National Library of Energy BETA

Sample records for research aerosol properties

  1. ARM - AOS Aerosol Properties Plots

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    XDC Data Viewers Aerosol Properties Plots SGP AMF NSA (BRW) AOS Aerosol Properties Plots ... are raw unedited data. Do not quote and cite. Aerosol Properties Plots SGP AMF NSA (BRW)

  2. ARM - Measurement - Aerosol optical properties

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    : Aerosol optical properties The optical properties of aerosols, including asymmetry factor, phase-function, single-scattering albedo, refractive index, and backscatter...

  3. Understanding the Effect of Aerosol Properties on Cloud Droplet...

    Office of Scientific and Technical Information (OSTI)

    5-055 ENERGY Science Understanding the Effect of Aerosol Properties on Cloud Droplet Formation during TCAP Field Campaign Report D Cziczo May 2016 ARM CLIMATE RESEARCH FACILITY ...

  4. Aerosol Properties Downwind of Biomass Burns Field Campaign Report

    Office of Scientific and Technical Information (OSTI)

    Science Aerosol Properties Downwind of Biomass Burns Field Campaign Report PR Buseck ... DOESC-ARM-15-076 Aerosol Properties Downwind of Biomass Burns Field Campaign Report PR ...

  5. Final Technical Report for Interagency Agreement No. DE-SC0005453 “Characterizing Aerosol Distributions, Types, and Optical and Microphysical Properties using the NASA Airborne High Spectral Resolution Lidar (HSRL) and the Research Scanning Polarimeter (RSP)”

    SciTech Connect (OSTI)

    Hostetler, Chris; Ferrare, Richard

    2015-01-13

    Measurements of the vertical profile of atmospheric aerosols and aerosol optical and microphysical characteristics are required to: 1) determine aerosol direct and indirect radiative forcing, 2) compute radiative flux and heating rate profiles, 3) assess model simulations of aerosol distributions and types, and 4) establish the ability of surface and space-based remote sensors to measure the indirect effect. Consequently the ASR program calls for a combination of remote sensing and in situ measurements to determine aerosol properties and aerosol influences on clouds and radiation. As part of our previous DOE ASP project, we deployed the NASA Langley airborne High Spectral Resolution Lidar (HSRL) on the NASA B200 King Air aircraft during major field experiments in 2006 (MILAGRO and MaxTEX), 2007 (CHAPS), 2009 (RACORO), and 2010 (CalNex and CARES). The HSRL provided measurements of aerosol extinction (532 nm), backscatter (532 and 1064 nm), and depolarization (532 and 1064 nm). These measurements were typically made in close temporal and spatial coincidence with measurements made from DOE-funded and other participating aircraft and ground sites. On the RACORO, CARES, and CalNEX missions, we also deployed the NASA Goddard Institute for Space Studies (GISS) Research Scanning Polarimeter (RSP). RSP provided intensity and degree of linear polarization over a broad spectral and angular range enabling column-average retrievals of aerosol optical and microphysical properties. Under this project, we analyzed observations and model results from RACORO, CARES, and CalNex and accomplished the following objectives. 1. Identified aerosol types, characterize the vertical distribution of the aerosol types, and partition aerosol optical depth by type, for CARES and CalNex using HSRL data as we have done for previous missions. 2. Investigated aerosol microphysical and macrophysical properties using the RSP. 3. Used the aerosol backscatter and extinction profiles measured by the HSRL

  6. ARM - Field Campaign - MASRAD: Marine Aerosol Properties

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsMASRAD: Marine Aerosol Properties Campaign Links AMF Point Reyes Website Comments? We would love to hear from you Send us a note below or call us at 1-888-ARM-DATA....

  7. ARM - Field Campaign - MASRAD - Aerosol Optical Properties

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsMASRAD - Aerosol Optical Properties Campaign Links AMF Point Reyes Website ARM Data Discovery Browse Data Related Campaigns MArine Stratus Radiation Aerosol and Drizzle (MASRAD) IOP 2005.03.14, Miller, AMF Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : MASRAD - Aerosol Optical Properties 2005.06.29 - 2005.08.30 Lead Scientist : Anthony Strawa For data sets, see below. Abstract Principal Investigators: J. Ogren, C.

  8. ARM AOS Processing Status and Aerosol Intensive Properties VAP

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AOS Processing Status and Aerosol Intensive Properties VAP A. S. Koontz and C. J. Flynn Pacific Northwest National Laboratory Richland, Washington J. A. Ogren, E. Andrews, and P....

  9. "Lidar Investigations of Aerosol, Cloud, and Boundary Layer Properties...

    Office of Scientific and Technical Information (OSTI)

    Technical Report: "Lidar Investigations of Aerosol, Cloud, and Boundary Layer Properties Over the ARM ACRF Sites" Citation Details In-Document Search Title: "Lidar Investigations ...

  10. ARM - Field Campaign - Cirrus Clouds and Aerosol Properties Campaign

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lead Scientist : Shadrian Strong For data sets, see below. Abstract Through the National Geospatial-Intelligence Agency Characterization of Cirrus and Aerosol Properties (CCAP) ...

  11. Evaluating Global Aerosol Models and Aerosol and Water Vapor Properties Near Clouds

    SciTech Connect (OSTI)

    Richard A. Ferrare; David D. Turner

    2011-09-01

    Project goals: (1) Use the routine surface and airborne measurements at the ARM SGP site, and the routine surface measurements at the NSA site, to continue our evaluations of model aerosol simulations; (2) Determine the degree to which the Raman lidar measurements of water vapor and aerosol scattering and extinction can be used to remotely characterize the aerosol humidification factor; (3) Use the high temporal resolution CARL data to examine how aerosol properties vary near clouds; and (4) Use the high temporal resolution CARL and Atmospheric Emitted Radiance Interferometer (AERI) data to quantify entrainment in optically thin continental cumulus clouds.

  12. Evaluating Global Aerosol Models and Aerosol and Water Vapor Properties Near Clouds

    SciTech Connect (OSTI)

    Turner, David, D.; Ferrare, Richard, A.

    2011-07-06

    The 'Evaluating Global Aerosol Models and Aerosol and Water Vapor Properties Near Clouds' project focused extensively on the analysis and utilization of water vapor and aerosol profiles derived from the ARM Raman lidar at the Southern Great Plains ARM site. A wide range of different tasks were performed during this project, all of which improved quality of the data products derived from the lidar or advanced the understanding of atmospheric processes over the site. These activities included: upgrading the Raman lidar to improve its sensitivity; participating in field experiments to validate the lidar aerosol and water vapor retrievals; using the lidar aerosol profiles to evaluate the accuracy of the vertical distribution of aerosols in global aerosol model simulations; examining the correlation between relative humidity and aerosol extinction, and how these change, due to horizontal distance away from cumulus clouds; inferring boundary layer turbulence structure in convective boundary layers from the high-time-resolution lidar water vapor measurements; retrieving cumulus entrainment rates in boundary layer cumulus clouds; and participating in a field experiment that provided data to help validate both the entrainment rate retrievals and the turbulent profiles derived from lidar observations.

  13. Connecting Organic Aerosol Climate-Relevant Properties to Chemical Mechanisms of Sources and Processing

    SciTech Connect (OSTI)

    Thornton, Joel

    2015-01-26

    The research conducted on this project aimed to improve our understanding of secondary organic aerosol (SOA) formation in the atmosphere, and how the properties of the SOA impact climate through its size, phase state, and optical properties. The goal of this project was to demonstrate that the use of molecular composition information to mechanistically connect source apportionment and climate properties can improve the physical basis for simulation of SOA formation and properties in climate models. The research involved developing and improving methods to provide online measurements of the molecular composition of SOA under atmospherically relevant conditions and to apply this technology to controlled simulation chamber experiments and field measurements. The science we have completed with the methodology will impact the simulation of aerosol particles in climate models.

  14. Characterizing Aerosol Distributions and Optical Properties Using the NASA Langley High Spectral Resolution Lidar

    SciTech Connect (OSTI)

    Hostetler, Chris; Ferrare, Richard

    2013-02-14

    The objective of this project was to provide vertically and horizontally resolved data on aerosol optical properties to assess and ultimately improve how models represent these aerosol properties and their impacts on atmospheric radiation. The approach was to deploy the NASA Langley Airborne High Spectral Resolution Lidar (HSRL) and other synergistic remote sensors on DOE Atmospheric Science Research (ASR) sponsored airborne field campaigns and synergistic field campaigns sponsored by other agencies to remotely measure aerosol backscattering, extinction, and optical thickness profiles. Synergistic sensors included a nadir-viewing digital camera for context imagery, and, later in the project, the NASA Goddard Institute for Space Studies (GISS) Research Scanning Polarimeter (RSP). The information from the remote sensing instruments was used to map the horizontal and vertical distribution of aerosol properties and type. The retrieved lidar parameters include profiles of aerosol extinction, backscatter, depolarization, and optical depth. Products produced in subsequent analyses included aerosol mixed layer height, aerosol type, and the partition of aerosol optical depth by type. The lidar products provided vertical context for in situ and remote sensing measurements from other airborne and ground-based platforms employed in the field campaigns and was used to assess the predictions of transport models. Also, the measurements provide a data base for future evaluation of techniques to combine active (lidar) and passive (polarimeter) measurements in advanced retrieval schemes to remotely characterize aerosol microphysical properties. The project was initiated as a 3-year project starting 1 January 2005. It was later awarded continuation funding for another 3 years (i.e., through 31 December 2010) followed by a 1-year no-cost extension (through 31 December 2011). This project supported logistical and flight costs of the NASA sensors on a dedicated aircraft, the subsequent

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Broadband Albedo Observations in the Southern Great Plains Submitter: Lamb, P. J., University of Oklahoma Area of Research: Aerosol Properties Working Group(s): Aerosol Journal...

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Nucleation Events Download a printable PDF Submitter: McMurry, P. ., University of Minnesota Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal ...

  17. Observed correlations between aerosol and cloud properties in an Indian Ocean trade cumulus regime

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Pistone, Kristina; Praveen, Puppala S.; Thomas, Rick M.; Ramanathan, Veerabhadran; Wilcox, Eric M.; Bender, Frida A.-M.

    2016-04-27

    There are many contributing factors which determine the micro- and macrophysical properties of clouds, including atmospheric vertical structure, dominant meteorological conditions, and aerosol concentration, all of which may be coupled to one another. In the quest to determine aerosol effects on clouds, these potential relationships must be understood. Here we describe several observed correlations between aerosol conditions and cloud and atmospheric properties in the Indian Ocean winter monsoon season.In the CARDEX (Cloud, Aerosol, Radiative forcing, Dynamics EXperiment) field campaign conducted in February and March 2012 in the northern Indian Ocean, continuous measurements were made of atmospheric precipitable water vapor (PWV)more » and the liquid water path (LWP) of trade cumulus clouds, concurrent with measurements of water vapor flux, cloud and aerosol vertical profiles, meteorological data, and surface and total-column aerosol from instrumentation at a ground observatory and on small unmanned aircraft. We present observations which indicate a positive correlation between aerosol and cloud LWP only when considering cases with low atmospheric water vapor (PWV < 40 kg m–2), a criterion which acts to filter the data to control for the natural meteorological variability in the region.We then use the aircraft and ground-based measurements to explore possible mechanisms behind this observed aerosol–LWP correlation. The increase in cloud liquid water is found to coincide with a lowering of the cloud base, which is itself attributable to increased boundary layer humidity in polluted conditions. High pollution is found to correlate with both higher temperatures and higher humidity measured throughout the boundary layer. A large-scale analysis, using satellite observations and meteorological reanalysis, corroborates these covariations: high-pollution cases are shown to originate as a highly polluted boundary layer air mass approaching the observatory from a

  18. FY 2010 Fourth Quarter Report: Evaluation of the Dependency of Drizzle Formation on Aerosol Properties

    SciTech Connect (OSTI)

    Lin, W; McGraw, R; Liu, Y; Wang, J; Vogelmann, A; Daum, PH

    2010-10-01

    Metric for Quarter 4: Report results of implementation of composite parameterization in single-column model (SCM) to explore the dependency of drizzle formation on aerosol properties. To better represent VOCALS conditions during a test flight, the Liu-Duam-McGraw (LDM) drizzle parameterization is implemented in the high-resolution Weather Research and Forecasting (WRF) model, as well as in the single-column Community Atmosphere Model (CAM), to explore this dependency.

  19. Optical Properties of Mixed Black Carbon, Inorganic and Secondary Organic Aerosols

    SciTech Connect (OSTI)

    Paulson, S E

    2012-05-30

    Summarizes the achievements of the project, which are divided into four areas: 1) Optical properties of secondary organic aerosols; 2) Development and of a polar nephelometer to measure aerosol optical properties and theoretical approaches to several optical analysis problems, 3) Studies on the accuracy of measurements of absorbing carbon by several methods, and 4) Environmental impacts of biodiesel.

  20. An AeroCom Initial Assessment - Optical Properties in Aerosol...

    Office of Scientific and Technical Information (OSTI)

    Since not only aot but also aab influence the aerosol impact on the radiative energy-balance, aerosol (direct) forcing uncertainty in modeling is larger than differences in aot ...

  1. Investigation of Absorption Properties of Submicron Aerosol in the Troposphere Over West Siberia

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Investigation of Absorption Properties of Submicron Aerosol in the Troposphere Over West Siberia M. V. Panchenko, V. S. Kozlov, and V. P. Shmargunov Institute of Atmospheric Optics Tomsk, Russia Introduction Improving radiative climate models for the cloudless atmosphere depends largely on the correct way to simulate single-scattering albedo of atmospheric aerosol. Solving this problem requires performing detailed experiments on the study of the aerosol absorption characteristics in the

  2. Aerosol Properties from Multi-spectral and Multi-angular Aircraft 4STAR Observations: Expected Advantages and Challenges

    SciTech Connect (OSTI)

    Kassianov, Evgueni I.; Flynn, Connor J.; Redemann, Jens; Schmid, Beat; Russell, P. B.; Sinyuk, Alexander

    2012-11-01

    The airborne Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR) is developed to retrieve aerosol microphysical and optical properties from multi-angular and multi-spectral measurements of sky radiance and direct-beam sun transmittance. The necessarily compact design of the 4STAR may cause noticeable apparent enhancement of sky radiance at small scattering angles. We assess the sensitivity of expected 4STAR-based aerosol retrieval to such enhancement by applying the operational AERONET retrieval code and constructed synthetic 4STARlike data. Also, we assess the sensitivity of the broadband fluxes and the direct aerosol radiative forcing to uncertainties in aerosol retrievals associated with the sky radiance enhancement. Our sensitivity study results suggest that the 4STARbased aerosol retrieval has limitations in obtaining detailed information on particle size distribution and scattering phase function. However, these limitations have small impact on the retrieved bulk optical parameters, such as the asymmetry factor (up to 4%, or 0.02) and single-scattering albedo (up to 2%, or 0.02), and the calculated direct aerosol radiative forcing (up to 6%, or 2 Wm-2).

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    First Observation-Based Estimates of Cloud-Free Aerosol Radiative Forcing Across China Download a printable PDF Submitter: Li, Z., University of Maryland Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: N/A Mean annual shortwave aerosol radiative forcing (SWARF) averaged across China. Spatial variation of the annual mean SW aerosol radiative forcing. Heavy loading of aerosols in China is widely known, but little is known about their impact on regional

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Experiment Results Featured in Technical Journal Submitter: Sheridan, P., U.S. Department of Commerce/NOAA Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Sheridan, P, W Arnott, J Ogren, E Andrews, D Atkinson, D Covert, H Moosmuller, A Petzold, B Schmid, A Strawa, R Varma, and A Virkkula. 2005. "The Reno Aerosol Optics Study: An evaluation of aerosol absorption measurement methods." Aerosol Science and Technology 39(1):1-16. This magnification

  5. Quantification of black carbon mixing state from traffic: Implications for aerosol optical properties

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Willis, Megan D.; Healy, Robert M.; Riemer, Nicole; West, Matthew; Wang, Jon M.; Jeong, Cheol -Heon; Wenger, John C.; Evans, Greg J.; Abbatt, Jonathan P. D.; Lee, Alex K. Y.

    2016-04-14

    The climatic impacts of black carbon (BC) aerosol, an important absorber of solar radiation in the atmosphere, remain poorly constrained and are intimately related to its particle-scale physical and chemical properties. Using particle-resolved modelling informed by quantitative measurements from a soot-particle aerosol mass spectrometer, we confirm that the mixing state (the distribution of co-emitted aerosol amongst fresh BC-containing particles) at the time of emission significantly affects BC-aerosol optical properties even after a day of atmospheric processing. Both single particle and ensemble aerosol mass spectrometry observations indicate that BC near the point of emission co-exists with hydrocarbon-like organic aerosol (HOA) inmore » two distinct particle types: HOA-rich and BC-rich particles. The average mass fraction of black carbon in HOA-rich and BC-rich particle classes was  < 0.1 and 0.8, respectively. Notably, approximately 90 % of BC mass resides in BC-rich particles. This new measurement capability provides quantitative insight into the physical and chemical nature of BC-containing particles and is used to drive a particle-resolved aerosol box model. Lastly, significant differences in calculated single scattering albedo (an increase of 0.1) arise from accurate treatment of initial particle mixing state as compared to the assumption of uniform aerosol composition at the point of BC injection into the atmosphere.« less

  6. “Lidar Investigations of Aerosol, Cloud, and Boundary Layer Properties Over the ARM ACRF Sites”

    SciTech Connect (OSTI)

    Ferrare, Richard; Turner, David

    2015-01-13

    Project goals; Characterize the aerosol and ice vertical distributions over the ARM NSA site, and in particular to discriminate between elevated aerosol layers and ice clouds in optically thin scattering layers; Characterize the water vapor and aerosol vertical distributions over the ARM Darwin site, how these distributions vary seasonally, and quantify the amount of water vapor and aerosol that is above the boundary layer; Use the high temporal resolution Raman lidar data to examine how aerosol properties vary near clouds; Use the high temporal resolution Raman lidar and Atmospheric Emitted Radiance Interferometer (AERI) data to quantify entrainment in optically thin continental cumulus clouds; and Use the high temporal Raman lidar data to continue to characterize the turbulence within the convective boundary layer and how the turbulence statistics (e.g., variance, skewness) is correlated with larger scale variables predicted by models.

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ARM Program Surface Measurements for Aerosol Profiles Shown to Represent Integrated Column Measurements Submitter: Andrews, E., University of Colorado Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Andrews, E., P. J. Sheridan, J. A. Ogren, and R. Ferrare (2004), In situ aerosol profiles over the Southern Great Plains cloud and radiation test bed site: 1. Aerosol optical properties, J. Geophys. Res., 109, D06208, doi:10.1029/2003JD004025. Delle Monache, L., K.

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MBL Aerosol Properties and Their Impact on CCN at the Azores-AMF Site Download a printable PDF Submitter: Dong, X., University of Arizona Area of Research: Aerosol Properties Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Logan T, B Xi, and X Dong. 2014. "Aerosol properties and their influences on marine boundary layer cloud condensation nuclei at the ARM mobile facility over the Azores." Journal of Geophysical Research - Atmospheres, 119(8),

  9. Wind-dependent desert aerosol model: radiative properties. Technical report, November 1986-April 1988

    SciTech Connect (OSTI)

    Longtin, D.R.; Shettle, E.P.; Hummel, J.R.; Pryce, J.D.

    1988-04-19

    This report presents a desert aerosol model that predicts aerosol radiative properties during background and severe dust-storm conditions. The model treats the desert aerosol as an external mixture of natural carbon, water soluble, and sand particles. The sand consists of two kinds of particles, pure quartz and quartz contaminated with a small amount of hematite. Mie calculations are performed using different size distributions and indices of refraction for each type of particle, and then a volume-weighting scheme is used to obtain the radiative properties of the aerosol as a whole. Attenuation coefficients, single scattering albedo, and asymmetry parameter are given for 68 wavelengths between 0.2 and 300 micro. The results indicate that extinction is wavelength-dependent for background conditions, but increases and becomes nearly constant for dust-storm conditions.

