National Library of Energy BETA

Sample records for research aerosol processes

  1. COLLABORATIVE RESEARCH: Study of Aerosol Sources and Processing at the GVAX Pantnagar Supersite

    SciTech Connect (OSTI)

    Worsnop, Douglas R.

    2014-07-28

    This project funded the participation of scientists from seven research groups, running more than thirty instruments, in the Winter Intensive Operating Period (January-February 2012) of the Clean Air for London (ClearfLo) campaign at a rural site in Detling, UK, 45 km southeast of central London. The primary science questions for the ClearfLo Winter IOP were, 1) what is the urban increment of particulate matter (PM) and other pollutants in the greater London area, and, 2) what is the contribution of solid fuel use for home heating to wintertime PM? An additional motivation for the Detling measurements was the question of whether coatings on black carbon particles enhance absorption. The following four key accomplishments have been identified so far: 1) Chemical, physical and optical characterization of PM from local and regional sources (Figures 2, 4, 5 and 6). 2) Measurement of urban increment in particulate matter and gases in London (Figure 3). 3) Measurement of optical properties and chemical composition of coatings on black carbon containing particles indicates absorption enhancement. 4) First deployment of chemical ionization instrument (MOVI-CI-TOFMS) to measure both particle-phase and gas-phase organic acids. (See final report from Joel Thornton, University of Washington, for details.) Analysis of the large dataset acquired in Detling is ongoing and will yield further key accomplishments. These measurements of urban and rural aerosol properties will contribute to improved modeling of regional aerosol emissions, and of atmospheric aging and removal. The measurement of absorption enhancement by coatings on black carbon will contribute to improved modeling of the direct radiative properties of PM.

  2. Collaborative research. Study of aerosol sources and processing at the GVAX Pantnagar Supersite

    SciTech Connect (OSTI)

    Worsnop, Doug; Volkamer, Rainer

    2012-08-13

    The Two Column Aerosol Project (TCAP) investigated uncertainties in the aerosol direct effect in the northern hemisphere mid-latitudes. The University of Colorado 2D-MAX-DOAS and LED-CE-DOAS instruments were collocated with DOE’s Atmospheric Radiation Measurement (ARM) Mobile Facility (AMF) and Mobile Aerosol Observing System (MAOS) during the TCAP-1 campaign at Cape Cod, MA (1 July to 13 August 2012). We have performed atmospheric radiation closure studies to evaluate the use of a novel parameter, i.e., the Raman Scattering Probability (RSP). We have performed first measurements of RSP almucantar scans, and measure RSP in spectra of scattered solar photons at 350nm and 430nm. Radiative Transfer Modelling of RSP demonstrate that the RSP measurement is maximally sensitive to infer even extremely low aerosol optical depth (AOD < 0.01) reliably by DOAS at low solar relative azimuth angles. We further assess the role of elevated aerosol layers on near surface observations of oxygen collision complexes, O 2-O2. Elevated aerosol layers modify the near surface absorption of O2-O2 and RSP. The combination of RSP and O2-O2 holds largely unexplored potential to better constrain elevated aerosol layers and measure column aerosol optical properties such as aerosol effective radius, extinction, aerosol phase functions and refractive indices. The TCAP deployment also provides a time series of reactive trace gas vertical profiles, i.e., nitrogen dioxide (NO2) and glyoxal (C2H2O2), which are measured simultaneously with the aerosol optical properties by DOAS. NO2 is an important precursor for ozone (O3) that modifies oxidative capacity. Glyoxal modifies oxidative capacity and is a source for brown carbon by forming secondary organic aerosol (SOA) via multiphase reactions in aerosol and cloud water. We have performed field measurements of these gases during TCAP, and conducted laboratory experiments to quantify for the first time the Setschenow salting constant, KS, of glyoxal in sulfate aerosols. Knowledge about KS is prerequisite to predict how increasing sulfate concentrations since pre-industrial times have modified the formation of SOA from biogenic gases in atmospheric models.

  3. Researchers Model Impact of Aerosols Over California

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Researchers Model Impact of Aerosols Over California Researchers Model Impact of Aerosols Over California Research may clarify the effectiveness of regional pollution controls May 28, 2013 Contact: Linda Vu, lvu@lbl.gov, (510) 495-2404 LosAngelesSmogv1.jpg Smog over downtown Los Angeles. Aerosols are microscopic particles-like dust, pollen and soot-that ubiquitously float around in our atmosphere. Despite their tiny stature, these particles can have a huge impact on human health, climate and the

  4. Natural Radionuclides and Isotopic Signatures for Determining Carbonaceous Aerosol Sources, Aerosol Lifetimes, and Washout Processes

    SciTech Connect (OSTI)

    Gaffney, Jeffrey

    2012-12-12

    This is the final technical report. The project description is as follows: to determine the role of aerosol radiative forcing on climate, the processes that control their atmospheric concentrations must be understood, and aerosol sources need to be determined for mitigation. Measurements of naturally occurring radionuclides and stable isotopic signatures allow the sources, removal and transport processes, as well as atmospheric lifetimes of fine carbonaceous aerosols, to be evaluated.

  5. ARM - Field Campaign - 2007 Cumulus Humilis Aerosol Process Study...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    would love to hear from you Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : 2007 Cumulus Humilis Aerosol Process Study (CHAPS) 2007.06.04 - 2007.06.25 Lead...

  6. Apartment Compartmentalization With an Aerosol-Based Sealing Process

    SciTech Connect (OSTI)

    Maxwell, S.; Berger, D.; Harrington, C.

    2015-03-01

    Air sealing of building enclosures is a difficult and time-consuming process. Current methods in new construction require laborers to physically locate small and sometimes large holes in multiple assemblies and then manually seal each of them. The innovation demonstrated under this research study was the automated air sealing and compartmentalization of buildings through the use of an aerosolized sealant, developed by the Western Cooling Efficiency Center at University of California Davis. CARB sought to demonstrate this new technology application in a multifamily building in Queens, NY. The effectiveness of the sealing process was evaluated by three methods: air leakage testing of overall apartment before and after sealing, point-source testing of individual leaks, and pressure measurements in the walls of the target apartment during sealing.

  7. ARM AOS Processing Status and Aerosol Intensive Properties VAP

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AOS Processing Status and Aerosol Intensive Properties VAP A. S. Koontz and C. J. Flynn Pacific Northwest National Laboratory Richland, Washington J. A. Ogren, E. Andrews, and P. J. Sheridan National Oceanic and Atmospheric Administration Boulder, Colorado Abstract The Atmospheric Radiation Measurement (ARM) Aerosol Observing System (AOS) has been operating at the Southern Great Plains (SGP) Central Facility since 1996. In response to the cross-cutting broad- band heating rate profile value

  8. Atmospheric Science Program Cumulus Humilis Aerosol Processing Study (CHAPS)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Program Cumulus Humilis Aerosol Processing Study (CHAPS) General Description 'Cumulus humilis' is the scientific term used to describe the small fair weather clouds that dot the summer skies over Oklahoma. During the month of June, scientists sponsored by the U.S. Department of Energy's Atmospheric Science Program will use aircraft and ground based instruments to obtain information about the physical and chemical properties of these clouds and the small airborne particles - called aerosols -

  9. Laboratory Studies of Processing of Carbonaceous Aerosols by Atmospheric Oxidants/Hygroscopicity and CCN Activity of Secondary & Processed Primary Organic Aerosols

    SciTech Connect (OSTI)

    Ziemann, P.J.; Arey, J.; Atkinson, R.; Kreidenweis, S.M.; Petters, M.D.

    2012-06-13

    The atmosphere is composed of a complex mixture of gases and suspended microscopic aerosol particles. The ability of these particles to take up water (hygroscopicity) and to act as nuclei for cloud droplet formation significantly impacts aerosol light scattering and absorption, and cloud formation, thereby influencing air quality, visibility, and climate in important ways. A substantial, yet poorly characterized component of the atmospheric aerosol is organic matter. Its major sources are direct emissions from combustion processes, which are referred to as primary organic aerosol (POA), or in situ processes in which volatile organic compounds (VOCs) are oxidized in the atmosphere to low volatility reaction products that subsequent condense to form particles that are referred to as secondary organic aerosol (SOA). POA and VOCs are emitted to the atmosphere from both anthropogenic and natural (biogenic) sources. The overall goal of this experimental research project was to conduct laboratory studies under simulated atmospheric conditions to investigate the effects of the chemical composition of organic aerosol particles on their hygroscopicity and cloud condensation nucleation (CCN) activity, in order to develop quantitative relationships that could be used to more accurately incorporate aerosol-cloud interactions into regional and global atmospheric models. More specifically, the project aimed to determine the products, mechanisms, and rates of chemical reactions involved in the processing of organic aerosol particles by atmospheric oxidants and to investigate the relationships between the chemical composition of organic particles (as represented by molecule sizes and the specific functional groups that are present) and the hygroscopicity and CCN activity of oxidized POA and SOA formed from the oxidation of the major classes of anthropogenic and biogenic VOCs that are emitted to the atmosphere, as well as model hydrocarbons. The general approach for this project was to carry out reactions of representative anthropogenic and biogenic VOCs and organic particles with ozone (O3), and hydroxyl (OH), nitrate (NO3), and chlorine (Cl) radicals, which are the major atmospheric oxidants, under simulated atmospheric conditions in large-volume environmental chambers. A combination of on-line and off-line analytical techniques were used to monitor the chemical and physical properties of the particles including their hygroscopicity and CCN activity. The results of the studies were used to (1) improve scientific understanding of the relationships between the chemical composition of organic particles and their hygroscopicity and CCN activity, (2) develop an improved molecular level theoretical framework for describing these relationships, and (3) establish a large database that is being used to develop parameterizations relating organic aerosol chemical properties and SOA sources to particle hygroscopicity and CCN activity for use in regional and global atmospheric air quality and climate models.

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Zhang, Q., University of California, Davis Fast, J. ., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal...

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Download a printable PDF Submitter: Moffet, R., University of the Pacific Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: O'Brien...

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    printable PDF Submitter: Kulkarni, G., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Kulkarni...

  13. Solar thermal aerosol flow reaction process

    DOE Patents [OSTI]

    Weimer, Alan W.; Dahl, Jaimee K.; Pitts, J. Roland; Lewandowski, Allan A.; Bingham, Carl; Tamburini, Joseph R.

    2005-03-29

    The present invention provides an environmentally beneficial process using concentrated sunlight to heat radiation absorbing particles to carry out highly endothermic gas phase chemical reactions ultimately resulting in the production of hydrogen or hydrogen synthesis gases.

  14. Technology Solutions Case Study: Apartment Compartmentalization with an Aerosol-Based Sealing Process

    SciTech Connect (OSTI)

    2015-07-01

    Air sealing of building enclosures is a difficult and time-consuming process. Current methods in new construction require laborers to physically locate small and sometimes large holes in multiple assemblies and then manually seal each of them. This research study by Building America team Consortium for Advanced Residential Buildings demonstrated the automated air sealing and compartmentalization of buildings through the use of an aerosolized sealant developed by the Western Cooling Efficiency Center at University of California Davis. CARB demonstrated this new technology application in a multifamily building in Queens, NY. The effectiveness of the sealing process was evaluated by three methods: air leakage testing of overall apartment before and after sealing, point-source testing of individual leaks, and pressure measurements in the walls of the target apartment during sealing. Aerosolized sealing was successful by several measures in this study. Many individual leaks that are labor-intensive to address separately were well sealed by the aerosol particles. In addition, many diffuse leaks that are difficult to identify and treat were also sealed. The aerosol-based sealing process resulted in an average reduction of 71% in air leakage across three apartments and an average apartment airtightness of 0.08 CFM50/SF of enclosure area.

  15. Project Overview: Cumulus Humilis Aerosol Processing Study (CHAPS): Proposed Summer 2007 ASP Field Campaign

    SciTech Connect (OSTI)

    Berkowitz, Carl M.; Berg, Larry K.; Ogren, J. A.; Hostetler, Chris A.; Ferrare, Richard

    2006-05-18

    This white paper presents the scientific motivation and preliminary logistical plans for a proposed ASP field campaign to be carried out in the summer of 2007. The primary objective of this campaign is to use the DOE Gulfstream-1 aircraft to make measurements characterizing the chemical, physical and optical properties of aerosols below, within and above large fields of fair weather cumulus and to use the NASA Langley Research Centers High Spectral Resolution Lidar (HSRL) to make independent measurements of aerosol backscatter and extinction profiles in the vicinity of these fields. Separate from the science questions to be addressed by these observations will be information to add in the development of a parameterized cumulus scheme capable of including multiple cloud fields within a regional or global scale model. We will also be able to compare and contrast the cloud and aerosol properties within and outside the Oklahoma City plume to study aerosol processes within individual clouds. Preliminary discussions with the Cloud and Land Surface Interaction Campaign (CLASIC) science team have identified overlap between the science questions posed for the CLASIC Intensive Operation Period (IOP) and the proposed ASP campaign, suggesting collaboration would benefit both teams.

  16. Scanning Transmission X-ray Microscopy: Applications in Atmospheric Aerosol Research

    SciTech Connect (OSTI)

    Moffet, Ryan C.; Tivanski, Alexei V.; Gilles, Mary K.

    2011-01-20

    Scanning transmission x-ray microscopy (STXM) combines x-ray microscopy and near edge x-ray absorption fine structure spectroscopy (NEXAFS). This combination provides spatially resolved bonding and oxidation state information. While there are reviews relevant to STXM/NEXAFS applications in other environmental fields (and magnetic materials) this chapter focuses on atmospheric aerosols. It provides an introduction to this technique in a manner approachable to non-experts. It begins with relevant background information on synchrotron radiation sources and a description of NEXAFS spectroscopy. The bulk of the chapter provides a survey of STXM/NEXAFS aerosol studies and is organized according to the type of aerosol investigated. The purpose is to illustrate the current range and recent growth of scientific investigations employing STXM-NEXAFS to probe atmospheric aerosol morphology, surface coatings, mixing states, and atmospheric processing.

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Laboratory Area of Research: Radiation Processes Working Group(s): Radiative Processes Journal Reference: NA Figure 1. MFRSR data from the TWP site (970910) Figure 2. Aerosol...

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Study Aerosol Humidity Effects Using the ARM Measurements Submitter: Li, Z., University of Maryland Area of Research: Radiation Processes Working Group(s): Aerosol Journal Reference: Jeong, M.-J., Z. Li, E. Andrews, and S.-C. Tsay (2007). Effect of aerosol humidification on the column aerosol optical thickness over the Atmospheric Radiation Measurement Southern Great Plains site, J. Geophys. Res., 112, D10202, doi:10.1029/2006JD007176. (a)-(j) Column-mean aerosol humidification factor as

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    A Dance of Aerosols Download a printable PDF Submitter: Song, C., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Song C, RA Zaveri, JE Shilling, ML Alexander, and M Newburn. 2011. "Effect of hydrophilic organic seed aerosols on secondary organic aerosol formation from ozonolysis of α-pinene." Environmental Science & Technology, 45(17), doi:10.1021/es201225c. The injection of alpha-pinene, a

  20. Improved Arctic Cloud and Aerosol Research and Model Parameterizations

    SciTech Connect (OSTI)

    Kenneth Sassen

    2007-03-01

    In this report are summarized our contributions to the Atmospheric Measurement (ARM) program supported by the Department of Energy. Our involvement commenced in 1990 during the planning stages of the design of the ARM Cloud and Radiation Testbed (CART) sites. We have worked continuously (up to 2006) on our ARM research objectives, building on our earlier findings to advance our knowledge in several areas. Below we summarize our research over this period, with an emphasis on the most recent work. We have participated in several aircraft-supported deployments at the SGP and NSA sites. In addition to deploying the Polarization Diversity Lidar (PDL) system (Sassen 1994; Noel and Sassen 2005) designed and constructed under ARM funding, we have operated other sophisticated instruments W-band polarimetric Doppler radar, and midinfrared radiometer for intercalibration and student training purposes. We have worked closely with University of North Dakota scientists, twice co-directing the Citation operations through ground-to-air communications, and serving as the CART ground-based mission coordinator with NASA aircraft during the 1996 SUCCESS/IOP campaign. We have also taken a leading role in initiating case study research involving a number of ARM coinvestigators. Analyses of several case studies from these IOPs have been reported in journal articles, as we show in Table 1. The PDL has also participated in other major field projects, including FIRE II and CRYSTAL-FACE. In general, the published results of our IOP research can be divided into two categories: comprehensive cloud case study analyses to shed light on fundamental cloud processes using the unique CART IOP measurement capabilities, and the analysis of in situ data for the testing of remote sensing cloud retrieval algorithms. One of the goals of the case study approach is to provide sufficiently detailed descriptions of cloud systems from the data-rich CART environment to make them suitable for application to cloud modeling groups, such as the GEWEX Cloud Simulation Study (GCSS) Cirrus Working Groups. In this paper we summarize our IOP-related accomplishments.

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosols Help Clouds Warm Up Arctic Submitter: Lubin, D., National Science Foundation Area of Research: Radiation Processes Working Group(s): Radiative Processes Journal Reference: Lubin, D., and A.M. Vogelmann, 2006: A climatologically significant aerosol longwave indirect effect in the Arctic, Nature, 439, 26 January, 453-456, doi:10.1038/nature04449 In a process known as the first aerosol indirect effect, enhanced aerosol concentrations cause the droplets in a cloud to be smaller and more

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Brass Ring of Climate Modeling Download a printable PDF Submitter: Ghan, S. J., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Ghan SJ, SJ Smith, M Wang, K Zhang, K Pringle, K Carslaw, J Pierce, S Bauer, and P Adams. 2013. "A simple model of global aerosol indirect effects." Journal of Geophysical Research - Atmospheres, 118, 1-20. The simple model of aerosol effects on clouds

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    a printable PDF Submitter: Marshak, A., NASA - Goddard Space Flight Center Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions...

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Burning on the Prairies Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation...

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference:...

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Download a printable PDF Submitter: Alexandrov, M. D., Columbia University Area of Research: Radiation Processes Working Group(s): Aerosol Journal Reference: Applied Optics,...

  7. Connecting Organic Aerosol Climate-Relevant Properties to Chemical Mechanisms of Sources and Processing

    SciTech Connect (OSTI)

    Thornton, Joel

    2015-01-26

    The research conducted on this project aimed to improve our understanding of secondary organic aerosol (SOA) formation in the atmosphere, and how the properties of the SOA impact climate through its size, phase state, and optical properties. The goal of this project was to demonstrate that the use of molecular composition information to mechanistically connect source apportionment and climate properties can improve the physical basis for simulation of SOA formation and properties in climate models. The research involved developing and improving methods to provide online measurements of the molecular composition of SOA under atmospherically relevant conditions and to apply this technology to controlled simulation chamber experiments and field measurements. The science we have completed with the methodology will impact the simulation of aerosol particles in climate models.

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Arctic Winter Frost Flowers Have Negligible Influence on Cloud Longwave Warming Download a printable PDF Submitter: Xu, L., University of California, San Diego Russell, L. M., Scripps Institution of Oceanography Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Xu L, LM Russell, RC Somerville, and PK Quinn. 2013. "Frost flower aerosol effects on Arctic wintertime longwave cloud radiative forcing."

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Carbonaceous Aerosol Aging Mechanisms Improve Agreement of Global Simulations with Data Download a printable PDF Submitter: Dubey, M. K., Los Alamos National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: N/A Longitudinal and vertical distribution of global zonal mean hydrophobic to hydrophilic conversion time for carbonaceous aerosols with new laboratory aging mechanism. Impact of new aging mechanism on global zonal mean black carbon

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Scale Shows True Weight of Aerosol Effects on Clouds Download a printable PDF Submitter: McComiskey, A. C., National Oceanic and Atmospheric Administration Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: McComiskey A and G Feingold. 2012. "The scale problem in quantifying aerosol indirect effects." Atmospheric Chemistry and Physics, 12, doi:10.5194/acp-12-1031-2012. Differing values: Values derived from aircraft and surface observations,

  11. Apartment Compartmentalization With an Aerosol-Based Sealing Process

    SciTech Connect (OSTI)

    Maxwell, Sean; Berger, David; Harrington, Curtis

    2015-03-01

    The U.S. Department of Energy Building America Team, Consortium for Advanced Residential Buildings, sought to demonstrate this new technology application in a new construction multifamily building in Queens, New York. The effectiveness of the sealing process was evaluated by three methods: air leakage testing of overall apartment before-and-after sealing, point-source testing of individual leaks, and pressure measurements in the walls of an apartment during sealing.

  12. Building America Case Study: Apartment Compartmentalization with an Aerosol-Based Sealing Process - Queens, NY; Technology Solutions for New and Existing Homes, Energy Efficiency & Renewable Energy (EERE)

    SciTech Connect (OSTI)

    2015-07-01

    Air sealing of building enclosures is a difficult and time-consuming process. Current methods in new construction require laborers to physically locate small and sometimes large holes in multiple assemblies and then manually seal each of them. The innovation demonstrated under this research study was the automated air sealing and compartmentalization of buildings through the use of an aerosolized sealant, developed by the Western Cooling Efficiency Center at University of California Davis.
    CARB sought to demonstrate this new technology application in a multifamily building in Queens, NY. The effectiveness of the sealing process was evaluated by three methods: air leakage testing of overall apartment before and after sealing, point-source testing of individual leaks, and pressure measurements in the walls of the target apartment during sealing. Aerosolized sealing was successful by several measures in this study. Many individual leaks that are labor-intensive to address separately were well sealed by the aerosol particles. In addition, many diffuse leaks that are difficult to identify and treat were also sealed. The aerosol-based sealing process resulted in an average reduction of 71% in air leakage across three apartments and an average apartment airtightness of 0.08 CFM50/SF of enclosure area.

  13. Laboratory Investigation of Contact Freezing and the Aerosol to Ice Crystal Transformation Process

    SciTech Connect (OSTI)

    Shaw, Raymond A.

    2014-10-28

    This project has been focused on the following objectives: 1. Investigations of the physical processes governing immersion versus contact nucleation, specifically surface-induced crystallization; 2. Development of a quadrupole particle trap with full thermodynamic control over the temperature range 0 to –40 °C and precisely controlled water vapor saturation ratios for continuous, single-particle measurement of the aerosol to ice crystal transformation process for realistic ice nuclei; 3. Understanding the role of ice nucleation in determining the microphysical properties of mixed-phase clouds, within a framework that allows bridging between laboratory and field measurements.

  14. A new WRF-Chem treatment for studying regional-scale impacts of cloud processes on aerosol and trace gases in parameterized cumuli

    SciTech Connect (OSTI)

    Berg, L. K.; Shrivastava, M.; Easter, R. C.; Fast, J. D.; Chapman, E. G.; Liu, Y.; Ferrare, R. A.

    2015-02-24

    A new treatment of cloud effects on aerosol and trace gases within parameterized shallow and deep convection, and aerosol effects on cloud droplet number, has been implemented in the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) version 3.2.1 that can be used to better understand the aerosol life cycle over regional to synoptic scales. The modifications to the model include treatment of the cloud droplet number mixing ratio; key cloud microphysical and macrophysical parameters (including the updraft fractional area, updraft and downdraft mass fluxes, and entrainment) averaged over the population of shallow clouds, or a single deep convective cloud; and vertical transport, activation/resuspension, aqueous chemistry, and wet removal of aerosol and trace gases in warm clouds. These changes have been implemented in both the WRF-Chem chemistry packages as well as the Kain–Fritsch (KF) cumulus parameterization that has been modified to better represent shallow convective clouds. Testing of the modified WRF-Chem has been completed using observations from the Cumulus Humilis Aerosol Processing Study (CHAPS). The simulation results are used to investigate the impact of cloud–aerosol interactions on regional-scale transport of black carbon (BC), organic aerosol (OA), and sulfate aerosol. Based on the simulations presented here, changes in the column-integrated BC can be as large as –50% when cloud–aerosol interactions are considered (due largely to wet removal), or as large as +40% for sulfate under non-precipitating conditions due to sulfate production in the parameterized clouds. The modifications to WRF-Chem are found to account for changes in the cloud droplet number concentration (CDNC) and changes in the chemical composition of cloud droplet residuals in a way that is consistent with observations collected during CHAPS. Efforts are currently underway to port the changes described here to the latest version of WRF-Chem, and it is anticipated that they will be included in a future public release of WRF-Chem.

  15. A new WRF-Chem treatment for studying regional-scale impacts of cloud processes on aerosol and trace gases in parameterized cumuli

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Berg, L. K.; Shrivastava, M.; Easter, R. C.; Fast, J. D.; Chapman, E. G.; Liu, Y.; Ferrare, R. A.

    2015-02-24

    A new treatment of cloud effects on aerosol and trace gases within parameterized shallow and deep convection, and aerosol effects on cloud droplet number, has been implemented in the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) version 3.2.1 that can be used to better understand the aerosol life cycle over regional to synoptic scales. The modifications to the model include treatment of the cloud droplet number mixing ratio; key cloud microphysical and macrophysical parameters (including the updraft fractional area, updraft and downdraft mass fluxes, and entrainment) averaged over the population of shallow clouds, or a single deep convectivemore » cloud; and vertical transport, activation/resuspension, aqueous chemistry, and wet removal of aerosol and trace gases in warm clouds. These changes have been implemented in both the WRF-Chem chemistry packages as well as the Kain–Fritsch (KF) cumulus parameterization that has been modified to better represent shallow convective clouds. Testing of the modified WRF-Chem has been completed using observations from the Cumulus Humilis Aerosol Processing Study (CHAPS). The simulation results are used to investigate the impact of cloud–aerosol interactions on regional-scale transport of black carbon (BC), organic aerosol (OA), and sulfate aerosol. Based on the simulations presented here, changes in the column-integrated BC can be as large as –50% when cloud–aerosol interactions are considered (due largely to wet removal), or as large as +40% for sulfate under non-precipitating conditions due to sulfate production in the parameterized clouds. The modifications to WRF-Chem are found to account for changes in the cloud droplet number concentration (CDNC) and changes in the chemical composition of cloud droplet residuals in a way that is consistent with observations collected during CHAPS. Efforts are currently underway to port the changes described here to the latest version of WRF-Chem, and it is anticipated that they will be included in a future public release of WRF-Chem.« less

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    "Invisible" Giants in the Sky Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Kassianov E, M Pekour, and J Barnard. 2012. "Aerosols in central California: Unexpectedly large contribution of coarse mode to aerosol radiative forcing." Geophysical Research Letters, 39, L20806, doi:10.1029/2012GL053469. Daily averaged values of (a, b) the direct

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Analyzing the Contribution of Aerosols to an Observed Increase in Direct Normal Irradiance Download a printable PDF Submitter: Long, C. N., NOAA Global Monitoring Division/CIRES Riihimaki, L., Pacific Northwest National Laboratory Vignola, F., University of Oregon Area of Research: Radiation Processes Working Group(s): Aerosol, Radiative Processes Journal Reference: Riihimaki LD, FE Vignola, and CN Long. 2009. "Analyzing the contribution of aerosols to an observed increase in direct normal

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Raman Lidar Observations of Aerosol Humidification Near Clouds Submitter: Ferrare, R. A., NASA LaRC Area of Research: Aerosol Properties Working Group(s): Aerosol Journal ...

  19. ARM - Measurement - Aerosol extinction

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol extinction The removal of radiant energy from an incident beam by the process of aerosol absorption ...

  20. Electrospray neutralization process and apparatus for generation of nano-aerosol and nano-structured materials

    DOE Patents [OSTI]

    Bailey, Charles L.; Morozov, Victor; Vsevolodov, Nikolai N.

    2010-08-17

    The claimed invention describes methods and apparatuses for manufacturing nano-aerosols and nano-structured materials based on the neutralization of charged electrosprayed products with oppositely charged electrosprayed products. Electrosprayed products include molecular ions, nano-clusters and nano-fibers. Nano-aerosols can be generated when neutralization occurs in the gas phase. Neutralization of electrospan nano-fibers with molecular ions and charged nano-clusters may result in the formation of fibrous aerosols or free nano-mats. Nano-mats can also be produced on a suitable substrate, forming efficient nano-filters.

  1. Automated Sealing of Home Enclosures with Aerosol Particles | Department of

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Energy Sealing of Home Enclosures with Aerosol Particles Automated Sealing of Home Enclosures with Aerosol Particles This presentation was delivered during a Building America webinar on October 14, 2011, by the Building Industry Research Alliance team member Mark Modera. PDF icon bira_webinar_10_14_11.pdf More Documents & Publications Building America Technology Solutions for New and Existing Homes: Apartment Compartmentalization with an Aerosol-Based Sealing Process Building America

  2. Process-model Simulations of Cloud Albedo Enhancement by Aerosols in the Arctic

    SciTech Connect (OSTI)

    Kravitz, Benjamin S.; Wang, Hailong; Rasch, Philip J.; Morrison, H.; Solomon, Amy

    2014-11-17

    A cloud-resolving model is used to simulate the effectiveness of Arctic marine cloud brightening via injection of cloud condensation nuclei (CCN). An updated cloud microphysical scheme is employed, with prognostic CCN and cloud particle numbers in both liquid and mixed-phase marine low clouds. Injection of CCN into the marine boundary layer can delay the collapse of the boundary layer and increase low-cloud albedo. Because nearly all of the albedo effects are in the liquid phase due to the removal of ice water by snowfall when ice processes are involved, albedo increases are stronger for pure liquid clouds than mixed-phase clouds. Liquid precipitation can be suppressed by CCN injection, whereas ice precipitation (snow) is affected less; thus the effectiveness of brightening mixed-phase clouds is lower than for liquid-only clouds. CCN injection into a clean regime results in a greater albedo increase than injection into a polluted regime, consistent with current knowledge about aerosol-cloud interactions. Unlike previous studies investigating warm clouds, dynamical changes in circulation due to precipitation changes are small.

  3. Electrically Driven Technologies for Radioactive Aerosol Abatement

    SciTech Connect (OSTI)

    David W. DePaoli; Ofodike A. Ezekoye; Costas Tsouris; Valmor F. de Almeida

    2003-01-28

    The purpose of this research project was to develop an improved understanding of how electriexecy driven processes, including electrocoalescence, acoustic agglomeration, and electric filtration, may be employed to efficiently treat problems caused by the formation of aerosols during DOE waste treatment operations. The production of aerosols during treatment and retrieval operations in radioactive waste tanks and during thermal treatment operations such as calcination presents a significant problem of cost, worker exposure, potential for release, and increased waste volume.

  4. 2010 Membranes: Materials & Processes Gordon Research Conference

    SciTech Connect (OSTI)

    Jerry Lin

    2010-07-30

    The GRC series on Membranes: Materials and Processes have gained significant international recognition, attracting leading experts on membranes and other related areas from around the world. It is now known for being an interdisciplinary and synergistic meeting. The next summer's edition will keep with the past tradition and include new, exciting aspects of material science, chemistry, chemical engineering, computer simulation with participants from academia, industry and national laboratories. This edition will focus on cutting edge topics of membranes for addressing several grand challenges facing our society, in particular, energy, water, health and more generally sustainability. During the technical program, we want to discuss new membrane structure and characterization techniques, the role of advanced membranes and membrane-based processes in sustainability/environment (including carbon dioxide capture), membranes in water processes, and membranes for biological and life support applications. As usual, the informal nature of the meeting, excellent quality of the oral presentations and posters, and ample opportunity to meet many outstanding colleagues make this an excellent conference for established scientists as well as for students. A Gordon Research Seminar (GRS) on the weekend prior to the GRC meeting will provide young researchers an opportunity to present their work and network with outstanding experts. It will also be a right warm-up for the conference participants to join and enjoy the main conference.

  5. A Research Park for Studying Processes in Unsaturated Fractured...

    Office of Scientific and Technical Information (OSTI)

    A Research Park for Studying Processes in Unsaturated Fractured Media Citation Details In-Document Search Title: A Research Park for Studying Processes in Unsaturated Fractured ...

  6. GE Global Research Sourcing External Document & Process Repository...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    GE Global Research Sourcing External Document & Process Repository Home > GE Global Research Sourcing External Document & Process Repository Supplier Integrity Guide Purchase Order...

  7. NREL: Photovoltaics Research - Process Development and Integration

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Laboratory Research Overhead photo a male standing next to a large circular piece of equipment. Work with Us Are you interested in collaborating with NREL scientists within the PDIL? Do you want to know more about its capabilities? We want to hear from you! To get the ball rolling, please apply by following steps 1 through 4 below. The Process Development and Integration Laboratory (PDIL) has one-of-a-kind capabilities for fabricating and studying a wide range of solar cell technologies.

