National Library of Energy BETA

Sample records for research aerosol properties

  1. ARM - AOS Aerosol Properties Plots

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ViewersAOS Aerosol Properties Plots XDC Data Viewers Aerosol Properties Plots SGP AMF NSA (BRW) AOS Aerosol Properties Plots These plots are designed to provide a quick look at the measured aerosol properties or review current station operations. Be aware that they are raw unedited data. Do not quote and cite. Aerosol Properties Plots SGP AMF NSA (BRW)

  2. ARM - Measurement - Aerosol optical properties

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    : Aerosol optical properties The optical properties of aerosols, including asymmetry factor, phase-function, single-scattering albedo, refractive index, and backscatter...

  3. ARM - Field Campaign - MASRAD - Aerosol Optical Properties

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsMASRAD - Aerosol Optical Properties Campaign Links AMF Point Reyes Website ARM Data Discovery Browse Data Related Campaigns MArine Stratus Radiation Aerosol and Drizzle...

  4. Researchers Model Impact of Aerosols Over California

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Researchers Model Impact of Aerosols Over California Researchers Model Impact of Aerosols Over California Research may clarify the effectiveness of regional pollution controls May 28, 2013 Contact: Linda Vu, lvu@lbl.gov, (510) 495-2404 LosAngelesSmogv1.jpg Smog over downtown Los Angeles. Aerosols are microscopic particles-like dust, pollen and soot-that ubiquitously float around in our atmosphere. Despite their tiny stature, these particles can have a huge impact on human health, climate and the

  5. ARM - Field Campaign - MASRAD: Marine Aerosol Properties

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsMASRAD: Marine Aerosol Properties Campaign Links AMF Point Reyes Website Comments? We would love to hear from you Send us a note below or call us at 1-888-ARM-DATA....

  6. Emerging Technology for Measuring Atmospheric Aerosol Properties

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Technology for Measuring Atmospheric Aerosol Properties Bruce Gandrud Greg Kok Droplet Measurement Technologies Darrel Baumgardner Centro de Ciencias de la Atmósfera Universidad Nacional Autónoma de México Acknowledgements * The DMT staff * Bob Bluth and Haflidi Jonsson * Pat Arnott * Greg Roberts and Thanos Nenes * Dave Fahey, Shuka Schwarz and Ru-Shan Gao * NSF, NASA, ONR, NOAA and DOE Introducing Droplet Measurement Technologies * Founded in 1987 * Specializing in aerosol and cloud

  7. ARM - Field Campaign - Cirrus Clouds and Aerosol Properties Campaign

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsCirrus Clouds and Aerosol Properties Campaign ARM Data Discovery Browse Data Related Campaigns Vaisala Laser Ceilometer CL51 Demonstration 2013.11.14, Winston, SGP...

  8. ARM AOS Processing Status and Aerosol Intensive Properties VAP

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AOS Processing Status and Aerosol Intensive Properties VAP A. S. Koontz and C. J. Flynn Pacific Northwest National Laboratory Richland, Washington J. A. Ogren, E. Andrews, and P....

  9. Evaluating Global Aerosol Models and Aerosol and Water Vapor Properties Near Clouds

    SciTech Connect (OSTI)

    Richard A. Ferrare; David D. Turner

    2011-09-01

    Project goals: (1) Use the routine surface and airborne measurements at the ARM SGP site, and the routine surface measurements at the NSA site, to continue our evaluations of model aerosol simulations; (2) Determine the degree to which the Raman lidar measurements of water vapor and aerosol scattering and extinction can be used to remotely characterize the aerosol humidification factor; (3) Use the high temporal resolution CARL data to examine how aerosol properties vary near clouds; and (4) Use the high temporal resolution CARL and Atmospheric Emitted Radiance Interferometer (AERI) data to quantify entrainment in optically thin continental cumulus clouds.

  10. Measurement and Modeling of Vertically Resolved Aerosol Optical Properties and Radiative Fluxes Over the ARM SGP Site During the May 2003 Aerosol IOP

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Measurement and Modeling of Vertically Resolved Aerosol Optical Properties and Radiative Fluxes Over the ARM SGP Site During the May 2003 Aerosol IOP B. Schmid and J. Redemann Bay Area Environmental Research Institute National Aeronautics and Space Administration Ames Research Center Moffett Field, California W. P. Arnott Desert Research Institute Reno, Nevada A. Bucholtz and J. Reid Naval Research Laboratory Monterey, California P. Colarco Earth System Science Interdisciplinary Center

  11. Evaluating Global Aerosol Models and Aerosol and Water Vapor Properties Near Clouds

    SciTech Connect (OSTI)

    Turner, David, D.; Ferrare, Richard, A.

    2011-07-06

    The 'Evaluating Global Aerosol Models and Aerosol and Water Vapor Properties Near Clouds' project focused extensively on the analysis and utilization of water vapor and aerosol profiles derived from the ARM Raman lidar at the Southern Great Plains ARM site. A wide range of different tasks were performed during this project, all of which improved quality of the data products derived from the lidar or advanced the understanding of atmospheric processes over the site. These activities included: upgrading the Raman lidar to improve its sensitivity; participating in field experiments to validate the lidar aerosol and water vapor retrievals; using the lidar aerosol profiles to evaluate the accuracy of the vertical distribution of aerosols in global aerosol model simulations; examining the correlation between relative humidity and aerosol extinction, and how these change, due to horizontal distance away from cumulus clouds; inferring boundary layer turbulence structure in convective boundary layers from the high-time-resolution lidar water vapor measurements; retrieving cumulus entrainment rates in boundary layer cumulus clouds; and participating in a field experiment that provided data to help validate both the entrainment rate retrievals and the turbulent profiles derived from lidar observations.

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Production Flux of Sea-Spray Aerosol Download a printable PDF Submitter: Schwartz, S. E., Brookhaven National Laboratory Area of Research: Aerosol Properties Working Group(s):...

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosols Help Heat Up the Yangtze River Delta in China Download a printable PDF Submitter: Flynn, C. J., Pacific Northwest National Laboratory Area of Research: Aerosol Properties...

  14. Connecting Organic Aerosol Climate-Relevant Properties to Chemical Mechanisms of Sources and Processing

    SciTech Connect (OSTI)

    Thornton, Joel

    2015-01-26

    The research conducted on this project aimed to improve our understanding of secondary organic aerosol (SOA) formation in the atmosphere, and how the properties of the SOA impact climate through its size, phase state, and optical properties. The goal of this project was to demonstrate that the use of molecular composition information to mechanistically connect source apportionment and climate properties can improve the physical basis for simulation of SOA formation and properties in climate models. The research involved developing and improving methods to provide online measurements of the molecular composition of SOA under atmospherically relevant conditions and to apply this technology to controlled simulation chamber experiments and field measurements. The science we have completed with the methodology will impact the simulation of aerosol particles in climate models.

  15. Characterizing Aerosol Distributions and Optical Properties Using the NASA Langley High Spectral Resolution Lidar

    SciTech Connect (OSTI)

    Hostetler, Chris; Ferrare, Richard

    2013-02-14

    The objective of this project was to provide vertically and horizontally resolved data on aerosol optical properties to assess and ultimately improve how models represent these aerosol properties and their impacts on atmospheric radiation. The approach was to deploy the NASA Langley Airborne High Spectral Resolution Lidar (HSRL) and other synergistic remote sensors on DOE Atmospheric Science Research (ASR) sponsored airborne field campaigns and synergistic field campaigns sponsored by other agencies to remotely measure aerosol backscattering, extinction, and optical thickness profiles. Synergistic sensors included a nadir-viewing digital camera for context imagery, and, later in the project, the NASA Goddard Institute for Space Studies (GISS) Research Scanning Polarimeter (RSP). The information from the remote sensing instruments was used to map the horizontal and vertical distribution of aerosol properties and type. The retrieved lidar parameters include profiles of aerosol extinction, backscatter, depolarization, and optical depth. Products produced in subsequent analyses included aerosol mixed layer height, aerosol type, and the partition of aerosol optical depth by type. The lidar products provided vertical context for in situ and remote sensing measurements from other airborne and ground-based platforms employed in the field campaigns and was used to assess the predictions of transport models. Also, the measurements provide a data base for future evaluation of techniques to combine active (lidar) and passive (polarimeter) measurements in advanced retrieval schemes to remotely characterize aerosol microphysical properties. The project was initiated as a 3-year project starting 1 January 2005. It was later awarded continuation funding for another 3 years (i.e., through 31 December 2010) followed by a 1-year no-cost extension (through 31 December 2011). This project supported logistical and flight costs of the NASA sensors on a dedicated aircraft, the subsequent analysis and archival of the data, and the presentation of results in conferences, workshops, and publications. DOE ASR field campaigns supported under this project included - MAX-Mex /MILAGRO (2006) - TexAQS 2006/GoMACCS (2006) - CHAPS (2007) - RACORO (2009) - CARE/CalNex (2010) In addition, data acquired on HSRL airborne field campaigns sponsored by other agencies were used extensively to fulfill the science objectives of this project and the data acquired have been made available to other DOE ASR investigators upon request.

  16. Researchers Model Impact of Aerosols Over California

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    cooling over California using supercomputers at the Department of Energy's National Energy Research Scientific Computing Center (NERSC) and at PNNL. The scientists found that...

  17. FY 2010 Fourth Quarter Report: Evaluation of the Dependency of Drizzle Formation on Aerosol Properties

    SciTech Connect (OSTI)

    Lin, W; McGraw, R; Liu, Y; Wang, J; Vogelmann, A; Daum, PH

    2010-10-01

    Metric for Quarter 4: Report results of implementation of composite parameterization in single-column model (SCM) to explore the dependency of drizzle formation on aerosol properties. To better represent VOCALS conditions during a test flight, the Liu-Duam-McGraw (LDM) drizzle parameterization is implemented in the high-resolution Weather Research and Forecasting (WRF) model, as well as in the single-column Community Atmosphere Model (CAM), to explore this dependency.

  18. Optical Properties of Mixed Black Carbon, Inorganic and Secondary Organic Aerosols

    SciTech Connect (OSTI)

    Paulson, S E

    2012-05-30

    Summarizes the achievements of the project, which are divided into four areas: 1) Optical properties of secondary organic aerosols; 2) Development and of a polar nephelometer to measure aerosol optical properties and theoretical approaches to several optical analysis problems, 3) Studies on the accuracy of measurements of absorbing carbon by several methods, and 4) Environmental impacts of biodiesel.

  19. Investigation of Absorption Properties of Submicron Aerosol in the Troposphere Over West Siberia

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Investigation of Absorption Properties of Submicron Aerosol in the Troposphere Over West Siberia M. V. Panchenko, V. S. Kozlov, and V. P. Shmargunov Institute of Atmospheric Optics Tomsk, Russia Introduction Improving radiative climate models for the cloudless atmosphere depends largely on the correct way to simulate single-scattering albedo of atmospheric aerosol. Solving this problem requires performing detailed experiments on the study of the aerosol absorption characteristics in the

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Experiment Results Featured in Technical Journal Submitter: Sheridan, P., U.S. Department of Commerce/NOAA Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Sheridan, P, W Arnott, J Ogren, E Andrews, D Atkinson, D Covert, H Moosmuller, A Petzold, B Schmid, A Strawa, R Varma, and A Virkkula. 2005. "The Reno Aerosol Optics Study: An evaluation of aerosol absorption measurement methods." Aerosol Science and Technology 39(1):1-16. This magnification

  1. Aerosol Properties from Multi-spectral and Multi-angular Aircraft 4STAR Observations: Expected Advantages and Challenges

    SciTech Connect (OSTI)

    Kassianov, Evgueni I.; Flynn, Connor J.; Redemann, Jens; Schmid, Beat; Russell, P. B.; Sinyuk, Alexander

    2012-11-01

    The airborne Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR) is developed to retrieve aerosol microphysical and optical properties from multi-angular and multi-spectral measurements of sky radiance and direct-beam sun transmittance. The necessarily compact design of the 4STAR may cause noticeable apparent enhancement of sky radiance at small scattering angles. We assess the sensitivity of expected 4STAR-based aerosol retrieval to such enhancement by applying the operational AERONET retrieval code and constructed synthetic 4STARlike data. Also, we assess the sensitivity of the broadband fluxes and the direct aerosol radiative forcing to uncertainties in aerosol retrievals associated with the sky radiance enhancement. Our sensitivity study results suggest that the 4STARbased aerosol retrieval has limitations in obtaining detailed information on particle size distribution and scattering phase function. However, these limitations have small impact on the retrieved bulk optical parameters, such as the asymmetry factor (up to 4%, or 0.02) and single-scattering albedo (up to 2%, or 0.02), and the calculated direct aerosol radiative forcing (up to 6%, or 2 Wm-2).

  2. Collaborative research. Study of aerosol sources and processing at the GVAX Pantnagar Supersite

    SciTech Connect (OSTI)

    Worsnop, Doug; Volkamer, Rainer

    2012-08-13

    The Two Column Aerosol Project (TCAP) investigated uncertainties in the aerosol direct effect in the northern hemisphere mid-latitudes. The University of Colorado 2D-MAX-DOAS and LED-CE-DOAS instruments were collocated with DOE’s Atmospheric Radiation Measurement (ARM) Mobile Facility (AMF) and Mobile Aerosol Observing System (MAOS) during the TCAP-1 campaign at Cape Cod, MA (1 July to 13 August 2012). We have performed atmospheric radiation closure studies to evaluate the use of a novel parameter, i.e., the Raman Scattering Probability (RSP). We have performed first measurements of RSP almucantar scans, and measure RSP in spectra of scattered solar photons at 350nm and 430nm. Radiative Transfer Modelling of RSP demonstrate that the RSP measurement is maximally sensitive to infer even extremely low aerosol optical depth (AOD < 0.01) reliably by DOAS at low solar relative azimuth angles. We further assess the role of elevated aerosol layers on near surface observations of oxygen collision complexes, O 2-O2. Elevated aerosol layers modify the near surface absorption of O2-O2 and RSP. The combination of RSP and O2-O2 holds largely unexplored potential to better constrain elevated aerosol layers and measure column aerosol optical properties such as aerosol effective radius, extinction, aerosol phase functions and refractive indices. The TCAP deployment also provides a time series of reactive trace gas vertical profiles, i.e., nitrogen dioxide (NO2) and glyoxal (C2H2O2), which are measured simultaneously with the aerosol optical properties by DOAS. NO2 is an important precursor for ozone (O3) that modifies oxidative capacity. Glyoxal modifies oxidative capacity and is a source for brown carbon by forming secondary organic aerosol (SOA) via multiphase reactions in aerosol and cloud water. We have performed field measurements of these gases during TCAP, and conducted laboratory experiments to quantify for the first time the Setschenow salting constant, KS, of glyoxal in sulfate aerosols. Knowledge about KS is prerequisite to predict how increasing sulfate concentrations since pre-industrial times have modified the formation of SOA from biogenic gases in atmospheric models.

  3. COLLABORATIVE RESEARCH: Study of Aerosol Sources and Processing at the GVAX Pantnagar Supersite

    SciTech Connect (OSTI)

    Worsnop, Douglas R.

    2014-07-28

    This project funded the participation of scientists from seven research groups, running more than thirty instruments, in the Winter Intensive Operating Period (January-February 2012) of the Clean Air for London (ClearfLo) campaign at a rural site in Detling, UK, 45 km southeast of central London. The primary science questions for the ClearfLo Winter IOP were, 1) what is the urban increment of particulate matter (PM) and other pollutants in the greater London area, and, 2) what is the contribution of solid fuel use for home heating to wintertime PM? An additional motivation for the Detling measurements was the question of whether coatings on black carbon particles enhance absorption. The following four key accomplishments have been identified so far: 1) Chemical, physical and optical characterization of PM from local and regional sources (Figures 2, 4, 5 and 6). 2) Measurement of urban increment in particulate matter and gases in London (Figure 3). 3) Measurement of optical properties and chemical composition of coatings on black carbon containing particles indicates absorption enhancement. 4) First deployment of chemical ionization instrument (MOVI-CI-TOFMS) to measure both particle-phase and gas-phase organic acids. (See final report from Joel Thornton, University of Washington, for details.) Analysis of the large dataset acquired in Detling is ongoing and will yield further key accomplishments. These measurements of urban and rural aerosol properties will contribute to improved modeling of regional aerosol emissions, and of atmospheric aging and removal. The measurement of absorption enhancement by coatings on black carbon will contribute to improved modeling of the direct radiative properties of PM.

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Raman Lidar Observations of Aerosol Humidification Near Clouds Submitter: Ferrare, R. A., NASA LaRC Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Ferrare, R., et al., Evaluation of Daytime Measurements of Aerosols and Water Vapor Made by an Operational Raman Lidar over the Southern Great Plains, J. Geophys. Res., 111, D05S08, doi:10.1029/2005JD005836, 2006. Relative humidity profiles derived from the Raman lidar during the ALIVE 2005 field experiment. Aerosol

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Influence of Dust Composition on Cloud Droplet Formation Download a printable PDF Submitter: Chuang, C., Lawrence Livermore National Laboratory Area of Research: Aerosol Properties...

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Arctic Aerosol Study Flies By Download a printable PDF Submitter: Schmid, B., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: ARM Climate Research Facility Operations Update, April 30, 2008, Edition Preliminary screening and analysis of images from the time-resolved aerosol collector indicate particles laden with carbon and sulfur. These data were obtained on April 8, 2008. Image courtesy of Alexander Laskin, PNNL. Images

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Atmospheric Aerosol Measurements on Cloudy Days: a New Method Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Ovchinnikov, M., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Kassianov, EI, and M Ovtchinnikov. 2008. "On reflectance ratios and aerosol optical depth retrieval in the presence of cumulus clouds." Geophysical Research Letters doi:10.1029/2008GL033231.

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Micropulse Lidar-Derived Aerosol Optical Depth Climatology at ARM Sites Worldwide Download a printable PDF Submitter: Kafle, D. N., NASA GSFC /ADNET Systems Coulter, R. L., Argonne National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Kafle DN and RL Coulter. 2013. "Micropulse lidar-derived aerosol optical depth climatology at ARM sites worldwide." Journal of Geophysical Research - Atmospheres, 118(13), 10.1002/jgrd.50536.

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Hemispherical Simulations Show Impact of Aerosols on Cloud Reflectivity Submitter: Rotstayn, L., Commonwealth Scientific and Industrial Research Organization Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Rotstayn, L., and Y. Liu, Sensitivity of the First Indirect Aerosol Effect to an Increase in Cloud Droplet Spectral Dispersion with Droplet Number Concentration, Journal of Climate: Vol. 16, No. 21, pp.3476-3481, May 2003. Figure 1. Measurements of the

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Overambitious Other Carbon Submitter: Church, J., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Song C, M Gyawali, RA Zaveri, JE Shilling, and WP Arnott. 2013. "Light absorption by secondary organic aerosol from α-pinene: Effects of oxidants, seed aerosol acidity, and relative humidity." Journal of Geophysical Research - Atmospheres, 118, doi:10.1002/jgrd.50767. Time-dependent Mass Absorption

  11. Ultraviolet high-spectral-resolution Doppler lidar for measuring wind field and aerosol optical properties

    SciTech Connect (OSTI)

    Imaki, Masaharu; Kobayashi, Takao

    2005-10-01

    An ultraviolet incoherent Doppler lidar that incorporates the high-spectral-resolution (HSR) technique has been developed for measuring the wind field and aerosol optical properties in the troposphere. An injection seeded and tripled Nd:YAG laser at an ultraviolet wavelength of 355 nm was used in the lidar system. The HRS technique can resolve the aerosol Mie backscatter and the molecular Rayleigh backscatter to derive the signal components. By detecting the Mie backscatter, a great increase in the Doppler filter sensitivity was realized compared to the conventional incoherent Doppler lidars that detected the Rayleigh backscatter. The wind velocity distribution in a two-dimensional cross section was measured. By using the HSR technique, multifunction and absolute value measurements were realized for aerosol extinction, and volume backscatter coefficients; the laser beam transmittance, the lidar ratio, and the backscatter ratio are derived from these measurements.

  12. Initial Assessment of the Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR)-Based Aerosol Retrieval: Sensitivity Study

    SciTech Connect (OSTI)

    Kassianov, Evgueni I.; Flynn, Connor J.; Redemann, Jens; Schmid, Beat; Russell, P. B.; Sinyuk, Alexander

    2012-10-24

    The Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR) being developed for airborne measurements will offer retrievals of aerosol microphysical and optical properties from multi-angular and multi-spectral measurements of sky radiance and direct-beam sun transmittance. In this study, we assess the expected accuracy of the 4STAR-based aerosol retrieval and its sensitivity to major sources of anticipated perturbations in the 4STAR measurements by adapting a theoretical approach previously developed for the AERONET measurements. The major anticipated perturbations are (1) an apparent enhancement of sky radiance at small scattering angles associated with the necessarily compact design of the 4STAR and (2) and an offset (i.e. uncertainty) of sky radiance calibration independent of scattering angle. The assessment is performed through application of the operational AERONET aerosol retrieval and constructed synthetic 4STAR-like data. Particular attention is given to the impact of these perturbations on the upwelling and downwelling broadband fluxes and the direct aerosol radiative forcing at the bottom and top of the atmosphere. The results from this study suggest that limitations in the accuracy of 4STAR-retrieved particle size distributions and scattering phase functions have diminished impact on the accuracy of retrieved bulk microphysical parameters, permitting quite accurate retrievals of properties including the effective radius (up to 10%, or 0.03), and the radiatively important optical properties, such as the asymmetry factor (up to 4%, or 0.02) and single-scattering albedo (up to 6%, or 0.04). Also, the obtained results indicate that the uncertainties in the retrieved aerosol optical properties are quite small in the context of the calculated fluxes and direct aerosol radiative forcing (up to 15%, or 3 Wm-2).

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    CCN Activity and Mixing Rules of Isoprene Secondary Organic Aerosol (SOA) and Sulfate Download a printable PDF Submitter: Martin, S. T., Harvard University Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: King SM, T Rosenoern, JH Shilling, Q Chen, Z Wang, G Biskos, KA McKinney, U Poeschl, and ST Martin. 2010. "Cloud droplet activation of mixed organic-sulfate particles produced by the photooxidation of

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    How Aerosols Affect Cloud Properties in Arctic Mixed-Phase Stratocumulus Download a printable PDF Submitter: McFarquhar, G., University of Illinois, Urbana Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Jackson RC, GM McFarquhar, AV Korolev, ME Earle, PS Liu, RP Lawson, S Brooks, M Wolde, A Laskin, and M Freer. 2012. "The dependence of ice microphysics on aerosol concentration in arctic mixed-phase

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Initial Aerosol Concentration Is Key Contributor to Low-Level Cloud Reflectivity Submitter: Penner, J. E., University of Michigan Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Penner, J., Dong, X., Chen. Y., Observational evidence of a change in radiative forcing due to the indirect aerosol effect, Nature, Vol. 427, 15 January 2004. Cloud optical depth, as determined from the parcel model, is indicated by the dots. Red lines show best fit data of cloud liquid

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Effects of Relative Humidity on Aerosols-Implications for Climate Submitter: Lacis, A. A., NASA - Goddard Institute for Space Studies Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: "Refractive Indices of Three Hygroscopic Aerosols and their Dependence on Relative Humidity," October 2001. Sponsored by the DOE Atmospheric Radiation Measurement (ARM) Program, science collaborators at the National Aeronautics and Space Administration (NASA) Goddard

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Even at High Humidity, Aerosols Stick Around: Slowly Evaporating Particles Refute Assumption Download a printable PDF Submitter: Zelenyuk-Imre, A., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Wilson J, D Imre, J Beránek, M Shrivastava, and A Zelenyuk. 2014. "Evaporation kinetics of laboratory-generated secondary organic aerosols at elevated relative humidity." Environmental Science & Technology,

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Arctic Haze: Effect of Anthropogenic and Biomass Burning Aerosols Transported from Europe to the Arctic Download a printable PDF Submitter: Fast, J. ., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Marelle L, J Raut, JL Thomas, KS Law, B Quennehen, G Ancellet, J Pelon, A Schwarzenboeck, and JD Fast. 2015. "Transport of anthropogenic and biomass burning aerosols from Europe to the

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Radiative and Thermodynamic Responses to Uncertainty in Aerosol Extinction Profiles Download a printable PDF Submitter: Feng, Y., Argonne National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Feng Y, R Kotamarthi, R Coulter, C Zhao, and M Cadeddu. 2016. "Radiative and Thermodynamic Responses to Aerosol Extinction Profiles during the Pre-monsoon Month over South Asia." Atmospheric Chemistry and Physics, 16(1), 247-264. WRF-Chem

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Retrieving Cloud and Aerosol Properties from the ARM Raman Lidar Download a printable PDF Submitter: Thorsen, T., NASA - Langley Research Center Fu, Q., University of Washington Area of Research: Cloud Distributions/Characterizations Working Group(s): Aerosol Life Cycle, Cloud Life Cycle Journal Reference: Thorsen TJ, Q Fu, RK Newsom, DD Turner, and JM Comstock. 2015. "Automated retrieval of cloud and aerosol properties from the ARM Raman lidar, Part I: Feature detection." Journal of

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Phase State and Physical Properties of Ambient and Lab Generated Aerosols: X-ray Microscopy Download a printable PDF Submitter: OBrien, R. E., Lawrence Berkeley National Laboratory Gilles, M., Lawrence Berkeley National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: O'Brien RE, A Neu, SA Epstein, AC MacMillan, B Wang, ST Kelly, SA Nizkorodov, A Laskin, RC Moffet, and MK Gilles. 2014. "Physical properties of ambient and

  2. Lidar Measurements of the Vertical Distribution of Aerosol Optical and Physical Properties over Central Asia

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Chen, Boris B.; Sverdlik, Leonid G.; Imashev, Sanjar A.; Solomon, Paul A.; Lantz, Jeffrey; Schauer, James J.; Shafer, Martin M.; Artamonova, Maria S.; Carmichael, Gregory R.

    2013-01-01

    The vertical structure of aerosol optical and physical properties was measured by Lidar in Eastern Kyrgyzstan, Central Asia, from June 2008 to May 2009. Lidar measurements were supplemented with surface-based measurements of PM 2.5 and PM 10 mass and chemical composition in both size fractions. Dust transported into the region is common, being detected 33% of the time. The maximum frequency occurred in the spring of 2009. Dust transported to Central Asia comes from regional sources, for example, Taklimakan desert and Aral Sea basin, and from long-range transport, for example, deserts of Arabia, Northeast Africa, Iran, and Pakistan. Regionalmore » sources are characterized by pollution transport with maximum values of coarse particles within the planetary boundary layer, aerosol optical thickness, extinction coefficient, integral coefficient of aerosol backscatter, and minimum values of the Ångström exponent. Pollution associated with air masses transported over long distances has different characteristics during autumn, winter, and spring. During winter, dust emissions were low resulting in high values of the Ångström exponent (about 0.51) and the fine particle mass fraction (64%). Dust storms were more frequent during spring with an increase in coarse dust particles in comparison to winter. The aerosol vertical profiles can be used to lower uncertainty in estimating radiative forcing.« less

  3. Global Distribution and Climate Forcing of Marine Organic Aerosol - Part 2: Effects on Cloud Properties and Radiative Forcing

    SciTech Connect (OSTI)

    Gantt, Brett; Xu, Jun; Meskhidze, N.; Zhang, Yang; Nenes, Athanasios; Ghan, Steven J.; Liu, Xiaohong; Easter, Richard C.; Zaveri, Rahul A.

    2012-07-25

    A series of simulations with the Community Atmosphere Model version 5 (CAM5) with a 7-mode Modal Aerosol Model were conducted to assess the changes in cloud microphysical properties and radiative forcing resulting from marine organic aerosols. Model simulations show that the anthropogenic aerosol indirect forcing (AIF) predicted by CAM5 is decreased in absolute magnitude by up to 0.09 Wm{sup -2} (7 %) when marine organic aerosols are included. Changes in the AIF from marine organic aerosols are associated with small global increases in low-level incloud droplet number concentration and liquid water path of 1.3 cm{sup -3} (1.5 %) and 0.22 gm{sup -2} (0.5 %), respectively. Areas especially sensitive to changes in cloud properties due to marine organic aerosol include the Southern Ocean, North Pacific Ocean, and North Atlantic Ocean, all of which are characterized by high marine organic emission rates. As climate models are particularly sensitive to the background aerosol concentration, this small but non-negligible change in the AIF due to marine organic aerosols provides a notable link for ocean-ecosystem marine low-level cloud interactions and may be a candidate for consideration in future earth system models.

  4. Improved Arctic Cloud and Aerosol Research and Model Parameterizations

    SciTech Connect (OSTI)

    Kenneth Sassen

    2007-03-01

    In this report are summarized our contributions to the Atmospheric Measurement (ARM) program supported by the Department of Energy. Our involvement commenced in 1990 during the planning stages of the design of the ARM Cloud and Radiation Testbed (CART) sites. We have worked continuously (up to 2006) on our ARM research objectives, building on our earlier findings to advance our knowledge in several areas. Below we summarize our research over this period, with an emphasis on the most recent work. We have participated in several aircraft-supported deployments at the SGP and NSA sites. In addition to deploying the Polarization Diversity Lidar (PDL) system (Sassen 1994; Noel and Sassen 2005) designed and constructed under ARM funding, we have operated other sophisticated instruments W-band polarimetric Doppler radar, and midinfrared radiometer for intercalibration and student training purposes. We have worked closely with University of North Dakota scientists, twice co-directing the Citation operations through ground-to-air communications, and serving as the CART ground-based mission coordinator with NASA aircraft during the 1996 SUCCESS/IOP campaign. We have also taken a leading role in initiating case study research involving a number of ARM coinvestigators. Analyses of several case studies from these IOPs have been reported in journal articles, as we show in Table 1. The PDL has also participated in other major field projects, including FIRE II and CRYSTAL-FACE. In general, the published results of our IOP research can be divided into two categories: comprehensive cloud case study analyses to shed light on fundamental cloud processes using the unique CART IOP measurement capabilities, and the analysis of in situ data for the testing of remote sensing cloud retrieval algorithms. One of the goals of the case study approach is to provide sufficiently detailed descriptions of cloud systems from the data-rich CART environment to make them suitable for application to cloud modeling groups, such as the GEWEX Cloud Simulation Study (GCSS) Cirrus Working Groups. In this paper we summarize our IOP-related accomplishments.

  5. Investigations of the Absorption Properties of Near-Ground Aerosol by the Methods of Optical-Acoustic Spectrometry and Diff...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Investigations of the Absorption Properties of Near-Ground Aerosol by the Methods of Optical-Acoustic Spectrometry and Diffuse Extinction V. S. Kozlov, M. V. Panchenko, A. B. Tikhomirov, and B. A. Tikhomirov Institute of Atmospheric Optics Tomsk, Russia Introduction Aerosol absorption is an important factor in the formation of non-selective radiation extinction in the visible wavelength range, and plays a great role in solving many radiative and climatic problems. The principal absorbing

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Cumuli Impact on Solar Radiation at Surface: Spectral Changes Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle, Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Kassianov E, J Barnard, LK Berg, CN Long, and C Flynn. 2011. "Shortwave spectral radiative forcing of cumulus clouds from surface observations." Geophysical Research Letters, 38, L07801,

  7. [Plasma properties research: Task 3

    SciTech Connect (OSTI)

    Not Available

    1992-01-01

    The principal research activities of the Magneto-Fluid Dynamics Division relate to magnetic fusion plasma physics. In addition, there is a modest amount of work in closely related areas, including space plasma physics, fluid dynamics, and dynamical systems. Members of the Magneto-Fluid Dynamics Division maintain close contacts with fusion researchers in the US and abroad. Some of the work of the Division is clearly directed towards ITER and TPX, while other problems relate to the broader development of fusion plasma physics and to the support of other issues arising in the many experimental programs. Topics of some note in the last year that are discussed in this report are: Application of sophisticated statistical techniques to tokamak data reduction, including time series analysis of TFTR fluctuation data and spline analysis of profile data. Continuing development of edge plasma and divertor modelling, including initial ergodic divertor studies. Analysis of energetic fusion products losses from TFTR plasmas. Examination of anomalous transport in dynamical systems induced by chaotic-like Hamiltonian motion. Numerical simulation of the development of singular MHD equilibria. Exploration of the validity of moment expansions of kinetic equations for weakly collisional systems. Studies of RF- and ripple-induced helium ash removal. Ballooning mode studies in fluids and rotating stars. Studies in dynamical systems, including explosive instabilities, development of chaos, and motion of collisionless particles in a domain with overlapping islands.

  8. [Plasma properties research: Task 3

    SciTech Connect (OSTI)

    Not Available

    1992-12-31

    The principal research activities of the Magneto-Fluid Dynamics Division relate to magnetic fusion plasma physics. In addition, there is a modest amount of work in closely related areas, including space plasma physics, fluid dynamics, and dynamical systems. Members of the Magneto-Fluid Dynamics Division maintain close contacts with fusion researchers in the US and abroad. Some of the work of the Division is clearly directed towards ITER and TPX, while other problems relate to the broader development of fusion plasma physics and to the support of other issues arising in the many experimental programs. Topics of some note in the last year that are discussed in this report are: Application of sophisticated statistical techniques to tokamak data reduction, including time series analysis of TFTR fluctuation data and spline analysis of profile data. Continuing development of edge plasma and divertor modelling, including initial ergodic divertor studies. Analysis of energetic fusion products losses from TFTR plasmas. Examination of anomalous transport in dynamical systems induced by chaotic-like Hamiltonian motion. Numerical simulation of the development of singular MHD equilibria. Exploration of the validity of moment expansions of kinetic equations for weakly collisional systems. Studies of RF- and ripple-induced helium ash removal. Ballooning mode studies in fluids and rotating stars. Studies in dynamical systems, including explosive instabilities, development of chaos, and motion of collisionless particles in a domain with overlapping islands.

  9. ARM - Measurement - Aerosol backscattered radiation

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    RLPROF : Raman LIDAR Vertical Profiles UW-AIR : University of Washington Airborne Aerosol Instruments Value-Added Products AIP : Aerosol Intensive Properties (Process) AIP1OGREN :...

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    From Fire to Ice Download a printable PDF Submitter: Kulkarni, G., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Kulkarni GR, M Nandasiri, A Zelenyuk, J Beranek, N Madaan, A Devaraj, V Shutthanandan, S Thevuthasan, and T Varga. 2015. "Effects of crystallographic properties on the ice nucleation properties of volcanic ash particles." Geophysical Research Letters, 42(8), doi:10.1002/2015GL063270. Tons of

  11. Coupling Between Oceanic Upwelling and Cloud-aerosol Properties at the AMF Point Reyes Site

    SciTech Connect (OSTI)

    Dunn, M.; Jensen, M.; Miller, M.; Kollias, P.; Bartholomew, M. J.; Turner, D.; Andrews, E.; Jefferson, A.; Daum, P.

    2008-03-10

    Cloud microphysical properties measured at the ARM Mobile Facility site located on the northern coast of California near Point Reyes, during the 2005 Marine Stratus Radiation, Aerosol and Drizzle experiment, were analyzed to determine their relationship to the coastal sea surface temperature (SST) which was characterized using measurements acquired from a National Oceanic and Atmospheric Administration offshore buoy. An increase in SST resulting from a relaxation of upwelling, occurring in the eastern Pacific Ocean off the coast of California in summer is observed to strongly correlate with nearby ground measured cloud microphysical properties and cloud condensation nuclei (CCN) concentrations. Correlations between these atmospheric and oceanic features provide insight into the interplay between the ocean and cloud radiative properties. We present evidence of this robust correlation and examine the factors controlling these features. The marine boundary layer is in direct contact with the sea surface and is strongly influenced by SST. Moisture and vertical motion are crucial ingredients for cloud development and so we examine the role of SST in providing these key components to the atmosphere. Although upwelling of cold subsurface waters is conventionally thought to increase aerosols in the region, thus increasing clouds, here we observed a relaxation of upwelling associated with changes in the structure of marine stratus clouds. As upwelling relaxes, the SST get warmer, thick clouds with high liquid water paths are observed and persist for a few days. This cycle is repeated throughout the summer upwelling season. A concomitant cyclic increase and decrease of CCN concentration is also observed. Forcing mechanisms and large-scale atmospheric features are discussed. Marine stratocumulus clouds are a critical component of the earth's radiation budget and this site provides an excellent opportunity to study the influence of SST on these clouds.

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Pollution Hitches Ride to Arctic Download a printable PDF Submitter: Zelenyuk-Imre, A., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Zelenyuk A, D Imre, J Beranek, E Abramson, J Wilson, and M Shrivastava. 2012. "Synergy between secondary organic aerosols and long-range transport of polycyclic aromatic hydrocarbons." Environmental Science & Technology, 46(22), doi:10.1021/es302743z. When airborne

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MBL Cloud and CCN Properties Under Coupled and Decoupled Conditions Submitter: Dong, X., University of North Dakota Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Dong X, A Schwantes, B Xi, and P Wu. 2015. "Investigation of the marine boundary layer cloud and CCN properties under coupled and decoupled conditions over the Azores." Journal of Geophysical Research - Atmospheres, , 1-13. ONLINE. A

  14. Aerosol Extinction Profiles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    and Thermodynamic Responses to Uncertainty in Aerosol Extinction Profiles For original submission and image(s), see ARM Research Highlights http://www.arm.gov/science/highlights/ Research Highlight Aerosol radiative effects are of great importance for climate simulations over South Asia. For quantifying aerosol direct radiative effect, aerosol optical depth (AOD) and single scattering albedo (SSA) are often compared with observations. These comparisons have revealed large AOD underestimation and

  15. One ARM, Two Columns and a Whole Lot of Aerosols | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    ARM, Two Columns and a Whole Lot of Aerosols One ARM, Two Columns and a Whole Lot of Aerosols July 25, 2012 - 5:49pm Addthis This observatory is part of an air particles research initiative at Cape Cod National Seashore in Massachusetts, and includes dozens of sophisticated instruments that take continuous ground-based measurements of clouds, aerosols, and other atmospheric properties. | Photo courtesy of the ARM Climate Research Facility. This observatory is part of an air particles research

  16. Los Alamos researchers uncover new properties in nanocomposite...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    New properties in nanocomposite oxide ceramics Los Alamos researchers uncover new properties in nanocomposite oxide ceramics for reactor fuel, fast-ion conductors In a...

  17. Intellectual Property Provisions (GLB-115) Grant Research, Development...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    GLB-115) Grant Research, Development, or Demonstration Large Business and Foreign Entity Intellectual Property Provisions (GLB-115) Grant Research, Development, or Demonstration...

  18. Intellectual Property Provisions (GSB-115) Grant Research, Development...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    GSB-115) Grant Research, Development, or Demonstration Domestic Small Business Intellectual Property Provisions (GSB-115) Grant Research, Development, or Demonstration Domestic...

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Climate Warming Due to Soot and Smoke? Maybe Not. Submitter: Penner, J. E., University of Michigan Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Penner, J.E., S.Y. Zhang, and C.C. Chuang, Soot and smoke aerosol may not warm climate, J. Geophys. Res., 108(D21), 4657, doi:10.1029/2003JD003409, 2003. New research results from the Department of Energy's Atmospheric Radiation Measurement (ARM) Program suggest that fossil fuel soot emissions and biomass smoke may

  20. Intellectual Property Provisions (CSB-115) Cooperative Agreement Research,

    Energy Savers [EERE]

    Development, or Demonstration Domestic Small Business | Department of Energy 15) Cooperative Agreement Research, Development, or Demonstration Domestic Small Business Intellectual Property Provisions (CSB-115) Cooperative Agreement Research, Development, or Demonstration Domestic Small Business PDF icon CSB-115.pdf More Documents & Publications Intellectual Property Provisions (CSB-1003) Cooperative Agreement Research, Development, or Demonstration Domestic Small Businesses Intellectual

  1. Direct Aerosol Forcing Uncertainty

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Mccomiskey, Allison

    2008-01-15

    Understanding sources of uncertainty in aerosol direct radiative forcing (DRF), the difference in a given radiative flux component with and without aerosol, is essential to quantifying changes in Earth's radiation budget. We examine the uncertainty in DRF due to measurement uncertainty in the quantities on which it depends: aerosol optical depth, single scattering albedo, asymmetry parameter, solar geometry, and surface albedo. Direct radiative forcing at the top of the atmosphere and at the surface as well as sensitivities, the changes in DRF in response to unit changes in individual aerosol or surface properties, are calculated at three locations representing distinct aerosol types and radiative environments. The uncertainty in DRF associated with a given property is computed as the product of the sensitivity and typical measurement uncertainty in the respective aerosol or surface property. Sensitivity and uncertainty values permit estimation of total uncertainty in calculated DRF and identification of properties that most limit accuracy in estimating forcing. Total uncertainties in modeled local diurnally averaged forcing range from 0.2 to 1.3 W m-2 (42 to 20%) depending on location (from tropical to polar sites), solar zenith angle, surface reflectance, aerosol type, and aerosol optical depth. The largest contributor to total uncertainty in DRF is usually single scattering albedo; however decreasing measurement uncertainties for any property would increase accuracy in DRF. Comparison of two radiative transfer models suggests the contribution of modeling error is small compared to the total uncertainty although comparable to uncertainty arising from some individual properties.

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Can Ice-Nucleating Aerosols Affect Arctic Seasonal Climate? Submitter: Prenni, A. J., Colorado State University Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Prenni, A. J., J. Y. Harrington, M. Tjernstrom, P. J. DeMott, A. Avramov, C. N. Long, S. M. Kreidenweis, P. Q. Olsson, and J. Verlinde, (2006): Can Ice-Nucleating Aerosols Affect Arctic Seasonal Climate?, BAMS, Vol.88, Iss. 4; pg. 541-550. ACIA, 2004: Impacts of a Warming

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    When Pollution Gets a Whiff of Trees Download a printable PDF Submitter: Shilling, J., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Shilling JE, RA Zaveri, JD Fast, L Kleinman, M Alexander, MR Canagaratna, E Fortner, JM Hubbe, JT Jayne, A Sedlacek, A Setyan, S Springston, DR Worsnop, and Q Zhang. 2013. "Enhanced SOA formation from mixed anthropogenic and biogenic emissions during the CARES campaign."

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Wildfires Lead to More Warming Than Climate Models Predict, a New Mexico Fire Study Reports Download a printable PDF Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: China S, C Mazzoleni, K Gorkowski, AC Aiken, and MK Dubey. 2013. "Morphology and mixing state of individual freshly emitted wildfire carbonaceous particles." Nature Communications, 4, 2122, doi:10.1038/ncomms3122.

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Reality Check: Estimates for Human-Caused Methane Emissions in the U.S. Appear Off by 50% Download a printable PDF Submitter: Biraud, S. C., Lawrence Berkeley National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Miller SM, SC Wofsy, AM Michalak, EA Kort, AE Andrews, SC Biraud, EJ Dlugokencky, J Elszkeiwicz, ML Fischer, G Janssens-Maenhout, BR Miller, JB Miller, SA Montzka, T Nehrkorn, and C Sweeney. 2013. "Anthropogenic emissions

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Observing Warm Clouds in 3D Using ARM Scanning Cloud Radars and a Novel Ensemble Method Download a printable PDF Submitter: Fielding, M. D., University of Reading Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Fielding MD, J Chiu, RJ Hogan, and G Feingold. 2014. "A novel ensemble method for retrieving properties of warm cloud in 3-D using ground-based scanning radar and zenith

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Broadband Albedo Observations in the Southern Great Plains Submitter: Lamb, P. J., University of Oklahoma Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Journal of Applied Meteorology and Climatology, Vol. 45, 2006, pp. 210-235. Figure 1 Figure 2 Because surface reflection of solar radiation plays a fundamental role in the surface energy budget, knowledge of its spatial and temporal variability is important for understanding the weather and climate of a

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Dark Side of Cold Clouds Download a printable PDF Submitter: Kulkarni, G., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: China S, G Kulkarni, BV Scarnato, N Sharma, M Pekour, JE Shilling, J Wilson, A Zelenyuk, D Chand, S Liu, AC Aiken, MK Dubey, A Laskin, RA Zaveri, and C Mazzoleni. 2015. "Morphology of diesel soot residuals from supercooled water droplets and ice crystals: implications for optical

  9. Intellectual Property Provisions (GSB-115) Grant Research, Development, or

    Energy Savers [EERE]

    Demonstration Domestic Small Business | Department of Energy GSB-115) Grant Research, Development, or Demonstration Domestic Small Business Intellectual Property Provisions (GSB-115) Grant Research, Development, or Demonstration Domestic Small Business PDF icon GSB-115.pdf More Documents & Publications GSB-1003.PDF&#0; Intellectual Property Provisions (CLB-115) Cooperative Agreement Research, Development, or Demonstration Large Business and Foreign Entity Intellectual Property

  10. Automated retrieval of cloud and aerosol properties from the ARM Raman lidar, part 1: feature detection

    SciTech Connect (OSTI)

    Thorsen, Tyler J.; Fu, Qiang; Newsom, Rob K.; Turner, David D.; Comstock, Jennifer M.