  10. Collaborative research. Study of aerosol sources and processing at the GVAX Pantnagar Supersite

    SciTech Connect (OSTI)

    Worsnop, Doug; Volkamer, Rainer

    2012-08-13

    The Two Column Aerosol Project (TCAP) investigated uncertainties in the aerosol direct effect in the northern hemisphere mid-latitudes. The University of Colorado 2D-MAX-DOAS and LED-CE-DOAS instruments were collocated with DOE’s Atmospheric Radiation Measurement (ARM) Mobile Facility (AMF) and Mobile Aerosol Observing System (MAOS) during the TCAP-1 campaign at Cape Cod, MA (1 July to 13 August 2012). We have performed atmospheric radiation closure studies to evaluate the use of a novel parameter, i.e., the Raman Scattering Probability (RSP). We have performed first measurements of RSP almucantar scans, and measure RSP in spectra of scattered solar photons at 350nm and 430nm. Radiative Transfer Modelling of RSP demonstrate that the RSP measurement is maximally sensitive to infer even extremely low aerosol optical depth (AOD < 0.01) reliably by DOAS at low solar relative azimuth angles. We further assess the role of elevated aerosol layers on near surface observations of oxygen collision complexes, O 2-O2. Elevated aerosol layers modify the near surface absorption of O2-O2 and RSP. The combination of RSP and O2-O2 holds largely unexplored potential to better constrain elevated aerosol layers and measure column aerosol optical properties such as aerosol effective radius, extinction, aerosol phase functions and refractive indices. The TCAP deployment also provides a time series of reactive trace gas vertical profiles, i.e., nitrogen dioxide (NO2) and glyoxal (C2H2O2), which are measured simultaneously with the aerosol optical properties by DOAS. NO2 is an important precursor for ozone (O3) that modifies oxidative capacity. Glyoxal modifies oxidative capacity and is a source for brown carbon by forming secondary organic aerosol (SOA) via multiphase reactions in aerosol and cloud water. We have performed field measurements of these gases

  11. COLLABORATIVE RESEARCH: Study of Aerosol Sources and Processing at the GVAX Pantnagar Supersite

    SciTech Connect (OSTI)

    Worsnop, Douglas R.

    2014-07-28

    This project funded the participation of scientists from seven research groups, running more than thirty instruments, in the Winter Intensive Operating Period (January-February 2012) of the Clean Air for London (ClearfLo) campaign at a rural site in Detling, UK, 45 km southeast of central London. The primary science questions for the ClearfLo Winter IOP were, 1) what is the urban increment of particulate matter (PM) and other pollutants in the greater London area, and, 2) what is the contribution of solid fuel use for home heating to wintertime PM? An additional motivation for the Detling measurements was the question of whether coatings on black carbon particles enhance absorption. The following four key accomplishments have been identified so far: 1) Chemical, physical and optical characterization of PM from local and regional sources (Figures 2, 4, 5 and 6). 2) Measurement of urban increment in particulate matter and gases in London (Figure 3). 3) Measurement of optical properties and chemical composition of coatings on black carbon containing particles indicates absorption enhancement. 4) First deployment of chemical ionization instrument (MOVI-CI-TOFMS) to measure both particle-phase and gas-phase organic acids. (See final report from Joel Thornton, University of Washington, for details.) Analysis of the large dataset acquired in Detling is ongoing and will yield further key accomplishments. These measurements of urban and rural aerosol properties will contribute to improved modeling of regional aerosol emissions, and of atmospheric aging and removal. The measurement of absorption enhancement by coatings on black carbon will contribute to improved modeling of the direct radiative properties of PM.

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Three Dimensions Are Better Than Two, When It Comes to Representing Aerosols PI Contact: Ching, J., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Ching J, RA Zaveri, RC Easter, N Riemer, and JD Fast. 2016. "A three-dimensional sectional representation of aerosol mixing state for simulating optical properties and cloud condensation nuclei." Journal of Geophysical Research - Atmospheres, 121(10),

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosols Help Heat Up the Yangtze River Delta in China Download a printable PDF Submitter: Flynn, C. J., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Liu J, Z Li, Y Zheng, C Flynn, and M Cribb. 2012. "Seasonal variations of aerosol optical properties, vertical distribution and associated radiative effects in the Yangtze Delta region of China." Journal of Geophysical Research, 117, D00K38,

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Raman Lidar Observations of Aerosol Humidification Near Clouds Submitter: Ferrare, R. A., NASA LaRC Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Ferrare, R., et al., Evaluation of Daytime Measurements of Aerosols and Water Vapor Made by an Operational Raman Lidar over the Southern Great Plains, J. Geophys. Res., 111, D05S08, doi:10.1029/2005JD005836, 2006. Relative humidity profiles derived from the Raman lidar during the ALIVE 2005 field experiment. Aerosol

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Climatology of Aerosol Optical Depth in North-Central Oklahoma: 1992-2008 Download a printable PDF Submitter: Michalsky, J. J., Cooperative Institute for Research in Environmental Sciences Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Michalsky J, F Denn, C Flynn, G Hodges, P Kiedron, A Koontz, J Schlemmer, and SE Schwartz. 2010. "Climatology of aerosol optical depth in north-central Oklahoma: 1992-2008." Journal of Geophysical Research -

  16. Ultraviolet high-spectral-resolution Doppler lidar for measuring wind field and aerosol optical properties

    SciTech Connect (OSTI)

    Imaki, Masaharu; Kobayashi, Takao

    2005-10-01

    An ultraviolet incoherent Doppler lidar that incorporates the high-spectral-resolution (HSR) technique has been developed for measuring the wind field and aerosol optical properties in the troposphere. An injection seeded and tripled Nd:YAG laser at an ultraviolet wavelength of 355 nm was used in the lidar system. The HRS technique can resolve the aerosol Mie backscatter and the molecular Rayleigh backscatter to derive the signal components. By detecting the Mie backscatter, a great increase in the Doppler filter sensitivity was realized compared to the conventional incoherent Doppler lidars that detected the Rayleigh backscatter. The wind velocity distribution in a two-dimensional cross section was measured. By using the HSR technique, multifunction and absolute value measurements were realized for aerosol extinction, and volume backscatter coefficients; the laser beam transmittance, the lidar ratio, and the backscatter ratio are derived from these measurements.

  17. Lidar Investigations of Aerosol, Cloud, and Boundary Layer Properties Over the ARM ACRF Sites

    SciTech Connect (OSTI)

    Turner, David D.; Ferrare, Richard

    2015-01-13

    The systematic and routine measurements of aerosol, water vapor, and clouds in the vertical column above the Atmospheric Radiation Measurement (ARM) sites from surface-based remote sensing systems provides a unique and comprehensive data source that can be used to characterize the boundary layer (i.e., the lowest 3 km of the atmosphere) and its evolution. New algorithms have been developed to provide critical datasets from ARM instruments, and these datasets have been used in long-term analyses to better understand the climatology of water vapor and aerosol over Darwin, the turbulent structure of the boundary layer and its statistical properties over Oklahoma, and to better determine the distribution of ice and aerosol particles over northern Alaska.

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Influence of Dust Composition on Cloud Droplet Formation Download a printable PDF Submitter: Chuang, C., Lawrence Livermore National Laboratory Area of Research: Aerosol Properties...

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Light Absorption of Primary Organic Aerosol Paper Named ACS Editors' Choice Download a printable PDF Submitter: Lu, Z., Argonne National Laboratory Streets, D. ., Argonne National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Lu Z, DG Streets, E Winijkul, F Yan, Y Chen, TC Bond, Y Feng, MK Dubey, S Liu, JP Pinto, and GR Carmichael. 2015. "Light absorption properties and radiative effects of primary organic aerosol emissions."

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Quantifying Error in the Radiative Forcing of the First Aerosol Indirect Effect Submitter: McComiskey, A. C., National Oceanic and Atmospheric Administration Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Submitted to Geophysical Research Letters, 06-27-2007. Radiative forcing of aerosol indirect as function of CCN number density and LWP in units of W/m2 per 5% IE error. A survey of recently published works shows that values used to represent the magnitude of

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Characterization of Atmospheric Aerosols Using MFRSR Measurements Download a printable PDF Submitter: Alexandrov, M. D., Columbia University Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Alexandrov, MD, AA Lacis, BE Carlson, and B Cairns. 2007. "Characterization of atmospheric aerosols using MFRSR measurements." (Journal of Geophysical Research 113, DO8204. Sample spectral optical depths of atmospheric constituents in 300 - 900 nm spectral range:

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Arctic Aerosol Study Flies By Download a printable PDF Submitter: Schmid, B., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: ARM Climate Research Facility Operations Update, April 30, 2008, Edition Preliminary screening and analysis of images from the time-resolved aerosol collector indicate particles laden with carbon and sulfur. These data were obtained on April 8, 2008. Image courtesy of Alexander Laskin, PNNL. Images

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Atmospheric Aerosol Measurements on Cloudy Days: a New Method Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Ovchinnikov, M., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Kassianov, EI, and M Ovtchinnikov. 2008. "On reflectance ratios and aerosol optical depth retrieval in the presence of cumulus clouds." Geophysical Research Letters doi:10.1029/2008GL033231.

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Hemispherical Simulations Show Impact of Aerosols on Cloud Reflectivity Submitter: Rotstayn, L., Commonwealth Scientific and Industrial Research Organization Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Rotstayn, L., and Y. Liu, Sensitivity of the First Indirect Aerosol Effect to an Increase in Cloud Droplet Spectral Dispersion with Droplet Number Concentration, Journal of Climate: Vol. 16, No. 21, pp.3476-3481, May 2003. Figure 1. Measurements of the

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Overambitious Other Carbon Submitter: Church, J., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Song C, M Gyawali, RA Zaveri, JE Shilling, and WP Arnott. 2013. "Light absorption by secondary organic aerosol from α-pinene: Effects of oxidants, seed aerosol acidity, and relative humidity." Journal of Geophysical Research - Atmospheres, 118, doi:10.1002/jgrd.50767. Time-dependent Mass Absorption

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Gas-Phase Dry Deposition as a Major Removal Mechanism for Secondary Organic Aerosols (SOA) Download a printable PDF Submitter: Hodzic, A., NCAR Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Hodzic A, B Aumont, C Knote, J Lee-Taylor, S Madronich, and G Tyndall. 2014. "Volatility dependence of Henry's law constants of condensable organics: Application to estimate depositional loss of secondary organic aerosols." Geophysical Research Letters,

  7. Initial Assessment of the Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR)-Based Aerosol Retrieval: Sensitivity Study

    SciTech Connect (OSTI)

    Kassianov, Evgueni I.; Flynn, Connor J.; Redemann, Jens; Schmid, Beat; Russell, P. B.; Sinyuk, Alexander

    2012-10-24

    The Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR) being developed for airborne measurements will offer retrievals of aerosol microphysical and optical properties from multi-angular and multi-spectral measurements of sky radiance and direct-beam sun transmittance. In this study, we assess the expected accuracy of the 4STAR-based aerosol retrieval and its sensitivity to major sources of anticipated perturbations in the 4STAR measurements by adapting a theoretical approach previously developed for the AERONET measurements. The major anticipated perturbations are (1) an apparent enhancement of sky radiance at small scattering angles associated with the necessarily compact design of the 4STAR and (2) and an offset (i.e. uncertainty) of sky radiance calibration independent of scattering angle. The assessment is performed through application of the operational AERONET aerosol retrieval and constructed synthetic 4STAR-like data. Particular attention is given to the impact of these perturbations on the upwelling and downwelling broadband fluxes and the direct aerosol radiative forcing at the bottom and top of the atmosphere. The results from this study suggest that limitations in the accuracy of 4STAR-retrieved particle size distributions and scattering phase functions have diminished impact on the accuracy of retrieved bulk microphysical parameters, permitting quite accurate retrievals of properties including the effective radius (up to 10%, or 0.03), and the radiatively important optical properties, such as the asymmetry factor (up to 4%, or 0.02) and single-scattering albedo (up to 6%, or 0.04). Also, the obtained results indicate that the uncertainties in the retrieved aerosol optical properties are quite small in the context of the calculated fluxes and direct aerosol radiative forcing (up to 15%, or 3 Wm-2).

  8. Lidar Measurements of the Vertical Distribution of Aerosol Optical and Physical Properties over Central Asia

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Chen, Boris B.; Sverdlik, Leonid G.; Imashev, Sanjar A.; Solomon, Paul A.; Lantz, Jeffrey; Schauer, James J.; Shafer, Martin M.; Artamonova, Maria S.; Carmichael, Gregory R.

    2013-01-01

    The vertical structure of aerosol optical and physical properties was measured by Lidar in Eastern Kyrgyzstan, Central Asia, from June 2008 to May 2009. Lidar measurements were supplemented with surface-based measurements of PM 2.5 and PM 10 mass and chemical composition in both size fractions. Dust transported into the region is common, being detected 33% of the time. The maximum frequency occurred in the spring of 2009. Dust transported to Central Asia comes from regional sources, for example, Taklimakan desert and Aral Sea basin, and from long-range transport, for example, deserts of Arabia, Northeast Africa, Iran, and Pakistan. Regionalmore » sources are characterized by pollution transport with maximum values of coarse particles within the planetary boundary layer, aerosol optical thickness, extinction coefficient, integral coefficient of aerosol backscatter, and minimum values of the Ångström exponent. Pollution associated with air masses transported over long distances has different characteristics during autumn, winter, and spring. During winter, dust emissions were low resulting in high values of the Ångström exponent (about 0.51) and the fine particle mass fraction (64%). Dust storms were more frequent during spring with an increase in coarse dust particles in comparison to winter. The aerosol vertical profiles can be used to lower uncertainty in estimating radiative forcing.« less

  9. Global Distribution and Climate Forcing of Marine Organic Aerosol - Part 2: Effects on Cloud Properties and Radiative Forcing

    SciTech Connect (OSTI)

    Gantt, Brett; Xu, Jun; Meskhidze, N.; Zhang, Yang; Nenes, Athanasios; Ghan, Steven J.; Liu, Xiaohong; Easter, Richard C.; Zaveri, Rahul A.

    2012-07-25

    A series of simulations with the Community Atmosphere Model version 5 (CAM5) with a 7-mode Modal Aerosol Model were conducted to assess the changes in cloud microphysical properties and radiative forcing resulting from marine organic aerosols. Model simulations show that the anthropogenic aerosol indirect forcing (AIF) predicted by CAM5 is decreased in absolute magnitude by up to 0.09 Wm{sup -2} (7 %) when marine organic aerosols are included. Changes in the AIF from marine organic aerosols are associated with small global increases in low-level incloud droplet number concentration and liquid water path of 1.3 cm{sup -3} (1.5 %) and 0.22 gm{sup -2} (0.5 %), respectively. Areas especially sensitive to changes in cloud properties due to marine organic aerosol include the Southern Ocean, North Pacific Ocean, and North Atlantic Ocean, all of which are characterized by high marine organic emission rates. As climate models are particularly sensitive to the background aerosol concentration, this small but non-negligible change in the AIF due to marine organic aerosols provides a notable link for ocean-ecosystem marine low-level cloud interactions and may be a candidate for consideration in future earth system models.

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Radiative and Thermodynamic Responses to Uncertainty in Aerosol Extinction Profiles Download a printable PDF Submitter: Feng, Y., Argonne National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Feng Y, R Kotamarthi, R Coulter, C Zhao, and M Cadeddu. 2016. "Radiative and Thermodynamic Responses to Aerosol Extinction Profiles during the Pre-monsoon Month over South Asia." Atmospheric Chemistry and Physics, 16(1), 247-264. WRF-Chem

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    CCN Activity and Mixing Rules of Isoprene Secondary Organic Aerosol (SOA) and Sulfate Download a printable PDF Submitter: Martin, S. T., Harvard University Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: King SM, T Rosenoern, JH Shilling, Q Chen, Z Wang, G Biskos, KA McKinney, U Poeschl, and ST Martin. 2010. "Cloud droplet activation of mixed organic-sulfate particles produced by the photooxidation of

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ice Nucleation Link to Aerosols for Global Models Download a printable PDF Submitter: DeMott, P. J., Colorado State University Liu, X., University of Wyoming Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: DeMott PJ, AJ Prenni, X Liu, SM Kreidenweis, MD Petters, CH Twohy, MS Richardson, T Eidhammer, and DC Rogers. 2010. "Predicting global atmospheric ice nuclei distributions and their impacts on

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    How Aerosols Affect Cloud Properties in Arctic Mixed-Phase Stratocumulus Download a printable PDF Submitter: McFarquhar, G., University of Illinois, Urbana Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Jackson RC, GM McFarquhar, AV Korolev, ME Earle, PS Liu, RP Lawson, S Brooks, M Wolde, A Laskin, and M Freer. 2012. "The dependence of ice microphysics on aerosol concentration in arctic mixed-phase

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Spectro-microscopic Measurements of Carbonaceous Aerosol Aging in Central California Download a printable PDF Submitter: Gilles, M., Lawrence Berkeley National Laboratory Moffet, R., University of the Pacific Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Moffet RC, TC Rödel, ST Kelly, XY Yu, GT Carroll, J Fast, RA Zaveri, A Laskin, and MK Gilles. 2013. "Spectro-microscopic measurements of carbonaceous aerosol aging in Central California."

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Initial Aerosol Concentration Is Key Contributor to Low-Level Cloud Reflectivity Submitter: Penner, J. E., University of Michigan Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Penner, J., Dong, X., Chen. Y., Observational evidence of a change in radiative forcing due to the indirect aerosol effect, Nature, Vol. 427, 15 January 2004. Cloud optical depth, as determined from the parcel model, is indicated by the dots. Red lines show best fit data of cloud liquid

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Effects of Relative Humidity on Aerosols-Implications for Climate Submitter: Lacis, A. A., NASA - Goddard Institute for Space Studies Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: "Refractive Indices of Three Hygroscopic Aerosols and their Dependence on Relative Humidity," October 2001. Sponsored by the DOE Atmospheric Radiation Measurement (ARM) Program, science collaborators at the National Aeronautics and Space Administration (NASA) Goddard

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Even at High Humidity, Aerosols Stick Around: Slowly Evaporating Particles Refute Assumption Download a printable PDF Submitter: Zelenyuk-Imre, A., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Wilson J, D Imre, J Beránek, M Shrivastava, and A Zelenyuk. 2014. "Evaporation kinetics of laboratory-generated secondary organic aerosols at elevated relative humidity." Environmental Science & Technology,

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Arctic Haze: Effect of Anthropogenic and Biomass Burning Aerosols Transported from Europe to the Arctic Download a printable PDF Submitter: Fast, J. D., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Marelle L, J Raut, JL Thomas, KS Law, B Quennehen, G Ancellet, J Pelon, A Schwarzenboeck, and JD Fast. 2015. "Transport of anthropogenic and biomass burning aerosols from Europe to the

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Phase State and Physical Properties of Ambient and Lab Generated Aerosols: X-ray Microscopy Download a printable PDF Submitter: OBrien, R. E., Lawrence Berkeley National Laboratory Gilles, M., Lawrence Berkeley National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: O'Brien RE, A Neu, SA Epstein, AC MacMillan, B Wang, ST Kelly, SA Nizkorodov, A Laskin, RC Moffet, and MK Gilles. 2014. "Physical properties of ambient and

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Retrieving Cloud and Aerosol Properties from the ARM Raman Lidar Download a printable PDF Submitter: Thorsen, T., NASA - Langley Research Center Fu, Q., University of Washington Area of Research: Cloud Distributions/Characterizations Working Group(s): Aerosol Life Cycle, Cloud Life Cycle Journal Reference: Thorsen TJ, Q Fu, RK Newsom, DD Turner, and JM Comstock. 2015. "Automated retrieval of cloud and aerosol properties from the ARM Raman lidar, Part I: Feature detection." Journal of

  1. Investigations of the Absorption Properties of Near-Ground Aerosol by the Methods of Optical-Acoustic Spectrometry and Diff...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Investigations of the Absorption Properties of Near-Ground Aerosol by the Methods of Optical-Acoustic Spectrometry and Diffuse Extinction V. S. Kozlov, M. V. Panchenko, A. B. Tikhomirov, and B. A. Tikhomirov Institute of Atmospheric Optics Tomsk, Russia Introduction Aerosol absorption is an important factor in the formation of non-selective radiation extinction in the visible wavelength range, and plays a great role in solving many radiative and climatic problems. The principal absorbing

  2. Improved Arctic Cloud and Aerosol Research and Model Parameterizations

    SciTech Connect (OSTI)

    Kenneth Sassen

    2007-03-01

    In this report are summarized our contributions to the Atmospheric Measurement (ARM) program supported by the Department of Energy. Our involvement commenced in 1990 during the planning stages of the design of the ARM Cloud and Radiation Testbed (CART) sites. We have worked continuously (up to 2006) on our ARM research objectives, building on our earlier findings to advance our knowledge in several areas. Below we summarize our research over this period, with an emphasis on the most recent work. We have participated in several aircraft-supported deployments at the SGP and NSA sites. In addition to deploying the Polarization Diversity Lidar (PDL) system (Sassen 1994; Noel and Sassen 2005) designed and constructed under ARM funding, we have operated other sophisticated instruments W-band polarimetric Doppler radar, and midinfrared radiometer for intercalibration and student training purposes. We have worked closely with University of North Dakota scientists, twice co-directing the Citation operations through ground-to-air communications, and serving as the CART ground-based mission coordinator with NASA aircraft during the 1996 SUCCESS/IOP campaign. We have also taken a leading role in initiating case study research involving a number of ARM coinvestigators. Analyses of several case studies from these IOPs have been reported in journal articles, as we show in Table 1. The PDL has also participated in other major field projects, including FIRE II and CRYSTAL-FACE. In general, the published results of our IOP research can be divided into two categories: comprehensive cloud case study analyses to shed light on fundamental cloud processes using the unique CART IOP measurement capabilities, and the analysis of in situ data for the testing of remote sensing cloud retrieval algorithms. One of the goals of the case study approach is to provide sufficiently detailed descriptions of cloud systems from the data-rich CART environment to make them suitable for application to

  3. Coupling Between Oceanic Upwelling and Cloud-aerosol Properties at the AMF Point Reyes Site

    SciTech Connect (OSTI)

    Dunn, M.; Jensen, M.; Miller, M.; Kollias, P.; Bartholomew, M. J.; Turner, D.; Andrews, E.; Jefferson, A.; Daum, P.