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Rotstayn, L., Commonwealth Scientific and Industrial Research Organization Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Rotstayn, L.,...

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    a printable PDF Submitter: Schmid, B., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: ARM Climate Research...

  10. Aerosol Optical Depth Value-Added Product Report

    SciTech Connect (OSTI)

    Koontz, A; Hodges, G; Barnard, J; Flynn, C; Michalsky, J

    2013-03-17

    This document describes the process applied to retrieve aerosol optical depth (AOD) from multifilter rotating shadowband radiometers (MFRSR) and normal incidence multifilter radiometers (NIMFR) operated at the ARM Climate Research Facility’s ground-based facilities.

  11. Use of the ARM Measurements of Spectral Zenith Radiance for Better Understanding of 3D Cloud-Radiation Processes & Aerosol-Cloud Interaction

    SciTech Connect (OSTI)

    Chiu, Jui-Yuan Christine

    2014-04-10

    This project focuses on cloud-radiation processes in a general three-dimensional cloud situation, with particular emphasis on cloud optical depth and effective particle size. The proposal has two main parts. Part one exploits the large number of new wavelengths offered by the Atmospheric Radiation Measurement (ARM) zenith-pointing ShortWave Spectrometer (SWS), to develop better retrievals not only of cloud optical depth but also of cloud particle size. We also take advantage of the SWS’ high sampling resolution to study the “twilight zone” around clouds where strong aerosol-cloud interactions are taking place. Part two involves continuing our cloud optical depth and cloud fraction retrieval research with ARM’s 2-channel narrow vield-of-view radiometer and sunphotometer instrument by, first, analyzing its data from the ARM Mobile Facility deployments, and second, making our algorithms part of ARM’s operational data processing.

  12. Study of Heterogeneouse Processes Related to the Chemistry of Tropospheric Oxidants and Aerosols

    SciTech Connect (OSTI)

    Davidovits, Paul; Worsnop, D R; Jayne, J T; Colb, C E

    2013-02-13

    The objective of the studies was to elucidate the heterogeneous chemistry of tropospheric aerosols. Experiments were designed to measure both specifically needed parameters, and to obtain systematic data required to build a fundamental understanding of the nature of gas-surface physical and chemical interactions

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    How to Catch Aerosols in the Act Download a printable PDF Submitter: Wang, M., Pacific Northwest National Laboratory Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle Journal Reference: Wang M, S Ghan, X Liu, TS L'Ecuyer, K Zhang, H Morrison, M Ovchinnikov, R Easter, R Marchand, D Chand, Y Qian, and JE Penner. 2012. "Constraining cloud lifetime effects of aerosols using A-Train satellite observations." Geophysical Research Letters, 39, L15709, doi:

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Variations of Meridional Aerosol Distribution and Solar Dimming Download a printable PDF Submitter: Long, C. N., NOAA Global Monitoring Division/CIRES Kishcha, P., Tel-Aviv University Starobinets, B., Tel-Aviv University Kalashnikova, O., Jet Propulsion Laboratory Alpert, P., Tel-Aviv University Area of Research: Radiation Processes Working Group(s): Aerosol, Radiative Processes Journal Reference: Kishcha P, B Starobinets, O Kalashnikova, CN Long, and P Alpert. 2009. "Variations of

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Optical Properties of the 1997 TWP Smoke Event Submitter: Spinhirne, J., University of Arizona Area of Research: Radiation Processes Working Group(s): Radiative Processes Journal Reference: N/A Figure 1. MPL image showing evolution of early September, 1997 smoke event at Manus, TWP. Figure 2. Selected aerosol extinction cross section profiles at the ARM TWP site during 1997 showing progression of aerosol loading. Figure 3. Cloud-cleared optical measurements at the TWP site from July 27 to

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Development and Validation of a Black Carbon Mixing State Resolved Three-Dimensional Model Download a printable PDF Submitter: Fast, J. ., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Matsui H, M Koike, Y Kondo, N Moteki, JD Fast, and RA Zaveri. 2013. "Development and validation of a black carbon mixing state resolved three-dimensional model: Aging processes and radiative impact." Journal of

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    China's Aerosol Malady Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Qiu Y, Q Wang, and F Hu. 2012. "Shouxian aerosol radiative properties measured by DOE AMF and compared with CERES-MODIS." Advanced Materials Research, 518-523(2), doi:10.4028/www.scientific.net/AMR.518-523.1973. Tiananmen tower enveloped by heavy fog and haze in January 2013. Many of

  18. NREL: Biomass Research - Projects in Biomass Process and Sustainabilit...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Projects in Biomass Process and Sustainability Analyses Researchers at NREL use biomass process and sustainability analyses to understand the economic, technical, and global ...

  19. NREL: Biomass Research - Capabilities in Biomass Process and...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Capabilities in Biomass Process and Sustainability Analyses A photo of a woman and four ... A team of NREL researchers uses biomass process and sustainability analyses to bridge the ...

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Nucleation Events Download a printable PDF Submitter: McMurry, P. ., University of Minnesota Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal ...

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Broadband Albedo Observations in the Southern Great Plains Submitter: Lamb, P. J., University of Oklahoma Area of Research: Aerosol Properties Working Group(s): Aerosol Journal...

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    a printable PDF Submitter: Laskin, A., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Aerosol Life Cycle...

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Wilson J, D Imre, J Bernek, M Shrivastava, and A Zelenyuk. 2014. "Evaporation ...

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    PDF Submitter: McComiskey, A. C., National Oceanic and Atmospheric Administration Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Aerosol Life Cycle,...

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Production Flux of Sea-Spray Aerosol Download a printable PDF Submitter: Schwartz, S. E., Brookhaven National Laboratory Area of Research: Aerosol Properties Working Group(s):...

  6. Responsible Science: Ensuring the Integrity of the Research Process

    SciTech Connect (OSTI)

    Arrison, Thomas Samuel

    2014-03-31

    This is the final technical report for DE-SC0005916 Responsible Science: Ensuring the Integrity of the Research Process.

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Does Glyoxal Contribute Significantly to Regional SOA Formation? Download a printable PDF Submitter: Knote, C., Atmospheric Chemistry Division Hodzic, A., NCAR Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Knote C, A Hodzic, J Jimenez, R Volkamer, JJ Orlando, S Baidar, J Brioude, J Fast, DR Gentner, AH Goldstein, PL Hayes, BW Knighton, H Oetjen, A Setyan, H Stark, R Thalman, G Tyndall, R Washenfelder, E Waxman, and Q Zhang. 2014. "Simulation of

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Organic Molecules Explaining New Particle Growth in the Boreal Forest Download a printable PDF Submitter: Thornton, J., University of Washington Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Ehn M, JA Thornton, E Kleist, M Sipila, H Junninen, I Pullinen, M Springer, F Rubach, R Tillmann, B Lee, F Lopez-Hilfiker, S Andres, I Acir, M Rissanen, T Jokinen, S Schobesberger, J Kangasluoma, J Kontkanen, T Nieminen, T Kurten, LB Nielsen, S Jorgensen, HG

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Scientists Uncover Combustion Mechanism to Better Predict Warming by Wildfires Download a printable PDF Submitter: Dubey, M. K., Los Alamos National Laboratory Donahue, N., Carnegie Mellon University Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Saleh R, E Robinson, D Tkacik, A Ahern, S Liu, A Aiken, R Sullivan, A Presto, M Dubey, R Yokelson, N Donahue, and A Robinson. 2014. "Brownness of organics in aerosols from biomass burning linked to

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Good Is Not Enough: Improving Measurements of Atmospheric Particles Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Kassianov E, LK Berg, M Pekour, J Barnard, D Chand, C Flynn, M Ovchinnikov, A Sedlacek, B Schmid, J Shilling, J Tomlinson, and J Fast. 2015. "Airborne aerosol in situ measurements during TCAP: A closure study of total scattering."

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Modelling Future Changes in Surface Ozone: a Parameterized Approach Download a printable PDF Submitter: Bergmann, D., Lawrence Livermore National Laboratory Chuang, C., Lawrence Livermore National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Wild O, AM Fiore, DT Shindell, RM Doherty, WJ Collins, FJ Dentener, MG Schultz, S Gong, IA MacKenzie, G Zeng, P Hess, DJ Bergmann, S Szopa, JE Jonson, TJ Keating, and A Zuber. 2012. "Modelling

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Mexico City Carbon-Containing Particle Composition Simulated Download a printable PDF Submitter: Zaveri, R., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Lee-Taylor J, S Madronich, B Aumont, M Camredon, A Hodzic, GS Tyndall, E Aperl, and RA Zaveri. 2012. "Explicit modeling of organic chemistry and secondary organic aerosol partitioning for Mexico City and its outflow plume." Atmospheric Chemistry and

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Influence of Regional Anthropogenic Emission Reductions on Aerosol Direct Radiative Forcing Download a printable PDF Submitter: Bergmann, D., Lawrence Livermore National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Yu H, M Chin, J West, C Atherton, N Bellouin, D Bergmann, I Bey, H Bian, T Diehl, G Forberth, P Hess, M Schulz, D Shindell, T Takemura, and Q Tan. 2012. "An HTAP multi-model assessment of the influence of regional

  14. Indirect and semi-direct aerosol campaign: The impact of Arctic aerosols on clouds

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    McFarquhar, Greg M.; Ghan, Steven; Verlinde, Johannes; Korolev, Alexei; Strapp, J. Walter; Schmid, Beat; Tomlinson, Jason M.; Wolde, Menqistu; Brooks, Sarah D.; Cziczo, Dan; et al

    2011-02-01

    A comprehensive dataset of microphysical and radiative properties of aerosols and clouds in the boundary layer in the vicinity of Barrow, Alaska, was collected in April 2008 during the Indirect and Semi-Direct Aerosol Campaign (ISDAC). ISDAC's primary aim was to examine the effects of aerosols, including those generated by Asian wildfires, on clouds that contain both liquid and ice. ISDAC utilized the Atmospheric Radiation Measurement Pro- gram's permanent observational facilities at Barrow and specially deployed instruments measuring aerosol, ice fog, precipitation, and radiation. The National Research Council of Canada Convair-580 flew 27 sorties and collected data using an unprecedented 41more » stateof- the-art cloud and aerosol instruments for more than 100 h on 12 different days. Aerosol compositions, including fresh and processed sea salt, biomassburning particles, organics, and sulfates mixed with organics, varied between flights. Observations in a dense arctic haze on 19 April and above, within, and below the single-layer stratocumulus on 8 and 26 April are enabling a process-oriented understanding of how aerosols affect arctic clouds. Inhomogeneities in reflectivity, a close coupling of upward and downward Doppler motion, and a nearly constant ice profile in the single-layer stratocumulus suggests that vertical mixing is responsible for its longevity observed during ISDAC. Data acquired in cirrus on flights between Barrow and Fairbanks, Alaska, are improving the understanding of the performance of cloud probes in ice. Furthermore, ISDAC data will improve the representation of cloud and aerosol processes in models covering a variety of spatial and temporal scales, and determine the extent to which surface measurements can provide retrievals of aerosols, clouds, precipitation, and radiative heating.« less

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Birth and Growth of an Aerosol Download a printable PDF Submitter: Fast, J. ., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: N/A An aerosol particle journey. New modeling approaches developed by a research team led by PNNL show how aerosol particles are born and grow to affect the atmosphere and ultimately climate. Tiny atmospheric aerosols are some of the most highly

  16. Building America Research-to-Market Process | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Research » Building America Research-to-Market Process Building America Research-to-Market Process Read the Building America Research-to-Market Plan. The Building America Program conducts applied research, development, and deployment in residential buildings. Building America projects are led by U.S. Department of Energy (DOE) national laboratories and expert building science teams in partnership with leading industry players (e.g., builders, contractors, and manufacturers). Building America's

  17. Initial Assessment of the Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR)-Based Aerosol Retrieval: Sensitivity Study

    SciTech Connect (OSTI)

    Kassianov, Evgueni I.; Flynn, Connor J.; Redemann, Jens; Schmid, Beat; Russell, P. B.; Sinyuk, Alexander

    2012-10-24

    The Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR) being developed for airborne measurements will offer retrievals of aerosol microphysical and optical properties from multi-angular and multi-spectral measurements of sky radiance and direct-beam sun transmittance. In this study, we assess the expected accuracy of the 4STAR-based aerosol retrieval and its sensitivity to major sources of anticipated perturbations in the 4STAR measurements by adapting a theoretical approach previously developed for the AERONET measurements. The major anticipated perturbations are (1) an apparent enhancement of sky radiance at small scattering angles associated with the necessarily compact design of the 4STAR and (2) and an offset (i.e. uncertainty) of sky radiance calibration independent of scattering angle. The assessment is performed through application of the operational AERONET aerosol retrieval and constructed synthetic 4STAR-like data. Particular attention is given to the impact of these perturbations on the upwelling and downwelling broadband fluxes and the direct aerosol radiative forcing at the bottom and top of the atmosphere. The results from this study suggest that limitations in the accuracy of 4STAR-retrieved particle size distributions and scattering phase functions have diminished impact on the accuracy of retrieved bulk microphysical parameters, permitting quite accurate retrievals of properties including the effective radius (up to 10%, or 0.03), and the radiatively important optical properties, such as the asymmetry factor (up to 4%, or 0.02) and single-scattering albedo (up to 6%, or 0.04). Also, the obtained results indicate that the uncertainties in the retrieved aerosol optical properties are quite small in the context of the calculated fluxes and direct aerosol radiative forcing (up to 15%, or 3 Wm-2).

  18. Environmental research program: FY 1987, annual report

    SciTech Connect (OSTI)

    Not Available

    1988-03-01

    This multidisciplinary research program includes fundamental and applied research in physics, chemistry, engineering, and biology, as well as research on the development of advanced methods of measurement and analysis. The Program's Annual Report contains summaries of research performed during FY 1987 in the areas of atmospheric aerosols, flue gas chemistry, combustion, membrane bioenergetics, and analytical chemistry. The main research interests of the Atmospheric Aerosol Research group concern the chemical and physical processes that occur in haze, clouds, and fogs. For their studies, the group is developing novel analytical and research methods for characterizing aerosol species. Aerosol research is performed in the laboratory and in the field. Studies of smoke emissions from fires and their possible effects on climatic change, especially as related to nuclear winter, are an example of the collaboration between the Atmospheric Aerosol Research and Combustion Research Groups.

  19. ARM - Field Campaign - Pajarito Aerosol Coupling to Ecosystems...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    (PJ) woodland site used for DOE sponsored ecosystem research to measure the aerosol life cycle of biogenic (secondary organic aerosol formation from sesquiterpenes) and smoke...

  20. The Indirect and Semi-Direct Aerosol Campaign

    SciTech Connect (OSTI)

    Ghan, Steve

    2014-03-24

    Research projects like the Indirect and Semi-Direct Aerosol Campaign, or ISDAC, increase our knowledge of atmospheric aerosol particles and cloud physics.

  1. The Indirect and Semi-Direct Aerosol Campaign

    ScienceCinema (OSTI)

    Ghan, Steve

    2014-06-12

    Research projects like the Indirect and Semi-Direct Aerosol Campaign, or ISDAC, increase our knowledge of atmospheric aerosol particles and cloud physics.

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Apparent Bluing of Aerosols Near Clouds Download a printable PDF Submitter: Marshak, A., NASA - Goddard Space Flight Center Area of Research: Radiation Processes Working Group(s): Radiative Processes Journal Reference: Marshak, A, G Wen, JA Coakley, LA Remer, NG Loeb, and RF Cahalan. 2008. "A simple model of the cloud adjacency effect and the apparent bluing of aerosols near clouds." Journal of Geophysical Research 113, D14S17, doi: 10.1029/2007JD009196. (upper panel) A schematic

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Experiment Results Featured in Technical Journal Submitter: Sheridan, P., U.S. Department of Commerce/NOAA Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Sheridan, P, W Arnott, J Ogren, E Andrews, D Atkinson, D Covert, H Moosmuller, A Petzold, B Schmid, A Strawa, R Varma, and A Virkkula. 2005. "The Reno Aerosol Optics Study: An evaluation of aerosol absorption measurement methods." Aerosol Science and Technology 39(1):1-16. This magnification

  4. Science Plan Biogenic Aerosols - Effects on Clouds and Climate...

    Office of Scientific and Technical Information (OSTI)

    In spite of recent advances in the understanding of aerosol formation processes and the links between aerosol dynamics and biosphere-atmosphere-climate interactions, great ...

  5. Biogenic Aerosols-Effects on Clouds and Climate (BAECC) Final...

    Office of Scientific and Technical Information (OSTI)

    In spite of recent advances in the understanding of aerosol formation processes and the links between aerosol dynamics and biosphere-atmosphere-climate interactions, great ...

  6. Indirect and Semi-Direct Aerosol Campaign: The Impact of Arctic Aerosols on Clouds

    SciTech Connect (OSTI)

    McFarquhar, Greg; Ghan, Steven J.; Verlinde, J.; Korolev, Alexei; Strapp, J. Walter; Schmid, Beat; Tomlinson, Jason M.; Wolde, Mengistu; Brooks, Sarah D.; Cziczo, Daniel J.; Dubey, Manvendra K.; Fan, Jiwen; Flynn, Connor J.; Gultepe, Ismail; Hubbe, John M.; Gilles, Mary K.; Laskin, Alexander; Lawson, Paul; Leaitch, W. R.; Liu, Peter S.; Liu, Xiaohong; Lubin, Dan; Mazzoleni, Claudio; Macdonald, A. M.; Moffet, Ryan C.; Morrison, H.; Ovchinnikov, Mikhail; Shupe, Matthew D.; Turner, David D.; Xie, Shaocheng; Zelenyuk, Alla; Bae, Kenny; Freer, Matthew; Glen, Andrew

    2011-02-01

    A comprehensive dataset of microphysical and radiative properties of aerosols and clouds in the arctic boundary layer in the vicinity of Barrow, Alaska was collected in April 2008 during the Indirect and Semi-Direct Aerosol Campaign (ISDAC) sponsored by the Department of Energy Atmospheric Radiation Measurement (ARM) and Atmospheric Science Programs. The primary aim of ISDAC was to examine indirect effects of aerosols on clouds that contain both liquid and ice water. The experiment utilized the ARM permanent observational facilities at the North Slope of Alaska (NSA) in Barrow. These include a cloud radar, a polarized micropulse lidar, and an atmospheric emitted radiance interferometer as well as instruments specially deployed for ISDAC measuring aerosol, ice fog, precipitation and spectral shortwave radiation. The National Research Council of Canada Convair-580 flew 27 sorties during ISDAC, collecting data using an unprecedented 42 cloud and aerosol instruments for more than 100 hours on 12 different days. Data were obtained above, below and within single-layer stratus on 8 April and 26 April 2008. These data enable a process-oriented understanding of how aerosols affect the microphysical and radiative properties of arctic clouds influenced by different surface conditions. Observations acquired on a heavily polluted day, 19 April 2008, are enhancing this understanding. Data acquired in cirrus on transit flights between Fairbanks and Barrow are improving our understanding of the performance of cloud probes in ice. Ultimately the ISDAC data will be used to improve the representation of cloud and aerosol processes in models covering a variety of spatial and temporal scales, and to determine the extent to which long-term surface-based measurements can provide retrievals of aerosols, clouds, precipitation and radiative heating in the Arctic.

  7. Wind Program Manufacturing Research Advances Processes and Reduces Costs |

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Department of Energy Manufacturing Research Advances Processes and Reduces Costs Wind Program Manufacturing Research Advances Processes and Reduces Costs March 31, 2014 - 11:22am Addthis Tower sections being installed for a 2-MW wind turbine. Knowing that reducing the overall cost of wind energy begins on the factory floor, the Department of Energy's (DOE's) Wind Program supports research and development efforts and funding opportunities that integrate new designs, materials, and advanced

  8. A Research Park for Studying Processes in Unsaturated Fractured Media

    Office of Scientific and Technical Information (OSTI)

    (Journal Article) | SciTech Connect A Research Park for Studying Processes in Unsaturated Fractured Media Citation Details In-Document Search Title: A Research Park for Studying Processes in Unsaturated Fractured Media A field research site has been developed to explore the combined use of physical experiments and mathematical modeling to analyze large-scale infiltration and chemical transport through the unsaturated media overlying the Snake River Plain Aquifer in southeastern Idaho. This

  9. DOE - Office of Legacy Management -- Processes Research Inc - OH 44

    Office of Legacy Management (LM)

    Processes Research Inc - OH 44 FUSRAP Considered Sites Site: PROCESSES RESEARCH, INC (OH.44) Eliminated from consideration under FUSRAP Designated Name: Not Designated Alternate Name: None Location: 2905 Vernon Place , Cincinnati , Ohio OH.44-1 Evaluation Year: 1991 OH.44-2 OH.44-3 Site Operations: Research and development of machining methods during the early 1950s; no indication of involvement with radioactive materials. OH.44-1 OH.44-3 Site Disposition: Eliminated - Potential for

  10. ARM - Research Highlights: Notable Findings

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    HighlightsNotable Research Findings Form Submit a New Research Highlight Sort Highlights Submitter Title Research Area Working Group Submission Date DOE Progress Reports Notable Research Findings for 2001-2006 Office of Science Abstracts Database Research Highlights Summaries Notable Research Findings for the Past Five Years Aerosols Cloud Parameterization and Modeling (Currently Cloud Modeling) Cloud Properties Instantaneous Radiative Flux (Currently Radiative Processes)

  11. ARM Cloud Aerosol Precipitation Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Precipitation Experiment a NOAA ship in the Pacific Ocean and on a DOE- sponsored plane over land and sea. These researchers will study: (1) water sources, evolution and structure of atmospheric rivers over the Pacific Ocean (2) long range transport of aerosols over the Pacific Ocean between Hawaii and the U.S. West Coast, and how aerosols interact with atmospheric rivers (3) the point where atmospheric rivers make landfall on the U.S. West Coast, especially how clouds form where

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Remote Sensing of Mineral Dust Using AERI Download a printable PDF Submitter: Hansell, R. A., University of California, Los Angeles Area of Research: Radiation Processes Working Group(s): Aerosol Journal Reference: Hansell R, KN Liou, SC Ou, SC Tsay, Q Ji, and JS Reid. 2008. "Remote sensing of mineral dust aerosol using AERI during the UAE2: A modeling and sensitivity study." Journal of Geophysical Research - Atmospheres, 113, D18202, doi:10.1029/2008JD010246. BT sensitivity to dust

  13. EM Marks Milestone at Separations Process Research Unit

    Broader source: Energy.gov [DOE]

    NISKAYUNA, N.Y. – EM met a major regulatory milestone at the Separations Process Research Unit (SPRU) by completing construction of enclosures and ventilation systems required for cleanup.

  14. Northwestern University Facility for Clean Catalytic Process Research

    SciTech Connect (OSTI)

    Marks, Tobin Jay

    2013-05-08

    Northwestern University with DOE support created a Facility for Clean Catalytic Process Research. This facility is designed to further strengthen our already strong catalysis research capabilities and thus to address these National challenges. Thus, state-of-the art instrumentation and experimentation facility was commissioned to add far greater breadth, depth, and throughput to our ability to invent, test, and understand catalysts and catalytic processes, hence to improve them via knowledge-based design and evaluation approaches.

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Two Faces of Aerosols Download a printable PDF Submitter: Ovink, J., Pacific Northwest National Laboratory Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle Journal Reference: Berg LK, M Shrivastava, RC Easter, JD Fast, EG Chapman, Y Liu, and RA Ferrare. 2015. "A New WRF-Chem Treatment for Studying Regional Scale Impacts of Cloud Processes on Aerosol and Trace Gases in Parameterized Cumuli." Geoscientific Model Development, 8, doi:10.5194/gmd-8-409-2015. A new

  16. Final Technical Report for Interagency Agreement No. DE-SC0005453 “Characterizing Aerosol Distributions, Types, and Optical and Microphysical Properties using the NASA Airborne High Spectral Resolution Lidar (HSRL) and the Research Scanning Polarimeter (RSP)”

    SciTech Connect (OSTI)

    Hostetler, Chris; Ferrare, Richard

    2015-01-13

    Measurements of the vertical profile of atmospheric aerosols and aerosol optical and microphysical characteristics are required to: 1) determine aerosol direct and indirect radiative forcing, 2) compute radiative flux and heating rate profiles, 3) assess model simulations of aerosol distributions and types, and 4) establish the ability of surface and space-based remote sensors to measure the indirect effect. Consequently the ASR program calls for a combination of remote sensing and in situ measurements to determine aerosol properties and aerosol influences on clouds and radiation. As part of our previous DOE ASP project, we deployed the NASA Langley airborne High Spectral Resolution Lidar (HSRL) on the NASA B200 King Air aircraft during major field experiments in 2006 (MILAGRO and MaxTEX), 2007 (CHAPS), 2009 (RACORO), and 2010 (CalNex and CARES). The HSRL provided measurements of aerosol extinction (532 nm), backscatter (532 and 1064 nm), and depolarization (532 and 1064 nm). These measurements were typically made in close temporal and spatial coincidence with measurements made from DOE-funded and other participating aircraft and ground sites. On the RACORO, CARES, and CalNEX missions, we also deployed the NASA Goddard Institute for Space Studies (GISS) Research Scanning Polarimeter (RSP). RSP provided intensity and degree of linear polarization over a broad spectral and angular range enabling column-average retrievals of aerosol optical and microphysical properties. Under this project, we analyzed observations and model results from RACORO, CARES, and CalNex and accomplished the following objectives. 1. Identified aerosol types, characterize the vertical distribution of the aerosol types, and partition aerosol optical depth by type, for CARES and CalNex using HSRL data as we have done for previous missions. 2. Investigated aerosol microphysical and macrophysical properties using the RSP. 3. Used the aerosol backscatter and extinction profiles measured by the HSRL to characterize the planetary boundary layer height (PBL) and the transition zone thickness, for the RACORO and CARES and CalNex campaigns as we have done for previous campaigns. 4. Investigated how optical properties measured by HSRL vary near clouds. 5. Assessed model simulations of aerosol spatial distributions and optical and microphysical properties.

  17. Oil shale, tar sand, coal research advanced exploratory process technology, jointly sponsored research

    SciTech Connect (OSTI)

    Speight, J.G.

    1992-01-01

    Accomplishments for the past quarter are presented for the following five tasks: oil shale; tar sand; coal; advanced exploratory process technology; and jointly sponsored research. Oil shale research covers oil shale process studies. Tar sand research is on process development of Recycle Oil Pyrolysis and Extraction (ROPE) Process. Coal research covers: coal combustion; integrated coal processing concepts; and solid waste management. Advanced exploratory process technology includes: advanced process concepts;advanced mitigation concepts; and oil and gas technology. Jointly sponsored research includes: organic and inorganic hazardous waste stabilization; CROW field demonstration with Bell Lumber and Pole; development and validation of a standard test method for sequential batch extraction fluid; PGI demonstration project; operation and evaluation of the CO[sub 2] HUFF-N-PUFF Process; fly ash binder for unsurfaced road aggregates; solid state NMR analysis of Mesaverde Group, Greater Green River Basin, tight gas sands; flow-loop testing of double-wall pipe for thermal applications; characterization of petroleum residue; shallow oil production using horizontal wells with enhanced oil recovery techniques; surface process study for oil recovery using a thermal extraction process; NMR analysis of samples from the ocean drilling program; in situ treatment of manufactured gas plant contaminated soils demonstration program; and solid state NMR analysis of naturally and artificially matured kerogens.

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ARM Program Surface Measurements for Aerosol Profiles Shown to Represent Integrated Column Measurements Submitter: Andrews, E., University of Colorado Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Andrews, E., P. J. Sheridan, J. A. Ogren, and R. Ferrare (2004), In situ aerosol profiles over the Southern Great Plains cloud and radiation test bed site: 1. Aerosol optical properties, J. Geophys. Res., 109, D06208, doi:10.1029/2003JD004025. Delle Monache, L., K.

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Cloud Droplet Spectral Shape Sheds New Light on Aerosol-Cloud-Interaction Regimes Download a printable PDF Submitter: Liu, Y., Brookhaven National Laboratory Zhang, M., Stony Brook University Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Chen J, Y Liu, M Zhang, and Y Peng. 2016. "New understanding and quantification of the regime dependence of aerosol-cloud interaction for studying aerosol indirect

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Climatology of Aerosol Optical Depth in North-Central Oklahoma: 1992-2008 Download a printable PDF Submitter: Michalsky, J. J., Cooperative Institute for Research in Environmental Sciences Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Michalsky J, F Denn, C Flynn, G Hodges, P Kiedron, A Koontz, J Schlemmer, and SE Schwartz. 2010. "Climatology of aerosol optical depth in north-central Oklahoma: 1992-2008." Journal of Geophysical Research -

  1. Carbonaceous Aerosols and Radiative...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    carbon, primary organic aerosols (POA), and secondary organic aerosols (SOA) from both man-made and biogenic sources. Black carbon and primary organic aerosols are emitted...

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MBL Cloud Properties Derived from the Azores-AMF Observations Submitter: Dong, X., University of North Dakota Area of Research: Cloud Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Dong X, B Xi, A Kennedy, P Minnis, and R Wood. 2014. "A 19-month record of marine aerosol-cloud-radiation properties derived from DOE ARM AMF deployment at the Azores: Part I: Cloud fraction and single-layered MBL cloud properties." Journal of Climate, 27(10),

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Probing the Birth of New Particles Download a printable PDF Submitter: Wang, J., Brookhaven National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Chen M, M Titcombe, J Jiang, C Jen, C Kuang, ML Fischer, FL Eisele, I Siepmann, DR Hanson, J Zhao, and PH McMurry. 2012. "Acid-base chemical reaction model for nucleation rates in the polluted atmospheric boundary layer." Proceedings of the National Academy of Sciences, 109(46),

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    A Decade and Counting Download a printable PDF Submitter: Long, C. N., NOAA Global Monitoring Division/CIRES Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Long CN, SA McFarlane, A Del Genio, P Minnis, TP Ackerman, J Mather, J Comstock, GG Mace, M Jensen, and C Jakob. 2013. "ARM research in the equatorial western Pacific - a decade and counting." Bulletin of the American Meteorological Society, 94(5),

  5. ARM - Two-Column Aerosol Project (TCAP)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    science objectives, the Atmospheric Radiation Measurement (ARM) Climate Research Facility will deploy the ARM Mobile Facility and the Mobile Aerosol Observing System on Cape...

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: China S, G Kulkarni, BV Scarnato, N Sharma, M Pekour, JE Shilling, J Wilson, A ...

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    To Rain or Not to Rain...Aerosols May Be the Answer Download a printable PDF Submitter: Li, Z., University of Maryland Area of Research: Cloud-Aerosol-Precipitation Interactions...

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Invisible Giants in the Sky Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Kassianov E, M Pekour, and J Barnard. 2012. "Aerosols in central California: Unexpectedly large contribution of coarse mode to aerosol radiative forcing." Geophysical Research Letters, 39, L20806, doi:10.1029/2012GL053469. Photo

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Overambitious Other Carbon Submitter: Church, J., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Song C, M Gyawali, RA Zaveri, JE Shilling, and WP Arnott. 2013. "Light absorption by secondary organic aerosol from α-pinene: Effects of oxidants, seed aerosol acidity, and relative humidity." Journal of Geophysical Research - Atmospheres, 118, doi:10.1002/jgrd.50767. Time-dependent Mass Absorption

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MBL Aerosol Properties and Their Impact on CCN at the Azores-AMF Site Download a printable PDF Submitter: Dong, X., University of North Dakota Area of Research: Aerosol Properties Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Logan T, B Xi, and X Dong. 2014. "Aerosol properties and their influences on marine boundary layer cloud condensation nuclei at the ARM mobile facility over the Azores." Journal of Geophysical Research - Atmospheres, 119(8),

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Quantifying Error in the Radiative Forcing of the First Aerosol Indirect Effect Submitter: McComiskey, A. C., National Oceanic and Atmospheric Administration Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Submitted to Geophysical Research Letters, 06-27-2007. Radiative forcing of aerosol indirect as function of CCN number density and LWP in units of W/m2 per 5% IE error. A survey of recently published works shows that values used to represent the magnitude of

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Characterization of Atmospheric Aerosols Using MFRSR Measurements Download a printable PDF Submitter: Alexandrov, M. D., Columbia University Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Alexandrov, MD, AA Lacis, BE Carlson, and B Cairns. 2007. "Characterization of atmospheric aerosols using MFRSR measurements." (Journal of Geophysical Research 113, DO8204. Sample spectral optical depths of atmospheric constituents in 300 - 900 nm spectral range:

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Atmospheric Aerosol Measurements on Cloudy Days: a New Method Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Ovchinnikov, M., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Kassianov, EI, and M Ovtchinnikov. 2008. "On reflectance ratios and aerosol optical depth retrieval in the presence of cumulus clouds." Geophysical Research Letters doi:10.1029/2008GL033231.

