a flat metal or other highly reflecting surface or substrate. In this second embodiment, an X-ray beam with a high degree of monochromaticity and spatial coherence is required.

  5. X-ray lithography using holographic images

    DOE Patents [OSTI]

    Howells, M.S.; Jacobsen, C.

    1997-03-18

    Methods for forming X-ray images having 0.25 {micro}m minimum line widths on X-ray sensitive material are presented. A holographic image of a desired circuit pattern is projected onto a wafer or other image-receiving substrate to allow recording of the desired image in photoresist material. In one embodiment, the method uses on-axis transmission and provides a high flux X-ray source having modest monochromaticity and coherence requirements. A layer of light-sensitive photoresist material on a wafer with a selected surface is provided to receive the image(s). The hologram has variable optical thickness and variable associated optical phase angle and amplitude attenuation for transmission of the X-rays. A second embodiment uses off-axis holography. The wafer receives the holographic image by grazing incidence reflection from a hologram printed on a flat metal or other highly reflecting surface or substrate. In this second embodiment, an X-ray beam with a high degree of monochromaticity and spatial coherence is required. 15 figs.

  6. Ultrafast X-Ray Coherent Control

    SciTech Connect (OSTI)

    Reis, David

    2009-05-01

    This main purpose of this grant was to develop the nascent #12;eld of ultrafast x-ray science using accelerator-based sources, and originally developed from an idea that a laser could modulate the di#11;racting properties of a x-ray di#11;racting crystal on a fast enough time scale to switch out in time a shorter slice from the already short x-ray pulses from a synchrotron. The research was carried out primarily at the Advanced Photon Source (APS) sector 7 at Argonne National Laboratory and the Sub-Picosecond Pulse Source (SPPS) at SLAC; in anticipation of the Linac Coherent Light Source (LCLS) x-ray free electron laser that became operational in 2009 at SLAC (all National User Facilities operated by BES). The research centered on the generation, control and measurement of atomic-scale dynamics in atomic, molecular optical and condensed matter systems with temporal and spatial resolution . It helped develop the ultrafast physics, techniques and scienti#12;c case for using the unprecedented characteristics of the LCLS. The project has been very successful with results have been disseminated widely and in top journals, have been well cited in the #12;eld, and have laid the foundation for many experiments being performed on the LCLS, the world's #12;rst hard x-ray free electron laser.

  7. X-Ray Data from the X-Ray Data Booklet Online

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Thompson, Albert C.; Attwood, David T.; Gullikson, Eric M.; Howells, Malcolm R.; Kortright, Jeffrey B.; Robinson, Arthur L.; Underwood, James H.; Kim, Kwang-Je; Kirz, Janos; Lindau, Ingolf; Pianetta, Piero; Winick, Herman; Williams, Gwyn P.; Scofield, James H.

    The original X-Ray Data Booklet, published in 1985, became a classic reference source. The online version has been significantly revised and updated to reflect today's science. Hundreds of pages of authoritative data provide the x-ray properties of elements, information on synchrotron radiation, scattering processes, optics and detectors, and other related calculations, formulas, and data tables.

  8. PROPX: An X-ray Manipulation Program

    SciTech Connect (OSTI)

    Kyrala, G.A.

    1992-05-01

    An interactive micro-computer program that performs some manipulations on an input x-ray spectrum is introduced and described. The program is used to calculate the effect of absorption of filters, transmission through fibers, responsivity of photocathodes, responsivity of absorptive detectors, folding of responses, plotting of cross sections, and calculation, as a function of electron temperature, of the response due to a bremsstrahlung spectrum. Fluorescence from the targets is not included. Two different x-ray libraries are offered, one covers the x-ray range 30--10,000 eV with 288 energy points, and the other covers the energy range 10 eV to 1 MeV with 250 energy points per decade. 7 refs.

  9. Spatially resolved high-resolution x-ray spectroscopy of high-current plasma-focus discharges

    SciTech Connect (OSTI)

    ZajaPc, S.; Rzadkiewicz, J.; Scholz, M.; Paduch, M.; Zielinska, E.; Rosmej, O.; Yongtao, Zhao; Gojska, A.

    2010-10-15

    Soft x-ray emission from a Mather-type plasma-focus device (PF-1000) operated at {approx}400 kJ was measured. The high density and temperature plasma were generated by the discharge in the deuterium-argon gas mixture in the modified (high-current) plasma-focus configuration. A spherically bent mica crystal spectrograph viewing the axial output of the pinch region was used to measure the x-ray spectra. Spatially resolved spectra including the characteristic x-ray lines of highly ionized Ar and continua were recorded by means of an x-ray film. The x-ray emission of PF-1000 device was studied at different areas of the pinch.

  10. Image plates as x-ray detectors in plasma physics experiments

    SciTech Connect (OSTI)

    Gales, S.G.; Bentley, C.D.

    2004-10-01

    The performance of image plates based on the photostimulable phosphor BaF(Br,l):Eu{sup 2+} has been investigated and compared with x-ray film. Evaluation of detective quantum efficiency (DQE), sensitivity, dynamic range, and linearity was carried out for several types of commercially available image plate, using the Excalibur soft x-ray calibration facility at AWE. Image plate response was found to be linear over a dynamic range of 5 orders of magnitude. One type of image plate was found to have a number of advantages for soft x-ray detection, with a measured sensitivity 1 order of magnitude greater than that of Kodak Industrex CX and DEF-5 x-ray film. The DQE of this plate was found to be superior to that of film at low [less than 10{sup 3} photons/(50 {mu}m){sup 2}] and high fluxes [greater than 10{sup 4} photons/(50 {mu}m){sup 2}]. The spatial resolution of image plates, scanned with several models of commercial image plate readers, has been evaluated using a USAF resolution test target. The highest spatial resolution measured is 35 {mu}m. Though this is significantly lower than the resolution possible with film, it is sufficient for many applications. Image plates were fielded in a refractive x-ray lens imaging diagnostic on the 1 TW Helen laser and these results are discussed.

  11. Differential phase contrast X-ray imaging system and components

    DOE Patents [OSTI]

    Stutman, Daniel; Finkenthal, Michael

    2014-07-01

    A differential phase contrast X-ray imaging system includes an X-ray illumination system, a beam splitter arranged in an optical path of the X-ray illumination system, and a detection system arranged in an optical path to detect X-rays after passing through the beam splitter.

  12. Radiobiological studies using gamma and x rays.

    SciTech Connect (OSTI)

    Potter, Charles Augustus; Longley, Susan W.; Scott, Bobby R. [Lovelace Respiratory Research Institute, Albuquerque, NM; Lin, Yong [Lovelace Respiratory Research Institute, Albuquerque, NM; Wilder, Julie [Lovelace Respiratory Research Institute, Albuquerque, NM; Hutt, Julie A. [Lovelace Respiratory Research Institute, Albuquerque, NM; Padilla, Mabel T. [Lovelace Respiratory Research Institute, Albuquerque, NM; Gott, Katherine M. [Lovelace Respiratory Research Institute, Albuquerque, NM

    2013-02-01

    There are approximately 500 self-shielded research irradiators used in various facilities throughout the U.S. These facilities use radioactive sources containing either 137Cs or 60Co for a variety of biological investigations. A report from the National Academy of Sciences[1] described the issues with security of particular radiation sources and the desire for their replacement. The participants in this effort prepared two peer-reviewed publications to document the results of radiobiological studies performed using photons from 320-kV x rays and 137Cs on cell cultures and mice. The effectiveness of X rays was shown to vary with cell type.

  13. Biological Imaging by Soft X-Ray Diffraction Microscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    reconstructions were obtained from eight angular orientations of the cell at 1 rotation intervals. The good agreement between the independently recovered structures provides...

  14. Biological Imaging by Soft X-Ray Diffraction Microscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    after passage through the cell. The phase information is represented as hue (see color map at left) and the magnitude as brightness. The labels indicate the nucleus (N),...

  15. Biological Imaging by Soft X-Ray Diffraction Microscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    objects opaque to visible light, and tomographic techniques related to those used in CAT scans give access to three-dimensional images. The rub is that lenses that can focus x...

  16. Electronic structure of titania aerogels: Soft x-ray absorption...

    Office of Scientific and Technical Information (OSTI)

    study Authors: Kucheyev, S O ; van Buuren, T ; Baumann, T F ; Satcher, Jr, J H ; Willey, T M ; Meulenberg, R W ; Felter, T E ; Poco, J F ; Gammon, S A ; Terminello, L J...

  17. Studies of magnetic microstructures with soft x-ray transmissionmicros...

    Office of Scientific and Technical Information (OSTI)

    Date: 2006-01-01 OSTI Identifier: 922805 Report Number(s): LBNL--60390 Journal ID: ISSN 0018-9197; IEJQA7; R&D Project: 509201; BnR: KC0202030; TRN: US200803%%455 DOE Contract...

  18. X-ray focal spot locating apparatus and method

    DOE Patents [OSTI]

    Gilbert, Hubert W. (Cedar Crest, NM)

    1985-07-30

    An X-ray beam finder for locating a focal spot of an X-ray tube includes a mass of X-ray opaque material having first and second axially-aligned, parallel-opposed faces connected by a plurality of substantially identical parallel holes perpendicular to the faces and a film holder for holding X-ray sensitive film tightly against one face while the other face is placed in contact with the window of an X-ray head.

  19. Small Angle X-Ray Scattering Detector

    DOE Patents [OSTI]

    Hessler, Jan P.

    2004-06-15

    A detector for time-resolved small-angle x-ray scattering includes a nearly constant diameter, evacuated linear tube having an end plate detector with a first fluorescent screen and concentric rings of first fiber optic bundles for low angle scattering detection and an annular detector having a second fluorescent screen and second fiber optic bundles concentrically disposed about the tube for higher angle scattering detection. With the scattering source, i.e., the specimen under investigation, located outside of the evacuated tube on the tube's longitudinal axis, scattered x-rays are detected by the fiber optic bundles, to each of which is coupled a respective photodetector, to provide a measurement resolution, i.e., dq/q, where q is the momentum transferred from an incident x-ray to an x-ray scattering specimen, of 2% over two (2) orders of magnitude in reciprocal space, i.e., q.sub.max /q.sub.min.congruent.100.

  20. Multiple wavelength X-ray monochromators

    DOE Patents [OSTI]

    Steinmeyer, P.A.

    1992-11-17

    An improved apparatus and method is provided for separating input x-ray radiation containing first and second x-ray wavelengths into spatially separate first and second output radiation which contain the first and second x-ray wavelengths, respectively. The apparatus includes a crystalline diffractor which includes a first set of parallel crystal planes, where each of the planes is spaced a predetermined first distance from one another. The crystalline diffractor also includes a second set of parallel crystal planes inclined at an angle with respect to the first set of crystal planes where each of the planes of the second set of parallel crystal planes is spaced a predetermined second distance from one another. In one embodiment, the crystalline diffractor is comprised of a single crystal. In a second embodiment, the crystalline diffractor is comprised of a stack of two crystals. In a third embodiment, the crystalline diffractor includes a single crystal that is bent for focusing the separate first and second output x-ray radiation wavelengths into separate focal points. 3 figs.

  1. Multiple wavelength X-ray monochromators

    DOE Patents [OSTI]

    Steinmeyer, Peter A. (Arvada, CO)

    1992-11-17

    An improved apparatus and method is provided for separating input x-ray radiation containing first and second x-ray wavelengths into spatially separate first and second output radiation which contain the first and second x-ray wavelengths, respectively. The apparatus includes a crystalline diffractor which includes a first set of parallel crystal planes, where each of the planes is spaced a predetermined first distance from one another. The crystalline diffractor also includes a second set of parallel crystal planes inclined at an angle with respect to the first set of crystal planes where each of the planes of the second set of parallel crystal planes is spaced a predetermined second distance from one another. In one embodiment, the crystalline diffractor is comprised of a single crystal. In a second embodiment, the crystalline diffractor is comprised of a stack of two crystals. In a third embodiment, the crystalline diffractor includes a single crystal that is bent for focussing the separate first and second output x-ray radiation wavelengths into separate focal points.

  2. SLAC All Access: X-ray Microscope

    ScienceCinema (OSTI)

    Nelson, Johanna; Liu, Yijin

    2014-06-13

    SLAC physicists Johanna Nelson and Yijin Liu give a brief overview of the X-ray microscope at the Stanford Synchrotron Radiation Lightsource (SSRL) that is helping improve rechargeable-battery technology by letting researchers peek into the inner workings of batteries as they operate.

  3. Bandpass x-ray diode and x-ray multiplier detector

    DOE Patents [OSTI]

    Wang, C.L.

    1982-09-27

    An absorption-edge of an x-ray absorption filter and a quantum jump of a photocathode determine the bandpass characteristics of an x-ray diode detector. An anode, which collects the photoelectrons emitted by the photocathode, has enhanced amplification provided by photoelectron-multiplying means which include dynodes or a microchannel-plate electron-multiplier. Suppression of undesired high frequency response for a bandpass x-ray diode is provided by subtracting a signal representative of energies above the passband from a signal representative of the overall response of the bandpass diode.

  4. X-ray imaging crystal spectrometer for extended X-ray sources

    DOE Patents [OSTI]

    Bitter, Manfred L. (Princeton, NJ); Fraenkel, Ben (Jerusalem, IL); Gorman, James L. (Bordentown, NJ); Hill, Kenneth W. (Lawrenceville, NJ); Roquemore, A. Lane (Cranbury, NJ); Stodiek, Wolfgang (Princeton, NJ); von Goeler, Schweickhard E. (Princeton, NJ)

    2001-01-01

    Spherically or toroidally curved, double focusing crystals are used in a spectrometer for X-ray diagnostics of an extended X-ray source such as a hot plasma produced in a tokomak fusion experiment to provide spatially and temporally resolved data on plasma parameters using the imaging properties for Bragg angles near 45. For a Bragg angle of 45.degree., the spherical crystal focuses a bundle of near parallel X-rays (the cross section of which is determined by the cross section of the crystal) from the plasma to a point on a detector, with parallel rays inclined to the main plain of diffraction focused to different points on the detector. Thus, it is possible to radially image the plasma X-ray emission in different wavelengths simultaneously with a single crystal.

  5. Rise time measurement for ultrafast X-ray pulses

    DOE Patents [OSTI]

    Celliers, Peter M. (Berkeley, CA); Weber, Franz A. (Oakland, CA); Moon, Stephen J. (Tracy, CA)

    2005-04-05

    A pump-probe scheme measures the rise time of ultrafast x-ray pulses. Conventional high speed x-ray diagnostics (x-ray streak cameras, PIN diodes, diamond PCD devices) do not provide sufficient time resolution to resolve rise times of x-ray pulses on the order of 50 fs or less as they are being produced by modern fast x-ray sources. Here, we are describing a pump-probe technique that can be employed to measure events where detector resolution is insufficient to resolve the event. The scheme utilizes a diamond plate as an x-ray transducer and a p-polarized probe beam.

  6. Rise Time Measurement for Ultrafast X-Ray Pulses

    DOE Patents [OSTI]

    Celliers, Peter M.; Weber, Franz A.; Moon, Stephen J.

    2005-04-05

    A pump-probe scheme measures the rise time of ultrafast x-ray pulses. Conventional high speed x-ray diagnostics (x-ray streak cameras, PIN diodes, diamond PCD devices) do not provide sufficient time resolution to resolve rise times of x-ray pulses on the order of 50 fs or less as they are being produced by modern fast x-ray sources. Here, we are describing a pump-probe technique that can be employed to measure events where detector resolution is insufficient to resolve the event. The scheme utilizes a diamond plate as an x-ray transducer and a p-polarized probe beam.

  7. X-ray radiography for container inspection

    DOE Patents [OSTI]

    Katz, Jonathan I.; Morris, Christopher L.