    2008-03-10

    Cloud microphysical properties measured at the ARM Mobile Facility site located on the northern coast of California near Point Reyes, during the 2005 Marine Stratus Radiation, Aerosol and Drizzle experiment, were analyzed to determine their relationship to the coastal sea surface temperature (SST) which was characterized using measurements acquired from a National Oceanic and Atmospheric Administration offshore buoy. An increase in SST resulting from a relaxation of upwelling, occurring in the eastern Pacific Ocean off the coast of California in summer is observed to strongly correlate with nearby ground measured cloud microphysical properties and cloud condensation nuclei (CCN) concentrations. Correlations between these atmospheric and oceanic features provide insight into the interplay between the ocean and cloud radiative properties. We present evidence of this robust correlation and examine the factors controlling these features. The marine boundary layer is in direct contact with the sea surface and is strongly influenced by SST. Moisture and vertical motion are crucial ingredients for cloud development and so we examine the role of SST in providing these key components to the atmosphere. Although upwelling of cold subsurface waters is conventionally thought to increase aerosols in the region, thus increasing clouds, here we observed a relaxation of upwelling associated with changes in the structure of marine stratus clouds. As upwelling relaxes, the SST get warmer, thick clouds with high liquid water paths are observed and persist for a few days. This cycle is repeated throughout the summer upwelling season. A concomitant cyclic increase and decrease of CCN concentration is also observed. Forcing mechanisms and large-scale atmospheric features are discussed. Marine stratocumulus clouds are a critical component of the earth's radiation budget and this site provides an excellent opportunity to study the influence of SST on these clouds.

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Cumuli Impact on Solar Radiation at Surface: Spectral Changes Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle, Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Kassianov E, J Barnard, LK Berg, CN Long, and C Flynn. 2011. "Shortwave spectral radiative forcing of cumulus clouds from surface observations." Geophysical Research Letters, 38, L07801,

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Production Flux of Sea-Spray Aerosol Download a printable PDF Submitter: Schwartz, S. E., Brookhaven National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: de Leeuw G, EL Andreas, MD Anguelova, ER Lewis, C O'Dowd, M Schulz, and SE Schwartz. 2011. "Production flux of sea-spray aerosol." Reviews of Geophysics, 49, RG2001, doi:10.1029/2010RG000349. Lewis ER and SE Schwartz. 2004. Sea Salt Aerosol Production: Mechanisms, Methods,

  6. [Plasma properties research: Task 3

    SciTech Connect (OSTI)

    Not Available

    1992-01-01

    The principal research activities of the Magneto-Fluid Dynamics Division relate to magnetic fusion plasma physics. In addition, there is a modest amount of work in closely related areas, including space plasma physics, fluid dynamics, and dynamical systems. Members of the Magneto-Fluid Dynamics Division maintain close contacts with fusion researchers in the US and abroad. Some of the work of the Division is clearly directed towards ITER and TPX, while other problems relate to the broader development of fusion plasma physics and to the support of other issues arising in the many experimental programs. Topics of some note in the last year that are discussed in this report are: Application of sophisticated statistical techniques to tokamak data reduction, including time series analysis of TFTR fluctuation data and spline analysis of profile data. Continuing development of edge plasma and divertor modelling, including initial ergodic divertor studies. Analysis of energetic fusion products losses from TFTR plasmas. Examination of anomalous transport in dynamical systems induced by chaotic-like Hamiltonian motion. Numerical simulation of the development of singular MHD equilibria. Exploration of the validity of moment expansions of kinetic equations for weakly collisional systems. Studies of RF- and ripple-induced helium ash removal. Ballooning mode studies in fluids and rotating stars. Studies in dynamical systems, including explosive instabilities, development of chaos, and motion of collisionless particles in a domain with overlapping islands.

  7. [Plasma properties research: Task 3

    SciTech Connect (OSTI)

    Not Available

    1992-12-31

    The principal research activities of the Magneto-Fluid Dynamics Division relate to magnetic fusion plasma physics. In addition, there is a modest amount of work in closely related areas, including space plasma physics, fluid dynamics, and dynamical systems. Members of the Magneto-Fluid Dynamics Division maintain close contacts with fusion researchers in the US and abroad. Some of the work of the Division is clearly directed towards ITER and TPX, while other problems relate to the broader development of fusion plasma physics and to the support of other issues arising in the many experimental programs. Topics of some note in the last year that are discussed in this report are: Application of sophisticated statistical techniques to tokamak data reduction, including time series analysis of TFTR fluctuation data and spline analysis of profile data. Continuing development of edge plasma and divertor modelling, including initial ergodic divertor studies. Analysis of energetic fusion products losses from TFTR plasmas. Examination of anomalous transport in dynamical systems induced by chaotic-like Hamiltonian motion. Numerical simulation of the development of singular MHD equilibria. Exploration of the validity of moment expansions of kinetic equations for weakly collisional systems. Studies of RF- and ripple-induced helium ash removal. Ballooning mode studies in fluids and rotating stars. Studies in dynamical systems, including explosive instabilities, development of chaos, and motion of collisionless particles in a domain with overlapping islands.

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    From Fire to Ice Download a printable PDF Submitter: Kulkarni, G., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Kulkarni GR, M Nandasiri, A Zelenyuk, J Beranek, N Madaan, A Devaraj, V Shutthanandan, S Thevuthasan, and T Varga. 2015. "Effects of crystallographic properties on the ice nucleation properties of volcanic ash particles." Geophysical Research Letters, 42(8), doi:10.1002/2015GL063270. Tons of

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Hiding in Plain Sight: a Less-Explored Secret of Secondary Organic Aerosols PI Contact: Shrivastava, M., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Shrivastava M, C Zhao, RC Easter, Y Qian, A Zelenyuk, JD Fast, Y Liu, Q Zhang, and A Guenther. 2016. "Sensitivity analysis of simulated SOA loadings using a variance-based statistical approach." Journal of Advances in Modeling Earth Systems, ,

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Anthropogenic Aerosols: a Clearer Understanding Submitter: Daum, P., Brookhaven National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Liu, Y., and P. H. Daum, 2002: "Indirect warming effect from dispersion forcing," Nature 419(6872):580-581. Figure 1. Key = Green symbols: triangle - FIRE, northeastern Pacific; Crossed circles - SOCEX, Southern Ocean; Filled circle - ACE1, Southern Ocean; Blue symbols: Filled circles - ASTEX 8,

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Pollution Hitches Ride to Arctic Download a printable PDF Submitter: Zelenyuk-Imre, A., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Zelenyuk A, D Imre, J Beranek, E Abramson, J Wilson, and M Shrivastava. 2012. "Synergy between secondary organic aerosols and long-range transport of polycyclic aromatic hydrocarbons." Environmental Science & Technology, 46(22), doi:10.1021/es302743z. When airborne

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Chemical Diffusivity and Viscosity of Secondary Organic Aerosols Download a printable PDF Submitter: Zelenyuk-Imre, A., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Abramson E, D Imre, J Beránek, J Wilson, and A Zelenyuk. 2013. "Experimental determination of chemical diffusion within secondary organic zerosol particles." Physical Chemistry Chemical Physics, 15, doi:10.1039/C2CP44013J. Determining the

  13. AERONET: The Aerosol Robotic Network

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    The AERONET (AErosol RObotic NETwork) program is a federation of ground-based remote sensing aerosol networks established by NASA and LOA-PHOTONS (CNRS) and is greatly expanded by collaborators from national agencies, institutes, universities, individual scientists, and partners. The program provides a long-term, continuous and readily accessible public domain database of aerosol optical, mircrophysical and radiative properties for aerosol research and characterization, validation of satellite retrievals, and synergism with other databases. The network imposes standardization of instruments, calibration, processing and distribution. AERONET collaboration provides globally distributed observations of spectral aerosol optical Depth (AOD), inversion products, and precipitable water in diverse aerosol regimes. Aerosol optical depth data are computed for three data quality levels: Level 1.0 (unscreened), Level 1.5 (cloud-screened), and Level 2.0 (cloud screened and quality-assured). Inversions, precipitable water, and other AOD-dependent products are derived from these levels and may implement additional quality checks.[Copied from http://aeronet.gsfc.nasa.gov/new_web/system_descriptions.html

  14. Aerosol Extinction Profiles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    and Thermodynamic Responses to Uncertainty in Aerosol Extinction Profiles For original submission and image(s), see ARM Research Highlights http://www.arm.gov/science/highlights/ Research Highlight Aerosol radiative effects are of great importance for climate simulations over South Asia. For quantifying aerosol direct radiative effect, aerosol optical depth (AOD) and single scattering albedo (SSA) are often compared with observations. These comparisons have revealed large AOD underestimation and

  15. One ARM, Two Columns and a Whole Lot of Aerosols | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    ARM, Two Columns and a Whole Lot of Aerosols One ARM, Two Columns and a Whole Lot of Aerosols July 25, 2012 - 5:49pm Addthis This observatory is part of an air particles research initiative at Cape Cod National Seashore in Massachusetts, and includes dozens of sophisticated instruments that take continuous ground-based measurements of clouds, aerosols, and other atmospheric properties. | Photo courtesy of the ARM Climate Research Facility. This observatory is part of an air particles research

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Mixed Bag of Aerosols over Northeastern China Download a printable PDF Submitter: Li, Z., University of Maryland Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Li C, JW Stehr, LT Marufu, Z Li, and RR Dickerson. 2012. "Aircraft measurements of SO2 and aerosols over northeastern China: Vertical profiles and the influence of weather on air quality." Atmospheric Environment, 62, doi:10.1016/j.atmosenv.2012.07.076. Altitude profiles of

  17. Scanning Transmission X-ray Microscopy: Applications in Atmospheric Aerosol Research

    SciTech Connect (OSTI)

    Moffet, Ryan C.; Tivanski, Alexei V.; Gilles, Mary K.

    2011-01-20

    Scanning transmission x-ray microscopy (STXM) combines x-ray microscopy and near edge x-ray absorption fine structure spectroscopy (NEXAFS). This combination provides spatially resolved bonding and oxidation state information. While there are reviews relevant to STXM/NEXAFS applications in other environmental fields (and magnetic materials) this chapter focuses on atmospheric aerosols. It provides an introduction to this technique in a manner approachable to non-experts. It begins with relevant background information on synchrotron radiation sources and a description of NEXAFS spectroscopy. The bulk of the chapter provides a survey of STXM/NEXAFS aerosol studies and is organized according to the type of aerosol investigated. The purpose is to illustrate the current range and recent growth of scientific investigations employing STXM-NEXAFS to probe atmospheric aerosol morphology, surface coatings, mixing states, and atmospheric processing.

  18. CLOUDS, AEROSOLS, RADIATION AND THE AIR-SEA INTERFACE OF THE SOUTHERN OCEAN: ESTABLISHING DIRECTIONS FOR FUTURE RESEARCH

    SciTech Connect (OSTI)

    Wood, Robert; Bretherton, Chris; McFarquhar, Greg; Protat, Alain; Quinn, Patricia; Siems, Steven; Jakob, Christian; Alexander, Simon; Weller, Bob

    2014-09-29

    A workshop sponsored by the Department of Energy was convened at the University of Washington to discuss the state of knowledge of clouds, aerosols and air-sea interaction over the Southern Ocean and to identify strategies for reducing uncertainties in their representation in global and regional models. The Southern Ocean plays a critical role in the global climate system and is a unique pristine environment, yet other than from satellite, there have been sparse observations of clouds, aerosols, radiation and the air-sea interface in this region. Consequently, much is unknown about atmospheric and oceanographic processes and their linkage in this region. Approximately 60 scientists, including graduate students, postdoctoral fellows and senior researchers working in atmospheric and oceanic sciences at U.S. and foreign universities and government laboratories, attended the Southern Ocean Workshop. It began with a day of scientific talks, partly in plenary and partly in two parallel sessions, discussing the current state of the science for clouds, aerosols and air-sea interaction in the Southern Ocean. After the talks, attendees broke into two working groups; one focused on clouds and meteorology, and one focused on aerosols and their interactions with clouds. This was followed by more plenary discussion to synthesize the two working group discussions and to consider possible plans for organized activities to study clouds, aerosols and the air-sea interface in the Southern Ocean. The agenda and talk slides, including short summaries of the highlights of the parallel session talks developed by the session chars, are available at http://www.atmos.washington.edu/socrates/presentations/SouthernOceanPresentations/.

  19. Intellectual Property Provisions (GLB-115) Grant Research, Development...

    Energy Savers [EERE]

    GLB-115) Grant Research, Development, or Demonstration Large Business and Foreign Entity Intellectual Property Provisions (GLB-115) Grant Research, Development, or Demonstration ...

  20. Intellectual Property Provisions (GSB-115) Grant Research, Development...

    Energy Savers [EERE]

    GSB-115) Grant Research, Development, or Demonstration Domestic Small Business Intellectual Property Provisions (GSB-115) Grant Research, Development, or Demonstration Domestic ...

  1. Direct Aerosol Forcing Uncertainty

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Mccomiskey, Allison

    2008-01-15

    Understanding sources of uncertainty in aerosol direct radiative forcing (DRF), the difference in a given radiative flux component with and without aerosol, is essential to quantifying changes in Earth's radiation budget. We examine the uncertainty in DRF due to measurement uncertainty in the quantities on which it depends: aerosol optical depth, single scattering albedo, asymmetry parameter, solar geometry, and surface albedo. Direct radiative forcing at the top of the atmosphere and at the surface as well as sensitivities, the changes in DRF in response to unit changes in individual aerosol or surface properties, are calculated at three locations representing distinct aerosol types and radiative environments. The uncertainty in DRF associated with a given property is computed as the product of the sensitivity and typical measurement uncertainty in the respective aerosol or surface property. Sensitivity and uncertainty values permit estimation of total uncertainty in calculated DRF and identification of properties that most limit accuracy in estimating forcing. Total uncertainties in modeled local diurnally averaged forcing range from 0.2 to 1.3 W m-2 (42 to 20%) depending on location (from tropical to polar sites), solar zenith angle, surface reflectance, aerosol type, and aerosol optical depth. The largest contributor to total uncertainty in DRF is usually single scattering albedo; however decreasing measurement uncertainties for any property would increase accuracy in DRF. Comparison of two radiative transfer models suggests the contribution of modeling error is small compared to the total uncertainty although comparable to uncertainty arising from some individual properties.

  2. Automated retrieval of cloud and aerosol properties from the ARM Raman lidar, part 1: feature detection

    SciTech Connect (OSTI)

    Thorsen, Tyler J.; Fu, Qiang; Newsom, Rob K.; Turner, David D.; Comstock, Jennifer M.

    2015-11-01

    A Feature detection and EXtinction retrieval (FEX) algorithm for the Atmospheric Radiation Measurement (ARM) program’s Raman lidar (RL) has been developed. Presented here is part 1 of the FEX algorithm: the detection of features including both clouds and aerosols. The approach of FEX is to use multiple quantities— scattering ratios derived using elastic and nitro-gen channel signals from two fields of view, the scattering ratio derived using only the elastic channel, and the total volume depolarization ratio— to identify features using range-dependent detection thresholds. FEX is designed to be context-sensitive with thresholds determined for each profile by calculating the expected clear-sky signal and noise. The use of multiple quantities pro-vides complementary depictions of cloud and aerosol locations and allows for consistency checks to improve the accuracy of the feature mask. The depolarization ratio is shown to be particularly effective at detecting optically-thin features containing non-spherical particles such as cirrus clouds. Improve-ments over the existing ARM RL cloud mask are shown. The performance of FEX is validated against a collocated micropulse lidar and observations from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite over the ARM Darwin, Australia site. While we focus on a specific lidar system, the FEX framework presented here is suitable for other Raman or high spectral resolution lidars.

  3. Improvement in Clouds and the Earth's Radiant Energy System/Surface and Atmosphere Radiation Budget Dust Aerosol Properties, Effects on Surface Validation of Clouds and Radiative Swath

    SciTech Connect (OSTI)

    Rutan, D.; Rose, F.; Charlock, T.P.