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Observations of the First Aerosol Indirect Effect in Shallow Cumuli Download a printable PDF Submitter: Berg, L., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Berg LK, CM Berkowitz, JC Barnard, G Senum, and SR Springston. 2011. "Observations of the first aerosol indirect effect in shallow cumuli." Geophysical Research Letters, 38, L03809, 10.1029/2010GL046047. Mean value of (a)

  15. Oil shale, tar sand, coal research, advanced exploratory process technology, jointly sponsored research

    SciTech Connect (OSTI)

    Not Available

    1992-01-01

    Progress made in five research programs is described. The subtasks in oil shale study include oil shale process studies and unconventional applications and markets for western oil shale.The tar sand study is on recycle oil pyrolysis and extraction (ROPE) process. Four tasks are described in coal research: underground coal gasification; coal combustion; integrated coal processing concepts; and sold waste management. Advanced exploratory process technology includes: advanced process concepts; advanced mitigation concepts; and oil and gas technology. Jointly sponsored research covers: organic and inorganic hazardous waste stabilization; CROW field demonstration with Bell Lumber and Pole; development and validation of a standard test method for sequential batch extraction fluid; PGI demonstration project; operation and evaluation of the CO[sub 2] HUFF-N-PUFF process; fly ash binder for unsurfaced road aggregates; solid state NMR analysis of Mesaverde group, Greater Green River Basin, tight gas sands; flow-loop testing of double-wall pipe for thermal applications; shallow oil production using horizontal wells with enhanced oil recovery techniques; NMR analysis of sample from the ocean drilling program; and menu driven access to the WDEQ hydrologic data management system.

  16. eDPS Aerosol Collection

    SciTech Connect (OSTI)

    Venzie, J.

    2015-10-13

    The eDPS Aerosol Collection project studies the fundamental physics of electrostatic aerosol collection for national security applications. The interpretation of aerosol data requires understanding and correcting for biases introduced from particle genesis through collection and analysis. The research and development undertaken in this project provides the basis for both the statistical correction of existing equipment and techniques; as well as, the development of new collectors and analytical techniques designed to minimize unwanted biases while improving the efficiency of locating and measuring individual particles of interest.

  17. 2004 research briefs :Materials and Process Sciences Center.

    SciTech Connect (OSTI)

    Cieslak, Michael J.

    2004-01-01

    This report is the latest in a continuing series that highlights the recent technical accomplishments associated with the work being performed within the Materials and Process Sciences Center. Our research and development activities primarily address the materials-engineering needs of Sandia's Nuclear-Weapons (NW) program. In addition, we have significant efforts that support programs managed by the other laboratory business units. Our wide range of activities occurs within six thematic areas: Materials Aging and Reliability, Scientifically Engineered Materials, Materials Processing, Materials Characterization, Materials for Microsystems, and Materials Modeling and Simulation. We believe these highlights collectively demonstrate the importance that a strong materials-science base has on the ultimate success of the NW program and the overall DOE technology portfolio.

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Modeling Aerosols in Fair-Weather Clouds During CHAPS Download a printable PDF Submitter: Shrivastava, M., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Shrivastava M, LK Berg, J Fast, R Easter, A Laskin, WI Gustafson, Y Liu, and CM Berkowitz. 2013. "Modeling aerosols and their interactions with shallow cumuli during the 2007 CHAPS field study." Journal of

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Initial Aerosol Concentration Is Key Contributor to Low-Level Cloud Reflectivity Submitter: Penner, J. E., University of Michigan Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Penner, J., Dong, X., Chen. Y., Observational evidence of a change in radiative forcing due to the indirect aerosol effect, Nature, Vol. 427, 15 January 2004. Cloud optical depth, as determined from the parcel model, is indicated by the dots. Red lines show best fit data of cloud liquid

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Light Absorption of Primary Organic Aerosol Paper Named ACS Editors' Choice Download a printable PDF Submitter: Lu, Z., Argonne National Laboratory Streets, D. ., Argonne National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Lu Z, DG Streets, E Winijkul, F Yan, Y Chen, TC Bond, Y Feng, MK Dubey, S Liu, JP Pinto, and GR Carmichael. 2015. "Light absorption properties and radiative effects of primary organic aerosol emissions."

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Arctic Haze: Effect of Anthropogenic and Biomass Burning Aerosols Transported from Europe to the Arctic Download a printable PDF Submitter: Fast, J. ., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Marelle L, J Raut, JL Thomas, KS Law, B Quennehen, G Ancellet, J Pelon, A Schwarzenboeck, and JD Fast. 2015. "Transport of anthropogenic and biomass burning aerosols from Europe to the

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Radiative and Thermodynamic Responses to Uncertainty in Aerosol Extinction Profiles Download a printable PDF Submitter: Feng, Y., Argonne National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Feng Y, R Kotamarthi, R Coulter, C Zhao, and M Cadeddu. 2016. "Radiative and Thermodynamic Responses to Aerosol Extinction Profiles during the Pre-monsoon Month over South Asia." Atmospheric Chemistry and Physics, 16(1), 247-264. WRF-Chem

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    CCN Activity and Mixing Rules of Isoprene Secondary Organic Aerosol (SOA) and Sulfate Download a printable PDF Submitter: Martin, S. T., Harvard University Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: King SM, T Rosenoern, JH Shilling, Q Chen, Z Wang, G Biskos, KA McKinney, U Poeschl, and ST Martin. 2010. "Cloud droplet activation of mixed organic-sulfate particles produced by the photooxidation of

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ice Nucleation Link to Aerosols for Global Models Download a printable PDF Submitter: DeMott, P. J., Colorado State University Liu, X., University of Wyoming Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: DeMott PJ, AJ Prenni, X Liu, SM Kreidenweis, MD Petters, CH Twohy, MS Richardson, T Eidhammer, and DC Rogers. 2010. "Predicting global atmospheric ice nuclei distributions and their impacts on

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Simulating the Impact of Aerosols on Tropical Deep Convection Download a printable PDF Submitter: Morrison, H. C., NCAR Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Morrison H and WW Grabowski. 2011. "Cloud-system resolving model simulations of aerosol indirect effects on tropical deep convection and its thermodynamic environment." Atmospheric Chemistry and Physics, 11(20),

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    CAM5 Shows Reasonable Aerosol First Indirect Effects on Non-Precipitating Low Liquid Clouds Download a printable PDF Submitter: Zhao, C., Beijing Normal University Klein, S., Lawrence Livermore National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Zhao C, SA Klein, S Xie, X Liu, JS Boyle, and Y Zhang. 2012. "Aerosol first indirect effects on non-precipitating low-level

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    How Aerosols Affect Cloud Properties in Arctic Mixed-Phase Stratocumulus Download a printable PDF Submitter: McFarquhar, G., University of Illinois, Urbana Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Jackson RC, GM McFarquhar, AV Korolev, ME Earle, PS Liu, RP Lawson, S Brooks, M Wolde, A Laskin, and M Freer. 2012. "The dependence of ice microphysics on aerosol concentration in arctic mixed-phase

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    A Tall Order: Climate Models Fall Short in Predicting African Sahel Rainfall Download a printable PDF Submitter: Roehrig, R., Meteo-France CNRM/GMME/MOANA Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Roehrig R, D Bouniol, F Guichard, F Hourdin, and JL Redelsperger. 2013. "The present and future of the West African Monsoon: A process-oriented assessment of CMIP5 simulations along

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Emergence of Open Source Software for the Weather Radar Community Download a printable PDF Submitter: Collis, S. M., Argonne National Laboratory Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Heistermann M, S Collis, MJ Dixon, SE Giangrande, JJ Helmus, B Kelley, J Koistinen, DB Michelson, P Markus, T Pfaff, and DB Wolff. 2014. "The Emergence of Open Source Software for the Weather Radar Community."

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Anatomy and Physics of ZDR Columns Submitter: Kumjian, M., Pennsylvania State University Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Kumjian MR, AP Khain, N Benmoshe, E Ilotoviz, AV Ryzhkov, and VT Phillips. 2014. "The anatomy and physics of ZDR columns: Investigating a polarimetric radar signature with a spectral bin microphysical model." Journal of Applied Meteorology and Climatology, 53(7),

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    A New Theory of Time-dependent Freezing and Its Application to Investigation of Formation of Hail Download a printable PDF Submitter: Khain, A., The Hebrew University of Jerusalem Phillips, V., University of Leeds Area of Research: Cloud Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Phillips VT, A Khain, N Benmoshe, E Ilotoviz, and A Ryzhkov. 2014. "Theory of time-dependent freezing. II: Scheme for freezing raindrops and simulations by a cloud model

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Modeling Dust as Component Minerals in the Community Atmosphere Model Download a printable PDF Submitter: Ghan, S. J., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Scanza R, N Mahowald, S Ghan, CS Zender, JF Kok, Y Zhang, and S Albani. 2015. "Modeling dust as component minerals in the Community Atmosphere Model: development of framework and impact on radiative forcing."

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Modeling Precipitating Cumulus Congestus Observed by the ARM Radar Suite During the MC3E Field Campaign Download a printable PDF Submitter: Mechem, D. B., University of Kansas Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Mechem DB, SE Giangrande, CS Wittman, P Borque, T Toto, and P Kollias. 2015. "Insights from modeling and observational evaluation of a precipitating continental cumulus event observed

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    An Improved Hindcast Approach for Evaluation and Diagnosis of Physical Processes in GCMs Download a printable PDF Submitter: Ma, H., Lawrence Livermore National Laboratory Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Ma H, C Chuang, SA Klein, M Lo, Y Zhang, S Xie, X Zheng, P Ma, Y Zhang, and TJ Phillips. 2015. "An improved hindcast approach for evaluation and

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Cloud Susceptibility Measures Potential Cloud Sensitivity to First Aerosol Indirect Effect Download a printable PDF Submitter: Oreopoulos, L., NASA Platnick, S., NASA - Goddard Space Flight Center Area of Research: Cloud Distributions/Characterizations Working Group(s): Radiative Processes Journal Reference: Platnick, S, and L Oreopoulos. 2008. "Radiative susceptibility of cloudy atmospheres to droplet number perturbations: 1. Theoretical analysis and examples from MODIS." Journal of

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Black Carbon Reduction of Snow Albedo Submitter: Kirchstetter, T. W., Lawrence Berkeley National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Hadley OL and TW Kirchstetter. 2012. "Black carbon reduction of snow albedo." Nature Climate Change, , doi:10.1038/nclimate1433. Spectrally weighted snow albedo over the 300-2,500 nm solar spectrum: derived from our experiments (dots, 1 standard deviation) and modelled using SNICAR

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Diurnal Cycle of Monsoon Clouds, Precipitation, and Surface Radiation Download a printable PDF Submitter: Long, C. N., NOAA Global Monitoring Division/CIRES May, P. T., Bureau of Meteorology Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: May PT, CN Long, and A Protat. 2012. "The diurnal cycle of the boundary layer, convection, clouds, and surface radiation in a coastal monsoon environment (Darwin

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Looking at the Full Spectrum for Water Vapor Download a printable PDF Submitter: Turner, D. D., National Oceanic and Atmospheric Administration Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Mlawer EJ, VH Payne, J Moncet, JS Delamere, MJ Alvarado, and DD Tobin. 2012. "Development and recent evaluation of the MT_CKD model of continuum absorption." Philosophical Transactions of The Royal Society A, 370, doi:

  19. Ganges Valley Aerosol Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ganges Valley Aerosol Experiment In northeastern India, the fertile land around the Ganges River supports several hundred million people. This river, the largest in India, is fed by monsoon rains and runoff from the nearby Himalayan Mountains. Through an intergovernmental agreement with India, the U.S. Department of Energy's Atmospheric Radiation Measurement (ARM) Climate Research Facility deployed its portable laboratory, the ARM Mobile Facility (AMF), to Nainital, India, in June 2011. During

  20. Aerosol Working Group Contributions Accomplishments for 2006

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Contributions Accomplishments for 2006 Aerosol IOP '03 Field Campaign Yields 18-Paper Special Issue of JGR The ARM Aerosol Intensive Operation Period (IOP) field campaign in 2003 has yielded an unprecedented eighteen peer-reviewed papers published in a special issue of the Journal of Geophysical Research. These papers capture the state of the science in terms of measurement of the optical properties of ambient-state aerosols. This special issue includes results from successful

  1. ARM - Measurement - Aerosol concentration

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    CSPHOT : Cimel Sunphotometer CPC : Condensation Particle Counter HTDMA : Humidified Tandem Differential Mobility Analyzer IAP : In-situ Aerosol Profiles (Cessna Aerosol Flights)...

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    to Lose Download a printable PDF Submitter: Laskin, A., Pacific Northwest National Laboratory Fast, J. ., Pacific Northwest National Laboratory Area of Research: Aerosol...

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Influence of Dust Composition on Cloud Droplet Formation Download a printable PDF Submitter: Chuang, C., Lawrence Livermore National Laboratory Area of Research: Aerosol Properties...

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Long-Term Impacts of Aerosols on the Vertical Development of Clouds and Precipitation Download a printable PDF Submitter: Li, Z., University of Maryland Area of Research:...

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Fog and Rain in the Amazon Download a printable PDF Submitter: Gentine, P., Columbia University Sobel, A., Columbia University Area of Research: Cloud-Aerosol-Precipitation...

  6. Final Technical Report for Collaborative Research: CRI-EaSM Multiscale Modeling Aerosol Indirect Effects on Decadal Timescales

    SciTech Connect (OSTI)

    Park, Sungsu

    2015-11-29

    Originally, the main role of the P.I. (Sungsu Park) in this project was to improve the treatment of cloud microphysics in the CAM5 shallow and deep convection scheme. During the progress of the project, however, the main research theme was changed to develop a new unified convection scheme (so called, UNICON) with the permission of the program manager.

  7. RESEARCH ON CARBON PRODUCTS FROM COAL USING AN EXTRACTIVE PROCESS

    SciTech Connect (OSTI)

    Peter G. Stansberry; Alfred H. Stiller; John W. Zondlo; Chong Chen; Brian Bland; David Fenton

    2002-03-31

    This report presents the results of a one-year effort directed at the exploration of the use of coal as a feedstock for a variety of industrially-relevant carbon products. The work was basically divided into three focus areas. The first area dealt with the acquisition of laboratory equipment to aid in the analysis and characterization of both the raw coal and the coal-derived feedstocks. Improvements were also made on the coal-extraction pilot plant which will now allow larger quantities of feedstock to be produced. Mass and energy balances were also performed on the pilot plant in an attempt to evaluate the scale-up potential of the process. The second focus area dealt with exploring hydrogenation conditions specifically aimed at testing several less-expensive candidate hydrogen-donor solvents. Through a process of filtration and vacuum distillation, viable pitch products were produced and evaluated. Moreover, a recycle solvent was also isolated so that the overall solvent balance in the system could be maintained. The effect of variables such as gas pressure and gas atmosphere were evaluated. The pitch product was analyzed and showed low ash content, reasonable yield, good coking value and a coke with anisotropic optical texture. A unique plot of coke yield vs. pitch softening point was discovered to be independent of reaction conditions or hydrogen-donor solvent. The third area of research centered on the investigation of alternate extraction solvents and processing conditions for the solvent extraction step. A wide variety of solvents, co-solvents and enhancement additives were tested with varying degrees of success. For the extraction of raw coal, the efficacy of the alternate solvents when compared to the benchmark solvent, N-methyl pyrrolidone, was not good. However when the same coal was partially hydrogenated prior to solvent extraction, all solvents showed excellent results even for extractions performed at room temperature. Standard analyses of the extraction products indicated that they had the requisite properties of viable carbon-product precursors.

  8. Thermochemical Process Development Unit: Researching Fuels from Biomass, Bioenergy Technologies (Fact Sheet)

    SciTech Connect (OSTI)

    Not Available

    2009-01-01

    The Thermochemical Process Development Unit (TCPDU) at the National Renewable Energy Laboratory (NREL) is a unique facility dedicated to researching thermochemical processes to produce fuels from biomass.

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Retrieving Cloud and Aerosol Properties from the ARM Raman Lidar Download a printable PDF Submitter: Thorsen, T., NASA - Langley Research Center Fu, Q., University of Washington Area of Research: Cloud Distributions/Characterizations Working Group(s): Aerosol Life Cycle, Cloud Life Cycle Journal Reference: Thorsen TJ, Q Fu, RK Newsom, DD Turner, and JM Comstock. 2015. "Automated retrieval of cloud and aerosol properties from the ARM Raman lidar, Part I: Feature detection." Journal of

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Birth and Growth of an Aerosol For original submission and image(s), see ARM Research Highlights http://www.arm.gov/science/highlights/ Research Highlight Tiny atmospheric aerosols are some of the most highly studied particles connected with Planet Earth, yet questions remain on how they are formed and how they affect climate. Now Pacific Northwest National Laboratory scientists have developed new approaches to accurately model the birth and growth of these important aerosols. "Most

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Cumuli Impact on Solar Radiation at Surface: Spectral Changes Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle, Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Kassianov E, J Barnard, LK Berg, CN Long, and C Flynn. 2011. "Shortwave spectral radiative forcing of cumulus clouds from surface observations." Geophysical Research Letters, 38, L07801,

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Pollution + Storm Clouds = Warmer Atmosphere Download a printable PDF Submitter: Fan, J., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Fan J, D Rosenfeld, Y Ding, L Leung, and Z Li. 2012. "Potential aerosol indirect effects on atmospheric circulation and radiative forcing through deep convection." Geophysical Research Letters, 39, L09806,

  13. Wind Program Manufacturing Research Advances Processes and Reduces...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    to Access Higher Wind Resources and Lower the Cost of Energy funding opportunity ... through the DOE's Small Business Innovation Research and Small Business ...

  14. FY 2011 Second Quarter: Demonstration of New Aerosol Measurement Verification Testbed for Present-Day Global Aerosol Simulations

    SciTech Connect (OSTI)

    Koch, D

    2011-03-20

    The regional-scale Weather Research and Forecasting (WRF) model is being used by a DOE Earth System Modeling (ESM) project titled Improving the Characterization of Clouds, Aerosols and the Cryosphere in Climate Models to evaluate the performance of atmospheric process modules that treat aerosols and aerosol radiative forcing in the Arctic. We are using a regional-scale modeling framework for three reasons: (1) It is easier to produce a useful comparison to observations with a high resolution model; (2) We can compare the behavior of the CAM parameterization suite with some of the more complex and computationally expensive parameterizations used in WRF; (3) we can explore the behavior of this parameterization suite at high resolution. Climate models like the Community Atmosphere Model version 5 (CAM5) being used within the Community Earth System Model (CESM) will not likely be run at mesoscale spatial resolutions (1020 km) until 510 years from now. The performance of the current suite of physics modules in CAM5 at such resolutions is not known, and current computing resources do not permit high-resolution global simulations to be performed routinely. We are taking advantage of two tools recently developed under PNNL Laboratory Directed Research and Development (LDRD) projects for this activity. The first is the Aerosol Modeling Testbed (Fast et al., 2011b), a new computational framework designed to streamline the process of testing and evaluating aerosol process modules over a range of spatial and temporal scales. The second is the CAM5 suite of physics parameterizations that have been ported into WRF so that their performance and scale dependency can be quantified at mesoscale spatial resolutions (Gustafson et al., 2010; with more publications in preparation).

  15. Particulate Matter Aerosols

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Particulate Matter Aerosols The study of atmospheric aerosols is important because of its adverse effects on health, air quality, visibility, cultural heritage, and Earth's radiation balance. Techniques that can help better characterize particulate matter are required to better understand the constituents, causes and sources of particulate matter (PM) aerosols. Carbon is one of the main constituents of atmospheric aerosols. Radiocarbon (14C) measurement performed on aerosol particulate matter

  16. Parameterizations of Cloud Microphysics and Indirect Aerosol Effects

    Office of Scientific and Technical Information (OSTI)

    (Technical Report) | SciTech Connect Parameterizations of Cloud Microphysics and Indirect Aerosol Effects Citation Details In-Document Search Title: Parameterizations of Cloud Microphysics and Indirect Aerosol Effects 1. OVERVIEW Aerosols and especially their effect on clouds are one of the key components of the climate system and the hydrological cycle [Ramanathan et al., 2001]. Yet, the aerosol effect on clouds remains largely unknown and the processes involved not well understood. A

  17. Assessing regional scale predictions of aerosols, marine stratocumulus, and their interactions during VOCALS-REx using WRF-Chem

    SciTech Connect (OSTI)

    Yang Q.; Lee Y.; Gustafson Jr., W. I.; Fast, J. D.; Wang, H.; Easter, R. C.; Morrison, H.; Chapman, E. G.; Spak, S. N.; Mena-Carrasco, M. A.

    2011-12-02

    This study assesses the ability of the recent chemistry version (v3.3) of the Weather Research and Forecasting (WRF-Chem) model to simulate boundary layer structure, aerosols, stratocumulus clouds, and energy fluxes over the Southeast Pacific Ocean. Measurements from the VAMOS Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-REx) and satellite retrievals (i.e., products from the MODerate resolution Imaging Spectroradiometer (MODIS), Clouds and Earth's Radiant Energy System (CERES), and GOES-10) are used for this assessment. The Morrison double-moment microphysics scheme is newly coupled with interactive aerosols in the model. The 31-day (15 October-16 November 2008) WRF-Chem simulation with aerosol-cloud interactions (AERO hereafter) is also compared to a simulation (MET hereafter) with fixed cloud droplet number concentrations in the microphysics scheme and simplified cloud and aerosol treatments in the radiation scheme. The well-simulated aerosol quantities (aerosol number, mass composition and optical properties), and the inclusion of full aerosol-cloud couplings lead to significant improvements in many features of the simulated stratocumulus clouds: cloud optical properties and microphysical properties such as cloud top effective radius, cloud water path, and cloud optical thickness. In addition to accounting for the aerosol direct and semi-direct effects, these improvements feed back to the simulation of boundary-layer characteristics and energy budgets. Particularly, inclusion of interactive aerosols in AERO strengthens the temperature and humidity gradients within the capping inversion layer and lowers the marine boundary layer (MBL) depth by 130 m from that of the MET simulation. These differences are associated with weaker entrainment and stronger mean subsidence at the top of the MBL in AERO. Mean top-of-atmosphere outgoing shortwave fluxes, surface latent heat, and surface downwelling longwave fluxes are in better agreement with observations in AERO, compared to the MET simulation. Nevertheless, biases in some of the simulated meteorological quantities (e.g., MBL temperature and humidity) and aerosol quantities (e.g., underestimations of accumulation mode aerosol number) might affect simulated stratocumulus and energy fluxes over the Southeastern Pacific, and require further investigation. The well-simulated timing and outflow patterns of polluted and clean episodes demonstrate the model's ability to capture daily/synoptic scale variations of aerosol and cloud properties, and suggest that the model is suitable for studying atmospheric processes associated with pollution outflow over the ocean. The overall performance of the regional model in simulating mesoscale clouds and boundary layer properties is encouraging and suggests that reproducing gradients of aerosol and cloud droplet concentrations and coupling cloud-aerosol-radiation processes are important when simulating marine stratocumulus over the Southeast Pacific.

  18. DOE - Office of Legacy Management -- Separations Process Research...

    Office of Legacy Management (LM)

    and operated by the Atomic Energy Commission as a pilot plant for developing and testing the chemical processes to extract both uranium and plutonium from irradiated fuel. ...

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Bimodal CCN Spectra Download a printable PDF Submitter: Hudson, J. G., Desert Research Institute Area of Research: Cloud Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: N/A Figure 1. Differential CCN concentrations (per cm3) against critical supersaturation (Sc) for MASE below cloud CCN spectra for each of the 8 modal categories. (a) cat 1, (b) cat 2, (c) cat 3, (d) cat 4, (e) cat 5, (f) cat 6, (g) cat 7, (h) cat 8. Sc in percent for, Hoppel minima are

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Improving the Treatment of Radiation in Climate Models Download a printable PDF Submitter: Delamere, J. S., Tech-X Corporation Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle, Cloud Life Cycle Journal Reference: Delamere JS, SA Clough, VH Payne, EJ Mlawer, DD Turner, and RR Gamache. 2010. "A far-infrared radiative closure study in the Arctic: Application to water vapor." Journal of Geophysical Research - Atmospheres, 115, D17106, 10.1029/2009JD012968. The

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Deciphering Raindrop Collisions with Dual-polarization Radar Download a printable PDF Submitter: Kumjian, M., Pennsylvania State University Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Kumjian MR and OP Prat. 2014. "The impact of raindrop collisional processes on the polarimetric radar variables." Journal of the Atmospheric Sciences, 71(8), doi:10.1175/JAS-D-13-0357.1. (a) Changes in ZDR as a function

  2. "Big Picture" Process Modeling Tools |GE Global Research

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Using process modeling tools to attain cost-effective results for GE customers Click to email this to a friend (Opens in new window) Share on Facebook (Opens in new window) Click ...

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Partly Cloudy with a Chance of Aerosol Download a printable PDF Submitter: Chand, D., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Chand D, R Wood, SJ Ghan, M Wang, M Ovchinnikov, PJ Rasch, S Miller, B Schichtel, and T Moore. 2012. "Aerosol optical depth increase in partly cloudy conditions." Journal of Geophysical Research, 117, D17207, doi:10.1029/2012JD017894. The sky can appear nearly clear or

  4. Study of Mechanisms of Aerosol Indirect Effects on Glaciated...

    Office of Scientific and Technical Information (OSTI)

    ... clouds, was seen to be of higher importance in regulating aerosol indirect effects ... DOE Contract Number: SC0007396 Resource Type: Technical Report Research Org: Leeds ...

  5. Light Absorption of Primary Organic Aerosol Paper Named ACS Editors...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Absorption of Primary Organic Aerosol Paper Named ACS Editors' Choice For original submission and image(s), see ARM Research Highlights http:www.arm.govsciencehighlights...

  6. BAECC Biogenic Aerosols - Effects on Clouds and Climate (Technical...

    Office of Scientific and Technical Information (OSTI)

    The main research goal was to understand the role of biogenic aerosols in cloud formation. ... Country of Publication: United States Language: English Subject: 54 ENVIRONMENTAL SCIENCES ...

  7. Aerosol mobility size spectrometer

    DOE Patents [OSTI]

    Wang, Jian; Kulkarni, Pramod

    2007-11-20

    A device for measuring aerosol size distribution within a sample containing aerosol particles. The device generally includes a spectrometer housing defining an interior chamber and a camera for recording aerosol size streams exiting the chamber. The housing includes an inlet for introducing a flow medium into the chamber in a flow direction, an aerosol injection port adjacent the inlet for introducing a charged aerosol sample into the chamber, a separation section for applying an electric field to the aerosol sample across the flow direction and an outlet opposite the inlet. In the separation section, the aerosol sample becomes entrained in the flow medium and the aerosol particles within the aerosol sample are separated by size into a plurality of aerosol flow streams under the influence of the electric field. The camera is disposed adjacent the housing outlet for optically detecting a relative position of at least one aerosol flow stream exiting the outlet and for optically detecting the number of aerosol particles within the at least one aerosol flow stream.

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Fair-Weather Clouds Hold Dirty Secret Download a printable PDF Submitter: Shrivastava, M., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Shrivastava MB, JD Fast, RC Easter, WI Gustafson, RA Zaveri, JL Jimenez, P Saide, and A Hodzic. 2011. "Modeling organic aerosols in a megacity: Comparison of simple and complex representations of the volatility basis set

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Phase State and Physical Properties of Ambient and Lab Generated Aerosols: X-ray Microscopy Download a printable PDF Submitter: OBrien, R. E., Lawrence Berkeley National Laboratory Gilles, M., Lawrence Berkeley National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: O'Brien RE, A Neu, SA Epstein, AC MacMillan, B Wang, ST Kelly, SA Nizkorodov, A Laskin, RC Moffet, and MK Gilles. 2014. "Physical properties of ambient and

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Clouds, Aerosol, and Precipitation in the Marine Boundary Layer: an ARM Mobile Facility Deployment Download a printable PDF Submitter: Wood, R., University of Washington Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: N/A Composite seasonal cycles of (a) cloud droplet concentration retrieved using a variety of methods; (b) surface measured cloud condensation nuclei concentrations at four supersaturations.

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    a Cloud-Resolving Model to Identify the Role of Aerosols on Clouds and Precipitation Download a printable PDF Submitter: GSFC, N., NASA GSFC Area of Research: Cloud Distributions/Characterizations Working Group(s): Aerosol, Cloud Modeling Journal Reference: Tao, W.-K., X. Li, A. Khain, T. Matsui, S. Lang, and J. Simpson, 2007: The role of atmospheric aerosol concentration on deep convective precipitation: Cloud-resolving model simulations. J. Geophy. Res., (accepted). Zeng, X., W.-K. Tao, S.

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Indirect Impact of Atmospheric Aerosols on an Ensemble of Deep Convective Clouds Download a printable PDF Submitter: Grabowski, W., NCAR Morrison, H. C., NCAR Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Grabowski WW and H Morrison. 2011. "Indirect impact of atmospheric aerosols in idealized simulations of convective-radiative quasi-equilibrium. Part II: Double-moment microphysics." Journal of

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Anthropogenic Aerosols: a Clearer Understanding Submitter: Daum, P., Brookhaven National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Liu, Y., and P. H. Daum, 2002: "Indirect warming effect from dispersion forcing," Nature 419(6872):580-581. Figure 1. Key = Green symbols: triangle - FIRE, northeastern Pacific; Crossed circles - SOCEX, Southern Ocean; Filled circle - ACE1, Southern Ocean; Blue symbols: Filled circles - ASTEX 8,

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Pollution Hitches Ride to Arctic Download a printable PDF Submitter: Zelenyuk-Imre, A., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Zelenyuk A, D Imre, J Beranek, E Abramson, J Wilson, and M Shrivastava. 2012. "Synergy between secondary organic aerosols and long-range transport of polycyclic aromatic hydrocarbons." Environmental Science & Technology, 46(22), doi:10.1021/es302743z. When airborne

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Strong Impacts of Vertical Velocity on Cloud Microphysics and Implications for Aerosol Indirect Download a printable PDF Submitter: Liu, Y., Brookhaven National Laboratory Lu, C., Nanjing University of Information Science and Technology Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Lu C, Y Liu, S Niu, and AM Vogelmann. 2012. "Observed impacts of vertical velocity on cloud

  16. NREL: Photovoltaics Research - New Materials, Devices, and Processes for

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Advanced Concepts New Materials, Devices, and Processes for Advanced Concepts Computational Science and Theory We can use high-performance computing tools in modeling and simulation studies of semiconductor and other solar materials. We also determine the performance of solar devices. Theoretical studies can help us understand underlying physical principles or predict useful chemical compositions and crystalline structures. Scientific Computing Experimental Materials Science Solid-State

  17. Research Challenge 3: Competing Radiative and Nonradiative Processes

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    3: Competing Radiative and Nonradiative Processes - Sandia Energy Energy Search Icon Sandia Home Locations Contact Us Employee Locator Energy & Climate Secure & Sustainable Energy Future Stationary Power Energy Conversion Efficiency Solar Energy Wind Energy Water Power Supercritical CO2 Geothermal Natural Gas Safety, Security & Resilience of the Energy Infrastructure Energy Storage Nuclear Power & Engineering Grid Modernization Battery Testing Nuclear Fuel Cycle Defense Waste

  18. ARM - Measurement - Aerosol image

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    would love to hear from you Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol image Images of aerosols from which one can derive characteristics such...

  19. Raman Lidar Measurements of Aerosols and Water Vapor During the May 2003 Aerosol IOP

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Raman Lidar Measurements of Aerosols and Water Vapor During the May 2003 Aerosol IOP R. A. Ferrare National Aeronautics and Space Administration Langley Research Center Hampton, Virginia D. D. Turner Pacific Northwest National Laboratory Richland, Washington M. Clayton Science Applications International Corporation National Aeronautics and Space Administration Langley Research Center Hampton, Virginia B. S. Schmid and J. Redemann BAER/NASA Ames Research Institute Moffett Field, California D.

  20. ARM - Measurement - Aerosol scattering

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    : Nephelometer PASS : Photoacoustic Soot Spectrometer RL : Raman Lidar TDMA : Tandem Differential Mobility Analyzer Field Campaign Instruments AMT : Aerosol Modeling...