    2011-06-07

    Arrangements of X-ray inspection systems are described for inspecting high-z materials in voluminous objects such as containers. Inspection methods may involve generating a radiographic image based on detected attenuation corresponding to a pulsed beams of radiation transmitted through a voluminous object. The pulsed beams of radiation are generated by a high-energy source and transmitted substantially downward along an incident angle, of approximately 1.degree. to 30.degree., to a vertical axis extending through the voluminous object. The generated radiographic image may be analyzed to detect on localized high attenuation representative of high-z materials and to discriminate high-z materials from lower and intermediate-z materials on the basis of the high density and greater attenuation of high-z material for higher energy (3-10 MeV) X-rays, and the compact nature of threatening masses of fissionable materials.

  8. Observation and modeling of geocoronal charge exchange X-ray emission during solar wind gusts

    SciTech Connect (OSTI)

    Wargelin, B. J.; Kornbleuth, M.; Juda, M.; Martin, P. L.

    2014-11-20

    Solar wind charge exchange (SWCX) X-rays are emitted when highly charged solar wind ions such as O{sup 7{sup +}} collide with neutral gas, including the Earth's tenuous outer atmosphere (exosphere or geocorona) and hydrogen and helium from the local interstellar medium drifting through the heliosphere. This geocoronal and heliospheric emission comprises a significant and varying fraction of the soft X-ray background (SXRB) and is seen in every X-ray observation, with the intensity dependent on solar wind conditions and observation geometry. Under the right conditions, geocoronal emission can increase the apparent SXRB by roughly an order of magnitude for an hour or more. In this work, we study a dozen occasions when the near-Earth solar wind flux was exceptionally high. These gusts of wind lead to abrupt changes in SWCX X-ray emission around Earth, which may or may not be seen by X-ray observatories depending on their line of sight. Using detailed three-dimensional magnetohydrodynamical simulations of the solar wind's interaction with the Earth's magnetosphere, and element abundances and ionization states measured by ACE, we model the time-dependent brightness of major geocoronal SWCX emission lines during those gusts and compare with changes in the X-ray background measured by the Chandra X-ray Observatory. We find reasonably good agreement between model and observation, with measured geocoronal line brightnesses averaged over 1 hr of up to 136 photons s{sup 1} cm{sup 2} sr{sup 1} in the O VII K? triplet around 564 eV.

  9. Probing nanoscale behavior of magnetic materials with soft x...

    Office of Scientific and Technical Information (OSTI)

    Probing nanoscale behavior of magnetic materials with soft x-ray spectromicroscopy Citation Details In-Document Search Title: Probing nanoscale behavior of magnetic materials with...

  10. Periodicities in the X-ray emission from the solar corona

    SciTech Connect (OSTI)

    Chowdhury, Partha; Jain, Rajmal; Awasthi, Arun K. E-mail: parthares@gmail.com E-mail: awasthi@prl.res.in

    2013-11-20

    We have studied the time series of full disk integrated soft and hard X-ray emission from the solar corona during 2004 January to 2008 December, covering the entire descending phase of solar cycle 23 from a global point of view. We employ the daily X-ray index derived from 1 s cadence X-ray observations from the Si and CZT detectors of the 'Solar X-ray Spectrometer' mission in seven different energy bands ranging between 6 and 56 keV. X-ray data in the energy bands 6-7, 7-10, 10-20, and 4-25 keV from the Si detector are considered, while 10-20, 20-30, and 30-56 keV high energy observations are taken from the CZT detector. The daily time series is subjected to power spectrum analysis after appropriate correction for noise. The Lomb-Scargle periodogram technique has shown prominent periods of ?13.5 days, ?27 days, and a near-Rieger period of ?181 days and ?1.24 yr in all energy bands. In addition to this, other periods like ?31, ?48, ?57, ?76, ?96, ?130, ?227, and ?303 days are also detected in different energy bands. We discuss our results in light of previous observations and existing numerical models.

  11. Characteristics of a molybdenum X-pinch X-ray source as a probe source for X-ray diffraction studies

    SciTech Connect (OSTI)

    Zucchini, F.; Chauvin, C.; Combes, P.; Sol, D.; Loyen, A.; Roques, B.; Grunenwald, J.; Bland, S. N.

    2015-03-15

    X-ray emission from a molybdenum X-pinch has been investigated as a potential probe for the high pressure states made in dynamic compression experiments. Studies were performed on a novel 300 kA, 400 ns generator which coupled the load directly to a low inductance capacitor and switch combination. The X-pinch load consisted of 4 crossed molybdenum wires of 13 μm diameter, crossed at an angle of 62°. The load height was 10 mm. An initial x-ray burst generated at the wire crossing point, radiated in the soft x-ray range (hυ < 10 keV). This was followed, 2–5 ns later, by at least one harder x-ray burst (hυ > 10 keV) whose power ranged from 1 to 7 MW. Time integrated spectral measurements showed that the harder bursts were dominated by K-alpha emission; though, a lower level, wide band continuum up to at least 30 keV was also present. Initial tests demonstrated that the source was capable of driving Laue diffraction experiments, probing uncompressed samples of LiF and aluminium.

  12. X-ray Science Division (XSD) | Advanced Photon Source

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    XSD Groups XSD Safety and Training XSD Strategic Plan XSD Visitor Program XSD Intranet X-ray Science Division (XSD) XSD enables world-class research using x-rays by developing...

  13. ALS X-Rays Shine a New Light on Catalysis

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ALS X-Rays Shine a New Light on Catalysis ALS X-Rays Shine a New Light on Catalysis Print Thursday, 21 May 2015 11:16 Electrocatalysts are responsible for expediting reactions in...

  14. Using Light to Control How X Rays Interact with Matter

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    that can be controlled by varying the properties of the optical control beam. Problems arise, however, when the probe pulse lies in the x-ray regime because x rays interact...

  15. A Spatially Resolving X-ray Crystal Spectrometer for Measurement...

    Office of Scientific and Technical Information (OSTI)

    A Spatially Resolving X-ray Crystal Spectrometer for Measurement of Ion-temperature and ... Title: A Spatially Resolving X-ray Crystal Spectrometer for Measurement of Ion-temperature ...

  16. X-Ray Diffraction Microscopy of Magnetic Structures

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-Ray Diffraction Microscopy of Magnetic Structures Print science brief icon Scientists working at ALS Beamline 12.0.2.2 have demonstrated a new x-ray technique for producing...

  17. NIF and OMEGA X-Ray Environments Summary (Technical Report) ...

    Office of Scientific and Technical Information (OSTI)

    Technical Report: NIF and OMEGA X-Ray Environments Summary Citation Details In-Document Search Title: NIF and OMEGA X-Ray Environments Summary You are accessing a document from...

  18. Using Light to Control How X Rays Interact with Matter

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Using Light to Control How X Rays Interact with Matter Using Light to Control How X Rays Interact with Matter Print Wednesday, 27 January 2010 00:00 Schemes that use one light...

  19. Sector 3 : High Resolution X-ray Scattering | Advanced Photon...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    & workshops IXN Group Useful Links Current APS status ESAF System GUP System X-Ray Science Division My APS Portal Sector 3 : High Resolution X-ray Scattering Sector 3 is...

  20. NIF and OMEGA X-Ray Environments Summary (Technical Report) ...

    Office of Scientific and Technical Information (OSTI)

    NIF and OMEGA X-Ray Environments Summary Citation Details In-Document Search Title: NIF and OMEGA X-Ray Environments Summary Abstract not provided. Authors: Fournier, K. B. 1 + ...

  1. X-Ray Interactions with Matter from the Center for X-Ray Optics (CXRO)

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Henke, B. L.; Gullikson, E. M.; Davis, J. C.

    The primary interactions of low-energy x-rays within condensed matter, viz. photoabsorption and coherent scattering, are described for photon energies outside the absorption threshold regions by using atomic scattering factors. The atomic scattering factors may be accurately determined from the atomic photoabsorption cross sections using modified Kramers-Kronig dispersion relations. From a synthesis of the currently available experimental data and recent theoretical calculations for photoabsorption, the angle-independent, forward-scattering components of the atomic scattering factors have been thus semiempirically determined and tabulated here for 92 elements and for the region 50-30,000 eV. Atomic scattering factors for all angles of coherent scattering and at the higher photon energies are obtained from these tabulated forward-scattering values by adding a simple angle-dependent form-factor correction. The incoherent scattering contributions that become significant for the light elements at the higher photon energies are similarly determined. The basic x-ray interaction relations that are used in applied x-ray physics are presented here in terms of the atomic scattering factors. The bulk optical constants are also related to the atomic scattering factors. These atomic and optical relations are applied to the detailed calculation of the reflectivity characteristics of a series of practical x-ray mirror, multilayer, and crystal monochromators. Comparisons of the results of this semiempirical,"atom-like", description of x-ray interactions for the low-energy region with those of experiment and ab initio theory are presented.

  2. Femtosecond laser-electron x-ray source

    DOE Patents [OSTI]

    Hartemann, Frederic V.; Baldis, Hector A.; Barty, Chris P.; Gibson, David J.; Rupp, Bernhard

    2004-04-20

    A femtosecond laser-electron X-ray source. A high-brightness relativistic electron injector produces an electron beam pulse train. A system accelerates the electron beam pulse train. The femtosecond laser-electron X-ray source includes a high intra-cavity power, mode-locked laser and an x-ray optics system.

  3. Maskelynite formation via solid-state transformation: Evidence of infrared and x-ray anisotropy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Jaret, Steven J.; Ehm, Lars; Woerner, William R.; Phillips, Brian L.; Nekvasil, Hanna; Wright, Shawn P.; Glotch, Timothy D.

    2015-03-24

    We present optical microscopy, micro-Raman spectroscopy, nuclear magnetic resonance (NMR) spectroscopy, high-energy X-ray total scattering experiments, and micro-Fourier transform infrared (micro-FTIR) spectroscopy on shocked labradorite from the Lonar Crater, India. We show that maskelynite of shock class 2 is structurally more similar to fused glass than to crystalline plagioclase. However, there are slight but significant differences – preservation of original pre-impact igneous zoning, anisotropy at Infrared wavelengths, X-ray anisotropy, and preservation of some intermediate range order – which are all consistent with a solid-state transformation formation of maskelynite.

  4. Maskelynite formation via solid-state transformation: Evidence of infrared and x-ray anisotropy

    SciTech Connect (OSTI)

    Jaret, Steven J.; Ehm, Lars; Woerner, William R.; Phillips, Brian L.; Nekvasil, Hanna; Wright, Shawn P.; Glotch, Timothy D.

    2015-03-24

    We present optical microscopy, micro-Raman spectroscopy, nuclear magnetic resonance (NMR) spectroscopy, high-energy X-ray total scattering experiments, and micro-Fourier transform infrared (micro-FTIR) spectroscopy on shocked labradorite from the Lonar Crater, India. We show that maskelynite of shock class 2 is structurally more similar to fused glass than to crystalline plagioclase. However, there are slight but significant differences preservation of original pre-impact igneous zoning, anisotropy at Infrared wavelengths, X-ray anisotropy, and preservation of some intermediate range order which are all consistent with a solid-state transformation formation of maskelynite.

  5. Hard X-ray spatial array diagnostics on Joint Texas Experimental Tokamak

    SciTech Connect (OSTI)

    Huang, D. W.; Chen, Z. Y. Luo, Y. H.; Tong, R. H.; Yan, W.; Jin, W.; Zhuang, G.

    2014-11-15

    A spatially distributed hard X-ray detection array has been developed to diagnose the loss of runaway electron with toroidal and poloidal resolution. The hard X-ray radiation in the energy ranges of 0.31 MeV resulted from runaway electrons can be measured. The detection array consists of 12 CdTe detectors which are arranged surrounding the tokamak. It is found that most runaway electrons which transport to plasma boundary tend to loss on limiters. The application of electrode biasing probe resulted in enhancement of local runaway loss. Resonant magnetic perturbations enhanced the runaway electrons diffusion and showed an asymmetric poloidal loss rate.

  6. Apparatus for X-ray diffraction microscopy and tomography of cryo specimens

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Beetz, T.; Howells, M. R.; Jacobsen, C.; Kao, C. -C.; Kirz, J.; Lima, E.; Mentes, T. O.; Miao, H.; Sanchez-Hanke, C.; Sayre, D.; et al

    2005-03-14

    An apparatus for diffraction microscopy of biological and materials science specimens is described. In this system, a coherent soft X-ray beam is selected with a pinhole, and the illuminated specimen is followed by an adjustable beamstop and CCD camera to record diffraction data from non-crystalline specimens. In addition, a Fresnel zone plate can be inserted to allow for direct imaging. The system makes use of a cryogenic specimen holder with cryotransfer capabilities to allow frozen hydrated specimens to be loaded. The specimen can be tilted over a range of ± 80 ° degrees for three-dimensional imaging; this is done bymore » computer-controlled motors, enabling automated alignment of the specimen through a tilt series. The system is now in use for experiments in soft X-ray diffraction microscopy.« less

  7. X-Ray Imaging Crystal Spectrometer for Extended X-Ray Sources

    SciTech Connect (OSTI)

    Bitter, Manfred L.; Fraekel, Benjamin; Gorman, James L.; Hill, Kenneth W.; Roquemore, Lane A.; Stodiek, Wolfgang; Goeler, Schweickhard von

    1999-05-01

    Spherically or toroidally curved, double focusing crystals are used in a spectrometer for X-ray diagnostics of an extended X-ray source such as a hot plasma produced in a tokamak fusion experiment to provide spatially and temporally resolved data on plasma parameters such as ion temperature, toroidal and poloidal rotation, electron temperature, impurity ion charge-state distributions, and impurity transport. The imaging properties of these spherically or toroidally curved crystals provide both spectrally and spatially resolved X-ray data from the plasma using only one small spherically or toroidally curved crystal, thus eliminating the requirement for a large array of crystal spectrometers and the need to cross-calibrate the various crystals.

  8. High efficiency replicated x-ray optics and fabrication method

    DOE Patents [OSTI]

    Barbee, Jr., Troy W.; Lane, Stephen M.; Hoffman, Donald E.

    2001-01-01

    Replicated x-ray optics are fabricated by sputter deposition of reflecting layers on a super-polished reusable mandrel. The reflecting layers are strengthened by a supporting multilayer that results in stronger stress-relieved reflecting surfaces that do not deform during separation from the mandrel. The supporting multilayer enhances the ability to part the replica from the mandrel without degradation in surface roughness. The reflecting surfaces are comparable in smoothness to the mandrel surface. An outer layer is electrodeposited on the supporting multilayer. A parting layer may be deposited directly on the mandrel before the reflecting surface to facilitate removal of the layered, tubular optic device from the mandrel without deformation. The inner reflecting surface of the shell can be a single layer grazing reflection mirror or a resonant multilayer mirror. The resulting optics can be used in a wide variety of applications, including lithography, microscopy, radiography, tomography, and crystallography.