    2005-03-18

    Within the Clouds and the Earth's Radiant Energy System (CERES) science team (Wielicki et al. 1996), the Surface and Atmospheric Radiation Budget (SARB) group is tasked with calculating vertical profiles of heating rates, globally, and continuously, beneath CERES footprint observations of Top of Atmosphere (TOA) fluxes. This is accomplished using a fast radiative transfer code originally developed by Qiang Fu and Kuo-Nan Liou (Fu and Liou 1993) and subsequently highly modified by the SARB team. Details on the code and its inputs can be found in Kato et al. (2005) and Rose and Charlock (2002). Among the many required inputs is characterization of the vertical column profile of aerosols beneath each footprint. To do this SARB combines aerosol optical depth information from the moderate-resolution imaging spectroradiometer (MODIS) instrument along with aerosol constituents specified by the Model for Atmosphere and Chemical Transport (MATCH) of Collins et al. (2001), and aerosol properties (e.g. single scatter albedo and asymmetry parameter) from Tegen and Lacis (1996) and OPAC (Hess et al. 1998). The publicly available files that include these flux profiles, called the Clouds and Radiative Swath (CRS) data product, available from the Langley Atmospheric Sciences Data Center (http://eosweb.larc.nasa.gov/). As various versions of the code are completed, publishable results are named ''Editions.'' After CRS Edition 2A was finalized it was found that dust aerosols were too absorptive. Dust aerosols have subsequently been modified using a new set of properties developed by Andy Lacis and results have been released in CRS Edition 2B. This paper discusses the effects of changing desert dust aerosol properties, which can be significant for the radiation budget in mid ocean, a few thousand kilometers from the source regions. Resulting changes are validated via comparison of surface observed fluxes from the Saudi Solar Village surface site (Myers et al. 1999), and the E13 site

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Climate Warming Due to Soot and Smoke? Maybe Not. Submitter: Penner, J. E., University of Michigan Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Penner, J.E., S.Y. Zhang, and C.C. Chuang, Soot and smoke aerosol may not warm climate, J. Geophys. Res., 108(D21), 4657, doi:10.1029/2003JD003409, 2003. New research results from the Department of Energy's Atmospheric Radiation Measurement (ARM) Program suggest that fossil fuel soot emissions and biomass smoke may

  5. Intellectual Property Provisions (CSB-115) Cooperative Agreement Research,

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Development, or Demonstration Domestic Small Business | Department of Energy 15) Cooperative Agreement Research, Development, or Demonstration Domestic Small Business Intellectual Property Provisions (CSB-115) Cooperative Agreement Research, Development, or Demonstration Domestic Small Business CSB-115.pdf (56.83 KB) More Documents & Publications Intellectual Property Provisions (CSB-1003) Cooperative Agreement Research, Development, or Demonstration Domestic Small Businesses

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Sub-micrometre Particulate Matter Is Primarily in Liquid Form over Amazon Rain Forest PI Contact: Zaveri, R., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Bateman AP, Z Gong, P Liu, B Sato, G Cirino, Y Zhang, P Artaxo, AK Bertram, AO Manzi, LV Rizzo, RA Souza, RA Zaveri, and ST Martin. 2016. "Sub-micrometre particulate matter is primarily in liquid form over Amazon rainforest."

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Can Ice-Nucleating Aerosols Affect Arctic Seasonal Climate? Submitter: Prenni, A. J., Colorado State University Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Prenni, A. J., J. Y. Harrington, M. Tjernstrom, P. J. DeMott, A. Avramov, C. N. Long, S. M. Kreidenweis, P. Q. Olsson, and J. Verlinde, (2006): Can Ice-Nucleating Aerosols Affect Arctic Seasonal Climate?, BAMS, Vol.88, Iss. 4; pg. 541-550. ACIA, 2004: Impacts of a Warming

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Optical Properties of the 1997 TWP Smoke Event Submitter: Spinhirne, J., University of Arizona Area of Research: Radiation Processes Working Group(s): Radiative Processes Journal Reference: N/A Figure 1. MPL image showing evolution of early September, 1997 smoke event at Manus, TWP. Figure 2. Selected aerosol extinction cross section profiles at the ARM TWP site during 1997 showing progression of aerosol loading. Figure 3. Cloud-cleared optical measurements at the TWP site from July 27 to

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    When Pollution Gets a Whiff of Trees Download a printable PDF Submitter: Shilling, J., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Shilling JE, RA Zaveri, JD Fast, L Kleinman, M Alexander, MR Canagaratna, E Fortner, JM Hubbe, JT Jayne, A Sedlacek, A Setyan, S Springston, DR Worsnop, and Q Zhang. 2013. "Enhanced SOA formation from mixed anthropogenic and biogenic emissions during the CARES campaign."

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Wildfires Lead to More Warming Than Climate Models Predict, a New Mexico Fire Study Reports Download a printable PDF Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: China S, C Mazzoleni, K Gorkowski, AC Aiken, and MK Dubey. 2013. "Morphology and mixing state of individual freshly emitted wildfire carbonaceous particles." Nature Communications, 4, 2122, doi:10.1038/ncomms3122.

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Dark Side of Cold Clouds Download a printable PDF Submitter: Kulkarni, G., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: China S, G Kulkarni, BV Scarnato, N Sharma, M Pekour, JE Shilling, J Wilson, A Zelenyuk, D Chand, S Liu, AC Aiken, MK Dubey, A Laskin, RA Zaveri, and C Mazzoleni. 2015. "Morphology of diesel soot residuals from supercooled water droplets and ice crystals: implications for optical

  12. Intellectual Property Provisions (GSB-115) Grant Research, Development, or

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Demonstration Domestic Small Business | Department of Energy GSB-115) Grant Research, Development, or Demonstration Domestic Small Business Intellectual Property Provisions (GSB-115) Grant Research, Development, or Demonstration Domestic Small Business GSB-115.pdf (46.58 KB) More Documents & Publications GSB-1003.PDF&#0; Intellectual Property Provisions (CSB-1003) Cooperative Agreement Research, Development, or Demonstration Domestic Small Businesses Intellectual Property Provisions

  13. Los Alamos researchers uncover new properties in nanocomposite...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Los Alamos researchers uncover new properties in nanocomposite oxide ceramics for reactor fuel, fast-ion conductors Alumni Link: Opportunities, News and Resources for Former ...

  14. Two-Column Aerosol Project (TCAP): Ground-Based Radiation and...

    Office of Scientific and Technical Information (OSTI)

    ... Sponsoring Org: USDOE Office of Science (SC), Biological and Environmental Research (BER) ... Subject: 54 ENVIRONMENTAL SCIENCES aerosols, aerosol optical depth, direct aerosol ...

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Two-Column Aerosol Project: Impact of Elevated Particle Layers on Particle Optical Depth PI Contact: Berg, L., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Berg LK, JD Fast, JC Barnard, SP Burton, B Cairns, D Chand, JM Comstock, S Dunagan, RA Ferrare, CJ Flynn, JW Hair, CA Hostetler, J Hubbe, A Jefferson, R Johnson, EI Kassianov, CD Kluzek, P Kollias, K Lamer, K Lantz, F Mei, MA Miller, J Michalsky, I Ortega, M

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Urban Emissions Significantly Enhance SOA Production at a Rural Site in the NE US PI Contact: Zhang, Q., University of California, Davis Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Zhou S, S Collier, J Xu, F Mei, J Wang, Y Lee, AI Sedlacek, SR Springston, Y Sun, and Q Zhang. 2016. "Influences of Upwind Emission Sources and Atmospheric Processing on Aerosol Chemistry and Properties at a Rural Location in the Northeastern US." Journal of

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Effects on Liquid-Water Path of Thin Stratocumulus Clouds Download a printable PDF Submitter: Penner, J. E., University of Michigan Lee, S., University of Michigan Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: n/a Thin clouds with mean liquid-water path (LWP) of ~ 50 g m-2 cover 27.5% of the globe and thus play an important role in the Earth's radiation budget. Radiative fluxes at the Earth's surface and top of atmosphere (TOA) are very sensitive to

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    More Like Shades of Gray: the Effects of Black Carbon in Aerosols Submitter: McComiskey, A. C., National Oceanic and Atmospheric Administration Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Cappa CD, TB Onasch, P Massoli, DR Worsnop, TS Bates, ES Cross, P Davidovits, J Hakala, KL Hayden, BT Jobson, KR Kolesar, DA Lack, BM Lerner, SM Li, D Mellon, I Nuaaman, JS Olfert, T Petaja, PK Quinn, C Song, R Subramanian, EJ Williams, and RA Zaveri. 2012.

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Dust in the Wind... and the Clouds... and the Atmosphere Submitter: Sassen, K., University of Alaska, Fairbanks Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Sassen, K., P.J. DeMott, J.M. Propsero, and M.R. Poellot, Saharan Dust Storms and Indirect Aerosol Effects on Clouds: CRYSTAL-FACE Results, Geophys. Res. Ltt., 30(12), 1633, doi:10/1029/2003GL017371, 2003. PDL linear depolarization ratio (color scale on top) and relative returned power (in gray scale) of

  20. Cloud Condensation Nuclei Activity of Aerosols during GoAmazon...

    Office of Scientific and Technical Information (OSTI)

    microphysical properties of the aerosol." The Observations and Modeling of the Green Ocean Amazon (GoAmazon 201415) study seeks to understand how aerosol and cloud life cycles ...

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MBL Cloud Properties Derived from the Azores-AMF Observations Submitter: Dong, X., University of Arizona Area of Research: Cloud Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Dong X, B Xi, A Kennedy, P Minnis, and R Wood. 2014. "A 19-month record of marine aerosol-cloud-radiation properties derived from DOE ARM AMF deployment at the Azores: Part I: Cloud fraction and single-layered MBL cloud properties." Journal of Climate, 27(10),

  2. Indirect and semi-direct aerosol campaign: The impact of Arctic aerosols on clouds

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    McFarquhar, Greg M.; Ghan, Steven; Verlinde, Johannes; Korolev, Alexei; Strapp, J. Walter; Schmid, Beat; Tomlinson, Jason M.; Wolde, Menqistu; Brooks, Sarah D.; Cziczo, Dan; et al

    2011-02-01

    A comprehensive dataset of microphysical and radiative properties of aerosols and clouds in the boundary layer in the vicinity of Barrow, Alaska, was collected in April 2008 during the Indirect and Semi-Direct Aerosol Campaign (ISDAC). ISDAC's primary aim was to examine the effects of aerosols, including those generated by Asian wildfires, on clouds that contain both liquid and ice. ISDAC utilized the Atmospheric Radiation Measurement Pro- gram's permanent observational facilities at Barrow and specially deployed instruments measuring aerosol, ice fog, precipitation, and radiation. The National Research Council of Canada Convair-580 flew 27 sorties and collected data using an unprecedented 41more » stateof- the-art cloud and aerosol instruments for more than 100 h on 12 different days. Aerosol compositions, including fresh and processed sea salt, biomassburning particles, organics, and sulfates mixed with organics, varied between flights. Observations in a dense arctic haze on 19 April and above, within, and below the single-layer stratocumulus on 8 and 26 April are enabling a process-oriented understanding of how aerosols affect arctic clouds. Inhomogeneities in reflectivity, a close coupling of upward and downward Doppler motion, and a nearly constant ice profile in the single-layer stratocumulus suggests that vertical mixing is responsible for its longevity observed during ISDAC. Data acquired in cirrus on flights between Barrow and Fairbanks, Alaska, are improving the understanding of the performance of cloud probes in ice. Furthermore, ISDAC data will improve the representation of cloud and aerosol processes in models covering a variety of spatial and temporal scales, and determine the extent to which surface measurements can provide retrievals of aerosols, clouds, precipitation, and radiative heating.« less

  3. Indirect and Semi-Direct Aerosol Campaign: The Impact of Arctic Aerosols on Clouds

    SciTech Connect (OSTI)

    McFarquhar, Greg; Ghan, Steven J.; Verlinde, J.; Korolev, Alexei; Strapp, J. Walter; Schmid, Beat; Tomlinson, Jason M.; Wolde, Mengistu; Brooks, Sarah D.; Cziczo, Daniel J.; Dubey, Manvendra K.; Fan, Jiwen; Flynn, Connor J.; Gultepe, Ismail; Hubbe, John M.; Gilles, Mary K.; Laskin, Alexander; Lawson, Paul; Leaitch, W. R.; Liu, Peter S.; Liu, Xiaohong; Lubin, Dan; Mazzoleni, Claudio; Macdonald, A. M.; Moffet, Ryan C.; Morrison, H.; Ovchinnikov, Mikhail; Shupe, Matthew D.; Turner, David D.; Xie, Shaocheng; Zelenyuk, Alla; Bae, Kenny; Freer, Matthew; Glen, Andrew

    2011-02-01

    A comprehensive dataset of microphysical and radiative properties of aerosols and clouds in the arctic boundary layer in the vicinity of Barrow, Alaska was collected in April 2008 during the Indirect and Semi-Direct Aerosol Campaign (ISDAC) sponsored by the Department of Energy Atmospheric Radiation Measurement (ARM) and Atmospheric Science Programs. The primary aim of ISDAC was to examine indirect effects of aerosols on clouds that contain both liquid and ice water. The experiment utilized the ARM permanent observational facilities at the North Slope of Alaska (NSA) in Barrow. These include a cloud radar, a polarized micropulse lidar, and an atmospheric emitted radiance interferometer as well as instruments specially deployed for ISDAC measuring aerosol, ice fog, precipitation and spectral shortwave radiation. The National Research Council of Canada Convair-580 flew 27 sorties during ISDAC, collecting data using an unprecedented 42 cloud and aerosol instruments for more than 100 hours on 12 different days. Data were obtained above, below and within single-layer stratus on 8 April and 26 April 2008. These data enable a process-oriented understanding of how aerosols affect the microphysical and radiative properties of arctic clouds influenced by different surface conditions. Observations acquired on a heavily polluted day, 19 April 2008, are enhancing this understanding. Data acquired in cirrus on transit flights between Fairbanks and Barrow are improving our understanding of the performance of cloud probes in ice. Ultimately the ISDAC data will be used to improve the representation of cloud and aerosol processes in models covering a variety of spatial and temporal scales, and to determine the extent to which long-term surface-based measurements can provide retrievals of aerosols, clouds, precipitation and radiative heating in the Arctic.

  4. ARM Aerosol Working Group Meeting

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    - all sites * Aerosol Sampling - SGP, NSA, AMF - scattering, absorption, number, size ... (Germany, 2007) * Near Future: - ISDAC (NSA, 2008) - AMF (China, 2008) AWG Research ...

  5. ARM - Field Campaign - Aerosol IOP

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ... Analyzer Order Data Arnott Desert Research Institute - airborne photo-acoustic aerosol extinction Order Data Bucholtz Aircraft Solar and IR Radiometers Order Data Jonsson Passive ...

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    PDF Submitter: McComiskey, A. C., National Oceanic and Atmospheric Administration Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Aerosol Life Cycle,...

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Chamber Studies Uncover New Pathways for Atmospheric Aerosol Growth PI Contact: Smith, J., University of California, Irvine Area of Research: Aerosol Processes Working Group(s): ...

  8. ARM - Research Highlights: Notable Findings

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    HighlightsNotable Research Findings Form Submit a New Research Highlight Sort Highlights Submitter Title Research Area Working Group Submission Date DOE Progress Reports Notable Research Findings for 2001-2006 Office of Science Abstracts Database Research Highlights Summaries Notable Research Findings for the Past Five Years Aerosols Cloud Parameterization and Modeling (Currently Cloud Modeling) Cloud Properties Instantaneous Radiative Flux (Currently Radiative Processes)

  9. The Indirect and Semi-Direct Aerosol Campaign

    SciTech Connect (OSTI)

    Ghan, Steve

    2014-03-24

    Research projects like the Indirect and Semi-Direct Aerosol Campaign, or ISDAC, increase our knowledge of atmospheric aerosol particles and cloud physics.

  10. The Indirect and Semi-Direct Aerosol Campaign

    ScienceCinema (OSTI)

    Ghan, Steve

    2014-06-12

    Research projects like the Indirect and Semi-Direct Aerosol Campaign, or ISDAC, increase our knowledge of atmospheric aerosol particles and cloud physics.

  11. Los Alamos researchers uncover new properties in nanocomposite...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Los Alamos researchers uncover new properties in nanocomposite oxide ceramics for reactor fuel, fast-ion conductors In a nanocomposite, the size of each of these grains is on the ...

  12. Intellectual Property Provisions (CLB-115) Cooperative Agreement Research,

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Development, or Demonstration Large Business and Foreign Entity | Department of Energy CLB-115) Cooperative Agreement Research, Development, or Demonstration Large Business and Foreign Entity Intellectual Property Provisions (CLB-115) Cooperative Agreement Research, Development, or Demonstration Large Business and Foreign Entity CLB-115.pdf (46.18 KB) More Documents & Publications CLB-1003.PDF&#0; CDLB-1003.PDF&#0; Intellectual Property Provisions (CDLB-115) Cooperative Agreement

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Birth and Growth of an Aerosol Download a printable PDF Submitter: Fast, J. D., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: N/A An aerosol particle journey. New modeling approaches developed by a research team led by PNNL show how aerosol particles are born and grow to affect the atmosphere and ultimately climate. Tiny atmospheric aerosols are some of the most highly

  14. Aerosol Observing System (AOS) Handbook

    SciTech Connect (OSTI)

    Jefferson, A

    2011-01-17

    The Aerosol Observing System (AOS) is a suite of in situ surface measurements of aerosol optical and cloud-forming properties. The instruments measure aerosol properties that influence the earths radiative balance. The primary optical measurements are those of the aerosol scattering and absorption coefficients as a function of particle size and radiation wavelength and cloud condensation nuclei (CCN) measurements as a function of percent supersaturation. Additional measurements include those of the particle number concentration and scattering hygroscopic growth. Aerosol optical measurements are useful for calculating parameters used in radiative forcing calculations such as the aerosol single-scattering albedo, asymmetry parameter, mass scattering efficiency, and hygroscopic growth. CCN measurements are important in cloud microphysical models to predict droplet formation.

  15. Intellectual Property Provisions (GLB-115) Grant Research, Development, or

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Demonstration Large Business and Foreign Entity | Department of Energy GLB-115) Grant Research, Development, or Demonstration Large Business and Foreign Entity Intellectual Property Provisions (GLB-115) Grant Research, Development, or Demonstration Large Business and Foreign Entity GLB-115.pdf (42.57 KB) More Documents & Publications GLB-1003.PDF&#0; CLB-1003.PDF&#0; CDLB

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Roles of Wind Shear at Different Vertical Levels in Cloud System Organization and Properties Download a printable PDF Submitter: Fan, J., Pacific Northwest National Laboratory Area of Research: Cloud Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Chen Q, J Fan, S Hagos, W Gustafson, and L Berg. 2015. "Roles of wind shear at different vertical levels, Part I: Cloud system organization and properties." Journal of Geophysical Research -

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Dust Takes Detour on Ice-Cloud Journey Download a printable PDF Submitter: Kulkarni, G., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Kulkarni G, C Sanders, K Zhang, X Liu, and C Zhao. 2014. "Ice nucleation of bare and sulfuric acid-coated mineral dust particles and implication for cloud properties." Journal of Geophysical Research - Atmospheres, 119(16), doi:10.1002/2014JD021567. Cirrus clouds are

  18. Science Overview Document Indirect and Semi-Direct Aerosol Campaign (ISDAC) April 2008

    SciTech Connect (OSTI)

    SJ Ghan; B Schmid; JM Hubbe; CJ Flynn; A Laskin; AA Zelenyuk; DJ Czizco; CN Long; G McFarquhar; J Verlinde; J Harrington; JW Strapp; P Liu; A Korolev; A McDonald; M Wolde; A Fridlind; T Garrett; G Mace; G Kok; S Brooks; D Collins; D Lubin; P Lawson; M Dubey; C Mazzoleni; M Shupe; S Xie; DD Turner; Q Min; EJ Mlawer; D Mitchell

    2007-11-01

    The ARM Climate Research Facility’s (ACRF) Aerial Vehicle Program (AVP) will deploy an intensive cloud and aerosol observing system to the ARM North Slope of Alaska (NSA) locale for a five week Indirect and Semi-Direct Aerosol Campaign (ISDAC) during period 29 March through 30 April 2008. The deployment period is within the International Polar Year, thus contributing to and benefiting from the many ancillary observing systems collecting data synergistically. We will deploy the Canadian National Research Council Convair 580 aircraft to measure temperature, humidity, total particle number, aerosol size distribution, single particle composition, concentrations of cloud condensation nuclei and ice nuclei, optical scattering and absorption, updraft velocity, cloud liquid water and ice contents, cloud droplet and crystal size distributions, cloud particle shape, and cloud extinction. In addition to these aircraft measurements, ISDAC will deploy two instruments at the ARM site in Barrow: a spectroradiometer to retrieve cloud optical depth and effective radius, and a tandem differential mobility analyzer to measure the aerosol size distribution and hygroscopicity. By using many of the same instruments used during Mixed-Phase Arctic Cloud Experiment (M-PACE), conducted in October 2004, we will be able to contrast the arctic aerosol and cloud properties during the fall and spring transitions. The aerosol measurements can be used in cloud models driven by objectively analyzed boundary conditions to test whether the cloud models can simulate the aerosol influence on the clouds. The influence of aerosol and boundary conditions on the simulated clouds can be separated by running the cloud models with all four combinations of M-PACE and ISDAC aerosol and boundary conditions: M-PACE aerosol and boundary conditions, M-PACE aerosol and ISDAC boundary conditions, ISDAC aerosol and M-PACE boundary conditions, and ISDAC aerosol and boundary conditions. ISDAC and M-PACE boundary