  1. Aerosol Observing System Upgraded

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    2 Aerosol Observing System Upgraded The Aerosol Observing System (AOS) at the SGP central facility recently received maintenance and was upgraded to improve its performance. The AOS measures the properties of the aerosol particles around it. Several AOS components were removed, repaired, and calibrated to operate within specifications. The system continuously gathers information about the way minute aerosol particles interact with solar radiation. A better understanding of these interactions

  2. Aerosol distribution apparatus

    DOE Patents [OSTI]

    Hanson, W.D.

    An apparatus for uniformly distributing an aerosol to a plurality of filters mounted in a plenum, wherein the aerosol and air are forced through a manifold system by means of a jet pump and released into the plenum through orifices in the manifold. The apparatus allows for the simultaneous aerosol-testing of all the filters in the plenum.

  3. Solid aerosol generator

    DOE Patents [OSTI]

    Prescott, Donald S.; Schober, Robert K.; Beller, John

    1992-01-01

    An improved solid aerosol generator used to produce a gas borne stream of dry, solid particles of predetermined size and concentration. The improved solid aerosol generator nebulizes a feed solution of known concentration with a flow of preheated gas and dries the resultant wet heated aerosol in a grounded, conical heating chamber, achieving high recovery and flow rates.

  4. Improved solid aerosol generator

    DOE Patents [OSTI]

    Prescott, D.S.; Schober, R.K.; Beller, J.

    1988-07-19

    An improved solid aerosol generator used to produce a gas borne stream of dry, solid particles of predetermined size and concentration. The improved solid aerosol generator nebulizes a feed solution of known concentration with a flow of preheated gas and dries the resultant wet heated aerosol in a grounded, conical heating chamber, achieving high recovery and flow rates. 2 figs.

  5. Solid aerosol generator

    DOE Patents [OSTI]

    Prescott, D.S.; Schober, R.K.; Beller, J.

    1992-03-17

    An improved solid aerosol generator used to produce a gas borne stream of dry, solid particles of predetermined size and concentration is disclosed. The improved solid aerosol generator nebulizes a feed solution of known concentration with a flow of preheated gas and dries the resultant wet heated aerosol in a grounded, conical heating chamber, achieving high recovery and flow rates. 2 figs.

  6. Study of Aerosol Indirect Effects in China

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Indirect Effects in China In 2008, the U.S. Department of Energy (DOE)'s Atmospheric Radiation Measurement (ARM) Climate Research Facility is providing the ARM Mobile Facility (AMF) to conduct a comprehensive investigation of regional aerosol impacts in China as part of a joint program with the Institute of Atmospheric Physics, Chinese Academy of Sciences. The joint program is under the "Climate Sciences" agreement established in 1987 between the DOE and China Ministry of

  7. Aerosol Characterization Data from the Asian Pacific Regional Aerosol Characterization Project (ACE-Asia)

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    The Aerosol Characterization Experiments (ACE) were designed to increase understanding of how atmospheric aerosol particles affect the Earth's climate system. These experiments integrated in-situ measurements, satellite observations, and models to reduce the uncertainty in calculations of the climate forcing due to aerosol particles and improve the ability of models to predict the influences of aerosols on the Earth's radiation balance. ACE-Asia was the fourth in a series of experiments organized by the International Global Atmospheric Chemistry (IGAC) Program (A Core Project of the International Geosphere Biosphere Program). The Intensive Field Phase for ACE-Asia took place during the spring of 2001 (mid-March through early May) off the coast of China, Japan and Korea. ACE-Asia pursued three specific objectives: 1) Determine the physical, chemical, and radiative properties of the major aerosol types in the Eastern Asia and Northwest Pacific region and investigate the relationships among these properties. 2) Quantify the physical and chemical processes controlling the evolution of the major aerosol types and in particular their physical, chemical, and radiative properties. 3) Develop procedures to extrapolate aerosol properties and processes from local to regional and global scales, and assess the regional direct and indirect radiative forcing by aerosols in the Eastern Asia and Northwest Pacific region [Edited and shortened version of summary at http://data.eol.ucar.edu/codiac/projs?ACE-ASIA]. The Ace-Asia collection contains 174 datasets.

  8. Final Report - Independent Verification Survey Activities at the Seperations Process Research Unit Sites, Niskayuna, New York

    SciTech Connect (OSTI)

    Evan Harpenau

    2011-03-15

    The Separations Process Research Unit (SPRU) complex located on the Knolls Atomic Power Laboratory (KAPL) site in Niskayuna, New York, was constructed in the late 1940s to research the chemical separation of plutonium and uranium (Figure A-1). SPRU operated as a laboratory scale research facility between February 1950 and October 1953. The research activities ceased following the successful development of the reduction oxidation and plutonium/uranium extraction processes. The oxidation and extraction processes were subsequently developed for large scale use by the Hanford and Savannah River sites (aRc 2008a). Decommissioning of the SPRU facilities began in October 1953 and continued through the 1990s.

  9. Signal and Image Processing Research at the Lawrence Livermore National Laboratory

    SciTech Connect (OSTI)

    Roberts, R S; Poyneer, L A; Kegelmeyer, L M; Carrano, C J; Chambers, D H; Candy, J V

    2009-06-29

    Lawrence Livermore National Laboratory is a large, multidisciplinary institution that conducts fundamental and applied research in the physical sciences. Research programs at the Laboratory run the gamut from theoretical investigations, to modeling and simulation, to validation through experiment. Over the years, the Laboratory has developed a substantial research component in the areas of signal and image processing to support these activities. This paper surveys some of the current research in signal and image processing at the Laboratory. Of necessity, the paper does not delve deeply into any one research area, but an extensive citation list is provided for further study of the topics presented.

  10. Basic research in engineering: process and systems dynamics and control. High priority research needs relevent to energy

    SciTech Connect (OSTI)

    Rabins, M.J.; Edgar, T.F.; Richardson, H.H.; Zaborszky, J.

    1980-02-01

    At a workshop held in Denver, Colorado, on June 20 to 23, 1979, Process and Systems Dynamics and Control (PSDC) is concerned with the development and control of system behavior, performance criteria, and theories of control and optimization. This report presents a set of high-priority basic engineering research needs in the PSDC field which are important to the development of future energy technologies. The ten high priority generic research areas were aggregeted into four major research needs recommended for DOE support: on-line optimization and control, systems methodology, measurement methodology and instrumentation, and modeling.

  11. Research investigations in oil shale, tar sand, coal research, advanced exploratory process technology, and advanced fuels research: Volume 1 -- Base program. Final report, October 1986--September 1993

    SciTech Connect (OSTI)

    Smith, V.E.

    1994-05-01

    Numerous studies have been conducted in five principal areas: oil shale, tar sand, underground coal gasification, advanced process technology, and advanced fuels research. In subsequent years, underground coal gasification was broadened to be coal research, under which several research activities were conducted that related to coal processing. The most significant change occurred in 1989 when the agreement was redefined as a Base Program and a Jointly Sponsored Research Program (JSRP). Investigations were conducted under the Base Program to determine the physical and chemical properties of materials suitable for conversion to liquid and gaseous fuels, to test and evaluate processes and innovative concepts for such conversions, to monitor and determine environmental impacts related to development of commercial-sized operations, and to evaluate methods for mitigation of potential environmental impacts. This report is divided into two volumes: Volume 1 consists of 28 summaries that describe the principal research efforts conducted under the Base Program in five topic areas. Volume 2 describes tasks performed within the JSRP. Research conducted under this agreement has resulted in technology transfer of a variety of energy-related research information. A listing of related publications and presentations is given at the end of each research topic summary. More specific and detailed information is provided in the topical reports referenced in the related publications listings.

  12. Final Report for Research Conducted at The Scripps Institution of Oceanography, University of California San Diego from 2/2002 to 8/2003 for ''Aerosol and Cloud-Field Radiative Effects in the Tropical Western Pacific: Analyses and General Circulation Model Parameterizations''

    SciTech Connect (OSTI)

    Vogelmann, A. M.

    2004-01-27

    OAK-B135 Final report from the University of California San Diego for an ongoing research project that was moved to Brookhaven National Laboratory where proposed work will be completed. The research uses measurements made by the Atmospheric Radiation Measurement (ARM) Program to quantify the effects of aerosols and clouds on the Earth's energy balance in the climatically important Tropical Western Pacific.

  13. ARM Cloud-Aerosol-Precipitation Experiment (ACAPEX) Field Campaign Report

    Office of Scientific and Technical Information (OSTI)

    (Program Document) | SciTech Connect SciTech Connect Search Results Program Document: ARM Cloud-Aerosol-Precipitation Experiment (ACAPEX) Field Campaign Report Citation Details In-Document Search Title: ARM Cloud-Aerosol-Precipitation Experiment (ACAPEX) Field Campaign Report The U.S. Department of Energy (DOE)'s Atmospheric Radiation Measurement (ARM) Climate Research Facility's ARM Cloud-Aerosol-Precipitation Experiment (ACAPEX) field campaign contributes to CalWater 2015, a multi-agency

  14. ARM - Publications: Science Team Meeting Documents: The SGP Aerosol

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Best-Estimate Value-Added Procedure and Its Impact on the BBHRP Project The SGP Aerosol Best-Estimate Value-Added Procedure and Its Impact on the BBHRP Project Turner, David Pacific Northwest National Laboratory Sivaraman, Chitra Pacific Northwest National Laboratory Flynn, Connor Pacific Northwest National Laboratory Mlawer, Eli Atmospheric & Environmental Research, Inc. The objective of the Aerosol Best-Estimate (ABE) Value-Added Procedure (VAP) is to provide estimates of aerosol

  15. Evaluating Global Aerosol Models and Aerosol and Water Vapor Properties Near Clouds

    SciTech Connect (OSTI)

    Turner, David, D.; Ferrare, Richard, A.

    2011-07-06

    The 'Evaluating Global Aerosol Models and Aerosol and Water Vapor Properties Near Clouds' project focused extensively on the analysis and utilization of water vapor and aerosol profiles derived from the ARM Raman lidar at the Southern Great Plains ARM site. A wide range of different tasks were performed during this project, all of which improved quality of the data products derived from the lidar or advanced the understanding of atmospheric processes over the site. These activities included: upgrading the Raman lidar to improve its sensitivity; participating in field experiments to validate the lidar aerosol and water vapor retrievals; using the lidar aerosol profiles to evaluate the accuracy of the vertical distribution of aerosols in global aerosol model simulations; examining the correlation between relative humidity and aerosol extinction, and how these change, due to horizontal distance away from cumulus clouds; inferring boundary layer turbulence structure in convective boundary layers from the high-time-resolution lidar water vapor measurements; retrieving cumulus entrainment rates in boundary layer cumulus clouds; and participating in a field experiment that provided data to help validate both the entrainment rate retrievals and the turbulent profiles derived from lidar observations.

  16. ARM - AOS Aerosol Properties Plots

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ViewersAOS Aerosol Properties Plots XDC Data Viewers Aerosol Properties Plots SGP AMF NSA (BRW) AOS Aerosol Properties Plots These plots are designed to provide a quick look at the...

  17. ARM - Measurement - Aerosol composition

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    quality assurance purposes. ARM Instruments PILS : Particle Into Liquid Sampler TDMA : Tandem Differential Mobility Analyzer Field Campaign Instruments AEROSMASSSPEC : Aerosol Mass...

  18. ARM - Measurement - Aerosol optical properties

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    : Aerosol optical properties The optical properties of aerosols, including asymmetry factor, phase-function, single-scattering albedo, refractive index, and backscatter...

  19. EMSP Final Report: Electrically Driven Technologies for Radioactive Aerosol Abatement

    SciTech Connect (OSTI)

    DePaoli, D.W.

    2003-01-22

    The purpose of this research project was to develop an improved understanding of how electrically driven processes, including electrocoalescence, acoustic agglomeration, and electric filtration, may be employed to efficiently treat problems caused by the formation of aerosols during DOE waste treatment operations. The production of aerosols during treatment and retrieval operations in radioactive waste tanks and during thermal treatment operations such as calcination presents a significant problem of cost, worker exposure, potential for release, and increased waste volume. There was anecdotal evidence in the literature that acoustic agglomeration and electrical coalescence could be used together to change the size distribution of aerosol particles in such a way as to promote easier filtration and less frequent maintenance of filtration systems. As such, those electrically driven technologies could potentially be used as remote technologies for improved treatment; however, existing theoretical models are not suitable for prediction and design. To investigate the physics of such systems, and also to prototype a system for such processes, a collaborative project was undertaken between Oak Ridge National Laboratory (ORNL) and the University of Texas at Austin (UT). ORNL was responsible for the larger-scale prototyping portion of the project, while UT was primarily responsible for the detailed physics in smaller scale unit reactors. It was found that both electrical coalescence and acoustic agglomeration do in fact increase the rate of aggregation of aerosols. Electrical coalescence requires significantly less input power than acoustic agglomeration, but it is much less effective in its ability to aggregate/coalesce aerosols. The larger-scale prototype showed qualitatively similar results as the unit reactor tests, but presented more difficulty in interpretation of the results because of the complex multi-physics coupling that necessarily occur in all larger-scale system tests. An additional finding from this work is that low-amplitude oscillation may provide an alternative, non-invasive, non-contact means of controlling settling and/or suspension of solids. Further investigation would be necessary to evaluate its utility for radioactive waste treatment applications. This project did not uncover a new technology for radioactive waste treatment. While it may be possible that an efficient electrically driven technology for aerosol treatment could be developed, it appears that other technologies, such as steel and ceramic HEPA filters, can suitably solve this problem. If further studies are to be undertaken, additional fundamental experimentation and modeling is necessary to fully capture the physics; in addition, larger-scale tests are needed to demonstrate the treatment of flowing gas streams through the coupling of acoustic agglomeration with electrocoalescence.

  20. Evaluating Membrane Processes for Air Conditioning; Highlights in Research and Development, NREL (National Renewable Energy Laboratory)

    SciTech Connect (OSTI)

    2015-06-01

    This NREL Highlight discusses a recent state-of-the-art review of membrane processes for air conditioning that identifies future research opportunities. This highlight is being developed for the June 2015 S&T Alliance Board meeting.

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Climate Warming Due to Soot and Smoke? Maybe Not. Submitter: Penner, J. E., University of Michigan Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Penner, J.E., S.Y. Zhang, and C.C. Chuang, Soot and smoke aerosol may not warm climate, J. Geophys. Res., 108(D21), 4657, doi:10.1029/2003JD003409, 2003. New research results from the Department of Energy's Atmospheric Radiation Measurement (ARM) Program suggest that fossil fuel soot emissions and biomass smoke may

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Research Masters the Misunderstood Mixed-Phase Cloud Download a printable PDF Submitter: Ovchinnikov, M., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Ovchinnikov M, AS Ackerman, A Avramov, A Cheng, J Fan, AM Fridland, S Ghan, J Harrington, C Hoose, A Korolev, GM McFarquhar, H Morrison, M Paukert, J Savre, BJ Shipway, MD Shupe, A Solomon, and K

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Are Increases in Thunderstorm Activity in Southeast China Related to Air Pollution? Download a printable PDF Submitter: Li, Z., UALBANY Cribb, M. C., University of Maryland Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Yang X and Z Li. 2014. "Increases in thunderstorm activity and relationships with air pollution in southeast China." Journal of Geophysical Research - Atmospheres, 119(4),

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    From Fire to Ice Download a printable PDF Submitter: Kulkarni, G., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Kulkarni GR, M Nandasiri, A Zelenyuk, J Beranek, N Madaan, A Devaraj, V Shutthanandan, S Thevuthasan, and T Varga. 2015. "Effects of crystallographic properties on the ice nucleation properties of volcanic ash particles." Geophysical Research Letters, 42(8), doi:10.1002/2015GL063270. Tons of

  5. Portable Aerosol Contaminant Extractor

    DOE Patents [OSTI]

    Carlson, Duane C.; DeGange, John J.; Cable-Dunlap, Paula

    2005-11-15

    A compact, portable, aerosol contaminant extractor having ionization and collection sections through which ambient air may be drawn at a nominal rate so that aerosol particles ionized in the ionization section may be collected on charged plate in the collection section, the charged plate being readily removed for analyses of the particles collected thereon.

  6. Direct Aerosol Forcing Uncertainty

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Mccomiskey, Allison

    2008-01-15

    Understanding sources of uncertainty in aerosol direct radiative forcing (DRF), the difference in a given radiative flux component with and without aerosol, is essential to quantifying changes in Earth's radiation budget. We examine the uncertainty in DRF due to measurement uncertainty in the quantities on which it depends: aerosol optical depth, single scattering albedo, asymmetry parameter, solar geometry, and surface albedo. Direct radiative forcing at the top of the atmosphere and at the surface as well as sensitivities, the changes in DRF in response to unit changes in individual aerosol or surface properties, are calculated at three locations representing distinct aerosol types and radiative environments. The uncertainty in DRF associated with a given property is computed as the product of the sensitivity and typical measurement uncertainty in the respective aerosol or surface property. Sensitivity and uncertainty values permit estimation of total uncertainty in calculated DRF and identification of properties that most limit accuracy in estimating forcing. Total uncertainties in modeled local diurnally averaged forcing range from 0.2 to 1.3 W m-2 (42 to 20%) depending on location (from tropical to polar sites), solar zenith angle, surface reflectance, aerosol type, and aerosol optical depth. The largest contributor to total uncertainty in DRF is usually single scattering albedo; however decreasing measurement uncertainties for any property would increase accuracy in DRF. Comparison of two radiative transfer models suggests the contribution of modeling error is small compared to the total uncertainty although comparable to uncertainty arising from some individual properties.

  7. Parameterizations of Cloud Microphysics and Indirect Aerosol Effects

    SciTech Connect (OSTI)

    Tao, Wei-Kuo

    2014-05-19

    1. OVERVIEW Aerosols and especially their effect on clouds are one of the key components of the climate system and the hydrological cycle [Ramanathan et al., 2001]. Yet, the aerosol effect on clouds remains largely unknown and the processes involved not well understood. A recent report published by the National Academy of Science states "The greatest uncertainty about the aerosol climate forcing - indeed, the largest of all the uncertainties about global climate forcing - is probably the indirect effect of aerosols on clouds [NRC, 2001]." The aerosol effect on clouds is often categorized into the traditional "first indirect (i.e., Twomey)" effect on the cloud droplet sizes for a constant liquid water path [Twomey, 1977] and the "semi-direct" effect on cloud coverage [e.g., Ackerman et al., 2000]. Enhanced aerosol concentrations can also suppress warm rain processes by producing a narrow droplet spectrum that inhibits collision and coalescence processes [e.g., Squires and Twomey, 1961; Warner and Twomey, 1967; Warner, 1968; Rosenfeld, 1999]. The aerosol effect on precipitation processes, also known as the second type of aerosol indirect effect [Albrecht, 1989], is even more complex, especially for mixed-phase convective clouds. Table 1 summarizes the key observational studies identifying the microphysical properties, cloud characteristics, thermodynamics and dynamics associated with cloud systems from high-aerosol continental environments. For example, atmospheric aerosol concentrations can influence cloud droplet size distributions, warm-rain process, cold-rain process, cloud-top height, the depth of the mixed phase region, and occurrence of lightning. In addition, high aerosol concentrations in urban environments could affect precipitation variability by providing an enhanced source of cloud condensation nuclei (CCN). Hypotheses have been developed to explain the effect of urban regions on convection and precipitation [van den Heever and Cotton, 2007 and Shepherd, 2005]. Recently, a detailed spectral-bin microphysical scheme was implemented into the Goddard Cumulus Ensemble (GCE) model. Atmospheric aerosols are also described using number density size-distribution functions. A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep tropical clouds in the west Pacific warm pool region and summertime convection over a mid-latitude continent with different concentrations of CCN: a low "clean" concentration and a high "dirty" concentration. The impact of atmospheric aerosol concentration on cloud and precipitation will be investigated. 2. MODEL DESCRIPTION AND CASE STUDIES 2.1 GCE MODEL The model used in this study is the 2D version of the GCE model. Modeled flow is anelastic. Second- or higher-order advection schemes can produce negative values in the solution. Thus, a Multi-dimensional Positive Definite Advection Transport Algorithm (MPDATA) has been implemented into the model. All scalar variables (potential temperature, water vapor, turbulent coefficient and all five hydrometeor classes) use forward time differencing and the MPDATA for advection. Dynamic variables, u, v and w, use a second-order accurate advection scheme and a leapfrog time integration (kinetic energy semi-conserving method). Short-wave (solar) and long-wave radiation as well as a subgrid-scale TKE turbulence scheme are also included in the model. Details of the model can be found in Tao and Simpson (1993) and Tao et al. (2003). 2.2 Microphysics (Bin Model) The formulation of the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (cloud droplets and raindrops), and six types of ice particles: pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail. Each type is described by a special size distribution function containing 33 categories (bins). Atmospheric aerosols are also described using number density size-distribution functions (containing 33 bins). Droplet nucleation (activation) is derived from the analytical calculation of super-saturation, which is used to determine the sizes of aerosol particles to be activated and the corresponding sizes of nucleated droplets. Primary nucleation of each type of ice crystal takes place within certain temperature ranges. A detailed description of these explicitly parameterized processes can be found in Khain and Sednev (1996) and Khain et al. (1999, 2001). 2.3 Case Studies Three cases, a tropical oceanic squall system observed during TOGA COARE (Tropical Ocean and Global Atmosphere Coupled Ocean-Atmosphere Response Experiment, which occurred over the Pacific Ocean warm pool from November 1992 to February 1993), a midlatitude continental squall system observed during PRESTORM (Preliminary Regional Experiment for STORM-Central, which occurred in Kansas and Oklahoma during May-June 1985), and mid-afternoon convection observed during CRYSTAL-FACE (Cirrus Regional Study of Tropical Anvils and Cirrus Layers – Florida Area Cumulus Experiment, which occurred in Florida during July 2002), will be used to examine the impact of aerosols on deep, precipitating systems. 3. SUMMARY of RESULTS • For all three cases, higher CCN produces smaller cloud droplets and a narrower spectrum. Dirty conditions delay rain formation, increase latent heat release above the freezing level, and enhance vertical velocities at higher altitude for all cases. Stronger updrafts, deeper mixed-phase regions, and more ice particles are simulated with higher CCN in good agreement with observations. • In all cases, rain reaches the ground early with lower CCN. Rain suppression is also evident in all three cases with high CCN in good agreement with observations (Rosenfeld, 1999, 2000 and others). Rain suppression, however, only occurs during the first hour of simulation. This result suggests that microphysical processes dominate the impact of aerosols on precipitation in the early stage of precipitation development. • During the mature stage of the simulations, the effect of increasing aerosol concentration ranges from rain suppression in the PRESTORM case to little effect on surface rainfall in the CRYSTAL-FACE case to rain enhancement in the TOGA COARE case. • The model results suggest that evaporative cooling is a key process in determining whether higher CCN reduces or enhances precipitation. Cold pool strength can be enhanced by stronger evaporation. When cold pool interacts with the near surface wind shear, the low-level convergence can be stronger, facilitating secondary cloud formation and more vigorous precipitation processes. Evaporative cooling is more than two times stronger at low levels with higher CCN for the TOGA COARE case during the early stages of precipitation development. However, evaporative cooling is slightly stronger at lower levels with lower CCN for the PRESTORM case. The early formation of rain in the clean environment could allow for the formation of an earlier and stronger cold pool compared to a dirty environment. PRESTORM has a very dry environment and both large and small rain droplets can evaporate. Consequently, the cold pool is relatively weaker, and the system is relatively less intense with higher CCN. • Sensitivity tests are conducted to determine the impact of ice processes on aerosol-precipitation interaction. The results suggested that ice processes are crucial for suppressing precipitation due to high CCN for the PRESTORM case. More and smaller ice particles are generated in the dirty case and transported to the trailing stratiform region. This reduces the heavy convective rain and contributes to the weakening of the cold pool. Warm rain processes dominate the TOGA COARE case. Therefore, ice processes only play a secondary role in terms of aerosol-precipitation interaction. • Two of the three cloud systems presented in this paper formed a line structure (squall system). A 2D simulation, therefore, gives a good approximation to such a line of convective clouds. Since the real atmosphere is 3D, further 3D cloud-resolving simulations are needed to address aerosol-precipitation interactions. 4. REFERENCES Tao, W.-K., X. Li, A. Khain, T. Matsui, S. Lang, and J. Simpson, 2007: The role of atmospheric aerosol concentration on deep convective precipitation: Cloud-resolving model simulations. J. Geophy. Res., 112, D24S18, doi:10.1029/2007JD008728. All other references can be found in above paper. 5. Acknowledgements The GCE model is mainly supported by the NASA Headquarters Atmospheric Dynamics and Thermodynamics Program and the NASA Tropical Rainfall Measuring Mission (TRMM). The research was also supported by the Office of Science (BER), U. S. Department of Energy/Atmospheric Radiation Measurement (DOE/ARM) Interagency. The authors acknowledge NASA Goddard Space Flight Center for computer time used in this research.

  8. Science Overview Document Indirect and Semi-Direct Aerosol Campaign (ISDAC)

    Office of Scientific and Technical Information (OSTI)

    April 2008 (Technical Report) | SciTech Connect Science Overview Document Indirect and Semi-Direct Aerosol Campaign (ISDAC) April 2008 Citation Details In-Document Search Title: Science Overview Document Indirect and Semi-Direct Aerosol Campaign (ISDAC) April 2008 The ARM Climate Research Facility's (ACRF) Aerial Vehicle Program (AVP) will deploy an intensive cloud and aerosol observing system to the ARM North Slope of Alaska (NSA) locale for a five week Indirect and Semi-Direct Aerosol

  9. ARM: 10-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    1998-03-01

    10-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  10. ARM: 1-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    2004-10-01

    1-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  11. ARM: 10-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    10-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  12. ARM: 1-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Chitra Sivaraman; Connor Flynn

    1-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  13. Climate implications of carbonaceous aerosols: An aerosol microphysical study using the GISS/MATRIX climate model

    SciTech Connect (OSTI)

    Bauer, Susanne E.; Menon, Surabi; Koch, Dorothy; Bond, Tami; Tsigaridis, Kostas

    2010-04-09

    Recently, attention has been drawn towards black carbon aerosols as a likely short-term climate warming mitigation candidate. However the global and regional impacts of the direct, cloud-indirect and semi-direct forcing effects are highly uncertain, due to the complex nature of aerosol evolution and its climate interactions. Black carbon is directly released as particle into the atmosphere, but then interacts with other gases and particles through condensation and coagulation processes leading to further aerosol growth, aging and internal mixing. A detailed aerosol microphysical scheme, MATRIX, embedded within the global GISS modelE includes the above processes that determine the lifecycle and climate impact of aerosols. This study presents a quantitative assessment of the impact of microphysical processes involving black carbon, such as emission size distributions and optical properties on aerosol cloud activation and radiative forcing. Our best estimate for net direct and indirect aerosol radiative forcing change is -0.56 W/m{sup 2} between 1750 and 2000. However, the direct and indirect aerosol effects are very sensitive to the black and organic carbon size distribution and consequential mixing state. The net radiative forcing change can vary between -0.32 to -0.75 W/m{sup 2} depending on these carbonaceous particle properties. Assuming that sulfates, nitrates and secondary organics form a coating shell around a black carbon core, rather than forming a uniformly mixed particles, changes the overall net radiative forcing from a negative to a positive number. Black carbon mitigation scenarios showed generally a benefit when mainly black carbon sources such as diesel emissions are reduced, reducing organic and black carbon sources such as bio-fuels, does not lead to reduced warming.

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Dust in the Wind... and the Clouds... and the Atmosphere Submitter: Sassen, K., University of Alaska, Fairbanks Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Sassen, K., P.J. DeMott, J.M. Propsero, and M.R. Poellot, Saharan Dust Storms and Indirect Aerosol Effects on Clouds: CRYSTAL-FACE Results, Geophys. Res. Ltt., 30(12), 1633, doi:10/1029/2003GL017371, 2003. PDL linear depolarization ratio (color scale on top) and relative returned power (in gray scale) of

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Clouds Re-gathered by Wind Shear Download a printable PDF Submitter: Yang, Q., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Yang Q, RC Easter, P Campuzano-Jost, JL Jimenez, JD Fast, SJ Ghan, H Wang, LK Berg, MC Barth, Y Liu, MB Shrivastava, B Singh, H Morrison, J Fan, CL Ziegler, M Bela, E Apel, GS Diskin, T Mikoviny, and A Wisthaler. 2015. "Aerosol transport and

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Effects on Liquid-Water Path of Thin Stratocumulus Clouds Download a printable PDF Submitter: Penner, J. E., University of Michigan Lee, S., University of Michigan Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: n/a Thin clouds with mean liquid-water path (LWP) of ~ 50 g m-2 cover 27.5% of the globe and thus play an important role in the Earth's radiation budget. Radiative fluxes at the Earth's surface and top of atmosphere (TOA) are very sensitive to

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    More Like Shades of Gray: the Effects of Black Carbon in Aerosols Submitter: McComiskey, A. C., National Oceanic and Atmospheric Administration Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Cappa CD, TB Onasch, P Massoli, DR Worsnop, TS Bates, ES Cross, P Davidovits, J Hakala, KL Hayden, BT Jobson, KR Kolesar, DA Lack, BM Lerner, SM Li, D Mellon, I Nuaaman, JS Olfert, T Petaja, PK Quinn, C Song, R Subramanian, EJ Williams, and RA Zaveri. 2012.

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Mingling in the Sky-A View from the Earth Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Madhavan BL, Y He, Y Wu, B Gross, F Moshary, and S Ahmed. 2012. "Development of a ground based remote sensing approach for direct evaluation of aerosol-cloud interaction." Atmosphere, 3(4), doi:10.3390/atmos3040468. Two different types of

  19. ARM - Measurement - Aerosol absorption

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption ARM Data Discovery Browse Data Comments? We would love to hear from you Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol absorption The...

  20. Monodisperse aerosol generator

    DOE Patents [OSTI]

    Ortiz, Lawrence W.; Soderholm, Sidney C.

    1990-01-01

    An aerosol generator is described which is capable of producing a monodisperse aerosol within narrow limits utilizing an aqueous solution capable of providing a high population of seed nuclei and an organic solution having a low vapor pressure. The two solutions are cold nebulized, mixed, vaporized, and cooled. During cooling, particles of the organic vapor condense onto the excess seed nuclei, and grow to a uniform particle size.

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Microphysical Piggybacking: Understanding the Coupling Between Cloud Dynamics and Microphysics PI Contact: Grabowski, W., NCAR Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Grabowski WW. 2014. "Extracting microphysical impacts in large-eddy simulations of shallow convection." Journal of the Atmospheric Sciences, 71(12), 10.1175/JAS-D-14-0231.1. Grabowski WW. 2015. "Untangling microphysical

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Wildfires Lead to More Warming Than Climate Models Predict, a New Mexico Fire Study Reports Download a printable PDF Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: China S, C Mazzoleni, K Gorkowski, AC Aiken, and MK Dubey. 2013. "Morphology and mixing state of individual freshly emitted wildfire carbonaceous particles." Nature Communications, 4, 2122, doi:10.1038/ncomms3122.