  9. Holographic Methods in X-ray Crystallography

    Energy Science and Technology Software Center (OSTI)

    1995-07-28

    The holographic method makes use of partially modeled electron density and experimentally-measured structure factor amplitudes to recover electron density corresponding to the unmodeled part of a crystal structure. This paper describes a fast algorithm that makes it possible to apply the holographic method to sizable crystallographic problems. The algorithm uses positivity constraints on the electron density, and can incorporate a target electron density, making it similar to solvent flattening. Using both synthetic and experimental data,morewe assess the potential for applying the holographic method to macromolecular x-ray crystallography.less

  10. Digital X-ray Pipe Inspector Software

    Energy Science and Technology Software Center (OSTI)

    2009-10-29

    The Digital X-ray Pipe Inspector software requires a digital x-ray image of a pipe as input to the program, such as the image in Attachment A Figure 1. The image may be in a variety of software formats such as bitmap, jpeg, tiff, DICOM or DICONDE. The software allows the user to interactively select a region of interest from the image for analysis. This software is used to analyze digital x-ray images of pipes tomore » evaluate loss of wall thickness. The software specifically provides tools to analyze the image in (a) the pipe walls, (b) between the pipe walls. Traditional software uses only the information at the pipe wall while this new software also evaluates the image between the pipewalls. This makes the inspection process faster, more thorough, more efficient, and reduces expensive reshots. Attachment A Figure 2 shows a region of interest (a green box) drawn by the user around an anomaly in the pipe wall. This area is automatically analyzed by the external pipe wall tool with the result shown in Attachment A Figure 3. The edges of the pipe wall are detected and highlighted in yellow and areas where the wall thickness in less the the minimum wall threshold are shown in red. These measurements are typically made manually in other software programs, which lead to errors and inconsistency because the location of the edges are estimated by the user. Attachment A Figure 4 shows a region of interest (a green box) drawn by the user between the pipe walls. As can be seen there are intensity anomalies that correspond to wall defects. However, this information is not used directly by other software programs. In order to fully investigate these anomalies, the pipe would be reinspected in a different orientation to attempt to obtain a view of the anomaly in the pipe wall rather than the interior of the pipe. The pipe may need to be x-rayed a number of times to obtain the correct orientation. This is very costly and time consuming. The new software can perform the analysis directly on the intensity information in the original image. Figures 5 through 9 in Attachment A show wall defects in red for various percents of wall thickness loss. For example, Figure 5 show defects (in red) where the wall thickness is 95% or less than the nominal wall thickness (or a 5% or greater wall thickness loss). Wall thicknesses can be given in absolute terms as well.« less

  11. Apparatus for monitoring X-ray beam alignment

    DOE Patents [OSTI]

    Steinmeyer, P.A.

    1991-10-08

    A self-contained, hand-held apparatus is provided for monitoring alignment of an X-ray beam in an instrument employing an X-ray source. The apparatus includes a transducer assembly containing a photoresistor for providing a range of electrical signals responsive to a range of X-ray beam intensities from the X-ray beam being aligned. A circuit, powered by a 7.5 VDC power supply and containing an audio frequency pulse generator whose frequency varies with the resistance of the photoresistor, is provided for generating a range of audible sounds. A portion of the audible range corresponds to low X-ray beam intensity. Another portion of the audible range corresponds to high X-ray beam intensity. The transducer assembly may include an a photoresistor, a thin layer of X-ray fluorescent material, and a filter layer transparent to X-rays but opaque to visible light. X-rays from the beam undergoing alignment penetrate the filter layer and excite the layer of fluorescent material. The light emitted from the fluorescent material alters the resistance of the photoresistor which is in the electrical circuit including the audio pulse generator and a speaker. In employing the apparatus, the X-ray beam is aligned to a complete alignment by adjusting the X-ray beam to produce an audible sound of the maximum frequency. 2 figures.

  12. Apparatus for monitoring X-ray beam alignment

    DOE Patents [OSTI]

    Steinmeyer, Peter A. (Arvada, CO)

    1991-10-08

    A self-contained, hand-held apparatus is provided for minitoring alignment of an X-ray beam in an instrument employing an X-ray source. The apparatus includes a transducer assembly containing a photoresistor for providing a range of electrical signals responsive to a range of X-ray beam intensities from the X-ray beam being aligned. A circuit, powered by a 7.5 VDC power supply and containing an audio frequency pulse generator whose frequency varies with the resistance of the photoresistor, is provided for generating a range of audible sounds. A portion of the audible range corresponds to low X-ray beam intensity. Another portion of the audible range corresponds to high X-ray beam intensity. The transducer assembly may include an a photoresistor, a thin layer of X-ray fluorescent material, and a filter layer transparent to X-rays but opaque to visible light. X-rays from the beam undergoing alignment penetrate the filter layer and excite the layer of fluorescent material. The light emitted from the fluorescent material alters the resistance of the photoresistor which is in the electrical circuit including the audio pulse generator and a speaker. In employing the apparatus, the X-ray beam is aligned to a complete alignment by adjusting the X-ray beam to produce an audible sound of the maximum frequency.

  13. High-Resolution Structure of the Photosynthetic Mn4Ca Catalyst from X-ray Spectroscopy

    SciTech Connect (OSTI)

    Yachandra, Vittal; Yano, Junko; Kern, Jan; Pushkar, Yulia; Sauer, Kenneth; Glatzel, Pieter; Bergmann, Uwe; Messinger, Johannes; Zouni, Athina; Yachandra, Vittal K.

    2007-08-01

    The application of high-resolution X-ray spectroscopy methods to study the photosynthetic water oxidizing complex, which contains a unique hetero-nuclear catalytic Mn4Ca cluster, are described. Issues of X-ray damage especially at the metal sites in the Mn4Ca cluster are discussed. The structure of the Mn4Ca catalyst at high-resolution which has so far eluded attempts of determination by X-ray diffraction, EXAFS and other spectroscopic techniques has been addressed using polarized EXAFS techniques applied to oriented PS II membrane preparations and PS II single crystals. A review of how the resolution of traditional EXAFS techniques can be improved, using methods such as range-extended EXAFS is presented, and the changes that occur in the structure of the cluster as it advances through the catalytic cycle are described. X-ray absorption and emission techniques (XANES and K? emission) have been used earlier to determine the oxidation states of the Mn4Ca cluster, and in this report we review the use of X-ray resonant Raman spectroscopy to understand the electronic structure of the Mn4Ca cluster as it cycles through the intermediate S-states.

  14. Boosting the Light: X-ray Physics in Confinement

    ScienceCinema (OSTI)

    Rhisberger, Ralf [HASYLAB/ DESY

    2010-01-08

    Remarkable effects are observed if light is confined to dimensions comparable to the wavelength of the light. The lifetime of atomic resonances excited by the radiation is strongly reduced in photonic traps, such as cavities or waveguides. Moreover, one observes an anomalous boost of the intensity scattered from the resonant atoms. These phenomena results from the strong enhancement of the photonic density of states in such geometries. Many of these effects are currently being explored in the regime of vsible light due to their relevance for optical information processing. It is thus appealing to study these phenomena also for much shorter wavelengths. This talk illuminates recent experiments where synchrotron x-rays were trapped in planar waveguides to resonantly excite atomos ([57]Fe nuclei_ embedded in them. In fact, one observes that the radiative decay of these excited atoms is strongly accelerated. The temporal acceleration of the decay goes along with a strong boost of the radiation coherently scattered from the confined atmos. This can be exploited to obtain a high signal-to-noise ratio from tiny quantities of material, leading to manifold applications in the investigation of nanostructured materials. One application is the use of ultrathin probe layers to image the internal structure of magnetic layer systems.

  15. A laboratory-based hard x-ray monochromator for high-resolution x-ray emission spectroscopy and x-ray absorption near edge structure measurements

    SciTech Connect (OSTI)

    Seidler, G. T. Mortensen, D. R.; Remesnik, A. J.; Pacold, J. I.; Ball, N. A.; Barry, N.; Styczinski, M.; Hoidn, O. R.

    2014-11-15

    We report the development of a laboratory-based Rowland-circle monochromator that incorporates a low power x-ray (bremsstrahlung) tube source, a spherically bent crystal analyzer, and an energy-resolving solid-state detector. This relatively inexpensive, introductory level instrument achieves 1-eV energy resolution for photon energies of ?5 keV to ?10 keV while also demonstrating a net efficiency previously seen only in laboratory monochromators having much coarser energy resolution. Despite the use of only a compact, air-cooled 10 W x-ray tube, we find count rates for nonresonant x-ray emission spectroscopy comparable to those achieved at monochromatized spectroscopy beamlines at synchrotron light sources. For x-ray absorption near edge structure, the monochromatized flux is small (due to the use of a low-powered x-ray generator) but still useful for routine transmission-mode studies of concentrated samples. These results indicate that upgrading to a standard commercial high-power line-focused x-ray tube or rotating anode x-ray generator would result in monochromatized fluxes of order 10{sup 6}10{sup 7} photons/s with no loss in energy resolution. This work establishes core technical capabilities for a rejuvenation of laboratory-based hard x-ray spectroscopies that could have special relevance for contemporary research on catalytic or electrical energy storage systems using transition-metal, lanthanide, or noble-metal active species.

  16. Gated monochromatic x-ray imager

    SciTech Connect (OSTI)

    Oertel, J.A.; Archuleta, T.; Clark, L.

    1995-09-01

    We have recently developed a gated monochromatic x-ray imaging diagnostic for the national Inertial-Confinement Fusion (ICF) program. This new imaging system will be one of the primary diagnostics to be utilized on University of Rochester`s Omega laser fusion facility. The new diagnostic is based upon a Kirkpatrick-Baez (KB) microscope dispersed by diffraction crystals, as first described by Marshall and Su. The dispersed images are gated by four individual proximity focused microchannel plates and recorded on film. Spectral coverage is tunable up to 8 keV, spectral resolution has been measured at 20 eV, temporal resolution is 80 ps, and spatial resolution is better than 10 {mu}m.

  17. Gray scale x-ray mask

    DOE Patents [OSTI]

    Morales, Alfredo M. (Livermore, CA); Gonzales, Marcela (Seattle, WA)

    2006-03-07

    The present invention describes a method for fabricating an embossing tool or an x-ray mask tool, providing microstructures that smoothly vary in height from point-to-point in etched substrates, i.e., structure which can vary in all three dimensions. The process uses a lithographic technique to transfer an image pattern in the surface of a silicon wafer by exposing and developing the resist and then etching the silicon substrate. Importantly, the photoresist is variably exposed so that when developed some of the resist layer remains. The remaining undeveloped resist acts as an etchant barrier to the reactive plasma used to etch the silicon substrate and therefore provides the ability etch structures of variable depths.

  18. Engineering Gilbert damping by dilute Gd doping in soft magnetic Fe thin films

    SciTech Connect (OSTI)

    Zhang, W. Jiang, S.; Sun, L.; Wang, Y. K.; Zhai, Y.; Wong, P. K. J.; Wang, K.; Jong, M. P. de; Wiel, W. G. van der; Laan, G. van der

    2014-05-07

    By analyzing the ferromagnetic resonance linewidth, we show that the Gilbert damping constant in soft magnetic Fe thin films can be enhanced by ?6 times with Gd doping of up to 20%. At the same time, the magnetic easy axis remains in the film plane while the coercivity is strongly reduced after Gd inclusion. X-ray magnetic circular dichroism measurements reveal a strong increase in the orbital-to-spin moment ratio of Fe with increasing Gd concentration, in full agreement with the increase in the Gilbert damping obtained for these thin films. Combined with x-ray diffraction and vibrating sample magnetometry, the results demonstrate that the FeGd thin films with dilute Gd doping of up to 20% are promising candidates for spin-transfer-torque applications in soft magnetic devices, in which an enhanced damping is required.

  19. Results from the NSTX X-ray Crystal Spectrometer

    SciTech Connect (OSTI)

    M. Bitter; K. Hill; L. Roquemore; P. Beiersdorfer; D. Thorn; Ming Feng Gu

    2003-01-14

    A high-resolution X-ray crystal spectrometer has recently been installed at the National Spherical Torus Experiment to record the satellite spectra of helium-like argon, ArXVII, in the wavelength range from 3.94 to 4.00 {angstrom} for measurements of ion and electron temperatures, and measurements of the ionization equilibrium of argon, which is of interest for studies of ion transport. The instrument presently consists of a spherically bent quartz crystal and a conventional one-dimensional position-sensitive multi-wire proportional counter, but it will soon be upgraded to a new type of X-ray imaging crystal spectrometer by the installation of a large size (10 cm x 30 cm) two-dimensional position-sensitive detector that will allow us to obtain temporally and spatially resolved spectra from an 80 cm high cross-section of the plasma. In its present configuration, the spectrometer has been optimized for high throughput so that it is possible to record spectra with small statistical errors with a time resolution of 10 ms by adding only small, nonperturbing amounts of argon to the plasma. The spectrometer is most valuable for measurements of the ion temperature in the absence of a neutral beam in ohmically heated and radio-frequency heated discharges, when charge exchange recombination spectroscopy does not function. Electron temperature measurements from the satellite-to-resonance line ratios have been important for a quantitative comparison with (and verification of) the Thomson scattering data. The paper will describe the instrumental details of the present and future spectrometer configurations, and present recent experimental results.

  20. Density gradient free electron collisionally excited x-ray laser

    DOE Patents [OSTI]

    Campbell, E.M.; Rosen, M.D.

    1984-11-29

    An operational x-ray laser is provided that amplifies 3p-3s transition x-ray radiation along an approximately linear path. The x-ray laser is driven by a high power optical laser. The driving line focused optical laser beam illuminates a free-standing thin foil that may be associated with a substrate for improved structural integrity. This illumination produces a generally cylindrically shaped plasma having an essentially uniform electron density and temperature, that exists over a long period of time, and provides the x-ray laser gain medium. The x-ray laser may be driven by more than one optical laser beam. The x-ray laser has been successfully demonstrated to function in a series of experimental tests.

  1. Density gradient free electron collisionally excited X-ray laser

    DOE Patents [OSTI]

    Campbell, Edward M. (Pleasanton, CA); Rosen, Mordecai D. (Berkeley, CA)

    1989-01-01

    An operational X-ray laser (30) is provided that amplifies 3p-3s transition X-ray radiation along an approximately linear path. The X-ray laser (30) is driven by a high power optical laser. The driving line focused optical laser beam (32) illuminates a free-standing thin foil (34) that may be associated with a substrate (36) for improved structural integrity. This illumination produces a generally cylindrically shaped plasma having an essentially uniform electron density and temperature, that exists over a long period of time, and provides the X-ray laser gain medium. The X-ray laser (30) may be driven by more than one optical laser beam (32, 44). The X-ray laser (30) has been successfully demonstrated to function in a series of experimental tests.

  2. X-ray transmission movies of spontaneous dynamic events

    SciTech Connect (OSTI)

    Smilowitz, L.; Henson, B. F.; Holmes, M.; Novak, A.; Oschwald, D.; Dolgonos, P.; Qualls, B.

    2014-11-15

    We describe a new x-ray radiographic imaging system which allows for continuous x-ray transmission imaging of spontaneous dynamic events. We demonstrate this method on thermal explosions in three plastic bonded formulations of the energetic material octahydro-1,3,5,7-tetranitro-1,3,5,7-tetrazocine. We describe the x-ray imaging system and triggering developed to enable the continuous imaging of a thermal explosion.

  3. X-ray interferometry with spherically bent crystals (abstract)

    SciTech Connect (OSTI)

    Koch, Jeffrey A.

    2001-01-01

    Recent progress in manufacturing high-quality spherically bent crystals allows highly monochromatic x-ray beams to be produced, and allows efficient x-ray imaging with {mu}m-scale resolution. This article explores some of the constraints for x-ray interferometry utilizing spherically bent crystals and laser-produced plasma sources, and discusses several shearing interferometer concepts that might be experimentally investigated.

  4. Generation of Coherent X-Ray Radiation through Modulation Compression

    Office of Scientific and Technical Information (OSTI)

    (Journal Article) | SciTech Connect Journal Article: Generation of Coherent X-Ray Radiation through Modulation Compression Citation Details In-Document Search Title: Generation of Coherent X-Ray Radiation through Modulation Compression In this paper, we propose a scheme to generate tunable coherent X-ray radiation for future light source applications. This scheme uses an energy chirped electron beam, a laser modulator, a laser chirper and two bunch compressors to generate a prebunched

  5. Legacy of the X-Ray Laser Program

    SciTech Connect (OSTI)

    Nilsen, J.