  19. Intellectual Property Provisions (CSB-1003) Cooperative Agreement Research,

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Development, or Demonstration Domestic Small Businesses | Department of Energy 003) Cooperative Agreement Research, Development, or Demonstration Domestic Small Businesses Intellectual Property Provisions (CSB-1003) Cooperative Agreement Research, Development, or Demonstration Domestic Small Businesses 01. FAR 52.227-1 Authorization and Consent (JUL 1995)-Alternate I (APR 1984) 02. FAR 52.227-2 Notice and Assistance Regarding Patent and Copyright Infringement (AUG 1996) This clause is not

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Dependence of the Single-Scattering Properties of Small Ice Crystals on Idealized Shape Models Download a printable PDF Submitter: Um, J., University of Illinois, Urbana McFarquhar, G., University of Illinois, Urbana Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Um J and GM McFarquhar. 2011. "Dependence of the single-scattering properties of small ice crystals on idealized shape

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Factors Influencing the Microphysics and Radiative Properties of Liquid-Dominated Arctic Clouds Download a printable PDF Submitter: Earle, M., Environment Canada Liu, P., Environment Canada Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Earle ME, PS Liu, JW Strapp, A Zelenyuk, D Imre, GM McFarquhar, NC Shantz, and WR Leaitch. 2011. "Factors influencing the microphysics and radiative properties of

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Turn Trash Into Treasure: Continental Warm Cloud Properties Derived from Unexploited Solar Background Signals Download a printable PDF Submitter: Chiu, J., University of Reading Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Chiu JC, JA Holmes, RJ Hogan, and EJ O'Connor. 2014. "The interdependence of continental warm cloud properties derived from unexploited solar background signals in

  3. Los Alamos researchers uncover new properties in nanocomposite oxide

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ceramics for reactor fuel, fast-ion conductors New properties in nanocomposite oxide ceramics Los Alamos researchers uncover new properties in nanocomposite oxide ceramics for reactor fuel, fast-ion conductors In a nanocomposite, the size of each of these grains is on the order of nanometers, roughly 1000 times smaller than the width of a human hair. September 23, 2014 Schematic depicting distinct dislocation networks for SrO- and TiO2-terminated SrTiO3/MgO interface. Schematic depicting

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Isoprene Photochemistry over the Amazon Rainforest PI Contact: Martin, S. T., Harvard University Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Liu Y, J Brito, MR Dorris, JC Rivera-Rios, R Seco, KH Bates, P Artaxo, S Duvoisin JR, FN Keutsch, S Kim, AH Goldstein, AB Guenther, AO Manzi, RA Souza, SR Springston, TB Watson, KA McKinney, and ST Martin. 2016. "Isoprene photochemistry over the Amazon rainforest." Proceedings of the National

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Comparison of Mixed-layer Heights from Airborne HSRL and WRF-Chem During CARES Download a printable PDF Submitter: Scarino, A. J., Science Systems and Applications, Inc. Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Scarino AJ, MD Obland, JD Fast, SP Burton, RA Ferrare, CA Hostetler, LK Berg, B Lefer, C Haman, JW Hair, RR Rogers, C Butler, AL Cook, and DB Harper. 2014. "Comparison of mixed layer heights from airborne high spectral resolution

  6. Holistic Interactions of Shallow Clouds, Aerosols, and Land-Ecosystems (HI-SCALE) Science Plan

    SciTech Connect (OSTI)

    Fast, JD; Berg, LK

    2015-12-01

    Cumulus convection is an important component in the atmospheric radiation budget and hydrologic cycle over the Southern Great Plains and over many regions of the world, particularly during the summertime growing season when intense turbulence induced by surface radiation couples the land surface to clouds. Current convective cloud parameterizations contain uncertainties resulting in part from insufficient coincident data that couples cloud macrophysical and microphysical properties to inhomogeneities in boundary layer and aerosol properties. The Holistic Interactions of Shallow Clouds, Aerosols, and Land-Ecosystems (HI-SCALE) campaign is designed to provide a detailed set of measurements that are needed to obtain a more complete understanding of the life cycle of shallow clouds by coupling cloud macrophysical and microphysical properties to land surface properties, ecosystems, and aerosols. HI-SCALE consists of 2, 4-week intensive observational periods, one in the spring and the other in the late summer, to take advantage of different stages and distribution of “greenness” for various types of vegetation in the vicinity of the Atmospheric Radiation and Measurement (ARM) Climate Research Facility’s Southern Great Plains (SGP) site as well as aerosol properties that vary during the growing season. Most of the proposed instrumentation will be deployed on the ARM Aerial Facility (AAF) Gulfstream 1 (G-1) aircraft, including those that measure atmospheric turbulence, cloud water content and drop size distributions, aerosol precursor gases, aerosol chemical composition and size distributions, and cloud condensation nuclei concentrations. Routine ARM aerosol measurements made at the surface will be supplemented with aerosol microphysical properties measurements. The G-1 aircraft will complete transects over the SGP Central Facility at multiple altitudes within the boundary layer, within clouds, and above clouds.

  7. CARES: Carbonaceous Aerosol and Radiative Effects Study Science Plan

    SciTech Connect (OSTI)

    Zaveri, RA; Shaw, WJ; Cziczo, DJ

    2010-05-27

    Carbonaceous aerosol components, which include black carbon (BC), urban primary organic aerosols (POA), biomass burning aerosols, and secondary organic aerosols (SOA) from both urban and biogenic precursors, have been previously shown to play a major role in the direct and indirect radiative forcing of climate. The primary objective of the CARES 2010 intensive field study is to investigate the evolution of carbonaceous aerosols of different types and their effects on optical and cloud formation properties.

  8. CARES: Carbonaceous Aerosol and Radiative Effects Study Operations Plan

    SciTech Connect (OSTI)

    Zaveri, RA; Shaw, WJ; Cziczo, DJ

    2010-07-12

    The CARES field campaign is motivated by the scientific issues described in the CARES Science Plan. The primary objectives of this field campaign are to investigate the evolution and aging of carbonaceous aerosols and their climate-affecting properties in the urban plume of Sacramento, California, a mid-size, mid-latitude city that is located upwind of a biogenic volatile organic compound (VOC) emission region. Our basic observational strategy is to make comprehensive gas, aerosol, and meteorological measurements upwind, within, and downwind of the urban area with the DOE G-1 aircraft and at strategically located ground sites so as to study the evolution of urban aerosols as they age and mix with biogenic SOA precursors. The NASA B-200 aircraft, equipped with the High Spectral Resolution Lidar (HSRL), digital camera, and the Research Scanning Polarimeter (RSP), will be flown in coordination with the G-1 to characterize the vertical and horizontal distribution of aerosols and aerosol optical properties, and to provide the vertical context for the G-1 and ground in situ measurements.

  9. ARM - Measurement - Aerosol optical depth

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Sky-Scanning, Sun Tracking Atmospheric Research SAM : Sun and Aureole Measurement UAV-GNAT : UAV-General Atomics GNAT Value-Added Products AOD : Aerosol Optical Depth, derived from ...

  10. ARM - Two-Column Aerosol Project (TCAP)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    science objectives, the Atmospheric Radiation Measurement (ARM) Climate Research Facility will deploy the ARM Mobile Facility and the Mobile Aerosol Observing System on Cape...

  11. Chemical composition, microstructure, and hygroscopic properties of aerosol particles at the Zotino Tall Tower Observatory (ZOTTO), Siberia, during a summer campaign

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Mikhailov, E. F.; Mironov, G. N.; Pöhlker, C.; Chi, X.; Krüger, M. L.; Shiraiwa, M.; Förster, J. -D.; Pöschl, U.; Vlasenko, S. S.; Ryshkevich, T. I.; et al

    2015-03-16

    In this study we describe the hygroscopic properties of accumulation- and coarse-mode aerosol particles sampled at the Zotino Tall Tower Observatory (ZOTTO) in Central Siberia (61° N; 89° E) from 16 to 21 June 2013. The hygroscopic growth measurements were supplemented with chemical analyses of the samples, including inorganic ions and organic/elemental carbon. In addition, the microstructure and chemical composition of aerosol particles were analyzed by X-ray micro-spectroscopy (STXM-NEXAFS) and transmission electron microscopy (TEM). A mass closure analysis indicates that organic carbon accounted for 61 and 38% of PM in the accumulation mode and coarse mode, respectively. The water solublemore » fraction of organic matter was estimated to be 52 and 8% of PM in these modes. Sulfate, predominantly in the form of ammoniated sulfate, was the dominant inorganic component in both size modes: ~ 34% in the accumulation vs. ~ 47% in the coarse mode. The hygroscopic growth measurements were conducted with a filter-based differential hygroscopicity analyzer (FDHA) over the range of 5–99.4% RH in the hydration and dehydration operation modes. The FDHA study indicates that both accumulation and coarse modes exhibit pronounced water uptake approximately at the same RH, starting at ~ 70%, while efflorescence occurred at different humidities, i.e., at ~ 35% RH for submicron particles vs. ~ 50% RH for supermicron particles. This ~ 15% RH difference was attributed to higher content of organic material in the submicron particles, which suppresses water release in the dehydration experiments. The kappa mass interaction model (KIM) was applied to characterize and parameterize non-ideal solution behavior and concentration-dependent water uptake by atmospheric aerosol samples in the 5–99.4% RH range. Based on KIM, the volume-based hygroscopicity parameter, κv, was calculated. The κv, ws value related to the water soluble (ws) fraction was estimated to be ~ 0.15 for the

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Study Aerosol Humidity Effects Using the ARM Measurements Submitter: Li, Z., University of Maryland Area of Research: Radiation Processes Working Group(s): Aerosol Journal Reference: Jeong, M.-J., Z. Li, E. Andrews, and S.-C. Tsay (2007). Effect of aerosol humidification on the column aerosol optical thickness over the Atmospheric Radiation Measurement Southern Great Plains site, J. Geophys. Res., 112, D10202, doi:10.1029/2006JD007176. (a)-(j) Column-mean aerosol humidification factor as

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    A Dance of Aerosols Download a printable PDF Submitter: Song, C., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Song C, RA Zaveri, JE Shilling, ML Alexander, and M Newburn. 2011. "Effect of hydrophilic organic seed aerosols on secondary organic aerosol formation from ozonolysis of α-pinene." Environmental Science & Technology, 45(17), doi:10.1021/es201225c. The injection of alpha-pinene, a

  14. Assessing regional scale predictions of aerosols, marine stratocumulus, and their interactions during VOCALS-REx using WRF-Chem

    SciTech Connect (OSTI)

    Yang Q.; Lee Y.; Gustafson Jr., W. I.; Fast, J. D.; Wang, H.; Easter, R. C.; Morrison, H.; Chapman, E. G.; Spak, S. N.; Mena-Carrasco, M. A.

    2011-12-02

    This study assesses the ability of the recent chemistry version (v3.3) of the Weather Research and Forecasting (WRF-Chem) model to simulate boundary layer structure, aerosols, stratocumulus clouds, and energy fluxes over the Southeast Pacific Ocean. Measurements from the VAMOS Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-REx) and satellite retrievals (i.e., products from the MODerate resolution Imaging Spectroradiometer (MODIS), Clouds and Earth's Radiant Energy System (CERES), and GOES-10) are used for this assessment. The Morrison double-moment microphysics scheme is newly coupled with interactive aerosols in the model. The 31-day (15 October-16 November 2008) WRF-Chem simulation with aerosol-cloud interactions (AERO hereafter) is also compared to a simulation (MET hereafter) with fixed cloud droplet number concentrations in the microphysics scheme and simplified cloud and aerosol treatments in the radiation scheme. The well-simulated aerosol quantities (aerosol number, mass composition and optical properties), and the inclusion of full aerosol-cloud couplings lead to significant improvements in many features of the simulated stratocumulus clouds: cloud optical properties and microphysical properties such as cloud top effective radius, cloud water path, and cloud optical thickness. In addition to accounting for the aerosol direct and semi-direct effects, these improvements feed back to the simulation of boundary-layer characteristics and energy budgets. Particularly, inclusion of interactive aerosols in AERO strengthens the temperature and humidity gradients within the capping inversion layer and lowers the marine boundary layer (MBL) depth by 130 m from that of the MET simulation. These differences are associated with weaker entrainment and stronger mean subsidence at the top of the MBL in AERO. Mean top-of-atmosphere outgoing shortwave fluxes, surface latent heat, and surface downwelling longwave fluxes are in better agreement with observations

  15. Direct Aerosol Forcing: Sensitivity to Uncertainty in Measurements of

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Optical and Situational Properties Direct Aerosol Forcing: Sensitivity to Uncertainty in Measurements of Aerosol Optical and Situational Properties McComiskey, Allison CIRES / NOAA Schwartz, Stephen Brookhaven National Laboratory Ricchiazzi, Paul University of California, Santa Barbara Lewis, Ernie Brookhaven National Laboratory Michalsky, Joseph DOC/NOAA/OAR/ESRL/GMD Ogren, John NOAA/CMDL Category: Radiation Understanding sources of uncertainty in estimating aerosol direct radiative

  16. eDPS Aerosol Collection

    SciTech Connect (OSTI)

    Venzie, J.

    2015-10-13

    The eDPS Aerosol Collection project studies the fundamental physics of electrostatic aerosol collection for national security applications. The interpretation of aerosol data requires understanding and correcting for biases introduced from particle genesis through collection and analysis. The research and development undertaken in this project provides the basis for both the statistical correction of existing equipment and techniques; as well as, the development of new collectors and analytical techniques designed to minimize unwanted biases while improving the efficiency of locating and measuring individual particles of interest.

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Capturing Biogenic Volatile Organic Compounds in a Coupled-Model System Compared to Observation PI Contact: Zhao, C., Pacific Northwest National Laboratory Area of Research: Surface Properties Working Group(s): Aerosol Life Cycle Journal Reference: Zhao C, M Huang, JD Fast, LK Berg, Y Qian, A Guenther, D Gu, M Shrivastava, Y Liu, S Walters, G Pfister, J Jin, JE Shilling, and C Warneke. 2016. "Sensitivity of biogenic volatile organic compounds to land surface parameterizations and vegetation

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    General Formulation for Representing Cloud-to-Rain Transition in Atmospheric Models Submitter: Liu, Y., Brookhaven National Laboratory Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Aerosol, Cloud Modeling, Cloud Properties Journal Reference: Liu, Y., P. H. Daum, R. McGraw, M. Miller, and S. Niu, 2007: Theoretical formulation for autoconversion rate of cloud droplet concentration. Geophys. Res. Lett., 34, L116821, doi:10.1029/2007GL030389

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    SGP Observations Help Validate Soil Temperature Simulations Download a printable PDF Submitter: Huang, M., Pacific Northwest National Laboratory Area of Research: Surface Properties Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Xia Y, M Ek, J Sheffield, B Livneh, M Huang, H Wei, S Feng, L Luo, J Meng, and E Wood. 2012. "Validation of Noah-simulated soil temperature in the North American Land Data Assimilation System Phase 2." Journal of Applied

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ground Stations Likely Get a Boost from Satellites to Estimate Carbon Dioxide Emissions Download a printable PDF Submitter: Roeder, L. R., Pacific Northwest National Laboratory Area of Research: Surface Properties Working Group(s): Aerosol Life Cycle Journal Reference: Basu S, S Guerlet, A Butz, S Houweling, OP Hasekamp, I Aben, PB Krummel, LP Steele, RL Langenfelds, MS Torn, SC Biraud, B Stephens, A Andrews, and D Worthy. 2013. "Global CO2 fluxes estimated from GOSAT retrievals of total

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Growing More Effective Ways to Measure Climate Change Download a printable PDF Submitter: Maseyk, K. S., Universite Pierre et Marie Curie, Paris 6 Area of Research: Surface Properties Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Maseyk K, JA Berry, D Billesbach, JE Campbell, MS Torn, M Zahniser, and U Seibt. 2014. "Sources and sinks of carbonyl sulfide in an agricultural field in the Southern Great Plains." Proceedings of the National Academy of

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    A Lidar View of Clouds in Southeastern China Download a printable PDF Submitter: Li, Z., University of Maryland Cribb, M. C., University of Maryland Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Liu J, Z Li, Y Zheng, and M Cribb. 2015. "Cloud-Base Distribution and Cirrus Properties Based on Micropulse Lidar Measurements at a Site in Southeastern China." Advances in Atmospheric Sciences, 32(7),

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Kulkarni G, S China, S Liu, M Nandasiri, N Sharma, J Wilson, AC Aiken, D Chand, A ...

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    To Rain or Not to Rain...Aerosols May Be the Answer Download a printable PDF Submitter: Li, Z., University of Maryland Area of Research: Cloud-Aerosol-Precipitation Interactions...

  5. The CU 2-D-MAX-DOAS instrument – Part 2: Raman scattering probability measurements and retrieval of aerosol optical properties

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Ortega, Ivan; Coburn, Sean; Berg, Larry K.; Lantz, Kathy; Michalsky, Joseph; Ferrare, Richard A.; Hair, Johnathan W.; Hostetler, Chris A.; Volkamer, Rainer

    2016-08-23

    The multiannual global mean of aerosol optical depth at 550 nm (AOD550) over land is ∼ 0.19, and that over oceans is ∼ 0.13. About 45 % of the Earth surface shows AOD550 smaller than 0.1. There is a need for measurement techniques that are optimized to measure aerosol optical properties under low AOD conditions. We present an inherently calibrated retrieval (i.e., no need for radiance calibration) to simultaneously measure AOD and the aerosol phase function parameter, g, based on measurements of azimuth distributions of the Raman scattering probability (RSP), the near-absolute rotational Raman scattering (RRS) intensity. We employ radiative transfer model simulations tomore » show that for solar azimuth RSP measurements at solar elevation and solar zenith angle (SZA) smaller than 80°, RSP is insensitive to the vertical distribution of aerosols and maximally sensitive to changes in AOD and g under near-molecular scattering conditions. The University of Colorado two-dimensional Multi-AXis Differential Optical Absorption Spectroscopy (CU 2-D-MAX-DOAS) instrument was deployed as part of the Two Column Aerosol Project (TCAP) at Cape Cod, MA, during the summer of 2012 to measure direct sun spectra and RSP from scattered light spectra at solar relative azimuth angles (SRAAs) between 5 and 170°. During two case study days with (1) high aerosol load (17 July, 0.3  <  AOD430 < 0.6) and (2) near-molecular scattering conditions (22 July, AOD430 < 0.13) we compare RSP-based retrievals of AOD430 and g with data from a co-located CIMEL sun photometer, Multi-Filter Rotating Shadowband Radiometer (MFRSR), and an airborne High Spectral Resolution Lidar (HSRL-2). The average difference (relative to DOAS) for AOD430 is +0.012 ± 0.023 (CIMEL), −0.012 ± 0.024 (MFRSR), −0.011 ± 0.014 (HSRL-2), and +0.023 ± 0.013 (CIMELAOD − MFRSRAOD) and yields the following expressions for correlations between different instruments

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Brass Ring of Climate Modeling Download a printable PDF Submitter: Ghan, S. J., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Ghan SJ, SJ Smith, M Wang, K Zhang, K Pringle, K Carslaw, J Pierce, S Bauer, and P Adams. 2013. "A simple model of global aerosol indirect effects." Journal of Geophysical Research - Atmospheres, 118, 1-20. The simple model of aerosol effects on clouds

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Invisible Giants in the Sky Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Kassianov E, M Pekour, and J Barnard. 2012. "Aerosols in central California: Unexpectedly large contribution of coarse mode to aerosol radiative forcing." Geophysical Research Letters, 39, L20806, doi:10.1029/2012GL053469. Photo

  8. Ganges Valley Aerosol Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ganges Valley Aerosol Experiment In northeastern India, the fertile land around the Ganges River supports several hundred million people. This river, the largest in India, is fed by monsoon rains and runoff from the nearby Himalayan Mountains. Through an intergovernmental agreement with India, the U.S. Department of Energy's Atmospheric Radiation Measurement (ARM) Climate Research Facility deployed its portable laboratory, the ARM Mobile Facility (AMF), to Nainital, India, in June 2011. During

  9. Cloud Properties Derived from Visible and Near-infrared Reflectance in the

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Presence of Aerosols Cloud Properties Derived from Visible and Near-infrared Reflectance in the Presence of Aerosols Hofmann, Odele University of Colorado at Boulder Pilewskie, Peter University of Colorado Gore, Warren NASA Ames Research Center Russell, Phil NASA Ames Research Center Livingston, John SRI International Redemann, Jens BAERI/NASA Ames Research Center Bergstrom, Robert Bay Area Environmental Research Institute Platnick, Steven NASA-GSFC Daniel, John NOAA Aeronomy Laboratory

  10. Chemical composition, microstructure, and hygroscopic properties of aerosol particles at the Zotino Tall Tower Observatory (ZOTTO), Siberia, during a summer campaign

    SciTech Connect (OSTI)

    Mikhailov, E. F.; Mironov, G. N.; Pöhlker, C.; Chi, X.; Krüger, M. L.; Shiraiwa, M.; Förster, J. -D.; Pöschl, U.; Vlasenko, S. S.; Ryshkevich, T. I.; Weigand, M.; Kilcoyne, A. L. D.; Andreae, M. O.