    2015-11-01

    A Feature detection and EXtinction retrieval (FEX) algorithm for the Atmospheric Radiation Measurement (ARM) program’s Raman lidar (RL) has been developed. Presented here is part 1 of the FEX algorithm: the detection of features including both clouds and aerosols. The approach of FEX is to use multiple quantities— scattering ratios derived using elastic and nitro-gen channel signals from two fields of view, the scattering ratio derived using only the elastic channel, and the total volume depolarization ratio— to identify features using range-dependent detection thresholds. FEX is designed to be context-sensitive with thresholds determined for each profile by calculating the expected clear-sky signal and noise. The use of multiple quantities pro-vides complementary depictions of cloud and aerosol locations and allows for consistency checks to improve the accuracy of the feature mask. The depolarization ratio is shown to be particularly effective at detecting optically-thin features containing non-spherical particles such as cirrus clouds. Improve-ments over the existing ARM RL cloud mask are shown. The performance of FEX is validated against a collocated micropulse lidar and observations from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite over the ARM Darwin, Australia site. While we focus on a specific lidar system, the FEX framework presented here is suitable for other Raman or high spectral resolution lidars.

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Effects on Liquid-Water Path of Thin Stratocumulus Clouds Download a printable PDF Submitter: Penner, J. E., University of Michigan Lee, S., University of Michigan Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: n/a Thin clouds with mean liquid-water path (LWP) of ~ 50 g m-2 cover 27.5% of the globe and thus play an important role in the Earth's radiation budget. Radiative fluxes at the Earth's surface and top of atmosphere (TOA) are very sensitive to

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    More Like Shades of Gray: the Effects of Black Carbon in Aerosols Submitter: McComiskey, A. C., National Oceanic and Atmospheric Administration Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Cappa CD, TB Onasch, P Massoli, DR Worsnop, TS Bates, ES Cross, P Davidovits, J Hakala, KL Hayden, BT Jobson, KR Kolesar, DA Lack, BM Lerner, SM Li, D Mellon, I Nuaaman, JS Olfert, T Petaja, PK Quinn, C Song, R Subramanian, EJ Williams, and RA Zaveri. 2012.

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Dust in the Wind... and the Clouds... and the Atmosphere Submitter: Sassen, K., University of Alaska, Fairbanks Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Sassen, K., P.J. DeMott, J.M. Propsero, and M.R. Poellot, Saharan Dust Storms and Indirect Aerosol Effects on Clouds: CRYSTAL-FACE Results, Geophys. Res. Ltt., 30(12), 1633, doi:10/1029/2003GL017371, 2003. PDL linear depolarization ratio (color scale on top) and relative returned power (in gray scale) of

  14. Nanoscale Material Properties | GE Global Research

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Nanotechnology Drives New Levels of Performance Click to email this to a friend (Opens in new window) Share on Facebook (Opens in new window) Click to share (Opens in new window) Click to share on LinkedIn (Opens in new window) Click to share on Tumblr (Opens in new window) Nanotechnology Drives New Levels of Performance GE scientists are discovering new material properties at the nanoscale that drive new performance levels in jet engines, gas and steam turbines, electronic devices and disease

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Zhang, Q., University of California, Davis Fast, J. ., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal...

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Probing the Birth of New Particles Download a printable PDF Submitter: Wang, J., Brookhaven National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life...

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    First Observation-Based Estimates of Cloud-Free Aerosol Radiative Forcing Across China Download a printable PDF Submitter: Li, Z., University of Maryland Area of Research: Aerosol...

  18. The Two-Column Aerosol Project (TCAP) Science Plan

    SciTech Connect (OSTI)

    Berkowitz, CM; Berg, LK; Cziczo, DJ; Flynn, CJ; Kassianov, EI; Fast, JD; Rasch, PJ; Shilling, JE; Zaveri, RA; Zelenyuk, A; Ferrare, RA; Hostetler, CA; Cairns, B; Russell, PB; Ervens, B

    2011-07-27

    The Two-Column Aerosol Project (TCAP) field campaign will provide a detailed set of observations with which to (1) perform radiative and cloud condensation nuclei (CCN) closure studies, (2) evaluate a new retrieval algorithm for aerosol optical depth (AOD) in the presence of clouds using passive remote sensing, (3) extend a previously developed technique to investigate aerosol indirect effects, and (4) evaluate the performance of a detailed regional-scale model and a more parameterized global-scale model in simulating particle activation and AOD associated with the aging of anthropogenic aerosols. To meet these science objectives, the Atmospheric Radiation Measurement (ARM) Climate Research Facility will deploy the ARM Mobile Facility (AMF) and the Mobile Aerosol Observing System (MAOS) on Cape Cod, Massachusetts, for a 12-month period starting in the summer of 2012 in order to quantify aerosol properties, radiation, and cloud characteristics at a location subject to both clear and cloudy conditions, and clean and polluted conditions. These observations will be supplemented by two aircraft intensive observation periods (IOPs), one in the summer and a second in the winter. Each IOP will deploy one, and possibly two, aircraft depending on available resources. The first aircraft will be equipped with a suite of in situ instrumentation to provide measurements of aerosol optical properties, particle composition and direct-beam irradiance. The second aircraft will fly directly over the first and use a multi-wavelength high spectral resolution lidar (HSRL) and scanning polarimeter to provide continuous optical and cloud properties in the column below.

  19. Intellectual Property Provisions (CLB-115) Cooperative Agreement Research,

    Energy Savers [EERE]

    Development, or Demonstration Large Business and Foreign Entity | Department of Energy CLB-115) Cooperative Agreement Research, Development, or Demonstration Large Business and Foreign Entity Intellectual Property Provisions (CLB-115) Cooperative Agreement Research, Development, or Demonstration Large Business and Foreign Entity PDF icon CLB-115.pdf More Documents & Publications CLB-1003.PDF&#0; CDLB-1003.PDF&#0; Intellectual Property Provisions (CDLB-115) Cooperative Agreement -

  20. Los Alamos researchers uncover new properties in nanocomposite oxide

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ceramics for reactor fuel, fast-ion conductors Los Alamos researchers uncover new properties in nanocomposite oxide ceramics for reactor fuel, fast-ion conductors Alumni Link: Opportunities, News and Resources for Former Employees Latest Issue:September 2015 all issues All Issues » submit Los Alamos researchers uncover new properties in nanocomposite oxide ceramics for reactor fuel, fast-ion conductors In a nanocomposite, the size of each of these grains is on the order of nanometers,

  1. ARM - Research Highlights: Notable Findings

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    HighlightsNotable Research Findings Form Submit a New Research Highlight Sort Highlights Submitter Title Research Area Working Group Submission Date DOE Progress Reports Notable Research Findings for 2001-2006 Office of Science Abstracts Database Research Highlights Summaries Notable Research Findings for the Past Five Years Aerosols Cloud Parameterization and Modeling (Currently Cloud Modeling) Cloud Properties Instantaneous Radiative Flux (Currently Radiative Processes)

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Roles of Wind Shear at Different Vertical Levels in Cloud System Organization and Properties Download a printable PDF Submitter: Fan, J., Pacific Northwest National Laboratory Area of Research: Cloud Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Chen Q, J Fan, S Hagos, W Gustafson, and L Berg. 2015. "Roles of wind shear at different vertical levels, Part I: Cloud system organization and properties." Journal of Geophysical Research -

  3. Intellectual Property Provisions (GLB-115) Grant Research, Development, or

    Energy Savers [EERE]

    Demonstration Large Business and Foreign Entity | Department of Energy GLB-115) Grant Research, Development, or Demonstration Large Business and Foreign Entity Intellectual Property Provisions (GLB-115) Grant Research, Development, or Demonstration Large Business and Foreign Entity PDF icon GLB-115.pdf More Documents & Publications GLB-1003.PDF&#0; CLB-1003.PDF&#0; CDLB

  4. Indirect and Semi-Direct Aerosol Campaign: The Impact of Arctic Aerosols on Clouds

    SciTech Connect (OSTI)

    McFarquhar, Greg; Ghan, Steven J.; Verlinde, J.; Korolev, Alexei; Strapp, J. Walter; Schmid, Beat; Tomlinson, Jason M.; Wolde, Mengistu; Brooks, Sarah D.; Cziczo, Daniel J.; Dubey, Manvendra K.; Fan, Jiwen; Flynn, Connor J.; Gultepe, Ismail; Hubbe, John M.; Gilles, Mary K.; Laskin, Alexander; Lawson, Paul; Leaitch, W. R.; Liu, Peter S.; Liu, Xiaohong; Lubin, Dan; Mazzoleni, Claudio; Macdonald, A. M.; Moffet, Ryan C.; Morrison, H.; Ovchinnikov, Mikhail; Shupe, Matthew D.; Turner, David D.; Xie, Shaocheng; Zelenyuk, Alla; Bae, Kenny; Freer, Matthew; Glen, Andrew

    2011-02-01

    A comprehensive dataset of microphysical and radiative properties of aerosols and clouds in the arctic boundary layer in the vicinity of Barrow, Alaska was collected in April 2008 during the Indirect and Semi-Direct Aerosol Campaign (ISDAC) sponsored by the Department of Energy Atmospheric Radiation Measurement (ARM) and Atmospheric Science Programs. The primary aim of ISDAC was to examine indirect effects of aerosols on clouds that contain both liquid and ice water. The experiment utilized the ARM permanent observational facilities at the North Slope of Alaska (NSA) in Barrow. These include a cloud radar, a polarized micropulse lidar, and an atmospheric emitted radiance interferometer as well as instruments specially deployed for ISDAC measuring aerosol, ice fog, precipitation and spectral shortwave radiation. The National Research Council of Canada Convair-580 flew 27 sorties during ISDAC, collecting data using an unprecedented 42 cloud and aerosol instruments for more than 100 hours on 12 different days. Data were obtained above, below and within single-layer stratus on 8 April and 26 April 2008. These data enable a process-oriented understanding of how aerosols affect the microphysical and radiative properties of arctic clouds influenced by different surface conditions. Observations acquired on a heavily polluted day, 19 April 2008, are enhancing this understanding. Data acquired in cirrus on transit flights between Fairbanks and Barrow are improving our understanding of the performance of cloud probes in ice. Ultimately the ISDAC data will be used to improve the representation of cloud and aerosol processes in models covering a variety of spatial and temporal scales, and to determine the extent to which long-term surface-based measurements can provide retrievals of aerosols, clouds, precipitation and radiative heating in the Arctic.

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Dust Takes Detour on Ice-Cloud Journey Download a printable PDF Submitter: Kulkarni, G., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Kulkarni G, C Sanders, K Zhang, X Liu, and C Zhao. 2014. "Ice nucleation of bare and sulfuric acid-coated mineral dust particles and implication for cloud properties." Journal of Geophysical Research - Atmospheres, 119(16), doi:10.1002/2014JD021567. Cirrus clouds are

  6. The Indirect and Semi-Direct Aerosol Campaign

    SciTech Connect (OSTI)

    Ghan, Steve

    2014-03-24

    Research projects like the Indirect and Semi-Direct Aerosol Campaign, or ISDAC, increase our knowledge of atmospheric aerosol particles and cloud physics.

  7. The Indirect and Semi-Direct Aerosol Campaign

    ScienceCinema (OSTI)

    Ghan, Steve

    2014-06-12

    Research projects like the Indirect and Semi-Direct Aerosol Campaign, or ISDAC, increase our knowledge of atmospheric aerosol particles and cloud physics.

  8. Intellectual Property Provisions (CSB-1003) Cooperative Agreement Research,

    Energy Savers [EERE]

    Development, or Demonstration Domestic Small Businesses | Department of Energy 003) Cooperative Agreement Research, Development, or Demonstration Domestic Small Businesses Intellectual Property Provisions (CSB-1003) Cooperative Agreement Research, Development, or Demonstration Domestic Small Businesses 01. FAR 52.227-1 Authorization and Consent (JUL 1995)-Alternate I (APR 1984) 02. FAR 52.227-2 Notice and Assistance Regarding Patent and Copyright Infringement (AUG 1996) This clause is not

  9. Aerosol Observing System (AOS) Handbook

    SciTech Connect (OSTI)

    Jefferson, A

    2011-01-17

    The Aerosol Observing System (AOS) is a suite of in situ surface measurements of aerosol optical and cloud-forming properties. The instruments measure aerosol properties that influence the earths radiative balance. The primary optical measurements are those of the aerosol scattering and absorption coefficients as a function of particle size and radiation wavelength and cloud condensation nuclei (CCN) measurements as a function of percent supersaturation. Additional measurements include those of the particle number concentration and scattering hygroscopic growth. Aerosol optical measurements are useful for calculating parameters used in radiative forcing calculations such as the aerosol single-scattering albedo, asymmetry parameter, mass scattering efficiency, and hygroscopic growth. CCN measurements are important in cloud microphysical models to predict droplet formation.

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Turn Trash Into Treasure: Continental Warm Cloud Properties Derived from Unexploited Solar Background Signals Download a printable PDF Submitter: Chiu, J., University of Reading Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Chiu JC, JA Holmes, RJ Hogan, and EJ O'Connor. 2014. "The interdependence of continental warm cloud properties derived from unexploited solar background signals in

  11. Los Alamos researchers uncover new properties in nanocomposite oxide

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ceramics for reactor fuel, fast-ion conductors New properties in nanocomposite oxide ceramics Los Alamos researchers uncover new properties in nanocomposite oxide ceramics for reactor fuel, fast-ion conductors In a nanocomposite, the size of each of these grains is on the order of nanometers, roughly 1000 times smaller than the width of a human hair. September 23, 2014 Schematic depicting distinct dislocation networks for SrO- and TiO2-terminated SrTiO3/MgO interface. Schematic depicting

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Comparison of Mixed-layer Heights from Airborne HSRL and WRF-Chem During CARES Download a printable PDF Submitter: Scarino, A. J., Science Systems and Applications, Inc. Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Scarino AJ, MD Obland, JD Fast, SP Burton, RA Ferrare, CA Hostetler, LK Berg, B Lefer, C Haman, JW Hair, RR Rogers, C Butler, AL Cook, and DB Harper. 2014. "Comparison of mixed layer heights from airborne high spectral resolution

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Higher Clouds Retain Less Energy Download a printable PDF Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle Journal Reference: Qiu Y, Q Wang, and F Hu. 2012. "Shouxian aerosol radiative properties measured by DOE AMF and compared with CERES-MODIS." Advanced Materials Research, 518-523(2), doi:10.4028/www.scientific.net/AMR.518-523.1973. Clouds with bases at different altitudes.

  14. ARM Cloud Aerosol Precipitation Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Precipitation Experiment a NOAA ship in the Pacific Ocean and on a DOE- sponsored plane over land and sea. These researchers will study: (1) water sources, evolution and structure of atmospheric rivers over the Pacific Ocean (2) long range transport of aerosols over the Pacific Ocean between Hawaii and the U.S. West Coast, and how aerosols interact with atmospheric rivers (3) the point where atmospheric rivers make landfall on the U.S. West Coast, especially how clouds form where

  15. Science Overview Document Indirect and Semi-Direct Aerosol Campaign (ISDAC) April 2008

    SciTech Connect (OSTI)

    SJ Ghan; B Schmid; JM Hubbe; CJ Flynn; A Laskin; AA Zelenyuk; DJ Czizco; CN Long; G McFarquhar; J Verlinde; J Harrington; JW Strapp; P Liu; A Korolev; A McDonald; M Wolde; A Fridlind; T Garrett; G Mace; G Kok; S Brooks; D Collins; D Lubin; P Lawson; M Dubey; C Mazzoleni; M Shupe; S Xie; DD Turner; Q Min; EJ Mlawer; D Mitchell

    2007-11-01

    The ARM Climate Research Facilitys (ACRF) Aerial Vehicle Program (AVP) will deploy an intensive cloud and aerosol observing system to the ARM North Slope of Alaska (NSA) locale for a five week Indirect and Semi-Direct Aerosol Campaign (ISDAC) during period 29 March through 30 April 2008. The deployment period is within the International Polar Year, thus contributing to and benefiting from the many ancillary observing systems collecting data synergistically. We will deploy the Canadian National Research Council Convair 580 aircraft to measure temperature, humidity, total particle number, aerosol size distribution, single particle composition, concentrations of cloud condensation nuclei and ice nuclei, optical scattering and absorption, updraft velocity, cloud liquid water and ice contents, cloud droplet and crystal size distributions, cloud particle shape, and cloud extinction. In addition to these aircraft measurements, ISDAC will deploy two instruments at the ARM site in Barrow: a spectroradiometer to retrieve cloud optical depth and effective radius, and a tandem differential mobility analyzer to measure the aerosol size distribution and hygroscopicity. By using many of the same instruments used during Mixed-Phase Arctic Cloud Experiment (M-PACE), conducted in October 2004, we will be able to contrast the arctic aerosol and cloud properties during the fall and spring transitions. The aerosol measurements can be used in cloud models driven by objectively analyzed boundary conditions to test whether the cloud models can simulate the aerosol influence on the clouds. The influence of aerosol and boundary conditions on the simulated clouds can be separated by running the cloud models with all four combinations of M-PACE and ISDAC aerosol and boundary conditions: M-PACE aerosol and boundary conditions, M-PACE aerosol and ISDAC boundary conditions, ISDAC aerosol and M-PACE boundary conditions, and ISDAC aerosol and boundary conditions. ISDAC and M-PACE boundary conditions are likely to be very different because of the much more extensive ocean water during M-PACE. The uniformity of the surface conditions during ISDAC greatly simplifies the objective analysis (surface fluxes and precipitation are very weak), so that it can largely rely on the European Centre for Medium-Range Weather Forecasts analysis. The aerosol measurements can also be used as input to the cloud models and to evaluate the aerosol retrievals. By running the cloud models with and without solar absorption by the aerosols, we can determine the semidirect effect of the aerosol on the clouds.

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Study Aerosol Humidity Effects Using the ARM Measurements Submitter: Li, Z., University of Maryland Area of Research: Radiation Processes Working Group(s): Aerosol Journal Reference: Jeong, M.-J., Z. Li, E. Andrews, and S.-C. Tsay (2007). Effect of aerosol humidification on the column aerosol optical thickness over the Atmospheric Radiation Measurement Southern Great Plains site, J. Geophys. Res., 112, D10202, doi:10.1029/2006JD007176. (a)-(j) Column-mean aerosol humidification factor as

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    A Dance of Aerosols Download a printable PDF Submitter: Song, C., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Song C, RA Zaveri, JE Shilling, ML Alexander, and M Newburn. 2011. "Effect of hydrophilic organic seed aerosols on secondary organic aerosol formation from ozonolysis of α-pinene." Environmental Science & Technology, 45(17), doi:10.1021/es201225c. The injection of alpha-pinene, a

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    What Exactly Do Metrics for Aerosol-Cloud Interactions Represent? Download a printable PDF Submitter: McComiskey, A. C., National Oceanic and Atmospheric Administration Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Aerosol Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: McComiskey A and G Feingold. 2012. "The scale problem in quantifying aerosol indirect effects." Atmospheric Chemistry and Physics, 12, doi:10.5194/acp-12-1031-2012.

  19. ARM - Cumulus Humilis Aerosol Processing Study (CHAPS)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Study (CHAPS) Campaign Details News Field Participants Resources Status and Actions ARM Data Discovery Browse Data Cumulus Humilis Aerosol Processing Study (CHAPS) Summer 2007 ASP Field Campaign The primary goal of the CHAPS campaign is to characterize and contrast freshly emitted aerosols above, within and below fields of cumulus humilis (or fair-weather cumulus). These observations will be used to examine the aerosol optical properties and cloud nucleating properties from both below-cloud and

  20. Holistic Interactions of Shallow Clouds, Aerosols, and Land-Ecosystems (HI-SCALE) Science Plan

    SciTech Connect (OSTI)

    Fast, JD; Berg, LK

    2015-12-01

    Cumulus convection is an important component in the atmospheric radiation budget and hydrologic cycle over the Southern Great Plains and over many regions of the world, particularly during the summertime growing season when intense turbulence induced by surface radiation couples the land surface to clouds. Current convective cloud parameterizations contain uncertainties resulting in part from insufficient coincident data that couples cloud macrophysical and microphysical properties to inhomogeneities in boundary layer and aerosol properties. The Holistic Interactions of Shallow Clouds, Aerosols, and Land-Ecosystems (HI-SCALE) campaign is designed to provide a detailed set of measurements that are needed to obtain a more complete understanding of the life cycle of shallow clouds by coupling cloud macrophysical and microphysical properties to land surface properties, ecosystems, and aerosols. HI-SCALE consists of 2, 4-week intensive observational periods, one in the spring and the other in the late summer, to take advantage of different stages and distribution of “greenness” for various types of vegetation in the vicinity of the Atmospheric Radiation and Measurement (ARM) Climate Research Facility’s Southern Great Plains (SGP) site as well as aerosol properties that vary during the growing season. Most of the proposed instrumentation will be deployed on the ARM Aerial Facility (AAF) Gulfstream 1 (G-1) aircraft, including those that measure atmospheric turbulence, cloud water content and drop size distributions, aerosol precursor gases, aerosol chemical composition and size distributions, and cloud condensation nuclei concentrations. Routine ARM aerosol measurements made at the surface will be supplemented with aerosol microphysical properties measurements. The G-1 aircraft will complete transects over the SGP Central Facility at multiple altitudes within the boundary layer, within clouds, and above clouds.

  1. CARES: Carbonaceous Aerosol and Radiative Effects Study Science Plan

    SciTech Connect (OSTI)

    Zaveri, RA; Shaw, WJ; Cziczo, DJ

    2010-05-27

    Carbonaceous aerosol components, which include black carbon (BC), urban primary organic aerosols (POA), biomass burning aerosols, and secondary organic aerosols (SOA) from both urban and biogenic precursors, have been previously shown to play a major role in the direct and indirect radiative forcing of climate. The primary objective of the CARES 2010 intensive field study is to investigate the evolution of carbonaceous aerosols of different types and their effects on optical and cloud formation properties.

  2. CARES: Carbonaceous Aerosol and Radiative Effects Study Operations Plan

    SciTech Connect (OSTI)

    Zaveri, RA; Shaw, WJ; Cziczo, DJ

    2010-07-12

    The CARES field campaign is motivated by the scientific issues described in the CARES Science Plan. The primary objectives of this field campaign are to investigate the evolution and aging of carbonaceous aerosols and their climate-affecting properties in the urban plume of Sacramento, California, a mid-size, mid-latitude city that is located upwind of a biogenic volatile organic compound (VOC) emission region. Our basic observational strategy is to make comprehensive gas, aerosol, and meteorological measurements upwind, within, and downwind of the urban area with the DOE G-1 aircraft and at strategically located ground sites so as to study the evolution of urban aerosols as they age and mix with biogenic SOA precursors. The NASA B-200 aircraft, equipped with the High Spectral Resolution Lidar (HSRL), digital camera, and the Research Scanning Polarimeter (RSP), will be flown in coordination with the G-1 to characterize the vertical and horizontal distribution of aerosols and aerosol optical properties, and to provide the vertical context for the G-1 and ground in situ measurements.

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Brass Ring of Climate Modeling Download a printable PDF Submitter: Ghan, S. J., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Ghan SJ, SJ Smith, M Wang, K Zhang, K Pringle, K Carslaw, J Pierce, S Bauer, and P Adams. 2013. "A simple model of global aerosol indirect effects." Journal of Geophysical Research - Atmospheres, 118, 1-20. The simple model of aerosol effects on clouds

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Invisible Giants in the Sky Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Kassianov E, M Pekour, and J Barnard. 2012. "Aerosols in central California: Unexpectedly large contribution of coarse mode to aerosol radiative forcing." Geophysical Research Letters, 39, L20806, doi:10.1029/2012GL053469. Photo

  5. Chemical composition, microstructure, and hygroscopic properties of aerosol particles at the Zotino Tall Tower Observatory (ZOTTO), Siberia, during a summer campaign

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Mikhailov, E. F.; Mironov, G. N.; Pöhlker, C.; Chi, X.; Krüger, M. L.; Shiraiwa, M.; Förster, J. -D.; Pöschl, U.; Vlasenko, S. S.; Ryshkevich, T. I.; et al

    2015-03-16

    In this study we describe the hygroscopic properties of accumulation- and coarse-mode aerosol particles sampled at the Zotino Tall Tower Observatory (ZOTTO) in Central Siberia (61° N; 89° E) from 16 to 21 June 2013. The hygroscopic growth measurements were supplemented with chemical analyses of the samples, including inorganic ions and organic/elemental carbon. In addition, the microstructure and chemical composition of aerosol particles were analyzed by X-ray micro-spectroscopy (STXM-NEXAFS) and transmission electron microscopy (TEM). A mass closure analysis indicates that organic carbon accounted for 61 and 38% of PM in the accumulation mode and coarse mode, respectively. The water solublemore » fraction of organic matter was estimated to be 52 and 8% of PM in these modes. Sulfate, predominantly in the form of ammoniated sulfate, was the dominant inorganic component in both size modes: ~ 34% in the accumulation vs. ~ 47% in the coarse mode. The hygroscopic growth measurements were conducted with a filter-based differential hygroscopicity analyzer (FDHA) over the range of 5–99.4% RH in the hydration and dehydration operation modes. The FDHA study indicates that both accumulation and coarse modes exhibit pronounced water uptake approximately at the same RH, starting at ~ 70%, while efflorescence occurred at different humidities, i.e., at ~ 35% RH for submicron particles vs. ~ 50% RH for supermicron particles. This ~ 15% RH difference was attributed to higher content of organic material in the submicron particles, which suppresses water release in the dehydration experiments. The kappa mass interaction model (KIM) was applied to characterize and parameterize non-ideal solution behavior and concentration-dependent water uptake by atmospheric aerosol samples in the 5–99.4% RH range. Based on KIM, the volume-based hygroscopicity parameter, κv, was calculated. The κv, ws value related to the water soluble (ws) fraction was estimated to be ~ 0.15 for the accumulation mode and ~ 0.36 for the coarse mode, respectively. The obtained κv, ws for the accumulation mode is in good agreement with earlier data reported for remote sites in the Amazon rain forest (κv ≈ 0.15) and a Colorado boreal forest (κv ≈ 0.16). We used the Zdanovskii–Stokes–Robinson (ZSR) mixing rule to predict the chemical composition dependent hygroscopicity, κv, p. The obtained κv, p values overestimate the experimental FDHA-KIM-derived κv, ws by factors of 1.8 and 1.5 for the accumulation and coarse modes, respectively. This divergence can be partly explained by incomplete dissolution of the hygroscopic inorganic compounds resulting from kinetic limitations due to a sparingly soluble organic coating. The TEM and STXM-NEXAFS results indicate that aged submicron (>300 nm) and supermicron aerosol particles possess core-shell structures with an inorganic core, and are enriched in organic carbon at the mixed particle surface. The direct FDHA kinetic studies provide a bulk diffusion coefficient of water of ~ 10−12 cm2 s−1 indicating a semi-solid state of the organic-rich phase leading to kinetic limitations of water uptake and release during hydration and dehydration cycles. Overall the present ZOTTO data set, obtained in the growing season, has revealed a strong influence of organic carbon on the hygroscopic properties of the ambient aerosols. The sparingly soluble organic coating controls hygroscopic growth, phase transitions, and microstructural rearrangement processes. The observed kinetic limitations can strongly influence the outcome of experiments performed on multi-second time scales, such as the commonly applied HTDMA (Hygroscopicity Tandem Differential Mobility Analyzer) and CCNC (Cloud Condensation Nuclei Counter) measurements.« less

  6. Chemical composition, microstructure, and hygroscopic properties of aerosol particles at the Zotino Tall Tower Observatory (ZOTTO), Siberia, during a summer campaign

    SciTech Connect (OSTI)

    Mikhailov, E. F.; Mironov, G. N.; Phlker, C.; Chi, X.; Krger, M. L.; Shiraiwa, M.; Frster, J. -D.; Pschl, U.; Vlasenko, S. S.; Ryshkevich, T. I.; Weigand, M.; Kilcoyne, A. L. D.; Andreae, M. O.

    2015-03-16

    In this study we describe the hygroscopic properties of accumulation- and coarse-mode aerosol particles sampled at the Zotino Tall Tower Observatory (ZOTTO) in Central Siberia (61 N; 89 E) from 16 to 21 June 2013. The hygroscopic growth measurements were supplemented with chemical analyses of the samples, including inorganic ions and organic/elemental carbon. In addition, the microstructure and chemical composition of aerosol particles were analyzed by X-ray micro-spectroscopy (STXM-NEXAFS) and transmission electron microscopy (TEM). A mass closure analysis indicates that organic carbon accounted for 61 and 38% of PM in the accumulation mode and coarse mode, respectively. The water soluble fraction of organic matter was estimated to be 52 and 8% of PM in these modes. Sulfate, predominantly in the form of ammoniated sulfate, was the dominant inorganic component in both size modes: ~ 34% in the accumulation vs. ~ 47% in the coarse mode.

    The hygroscopic growth measurements were conducted with a filter-based differential hygroscopicity analyzer (FDHA) over the range of 599.4% RH in the hydration and dehydration operation modes. The FDHA study indicates that both accumulation and coarse modes exhibit pronounced water uptake approximately at the same RH, starting at ~ 70%, while efflorescence occurred at different humidities, i.e., at ~ 35% RH for submicron particles vs. ~ 50% RH for supermicron particles. This ~ 15% RH difference was attributed to higher content of organic material in the submicron particles, which suppresses water release in the dehydration experiments.

    The kappa mass interaction model (KIM) was applied to characterize and parameterize non-ideal solution behavior and concentration-dependent water uptake by atmospheric aerosol samples in the 599.4% RH range. Based on KIM, the volume-based hygroscopicity parameter, ?v, was calculated. The ?v, ws value related to the water soluble (ws) fraction was estimated to be ~ 0.15 for the accumulation mode and ~ 0.36 for the coarse mode, respectively. The obtained ?v, ws for the accumulation mode is in good agreement with earlier data reported for remote sites in the Amazon rain forest (?v ≈ 0.15) and a Colorado boreal forest (?v ≈ 0.16).

    We used the ZdanovskiiStokesRobinson (ZSR) mixing rule to predict the chemical composition dependent hygroscopicity, ?v, p. The obtained ?v, p values overestimate the experimental FDHA-KIM-derived ?v, ws by factors of 1.8 and 1.5 for the accumulation and coarse modes, respectively. This divergence can be partly explained by incomplete dissolution of the hygroscopic inorganic compounds resulting from kinetic limitations due to a sparingly soluble organic coating. The TEM and STXM-NEXAFS results indicate that aged submicron (>300 nm) and supermicron aerosol particles possess core-shell structures with an inorganic core, and are enriched in organic carbon at the mixed particle surface. The direct FDHA kinetic studies provide a bulk diffusion coefficient of water of ~ 10?12 cm2 s?1 indicating a semi-solid state of the organic-rich phase leading to kinetic limitations of water uptake and release during hydration and dehydration cycles. Overall the present ZOTTO data set, obtained in the growing season, has revealed a strong influence of organic carbon on the hygroscopic properties of the ambient aerosols. The sparingly soluble organic coating controls hygroscopic growth, phase transitions, and microstructural rearrangement processes. The observed kinetic limitations can strongly influence the outcome of experiments performed on multi-second time scales, such as the commonly applied HTDMA (Hygroscopicity Tandem Differential Mobility Analyzer

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    energy balance due to aerosol-radiation interactions, but the effect depends on the dust optical properties assumed in the simulations without mineralogy. More importantly, the...

  8. eDPS Aerosol Collection

    SciTech Connect (OSTI)

    Venzie, J.

    2015-10-13

    The eDPS Aerosol Collection project studies the fundamental physics of electrostatic aerosol collection for national security applications. The interpretation of aerosol data requires understanding and correcting for biases introduced from particle genesis through collection and analysis. The research and development undertaken in this project provides the basis for both the statistical correction of existing equipment and techniques; as well as, the development of new collectors and analytical techniques designed to minimize unwanted biases while improving the efficiency of locating and measuring individual particles of interest.

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Simulating the Impact of Aerosols on Tropical Deep Convection Download a printable PDF Submitter: Morrison, H. C., NCAR Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Morrison H and WW Grabowski. 2011. "Cloud-system resolving model simulations of aerosol indirect effects on tropical deep convection and its thermodynamic environment." Atmospheric Chemistry and Physics, 11(20),

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Mixing State of Carbonaceous Aerosol Particles in Northern and Southern California Measured During CARES and CalNex Download a printable PDF Submitter: Zaveri, R., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Cahill JF, K Suski, JH Seinfeld, RA Zaveri, and KA Prather. 2012. "The mixing state of carbonaceous aerosol particles in Northern and Southern California measured during CARES and CalNex

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Parameterizing the Mixing State of Complex Submicron Aerosols Using Chemical Imaging Download a printable PDF Submitter: Moffet, R., University of the Pacific Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: O'Brien RE, B Wang, A Laskin, N Riemer, M West, Q Zhang, Y Sun, X Yu, P Alpert, DA Knopf, MK Gilles, and RC Moffet. 2015. "Chemical imaging of ambient aerosol particles: Observational constraints on mixing state parameterization." Journal

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosols Help Clouds Warm Up Arctic Submitter: Lubin, D., National Science Foundation Area of Research: Radiation Processes Working Group(s): Radiative Processes Journal Reference: Lubin, D., and A.M. Vogelmann, 2006: A climatologically significant aerosol longwave indirect effect in the Arctic, Nature, 439, 26 January, 453-456, doi:10.1038/nature04449 In a process known as the first aerosol indirect effect, enhanced aerosol concentrations cause the droplets in a cloud to be smaller and more

  13. Ganges Valley Aerosol Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ganges Valley Aerosol Experiment In northeastern India, the fertile land around the Ganges River supports several hundred million people. This river, the largest in India, is fed by monsoon rains and runoff from the nearby Himalayan Mountains. Through an intergovernmental agreement with India, the U.S. Department of Energy's Atmospheric Radiation Measurement (ARM) Climate Research Facility deployed its portable laboratory, the ARM Mobile Facility (AMF), to Nainital, India, in June 2011. During

  14. Cloud Properties Derived from Visible and Near-infrared Reflectance in the

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Presence of Aerosols Cloud Properties Derived from Visible and Near-infrared Reflectance in the Presence of Aerosols Hofmann, Odele University of Colorado at Boulder Pilewskie, Peter University of Colorado Gore, Warren NASA Ames Research Center Russell, Phil NASA Ames Research Center Livingston, John SRI International Redemann, Jens BAERI/NASA Ames Research Center Bergstrom, Robert Bay Area Environmental Research Institute Platnick, Steven NASA-GSFC Daniel, John NOAA Aeronomy Laboratory

  15. Building America Webinar: Sealing of Home Enclosures with Aerosol...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Sealing of Home Enclosures with Aerosol Particles This webinar was presented by research team Building Industry Research Alliance (BIRA), and provided information about a project...

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Quantifying Error in the Radiative Forcing of the First Aerosol Indirect Effect Submitter: McComiskey, A. C., National Oceanic and Atmospheric Administration Area of Research:...

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Burning on the Prairies Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation...

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    energy budget of the atmospheric column. Researchers used measurements of atmospheric temperature and humidity profiles and ground-based retrievals of aerosol optical...

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    a printable PDF Submitter: Marshak, A., NASA - Goddard Space Flight Center Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions...

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Fog and Rain in the Amazon Download a printable PDF Submitter: Gentine, P., Columbia University Sobel, A., Columbia University Area of Research: Cloud-Aerosol-Precipitation...

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    to Lose Download a printable PDF Submitter: Laskin, A., Pacific Northwest National Laboratory Fast, J. ., Pacific Northwest National Laboratory Area of Research: Aerosol...

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Black Carbon Aerosols and the Third Polar Ice Cap Submitter: Menon, S., Lawrence Berkeley National Laboratory Area of Research: General Circulation and Single Column Models...

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Pollution + Storm Clouds Warmer Atmosphere Download a printable PDF Submitter: Fan, J., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation...

  4. ARM - Measurement - Aerosol concentration

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    CSPHOT : Cimel Sunphotometer CPC : Condensation Particle Counter HTDMA : Humidified Tandem Differential Mobility Analyzer IAP : In-situ Aerosol Profiles (Cessna Aerosol Flights)...

  5. Cloud Properties Working Group Low Clouds Update

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    radiative fluxes, and Optical properties and radiative fluxes, and Associated aerosol prop. & atmospheric state Associated aerosol prop. & atmospheric state Long Long - - term...

  6. ARM - AIP1OGREN: AOS Intensive Properties

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govDataAIP1OGREN: AOS Intensive Properties AIP1OGREN: AOS Intensive Properties The aip1ogren value-added product produces aerosol intensive properties from Aerosol Observing Station data. Information Last Updated: October 2008 General Description The aip1ogren value-added product (VAP) computes several aerosol intensive properties. It requires as input calibrated, corrected, aerosol extensive properties (scattering and absorption coefficients, primarily) from the Aerosol Observing Station (AOS).

  7. Final Technical Report for Collaborative Research: CRI-EaSM Multiscale Modeling Aerosol Indirect Effects on Decadal Timescales

    SciTech Connect (OSTI)

    Park, Sungsu

    2015-11-29

    Originally, the main role of the P.I. (Sungsu Park) in this project was to improve the treatment of cloud microphysics in the CAM5 shallow and deep convection scheme. During the progress of the project, however, the main research theme was changed to develop a new unified convection scheme (so called, UNICON) with the permission of the program manager.

  8. ARM - Field Campaign - Two-Column Aerosol Project (TCAP): Winter...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    on atmospheric particulate matter. The effect of aerosol properties such as size, morphology and composition on cloud droplet formation has been studied theoretically as well as...

  9. Preliminary Results of in-situ Measurements of Aerosol Optical...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    of Aerosol Optical and Water Uptake Properties from the ARM Mobile Facility in Niger Jefferson, Anne NOAA CMDL Ogren, John NOAACMDL Category: Field Campaigns The second...

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    "Invisible" Giants in the Sky Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Kassianov E, M Pekour, and J Barnard. 2012. "Aerosols in central California: Unexpectedly large contribution of coarse mode to aerosol radiative forcing." Geophysical Research Letters, 39, L20806, doi:10.1029/2012GL053469. Daily averaged values of (a, b) the direct

  11. Aerosol Characterization Data from the Asian Pacific Regional Aerosol Characterization Project (ACE-Asia)

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    The Aerosol Characterization Experiments (ACE) were designed to increase understanding of how atmospheric aerosol particles affect the Earth's climate system. These experiments integrated in-situ measurements, satellite observations, and models to reduce the uncertainty in calculations of the climate forcing due to aerosol particles and improve the ability of models to predict the influences of aerosols on the Earth's radiation balance. ACE-Asia was the fourth in a series of experiments organized by the International Global Atmospheric Chemistry (IGAC) Program (A Core Project of the International Geosphere Biosphere Program). The Intensive Field Phase for ACE-Asia took place during the spring of 2001 (mid-March through early May) off the coast of China, Japan and Korea. ACE-Asia pursued three specific objectives: 1) Determine the physical, chemical, and radiative properties of the major aerosol types in the Eastern Asia and Northwest Pacific region and investigate the relationships among these properties. 2) Quantify the physical and chemical processes controlling the evolution of the major aerosol types and in particular their physical, chemical, and radiative properties. 3) Develop procedures to extrapolate aerosol properties and processes from local to regional and global scales, and assess the regional direct and indirect radiative forcing by aerosols in the Eastern Asia and Northwest Pacific region [Edited and shortened version of summary at http://data.eol.ucar.edu/codiac/projs?ACE-ASIA]. The Ace-Asia collection contains 174 datasets.

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Seasonal and Interannual Variability in 13C of Ecosystem Carbon Fluxes from 2002-2009 Submitter: Torn, M. S., Lawrence Berkeley National Laboratory Area of Research: Surface Properties Working Group(s): Aerosol Life Cycle Journal Reference: Torn MS, SC Biraud, CJ Still, WJ Riley, and JA Berry. 2011. "Seasonal and inter-annual variability in δ13C of net ecosystem carbon exchanges from 2002-2009 in the U.S. Southern Great Plains." Tellus, 63(2), 10.1111/j.1600-0889.2010.00519.x. Time

  13. Study of Aerosol Indirect Effects in China

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Indirect Effects in China In 2008, the U.S. Department of Energy (DOE)'s Atmospheric Radiation Measurement (ARM) Climate Research Facility is providing the ARM Mobile...

  14. Light Absorption of Primary Organic Aerosol Paper Named ACS Editors...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Absorption of Primary Organic Aerosol Paper Named ACS Editors' Choice For original submission and image(s), see ARM Research Highlights http:www.arm.govsciencehighlights...

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Indirect Impact of Atmospheric Aerosols on an Ensemble of Deep Convective Clouds Download a printable PDF Submitter: Grabowski, W., NCAR Morrison, H. C., NCAR Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Grabowski WW and H Morrison. 2011. "Indirect impact of atmospheric aerosols in idealized simulations of convective-radiative quasi-equilibrium. Part II: Double-moment microphysics." Journal of

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Improving Estimates of Cloud Condensation Nuclei Concentration Download a printable PDF Submitter: Li, Z., University of Maryland Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Liu J and Z Li. 2014. "Estimation of cloud condensation nuclei concentration from aerosol optical quantities: influential factors and uncertainties." Atmospheric Chemistry and Physics, 14(1), doi:10.5194/acp-14-1-2014.

  17. Aerosol mobility size spectrometer

    DOE Patents [OSTI]

    Wang, Jian (Port Jefferson, NY); Kulkarni, Pramod (Port Jefferson Station, NY)

    2007-11-20

    A device for measuring aerosol size distribution within a sample containing aerosol particles. The device generally includes a spectrometer housing defining an interior chamber and a camera for recording aerosol size streams exiting the chamber. The housing includes an inlet for introducing a flow medium into the chamber in a flow direction, an aerosol injection port adjacent the inlet for introducing a charged aerosol sample into the chamber, a separation section for applying an electric field to the aerosol sample across the flow direction and an outlet opposite the inlet. In the separation section, the aerosol sample becomes entrained in the flow medium and the aerosol particles within the aerosol sample are separated by size into a plurality of aerosol flow streams under the influence of the electric field. The camera is disposed adjacent the housing outlet for optically detecting a relative position of at least one aerosol flow stream exiting the outlet and for optically detecting the number of aerosol particles within the at least one aerosol flow stream.

  18. Laboratory Studies of Processing of Carbonaceous Aerosols by Atmospheric Oxidants/Hygroscopicity and CCN Activity of Secondary & Processed Primary Organic Aerosols

    SciTech Connect (OSTI)

    Ziemann, P.J.; Arey, J.; Atkinson, R.; Kreidenweis, S.M.; Petters, M.D.