    1993-08-06

    The X-Ray Laser Program has evolved from a design effort focusing on developing a Strategic Defense Initiative weapon that protects against Soviet ICBMs to a scientific project that is producing new technologies for industrial and medical research. While the great technical successes and failures of the X-ray laser itself cannot be discussed, this article presents the many significant achievements made as part of the X-ray laser effort that are now being used for other applications at LLNL.

  6. Characterization of spatially resolved high resolution x-ray spectrometers

    Office of Scientific and Technical Information (OSTI)

    for high energy density physics and light source experiments (Journal Article) | SciTech Connect Characterization of spatially resolved high resolution x-ray spectrometers for high energy density physics and light source experiments Citation Details In-Document Search Title: Characterization of spatially resolved high resolution x-ray spectrometers for high energy density physics and light source experiments A high resolution 1D imaging x-ray spectrometer concept comprising a spherically

  7. Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism Print Wednesday, 29 August 2007 00:00 Using spectroscopic information for magnetometry and magnetic microscopy obviously requires detailed theoretical understanding of spectral shape and magnitude of dichroism signals. A research team at ALS Beamline 4.0.2 has now shown unambiguously that, contrary to common belief, spectral shape and magnitude of x-ray magnetic

  8. Femtosecond nanocrystallography using X-ray lasers for membrane protein

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    structure determination Femtosecond nanocrystallography using X-ray lasers for membrane protein structure determination Authors: Fromme, P., and Spence, J. C. H. Title: Femtosecond nanocrystallography using X-ray lasers for membrane protein structure determination Source: Current Opinion in Structural Biology Year: 2011 Volume: 21 Pages: 509-516 ABSTRACT: The invention of free electron X-ray lasers has opened a new era for membrane protein structure determination with the recent first

  9. 14.05.14 RH Synchrotron X-ray - JCAP

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    High-Throughput Synchrotron X-Ray Experimentation for Combinatorial Phase Matching Gregoire, J. M. et al. High-throughput synchrotron X-ray diffraction for combinatorial phase mapping. Journal of Synchrotron Radiation 21, 1262-1268, DOI: 10.1107/s1600577514016488 (2014). Scientific Achievement Development of new synchrotron X-ray diffraction and fluorescence methods for rapid characterization of material libraries. Significance & impact First demonstration of prototype facility capable of

  10. ANL CT Reconstruction Algorithm for Utilizing Digital X-ray

    Energy Science and Technology Software Center (OSTI)

    2004-05-01

    Reconstructs X-ray computed tomographic images from large data sets known as 16-bit binary sinograms when using a massively parallelized computer architecture such as a Beowuif cluster by parallelizing the X-ray CT reconstruction routine. The algorithm uses the concept of generation of an image from carefully obtained multiple 1-D or 2-D X-ray projections. The individual projections are filtered using a digital Fast Fourier Transform. The literature refers to this as filtered back projection.

  11. Ultra-short wavelength x-ray system

    DOE Patents [OSTI]

    Umstadter, Donald (Ann Arbor, MI); He, Fei (Ann Arbor, MI); Lau, Yue-Ying (Potomac, MD)

    2008-01-22

    A method and apparatus to generate a beam of coherent light including x-rays or XUV by colliding a high-intensity laser pulse with an electron beam that is accelerated by a synchronized laser pulse. Applications include x-ray and EUV lithography, protein structural analysis, plasma diagnostics, x-ray diffraction, crack analysis, non-destructive testing, surface science and ultrafast science.

  12. X-ray compass for determining device orientation

    DOE Patents [OSTI]

    Da Silva, L.B.; Matthews, D.L.; Fitch, J.P.; Everett, M.J.; Colston, B.W.; Stone, G.F.

    1999-06-15

    An apparatus and method for determining the orientation of a device with respect to an x-ray source are disclosed. In one embodiment, the present invention is coupled to a medical device in order to determine the rotational orientation of the medical device with respect to the x-ray source. In such an embodiment, the present invention is comprised of a scintillator portion which is adapted to emit photons upon the absorption of x-rays emitted from the x-ray source. An x-ray blocking portion is coupled to the scintillator portion. The x-ray blocking portion is disposed so as to vary the quantity of x-rays which penetrate the scintillator portion based upon the particular rotational orientation of the medical device with respect to the x-ray source. A photon transport mechanism is also coupled to the scintillator portion. The photon transport mechanism is adapted to pass the photons emitted from the scintillator portion to an electronics portion. By analyzing the quantity of the photons, the electronics portion determines the rotational orientation of the medical device with respect to the x-ray source. 25 figs.

  13. ALS X-Rays Shine a New Light on Catalysis

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ALS X-Rays Shine a New Light on Catalysis Print Electrocatalysts are responsible for expediting reactions in many promising renewable energy technologies. However, the extreme...

  14. Self-terminating diffraction gates femtosecond X-ray nanocrystallograp...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The shortest apparent pulse lengths occur at the highest resolution, and our measurements indicate that current X-ray free-electron laser technology5 should enable structural ...

  15. Stimulated X-Ray Emission for Spectroscopy | Stanford Synchrotron...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Room 108A Speaker: Clemens Weninger, Max Planck Institute for the Physics of Complex Systems Program Description The recent advance of x-ray free electron lasers (XFELs)...

  16. High intensity x-ray source using liquid gallium target

    DOE Patents [OSTI]

    Smither, Robert K. (Hinsdale, IL); Knapp, Gordon S. (Cupertino, CA); Westbrook, Edwin M. (Chicago, IL); Forster, George A. (Westmont, IL)

    1990-01-01

    A high intensity x-ray source that uses a flowing stream of liquid gallium as a target with the electron beam impinging directly on the liquid metal.

  17. Crystallization and preliminary X-ray crystallographic studies...

    Office of Scientific and Technical Information (OSTI)

    protein from Drosophila melanogaster Citation Details In-Document Search Title: Crystallization and preliminary X-ray crystallographic studies of Drep-3, a DFF-related protein ...

  18. X-ray Diffuse Scattering Measurements of Nucleation Dynamics...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-ray Diffuse Scattering Measurements of Nucleation Dynamics at Femtosecond Resolution Real-time measurement and control of the non-equilibrium properties of materials represents ...

  19. Staff Research Physicist (X-Ray Spectroscopy) | Princeton Plasma...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    of X-ray spectrometers for high energy density plasma at the National Ignition Facility (NIF) at the Lawrence Livermore National Laboratory (LLNL, Livermore, California). In...

  20. X-ray image reconstruction from a diffraction pattern alone

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Marchesini, Stefano

    2015-03-16

    X-ray diffraction pattern of a sample of 50 nm colloidal gold particles, recorded at a wavelength of 2.1 nm.

  1. X-Ray Microscopy Capabilities | Argonne National Laboratory

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Hard X-Ray Nanoprobe (HXN) facility provides scanning fluorescence, scanning diffraction, and full-field transmission and tomographic imaging capabilities with a spatial...

  2. X-Ray Fluorescence (XRF) | Open Energy Information

    Open Energy Info (EERE)

    Dispersive Spectroscopy (WDS) typically performed using a SEM or EPMA, and X-Ray Diffraction (XRD) analyses. Rock Lab Analysis Core Analysis Cuttings Analysis Isotopic...

  3. Using Light to Control How X Rays Interact with Matter

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    the microscopic world, can have unwanted consequences for the materials they probe. Radiation damage due to x-ray absorption is, for instance, an unwanted consequence of using...

  4. ALS X-Rays Shine a New Light on Catalysis

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    were able to directly observe redox processes in thin-film iron and cobalt perovskite oxide electrocatalysts using surface-sensitive, x-ray absorption spectroscopy while...

  5. Diagnostics Implemented on NIF - X-ray Diagnostics

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-ray Diagnostics Diagnostic acronym Diangostic Port location Built and commisioned by Description of function Published references ARIANE Active Readout in a Neutron Environment (gated x-ray imager) 90-89 (but uses DIM) LLNL ARIANE is a gated x-ray detector measuring x-ray output at yields up to ~1E16 neutrons from TCC. ARIANE uses gated MCP technology adapted to operate in this neutron regime by moving the detector to a position just outside of the target chamber wall. ARIANE is typically used

  6. Simulating Wavefront Correction via Deformable Mirrors at X-Ray...

    Office of Scientific and Technical Information (OSTI)

    Resource Type: Conference Resource Relation: Conference: Presented at: X-ray Adaptive Optics, San Diego, CA, United States, Aug 14 - Aug 14, 2012 Research Org: Lawrence Livermore...

  7. X-Ray Diffraction Microscopy of Magnetic Structures (Journal...

    Office of Scientific and Technical Information (OSTI)

    Prev Next Title: X-Ray Diffraction Microscopy of Magnetic Structures Authors: Turner, Joshua J. ; Huang, Xiaojing ; Krupin, Oleg ; Seu, Keoki A. ; Parks, Daniel ; Kevan,...

  8. Portable X-Ray Diffraction (XRD) | Open Energy Information

    Open Energy Info (EERE)

    X-ray powder diffraction, which has traditionally been used in geology, environmental science, material science, and engineering to rapidly identify unknown crystalline...

  9. X-Ray Diffraction (XRD) | Open Energy Information

    Open Energy Info (EERE)

    under investigation. X-ray powder diffraction is widely used in geology, environmental science, material science, and engineering to rapidly identify unknown crystalline substances...

  10. XRMS: X-Ray Spectroscopy of Magnetic Solids

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    XRMS: X-Ray Spectroscopy of Magnetic Solids October 22-23, 2011 SLAC National Accelerator Laboratory, Menlo Park, CA More information...

  11. X-ray compass for determining device orientation

    DOE Patents [OSTI]

    Da Silva, Luiz B. (Danville, CA); Matthews, Dennis L. (Moss Beach, CA); Fitch, Joseph P. (Livermore, CA); Everett, Matthew J. (Pleasanton, CA); Colston, Billy W. (Livermore, CA); Stone, Gary F. (Livermore, CA)

    1999-01-01

    An apparatus and method for determining the orientation of a device with respect to an x-ray source. In one embodiment, the present invention is coupled to a medical device in order to determine the rotational orientation of the medical device with respect to the x-ray source. In such an embodiment, the present invention is comprised of a scintillator portion which is adapted to emit photons upon the absorption of x-rays emitted from the x-ray source. An x-ray blocking portion is coupled to the scintillator portion. The x-ray blocking portion is disposed so as to vary the quantity of x-rays which penetrate the scintillator portion based upon the particular rotational orientation of the medical device with respect to the x-ray source. A photon transport mechanism is also coupled to the scintillator portion. The photon transport mechanism is adapted to pass the photons emitted from the scintillator portion to an electronics portion. By analyzing the quantity of the photons, the electronics portion determines the rotational orientation of the medical device with respect to the x-ray source.

  12. Integrated X-ray Reflectivity Measurements for Elliptically Curved...

    Office of Scientific and Technical Information (OSTI)

    The elliptically curved pentaerythritol (PET) crystals used in the Supersnout 2 X-ray spectrometer on the National Ignition Facility (NIF) at Lawrence Livermore National Laboratory ...

  13. The 2011 outburst of recurrent nova T Pyx: X-ray observations expose the white dwarf mass and ejection dynamics

    SciTech Connect (OSTI)

    Chomiuk, Laura; Nelson, Thomas; Mukai, Koji; Rupen, Michael P.; Mioduszewski, Amy J.; Krauss, Miriam I.; Page, Kim L.; Osborne, Julian P.; Kuulkers, Erik; Roy, Nirupam

    2014-06-20

    The recurrent nova T Pyx underwent its sixth historical outburst in 2011, and became the subject of an intensive multi-wavelength observational campaign. We analyze data from the Swift and Suzaku satellites to produce a detailed X-ray light curve augmented by epochs of spectral information. X-ray observations yield mostly non-detections in the first four months of outburst, but both a super-soft and hard X-ray component rise rapidly after Day 115. The super-soft X-ray component, attributable to the photosphere of the nuclear-burning white dwarf, is relatively cool (?45 eV) and implies that the white dwarf in T Pyx is significantly below the Chandrasekhar mass (?1 M {sub ?}). The late turn-on time of the super-soft component yields a large nova ejecta mass (? 10{sup 5} M {sub ?}), consistent with estimates at other wavelengths. The hard X-ray component is well fit by a ?1 keV thermal plasma, and is attributed to shocks internal to the 2011 nova ejecta. The presence of a strong oxygen line in this thermal plasma on Day 194 requires a significantly super-solar abundance of oxygen and implies that the ejecta are polluted by white dwarf material. The X-ray light curve can be explained by a dual-phase ejection, with a significant delay between the first and second ejection phases, and the second ejection finally released two months after outburst. A delayed ejection is consistent with optical and radio observations of T Pyx, but the physical mechanism producing such a delay remains a mystery.

  14. SWIFT X-RAY AND ULTRAVIOLET MONITORING OF THE CLASSICAL NOVA V458 VUL (NOVA VUL 2007)

    SciTech Connect (OSTI)

    Ness, J.-U. [European Space Astronomy Centre, P.O. Box 78, 28691 Villanueva de la Canada, Madrid (Spain); Drake, J. J. [Harvard-Smithsonian Center for Astrophysics, 60 Garden Street, Cambridge, MA 02138 (United States); Beardmore, A. P.; Evans, P. A.; Osborne, J. P.; Page, K. L. [Department of Physics and Astronomy, University of Leicester, Leicester LE1 7RH (United Kingdom); Boyd, D. [BAA VSS, 5 Silver Lane, West Challow, Wantage, OX12 9TX (United Kingdom); Bode, M. F. [Astrophysics Research Institute, Liverpool John Moores University, Twelve Quays House, Egerton Wharf, Birkenhead CH41 1LD (United Kingdom); Brady, S. [AAVSO, 5 Melba Drive, Hudson, NH 03051 (United States); Gaensicke, B. T.; Steeghs, D. [Department of Physics, University of Warwick, Coventry CV4 7AL (United Kingdom); Kitamoto, S.; Takei, D. [Department of Physics, Rikkyo University, 3-34-1 Nishi-Ikebukuro, Toshima, Tokyo 171-8501 (Japan); Knigge, C. [School of Physics and Astronomy, University of Southampton, Southampton SO17 1BJ (United Kingdom); Miller, I. [BAA VSS, Furzehill House, Ilston, Swansea SA2 7LE (United Kingdom); Rodriguez-Gil, P. [Isaac Newton Group, PO Ap. de Correos 321, 38700 Sta. Cruz de la Palma (Spain); Schwarz, G. [Department of Geology and Astronomy, West Chester University, West Chester, PA 19383 (United States); Staels, B. [CBA Flanders, Alan Guth Observatory, Koningshofbaan 51, Hofstade, Aalst (Belgium); Tsujimoto, M. [Department of Astronomy and Astrophysics, Pennsylvania State University, 525 Davey Laboratory, University Park, PA 16802 (United States); Wesson, R. [Department of Physics and Astronomy, University College London, Gower Street, London WC1E 6BT (United Kingdom)], E-mail: juness@sciops.esa.int (and others)

    2009-05-15

    We describe the highly variable X-ray and UV emission of V458 Vul (Nova Vul 2007), observed by Swift between 1 and 422 days after outburst. Initially bright only in the UV, V458 Vul became a variable hard X-ray source due to optically thin thermal emission at kT = 0.64 keV with an X-ray band unabsorbed luminosity of 2.3 x 10{sup 34} erg s{sup -1} during days 71-140. The X-ray spectrum at this time requires a low Fe abundance (0.2{sup +0.3} {sub -0.1} solar), consistent with a Suzaku measurement around the same time. On day 315 we find a new X-ray spectral component which can be described by a blackbody with temperature of kT = 23{sup +9} {sub -5} eV, while the previous hard X-ray component has declined by a factor of 3.8. The spectrum of this soft X-ray component resembles those typically seen in the class of supersoft sources (SSS) which suggests that the nova ejecta were starting to clear and/or that the white dwarf photosphere is shrinking to the point at which its thermal emission reaches into the X-ray band. We find a high degree of variability in the soft component with a flare rising by an order of magnitude in count rate in 0.2 days. In the following observations on days 342.4-383.6, the soft component was not seen, only to emerge again on day 397. The hard component continued to evolve, and we found an anticorrelation between the hard X-ray emission and the UV emission, yielding a Spearman rank probability of 97%. After day 397, the hard component was still present, was variable, and continued to fade at an extremely slow rate but could not be analyzed owing to pile-up contamination from the bright SSS component.