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Modified Climate Model Better Replicates Global Rainfall Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Song X, GJ Zhang, and JF Li. 2012. "Evaluation of microphysics parameterization for convective clouds in the NCAR Community Atmosphere Model CAM5." Journal of Climate, 25(24), doi:10.1175/JCLI-D-11-00563.1. Rainfall in the

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Reality Check: Estimates for Human-Caused Methane Emissions in the U.S. Appear Off by 50% Download a printable PDF Submitter: Biraud, S. C., Lawrence Berkeley National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Miller SM, SC Wofsy, AM Michalak, EA Kort, AE Andrews, SC Biraud, EJ Dlugokencky, J Elszkeiwicz, ML Fischer, G Janssens-Maenhout, BR Miller, JB Miller, SA Montzka, T Nehrkorn, and C Sweeney. 2013. "Anthropogenic emissions

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Can Ice-Nucleating Aerosols Affect Arctic Seasonal Climate? Submitter: Prenni, A. J., Colorado State University Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Prenni, A. J., J. Y. Harrington, M. Tjernstrom, P. J. DeMott, A. Avramov, C. N. Long, S. M. Kreidenweis, P. Q. Olsson, and J. Verlinde, (2006): Can Ice-Nucleating Aerosols Affect Arctic Seasonal Climate?, BAMS, Vol.88, Iss. 4; pg. 541-550. ACIA, 2004: Impacts of a Warming

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Black Carbon Aerosols and the Third Polar Ice Cap Submitter: Menon, S., Lawrence Berkeley National Laboratory Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Cloud Modeling Journal Reference: Menon S, D Koch, G Beig, S Sahu, J Fasullo, and D Orlikowski. 2009. "Black carbon aerosols and the third polar ice cap." Atmospheric Chemistry and Physics, 9, 26593-26625. Recent thinning of glaciers over the Himalayas (sometimes referred to as

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    New Insight on the Atmosphere's Tiniest Particles Download a printable PDF Submitter: Smith, J., University of California, Irvine McMurry, P. ., University of Minnesota Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Smith JN, KC Barsanti, HR Friedli, M Ehn, M Kulmala, DR Collins, JH Scheckman, BJ Williams, and PH McMurry. 2010. "Observations of aminium salts in atmospheric nanoparticles and possible climatic implications." Proceedings of

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Influence of Humidified Aerosols on Lidar Depolarization Below Ice-Precipitating Arctic Clouds Download a printable PDF Submitter: Fridlind, A. M., NASA - Goddard Institute for Space Studies van Diedenhoven, B., NASA - Goddard Institute for Space Studies Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle Journal Reference: van Diedenhoven B, AM Fridlind, and AS Ackerman. 2011. "Influence of humidified aerosol on lidar depolarization measurements below

  9. One ARM, Two Columns and a Whole Lot of Aerosols | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    ARM, Two Columns and a Whole Lot of Aerosols One ARM, Two Columns and a Whole Lot of Aerosols July 25, 2012 - 5:49pm Addthis This observatory is part of an air particles research initiative at Cape Cod National Seashore in Massachusetts, and includes dozens of sophisticated instruments that take continuous ground-based measurements of clouds, aerosols, and other atmospheric properties. | Photo courtesy of the ARM Climate Research Facility. This observatory is part of an air particles research

  10. Cloud Droplet Spectral Shape Sheds New Light on Aerosol- Cloud-Interaction Regimes

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Droplet Spectral Shape Sheds New Light on Aerosol- Cloud-Interaction Regimes For original submission and image(s), see ARM Research Highlights http://www.arm.gov/science/highlights/ Research Highlight Despite decades of research, aerosol indirect effects remain among the most uncertain climate forcings according to the latest Intergovernmental Panel on Climate Change report. Furthermore, climate models tend to overestimate the cooling of aerosol indirect effects and are more susceptible than

  11. Enhancing Cloud Radiative Processes and Radiation Efficiency in the Advanced Research Weather Research and Forecasting (WRF) Model

    SciTech Connect (OSTI)

    Iacono, Michael J.

    2015-03-09

    The objective of this research has been to evaluate and implement enhancements to the computational performance of the RRTMG radiative transfer option in the Advanced Research version of the Weather Research and Forecasting (WRF) model. Efficiency is as essential as accuracy for effective numerical weather prediction, and radiative transfer is a relatively time-consuming component of dynamical models, taking up to 30-50 percent of the total model simulation time. To address this concern, this research has implemented and tested a version of RRTMG that utilizes graphics processing unit (GPU) technology (hereinafter RRTMGPU) to greatly improve its computational performance; thereby permitting either more frequent simulation of radiative effects or other model enhancements. During the early stages of this project the development of RRTMGPU was completed at AER under separate NASA funding to accelerate the code for use in the Goddard Space Flight Center (GSFC) Goddard Earth Observing System GEOS-5 global model. It should be noted that this final report describes results related to the funded portion of the originally proposed work concerning the acceleration of RRTMG with GPUs in WRF. As a k-distribution model, RRTMG is especially well suited to this modification due to its relatively large internal pseudo-spectral (g-point) dimension that, when combined with the horizontal grid vector in the dynamical model, can take great advantage of the GPU capability. Thorough testing under several model configurations has been performed to ensure that RRTMGPU improves WRF model run time while having no significant impact on calculated radiative fluxes and heating rates or on dynamical model fields relative to the RRTMG radiation. The RRTMGPU codes have been provided to NCAR for possible application to the next public release of the WRF forecast model.

  12. Selection Process and Notification for Small Business Innovation Research and Small Business Technology Transfer Awards

    Broader source: Energy.gov [DOE]

    Once you apply for a U.S. Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE) Small Business Innovation Research Program (SBIR) grant, the selection process begins, which includes an initial review, technical merit review, discussions, and notifications.

  13. Industrial Technologies Program Research Plan for Energy-Intensive Process Industries

    SciTech Connect (OSTI)

    Chapas, Richard B.; Colwell, Jeffery A.

    2007-10-01

    In this plan, the Industrial Technologies Program (ITP) identifies the objectives of its cross-cutting strategy for conducting research in collaboration with industry and U.S. Department of Energy national laboratories to develop technologies that improve the efficiencies of energy-intensive process industries.

  14. EM Celebrates Milestone with Removal of Last Waste Tank at Separations Process Research Unit

    Broader source: Energy.gov [DOE]

    NISKAYUNA, N.Y. – EM recently marked a notable milestone at the Separations Process Research Unit (SPRU) when workers removed the last of seven large waste storage tanks from a vault and shipped it to an offsite low-level radioactive waste disposal facility.

  15. Research prioritization using the Analytic Hierarchy Process: basic methods. Volume 1

    SciTech Connect (OSTI)

    Vesely, W.E.; Shafaghi, A.; Gary, I. Jr.; Rasmuson, D.M.

    1983-08-01

    This report describes a systematic approach for prioritizing research needs and research programs. The approach is formally called the Analytic Hierarchy Process which was developed by T.L. Saaty and is described in several of his texts referenced in the report. The Analytic Hierarchy Process, or AHP for short, has been applied to a wide variety of prioritization problems and has a good record of success as documented in Saaty's texts. The report develops specific guidelines for constructing the hierarchy and for prioritizing the research programs. Specific examples are given to illustrate the steps in the AHP. As part of the work, a computer code has been developed and the use of the code is described. The code allows the prioritizations to be done in a codified and efficient manner; sensitivity and parametric studies can also be straightforwardly performed to gain a better understanding of the prioritization results. Finally, as an important part of the work, an approach is developed which utilizes probabilistic risk analyses (PRAs) to systematically identify and prioritize research needs and research programs. When utilized in an AHP framework, the PRA's which have been performed to date provide a powerful information source for focusing research on those areas most impacting risk and risk uncertainty.

  16. ARM - Field Campaign - In-situ Aerosol Profiles (Cessna Aerosol...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    would love to hear from you Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : In-situ Aerosol Profiles (Cessna Aerosol Flights) 2000.03.01 - 2007.10.31 Lead...

  17. ARM - Measurement - Aerosol effective radius

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    would love to hear from you Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol effective radius Aerosol effective radius is the ratio of the third and...

  18. Research investigations in oil shale, tar sand, coal research, advanced exploratory process technology, and advanced fuels research: Volume 2 -- Jointly sponsored research program. Final report, October 1986--September 1993

    SciTech Connect (OSTI)

    Smith, V.E.

    1994-09-01

    Numerous studies have been conducted in five principal areas: oil shale, tar sand, underground coal gasification, advanced process technology, and advanced fuels research. In subsequent years, underground coal gasification was broadened to be coal research, under which several research activities were conducted that related to coal processing. The most significant change occurred in 1989 when the agreement was redefined as a Base Program and a Jointly Sponsored Research Program (JSRP). Investigations were conducted under the Base Program to determine the physical and chemical properties of materials suitable for conversion to liquid and gaseous fuels, to test and evaluate processes and innovative concepts for such conversions, to monitor and determine environmental impacts related to development of commercial-sized operations, and to evaluate methods for mitigation of potential environmental impacts. This report is divided into two volumes: Volume 1 consists of 28 summaries that describe the principal research efforts conducted under the Base Program in five topic areas. Volume 2 describes tasks performed within the JSRP. Research conducted under this agreement has resulted in technology transfer of a variety of energy-related research information. A listing of related publications and presentations is given at the end of each research topic summary. More specific and detailed information is provided in the topical reports referenced in the related publications listings.

  19. Review of internal combustion engine combustion chamber process studies at NASA Lewis Research Center

    SciTech Connect (OSTI)

    Schock, H.J.

    1984-01-01

    The performance of internal combustion stratified-charge engines is highly dependent on the in-cylinder fuel-air mixing processes occurring in these engines. Current research concerning the in-cylinder airflow characteristics of rotary and piston engines is presented. Results showing the output of multidimensional models, laser velocimetry measurements and the application of a holographic optical element are described. Models which simulate the four-stroke cycle and seal dynamics of rotary engines are also discussed.

  20. Highly stable aerosol generator

    DOE Patents [OSTI]

    DeFord, H.S.; Clark, M.L.

    1981-11-03

    An improved compressed air nebulizer has been developed such that a uniform aerosol particle size and concentration may be produced over long time periods. This result is achieved by applying a vacuum pressure to the makeup assembly and by use of a vent tube between the atmosphere and the makeup solution. By applying appropriate vacuum pressures to the makeup solution container and by proper positioning of the vent tube, a constant level of aspirating solution may be maintained within the aspirating assembly with aspirating solution continuously replaced from the makeup solution supply. This device may also be adapted to have a plurality of aerosol generators and only one central makeup assembly. 2 figs.

  1. Highly stable aerosol generator

    DOE Patents [OSTI]

    DeFord, Henry S.; Clark, Mark L.

    1981-01-01

    An improved compressed air nebulizer has been developed such that a uniform aerosol particle size and concentration may be produced over long time periods. This result is achieved by applying a vacuum pressure to the makeup assembly and by use of a vent tube between the atmosphere and the makeup solution. By applying appropriate vacuum pressures to the makeup solution container and by proper positioning of the vent tube, a constant level of aspirating solution may be maintained within the aspirating assembly with aspirating solution continuously replaced from the makeup solution supply. This device may also be adapted to have a plurality of aerosol generators and only one central makeup assembly.

  2. Oil shale, tar sand, coal research advanced exploratory process technology, jointly sponsored research. Quarterly technical progress report, October--December 1992

    SciTech Connect (OSTI)

    Speight, J.G.

    1992-12-31

    Accomplishments for the past quarter are presented for the following five tasks: oil shale; tar sand; coal; advanced exploratory process technology; and jointly sponsored research. Oil shale research covers oil shale process studies. Tar sand research is on process development of Recycle Oil Pyrolysis and Extraction (ROPE) Process. Coal research covers: coal combustion; integrated coal processing concepts; and solid waste management. Advanced exploratory process technology includes: advanced process concepts;advanced mitigation concepts; and oil and gas technology. Jointly sponsored research includes: organic and inorganic hazardous waste stabilization; CROW field demonstration with Bell Lumber and Pole; development and validation of a standard test method for sequential batch extraction fluid; PGI demonstration project; operation and evaluation of the CO{sub 2} HUFF-N-PUFF Process; fly ash binder for unsurfaced road aggregates; solid state NMR analysis of Mesaverde Group, Greater Green River Basin, tight gas sands; flow-loop testing of double-wall pipe for thermal applications; characterization of petroleum residue; shallow oil production using horizontal wells with enhanced oil recovery techniques; surface process study for oil recovery using a thermal extraction process; NMR analysis of samples from the ocean drilling program; in situ treatment of manufactured gas plant contaminated soils demonstration program; and solid state NMR analysis of naturally and artificially matured kerogens.

  3. Tanks Focus Area Alternative Salt Processing Research and Development Program Plan

    SciTech Connect (OSTI)

    Harmon, Harry D.

    2000-11-30

    In March 2000, DOE-Headquarters (HQ) requested the Tanks Focus Area (TFA) to assume management responsibility for the Salt Processing Project technology development program at Savannah River Site. The TFA was requested to conduct several activities, including review and revision of the technology development roadmaps, development of down-selection criteria, and preparation of a comprehensive Research and Development (R&D) Program Plan for three candidate cesium removal technologies, as well as the Alpha and strontium removal processes that must also be carried out. The three cesium removal candidate technologies are Crystalline Silicotitanate (CST) Non-Elutable Ion Exchange, Caustic Side Solvent Extraction (CSSX), and Small Tank Tetraphenylborate Precipitation (STTP). This plan describes the technology development needs for each process that must be satisfied in order to reach a down-selection decision, as well as continuing technology development required to support conceptual design activities.

  4. Tanks Focus Area Alternative Salt Processing Research and Development Program Plan

    SciTech Connect (OSTI)

    Harmon, Harry D.

    2000-05-15

    In March 2000, DOE-Headquarters (HQ) requested the Tanks Focus Area (TFA)to assume management responsibility for the Salt Processing Project technology development program at Savannah River Site. The TFA was requested to conduct several activities, including review and revision of the technology development roadmaps, development of down-selection criteria, and preparation of a comprehensive Research and Development (R&D) Program Plan for three candidate cesium removal technologies, as well as the Alpha and strontium removal processes that must also be carried out. The three cesium removal candidate technologies are Crystalline Silicotitanate (CST) Non-Elutable Ion Exchange, Caustic Side Solvent Extraction (CSSX), and Small Tank Tetraphenylborate Precipitation (STTP). This plan describes the technology development needs for each process that must be satisfied in order to reach a down-selection decision, as well as continuing technology development required to support conceptual design activities.

  5. Field Trial of an Aerosol-Based Enclosure Sealing Technology

    SciTech Connect (OSTI)

    Harrington, Curtis; Springer, David

    2015-09-01

    This report presents the results from several demonstrations of a new method for sealing building envelope air leaks using an aerosol sealing process developed by the Western Cooling Efficiency Center at UC Davis. The process involves pressurizing a building while applying an aerosol sealant to the interior. As air escapes through leaks in the building envelope, the aerosol particles are transported to the leaks where they collect and form a seal that blocks the leak. Standard blower door technology is used to facilitate the building pressurization, which allows the installer to track the sealing progress during the installation and automatically verify the final building tightness. Each aerosol envelope sealing installation was performed after drywall was installed and taped, and the process did not appear to interrupt the construction schedule or interfere with other trades working in the homes. The labor needed to physically seal bulk air leaks in typical construction will not be replaced by this technology.

  6. Incorporating an advanced aerosol activation parameterization into WRF-CAM5: Model evaluation and parameterization intercomparison

    SciTech Connect (OSTI)

    Zhang, Yang; Zhang, Xin; Wang, Kai; He, Jian; Leung, Lai-Yung R.; Fan, Jiwen; Nenes, Athanasios

    2015-07-22

    Aerosol activation into cloud droplets is an important process that governs aerosol indirect effects. The advanced treatment of aerosol activation by Fountoukis and Nenes (2005) and its recent updates, collectively called the FN series, have been incorporated into a newly developed regional coupled climate-air quality model based on the Weather Research and Forecasting model with the physics package of the Community Atmosphere Model version 5 (WRF-CAM5) to simulate aerosol-cloud interactions in both resolved and convective clouds. The model is applied to East Asia for two full years of 2005 and 2010. A comprehensive model evaluation is performed for model predictions of meteorological, radiative, and cloud variables, chemical concentrations, and column mass abundances against satellite data and surface observations from air quality monitoring sites across East Asia. The model performs overall well for major meteorological variables including near-surface temperature, specific humidity, wind speed, precipitation, cloud fraction, precipitable water, downward shortwave and longwave radiation, and column mass abundances of CO, SO2, NO2, HCHO, and O3 in terms of both magnitudes and spatial distributions. Larger biases exist in the predictions of surface concentrations of CO and NOx at all sites and SO2, O3, PM2.5, and PM10 concentrations at some sites, aerosol optical depth, cloud condensation nuclei over ocean, cloud droplet number concentration (CDNC), cloud liquid and ice water path, and cloud optical thickness. Compared with the default Abdul-Razzack Ghan (2000) parameterization, simulations with the FN series produce ~107113% higher CDNC, with half of the difference attributable to the higher aerosol activation fraction by the FN series and the remaining half due to feedbacks in subsequent cloud microphysical processes. With the higher CDNC, the FN series are more skillful in simulating cloud water path, cloud optical thickness, downward shortwave radiation, shortwave cloud forcing, and precipitation. The model evaluation identifies several areas of provements including emissions and their vertical allocation as well as model formulations such as aerosol formation, cloud droplet nucleation, and ice nucleation.

  7. Development of an aerosol microphysical module: Aerosol Two-dimensional bin module for foRmation and Aging Simulation (ATRAS)

    SciTech Connect (OSTI)

    Matsui, H.; Koike, Makoto; Kondo, Yutaka; Fast, Jerome D.; Takigawa, M.

    2014-09-30

    Number concentrations, size distributions, and mixing states of aerosols are essential parameters for accurate estimation of aerosol direct and indirect effects. In this study, we developed an aerosol module, designated Aerosol Two-dimensional bin module for foRmation and Aging Simulation (ATRAS), that can represent these parameters explicitly by considering new particle formation (NPF), black carbon (BC) aging, and secondary organic aerosol (SOA) processes. A two-dimensional bin representation is used for particles with dry diameters from 40 nm to 10 m to resolve both aerosol size (12 bins) and BC mixing state (10 bins) for a total of 120 bins. The particles with diameters from 1 to 40 nm are resolved using an additional 8 size bins to calculate NPF. The ATRAS module was implemented in the WRF-chem model and applied to examine the sensitivity of simulated mass, number, size distributions, and optical and radiative parameters of aerosols to NPF, BC aging and SOA processes over East Asia during the spring of 2009. BC absorption enhancement by coating materials was about 50% over East Asia during the spring, and the contribution of SOA processes to the absorption enhancement was estimated to be 10 20% over northern East Asia and 20 35% over southern East Asia. A clear north-south contrast was also found between the impacts of NPF and SOA processes on cloud condensation nuclei (CCN) concentrations: NPF increased CCN concentrations at higher supersaturations (smaller particles) over northern East Asia, whereas SOA increased CCN concentrations at lower supersaturations (larger particles) over southern East Asia. Application of ATRAS to East Asia also showed that the impact of each process on each optical and radiative parameter depended strongly on the process and the parameter in question. The module can be used in the future as a benchmark model to evaluate the accuracy of simpler aerosol models and examine interactions between NPF, BC aging, and SOA processes under different meteorological conditions and emissions.

  8. Research on the pyrolysis of hardwood in an entrained bed process development unit

    SciTech Connect (OSTI)

    Kovac, R.J.; Gorton, C.W.; Knight, J.A.; Newman, C.J.; O'Neil, D.J. . Research Inst.)

    1991-08-01

    An atmospheric flash pyrolysis process, the Georgia Tech Entrained Flow Pyrolysis Process, for the production of liquid biofuels from oak hardwood is described. The development of the process began with bench-scale studies and a conceptual design in the 1978--1981 timeframe. Its development and successful demonstration through research on the pyrolysis of hardwood in an entrained bed process development unit (PDU), in the period of 1982--1989, is presented. Oil yields (dry basis) up to 60% were achieved in the 1.5 ton-per-day PDU, far exceeding the initial target/forecast of 40% oil yields. Experimental data, based on over forty runs under steady-state conditions, supported by material and energy balances of near-100% closures, have been used to establish a process model which indicates that oil yields well in excess of 60% (dry basis) can be achieved in a commercial reactor. Experimental results demonstrate a gross product thermal efficiency of 94% and a net product thermal efficiency of 72% or more; the highest values yet achieved with a large-scale biomass liquefaction process. A conceptual manufacturing process and an economic analysis for liquid biofuel production at 60% oil yield from a 200-TPD commercial plant is reported. The plant appears to be profitable at contemporary fuel costs of $21/barrel oil-equivalent. Total capital investment is estimated at under $2.5 million. A rate-of-return on investment of 39.4% and a pay-out period of 2.1 years has been estimated. The manufacturing cost of the combustible pyrolysis oil is $2.70 per gigajoule. 20 figs., 87 tabs.

  9. Biogenic Aerosols-Effects on Clouds and Climate: Snowfall Experiment

    Office of Scientific and Technical Information (OSTI)

    Field Campaign Report (Program Document) | SciTech Connect SciTech Connect Search Results Program Document: Biogenic Aerosols-Effects on Clouds and Climate: Snowfall Experiment Field Campaign Report Citation Details In-Document Search Title: Biogenic Aerosols-Effects on Clouds and Climate: Snowfall Experiment Field Campaign Report The snowfall measurement campaign took place during deployment of the U.S. Department of Energy (DOE)'s Atmospheric Radiation Measurement (ARM) Climate Research

  10. Sources and composition of submicron organic mass in marine aerosol particles: Marine Aerosol Organic Mass Composition

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Frossard, Amanda A.; Russell, Lynn M.; Burrows, Susannah M.; Elliott, Scott M.; Bates, Timothy S.; Quinn, Patricia K.

    2014-11-26

    Recent studies have proposed a variety of interpretations of the sources and composition of atmospheric marine aerosol particles (aMA) based on a range of physical and chemical measurements collected during open-ocean research cruises. To investigate the processes that affect marine organic particles, this study uses the characteristic functional group composition (from Fourier transform infrared (FTIR) spectroscopy) of aMAP from five ocean regions to show that: (i) The organic functional group composition of aMAP that can be identified as atmospheric primary marine (ocean-derived) aerosol (aPMA) is 6512% hydroxyl, 219% alkane, 66% amine, and 78% carboxylic acid functional groups. Contributions from photochemicalmorereactions add carboxylic acid groups (15%-25%), shipping effluent in seawater and ship emissions add additional alkane groups (up to 70%), and coastal emissions mix in alkane and carboxylic acid groups from coastal pollution sources. (ii) The organic composition of aPMA is nearly identical to model generated primary marine aerosol particles (gPMA) from bubbled seawater (55% hydroxyl, 32% alkane, and 13% amine functional groups), indicating that its overall functional group composition is the direct consequence of the organic constituents of the seawater source. (iii) While the seawater organic functional group composition was nearly invariant across all three ocean regions studied, the gPMA alkane group fraction increased with chlorophyll-a concentrations (r = 0.79). gPMA from productive seawater had a larger fraction of alkane functional groups (35%) compared to gPMA from non-productive seawater (16%), likely due to the presence of surfactants in productive seawater that stabilize the bubble film and lead to preferential drainage of the more soluble (lower alkane group fraction) organic components. gPMA has a hydroxyl group absorption peak location characteristic of monosaccharides and disaccharides, where the seawater OM hydroxyl group peak location is closer to that of polysaccharides. This may result from the larger saccharides preferentially remaining in the seawater during gPMA and aPMA productionless

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Predicting Arctic Sea Ice Loss Download a printable PDF Submitter: Liu, X., University of Wyoming Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Liu X, S Xie, J Boyle, SA Klein, X Shi, Z Wang, W Lin, SJ Ghan, M Earle, PS Liu, and A Zelenyuk. 2011. "Testing cloud microphysics parameterizations in NCAR CAM5 with ISDAC and M-PACE observations." Journal of Geophysical Research, 116, D00T11,

  12. Organic Aerosol Component (OACOMP) Value-Added Product Report

    SciTech Connect (OSTI)

    Fast, J; Zhang, Q; Tilp, A; Shippert, T; Parworth, C; Mei, F

    2013-08-23

    Significantly improved returns in their aerosol chemistry data can be achieved via the development of a value-added product (VAP) of deriving OA components, called Organic Aerosol Components (OACOMP). OACOMP is primarily based on multivariate analysis of the measured organic mass spectral matrix. The key outputs of OACOMP are the concentration time series and the mass spectra of OA factors that are associated with distinct sources, formation and evolution processes, and physicochemical properties.

  13. ARM Cloud Aerosol Precipitation Experiment (ACAPEX) Science Plan (Program

    Office of Scientific and Technical Information (OSTI)

    Document) | SciTech Connect ARM Cloud Aerosol Precipitation Experiment (ACAPEX) Science Plan Citation Details In-Document Search Title: ARM Cloud Aerosol Precipitation Experiment (ACAPEX) Science Plan The western U.S. receives precipitation predominantly during the cold season when storms approach from the Pacific Ocean. The snowpack that accumulates during winter storms provides about 70-90% of water supply for the region. Understanding and modeling the fundamental processes that govern the

  14. A new scenario framework for climate change research: background, process, and future directions

    SciTech Connect (OSTI)

    Ebi, Kristie L.; Hallegatte, Stephane; Kram, Tom; Arnell, Nigel; Carter, Tim; Edmonds, James A.; Kriegler, Elmar; Mathur, Ritu; O'Neill, Brian; Riahi, Keywan; Winkler, Harald; Van Vuuren, Detlef; Zwickel, Timm

    2014-02-01

    The scientific community is developing new integrated global, regional, and sectoral scenarios to facilitate interdisciplinary research and assessment to explore the range of possible future climates and related physical changes could pose to human and natural systems; how these could interact with social, economic, and environmental development pathways; the degree to which mitigation and adaptation policies can avoid and reduce those risks; the costs and benefits of various policy mixes; residual impacts under alternative pathways; and the relationship with sustainable development. This paper provides the background to, and process of, developing the conceptual framework for these scenarios, described in three other papers in this Special Issue (van Vuuren et al.; O'Neill et al.; Kriegler et al.). The paper also discusses research needs to further develop and apply this framework. The goal is to encourage climate change researchers from a broad range of perspectives and disciplines to work together to develop policy-relevant scenarios and explore the implications of different possible futures for the challenges and opportunities human and natural systems could face with increasing climate change.

  15. The Radiative Role of Free Tropospheric Aerosols and Marine Clouds over the Central North Atlantic

    SciTech Connect (OSTI)

    Mazzoleni, Claudio; Kumar, Sumit; Wright, Kendra; Kramer, Louisa; Mazzoleni, Lynn; Owen, Robert; Helmig, Detlev

    2014-12-09

    The scientific scope of the project was to exploit the unique location of the Pico Mountain Observatory (PMO) located in the summit caldera of the Pico Volcano in Pico Island in the Azores, for atmospheric studies. The observatory, located at 2225m a.s.l., typically samples free tropospheric aerosols laying above the marine low-level clouds and long-range transported from North America. The broad purpose of this research was to provide the scientific community with a better understanding of fundamental physical processes governing the effects of aerosols on radiative forcing and climate; with the ultimate goal of improving our abilities to understand past climate and to predict future changes through numerical models. The project was 'exploratory' in nature, with the plan to demonstrate the feasibility of deploying for the first time, an extensive aerosol research package at PMO. One of the primary activities was to test the deployment of these instruments at the site, to collect data during the 2012 summer season, and to further develop the infrastructure and the knowledge for performing novel research at PMO in follow-up longer-term aerosol-cloud studies. In the future, PMO could provide an elevated research outpost to support the renewed DOE effort in the Azores that was intensified in 2013 with the opening of the new sea-level ARM-DOE Eastern North Atlantic permanent facility at Graciosa Island. During the project period, extensive new data sets were collected for the planned 2012 season. Thanks to other synergistic activities and opportunities, data collection was then successfully extended to 2013 and 2014. Highlights of the scientific findings during this project include: a) biomass burning contribute significantly to the aerosol loading in the North Atlantic free troposphere; however, long-range transported black carbon concentrations decreased substantially in the last decade. b) Single black carbon particles – analyzed off-line at the electron microscope – were often very compacted, suggesting cloud processing and exhibiting different optical properties from fresh emissions. In addition, black carbon was found to be sometimes mixed with mineral dust, affecting its optical properties and potential forcing. c) Some aerosols collected at PMO acted as ice nuclei, potentially contributing to cirrus cloud formation during their transport in the upper free troposphere. Identified good ice nuclei were often mineral dust particles. d) The free tropospheric aerosols studied at PMO have relevance to low level marine clouds due, for example, to synoptic subsidence entraining free tropospheric aerosols into the marine boundary layer. This has potentially large consequences on cloud condensation nuclei concentrations and compositions in the marine boundary layer; therefore, having an effect on the marine stratus clouds, with potentially important repercussions on the radiative forcing. The scientific products of this project currently include contributions to two papers published in the Nature Publishing group (Nature Communications and Scientific Reports), one paper under revision for Atmospheric Chemistry and Physics, one in review in Geophysical Research Letters and one recently submitted to Atmospheric Chemistry and Physics Discussion. In addition, four manuscripts are in advanced state of preparation. Finally, twenty-eight presentations were given at international conferences, workshops and seminars.

  16. The Design-Build Process for the Research Support Facility (RSF), Energy Efficiency & Renewable Energy (EERE)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Design-Build Process for the Research Support Facility An in-depth look at how the U.S. Department of Energy and the National Renewable Energy Laboratory used a performance-based design-build contract process to build one of the most energy efficient office buildings in the world. Table of Contents The Design-Build Process for the Research Support Facility | 1 Table of Contents Executive Summary . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    atmospheric radiative forcing and cloud-aerosol interactions is due to lack of sufficient observational data describing vertical profiles of aerosol particles and aerosol optical...

  18. Aerosol Observing System (AOS) Handbook

    SciTech Connect (OSTI)

    Jefferson, A

    2011-01-17

    The Aerosol Observing System (AOS) is a suite of in situ surface measurements of aerosol optical and cloud-forming properties. The instruments measure aerosol properties that influence the earths radiative balance. The primary optical measurements are those of the aerosol scattering and absorption coefficients as a function of particle size and radiation wavelength and cloud condensation nuclei (CCN) measurements as a function of percent supersaturation. Additional measurements include those of the particle number concentration and scattering hygroscopic growth. Aerosol optical measurements are useful for calculating parameters used in radiative forcing calculations such as the aerosol single-scattering albedo, asymmetry parameter, mass scattering efficiency, and hygroscopic growth. CCN measurements are important in cloud microphysical models to predict droplet formation.

  19. Research

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Isotopes produced at Los Alamos National Laboratory are saving lives, advancing cutting-edge research and keeping the U.S. safe. Research thorium test foil A thorium test foil ...

  20. Cantera Aerosol Dynamics Simulator

    Energy Science and Technology Software Center (OSTI)

    2004-09-01

    The Cantera Aerosol Dynamics Simulator (CADS) package is a general library for aerosol modeling to address aerosol general dynamics, including formation from gas phase reactions, surface chemistry (growth and oxidation), bulk particle chemistry, transport by Brownian diffusion, thermophoresis, and diffusiophoresis with linkage to DSMC studies, and thermal radiative transport. The library is based upon Cantera, a C++ Cal Tech code that handles gas phase species transport, reaction, and thermodynamics. The method uses a discontinuous galerkinmore » formulation for the condensation and coagulation operator that conserves particles, elements, and enthalpy up to round-off error. Both O-D and 1-D time dependent applications have been developed with the library. Multiple species in the solid phase are handled as well. The O-D application, called Tdcads (Time Dependent CADS) is distributed with the library. Tdcads can address both constant volume and constant pressure adiabatic homogeneous problems. An extensive set of sample problems for Tdcads is also provided.« less

  1. Laboratory Experiments and Instrument Intercomparison Studies of Carbonaceous Aerosol Particles

    SciTech Connect (OSTI)

    Davidovits, Paul

    2015-10-20

    Aerosols containing black carbon (and some specific types of organic particulate matter) directly absorb incoming light, heating the atmosphere. In addition, all aerosol particles backscatter solar light, leading to a net-cooling effect. Indirect effects involve hydrophilic aerosols, which serve as cloud condensation nuclei (CCN) that affect cloud cover and cloud stability, impacting both atmospheric radiation balance and precipitation patterns. At night, all clouds produce local warming, but overall clouds exert a net-cooling effect on the Earth. The effect of aerosol radiative forcing on climate may be as large as that of the greenhouse gases, but predominantly opposite in sign and much more uncertain. The uncertainties in the representation of aerosol interactions in climate models makes it problematic to use model projections to guide energy policy. The objective of our program is to reduce the uncertainties in the aerosol radiative forcing in the two areas highlighted in the ASR Science and Program Plan. That is, (1) addressing the direct effect by correlating particle chemistry and morphology with particle optical properties (i.e. absorption, scattering, extinction), and (2) addressing the indirect effect by correlating particle hygroscopicity and CCN activity with particle size, chemistry, and morphology. In this connection we are systematically studying particle formation, oxidation, and the effects of particle coating. The work is specifically focused on carbonaceous particles where the uncertainties in the climate relevant properties are the highest. The ongoing work consists of laboratory experiments and related instrument inter-comparison studies both coordinated with field and modeling studies, with the aim of providing reliable data to represent aerosol processes in climate models. The work is performed in the aerosol laboratory at Boston College. At the center of our laboratory setup are two main sources for the production of aerosol particles: (a) two well-characterized source of soot particles and (b) a flow reactor for controlled OH and/or O3 oxidation of relevant gas phase species to produce well-characterized SOA particles. After formation, the aerosol particles are subjected to physical and chemical processes that simulate aerosol growth and aging. A suite of instruments in our laboratory is used to characterize the physical and chemical properties of aerosol particles before and after processing. The Time of Flight Aerosol Mass Spectrometer (ToF-AMS) together with a Scanning Mobility Particle Sizer (SMPS) measures particle mass, volume, density, composition (including black carbon content), dynamic shape factor, and fractal dimension. The–ToF-AMS was developed at ARI with Boston College participation. About 120 AMS instruments are now in service (including 5 built for DOE laboratories) performing field and laboratory studies world-wide. Other major instruments include a thermal denuder, two Differential Mobility Analyzers (DMA), a Cloud Condensation Nuclei Counter (CCN), a Thermal desorption Aerosol GC/MS (TAG) and the new Soot Particle Aerosol Mass Spectrometer (SP-AMS). Optical instrumentation required for the studies have been brought to our laboratory as part of ongoing and planned collaborative projects with colleagues from DOE, NOAA and university laboratories. Optical instruments that will be utilized include a Photoacoustic Spectrometer (PAS), a Cavity Ring Down Aerosol Extinction Spectrometer (CRD-AES), a Photo Thermal Interferometer (PTI), a new 7-wavelength Aethalometer and a Cavity Attenuated Phase Shift Extinction Monitor (CAPS). These instruments are providing aerosol absorption, extinction and scattering coefficients at a range of atmospherically relevant wavelengths. During the past two years our work has continued along the lines of our original proposal. We report on 12 completed and/or continuing projects conducted during the period 08/14 to 0814/2015. These projects are described in 17 manuscripts published in refereed journals.