    2012-06-13

    The atmosphere is composed of a complex mixture of gases and suspended microscopic aerosol particles. The ability of these particles to take up water (hygroscopicity) and to act as nuclei for cloud droplet formation significantly impacts aerosol light scattering and absorption, and cloud formation, thereby influencing air quality, visibility, and climate in important ways. A substantial, yet poorly characterized component of the atmospheric aerosol is organic matter. Its major sources are direct emissions from combustion processes, which are referred to as primary organic aerosol (POA), or in situ processes in which volatile organic compounds (VOCs) are oxidized in the atmosphere to low volatility reaction products that subsequent condense to form particles that are referred to as secondary organic aerosol (SOA). POA and VOCs are emitted to the atmosphere from both anthropogenic and natural (biogenic) sources. The overall goal of this experimental research project was to conduct laboratory studies under simulated atmospheric conditions to investigate the effects of the chemical composition of organic aerosol particles on their hygroscopicity and cloud condensation nucleation (CCN) activity, in order to develop quantitative relationships that could be used to more accurately incorporate aerosol-cloud interactions into regional and global atmospheric models. More specifically, the project aimed to determine the products, mechanisms, and rates of chemical reactions involved in the processing of organic aerosol particles by atmospheric oxidants and to investigate the relationships between the chemical composition of organic particles (as represented by molecule sizes and the specific functional groups that are present) and the hygroscopicity and CCN activity of oxidized POA and SOA formed from the oxidation of the major classes of anthropogenic and biogenic VOCs that are emitted to the atmosphere, as well as model hydrocarbons. The general approach for this project was to carry out reactions of representative anthropogenic and biogenic VOCs and organic particles with ozone (O3), and hydroxyl (OH), nitrate (NO3), and chlorine (Cl) radicals, which are the major atmospheric oxidants, under simulated atmospheric conditions in large-volume environmental chambers. A combination of on-line and off-line analytical techniques were used to monitor the chemical and physical properties of the particles including their hygroscopicity and CCN activity. The results of the studies were used to (1) improve scientific understanding of the relationships between the chemical composition of organic particles and their hygroscopicity and CCN activity, (2) develop an improved molecular level theoretical framework for describing these relationships, and (3) establish a large database that is being used to develop parameterizations relating organic aerosol chemical properties and SOA sources to particle hygroscopicity and CCN activity for use in regional and global atmospheric air quality and climate models.

  19. Raman Lidar Measurements of Aerosols and Water Vapor During the May 2003 Aerosol IOP

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Raman Lidar Measurements of Aerosols and Water Vapor During the May 2003 Aerosol IOP R. A. Ferrare National Aeronautics and Space Administration Langley Research Center Hampton, Virginia D. D. Turner Pacific Northwest National Laboratory Richland, Washington M. Clayton Science Applications International Corporation National Aeronautics and Space Administration Langley Research Center Hampton, Virginia B. S. Schmid and J. Redemann BAER/NASA Ames Research Institute Moffett Field, California D.

  20. ARM - Measurement - Aerosol scattering

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    : Nephelometer PASS : Photoacoustic Soot Spectrometer RL : Raman Lidar TDMA : Tandem Differential Mobility Analyzer Field Campaign Instruments AMT : Aerosol Modeling...

  1. Building America Webinar: Sealing of Home Enclosures with Aerosol Particles

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    | Department of Energy Sealing of Home Enclosures with Aerosol Particles Building America Webinar: Sealing of Home Enclosures with Aerosol Particles This webinar was presented by research team Building Industry Research Alliance (BIRA), and provided information about a project that uses existing aerosol duct sealing technology to seal the entire building enclosure in order to achieve greater airtightness and energy and cost savings. File webinar_bira_20111014.wmv More Documents &

  2. Solid aerosol generator

    DOE Patents [OSTI]

    Prescott, D.S.; Schober, R.K.; Beller, J.

    1992-03-17

    An improved solid aerosol generator used to produce a gas borne stream of dry, solid particles of predetermined size and concentration is disclosed. The improved solid aerosol generator nebulizes a feed solution of known concentration with a flow of preheated gas and dries the resultant wet heated aerosol in a grounded, conical heating chamber, achieving high recovery and flow rates. 2 figs.

  3. Solid aerosol generator

    DOE Patents [OSTI]

    Prescott, Donald S. (Shelley, ID); Schober, Robert K. (Midwest City, OK); Beller, John (Idaho Falls, ID)

    1992-01-01

    An improved solid aerosol generator used to produce a gas borne stream of dry, solid particles of predetermined size and concentration. The improved solid aerosol generator nebulizes a feed solution of known concentration with a flow of preheated gas and dries the resultant wet heated aerosol in a grounded, conical heating chamber, achieving high recovery and flow rates.

  4. Improved solid aerosol generator

    DOE Patents [OSTI]

    Prescott, D.S.; Schober, R.K.; Beller, J.

    1988-07-19

    An improved solid aerosol generator used to produce a gas borne stream of dry, solid particles of predetermined size and concentration. The improved solid aerosol generator nebulizes a feed solution of known concentration with a flow of preheated gas and dries the resultant wet heated aerosol in a grounded, conical heating chamber, achieving high recovery and flow rates. 2 figs.

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Long-Term Impacts of Aerosols on the Vertical Development of Clouds and Precipitation Download a printable PDF Submitter: Li, Z., University of Maryland Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Li Z, F Niu, J Fan, Y Liu, and D Rosenfeld. 2011. "The long-term impacts of aerosols on the vertical development of clouds and precipitation." Nature-Geoscience, 4, doi:10.1038/NGEO1313. Changes

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    To Rain or Not to Rain...Aerosols May Be the Answer Download a printable PDF Submitter: Li, Z., University of Maryland Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Niu F and Z Li. 2012. "Systematic variations of cloud top temperature and precipitation rate with aerosols over the global tropics." Atmospheric Chemistry and Physics, 12, doi:10.5194/acp-12-8491-2012. Cloud-top temperature (A, C) and

  7. Ash Deposit Formation and Deposit Properties. A Comprehensive Summary of Research Conducted at Sandia's Combustion Research Facility

    SciTech Connect (OSTI)

    Larry L. Baxter

    2000-08-01

    This report summarizes experimental and theoretical work performed at Sandia's Combustion Research Facility over the past eight years on the fate of inorganic material during coal combustion. This work has been done under four broad categories: coal characterization, fly ash formation, ash deposition, and deposit property development. The objective was to provide sufficient understanding of these four areas to be able to predict coal behavior in current and advanced conversion systems. This work has led to new characterization techniques for fuels that provide, for the first time, systematic and species specific information regarding the inorganic material. The transformations of inorganic material during combustion can be described in terms of the net effects of the transformations of these individual species. Deposit formation mechanisms provide a framework for predicting deposition rates for abroad range of particle sizes. Predictions based on these rates many times are quite accurate although there are important exceptions. A rigorous framework for evaluating deposit has been established. Substantial data have been obtained with which to exercise this framework, but this portion of the work is less mature than is any other. Accurate prediction of deposit properties as functions of fuel properties, boiler design, and boiler operating conditions represents the single most critical area where additional research is needed.

  8. Electrically Driven Technologies for Radioactive Aerosol Abatement

    SciTech Connect (OSTI)

    David W. DePaoli; Ofodike A. Ezekoye; Costas Tsouris; Valmor F. de Almeida

    2003-01-28

    The purpose of this research project was to develop an improved understanding of how electriexecy driven processes, including electrocoalescence, acoustic agglomeration, and electric filtration, may be employed to efficiently treat problems caused by the formation of aerosols during DOE waste treatment operations. The production of aerosols during treatment and retrieval operations in radioactive waste tanks and during thermal treatment operations such as calcination presents a significant problem of cost, worker exposure, potential for release, and increased waste volume.

  9. East Asian Studies of Tropospheric Aerosols and their Impact on Regional Climate (EAST-AIRC): An Overview

    SciTech Connect (OSTI)

    Li, Zhanqing; Li, C.; Chen, H.; Tsay, S. C.; Holben, B. N.; Huang, J.; Li, B.; Maring, H.; Qian, Yun; Shi, Guangyu; Xia, X.; Yin, Y.; Zheng, Y.; Zhuang, G.

    2011-02-01

    As the most populated region of the world, Asia is a major source of aerosols with potential large impact over vast downstream areas. Papers published in this special section describe the variety of aerosols observed in China and their effects and interactions with the regional climate as part of the East Asian Study of Tropospheric Aerosols and Impact on Regional Climate (EAST-AIRC). The majority of the papers are based on analyses of observations made under three field projects, namely, the Atmospheric Radiation Measurements (ARM) Mobile Facility mission in China (AMF10 China), the East Asian Study of Tropospheric Aerosols: an International Regional Experiment (EAST-AIRE), and the Atmospheric Aerosols of China and their Climate Effects (AACCE). The former two are US-China collaborative projects and the latter is a part of the China’s National Basic Research program (or often referred to as “973 project”). Routine meteorological data of China are also employed in some studies. The wealth of general and specialized measurements lead to extensive and close-up investigations of the optical, physical and chemical properties of anthropogenic, natural, and mixed aerosols; their sources, formation and transport mechanisms; horizontal, vertical and temporal variations; direct and indirect effects and interactions with the East Asian monsoon system. Particular efforts are made to advance our understanding of the mixing and interaction between dust and anthropogenic pollutants during transport. Several modeling studies were carried out to simulate aerosol impact on radiation budget, temperature, precipitation, wind and atmospheric circulation, fog, etc. In addition, impacts of the Asian monsoon system on aerosol loading are also simulated.

  10. Final Report for Research Conducted at The Scripps Institution of Oceanography, University of California San Diego from 2/2002 to 8/2003 for ''Aerosol and Cloud-Field Radiative Effects in the Tropical Western Pacific: Analyses and General Circulation Model Parameterizations''

    SciTech Connect (OSTI)

    Vogelmann, A. M.

    2004-01-27

    OAK-B135 Final report from the University of California San Diego for an ongoing research project that was moved to Brookhaven National Laboratory where proposed work will be completed. The research uses measurements made by the Atmospheric Radiation Measurement (ARM) Program to quantify the effects of aerosols and clouds on the Earth's energy balance in the climatically important Tropical Western Pacific.

  11. ARM - Publications: Science Team Meeting Documents: A decade long aerosol

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    and cloud statistics and aerosol indirect effect at the ARM SGP site A decade long aerosol and cloud statistics and aerosol indirect effect at the ARM SGP site Min, Qilong State University of New York at Albany Duan, Minzheng State University of New York at Albany Harrison, Lee State University of New York Joseph, Everette Howard University Twelve-year data of MFRSR and MWR have been used to derive aerosol and cloud optical properties at the ARM SGP. Diurnal, monthly, seasonal and

  12. Aerodynamic Focusing Of High-Density Aerosols

    SciTech Connect (OSTI)

    Ruiz, D. E.; Fisch, Nathaniel

    2014-02-24

    High-density micron-sized particle aerosols might form the basis for a number of applications in which a material target with a particular shape might be quickly ionized to form a cylindrical or sheet shaped plasma. A simple experimental device was built in order to study the properties of high-density aerosol focusing for 1#22; m silica spheres. Preliminary results recover previous findings on aerodynamic focusing at low densities. At higher densities, it is demonstrated that the focusing properties change in a way which is consistent with a density dependent Stokes number.

  13. Project Overview: Cumulus Humilis Aerosol Processing Study (CHAPS): Proposed Summer 2007 ASP Field Campaign

    SciTech Connect (OSTI)

    Berkowitz, Carl M.; Berg, Larry K.; Ogren, J. A.; Hostetler, Chris A.; Ferrare, Richard

    2006-05-18

    This white paper presents the scientific motivation and preliminary logistical plans for a proposed ASP field campaign to be carried out in the summer of 2007. The primary objective of this campaign is to use the DOE Gulfstream-1 aircraft to make measurements characterizing the chemical, physical and optical properties of aerosols below, within and above large fields of fair weather cumulus and to use the NASA Langley Research Centers High Spectral Resolution Lidar (HSRL) to make independent measurements of aerosol backscatter and extinction profiles in the vicinity of these fields. Separate from the science questions to be addressed by these observations will be information to add in the development of a parameterized cumulus scheme capable of including multiple cloud fields within a regional or global scale model. We will also be able to compare and contrast the cloud and aerosol properties within and outside the Oklahoma City plume to study aerosol processes within individual clouds. Preliminary discussions with the Cloud and Land Surface Interaction Campaign (CLASIC) science team have identified overlap between the science questions posed for the CLASIC Intensive Operation Period (IOP) and the proposed ASP campaign, suggesting collaboration would benefit both teams.

  14. ARM - Measurement - Aerosol extinction

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    extinction ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol extinction The removal of radiant energy from an incident beam by the process of aerosol absorption and/or scattering. Categories Aerosols Instruments The above measurement is considered scientifically relevant for the following instruments. Refer to the datastream (netcdf) file headers of each instrument for a list of all available

  15. ARM - Measurement - Aerosol image

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    image ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol image Images of aerosols from which one can derive characteristics such as size and shape. Categories Aerosols Instruments The above measurement is considered scientifically relevant for the following instruments. Refer to the datastream (netcdf) file headers of each instrument for a list of all available measurements, including those

  16. Two-Column Aerosol Project

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Column Aerosol Project Tiny particles in the sky known as "aerosols" come in many forms-dust, soot, and sea salt, for example. Depending on the type of aerosol, it can either...

  17. Particulate Matter Aerosols

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The study of atmospheric aerosols is important because of its adverse effects on health, air quality, visibility, cultural heritage, and Earth's radiation balance. Techniques that...

  18. ARM - Measurement - Aerosol composition

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    quality assurance purposes. ARM Instruments PILS : Particle Into Liquid Sampler TDMA : Tandem Differential Mobility Analyzer Field Campaign Instruments AEROSMASSSPEC : Aerosol Mass...

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Effect of Dry Deposition of Condensable Organic Vapors on SOA Formation in the Urban Plume Download a printable PDF Submitter: Hodzic, A., NCAR Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Hodzic A, S Madronich, B Aumont, J Lee-Taylor, T Karl, M Camredon, and C Mouchel-Vallon. 2014. "Limited influence of dry deposition of semi-volatile organic vapors on secondary organic aerosol formation in the urban plume." Geophysical Research Letters,

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lord of the Wings: Elevated Particles a Rising Star Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Kassianov E, C Flynn, J Redemann, B Schmid, PB Russell, and A Sinyuk. 2012. "Initial assessment of the Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR)-based aerosol retrieval: Sensitivity study." Atmosphere, 3,

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Twenty Years Serving Climate Science Download a printable PDF Submitter: Mather, J. H., Pacific Northwest National Laboratory Area of Research: Cloud Processes Working Group(s): Aerosol Life Cycle, Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Mather JH and JW Voyles. 2013. "The ARM Climate Research Facility: a review of structure and capabilities." Bulletin of the American Meteorological Society, 94(3), doi:10.1175/BAMS-D-11-00218.1. A scanning ARM

  2. 2010 Atmospheric System Research (ASR) Science Team Meeting Summary

    SciTech Connect (OSTI)

    Dupont, DL

    2011-05-04

    This document contains the summaries of papers presented in poster format at the March 2010 Atmospheric System Research Science Team Meeting held in Bethesda, Maryland. More than 260 posters were presented during the Science Team Meeting. Posters were sorted into the following subject areas: aerosol-cloud-radiation interactions, aerosol properties, atmospheric state and surface, cloud properties, field campaigns, infrastructure and outreach, instruments, modeling, and radiation. To put these posters in context, the status of ASR at the time of the meeting is provided here.

  3. Portable Aerosol Contaminant Extractor

    DOE Patents [OSTI]

    Carlson, Duane C. (N. Augusta, SC); DeGange, John J. (Aiken, SC); Cable-Dunlap, Paula (Waynesville, NC)

    2005-11-15

    A compact, portable, aerosol contaminant extractor having ionization and collection sections through which ambient air may be drawn at a nominal rate so that aerosol particles ionized in the ionization section may be collected on charged plate in the collection section, the charged plate being readily removed for analyses of the particles collected thereon.

  4. Techniques and Methods Used to Determine the Aerosol Best Estimate...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    I: Aerosol Optical Properties. J. Geophys. Res., 109, D06208, doi:10.10292003JD004025. Daniel, J. S., and coauthors, 2002: Cloud liquid water and ice measurements from...

  5. Study of in-duct spray drying using condensation aerosol

    SciTech Connect (OSTI)

    Chen, W.J.R.; Chang, S.M.; Adikesavalu, R. )

    1992-06-01

    Sulfur removal efficiency of in-duct spray drying is limited by sorbent content and surface properties of the sorbent-water aerosol. It was the purpose of this study to improve the sulfur removal efficiency for in-duct spray drying by injecting condensation aerosol instead of conventional dispersion aerosol. The program was composed of three phases. In Phase I, a novel pulsed fluid bed feeder was developed and was used to feed hydrated lime for subsequent experiments. A small condensation aerosol generator was then built, which produces a lime-water condensation aerosol by condensing steam on lime particles. The results show that novel lime-water aerosols less than 10 microns were generated. The central task in Phase II was to simulate experimentally in-duct spray drying using condensation aerosols and compare the results with those using dispersion aerosols reported in the literature. A small entrained-flow reactor was constructed to simulate an in-duct spray dryer. The condensation aerosol was then introduced to the reactor at various approach to saturation temperature, calcium/sulfur stoichiometry and sulfur dioxide concentration for desulfurization study. The results show that we have improved the sulfur removal efficiency for in-duct spray drying to 90 percent or above. Thus we have met and exceeded the stated project goal of 70 percent sulfur removal. A comprehensive computer code was employed to calculate sulfur removal efficiency in Phase III.

  6. Climate implications of carbonaceous aerosols: An aerosol microphysical study using the GISS/MATRIX climate model

    SciTech Connect (OSTI)

    Bauer, Susanne E.; Menon, Surabi; Koch, Dorothy; Bond, Tami; Tsigaridis, Kostas

    2010-04-09

    Recently, attention has been drawn towards black carbon aerosols as a likely short-term climate warming mitigation candidate. However the global and regional impacts of the direct, cloud-indirect and semi-direct forcing effects are highly uncertain, due to the complex nature of aerosol evolution and its climate interactions. Black carbon is directly released as particle into the atmosphere, but then interacts with other gases and particles through condensation and coagulation processes leading to further aerosol growth, aging and internal mixing. A detailed aerosol microphysical scheme, MATRIX, embedded within the global GISS modelE includes the above processes that determine the lifecycle and climate impact of aerosols. This study presents a quantitative assessment of the impact of microphysical processes involving black carbon, such as emission size distributions and optical properties on aerosol cloud activation and radiative forcing. Our best estimate for net direct and indirect aerosol radiative forcing change is -0.56 W/m{sup 2} between 1750 and 2000. However, the direct and indirect aerosol effects are very sensitive to the black and organic carbon size distribution and consequential mixing state. The net radiative forcing change can vary between -0.32 to -0.75 W/m{sup 2} depending on these carbonaceous particle properties. Assuming that sulfates, nitrates and secondary organics form a coating shell around a black carbon core, rather than forming a uniformly mixed particles, changes the overall net radiative forcing from a negative to a positive number. Black carbon mitigation scenarios showed generally a benefit when mainly black carbon sources such as diesel emissions are reduced, reducing organic and black carbon sources such as bio-fuels, does not lead to reduced warming.

  7. Effect of Aerosol Humidification on the Column Aerosol Optical Thickness

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    over the ARM Southern Great Plains Site Effect of Aerosol Humidification on the Column Aerosol Optical Thickness over the ARM Southern Great Plains Site Li, Zhanqing University of Maryland Jeong, Myeong-Jae University of Maryland Category: Aerosols This study investigates the aerosol humidification effect (AHE) using seventy profiles of the aerosol scattering and absorption coefficients at high (~85%) and low (~40%) relative humidity (RH) levels obtained over the Southern Great Plains (SGP)

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Mingling in the Sky-A View from the Earth Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Madhavan BL, Y He, Y Wu, B Gross, F Moshary, and S Ahmed. 2012. "Development of a ground based remote sensing approach for direct evaluation of aerosol-cloud interaction." Atmosphere, 3(4), doi:10.3390/atmos3040468. Two different types of

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Clouds Re-gathered by Wind Shear Download a printable PDF Submitter: Yang, Q., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Yang Q, RC Easter, P Campuzano-Jost, JL Jimenez, JD Fast, SJ Ghan, H Wang, LK Berg, MC Barth, Y Liu, MB Shrivastava, B Singh, H Morrison, J Fan, CL Ziegler, M Bela, E Apel, GS Diskin, T Mikoviny, and A Wisthaler. 2015. "Aerosol transport and

  10. ARM: 10-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    1998-03-01

    10-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  11. ARM: 1-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    2004-10-01

    1-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  12. ARM: 10-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    10-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  13. ARM: 1-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    1-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  14. Final Technical Report for "Ice nuclei relation to aerosol properties: Data analysis and model parameterization for IN in mixed-phase clouds"? (DOE/SC00002354)

    SciTech Connect (OSTI)

    Paul J. DeMott, Anthony J. Prenni; Sonia M. Kreidenweis

    2012-09-28

    Clouds play an important role in weather and climate. In addition to their key role in the hydrologic cycle, clouds scatter incoming solar radiation and trap infrared radiation from the surface and lower atmosphere. Despite their importance, feedbacks involving clouds remain as one of the largest sources of uncertainty in climate models. To better simulate cloud processes requires better characterization of cloud microphysical processes, which can affect the spatial extent, optical depth and lifetime of clouds. To this end, we developed a new parameterization to be used in numerical models that describes the variation of ice nuclei (IN) number concentrations active to form ice crystals in mixed-phase (water droplets and ice crystals co-existing) cloud conditions as these depend on existing aerosol properties and temperature. The parameterization is based on data collected using the Colorado State University continuous flow diffusion chamber in aircraft and ground-based campaigns over a 14-year period, including data from the DOE-supported Mixed-Phase Arctic Cloud Experiment. The resulting relationship is shown to more accurately represent the variability of ice nuclei distributions in the atmosphere compared to currently used parameterizations based on temperature alone. When implemented in one global climate model, the new parameterization predicted more realistic annually averaged cloud water and ice distributions, and cloud radiative properties, especially for sensitive higher latitude mixed-phase cloud regions. As a test of the new global IN scheme, it was compared to independent data collected during the 2008 DOE-sponsored Indirect and Semi-Direct Aerosol Campaign (ISDAC). Good agreement with this new data set suggests the broad applicability of the new scheme for describing general (non-chemically specific) aerosol influences on IN number concentrations feeding mixed-phase Arctic stratus clouds. Finally, the parameterization was implemented into a regional cloud-resolving model to compare predictions of ice crystal concentrations and other cloud properties to those observed in two intensive case studies of Arctic stratus during ISDAC. Our implementation included development of a prognostic scheme of ice activation using the IN parameterization so that the most realistic treatment of ice nuclei, including their budget (gains and losses), was achieved. Many cloud microphysical properties and cloud persistence were faithfully reproduced, despite a tendency to under-predict (by a few to several times) ice crystal number concentrations and cloud ice mass, in agreement with some other studies. This work serves generally as the basis for improving predictive schemes for cloud ice crystal activation in cloud and climate models, and more specifically as the basis for such a scheme to be used in a Multi-scale Modeling Format (MMF) that utilizes a connected system of cloud-resolving models on a global grid in an effort to better resolve cloud processes and their influence on climate.

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Mexico City Carbon-Containing Particle Composition Simulated Download a printable PDF Submitter: Zaveri, R., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Lee-Taylor J, S Madronich, B Aumont, M Camredon, A Hodzic, GS Tyndall, E Aperl, and RA Zaveri. 2012. "Explicit modeling of organic chemistry and secondary organic aerosol partitioning for Mexico City and its outflow plume." Atmospheric Chemistry and

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Influence of Regional Anthropogenic Emission Reductions on Aerosol Direct Radiative Forcing Download a printable PDF Submitter: Bergmann, D., Lawrence Livermore National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Yu H, M Chin, J West, C Atherton, N Bellouin, D Bergmann, I Bey, H Bian, T Diehl, G Forberth, P Hess, M Schulz, D Shindell, T Takemura, and Q Tan. 2012. "An HTAP multi-model assessment of the influence of regional

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Measured Radiative Cooling from Reflective Roofs in India Download a printable PDF Submitter: Fischer, M. L., Lawrence Berkeley National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle, Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Salamanca F, S Tonse, S Menon, V Garg, KP Singh, M Naja, and ML Fischer. 2012. "Top-of-atmosphere radiative cooling with white roofs: Experimental verification and model-based evaluation."

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Development and Validation of a Black Carbon Mixing State Resolved Three-Dimensional Model Download a printable PDF Submitter: Fast, J. ., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Matsui H, M Koike, Y Kondo, N Moteki, JD Fast, and RA Zaveri. 2013. "Development and validation of a black carbon mixing state resolved three-dimensional model: Aging processes and radiative impact." Journal of

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Forecast Calls for Better Models: Examining the Core Components of Arctic Clouds to Clear Their Influence on Climate Download a printable PDF Submitter: Laskin, A., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Aerosol Life Cycle Journal Reference: Hiranuma N, SD Brooks, RC Moffet, A Glen, A Laskin, MK Gilles, P Liu, AM Macdonald, JW Strapp, and GM McFarquhar. 2013. "Chemical characterization of individual particles and

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Scientists Uncover Combustion Mechanism to Better Predict Warming by Wildfires Download a printable PDF Submitter: Dubey, M. K., Los Alamos National Laboratory Donahue, N., Carnegie Mellon University Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Saleh R, E Robinson, D Tkacik, A Ahern, S Liu, A Aiken, R Sullivan, A Presto, M Dubey, R Yokelson, N Donahue, and A Robinson. 2014. "Brownness of organics in aerosols from biomass burning linked to

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    KDP Columns: Characterizing Deep Thunderstorm Updrafts Using Polarimetric Radar Download a printable PDF Submitter: van Lier-Walqui, M., NASA Fridlind, A. M., NASA - Goddard Institute for Space Studies Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: van Lier-Walqui M, AM Fridlind, AS Ackerman, S Collis, J Helmus, DR MacGorman, K North, P Kollias, and DJ Posselt. 2015. "On polarimetric radar signatures

  2. ARM - Measurement - Aerosol absorption

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption ARM Data Discovery Browse Data Comments? We would love to hear from you Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol absorption The...

  3. Monodisperse aerosol generator

    DOE Patents [OSTI]

    Ortiz, Lawrence W. (Los Alamos, NM); Soderholm, Sidney C. (Pittsford, NY)

    1990-01-01

    An aerosol generator is described which is capable of producing a monodisperse aerosol within narrow limits utilizing an aqueous solution capable of providing a high population of seed nuclei and an organic solution having a low vapor pressure. The two solutions are cold nebulized, mixed, vaporized, and cooled. During cooling, particles of the organic vapor condense onto the excess seed nuclei, and grow to a uniform particle size.

  4. Aerosol Optical Depth Value-Added Product Report

    SciTech Connect (OSTI)

    Koontz, A; Hodges, G; Barnard, J; Flynn, C; Michalsky, J

    2013-03-17

    This document describes the process applied to retrieve aerosol optical depth (AOD) from multifilter rotating shadowband radiometers (MFRSR) and normal incidence multifilter radiometers (NIMFR) operated at the ARM Climate Research Facility’s ground-based facilities.

  5. Lidar Investigation of Tropical Nocturnal Boundary Layer Aerosols and Cloud Macrophysics

    SciTech Connect (OSTI)

    Manoj, M. G.; Devara, PC S.; Taraphdar, Sourav

    2013-10-01

    Observational evidence of two-way association between nocturnal boundary layer aerosols and cloud macrophysical properties under different meteorological conditions is reported in this paper. The study has been conducted during 2008-09 employing a high space-time resolution polarimetric micro-pulse lidar over a tropical urban station in India. Firstly, the study highlights the crucial role of boundary layer aerosols and background meteorology on the formation and structure of low-level stratiform clouds in the backdrop of different atmospheric stability conditions. Turbulent mixing induced by the wind shear at the station, which is associated with a complex terrain, is found to play a pivotal role in the formation and structural evolution of nocturnal boundary layer clouds. Secondly, it is shown that the trapping of energy in the form of outgoing terrestrial radiation by the overlying low-level clouds can enhance the aerosol mixing height associated with the nocturnal boundary layer. To substantiate this, the long-wave heating associated with cloud capping has been quantitatively estimated in an indirect way by employing an Advanced Research Weather Research and Forecasting (WRF-ARW) model version 2.2 developed by National Center for Atmospheric Research (NCAR), Colorado, USA, and supplementary data sets; and differentiated against other heating mechanisms. The present investigation as well establishes the potential of lidar remote-sensing technique in exploring some of the intriguing aspects of the cloud-environment relationship.

  6. ARM - Field Campaign - In-situ Aerosol Profiles (Cessna Aerosol...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    would love to hear from you Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : In-situ Aerosol Profiles (Cessna Aerosol Flights) 2000.03.01 - 2007.10.31 Lead...

  7. Organic Aerosol Component (OACOMP) Value-Added Product Report

    SciTech Connect (OSTI)

    Fast, J; Zhang, Q; Tilp, A; Shippert, T; Parworth, C; Mei, F

    2013-08-23

    Significantly improved returns in their aerosol chemistry data can be achieved via the development of a value-added product (VAP) of deriving OA components, called Organic Aerosol Components (OACOMP). OACOMP is primarily based on multivariate analysis of the measured organic mass spectral matrix. The key outputs of OACOMP are the concentration time series and the mass spectra of OA factors that are associated with distinct sources, formation and evolution processes, and physicochemical properties.

  8. Indirect and Semi-Direct Aerosol Campaign

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Campaign For the month of April, researchers are descending on and above Barrow, Alaska, to obtain data from the atmosphere that will help them understand the impacts that aerosols have on Arctic clouds and climate. Scientists sponsored by the U.S. Department of Energy's Atmospheric Radiation Measurement (ARM) Climate Research Facility are using a heavily instrumented aircraft to collect data from the sky, while instruments based at surface sites in Barrow and Atqasuk, Alaska, are obtaining

  9. ARM - Measurement - Aerosol effective radius

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    effective radius ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol effective radius Aerosol effective radius is the ratio of the third and second moments of the number size distribution of aerosol particles. Categories Aerosols Instruments The above measurement is considered scientifically relevant for the following instruments. Refer to the datastream (netcdf) file headers of each instrument for

  10. Parameterizations of Cloud Microphysics and Indirect Aerosol Effects

    SciTech Connect (OSTI)

    Tao, Wei-Kuo

    2014-05-19

    1. OVERVIEW Aerosols and especially their effect on clouds are one of the key components of the climate system and the hydrological cycle [Ramanathan et al., 2001]. Yet, the aerosol effect on clouds remains largely unknown and the processes involved not well understood. A recent report published by the National Academy of Science states "The greatest uncertainty about the aerosol climate forcing - indeed, the largest of all the uncertainties about global climate forcing - is probably the indirect effect of aerosols on clouds [NRC, 2001]." The aerosol effect on clouds is often categorized into the traditional "first indirect (i.e., Twomey)" effect on the cloud droplet sizes for a constant liquid water path [Twomey, 1977] and the "semi-direct" effect on cloud coverage [e.g., Ackerman et al., 2000]. Enhanced aerosol concentrations can also suppress warm rain processes by producing a narrow droplet spectrum that inhibits collision and coalescence processes [e.g., Squires and Twomey, 1961; Warner and Twomey, 1967; Warner, 1968; Rosenfeld, 1999]. The aerosol effect on precipitation processes, also known as the second type of aerosol indirect effect [Albrecht, 1989], is even more complex, especially for mixed-phase convective clouds. Table 1 summarizes the key observational studies identifying the microphysical properties, cloud characteristics, thermodynamics and dynamics associated with cloud systems from high-aerosol continental environments. For example, atmospheric aerosol concentrations can influence cloud droplet size distributions, warm-rain process, cold-rain process, cloud-top height, the depth of the mixed phase region, and occurrence of lightning. In addition, high aerosol concentrations in urban environments could affect precipitation variability by providing an enhanced source of cloud condensation nuclei (CCN). Hypotheses have been developed to explain the effect of urban regions on convection and precipitation [van den Heever and Cotton, 2007 and Shepherd, 2005]. Recently, a detailed spectral-bin microphysical scheme was implemented into the Goddard Cumulus Ensemble (GCE) model. Atmospheric aerosols are also described using number density size-distribution functions. A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep tropical clouds in the west Pacific warm pool region and summertime convection over a mid-latitude continent with different concentrations of CCN: a low "clean" concentration and a high "dirty" concentration. The impact of atmospheric aerosol concentration on cloud and precipitation will be investigated. 2. MODEL DESCRIPTION AND CASE STUDIES 2.1 GCE MODEL The model used in this study is the 2D version of the GCE model. Modeled flow is anelastic. Second- or higher-order advection schemes can produce negative values in the solution. Thus, a Multi-dimensional Positive Definite Advection Transport Algorithm (MPDATA) has been implemented into the model. All scalar variables (potential temperature, water vapor, turbulent coefficient and all five hydrometeor classes) use forward time differencing and the MPDATA for advection. Dynamic variables, u, v and w, use a second-order accurate advection scheme and a leapfrog time integration (kinetic energy semi-conserving method). Short-wave (solar) and long-wave radiation as well as a subgrid-scale TKE turbulence scheme are also included in the model. Details of the model can be found in Tao and Simpson (1993) and Tao et al. (2003). 2.2 Microphysics (Bin Model) The formulation of the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (cloud droplets and raindrops), and six types of ice particles: pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail. Each type is described by a special size distribution function containing 33 categories (bins). Atmospheric aerosols are also described using number density size-distribution functions (containing 33 bins). Droplet nucleation (activation) is derived from the analytical calculation of super-saturation, which is used to determine the sizes of aerosol particles to be activated and the corresponding sizes of nucleated droplets. Primary nucleation of each type of ice crystal takes place within certain temperature ranges. A detailed description of these explicitly parameterized processes can be found in Khain and Sednev (1996) and Khain et al. (1999, 2001). 2.3 Case Studies Three cases, a tropical oceanic squall system observed during TOGA COARE (Tropical Ocean and Global Atmosphere Coupled Ocean-Atmosphere Response Experiment, which occurred over the Pacific Ocean warm pool from November 1992 to February 1993), a midlatitude continental squall system observed during PRESTORM (Preliminary Regional Experiment for STORM-Central, which occurred in Kansas and Oklahoma during May-June 1985), and mid-afternoon convection observed during CRYSTAL-FACE (Cirrus Regional Study of Tropical Anvils and Cirrus Layers – Florida Area Cumulus Experiment, which occurred in Florida during July 2002), will be used to examine the impact of aerosols on deep, precipitating systems. 3. SUMMARY of RESULTS • For all three cases, higher CCN produces smaller cloud droplets and a narrower spectrum. Dirty conditions delay rain formation, increase latent heat release above the freezing level, and enhance vertical velocities at higher altitude for all cases. Stronger updrafts, deeper mixed-phase regions, and more ice particles are simulated with higher CCN in good agreement with observations. • In all cases, rain reaches the ground early with lower CCN. Rain suppression is also evident in all three cases with high CCN in good agreement with observations (Rosenfeld, 1999, 2000 and others). Rain suppression, however, only occurs during the first hour of simulation. This result suggests that microphysical processes dominate the impact of aerosols on precipitation in the early stage of precipitation development. • During the mature stage of the simulations, the effect of increasing aerosol concentration ranges from rain suppression in the PRESTORM case to little effect on surface rainfall in the CRYSTAL-FACE case to rain enhancement in the TOGA COARE case. • The model results suggest that evaporative cooling is a key process in determining whether higher CCN reduces or enhances precipitation. Cold pool strength can be enhanced by stronger evaporation. When cold pool interacts with the near surface wind shear, the low-level convergence can be stronger, facilitating secondary cloud formation and more vigorous precipitation processes. Evaporative cooling is more than two times stronger at low levels with higher CCN for the TOGA COARE case during the early stages of precipitation development. However, evaporative cooling is slightly stronger at lower levels with lower CCN for the PRESTORM case. The early formation of rain in the clean environment could allow for the formation of an earlier and stronger cold pool compared to a dirty environment. PRESTORM has a very dry environment and both large and small rain droplets can evaporate. Consequently, the cold pool is relatively weaker, and the system is relatively less intense with higher CCN. • Sensitivity tests are conducted to determine the impact of ice processes on aerosol-precipitation interaction. The results suggested that ice processes are crucial for suppressing precipitation due to high CCN for the PRESTORM case. More and smaller ice particles are generated in the dirty case and transported to the trailing stratiform region. This reduces the heavy convective rain and contributes to the weakening of the cold pool. Warm rain processes dominate the TOGA COARE case. Therefore, ice processes only play a secondary role in terms of aerosol-precipitation interaction. • Two of the three cloud systems presented in this paper formed a line structure (squall system). A 2D simulation, therefore, gives a good approximation to such a line of convective clouds. Since the real atmosphere is 3D, further 3D cloud-resolving simulations are needed to address aerosol-precipitation interactions. 4. REFERENCES Tao, W.-K., X. Li, A. Khain, T. Matsui, S. Lang, and J. Simpson, 2007: The role of atmospheric aerosol concentration on deep convective precipitation: Cloud-resolving model simulations. J. Geophy. Res., 112, D24S18, doi:10.1029/2007JD008728. All other references can be found in above paper. 5. Acknowledgements The GCE model is mainly supported by the NASA Headquarters Atmospheric Dynamics and Thermodynamics Program and the NASA Tropical Rainfall Measuring Mission (TRMM). The research was also supported by the Office of Science (BER), U. S. Department of Energy/Atmospheric Radiation Measurement (DOE/ARM) Interagency. The authors acknowledge NASA Goddard Space Flight Center for computer time used in this research.

  11. The Radiative Role of Free Tropospheric Aerosols and Marine Clouds over the Central North Atlantic

    SciTech Connect (OSTI)

    Mazzoleni, Claudio; Kumar, Sumit; Wright, Kendra; Kramer, Louisa; Mazzoleni, Lynn; Owen, Robert; Helmig, Detlev

    2014-12-09

    The scientific scope of the project was to exploit the unique location of the Pico Mountain Observatory (PMO) located in the summit caldera of the Pico Volcano in Pico Island in the Azores, for atmospheric studies. The observatory, located at 2225m a.s.l., typically samples free tropospheric aerosols laying above the marine low-level clouds and long-range transported from North America. The broad purpose of this research was to provide the scientific community with a better understanding of fundamental physical processes governing the effects of aerosols on radiative forcing and climate; with the ultimate goal of improving our abilities to understand past climate and to predict future changes through numerical models. The project was 'exploratory' in nature, with the plan to demonstrate the feasibility of deploying for the first time, an extensive aerosol research package at PMO. One of the primary activities was to test the deployment of these instruments at the site, to collect data during the 2012 summer season, and to further develop the infrastructure and the knowledge for performing novel research at PMO in follow-up longer-term aerosol-cloud studies. In the future, PMO could provide an elevated research outpost to support the renewed DOE effort in the Azores that was intensified in 2013 with the opening of the new sea-level ARM-DOE Eastern North Atlantic permanent facility at Graciosa Island. During the project period, extensive new data sets were collected for the planned 2012 season. Thanks to other synergistic activities and opportunities, data collection was then successfully extended to 2013 and 2014. Highlights of the scientific findings during this project include: a) biomass burning contribute significantly to the aerosol loading in the North Atlantic free troposphere; however, long-range transported black carbon concentrations decreased substantially in the last decade. b) Single black carbon particles analyzed off-line at the electron microscope were often very compacted, suggesting cloud processing and exhibiting different optical properties from fresh emissions. In addition, black carbon was found to be sometimes mixed with mineral dust, affecting its optical properties and potential forcing. c) Some aerosols collected at PMO acted as ice nuclei, potentially contributing to cirrus cloud formation during their transport in the upper free troposphere. Identified good ice nuclei were often mineral dust particles. d) The free tropospheric aerosols studied at PMO have relevance to low level marine clouds due, for example, to synoptic subsidence entraining free tropospheric aerosols into the marine boundary layer. This has potentially large consequences on cloud condensation nuclei concentrations and compositions in the marine boundary layer; therefore, having an effect on the marine stratus clouds, with potentially important repercussions on the radiative forcing. The scientific products of this project currently include contributions to two papers published in the Nature Publishing group (Nature Communications and Scientific Reports), one paper under revision for Atmospheric Chemistry and Physics, one in review in Geophysical Research Letters and one recently submitted to Atmospheric Chemistry and Physics Discussion. In addition, four manuscripts are in advanced state of preparation. Finally, twenty-eight presentations were given at international conferences, workshops and seminars.

  12. Highly stable aerosol generator

    DOE Patents [OSTI]

    DeFord, Henry S. (Kennewick, WA); Clark, Mark L. (Kennewick, WA)

    1981-01-01

    An improved compressed air nebulizer has been developed such that a uniform aerosol particle size and concentration may be produced over long time periods. This result is achieved by applying a vacuum pressure to the makeup assembly and by use of a vent tube between the atmosphere and the makeup solution. By applying appropriate vacuum pressures to the makeup solution container and by proper positioning of the vent tube, a constant level of aspirating solution may be maintained within the aspirating assembly with aspirating solution continuously replaced from the makeup solution supply. This device may also be adapted to have a plurality of aerosol generators and only one central makeup assembly.

  13. Highly stable aerosol generator

    DOE Patents [OSTI]

    DeFord, H.S.; Clark, M.L.

    1981-11-03

    An improved compressed air nebulizer has been developed such that a uniform aerosol particle size and concentration may be produced over long time periods. This result is achieved by applying a vacuum pressure to the makeup assembly and by use of a vent tube between the atmosphere and the makeup solution. By applying appropriate vacuum pressures to the makeup solution container and by proper positioning of the vent tube, a constant level of aspirating solution may be maintained within the aspirating assembly with aspirating solution continuously replaced from the makeup solution supply. This device may also be adapted to have a plurality of aerosol generators and only one central makeup assembly. 2 figs.

  14. Implementing marine organic aerosols into the GEOS-Chem model

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Gantt, B.; Johnson, M. S.; Crippa, M.; Prévôt, A. S. H.; Meskhidze, N.

    2015-03-17

    Marine-sourced organic aerosols (MOAs) have been shown to play an important role in tropospheric chemistry by impacting surface mass, cloud condensation nuclei, and ice nuclei concentrations over remote marine and coastal regions. In this work, an online marine primary organic aerosol emission parameterization, designed to be used for both global and regional models, was implemented into the GEOS-Chem (Global Earth Observing System Chemistry) model. The implemented emission scheme improved the large underprediction of organic aerosol concentrations in clean marine regions (normalized mean bias decreases from -79% when using the default settings to -12% when marine organic aerosols are added). Modelmore » predictions were also in good agreement (correlation coefficient of 0.62 and normalized mean bias of -36%) with hourly surface concentrations of MOAs observed during the summertime at an inland site near Paris, France. Our study shows that MOAs have weaker coastal-to-inland concentration gradients than sea-salt aerosols, leading to several inland European cities having >10% of their surface submicron organic aerosol mass concentration with a marine source. The addition of MOA tracers to GEOS-Chem enabled us to identify the regions with large contributions of freshly emitted or aged aerosol having distinct physicochemical properties, potentially indicating optimal locations for future field studies.« less

  15. Implementing marine organic aerosols into the GEOS-Chem model

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Gantt, B.; Johnson, M. S.; Crippa, M.; Prévôt, A. S. H.; Meskhidze, N.