    2015-03-16

    In this study we describe the hygroscopic properties of accumulation- and coarse-mode aerosol particles sampled at the Zotino Tall Tower Observatory (ZOTTO) in Central Siberia (61° N; 89° E) from 16 to 21 June 2013. The hygroscopic growth measurements were supplemented with chemical analyses of the samples, including inorganic ions and organic/elemental carbon. In addition, the microstructure and chemical composition of aerosol particles were analyzed by X-ray micro-spectroscopy (STXM-NEXAFS) and transmission electron microscopy (TEM). A mass closure analysis indicates that organic carbon accounted for 61 and 38% of PM in the accumulation mode and coarse mode, respectively. The water soluble fraction of organic matter was estimated to be 52 and 8% of PM in these modes. Sulfate, predominantly in the form of ammoniated sulfate, was the dominant inorganic component in both size modes: ~ 34% in the accumulation vs. ~ 47% in the coarse mode.

    The hygroscopic growth measurements were conducted with a filter-based differential hygroscopicity analyzer (FDHA) over the range of 5–99.4% RH in the hydration and dehydration operation modes. The FDHA study indicates that both accumulation and coarse modes exhibit pronounced water uptake approximately at the same RH, starting at ~ 70%, while efflorescence occurred at different humidities, i.e., at ~ 35% RH for submicron particles vs. ~ 50% RH for supermicron particles. This ~ 15% RH difference was attributed to higher content of organic material in the submicron particles, which suppresses water release in the dehydration experiments.

    The kappa mass interaction model (KIM) was applied to characterize and parameterize non-ideal solution behavior and concentration-dependent water uptake by atmospheric aerosol samples in the 5–99.4% RH range. Based on KIM, the volume-based hygroscopicity parameter, κv, was calculated. The κv, ws value related to the water soluble (ws) fraction was

  11. ARM - Measurement - Aerosol concentration

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    CSPHOT : Cimel Sunphotometer CPC : Condensation Particle Counter HTDMA : Humidified Tandem Differential Mobility Analyzer IAP : In-situ Aerosol Profiles (Cessna Aerosol Flights)...

  12. ARM - Field Campaign - Two-Column Aerosol Project (TCAP): Winter...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    on atmospheric particulate matter. The effect of aerosol properties such as size, morphology and composition on cloud droplet formation has been studied theoretically as well as...

  13. Preliminary Results of in-situ Measurements of Aerosol Optical...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    of Aerosol Optical and Water Uptake Properties from the ARM Mobile Facility in Niger Jefferson, Anne NOAA CMDL Ogren, John NOAACMDL Category: Field Campaigns The second...

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Simulating the Impact of Aerosols on Tropical Deep Convection Download a printable PDF Submitter: Morrison, H. C., NCAR Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Morrison H and WW Grabowski. 2011. "Cloud-system resolving model simulations of aerosol indirect effects on tropical deep convection and its thermodynamic environment." Atmospheric Chemistry and Physics, 11(20),

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Carbonaceous Aerosol Aging Mechanisms Improve Agreement of Global Simulations with Data Download a printable PDF Submitter: Dubey, M. K., Los Alamos National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: N/A Longitudinal and vertical distribution of global zonal mean hydrophobic to hydrophilic conversion time for carbonaceous aerosols with new laboratory aging mechanism. Impact of new aging mechanism on global zonal mean black carbon

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Scale Shows True Weight of Aerosol Effects on Clouds Download a printable PDF Submitter: McComiskey, A. C., National Oceanic and Atmospheric Administration Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: McComiskey A and G Feingold. 2012. "The scale problem in quantifying aerosol indirect effects." Atmospheric Chemistry and Physics, 12, doi:10.5194/acp-12-1031-2012. Differing values: Values derived from aircraft and surface observations,

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Mixing State of Carbonaceous Aerosol Particles in Northern and Southern California Measured During CARES and CalNex Download a printable PDF Submitter: Zaveri, R., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Cahill JF, K Suski, JH Seinfeld, RA Zaveri, and KA Prather. 2012. "The mixing state of carbonaceous aerosol particles in Northern and Southern California measured during CARES and CalNex

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Modeling Aerosols in Fair-Weather Clouds During CHAPS Download a printable PDF Submitter: Shrivastava, M., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Shrivastava M, LK Berg, J Fast, R Easter, A Laskin, WI Gustafson, Y Liu, and CM Berkowitz. 2013. "Modeling aerosols and their interactions with shallow cumuli during the 2007 CHAPS field study." Journal of

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Arctic Winter Frost Flowers Have Negligible Influence on Cloud Longwave Warming Download a printable PDF Submitter: Xu, L., University of California, San Diego Russell, L. M., Scripps Institution of Oceanography Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Xu L, LM Russell, RC Somerville, and PK Quinn. 2013. "Frost flower aerosol effects on Arctic wintertime longwave cloud radiative forcing."

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Parameterizing the Mixing State of Complex Submicron Aerosols Using Chemical Imaging Download a printable PDF Submitter: Moffet, R., University of the Pacific Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: O'Brien RE, B Wang, A Laskin, N Riemer, M West, Q Zhang, Y Sun, X Yu, P Alpert, DA Knopf, MK Gilles, and RC Moffet. 2015. "Chemical imaging of ambient aerosol particles: Observational constraints on mixing state parameterization." Journal

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosols Help Clouds Warm Up Arctic Submitter: Lubin, D., Scripps Institution of Oceanography Area of Research: Radiation Processes Working Group(s): Radiative Processes Journal Reference: Lubin, D., and A.M. Vogelmann, 2006: A climatologically significant aerosol longwave indirect effect in the Arctic, Nature, 439, 26 January, 453-456, doi:10.1038/nature04449 In a process known as the first aerosol indirect effect, enhanced aerosol concentrations cause the droplets in a cloud to be smaller and

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Observations of Microphysical Properties of Single-Layer Stratocumulus During the Mixed-Phase Arctic Cloud Experiment Submitter: McFarquhar, G., University of Illinois, Urbana Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Fridlind, A.M., A.S. Ackerman, G.M. McFarquhar, G. Zhang, M.R. Poellot, P.J. DeMott, A.J. Prenni and A.J. Heymsfield, 2007: Ice properties of single-layer stratocumulus during the

  3. Aerosol Characterization Data from the Asian Pacific Regional Aerosol Characterization Project (ACE-Asia)

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    The Aerosol Characterization Experiments (ACE) were designed to increase understanding of how atmospheric aerosol particles affect the Earth's climate system. These experiments integrated in-situ measurements, satellite observations, and models to reduce the uncertainty in calculations of the climate forcing due to aerosol particles and improve the ability of models to predict the influences of aerosols on the Earth's radiation balance. ACE-Asia was the fourth in a series of experiments organized by the International Global Atmospheric Chemistry (IGAC) Program (A Core Project of the International Geosphere Biosphere Program). The Intensive Field Phase for ACE-Asia took place during the spring of 2001 (mid-March through early May) off the coast of China, Japan and Korea. ACE-Asia pursued three specific objectives: 1) Determine the physical, chemical, and radiative properties of the major aerosol types in the Eastern Asia and Northwest Pacific region and investigate the relationships among these properties. 2) Quantify the physical and chemical processes controlling the evolution of the major aerosol types and in particular their physical, chemical, and radiative properties. 3) Develop procedures to extrapolate aerosol properties and processes from local to regional and global scales, and assess the regional direct and indirect radiative forcing by aerosols in the Eastern Asia and Northwest Pacific region [Edited and shortened version of summary at http://data.eol.ucar.edu/codiac/projs?ACE-ASIA]. The Ace-Asia collection contains 174 datasets.

  4. Particulate Matter Aerosols

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    particulate matter aerosols Particulate Matter Aerosols The study of atmospheric aerosols is important because of its adverse effects on health, air quality, visibility, cultural heritage, and Earth's radiation balance. Techniques that can help better characterize particulate matter are required to better understand the constituents, causes and sources of particulate matter (PM) aerosols. Carbon is one of the main constituents of atmospheric aerosols. Radiocarbon (14C) measurement performed on

  5. Final Technical Report for Collaborative Research: CRI-EaSM Multiscale Modeling Aerosol Indirect Effects on Decadal Timescales

    SciTech Connect (OSTI)

    Park, Sungsu

    2015-11-29

    Originally, the main role of the P.I. (Sungsu Park) in this project was to improve the treatment of cloud microphysics in the CAM5 shallow and deep convection scheme. During the progress of the project, however, the main research theme was changed to develop a new unified convection scheme (so called, UNICON) with the permission of the program manager.

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    a printable PDF Submitter: Marshak, A., NASA - Goddard Space Flight Center Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions...

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Burning on the Prairies Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation...

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Long-Term Impacts of Aerosols on the Vertical Development of Clouds and Precipitation Download a printable PDF Submitter: Li, Z., University of Maryland Area of Research:...

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    to Lose Download a printable PDF Submitter: Laskin, A., Pacific Northwest National Laboratory Fast, J. ., Pacific Northwest National Laboratory Area of Research: Aerosol...

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Fog and Rain in the Amazon Download a printable PDF Submitter: Gentine, P., Columbia University Sobel, A., Columbia University Area of Research: Cloud-Aerosol-Precipitation...

  11. Study of Mechanisms of Aerosol Indirect Effects on Glaciated...

    Office of Scientific and Technical Information (OSTI)

    ... clouds, was seen to be of higher importance in regulating aerosol indirect effects ... DOE Contract Number: SC0007396 Resource Type: Technical Report Research Org: Leeds ...

  12. ARM - Field Campaign - Pajarito Aerosol Coupling to Ecosystems...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    woodland site used for DOE sponsored ecosystem research to measure the aerosol life ... PACE will measure changes in biogenic volatile organic from PJ ecosystem, the ...

  13. Light Absorption of Primary Organic Aerosol Paper Named ACS Editors...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Absorption of Primary Organic Aerosol Paper Named ACS Editors' Choice For original submission and image(s), see ARM Research Highlights http:www.arm.govsciencehighlights...

  14. Predicting Aerosol Direct Radiative Forcing over Mexico using...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Use Weather Research and Forecasting (WRF) model as the foundation of computational framework * Fully-coupled aerosol-radiation-cloud-chemistry interactions * Handles multiple ...

  15. BAECC Biogenic Aerosols - Effects on Clouds and Climate (Technical...

    Office of Scientific and Technical Information (OSTI)

    The main research goal was to understand the role of biogenic aerosols in cloud formation. ... Country of Publication: United States Language: English Subject: 54 ENVIRONMENTAL SCIENCES ...

  16. Characterization of aerosols produced by surgical procedures

    SciTech Connect (OSTI)

    Yeh, H.C.; Muggenburg, B.A.; Lundgren, D.L.; Guilmette, R.A.; Snipes, M.B.; Jones, R.K.; Turner, R.S.

    1994-07-01

    In many surgeries, especially orthopedic procedures, power tools such as saws and drills are used. These tools may produce aerosolized blood and other biological material from bone and soft tissues. Surgical lasers and electrocautery tools can also produce aerosols when tissues are vaporized and condensed. Studies have been reported in the literature concerning production of aerosols during surgery, and some of these aerosols may contain infectious material. Garden et al. (1988) reported the presence of papilloma virus DNA in the fumes produced from laser surgery, but the infectivity of the aerosol was not assessed. Moon and Nininger (1989) measured the size distribution and production rate of emissions from laser surgery and found that particles were generally less than 0.5 {mu}m diameter. More recently there has been concern expressed over the production of aerosolized blood during surgical procedures that require power tools. In an in vitro study, the production of an aerosol containing the human immunodeficiency virus (HIV) was reported when power tools were used to cut tissues with blood infected with HIV. Another study measured the size distribution of blood aerosols produced by surgical power tools and found blood-containing particles in a number of size ranges. Health care workers are anxious and concerned about whether surgically produced aerosols are inspirable and can contain viable pathogens such as HIV. Other pathogens such as hepatitis B virus (HBV) are also of concern. The Occupational Safety and Health funded a project at the National Institute for Inhalation Toxicology Research Institute to assess the extent of aerosolization of blood and other tissues during surgical procedures. This document reports details of the experimental and sampling approach, methods, analyses, and results on potential production of blood-associated aerosols from surgical procedures in the laboratory and in the hospital surgical suite.

  17. Aerosol mobility size spectrometer

    DOE Patents [OSTI]

    Wang, Jian; Kulkarni, Pramod

    2007-11-20

    A device for measuring aerosol size distribution within a sample containing aerosol particles. The device generally includes a spectrometer housing defining an interior chamber and a camera for recording aerosol size streams exiting the chamber. The housing includes an inlet for introducing a flow medium into the chamber in a flow direction, an aerosol injection port adjacent the inlet for introducing a charged aerosol sample into the chamber, a separation section for applying an electric field to the aerosol sample across the flow direction and an outlet opposite the inlet. In the separation section, the aerosol sample becomes entrained in the flow medium and the aerosol particles within the aerosol sample are separated by size into a plurality of aerosol flow streams under the influence of the electric field. The camera is disposed adjacent the housing outlet for optically detecting a relative position of at least one aerosol flow stream exiting the outlet and for optically detecting the number of aerosol particles within the at least one aerosol flow stream.

  18. Priorities for In-situ Aerosol Measurements

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Priorities for In-situ Aerosol Measurements Parameters * Aerosol light absorption coefficient - spectral, including UV, vis, and IR - as f(RH), and at ambient RH * Phase function - or relevant integral properties (how many?) * Ice nuclei * Scattering vs. RH, for RH>90% * CCN, as f(S, D p ) * Size distribution * Chemical composition - for determining climate forcing, vs. radiative effect Calibration * Number concentration * Size and shape * Light absorption reference method Characterization *

  19. Laboratory Studies of Processing of Carbonaceous Aerosols by Atmospheric Oxidants/Hygroscopicity and CCN Activity of Secondary & Processed Primary Organic Aerosols

    SciTech Connect (OSTI)

    Ziemann, P.J.; Arey, J.; Atkinson, R.; Kreidenweis, S.M.; Petters, M.D.

    2012-06-13

    The atmosphere is composed of a complex mixture of gases and suspended microscopic aerosol particles. The ability of these particles to take up water (hygroscopicity) and to act as nuclei for cloud droplet formation significantly impacts aerosol light scattering and absorption, and cloud formation, thereby influencing air quality, visibility, and climate in important ways. A substantial, yet poorly characterized component of the atmospheric aerosol is organic matter. Its major sources are direct emissions from combustion processes, which are referred to as primary organic aerosol (POA), or in situ processes in which volatile organic compounds (VOCs) are oxidized in the atmosphere to low volatility reaction products that subsequent condense to form particles that are referred to as secondary organic aerosol (SOA). POA and VOCs are emitted to the atmosphere from both anthropogenic and natural (biogenic) sources. The overall goal of this experimental research project was to conduct laboratory studies under simulated atmospheric conditions to investigate the effects of the chemical composition of organic aerosol particles on their hygroscopicity and cloud condensation nucleation (CCN) activity, in order to develop quantitative relationships that could be used to more accurately incorporate aerosol-cloud interactions into regional and global atmospheric models. More specifically, the project aimed to determine the products, mechanisms, and rates of chemical reactions involved in the processing of organic aerosol particles by atmospheric oxidants and to investigate the relationships between the chemical composition of organic particles (as represented by molecule sizes and the specific functional groups that are present) and the hygroscopicity and CCN activity of oxidized POA and SOA formed from the oxidation of the major classes of anthropogenic and biogenic VOCs that are emitted to the atmosphere, as well as model hydrocarbons. The general approach for this project was

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Pollution + Storm Clouds = Warmer Atmosphere Download a printable PDF Submitter: Fan, J., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Fan J, D Rosenfeld, Y Ding, L Leung, and Z Li. 2012. "Potential aerosol indirect effects on atmospheric circulation and radiative forcing through deep convection." Geophysical Research Letters, 39, L09806,

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    "Invisible" Giants in the Sky Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Kassianov E, M Pekour, and J Barnard. 2012. "Aerosols in central California: Unexpectedly large contribution of coarse mode to aerosol radiative forcing." Geophysical Research Letters, 39, L20806, doi:10.1029/2012GL053469. Daily averaged values of (a, b) the direct

  2. ARM - Measurement - Aerosol image

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    would love to hear from you Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol image Images of aerosols from which one can derive characteristics such...

  3. ARM - Measurement - Aerosol extinction

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol extinction The removal of radiant energy from an incident beam by the process of aerosol absorption ...

  4. ARM - Measurement - Aerosol scattering

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    : Nephelometer PASS : Photoacoustic Soot Spectrometer RL : Raman Lidar TDMA : Tandem Differential Mobility Analyzer Field Campaign Instruments AMT : Aerosol Modeling...

  5. Storm Peak Lab Cloud Property Validation

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Peak Lab Cloud Property Validation Experiment (STORMVEX) Operated by the Atmospheric Radiation Measurement (ARM) Climate Research Facility for the U.S. Department of Energy, the second ARM Mobile Facility (AMF2) begins its inaugural deployment November 2010 in Steamboat Springs, Colorado, for the Storm Peak Lab Cloud Property Validation Experiment, or STORMVEX. For six months, the comprehensive suite of AMF2 instruments will obtain measurements of cloud and aerosol properties at various sites

  6. Solid aerosol generator

    DOE Patents [OSTI]

    Prescott, Donald S.; Schober, Robert K.; Beller, John

    1992-01-01

    An improved solid aerosol generator used to produce a gas borne stream of dry, solid particles of predetermined size and concentration. The improved solid aerosol generator nebulizes a feed solution of known concentration with a flow of preheated gas and dries the resultant wet heated aerosol in a grounded, conical heating chamber, achieving high recovery and flow rates.

  7. Improved solid aerosol generator

    DOE Patents [OSTI]

    Prescott, D.S.; Schober, R.K.; Beller, J.

    1988-07-19

    An improved solid aerosol generator used to produce a gas borne stream of dry, solid particles of predetermined size and concentration. The improved solid aerosol generator nebulizes a feed solution of known concentration with a flow of preheated gas and dries the resultant wet heated aerosol in a grounded, conical heating chamber, achieving high recovery and flow rates. 2 figs.

  8. Solid aerosol generator

    DOE Patents [OSTI]

    Prescott, D.S.; Schober, R.K.; Beller, J.