  2. Aerosol Oxidation Speeds Up in Smoggy Air

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Oxidation Speeds Up in Smoggy Air Aerosol Oxidation Speeds Up in Smoggy Air Print Wednesday, 17 February 2016 11:37 Organic aerosols (nanometer-sized liquid or solid ...

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    A Partial Mechanistic Understanding of the North American Monsoon Download a printable PDF Submitter: Erfani, E., Desert Research Institute Area of Research: Atmospheric Thermodynamics and Vertical Structures Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Erfani E and DL Mitchell. 2014. "A partial mechanistic understanding of the North American monsoon." Journal of Geophysical Research - Atmospheres, 119(23), 10.1002/2014JD022038. a) Dependence of

  4. ARM - Measurement - Aerosol optical depth

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Modeling Testbed AOD : Aerosol Optical Depth, derived from atmospheric extinction of solar irradiance AATS : Ames Airborne Tracking Sunphotometer CSPHOT : Cimel Sunphotometer...

  5. ARM: 10-minute TEMPORARY Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Sivaraman, Chitra; Flynn, Connor

    2010-12-15

    10-minute TEMPORARY Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  6. ARM: 10-minute TEMPORARY Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Sivaraman, Chitra; Flynn, Connor

    10-minute TEMPORARY Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

  7. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion...

  8. ARM - Campaign Instrument - aerosol-tower-eml

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    (AEROSOL-TOWER-EML) Instrument Categories Aerosols Campaigns Remote Cloud Sensing (RCS) Field Evaluation Download Data Southern Great Plains, 1994.04.01 - 1994.05.31...

  9. ARM - Evaluation Product - Organic Aerosol Component VAP

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    mass spectral matrix data collected by the aerosol chemical speciation monitor and multivariate analysis to obtain an estimate of the types of organic aerosols. Currently, time...

  10. ARM - Field Campaign - MASRAD - Aerosol Optical Properties

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsMASRAD - Aerosol Optical Properties Campaign Links AMF Point Reyes Website ARM Data Discovery Browse Data Related Campaigns MArine Stratus Radiation Aerosol and Drizzle...

  11. Aerosol Oxidation Speeds Up in Smoggy Air

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Oxidation Speeds Up in Smoggy Air Print Organic aerosols (nanometer-sized liquid or solid particles suspended in air) are important constituents of the troposphere, and ...

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Comparison of Mixed-layer Heights from Airborne HSRL and WRF-Chem During CARES Download a printable PDF Submitter: Scarino, A. J., Science Systems and Applications, Inc. Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Scarino AJ, MD Obland, JD Fast, SP Burton, RA Ferrare, CA Hostetler, LK Berg, B Lefer, C Haman, JW Hair, RR Rogers, C Butler, AL Cook, and DB Harper. 2014. "Comparison of mixed layer heights from airborne high spectral resolution

  13. Researchers Model Impact of Aerosols Over California

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ... Radiative forcing is the difference between the radiant energy received by earth and the energy radiated back to space. According to Zhao, California is an interesting case study ...

  14. Research

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Research Research Isotopes produced at Los Alamos National Laboratory are saving lives, advancing cutting-edge research and keeping the U.S. safe. Research thorium test foil A thorium test foil target for proof-of-concept actinium-225 production In addition to our routine isotope products, the LANL Isotope Program is focused on developing the next suite of isotopes and services to meet the Nation's emerging needs. The LANL Isotope Program's R&D strategy is focused on four main areas (see

  15. Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Feng, Y.; Kotamarthi, V. R.; Coulter, R.; Zhao, C.; Cadeddu, M.

    2015-06-19

    Aerosol radiative effects and thermodynamic responses over South Asia are examined with a version of the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of Aerosol Optical Depth (AOD) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in the northern India. The WRF-Chem model is found to underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model low-bias is due to aerosol extinctions below ~2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AODmoreand extinction profiles averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7 K day?1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond differently between Case I and Case II underlying the importance of determining the exact portion of scattering or absorbing aerosols that lead to the underestimation of aerosol optical depth in the model. In addition, the model results suggest that both direct radiative effect and rapid thermodynamic responses need to be quantified for understanding aerosol radiative impacts.less

  16. Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

    SciTech Connect (OSTI)

    Feng, Y.; Kotamarthi, V. R.; Coulter, R.; Zhao, C.; Cadeddu, M.

    2015-06-19

    Aerosol radiative effects and thermodynamic responses over South Asia are examined with a version of the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of Aerosol Optical Depth (AOD) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in the northern India. The WRF-Chem model is found to underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model low-bias is due to aerosol extinctions below ~2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AOD and extinction profiles averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7 K day−1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond differently between Case I and Case II underlying the importance of determining the exact portion of scattering or absorbing aerosols that lead to the underestimation of aerosol optical depth in the model. In addition, the model results suggest that both direct radiative effect and rapid thermodynamic responses need to be quantified for understanding aerosol radiative impacts.

  17. Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Feng, Y.; Kotamarthi, V. R.; Coulter, R.; Zhao, C.; Cadeddu, M.

    2016-01-18

    In this study, aerosol radiative effects and thermodynamic responses over South Asia are examined with the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of aerosol optical depths (AODs) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in northern India. The WRF-Chem model is found to heavily underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model's low bias is due to aerosol extinctions below ~2km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AOD andmore » extinction profiles averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to –0.7 K day−1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond differently between Case I and Case II, underlining the importance of determining the exact portion of scattering or absorbing aerosols that lead to the underestimation of aerosol optical depth in the model. In addition, the model results suggest that both the direct radiative effect and rapid thermodynamic responses need to be quantified for understanding aerosol radiative impacts.« less

  18. Radiative and thermodynamic responses to aerosol extinction profiles during the pre-monsoon month over South Asia

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Feng, Y.; Kotamarthi, V. R.; Coulter, R.; Zhao, C.; Cadeddu, M.

    2015-06-19

    Aerosol radiative effects and thermodynamic responses over South Asia are examined with a version of the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of Aerosol Optical Depth (AOD) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in the northern India. The WRF-Chem model is found to underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model low-bias is due to aerosol extinctions below ~2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AODmore » and extinction profiles averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to -0.7 K day−1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond differently between Case I and Case II underlying the importance of determining the exact portion of scattering or absorbing aerosols that lead to the underestimation of aerosol optical depth in the model. In addition, the model results suggest that both direct radiative effect and rapid thermodynamic responses need to be quantified for understanding aerosol radiative impacts.« less

  19. Building America Webinar: Sealing of Home Enclosures with Aerosol Particles

    Broader source: Energy.gov [DOE]

    This webinar was presented by research team Building Industry Research Alliance (BIRA), and provided information about a project that uses existing aerosol duct sealing technology to seal the entire building enclosure in order to achieve greater airtightness and energy and cost savings.

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    aerosol, allowing carefully controlled and reproducible conditions. Benchmarking with humidified ammonium sulfate aerosol indicated that the optical measurements...

  1. Oil shale, tar sand, coal research, advanced exploratory process technology, jointly sponsored research. Quarterly technical progress report, July--September 1992

    SciTech Connect (OSTI)

    Not Available

    1992-12-31

    Progress made in five research programs is described. The subtasks in oil shale study include oil shale process studies and unconventional applications and markets for western oil shale.The tar sand study is on recycle oil pyrolysis and extraction (ROPE) process. Four tasks are described in coal research: underground coal gasification; coal combustion; integrated coal processing concepts; and sold waste management. Advanced exploratory process technology includes: advanced process concepts; advanced mitigation concepts; and oil and gas technology. Jointly sponsored research covers: organic and inorganic hazardous waste stabilization; CROW field demonstration with Bell Lumber and Pole; development and validation of a standard test method for sequential batch extraction fluid; PGI demonstration project; operation and evaluation of the CO{sub 2} HUFF-N-PUFF process; fly ash binder for unsurfaced road aggregates; solid state NMR analysis of Mesaverde group, Greater Green River Basin, tight gas sands; flow-loop testing of double-wall pipe for thermal applications; shallow oil production using horizontal wells with enhanced oil recovery techniques; NMR analysis of sample from the ocean drilling program; and menu driven access to the WDEQ hydrologic data management system.

  2. Impact of aerosol size representation on modeling aerosol-cloud interactions: AEROSOL SIZE REPRESENTATION

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Zhang, Y.; Easter, R. C.; Ghan, S. J.; Abdul-Razzak, H.

    2002-11-07

    We use a 1-D version of a climate-aerosol-chemistry model with both modal and sectional aerosol size representations to evaluate the impact of aerosol size representation on modeling aerosol-cloud interactions in shallow stratiform clouds observed during the 2nd Aerosol Characterization Experiment. Both the modal (with prognostic aerosol number and mass or prognostic aerosol number, surface area and mass, referred to as the Modal-NM and Modal-NSM) and the sectional approaches (with 12 and 36 sections) predict total number and mass for interstitial and activated particles that are generally within several percent of references from a high resolution 108-section approach. The modal approachmore » with prognostic aerosol mass but diagnostic number (referred to as the Modal-M) cannot accurately predict the total particle number and surface areas, with deviations from the references ranging from 7-161%. The particle size distributions are sensitive to size representations, with normalized absolute differences of up to 12% and 37% for the 36- and 12-section approaches, and 30%, 39%, and 179% for the Modal-NSM, Modal-NM, and Modal-M, respectively. For the Modal-NSM and Modal-NM, differences from the references are primarily due to the inherent assumptions and limitations of the modal approach. In particular, they cannot resolve the abrupt size transition between the interstitial and activated aerosol fractions. For the 12- and 36-section approaches, differences are largely due to limitations of the parameterized activation for non-log-normal size distributions, plus the coarse resolution for the 12-section case. Differences are larger both with higher aerosol (i.e., less complete activation) and higher SO2 concentrations (i.e., greater modification of the initial aerosol distribution).« less

  3. Research

    SciTech Connect (OSTI)

    1999-10-01

    Subjects covered in this section are: (1) PCAST panel promotes energy research cooperation; (2) Letter issued by ANS urges funding balance in FFTF restart consideration and (3) FESAC panel releases report on priorities and balance.

  4. Advancing Climate Science with Global Research Facilities | Department...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Research at the facilities focuses on four areas: how aerosols affect the global climate; the various stages of cloud evolution; the impact of aerosols on the radiative balance of ...

  5. Laboratory Experiments and Instrument Development for the Study of Atmospheric Aerosols

    SciTech Connect (OSTI)

    Davidovits, Paul

    2011-12-10

    Soot particles are generated by incomplete combustion of fossil and biomass fuels. Through direct effects clear air aerosols containing black carbon (BC) such as soot aerosols, absorb incoming light heating the atmosphere, while most other aerosols scatter light and produce cooling. Even though BC represents only 1-2% of the total annual emissions of particulate mass to the atmosphere, it has been estimated that the direct radiative effect of BC is the second-most important contributor to global warming after absorption by CO2. Ongoing studies continue to underscore the climate forcing importance of black carbon. However, estimates of the radiative effects of black carbon on climate remain highly uncertain due to the complexity of particles containing black carbon. Quantitative measurement of BC is challenging because BC often occurs in highly non-spherical soot particles of complex morphology. Freshly emitted soot particles are typically fractal hydrophobic aggregates. The aggregates consist of black carbon spherules with diameters typically in the range of about 15-40 nm, and they are usually coated by adsorbed polyaromatic hydrocarbons (PAHs) produced during combustion. Diesel-generated soot particles are often emitted with an organic coating composed primarily of lubricating oil and unburned fuel, as well as well as PAH compounds. Sulfuric acid has also been detected in diesel and aircraft-emitted soot particles. In the course of aging, these particle coatings may be substantially altered by chemical reactions and/or the deposition of other materials. Such processes transform the optical and CCN properties of the soot aerosols in ways that are not yet well understood. Our work over the past seven years consisted of laboratory research, instrument development and characterization, and field studies with the central focus of improving our understanding of the black carbon aerosol climate impacts. During the sixth year as well as during this seventh year (no-cost extension period) of our grant, we extended our studies to perform experiments on the controlled production and characterization of secondary organic aerosol.

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Pointing Scanning Cloud Radar in the Right Direction Download a printable PDF Submitter: Fielding, M. D., University of Reading Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Fielding MD, JC Chiu, RJ Hogan, and G Feingold. 2013. "3D cloud reconstructions: Evaluation of scanning radar scan strategy with a view to surface shortwave radiation closure." Journal of Geophysical Research -

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Role of Ice Nuclei Recycling in the Maintenance of Cloud Ice in Arctic Mixed-phase Stratocumulus Download a printable PDF Submitter: Solomon, A., NOAA/ESRL/Physical Sciences Division Feingold, G., NOAA - Earth System Research Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud Life Cycle Journal Reference: Solomon A, G Feingold, and MD Shupe. 2015. "The role of ice nuclei recycling in the maintenance of cloud ice in Arctic mixed-phase

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Adoption of RRTMG in the NCAR CAM5 and CESM1 Global Climate Models Download a printable PDF Submitter: Iacono, M. J., Atmospheric & Environmental Research, Inc. Collins, W. D., Lawrence Berkeley National Laboratory Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: N/A Figure 1. Shortwave cloud forcing for three versions of the NCAR Community Atmosphere Model (CAM) with CERES

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Possible Impact of Homogeneous Freezing Nucleation on in Situ Measurements Download a printable PDF Submitter: Mitchell, D. L., Desert Research Institute Mishra, S., DOE - SunShot Initiative, AAAS S&T Policy Fellow Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Mitchell DL, S Mishra, and RP Lawson. 2011. Cirrus Clouds and Climate Engineering: New Findings on Ice Nucleation and Theoretical

  10. research

    National Nuclear Security Administration (NNSA)

    care data.

    Hydrothermal Processing to Convert Wet Biomass into Biofuels

    The ability to make useful fuels out of biological materials like plants...

  11. ARM - Cumulus Humilis Aerosol Processing Study (CHAPS)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    an airborne LIDAR provides look-down information on those same clouds from NASA's Beech King Air 200. The scientific goals of the campaign were intended to reduce uncertainties...

  12. Enhanced Geothermal Systems Research and Development: Models of Subsurface Chemical Processes Affecting Fluid Flow

    SciTech Connect (OSTI)

    Moller, Nancy; Weare J. H.

    2008-05-29

    Successful exploitation of the vast amount of heat stored beneath the earth’s surface in hydrothermal and fluid-limited, low permeability geothermal resources would greatly expand the Nation’s domestic energy inventory and thereby promote a more secure energy supply, a stronger economy and a cleaner environment. However, a major factor limiting the expanded development of current hydrothermal resources as well as the production of enhanced geothermal systems (EGS) is insufficient knowledge about the chemical processes controlling subsurface fluid flow. With funding from past grants from the DOE geothermal program and other agencies, we successfully developed advanced equation of state (EOS) and simulation technologies that accurately describe the chemistry of geothermal reservoirs and energy production processes via their free energies for wide XTP ranges. Using the specific interaction equations of Pitzer, we showed that our TEQUIL chemical models can correctly simulate behavior (e.g., mineral scaling and saturation ratios, gas break out, brine mixing effects, down hole temperatures and fluid chemical composition, spent brine incompatibilities) within the compositional range (Na-K-Ca-Cl-SO4-CO3-H2O-SiO2-CO2(g)) and temperature range (T < 350°C) associated with many current geothermal energy production sites that produce brines with temperatures below the critical point of water. The goal of research carried out under DOE grant DE-FG36-04GO14300 (10/1/2004-12/31/2007) was to expand the compositional range of our Pitzer-based TEQUIL fluid/rock interaction models to include the important aluminum and silica interactions (T < 350°C). Aluminum is the third most abundant element in the earth’s crust; and, as a constituent of aluminosilicate minerals, it is found in two thirds of the minerals in the earth’s crust. The ability to accurately characterize effects of temperature, fluid mixing and interactions between major rock-forming minerals and hydrothermal and/or injected fluids is critical to predict important chemical behaviors affecting fluid flow, such as mineral precipitation/dissolution reactions. We successfully achieved the project goal and objectives by demonstrating the ability of our modeling technology to correctly predict the complex pH dependent solution chemistry of the Al3+ cation and its hydrolysis species: Al(OH)2+, Al(OH)2+, Al(OH)30, and Al(OH)4- as well as the solubility of common aluminum hydroxide and aluminosilicate minerals in aqueous brines containing components (Na, K, Cl) commonly dominating hydrothermal fluids. In the sodium chloride system, where experimental data for model parameterization are most plentiful, the model extends to 300°C. Determining the stability fields of aluminum species that control the solubility of aluminum-containing minerals as a function of temperature and composition has been a major objective of research in hydrothermal chemistry.

  13. LMFBR aerosol release and transport program. Quarterly progress report, July-September 1981

    SciTech Connect (OSTI)

    Kress, T.S.; Tobias, M.L.

    1982-01-01

    This report summarizes progress for the Aerosol Release and Transport Program sponsored by the Office of Nuclear Regulatory Research, Division of Accident Evaluation of the Nuclear Regulatory Commission for the period July-September 1981. Topics discussed include (1) preparations for under-sodium tests at the Fast Aerosol Simulant Test Facility, (2) progress in interpretation of Oak Ridge National Laboratory-Sandia Laboratory normalization test results, (3) U/sub 3/O/sub 8/ in steam (light-water reactor accident) aerosol experiments conducted in the Nuclear Safety Power Plant, (4) experiments on B/sub 2/O/sub 3/ and SiO/sub 2/ aerosols at the Containment Research Installation-II Facility, (5) fuel-melting tests in small-scale experimental facilities for the core-melt aerosol program, (6) analytical comparison of simple adiabatic nonlinear and linear analytical models of bubble oscillation phenomena with experimental data.

  14. ARM - Campaign Instrument - drum-aerosol

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govInstrumentsdrum-aerosol Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign Instrument : Drum Aerosol Sampler (DRUM-AEROSOL) Instrument Categories Aerosols Campaigns Aerosol IOP [ Download Data ] Southern Great Plains, 2003.05.01 - 2003.05.31 Primary Measurements Taken The following measurements are those considered scientifically relevant. Refer to the datastream (netcdf) file headers for the list of all available measurements, including

  15. Two-Column Aerosol Project

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Column Aerosol Project Tiny particles in the sky known as "aerosols" come in many forms-dust, soot, and sea salt, for example. Depending on the type of aerosol, it can either absorb or reflect sunlight, which in turn can cause either a warming or cooling effect in the atmosphere. But to what extent? The answer to this question is critical for scientists trying to envision what Earth's climate could be like 10, 50, and even 100 years from now. To help find the answer, the Department of

  16. AERONET: The Aerosol Robotic Network

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    AERONET collaboration provides globally distributed observations of spectral aerosol optical Depth (AOD), inversion products, and precipitable water in diverse aerosol regimes. Aerosol optical depth data are computed for three data quality levels: Level 1.0 (unscreened), Level 1.5 (cloud-screened), and Level 2.0 (cloud screened and quality-assured). Inversions, precipitable water, and other AOD-dependent products are derived from these levels and may implement additional quality checks.[Copied from http://aeronet.gsfc.nasa.gov/new_web/system_descriptions.html

  17. Stratospheric aerosol geoengineering

    SciTech Connect (OSTI)

    Robock, Alan

    2015-03-30

    The Geoengineering Model Intercomparison Project, conducting climate model experiments with standard stratospheric aerosol injection scenarios, has found that insolation reduction could keep the global average temperature constant, but global average precipitation would reduce, particularly in summer monsoon regions around the world. Temperature changes would also not be uniform; the tropics would cool, but high latitudes would warm, with continuing, but reduced sea ice and ice sheet melting. Temperature extremes would still increase, but not as much as without geoengineering. If geoengineering were halted all at once, there would be rapid temperature and precipitation increases at 5–10 times the rates from gradual global warming. The prospect of geoengineering working may reduce the current drive toward reducing greenhouse gas emissions, and there are concerns about commercial or military control. Because geoengineering cannot safely address climate change, global efforts to reduce greenhouse gas emissions and to adapt are crucial to address anthropogenic global warming.

  18. Assessing the Effects of Anthropogenic Aerosols on Pacific Storm Track Using a Multiscale Global Climate Model

    SciTech Connect (OSTI)

    Wang, Yuan; Wang, Minghuai; Zhang, Renyi; Ghan, Steven J.; Lin, Yun; Hu, Jiaxi; Pan, Bowen; Levy, Misti; Jiang, Jonathan; Molina, Mario J.

    2014-05-13

    Atmospheric aerosols impact weather and global general circulation by modifying cloud and precipitation processes, but the magnitude of cloud adjustment by aerosols remains poorly quantified and represents the largest uncertainty in estimated forcing of climate change. Here we assess the impacts of anthropogenic aerosols on the Pacific storm track using a multi-scale global aerosol-climate model (GCM). Simulations of two aerosol scenarios corresponding to the present day and pre-industrial conditions reveal long-range transport of anthropogenic aerosols across the north Pacific and large resulting changes in the aerosol optical depth, cloud droplet number concentration, and cloud and ice water paths. Shortwave and longwave cloud radiative forcing at the top of atmosphere are changed by - 2.5 and + 1.3 W m-2, respectively, by emission changes from pre-industrial to present day, and an increased cloud-top height indicates invigorated mid-latitude cyclones. The overall increased precipitation and poleward heat transport reflect intensification of the Pacific storm track by anthropogenic aerosols. Hence, this work provides for the first time a global perspective of the impacts of Asian pollution outflows from GCMs. Furthermore, our results suggest that the multi-scale modeling framework is essential in producing the aerosol invigoration effect of deep convective clouds on the global scale.

  19. Ganges Valley Aerosol Experiment: Science and Operations Plan

    SciTech Connect (OSTI)

    Kotamarthi, VR

    2010-06-21

    The Ganges Valley region is one of the largest and most rapidly developing sections of the Indian subcontinent. The Ganges River, which provides the region with water needed for sustaining life, is fed primarily by snow and rainfall associated with Indian summer monsoons. Impacts of changes in precipitation patterns, temperature, and the flow of the snow-fed rivers can be immense. Recent satellite-based measurements have indicated that the upper Ganges Valley has some of the highest persistently observed aerosol optical depth values. The aerosol layer covers a vast region, extending across the Indo-Gangetic Plain to the Bay of Bengal during the winter and early spring of each year. The persistent winter fog in the region is already a cause of much concern, and several studies have been proposed to understand the economic, scientific, and societal dimensions of this problem. During the INDian Ocean EXperiment (INDOEX) field studies, aerosols from this region were shown to affect cloud formation and monsoon activity over the Indian Ocean. This is one of the few regions showing a trend toward increasing surface dimming and enhanced mid-tropospheric warming. Increasing air pollution over this region could modify the radiative balance through direct, indirect, and semi-indirect effects associated with aerosols. The consequences of aerosols and associated pollution for surface insolation over the Ganges Valley and monsoons, in particular, are not well understood. The proposed field study is designed for use of (1) the ARM Mobile Facility (AMF) to measure relevant radiative, cloud, convection, and aerosol optical characteristics over mainland India during an extended period of 912 months and (2) the G-1 aircraft and surface sites to measure relevant aerosol chemical, physical, and optical characteristics in the Ganges Valley during a period of 612 weeks. The aerosols in this region have complex sources, including burning of coal, biomass, and biofuels; automobile emissions; and dust. The extended AMF deployment will enable measurements under different regimes of the climate and aerosol abundancein the wet monsoon period with low aerosol loading; in the dry, hot summer with aerosols dispersed throughout the atmospheric column; and in the cool, dry winter with aerosols confined mostly to the boundary later and mid-troposphere. Each regime, in addition, has its own distinct radiative and atmospheric dynamic drivers. The aircraft operational phase will assist in characterizing the aerosols at times when they have been observed to be at the highest concentrations. A number of agencies in India will collaborate with the proposed field study and provide support in terms of planning, aircraft measurements, and surface sites. The high concentration of aerosols in the upper Ganges Valley, together with hypotheses involving several possible mechanisms with direct impacts on the hydrologic cycle of the region, gives us a unique opportunity to generate data sets that will be useful both in understanding the processes at work and in providing answers regarding the effects of aerosols on climate in a region where the perturbation is the highest.

  20. Thin Film Materials and Processing Techniques for a Next Generation Photovoltaic Device: Cooperative Research and Development Final Report, CRADA Number CRD-12-470

    SciTech Connect (OSTI)

    van Hest, M.

    2013-08-01

    This research extends thin film materials and processes relevant to the development and production of a next generation photovoltaic device.

  1. Evaluating Membrane Processes for Air Conditioning, Highlights in Research and Development (Fact Sheet), NREL (National Renewable Energy Laboratory)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    NREL compiles state-of-the-art review on membrane processes for air conditioning to identify future research opportunities. Researchers are pursuing alternatives to conventional heating, ventilating, and air-conditioning (HVAC) practices, especially cool- ing and dehumidification, because of high energy use, environmentally harmful refrigerants, and a need for better humidity control. Advancements in membrane technology enable new possibilities in this area. Membranes are traditionally used for

  2. ARM - Measurement - Aerosol backscattered radiation

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol backscattered radiation The scattering of radiant energy into the hemisphere of space bounded by a ...

  3. Science Plan Biogenic Aerosols – Effects on Clouds and Climate (BAECC)

    SciTech Connect (OSTI)

    Petäjä, T

    2013-12-01

    Atmospheric aerosol particles impact human health in urban environments, while on regional and global scales they can affect climate patterns, the hydrological cycle, and the intensity of radiation that reaches the Earth’s surface. In spite of recent advances in the understanding of aerosol formation processes and the links between aerosol dynamics and biosphere-atmosphere-climate interactions, great challenges remain in the analysis of related processes on a global scale. Boreal forests, situated in a circumpolar belt in the northern latitudes throughout the United States, Canada, Russia and Scandinavia, are among the most active areas of atmospheric aerosol formation among all biomes. The formation of aerosol particles and their growth to the sizes of cloud condensation nuclei in these areas are associated with biogenic volatile organic emissions from vegetation and soil.

  4. Method for producing monodisperse aerosols

    DOE Patents [OSTI]

    Ortiz, Lawrence W.; Soderholm, Sidney C.

    1990-01-01

    An aerosol generator is described which is capable of producing a monodisperse aerosol within narrow limits utilizing an aqueous solution capable of providing a high population of seed nuclei and an organic solution having a low vapor pressure. The two solutions are cold nebulized, mixed, vaporized, and cooled. During cooling, particles of the organic vapor condense onto the excess seed nuclei, and grow to a uniform particle size.

  5. ARM Aerosol Working Group Meeting

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Report ARM STM 2008 Norfolk, VA Connor Flynn for B Schmid and AWG Members AWG Instruments * Raman Lidar - SGP * Micropulse Lidars - all sites * Aerosol Sampling - SGP, NSA, AMF - scattering, absorption, number, size distribution, hygroscopicity, CCN, composition (major ions). * In situ Aerosol Profile (Cessna) - scattering, absorption, number, hygroscopicity, * Radiometers: - MFRSR, NIMFR, RSS, Cimel, AERI, SWS AWG-related Field Campaigns * Recent Past: - MASRAD (Marine Stratus Radiation,

  6. Final Project Report - ARM CLASIC CIRPAS Twin Otter Aerosol

    SciTech Connect (OSTI)

    John A. Ogren

    2010-04-05

    The NOAA/ESRL/GMD aerosol group made three types of contributions related to airborne measurements of aerosol light scattering and absorption for the Cloud and Land Surface Interaction Campaign (CLASIC) in June 2007 on the Twin Otter research airplane operated by the Center for Interdisciplinary Remotely-Piloted Aircraft Studies (CIRPAS). GMD scientists served as the instrument mentor for the integrating nephelometer and particle soot absorption photometer (PSAP) on the Twin Otter during CLASIC, and were responsible for (1) instrument checks/comparisons; (2) instrument trouble shooting/repair; and (3) data quality control (QC) and submittal to the archive.

  7. In-tank precipitation with tetraphenylborate: recent process and research results

    SciTech Connect (OSTI)

    Walker, D.D.; Barnes, M.J.; Crawford, C.L.; Peterson, R.A.; Swingle, R.F.; Fink, S.D.

    1997-09-01

    At the Savannah River Site, the In-Tank Precipitation process uses sodium tetraphenylborate to decontaminate soluble waste by precipitating cesium-137.

  8. Applied research and evaluation of process concepts for liquefaction and gasification of western coals. Final report

    SciTech Connect (OSTI)

    Wiser, W. H.

    1980-09-01

    Fourteen sections, including five subsections, of the final report covering work done between June 1, 1975 to July 31, 1980 on research programs in coal gasification and liquefaction have been entered individually into EDB and ERA. (LTN)

  9. CARES: Carbonaceous Aerosol and Radiative Effects Study Operations Plan

    SciTech Connect (OSTI)

    Zaveri, RA; Shaw, WJ; Cziczo, DJ

    2010-07-12

    The CARES field campaign is motivated by the scientific issues described in the CARES Science Plan. The primary objectives of this field campaign are to investigate the evolution and aging of carbonaceous aerosols and their climate-affecting properties in the urban plume of Sacramento, California, a mid-size, mid-latitude city that is located upwind of a biogenic volatile organic compound (VOC) emission region. Our basic observational strategy is to make comprehensive gas, aerosol, and meteorological measurements upwind, within, and downwind of the urban area with the DOE G-1 aircraft and at strategically located ground sites so as to study the evolution of urban aerosols as they age and mix with biogenic SOA precursors. The NASA B-200 aircraft, equipped with the High Spectral Resolution Lidar (HSRL), digital camera, and the Research Scanning Polarimeter (RSP), will be flown in coordination with the G-1 to characterize the vertical and horizontal distribution of aerosols and aerosol optical properties, and to provide the vertical context for the G-1 and ground in situ measurements.

  10. Aerosols and Clouds: In Cahoots to Change Climate

    ScienceCinema (OSTI)

    Berg, Larry

    2014-06-02

    Key knowledge gaps persist despite advances in the scientific understanding of how aerosols and clouds evolve and affect climate. The Two-Column Aerosol Project, or TCAP, was designed to provide a detailed set of observations to tackle this area of unknowns. Led by PNNL atmospheric scientist Larry Berg, ARM's Climate Research Facility was deployed in Cape Cod, Massachusetts for the 12-month duration of TCAP, which came to a close in June 2013. "We are developing new tools to look at particle chemistry, like our mass spectrometer used in TCAP that can tell us the individual chemical composition of an aerosol," said Berg. "Then, we'll run our models and compare it with the data that we have to make sure we're getting correct answers and make sure our climate models are reflecting the best information."

  11. Aerosols and Clouds: In Cahoots to Change Climate

    SciTech Connect (OSTI)

    Berg, Larry

    2014-03-29

    Key knowledge gaps persist despite advances in the scientific understanding of how aerosols and clouds evolve and affect climate. The Two-Column Aerosol Project, or TCAP, was designed to provide a detailed set of observations to tackle this area of unknowns. Led by PNNL atmospheric scientist Larry Berg, ARM's Climate Research Facility was deployed in Cape Cod, Massachusetts for the 12-month duration of TCAP, which came to a close in June 2013. "We are developing new tools to look at particle chemistry, like our mass spectrometer used in TCAP that can tell us the individual chemical composition of an aerosol," said Berg. "Then, we'll run our models and compare it with the data that we have to make sure we're getting correct answers and make sure our climate models are reflecting the best information."