    2014-09-09

    Marine organic aerosols (MOA) have been shown to play an important role in tropospheric chemistry by impacting surface mass, cloud condensation nuclei, and ice nuclei concentrations over remote marine and coastal regions. In this work, an online marine primary organic aerosol emission parameterization, designed to be used for both global and regional models, was implemented into the GEOS-Chem model. The implemented emission scheme improved the large underprediction of organic aerosol concentrations in clean marine regions (normalized mean bias decreases from -79% when using the default settings to -12% when marine organic aerosols are added). Model predictions were also in goodmore » agreement (correlation coefficient of 0.62 and normalized mean bias of -36%) with hourly surface concentrations of MOA observed during the summertime at an inland site near Paris, France. Our study shows that MOA have weaker coastal-to-inland concentration gradients than sea-salt aerosols, leading to several inland European cities having > 10% of their surface submicron organic aerosol mass concentration with a marine source. The addition of MOA tracers to GEOS-Chem enabled us to identify the regions with large contributions of freshly-emitted or aged aerosol having distinct physicochemical properties, potentially indicating optimal locations for future field studies.« less

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Predicting Arctic Sea Ice Loss Download a printable PDF Submitter: Liu, X., University of Wyoming Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Liu X, S Xie, J Boyle, SA Klein, X Shi, Z Wang, W Lin, SJ Ghan, M Earle, PS Liu, and A Zelenyuk. 2011. "Testing cloud microphysics parameterizations in NCAR CAM5 with ISDAC and M-PACE observations." Journal of Geophysical Research, 116, D00T11,

  17. Laboratory Experiments and Instrument Intercomparison Studies of Carbonaceous Aerosol Particles

    SciTech Connect (OSTI)

    Davidovits, Paul

    2015-10-20

    Aerosols containing black carbon (and some specific types of organic particulate matter) directly absorb incoming light, heating the atmosphere. In addition, all aerosol particles backscatter solar light, leading to a net-cooling effect. Indirect effects involve hydrophilic aerosols, which serve as cloud condensation nuclei (CCN) that affect cloud cover and cloud stability, impacting both atmospheric radiation balance and precipitation patterns. At night, all clouds produce local warming, but overall clouds exert a net-cooling effect on the Earth. The effect of aerosol radiative forcing on climate may be as large as that of the greenhouse gases, but predominantly opposite in sign and much more uncertain. The uncertainties in the representation of aerosol interactions in climate models makes it problematic to use model projections to guide energy policy. The objective of our program is to reduce the uncertainties in the aerosol radiative forcing in the two areas highlighted in the ASR Science and Program Plan. That is, (1) addressing the direct effect by correlating particle chemistry and morphology with particle optical properties (i.e. absorption, scattering, extinction), and (2) addressing the indirect effect by correlating particle hygroscopicity and CCN activity with particle size, chemistry, and morphology. In this connection we are systematically studying particle formation, oxidation, and the effects of particle coating. The work is specifically focused on carbonaceous particles where the uncertainties in the climate relevant properties are the highest. The ongoing work consists of laboratory experiments and related instrument inter-comparison studies both coordinated with field and modeling studies, with the aim of providing reliable data to represent aerosol processes in climate models. The work is performed in the aerosol laboratory at Boston College. At the center of our laboratory setup are two main sources for the production of aerosol particles: (a) two well-characterized source of soot particles and (b) a flow reactor for controlled OH and/or O3 oxidation of relevant gas phase species to produce well-characterized SOA particles. After formation, the aerosol particles are subjected to physical and chemical processes that simulate aerosol growth and aging. A suite of instruments in our laboratory is used to characterize the physical and chemical properties of aerosol particles before and after processing. The Time of Flight Aerosol Mass Spectrometer (ToF-AMS) together with a Scanning Mobility Particle Sizer (SMPS) measures particle mass, volume, density, composition (including black carbon content), dynamic shape factor, and fractal dimension. The–ToF-AMS was developed at ARI with Boston College participation. About 120 AMS instruments are now in service (including 5 built for DOE laboratories) performing field and laboratory studies world-wide. Other major instruments include a thermal denuder, two Differential Mobility Analyzers (DMA), a Cloud Condensation Nuclei Counter (CCN), a Thermal desorption Aerosol GC/MS (TAG) and the new Soot Particle Aerosol Mass Spectrometer (SP-AMS). Optical instrumentation required for the studies have been brought to our laboratory as part of ongoing and planned collaborative projects with colleagues from DOE, NOAA and university laboratories. Optical instruments that will be utilized include a Photoacoustic Spectrometer (PAS), a Cavity Ring Down Aerosol Extinction Spectrometer (CRD-AES), a Photo Thermal Interferometer (PTI), a new 7-wavelength Aethalometer and a Cavity Attenuated Phase Shift Extinction Monitor (CAPS). These instruments are providing aerosol absorption, extinction and scattering coefficients at a range of atmospherically relevant wavelengths. During the past two years our work has continued along the lines of our original proposal. We report on 12 completed and/or continuing projects conducted during the period 08/14 to 0814/2015. These projects are described in 17 manuscripts published in refereed journals.

  18. Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Feng, Y.; Kotamarthi, V. R.; Coulter, R.; Zhao, C.; Cadeddu, M.

    2015-06-19

    Aerosol radiative effects and thermodynamic responses over South Asia are examined with a version of the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of Aerosol Optical Depth (AOD) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in the northern India. The WRF-Chem model is found to underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model low-bias is due to aerosol extinctions below ~2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AODmore » and extinction profiles averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7 K day−1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond differently between Case I and Case II underlying the importance of determining the exact portion of scattering or absorbing aerosols that lead to the underestimation of aerosol optical depth in the model. In addition, the model results suggest that both direct radiative effect and rapid thermodynamic responses need to be quantified for understanding aerosol radiative impacts.« less

  19. Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Feng, Y.; Kotamarthi, V. R.; Coulter, R.; Zhao, C.; Cadeddu, M.

    2015-06-19

    Aerosol radiative effects and thermodynamic responses over South Asia are examined with a version of the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of Aerosol Optical Depth (AOD) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in the northern India. The WRF-Chem model is found to underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model low-bias is due to aerosol extinctions below ~2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AODmoreand extinction profiles averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7 K day?1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond differently between Case I and Case II underlying the importance of determining the exact portion of scattering or absorbing aerosols that lead to the underestimation of aerosol optical depth in the model. In addition, the model results suggest that both direct radiative effect and rapid thermodynamic responses need to be quantified for understanding aerosol radiative impacts.less

  20. Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

    SciTech Connect (OSTI)

    Feng, Y.; Kotamarthi, V. R.; Coulter, R.; Zhao, C.; Cadeddu, M.

    2015-06-19

    Aerosol radiative effects and thermodynamic responses over South Asia are examined with a version of the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of Aerosol Optical Depth (AOD) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in the northern India. The WRF-Chem model is found to underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model low-bias is due to aerosol extinctions below ~2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AOD and extinction profiles averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7 K day?1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond differently between Case I and Case II underlying the importance of determining the exact portion of scattering or absorbing aerosols that lead to the underestimation of aerosol optical depth in the model. In addition, the model results suggest that both direct radiative effect and rapid thermodynamic responses need to be quantified for understanding aerosol radiative impacts.

  1. Carbonaceous Aerosols and Radiative Effects Study (CARES), g1-aircraft, sedlacek sp2

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Sedlacek, Art

    The primary objective of the Carbonaceous Aerosol and Radiative Effects Study (CARES) in 2010 was to investigate the evolution of carbonaceous aerosols of different types and their optical and hygroscopic properties in central California, with a focus on the Sacramento urban plume.

  2. Carbonaceous Aerosols and Radiative Effects Study (CARES), g1-aircraft, sedlacek sp2

    SciTech Connect (OSTI)

    Sedlacek, Art

    2011-08-30

    The primary objective of the Carbonaceous Aerosol and Radiative Effects Study (CARES) in 2010 was to investigate the evolution of carbonaceous aerosols of different types and their optical and hygroscopic properties in central California, with a focus on the Sacramento urban plume.

  3. Cantera Aerosol Dynamics Simulator

    Energy Science and Technology Software Center (OSTI)

    2004-09-01

    The Cantera Aerosol Dynamics Simulator (CADS) package is a general library for aerosol modeling to address aerosol general dynamics, including formation from gas phase reactions, surface chemistry (growth and oxidation), bulk particle chemistry, transport by Brownian diffusion, thermophoresis, and diffusiophoresis with linkage to DSMC studies, and thermal radiative transport. The library is based upon Cantera, a C++ Cal Tech code that handles gas phase species transport, reaction, and thermodynamics. The method uses a discontinuous galerkinmore » formulation for the condensation and coagulation operator that conserves particles, elements, and enthalpy up to round-off error. Both O-D and 1-D time dependent applications have been developed with the library. Multiple species in the solid phase are handled as well. The O-D application, called Tdcads (Time Dependent CADS) is distributed with the library. Tdcads can address both constant volume and constant pressure adiabatic homogeneous problems. An extensive set of sample problems for Tdcads is also provided.« less

  4. ARM - Measurement - Aerosol optical depth

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    depth ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol optical depth A measure of how much light aerosols prevent from passing through a column of atmosphere. Categories Aerosols Instruments The above measurement is considered scientifically relevant for the following instruments. Refer to the datastream (netcdf) file headers of each instrument for a list of all available measurements, including

  5. Research

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Research Research Isotopes produced at Los Alamos National Laboratory are saving lives, advancing cutting-edge research and keeping the U.S. safe. Research thorium test foil A thorium test foil target for proof-of-concept actinium-225 production In addition to our routine isotope products, the LANL Isotope Program is focused on developing the next suite of isotopes and services to meet the Nation's emerging needs. The LANL Isotope Program's R&D strategy is focused on four main areas (see

  6. ARM - Surface Aerosol Observing System

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    2009-2010 Shouxian, China, 2008 Black Forest, Germany, 2007 Niamey, Niger, 2006 Point Reyes, California, 2005 Surface Aerosol Observing System The ARM Mobile Facility (AMF) is...

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Two Faces of Aerosols Download a printable PDF Submitter: Ovink, J., Pacific Northwest National Laboratory Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle Journal Reference: Berg LK, M Shrivastava, RC Easter, JD Fast, EG Chapman, Y Liu, and RA Ferrare. 2015. "A New WRF-Chem Treatment for Studying Regional Scale Impacts of Cloud Processes on Aerosol and Trace Gases in Parameterized Cumuli." Geoscientific Model Development, 8, doi:10.5194/gmd-8-409-2015. A new

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    An Update on Unmanned Platforms at Oliktok Point Download a printable PDF Submitter: de Boer, G., University of Colorado, Boulder/CIRES Area of Research: Atmospheric Thermodynamics and Vertical Structures Working Group(s): Aerosol Life Cycle, Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: de Boer G, MD Ivey, B Schmid, S McFarlane, and R Petty. 2016. "Unmanned platforms monitor the Arctic atmosphere." EOS, 97, doi:10.1029/2016EO046441. Figure 1: Gijs de

  9. Laboratory Experiments and Instrument Development for the Study of Atmospheric Aerosols

    SciTech Connect (OSTI)

    Davidovits, Paul

    2011-12-10

    Soot particles are generated by incomplete combustion of fossil and biomass fuels. Through direct effects clear air aerosols containing black carbon (BC) such as soot aerosols, absorb incoming light heating the atmosphere, while most other aerosols scatter light and produce cooling. Even though BC represents only 1-2% of the total annual emissions of particulate mass to the atmosphere, it has been estimated that the direct radiative effect of BC is the second-most important contributor to global warming after absorption by CO2. Ongoing studies continue to underscore the climate forcing importance of black carbon. However, estimates of the radiative effects of black carbon on climate remain highly uncertain due to the complexity of particles containing black carbon. Quantitative measurement of BC is challenging because BC often occurs in highly non-spherical soot particles of complex morphology. Freshly emitted soot particles are typically fractal hydrophobic aggregates. The aggregates consist of black carbon spherules with diameters typically in the range of about 15-40 nm, and they are usually coated by adsorbed polyaromatic hydrocarbons (PAHs) produced during combustion. Diesel-generated soot particles are often emitted with an organic coating composed primarily of lubricating oil and unburned fuel, as well as well as PAH compounds. Sulfuric acid has also been detected in diesel and aircraft-emitted soot particles. In the course of aging, these particle coatings may be substantially altered by chemical reactions and/or the deposition of other materials. Such processes transform the optical and CCN properties of the soot aerosols in ways that are not yet well understood. Our work over the past seven years consisted of laboratory research, instrument development and characterization, and field studies with the central focus of improving our understanding of the black carbon aerosol climate impacts. During the sixth year as well as during this seventh year (no-cost extension period) of our grant, we extended our studies to perform experiments on the controlled production and characterization of secondary organic aerosol.

  10. ARM: 10-minute TEMPORARY Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Sivaraman, Chitra; Flynn, Connor

    2010-12-15

    10-minute TEMPORARY Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  11. ARM: 10-minute TEMPORARY Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Sivaraman, Chitra; Flynn, Connor

    10-minute TEMPORARY Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  12. Atmospheric Science Program Cumulus Humilis Aerosol Processing...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    aerosols - within and around them. Aerosols - particularly those associated with human activity - are thought to be changing the brightness, the lifetime, the amount of...

  13. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion...

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    aerosol, allowing carefully controlled and reproducible conditions. Benchmarking with humidified ammonium sulfate aerosol indicated that the optical measurements...

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    atmospheric emitted radiance interferometer (AERI) during the United Arab Emirates Unified Aerosol Experiment for detectingretrieving dust aerosols. The objectives of...

  16. Environmental research program: FY 1987, annual report

    SciTech Connect (OSTI)

    Not Available

    1988-03-01

    This multidisciplinary research program includes fundamental and applied research in physics, chemistry, engineering, and biology, as well as research on the development of advanced methods of measurement and analysis. The Program's Annual Report contains summaries of research performed during FY 1987 in the areas of atmospheric aerosols, flue gas chemistry, combustion, membrane bioenergetics, and analytical chemistry. The main research interests of the Atmospheric Aerosol Research group concern the chemical and physical processes that occur in haze, clouds, and fogs. For their studies, the group is developing novel analytical and research methods for characterizing aerosol species. Aerosol research is performed in the laboratory and in the field. Studies of smoke emissions from fires and their possible effects on climatic change, especially as related to nuclear winter, are an example of the collaboration between the Atmospheric Aerosol Research and Combustion Research Groups.

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Field Experiments to Improve the Treatment of Radiation in the Mid-to-Upper Troposphere Download a printable PDF Submitter: Turner, D. D., National Oceanic and Atmospheric Administration Mlawer, E. J., Atmospheric & Environmental Research, Inc. Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Turner DD and EJ Mlawer. 2010. "The Radiative Heating in Underexplored Bands Campaigns (RHUBC)." Bulletin of the American

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ice Heating Up Cold Clouds Download a printable PDF Submitter: Ovchinnikov, M., Pacific Northwest National Laboratory Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Ovchinnikov M, A Korolev, and J Fan. 2011. "Effects of ice number concentration on dynamics of a shallow mixed-phase stratiform cloud." Journal of Geophysical Research - Atmospheres, 116, D00T06, doi:10.1029/2011JD015888. The mighty cloud

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    First Ground-Based Spectral Observations of the Entire Infrared Band Download a printable PDF Submitter: Turner, D. D., National Oceanic and Atmospheric Administration Mlawer, E. J., Atmospheric & Environmental Research, Inc. Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle, Cloud Life Cycle Journal Reference: Turner DD, EJ Mlawer, G Bianchini, MP Cadeddu, S Crewell, JS Delamere, RO Knuteson, G Maschwitz, M Mlynzcak, S Paine, L Palchetti, and DC Tobin. 2012.

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Role of Ice Nuclei Recycling in the Maintenance of Cloud Ice in Arctic Mixed-phase Stratocumulus Download a printable PDF Submitter: Solomon, A., NOAA/ESRL/Physical Sciences Division Feingold, G., NOAA - Earth System Research Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud Life Cycle Journal Reference: Solomon A, G Feingold, and MD Shupe. 2015. "The role of ice nuclei recycling in the maintenance of cloud ice in Arctic mixed-phase

  1. FACT SHEET U.S. Department of Energy ARM Aerial Facility G-1 Research Aircraft

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Facility G-1 Research Aircraft The Gulfstream-159 (G-1) twin turboprop aircraft, owned by Battelle Memorial Institute since 1988 and operated by the Pacific Northwest National Laboratory for the U.S. Department of Energy (DOE), serves as an airborne atmospheric research laboratory for DOE and other users. The aircraft can measure a wide range of radiative, aerosol, and cloud properties, as well as collect gas-phase measurements. It is capable of taking measurements at altitudes approaching

  2. Model analysis of the anthropogenic aerosol effect on clouds over East Asia

    SciTech Connect (OSTI)

    Gao, Yi; Zhang, Meigen; Liu, Xiaohong; Zhao, Chun

    2012-01-16

    A coupled meteorology and aerosol/chemistry model WRF-Chem (Weather Research and Forecast model coupled with Chemistry) was used to conduct a pair of simulations with present-day (PD) and preindustrial (PI) emissions over East Asia to examine the aerosol indirect effect on clouds. As a result of an increase in aerosols in January, the cloud droplet number increased by 650 cm{sup -3} over the ocean and East China, 400 cm{sup -3} over Central and Southwest China, and less than 200 cm{sup -3} over North China. The cloud liquid water path (LWP) increased by 40-60 g m{sup -2} over the ocean and Southeast China and 30 g m{sup -2} over Central China; the LWP increased less than 5 g m{sup -2} or decreased by 5 g m{sup -2} over North China. The effective radius (Re) decreased by more than 4 {mu}m over Southwest, Central, and Southeast China and 2 {mu}m over North China. In July, variations in cloud properties were more uniform; the cloud droplet number increased by approximately 250-400 cm{sup -3}, the LWP increased by approximately 30-50 g m{sup -2}, and Re decreased by approximately 3 {mu}m over most regions of China. In response to cloud property changes from PI to PD, shortwave (SW) cloud radiative forcing strengthened by 30 W m{sup -2} over the ocean and 10 W m{sup -2} over Southeast China, and it weakened slightly by approximately 2-10 W m{sup -2} over Central and Southwest China in January. In July, SW cloud radiative forcing strengthened by 15 W m{sup -2} over Southeast and North China and weakened by 10 W m{sup -2} over Central China. The different responses of SW cloud radiative forcing in different regions was related to cloud feedbacks and natural variability.

  3. Carbonaceous Aerosols and Radiative Effects Study

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Carbonaceous Aerosols and Radiative Effects Study Science Objective This field campaign is designed to increase scientific knowledge about the evolution of black carbon, primary organic aerosols (POA), and secondary organic aerosols (SOA) from both man-made and biogenic sources. Black carbon and primary organic aerosols are emitted directly into the atmosphere through diesel and gasoline vehicle exhaust, as well as during meat cooking and biomass burning; secondary organic aerosols are formed

  4. ARM - Campaign Instrument - drum-aerosol

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govInstrumentsdrum-aerosol Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign Instrument : Drum Aerosol Sampler (DRUM-AEROSOL) Instrument Categories Aerosols Campaigns Aerosol IOP [ Download Data ] Southern Great Plains, 2003.05.01 - 2003.05.31 Primary Measurements Taken The following measurements are those considered scientifically relevant. Refer to the datastream (netcdf) file headers for the list of all available measurements, including

  5. AERONET: The Aerosol Robotic Network

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    AERONET collaboration provides globally distributed observations of spectral aerosol optical Depth (AOD), inversion products, and precipitable water in diverse aerosol regimes. Aerosol optical depth data are computed for three data quality levels: Level 1.0 (unscreened), Level 1.5 (cloud-screened), and Level 2.0 (cloud screened and quality-assured). Inversions, precipitable water, and other AOD-dependent products are derived from these levels and may implement additional quality checks.[Copied from http://aeronet.gsfc.nasa.gov/new_web/system_descriptions.html

  6. Development of Aerosol Models for Radiative Flux Calculations at ARM Sites

    SciTech Connect (OSTI)

    Ogren, John A.; Dutton, Ellsworth G.; McComiskey, Allison C.

    2006-09-30

    The direct radiative forcing (DRF) of aerosols, the change in net radiative flux due to aerosols in non-cloudy conditions, is an essential quantity for understanding the human impact on climate change. Our work has addressed several key issues that determine the accuracy, and identify the uncertainty, with which aerosol DRF can be modeled. These issues include the accuracy of several radiative transfer models when compared to measurements and to each other in a highly controlled closure study using data from the ARM 2003 Aerosol IOP. The primary focus of our work has been to determine an accurate approach to assigning aerosol properties appropriate for modeling over averaged periods of time and space that represent the observed regional variability of these properties. We have also undertaken a comprehensive analysis of the aerosol properties that contribute most to uncertainty in modeling aerosol DRF, and under what conditions they contribute the most uncertainty. Quantification of these issues enables the community to better state accuracies of radiative forcing calculations and to concentrate efforts in areas that will decrease uncertainties in these calculations in the future.

  7. Stratospheric aerosol geoengineering

    SciTech Connect (OSTI)

    Robock, Alan

    2015-03-30

    The Geoengineering Model Intercomparison Project, conducting climate model experiments with standard stratospheric aerosol injection scenarios, has found that insolation reduction could keep the global average temperature constant, but global average precipitation would reduce, particularly in summer monsoon regions around the world. Temperature changes would also not be uniform; the tropics would cool, but high latitudes would warm, with continuing, but reduced sea ice and ice sheet melting. Temperature extremes would still increase, but not as much as without geoengineering. If geoengineering were halted all at once, there would be rapid temperature and precipitation increases at 510 times the rates from gradual global warming. The prospect of geoengineering working may reduce the current drive toward reducing greenhouse gas emissions, and there are concerns about commercial or military control. Because geoengineering cannot safely address climate change, global efforts to reduce greenhouse gas emissions and to adapt are crucial to address anthropogenic global warming.

  8. Fuels for Advanced Combustion Engines Research Diesel Fuels: Analysis of Physical and Chemical Properties

    SciTech Connect (OSTI)

    Gallant, Tom; Franz, Jim; Alnajjar, Mikhail; Storey, John Morse; Lewis Sr, Samuel Arthur; Sluder, Scott; Cannella, William C; Fairbridge, Craig; Hager, Darcy; Dettman, Heather; Luecke, Jon; Ratcliff, Matthew A.; Zigler, Brad

    2009-01-01

    The CRC Fuels for Advanced Combustion Engines working group has worked to identify a matrix of research diesel fuels for use in advanced combustion research applications. Nine fuels were specified and formulated to investigate the effects of cetane number aromatic content and 90% distillation fraction. Standard ASTM analyses were performed on the fuels as well as GC/MS and /u1H//u1/u3C NMR analyses and thermodynamic characterizations. Details of the actual results of the fuel formulations compared with the design values are presented, as well as results from standard analyses, such as heating value, viscosity and density. Cetane number characterizations were accomplished by using both the engine method and the Ignition Quality Tester (IQT/sT) apparatus.

  9. Property

    Energy Savers [EERE]

    ER-B-98-07 AUDIT REPORT PERSONAL PROPERTY AT THE OAK RIDGE OPERATIONS OFFICE AND THE OFFICE OF SCIENTIFIC AND TECHNICAL INFORMATION U.S. DEPARTMENT OF ENERGY OFFICE OF INSPECTOR GENERAL OFFICE OF AUDIT SERVICES APRIL 1998 Page 10 DEPARTMENT OF ENERGY Washington, DC 20585 April 6, 1998 MEMORANDUM FOR THE MANAGER, OAK RIDGE OPERATIONS OFFICE AND THE DIRECTOR, OFFICE OF SCIENTIFIC AND TECHNICAL INFORMATION FROM: Terry L. Brendlinger Eastern Regional Audit Office Office of Inspector General SUBJECT:

  10. ARM Aerosol Working Group Meeting

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Report ARM STM 2008 Norfolk, VA Connor Flynn for B Schmid and AWG Members AWG Instruments * Raman Lidar - SGP * Micropulse Lidars - all sites * Aerosol Sampling - SGP, NSA, AMF - scattering, absorption, number, size distribution, hygroscopicity, CCN, composition (major ions). * In situ Aerosol Profile (Cessna) - scattering, absorption, number, hygroscopicity, * Radiometers: - MFRSR, NIMFR, RSS, Cimel, AERI, SWS AWG-related Field Campaigns * Recent Past: - MASRAD (Marine Stratus Radiation,

  11. Final Project Report - ARM CLASIC CIRPAS Twin Otter Aerosol

    SciTech Connect (OSTI)

    John A. Ogren

    2010-04-05

    The NOAA/ESRL/GMD aerosol group made three types of contributions related to airborne measurements of aerosol light scattering and absorption for the Cloud and Land Surface Interaction Campaign (CLASIC) in June 2007 on the Twin Otter research airplane operated by the Center for Interdisciplinary Remotely-Piloted Aircraft Studies (CIRPAS). GMD scientists served as the instrument mentor for the integrating nephelometer and particle soot absorption photometer (PSAP) on the Twin Otter during CLASIC, and were responsible for (1) instrument checks/comparisons; (2) instrument trouble shooting/repair; and (3) data quality control (QC) and submittal to the archive.

  12. BAECC Biogenic Aerosols - Effects on Clouds and Climate

    SciTech Connect (OSTI)

    Petäjä, Tuukka; Moisseev, Dmitri; Sinclair, Victoria; O'Connor, Ewan J.; Manninen, Antti J.; Levula, Janne; Väänänen, Riikka; Heikkinen, Liine; Äijälä, Mikko; Aalto, Juho; Bäck, Jaana

    2015-11-01

    “Biogenic Aerosols - Effects on Clouds and Climate (BAECC)”, featured the U.S. Department of Energy’s Atmospheric Radiation Measurement (ARM) Program’s 2nd Mobile Facility (AMF2) in Hyytiälä, Finland. It operated for an 8-month intensive measurement campaign from February to September 2014. The main research goal was to understand the role of biogenic aerosols in cloud formation. One of the reasons to perform BAECC study in Hyytiälä was the fact that it hosts SMEAR-II (Station for Measuring Forest Ecosystem-Atmosphere Relations), which is one of the world’s most comprehensive surface in-situ observation sites in a boreal forest environment. The station has been measuring atmospheric aerosols, biogenic emissions and an extensive suite of parameters relevant to atmosphere-biosphere interactions continuously since 1996. The BAECC enables combining vertical profiles from AMF2 with surface-based in-situ SMEAR-II observations and allows the processes at the surface to be directly related to processes occurring throughout the entire tropospheric column. With the inclusion of extensive surface precipitation measurements, and intensive observation periods involving aircraft flights and novel radiosonde launches, the complementary observations of AMF2 and SMEAR-II provide a unique opportunity for investigating aerosol-cloud interactions, and cloud-to-precipitation processes. The BAECC dataset will initiate new opportunities for evaluating and improving models of aerosol sources and transport, cloud microphysical processes, and boundary-layer structures.

  13. Aerosols and Clouds: In Cahoots to Change Climate

    SciTech Connect (OSTI)

    Berg, Larry

    2014-03-29

    Key knowledge gaps persist despite advances in the scientific understanding of how aerosols and clouds evolve and affect climate. The Two-Column Aerosol Project, or TCAP, was designed to provide a detailed set of observations to tackle this area of unknowns. Led by PNNL atmospheric scientist Larry Berg, ARM's Climate Research Facility was deployed in Cape Cod, Massachusetts for the 12-month duration of TCAP, which came to a close in June 2013. "We are developing new tools to look at particle chemistry, like our mass spectrometer used in TCAP that can tell us the individual chemical composition of an aerosol," said Berg. "Then, we'll run our models and compare it with the data that we have to make sure we're getting correct answers and make sure our climate models are reflecting the best information."

  14. Aerosols and Clouds: In Cahoots to Change Climate

    ScienceCinema (OSTI)

    Berg, Larry

    2014-06-02

    Key knowledge gaps persist despite advances in the scientific understanding of how aerosols and clouds evolve and affect climate. The Two-Column Aerosol Project, or TCAP, was designed to provide a detailed set of observations to tackle this area of unknowns. Led by PNNL atmospheric scientist Larry Berg, ARM's Climate Research Facility was deployed in Cape Cod, Massachusetts for the 12-month duration of TCAP, which came to a close in June 2013. "We are developing new tools to look at particle chemistry, like our mass spectrometer used in TCAP that can tell us the individual chemical composition of an aerosol," said Berg. "Then, we'll run our models and compare it with the data that we have to make sure we're getting correct answers and make sure our climate models are reflecting the best information."

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Optical Depth Measurements by Shadowband Radiometers and Their Uncertainties Download a printable PDF Submitter: Alexandrov, M. D., Columbia University Area of Research: Radiation Processes Working Group(s): Aerosol Journal Reference: Applied Optics, accepted Sept. 2007. Effective offset to measured optical depths due to tilt of 1-degree in different directions. Offset observed in C1 MFRSR AOD relative to Cimel and representative offset due to tilt. Appearance of shading failure and effect on

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Cloud Susceptibility Measures Potential Cloud Sensitivity to First Aerosol Indirect Effect Download a printable PDF Submitter: Oreopoulos, L., NASA Platnick, S., NASA - Goddard Space Flight Center Area of Research: Cloud Distributions/Characterizations Working Group(s): Radiative Processes Journal Reference: Platnick, S, and L Oreopoulos. 2008. "Radiative susceptibility of cloudy atmospheres to droplet number perturbations: 1. Theoretical analysis and examples from MODIS." Journal of

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Estimating the Ice Crystal Enhancement Factor in the Tropics Download a printable PDF Submitter: Zeng, X., Morgan State University GSFC, N., NASA GSFC Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Zeng X, W Tao, T Matsui, S Xie, S Lang, M Zhang, DO Starr, and X Li. 2011. "Estimating the ice crystal enhancement factor in the tropics." Journal of the

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Understanding Ice Formation in Arctic Mixed-Phase Boundary-Layer Clouds During ISDAC Download a printable PDF Submitter: Ackerman, A., NASA - Goddard Institute for Space Studies Fridlind, A. M., NASA - Goddard Institute for Space Studies Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Avramov A, AS Ackerman, AM Fridlind, B van Diedenhoven, G Botta, K Aydin, J Verlinde, KV Alexei, W Strapp, GM McFarquhar, R

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Trends in Downwelling Longwave Radiation over SGP Download a printable PDF Submitter: Gero, J., University of Wisconsin Turner, D. D., National Oceanic and Atmospheric Administration Area of Research: Radiation Processes Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Gero P and DD Turner. 2011. "Long-term trends in downwelling spectral infrared radiance over the U.S. Southern Great Plains." Journal of Climate, 24(18),

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Spectrally Invariant Approximation Within Atmospheric Radiative Transfer Download a printable PDF Submitter: Marshak, A., NASA - Goddard Space Flight Center Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Marshak A, Y Knyazikhin, JC Chiu, and WJ Wiscombe. 2011. "Spectrally-invariant approximation within atmospheric radiative transfer." Journal of the Atmospheric Sciences, 68(12), doi:10.1175/JAS-D-11-060.1. Ratio of

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Tropical Rain Clouds Still a Challenge to Cloud-Resolving Models Download a printable PDF Submitter: Fridlind, A. M., NASA - Goddard Institute for Space Studies Ackerman, A., NASA - Goddard Institute for Space Studies Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Fridlind AM, AS Ackerman, J Chaboureau, J Fan, WW Grabowski, AA Hill, TR Jones, MM Khaiyer, G Liu, P Minnis, H Morrison, L Nguyen,

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Diurnal Cycle of Monsoon Clouds, Precipitation, and Surface Radiation Download a printable PDF Submitter: Long, C. N., NOAA Global Monitoring Division/CIRES May, P. T., Bureau of Meteorology Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: May PT, CN Long, and A Protat. 2012. "The diurnal cycle of the boundary layer, convection, clouds, and surface radiation in a coastal monsoon environment (Darwin

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    2007 Floods Not a Complete Washout in U.S. Great Plains Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Atmospheric Thermodynamics and Vertical Structures Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Lamb PJ, DH Portis, and A Zangvil. 2012. "Investigation of Large-Scale Atmospheric Moisture Budget and Land Surface Interactions over U.S. Southern Great Plains including for CLASIC (June 2007)." Journal of

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Linking Ice Nucleation to Aerosols and Its Impact on CAM5 Simulated Arctic Clouds and Radiation Download a printable PDF Submitter: Xie, S., Lawrence Livermore National Laboratory Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Cloud Life Cycle Journal Reference: Xie S, X Liu, C Zhao, and Y Zhang. 2013. "Sensitivity of CAM5 simulated arctic clouds and radiation to ice nucleation parameterization." Journal of Climate, 26(16),

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Arctic Mixed-phase Clouds Persist with Little Help from the Local Surface Download a printable PDF Submitter: Shupe, M., University of Colorado Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Shupe MD, OG Persson, IM Brooks, M Tjernstrom, J Sedlar, T Mauritsen, S Sjogren, and C Leck. 2013. "Cloud and boundary layer interactions over the Arctic sea ice in late summer." Atmospheric Chemistry and Physics,

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    A New Theory of Time-dependent Freezing and Its Application to Investigation of Formation of Hail Download a printable PDF Submitter: Khain, A., The Hebrew University of Jerusalem Phillips, V., University of Leeds Area of Research: Cloud Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Phillips VT, A Khain, N Benmoshe, E Ilotoviz, and A Ryzhkov. 2014. "Theory of time-dependent freezing. II: Scheme for freezing raindrops and simulations by a cloud model

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    On the Right Track for Tropical Clouds Download a printable PDF Submitter: Hagos, S. M., Pacific Northwest National Laboratory Area of Research: Atmospheric Thermodynamics and Vertical Structures Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Hagos SM, Z Feng, K Landu, and C Long. 2014. "Advection, moistening, and shallow-to-deep convection transitions during the initiation and propagation of Madden-Julian Oscillation." Journal of Advances in Earth System

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Satellite Inference of Thermals and Cloud Base Updraft Speeds Download a printable PDF Submitter: Zheng, Y., University of Maryland Area of Research: Vertical Velocity Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Zheng Y, D Rosenfeld, and Z Li. 2015. "Satellite inference of thermals and cloud base updraft speeds based on retrieved surface and cloud base temperatures." Journal of the Atmospheric Sciences, , . ONLINE. Validation of satellite-estimated

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Modeling Precipitating Cumulus Congestus Observed by the ARM Radar Suite During the MC3E Field Campaign Download a printable PDF Submitter: Mechem, D. B., University of Kansas Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Mechem DB, SE Giangrande, CS Wittman, P Borque, T Toto, and P Kollias. 2015. "Insights from modeling and observational evaluation of a precipitating continental cumulus event observed

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Developing and Evaluating Ice Cloud Parameterizations by Combining Radar and in Situ Observations Download a printable PDF Submitter: Maahn, M., University of Cologne Loehnert, U., University of Cologne Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Maahn M, U Löhnert, P Kollias, RC Jackson, and GM McFarquhar. 2015. "Developing and Evaluating Ice Cloud Parameterizations for Forward Modeling of Radar Moments

  11. Research on the electronic and optical properties of polymer and other organic molecular thin films

    SciTech Connect (OSTI)

    1997-02-01

    The main goal of the work is to find materials and methods of optimization of organic layered electroluminescent cells and to study such properties of polymers and other organic materials that can be used in various opto-electronic devices. The summary of results obtained during the first year of work is presented. They are: (1) the possibility to produce electroluminescent cells using a vacuum deposition photoresist technology for commercial photoresists has been demonstrated; (2) the idea to replace the polyaryl polymers by other polymers with weaker hole conductivity for optimization of electroluminescent cells with ITO-Al electrodes has been suggested. The goal is to obtain amorphous processable thin films of radiative recombination layers in electroluminescent devices; (3) procedures of preparation of high-quality vacuum-deposited poly (p-phenylene) (PPP) films on various substrates have been developed; (4) it was found for the first time that the fluorescence intensity of PPP films depends on the degree of polymerization; (5) the role of interfaces between organic compounds, on one side, and metals or semiconductors, on the other side, has been studied and quenching of the fluorescence caused by semiconductor layer in thin sandwiches has been observed; (6) studies of the dynamics of photoexcitations revealed the exciton self-trapping in quasi-one-dimensional aggregates; and (7) conditions for preparation of highly crystalline fullerene C{sub 60} films by vacuum deposition have been found. Composites of C{sub 60} with conjugated polymers have been prepared.

  12. ARM Climate Research Facility Annual Report 2005

    SciTech Connect (OSTI)

    J. Voyles

    2005-12-31

    Through the ARM Program, the DOE funded the development of several highly instrumented ground stations for studying cloud formation processes and their influence on radiative transfer, and for measuring other parameters that determine the radiative properties of the atmosphere. This scientific infrastructure, and resultant data archive, is a valuable national and international asset for advancing scientific knowledge of Earth systems. In fiscal year (FY) 2003, the DOE designated ARM sites as a national scientific user facility: the ARM Climate Research (ACRF). The ACRF has enormous potential to contribute to a wide range interdisciplinary science in areas such as meteorology, atmospheric aerosols, hydrology, biogeochemical cycling, and satellite validation, to name only a few.

  13. Simulation of aerosol direct radiative forcing with RAMS-CMAQ in East Asia

    SciTech Connect (OSTI)

    Han, Xiao; Zhang, Meigen; Han, Zhiewi; Xin, Jin-Yuan; Liu, Xiaohong

    2011-11-14

    The air quality modeling system RAMS-CMAQ is developed to assess aerosol direct radiative forcing by linking simulated meteorological parameters and aerosol mass concentration with the aerosol optical properties/radiative transfer module in this study. The module is capable of accounting for important factors that affect aerosol optical properties and radiative effect, such as incident wave length, aerosol size distribution, water uptake, and internal mixture. Subsequently, the modeling system is applied to simulate the temporal and spatial variations in mass burden, optical properties, and direct radiative forcing of diverse aerosols, including sulfate, nitrate, ammonium, black carbon, organic carbon, dust, and sea salt over East Asia throughout 2005. Model performance is fully evaluated using various observational data, including satellite monitoring of MODIS and surface measurements of EANET (Acid Deposition Monitoring Network), AERONET (Aerosol Robotic Network), and CSHNET (Chinese Sun Hazemeter Network). The correlation coefficients of the comparisons of daily average mass concentrations of sulfate, PM2.5, and PM10 between simulations and EANET measurements are 0.70, 0.61, and 0.64, respectively. It is also determined that the modeled aerosol optical depth (AOD) is in congruence with the observed results from the AERONET, the CSHNET, and the MODIS. The model results suggest that the high AOD values ranging from 0.8 to 1.2 are mainly distributed over the Sichuan Basin as well as over central and southeastern China, in East Asia. The aerosol direct radiative forcing patterns generally followed the AOD patterns. The strongest forcing effect ranging from -12 to -8 W m-2 was mainly distributed over the Sichuan Basin and the eastern China's coastal regions in the all-sky case at TOA, and the forcing effect ranging from -8 to -4 W m-2 could be found over entire eastern China, Korea, Japan, East China Sea, and the sea areas of Japan

  14. Overview of the 2010 Carbonaceous Aerosols and Radiative Effects Study (CARES)

    SciTech Connect (OSTI)

    Zaveri, Rahul A.; Shaw, William J.; Cziczo, D. J.; Schmid, Beat; Ferrare, R.; Alexander, M. L.; Alexandrov, Mikhail; Alvarez, R. J.; Arnott, W. P.; Atkinson, D.; Baidar, Sunil; Banta, Robert M.; Barnard, James C.; Beranek, Josef; Berg, Larry K.; Brechtel, Fred J.; Brewer, W. A.; Cahill, John F.; Cairns, Brian; Cappa, Christopher D.; Chand, Duli; China, Swarup; Comstock, Jennifer M.; Dubey, Manvendra K.; Easter, Richard C.; Erickson, Matthew H.; Fast, Jerome D.; Floerchinger, Cody; Flowers, B. A.; Fortner, Edward; Gaffney, Jeffrey S.; Gilles, Mary K.; Gorkowski, K.; Gustafson, William I.; Gyawali, Madhu S.; Hair, John; Hardesty, Michael; Harworth, J. W.; Herndon, Scott C.; Hiranuma, Naruki; Hostetler, Chris A.; Hubbe, John M.; Jayne, J. T.; Jeong, H.; Jobson, Bertram T.; Kassianov, Evgueni I.; Kleinman, L. I.; Kluzek, Celine D.; Knighton, B.; Kolesar, K. R.; Kuang, Chongai; Kubatova, A.; Langford, A. O.; Laskin, Alexander; Laulainen, Nels S.; Marchbanks, R. D.; Mazzoleni, Claudio; Mei, F.; Moffet, Ryan C.; Nelson, Danny A.; Obland, Michael; Oetjen, Hilke; Onasch, Timothy B.; Ortega, Ivan; Ottaviani, M.; Pekour, Mikhail S.; Prather, Kimberly A.; Radney, J. G.; Rogers, Ray; Sandberg, S. P.; Sedlacek, Art; Senff, Christoph; Senum, Gunar; Setyan, Ari; Shilling, John E.; Shrivastava, ManishKumar B.; Song, Chen; Springston, S. R.; Subramanian, R.; Suski, Kaitlyn; Tomlinson, Jason M.; Volkamer, Rainer M.; Wallace, Hoyt A.; Wang, J.; Weickmann, A. M.; Worsnop, Douglas R.; Yu, Xiao-Ying; Zelenyuk, Alla; Zhang, Qi

    2012-08-22

    Substantial uncertainties still exist in the scientific understanding of the possible interactions between urban and natural (biogenic) emissions in the production and transformation of atmospheric aerosol and the resulting impact on climate change. The U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) program's Carbonaceous Aerosol and Radiative Effects Study (CARES) carried out in June 2010 in Central Valley, California, was a comprehensive effort designed to improve this understanding. The primary objective of the field study was to investigate the evolution of secondary organic and black carbon aerosols and their climate-related properties in the Sacramento urban plume as it was routinely transported into the forested Sierra Nevada foothills area. Urban aerosols and trace gases experienced significant physical and chemical transformations as they mixed with the reactive biogenic hydrocarbons emitted from the forest. Two heavily-instrumented ground sites - one within the Sacramento urban area and another about 40 km to the northeast in the foothills area - were set up to characterize the evolution of meteorological variables, trace gases, aerosol precursors, aerosol size, composition, and climate-related properties in freshly polluted and 'aged' urban air. On selected days, the DOE G-1 aircraft was deployed to make similar measurements upwind and across the evolving Sacramento plume in the morning and again in the afternoon. The NASA B-200 aircraft, carrying remote sensing instruments, was also deployed to characterize the vertical and horizontal distribution of aerosols and aerosol optical properties within and around the plume. This overview provides: a) the scientific background and motivation for the study, b) the operational and logistical information pertinent to the execution of the study, c) an overview of key observations and initial results from the aircraft and ground-based sampling platforms, and d) a roadmap of planned data analyses and focused modeling efforts that will facilitate the integration of new knowledge into improved representations of key aerosol processes in climate models.

  15. Effects of Ocean Ecosystem on Marine Aerosol-Cloud Interaction

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Meskhidze, Nicholas; Nenes, Athanasios

    2010-01-01

    Using smore » atellite data for the surface ocean, aerosol optical depth (AOD), and cloud microphysical parameters, we show that statistically significant positive correlations exist between ocean ecosystem productivity, the abundance of submicron aerosols, and cloud microphysical properties over different parts of the remote oceans. The correlation coefficient for remotely sensed surface chlorophyll a concentration ([Chl- a ]) and liquid cloud effective radii over productive areas of the oceans varies between − 0.2 and − 0.6 . Special attention is given to identifying (and addressing) problems from correlation analysis used in the previous studies that can lead to erroneous conclusions. A new approach (using the difference between retrieved AOD and predicted sea salt aerosol optical depth, AOD diff ) is developed to explore causal links between ocean physical and biological systems and the abundance of cloud condensation nuclei (CCN) in the remote marine atmosphere. We have found that over multiple time periods, 550 nm AOD diff (sensitive to accumulation mode aerosol, which is the prime contributor to CCN) correlates well with [Chl- a ] over the productive waters of the Southern Ocean. Since [Chl- a ] can be used as a proxy of ocean biological productivity, our analysis demonstrates the role of ocean ecology in contributing CCN, thus shaping the microphysical properties of low-level marine clouds.« less

  16. The impact of biogenic carbon emissions on aerosol absorption inMexico City

    SciTech Connect (OSTI)

    Marley, N; Gaffney, J; Tackett, M J; Sturchio, N; Hearty, L; Martinez, N; Hardy, K D; Machany-Rivera, A; Guilderson, T P; MacMillan, A; Steelman, K

    2009-02-24

    In order to determine the wavelength dependence of atmospheric aerosol absorption in the Mexico City area, the absorption angstrom exponents (AAEs) were calculated from aerosol absorption measurements at seven wavelengths obtained with a seven-channel aethalometer during two field campaigns, the Mexico City Metropolitan Area study in April 2003 (MCMA 2003) and the Megacity Initiative: Local and Global Research Observations in March 2006 (MILAGRO). The AAEs varied from 0.76 to 1.56 in 2003 and from 0.54 to 1.52 in 2006. The AAE values determined in the afternoon were consistently higher than the corresponding morning values, suggesting the photochemical formation of absorbing secondary organic aerosols (SOA) in the afternoon. The AAE values were compared to stable and radiocarbon isotopic measurements of aerosol samples collected at the same time to determine the sources of the aerosol carbon. The fraction of modern carbon (fM) in the aerosol samples, as determined from {sup 14}C analysis, showed that 70% of the carbonaceous aerosols in Mexico City were from modern sources, indicating a significant impact from biomass burning during both field campaigns. The {sup 13}C/{sup 12}C ratios of the aerosol samples illustrate the significant impact of Yucatan forest fires (C-3 plants) in 2003 and local grass fires (C-4 plants) at site T1 in 2006. A direct comparison of the fM values, stable carbon isotope ratios, and calculated aerosol AAEs suggested that the wavelength dependence of the aerosol absorption was controlled by the biogenically derived aerosol components.