  15. X-ray laser system, x-ray laser and method

    DOE Patents [OSTI]

    London, Richard A. (Oakland, CA); Rosen, Mordecai D. (Berkeley, CA); Strauss, Moshe (Omer, IL)

    1992-01-01

    Disclosed is an x-ray laser system comprising a laser containing generating means for emitting short wave length radiation, and means external to said laser for energizing said generating means, wherein when the laser is in an operative mode emitting radiation, the radiation has a transverse coherence length to width ratio of from about 0.05 to 1. Also disclosed is a method of adjusting the parameters of the laser to achieve the desired coherence length to laser width ratio.

  16. Femtosecond x-ray absorption spectroscopy with hard x-ray free electron laser

    SciTech Connect (OSTI)

    Katayama, Tetsuo; Togashi, Tadashi; Tono, Kensuke; Kameshima, Takashi; Inubushi, Yuichi; Sato, Takahiro; Hatsui, Takaki; Yabashi, Makina; Obara, Yuki; Misawa, Kazuhiko; Bhattacharya, Atanu; Kurahashi, Naoya; Ogi, Yoshihiro; Suzuki, Toshinori; Molecular Reaction Dynamics Research Team, RIKEN Center for Advanced Photonics, 2-1 Hirosawa, Wako 351-0198

    2013-09-23

    We have developed a method of dispersive x-ray absorption spectroscopy with a hard x-ray free electron laser (XFEL), generated by a self-amplified spontaneous emission (SASE) mechanism. A transmission grating was utilized for splitting SASE-XFEL light, which has a relatively large bandwidth (ΔE/E ∼ 5 × 10{sup −3}), into several branches. Two primary split beams were introduced into a dispersive spectrometer for measuring signal and reference spectra simultaneously. After normalization, we obtained a Zn K-edge absorption spectrum with a photon-energy range of 210 eV, which is in excellent agreement with that measured by a conventional wavelength-scanning method. From the analysis of the difference spectra, the noise ratio was evaluated to be ∼3 × 10{sup −3}, which is sufficiently small to trace minute changes in transient spectra induced by an ultrafast optical laser. This scheme enables us to perform single-shot, high-accuracy x-ray absorption spectroscopy with femtosecond time resolution.

  17. Magnetism studies using resonant, coherent, x-ray scattering...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    where the scattering vector q that can only be reached in reflection. The method is Fourier transform holography, where the exit wave from a sample interferes with a reference...

  18. X-ray imaging of Nonlinear Resonant Gyrotropic Magnetic Vortex...

    Office of Scientific and Technical Information (OSTI)

    Springfield, VA at www.ntis.gov. Authors: Mesler, Brooke ; Buchanan, Kristen ; Im, Mi-Young ; Fischer, Peter Publication Date: 2011-09-30 OSTI Identifier: 1172262 Report...

  19. Automated high pressure cell for pressure jump x-ray diffraction

    SciTech Connect (OSTI)

    Brooks, Nicholas J.; Gauthe, Beatrice L. L. E.; Templer, Richard H.; Ces, Oscar; Seddon, John M.; Terrill, Nick J.; Rogers, Sarah E.

    2010-06-15

    A high pressure cell for small and wide-angle x-ray diffraction measurements of soft condensed matter samples has been developed, incorporating a fully automated pressure generating network. The system allows both static and pressure jump measurements in the range of 0.1-500 MPa. Pressure jumps can be performed as quickly as 5 ms, both with increasing and decreasing pressures. Pressure is generated by a motorized high pressure pump, and the system is controlled remotely via a graphical user interface to allow operation by a broad user base, many of whom may have little previous experience of high pressure technology. Samples are loaded through a dedicated port allowing the x-ray windows to remain in place throughout an experiment; this facilitates accurate subtraction of background scattering. The system has been designed specifically for use at beamline I22 at the Diamond Light Source, United Kingdom, and has been fully integrated with the I22 beamline control systems.

  20. High resolution energy-sensitive digital X-ray

    DOE Patents [OSTI]

    Nygren, D.R.

    1995-07-18

    An apparatus and method for detecting an x-ray and for determining the depth of penetration of an x-ray into a semiconductor strip detector. In one embodiment, a semiconductor strip detector formed of semiconductor material is disposed in an edge-on orientation towards an x-ray source such that x-rays from the x-ray source are incident upon and substantially perpendicular to the front edge of the semiconductor strip detector. The semiconductor strip detector is formed of a plurality of segments. The segments are coupled together in a collinear arrangement such that the semiconductor strip detector has a length great enough such that substantially all of the x-rays incident on the front edge of the semiconductor strip detector interact with the semiconductor material which forms the semiconductor strip detector. A plurality of electrodes are connected to the semiconductor strip detector such that each one of the semiconductor strip detector segments has at least one of the of electrodes coupled thereto. A signal processor is also coupled to each one of the electrodes. The present detector detects an interaction within the semiconductor strip detector, between an x-ray and the semiconductor material, and also indicates the depth of penetration of the x-ray into the semiconductor strip detector at the time of the interaction. 5 figs.

  1. High resolution energy-sensitive digital X-ray

    DOE Patents [OSTI]

    Nygren, David R. (Berkeley, CA)

    1995-01-01

    An apparatus and method for detecting an x-ray and for determining the depth of penetration of an x-ray into a semiconductor strip detector. In one embodiment, a semiconductor strip detector formed of semiconductor material is disposed in an edge-on orientation towards an x-ray source such that x-rays From the x-ray source are incident upon and substantially perpendicular to the front edge of the semiconductor strip detector. The semiconductor strip detector is formed of a plurality of segments. The segments are coupled together in a collinear arrangement such that the semiconductor strip detector has a length great enough such that substantially all of the x-rays incident on the front edge of the semiconductor strip detector interact with the semiconductor material which forms the semiconductor strip detector. A plurality of electrodes are connected to the semiconductor strip detect or such that each one of the of semiconductor strip detector segments has at least one of the of electrodes coupled thereto. A signal processor is also coupled to each one of the electrodes. The present detector detects an interaction within the semiconductor strip detector, between an x-ray and the semiconductor material, and also indicates the depth of penetration of the x-ray into the semiconductor strip detector at the time of the interaction.

  2. High energy x-ray phase contrast CT using glancing-angle grating interferometers

    SciTech Connect (OSTI)

    Sarapata, A.; Stayman, J. W.; Siewerdsen, J. H.; Finkenthal, M.; Stutman, D.; Pfeiffer, F.

    2014-02-15

    Purpose: The authors present initial progress toward a clinically compatible x-ray phase contrast CT system, using glancing-angle x-ray grating interferometry to provide high contrast soft tissue images at estimated by computer simulation dose levels comparable to conventional absorption based CT. Methods: DPC-CT scans of a joint phantom and of soft tissues were performed in order to answer several important questions from a clinical setup point of view. A comparison between high and low fringe visibility systems is presented. The standard phase stepping method was compared with sliding window interlaced scanning. Using estimated dose values obtained with a Monte-Carlo code the authors studied the dependence of the phase image contrast on exposure time and dose. Results: Using a glancing angle interferometer at high x-ray energy (∼45 keV mean value) in combination with a conventional x-ray tube the authors achieved fringe visibility values of nearly 50%, never reported before. High fringe visibility is shown to be an indispensable parameter for a potential clinical scanner. Sliding window interlaced scanning proved to have higher SNRs and CNRs in a region of interest and to also be a crucial part of a low dose CT system. DPC-CT images of a soft tissue phantom at exposures in the range typical for absorption based CT of musculoskeletal extremities were obtained. Assuming a human knee as the CT target, good soft tissue phase contrast could be obtained at an estimated absorbed dose level around 8 mGy, similar to conventional CT. Conclusions: DPC-CT with glancing-angle interferometers provides improved soft tissue contrast over absorption CT even at clinically compatible dose levels (estimated by a Monte-Carlo computer simulation). Further steps in image processing, data reconstruction, and spectral matching could make the technique fully clinically compatible. Nevertheless, due to its increased scan time and complexity the technique should be thought of not as replacing, but as complimentary to conventional CT, to be used in specific applications.

  3. Broadband high resolution X-ray spectral analyzer

    DOE Patents [OSTI]

    Silver, E.H.; Legros, M.; Madden, N.W.; Goulding, F.; Landis, D.

    1998-07-07

    A broad bandwidth high resolution X-ray fluorescence spectrometer has a performance that is superior in many ways to those currently available. It consists of an array of 4 large area microcalorimeters with 95% quantum efficiency at 6 keV and it produces X-ray spectra between 0.2 keV and 7 keV with an energy resolution of 7 to 10 eV. The resolution is obtained at input count rates per array element of 10 to 50 Hz in real-time, with analog pulse processing and thermal pile-up rejection. This performance cannot be matched by currently available X-ray spectrometers. The detectors are incorporated into a compact and portable cryogenic refrigerator system that is ready for use in many analytical spectroscopy applications as a tool for X-ray microanalysis or in research applications such as laboratory and astrophysical X-ray and particle spectroscopy. 6 figs.

  4. Broadband high resolution X-ray spectral analyzer

    DOE Patents [OSTI]

    Silver, Eric H. (Berkeley, CA); Legros, Mark (Berkeley, CA); Madden, Norm W. (Livermore, CA); Goulding, Fred (Lafayette, CA); Landis, Don (Pinole, CA)

    1998-01-01

    A broad bandwidth high resolution x-ray fluorescence spectrometer has a performance that is superior in many ways to those currently available. It consists of an array of 4 large area microcalorimeters with 95% quantum efficiency at 6 keV and it produces x-ray spectra between 0.2 keV and 7 keV with an energy resolution of 7 to 10 eV. The resolution is obtained at input count rates per array element of 10 to 50 Hz in real-time, with analog pulse processing and thermal pile-up rejection. This performance cannot be matched by currently available x-ray spectrometers. The detectors are incorporated into a compact and portable cryogenic refrigerator system that is ready for use in many analytical spectroscopy applications as a tool for x-ray microanalysis or in research applications such as laboratory and astrophysical x-ray and particle spectroscopy.

  5. Apparatus for generating x-ray holograms

    DOE Patents [OSTI]

    Rhodes, Charles K.; Boyer, Keith; Solem, Johndale C.; Haddad, Waleed S.

    1990-01-01

    Apparatus for x-ray microholography of living biological materials. A Fourier transform holographic configuration is described as being most suitable for the 3-dimensional recording of the physical characteristics of biological specimens. The use of a spherical scatterer as a reference and a charge-coupled device two-dimensional detector array placed in the forward direction relative to the incident x-radiation for viewing electromagnetic radiation simultaneously scattered from both the specimen and the reference scatterer permits the ready reconstruction of the details of the specimen from the fringe pattern detected by the charge-coupled device. For example, by using a nickel reference scatter at 4.5 nm, sufficient reference illumination is provided over a wide enough angle to allow similar resolution in both transverse and longitudinal directions. Both laser and synchrotron radiation sources are feasible for generating microholographs. Operation in the water window (2.4 to 4.5 nm) should provide maximum contrast for features of the specimen and spatial resolution on the order of the wavelength of x-radiation should be possible in all three dimensions, which is sufficient for the visualization of many biological features. It is anticipated that the present apparatus will find utility in other areas as well where microscopic physical details of a specimen are important. A computational procedure which enables the holographic data collected by the detector to be used to correct for misalignments introduced by inexact knowledge of the relative positions of the spherical reference scatterer and the sample under investigation has been developed. If the correction is performed prior to reconstruction, full compensation can be achieved and a faithfully reconstructed image produced.

  6. Apparatus for generating x-ray holograms

    DOE Patents [OSTI]

    Rhodes, C.K.; Boyer, K.; Solem, J.C.; Haddad, W.S.

    1990-09-11

    Apparatus for x-ray microholography of living biological materials. A Fourier transform holographic configuration is described as being most suitable for the 3-dimensional recording of the physical characteristics of biological specimens. The use of a spherical scatterer as a reference and a charge-coupled device two-dimensional detector array placed in the forward direction relative to the incident x-radiation for viewing electromagnetic radiation simultaneously scattered from both the specimen and the reference scatterer permits the ready reconstruction of the details of the specimen from the fringe pattern detected by the charge-coupled device. For example, by using a nickel reference scatter at 4.5 nm, sufficient reference illumination is provided over a wide enough angle to allow similar resolution in both transverse and longitudinal directions. Both laser and synchrotron radiation sources are feasible for generating microholographs. Operation in the water window (2.4 to 4.5 nm) should provide maximum contrast for features of the specimen and spatial resolution on the order of the wavelength of x-radiation should be possible in all three dimensions, which is sufficient for the visualization of many biological features. It is anticipated that the present apparatus will find utility in other areas as well where microscopic physical details of a specimen are important. A computational procedure which enables the holographic data collected by the detector to be used to correct for misalignments introduced by inexact knowledge of the relative positions of the spherical reference scatterer and the sample under investigation has been developed. If the correction is performed prior to reconstruction, full compensation can be achieved and a faithfully reconstructed image produced. 7 figs.

  7. NEW X-RAY DETECTIONS OF WNL STARS

    SciTech Connect (OSTI)

    Skinner, Stephen L.; Zhekov, Svetozar A.; Guedel, Manuel; Schmutz, Werner; Sokal, Kimberly R.

    2012-05-15

    Previous studies have demonstrated that putatively single nitrogen-type Wolf-Rayet stars (WN stars) without known companions are X-ray sources. However, almost all WN star X-ray detections so far have been of earlier WN2-WN6 spectral subtypes. Later WN7-WN9 subtypes (also known as WNL stars) have proved more difficult to detect, an important exception being WR 79a (WN9ha). We present here new X-ray detections of the WNL stars WR 16 (WN8h) and WR 78 (WN7h). These new results, when combined with previous detections, demonstrate that X-ray emission is present in WN stars across the full range of spectral types, including later WNL stars. The two WN8 stars observed to date (WR 16 and WR 40) show unusually low X-ray luminosities (L{sub x} ) compared to other WN stars, and it is noteworthy that they also have the lowest terminal wind speeds (v{sub {infinity}}). Existing X-ray detections of about a dozen WN stars reveal a trend of increasing L{sub x} with wind luminosity L{sub wind} = (1/2)M-dot v{sup 2}{sub {infinity}}, suggesting that wind kinetic energy may play a key role in establishing X-ray luminosity levels in WN stars.

  8. WHOLE CELL TOMOGRAPHY/MOLECULAR BIOLOGY/STRUCTURAL BIOLOGY: Affordable x-ray microscopy with nanoscale resolution

    SciTech Connect (OSTI)

    Evans, James E.; Blackborow, Paul; Horne, Stephen J.; Gelb, Jeff

    2013-03-01

    Biological research spans 10 orders of magnitude from angstroms to meters. While electron microscopy can reveal structural details at most of these spatial length scales, transmission electron tomography only reliably reconstructs three-dimensional (3-D) volumes of cellular material with a spatial resolution between 1-5 nm from samples less than 500 nm thick1. Most biological cells are 2-30 times thicker than this threshold, which means that a cell must be cut into consecutive slices with each slice reconstructed individually in order to approximate the contextual information of the entire cell. Fortunately, due to a larger penetration depth2, X-ray computed tomography bypasses the need to physically section a cell and enables imaging of intact cells and tissues on the micrometer or larger scale with tens to hundreds of nanometer spatial resolution. While the technique of soft x-ray microscopy has been extensively developed in synchrotron facilities, advancements in laboratory x-ray source designs now increase its accessibility by supporting commercial systems suitable for a standard laboratory. In this paper, we highlight a new commercial compact cryogenic soft x-ray microscope designed for a standard laboratory setting and explore its capabilities for mesoscopic investigations of intact prokaryotic and eukaryotic cells.