  12. The impact of biogenic carbon emissions on aerosol absorption inMexico City

    SciTech Connect (OSTI)

    Marley, N; Gaffney, J; Tackett, M J; Sturchio, N; Hearty, L; Martinez, N; Hardy, K D; Machany-Rivera, A; Guilderson, T P; MacMillan, A; Steelman, K

    2009-02-24

    In order to determine the wavelength dependence of atmospheric aerosol absorption in the Mexico City area, the absorption angstrom exponents (AAEs) were calculated from aerosol absorption measurements at seven wavelengths obtained with a seven-channel aethalometer during two field campaigns, the Mexico City Metropolitan Area study in April 2003 (MCMA 2003) and the Megacity Initiative: Local and Global Research Observations in March 2006 (MILAGRO). The AAEs varied from 0.76 to 1.56 in 2003 and from 0.54 to 1.52 in 2006. The AAE values determined in the afternoon were consistently higher than the corresponding morning values, suggesting the photochemical formation of absorbing secondary organic aerosols (SOA) in the afternoon. The AAE values were compared to stable and radiocarbon isotopic measurements of aerosol samples collected at the same time to determine the sources of the aerosol carbon. The fraction of modern carbon (fM) in the aerosol samples, as determined from {sup 14}C analysis, showed that 70% of the carbonaceous aerosols in Mexico City were from modern sources, indicating a significant impact from biomass burning during both field campaigns. The {sup 13}C/{sup 12}C ratios of the aerosol samples illustrate the significant impact of Yucatan forest fires (C-3 plants) in 2003 and local grass fires (C-4 plants) at site T1 in 2006. A direct comparison of the fM values, stable carbon isotope ratios, and calculated aerosol AAEs suggested that the wavelength dependence of the aerosol absorption was controlled by the biogenically derived aerosol components.

  13. ARM: Tandem Differential Mobility Analyzer Aerosol Particle Sizer...

    Office of Scientific and Technical Information (OSTI)

    Subject: 54 Environmental Sciences Aerosol concentration; Aerosol particle size distribution; Hygroscopic growth; Particle number concentration; Particle size distribution Dataset ...

  14. Thermophoretic separation of aerosol particles from a sampled gas stream

    DOE Patents [OSTI]

    Postma, A.K.

    1984-09-07

    This disclosure relates to separation of aerosol particles from gas samples withdrawn from within a contained atmosphere, such as containment vessels for nuclear reactors or other process equipment where remote gaseous sampling is required. It is specifically directed to separation of dense aerosols including particles of any size and at high mass loadings and high corrosivity. The United States Government has rights in this invention pursuant to Contract DE-AC06-76FF02170 between the US Department of Energy and Westinghouse Electric Corporation.

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Linking Ice Nucleation to Aerosols and Its Impact on CAM5 Simulated Arctic Clouds and Radiation Download a printable PDF Submitter: Xie, S., Lawrence Livermore National Laboratory Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Cloud Life Cycle Journal Reference: Xie S, X Liu, C Zhao, and Y Zhang. 2013. "Sensitivity of CAM5 simulated arctic clouds and radiation to ice nucleation parameterization." Journal of Climate, 26(16),

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Determining the Future of CO2 Using an Earth System Model Download a printable PDF Submitter: Keppel-Aleks, G., University of Michigan Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Aerosol Life Cycle Journal Reference: Keppel-Aleks G, JT Randerson, K Lindsay, BB Stephens, JK Moore, SC Doney, PE Thornton, NM Mahowald, FM Hoffman, C Sweeney, PP Tans, PO Wennberg, and SC Wofsy. 2013. "Atmospheric carbon dioxide variability in the Community

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ground Stations Likely Get a Boost from Satellites to Estimate Carbon Dioxide Emissions Download a printable PDF Submitter: Roeder, L. R., Pacific Northwest National Laboratory Area of Research: Surface Properties Working Group(s): Aerosol Life Cycle Journal Reference: Basu S, S Guerlet, A Butz, S Houweling, OP Hasekamp, I Aben, PB Krummel, LP Steele, RL Langenfelds, MS Torn, SC Biraud, B Stephens, A Andrews, and D Worthy. 2013. "Global CO2 fluxes estimated from GOSAT retrievals of total

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Growing More Effective Ways to Measure Climate Change Download a printable PDF Submitter: Maseyk, K. S., Universite Pierre et Marie Curie, Paris 6 Area of Research: Surface Properties Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Maseyk K, JA Berry, D Billesbach, JE Campbell, MS Torn, M Zahniser, and U Seibt. 2014. "Sources and sinks of carbonyl sulfide in an agricultural field in the Southern Great Plains." Proceedings of the National Academy of

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Satellite Inference of Thermals and Cloud Base Updraft Speeds Download a printable PDF Submitter: Zheng, Y., University of Maryland Area of Research: Vertical Velocity Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Zheng Y, D Rosenfeld, and Z Li. 2015. "Satellite inference of thermals and cloud base updraft speeds based on retrieved surface and cloud base temperatures." Journal of the Atmospheric Sciences, , . ONLINE. Validation of satellite-estimated

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    General Formulation for Representing Cloud-to-Rain Transition in Atmospheric Models Submitter: Liu, Y., Brookhaven National Laboratory Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Aerosol, Cloud Modeling, Cloud Properties Journal Reference: Liu, Y., P. H. Daum, R. McGraw, M. Miller, and S. Niu, 2007: Theoretical formulation for autoconversion rate of cloud droplet concentration. Geophys. Res. Lett., 34, L116821, doi:10.1029/2007GL030389

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ground-Based Measurements in Support of Liquid-Dependent Ice Nucleation in Arctic Clouds Download a printable PDF Submitter: de Boer, G., University of Colorado, Boulder/CIRES Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: de Boer G, H Morrison, MD Shupe, and R Hildner. 2011. "Evidence of liquid dependent ice nucleation in high-latitude stratiform clouds from surface remote

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Estimating the Ice Crystal Enhancement Factor in the Tropics Download a printable PDF Submitter: Zeng, X., Morgan State University GSFC, N., NASA GSFC Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Zeng X, W Tao, T Matsui, S Xie, S Lang, M Zhang, DO Starr, and X Li. 2011. "Estimating the ice crystal enhancement factor in the tropics." Journal of the

  3. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Dependence of the Single-Scattering Properties of Small Ice Crystals on Idealized Shape Models Download a printable PDF Submitter: Um, J., University of Illinois, Urbana McFarquhar, G., University of Illinois, Urbana Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Um J and GM McFarquhar. 2011. "Dependence of the single-scattering properties of small ice crystals on idealized shape

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Factors Influencing the Microphysics and Radiative Properties of Liquid-Dominated Arctic Clouds Download a printable PDF Submitter: Earle, M., Environment Canada Liu, P., Environment Canada Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Earle ME, PS Liu, JW Strapp, A Zelenyuk, D Imre, GM McFarquhar, NC Shantz, and WR Leaitch. 2011. "Factors influencing the microphysics and radiative properties of

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Birth of a Cloud Droplet Download a printable PDF Submitter: Ghan, S. J., Pacific Northwest National Laboratory Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Ghan SJ, H Abdul-Razzak, A Nenes, Y Ming, X Liu, M Ovchinnikov, B Shipway, N Meskhidze, J Xu, and X Shi. 2011. "Droplet nucleation: Physically-based parameterizations and comparative evaluation." Journal of Advances

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Tropical Rain Clouds Still a Challenge to Cloud-Resolving Models Download a printable PDF Submitter: Fridlind, A. M., NASA - Goddard Institute for Space Studies Ackerman, A., NASA - Goddard Institute for Space Studies Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Fridlind AM, AS Ackerman, J Chaboureau, J Fan, WW Grabowski, AA Hill, TR Jones, MM Khaiyer, G Liu, P Minnis, H Morrison, L Nguyen,

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Regional Controls on Ozone Precursors Will Have Different Impacts on Future Climate Download a printable PDF Submitter: Bergmann, D., Lawrence Livermore National Laboratory Chuang, C., Lawrence Livermore National Laboratory Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Aerosol Life Cycle Journal Reference: Fry MM, V Naik, JJ West, MD Schwartzkopf, AM Fiore, WJ Collins, FJ Dentener, DT Shindell, C Atherton, D Bergmann, BN Duncan, P Hess, IA

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    2007 Floods Not a Complete Washout in U.S. Great Plains Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Atmospheric Thermodynamics and Vertical Structures Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Lamb PJ, DH Portis, and A Zangvil. 2012. "Investigation of Large-Scale Atmospheric Moisture Budget and Land Surface Interactions over U.S. Southern Great Plains including for CLASIC (June 2007)." Journal of

  9. RESEARCH AND DEVELOPMENT OF AN INTEGRAL SEPARATOR FOR A CENTRIFUGAL GAS PROCESSING FACILITY

    SciTech Connect (OSTI)

    LANCE HAYS

    2007-02-27

    A COMPACT GAS PROCESSING DEVICE WAS INVESTIGATED TO INCREASE GAS PRODUCTION FROM REMOTE, PREVIOUSLY UN-ECONOMIC RESOURCES. THE UNIT WAS TESTED ON AIR AND WATER AND WITH NATURAL GAS AND LIQUID. RESULTS ARE REPORTED WITH RECOMMENDATIONS FOR FUTURE WORK.

  10. Research Summary: Corrosion Considerations for Thermochemical Biomass Liquefaction Process Systems in Biofuel Production

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Brady, Michael P; Keiser, James R; Leonard, Donovan N; Whitmer, Lysle; Thomson, Jeffery K

    2014-01-01

    Thermochemical liquifaction processing of biomass to produce bio-derived fuels (e.g. gasoline, jet fuel, diesel, home heating oil, etc.) is of great recent interest as a renewable energy source. Approaches under investigation include direct liquefaction, hydrothermal liquefaction, hydropyrolysis, fast pyrolysis, etc. to produce energy dense liquids that can be utilized as produced or further processed to provide products of higher value. An issue with bio-oils is that they tend to contain significant concentrations of organic compounds, which make the bio-oil acidic and a potential source of corrosion issues in in transport, storage, and use. Efforts devoted to modified/further processing of bio-oilsmore » to make them less corrosive are currently being widely pursued. Another aspect that must also be addressed is potential corrosion issues in the bio-oil liquefaction process equipment itself. Depending on the specific process, bio-oil liquefaction production temperatures can reach up to 400-600 C, and involve the presence of aggressive sulfur, and halide species from both the biomass used and/or process additives. Detailed knowledge of the corrosion resistance of candidate process equipment alloys in these bio-oil production environments is currently lacking. This paper summarizes our recent, ongoing efforts to assess the extent to which corrosion of bio-oil process equipment may be an issue, with the ultimate goal of providing the basis to select the lowest cost alloy grades capable of providing the long-term corrosion resistance needed for future bio-oil production plants.« less

  11. Research Summary: Corrosion Considerations for Thermochemical Biomass Liquefaction Process Systems in Biofuel Production

    SciTech Connect (OSTI)

    Brady, Michael P; Keiser, James R; Leonard, Donovan N; Whitmer, Lysle; Thomson, Jeffery K

    2014-01-01

    Thermochemical liquifaction processing of biomass to produce bio-derived fuels (e.g. gasoline, jet fuel, diesel, home heating oil, etc.) is of great recent interest as a renewable energy source. Approaches under investigation include direct liquefaction, hydrothermal liquefaction, hydropyrolysis, fast pyrolysis, etc. to produce energy dense liquids that can be utilized as produced or further processed to provide products of higher value. An issue with bio-oils is that they tend to contain significant concentrations of organic compounds, which make the bio-oil acidic and a potential source of corrosion issues in in transport, storage, and use. Efforts devoted to modified/further processing of bio-oils to make them less corrosive are currently being widely pursued. Another aspect that must also be addressed is potential corrosion issues in the bio-oil liquefaction process equipment itself. Depending on the specific process, bio-oil liquefaction production temperatures can reach up to 400-600 C, and involve the presence of aggressive sulfur, and halide species from both the biomass used and/or process additives. Detailed knowledge of the corrosion resistance of candidate process equipment alloys in these bio-oil production environments is currently lacking. This paper summarizes our recent, ongoing efforts to assess the extent to which corrosion of bio-oil process equipment may be an issue, with the ultimate goal of providing the basis to select the lowest cost alloy grades capable of providing the long-term corrosion resistance needed for future bio-oil production plants.

  12. About the Rhythms of Variability of the Submicron Aerosol Characteristics in the Near-Ground Air Layer in West Siberia

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    the Rhythms of Variability of the Submicron Aerosol Characteristics in the Near-Ground Air Layer in West Siberia M. V. Panchenko, V. S. Kozlov, S. A. Terpugova, and E. P. Yausheva Institute of Atmospheric Optics Tomsk, Russia Introduction The study of the role of atmospheric aerosol in climate change and radiative processes in the lower atmosphere requires knowing the peculiarities of the variability of the aerosol characteristics under the effect of geophysical factors of different temporal and

  13. Design-Build Process for the Research Support Facility (RSF) (Book)

    SciTech Connect (OSTI)

    Not Available

    2012-06-01

    An in-depth look at how the U.S. DOE and NREL used a performance-based design-build contract to build the Research Support Facility (RSF); one of the most energy efficient office buildings in the world.

  14. ARM - Field Campaign - Fall 1997 Aerosol IOP

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Send Campaign : Fall 1997 Aerosol IOP 1997.09.15 - 1997.10.05 Lead Scientist : Stephen Schwartz For data sets, see below. Summary The Aerosol IOP was highlighted by the...

  15. "Big Picture" Process Modeling Tools |GE Global Research

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Using process modeling tools to attain cost-effective results for GE customers Click to email this to a friend (Opens in new window) Share on Facebook (Opens in new window) Click to share (Opens in new window) Click to share on LinkedIn (Opens in new window) Click to share on Tumblr (Opens in new window) Using process modeling tools to attain cost-effective results for GE customers Jimmy Lopez 2015.03.26 Sometimes, we need to look outside the box to realize the powerful tools we have inside.

  16. ARM - Measurement - Aerosol particle size distribution

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AOS : Aerosol Observing System CSPHOT : Cimel Sunphotometer HTDMA : Humidified Tandem Differential Mobility Analyzer SMPS : Scanning mobility particle sizer TDMA : Tandem...

  17. Aerosol Oxidation Speeds Up in Smoggy Air

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Oxidation Speeds Up in Smoggy Air Aerosol Oxidation Speeds Up in Smoggy Air Print Wednesday, 17 February 2016 11:37 Organic aerosols (nanometer-sized liquid or solid particles suspended in air) are important constituents of the troposphere, and their chemistry has large-scale impacts on climate, pollution, and health. Accurate predictions of these aerosol impacts require a robust microphysical understanding of all relevant chemical reaction mechanisms and time scales, including those

  18. Aerosol Remote Sealing System - Energy Innovation Portal

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Remote Sealing System Lawrence Berkeley National Laboratory Contact LBL About This Technology Technology Marketing SummaryMark Modera and Francois Remi Carrie from Berkeley National Laboratory have developed a rapid, economical technique to seal duct and other enclosed systems by means of an internally injected aerosol. DescriptionBerkeley National Laboratory's aerosol compound seals holes in enclosed systems and is effective even after bends and junctions. A unique, in situ aerosol

  19. Field Trial of an Aerosol-Based Enclosure Sealing Technology

    SciTech Connect (OSTI)

    Harrington, Curtis; Springer, David

    2015-09-01

    This report presents the results from several demonstrations of a new method for sealing building envelope air leaks using an aerosol sealing process developed by the Western Cooling Efficiency Center at UC Davis. The process involves pressurizing a building while applying an aerosol sealant to the interior. As air escapes through leaks in the building envelope, the aerosol particles are transported to the leaks where they collect and form a seal that blocks the leak. Standard blower door technology is used to facilitate the building pressurization, which allows the installer to track the sealing progress during the installation and automatically verify the final building tightness. Each aerosol envelope sealing installation was performed after drywall was installed and taped, and the process did not appear to interrupt the construction schedule or interfere with other trades working in the homes. The labor needed to physically seal bulk air leaks in typical construction will not be replaced by this technology. However, this technology is capable of bringing the air leakage of a building that was built with standard construction techniques and HERS-verified sealing down to levels that would meet DOE Zero Energy Ready Homes program requirements. When a developer is striving to meet a tighter envelope leakage specification, this technology could greatly reduce the cost to achieve that goal by providing a simple and relatively low cost method for reducing the air leakage of a building envelope with little to no change in their common building practices.

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    First Observation-Based Estimates of Cloud-Free Aerosol Radiative Forcing Across China ... Mean annual shortwave aerosol radiative forcing (SWARF) averaged across China. Spatial ...

  1. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    and aerosol optical quantities for some distinct aerosol types using an extensive set of observational data collected at multiple Atmospheric Radiation Measurement (ARM) Climate...

  2. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    from size distribution and light scattering data: Weakly absorbing aerosol." Atmospheric Measurement Techniques, 7, doi:10.5194amt-7-3247-2014. Observing Aerosols. The ARM...

  3. Real time infrared aerosol analyzer

    DOE Patents [OSTI]

    Johnson, Stanley A.; Reedy, Gerald T.; Kumar, Romesh

    1990-01-01

    Apparatus for analyzing aerosols in essentially real time includes a virtual impactor which separates coarse particles from fine and ultrafine particles in an aerosol sample. The coarse and ultrafine particles are captured in PTFE filters, and the fine particles impact onto an internal light reflection element. The composition and quantity of the particles on the PTFE filter and on the internal reflection element are measured by alternately passing infrared light through the filter and the internal light reflection element, and analyzing the light through infrared spectrophotometry to identify the particles in the sample.

  4. Reducing Plug and Process Loads for a Large Scale, Low Energy Office Building: NREL's Research Support Facility: Preprint

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Reducing Plug and Process Loads for a Large Scale, Low Energy Office Building: NREL's Research Support Facility Preprint Chad Lobato, Shanti Pless, Michael Sheppy, and Paul Torcellini Presented at the ASHRAE Winter Conference Las Vegas, Nevada January 29 - February 2, 2011 Conference Paper NREL/CP-5500-49002 February 2011 NOTICE The submitted manuscript has been offered by an employee of the Alliance for Sustainable Energy, LLC (Alliance), a contractor of the US Government under Contract No.

  5. ARM - PI Product - Black Carbon aerosol mass concentration in snow and rain

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    samples over Barrow in the Arctic ProductsBlack Carbon aerosol mass concentration in snow and rain samples over Barrow in the Arctic ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send PI Product : Black Carbon aerosol mass concentration in snow and rain samples over Barrow in the Arctic [ ARM research ] Deposition of black carbon aerosol (BC) on snow (i.e. wet deposition) is considered to lower snow albedo and

  6. Quantifying the Uncertainties of Aerosol Indirect Effects and Impacts on Decadal-Scale Climate Variability in NCAR CAM5 and CESM1

    SciTech Connect (OSTI)

    Park, Sungsu

    2014-12-12

    The main goal of this project is to systematically quantify the major uncertainties of aerosol indirect effects due to the treatment of moist turbulent processes that drive aerosol activation, cloud macrophysics and microphysics in response to anthropogenic aerosol perturbations using the CAM5/CESM1. To achieve this goal, the P.I. hired a postdoctoral research scientist (Dr. Anna Fitch) who started her work from the Nov.1st.2012. In order to achieve the project goal, the first task that the Postdoc. and the P.I. did was to quantify the role of subgrid vertical velocity variance on the activation and nucleation of cloud liquid droplets and ice crystals and its impact on the aerosol indirect effect in CAM5. First, we analyzed various LES cases (from dry stable to cloud-topped PBL) to check whether this isotropic turbulence assumption used in CAM5 is really valid. It turned out that this isotropic turbulence assumption is not universally valid. Consequently, from the analysis of LES, we derived an empirical formulation relaxing the isotropic turbulence assumption used for the CAM5 aerosol activation and ice nucleation, and implemented the empirical formulation into CAM5/CESM1, and tested in the single-column and global simulation modes, and examined how it changed aerosol indirect effects in the CAM5/CESM1. These results were reported in the poster section in the 18th Annual CESM workshop held in Breckenridge, CO during Jun.17-20.2013. While we derived an empirical formulation from the analysis of couple of LES from the first task, the general applicability of that empirical formulation was questionable, because it was obtained from the limited number of LES simulations. The second task we did was to derive a more fundamental analytical formulation relating vertical velocity variance to TKE using other information starting from basic physical principles. This was a somewhat challenging subject, but if this could be done in a successful way, it could be directly implemented into the CAM5 as a practical parameterization, and substantially contributes to achieving the project goal. Through an intensive research for about one year, we found appropriate mathematical formulation and tried to implement it into the CAM5 PBL and activation routine as a practical parameterized numerical code. During these processes, however, the Postdoc applied for another position in Sweden, Europe, and accepted a job offer there, and left NCAR in August 2014. In Sweden, Dr. Anna Fitch is still working on this subject in a part time, planning to finalize the research and to write the paper in a near future.

  7. Hyperspectral Aerosol Optical Depths from TCAP Flights

    SciTech Connect (OSTI)

    Shinozuka, Yohei; Johnson, Roy R.; Flynn, Connor J.; Russell, P. B.; Schmid, Beat; Redemann, Jens; Dunagan, Stephen; Kluzek, Celine D.; Hubbe, John M.; Segal-Rosenheimer, Michal; Livingston, J. M.; Eck, T.; Wagener, Richard; Gregory, L.; Chand, Duli; Berg, Larry K.; Rogers, Ray; Ferrare, R. A.; Hair, John; Hostetler, Chris A.; Burton, S. P.

    2013-11-13

    4STAR (Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research), the worlds first hyperspectral airborne tracking sunphotometer, acquired aerosol optical depths (AOD) at 1 Hz during all July 2012 flights of the Two Column Aerosol Project (TCAP). Root-mean square differences from AERONET ground-based observations were 0.01 at wavelengths between 500-1020 nm, 0.02 at 380 and 1640 nm and 0.03 at 440 nm in four clear-sky fly-over events, and similar in ground side-by-side comparisons. Changes in the above-aircraft AOD across 3-km-deep spirals were typically consistent with integrals of coincident in situ (on DOE Gulfstream 1 with 4STAR) and lidar (on NASA B200) extinction measurements within 0.01, 0.03, 0.01, 0.02, 0.02, 0.02 at 355, 450, 532, 550, 700, 1064 nm, respectively, despite atmospheric variations and combined measurement uncertainties. Finer vertical differentials of the 4STAR measurements matched the in situ ambient extinction profile within 14% for one homogeneous column. For the AOD observed between 350-1660 nm, excluding strong water vapor and oxygen absorption bands, estimated uncertainties were ~0.01 and dominated by (then) unpredictable throughput changes, up to +/-0.8%, of the fiber optic rotary joint. The favorable intercomparisons herald 4STARs spatially-resolved high-frequency hyperspectral products as a reliable tool for climate studies and satellite validation.

  8. Laboratory Testing of Aerosol for Enclosure Air Sealing

    SciTech Connect (OSTI)

    Harrington, C.; Modera, M.

    2012-05-01

    Space conditioning energy use can be significantly reduced by addressing uncontrolled infiltration and exfiltration through the envelope of a building. A process for improving the air tightness of a building envelope by sealing shell leaks with an aerosol sealing technology is presented. Both retrofit and new construction applications are possible through applying this process either in attics and crawlspaces or during rough-in stage.

  9. Externally pressurized porous cylinder for multiple surface aerosol generation and method of generation

    DOE Patents [OSTI]

    Apel, Charles T.; Layman, Lawrence R.; Gallimore, David L.

    1988-01-01

    A nebulizer for generating aerosol having small droplet sizes and high efficiency at low sample introduction rates. The nebulizer has a cylindrical gas permeable active surface. A sleeve is disposed around the cylinder and gas is provided from the sleeve to the interior of the cylinder formed by the active surface. In operation, a liquid is provided to the inside of the gas permeable surface. The gas contacts the wetted surface and forms small bubbles which burst to form an aerosol. Those bubbles which are large are carried by momentum to another part of the cylinder where they are renebulized. This process continues until the entire sample is nebulized into aerosol sized droplets.

  10. Use of Aeronet Aerosol Retrievals to Calculate Clear-Sky Irradiance at the Surface

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AERONET Aerosol Retrievals to Calculate Clear-Sky Irradiance at the Surface G. L. Schuster National Aeronautics and Space Administration Langley Research Center Hampton, Virginia O. Dubovik National Aeronautics and Space Administration Goddard Space Flight Center Laboratory for Terrestrial Physics Greenbelt, Maryland Motivation The worldwide aerosol robotic network (AERONET) of ground-based radiometers was developed (in part) as a satellite validation tool (Holben et al. 1998). These sites

  11. Aerosol Radiative Forcing During Spring-Summer 2002 from Measurements at IAP Scientific Station Near Moscow

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Forcing During Spring-Summer 2002 from Measurements at IAP Scientific Station Near Moscow G. S. Golitsyn, I. A. Gorchakova, and I. I. Mokhov A. M. Obukohov Institute of Atmospheric Physics Russian Academy of Science Moscow, Russia A. N. Rublev Russian Research Center Kurchatov Institute Moscow, Russia Introduction Aerosol Radiative Forcing (ARF) is estimated for spring-summer conditions from measurements during the Cloud-Aerosol-Radiation Experiment in 2002 (ZCAREX-2002) at the Zvenigorod

  12. PHASE II CALDERON PROCESS TO PRODUCE DIRECT REDUCED IRON RESEARCH AND DEVELOPMENT PROJECT

    SciTech Connect (OSTI)

    Albert Calderon

    2005-10-14

    The commercialization path of the Calderon technology for making a feedstock for steelmaking with assistance from DOE initially focused on making coke and work was done which proved that the Calderon technology is capable of making good coke for hard driving blast furnaces. U.S. Steel which participated in such demonstration felt that the Calderon technology would be more meaningful in lowering the costs of making steel by adapting it to the making of iron--thus obviating the need for coke. U.S. Steel and Calderon teamed up to jointly work together to demonstrate that the Calderon technology will produce in a closed system iron units from iron concentrate (ore) and coal competitively by eliminating pelletizing, sintering, coking and blast furnace operation. If such process steps could be eliminated, a huge reduction in polluting emissions and greenhouse gases (including CO{sub 2}) relating to steelmaking would ensue. Such reduction will restructure the steel industry away from the very energy-intensive steelmaking steps currently practiced and drastically reduce costs of making steel. The development of a technology to lower U.S. steelmaking costs and become globally competitive is a priority of major importance. Therefore, the development work which Calderon is conducting presently under this Agreement with the U.S. Department of Energy becomes more crucial than ever. During the 3rd quarter of 2005 which the present report covers, virtually all the effort to advance the Calderon technology to make iron units was concentrated towards forming a team with a steelmaker who needs both iron units in the form of hot metal and a substitute for natural gas (SNG), both being major contributors to higher costs in steelmaking. Calderon felt that a very good candidate would be Steel Dynamics (SDI) by virtue that it operates a rotary hearth facility in Butler, Indiana that uses large amounts of natural gas to reduce briquettes made from ore and coal that they subsequently melt in a submerged arc furnace that is a large consumer of electric power. This facility is operated as a division of SDI under the name of Iron Dynamics (IDI). It is no secret that IDI has had and still has a great number of operational problems, including high cost for natural gas.

  13. Research on Anaerobic Digestion: Optimization and Scalability of Mixed High-strength Food Processing Wastes for Renewable Biogas Energy

    SciTech Connect (OSTI)

    Yu, Zhongtang; Hitzhusen, Fredrick

    2012-12-27

    This research project developed and improved anaerobic digestion technologies, created a comprehensive Inventory of Ohio Biomass and a database of microorganisms of anaerobic digesters, and advanced knowledge and understanding of the underpinning microbiology of the anaerobic digestion process. The results and finding of this research project may be useful for future development and implementation of anaerobic digesters, especially at livestock farms. Policy makers and investors may also find the information on the biomass availability in Ohio and valuation of energy projects useful in policy making and making of investment decisions. The public may benefit from the information on biogas as an energy source and the potential impact of anaerobic digester projects on their neighborhoods.

  14. Aerosol Extinction Profiles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    (Technical Report) | SciTech Connect Aerogel-Based Insulation for High-Temperature Industrial Processes Citation Details In-Document Search Title: Aerogel-Based Insulation for High-Temperature Industrial Processes Under this program, Aspen Aerogels has developed an industrial insulation called Pyrogel HT, which is 4-5 times more thermally efficient than current non-aerogel technology. Derived from nanoporous silica aerogels, Pyrogel HT was specifically developed to address a high temperature

  15. Organization by Gordon Research Conferences of the 2012 Plasma Processing Science Conference 22-27 July 2012

    SciTech Connect (OSTI)

    Jane Chang

    2012-07-27

    The 2012 Gordon Research Conference on Plasma Processing Science will feature a comprehensive program that will highlight the most cutting edge scientific advances in plasma science and technology as well as explore the applications of this nonequilibrium medium in possible approaches relative to many grand societal challenges. Fundamental science sessions will focus on plasma kinetics and chemistry, plasma surface interactions, and recent trends in plasma generation and multi-phase plasmas. Application sessions will explore the impact of plasma technology in renewable energy, the production of fuels from renewable feedstocks and carbon dioxide neutral solar fuels (from carbon dioxide and water), and plasma-enabled medicine and sterilization.

  16. LESSONS LEARNED IN AEROSOL MONITORING WITH THE RASA

    SciTech Connect (OSTI)

    Forrester, Joel B.; Bowyer, Ted W.; Carty, Fitz; Comes, Laura; Eslinger, Paul W.; Greenwood, Lawrence R.; Haas, Derek A.; Hayes, James C.; Kirkham, Randy R.; Lepel, Elwood A.; Litke, Kevin E.; Miley, Harry S.; Morris, Scott J.; Schrom, Brian T.; Van Davelaar, Peter; Woods, Vincent T.

    2011-09-14

    The Radionuclide Aerosol Sampler/Analyzer (RASA) is an automated aerosol collection and analysis system designed by Pacific Northwest National Laboratory (PNNL) in the 1990's and is deployed in several locations around the world as part of the International Monitoring System (IMS) required under the Comprehensive Nuclear-Test-Ban Treaty (CTBT). The RASA operates unattended, save for regularly scheduled maintenance, iterating samples through a three-step process on a 24-hour interval. In its 15-year history, much has been learned from the operation and maintenance of the RASA that can benefit engineering updates or future aerosol systems. On 11 March 2011, a 9.0 magnitude earthquake and tsunami rocked the eastern coast of Japan, resulting in power loss and cooling failures at the Daiichi nuclear power plants in Fukushima Prefecture. Aerosol collections were conducted with the RASA in Richland, WA. We present a summary of the lessons learned over the history of the RASA, including lessons taken from the Fukushima incident, regarding the RASA IMS stations operated by the United States.

  17. X-ray Vision for Aerosol Scientists: LCLS Snapshots of Soot (Narrated)

    ScienceCinema (OSTI)

    None

    2014-06-03

    This short conceptual animation depicts how scientists can now simultaneously capture fractal morphology (structure), chemical composition and nanoscale imagery of individual aerosol particles in flight. These particles, known as "PM2.5" because they are smaller than 2.5 microns in diameter, affect climate by interacting with sunlight and impact human health by entering the lungs. The single LCLS laser pulses travel to the Atomic, Molecular and Optical Sciences (AMO) laboratory in the Near Experimental Hall. As we zoom in, we see deep inside a simplified aerosol inlet, where the complex fractal structure of the soot particles, each one completely unique, is shown. Individual soot particles are then delivered into the pulses of the LCLS beam, which destroys them. X-rays are scattered to the detector before the particle is destroyed, giving information about the morphology of the particle. Ion fragments released in the explosion are sent into a mass spectrometer, which measures their mass-to-charge ratio -- giving scientists information about the chemical composition of the particle. Many different particles are analyzed in this manner, allowing scientists to probe variations in the particles due to changes in their environment before being sent through the aerosol inlet. The final visual of aerosols emitted from a factory is representative of the goal that such LCLS aerosol dynamics experiments can provide critical feedback into modeling and understanding combustion, aerosol processes in manufacturing or aerosol effects on climate change.