  17. Constraining the atmospheric composition of the day-night terminators of HD 189733b: Atmospheric retrieval with aerosols

    SciTech Connect (OSTI)

    Lee, Jae-Min; Irwin, Patrick G. J.; Fletcher, Leigh N.; Barstow, Joanna K.; Heng, Kevin

    2014-07-01

    A number of observations have shown that Rayleigh scattering by aerosols dominates the transmission spectrum of HD 189733b at wavelengths shortward of 1 ?m. In this study, we retrieve a range of aerosol distributions consistent with transmission spectroscopy between 0.3-24 ?m that were recently re-analyzed by Pont et al. To constrain the particle size and the optical depth of the aerosol layer, we investigate the degeneracies between aerosol composition, temperature, planetary radius, and molecular abundances that prevent unique solutions for transit spectroscopy. Assuming that the aerosol is composed of MgSiO{sub 3}, we suggest that a vertically uniform aerosol layer over all pressures with a monodisperse particle size smaller than about 0.1 ?m and an optical depth in the range 0.002-0.02 at 1 ?m provides statistically meaningful solutions for the day/night terminator regions of HD 189733b. Generally, we find that a uniform aerosol layer provide adequate fits to the data if the optical depth is less than 0.1 and the particle size is smaller than 0.1 ?m, irrespective of the atmospheric temperature, planetary radius, aerosol composition, and gaseous molecules. Strong constraints on the aerosol properties are provided by spectra at wavelengths shortward of 1 ?m as well as longward of 8 ?m, if the aerosol material has absorption features in this region. We show that these are the optimal wavelengths for quantifying the effects of aerosols, which may guide the design of future space observations. The present investigation indicates that the current data offer sufficient information to constrain some of the aerosol properties of HD189733b, but the chemistry in the terminator regions remains uncertain.

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Chinese Researchers Report Reliable Method for Monitoring Soil Moisture Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Surface Properties...

  19. An Observed Signature of Aerosol Effect on Cloud Droplet Radii from a

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Decade of Observations at a Mid-Continental Site An Observed Signature of Aerosol Effect on Cloud Droplet Radii from a Decade of Observations at a Mid-Continental Site Min, Qilong State University of New York at Albany Duan, Minzheng State University of New York at Albany Harrison, Lee State University of New York Joseph, Everette Howard University Category: Aerosols Continuing observations of aerosol and cloud optical property have been made using MFRSR and MWR at the ARM SGP site since

  20. Atmospheric Radiation Measurement Climate Research Facility (ACRF) Annual Report 2008

    SciTech Connect (OSTI)

    LR Roeder

    2008-12-01

    The Importance of Clouds and Radiation for Climate Change: The Earths surface temperature is determined by the balance between incoming solar radiation and thermal (or infrared) radiation emitted by the Earth back to space. Changes in atmospheric composition, including greenhouse gases, clouds, and aerosols, can alter this balance and produce significant climate change. Global climate models (GCMs) are the primary tool for quantifying future climate change; however, there remain significant uncertainties in the GCM treatment of clouds, aerosol, and their effects on the Earths energy balance. In 1989, the U.S. Department of Energy (DOE) Office of Science created the Atmospheric Radiation Measurement (ARM) Program to address scientific uncertainties related to global climate change, with a specific focus on the crucial role of clouds and their influence on the transfer of radiation in the atmosphere. To reduce these scientific uncertainties, the ARM Program uses a unique twopronged approach: The ARM Climate Research Facility, a scientific user facility for obtaining long-term measurements of radiative fluxes, cloud and aerosol properties, and related atmospheric characteristics in diverse climate regimes; and The ARM Science Program, focused on the analysis of ACRF and other data to address climate science issues associated with clouds, aerosols, and radiation, and to improve GCMs. This report provides an overview of each of these components and a sample of achievements for each in fiscal year (FY) 2008.

  1. Dispersion of Cloud Droplet Size Distributions, Cloud Parameterizations and Indirect Aerosol Effects

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Dispersion of Cloud Droplet Size Distributions, Cloud Parameterizations, and Indirect Aerosol Effects P. H. Daum and Y. Liu Brookhaven National Laboratory Upton, New York Introduction Most studies of the effect of aerosols on cloud radiative properties have considered only changes in the cloud droplet concentration, neglecting changes in the spectral shape of the cloud droplet size distribution. However, it has been shown that that the spectral dispersion of the cloud droplet size distribution

  2. Aerosol Remote Sealing System - Energy Innovation Portal

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Remote Sealing System Lawrence Berkeley National Laboratory Contact LBL About This Technology Technology Marketing SummaryMark Modera and Francois Remi Carrie from Berkeley National Laboratory have developed a rapid, economical technique to seal duct and other enclosed systems by means of an internally injected aerosol. DescriptionBerkeley National Laboratory's aerosol compound seals holes in enclosed systems and is effective even after bends and junctions. A unique, in situ aerosol

  3. ARM - PI Product - Direct Aerosol Forcing Uncertainty

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ProductsDirect Aerosol Forcing Uncertainty ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send PI Product : Direct Aerosol Forcing Uncertainty Understanding sources of uncertainty in aerosol direct radiative forcing (DRF), the difference in a given radiative flux component with and without aerosol, is essential to quantifying changes in Earth's radiation budget. We examine the uncertainty in DRF due to measurement

  4. Aerosol Oxidation Speeds Up in Smoggy Air

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Oxidation Speeds Up in Smoggy Air Aerosol Oxidation Speeds Up in Smoggy Air Print Wednesday, 17 February 2016 11:37 Organic aerosols (nanometer-sized liquid or solid particles suspended in air) are important constituents of the troposphere, and their chemistry has large-scale impacts on climate, pollution, and health. Accurate predictions of these aerosol impacts require a robust microphysical understanding of all relevant chemical reaction mechanisms and time scales, including those

  5. ARM - Measurement - Aerosol particle size distribution

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AOS : Aerosol Observing System CSPHOT : Cimel Sunphotometer HTDMA : Humidified Tandem Differential Mobility Analyzer SMPS : Scanning mobility particle sizer TDMA : Tandem...

  6. Evolution of organic aerosol mass spectra upon heating: implications for OA phase and partitioning behavior

    SciTech Connect (OSTI)

    UC Davis; Cappa, Christopher D.; Wilson, Kevin R.

    2010-10-28

    Vacuum Ultraviolet (VUV) photoionization mass spectrometry has been used to measure the evolution of chemical composition for two distinct organic aerosol types as they are passed through a thermodenuder at different temperatures. The two organic aerosol types considered are primary lubricating oil (LO) aerosol and secondary aerosol from the alpha-pinene + O3 reaction (alphaP). The evolution of the VUV mass spectra for the two aerosol types with temperature are observed to differ dramatically. For LO particles, the spectra exhibit distinct changes with temperature in which the lower m/z peaks, corresponding to compounds with higher vapor pressures, disappear more rapidly than the high m/z peaks. In contrast, the alphaP aerosol spectrum is essentially unchanged by temperature even though the particles experience significant mass loss due to evaporation. The variations in the LO spectra are found to be quantitatively in agreement with expectations from absorptive partitioning theory whereas the alphaP spectra suggest that the evaporation of alphaP derived aerosol appears to not be governed by partitioning theory. We postulate that this difference arises from the alphaP particles existing as in a glassy state instead of having the expected liquid-like behavior. To reconcile these observations with decades of aerosol growth measurements, which indicate that OA formation is described by equilibrium partitioning, we present a conceptual model wherein the secondary OA is formed and then rapidly converted from an absorbing form to a non-absorbing form. The results suggest that although OA growth may be describable by equilibrium partitioning theory, the properties of organic aerosol once formed may differ significantly from the properties determined in the equilibrium framework.

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    from size distribution and light scattering data: Weakly absorbing aerosol." Atmospheric Measurement Techniques, 7, doi:10.5194amt-7-3247-2014. Observing Aerosols. The ARM...

  8. ARM - Field Campaign - Aerosol IOP

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsAerosol IOP Campaign Links Science Plan (PDF document) ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : Aerosol IOP 2003.05.01 - 2003.05.31 Lead Scientist : Richard Ferrare Data Availability The IOP participants examined the individual instrument data to assess data quality, and to initiate other data analyses. Authorized participants can read reports of planning and debrief meetings,

  9. Real time infrared aerosol analyzer

    DOE Patents [OSTI]

    Johnson, Stanley A. (Countryside, IL); Reedy, Gerald T. (Bourbonnais, IL); Kumar, Romesh (Naperville, IL)

    1990-01-01

    Apparatus for analyzing aerosols in essentially real time includes a virtual impactor which separates coarse particles from fine and ultrafine particles in an aerosol sample. The coarse and ultrafine particles are captured in PTFE filters, and the fine particles impact onto an internal light reflection element. The composition and quantity of the particles on the PTFE filter and on the internal reflection element are measured by alternately passing infrared light through the filter and the internal light reflection element, and analyzing the light through infrared spectrophotometry to identify the particles in the sample.

  10. Study of in-duct spray drying using condensation aerosol. Final report, June 16, 1990--June 15, 1992

    SciTech Connect (OSTI)

    Chen, W.J.R.; Chang, S.M.; Adikesavalu, R.

    1992-06-01

    Sulfur removal efficiency of in-duct spray drying is limited by sorbent content and surface properties of the sorbent-water aerosol. It was the purpose of this study to improve the sulfur removal efficiency for in-duct spray drying by injecting condensation aerosol instead of conventional dispersion aerosol. The program was composed of three phases. In Phase I, a novel pulsed fluid bed feeder was developed and was used to feed hydrated lime for subsequent experiments. A small condensation aerosol generator was then built, which produces a lime-water condensation aerosol by condensing steam on lime particles. The results show that novel lime-water aerosols less than 10 microns were generated. The central task in Phase II was to simulate experimentally in-duct spray drying using condensation aerosols and compare the results with those using dispersion aerosols reported in the literature. A small entrained-flow reactor was constructed to simulate an in-duct spray dryer. The condensation aerosol was then introduced to the reactor at various approach to saturation temperature, calcium/sulfur stoichiometry and sulfur dioxide concentration for desulfurization study. The results show that we have improved the sulfur removal efficiency for in-duct spray drying to 90 percent or above. Thus we have met and exceeded the stated project goal of 70 percent sulfur removal. A comprehensive computer code was employed to calculate sulfur removal efficiency in Phase III.

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Improving the Treatment of Radiation in Climate Models Download a printable PDF Submitter: Delamere, J. S., Tech-X Corporation Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle, Cloud Life Cycle Journal Reference: Delamere JS, SA Clough, VH Payne, EJ Mlawer, DD Turner, and RR Gamache. 2010. "A far-infrared radiative closure study in the Arctic: Application to water vapor." Journal of Geophysical Research - Atmospheres, 115, D17106, 10.1029/2009JD012968. The

  12. ARM - PI Product - Black Carbon aerosol mass concentration in snow and rain

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    samples over Barrow in the Arctic ProductsBlack Carbon aerosol mass concentration in snow and rain samples over Barrow in the Arctic ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send PI Product : Black Carbon aerosol mass concentration in snow and rain samples over Barrow in the Arctic [ ARM research ] Deposition of black carbon aerosol (BC) on snow (i.e. wet deposition) is considered to lower snow albedo and

  13. Efficacy of Aerosol-Cloud Interactions Under Varying Meteorological Conditions: Southern Great Plains Vs. Pt. Reyes

    SciTech Connect (OSTI)

    Dunn, M.; Schwartz, S.; Kim, B.-G.; Miller, M.; Liu, Y.; Min, Q.

    2008-03-10

    Several studies have demonstrated that cloud dynamical processes such as entrainment mixing may be the primary modulator of cloud optical properties in certain situations. For example, entrainment of dry air alters the cloud drop size distribution by enhancing drop evaporation. However, the effect of entrainment mixing and other forms or turbulence is still quite uncertain. Although these factors and aerosol-cloud interactions should be considered together when evaluating the efficacy of aerosol indirect effects, the underlying mechanisms appear to be dependent upon each other. In addition, accounting for them is impossible with the current understanding of aerosol indirect effect. Therefore, careful objective screening and analysis of observations are needed to determine the extent to which mixing related properties affect cloud optical properties, apart from the aerosol first indirect effect. This study addresses the role of aerosol-cloud interactions in the context of varying meteorological conditions based on ARM data obtained at the Southern Great Plains (SGP) site in Oklahoma and at Pt. Reyes, California. Previous analyses of the continental stratiform clouds at the SGP site have shown that the thicker clouds of high liquid water path (LWP) tend to contain sub adiabatic LWPs. These sub adiabatic LWPs, which result from active mixing processes, correspond to a lower susceptibility of the clouds to aerosol-cloud interactions, and, hence, to reduced aerosol indirect effects. In contrast, the consistently steady and thin maritime stratus clouds observed at Pt. Reyes are much closer to adiabatic. These clouds provide an excellent benchmark for the study of the aerosol influence on modified marine clouds relative to continental clouds, since they form in a much more homogeneous meteorological environment than those at the continental site.

  14. Hyperspectral Aerosol Optical Depths from TCAP Flights

    SciTech Connect (OSTI)

    Shinozuka, Yohei; Johnson, Roy R.; Flynn, Connor J.; Russell, P. B.; Schmid, Beat; Redemann, Jens; Dunagan, Stephen; Kluzek, Celine D.; Hubbe, John M.; Segal-Rosenheimer, Michal; Livingston, J. M.; Eck, T.; Wagener, Richard; Gregory, L.; Chand, Duli; Berg, Larry K.; Rogers, Ray; Ferrare, R. A.; Hair, John; Hostetler, Chris A.; Burton, S. P.

    2013-11-13

    4STAR (Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research), the worlds first hyperspectral airborne tracking sunphotometer, acquired aerosol optical depths (AOD) at 1 Hz during all July 2012 flights of the Two Column Aerosol Project (TCAP). Root-mean square differences from AERONET ground-based observations were 0.01 at wavelengths between 500-1020 nm, 0.02 at 380 and 1640 nm and 0.03 at 440 nm in four clear-sky fly-over events, and similar in ground side-by-side comparisons. Changes in the above-aircraft AOD across 3-km-deep spirals were typically consistent with integrals of coincident in situ (on DOE Gulfstream 1 with 4STAR) and lidar (on NASA B200) extinction measurements within 0.01, 0.03, 0.01, 0.02, 0.02, 0.02 at 355, 450, 532, 550, 700, 1064 nm, respectively, despite atmospheric variations and combined measurement uncertainties. Finer vertical differentials of the 4STAR measurements matched the in situ ambient extinction profile within 14% for one homogeneous column. For the AOD observed between 350-1660 nm, excluding strong water vapor and oxygen absorption bands, estimated uncertainties were ~0.01 and dominated by (then) unpredictable throughput changes, up to +/-0.8%, of the fiber optic rotary joint. The favorable intercomparisons herald 4STARs spatially-resolved high-frequency hyperspectral products as a reliable tool for climate studies and satellite validation.

  15. ARM - Field Campaign - Fall 1997 Aerosol IOP

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsFall 1997 Aerosol IOP ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : Fall 1997 Aerosol IOP 1997.09.15 - 1997.10.05 Lead Scientist : Stephen Schwartz For data sets, see below. Summary The Aerosol IOP was highlighted by the Gulfstream-1 aircraft flying clear-sky aerosol missions over the Central Facility to study the effect of aerosol loading on clear sky radiation fields, with weather

  16. ARM - Evaluation Product - Organic Aerosol Component VAP

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ProductsOrganic Aerosol Component VAP ARM Data Discovery Browse Data Documentation Use the Data File Inventory tool to view data availability at the file level. Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Evaluation Product : Organic Aerosol Component VAP Organic aerosol (OA, i.e., the organic fraction of particles) accounts for 10-90% of the fine aerosol mass globally and is a key determinant of aerosol radiative forcing. But atmospheric OA

  17. Aerosol Impacts on California Winter Clouds and Precipitation during CalWater 2011: Local Pollution versus Long-Range Transported Dust

    SciTech Connect (OSTI)

    Fan, Jiwen; Leung, Lai-Yung R.; DeMott, Paul J.; Comstock, Jennifer M.; Singh, Balwinder; Rosenfeld, Daniel; Tomlinson, Jason M.; White, Allen B.; Prather, Kimberly; Minnis, Patrick; Ayers, J. K.; Min, Qilong

    2014-01-03

    Mineral dust aerosols often observed over California in winter and spring, associated with long-range transport from Asia and Sahara, have been linked to enhanced precipitation based on observations. Local anthropogenic pollution, on the other hand, was shown in previous observational and modeling studies to reduce precipitation. Here we incorporate recent developments in ice nucleation parameterizations to link aerosols with ice crystal formation in a spectral-bin cloud microphysical model coupled with the Weather Research and Forecasting (WRF) model, to examine the relative and combined impacts of dust and local pollution particles on cloud properties and precipitation type and intensity. Simulations are carried out for two cloud cases with contrasting meteorology and cloud dynamics that occurred on February 16 (FEB16) and March 02 (MAR02) from the CalWater 2011 field campaign. In both cases, observations show the presence of dust and biological particles in a relative pristine environment. The simulated cloud microphysical properties and precipitation show reasonable agreement with aircraft and surface measurements. Model sensitivity experiments indicate that in the pristine environment, the dust and biological aerosol layers increase the accumulated precipitation by 10-20% from the Central Valley to the Sierra Nevada Mountains for both FEB16 and MAR02 due to a ~40% increase in snow formation, validating the observational hypothesis. Model results show that local pollution increases precipitation over the windward slope of the mountains by few percent due to increased snow formation when dust is present but reduces precipitation by 5-8% if dust is removed on FEB16. The effects of local pollution on cloud microphysics and precipitation strongly depend on meteorology including the strength of the Sierra Barrier Jet, and cloud dynamics. This study further underscores the importance of the interactions between local pollution, dust, and environmental conditions for assessing aerosol effects on cold season precipitation in California.

  18. Aerosol Radiative Forcing During Spring-Summer 2002 from Measurements at IAP Scientific Station Near Moscow

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Forcing During Spring-Summer 2002 from Measurements at IAP Scientific Station Near Moscow G. S. Golitsyn, I. A. Gorchakova, and I. I. Mokhov A. M. Obukohov Institute of Atmospheric Physics Russian Academy of Science Moscow, Russia A. N. Rublev Russian Research Center Kurchatov Institute Moscow, Russia Introduction Aerosol Radiative Forcing (ARF) is estimated for spring-summer conditions from measurements during the Cloud-Aerosol-Radiation Experiment in 2002 (ZCAREX-2002) at the Zvenigorod

  19. Effective Radius of Cloud Droplets by Ground-Based Remote Sensing: Relationships to Aerosol?

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Effective Radius of Cloud Droplets by Ground-Based Remote Sensing: Relationships to Aerosol? B.-G. Kim, S. E. Schwartz, and M. A. Miller Environmental Sciences Department Brookhaven National Laboratory Upton, New York Q.-L. Min Atmospheric Science Research Center State University of New York Albany, New York Introduction Aerosol Indirect Effect Increases in anthropogenic sources of cloud condensation nuclei can increase cloud albedo by increasing the concentration and reducing the size of cloud

  20. Transport of anthropogenic and biomass burning aerosols from Europe to the Arctic during spring 2008

    SciTech Connect (OSTI)

    Marelle, L.; Raut, Jean-Christophe; Thomas, J. L.; Law, K. S.; Quennehen, Boris; Ancellet, G.; Pelon, J.; Schwarzenboeck, A.; Fast, Jerome D.

    2015-04-10

    During the POLARCAT-France airborne campaign in April 2008, pollution originating from anthropogenic and biomass burning emissions was measured in the European Arctic. We compare these aircraft measurements with simulations using the WRF-Chem model to investigate model representation of aerosols transported from Europe to the Arctic. Modeled PM2.5 is evaluated using European Monitoring and Evaluation Programme (EMEP) measurements in source regions and POLARCAT aircraft measurements in the Scandinavian Arctic. Total PM2.5 agrees well with the measurements, although the model overestimates nitrate and underestimates organic carbon in source regions. Using WRF-Chem in combination with the Lagrangian model FLEXPART-WRF, we find that during the campaign the research aircraft sampled two different types of European plumes: mixed anthropogenic and fire plumes from eastern Europe and Russia transported below 2 km, and anthropogenic plumes from central Europe uplifted by warm conveyor belt circulations to 56 km. Both modeled plume types had undergone significant wet scavenging (> 50% PM10) during transport. Modeled aerosol vertical distributions and optical properties below the aircraft are evaluated in the Arctic using airborne lidar measurements. Model results show that the pollution event transported aerosols into the Arctic (> 66.6 N) for a 4-day period. During this 4-day period, biomass burning emissions have the strongest influence on concentrations between 2.5 and 3 km altitudes, while European anthropogenic emissions influence aerosols at both lower (~ 1.5 km) and higher altitudes (~ 4.5 km). As a proportion of PM2.5, modeled black carbon and SO4= concentrations are more enhanced near the surface in anthropogenic plumes. The European plumes sampled during the POLARCAT-France campaign were transported over the region of springtime snow cover in northern Scandinavia, where they had a significant local atmospheric warming effect. We find that, during this transport event, the average modeled top-of-atmosphere (TOA) shortwave direct and semi-direct radiative effect (DSRE) north of 60 N over snow and ice-covered surfaces reaches +0.58 W m?2, peaking at +3.3 W m?2 at noon over Scandinavia and Finland.

  1. Transport of anthropogenic and biomass burning aerosols from Europe to the Arctic during spring 2008

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Marelle, L.; Raut, Jean-Christophe; Thomas, J. L.; Law, K. S.; Quennehen, Boris; Ancellet, G.; Pelon, J.; Schwarzenboeck, A.; Fast, Jerome D.

    2015-04-10

    During the POLARCAT-France airborne campaign in April 2008, pollution originating from anthropogenic and biomass burning emissions was measured in the European Arctic. We compare these aircraft measurements with simulations using the WRF-Chem model to investigate model representation of aerosols transported from Europe to the Arctic. Modeled PM2.5 is evaluated using European Monitoring and Evaluation Programme (EMEP) measurements in source regions and POLARCAT aircraft measurements in the Scandinavian Arctic. Total PM2.5 agrees well with the measurements, although the model overestimates nitrate and underestimates organic carbon in source regions. Using WRF-Chem in combination with the Lagrangian model FLEXPART-WRF, we find that duringmore » the campaign the research aircraft sampled two different types of European plumes: mixed anthropogenic and fire plumes from eastern Europe and Russia transported below 2 km, and anthropogenic plumes from central Europe uplifted by warm conveyor belt circulations to 5–6 km. Both modeled plume types had undergone significant wet scavenging (> 50% PM10) during transport. Modeled aerosol vertical distributions and optical properties below the aircraft are evaluated in the Arctic using airborne lidar measurements. Model results show that the pollution event transported aerosols into the Arctic (> 66.6° N) for a 4-day period. During this 4-day period, biomass burning emissions have the strongest influence on concentrations between 2.5 and 3 km altitudes, while European anthropogenic emissions influence aerosols at both lower (~ 1.5 km) and higher altitudes (~ 4.5 km). As a proportion of PM2.5, modeled black carbon and SO4= concentrations are more enhanced near the surface in anthropogenic plumes. The European plumes sampled during the POLARCAT-France campaign were transported over the region of springtime snow cover in northern Scandinavia, where they had a significant local atmospheric warming effect. We find that, during this transport event, the average modeled top-of-atmosphere (TOA) shortwave direct and semi-direct radiative effect (DSRE) north of 60° N over snow and ice-covered surfaces reaches +0.58 W m−2, peaking at +3.3 W m−2 at noon over Scandinavia and Finland.« less

  2. FY 2011 Second Quarter: Demonstration of New Aerosol Measurement Verification Testbed for Present-Day Global Aerosol Simulations

    SciTech Connect (OSTI)

    Koch, D

    2011-03-20

    The regional-scale Weather Research and Forecasting (WRF) model is being used by a DOE Earth System Modeling (ESM) project titled Improving the Characterization of Clouds, Aerosols and the Cryosphere in Climate Models to evaluate the performance of atmospheric process modules that treat aerosols and aerosol radiative forcing in the Arctic. We are using a regional-scale modeling framework for three reasons: (1) It is easier to produce a useful comparison to observations with a high resolution model; (2) We can compare the behavior of the CAM parameterization suite with some of the more complex and computationally expensive parameterizations used in WRF; (3) we can explore the behavior of this parameterization suite at high resolution. Climate models like the Community Atmosphere Model version 5 (CAM5) being used within the Community Earth System Model (CESM) will not likely be run at mesoscale spatial resolutions (1020 km) until 510 years from now. The performance of the current suite of physics modules in CAM5 at such resolutions is not known, and current computing resources do not permit high-resolution global simulations to be performed routinely. We are taking advantage of two tools recently developed under PNNL Laboratory Directed Research and Development (LDRD) projects for this activity. The first is the Aerosol Modeling Testbed (Fast et al., 2011b), a new computational framework designed to streamline the process of testing and evaluating aerosol process modules over a range of spatial and temporal scales. The second is the CAM5 suite of physics parameterizations that have been ported into WRF so that their performance and scale dependency can be quantified at mesoscale spatial resolutions (Gustafson et al., 2010; with more publications in preparation).

  3. Atmospheric Radiation Measurement (ARM) Data from Point Reyes, California for the Marine Stratus, Radiation, Aerosol, and Drizzle (MASRAD) Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Point Reyes National Seashore, on the California coast north of San Francisco, was the location of the first deployment of the DOE's Atmospheric Radiation Measurement (ARM) Mobile Facility (AMF). The ARM Program collaborated with the U.S. Office of Naval Research and DOE's Aerosol Science Program in the Marine Stratus, Radiation, Aerosol, and Drizzle (MASRAD) project. Their objectives were to collect data from cloud/aerosol interactions and to improve understanding of cloud organization that is often associated with patches of drizzle. Between March and September 2005, the AMF and at least two research aircraft were used to collect data.

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Using ARM Cloud Data to Evaluate the Effect of a Land Surface on Clouds Download a printable PDF Submitter: GSFC, N., NASA GSFC Area of Research: Cloud Distributions/Characterizations Working Group(s): Aerosol, Cloud Modeling Journal Reference: Zeng, X., W.-K. Tao, M. Zhang, C. Peters-Lidard, S. Lang, J. Simpson, S. Kumar, S. Xie, J. L. Eastman, C.-L. Shie, and J. V. Geiger, 2007: Evaluating clouds in long-term cloud-resolving model simulations with observational data. J. Atmos. Sci. (in press).

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Preview of TWP MFRSR Data Submitter: Chuang, C., Lawrence Livermore National Laboratory Area of Research: Radiation Processes Working Group(s): Radiative Processes Journal Reference: N/A Figure 1. MFRSR data from the TWP site (97/09/10) Figure 2. Aerosol optical depth and Angstrom exponent Figure 3. Water vapor derived from MFRSR and MWR Key contributors to this work are Jim Barnard and Will Shaw. The Multi-Filter Rotating Shadowband Radiometer (MFRSR) is a ground-based radiometer that uses

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Deciphering Raindrop Collisions with Dual-polarization Radar Download a printable PDF Submitter: Kumjian, M., Pennsylvania State University Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Kumjian MR and OP Prat. 2014. "The impact of raindrop collisional processes on the polarimetric radar variables." Journal of the Atmospheric Sciences, 71(8), doi:10.1175/JAS-D-13-0357.1. (a) Changes in ZDR as a function

  7. ARM - Mobile Aerosol Observing System

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    FacilitiesMobile Aerosol Observing System AMF Information Science Architecture Baseline Instruments AMF1 AMF2 AMF3 MAOS Data Operations AMF Fact Sheet Images Contacts AMF Deployments McMurdo Station, Antarctica, 2015-2016 Pearl Harbor, Hawaii, to San Francisco, California, 2015 Hyytiälä, Finland, 2014 Manacapuru, Brazil, 2014 Oliktok Point, Alaska, 2013 Los Angeles, California, to Honolulu, Hawaii, 2012 Cape Cod, Massachusetts, 2012 Gan Island, Maldives, 2011 Ganges Valley, India, 2011

  8. Aerosol Oxidation Speeds Up in Smoggy Air

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Oxidation Speeds Up in Smoggy Air Print Organic aerosols (nanometer-sized liquid or solid particles suspended in air) are important constituents of the troposphere, and their chemistry has large-scale impacts on climate, pollution, and health. Accurate predictions of these aerosol impacts require a robust microphysical understanding of all relevant chemical reaction mechanisms and time scales, including those involving highly reactive free-radical molecules. However, detailed modeling is

  9. Aerosol Oxidation Speeds Up in Smoggy Air

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Oxidation Speeds Up in Smoggy Air Print Organic aerosols (nanometer-sized liquid or solid particles suspended in air) are important constituents of the troposphere, and their chemistry has large-scale impacts on climate, pollution, and health. Accurate predictions of these aerosol impacts require a robust microphysical understanding of all relevant chemical reaction mechanisms and time scales, including those involving highly reactive free-radical molecules. However, detailed modeling is

  10. Aerosol Oxidation Speeds Up in Smoggy Air

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Oxidation Speeds Up in Smoggy Air Print Organic aerosols (nanometer-sized liquid or solid particles suspended in air) are important constituents of the troposphere, and their chemistry has large-scale impacts on climate, pollution, and health. Accurate predictions of these aerosol impacts require a robust microphysical understanding of all relevant chemical reaction mechanisms and time scales, including those involving highly reactive free-radical molecules. However, detailed modeling is

  11. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused

  12. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused

  13. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused

  14. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Composition and Reactions of Atmospheric Aerosol Particles Print Wednesday, 29 June 2005 00:00 Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the

  15. Aerosol Oxidation Speeds Up in Smoggy Air

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Oxidation Speeds Up in Smoggy Air Print Organic aerosols (nanometer-sized liquid or solid particles suspended in air) are important constituents of the troposphere, and their chemistry has large-scale impacts on climate, pollution, and health. Accurate predictions of these aerosol impacts require a robust microphysical understanding of all relevant chemical reaction mechanisms and time scales, including those involving highly reactive free-radical molecules. However, detailed modeling is

  16. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused

  17. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused

  18. ARM - Campaign Instrument - aerosol-tower-eml

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govInstrumentsaerosol-tower-eml Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign Instrument : EML Tower based Aerosol Measurements (AEROSOL-TOWER-EML) Instrument Categories Aerosols Campaigns Remote Cloud Sensing (RCS) Field Evaluation [ Download Data ] Southern Great Plains, 1994.04.01 - 1994.05.31 Primary Measurements Taken The following measurements are those considered scientifically relevant. Refer to the datastream (netcdf) file

  19. Unintended consequences of atmospheric injection of sulphate aerosols.

    SciTech Connect (OSTI)

    Brady, Patrick Vane; Kobos, Peter Holmes; Goldstein, Barry

    2010-10-01

    Most climate scientists believe that climate geoengineering is best considered as a potential complement to the mitigation of CO{sub 2} emissions, rather than as an alternative to it. Strong mitigation could achieve the equivalent of up to -4Wm{sup -2} radiative forcing on the century timescale, relative to a worst case scenario for rising CO{sub 2}. However, to tackle the remaining 3Wm{sup -2}, which are likely even in a best case scenario of strongly mitigated CO{sub 2} releases, a number of geoengineering options show promise. Injecting stratospheric aerosols is one of the least expensive and, potentially, most effective approaches and for that reason an examination of the possible unintended consequences of the implementation of atmospheric injections of sulphate aerosols was made. Chief among these are: reductions in rainfall, slowing of atmospheric ozone rebound, and differential changes in weather patterns. At the same time, there will be an increase in plant productivity. Lastly, because atmospheric sulphate injection would not mitigate ocean acidification, another side effect of fossil fuel burning, it would provide only a partial solution. Future research should aim at ameliorating the possible negative unintended consequences of atmospheric injections of sulphate injection. This might include modeling the optimum rate and particle type and size of aerosol injection, as well as the latitudinal, longitudinal and altitude of injection sites, to balance radiative forcing to decrease negative regional impacts. Similarly, future research might include modeling the optimum rate of decrease and location of injection sites to be closed to reduce or slow rapid warming upon aerosol injection cessation. A fruitful area for future research might be system modeling to enhance the possible positive increases in agricultural productivity. All such modeling must be supported by data collection and laboratory and field testing to enable iterative modeling to increase the accuracy and precision of the models, while reducing epistemic uncertainties.

  20. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused particle growth while...

  1. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    will help climate scientists refine the computer models used to predict climate change. Tiny Specks with Large Effects Most people equate aerosols with hairspray and...

  2. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    results will help climate scientists refine the computer models used to predict climate change. Tiny Specks with Large Effects Most people equate aerosols with hairspray and...

  3. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    refine the computer models used to predict climate change. Tiny Specks with Large Effects Most people equate aerosols with hairspray and household cleaning products, but a...

  4. The LANL Cloud-Aerosol Model

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    that incorporates two unique aspects in its formulation. First, the model employs a nonlinear solver that requires cloud-aerosol parameterizations be smooth or contain reasonable...

  5. THE INFLUENCE OF BENZENE AS A TRACE REACTANT IN TITAN AEROSOL ANALOGS

    SciTech Connect (OSTI)

    Trainer, Melissa G.; Sebree, Joshua A.; Heidi Yoon, Y.; Tolbert, Margaret A.

    2013-03-20

    Benzene has been detected in Titan's atmosphere by Cassini instruments, with concentrations ranging from sub-ppb in the stratosphere to ppm in the ionosphere. Sustained levels of benzene in the haze formation region could signify that it is an important reactant in the formation of Titan's organic aerosol. To date, there have not been laboratory investigations to assess the influence of benzene on aerosol properties. We report a laboratory study on the chemical composition of organic aerosol formed from C{sub 6}H{sub 6}/CH{sub 4}/N{sub 2} via far ultraviolet irradiation (120-200 nm). The compositional results are compared to those from aerosol generated by a more ''traditional Titan'' mixture of CH{sub 4}/N{sub 2}. Our results show that even a trace amount of C{sub 6}H{sub 6} (10 ppm) has significant impact on the chemical composition and production rates of organic aerosol. There are several pathways by which photolyzed benzene may react to form larger molecules, both with and without the presence of CH{sub 4}, but many of these reaction mechanisms are only beginning to be explored for the conditions at Titan. Continued work investigating the influence of benzene in aerosol growth will advance understanding of this previously unstudied reaction system.

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Submitter: Westwater, E. R., University of Colorado Area of Research: Atmospheric Thermodynamics and Vertical Structures Working Group(s): Cloud Properties Journal Reference:...

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Liljegren, J. C., Argonne National Laboratory Area of Research: Atmospheric Thermodynamics and Vertical Structures Working Group(s): Cloud Properties, Radiative Processes...

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lovejoy, S., McGill University Area of Research: Atmospheric Thermodynamics and Vertical Structures Working Group(s): Cloud Properties Journal Reference: Lovejoy, S., D....

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    of MBL Cloud Properties over the Azores Download a printable PDF Submitter: Dong, X., University of North Dakota Area of Research: Radiation Processes Working Group(s): Cloud...

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Climate Change Download a printable PDF Submitter: Maseyk, K. S., Universite Pierre et Marie Curie, Paris 6 Area of Research: Surface Properties Working Group(s):...

  11. ARM - Field Campaign - Aerosol and Cloud Experiments in the Eastern...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    horizontal variabilities of aerosol, trace gases, cloud, drizzle, and atmospheric thermodynamics are critically needed for understanding and quantifying the budget of MBL aerosol,...

  12. Analysis of Langley optical depth data, with aerosol and gas...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Columbia University - NASAGISS Lacis, Andrew NASAGoddard Institute for Space Studies Carlson, Barbara NASAGoddard Institute for Space Studies Category: Aerosols Bimodal aerosol...

  13. ARM - Field Campaign - Carbonaceous Aerosol and Radiative Effects...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsCarbonaceous Aerosol and Radiative Effects Study (CARES) Campaign Links CARES Website ARM Data Discovery Browse Data Related Campaigns Carbonaceous Aerosol and...

  14. ARM - Field Campaign - Carbonaceous Aerosol and Radiation Effects...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Photo-Acoustic Aerosol Light Absorption and Scattering Campaign Links ARM Data Discovery Browse Data Related Campaigns Carbonaceous Aerosol and Radiative Effects Study (CARES)...

  15. ARM - Facility News Article

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    aerosol properties, aerosol indirect effects, precipitation, visibility (extinction), particle spectra, and ice crystal processes. Researchers from Environment Canada filled the...

  16. AEROSOL PARTICLE COLLECTOR DESIGN STUDY

    SciTech Connect (OSTI)

    Lee, S; Richard Dimenna, R

    2007-09-27

    A computational evaluation of a particle collector design was performed to evaluate the behavior of aerosol particles in a fast flowing gas stream. The objective of the work was to improve the collection efficiency of the device while maintaining a minimum specified air throughput, nominal collector size, and minimal power requirements. The impact of a range of parameters was considered subject to constraints on gas flow rate, overall collector dimensions, and power limitations. Potential improvements were identified, some of which have already been implemented. Other more complex changes were identified and are described here for further consideration. In addition, fruitful areas for further study are proposed.

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Group(s): Aerosol Journal Reference: McComiskey, A, SE Schwartz, B Schmid, H Guan, ER Lewis, P Ricchiazzi, and JA Ogren. 2008. "Direct aerosol forcing: Calculation from...

  18. Large-Scale Spray Releases: Additional Aerosol Test Results

    SciTech Connect (OSTI)

    Daniel, Richard C.; Gauglitz, Phillip A.; Burns, Carolyn A.; Fountain, Matthew S.; Shimskey, Rick W.; Billing, Justin M.; Bontha, Jagannadha R.; Kurath, Dean E.; Jenks, Jeromy WJ; MacFarlan, Paul J.; Mahoney, Lenna A.

    2013-08-01

    One of the events postulated in the hazard analysis for the Waste Treatment and Immobilization Plant (WTP) and other U.S. Department of Energy (DOE) nuclear facilities is a breach in process piping that produces aerosols with droplet sizes in the respirable range. The current approach for predicting the size and concentration of aerosols produced in a spray leak event involves extrapolating from correlations reported in the literature. These correlations are based on results obtained from small engineered spray nozzles using pure liquids that behave as a Newtonian fluid. The narrow ranges of physical properties on which the correlations are based do not cover the wide range of slurries and viscous materials that will be processed in the WTP and in processing facilities across the DOE complex. To expand the data set upon which the WTP accident and safety analyses were based, an aerosol spray leak testing program was conducted by Pacific Northwest National Laboratory (PNNL). PNNLs test program addressed two key technical areas to improve the WTP methodology (Larson and Allen 2010). The first technical area was to quantify the role of slurry particles in small breaches where slurry particles may plug the hole and prevent high-pressure sprays. The results from an effort to address this first technical area can be found in Mahoney et al. (2012a). The second technical area was to determine aerosol droplet size distribution and total droplet volume from prototypic breaches and fluids, including sprays from larger breaches and sprays of slurries for which literature data are mostly absent. To address the second technical area, the testing program collected aerosol generation data at two scales, commonly referred to as small-scale and large-scale testing. The small-scale testing and resultant data are described in Mahoney et al. (2012b), and the large-scale testing and resultant data are presented in Schonewill et al. (2012). In tests at both scales, simulants were used to mimic the relevant physical properties projected for actual WTP process streams.

  19. Small-Scale Spray Releases: Additional Aerosol Test Results

    SciTech Connect (OSTI)

    Schonewill, Philip P.; Gauglitz, Phillip A.; Kimura, Marcia L.; Brown, G. N.; Mahoney, Lenna A.; Tran, Diana N.; Burns, Carolyn A.; Kurath, Dean E.

    2013-08-01

    One of the events postulated in the hazard analysis at the Waste Treatment and Immobilization Plant (WTP) and other U.S. Department of Energy (DOE) nuclear facilities is a breach in process piping that produces aerosols with droplet sizes in the respirable range. The current approach for predicting the size and concentration of aerosols produced in a spray leak involves extrapolating from correlations reported in the literature. These correlations are based on results obtained from small engineered spray nozzles using pure liquids with Newtonian fluid behavior. The narrow ranges of physical properties on which the correlations are based do not cover the wide range of slurries and viscous materials that will be processed in the WTP and across processing facilities in the DOE complex. To expand the data set upon which the WTP accident and safety analyses were based, an aerosol spray leak testing program was conducted by Pacific Northwest National Laboratory (PNNL). PNNLs test program addressed two key technical areas to improve the WTP methodology (Larson and Allen 2010). The first technical area was to quantify the role of slurry particles in small breaches where slurry particles may plug the hole and prevent high-pressure sprays. The results from an effort to address this first technical area can be found in Mahoney et al. (2012a). The second technical area was to determine aerosol droplet size distribution and total droplet volume from prototypic breaches and fluids, including sprays from larger breaches and sprays of slurries for which literature data are largely absent. To address the second technical area, the testing program collected aerosol generation data at two scales, commonly referred to as small-scale and large-scale. The small-scale testing and resultant data are described in Mahoney et al. (2012b) and the large-scale testing and resultant data are presented in Schonewill et al. (2012). In tests at both scales, simulants were used to mimic the relevant physical properties projected for actual WTP process streams.

  20. EMSP Final Report: Electrically Driven Technologies for Radioactive Aerosol Abatement

    SciTech Connect (OSTI)

    DePaoli, D.W.

    2003-01-22

    The purpose of this research project was to develop an improved understanding of how electrically driven processes, including electrocoalescence, acoustic agglomeration, and electric filtration, may be employed to efficiently treat problems caused by the formation of aerosols during DOE waste treatment operations. The production of aerosols during treatment and retrieval operations in radioactive waste tanks and during thermal treatment operations such as calcination presents a significant problem of cost, worker exposure, potential for release, and increased waste volume. There was anecdotal evidence in the literature that acoustic agglomeration and electrical coalescence could be used together to change the size distribution of aerosol particles in such a way as to promote easier filtration and less frequent maintenance of filtration systems. As such, those electrically driven technologies could potentially be used as remote technologies for improved treatment; however, existing theoretical models are not suitable for prediction and design. To investigate the physics of such systems, and also to prototype a system for such processes, a collaborative project was undertaken between Oak Ridge National Laboratory (ORNL) and the University of Texas at Austin (UT). ORNL was responsible for the larger-scale prototyping portion of the project, while UT was primarily responsible for the detailed physics in smaller scale unit reactors. It was found that both electrical coalescence and acoustic agglomeration do in fact increase the rate of aggregation of aerosols. Electrical coalescence requires significantly less input power than acoustic agglomeration, but it is much less effective in its ability to aggregate/coalesce aerosols. The larger-scale prototype showed qualitatively similar results as the unit reactor tests, but presented more difficulty in interpretation of the results because of the complex multi-physics coupling that necessarily occur in all larger-scale system tests. An additional finding from this work is that low-amplitude oscillation may provide an alternative, non-invasive, non-contact means of controlling settling and/or suspension of solids. Further investigation would be necessary to evaluate its utility for radioactive waste treatment applications. This project did not uncover a new technology for radioactive waste treatment. While it may be possible that an efficient electrically driven technology for aerosol treatment could be developed, it appears that other technologies, such as steel and ceramic HEPA filters, can suitably solve this problem. If further studies are to be undertaken, additional fundamental experimentation and modeling is necessary to fully capture the physics; in addition, larger-scale tests are needed to demonstrate the treatment of flowing gas streams through the coupling of acoustic agglomeration with electrocoalescence.