  9. Spatiotemporal focusing dynamics in plasmas at X-ray wavelength

    SciTech Connect (OSTI)

    Sharma, A., E-mail: a-physics2001@yahoo.com; Tibai, Z. [Institute of Physics, University of Pecs, Pecs7624 (Hungary)] [Institute of Physics, University of Pecs, Pecs7624 (Hungary); Hebling, J. [Institute of Physics, University of Pecs, Pecs7624 (Hungary) [Institute of Physics, University of Pecs, Pecs7624 (Hungary); Szentagothai Research Centre, University of Pecs, Pecs-7624 (Hungary); Mishra, S. K. [Institute for Plasma Research, Gandhinagar (India)] [Institute for Plasma Research, Gandhinagar (India)

    2014-03-15

    Using a finite curvature beam, we investigate here the spatiotemporal focusing dynamics of a laser pulse in plasmas at X-ray wavelength. We trace the dependence of curvature parameter on the focusing of laser pulse and recognize that the self-focusing in plasma is more intense for the X-ray laser pulse with curved wavefront than with flat wavefront. The simulation results demonstrate that spatiotemporal focusing dynamics in plasmas can be controlled with the appropriate choice of beam-plasma parameters to explore the high intensity effects in X-ray regime.

  10. Laser-Produced Coherent X-Ray Sources

    SciTech Connect (OSTI)

    Donald Umstadter

    2007-01-31

    We study the generation of x-rays from the interaction of relativistic electrons with ultra-intense laser pulse either directly or via laser generated ion channels. The laser pulse acts as the accelerator and wiggler leading to an all-optical synchrotron-like x-ray source. The mm sized accelerator and micron-sized wiggler leads to a compact source of high brightness, ultrafast x-rays with applications in relativistic nonlinear optics, ultrafast chemistry, biology, inner-shell electronic processes and phase transitions.

  11. Characterization of X-ray generator beam profiles.

    SciTech Connect (OSTI)

    Mitchell, Dean J; Harding, Lee T.; Thoreson, Gregory G.; Theisen, Lisa Anne; Parmeter, John Ethan; Thompson, Kyle Richard

    2013-07-01

    T to compute the radiography properties of various materials, the flux profiles of X-ray sources must be characterized. This report describes the characterization of X-ray beam profiles from a Kimtron industrial 450 kVp radiography system with a Comet MXC-45 HP/11 bipolar oil-cooled X-ray tube. The empirical method described here uses a detector response function to derive photon flux profiles based on data collected with a small cadmium telluride detector. The flux profiles are then reduced to a simple parametric form that enables computation of beam profiles for arbitrary accelerator energies.

  12. X-ray backscatter imaging of nuclear materials

    DOE Patents [OSTI]

    Chapman, Jeffrey Allen; Gunning, John E; Hollenbach, Daniel F; Ott, Larry J; Shedlock, Daniel

    2014-09-30

    The energy of an X-ray beam and critical depth are selected to detect structural discontinuities in a material having an atomic number Z of 57 or greater. The critical depth is selected by adjusting the geometry of a collimator that blocks backscattered radiation so that backscattered X-ray originating from a depth less than the critical depth is not detected. Structures of Lanthanides and Actinides, including nuclear fuel rod materials, can be inspected for structural discontinuities such as gaps, cracks, and chipping employing the backscattered X-ray.

  13. Development of Ta-based Superconducting Tunnel Junction X-ray Detectors for Fluorescence XAS

    SciTech Connect (OSTI)

    Friedrich, S; Drury, O; Hall, J; Cantor, R

    2009-09-23

    We are developing superconducting tunnel junction (STJ) soft X-ray detectors for chemical analysis of dilute samples by fluorescence-detected X-ray absorption spectroscopy (XAS). Our 36-pixel Nb-based STJ spectrometer covers a solid angle {Omega}/4{pi} {approx} 10{sup -3}, offers an energy resolution of {approx}10-20 eV FWHM for energies up to {approx}1 keV, and can be operated at total count rates of {approx}10{sup 6} counts/s. For increased quantum efficiency and cleaner response function, we have now started the development of Ta-based STJ detector arrays. Initial devices modeled after our Nb-based STJs have an energy resolution below 10 eV FWHM for X-ray energies below 1 keV, and pulse rise time discrimination can be used to improve their response function for energies up to several keV. We discuss the performance of the Ta-STJs and outline steps towards the next-generation of large STJ detector arrays with higher sensitivity.

  14. High-resolution monochromatic x-ray imaging system based on spherically bent crystals

    SciTech Connect (OSTI)

    Aglitskiy, Y.; Lehecka, T.; Obenschain, S.; Bodner, S.; Pawley, C.; Gerber, K.; Sethian, J.; Brown, C.M.; Seely, J.; Feldman, U.; Holland, G.

    1998-08-01

    We have developed an improved x-ray imaging system based on spherically curve crystals. It is designed and used for diagnostics of targets ablatively accelerated by the Nike KrF laser. A spherically curved quartz crystal (2d=6.687 {Angstrom}, R=200 mm) has been used to produce monochromatic backlit images with the He-like Si resonance line (1865 eV) as the source of radiation. The spatial resolution of the x-ray optical system is 1.7 {mu}m in selected places and 2{endash}3 {mu}m over a larger area. Time-resolved backlit monochromatic images of polystyrene planar targets driven by the Nike facility have been obtained with a spatial resolution of 2.5 {mu}m in selected places and 5 {mu}m over the focal spot of the Nike laser. {copyright} 1998 Optical Society of America

  15. High resolution monochromatic X-ray imaging system based on spherically bent crystals

    SciTech Connect (OSTI)

    Aglitskiy, Y.; Lehecka, T.; Obenschain, S.; Bodner, S.; Pawley, C.; Gerber, K.; Sethian, J.; Brown, C. M.; Seely, J.; Feldman, U.; Holland, G.

    1997-05-05

    We have developed a new X-ray imaging system based on spherically curved crystals. It is designed and used for diagnostics of targets ablatively accelerated by the Nike KrF laser. The imaging system is used for plasma diagnostics of the main target and for characterization of potential backlighters. A spherically curved quartz crystal (2d=6.687 A, R=200 mm) is used to produce monochromatic backlit images with the He-like Si resonance line (1865 eV) as the source of radiation. The spatial resolution of the X-ray optical system is 3-4 {mu}m. Time resolved backlit monochromatic images of CH planar targets driven by the Nike facility have been obtained with 6-7 {mu}m spatial resolution.

  16. High resolution monochromatic X-ray imaging system based on spherically bent crystals

    SciTech Connect (OSTI)

    Aglitskiy, Y.; Lehecka, T.; Obenschain, S.; Bodner, S.; Pawley, C.; Gerber, K.; Sethian, J.; Brown, C.M.; Seely, J.; Feldman, U.; Holland, G.

    1997-05-01

    We have developed a new X-ray imaging system based on spherically curved crystals. It is designed and used for diagnostics of targets ablatively accelerated by the Nike KrF laser [1,2]. The imaging system is used for plasma diagnostics of the main target and for characterization of potential backlighters. A spherically curved quartz crystal (2d=6.687{Angstrom}, R=200mm) is used to produce monochromatic backlit images with the He-like Si resonance line (1865 eV) as the source of radiation. The spatial resolution of the X-ray optical system is 3{endash}4 {mu}m. Time resolved backlit monochromatic images of CH planar targets driven by the Nike facility have been obtained with 6{endash}7 {mu}m spatial resolution. {copyright} {ital 1997 American Institute of Physics.}

  17. 1-to 10-keV x-ray backlighting of annular wire arrays on the Sandia Z-machine using bent-crystal imaging techniques.

    SciTech Connect (OSTI)

    Rambo, Patrick K.; Wenger, David Franklin; Bennett, Guy R.; Sinars, Daniel Brian; Smith, Ian Craig; Porter, John Larry, Jr.; Cuneo, Michael Edward; Rovang, Dean Curtis; Anderson, Jessica E.

    2003-07-01

    Annular wire array implosions on the Sandia Z-machine can produce >200 TW and 1-2 MJ of soft x rays in the 0.1-10 keV range. The x-ray flux and debris in this environment present significant challenges for radiographic diagnostics. X-ray backlighting diagnostics at 1865 and 6181 eV using spherically-bent crystals have been fielded on the Z-machine, each with a {approx}0.6 eVspectral bandpass, 10 {micro}m spatial resolution, and a 4 mm by 20mm field of view. The Z-Beamlet laser, a 2-TW, 2-kJ Nd:glass laser({lambda} = 527 nm), is used to produce 0.1-1 J x-ray sources for radiography. The design, calibration, and performance of these diagnostics is presented.

  18. The diagnostic capability of x-ray scattering parameters for the characterization of breast cancer

    SciTech Connect (OSTI)

    Elshemey, Wael M.; Desouky, Omar S.; Fekry, Mostafa M.; Talaat, Sahar M.; Elsayed, Anwar A.

    2010-08-15

    Purpose: The evaluation of the diagnostic capability of easy to measure x-ray scattering profile characterization parameters for the detection of breast cancer in excised samples. The selected parameters are the full width at half maximum (FWHM) and area under the x-ray scattering profile of breast tissue in addition to the ratio of scattering intensities (I{sub 2}/I{sub 1}%) at 1.6 nm{sup -1} to that at 1.1 nm{sup -1} (corresponding to scattering from soft and adipose tissues, respectively). Methods: A histopathologist is asked to classify 36 excised breast tissue samples into healthy or malignant. A conventional x-ray diffractometer is used to acquire the scattering profiles of the investigated samples. The values of three profile characterization parameters are calculated and the diagnostic capability of each is evaluated by determining the optimal cutoffs of scatter diagrams, calculating the diagnostic indices, and plotting the receiver operating characteristic (ROC) curves. Results: At the calculated optimal cutoff for each of the examined parameters, the sensitivity ranged from 78% (for area under curve) up to 94% (for FWHM), the specificity ranged from 94%[for I{sub 2}/I{sub 1}% and area under curve] up to 100% (for FWHM), and the diagnostic accuracy ranged from 86% (for area under curve) up to 97% (for FWHM). The area under the ROC curves is greater than 0.95 for all of the investigated parameters, reflecting a highly accurate diagnostic performance. Conclusions: The discussed tests offered a means to quantitatively evaluate the performance of the suggested breast tissue x-ray scattering characterization parameters. The performance results are promising, indicating that the evaluated parameters would be considered a tool for fast, on spot probing of breast cancer in excised tissue samples.

  19. Experimental X-ray characterization of Gekko XII laser propagation...

    Office of Scientific and Technical Information (OSTI)

    Experimental X-ray characterization of Gekko XII laser propagation through very low density aerogels (2-5 mgcc) creating multi-keV photons from a titanium solid foil Citation...

  20. X-ray crystallographic analysis of adipocyte fatty acid binding...

    Office of Scientific and Technical Information (OSTI)

    binding protein (aP2) modified with 4-hydroxy-2-nonenal Citation Details In-Document Search Title: X-ray crystallographic analysis of adipocyte fatty acid binding protein (aP2) ...

  1. ALS X-Rays Shine a New Light on Catalysis

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    vice versa. At the ALS, researchers were able to directly observe redox processes in thin-film iron and cobalt perovskite oxide electrocatalysts using surface-sensitive, x-ray...

  2. Systems and methods for detecting x-rays

    DOE Patents [OSTI]

    Bross, Alan D.; Mellott, Kerry L.; Pla-Dalmau, Anna

    2006-05-02

    Systems and methods for detecting x-rays are disclosed herein. One or more x-ray-sensitive scintillators can be configured from a plurality of heavy element nano-sized particles and a plastic material, such as polystyrene. As will be explained in greater detail herein, the heavy element nano-sized particles (e.g., PbWO4) can be compounded into the plastic material with at least one dopant that permits the plastic material to scintillate. X-rays interact with the heavy element nano-sized particles to produce electrons that can deposit energy in the x-ray sensitive scintillator, which in turn can produce light.

  3. In situ Nanotomography and Operando Transmission X-ray Microscopy...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    and Operando Transmission X-ray Microscopy of Micron-sized Ge Particles in Battery Anodes Friday, August 29, 2014 Ge fig1 Figure 1. Schematic of the irreversible...

  4. X-ray mask and method for making

    DOE Patents [OSTI]

    Morales, Alfredo M.

    2004-10-26

    The present invention describes a method for fabricating an x-ray mask tool which is a contact lithographic mask which can provide an x-ray exposure dose which is adjustable from point-to-point. The tool is useful in the preparation of LIGA plating molds made from PMMA, or similar materials. In particular the tool is useful for providing an ability to apply a graded, or "stepped" x-ray exposure dose across a photosensitive substrate. By controlling the x-ray radiation dose from point-to-point, it is possible to control the development process for removing exposed portions of the substrate; adjusting it such that each of these portions develops at a more or less uniformly rate regardless of feature size or feature density distribution.

  5. Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    of the XMLD signal across the Ni L2,3 edges was determined by rotating the orientation of x-ray polarization E and external magnetic field H relative to the crystalline axes. ...

  6. Development of a Spatially Resolving X-Ray Crystal Spectrometer...

    Office of Scientific and Technical Information (OSTI)

    Fusion Links Development of a spatially resolving x-ray crystal spectrometer for measurement of ion-temperature "T i ... and rotation-velocity "v... profiles in ITER a... ...

  7. X-ray Diffraction from Membrane Protein Nanocrystals

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-ray Diffraction from Membrane Protein Nanocrystals Authors: Hunter, M.S., DePonte, D.P., Shapiro, D.A., Kirian, R.A., Wang, X., Starodub, D., Marchesini, S., Weierstall, U.,...

  8. X-ray Microscopy and Imaging (XSD-XMI)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    and (c) technical R&D in collaborations with other groups on nano-focusing x-ray optics, image contrast mechanisms, phase-retrieval methodology, detectors and data...

  9. X-Ray Photoelectron Spectroscopy (XPS) Applied to Soot & What...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Photoelectron Spectroscopy (XPS) Applied to Soot & What It Can Do for You X-Ray Photoelectron Spectroscopy (XPS) Applied to Soot & What It Can Do for You Presentation given at DEER...

  10. Using Light to Control How X Rays Interact with Matter

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Using Light to Control How X Rays Interact with Matter Print Schemes that use one light pulse to manipulate interactions of another with matter are well developed in the...

  11. X-Ray Diffraction Microscopy of Magnetic Structures

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lensless Imaging of Magnetic Nanostructures Work performed on ALS Beamline 12.0.2.2 Citation: J.J. Turner et al., "X-Ray Diffraction Microscopy of Magnetic Structures," Phys....

  12. Experimental X-ray characterization of Gekko XII laser propagation...

    Office of Scientific and Technical Information (OSTI)

    very low density aerogels (2-5 mgcc) creating multi-keV photons from a titanium solid foil Citation Details In-Document Search Title: Experimental X-ray characterization of...

  13. High performance x-ray anti-scatter grid

    DOE Patents [OSTI]

    Logan, Clinton M.

    1995-01-01

    An x-ray anti-scatter grid for x-ray imaging, particularly for screening mammography, and method for fabricating same, x-rays incident along a direct path pass through a grid composed of a plurality of parallel or crossed openings, microchannels, grooves, or slots etched in a substrate, such as silicon, having the walls of the microchannels or slots coated with a high opacity material, such as gold, while x-rays incident at angels with respect to the slots of the grid, arising from scatter, are blocked. The thickness of the substrate is dependent on the specific application of the grid, whereby a substrate of the grid for mammography would be thinner than one for chest radiology. Instead of coating the walls of the slots, such could be filed with an appropriate liquid, such as mercury.