    1992-03-17

    An improved solid aerosol generator used to produce a gas borne stream of dry, solid particles of predetermined size and concentration is disclosed. The improved solid aerosol generator nebulizes a feed solution of known concentration with a flow of preheated gas and dries the resultant wet heated aerosol in a grounded, conical heating chamber, achieving high recovery and flow rates. 2 figs.

  9. Aerosol distribution apparatus

    DOE Patents [OSTI]

    Hanson, W.D.

    An apparatus for uniformly distributing an aerosol to a plurality of filters mounted in a plenum, wherein the aerosol and air are forced through a manifold system by means of a jet pump and released into the plenum through orifices in the manifold. The apparatus allows for the simultaneous aerosol-testing of all the filters in the plenum.

  10. Building America Webinar: Sealing of Home Enclosures with Aerosol Particles

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    | Department of Energy Sealing of Home Enclosures with Aerosol Particles Building America Webinar: Sealing of Home Enclosures with Aerosol Particles This webinar was presented by research team Building Industry Research Alliance (BIRA), and provided information about a project that uses existing aerosol duct sealing technology to seal the entire building enclosure in order to achieve greater airtightness and energy and cost savings. webinar_bira_20111014.wmv (11.57 MB) More Documents &

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Seasonal and Interannual Variability in 13C of Ecosystem Carbon Fluxes from 2002-2009 Submitter: Torn, M. S., Lawrence Berkeley National Laboratory Area of Research: Surface Properties Working Group(s): Aerosol Life Cycle Journal Reference: Torn MS, SC Biraud, CJ Still, WJ Riley, and JA Berry. 2011. "Seasonal and inter-annual variability in δ13C of net ecosystem carbon exchanges from 2002-2009 in the U.S. Southern Great Plains." Tellus, 63(2), 10.1111/j.1600-0889.2010.00519.x. Time

  12. Research Highlights Sorted by Working Group

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Working Group Aerosol Life Cycle | Cloud Life Cycle | Cloud-Aerosol-Precipitation Interactions | Aerosol | Cloud Modeling | Cloud Properties | Radiative Processes Aerosol Life Cycle 2016 Berg, L. Two-Column Aerosol Project: Impact of Elevated Particle Layers on Particle Optical Depth ASR Ching, J. Three Dimensions Are Better Than Two, When It Comes to Representing Aerosols ASR de Boer, G. An Update on Unmanned Platforms at Oliktok Point ARM ASR Fast, J. D. Impact of External Industrial Sources

  13. Electrically Driven Technologies for Radioactive Aerosol Abatement

    SciTech Connect (OSTI)

    David W. DePaoli; Ofodike A. Ezekoye; Costas Tsouris; Valmor F. de Almeida

    2003-01-28

    The purpose of this research project was to develop an improved understanding of how electriexecy driven processes, including electrocoalescence, acoustic agglomeration, and electric filtration, may be employed to efficiently treat problems caused by the formation of aerosols during DOE waste treatment operations. The production of aerosols during treatment and retrieval operations in radioactive waste tanks and during thermal treatment operations such as calcination presents a significant problem of cost, worker exposure, potential for release, and increased waste volume.

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    a Cloud-Resolving Model to Identify the Role of Aerosols on Clouds and Precipitation Download a printable PDF Submitter: GSFC, N., NASA GSFC Area of Research: Cloud Distributions/Characterizations Working Group(s): Aerosol, Cloud Modeling Journal Reference: Tao, W.-K., X. Li, A. Khain, T. Matsui, S. Lang, and J. Simpson, 2007: The role of atmospheric aerosol concentration on deep convective precipitation: Cloud-resolving model simulations. J. Geophy. Res., (accepted). Zeng, X., W.-K. Tao, S.

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Analyzing the Contribution of Aerosols to an Observed Increase in Direct Normal Irradiance Download a printable PDF Submitter: Long, C. N., NOAA Global Monitoring Division/CIRES Riihimaki, L., Pacific Northwest National Laboratory Vignola, F., University of Oregon Area of Research: Radiation Processes Working Group(s): Aerosol, Radiative Processes Journal Reference: Riihimaki LD, FE Vignola, and CN Long. 2009. "Analyzing the contribution of aerosols to an observed increase in direct normal

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Indirect Impact of Atmospheric Aerosols on an Ensemble of Deep Convective Clouds Download a printable PDF Submitter: Grabowski, W., NCAR Morrison, H. C., NCAR Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Grabowski WW and H Morrison. 2011. "Indirect impact of atmospheric aerosols in idealized simulations of convective-radiative quasi-equilibrium. Part II: Double-moment microphysics." Journal of

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Impact of Anthropogenic Emissions on Organic Aerosols During CARES Submitter: Zhang, Q., University of California, Davis Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Setyan A, Q Zhang, M Merkel, WB Knighton, Y Sun, C Song, J Shilling, TB Onasch, S Herndon, D Worsnop, JD Fast, R Zaveri, LK Berg, A Wiedensohler, BA Flowers, MK Dubey, and R Subramanian. 2012. "Characterization of submicron particles influenced by mixed biogenic and anthropogenic

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Strong Impacts of Vertical Velocity on Cloud Microphysics and Implications for Aerosol Indirect Download a printable PDF Submitter: Liu, Y., Brookhaven National Laboratory Lu, C., Nanjing University of Information Science and Technology Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Lu C, Y Liu, S Niu, and AM Vogelmann. 2012. "Observed impacts of vertical velocity on cloud

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Improving Estimates of Cloud Condensation Nuclei Concentration Download a printable PDF Submitter: Li, Z., University of Maryland Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Liu J and Z Li. 2014. "Estimation of cloud condensation nuclei concentration from aerosol optical quantities: influential factors and uncertainties." Atmospheric Chemistry and Physics, 14(1), doi:10.5194/acp-14-1-2014.

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Clouds, Aerosol, and Precipitation in the Marine Boundary Layer: an ARM Mobile Facility Deployment Download a printable PDF Submitter: Wood, R., University of Washington Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: N/A Composite seasonal cycles of (a) cloud droplet concentration retrieved using a variety of methods; (b) surface measured cloud condensation nuclei concentrations at four supersaturations.

  1. East Asian Studies of Tropospheric Aerosols and their Impact on Regional Climate (EAST-AIRC): An Overview

    SciTech Connect (OSTI)

    Li, Zhanqing; Li, C.; Chen, H.; Tsay, S. C.; Holben, B. N.; Huang, J.; Li, B.; Maring, H.; Qian, Yun; Shi, Guangyu; Xia, X.; Yin, Y.; Zheng, Y.; Zhuang, G.

    2011-02-01

    As the most populated region of the world, Asia is a major source of aerosols with potential large impact over vast downstream areas. Papers published in this special section describe the variety of aerosols observed in China and their effects and interactions with the regional climate as part of the East Asian Study of Tropospheric Aerosols and Impact on Regional Climate (EAST-AIRC). The majority of the papers are based on analyses of observations made under three field projects, namely, the Atmospheric Radiation Measurements (ARM) Mobile Facility mission in China (AMF10 China), the East Asian Study of Tropospheric Aerosols: an International Regional Experiment (EAST-AIRE), and the Atmospheric Aerosols of China and their Climate Effects (AACCE). The former two are US-China collaborative projects and the latter is a part of the China’s National Basic Research program (or often referred to as “973 project”). Routine meteorological data of China are also employed in some studies. The wealth of general and specialized measurements lead to extensive and close-up investigations of the optical, physical and chemical properties of anthropogenic, natural, and mixed aerosols; their sources, formation and transport mechanisms; horizontal, vertical and temporal variations; direct and indirect effects and interactions with the East Asian monsoon system. Particular efforts are made to advance our understanding of the mixing and interaction between dust and anthropogenic pollutants during transport. Several modeling studies were carried out to simulate aerosol impact on radiation budget, temperature, precipitation, wind and atmospheric circulation, fog, etc. In addition, impacts of the Asian monsoon system on aerosol loading are also simulated.

  2. Aerodynamic Focusing Of High-Density Aerosols

    SciTech Connect (OSTI)

    Ruiz, D. E.; Fisch, Nathaniel

    2014-02-24

    High-density micron-sized particle aerosols might form the basis for a number of applications in which a material target with a particular shape might be quickly ionized to form a cylindrical or sheet shaped plasma. A simple experimental device was built in order to study the properties of high-density aerosol focusing for 1#22; m silica spheres. Preliminary results recover previous findings on aerodynamic focusing at low densities. At higher densities, it is demonstrated that the focusing properties change in a way which is consistent with a density dependent Stokes number.

  3. Evaluating aerosol indirect effect through marine stratocumulus clouds

    SciTech Connect (OSTI)

    Kogan, Z.N.; Kogan, Y.L.; Lilly, D.K.

    1996-04-01

    During the last decade much attention has been focused on anthropogenic aerosols and their radiative influence on the global climate. Charlson et al. and Penner et al. have demonstrated that tropospheric aerosols and particularly anthropogenic sulfate aerosols may significantly contribute to the radiative forcing exerting a cooling influence on climate (-1 to -2 W/m{sup 2}) which is comparable in magnitude to greenhouse forcing, but opposite in sign. Aerosol particles affect the earth`s radiative budget either directly by scattering and absorption of solar radiation by themselves or indirectly by altering the cloud radiative properties through changes in cloud microstructure. Marine stratocumulus cloud layers and their possible cooling influence on the atmosphere as a result of pollution are of special interest because of their high reflectivity, durability, and large global cover. We present an estimate of thet aerosol indirect effect, or, forcing due to anthropogenic sulfate aerosols.

  4. The mixing state of carbonaceous aerosol particles in northern and southern California measured during CARES and CalNex 2010

    SciTech Connect (OSTI)

    Cahill, John F.; Suski, Kaitlyn; Seinfeld, John H.; Zaveri, Rahul A.; Prather, Kimberly A.

    2012-11-21

    Carbonaceous aerosols impact climate directly by scattering and absorbing radiation, and hence play a major, although highly uncertain, role in global radiative forcing. Commonly, ambient carbonaceous aerosols are internally mixed with secondary species such as nitrate, sulfate, and ammonium, which influence their climate impacts through optical properties, hygroscopicity, and atmospheric lifetime. Aircraft-aerosol time-of-flight mass spectrometry (A-ATOFMS), which measures single-particle mixing state, was used to determine the fraction of organic and soot aerosols that were internally mixed and the variability of their mixing state in California during the Carbonaceous Aerosol and Radiative Effects Study (CARES) and the Research at the Nexus of Air Quality and Climate Change (CalNex) field campaigns in the late spring and early summer of 2010. Nearly 88% of all A-ATOFMS measured particles (100-1000 nm in diameter) were internally mixed with secondary species, with 96% and 75% of particles internally mixed with nitrate and/or sulfate in southern and northern California, respectively. Even though atmospheric particle composition in both regions was primarily influenced by urban sources, the mixing state was found to vary greatly, with nitrate and soot being the dominant species in southern California, and sulfate and organic carbon in northern California. Furthermore, mixing state varied temporally in northern California, with soot becoming the prevalent particle type towards the end of the study as regional pollution levels increased. The results from these studies demonstrate that the majority of ambient carbonaceous particles are internally mixed and are heavily influenced by secondary species that are most predominant in each region. Based on these findings, considerations of regionally dominant sources and secondary species, as well as temporal variations of aerosol physical and optical properties, will be required to obtain more accurate predictions of the

  5. Project Overview: Cumulus Humilis Aerosol Processing Study (CHAPS): Proposed Summer 2007 ASP Field Campaign

    SciTech Connect (OSTI)

    Berkowitz, Carl M.; Berg, Larry K.; Ogren, J. A.; Hostetler, Chris A.; Ferrare, Richard

    2006-05-18

    This white paper presents the scientific motivation and preliminary logistical plans for a proposed ASP field campaign to be carried out in the summer of 2007. The primary objective of this campaign is to use the DOE Gulfstream-1 aircraft to make measurements characterizing the chemical, physical and optical properties of aerosols below, within and above large fields of fair weather cumulus and to use the NASA Langley Research Centers High Spectral Resolution Lidar (HSRL) to make independent measurements of aerosol backscatter and extinction profiles in the vicinity of these fields. Separate from the science questions to be addressed by these observations will be information to add in the development of a parameterized cumulus scheme capable of including multiple cloud fields within a regional or global scale model. We will also be able to compare and contrast the cloud and aerosol properties within and outside the Oklahoma City plume to study aerosol processes within individual clouds. Preliminary discussions with the Cloud and Land Surface Interaction Campaign (CLASIC) science team have identified overlap between the science questions posed for the CLASIC Intensive Operation Period (IOP) and the proposed ASP campaign, suggesting collaboration would benefit both teams.

  6. Effect of Aerosol Humidification on the Column Aerosol Optical...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    of Aerosol Humidification on the Column Aerosol Optical Thickness over the ARM Southern Great Plains Site Li, Zhanqing University of Maryland Jeong, Myeong-Jae University of...

  7. Two-Column Aerosol Project

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Column Aerosol Project Tiny particles in the sky known as "aerosols" come in many forms-dust, soot, and sea salt, for example. Depending on the type of aerosol, it can either...

  8. ARM - Measurement - Aerosol composition

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    quality assurance purposes. ARM Instruments PILS : Particle Into Liquid Sampler TDMA : Tandem Differential Mobility Analyzer Field Campaign Instruments AEROSMASSSPEC : Aerosol Mass...

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol-mediated Changes in Deep Convective Cloud Radiative Forcing over the SGP Download a printable PDF Submitter: Cribb, M. C., University of Maryland Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Yan H, Z Li, J Huang, M Cribb, and J Liu. 2014. "Long-term aerosol-mediated changes in cloud radiative forcing of deep clouds at the top and bottom of the atmosphere over the Southern Great Plains."

  10. Final Report for Research Conducted at The Scripps Institution of Oceanography, University of California San Diego from 2/2002 to 8/2003 for ''Aerosol and Cloud-Field Radiative Effects in the Tropical Western Pacific: Analyses and General Circulation Model Parameterizations''

    SciTech Connect (OSTI)

    Vogelmann, A. M.

    2004-01-27

    OAK-B135 Final report from the University of California San Diego for an ongoing research project that was moved to Brookhaven National Laboratory where proposed work will be completed. The research uses measurements made by the Atmospheric Radiation Measurement (ARM) Program to quantify the effects of aerosols and clouds on the Earth's energy balance in the climatically important Tropical Western Pacific.

  11. Ash Deposit Formation and Deposit Properties. A Comprehensive Summary of Research Conducted at Sandia's Combustion Research Facility

    SciTech Connect (OSTI)

    Larry L. Baxter

    2000-08-01

    This report summarizes experimental and theoretical work performed at Sandia's Combustion Research Facility over the past eight years on the fate of inorganic material during coal combustion. This work has been done under four broad categories: coal characterization, fly ash formation, ash deposition, and deposit property development. The objective was to provide sufficient understanding of these four areas to be able to predict coal behavior in current and advanced conversion systems. This work has led to new characterization techniques for fuels that provide, for the first time, systematic and species specific information regarding the inorganic material. The transformations of inorganic material during combustion can be described in terms of the net effects of the transformations of these individual species. Deposit formation mechanisms provide a framework for predicting deposition rates for abroad range of particle sizes. Predictions based on these rates many times are quite accurate although there are important exceptions. A rigorous framework for evaluating deposit has been established. Substantial data have been obtained with which to exercise this framework, but this portion of the work is less mature than is any other. Accurate prediction of deposit properties as functions of fuel properties, boiler design, and boiler operating conditions represents the single most critical area where additional research is needed.

  12. The Two-Column Aerosol Project (TCAP) Science Plan (Program Document...

    Office of Scientific and Technical Information (OSTI)

    To meet these science objectives, the Atmospheric Radiation Measurement (ARM) Climate ... of aerosol optical properties, particle composition and direct-beam irradiance. ...

  13. Portable Aerosol Contaminant Extractor

    DOE Patents [OSTI]

    Carlson, Duane C.; DeGange, John J.; Cable-Dunlap, Paula

    2005-11-15

    A compact, portable, aerosol contaminant extractor having ionization and collection sections through which ambient air may be drawn at a nominal rate so that aerosol particles ionized in the ionization section may be collected on charged plate in the collection section, the charged plate being readily removed for analyses of the particles collected thereon.

  14. Development of Aerosol Models for Radiative Flux Calculations...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Plains (SGP), and North Slope of Alaska (NSA) sites to begin development of a set of ... Aerosol properties at the SGP and NSA sites show considerable variability on multiple time ...

  15. Study of in-duct spray drying using condensation aerosol

    SciTech Connect (OSTI)

    Chen, W.J.R.; Chang, S.M.; Adikesavalu, R. )

    1992-06-01

    Sulfur removal efficiency of in-duct spray drying is limited by sorbent content and surface properties of the sorbent-water aerosol. It was the purpose of this study to improve the sulfur removal efficiency for in-duct spray drying by injecting condensation aerosol instead of conventional dispersion aerosol. The program was composed of three phases. In Phase I, a novel pulsed fluid bed feeder was developed and was used to feed hydrated lime for subsequent experiments. A small condensation aerosol generator was then built, which produces a lime-water condensation aerosol by condensing steam on lime particles. The results show that novel lime-water aerosols less than 10 microns were generated. The central task in Phase II was to simulate experimentally in-duct spray drying using condensation aerosols and compare the results with those using dispersion aerosols reported in the literature. A small entrained-flow reactor was constructed to simulate an in-duct spray dryer. The condensation aerosol was then introduced to the reactor at various approach to saturation temperature, calcium/sulfur stoichiometry and sulfur dioxide concentration for desulfurization study. The results show that we have improved the sulfur removal efficiency for in-duct spray drying to 90 percent or above. Thus we have met and exceeded the stated project goal of 70 percent sulfur removal. A comprehensive computer code was employed to calculate sulfur removal efficiency in Phase III.

  16. Climate implications of carbonaceous aerosols: An aerosol microphysical study using the GISS/MATRIX climate model

    SciTech Connect (OSTI)

    Bauer, Susanne E.; Menon, Surabi; Koch, Dorothy; Bond, Tami; Tsigaridis, Kostas

    2010-04-09

    Recently, attention has been drawn towards black carbon aerosols as a likely short-term climate warming mitigation candidate. However the global and regional impacts of the direct, cloud-indirect and semi-direct forcing effects are highly uncertain, due to the complex nature of aerosol evolution and its climate interactions. Black carbon is directly released as particle into the atmosphere, but then interacts with other gases and particles through condensation and coagulation processes leading to further aerosol growth, aging and internal mixing. A detailed aerosol microphysical scheme, MATRIX, embedded within the global GISS modelE includes the above processes that determine the lifecycle and climate impact of aerosols. This study presents a quantitative assessment of the impact of microphysical processes involving black carbon, such as emission size distributions and optical properties on aerosol cloud activation and radiative forcing. Our best estimate for net direct and indirect aerosol radiative forcing change is -0.56 W/m{sup 2} between 1750 and 2000. However, the direct and indirect aerosol effects are very sensitive to the black and organic carbon size distribution and consequential mixing state. The net radiative forcing change can vary between -0.32 to -0.75 W/m{sup 2} depending on these carbonaceous particle properties. Assuming that sulfates, nitrates and secondary organics form a coating shell around a black carbon core, rather than forming a uniformly mixed particles, changes the overall net radiative forcing from a negative to a positive number. Black carbon mitigation scenarios showed generally a benefit when mainly black carbon sources such as diesel emissions are reduced, reducing organic and black carbon sources such as bio-fuels, does not lead to reduced warming.

  17. Implementation of the Research Performance Progress Report (RPPR) and the SF-428 Tangible Personal Property Report Forms Family

    Broader source: Energy.gov [DOE]

    The new Research Performance Progress Report (RPPR) and SF-428 Tangible Personal Property Report Forms Family are now available for use.

  18. 2010 Atmospheric System Research (ASR) Science Team Meeting Summary

    SciTech Connect (OSTI)

    Dupont, DL

    2011-05-04

    This document contains the summaries of papers presented in poster format at the March 2010 Atmospheric System Research Science Team Meeting held in Bethesda, Maryland. More than 260 posters were presented during the Science Team Meeting. Posters were sorted into the following subject areas: aerosol-cloud-radiation interactions, aerosol properties, atmospheric state and surface, cloud properties, field campaigns, infrastructure and outreach, instruments, modeling, and radiation. To put these posters in context, the status of ASR at the time of the meeting is provided here.