  1. Global distribution and climate forcing of marine organic aerosol: 1. Model improvements and evaluation

    SciTech Connect (OSTI)

    Meskhidze, N.; Xu, J.; Gantt, Brett; Zhang, Yang; Nenes, Athanasios; Ghan, Steven J.; Liu, Xiaohong; Easter, Richard C.; Zaveri, Rahul A.

    2011-11-23

    Marine organic aerosol emissions have been implemented and evaluated within the National Center of Atmospheric Research (NCAR)'s Community Atmosphere Model (CAM5) with the Pacific Northwest National Laboratory's 7-mode Modal Aerosol Module (MAM-7). Emissions of marine primary organic aerosols (POA), phytoplanktonproduced isoprene- and monoterpenes-derived secondary organic aerosols (SOA) and methane sulfonate (MS{sup -}) are shown to affect surface concentrations of organic aerosols in remote marine regions. Global emissions of submicron marine POA is estimated to be 7.9 and 9.4 Tg yr{sup -1}, for the Gantt et al. (2011) and Vignati et al. (2010) emission parameterizations, respectively. Marine sources of SOA and particulate MS{sup -} (containing both sulfur and carbon atoms) contribute an additional 0.2 and 5.1 Tg yr{sup -1}, respectively. Widespread areas over productive waters of the Northern Atlantic, Northern Pacific, and the Southern Ocean show marine-source submicron organic aerosol surface concentrations of 100 ngm{sup -3}, with values up to 400 ngm{sup -3} over biologically productive areas. Comparison of long-term surface observations of water insoluble organic matter (WIOM) with POA concentrations from the two emission parameterizations shows that despite revealed discrepancies (often more than a factor of 2), both Gantt et al. (2011) and Vignati et al. (2010) formulations are able to capture the magnitude of marine organic aerosol concentrations, with the Gantt et al. (2011) parameterization attaining better seasonality. Model simulations show that the mixing state of the marine POA can impact the surface number concentration of cloud condensation nuclei (CCN). The largest increases (up to 20 %) in CCN (at a supersaturation (S) of 0.2 %) number concentration are obtained over biologically productive ocean waters when marine organic aerosol is assumed to be externally mixed with sea-salt. Assuming marine organics are internally-mixed with sea-salt provides diverse results with increases and decreases in the concentration of CCN over different parts of the ocean. The sign of the CCN change due to the addition of marine organics to seasalt aerosol is determined by the relative significance of the increase in mean modal diameter due to addition of mass, and the decrease in particle hygroscopicity due to compositional changes in marine aerosol. Based on emerging evidence for increased CCN concentration over biologically active surface ocean areas/periods, our study suggests that treatment of sea spray in global climate models (GCMs) as an internal mixture of marine organic aerosols and sea-salt will likely lead to an underestimation in CCN number concentration.

  2. New Analysis Methods Estimate a Critical Property of Ethanol Fuel Blends (Fact Sheet), Highlights in Research & Development, NREL (National Renewable Energy Laboratory)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Methods developed at NREL disclose the impact of ethanol on gasoline blend heat of vaporization with potential for improved efficiency of spark-ignition engines. More stringent standards for fuel economy, regulation of greenhouse gas emissions, and the mandated increase in the use of renew- able fuel are driving research to improve the efficiency of spark ignition engines. When fuel properties such as octane number and evaporative cooling (heat of vaporization or HOV) are insufficient, they

  3. Final Report, The Influence of Organic-Aerosol Emissions and Aging on Regional and Global Aerosol Size Distributions and the CCN Number Budget

    SciTech Connect (OSTI)

    Donahue, Neil M.

    2015-12-23

    We conducted laboratory experiments and analyzed data on aging of organic aerosol and analysis of field data on volatility and CCN activity. With supplemental ASR funding we participated in the FLAME-IV campaign in Missoula MT in the Fall of 2012, deploying a two-chamber photochemical aging system to enable experimental exploration of photochemical aging of biomass burning emissions. Results from that campaign will lead to numerous publications, including demonstration of photochemical production of Brown Carbon (BrC) from secondary organic aerosol associated with biomass burning emissions as well as extensive characterization of the effect of photochemical aging on the overall concentrations of biomass burning organic aerosol. Excluding publications arising from the FLAME-IV campaign, project research resulted in 8 papers: [11, 5, 3, 10, 12, 4, 8, 7], including on in Nature Geoscience addressing the role of organic compounds in nanoparticle growth [11

  4. ARM - Field Campaign - Two-Column Aerosol Project (TCAP)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsTwo-Column Aerosol Project (TCAP) Campaign Links TCAP website ARM Data Discovery Browse Data Related Campaigns Two-Column Aerosol Project (TCAP): Field Evaluation of Real-time Cloud OD Sensor TWST 2013.04.15, Scott, AMF Two-Column Aerosol Project (TCAP): Winter Aerosol Effects on Cloud Formation 2013.02.04, Cziczo, AMF Two-Column Aerosol Project (TCAP): CU GMAX-DOAS Deployment 2012.07.15, Volkamer, AMF Two-Column Aerosol Project (TCAP): Aerosol Light Extinction Measurements

  5. Large-Scale Spray Releases: Initial Aerosol Test Results

    SciTech Connect (OSTI)

    Schonewill, Philip P.; Gauglitz, Phillip A.; Bontha, Jagannadha R.; Daniel, Richard C.; Kurath, Dean E.; Adkins, Harold E.; Billing, Justin M.; Burns, Carolyn A.; Davis, James M.; Enderlin, Carl W.; Fischer, Christopher M.; Jenks, Jeromy WJ; Lukins, Craig D.; MacFarlan, Paul J.; Shutthanandan, Janani I.; Smith, Dennese M.

    2012-12-01

    One of the events postulated in the hazard analysis at the Waste Treatment and Immobilization Plant (WTP) and other U.S. Department of Energy (DOE) nuclear facilities is a breach in process piping that produces aerosols with droplet sizes in the respirable range. The current approach for predicting the size and concentration of aerosols produced in a spray leak involves extrapolating from correlations reported in the literature. These correlations are based on results obtained from small engineered spray nozzles using pure liquids with Newtonian fluid behavior. The narrow ranges of physical properties on which the correlations are based do not cover the wide range of slurries and viscous materials that will be processed in the WTP and across processing facilities in the DOE complex. Two key technical areas were identified where testing results were needed to improve the technical basis by reducing the uncertainty due to extrapolating existing literature results. The first technical need was to quantify the role of slurry particles in small breaches where the slurry particles may plug and result in substantially reduced, or even negligible, respirable fraction formed by high-pressure sprays. The second technical need was to determine the aerosol droplet size distribution and volume from prototypic breaches and fluids, specifically including sprays from larger breaches with slurries where data from the literature are scarce. To address these technical areas, small- and large-scale test stands were constructed and operated with simulants to determine aerosol release fractions and generation rates from a range of breach sizes and geometries. The properties of the simulants represented the range of properties expected in the WTP process streams and included water, sodium salt solutions, slurries containing boehmite or gibbsite, and a hazardous chemical simulant. The effect of anti-foam agents was assessed with most of the simulants. Orifices included round holes and rectangular slots. The round holes ranged in size from 0.2 to 4.46 mm. The slots ranged from (width × length) 0.3 × 5 to 2.74 × 76.2 mm. Most slots were oriented longitudinally along the pipe, but some were oriented circumferentially. In addition, a limited number of multi-hole test pieces were tested in an attempt to assess the impact of a more complex breach. Much of the testing was conducted at pressures of 200 and 380 psi, but some tests were conducted at 100 psi. Testing the largest postulated breaches was deemed impractical because of the large size of some of the WTP equipment. The purpose of this report is to present the experimental results and analyses for the aerosol measurements obtained in the large-scale test stand. The report includes a description of the simulants used and their properties, equipment and operations, data analysis methodology, and test results. The results of tests investigating the role of slurry particles in plugging of small breaches are reported in Mahoney et al. 2012a. The results of the aerosol measurements in the small-scale test stand are reported in Mahoney et al. (2012b).

  6. Small-Scale Spray Releases: Initial Aerosol Test Results

    SciTech Connect (OSTI)

    Mahoney, Lenna A.; Gauglitz, Phillip A.; Kimura, Marcia L.; Brown, Garrett N.; Kurath, Dean E.; Buchmiller, William C.; Smith, Dennese M.; Blanchard, Jeremy; Song, Chen; Daniel, Richard C.; Wells, Beric E.; Tran, Diana N.; Burns, Carolyn A.

    2012-11-01

    One of the events postulated in the hazard analysis at the Waste Treatment and Immobilization Plant (WTP) and other U.S. Department of Energy (DOE) nuclear facilities is a breach in process piping that produces aerosols with droplet sizes in the respirable range. The current approach for predicting the size and concentration of aerosols produced in a spray leak involves extrapolating from correlations reported in the literature. These correlations are based on results obtained from small engineered spray nozzles using pure liquids with Newtonian fluid behavior. The narrow ranges of physical properties on which the correlations are based do not cover the wide range of slurries and viscous materials that will be processed in the WTP and across processing facilities in the DOE complex. Two key technical areas were identified where testing results were needed to improve the technical basis by reducing the uncertainty due to extrapolating existing literature results. The first technical need was to quantify the role of slurry particles in small breaches where the slurry particles may plug and result in substantially reduced, or even negligible, respirable fraction formed by high-pressure sprays. The second technical need was to determine the aerosol droplet size distribution and volume from prototypic breaches and fluids, specifically including sprays from larger breaches with slurries where data from the literature are scarce. To address these technical areas, small- and large-scale test stands were constructed and operated with simulants to determine aerosol release fractions and generation rates from a range of breach sizes and geometries. The properties of the simulants represented the range of properties expected in the WTP process streams and included water, sodium salt solutions, slurries containing boehmite or gibbsite, and a hazardous chemical simulant. The effect of anti-foam agents was assessed with most of the simulants. Orifices included round holes and rectangular slots. The round holes ranged in size from 0.2 to 4.46 mm. The slots ranged from (width × length) 0.3 × 5 to 2.74 × 76.2 mm. Most slots were oriented longitudinally along the pipe, but some were oriented circumferentially. In addition, a limited number of multi-hole test pieces were tested in an attempt to assess the impact of a more complex breach. Much of the testing was conducted at pressures of 200 and 380 psi, but some tests were conducted at 100 psi. Testing the largest postulated breaches was deemed impractical because of the large size of some of the WTP equipment. This report presents the experimental results and analyses for the aerosol measurements obtained in the small-scale test stand. It includes a description of the simulants used and their properties, equipment and operations, data analysis methodologies, and test results. The results of tests investigating the role of slurry particles in plugging small breaches are reported in Mahoney et al. (2012). The results of the aerosol measurements in the large-scale test stand are reported in Schonewill et al. (2012) along with an analysis of the combined results from both test scales.

  7. Small-Scale Spray Releases: Initial Aerosol Test Results

    SciTech Connect (OSTI)

    Mahoney, Lenna A.; Gauglitz, Phillip A.; Kimura, Marcia L.; Brown, Garrett N.; Kurath, Dean E.; Buchmiller, William C.; Smith, Dennese M.; Blanchard, Jeremy; Song, Chen; Daniel, Richard C.; Wells, Beric E.; Tran, Diana N.; Burns, Carolyn A.

    2013-05-29

    One of the events postulated in the hazard analysis at the Waste Treatment and Immobilization Plant (WTP) and other U.S. Department of Energy (DOE) nuclear facilities is a breach in process piping that produces aerosols with droplet sizes in the respirable range. The current approach for predicting the size and concentration of aerosols produced in a spray leak involves extrapolating from correlations reported in the literature. These correlations are based on results obtained from small engineered spray nozzles using pure liquids with Newtonian fluid behavior. The narrow ranges of physical properties on which the correlations are based do not cover the wide range of slurries and viscous materials that will be processed in the WTP and across processing facilities in the DOE complex. Two key technical areas were identified where testing results were needed to improve the technical basis by reducing the uncertainty due to extrapolating existing literature results. The first technical need was to quantify the role of slurry particles in small breaches where the slurry particles may plug and result in substantially reduced, or even negligible, respirable fraction formed by high-pressure sprays. The second technical need was to determine the aerosol droplet size distribution and volume from prototypic breaches and fluids, specifically including sprays from larger breaches with slurries where data from the literature are scarce. To address these technical areas, small- and large-scale test stands were constructed and operated with simulants to determine aerosol release fractions and net generation rates from a range of breach sizes and geometries. The properties of the simulants represented the range of properties expected in the WTP process streams and included water, sodium salt solutions, slurries containing boehmite or gibbsite, and a hazardous chemical simulant. The effect of antifoam agents was assessed with most of the simulants. Orifices included round holes and rectangular slots. For the combination of both test stands, the round holes ranged in size from 0.2 to 4.46 mm. The slots ranged from (width × length) 0.3 × 5 to 2.74 × 76.2 mm. Most slots were oriented longitudinally along the pipe, but some were oriented circumferentially. In addition, a limited number of multi-hole test pieces were tested in an attempt to assess the impact of a more complex breach. Much of the testing was conducted at pressures of 200 and 380 psi, but some tests were conducted at 100 psi. Testing the largest postulated breaches was deemed impractical because of the much larger flow rates and equipment that would be required. This report presents the experimental results and analyses for the aerosol measurements obtained in the small-scale test stand. It includes a description of the simulants used and their properties, equipment and operations, data analysis methodologies, and test results. The results of tests investigating the role of slurry particles in plugging small breaches are reported in Mahoney et al. (2012). The results of the aerosol measurements in the large-scale test stand are reported in Schonewill et al. (2012) along with an analysis of the combined results from both test scales.

  8. Clouds, aerosol, and precipitation in the Marine Boundary Layer: An ARM mobile facility deployment

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Wood, Robert; Luke, Ed; Wyant, Matthew; Bretherton, Christopher S.; Remillard, Jasmine; Kollias, Pavlos; Fletcher, Jennifer; Stemmler, Jayson; deSzoeke, S.; Yuter, Sandra; et al

    2014-04-27

    The Clouds, Aerosol, and Precipitation in the Marine Boundary Layer (CAP-MBL) deployment at Graciosa Island in the Azores generated a 21-month (April 2009-December 2010) comprehensive dataset documenting clouds, aerosols, and precipitation using the Atmospheric Radiation Measurement Program (ARM) Mobile Facility (AMF). The scientific aim of the deployment is to gain improved understanding of the interactions of clouds, aerosols, and precipitation in the marine boundary layer. Graciosa Island straddles the boundary between the subtropics and midlatitudes in the Northeast Atlantic Ocean and consequently experiences a great diversity of meteorological and cloudiness conditions. Low clouds are the dominant cloud type, with stratocumulusmore » and cumulus occurring regularly. Approximately half of all clouds contained precipitation detectable as radar echoes below the cloud base. Radar and satellite observations show that clouds with tops from 1-11 km contribute more or less equally to surface-measured precipitation at Graciosa. A wide range of aerosol conditions was sampled during the deployment consistent with the diversity of sources as indicated by back-trajectory analysis. Preliminary findings suggest important two-way interactions between aerosols and clouds at Graciosa, with aerosols affecting light precipitation and cloud radiative properties while being controlled in part by precipitation scavenging.The data from Graciosa are being compared with short-range forecasts made with a variety of models. A pilot analysis with two climate and two weather forecast models shows that they reproduce the observed time-varying vertical structure of lower-tropospheric cloud fairly well but the cloud-nucleating aerosol concentrations less well. The Graciosa site has been chosen to be a permanent fixed ARM site that became operational in October 2013.« less

  9. Clouds, aerosol, and precipitation in the Marine Boundary Layer: An ARM mobile facility deployment

    SciTech Connect (OSTI)

    Wood, Robert; Luke, Ed; Wyant, Matthew; Bretherton, Christopher S.; Remillard, Jasmine; Kollias, Pavlos; Fletcher, Jennifer; Stemmler, Jayson; deSzoeke, S.; Yuter, Sandra; Miller, Matthew; Mechem, David; Tselioudis, George; Chiu, Christine; Mann, Julia; O Connor, Ewan; Hogan, Robin; Dong, Xiquan; Miller, Mark; Ghate, Virendra; Jefferson, Anne; Min, Qilong; Minnis, Patrick; Palinkonda, Rabindra; Albrecht, Bruce; Hannay, Cecile; Lin, Yanluan

    2014-04-27

    The Clouds, Aerosol, and Precipitation in the Marine Boundary Layer (CAP-MBL) deployment at Graciosa Island in the Azores generated a 21-month (April 2009-December 2010) comprehensive dataset documenting clouds, aerosols, and precipitation using the Atmospheric Radiation Measurement Program (ARM) Mobile Facility (AMF). The scientific aim of the deployment is to gain improved understanding of the interactions of clouds, aerosols, and precipitation in the marine boundary layer. Graciosa Island straddles the boundary between the subtropics and midlatitudes in the Northeast Atlantic Ocean and consequently experiences a great diversity of meteorological and cloudiness conditions. Low clouds are the dominant cloud type, with stratocumulus and cumulus occurring regularly. Approximately half of all clouds contained precipitation detectable as radar echoes below the cloud base. Radar and satellite observations show that clouds with tops from 1-11 km contribute more or less equally to surface-measured precipitation at Graciosa. A wide range of aerosol conditions was sampled during the deployment consistent with the diversity of sources as indicated by back-trajectory analysis. Preliminary findings suggest important two-way interactions between aerosols and clouds at Graciosa, with aerosols affecting light precipitation and cloud radiative properties while being controlled in part by precipitation scavenging.The data from Graciosa are being compared with short-range forecasts made with a variety of models. A pilot analysis with two climate and two weather forecast models shows that they reproduce the observed time-varying vertical structure of lower-tropospheric cloud fairly well but the cloud-nucleating aerosol concentrations less well. The Graciosa site has been chosen to be a permanent fixed ARM site that became operational in October 2013.

  10. Spectrometer for Sky-Scanning Sun-Tracking Atmospheric Research (4STAR): Instrument Technology

    SciTech Connect (OSTI)

    Dunagan, Stephen; Johnson, Roy; Zavaleta, Jhony; Russell, P. B.; Schmid, Beat; Flynn, Connor J.; Redemann, Jens; Shinozuka, Yohei; Livingston, J.; Segal Rozenhaimer, Michal

    2013-08-06

    The Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR) combines airborne sun tracking and sky scanning with diffraction spectroscopy, to improve knowledge of atmospheric constituents and their links to air-pollution/climate. Direct beam hyper-spectral measurement of optical depth improves retrievals of gas constituents and determination of aerosol properties. Sky scanning enhances retrievals of aerosol type and size distribution. 4STAR measurements will tighten the closure between satellite and ground-based measurements. 4STAR incorporates a modular sun-tracking/ sky-scanning optical head with fiber optic signal transmission to rack mounted spectrometers, permitting miniaturization of the external optical head, and future detector evolution. Technical challenges include compact optical collector design, radiometric dynamic range and stability, and broad spectral coverage. Test results establishing the performance of the instrument against the full range of operational requirements are presented, along with calibration, engineering flight test, and scientific field campaign data and results.

  11. Natural Radionuclides and Isotopic Signatures for Determining Carbonaceous Aerosol Sources, Aerosol Lifetimes, and Washout Processes

    SciTech Connect (OSTI)

    Gaffney, Jeffrey

    2012-12-12

    This is the final technical report. The project description is as follows: to determine the role of aerosol radiative forcing on climate, the processes that control their atmospheric concentrations must be understood, and aerosol sources need to be determined for mitigation. Measurements of naturally occurring radionuclides and stable isotopic signatures allow the sources, removal and transport processes, as well as atmospheric lifetimes of fine carbonaceous aerosols, to be evaluated.

  12. Aerosol characterization study using multi-spectrum remote sensing measurement techniques.

    SciTech Connect (OSTI)

    Glen, Crystal Chanea; Sanchez, Andres L.; Lucero, Gabriel Anthony; Schmitt, Randal L.; Johnson, Mark S.; Tezak, Matthew Stephen; Servantes, Brandon Lee

    2013-09-01

    A unique aerosol flow chamber coupled with a bistatic LIDAR system was implemented to measure the optical scattering cross sections and depolarization ratio of common atmospheric particulates. Each of seven particle types (ammonium sulfate, ammonium nitrate, sodium chloride, potassium chloride, black carbon and Arizona road dust) was aged by three anthropogenically relevant mechanisms: 1. Sulfuric acid deposition, 2. Toluene ozonolysis reactions, and 3. m-Xylene ozonolysis reactions. The results of pure particle scattering properties were compared with their aged equivalents. Results show that as most particles age under industrial plume conditions, their scattering cross sections are similar to pure black carbon, which has significant impacts to our understanding of aerosol impacts on climate. In addition, evidence emerges that suggest chloride-containing aerosols are chemically altered during the organic aging process. Here we present the direct measured scattering cross section and depolarization ratios for pure and aged atmospheric particulates.

  13. Sources and composition of submicron organic mass in marine aerosol particles: Marine Aerosol Organic Mass Composition

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Frossard, Amanda A.; Russell, Lynn M.; Burrows, Susannah M.; Elliott, Scott M.; Bates, Timothy S.; Quinn, Patricia K.

    2014-11-26

    Recent studies have proposed a variety of interpretations of the sources and composition of atmospheric marine aerosol particles (aMA) based on a range of physical and chemical measurements collected during open-ocean research cruises. To investigate the processes that affect marine organic particles, this study uses the characteristic functional group composition (from Fourier transform infrared (FTIR) spectroscopy) of aMAP from five ocean regions to show that: (i) The organic functional group composition of aMAP that can be identified as atmospheric primary marine (ocean-derived) aerosol (aPMA) is 6512% hydroxyl, 219% alkane, 66% amine, and 78% carboxylic acid functional groups. Contributions from photochemicalmorereactions add carboxylic acid groups (15%-25%), shipping effluent in seawater and ship emissions add additional alkane groups (up to 70%), and coastal emissions mix in alkane and carboxylic acid groups from coastal pollution sources. (ii) The organic composition of aPMA is nearly identical to model generated primary marine aerosol particles (gPMA) from bubbled seawater (55% hydroxyl, 32% alkane, and 13% amine functional groups), indicating that its overall functional group composition is the direct consequence of the organic constituents of the seawater source. (iii) While the seawater organic functional group composition was nearly invariant across all three ocean regions studied, the gPMA alkane group fraction increased with chlorophyll-a concentrations (r = 0.79). gPMA from productive seawater had a larger fraction of alkane functional groups (35%) compared to gPMA from non-productive seawater (16%), likely due to the presence of surfactants in productive seawater that stabilize the bubble film and lead to preferential drainage of the more soluble (lower alkane group fraction) organic components. gPMA has a hydroxyl group absorption peak location characteristic of monosaccharides and disaccharides, where the seawater OM hydroxyl group peak location is closer to that of polysaccharides. This may result from the larger saccharides preferentially remaining in the seawater during gPMA and aPMA productionless

  14. Lidar techniques for chemical and aerosol air pollution studies

    SciTech Connect (OSTI)

    Hardesty, R.M.

    1993-12-31

    At the Wave Propagation Laboratory (WPL), lidar methods are being applied in several areas of air pollution research. Differential absorption lidar (DIAL) systems for measuring ozone, ethylene, and other pollutants have been recently developed. The ozone instrument profiles ozone concentration in the boundary layer and lower troposphere to study sources, sinks, and transport of ozone. A goal is to combine DIAL and Doppler lidar techniques for measurement of the vertical fluxes of ozone and other pollutants. Doppler lidars have been also used at WPL to study visibility reduction caused by aerosol pollutants at the Grand Canyon, and to investigate dispersion of hazardous emissions near the Rocky Flats nuclear plant.

  15. Long-Term Measurements of Submicrometer Aerosol

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    non-refractory submicron particulate matter (NR-PM1) including organic aerosol (OA), sulfate (SO 4 2- ), nitrate (NO 3 - ), ammonium (NH 4 + ), and chloride (Cl-). In this study,...

  16. ARM - Field Campaign - Aerosol Lidar Validation Experiment -...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsAerosol Lidar Validation Experiment - ALIVE Campaign Links ALIVE Website ARM Data Discovery Browse Data Comments? We would love to hear from you Send us a note below...

  17. ARM - Evaluation Product - Aerosol Modeling Testbed

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    and satellite aerosol optical depth data is included to supplement and enhance the value of the CARES data. The software that is provided in AMT extracts model output from...

  18. Aerosol remote sensing in polar regions

    SciTech Connect (OSTI)

    Tomasi, Claudio; Kokhanovsky, Alexander A.; Lupi, Angelo; Ritter, Christoph; Smirnov, Alexander; O'Neill, Norman T.; Stone, Robert S.; Holben, Brent N.; Nyeki, Stephan; Mazzola, Mauro; Lanconelli, Christian; Vitale, Vito; Stebel, Kerstin; Aaltonen, Veijo; de Leeuw, Gerrit; Rodriguez, Edith; Herber, Andreas B.; Radionov, Vladimir F.; Zielinski, Tymon; Petelski, Tomasz; Sakerin, Sergey M.; Kabanov, Dmitry M.; Xue, Yong; Mei, Linlu; Istomina, Larysa; Wagener, Richard; McArthur, Bruce; Sobolewski, Piotr S.; Kivi, Rigel; Courcoux, Yann; Larouche, Pierre; Broccardo, Stephen; Piketh, Stuart J.

    2015-01-01

    Multi-year sets of ground-based sun-photometer measurements conducted at 12 Arctic sites and 9 Antarctic sites were examined to determine daily mean values of aerosol optical thickness ?(?) at visible and near-infrared wavelengths, from which best-fit values of ngstrm's exponent ? were calculated. Analysing these data, the monthly mean values of ?(0.50 ?m) and ? and the relative frequency histograms of the daily mean values of both parameters were determined for winterspring and summerautumn in the Arctic and for austral summer in Antarctica. The Arctic and Antarctic covariance plots of the seasonal median values of ? versus ?(0.50 ?m) showed: (i) a considerable increase in ?(0.50 ?m) for the Arctic aerosol from summer to winterspring, without marked changes in ?; and (ii) a marked increase in ?(0.50 ?m) passing from the Antarctic Plateau to coastal sites, whereas ? decreased considerably due to the larger fraction of sea-salt aerosol. Good agreement was found when comparing ground-based sun-photometer measurements of ?(?) and ? at Arctic and Antarctic coastal sites with Microtops measurements conducted during numerous AERONET/MAN cruises from 2006 to 2013 in three Arctic Ocean sectors and in coastal and off-shore regions of the Southern Atlantic, Pacific, and Indian Oceans, and the Antarctic Peninsula. Lidar measurements were also examined to characterise vertical profiles of the aerosol backscattering coefficient measured throughout the year at Ny-lesund. Satellite-based MODIS, MISR, and AATSR retrievals of ?(?) over large parts of the oceanic polar regions during spring and summer were in close agreement with ship-borne and coastal ground-based sun-photometer measurements. An overview of the chemical composition of mode particles is also presented, based on in-situ measurements at Arctic and Antarctic sites. Fourteen log-normal aerosol number size-distributions were defined to represent the average features of nuclei, accumulation and coarse mode particles for Arctic haze, summer background aerosol, Asian dust and boreal forest fire smoke, and for various background austral summer aerosol types at coastal and high-altitude Antarctic sites. The main columnar aerosol optical characteristics were determined for all 14 particle modes, based on in-situ measurements of the scattering and absorption coefficients. Diurnally averaged direct aerosol-induced radiative forcing and efficiency were calculated for a set of multimodal aerosol extinction models, using various Bidirectional Reflectance Distribution Function models over vegetation-covered, oceanic and snow-covered surfaces. These gave a reliable measure of the pronounced effects of aerosols on the radiation balance of the surfaceatmosphere system over polar regions.

  19. Aerosol fabrication methods for monodisperse nanoparticles

    DOE Patents [OSTI]

    Jiang, Xingmao; Brinker, C Jeffrey

    2014-10-21

    Exemplary embodiments provide materials and methods for forming monodisperse particles. In one embodiment, the monodisperse particles can be formed by first spraying a nanoparticle-containing dispersion into aerosol droplets and then heating the aerosol droplets in the presence of a shell precursor to form core-shell particles. By removing either the shell layer or the nanoparticle core of the core-shell particles, monodisperse nanoparticles can be formed.

  20. Collider Detector at Fermilab (CDF): Data from the QCD Group's Research into Properties of the Strong Interaction

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    ,

    The Collider Detector at Fermilab (CDF) is a Tevatron experiment at Fermilab. The Tevatron, a powerful particle accelerator, accelerates protons and antiprotons close to the speed of light, and then makes them collide head-on inside the CDF detector. The CDF detector is used to study the products of such collisions. The CDF Physics Group at Fermilab is organized into six working groups, each with a specific focus. The QCD group studies the properties of the strong interaction. Their public web page makes data and numerous figures available from both CDF Runs I and II.

  1. WRF-Chem Simulations of Aerosols and Anthropogenic Aerosol Radiative Forcing in East Asia

    SciTech Connect (OSTI)

    Gao, Yi; Zhao, Chun; Liu, Xiaohong; Zhang, Meigen; Leung, Lai-Yung R.

    2014-08-01

    This study aims to provide a first comprehensive evaluation of WRF-Chem for modeling aerosols and anthropogenic aerosol radiative forcing (RF) over East Asia. Several numerical experiments were conducted from November 2007 to December 2008. Comparison between model results and observations shows that the model can generally reproduce the observed spatial distributions of aerosol concentration, aerosol optical depth (AOD) and single scattering albedo (SSA) from measurements at different sites, including the relatively higher aerosol concentration and AOD over East China and the relatively lower AOD over Southeast Asia, Korean, and Japan. The model also depicts the seasonal variation and transport of pollutions over East Asia. Particulate matter of 10 um or less in the aerodynamic diameter (PM10), black carbon (BC), sulfate (SO42-), nitrate (NO3-) and ammonium (NH4+) concentrations are higher in spring than other seasons in Japan due to the pollutant transport from polluted area of East Asia. AOD is high over Southwest and Central China in winter, spring and autumn and over North China in summer while is low over South China in summer due to monsoon precipitation. SSA is lowest in winter and highest in summer. The model also captures the dust events at the Zhangye site in the semi-arid region of China. Anthropogenic aerosol RF is estimated to range from -5 to -20 W m-2 over land and -20 to -40 W m-2 over ocean at the top of atmosphere (TOA), 5 to 30 W m-2 in the atmosphere (ATM) and -15 to -40 W m-2 at the bottom (BOT). The warming effect of anthropogenic aerosol in ATM results from BC aerosol while the negative aerosol RF at TOA is caused by scattering aerosols such as SO4 2-, NO3 - and NH4+. Positive BC RF at TOA compensates 40~50% of the TOA cooling associated with anthropogenic aerosol.

  2. The First Aerosol Indirect Effect: Beyond Twomey

    SciTech Connect (OSTI)

    Liu, Y.; Dunn, M.; Daum, P.

    2008-03-10

    The traditional first aerosol indirect effect or the Twomey effect involves several fundamental assumptions. Some of the assumptions (e.g., constant liquid water content) are explicitly stated in studies of the Twomey effect whereas others are only implicitly embedded in the quantitative formulation. This work focuses on examining the implicit assumptions. In particular, we will show that anthropogenic pollution not only increases aerosol loading and droplet concentrations but also alters the relative dispersions of both the aerosol and subsequent droplet size distributions. The indirect effects resulting from the two altered relative dispersions (aerosol dispersion effect and droplet dispersion effect) are likely opposite in sign and proportional in magnitude to the conventional Twomey effect. This result suggests that the outstanding problems of the Twomey effect (i.e., large uncertainty and overestimation reported in literature) may lie with violation of the constant spectral shapes of aerosol and droplet size distributions implicitly assumed in evaluation of the Twomey effect, and therefore, further progress in understanding and quantification of the first aerosol indirect effect demands moving beyond the traditional paradigm originally conceived by Twomey.

  3. Development of a Fast Time-Resolved Aerosol Collector (Fast TRAC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Yu & James Cowin PNNL Fast Time-Resolved Aerosol Collector ......Fast TRAC...... Xiao-Ying Yu, Ali Hashim, Martin Iedema, and James Cowin Atmospheric Sciences, Chemical Sciences Pacific Northwest National Laboratory Richland, WA Research is supported by NOAA & DOE. *Patent Pending Xiao-Ying Yu & James Cowin PNNL Cloud Microstructures ≤ 1 m Want to know the aerosols at this resolution Aircraft flies at 150 m/s Need time resolution 1 m/150 m/s = 6 ms (!!!!!) Xiao-Ying Yu & James

  4. Development of a Fast Time-Resolved Aerosol Collector (Fast TRAC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Yu, James Cowin PNNL Probing Aerosols in Cloud Microstructures with Single Particle "Fast TRAC" Xiao-Ying Yu, Martin Iedema, and James Cowin Atmospheric Sciences, Chemical Sciences Pacific Northwest National Laboratory Richland, WA Research is supported by NOAA & DOE. *Patent Pending Xiao-Ying Yu, James Cowin PNNL Cloud Microstructures ≤ 1 m Want to know the aerosols at this resolution Aircraft flies at 150 m/s Need time resolution 1 m/150 m/s = 6 ms (!!!!!) Xiao-Ying Yu, James

  5. Impact of aerosol on mixed-phase stratocumulus during MPACE in a mesoscale

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    model with two-moment microphysics Impact of aerosol on mixed-phase stratocumulus during MPACE in a mesoscale model with two-moment microphysics Morrison, Hugh MMM/ASP National Center for Atmospheric Research Pinto, James University of Colorado Curry, Judith Georgia Institute of Technology Category: Modeling The Penn State/NCAR mesoscale model MM5 is coupled to a new microphysics scheme to examine the impact of aerosol on mixed-phase stratocumulus during the Mixed-Phase Arctic Stratus

  6. ARM Aerosol Working Group Meeting

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    series of retrieved dust properties, based on results from the AMF deployment in Niger, Africa. Lidar data survey Lidar profiles: fully-corrected MPL attenuated backscatter...

  7. Atmospheric Radiation Measurement (ARM) Data from Steamboat Springs, Colorado, for the Storm Peak Laboratory Cloud Property Validation Experiment (STORMVEX)

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    In October 2010, the initial deployment of the second ARM Mobile Facility (AMF2) took place at Steamboat Springs, Colorado, for the Storm Peak Laboratory Cloud Property Validation Experiment (STORMVEX). The objective of this field campaign was to obtain data about liquid and mixed-phase clouds using AMF2 instruments in conjunction with Storm Peak Laboratory (located at an elevation of 3220 meters on Mt. Werner), a cloud and aerosol research facility operated by the Desert Research Institute. STORMVEX datasets are freely available for viewing and download. Users are asked to register with the ARM Archive; the user's email address is used from that time forward as the login name.

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Area of Research: Cloud DistributionsCharacterizations Working Group(s): Cloud Properties Journal Reference: Wang X, KN Liou, SS Ou, GG Mace, and M Deng. 2009. "Remote sensing of ...

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Detection and Retrieval of Cirrus Clouds in the Tropics from AIRS: Validation from ARM Data Submitter: Yue, Q., Jet Propulsion Laboratory/California Institute of Technology Liou, K., University of California, Los Angeles Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Yue Q and KN Liou. 2009. "Cirrus cloud optical and microphysical properties determined from AIRS infrared spectra." Geophysical Research Letters, 36, L05810,

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Evaluation of Cloud Properties in Major Reanalyses Download a printable PDF Submitter: Liu, Y., Brookhaven National Laboratory Wu, W., Brookhaven National Laboratory Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle Journal Reference: Wu W, YG Liu, and AK Betts. 2012. "Observationally based evaluation of NWP reanalyses in modeling cloud properties over the Southern Great Plains." Journal of Geophysical Research - Atmospheres, 117, D12202,

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    A Climatology of Midlatitude Continental Cloud Properties and Their Impact on the Surface Radiation Budget Submitter: Dong, X., University of North Dakota Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Dong, X., P. Minnis, and B. Xi, 2005: A climatology of midlatitude continental clouds from ARM SGP site. Part I: Low-level Cloud Macrophysical, microphysical and radiative properties. J. Climate. 18, 1391-1410. Dong, X., B. Xi, and P.

  12. Evaluating Clouds, Aerosols, and their Interactions in Three Global Climate Models using COSP and Satellite Observations

    SciTech Connect (OSTI)

    Ban-Weiss, George; Jin, Ling; Bauer, S.; Bennartz, Ralph; Liu, Xiaohong; Zhang, Kai; Ming, Yi; Guo, Huan; Jiang, Jonathan

    2014-09-23

    Accurately representing aerosol-cloud interactions in global climate models is challenging. As parameterizations evolve, it is important to evaluate their performance with appropriate use of observations. In this work we compare aerosols, clouds, and their interactions in three climate models (AM3, CAM5, ModelE) to MODIS satellite observations. Modeled cloud properties were diagnosed using the CFMIP Observations Simulator Package (COSP). Cloud droplet number concentrations (N) were derived using the same algorithm for both satellite-simulated model values and observations. We find that aerosol optical depth tau simulated by models is similar to observations. For N, AM3 and CAM5 capture the observed spatial pattern of higher values in near-coast versus remote ocean regions, though modeled values in general are higher than observed. In contrast, ModelE simulates lower N in most near-coast versus remote regions. Aerosol- cloud interactions were computed as the sensitivity of N to tau for marine liquid clouds off the coasts of South Africa and Eastern Asia where aerosol pollution varies in time. AM3 and CAM5 are in most cases more sensitive than observations, while the sensitivity for ModelE is statistically insignificant. This widely used sensitivity could be subject to misinterpretation due to the confounding influence of meteorology on both aerosols and clouds. A simple framework for assessing the N tau sensitivity at constant meteorology illustrates that observed sensitivity can change from positive to statistically insignificant when including the confounding influence of relative humidity. Satellite simulated values of N were compared to standard model output and found to be higher with a bias of 83 cm-3.

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Measured Parameterization of Fire Aerosol Single Scattering Albedo Using Combustion Efficiency Download a printable PDF Submitter: Dubey, M. K., Los Alamos National Laboratory Area...

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Modeling Journal Reference: Tao, W.-K., X. Li, A. Khain, T. Matsui, S. Lang, and J. Simpson, 2007: The role of atmospheric aerosol concentration on deep convective...

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Analyzing the Contribution of Aerosols to an Observed Increase in Direct Normal Irradiance Download a printable PDF Submitter: Long, C. N., NOAA Global Monitoring DivisionCIRES...

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    function of liquid water path for all profiles through liquid-dominated cloud in clean (grey markers) and polluted (white markers) aerosol conditions. Flight dates flight numbers...

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Yang F, M Ovchinnikov, and RA Shaw. 2014. "Microphysical consequences of the spatial...

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Cloud-Aerosol-Precipitation Interactions Journal Reference: Qian Y, MY Huang, B Yang, and LK Berg. 2013. "A modeling study of irrigation effects on surface fluxes and...

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    of changing components in climate simulations (e.g., aerosols). The purpose of this study is to compute longwave radiative transfer results for the third phase of the...

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    organic aerosol and size distribution dynamics: Representing effects of volatility, phase state, and particle-phase reaction." Atmospheric Chemistry and Physics, 14, doi:10.5194...

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Download a printable PDF Submitter: Smith, J., University of California, Irvine ... Working Group(s): Aerosol Life Cycle Journal Reference: Smith JN, KC Barsanti, HR Friedli, ...

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Organic matter is a major contributor to total ambient aerosol load. Therefore, understanding its formation and removal is key to mitigate air pollution problems and climate ...

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    rates, and changes to liquid droplet nucleation and growth rates. Freezing point depression resulting from soluble material associated with aerosol particles was demonstrated...

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Life Cycle Journal Reference: Michalsky J, F Denn, C Flynn, G Hodges, P Kiedron, A Koontz, J Schlemmer, and SE Schwartz. 2010. "Climatology of aerosol optical depth in...

  5. Evaluate and characterize mechanisms controlling transport, fate, and effects of army smokes in the aerosol wind tunnel: Transport, transformations, fate, and terrestrial ecological effects of hexachloroethane obscurant smokes

    SciTech Connect (OSTI)

    Cataldo, D.A.; Ligotke, M.W.; Bolton, H. Jr.; Fellows, R.J.; Van Voris, P.; McVeety, B.D.; Li, Shu-mei W.; McFadden, K.M.

    1989-09-01

    The terrestrial transport, chemical fate, and ecological effects of hexachloroethane (HC) smoke were evaluated under controlled wind tunnel conditions. The primary objectives of this research program are to characterize and assess the impacts of smoke and obscurants on: (1) natural vegetation characteristic of US Army training sites in the United States; (2) physical and chemical properties of soils representative of these training sites; and (3) soil microbiological and invertebrate communities. Impacts and dose/responses were evaluated based on exposure scenarios, including exposure duration, exposure rate, and sequential cumulative dosing. Key to understanding the environmental impacts of HC smoke/obscurants is establishing the importance of environmental parameters such as relative humidity and wind speed on airborne aerosol characteristics and deposition to receptor surfaces. Direct and indirect biotic effects were evaluated using five plant species and two soil types. HC aerosols were generated in a controlled atmosphere wind tunnel by combustion of hexachloroethane mixtures prepared to simulate normal pot burn rates and conditions. The aerosol was characterized and used to expose plant, soil, and other test systems. Particle sizes of airborne HC ranged from 1.3 to 2.1 {mu}m mass median aerodynamic diameter (MMAD), and particle size was affected by relative humidity over a range of 20% to 85%. Air concentrations employed ranged from 130 to 680 mg/m{sup 3}, depending on exposure scenario. Chlorocarbon concentrations within smokes, deposition rates for plant and soil surfaces, and persistence were determined. The fate of principal inorganic species (Zn, Al, and Cl) in a range of soils was assessed.

  6. ARM - Publications: Science Team Meeting Documents: Aerosol Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ice cloud formation at unusually warm temperatures and low ice supersaturations (via deposition nucleation) involving transported Asian dust layers (as will be reported in Nature)...

  7. Aerosol beam-focus laser-induced plasma spectrometer device

    DOE Patents [OSTI]

    Cheng, Meng-Dawn (Oak Ridge, TN)

    2002-01-01

    An apparatus for detecting elements in an aerosol includes an aerosol beam focuser for concentrating aerosol into an aerosol beam; a laser for directing a laser beam into the aerosol beam to form a plasma; a detection device that detects a wavelength of a light emission caused by the formation of the plasma. The detection device can be a spectrometer having at least one grating and a gated intensified charge-coupled device. The apparatus may also include a processor that correlates the wavelength of the light emission caused by the formation of the plasma with an identity of an element that corresponds to the wavelength. Furthermore, the apparatus can also include an aerosol generator for forming an aerosol beam from bulk materials. A method for detecting elements in an aerosol is also disclosed.

  8. ARM - Field Campaign - Two-Column Aerosol Project (TCAP): Aerial...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsTwo-Column Aerosol Project (TCAP): Aerial Campaign ARM Data Discovery Browse Data Related Campaigns Two-Column Aerosol Project (TCAP) 2012.07.01, Berg, AMF Comments? We...

  9. Apparatus for rapid measurement of aerosol bulk chemical composition

    DOE Patents [OSTI]

    Lee, Yin-Nan E. (East Setauket, NY); Weber, Rodney J. (Atlanta, GA)

    2003-01-01

    An apparatus and method for continuous on-line measurement of chemical composition of aerosol particles with a fast time resolution are provided. The apparatus includes a modified particle size magnifier for producing activated aerosol particles and a collection device which collects the activated aerosol particles into a liquid stream for quantitative analysis by analytical methods. The method provided for on-line measurement of chemical composition of aerosol particles includes exposing aerosol carrying sample air to hot saturated steam thereby forming activated aerosol particles; collecting the activated aerosol particles by a collection device for delivery as a jet stream onto an impaction surface; flushing off the activated aerosol particles from the impaction surface into a liquid stream for delivery of the collected liquid stream to an analytical instrument for quantitative measurement.