  14. High order reflectivity of graphite (HOPG) crystals for x ray...

    Office of Scientific and Technical Information (OSTI)

    High order reflectivity of graphite (HOPG) crystals for x ray energies up to 22 keV Citation Details In-Document Search Title: High order reflectivity of graphite (HOPG) crystals...

  15. Lensless Imaging of Magnetic Nanostructures by X-ray Spectro...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    J. Lning, W. F. Schlotter and J. Sthr (SSRL) The unprecedented properties of X-ray free electron lasers (X-FELs) under development world wide will open the door for entirely...

  16. High performance x-ray anti-scatter grid

    DOE Patents [OSTI]

    Logan, C.M.

    1995-05-23

    Disclosed are an x-ray anti-scatter grid for x-ray imaging, particularly for screening mammography, and method for fabricating same, x-rays incident along a direct path pass through a grid composed of a plurality of parallel or crossed openings, microchannels, grooves, or slots etched in a substrate, such as silicon, having the walls of the microchannels or slots coated with a high opacity material, such as gold, while x-rays incident at angels with respect to the slots of the grid, arising from scatter, are blocked. The thickness of the substrate is dependent on the specific application of the grid, whereby a substrate of the grid for mammography would be thinner than one for chest radiology. Instead of coating the walls of the slots, such could be filed with an appropriate liquid, such as mercury. 4 Figs.

  17. Vitreous carbon mask substrate for X-ray lithography

    DOE Patents [OSTI]

    Aigeldinger, Georg; Skala, Dawn M.; Griffiths, Stewart K.; Talin, Albert Alec; Losey, Matthew W.; Yang, Chu-Yeu Peter

    2009-10-27

    The present invention is directed to the use of vitreous carbon as a substrate material for providing masks for X-ray lithography. The new substrate also enables a small thickness of the mask absorber used to pattern the resist, and this enables improved mask accuracy. An alternative embodiment comprised the use of vitreous carbon as a LIGA substrate wherein the VC wafer blank is etched in a reactive ion plasma after which an X-ray resist is bonded. This surface treatment provides a surface enabling good adhesion of the X-ray photoresist and subsequent nucleation and adhesion of the electrodeposited metal for LIGA mold-making while the VC substrate practically eliminates secondary radiation effects that lead to delamination of the X-ray resist form the substrate, the loss of isolated resist features, and the formation of a resist layer adjacent to the substrate that is insoluble in the developer.

  18. X-ray imaging reveals secrets in battery materials | Argonne...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-ray imaging reveals secrets in battery materials June 22, 2015 Tweet EmailPrint Imaging and data analysis techniques offer new approach to probing material properties In a new...

  19. HIgh Rate X-ray Fluorescence Detector

    SciTech Connect (OSTI)

    Grudberg, Peter Matthew

    2013-04-30

    The purpose of this project was to develop a compact, modular multi-channel x-ray detector with integrated electronics. This detector, based upon emerging silicon drift detector (SDD) technology, will be capable of high data rate operation superior to the current state of the art offered by high purity germanium (HPGe) detectors, without the need for liquid nitrogen. In addition, by integrating the processing electronics inside the detector housing, the detector performance will be much less affected by the typically noisy electrical environment of a synchrotron hutch, and will also be much more compact than current systems, which can include a detector involving a large LN2 dewar and multiple racks of electronics. The combined detector/processor system is designed to match or exceed the performance and features of currently available detector systems, at a lower cost and with more ease of use due to the small size of the detector. In addition, the detector system is designed to be modular, so a small system might just have one detector module, while a larger system can have many ?? you can start with one detector module, and add more as needs grow and budget allows. The modular nature also serves to simplify repair. In large part, we were successful in achieving our goals. We did develop a very high performance, large area multi-channel SDD detector, packaged with all associated electronics, which is easy to use and requires minimal external support (a simple power supply module and a closed-loop water cooling system). However, we did fall short of some of our stated goals. We had intended to base the detector on modular, large-area detectors from Ketek GmbH in Munich, Germany; however, these were not available in a suitable time frame for this project, so we worked instead with pnDetector GmbH (also located in Munich). They were able to provide a front-end detector module with six 100 m^2 SDD detectors (two monolithic arrays of three elements each) along with associated preamplifiers; these detectors surpassed the performance we expected to get from the Ketek detectors, however they are housed in a sealed module, which does not offer the ease of repair and expandability we??d hoped to achieve with the Ketek SDD??s. Our packaging efforts were quite successful, as we came up with a very compact way to mount the detector and to house the associated electronics, as well as a very effective way to reliably take out the heat (from the electronics as well as the detector??s Peltier coolers) without risk of condensation and without external airflow or vibration, which could create problems for the target applications. While we were able to design compact processing electronics that fit into the detector assembly, they are still at the prototype stage, and would require a significant redesign to achieve product status. We have not yet tested this detector at a synchrotron facility; we do still plan on working with some close contacts at the nearby Stanford Synchrotron Radiation Laboratory (SSRL) to get some testing with the beam (using existing commercial electronics for readout, as the integrated processor is not ready for use).

  20. Dose optimization in cardiac x-ray imaging

    SciTech Connect (OSTI)

    Gislason-Lee, Amber J.; McMillan, Catherine; Cowen, Arnold R.; Davies, Andrew G.

    2013-09-15

    Purpose: The aim of this research was to optimize x-ray image quality to dose ratios in the cardiac catheterization laboratory. This study examined independently the effects of peak x-ray tube voltage (kVp), copper (Cu), and gadolinium (Gd) x-ray beam filtration on the image quality to radiation dose balance for adult patient sizes.Methods: Image sequences of polymethyl methacrylate (PMMA) phantoms representing two adult patient sizes were captured using a modern flat panel detector based x-ray imaging system. Tin and copper test details were used to simulate iodine-based contrast medium and stents/guide wires respectively, which are used in clinical procedures. Noise measurement for a flat field image and test detail contrast were used to calculate the contrast to noise ratio (CNR). Entrance surface dose (ESD) and effective dose measurements were obtained to calculate the figure of merit (FOM), CNR{sup 2}/dose. This FOM determined the dose efficiency of x-ray spectra investigated. Images were captured with 0.0, 0.1, 0.25, 0.4, and 0.9 mm Cu filtration and with a range of gadolinium oxysulphide (Gd{sub 2}O{sub 2}S) filtration.Results: Optimum x-ray spectra were the same for the tin and copper test details. Lower peak tube voltages were generally favored. For the 20 cm phantom, using 2 Lanex Fast Back Gd{sub 2}O{sub 2}S screens as x-ray filtration at 65 kVp provided the highest FOM considering ESD and effective dose. Considering ESD, this FOM was only marginally larger than that from using 0.4 mm Cu at 65 kVp. For the 30 cm phantom, using 0.25 mm copper filtration at 80 kVp was most optimal; considering effective dose the FOM was highest with no filtration at 65 kVp.Conclusions: These settings, adjusted for x-ray tube loading limits and clinically acceptable image quality, should provide a useful option for optimizing patient dose to image quality in cardiac x-ray imaging. The same optimal x-ray beam spectra were found for both the tin and copper details, suggesting that iodine contrast based imaging and visualization of interventional devices could potentially be optimized for dose using similar x-ray beam spectra.

  1. Self-cleaning rotating anode X-ray source

    DOE Patents [OSTI]

    Paulikas, Arvydas P.

    1989-01-01

    A self-cleaning rotating anode x-ray source comprising an evacuable housing, a rotatable cylindrical anode within the housing, a source of electrons within the housing which electrons are caused to impinge upon the anode to produce x-rays, and means for ionizing residual particles within the housing and accelerating such ions so as to impinge upon the anode to sputter impurities from the surface thereof.

  2. Self-cleaning rotating anode x-ray source

    DOE Patents [OSTI]

    Paulikas, A.P.

    1987-06-02

    A self-cleaning rotating anode x-ray source comprising and evacuable housing, a rotatable cylindrical anode within the housing, a source of electrons within the housing which electrons are caused to impinge upon the anode to produce x-rays, and means for ionizing residual particles within the housing and accelerating such ions so as to impinge upon the anode to sputter impurities from the surface thereof. 2 figs.

  3. Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism Print Using spectroscopic information for magnetometry and magnetic microscopy obviously requires detailed theoretical understanding of spectral shape and magnitude of dichroism signals. A research team at ALS Beamline 4.0.2 has now shown unambiguously that, contrary to common belief, spectral shape and magnitude of x-ray magnetic linear dichroism (XMLD) are not only determined by the relative orientation of magnetic moments and

  4. Polarized X-Rays Reveal Molecular Alignment in Printed Electronics

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Polarized X-Rays Reveal Molecular Alignment in Printed Electronics Polarized X-Rays Reveal Molecular Alignment in Printed Electronics Print Wednesday, 31 October 2012 00:00 The printing of electronic devices using giant roll-to-roll presses or inkjet-style printers has recently been made possible by the development of solution-processable organic materials with optoelectronic properties. Organic light-emitting diodes (OLEDs) are already being produced commercially, and sensors, organic thin-film

  5. ALS X-Rays Shine a New Light on Catalysis

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ALS X-Rays Shine a New Light on Catalysis Print Electrocatalysts are responsible for expediting reactions in many promising renewable energy technologies. However, the extreme sensitivity of their surface redox states to temperatures, to gas pressures, and to electrochemical reaction conditions renders them difficult to investigate by conventional surface-science techniques. Recently a team of Stanford and Berkeley Lab researchers used x-rays at the ALS in a novel way to observe the behavior of

  6. ALS X-Rays Shine a New Light on Catalysis

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ALS X-Rays Shine a New Light on Catalysis Print Electrocatalysts are responsible for expediting reactions in many promising renewable energy technologies. However, the extreme sensitivity of their surface redox states to temperatures, to gas pressures, and to electrochemical reaction conditions renders them difficult to investigate by conventional surface-science techniques. Recently a team of Stanford and Berkeley Lab researchers used x-rays at the ALS in a novel way to observe the behavior of

  7. ALS X-Rays Shine a New Light on Catalysis

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ALS X-Rays Shine a New Light on Catalysis Print Electrocatalysts are responsible for expediting reactions in many promising renewable energy technologies. However, the extreme sensitivity of their surface redox states to temperatures, to gas pressures, and to electrochemical reaction conditions renders them difficult to investigate by conventional surface-science techniques. Recently a team of Stanford and Berkeley Lab researchers used x-rays at the ALS in a novel way to observe the behavior of

  8. ALS X-Rays Shine a New Light on Catalysis

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ALS X-Rays Shine a New Light on Catalysis Print Electrocatalysts are responsible for expediting reactions in many promising renewable energy technologies. However, the extreme sensitivity of their surface redox states to temperatures, to gas pressures, and to electrochemical reaction conditions renders them difficult to investigate by conventional surface-science techniques. Recently a team of Stanford and Berkeley Lab researchers used x-rays at the ALS in a novel way to observe the behavior of

  9. ALS X-Rays Shine a New Light on Catalysis

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ALS X-Rays Shine a New Light on Catalysis ALS X-Rays Shine a New Light on Catalysis Print Thursday, 21 May 2015 11:16 Electrocatalysts are responsible for expediting reactions in many promising renewable energy technologies. However, the extreme sensitivity of their surface redox states to temperatures, to gas pressures, and to electrochemical reaction conditions renders them difficult to investigate by conventional surface-science techniques. Recently a team of Stanford and Berkeley Lab

  10. New focusing multilayer structures for X-ray plasma spectroscopy

    SciTech Connect (OSTI)

    Bibishkin, M S; Luchin, V I; Salashchenko, N N; Chernov, V V; Chkhalo, N I; Kazakov, E D; Shevelko, A P

    2008-02-28

    New focusing short-period multilayer structures are developed which opens up wide possibilities for X-ray and VUV spectroscopy. Multilayer structures are deposited on a flat surface of a mica crystal which is then bent to a small-radius cylinder. The use of this structure in a von Hamos spectrometer for X-ray laser plasma diagnostics is demonstrated. (interaction of laser radiation with matter. laser plasma)

  11. Integrated X-Ray Reflectivity Measurements for Elliptically Curved PET

    Office of Scientific and Technical Information (OSTI)

    Crystals (Conference) | SciTech Connect Integrated X-Ray Reflectivity Measurements for Elliptically Curved PET Crystals Citation Details In-Document Search Title: Integrated X-Ray Reflectivity Measurements for Elliptically Curved PET Crystals Spectroscopy provides valuable information about the temperature and density of a compressed pellet in a plasma. Elliptically curved pentaerythritol (PET) crystals are used as components for spectrometers. Their elliptical geometry gives several

  12. Integrated X-ray Reflectivity Measurements for Elliptically Curved PET

    Office of Scientific and Technical Information (OSTI)

    Crystals (Conference) | SciTech Connect ray Reflectivity Measurements for Elliptically Curved PET Crystals Citation Details In-Document Search Title: Integrated X-ray Reflectivity Measurements for Elliptically Curved PET Crystals The elliptically curved pentaerythritol (PET) crystals used in the Supersnout 2 X-ray spectrometer on the National Ignition Facility (NIF) at Lawrence Livermore National Laboratory (LLNL) have been calibrated photometrically in the range of 5.5 to 16 keV. The

  13. Enabling X-ray free electron laser crystallography for challenging

    Office of Scientific and Technical Information (OSTI)

    biological systems from a limited number of crystals (Journal Article) | SciTech Connect Enabling X-ray free electron laser crystallography for challenging biological systems from a limited number of crystals Citation Details In-Document Search Title: Enabling X-ray free electron laser crystallography for challenging biological systems from a limited number of crystals Authors: Uervirojnangkoorn, Monarin ; Zeldin, Oliver B. ; Lyubimov, Artem Y. ; Hattne, Johan Search SciTech Connect for

  14. Elastic wave velocity measurement combined with synchrotron X-ray

    Office of Scientific and Technical Information (OSTI)

    measurements at high pressure and high temperature conditions: Towards prediction and reproduction of MoHole rocks (Journal Article) | SciTech Connect Elastic wave velocity measurement combined with synchrotron X-ray measurements at high pressure and high temperature conditions: Towards prediction and reproduction of MoHole rocks Citation Details In-Document Search Title: Elastic wave velocity measurement combined with synchrotron X-ray measurements at high pressure and high temperature

  15. Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism Print Using spectroscopic information for magnetometry and magnetic microscopy obviously requires detailed theoretical understanding of spectral shape and magnitude of dichroism signals. A research team at ALS Beamline 4.0.2 has now shown unambiguously that, contrary to common belief, spectral shape and magnitude of x-ray magnetic linear dichroism (XMLD) are not only determined by the relative orientation of magnetic moments and

  16. Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism Print Using spectroscopic information for magnetometry and magnetic microscopy obviously requires detailed theoretical understanding of spectral shape and magnitude of dichroism signals. A research team at ALS Beamline 4.0.2 has now shown unambiguously that, contrary to common belief, spectral shape and magnitude of x-ray magnetic linear dichroism (XMLD) are not only determined by the relative orientation of magnetic moments and

  17. Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism Print Using spectroscopic information for magnetometry and magnetic microscopy obviously requires detailed theoretical understanding of spectral shape and magnitude of dichroism signals. A research team at ALS Beamline 4.0.2 has now shown unambiguously that, contrary to common belief, spectral shape and magnitude of x-ray magnetic linear dichroism (XMLD) are not only determined by the relative orientation of magnetic moments and