  19. ARM: 10-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    1998-03-01

    10-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  20. ARM: 1-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    2004-10-01

    1-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  1. ARM: 10-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    10-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  2. ARM: 1-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    1-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  3. Final Technical Report for "Ice nuclei relation to aerosol properties: Data analysis and model parameterization for IN in mixed-phase clouds" (DOE/SC00002354)

    SciTech Connect (OSTI)

    Paul J. DeMott, Anthony J. Prenni; Sonia M. Kreidenweis

    2012-09-28

    Clouds play an important role in weather and climate. In addition to their key role in the hydrologic cycle, clouds scatter incoming solar radiation and trap infrared radiation from the surface and lower atmosphere. Despite their importance, feedbacks involving clouds remain as one of the largest sources of uncertainty in climate models. To better simulate cloud processes requires better characterization of cloud microphysical processes, which can affect the spatial extent, optical depth and lifetime of clouds. To this end, we developed a new parameterization to be used in numerical models that describes the variation of ice nuclei (IN) number concentrations active to form ice crystals in mixed-phase (water droplets and ice crystals co-existing) cloud conditions as these depend on existing aerosol properties and temperature. The parameterization is based on data collected using the Colorado State University continuous flow diffusion chamber in aircraft and ground-based campaigns over a 14-year period, including data from the DOE-supported Mixed-Phase Arctic Cloud Experiment. The resulting relationship is shown to more accurately represent the variability of ice nuclei distributions in the atmosphere compared to currently used parameterizations based on temperature alone. When implemented in one global climate model, the new parameterization predicted more realistic annually averaged cloud water and ice distributions, and cloud radiative properties, especially for sensitive higher latitude mixed-phase cloud regions. As a test of the new global IN scheme, it was compared to independent data collected during the 2008 DOE-sponsored Indirect and Semi-Direct Aerosol Campaign (ISDAC). Good agreement with this new data set suggests the broad applicability of the new scheme for describing general (non-chemically specific) aerosol influences on IN number concentrations feeding mixed-phase Arctic stratus clouds. Finally, the parameterization was implemented into a regional

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Effect of Dry Deposition of Condensable Organic Vapors on SOA Formation in the Urban Plume Download a printable PDF Submitter: Hodzic, A., NCAR Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Hodzic A, S Madronich, B Aumont, J Lee-Taylor, T Karl, M Camredon, and C Mouchel-Vallon. 2014. "Limited influence of dry deposition of semi-volatile organic vapors on secondary organic aerosol formation in the urban plume." Geophysical Research Letters,

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Multiday Production of SOA in Urban and Forest Outflow Submitter: Lee-Taylor, J., NCAR Madronich, S., National Center for Atmospheric Research Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Lee-Taylor J, A Hodzic, S Madronich, B Aumont, M Camredon, and R Valorso. 2015. "Multiday production of condensing organic aerosol mass in urban and forest outflow." Atmospheric Chemistry and Physics, 15, doi:10.5194/acp-15-595-2015. Simulated SOA in

  6. Monodisperse aerosol generator

    DOE Patents [OSTI]

    Ortiz, Lawrence W.; Soderholm, Sidney C.

    1990-01-01

    An aerosol generator is described which is capable of producing a monodisperse aerosol within narrow limits utilizing an aqueous solution capable of providing a high population of seed nuclei and an organic solution having a low vapor pressure. The two solutions are cold nebulized, mixed, vaporized, and cooled. During cooling, particles of the organic vapor condense onto the excess seed nuclei, and grow to a uniform particle size.

  7. Cloud Droplet Spectral Shape Sheds New Light on Aerosol- Cloud-Interaction Regimes

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Droplet Spectral Shape Sheds New Light on Aerosol- Cloud-Interaction Regimes For original submission and image(s), see ARM Research Highlights http://www.arm.gov/science/highlights/ Research Highlight Despite decades of research, aerosol indirect effects remain among the most uncertain climate forcings according to the latest Intergovernmental Panel on Climate Change report. Furthermore, climate models tend to overestimate the cooling of aerosol indirect effects and are more susceptible than

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lord of the Wings: Elevated Particles a Rising Star Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Kassianov E, C Flynn, J Redemann, B Schmid, PB Russell, and A Sinyuk. 2012. "Initial assessment of the Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR)-based aerosol retrieval: Sensitivity study." Atmosphere, 3,

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Twenty Years Serving Climate Science Download a printable PDF Submitter: Mather, J. H., Pacific Northwest National Laboratory Area of Research: Cloud Processes Working Group(s): Aerosol Life Cycle, Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Mather JH and JW Voyles. 2013. "The ARM Climate Research Facility: a review of structure and capabilities." Bulletin of the American Meteorological Society, 94(3), doi:10.1175/BAMS-D-11-00218.1. A scanning ARM

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    CCN and Vertical Velocity Influences Submitter: Hudson, J. G., Desert Research Institute Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Hudson JG and S Noble. 2013. "CCN and vertical velocity influences on droplet concentrations and supersaturations in clean and polluted stratus clouds." Journal of the Atmospheric Sciences, 71(1), 10.1175/JAS-D-13-086.1. Figure 1. Effective cloud supersaturation

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Research Masters the Misunderstood Mixed-Phase Cloud Download a printable PDF Submitter: Ovchinnikov, M., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Ovchinnikov M, AS Ackerman, A Avramov, A Cheng, J Fan, AM Fridland, S Ghan, J Harrington, C Hoose, A Korolev, GM McFarquhar, H Morrison, M Paukert, J Savre, BJ Shipway, MD Shupe, A Solomon, and K

  12. Aerosol Optical Depth Value-Added Product Report

    SciTech Connect (OSTI)

    Koontz, A; Hodges, G; Barnard, J; Flynn, C; Michalsky, J

    2013-03-17

    This document describes the process applied to retrieve aerosol optical depth (AOD) from multifilter rotating shadowband radiometers (MFRSR) and normal incidence multifilter radiometers (NIMFR) operated at the ARM Climate Research Facility’s ground-based facilities.

  13. Lidar Investigation of Tropical Nocturnal Boundary Layer Aerosols and Cloud Macrophysics

    SciTech Connect (OSTI)

    Manoj, M. G.; Devara, PC S.; Taraphdar, Sourav

    2013-10-01

    Observational evidence of two-way association between nocturnal boundary layer aerosols and cloud macrophysical properties under different meteorological conditions is reported in this paper. The study has been conducted during 2008-09 employing a high space-time resolution polarimetric micro-pulse lidar over a tropical urban station in India. Firstly, the study highlights the crucial role of boundary layer aerosols and background meteorology on the formation and structure of low-level stratiform clouds in the backdrop of different atmospheric stability conditions. Turbulent mixing induced by the wind shear at the station, which is associated with a complex terrain, is found to play a pivotal role in the formation and structural evolution of nocturnal boundary layer clouds. Secondly, it is shown that the trapping of energy in the form of outgoing terrestrial radiation by the overlying low-level clouds can enhance the aerosol mixing height associated with the nocturnal boundary layer. To substantiate this, the long-wave heating associated with cloud capping has been quantitatively estimated in an indirect way by employing an Advanced Research Weather Research and Forecasting (WRF-ARW) model version 2.2 developed by National Center for Atmospheric Research (NCAR), Colorado, USA, and supplementary data sets; and differentiated against other heating mechanisms. The present investigation as well establishes the potential of lidar remote-sensing technique in exploring some of the intriguing aspects of the cloud-environment relationship.

  14. ARM - Field Campaign - MArine Stratus Radiation Aerosol and Drizzle

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    (MASRAD) IOP govCampaignsMArine Stratus Radiation Aerosol and Drizzle (MASRAD) IOP Campaign Links Science Plan AMF Point Reyes Website AMF Point Reyes Data Plots ARM Data Discovery Browse Data Related Campaigns MASRAD: Pt. Reyes Stratus Cloud and Drizzle Study 2005.07.07, Coulter, AMF MASRAD: Cloud Condensate Nuclei Chemistry Measurements 2005.07.01, Berkowitz, AMF MASRAD - Aerosol Optical Properties 2005.06.29, Strawa, AMF MASRAD:Sub-Micron Aerosol Measurements 2005.06.20, Wang, AMF MASRAD:

  15. Surface based remote sensing of aerosol-cloud interactions

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Surface based remote sensing of aerosol-cloud interactions Feingold, Graham NOAA/Environmental Technology Laboratory Frisch, Shelby NOAA/Environmental Technology Laboratory Min, Qilong State University of New York at Albany Category: Cloud Properties We will present an analysis of the effect of aerosol on clouds at the Southern Great Plains ARM site. New methods for retrieving cloud droplet effective radius with radar (MMCR), multifilter rotating shadowband radiometer (MFRSR), and microwave

  16. Organic Aerosol Component (OACOMP) Value-Added Product Report

    SciTech Connect (OSTI)

    Fast, J; Zhang, Q; Tilp, A; Shippert, T; Parworth, C; Mei, F

    2013-08-23

    Significantly improved returns in their aerosol chemistry data can be achieved via the development of a value-added product (VAP) of deriving OA components, called Organic Aerosol Components (OACOMP). OACOMP is primarily based on multivariate analysis of the measured organic mass spectral matrix. The key outputs of OACOMP are the concentration time series and the mass spectra of OA factors that are associated with distinct sources, formation and evolution processes, and physicochemical properties.

  17. Atmospheric Science Program Cumulus Humilis Aerosol Processing Study (CHAPS)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Program Cumulus Humilis Aerosol Processing Study (CHAPS) General Description 'Cumulus humilis' is the scientific term used to describe the small fair weather clouds that dot the summer skies over Oklahoma. During the month of June, scientists sponsored by the U.S. Department of Energy's Atmospheric Science Program will use aircraft and ground based instruments to obtain information about the physical and chemical properties of these clouds and the small airborne particles - called aerosols -

  18. ARM - Measurement - Aerosol effective radius

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    would love to hear from you Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol effective radius Aerosol effective radius is the ratio of the third and...

  19. Parameterizations of Cloud Microphysics and Indirect Aerosol Effects

    SciTech Connect (OSTI)

    Tao, Wei-Kuo

    2014-05-19

    1. OVERVIEW Aerosols and especially their effect on clouds are one of the key components of the climate system and the hydrological cycle [Ramanathan et al., 2001]. Yet, the aerosol effect on clouds remains largely unknown and the processes involved not well understood. A recent report published by the National Academy of Science states "The greatest uncertainty about the aerosol climate forcing - indeed, the largest of all the uncertainties about global climate forcing - is probably the indirect effect of aerosols on clouds [NRC, 2001]." The aerosol effect on clouds is often categorized into the traditional "first indirect (i.e., Twomey)" effect on the cloud droplet sizes for a constant liquid water path [Twomey, 1977] and the "semi-direct" effect on cloud coverage [e.g., Ackerman et al., 2000]. Enhanced aerosol concentrations can also suppress warm rain processes by producing a narrow droplet spectrum that inhibits collision and coalescence processes [e.g., Squires and Twomey, 1961; Warner and Twomey, 1967; Warner, 1968; Rosenfeld, 1999]. The aerosol effect on precipitation processes, also known as the second type of aerosol indirect effect [Albrecht, 1989], is even more complex, especially for mixed-phase convective clouds. Table 1 summarizes the key observational studies identifying the microphysical properties, cloud characteristics, thermodynamics and dynamics associated with cloud systems from high-aerosol continental environments. For example, atmospheric aerosol concentrations can influence cloud droplet size distributions, warm-rain process, cold-rain process, cloud-top height, the depth of the mixed phase region, and occurrence of lightning. In addition, high aerosol concentrations in urban environments could affect precipitation variability by providing an enhanced source of cloud condensation nuclei (CCN). Hypotheses have been developed to explain the effect of urban regions on convection and precipitation [van den Heever and Cotton, 2007 and Shepherd

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Mingling in the Sky-A View from the Earth Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Madhavan BL, Y He, Y Wu, B Gross, F Moshary, and S Ahmed. 2012. "Development of a ground based remote sensing approach for direct evaluation of aerosol-cloud interaction." Atmosphere, 3(4), doi:10.3390/atmos3040468. Two different types of

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Clouds Re-gathered by Wind Shear Download a printable PDF Submitter: Yang, Q., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Yang Q, RC Easter, P Campuzano-Jost, JL Jimenez, JD Fast, SJ Ghan, H Wang, LK Berg, MC Barth, Y Liu, MB Shrivastava, B Singh, H Morrison, J Fan, CL Ziegler, M Bela, E Apel, GS Diskin, T Mikoviny, and A Wisthaler. 2015. "Aerosol transport and

  2. Highly stable aerosol generator

    DOE Patents [OSTI]

    DeFord, H.S.; Clark, M.L.

    1981-11-03

    An improved compressed air nebulizer has been developed such that a uniform aerosol particle size and concentration may be produced over long time periods. This result is achieved by applying a vacuum pressure to the makeup assembly and by use of a vent tube between the atmosphere and the makeup solution. By applying appropriate vacuum pressures to the makeup solution container and by proper positioning of the vent tube, a constant level of aspirating solution may be maintained within the aspirating assembly with aspirating solution continuously replaced from the makeup solution supply. This device may also be adapted to have a plurality of aerosol generators and only one central makeup assembly. 2 figs.

  3. Highly stable aerosol generator

    DOE Patents [OSTI]

    DeFord, Henry S.; Clark, Mark L.

    1981-01-01

    An improved compressed air nebulizer has been developed such that a uniform aerosol particle size and concentration may be produced over long time periods. This result is achieved by applying a vacuum pressure to the makeup assembly and by use of a vent tube between the atmosphere and the makeup solution. By applying appropriate vacuum pressures to the makeup solution container and by proper positioning of the vent tube, a constant level of aspirating solution may be maintained within the aspirating assembly with aspirating solution continuously replaced from the makeup solution supply. This device may also be adapted to have a plurality of aerosol generators and only one central makeup assembly.

  4. The Radiative Role of Free Tropospheric Aerosols and Marine Clouds over the Central North Atlantic

    SciTech Connect (OSTI)

    Mazzoleni, Claudio; Kumar, Sumit; Wright, Kendra; Kramer, Louisa; Mazzoleni, Lynn; Owen, Robert; Helmig, Detlev

    2014-12-09

    microscope – were often very compacted, suggesting cloud processing and exhibiting different optical properties from fresh emissions. In addition, black carbon was found to be sometimes mixed with mineral dust, affecting its optical properties and potential forcing. c) Some aerosols collected at PMO acted as ice nuclei, potentially contributing to cirrus cloud formation during their transport in the upper free troposphere. Identified good ice nuclei were often mineral dust particles. d) The free tropospheric aerosols studied at PMO have relevance to low level marine clouds due, for example, to synoptic subsidence entraining free tropospheric aerosols into the marine boundary layer. This has potentially large consequences on cloud condensation nuclei concentrations and compositions in the marine boundary layer; therefore, having an effect on the marine stratus clouds, with potentially important repercussions on the radiative forcing. The scientific products of this project currently include contributions to two papers published in the Nature Publishing group (Nature Communications and Scientific Reports), one paper under revision for Atmospheric Chemistry and Physics, one in review in Geophysical Research Letters and one recently submitted to Atmospheric Chemistry and Physics Discussion. In addition, four manuscripts are in advanced state of preparation. Finally, twenty-eight presentations were given at international conferences, workshops and seminars.

  5. Implementing marine organic aerosols into the GEOS-Chem model

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Gantt, B.; Johnson, M. S.; Crippa, M.; Prévôt, A. S. H.; Meskhidze, N.

    2014-09-09

    Marine organic aerosols (MOA) have been shown to play an important role in tropospheric chemistry by impacting surface mass, cloud condensation nuclei, and ice nuclei concentrations over remote marine and coastal regions. In this work, an online marine primary organic aerosol emission parameterization, designed to be used for both global and regional models, was implemented into the GEOS-Chem model. The implemented emission scheme improved the large underprediction of organic aerosol concentrations in clean marine regions (normalized mean bias decreases from -79% when using the default settings to -12% when marine organic aerosols are added). Model predictions were also in goodmore » agreement (correlation coefficient of 0.62 and normalized mean bias of -36%) with hourly surface concentrations of MOA observed during the summertime at an inland site near Paris, France. Our study shows that MOA have weaker coastal-to-inland concentration gradients than sea-salt aerosols, leading to several inland European cities having > 10% of their surface submicron organic aerosol mass concentration with a marine source. The addition of MOA tracers to GEOS-Chem enabled us to identify the regions with large contributions of freshly-emitted or aged aerosol having distinct physicochemical properties, potentially indicating optimal locations for future field studies.« less

  6. Implementing marine organic aerosols into the GEOS-Chem model

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Gantt, B.; Johnson, M. S.; Crippa, M.; Prévôt, A. S. H.; Meskhidze, N.

    2015-03-17

    Marine-sourced organic aerosols (MOAs) have been shown to play an important role in tropospheric chemistry by impacting surface mass, cloud condensation nuclei, and ice nuclei concentrations over remote marine and coastal regions. In this work, an online marine primary organic aerosol emission parameterization, designed to be used for both global and regional models, was implemented into the GEOS-Chem (Global Earth Observing System Chemistry) model. The implemented emission scheme improved the large underprediction of organic aerosol concentrations in clean marine regions (normalized mean bias decreases from -79% when using the default settings to -12% when marine organic aerosols are added). Modelmore » predictions were also in good agreement (correlation coefficient of 0.62 and normalized mean bias of -36%) with hourly surface concentrations of MOAs observed during the summertime at an inland site near Paris, France. Our study shows that MOAs have weaker coastal-to-inland concentration gradients than sea-salt aerosols, leading to several inland European cities having >10% of their surface submicron organic aerosol mass concentration with a marine source. The addition of MOA tracers to GEOS-Chem enabled us to identify the regions with large contributions of freshly emitted or aged aerosol having distinct physicochemical properties, potentially indicating optimal locations for future field studies.« less

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Pollution from a Megacity in the Amazon: the Case of Manaus, Brazil PI Contact: Fan, J., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Martin ST, P Artaxo, L Machado, AO Manzi, RA Souza, C Schumacher, J Wang, MO Andreae, HJ Barbosa, J Fan, G Fisch, AH Goldstein, A Guenther, JL Jimenez, U Poschl, MA Silva Dias, J Smith, and M Wendisch. 2016. "Introduction:

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Variations of Meridional Aerosol Distribution and Solar Dimming Download a printable PDF Submitter: Long, C. N., NOAA Global Monitoring Division/CIRES Kishcha, P., Tel-Aviv University Starobinets, B., Tel-Aviv University Kalashnikova, O., Jet Propulsion Laboratory Alpert, P., Tel-Aviv University Area of Research: Radiation Processes Working Group(s): Aerosol, Radiative Processes Journal Reference: Kishcha P, B Starobinets, O Kalashnikova, CN Long, and P Alpert. 2009. "Variations of

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Black Carbon Aerosols and the Third Polar Ice Cap Submitter: Menon, S., Lawrence Berkeley National Laboratory Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Cloud Modeling Journal Reference: Menon S, D Koch, G Beig, S Sahu, J Fasullo, and D Orlikowski. 2009. "Black carbon aerosols and the third polar ice cap." Atmospheric Chemistry and Physics, 9, 26593-26625. Recent thinning of glaciers over the Himalayas (sometimes referred to as

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Influence of Humidified Aerosols on Lidar Depolarization Below Ice-Precipitating Arctic Clouds Download a printable PDF Submitter: Fridlind, A. M., NASA - Goddard Institute for Space Studies van Diedenhoven, B., NASA - Goddard Institute for Space Studies Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle Journal Reference: van Diedenhoven B, AM Fridlind, and AS Ackerman. 2011. "Influence of humidified aerosol on lidar depolarization measurements below