  10. Apparatus for rapid measurement of aerosol bulk chemical composition

    DOE Patents [OSTI]

    Lee, Yin-Nan E.; Weber, Rodney J.; Orsini, Douglas

    2006-04-18

    An apparatus for continuous on-line measurement of chemical composition of aerosol particles with a fast time resolution is provided. The apparatus includes an enhanced particle size magnifier for producing activated aerosol particles and an enhanced collection device which collects the activated aerosol particles into a liquid stream for quantitative analysis by analytical means. Methods for on-line measurement of chemical composition of aerosol particles are also provided, the method including exposing aerosol carrying sample air to hot saturated steam thereby forming activated aerosol particles; collecting the activated aerosol particles by a collection device for delivery as a jet stream onto an impaction surface; and flushing off the activated aerosol particles from the impaction surface into a liquid stream for delivery of the collected liquid stream to an analytical instrument for quantitative measurement.

  11. Vertical Variability of Aerosols and Water Vapor Over the Southern Great Plains

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Vertical Variability of Aerosols and Water Vapor Over the Southern Great Plains R. A. Ferrare National Aeronautics and Space Administration Langley Research Center Hampton, Virginia D. D. Turner Pacific Northwest National Laboratory Richland, Washington M. Clayton and V. Brackett Science Applications International Corporation National Aeronautics and Space Administration Langley Research Center Hampton, Virginia T. P. Tooman and J. E. M. Goldsmith Sandia National Laboratories Livermore,

  12. Aerodyne Develops an Aircraft-Deployable Precision Aerosol Analyzer | U.S.

    Office of Science (SC) Website

    DOE Office of Science (SC) Aerodyne Develops an Aircraft-Deployable Precision Aerosol Analyzer Small Business Innovation Research (SBIR) and Small Business Technology Transfer (STTR) SBIR/STTR Home About Funding Opportunity Announcements (FOAs) Applicant and Awardee Resources Commercialization Assistance Other Resources Awards SBIR/STTR Highlights Reporting Fraud Contact Information Small Business Innovation Research and Small Business Technology Transfer U.S. Department of Energy

  13. Study of Mechanisms of Aerosol Indirect Effects on Glaciated Clouds: Progress during the Project Final Technical Report

    SciTech Connect (OSTI)

    2013-10-18

    This 3-year project has studied how aerosol pollution influences glaciated clouds. The tool applied has been an 'aerosol-cloud model'. It is a type of Cloud-System Resolving Model (CSRM) modified to include 2-moment bulk microphysics and 7 aerosol species, as described by Phillips et al. (2009, 2013). The study has been done by, first, improving the model and then performing sensitivity studies with validated simulations of a couple of observed cases from ARM. These are namely the Tropical Warm Pool International Cloud Experiment (TWP-ICE) over the tropical west Pacific and the Cloud and Land Surface Interaction Campaign (CLASIC) over Oklahoma. During the project, sensitivity tests with the model showed that in continental clouds, extra liquid aerosols (soluble aerosol material) from pollution inhibited warm rain processes for precipitation production. This promoted homogeneous freezing of cloud droplets and aerosols. Mass and number concentrations of cloud-ice particles were boosted. The mean sizes of cloud-ice particles were reduced by the pollution. Hence, the lifetime of glaciated clouds, especially ice-only clouds, was augmented due to inhibition of sedimentation and ice-ice aggregation. Latent heat released from extra homogeneous freezing invigorated convective updrafts, and raised their maximum cloud-tops, when aerosol pollution was included. In the particular cases simulated in the project, the aerosol indirect effect of glaciated clouds was twice than of (warm) water clouds. This was because glaciated clouds are higher in the troposphere than water clouds and have the first interaction with incoming solar radiation. Ice-only clouds caused solar cooling by becoming more extensive as a result of aerosol pollution. This 'lifetime indirect effect' of ice-only clouds was due to higher numbers of homogeneously nucleated ice crystals causing a reduction in their mean size, slowing the ice-crystal process of snow production and slowing sedimentation. In addition to the known indirect effects (glaciation, riming and thermodynamic), new indirect effects were discovered and quantified due to responses of sedimentation, aggregation and coalescence in glaciated clouds to changing aerosol conditions. In summary, the change in horizontal extent of the glaciated clouds ('lifetime indirect effects'), especially of ice-only clouds, was seen to be of higher importance in regulating aerosol indirect effects than changes in cloud properties ('cloud albedo indirect effects').

  14. he Impact of Primary Marine Aerosol on Atmospheric Chemistry, Radiation and Climate: A CCSM Model Development Study

    SciTech Connect (OSTI)

    Keene, William C.; Long, Michael S.

    2013-05-20

    This project examined the potential large-scale influence of marine aerosol cycling on atmospheric chemistry, physics and radiative transfer. Measurements indicate that the size-dependent generation of marine aerosols by wind waves at the ocean surface and the subsequent production and cycling of halogen-radicals are important but poorly constrained processes that influence climate regionally and globally. A reliable capacity to examine the role of marine aerosol in the global-scale atmospheric system requires that the important size-resolved chemical processes be treated explicitly. But the treatment of multiphase chemistry across the breadth of chemical scenarios encountered throughout the atmosphere is sensitive to the initial conditions and the precision of the solution method. This study examined this sensitivity, constrained it using high-resolution laboratory and field measurements, and deployed it in a coupled chemical-microphysical 3-D atmosphere model. First, laboratory measurements of fresh, unreacted marine aerosol were used to formulate a sea-state based marine aerosol source parameterization that captured the initial organic, inorganic, and physical conditions of the aerosol population. Second, a multiphase chemical mechanism, solved using the Max Planck Institute for Chemistry??s MECCA (Module Efficiently Calculating the Chemistry of the Atmosphere) system, was benchmarked across a broad set of observed chemical and physical conditions in the marine atmosphere. Using these results, the mechanism was systematically reduced to maximize computational speed. Finally, the mechanism was coupled to the 3-mode modal aerosol version of the NCAR Community Atmosphere Model (CAM v3.6.33). Decadal-scale simulations with CAM v.3.6.33, were run both with and without reactive-halogen chemistry and with and without explicit treatment of particulate organic carbon in the marine aerosol source function. Simulated results were interpreted (1) to evaluate influences of marine aerosol production on the microphysical properties of aerosol populations and clouds over the ocean and the corresponding direct and indirect effects on radiative transfer; (2) atmospheric burdens of reactive halogen species and their impacts on O3, NOx, OH, DMS, and particulate non-sea-salt SO42-; and (3) the global production and influences of marine-derived particulate organic carbon. The model reproduced major characteristics of the marine aerosol system and demonstrated the potential sensitivity of global, decadal-scale climate metrics to multiphase marine-derived components of Earth??s troposphere. Due to the combined computational burden of the coupled system, the currently available computational resources were the limiting factor preventing the adequate statistical analysis of the overall impact that multiphase chemistry might have on climate-scale radiative transfer and climate.

  15. Long-term Measurements of Submicrometer Aerosol Chemistry at the Southern Great Plains (SGP) Using an Aerosol Chemical Speciation Monitor (ACSM)

    SciTech Connect (OSTI)

    Parworth, Caroline; Fast, Jerome D.; Mei, Fan; Shippert, Timothy R.; Sivaraman, Chitra; Tilp, Alison; Watson, Thomas; Zhang, Qi

    2015-04-01

    In this study the long-term trends of non-refractory submicrometer aerosol (NR-PM1) composition and mass concentration measured by an Aerosol Chemical Speciation Monitor (ACSM) at the U.S. Department of Energy’s Southern Great Plains (SGP) site are discussed. Over the period of 19 months (Nov. 20, 2010 – June 2012) highly time resolved (~30 min.) NR-PM1 data was recorded. Using this dataset the value-added product (VAP) of deriving organic aerosol components (OACOMP) is introduced. With this VAP, multivariate analysis of the measured organic mass spectral matrix can be performed on long term data to return organic aerosol (OA) factors that are associated with distinct sources, evolution processes, and physiochemical properties. Three factors were obtained from this VAP including two oxygenated OA (OOA) factors, differing in degrees of oxidation, and a biomass burning OA (BBOA) factor. Back trajectory analyses were performed to investigate possible sources of major NR-PM1 species at the SGP site. Organics dominated NR-PM1 mass concentration for the majority of the study with the exception of winter, when nitrate increased due to transport of precursor species from surrounding urban and agricultural areas and also due to cooler temperatures. Sulfate mass concentrations showed little seasonal variation with mixed regional and local sources. In the spring BBOA emissions increased and were mainly associated with local fires. Isoprene and carbon monoxide emission rates were computed by the Model of Emissions of Gases and Aerosols from Nature (MEGAN) to represent the spatial distribution of biogenic and anthropogenic sources, respectively. From this model there is evidence to support that biogenic emissions from the southeast contribute to SOA formation at the SGP site during the summer.

  16. Aerosol can puncture device test report

    SciTech Connect (OSTI)

    Leist, K.J.

    1994-10-01

    This test report documents the evaluation of an aerosol can puncture device to replace a system currently identified for use in the WRAP-1 facility. The new system is based upon a commercially available puncture device, as recommended by WHC Fire Protection. With modifications found necessary through the testing program, the Aerosol Can Puncture Device was found able to puncture and drain aerosol cans without incident. Modifications include the addition of a secondary collection bottle and the modification of the can puncture needle. In the course of testing, a variety of absorbents were tested to determine their performance in immobilizing drained fluids. The visibility of the puncture with Non-Destructive Examination techniques were also reviewed.

  17. Aerosol Radiative Effects and Single-Scattering Properties in...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Institution of Oceanography University of California San Diego, California M. A. Miller, M. J. Bartholomew, and R. M. Reynolds Brookhaven National Laboratory Upton, New York...

  18. Apparatus for sampling and characterizing aerosols

    DOE Patents [OSTI]

    Dunn, Patrick F. (Downers Grove, IL); Herceg, Joseph E. (Naperville, IL); Klocksieben, Robert H. (Park Forest, IL)

    1986-01-01

    Apparatus for sampling and characterizing aerosols having a wide particle size range at relatively low velocities may comprise a chamber having an inlet and an outlet, the chamber including: a plurality of vertically stacked, successive particle collection stages; each collection stage includes a separator plate and a channel guide mounted transverse to the separator plate, defining a labyrinthine flow path across the collection stage. An opening in each separator plate provides a path for the aerosols from one collection stage to the next. Mounted within each collection stage are one or more particle collection frames.

  19. ARM - PI Product - Niamey Aerosol Optical Depths

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Optical Depths ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send PI Product : Niamey Aerosol Optical Depths MFRSR irradiance data collected during the ACRF AMF deployment in Niamey, Niger have been used to derive AOD for five wavelength channels of the MFRSR. These data have been corrected to adjust for filter drift over the course of the campaign and contamination due to forward scattering as a result of

  20. Surrogate/spent fuel sabotage aerosol ratio testing:phase 1 summary and results.

    SciTech Connect (OSTI)

    Vigil, Manuel Gilbert; Sorenson, Ken Bryce; Lange, F. , Germany); Nolte, O. (Fraunhofer Institut fur Toxikologie und Experimentelle Medizin, Germany); Koch, W. (Fraunhofer Institut fur Toxikologie und Experimentelle Medizin, Germany); Dickey, Roy R.; Yoshimura, Richard Hiroyuki; Molecke, Martin Alan; Autrusson, Bruno (Institut de Radioprotection et de Surete Nucleaire , France); Young, F. I.; Pretzsch, Gunter Guido (Gesellschaft fur Anlagen- und reaktorsicherheit , Germany)

    2005-10-01

    This multinational test program is quantifying the aerosol particulates produced when a high energy density device (HEDD) impacts surrogate material and actual spent fuel test rodlets. The experimental work, performed in four consecutive test phases, has been in progress for several years. The overall program provides needed data that are relevant to some sabotage scenarios in relation to spent fuel transport and storage casks, and associated risk assessments. This program also provides significant political benefits in international cooperation for nuclear security related evaluations. The spent fuel sabotage--aerosol test program is coordinated with the international Working Group for Sabotage Concerns of Transport and Storage Casks (WGSTSC), and supported by both the U.S. Department of Energy and Nuclear Regulatory Commission. This report summarizes the preliminary, Phase 1 work performed in 2001 and 2002 at Sandia National Laboratories and the Fraunhofer Institute, Germany, and documents the experimental results obtained, observations, and preliminary interpretations. Phase 1 testing included: performance quantifications of the HEDD devices; characterization of the HEDD or conical shaped charge (CSC) jet properties with multiple tests; refinement of the aerosol particle collection apparatus being used; and, CSC jet-aerosol tests using leaded glass plates and glass pellets, serving as representative brittle materials. Phase 1 testing was quite important for the design and performance of the following Phase 2 test program and test apparatus.

  1. Aerosol remote sensing in polar regions

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Tomasi, Claudio; Kokhanovsky, Alexander A.; Lupi, Angelo; Ritter, Christoph; Smirnov, Alexander; O'Neill, Norman T.; Stone, Robert S.; Holben, Brent N.; Nyeki, Stephan; Wehrli, Christoph; et al

    2015-01-01

    Multi-year sets of ground-based sun-photometer measurements conducted at 12 Arctic sites and 9 Antarctic sites were examined to determine daily mean values of aerosol optical thickness τ(λ) at visible and near-infrared wavelengths, from which best-fit values of Ångström's exponent α were calculated. Analysing these data, the monthly mean values of τ(0.50 μm) and α and the relative frequency histograms of the daily mean values of both parameters were determined for winter–spring and summer–autumn in the Arctic and for austral summer in Antarctica. The Arctic and Antarctic covariance plots of the seasonal median values of α versus τ(0.50 μm) showed: (i)more » a considerable increase in τ(0.50 μm) for the Arctic aerosol from summer to winter–spring, without marked changes in α; and (ii) a marked increase in τ(0.50 μm) passing from the Antarctic Plateau to coastal sites, whereas α decreased considerably due to the larger fraction of sea-salt aerosol. Good agreement was found when comparing ground-based sun-photometer measurements of τ(λ) and α at Arctic and Antarctic coastal sites with Microtops measurements conducted during numerous AERONET/MAN cruises from 2006 to 2013 in three Arctic Ocean sectors and in coastal and off-shore regions of the Southern Atlantic, Pacific, and Indian Oceans, and the Antarctic Peninsula. Lidar measurements were also examined to characterise vertical profiles of the aerosol backscattering coefficient measured throughout the year at Ny-Ålesund. Satellite-based MODIS, MISR, and AATSR retrievals of τ(λ) over large parts of the oceanic polar regions during spring and summer were in close agreement with ship-borne and coastal ground-based sun-photometer measurements. An overview of the chemical composition of mode particles is also presented, based on in-situ measurements at Arctic and Antarctic sites. Fourteen log-normal aerosol number size-distributions were defined to represent the average features of nuclei, accumulation and coarse mode particles for Arctic haze, summer background aerosol, Asian dust and boreal forest fire smoke, and for various background austral summer aerosol types at coastal and high-altitude Antarctic sites. The main columnar aerosol optical characteristics were determined for all 14 particle modes, based on in-situ measurements of the scattering and absorption coefficients. Diurnally averaged direct aerosol-induced radiative forcing and efficiency were calculated for a set of multimodal aerosol extinction models, using various Bidirectional Reflectance Distribution Function models over vegetation-covered, oceanic and snow-covered surfaces. These gave a reliable measure of the pronounced effects of aerosols on the radiation balance of the surface–atmosphere system over polar regions.« less

  2. Long-term measurements of submicrometer aerosol chemistry at the Southern Great Plains (SGP) using an Aerosol Chemical Speciation Monitor (ACSM)

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Parworth, Caroline; Tilp, Alison; Fast, Jerome; Mei, Fan; Shippert, Tim; Sivaraman, Chitra; Watson, Thomas; Zhang, Qi

    2015-04-01

    In this study the long-term trends of non-refractory submicrometer aerosol (NR-PM1) composition and mass concentration measured by an Aerosol Chemical Speciation Monitor (ACSM) at the Atmospheric Radiation Measurement (ARM) program's Southern Great Plains (SGP) site are discussed. NR-PM1 data was recorded at ~30 min intervals over a period of 19 months between November 2010 and June 2012. Positive Matrix Factorization (PMF) was performed on the measured organic mass spectral matrix using a rolling window technique to derive factors associated with distinct sources, evolution processes, and physiochemical properties. The rolling window approach also allows us to capture the dynamic variations ofmore » the chemical properties in the organic aerosol (OA) factors over time. Three OA factors were obtained including two oxygenated OA (OOA) factors, differing in degrees of oxidation, and a biomass burning OA (BBOA) factor. Back trajectory analyses were performed to investigate possible sources of major NR-PM1 species at the SGP site. Organics dominated NR-PM1 mass concentration for the majority of the study with the exception of winter, when ammonium nitrate increases due to transport of precursor species from surrounding urban and agricultural areas and also due to cooler temperatures. Sulfate mass concentrations have little seasonal variation with mixed regional and local sources. In the spring BBOA emissions increase and are mainly associated with local fires. Isoprene and carbon monoxide emission rates were obtained by the Model of Emissions of Gases and Aerosols from Nature (MEGAN) and the 2011 U.S. National Emissions Inventory to represent the spatial distribution of biogenic and anthropogenic sources, respectively. The combined spatial distribution of isoprene emissions and air mass trajectories suggest that biogenic emissions from the southeast contribute to SOA formation at the SGP site during the summer.« less

  3. Long-term measurements of submicrometer aerosol chemistry at the Southern Great Plains (SGP) using an Aerosol Chemical Speciation Monitor (ACSM)

    SciTech Connect (OSTI)

    Parworth, Caroline; Tilp, Alison; Fast, Jerome; Mei, Fan; Shippert, Tim; Sivaraman, Chitra; Watson, Thomas; Zhang, Qi

    2015-04-01

    In this study the long-term trends of non-refractory submicrometer aerosol (NR-PM1) composition and mass concentration measured by an Aerosol Chemical Speciation Monitor (ACSM) at the Atmospheric Radiation Measurement (ARM) program's Southern Great Plains (SGP) site are discussed. NR-PM1 data was recorded at ~30 min intervals over a period of 19 months between November 2010 and June 2012. Positive Matrix Factorization (PMF) was performed on the measured organic mass spectral matrix using a rolling window technique to derive factors associated with distinct sources, evolution processes, and physiochemical properties. The rolling window approach also allows us to capture the dynamic variations of the chemical properties in the organic aerosol (OA) factors over time. Three OA factors were obtained including two oxygenated OA (OOA) factors, differing in degrees of oxidation, and a biomass burning OA (BBOA) factor. Back trajectory analyses were performed to investigate possible sources of major NR-PM1 species at the SGP site. Organics dominated NR-PM1 mass concentration for the majority of the study with the exception of winter, when ammonium nitrate increases due to transport of precursor species from surrounding urban and agricultural areas and also due to cooler temperatures. Sulfate mass concentrations have little seasonal variation with mixed regional and local sources. In the spring BBOA emissions increase and are mainly associated with local fires. Isoprene and carbon monoxide emission rates were obtained by the Model of Emissions of Gases and Aerosols from Nature (MEGAN) and the 2011 U.S. National Emissions Inventory to represent the spatial distribution of biogenic and anthropogenic sources, respectively. The combined spatial distribution of isoprene emissions and air mass trajectories suggest that biogenic emissions from the southeast contribute to SOA formation at the SGP site during the summer.

  4. Two Hundred Fifty Years of Aerosols and Climate: The End of the Age of Aerosols

    SciTech Connect (OSTI)

    Smith, Steven J.; Bond, Tami C.

    2014-01-20

    Carbonaceous and sulfur aerosols have a substantial global and regional influence on climate in addition to their impact on health and ecosystems. The magnitude of this influence has changed substantially over the past and is expected to continue to change into the future. An integrated picture of the changing climatic influence of black carbon, organic carbon and sulfate over the period 1850 through 2100, focusing on uncertainty, is presented using updated historical inventories and a coordinated set of emission projections. While aerosols have had a substantial impact on climate over the past century, by the end of the 21st century aerosols will likely be only a minor contributor to radiative forcing due to increases in greenhouse gas forcing and a global decrease in pollutant emissions. This outcome is even more certain under a successful implementation of a policy to limit greenhouse gas emissions as low-carbon energy technologies that do not emit appreciable aerosol or SO2 are deployed.

  5. Near real time vapor detection and enhancement using aerosol adsorption

    DOE Patents [OSTI]

    Novick, V.J.; Johnson, S.A.

    1999-08-03

    A vapor sample detection method is described where the vapor sample contains vapor and ambient air and surrounding natural background particles. The vapor sample detection method includes the steps of generating a supply of aerosol that have a particular effective median particle size, mixing the aerosol with the vapor sample forming aerosol and adsorbed vapor suspended in an air stream, impacting the suspended aerosol and adsorbed vapor upon a reflecting element, alternatively directing infrared light to the impacted aerosol and adsorbed vapor, detecting and analyzing the alternatively directed infrared light in essentially real time using a spectrometer and a microcomputer and identifying the vapor sample. 13 figs.

  6. Near real time vapor detection and enhancement using aerosol adsorption

    DOE Patents [OSTI]

    Novick, Vincent J. (Downers Grove, IL); Johnson, Stanley A. (Countryside, IL)

    1999-01-01

    A vapor sample detection method where the vapor sample contains vapor and ambient air and surrounding natural background particles. The vapor sample detection method includes the steps of generating a supply of aerosol that have a particular effective median particle size, mixing the aerosol with the vapor sample forming aerosol and adsorbed vapor suspended in an air stream, impacting the suspended aerosol and adsorbed vapor upon a reflecting element, alternatively directing infrared light to the impacted aerosol and adsorbed vapor, detecting and analyzing the alternatively directed infrared light in essentially real time using a spectrometer and a microcomputer and identifying the vapor sample.

  7. Custom data support for the FAst -physics System Testbed and Research (FASTER) Project

    SciTech Connect (OSTI)

    Toto, T.; Jensen, M.; Vogelmann, A.; Wagener, R.; Liu, Y.; Lin, W.

    2010-03-15

    The multi-institution FAst -physics System Testbed and Research (FASTER) project, funded by the DOE Earth System Modeling program, aims to evaluate and improve the parameterizations of fast processes (those involving clouds, precipitation and aerosols) in global climate models, using a combination of numerical prediction models, single column models, cloud resolving models, large-eddy simulations, full global climate model output and ARM active and passive remote sensing and in-situ data. This poster presents the Custom Data Support effort for the FASTER project. The effort will provide tailored datasets, statistics, best estimates and quality control data, as needed and defined by FASTER participants, for use in evaluating and improving parameterizations of fast processes in GCMs. The data support will include custom gridding and averaging, for the model of interest, using high time resolution and pixel level data from continuous ARM observations and complementary datasets. In addition to the FASTER team, these datasets will be made available to the ARM Science Team. Initial efforts with respect to data product development, priorities, availability and distribution are summarized here with an emphasis on cloud, atmospheric state and aerosol properties as observed during the Spring 2000 Cloud IOP and the Spring 2003 Aerosol IOP at the ARM Southern Great Plains site.

  8. Radiological/biological/aerosol removal system

    DOE Patents [OSTI]

    Haslam, Jeffery J

    2015-03-17

    An air filter replacement system for existing buildings, vehicles, arenas, and other enclosed airspaces includes a replacement air filter for replacing a standard air filter. The replacement air filter has dimensions and air flow specifications that allow it to replace the standard air filter. The replacement air filter includes a filter material that removes radiological or biological or aerosol particles.

  9. Atmospheric Radiation Measurement (ARM) Data from Shouxian, China for the Study of Aerosol Indirect Effects in China

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    In a complex ARM Mobile Facility (AMF) deployment, monitoring data was collected at four locations in China during 2008. The various sites are located in regions with different climate regimes and with high aerosol loadings of different optical, physical, and chemical properties. Measurements obtained at all the AMF sites during the 8-month deployment in China will help scientists to validate satellite-based findings, understand the mechanisms of the aerosol indirect effects in the region, and examine the roles of aerosols in affecting regional climate and atmospheric circulation, with a special focus on the impact of the East Asian monsoon system. As with other collections from the ARM Mobile Facility, the datasets are available from the ARM Archive. The ARM Archive physically resides at the Oak Ridge National Laboratory.

  10. Technology Solutions Case Study: Apartment Compartmentalization with an Aerosol-Based Sealing Process

    SciTech Connect (OSTI)

    2015-07-01

    Air sealing of building enclosures is a difficult and time-consuming process. Current methods in new construction require laborers to physically locate small and sometimes large holes in multiple assemblies and then manually seal each of them. This research study by Building America team Consortium for Advanced Residential Buildings demonstrated the automated air sealing and compartmentalization of buildings through the use of an aerosolized sealant developed by the Western Cooling Efficiency Center at University of California Davis. CARB demonstrated this new technology application in a multifamily building in Queens, NY. The effectiveness of the sealing process was evaluated by three methods: air leakage testing of overall apartment before and after sealing, point-source testing of individual leaks, and pressure measurements in the walls of the target apartment during sealing. Aerosolized sealing was successful by several measures in this study. Many individual leaks that are labor-intensive to address separately were well sealed by the aerosol particles. In addition, many diffuse leaks that are difficult to identify and treat were also sealed. The aerosol-based sealing process resulted in an average reduction of 71% in air leakage across three apartments and an average apartment airtightness of 0.08 CFM50/SF of enclosure area.

  11. Clouds, Aerosol, and Precipitation in the Marine Boundary Layer (CAP-MBL) Final Campaign Report

    SciTech Connect (OSTI)

    Wood, R.

    2016-01-01

    The extensive coverage of low clouds over the subtropical eastern oceans greatly impacts the current climate. In addition, the response of low clouds to changes in atmospheric greenhouse gases and aerosols is a major source of uncertainty, which thwarts accurate prediction of future climate change. Low clouds are poorly simulated in climate models, partly due to inadequate long-term simultaneous observations of their macrophysical and microphysical structure, radiative effects, and associated aerosol distribution in regions where their impact is greatest. The thickness and extent of subtropical low clouds is dependent on tight couplings between surface fluxes of heat and moisture, radiative cooling, boundary layer turbulence, and precipitation (much of which evaporates before reaching the ocean surface and is closely connected to the abundance of cloud condensation nuclei). These couplings have been documented as a result of past field programs and model studies. However, extensive research is still required to achieve a quantitative understanding sufficient for developing parameterizations, which adequately predict aerosol indirect effects and low cloud response to climate perturbations. This is especially true of the interactions between clouds, aerosol, and precipitation. These processes take place in an ever-changing synoptic environment that can confound interpretation of short time period observations.

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Significance of Multilayer Cloud Systems in Tropical Convection Download a printable PDF Submitter: Stephens, G. L., Colorado State University Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Stephens, GL, and NB Wood. 2007. "Properties of tropical convection observed by millimeter-wave radar systems." Monthly Weather Review 135: 821-842. Storm classifications (derived from k-means clustering analysis) applied to MWR

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Validation of Climate Model Ice Cloud Properties Download a printable PDF Submitter: Eidhammer, T., NCAR Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle Journal Reference: Eidhammer T, H Morrison, A Bansemer, A Gettelman, and AJ Heymsfield. 2014. "Comparison of ice cloud properties simulated by the Community Atmosphere Model (CAM5) with in situ observations." Atmospheric Chemistry and Physics, 14(18), doi:10.5194/acp-14-10103-2014. Mass weighted terminal fall

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    DCS Ice Cloud Microphysical Properties Derived from Aircraft Data During MC3E Submitter: Dong, X., University of North Dakota Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle Journal Reference: Wang J, X Dong, and B Xi. 2015. "Investigation of ice cloud microphysical properties of DCSs using aircraft in situ measurements during MC3E over the ARM SGP site." Journal of Geophysical Research - Atmospheres, 120(8), 3533-3552. Figure 1. The observed PSDs at different

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Observations of Microphysical Properties of Single Layer Stratocumulus During the Mixed-Phase Arctic Cloud Experiment Submitter: McFarquhar, G., University of Illinois, Urbana Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Fridlind, A.M., A.S. Ackerman, G.M. McFarquhar, G. Zhang, M.R. Poellot, P.J. DeMott, A.J. Prenni and A.J. Heymsfield, 2007: Ice properties of single-layer stratocumulus during the Mixed-Phase Arctic Cloud

  16. Apartment Compartmentalization With an Aerosol-Based Sealing Process

    SciTech Connect (OSTI)

    Maxwell, S.; Berger, D.; Harrington, C.

    2015-03-01

    Air sealing of building enclosures is a difficult and time-consuming process. Current methods in new construction require laborers to physically locate small and sometimes large holes in multiple assemblies and then manually seal each of them. The innovation demonstrated under this research study was the automated air sealing and compartmentalization of buildings through the use of an aerosolized sealant, developed by the Western Cooling Efficiency Center at University of California Davis. CARB sought to demonstrate this new technology application in a multifamily building in Queens, NY. The effectiveness of the sealing process was evaluated by three methods: air leakage testing of overall apartment before and after sealing, point-source testing of individual leaks, and pressure measurements in the walls of the target apartment during sealing.

  17. The ARM Climate Research Facility: A Review of Structure and Capabilities

    SciTech Connect (OSTI)

    Mather, James H.; Voyles, Jimmy W.

    2013-03-01

    The Atmospheric Radiation Measurement (ARM) program (www.arm.gov) is a Department of Energy, Office of Science, climate research user facility that provides atmospheric observations from diverse climatic regimes around the world. Use of ARM data is free and available to anyone through the ARM data archive. ARM is approaching 20 years of operations. In recent years, the facility has grown to add two mobile facilities and an aerial facility to its network of fixed-location sites. Over the past year, ARM has enhanced its observational capabilities with a broad array of new instruments at its fixed and mobile sites and the aerial facility. Instruments include scanning millimeter- and centimeter-wavelength radars; water vapor, cloud/aerosol extinction, and Doppler lidars; a suite of aerosol instruments for measuring optical, physical, and chemical properties; instruments including eddy correlation systems to expand measurements of the surface and boundary layer; and aircraft probes for measuring cloud and aerosol properties. Taking full advantage of these instruments will involve the development of complex data products. This work is underway but will benefit from engagement with the broader scientific community. In this article we will describe the current status of the ARM program with an emphasis on developments over the past eight years since ARM was designated a DOE scientific user facility. We will also describe the new measurement capabilities and provide thoughts for how these new measurements can be used to serve the climate research community with an invitation to the community to engage in the development and use of these data products.

  18. ARM Climate Research Facility

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ... 3 2.4 Aerosol Observing System Humidified Tandem Differential Mobility Analyzer (AOS- HTDMA) ......

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Threshold Radar Reflectivity Separating Precipitating from Non-Precipitating Clouds Download a printable PDF Submitter: Liu, Y., Brookhaven National Laboratory Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Liu, Y, B Geerts, PH Daum, R McGraw, and M Miller. 2008. "Threshold radar reflectivity for drizzling clouds." Geophysical Research Letters 35, L03807, doi:10.1029/2007GL031201. Figure 1 shows the comparison of the

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Small Ice Crystals on Ice Sedimentation Rates in Cirrus Clouds and GCM Simulations Download a printable PDF Submitter: Mitchell, D. L., Desert Research Institute Rasch, P., Pacific Northwest National Laboratory Ivanova, D., Embry-Riddle Aeronautical University McFarquhar, G., University of Illinois, Urbana Nousiainen, T. P., University of Helsinki Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Cloud Properties Journal Reference: Mitchell, DL, P

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Surprisingly Large Contribution of Small Marine Clouds to Cloud Fraction and Reflectance Download a printable PDF Submitter: Oreopoulos, L., NASA Feingold, G., NOAA - Earth System Research Laboratory Koren, I., Weizmann Institute of Science Remer, L., NASA - GSFC, Laboratory for Atmospheres Area of Research: Clouds with Low Optical [Water] Depths (CLOWD) Working Group(s): Cloud Properties Journal Reference: Koren, I, L Oreopoulos, G Feingold, LA Remer, and O Altaratz. 2008. "How small

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Thin Is In Download a printable PDF Submitter: Tomlinson, J., Pacific Northwest National Laboratory Long, C. N., NOAA Global Monitoring Division/CIRES Comstock, J. M., Pacific Northwest National Laboratory Ronfeld, D., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Cloud Properties Journal Reference: N/A The Twin Otter takes off to test the onboard instruments for the RACORO field campaign that began in January 2009. Researchers are gathering data

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    New Method for Retrieving Cloud Heights from Satellite Data Download a printable PDF Submitter: Chang, F., Science Systems and Applications, Inc. Minnis, P., NASA - Langley Research Center Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Chang F, P Minnis, B Lin, MM Khaiyer, R Palikonda, and DA Spangenberg. 2010. "A modified method for inferring cloud top height using GOES-12 imager 10.7- and 13.3-µm data." Journal of

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Observational Analysis of Land-Atmosphere Coupling for Climate Model Evaluation Download a printable PDF Submitter: Phillips, T. J., Lawrence Livermore National Laboratory Klein, S., Lawrence Livermore National Laboratory Area of Research: Surface Properties Working Group(s): Cloud Life Cycle Journal Reference: Phillips TJ and SA Klein. 2014. "Land-atmosphere coupling manifested in warm-season observations on the U.S. southern great plains." Journal of Geophysical Research -

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    A Revealing Look Inside Northern Australian Wet Season Precipitation Download a printable PDF Submitter: Giangrande, S., Brookhaven National Laboratory Area of Research: Surface Properties Working Group(s): Cloud Life Cycle Journal Reference: Giangrande SE, M Bartholomew, M Pope, S Collis, and MP Jensen. 2014. "A Summary of Precipitation Characteristics from the 2006-2011 Northern Australian Wet Seasons as Revealed by ARM Disdrometer Research Facilities (Darwin, Australia)." Journal of

  6. Stackable differential mobility analyzer for aerosol measurement

    DOE Patents [OSTI]

    Cheng, Meng-Dawn; Chen, Da-Ren

    2007-05-08

    A multi-stage differential mobility analyzer (MDMA) for aerosol measurements includes a first electrode or grid including at least one inlet or injection slit for receiving an aerosol including charged particles for analysis. A second electrode or grid is spaced apart from the first electrode. The second electrode has at least one sampling outlet disposed at a plurality different distances along its length. A volume between the first and the second electrode or grid between the inlet or injection slit and a distal one of the plurality of sampling outlets forms a classifying region, the first and second electrodes for charging to suitable potentials to create an electric field within the classifying region. At least one inlet or injection slit in the second electrode receives a sheath gas flow into an upstream end of the classifying region, wherein each sampling outlet functions as an independent DMA stage and classifies different size ranges of charged particles based on electric mobility simultaneously.

  7. Aerosol Retrievals from ARM SGP MFRSR Data

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Alexandrov, Mikhail

    2008-01-15

    The Multi-Filter Rotating Shadowband Radiometer (MFRSR) makes precise simultaneous measurements of the solar direct normal and diffuse horizontal irradiances at six wavelengths (nominally 415, 500, 615, 673, 870, and 940 nm) at short intervals (20 sec for ARM instruments) throughout the day. Time series of spectral optical depth are derived from these measurements. Besides water vapor at 940 nm, the other gaseous absorbers within the MFRSR channels are NO2 (at 415, 500, and 615 nm) and ozone (at 500, 615, and 670 nm). Aerosols and Rayleigh scattering contribute atmospheric extinction in all MFRSR channels. Our recently updated MFRSR data analysis algorithm allows us to partition the spectral aerosol optical depth into fine and coarse modes and to retrieve the fine mode effective radius. In this approach we rely on climatological amounts of NO2 from SCIAMACHY satellite retrievals and use daily ozone columns from TOMS.

  8. Incorporating an advanced aerosol activation parameterization into WRF-CAM5: Model evaluation and parameterization intercomparison

    SciTech Connect (OSTI)

    Zhang, Yang; Zhang, Xin; Wang, Kai; He, Jian; Leung, Lai-Yung R.; Fan, Jiwen; Nenes, Athanasios

    2015-07-22

    Aerosol activation into cloud droplets is an important process that governs aerosol indirect effects. The advanced treatment of aerosol activation by Fountoukis and Nenes (2005) and its recent updates, collectively called the FN series, have been incorporated into a newly developed regional coupled climate-air quality model based on the Weather Research and Forecasting model with the physics package of the Community Atmosphere Model version 5 (WRF-CAM5) to simulate aerosol-cloud interactions in both resolved and convective clouds. The model is applied to East Asia for two full years of 2005 and 2010. A comprehensive model evaluation is performed for model predictions of meteorological, radiative, and cloud variables, chemical concentrations, and column mass abundances against satellite data and surface observations from air quality monitoring sites across East Asia. The model performs overall well for major meteorological variables including near-surface temperature, specific humidity, wind speed, precipitation, cloud fraction, precipitable water, downward shortwave and longwave radiation, and column mass abundances of CO, SO2, NO2, HCHO, and O3 in terms of both magnitudes and spatial distributions. Larger biases exist in the predictions of surface concentrations of CO and NOx at all sites and SO2, O3, PM2.5, and PM10 concentrations at some sites, aerosol optical depth, cloud condensation nuclei over ocean, cloud droplet number concentration (CDNC), cloud liquid and ice water path, and cloud optical thickness. Compared with the default Abdul-Razzack Ghan (2000) parameterization, simulations with the FN series produce ~107113% higher CDNC, with half of the difference attributable to the higher aerosol activation fraction by the FN series and the remaining half due to feedbacks in subsequent cloud microphysical processes. With the higher CDNC, the FN series are more skillful in simulating cloud water path, cloud optical thickness, downward shortwave radiation, shortwave cloud forcing, and precipitation. The model evaluation identifies several areas of provements including emissions and their vertical allocation as well as model formulations such as aerosol formation, cloud droplet nucleation, and ice nucleation.

  9. Total aerosol effect: forcing or radiative flux perturbation?

    SciTech Connect (OSTI)

    Lohmann, Ulrike; Storelvmo, Trude; Jones, Andy; Rotstayn, Leon; Menon, Surabi; Quaas, Johannes; Ekman, Annica; Koch, Dorothy; Ruedy, Reto

    2009-09-25

    Uncertainties in aerosol forcings, especially those associated with clouds, contribute to a large extent to uncertainties in the total anthropogenic forcing. The interaction of aerosols with clouds and radiation introduces feedbacks which can affect the rate of rain formation. Traditionally these feedbacks were not included in estimates of total aerosol forcing. Here we argue that they should be included because these feedbacks act quickly compared with the time scale of global warming. We show that for different forcing agents (aerosols and greenhouse gases) the radiative forcings as traditionally defined agree rather well with estimates from a method, here referred to as radiative flux perturbations (RFP), that takes these fast feedbacks and interactions into account. Thus we propose replacing the direct and indirect aerosol forcing in the IPCC forcing chart with RFP estimates. This implies that it is better to evaluate the total anthropogenic aerosol effect as a whole.

  10. Climate Engineering with Stratospheric Aerosols and Associated Engineering Parameters

    SciTech Connect (OSTI)

    Kravitz, Benjamin S.

    2013-02-12

    Climate engineering with stratospheric aerosols, an idea inspired by large volcaniceruptions, could cool the Earths surface and thus alleviate some of the predicted dangerous impacts of anthropogenic climate change. However, the effectiveness of climate engineering to achieve a particular climate goal, and any associated side effects, depend on certain aerosol parameters and how the aerosols are deployed in the stratosphere. Through the examples of sulfate and black carbon aerosols, this paper examines "engineering" parameters-aerosol composition, aerosol size, and spatial and temporal variations in deployment-for stratospheric climate engineering. The effects of climate engineering are sensitive to these parameters, suggesting that a particle could be found ordesigned to achieve specific desired climate outcomes. This prospect opens the possibility for discussion of societal goals for climate engineering.

  11. Indirect and Semi-Direct Aerosol Campaign

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Campaign (ISDAC) The Influence of Arctic Aerosol on Clouds PIs: Steve Ghan, Greg McFarquhar, Hans Verlinde ARM AVP: Beat Schmid, Greg McFarquhar, John Hubbe, Debbie Ronfeld In situ measurements: Sarah Brooks, Don Collins, Dan Cziczo, Manvendra Dubey, Greg Kok, Alexei Korolev, Alex Laskin, Paul Lawson, Peter Liu, Claudio Mazzoleni, Ann-Marie McDonald, Greg McFarquhar, Walter Strapp, Alla Zelenyuk Retrievals: Connor Flynn, Dan Lubin, Mengistu Wolde, David Mitchell, Matthew Shupe, David Turner

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    118(23), doi:10.10022013JD020554. Figure 1. a) Observed and fitted mean aerosol size distribution in Barrow, Alaska, averaged during the period from November 2008 to...

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    two competitive "aerosol+NO2" models fitting the solid curve within 0.01 error margin (grey area). Point-by-point intercomparison between total, fine, and coarse mode AODs...

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Chand D, R Wood, SJ Ghan, M Wang, M Ovchinnikov, PJ Rasch, S Miller, B Schichtel, and T Moore. 2012. "Aerosol optical depth increase in partly cloudy conditions." Journal of...

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    and aerosols over northeastern China: Vertical profiles and the influence of weather on air quality." Atmospheric Environment, 62, doi:10.1016j.atmosenv.2012.07.076. Altitude...

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    data set from the Clouds, Aerosol, and Precipitation in the Marine Boundary Layer (CAP-MBL) Graciosa, Azores, 2009-2010 field campaign was used to investigate how continental...

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    using high-resolution aerosol mass spectrometry: Results from CARES." Atmospheric Chemistry and Physics, 12, doi:10.5194acp-12-8131-2012. High-resolution mass spectra (colored...

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    data, which represent data aggregated at a range of levels. Currently, many climate change models treat the two types of data the same. Aerosols-tiny airborne particles from...

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    organic aerosol mass in urban and forest outflow." Atmospheric Chemistry and Physics, 15, doi:10.5194acp-15-595-2015. Simulated SOA in outflow from case studies based on...

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    of carbonaceous aerosol aging in Central California." Atmospheric Chemistry and Physics, 13, doi:10.5194acpd-13-9179-2013. Fractions of STXM-derived particle types for...

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    J. Geophys. Res., 109, D06208, doi:10.10292003JD004025. Delle Monache, L., K. D. Perry, R. T. Cederwall, and J. A. Ogren (2004), In situ aerosol profiles over the Southern...

  2. A New Assessment of the Aerosol First Indirect Effect

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    New Assessment of the Aerosol First Indirect Effect Shao, Hongfei Florida State University Liu, Guosheng Florida State University Category: Aerosols The aerosol first indirect effect is known to cool the Earth radiatively. However, its magnitude is very uncertain; large discrepancies exist among the observed values published in the literature. In this study, we first survey the published values of those parameters used for describing the first indirect effect. By analyzing the discrepancies

  3. Aerosol Simulations by LLNL IMPACT and Comparisons with Field Measurements

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Simulations by LLNL IMPACT and Comparisons with Field Measurements C. C. Chuang, D. Bergman, J. Dignon, and P. Connell Lawrence Livermore National Laboratory Livermore, California Introduction The first step needed to assess aerosol climate effects is to provide the global concentrations and vertical profiles of different aerosol components. These distributions cannot be easily obtained from satellite retrievals or field measurements but are key to estimating the magnitude of aerosol forcing. A

  4. Discrimination between thin cirrus and and tropospheric aerosol using

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    multiple measurements from Darwin ARCS Discrimination between thin cirrus and and tropospheric aerosol using multiple measurements from Darwin ARCS Mitchell, Ross CSIRO Category: Aerosols Thin cirrus cloud occurs frequently in the tropics, and is often difficult to distinguish from tropospheric aerosol on the basis of temporal variations in ground based measurements, since both can be rather spatially uniform. In this study we investigate their discrimination by combining data from three

  5. Importance of Iron Mineralogy to Aerosol Solubility: Potential Effects of

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Source on Ocean Photosynthesis Importance of Iron Mineralogy to Aerosol Solubility: Potential Effects of Aerosol Source on Ocean Photosynthesis figure 1 Figure 1. Dust storm blowing glacial dusts from the Copper River Basin of southeast Alaska into the North Pacific Ocean, which depends on this and other external iron sources to support its biological communities. (Image: NASA MODIS satellite image, Nov. 1, 2006. http://earthobservatory.nasa.gov/IOTD/view.php?id=7094) Iron is one of

  6. Toward a Minimal Representation of Aerosols in Climate Models: Description

    Office of Scientific and Technical Information (OSTI)

    and Evaluation in the Community Atmosphere Model CAM5 (Journal Article) | SciTech Connect Toward a Minimal Representation of Aerosols in Climate Models: Description and Evaluation in the Community Atmosphere Model CAM5 Citation Details In-Document Search Title: Toward a Minimal Representation of Aerosols in Climate Models: Description and Evaluation in the Community Atmosphere Model CAM5 A modal aerosol module (MAM) has been developed for the Community Atmosphere Model version 5 (CAM5), the

  7. Quantifying Aerosol Direct Effects from Broadband Irradiance and Spectral Aerosol Optical Depth Observations

    SciTech Connect (OSTI)

    Creekmore, Torreon N.; Joseph, Everette; Long, Charles N.; Li, Siwei

    2014-05-16

    We outline a methodology using broadband and spectral irradiances to quantify aerosol direct effects on the surface diffuse shortwave (SW) irradiance. Best Estimate Flux data span a 13 year timeframe at the Department of Energy Atmospheric Radiation Measurement Program’s Southern Great Plains (SGP) site. Screened clear-sky irradiances and aerosol optical depth (AOD), for solar zenith angles ≤ 65°, are used to estimate clear-sky diffuse irradiances. We validate against detected clear-sky observations from SGP’s Basic Radiation System (BRS). BRS diffuse irradiances were in accordance with estimates, producing a root-mean-square error and mean bias errors of 4.0 W/m2 and -1.4 W/m2, respectively. Absolute differences show 99% of estimates within ±10 W/m2 (10%) of the mean BRS observations. Clear-sky diffuse estimates are used to derive quantitative estimates of aerosol radiative effects, represented as the aerosol diffuse irradiance (ADI). ADI is the contribution of diffuse SW to global SW, attributable to scattering of atmospheric transmission by natural plus anthropogenic aerosols. Estimated slope for the ADI as a function of AOD indicates an increase of ~22 W/m2 in diffuse SW for every 0.1 increase in AOD. Such significant increases in the diffuse fraction could possibly increase photosynthesis. Annual mean ADI is 28.2 W/m2, and heavy aerosol loading at SGP provides up to a maximum increase of 120 W/m2 in diffuse SW over background conditions. With regard to seasonal variation, the mean diffuse forcings are 17.2, 33.3, 39.0, and 23.6 W/m2 for winter, spring, summer, and fall, respectively.