  18. Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Unexpected Angular Dependence of X-Ray Magnetic Linear Dichroism Print Using spectroscopic information for magnetometry and magnetic microscopy obviously requires detailed theoretical understanding of spectral shape and magnitude of dichroism signals. A research team at ALS Beamline 4.0.2 has now shown unambiguously that, contrary to common belief, spectral shape and magnitude of x-ray magnetic linear dichroism (XMLD) are not only determined by the relative orientation of magnetic moments and

  19. Using Light to Control How X Rays Interact with Matter

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Using Light to Control How X Rays Interact with Matter Using Light to Control How X Rays Interact with Matter Print Wednesday, 27 January 2010 00:00 Schemes that use one light pulse to manipulate interactions of another with matter are well developed in the visible-light regime where an optical control pulse influences how an optical probe pulse interacts with a medium. This approach has opened new research directions in fields like quantum computing and nonlinear optics, while also spawning

  20. Probing Spatial, Electronic Structures with X-ray Scattering, Spectroscopic

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Techniques | Stanford Synchrotron Radiation Lightsource Probing Spatial, Electronic Structures with X-ray Scattering, Spectroscopic Techniques Wednesday, September 5, 2012 - 10:45am SLAC, Bldg. 137, Room 226 Gang Chen Seminar: Structures at atomic scales are traditionally determined through X-ray crystallography that amplifies scattering intensities by introducing spatial periodicity. For amorphous materials and many macromolecules, such as viruses, proteins and biofilms, it is hard to

  1. 15.05.29 RH Operando X-ray - JCAP

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Direct Observation of a Semiconductor/Liquid Junction by Operando X-Ray Photoelectron Spectroscopy (XPS) Lichterman , M. F. et al. Direct Observation of the Energetics at a Semiconductor/Liquid Junction by Operando X-Ray Photoelectron Spectroscopy. Energy Environ. Sci ., 2015, DOI: 10.1039/C5EE01014D (2015). Scientific Achievement We demonstrated that the operando XPS technique, applied to a semiconductor/liquid junction, can directly measure the positions of the electronic states of the

  2. NREL: Measurements and Characterization - X-Ray and UV Photoelectron

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Spectroscopy X-Ray and UV Photoelectron Spectroscopy Example of graph made with cluster tool; plots counts (Y-axis) vs. binding energy (X-axis) for PET Carbon 1S. High-resolution XPS spectra of carbon 1s from polyethylene terephthalate backsheet material, showing excellent quantitative agreement between measured and predicted peak area ratios. Subtle differences in polymer functionality are assessed by deviations from stoichiometry. In photoemission techniques, we use either X-rays or

  3. ALS X-Rays Shine a New Light on Catalysis

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ALS X-Rays Shine a New Light on Catalysis Print Electrocatalysts are responsible for expediting reactions in many promising renewable energy technologies. However, the extreme sensitivity of their surface redox states to temperatures, to gas pressures, and to electrochemical reaction conditions renders them difficult to investigate by conventional surface-science techniques. Recently a team of Stanford and Berkeley Lab researchers used x-rays at the ALS in a novel way to observe the behavior of

  4. ALS X-Rays Shine a New Light on Catalysis

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ALS X-Rays Shine a New Light on Catalysis Print Electrocatalysts are responsible for expediting reactions in many promising renewable energy technologies. However, the extreme sensitivity of their surface redox states to temperatures, to gas pressures, and to electrochemical reaction conditions renders them difficult to investigate by conventional surface-science techniques. Recently a team of Stanford and Berkeley Lab researchers used x-rays at the ALS in a novel way to observe the behavior of

  5. New Directions in X-Ray Light Sources

    ScienceCinema (OSTI)

    Falcone, Roger

    2010-01-08

    July 15, 2008 Berkeley Lab lecture: Molecular movies of chemical reactions and material phase transformations need a strobe of x-rays, the penetrating light that reveals how atoms and molecules assemble in chemical and biological systems and complex materials. Roger Falcone, Director of the Advanced Light Source,will discuss a new generation of x ray sources that will enable a new science of atomic dynamics on ultrafast timescales.

  6. X-ray tube with magnetic electron steering

    DOE Patents [OSTI]

    Reed, Kim W. (Albuquerque, NM); Turman, Bobby N. (Albuquerque, NM); Kaye, Ronald J. (Albuquerque, NM); Schneider, Larry X. (Albuquerque, NM)

    2000-01-01

    An X-ray tube uses a magnetic field to steer electrons. The magnetic field urges electrons toward the anode, increasing the proportion of electrons emitted from the cathode that reach desired portions of the anode and consequently contribute to X-ray production. The magnetic field also urges electrons reflected from the anode back to the anode, further increasing the efficiency of the tube.

  7. X-ray transient absorption and picosecond IR spectroscopy of

    Office of Scientific and Technical Information (OSTI)

    fulvalene(tetracarbonyl)diruthenium on photoexcitation (Journal Article) | SciTech Connect X-ray transient absorption and picosecond IR spectroscopy of fulvalene(tetracarbonyl)diruthenium on photoexcitation Citation Details In-Document Search Title: X-ray transient absorption and picosecond IR spectroscopy of fulvalene(tetracarbonyl)diruthenium on photoexcitation Authors: Harpham, M. R. ; Nguyen, S. C. ; Hou, Z. ; Grossman, J. C. ; Harris, C. B. ; Mara, M. W. ; Stickrath, A. B. ; Kanai, Y. ;

  8. X-Ray Characterization of Diesel Sprays | Department of Energy

    Broader source: Energy.gov (indexed) [DOE]

    5 Diesel Engine Emissions Reduction (DEER) Conference Presentations and Posters PDF icon 2005_deer_powell.pdf More Documents & Publications X-Ray Characterization of Diesel Sprays and the Effects of Nozzle Geometry Ultrafast X-ray Phase-Enhanced Microimaging for Visualizing Fuel Injection Process and Diesel Sprays Integrated Nozzle Flow, Spray, Combustion, & Emission Modeling using KH-ACT Primary Breakup Model & Detailed Chemistry

  9. Internal energy dissipation of gamma-ray bursts observed with Swift: Precursors, prompt gamma-rays, extended emission, and late X-ray flares

    SciTech Connect (OSTI)

    Hu, You-Dong; Liang, En-Wei; Xi, Shao-Qiang; Peng, Fang-Kun; Lu, Rui-Jing; L, Lian-Zhong [Department of Physics and GXU-NAOC Center for Astrophysics and Space Sciences, Guangxi University, Nanning 530004 (China); Zhang, Bing, E-mail: lew@gxu.edu.cn, E-mail: Zhang@physics.unlv.edu [Department of Physics and Astronomy, University of Nevada, Las Vegas, NV 89154 (United States)

    2014-07-10

    We jointly analyze the gamma-ray burst (GRB) data observed with Burst Alert Telescope (BAT) and X-ray Telescope on board the Swift mission to present a global view on the internal energy dissipation processes in GRBs, including precursors, prompt gamma-ray emission, extended soft gamma-ray emission, and late X-ray flares. The Bayesian block method is utilized to analyze the BAT light curves to identify various emission episodes. Our results suggest that these emission components likely share the same physical origin, which is the repeated activation of the GRB central engine. What we observe in the gamma-ray band may be a small part of more extended underlying activities. The precursor emission, which is detected in about 10% of Swift GRBs, is preferably detected in those GRBs that have a massive star core-collapse origin. The soft extended emission tail, on the other hand, is preferably detected in those GRBs that have a compact star merger origin. Bright X-ray emission is detected during the BAT quiescent phases prior to subsequent gamma-ray peaks, implying that X-ray emission may be detectable prior the BAT trigger time. Future GRB alert instruments with soft X-ray capability are essential for revealing the early stages of GRB central engine activities, and shedding light on jet composition and the jet launching mechanism in GRBs.

  10. A New Scheme for Stigmatic X-ray Imaging with Large Magnification...

    Office of Scientific and Technical Information (OSTI)

    F; Beiersdorfer, P; Wang, E; Sanchez del Rio, M; Caughey, T A 70 PLASMA PHYSICS AND FUSION TECHNOLOGY X-ray Imaging X-ray Imaging This paper describes a new x-ray scheme for...

  11. Evaluation of partial coherence correction in X-ray ptychography

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Burdet, Nicolas; Shi, Xiaowen; Parks, Daniel; Clark, Jesse N.; Huang, Xiaojing; Kevan, Stephen D.; Robinson, Ian K.

    2015-02-23

    Coherent X-ray Diffraction Imaging (CDI) and X-ray ptychography both heavily rely on the high degree of spatial coherence of the X-ray illumination for sufficient experimental data quality for reconstruction convergence. Nevertheless, the majority of the available synchrotron undulator sources have a limited degree of partial coherence, leading to reduced data quality and a lower speckle contrast in the coherent diffraction patterns. It is still an open question whether experimentalists should compromise the coherence properties of an X-ray source in exchange for a higher flux density at a sample, especially when some materials of scientific interest are relatively weak scatterers. Amoreprevious study has suggested that in CDI, the best strategy for the study of strong phase objects is to maintain a high degree of coherence of the illuminating X-rays because of the broadening of solution space resulting from the strong phase structures. In this article, we demonstrate the first systematic analysis of the effectiveness of partial coherence correction in ptychography as a function of the coherence properties, degree of complexity of illumination (degree of phase diversity of the probe) and sample phase complexity. We have also performed analysis of how well ptychographic algorithms refine X-ray probe and complex coherence functions when those variables are unknown at the start of reconstructions, for noise-free simulated data, in the case of both real-valued and highly-complex objects.less

  12. Normal incidence X-ray mirror for chemical microanalysis

    DOE Patents [OSTI]

    Carr, Martin J. (Tijeras, NM); Romig, Jr., Alton D. (Albuquerque, NM)

    1990-01-01

    A non-planar, focusing mirror, to be utilized in both electron column instruments and micro-x-ray fluorescence instruments for performing chemical microanalysis on a sample, comprises a concave, generally spherical base substrate and a predetermined number of alternating layers of high atomic number material and low atomic number material contiguously formed on the base substrate. The thickness of each layer is an integral multiple of the wavelength being reflected and may vary non-uniformly according to a predetermined design. The chemical analytical instruments in which the mirror is used also include a predetermined energy source for directing energy onto the sample and a detector for receiving and detecting the x-rays emitted from the sample; the non-planar mirror is located between the sample and detector and collects the x-rays emitted from the sample at a large solid angle and focuses the collected x-rays to the sample. For electron column instruments, the wavelengths of interest lie above 1.5 nm, while for x-ray fluorescence instruments, the range of interest is below 0.2 nm. Also, x-ray fluorescence instruments include an additional non-planar focusing mirror, formed in the same manner as the previously described m The invention described herein was made in the performance of work under contract with the Department of Energy, Contract No. DE-AC04-76DP00789, and the United States Government has rights in the invention pursuant to this contract.

  13. Preparation and in situ Characterization of Surfaces Using Soft-Landing in a Fourier Transform Ion Cyclotron Resonance Mass Spectrometer

    SciTech Connect (OSTI)

    Alvarez, Jormarie; Cooks, Robert G.; Barlow, Stephan E.; Gaspar, Dan J.; Futrell, Jean H.; Laskin, Julia

    2005-06-01

    Mass-selected peptide ions produced by electrospray ionization were deposited onto fluorinated self-assembled monolayer surfaces (FSAM) surfaces by soft-landing using a Fourier transform ion cyclotron resonance mass spectrometer (FT-ICR MS) specially designed for studying interactions of large ions with surfaces. Analysis of the modified surface was performed in situ by combining 2 keV Cs+ secondary ion mass spectrometry with FT-ICR detection of the sputtered ions (FT-ICR-SIMS). Regardless of the initial charge state of the precursor ion, the SIMS mass spectra included singly-protonated peptide fragment ions and peaks characteristic of the surfaces in all cases. In some experiments multiply-protonated peptide ions and [M+Au]+ ions were also observed upon SIMS analysis of modified surfaces. For comparison with the in situ analysis of the modified surfaces, ex situ analysis of some of the modified surfaces was performed by 25 kV Ga+ time of flight ? secondary ion mass spectrometry (ToF-SIMS). The ex situ analysis demonstrated that a significant number of soft-landed peptide ions remain charged on the surface even when exposed to air for several hours after deposition. Charge retention of soft-landed ions dramatically increases the ion yields obtained during SIMS analysis very sensitive detection of deposited material at less than 1% of monolayer coverage. Accumulation of charged species on the surface undergoes saturation due to Coulomb repulsion between charges at close to 30% coverage. We estimated that close to 1 ng of peptide could be deposited on the spot area of 4 mm2 of the FSAM surface without reaching saturation.

  14. Johann Spectrometer for High Resolution X-ray Spectroscopy

    SciTech Connect (OSTI)

    Machek, Pavel; Froeba, Michael; Welter, Edmund; Caliebe, Wolfgang; Brueggmann, Ulf; Draeger, Guenter

    2007-01-19

    A newly designed vacuum Johann spectrometer with a large focusing analyzer crystal for inelastic x-ray scattering and high resolution fluorescence spectroscopy has been installed at the DORIS III storage ring. Spherically bent crystals with a maximum diameter of 125 mm, and cylindrically bent crystals are employed as dispersive optical elements. Standard radius of curvature of the crystals is 1000 mm, however, the design of the mechanical components also facilitates measurements with smaller and larger bending radii. Up to four crystals are mounted on a revolving crystal changer which enables crystal changes without breaking the vacuum. The spectrometer works at fixed Bragg angle. It is preferably designed for the measurements in non-scanning mode with a broad beam spot, and offers a large flexibility to set the sample to the optimum position inside the Rowland circle. A deep depletion CCD camera is employed as a position sensitive detector to collect the energy-analyzed photons on the circumference of the Rowland circle. The vacuum in the spectrometer tank is typically 10-6 mbar. The sample chamber is separated from the tank either by 25 {mu}m thick Kapton windows, which allows samples to be measured under ambient conditions, or by two gate valves. The spectrometer is currently installed at wiggler beamline W1 whose working range is 4-10.5 keV with typical flux at the sample of 5x1010photons/s/mm2. The capabilities of the spectrometer are illustrated by resonant inelastic experiments on 3d transition metals and rare earth compounds, and by chemical shift measurements on chromium compounds.

  15. Achieving hard X-ray nanofocusing using a wedged multilayer Laue...

    Office of Scientific and Technical Information (OSTI)

    anticipate that continuous development on wedged MLLs will advance x-ray nanofocusing optics to new frontiers and enrich capabilities and opportunities for hard X-ray microscopy....

  16. Proposed New Accelerator Design for Homeland Security X-Ray Applicatio...

    Office of Scientific and Technical Information (OSTI)

    Proposed New Accelerator Design for Homeland Security X-Ray Applications Citation Details In-Document Search Title: Proposed New Accelerator Design for Homeland Security X-Ray...

  17. Proposed New Accelerator Design for Homeland Security X-Ray Applicatio...

    Office of Scientific and Technical Information (OSTI)

    Proposed New Accelerator Design for Homeland Security X-Ray Applications Citation Details In-Document Search Title: Proposed New Accelerator Design for Homeland Security X-Ray ...

  18. Towards three-dimensional and attosecond x-ray imaging at the...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    x-ray wavelength appears desirable to achieve maximal spatial resolution in x-ray diffraction experiments, longer wavelengths turns out to enable the identification of...

  19. Ultrafast X-ray Phase-Enhanced Microimaging for Visualizing Fuel...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Ultrafast X-ray Phase-Enhanced Microimaging for Visualizing Fuel Injection Process and Diesel Sprays Ultrafast X-ray Phase-Enhanced Microimaging for Visualizing Fuel Injection ...

  20. X-Ray Diffraction > Analytical Resources > Research > The Energy Materials

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Center at Cornell Analytical Resources In This Section Differential Electrochemical Mass Spectroscopy (DEMS) Electron Microscopy X-Ray Diffraction X-Ray Diffraction