  8. Parameterizing the Mixing State of Complex Submicron Aerosols...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    DA Knopf, MK Gilles, and RC Moffet. 2015. "Chemical imaging of ambient aerosol particles: Observational constraints on mixing state parameterization." Journal of Geophysical...

  9. ARM - Field Campaign - Azores: Clouds, Aerosol and Precipitation...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Campaigns Azores: Above-Cloud Radiation Budget near Graciosa Island 2010.04.15, Miller, AMF Azores: Extension to Clouds, Aerosol and Precipitation in the Marine Boundary...

  10. ARM - Field Campaign - Carbonaceous Aerosol and Radiative Effects...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    of representative organic aerosols within the boundary layer. By combining a SMPS and a dual column CCN counter, the size-resolved CCN concentrations were measured. This allowed...

  11. Clouds, Aerosols and Precipitation in the Marine Boundary Layer...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Framework, extend to investigation of aerosol-cloud interactions in models - Ensemble Kalman Filter (DART) Satellite activities with CAP-MBL Minnis: CAP-MBL subset MBL depth,...

  12. ARM - Field Campaign - Carbonaceous Aerosol and Radiation Effects...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    - Surface Meteorological Sounding Campaign Links ARM Data Discovery Browse Data Related Campaigns Carbonaceous Aerosol and Radiative Effects Study (CARES) 2010.06.02, Zaveri, AAF...

  13. ARM - Field Campaign - Indirect and Semi-Direct Aerosol Campaign...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsIndirect and Semi-Direct Aerosol Campaign (ISDAC) Campaign Links ISDAC Website ARM Data Discovery Browse Data Related Campaigns Parameterization of Extinction...

  14. Analysis of Aerosol Indirect Effects in California Coastal Stratus...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Andrew Brookhaven National Laboratory Andrews, Betsy NOAACMDL Ogren, John NOAACMDL Turner, David University of Wisconsin-Madison Category: Field Campaigns Impacts of aerosol...

  15. ARM - Field Campaign - Biogenic Aerosols - Effects on Clouds...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    relevant to DOE's goals in understanding the impact of clouds and aerosols on climate change. TWST contributes significantly to the body of data used for extracting cloud...

  16. Toward a Minimal Representation of Aerosols in Climate Models...

    Office of Scientific and Technical Information (OSTI)

    Minimal Representation of Aerosols in Climate Models: Description and Evaluation in the Community Atmosphere Model CAM5 Citation Details In-Document Search Title: Toward a Minimal ...

  17. The Radiative Role of Free Tropospheric Aerosols and Marine Clouds...

    Office of Scientific and Technical Information (OSTI)

    Technical Report: The Radiative Role of Free Tropospheric Aerosols and Marine Clouds over the Central North Atlantic Citation Details In-Document Search Title: The Radiative Role...

  18. ARM - Publications: Science Team Meeting Documents: The SGP Aerosol...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The SGP Aerosol Best-Estimate Value-Added Procedure and Its Impact on the BBHRP Project Turner, David Pacific Northwest National Laboratory Sivaraman, Chitra Pacific Northwest...

  19. About the Rhythms of Variability of the Submicron Aerosol Characterist...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    of the distribution of the aerosol characteristics were considered. The periodograms (Fourier spectra of the discrete data set) were calculated for all data arrays using...

  20. A New Approach to Modeling Aerosol Effects on East Asian Climate: Parametric Uncertainties Associated with Emissions, Cloud Microphysics and their Interactions

    SciTech Connect (OSTI)

    Yan, Huiping; Qian, Yun; Zhao, Chun; Wang, Hailong; Wang, Minghuai; Yang, Ben; Liu, Xiaohong; Fu, Qiang

    2015-09-16

    In this study, we adopt a parametric sensitivity analysis framework that integrates the quasi-Monte Carlo parameter sampling approach and a surrogate model to examine aerosol effects on the East Asian Monsoon climate simulated in the Community Atmosphere Model (CAM5). A total number of 256 CAM5 simulations are conducted to quantify the model responses to the uncertain parameters associated with cloud microphysics parameterizations and aerosol (e.g., sulfate, black carbon (BC), and dust) emission factors and their interactions. Results show that the interaction terms among parameters are important for quantifying the sensitivity of fields of interest, especially precipitation, to the parameters. The relative importance of cloud-microphysics parameters and emission factors (strength) depends on evaluation metrics or the model fields we focused on, and the presence of uncertainty in cloud microphysics imposes an additional challenge in quantifying the impact of aerosols on cloud and climate. Due to their different optical and microphysical properties and spatial distributions, sulfate, BC, and dust aerosols have very different impacts on East Asian Monsoon through aerosol-cloud-radiation interactions. The climatic effects of aerosol do not always have a monotonic response to the change of emission factors. The spatial patterns of both sign and magnitude of aerosol-induced changes in radiative fluxes, cloud, and precipitation could be different, depending on the aerosol types, when parameters are sampled in different ranges of values. We also identify the different cloud microphysical parameters that show the most significant impact on climatic effect induced by sulfate, BC and dust, respectively, in East Asia.

  1. Aerosol, Cloud, and Climate: From Observation to Model (457th Brookhaven Lecture)

    SciTech Connect (OSTI)

    Wang, Jian

    2010-05-12

    In the last 100 years, the Earth has warmed by about 1F, glaciers and sea ice have been melting more quickly than previously, especially during the past decade, and the level of the sea has risen about 6-8 inches worldwide. Scientists have long been investigating this phenomenon of global warming, which is believed to be at least partly due to the increased carbon dioxide (CO2) concentration in the air from burning fossil fuels. Funded by DOE, teams of researchers from BNL and other national labs have been gathering data in the U.S. and internationally to build computer models of climate and weather to help in understanding general patterns, causes, and perhaps, solutions. Among many findings, researchers observed that atmospheric aerosols, minute particles in the atmosphere, can significantly affect global energy balance and climate. Directly, aerosols scatter and absorb sunlight. Indirectly, increased aerosol concentration can lead to smaller cloud droplets, changing clouds in ways that tend to cool global climate and potentially mask overall warming from man-made CO2.

  2. Aerosol, Cloud, and Climate: From Observation to Model (457th Brookhaven Lecture)

    ScienceCinema (OSTI)

    Wang, Jian [Ph.D., Environmental Sciences Department

    2010-09-01

    In the last 100 years, the Earth has warmed by about 1ºF, glaciers and sea ice have been melting more quickly than previously, especially during the past decade, and the level of the sea has risen about 6-8 inches worldwide. Scientists have long been investigating this phenomenon of ?global warming,? which is believed to be at least partly due to the increased carbon dioxide (CO2) concentration in the air from burning fossil fuels. Funded by DOE, teams of researchers from BNL and other national labs have been gathering data in the U.S. and internationally to build computer models of climate and weather to help in understanding general patterns, causes, and perhaps, solutions. Among many findings, researchers observed that atmospheric aerosols, minute particles in the atmosphere, can significantly affect global energy balance and climate. Directly, aerosols scatter and absorb sunlight. Indirectly, increased aerosol concentration can lead to smaller cloud droplets, changing clouds in ways that tend to cool global climate and potentially mask overall warming from man-made CO2.

  3. Research Techniques

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Research Techniques Research Techniques Print Coming Soon

  4. Optical Properties of Moderately-Absorbing Organic and Mixed Organic/Inorganic Particles at Very High Humidities

    SciTech Connect (OSTI)

    Bond, Tami C; Rood, Mark J; Brem, Benjamin T; Mena-Gonzalez, Francisco C; Chen, Yanju

    2012-04-16

    Relative humidity (RH) affects the water content of an aerosol, altering its ability to scatter and absorb light, which is important for aerosol effects on climate and visibility. This project involves in situ measurement and modeling of aerosol optical properties including absorption, scattering and extinction at three visible wavelengths (467, 530, 660 nm), for organic carbon (OC) generated by pyrolysis of biomass, ammonium sulfate and sodium chloride, and their mixtures at controlled RH conditions. Novel components of this project include investigation of: (1) Changes in all three of these optical properties at scanned RH conditions; (2) Optical properties at RH values up to 95%, which are usually extrapolated instead of measured; and (3) Examination of aerosols generated by the pyrolysis of wood, which is representative of primary atmospheric organic carbon, and its mixture with inorganic aerosol. Scattering and extinction values were used to determine light absorption by difference and single scattering albedo values. Extensive instrumentation development and benchmarking with independently measured and modeled values were used to obtain and evaluate these new results. The single scattering albedo value for a dry absorbing polystyrene microsphere benchmark agreed within 0.02 (absolute value) with independently published results at 530 nm. Light absorption by a nigrosin (sample light-absorbing) benchmark increased by a factor of 1.24 +/-0.06 at all wavelengths as RH increased from 38 to 95%. Closure modeling with Mie theory was able to reproduce this increase with the linear volume average (LVA) refractive index mixing rule for this water soluble compound. Absorption by biomass OC aerosol increased by a factor of 2.1 +/- 0.7 and 2.3 +/- 1.2 between 32 and 95% RH at 467 nm and 530 nm, but there was no detectable absorption at 660 nm. Additionally, the spectral dependence of absorption by OC that was observed with filter measurements was confirmed qualitatively in situ at 467 and 530 nm. Closure modeling with the dynamic effective medium approximation (DEMA) refractive index model was able to capture the increasing absorption trend with RH indicating that the droplets were heterogeneously mixed while containing dispersed insoluble absorbing material within those droplets. Seven other refractive index mixing models including LVA did not adequately describe the measurements for OC. Mixing the biomass OC aerosol with select mass fractions of ammonium sulfate ranging from 25 to 36% and sodium chloride ranging from 21 to 30% resulted in an increase in light scattering and extinction with RH and inorganic mass fraction. However, no detectable difference in light absorption behavior in comparison to pure biomass OC was observed. The main finding of this research is a measured increase in absorption with increasing RH, which is currently not represented in radiative transfer models even though biomass burning produces most of the primary OC aerosol in the atmosphere.

  5. Method of dispersing particulate aerosol tracer

    DOE Patents [OSTI]

    O'Holleran, Thomas P. (Belleville, MI)

    1988-01-01

    A particulate aerosol tracer which comprises a particulate carrier of sheet silicate composition having a particle size up to one micron, and a cationic dopant chemically absorbed in solid solution in the carrier. The carrier is preferably selected from the group consisting of natural mineral clays such as bentonite, and the dopant is selected from the group consisting of rare earth elements and transition elements. The tracers are dispersed by forming an aqueous salt solution with the dopant present as cations, dispersing the carriers in the solution, and then atomizing the solution under heat sufficient to superheat the solution droplets at a level sufficient to prevent reagglomeration of the carrier particles.

  6. Evaluate and characterize mechanisms controlling transport, fate and effects of army smokes in an aerosol wind tunnel: Transport, transformations, fate and terrestrial ecological effects of fog oil obscurant smokes: Final report

    SciTech Connect (OSTI)

    Cataldo, D.A.; Van Voris, P.; Ligotke, M.W.; Fellows, R.J.; McVeety, B.D.; Li, Shu-mei W.; Bolton, H. Jr.; Fredrickson, J.K.

    1989-01-01

    The terrestrial transport, chemical fate, and ecological effects of fog oil (FO) smoke obscurants were evaluated under controlled wind tunnel conditions. The primary objectives of this research program are to characterize and assess the impacts of smoke and obscurants on: (1) natural vegetation characteristic of US Army training sites in the United States; (2) physical and chemical properties of soils representative of these training sites; and (3) soil microbiological and invertebrate communities. Impacts and dose/responses were evaluated based on an exposure scenario, including exposure duration, exposure rate, and sequential cumulative dosing. Key to understanding the environmental impacts of fog oil smoke/obscurants is establishing the importance of environmental parameters, such as relative humidity and wind speed on airborne aerosol characteristics and deposition to receptor surfaces. Direct and indirect biotic effects were evaluated using five plant species and three soil types. 29 refs., 35 figs., 32 tabs.

  7. Chemical distribution in high-solids paint overspray aerosols

    SciTech Connect (OSTI)

    D'Arcy, J.B.; Chan, T.L. )

    1990-03-01

    The chemical composition of high-solids basecoat paint overspray aerosols was determined as a function of particle size. Detailed information on the chemical composition of the overspray aerosols is important in health hazard evaluation since the composition and distribution within the airborne particles may differ significantly from the bulk paint material. This study was conducted in a typical down-draft paint booth equipped with air-atomized spray painting equipment. A fixed paint target was used to simulate typical overspray generation conditions and the aerosols were collected isokinetically with a seven-stage cascade impactor for size-fractionated analysis. The overspray aerosol from six paints consisted of organic paint binders with varying amounts of inorganic species as pigments or luster enhancers. These overspray aerosols had mass median aerodynamic diameters (MMAD) ranging from 2.9 to 9.7 microns. The size-fractionated paint samples collected on the impaction stages were analyzed by energy dispersive X-ray spectrometry on a scanning electron microscope (SEM-EDXRS) to identify the metallic elements. Atomic absorption spectrometry was used to determine the mass distribution of aluminum and iron as indicators of nonuniform distribution. Three of the aerosols containing aluminum were found to have bimodal distributions with most aluminum distributions having cumulative MMADs larger than the total aerosol. Iron in the aerosols was bimodal for three of the paints with all samples having an overall iron MMAD less than or equal to the overspray aerosol MMAD. Analysis using ultraviolet spectrometry revealed that the organic compounds present in the size-fractionated particulate samples consisted of a single, polydispersed mode with an MMAD similar to that of the total overspray aerosol.

  8. Sandia National Laboratories: Research: Research Foundations: Geoscience

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Geoscience Bioscience Computing and Information Science Electromagnetics Engineering Science Geoscience Materials Science Nanodevices and Microsystems Radiation Effects and High Energy Density Science Research Geoscience Geoscience photo The Geoscience Research Foundation performs recognized world-class earth and atmospheric sciences research and development to support Sandia's national security missions. Why our work matters Knowledge of the Earth's subsurface properties, structure and

  9. Contributions of the Atmospheric Radiation Measurement (ARM) Program and the ARM Climate Research Facility to the U.S. Climate Change Science Program

    SciTech Connect (OSTI)

    SA Edgerton; LR Roeder

    2008-09-30

    The Earth’s surface temperature is determined by the balance between incoming solar radiation and thermal (or infrared) radiation emitted by the Earth back to space. Changes in atmospheric composition, including greenhouse gases, clouds, and aerosols can alter this balance and produce significant climate change. Global climate models (GCMs) are the primary tool for quantifying future climate change; however, there remain significant uncertainties in the GCM treatment of clouds, aerosol, and their effects on the Earth’s energy balance. The 2007 assessment (AR4) by the Intergovernmental Panel on Climate Change (IPCC) reports a substantial range among GCMs in climate sensitivity to greenhouse gas emissions. The largest contributor to this range lies in how different models handle changes in the way clouds absorb or reflect radiative energy in a changing climate (Solomon et al. 2007). In 1989, the U.S. Department of Energy (DOE) Office of Science created the Atmospheric Radiation Measurement (ARM) Program within the Office of Biological and Environmental Research (BER) to address scientific uncertainties related to global climate change, with a specific focus on the crucial role of clouds and their influence on the transfer of radiation in the atmosphere. To address this problem, BER has adopted a unique two-pronged approach: * The ARM Climate Research Facility (ACRF), a scientific user facility for obtaining long-term measurements of radiative fluxes, cloud and aerosol properties, and related atmospheric characteristics in diverse climate regimes. * The ARM Science Program, focused on the analysis of ACRF data to address climate science issues associated with clouds, aerosols, and radiation, and to improve GCMs. This report describes accomplishments of the BER ARM Program toward addressing the primary uncertainties related to climate change prediction as identified by the IPCC.

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ARM Measurements Validate New Satellite Multilayer Cloud Remote Sensing Method Submitter: Minnis, P., NASA - Langley Research Center Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Huang, J., P. Minnis, B. Lin, Y. Yi, T.-F. Fan, S. Sun-Mack, and J. K. Ayers, 2006: Determination of ice water path in ice-over-water cloud systems using combined MODIS and AMSR-E measurements. Geophys. Res. Lett., 33, L21801, 10.1029/2006GL027038. Minnis,

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ARM Program Achieves Milestone in Global Cloud Properties Research Submitter: Revercomb, H. E., University of Wisconsin, Madison Area of Research: Radiation Processes Working Group(s): Radiative Processes Journal Reference: Knuteson, R.O., Best, F.A., Dedecker, R.G., Feltz, W.F., Revercomb, H.E., and Tobin, D.C., 2004: "10 Years of AERI Data from the DOE ARM Southern Great Plains Site," In Proceedings from the Fourteenth ARM Science Team Meeting, U.S. Department of Energy,Washington,

  12. Laboratory Investigation of Contact Freezing and the Aerosol to Ice Crystal Transformation Process

    SciTech Connect (OSTI)

    Shaw, Raymond A.

    2014-10-28

    This project has been focused on the following objectives: 1. Investigations of the physical processes governing immersion versus contact nucleation, specifically surface-induced crystallization; 2. Development of a quadrupole particle trap with full thermodynamic control over the temperature range 0 to 40 C and precisely controlled water vapor saturation ratios for continuous, single-particle measurement of the aerosol to ice crystal transformation process for realistic ice nuclei; 3. Understanding the role of ice nucleation in determining the microphysical properties of mixed-phase clouds, within a framework that allows bridging between laboratory and field measurements.

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Vertical Structure of Cloud Radiative Forcing at the ACRF SGP Revealed by 8 Years of Continuous Measurements Submitter: Mace, G., University of Utah Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Modeling, Cloud Properties Journal Reference: Accepted to Journal of Climate, 2007. Figure 1. Cloud occurrence, coverage, radiative forcing, and radiation effects over a composite annual cycle that is derived by averaging all observations collected during a

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Mixed-Phase Cloud Vertical Velocities and Dynamical-Microphysical Interactions Download a printable PDF Submitter: Shupe, M., University of Colorado Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Shupe, MD, P Kollias, M Poellot, and E Eloranta. 2008. "On deriving vertical air motions from cloud radar Doppler spectra." Journal of Atmospheric and Oceanic Technology 25: 547-557. Shupe, MD, P Kollias, POG Persson, and GM

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Characterizing Mixed-Phase Clouds from the Ground: a Status Report Download a printable PDF Submitter: Shupe, M., University of Colorado Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Shupe, MD, JS Daniel, G De Boer, EW Eloranta, P Kollias, E Luke, CN Long, DD Turner, and J Verlinde. 2008. "A focus on mixed-phase clouds: The status of ground-ba sed observational methods." Bulletin of the American Meteorological Society,

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Assessment of CloudSat Using ARM, AMF, and CloudNet Observations Download a printable PDF Submitter: Protat, A., Australian Bureau of Meterology May, P. T., Bureau of Meteorology O'Connor, E. J., University of Reading Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Submitted. PDF of cloud reflectivity (upper-left), cloud top height (upper-right), thickness (lower-left), and cloud base height (lower right) as measured by the Darwin

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Vertical Variation of Cloud Droplet Size Using Ship and Space-borne R/S Data Download a printable PDF Submitter: Li, Z., University of Maryland Chen, R., University of Maryland Wood, R., University of Washington Chang, F., Science Systems and Applications, Inc. Ferraro, R., NOAA/NESDIS, WWBG Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Chen, R, R Wood, Z Li, R Ferraro, and F Chang. 2008. "Studying the vertical variation of

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    A New Method for Satellite/Surface Comparisons Download a printable PDF Submitter: Long, C. N., NOAA Global Monitoring Division/CIRES Area of Research: Radiation Processes Working Group(s): Cloud Properties, Radiative Processes Journal Reference: Zhang Y, CN Long, WB Rossow, and EG Dutton. 2010. "Exploiting diurnal variations to evaluate the ISCCP-FD flux calculations and radiative-flux-analysis-processed surface observations from BSRN, ARM, and SURFRAD." Journal of Geophysical

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Increased Accuracy for Sky Imager Retrievals Download a printable PDF Submitter: Long, C. N., NOAA Global Monitoring Division/CIRES Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Long CN. 2010. "Correcting for circumsolar and near-horizon errors in sky cover retrievals from sky images." The Open Atmospheric Science Journal, 4, doi:10.2174/1874282301004010045. Long CN, JM Sabburg, J Calbo, and D Pages. 2006. "Retrieving

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Characterizing Clouds at Arctic Atmospheric Observatories Download a printable PDF Submitter: Shupe, M., University of Colorado Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle Journal Reference: Shupe MD, VP Walden, E Eloranta, T Uttal, JR Campbell, SM Starkweather, and M Shiobara. 2011. "Clouds at Arctic atmospheric observatories, part I: occurrence and macrophysical properties." Journal of Applied Meteorology and Climatology, 50(3), 626-644.

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Modeling from a Tropical State of Mind Download a printable PDF Submitter: Del Genio, A. D., National Aeronautics and Space Administration Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle Journal Reference: Mrowiec AA, C Rio, AM Fridlind, AS Ackerman, AD Del Genio, OM Pauluis, AC Varble, and J Fan. 2012. "Analysis of cloud-resolving simulations of a tropical mesoscale convective system observed during TWP-ICE: Vertical fluxes and draft properties in convective and

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    High and Dry - Probing Greenland's Atmosphere and Clouds Download a printable PDF Submitter: Shupe, M., University of Colorado Turner, D. D., National Oceanic and Atmospheric Administration Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle Journal Reference: Shupe MD, DD Turner, VP Walden, R Bennartz, M Cadeddu, B Castellani, C Cox, D Hudak, M Kulie, N Miller, RR Neely, III, W Neff, and PM Rowe. 2013. "High and Dry: New observations of tropospheric and cloud properties

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    For Estimates of Cloud Optical Thickness, Simple Equation Is Good Enough Submitter: Barnard, J., University of Nevada Reno Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Barnard, J. C., and C. N. Long, (2004): A Simple Empirical Equation to Calculate Cloud Optical Thickness Using Shortwave Broadband Measurement, JAM, 43, 1057-1066. Distributions of cloud optical thickness reveal that the empirical method (dashed line) closely

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Self-Regulation Strikes a Balance Between Hydrological Cycle, Radiation Processes, and Intraseasonal Dynamic Variations Submitter: Stephens, G. L., Colorado State University Area of Research: Atmospheric Thermodynamics and Vertical Structures Working Group(s): Cloud Properties Journal Reference: Stephens, Graeme L., Webster, Peter J., Johnson, Richard H., Engelen, Richard, L'Ecuyer, Tristan. 2004: Observational Evidence for the Mutual Regulation of the Tropical Hydrological Cycle and Tropical

  5. CARES Helps Explain Secondary Organic Aerosols

    SciTech Connect (OSTI)

    Zaveri, Rahul

    2014-03-28

    What happens when urban man-made pollution mixes with what we think of as pristine forest air? To know more about what this interaction means for the climate, the Carbonaceous Aerosol and Radiative Effects Study, or CARES, field campaign was designed in 2010. The sampling strategy during CARES was coordinated with CalNex 2010, another major field campaign that was planned in California in 2010 by the California Air Resources Board (CARB), the National Oceanic and Atmospheric Administration (NOAA), and the California Energy Commission (CEC). "We found two things. When urban pollution mixes with forest pollutions we get more secondary organic aerosols," said Rahul Zaveri, FCSD scientist and project lead on CARES. "SOAs are thought to be formed primarily from forest emissions but only when they interact with urban emissions. The data is saying that there will be climate cooling over the central California valley because of these interactions." Knowledge gained from detailed analyses of data gathered during the CARES campaign, together with laboratory experiments, is being used to improve existing climate models.

  6. Asthmatic responses to airborne acid aerosols

    SciTech Connect (OSTI)

    Ostro, B.D.; Lipsett, M.J.; Wiener, M.B.; Selner, J.C. )

    1991-06-01

    Controlled exposure studies suggest that asthmatics may be more sensitive to the respiratory effects of acidic aerosols than individuals without asthma. This study investigates whether acidic aerosols and other air pollutants are associated with respiratory symptoms in free-living asthmatics. Daily concentrations of hydrogen ion (H+), nitric acid, fine particulates, sulfates and nitrates were obtained during an intensive air monitoring effort in Denver, Colorado, in the winter of 1987-88. A panel of 207 asthmatics recorded respiratory symptoms, frequency of medication use, and related information in daily diaries. We used a multiple regression time-series model to analyze which air pollutants, if any, were associated with health outcomes reported by study participants. Airborne H+ was found to be significantly associated with several indicators of asthma status, including moderate or severe cough and shortness of breath. Cough was also associated with fine particulates, and shortness of breath with sulfates. Incorporating the participants' time spent outside and exercise intensity into the daily measure of exposure strengthened the association between these pollutants and asthmatic symptoms. Nitric acid and nitrates were not significantly associated with any respiratory symptom analyzed. In this population of asthmatics, several outdoor air pollutants, particularly airborne acidity, were associated with daily respiratory symptoms.

  7. CARES Helps Explain Secondary Organic Aerosols

    ScienceCinema (OSTI)

    Zaveri, Rahul

    2014-06-02

    What happens when urban man-made pollution mixes with what we think of as pristine forest air? To know more about what this interaction means for the climate, the Carbonaceous Aerosol and Radiative Effects Study, or CARES, field campaign was designed in 2010. The sampling strategy during CARES was coordinated with CalNex 2010, another major field campaign that was planned in California in 2010 by the California Air Resources Board (CARB), the National Oceanic and Atmospheric Administration (NOAA), and the California Energy Commission (CEC). "We found two things. When urban pollution mixes with forest pollutions we get more secondary organic aerosols," said Rahul Zaveri, FCSD scientist and project lead on CARES. "SOAs are thought to be formed primarily from forest emissions but only when they interact with urban emissions. The data is saying that there will be climate cooling over the central California valley because of these interactions." Knowledge gained from detailed analyses of data gathered during the CARES campaign, together with laboratory experiments, is being used to improve existing climate models.

  8. Intellectual Property Provisions (CSB-115) Cooperative Agreement...

    Energy Savers [EERE]

    15) Cooperative Agreement Research, Development, or Demonstration Domestic Small Business Intellectual Property Provisions (CSB-115) Cooperative Agreement Research, Development, or...

  9. Intellectual Property Provisions (CLB-115) Cooperative Agreement...

    Office of Environmental Management (EM)

    Agreement Research, Development, or Demonstration Large Business and Foreign Entity Intellectual Property Provisions (CLB-115) Cooperative Agreement Research, Development, or...

  10. Method and apparatus for aerosol particle absorption spectroscopy

    DOE Patents [OSTI]

    Campillo, Anthony J.; Lin, Horn-Bond

    1983-11-15

    A method and apparatus for determining the absorption spectra, and other properties, of aerosol particles. A heating beam source provides a beam of electromagnetic energy which is scanned through the region of the spectrum which is of interest. Particles exposed to the heating beam which have absorption bands within the band width of the heating beam absorb energy from the beam. The particles are also illuminated by light of a wave length such that the light is scattered by the particles. The absorption spectra of the particles can thus be determined from an analysis of the scattered light since the absorption of energy by the particles will affect the way the light is scattered. Preferably the heating beam is modulated to simplify the analysis of the scattered light. In one embodiment the heating beam is intensity modulated so that the scattered light will also be intensity modulated when the particles absorb energy. In another embodiment the heating beam passes through an interferometer and the scattered light reflects the Fourier Transform of the absorption spectra.

  11. ARM: 10-second Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    2004-10-01

    10-second Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

  12. ARM: 2-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    2004-10-01

    2-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

  13. ARM: 1-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    2004-10-01

    1-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

  14. ARM: 10-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Newsom, Rob; Goldsmith, John

    1998-03-01

    10-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

  15. ARM: 10-second Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    10-second Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

  16. ARM: 10-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    10-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

  17. ARM: 2-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Sivaraman, Chitra; Flynn, Connor

    2-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

  18. ARM: 1-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    1-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

  19. Effect of Terrestrial and Marine Organic Aerosol on Regional and Global Climate: Model Development, Application, and Verification with Satellite Data

    SciTech Connect (OSTI)

    Meskhidze, Nicholas; Zhang, Yang; Kamykowski, Daniel

    2012-03-28

    In this DOE project the improvements to parameterization of marine primary organic matter (POM) emissions, hygroscopic properties of marine POM, marine isoprene derived secondary organic aerosol (SOA) emissions, surfactant effects, new cloud droplet activation parameterization have been implemented into Community Atmosphere Model (CAM 5.0), with a seven mode aerosol module from the Pacific Northwest National Laboratory (PNNL)???¢????????s Modal Aerosol Model (MAM7). The effects of marine aerosols derived from sea spray and ocean emitted biogenic volatile organic compounds (BVOCs) on microphysical properties of clouds were explored by conducting 10 year CAM5.0-MAM7 model simulations at a grid resolution 1.9???????°????????2.5???????° with 30 vertical layers. Model-predicted relationship between ocean physical and biological systems and the abundance of CCN in remote marine atmosphere was compared to data from the A-Train satellites (MODIS, CALIPSO, AMSR-E). Model simulations show that on average, primary and secondary organic aerosol emissions from the ocean can yield up to 20% increase in Cloud Condensation Nuclei (CCN) at 0.2% Supersaturation, and up to 5% increases in droplet number concentration of global maritime shallow clouds. Marine organics were treated as internally or externally mixed with sea salt. Changes associated with cloud properties reduced (absolute value) the model-predicted short wave cloud forcing from -1.35 Wm-2 to -0.25 Wm-2. By using different emission scenarios, and droplet activation parameterizations, this study suggests that addition of marine primary aerosols and biologically generated reactive gases makes an important difference in radiative forcing assessments. All baseline and sensitivity simulations for 2001 and 2050 using global-through-urban WRF/Chem (GU-WRF) were completed. The main objective of these simulations was to evaluate the capability of GU-WRF for an accurate representation of the global atmosphere by exploring the most accurate configuration of physics options in GWRF for global scale modeling in 2001 at a horizontal grid resolution of 1???????° x 1???????°. GU-WRF model output was evaluated using observational datasets from a variety of sources including surface based observations (NCDC and BSRN), model reanalysis (NCEP/ NCAR Reanalysis and CMAP), and remotely-sensed data (TRMM) to evaluate the ability of GU-WRF to simulate atmospheric variables at the surface as well as aloft. Explicit treatment of nanoparticles produced from new particle formation in GU-WRF/Chem-MADRID was achieved by expanding particle size sections from 8 to 12 to cover particles with the size range of 1.16 nm to 11.6 ???????µm. Simulations with two different nucleation parameterizations were conducted for August 2002 over a global domain at a 4???????º by 5???????º horizontal resolution. The results are evaluated against field measurement data from the 2002 Aerosol Nucleation and Real Time Characterization Experiment (ANARChE) in Atlanta, Georgia, as well as satellite and reanalysis data. We have also explored the relationship between ???¢????????clean marine???¢??????? aerosol optical properties and ocean surface wind speed using remotely sensed data from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) on board the CALIPSO satellite and the Advanced Microwave Scanning Radiometer (AMSR-E) on board the AQUA satellite. Detailed data analyses

  20. Intellectual Property Provisions

    Office of Environmental Management (EM)

    GNP-115 1 Intellectual Property Provisions (GNP-115) Grant and Cooperative Agreement Research, Development, or Demonstration Non-Federal Entity (State, Local government, Indian tribe, Institution of higher education, or Nonprofit organization) A Non-Federal Entity is subject to the intellectual property requirements at 2 CFR 200.315. 2 CFR 200.315 Intangible Property (a) Title to intangible property (see §200.59 Intangible property) acquired under a Federal award vests upon acquisition in the

  1. Fire aerosol experiment and comparisons with computer code predictions

    SciTech Connect (OSTI)

    Gregory, W.S.; Nichols, B.D.; White, B.W.; Smith, P.R.; Leslie, I.H.; Corkran, J.R.

    1988-01-01

    Los Alamos National Laboratory, in cooperation with New Mexico State University, has carried on a series of tests to provide experimental data on fire-generated aerosol transport. These data will be used to verify the aerosol transport capabilities of the FIRAC computer code. FIRAC was developed by Los Alamos for the US Nuclear Regulatory Commission. It is intended to be used by safety analysts to evaluate the effects of hypothetical fires on nuclear plants. One of the most significant aspects of this analysis deals with smoke and radioactive material movement throughout the plant. The tests have been carried out using an industrial furnace that can generate gas temperatures to 300/degree/C. To date, we have used quartz aerosol with a median diameter of about 10 ..mu..m as the fire aerosol simulant. We also plan to use fire-generated aerosols of polystyrene and polymethyl methacrylate (PMMA). The test variables include two nominal gas flow rates (150 and 300 ft/sup 3//min) and three nominal gas temperatures (ambient, 150/degree/C, and 300/degree/C). The test results are presented in the form of plots of aerosol deposition vs length of duct. In addition, the mass of aerosol caught in a high-efficiency particulate air (HEPA) filter during the tests is reported. The tests are simulated with the FIRAC code, and the results are compared with the experimental data. 3 refs., 10 figs., 1 tab.

  2. GCM parameterization of radiative forcing by Pinatubo aerosols

    SciTech Connect (OSTI)

    Lacis, A.A.; Mishchenko, M.I.

    1996-12-31

    This paper addresses the question of whether the general circulation model (GCM) parameterization of volcanic aerosol forcing can be adequately described in terms of just two physical aerosol parameters: (1) the aerosol column optical thickness and (2) the effective radius of the aerosol size distribution. Data recorded from the eruption of Mt. Pinatubo in the Philippines in June 1991 was analyzed to attempt to answer this question. The spatial distribution of the particle size showed considerable variability and was found to increase steadily following the eruption. The time evolution of the Pinatubo aerosol particle size distribution as derived from satellite data differed significantly, particularly in the early phases of the eruption, from that assumed in the initial GCM simulation of the Pinatubo eruption. A bimodal distribution was used to examine the possibility that the actual size distribution of the volcanic aerosol was multimodal. However, results suggested that in most cases the aerosol size distribution was essentially monomodal in nature. Results from the radiative model used in the calculations are also presented. 11 refs., 6 figs.

  3. ARM Climate Research Facility

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    for ARM Radiation Data (QCRAD) ... 13 2.35 Raman Lidar Profiles-Aerosol Scattering Ratio (RLPROFASR) ......

  4. ARM Climate Research Facility

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    for ARM Radiation Data (QCRAD) ... 12 2.31 Raman Lidar Profiles-Aerosol Scattering Ratio (RLPROFASR) ......

  5. Building America Case Study: Apartment Compartmentalization with an Aerosol-Based Sealing Process - Queens, NY (Fact Sheet), Technology Solutions for New and Existing Homes, Energy Efficiency & Renewable Energy (EERE)

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Apartment Compartmentalization with an Aerosol-Based Sealing Process Queens, New York PROJECT INFORMATION Construction: New Type: Multifamily Partners: Builder: Bluestone Organization, bluestoneorg.com Consortium for Advanced Residential Buildings, carb-swa.com Research Topic: Air sealing building enclosures Date Completed: 2014 Climate Zones: All PERFORMANCE DATA The aerosol process resulted in an average reduction of 71% in air leakage and an average apartment airtightness of 0.08 CFM50/ft 2

  6. Method of Producing Ultra-heavy Homogeneous Aerosol of Sub-micron Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ernest J. Valeo and Nathaniel J. Fisch | Princeton Plasma Physics Lab Method of Producing Ultra-heavy Homogeneous Aerosol of Sub-micron Particles Ernest J. Valeo and Nathaniel J. Fisch This invention forms a heavy homogeneous aerosol by agitating sub-micron particles throughacoustic forces and then releasing the aerosol into a low-pressure reservoir. Through this method, the aerosol particulates comprise the dominant mass of the aerosol to produce plasma of the requisite homogeneity,

  7. ARM - Field Campaign - Pajarito Aerosol Coupling to Ecosystems PACE

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsPajarito Aerosol Coupling to Ecosystems PACE ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : Pajarito Aerosol Coupling to Ecosystems PACE 2011.12.16 - 2012.04.29 Lead Scientist : Manvendra Dubey For data sets, see below. Abstract The primary goal of the Pajarito Aerosol Couplings to Ecosystems (PACE) IOP is to demonstrate routine MAOS field operations and finesse instrumental and operational

  8. ARM - Field Campaign - Shortwave Radiation and Aerosol Intensive

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Observation Periods govCampaignsShortwave Radiation and Aerosol Intensive Observation Periods ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : Shortwave Radiation and Aerosol Intensive Observation Periods 1998.08.03 - 1998.08.28 Lead Scientist : Warren Wiscombe For data sets, see below. Summary Wednesday, August 5, 1998: IOP Opening Activities: The IOP updates for the Shortwave/Aerosol/BDRF will be

  9. Aerosol mass spectrometry systems and methods

    DOE Patents [OSTI]

    Fergenson, David P.; Gard, Eric E.

    2013-08-20

    A system according to one embodiment includes a particle accelerator that directs a succession of polydisperse aerosol particles along a predetermined particle path; multiple tracking lasers for generating beams of light across the particle path; an optical detector positioned adjacent the particle path for detecting impingement of the beams of light on individual particles; a desorption laser for generating a beam of desorbing light across the particle path about coaxial with a beam of light produced by one of the tracking lasers; and a controller, responsive to detection of a signal produced by the optical detector, that controls the desorption laser to generate the beam of desorbing light. Additional systems and methods are also disclosed.

  10. Final Report for ?¢????Cloud-Aerosol Physics in Super-Parameterized Atmospheric Regional Climate Simulations (CAP-SPARCS)?¢??? (DE-SC0002003) for 8/15/2009 through 8/14/2012

    SciTech Connect (OSTI)

    Lynn M. Russell; Richard C.J. Somerville

    2012-11-05

    Improving the representation of local and non-local aerosol interactions in state-of-the-science regional climate models is a priority for the coming decade (Zhang, 2008). With this aim in mind, we have combined two new technologies that have a useful synergy: (1) an aerosol-enabled regional climate model (Advanced Weather Research and Forecasting Model with Chemistry WRF-Chem), whose primary weakness is a lack of high quality boundary conditions and (2) an aerosol-enabled multiscale modeling framework (PNNL Multiscale Aerosol Climate Model (MACM)), which is global but captures aerosol-convection-cloud feedbacks, and thus an ideal source of boundary conditions. Combining these two approaches has resulted in an aerosol-enabled modeling framework that not only resolves high resolution details in a particular region, but crucially does so within a global context that is similarly faithful to multi-scale aerosol-climate interactions. We have applied and improved the representation of aerosol interactions by evaluating model performance over multiple domains, with (1) an extensive evaluation of mid-continent precipitation representation by multiscale modeling, (2) two focused comparisons to transport of aerosol plumes to the eastern United States for comparison with observations made as part of the International Consortium for Atmospheric Research on Transport and Transformation (ICARTT), with the first being idealized and the second being linked to an extensive wildfire plume, and (3) the extension of these ideas to the development of a new approach to evaluating aerosol indirect effects with limited-duration model runs by ?¢????nudging?¢??? to observations. This research supported the work of one postdoc (Zhan Zhao) for two years and contributed to the training and research of two graduate students. Four peer-reviewed publications have resulted from this work, and ground work for a follow-on project was completed.

  11. Observations and Modeling of Shallow Convective Clouds: Implications for the Indirect Aerosol Effects

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    and Modeling of Shallow Convective Clouds: Implications for the Indirect Aerosol Effects Sylwester Arabas 1 , Joanna Slawinska 1 , Wojciech Grabowski 2 , Hugh Morrison 2 , Hanna Pawlowska 1 1 : Institute of Geophysics, University of Warsaw, Poland 2 : National Center for Atmospheric Research, Boulder, Colorado, USA 348 constants for reference state and lateral boundary conditions 349 ibcx=icyx 350 ibcy=icyy*j3 351 ibcz=icyz 352 irlx=irelx 353 irly=irely*j3 354 irdbc=0 355 fcr0=fcr0*icorio 356

  12. Pressure-flow reducer for aerosol focusing devices

    DOE Patents [OSTI]

    Gard, Eric (San Francisco, CA); Riot, Vincent (Oakland, CA); Coffee, Keith (Diablo Grande, CA); Woods, Bruce (Livermore, CA); Tobias, Herbert (Kensington, CA); Birch, Jim (Albany, CA); Weisgraber, Todd (Brentwood, CA)

    2008-04-22

    A pressure-flow reducer, and an aerosol focusing system incorporating such a pressure-flow reducer, for performing high-flow, atmosphere-pressure sampling while delivering a tightly focused particle beam in vacuum via an aerodynamic focusing lens stack. The pressure-flow reducer has an inlet nozzle for adjusting the sampling flow rate, a pressure-flow reduction region with a skimmer and pumping ports for reducing the pressure and flow to enable interfacing with low pressure, low flow aerosol focusing devices, and a relaxation chamber for slowing or stopping aerosol particles. In this manner, the pressure-flow reducer decouples pressure from flow, and enables aerosol sampling at atmospheric pressure and at rates greater than 1 liter per minute.

  13. Overview of the COPS Aerosol and Cloud Microphysics (ACM) Subgroup...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    at the AMF for Jun-Aug 2007 - Multi-wavelength aerosol and water vapor lidar (BERTHA) - Doppler wind lidar * Mainly in vertical-pointing mode * Operated primarily in the daytime,...

  14. Microsoft Word - Aerosol Working Group_Norfolk 2008.doc

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Interactions Under Varying Meteorological Conditions: Southern Great Plains Vs. Pt. Reyes 15:52 0:13 Jefferson AOS mentor report 16:05 0:13 Kassianov Retrieval of Aerosol...

  15. ARM - Field Campaign - ARM Cloud Aerosol Precipitation Experiment...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    would love to hear from you Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : ARM Cloud Aerosol Precipitation Experiment (ACAPEX) 2015.01.14 - 2015.02.12 Lead...

  16. ARM - Field Campaign - MArine Stratus Radiation Aerosol and Drizzle...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsMArine Stratus Radiation Aerosol and Drizzle (MASRAD) IOP Campaign Links Science Plan AMF Point Reyes Website AMF Point Reyes Data Plots ARM Data Discovery Browse Data...

  17. ARM - Field Campaign - Aerosol Life Cycle IOP at BNL

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