  18. Residence times of fine tropospheric aerosols as determined by {sup 210}Pb progeny.

    SciTech Connect (OSTI)

    Marley, N. A.; Gaffney, J. S.; Drayton, P. J.; Cunningham, M. M.; Mielcarek, C.; Ravelo, R.; Wagner, C.

    1999-10-05

    Fine tropospheric aerosols can play important roles in the radiative balance of the atmosphere. The fine aerosols can act directly to cool the atmosphere by scattering incoming solar radiation, as well as indirectly by serving as cloud condensation nuclei. Fine aerosols, particularly carbonaceous soots, can also warm the atmosphere by absorbing incoming solar radiation. In addition, aerosols smaller than 2.5 {micro}m have recently been implicated in the health effects of air pollution. Aerosol-active radioisotopes are ideal tracers for the study of atmospheric transport processes. The source terms of these radioisotopes are relatively well known, and they are removed from the atmosphere only by radioactive decay or by wet or dry deposition of the host aerosol. The progeny of the primordial radionuclide {sup 238}U are of particular importance to atmospheric studies. Uranium-238 is common throughout Earth's crust and decays to the inert gas {sup 222}Rn, which escapes into the atmosphere. Radon-222 decays by the series of alpha and beta emissions shown in Figure 1 to the long-lived {sup 210}Pb. Once formed, {sup 210}Pb becomes attached to aerosol particles with average attachment times of 40 s to 3 min.

  19. REVISED FINAL REPORT – INDEPENDENT VERIFICATION SURVEY ACTIVITIES AT THE SEPARATIONS PROCESS RESEARCH UNIT SITES, NISKAYUNA, NEW YORK – DCN 0496-SR-06-1

    SciTech Connect (OSTI)

    Evan Harpenau

    2011-10-10

    The Separations Process Research Unit (SPRU) complex located on the Knolls Atomic Power Laboratory (KAPL) site in Niskayuna, New York, was constructed in the late 1940s to research the chemical separation of plutonium and uranium (Figure A-1). SPRU operated as a laboratory scale research facility between February 1950 and October 1953. The research activities ceased following the successful development of the reduction oxidation and plutonium/uranium extraction processes. The oxidation and extraction processes were subsequently developed for large scale use by the Hanford and Savannah River sites (aRc 2008a). Decommissioning of the SPRU facilities began in October 1953 and continued through the 1990s.

  20. Caused? A Monsoon Example: India Ganges Valley Aerosol Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    issue: What is a Monsoon? How are Monsoons Caused? A Monsoon Example: India Ganges Valley Aerosol Experiment Definitions Activity About ARM: The Atmospheric Radiation Measurement (ARM) Climate Research Facility is a U.S. Department of Energy scientific user facility for the study of global climate change. As part of its outreach program, ARM provides education resources for students, teachers, and communities. www.arm.gov EDUCATION NEWS Monsoons: Bring on the Rain Imagine weeks of hot, dry heat,

  1. ARM Climate Research Facility Annual Report 2005

    SciTech Connect (OSTI)

    J. Voyles

    2005-12-31

    Through the ARM Program, the DOE funded the development of several highly instrumented ground stations for studying cloud formation processes and their influence on radiative transfer, and for measuring other parameters that determine the radiative properties of the atmosphere. This scientific infrastructure, and resultant data archive, is a valuable national and international asset for advancing scientific knowledge of Earth systems. In fiscal year (FY) 2003, the DOE designated ARM sites as a national scientific user facility: the ARM Climate Research (ACRF). The ACRF has enormous potential to contribute to a wide range interdisciplinary science in areas such as meteorology, atmospheric aerosols, hydrology, biogeochemical cycling, and satellite validation, to name only a few.

  2. Application of electrolytic in-process dressing for high-efficiency grinding of ceramic parts. Research activities 1995--96

    SciTech Connect (OSTI)

    Bandyopadhyay, B.P.

    1997-02-01

    The application of Electrolytic In-Process Dressing (ELID) for highly efficient and stable grinding of ceramic parts is discussed. This research was performed at the Institute of Physical and Chemical Research (RIKEN), Tokyo, Japan, June 1995 through August 1995. Experiments were conducted using a vertical machining center. The silicon nitride work material, of Japanese manufacture and supplied in the form of a rectangular block, was clamped to a vice which was firmly fixed on the base of a strain gage dynamometer. The dynamometer was clamped on the machining center table. Reciprocating grinding was performed with a flat-faced diamond grinding wheel. The output from the dynamometer was recorded with a data acquisition system and the normal component of the force was monitored. Experiments were carried out under various cutting conditions, different ELID conditions, and various grinding wheel bonds types. Rough grinding wheels of grit sizes {number_sign}170 and {number_sign}140 were used in the experiments. Compared to conventional grinding, there was a significant reduction in grinding force with ELID grinding. Therefore, ELID grinding can be recommended for high material removal rate grinding, low rigidity machines, and low rigidity workpieces. Compared to normal grinding, a reduction in grinding ratio was observed when ELID grinding was performed. A negative aspect of the process, this reduced G-ratio derives from bond erosion and can be improved somewhat by adjustments in the ELID current. The results of this investigation are discussed in detail in this report.

  3. Atmospheric Radiation Measurement (ARM) Data from Point Reyes, California for the Marine Stratus, Radiation, Aerosol, and Drizzle (MASRAD) Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Point Reyes National Seashore, on the California coast north of San Francisco, was the location of the first deployment of the DOE's Atmospheric Radiation Measurement (ARM) Mobile Facility (AMF). The ARM Program collaborated with the U.S. Office of Naval Research and DOE's Aerosol Science Program in the Marine Stratus, Radiation, Aerosol, and Drizzle (MASRAD) project. Their objectives were to collect data from cloud/aerosol interactions and to improve understanding of cloud organization that is often associated with patches of drizzle. Between March and September 2005, the AMF and at least two research aircraft were used to collect data.

  4. ARM - Surface Aerosol Observing System

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    FacilitiesSurface Aerosol Observing System AMF Information Science Architecture Baseline Instruments AMF1 AMF2 AMF3 MAOS Data Operations AMF Fact Sheet Images Contacts AMF Deployments McMurdo Station, Antarctica, 2015-2016 Pearl Harbor, Hawaii, to San Francisco, California, 2015 Hyytiälä, Finland, 2014 Manacapuru, Brazil, 2014 Oliktok Point, Alaska, 2013 Los Angeles, California, to Honolulu, Hawaii, 2012 Cape Cod, Massachusetts, 2012 Gan Island, Maldives, 2011 Ganges Valley, India, 2011

  5. ARM Aerosol Working Group Meeting

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    and MFRSR Measurements ARM STM 2008 Norfolk, VA Connor Flynn 1 , Annette Koontz 1 , Anne Jefferson 2 , Jim Barnard 1 , Sally McFarlane 1 1 Pacific Northwest National Laboratory 2 CIRES, University of Colorado, Boulder Progress towards ARM DOE 2008 Performance Metric 3 & 4 * Produce and make available new continuous time series of aerosol total column depth, based on results from the AMF deployment in Niger, Africa. * Produce and make available new continuous time series of retrieved dust

  6. Two-Column Aerosol Project (TCAP): Ground-Based Radiation and Aerosol

    Office of Scientific and Technical Information (OSTI)

    Validation Using the NOAA Mobile SURFRAD Station Field Campaign Report (Technical Report) | SciTech Connect SciTech Connect Search Results Technical Report: Two-Column Aerosol Project (TCAP): Ground-Based Radiation and Aerosol Validation Using the NOAA Mobile SURFRAD Station Field Campaign Report Citation Details In-Document Search Title: Two-Column Aerosol Project (TCAP): Ground-Based Radiation and Aerosol Validation Using the NOAA Mobile SURFRAD Station Field Campaign Report The National

  7. Overview of the 2010 Carbonaceous Aerosols and Radiative Effects Study (CARES)

    SciTech Connect (OSTI)

    Zaveri, Rahul A.; Shaw, William J.; Cziczo, D. J.; Schmid, Beat; Ferrare, R.; Alexander, M. L.; Alexandrov, Mikhail; Alvarez, R. J.; Arnott, W. P.; Atkinson, D.; Baidar, Sunil; Banta, Robert M.; Barnard, James C.; Beranek, Josef; Berg, Larry K.; Brechtel, Fred J.; Brewer, W. A.; Cahill, John F.; Cairns, Brian; Cappa, Christopher D.; Chand, Duli; China, Swarup; Comstock, Jennifer M.; Dubey, Manvendra K.; Easter, Richard C.; Erickson, Matthew H.; Fast, Jerome D.; Floerchinger, Cody; Flowers, B. A.; Fortner, Edward; Gaffney, Jeffrey S.; Gilles, Mary K.; Gorkowski, K.; Gustafson, William I.; Gyawali, Madhu S.; Hair, John; Hardesty, Michael; Harworth, J. W.; Herndon, Scott C.; Hiranuma, Naruki; Hostetler, Chris A.; Hubbe, John M.; Jayne, J. T.; Jeong, H.; Jobson, Bertram T.; Kassianov, Evgueni I.; Kleinman, L. I.; Kluzek, Celine D.; Knighton, B.; Kolesar, K. R.; Kuang, Chongai; Kubatova, A.; Langford, A. O.; Laskin, Alexander; Laulainen, Nels S.; Marchbanks, R. D.; Mazzoleni, Claudio; Mei, F.; Moffet, Ryan C.; Nelson, Danny A.; Obland, Michael; Oetjen, Hilke; Onasch, Timothy B.; Ortega, Ivan; Ottaviani, M.; Pekour, Mikhail S.; Prather, Kimberly A.; Radney, J. G.; Rogers, Ray; Sandberg, S. P.; Sedlacek, Art; Senff, Christoph; Senum, Gunar; Setyan, Ari; Shilling, John E.; Shrivastava, ManishKumar B.; Song, Chen; Springston, S. R.; Subramanian, R.; Suski, Kaitlyn; Tomlinson, Jason M.; Volkamer, Rainer M.; Wallace, Hoyt A.; Wang, J.; Weickmann, A. M.; Worsnop, Douglas R.; Yu, Xiao-Ying; Zelenyuk, Alla; Zhang, Qi

    2012-08-22

    Substantial uncertainties still exist in the scientific understanding of the possible interactions between urban and natural (biogenic) emissions in the production and transformation of atmospheric aerosol and the resulting impact on climate change. The U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) program's Carbonaceous Aerosol and Radiative Effects Study (CARES) carried out in June 2010 in Central Valley, California, was a comprehensive effort designed to improve this understanding. The primary objective of the field study was to investigate the evolution of secondary organic and black carbon aerosols and their climate-related properties in the Sacramento urban plume as it was routinely transported into the forested Sierra Nevada foothills area. Urban aerosols and trace gases experienced significant physical and chemical transformations as they mixed with the reactive biogenic hydrocarbons emitted from the forest. Two heavily-instrumented ground sites - one within the Sacramento urban area and another about 40 km to the northeast in the foothills area - were set up to characterize the evolution of meteorological variables, trace gases, aerosol precursors, aerosol size, composition, and climate-related properties in freshly polluted and 'aged' urban air. On selected days, the DOE G-1 aircraft was deployed to make similar measurements upwind and across the evolving Sacramento plume in the morning and again in the afternoon. The NASA B-200 aircraft, carrying remote sensing instruments, was also deployed to characterize the vertical and horizontal distribution of aerosols and aerosol optical properties within and around the plume. This overview provides: a) the scientific background and motivation for the study, b) the operational and logistical information pertinent to the execution of the study, c) an overview of key observations and initial results from the aircraft and ground-based sampling platforms, and d) a roadmap of planned data analyses and focused modeling efforts that will facilitate the integration of new knowledge into improved representations of key aerosol processes in climate models.

  8. The LANL Cloud-Aerosol Model

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The K-25 Story The K-25 Story Addthis Description The K-25 Story

    The LANL Cloud-Aerosol Model Reisner, Jon Los Alamos National Laboratory Category: Modeling Additional Authors: Dubey Manvendra, Chris Jeffery, Miroslaw Andrejczuk, and Dave Moulton A cloud-aerosol modeling framework is being developed at Los Alamos National Laboratory that incorporates two unique aspects in its formulation. First, the model employs a nonlinear solver that requires cloud-aerosol parameterizations be smooth or

  9. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused

  10. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused

  11. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused

  12. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Composition and Reactions of Atmospheric Aerosol Particles Print Wednesday, 29 June 2005 00:00 Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the

  13. Aerosol Oxidation Speeds Up in Smoggy Air

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Oxidation Speeds Up in Smoggy Air Print Organic aerosols (nanometer-sized liquid or solid particles suspended in air) are important constituents of the troposphere, and their chemistry has large-scale impacts on climate, pollution, and health. Accurate predictions of these aerosol impacts require a robust microphysical understanding of all relevant chemical reaction mechanisms and time scales, including those involving highly reactive free-radical molecules. However, detailed modeling is

  14. Aerosol Oxidation Speeds Up in Smoggy Air

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Oxidation Speeds Up in Smoggy Air Print Organic aerosols (nanometer-sized liquid or solid particles suspended in air) are important constituents of the troposphere, and their chemistry has large-scale impacts on climate, pollution, and health. Accurate predictions of these aerosol impacts require a robust microphysical understanding of all relevant chemical reaction mechanisms and time scales, including those involving highly reactive free-radical molecules. However, detailed modeling is

  15. Aerosol Oxidation Speeds Up in Smoggy Air

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosol Oxidation Speeds Up in Smoggy Air Print Organic aerosols (nanometer-sized liquid or solid particles suspended in air) are important constituents of the troposphere, and their chemistry has large-scale impacts on climate, pollution, and health. Accurate predictions of these aerosol impacts require a robust microphysical understanding of all relevant chemical reaction mechanisms and time scales, including those involving highly reactive free-radical molecules. However, detailed modeling is

  16. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused

  17. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused

  18. Unintended consequences of atmospheric injection of sulphate aerosols.

    SciTech Connect (OSTI)

    Brady, Patrick Vane; Kobos, Peter Holmes; Goldstein, Barry

    2010-10-01

    Most climate scientists believe that climate geoengineering is best considered as a potential complement to the mitigation of CO{sub 2} emissions, rather than as an alternative to it. Strong mitigation could achieve the equivalent of up to -4Wm{sup -2} radiative forcing on the century timescale, relative to a worst case scenario for rising CO{sub 2}. However, to tackle the remaining 3Wm{sup -2}, which are likely even in a best case scenario of strongly mitigated CO{sub 2} releases, a number of geoengineering options show promise. Injecting stratospheric aerosols is one of the least expensive and, potentially, most effective approaches and for that reason an examination of the possible unintended consequences of the implementation of atmospheric injections of sulphate aerosols was made. Chief among these are: reductions in rainfall, slowing of atmospheric ozone rebound, and differential changes in weather patterns. At the same time, there will be an increase in plant productivity. Lastly, because atmospheric sulphate injection would not mitigate ocean acidification, another side effect of fossil fuel burning, it would provide only a partial solution. Future research should aim at ameliorating the possible negative unintended consequences of atmospheric injections of sulphate injection. This might include modeling the optimum rate and particle type and size of aerosol injection, as well as the latitudinal, longitudinal and altitude of injection sites, to balance radiative forcing to decrease negative regional impacts. Similarly, future research might include modeling the optimum rate of decrease and location of injection sites to be closed to reduce or slow rapid warming upon aerosol injection cessation. A fruitful area for future research might be system modeling to enhance the possible positive increases in agricultural productivity. All such modeling must be supported by data collection and laboratory and field testing to enable iterative modeling to increase the accuracy and precision of the models, while reducing epistemic uncertainties.

  19. Aerosol Properties Downwind of Biomass Burns Field Campaign Report

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    6 Aerosol Properties Downwind of Biomass Burns Field Campaign Report April 2016 PR Buseck DISCLAIMER This report was prepared as an account of work sponsored by the U.S. Government. Neither the United States nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not

  20. Aerosol Observing System Greenhouse Gas (AOS GHG) Handbook

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    5 Aerosol Observing System Greenhouse Gas (AOS GHG) Monitor Handbook SC Biraud K Reichl March 2016 DISCLAIMER This report was prepared as an account of work sponsored by the U.S. Government. Neither the United States nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would

  1. Potential Aerosol Indirect Effects on Atmospheric Circulation...

    Office of Scientific and Technical Information (OSTI)

    We further elucidated how aerosols change convective intensity, diabatic heating, and regional circulation under different environmental conditions and concluded that wind shear ...

  2. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    refine the computer models used to predict climate change. Tiny Specks with Large Effects Most people equate aerosols with hairspray and household cleaning products, but a...

  3. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused particle growth while...

  4. ARM: Ultrahigh Sensitivity Aerosol Spectrometer (Dataset) | Data...

    Office of Scientific and Technical Information (OSTI)

    Ultrahigh Sensitivity Aerosol Spectrometer Authors: Cynthia Salwen ; Derek Hageman ; Bill Behrens ; Scott Smith ; Janek Uin ; Janek Uin ; Cynthia Salwen ; Annette Koontz ; Annette ...

  5. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    results will help climate scientists refine the computer models used to predict climate change. Tiny Specks with Large Effects Most people equate aerosols with hairspray and...

  6. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    will help climate scientists refine the computer models used to predict climate change. Tiny Specks with Large Effects Most people equate aerosols with hairspray and...

  7. Aerosol indirect effects - general circulation model intercomparison...

    Office of Scientific and Technical Information (OSTI)

    We compute statistical relationships between aerosol optical depth (a) and various cloud ... Nevertheless, the strengths of the statistical relationships are good predictors for the ...

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Using ARM Cloud Data to Evaluate the Effect of a Land Surface on Clouds Download a printable PDF Submitter: GSFC, N., NASA GSFC Area of Research: Cloud Distributions/Characterizations Working Group(s): Aerosol, Cloud Modeling Journal Reference: Zeng, X., W.-K. Tao, M. Zhang, C. Peters-Lidard, S. Lang, J. Simpson, S. Kumar, S. Xie, J. L. Eastman, C.-L. Shie, and J. V. Geiger, 2007: Evaluating clouds in long-term cloud-resolving model simulations with observational data. J. Atmos. Sci. (in press).

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Seasonal and Interannual Variability in 13C of Ecosystem Carbon Fluxes from 2002-2009 Submitter: Torn, M. S., Lawrence Berkeley National Laboratory Area of Research: Surface Properties Working Group(s): Aerosol Life Cycle Journal Reference: Torn MS, SC Biraud, CJ Still, WJ Riley, and JA Berry. 2011. "Seasonal and inter-annual variability in δ13C of net ecosystem carbon exchanges from 2002-2009 in the U.S. Southern Great Plains." Tellus, 63(2), 10.1111/j.1600-0889.2010.00519.x. Time

  10. Design characteristics for facilities which process hazardous particulate

    SciTech Connect (OSTI)

    Abeln, S.P.; Creek, K.; Salisbury, S.

    1998-12-01

    Los Alamos National Laboratory is establishing a research and processing capability for beryllium. The unique properties of beryllium, including light weight, rigidity, thermal conductivity, heat capacity, and nuclear properties make it critical to a number of US defense and aerospace programs. Concomitant with the unique engineering properties are the health hazards associated with processing beryllium in a particulate form and the potential for worker inhalation of aerosolized beryllium. Beryllium has the lowest airborne standard for worker protection compared to all other nonradioactive metals by more than an order of magnitude. This paper describes the design characteristics of the new beryllium facility at Los Alamos as they relate to protection of the workforce. Design characteristics to be reviewed include; facility layout, support systems to minimize aerosol exposure and spread, and detailed review of the ventilation system design for general room air cleanliness and extraction of particulate at the source.

  11. Aerosol Resuspension Model for MELCOR for Fusion and Very High Temperature Reactor Applications

    SciTech Connect (OSTI)

    B.J. Merrill

    2011-01-01

    Dust is generated in fusion reactors from plasma erosion of plasma facing components within the reactors vacuum vessel (VV) during reactor operation. This dust collects in cooler regions on interior surfaces of the VV. Because this dust can be radioactive, toxic, and/or chemically reactive, it poses a safety concern, especially if mobilized by the process of resuspension during an accident and then transported as an aerosol though out the reactor confinement building, and possibly released to the environment. A computer code used at the Idaho National Laboratory (INL) to model aerosol transport for safety consequence analysis is the MELCOR code. A primary reason for selecting MELCOR for this application is its aerosol transport capabilities. The INL Fusion Safety Program (FSP) organization has made fusion specific modifications to MELCOR. Recent modifications include the implementation of aerosol resuspension models in MELCOR 1.8.5 for Fusion. This paper presents the resuspension models adopted and the initial benchmarking of these models.

  12. ARM - Field Campaign - Measurement of Aerosols, Radiation and...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    the Southern Ocean Clouds Radiation Transport Aerosol Transport Experimental Study (SOCRATES) has been proposed to improve our understanding of clouds, aerosols, air-sea...

  13. Natural Aerosols Explain Seasonal and Spatial Patterns of Southern...

    Office of Scientific and Technical Information (OSTI)

    that modeled natural aerosols, principally marine biogenic primary and secondary aerosol sources, explain more than half of the spatiotemporal variability in satellite-observed Nd. ...

  14. ARM: 10-minute TEMPORARY Raman Lidar: aerosol extinction profiles...

    Office of Scientific and Technical Information (OSTI)

    extinction profiles and aerosol optical thickness, from first Ferrare algorithm Citation Details In-Document Search Title: ARM: 10-minute TEMPORARY Raman Lidar: aerosol extinction ...

  15. Aerosol Retrievals from ARM SGP MFRSR Data (Dataset) | Data Explorer

    Office of Scientific and Technical Information (OSTI)

    Aerosol Retrievals from ARM SGP MFRSR Data Title: Aerosol Retrievals from ARM SGP MFRSR Data The Multi-Filter Rotating Shadowband Radiometer (MFRSR) makes precise simultaneous ...

  16. Long-term measurements of submicrometer aerosol chemistry at...

    Office of Scientific and Technical Information (OSTI)

    Great Plains (SGP) using an Aerosol Chemical Speciation Monitor (ACSM) Citation ... Great Plains (SGP) using an Aerosol Chemical Speciation Monitor (ACSM) In this study ...

  17. ARM - Field Campaign - Aerosol and Cloud Experiments in the Eastern...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    horizontal variabilities of aerosol, trace gases, cloud, drizzle, and atmospheric thermodynamics are critically needed for understanding and quantifying the budget of MBL aerosol,...

  18. ARM - Field Campaign - Carbonaceous Aerosol and Radiative Effects...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsCarbonaceous Aerosol and Radiative Effects Study (CARES) Campaign Links CARES Website ARM Data Discovery Browse Data Related Campaigns Carbonaceous Aerosol and...

  19. ARM - Field Campaign - Carbonaceous Aerosol and Radiation Effects...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Photo-Acoustic Aerosol Light Absorption and Scattering Campaign Links ARM Data Discovery Browse Data Related Campaigns Carbonaceous Aerosol and Radiative Effects Study (CARES)...

  20. ARM: Aerosol Observing System (AOS): cloud condensation nuclei...

    Office of Scientific and Technical Information (OSTI)

    Title: ARM: Aerosol Observing System (AOS): cloud condensation nuclei data Aerosol Observing System (AOS): cloud condensation nuclei data Authors: Scott Smith ; Cynthia Salwen ; ...

  1. Cloud Condensation Nuclei Activity of Aerosols during GoAmazon...

    Office of Scientific and Technical Information (OSTI)

    microphysical properties of the aerosol." The Observations and Modeling of the Green Ocean Amazon (GoAmazon 201415) study seeks to understand how aerosol and cloud life cycles ...

  2. Aerosol specification in single-column Community Atmosphere Model...

    Office of Scientific and Technical Information (OSTI)

    Aerosol specification in single-column Community Atmosphere Model version 5 Title: Aerosol specification in single-column Community Atmosphere Model version 5 Single-column model ...

  3. Discrimination between thin cirrus and and tropospheric aerosol...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Discrimination between thin cirrus and and tropospheric aerosol using multiple measurements from Darwin ARCS Mitchell, Ross CSIRO Category: Aerosols Thin cirrus cloud occurs...

  4. Efficacy of Aerosol-Cloud Interactions Under Varying Meteorological Conditions: Southern Great Plains Vs. Pt. Reyes

    SciTech Connect (OSTI)

    Dunn, M.; Schwartz, S.; Kim, B.-G.; Miller, M.; Liu, Y.; Min, Q.

    2008-03-10

    Several studies have demonstrated that cloud dynamical processes such as entrainment mixing may be the primary modulator of cloud optical properties in certain situations. For example, entrainment of dry air alters the cloud drop size distribution by enhancing drop evaporation. However, the effect of entrainment mixing and other forms or turbulence is still quite uncertain. Although these factors and aerosol-cloud interactions should be considered together when evaluating the efficacy of aerosol indirect effects, the underlying mechanisms appear to be dependent upon each other. In addition, accounting for them is impossible with the current understanding of aerosol indirect effect. Therefore, careful objective screening and analysis of observations are needed to determine the extent to which mixing related properties affect cloud optical properties, apart from the aerosol first indirect effect. This study addresses the role of aerosol-cloud interactions in the context of varying meteorological conditions based on ARM data obtained at the Southern Great Plains (SGP) site in Oklahoma and at Pt. Reyes, California. Previous analyses of the continental stratiform clouds at the SGP site have shown that the thicker clouds of high liquid water path (LWP) tend to contain sub adiabatic LWPs. These sub adiabatic LWPs, which result from active mixing processes, correspond to a lower susceptibility of the clouds to aerosol-cloud interactions, and, hence, to reduced aerosol indirect effects. In contrast, the consistently steady and thin maritime stratus clouds observed at Pt. Reyes are much closer to adiabatic. These clouds provide an excellent benchmark for the study of the aerosol influence on modified marine clouds relative to continental clouds, since they form in a much more homogeneous meteorological environment than those at the continental site.

  5. Liquid Metal Processing and Casting Experiences at the U.S. Department of Energy's Albany Research Center

    SciTech Connect (OSTI)

    Jablonski, Paul D.; Turner, Paul C.

    2005-09-01

    In this paper we will discuss some of the early pioneering work as well as some of our more recent research. The Albany Research Center (ARC) has been involved with the melting and processing of metals since it was established in 1942. In the early days, hardly anything was known about melting refractory or reactive metals and as such, virtually everything had to be developed in-house. Besides the more common induction heated air-melt furnaces, ARC has built and/or utilized a wide variety of furnaces including vacuum arc remelt ingot and casting furnaces, cold wall induction furnaces, electric arc furnaces, cupola furnaces and reverberatory furnaces. The melt size of these furnaces range from several grams to a ton or more. We have used these furnaces to formulate custom alloys for wrought applications as well as for such casting techniques as spin casting, investment casting and lost foam casting among many. Two early spin-off industrializations were Wah Chang (wrought zirconium alloys for military and commercial nuclear applications) and Oremet (both wrought and cast Ti). Both of these companies are now part of the ATI Allegheny Ludlum Corporation.

  6. Composition of carbonaceous smoke particles from prescribed burning of a Canadian boreal forest: 1. Organic aerosol characterization by gas chromatography

    SciTech Connect (OSTI)

    Mazurek, M.A.; Laterza, C.; Newman, L.; Daum, P.; Cofer, W.R. III; Levine, J.S.; Winstead, E.L.

    1995-06-01

    In this study we examine the molecular organic constituents (C8 to C40 lipid compounds) collected as smoke particles from a Canadian boreal forest prescribed burn. Of special interest are (1) the molecular identity of polar organic aerosols, and (2) the amount of polar organic matter relative to the total mass of aerosol particulate carbon. Organic extracts of smoke aerosol particles show complex distributions of the lipid compounds when analyzed by capillary gas chromatography/mass spectrometry. The molecular constituents present as smoke aerosol are grouped into non-polar (hydrocarbons) and polar {minus}2 oxygen atoms) subtractions. The dominant chemical species found in the boreal forest smoke aerosol are unaltered resin compounds (C20 terpenes) which are abundant in unburned conifer wood, plus thermally altered wood lignins and other polar aromatic hydrocarbons. Our results show that smoke aerosols contain molecular tracers which are related to the biofuel consumed. These smoke tracers can be related structurally back to the consumed softwood and hardwood vegetation. In addition, combustion of boreal forest materials produces smoke aerosol particles that are both oxygen-rich and chemically complex, yielding a carbonaceous aerosol matrix that is enriched in polar substances. As a consequence, emissions of carbonaceous smoke particles from large-scale combustion of boreal forest land may have a disproportionate effect on regional atmospheric chemistry and on cloud microphysical processes.

  7. AEROSOL PARTICLE COLLECTOR DESIGN STUDY

    SciTech Connect (OSTI)

    Lee, S; Richard Dimenna, R

    2007-09-27

    A computational evaluation of a particle collector design was performed to evaluate the behavior of aerosol particles in a fast flowing gas stream. The objective of the work was to improve the collection efficiency of the device while maintaining a minimum specified air throughput, nominal collector size, and minimal power requirements. The impact of a range of parameters was considered subject to constraints on gas flow rate, overall collector dimensions, and power limitations. Potential improvements were identified, some of which have already been implemented. Other more complex changes were identified and are described here for further consideration. In addition, fruitful areas for further study are proposed.

  8. Observations of the first aerosol indirect effect in shallow cumuli

    SciTech Connect (OSTI)

    Berg, Larry K.; Berkowitz, Carl M.; Barnard, James C.; Senum, Gunar; Springston, Stephen R.

    2011-02-08

    Data from the Cumulus Humilis Aerosol Processing Study (CHAPS) are used to estimate the impact of both aerosol indirect effects and cloud dynamics on the microphysical and optical properties of shallow cumuli observed in the vicinity of Oklahoma City, Oklahoma. Not surprisingly, we find that the amount of light scattered by the clouds is dominated by their liquid water content (LWC), which in turn is driven by cloud dynamics. However, removing the effect of cloud dynamics by examining the scattering normalized by LWC shows a strong sensitivity of scattering to pollutant loading. These results suggest that even moderately sized cities, like Oklahoma City, can have a measureable impact on the optical properties of shallow cumuli.

  9. Holistic Interactions of Shallow Clouds, Aerosols, and Land-Ecosystems (HI-SCALE) Science Plan

    SciTech Connect (OSTI)

    Fast, JD; Berg, LK

    2015-12-01

    Cumulus convection is an important component in the atmospheric radiation budget and hydrologic cycle over the Southern Great Plains and over many regions of the world, particularly during the summertime growing season when intense turbulence induced by surface radiation couples the land surface to clouds. Current convective cloud parameterizations contain uncertainties resulting in part from insufficient coincident data that couples cloud macrophysical and microphysical properties to inhomogeneities in boundary layer and aerosol properties. The Holistic Interactions of Shallow Clouds, Aerosols, and Land-Ecosystems (HI-SCALE) campaign is designed to provide a detailed set of measurements that are needed to obtain a more complete understanding of the life cycle of shallow clouds by coupling cloud macrophysical and microphysical properties to land surface properties, ecosystems, and aerosols. HI-SCALE consists of 2, 4-week intensive observational periods, one in the spring and the other in the late summer, to take advantage of different stages and distribution of “greenness” for various types of vegetation in the vicinity of the Atmospheric Radiation and Measurement (ARM) Climate Research Facility’s Southern Great Plains (SGP) site as well as aerosol properties that vary during the growing season. Most of the proposed instrumentation will be deployed on the ARM Aerial Facility (AAF) Gulfstream 1 (G-1) aircraft, including those that measure atmospheric turbulence, cloud water content and drop size distributions, aerosol precursor gases, aerosol chemical composition and size distributions, and cloud condensation nuclei concentrations. Routine ARM aerosol measurements made at the surface will be supplemented with aerosol microphysical properties measurements. The G-1 aircraft will complete transects over the SGP Central Facility at multiple altitudes within the boundary layer, within clouds, and above clouds.

  10. In situ measurements of heterogeneous reactions on ambient aerosol particles: Impacts on atmospheric chemistry and climate

    SciTech Connect (OSTI)

    Bertram, Timothy

    2015-02-11

    Aerosol particles play a critical role in the Earth’s energy budget through the absorption and scattering of radiation, and/or through their ability to form clouds and alter cloud lifetime. Heterogeneous and multi-phase reactions alter the climate-relevant properties of aerosol particles and catalyze reaction pathways that are energetically unfavorable in the gas phase. The chemical composition of aerosol particles dictates the kinetics of heterogeneous and multi-phase reactions. At present, the vast majority of the molecular level information on these processes has been determined in laboratory investigations on model aerosol systems. The work described here provides a comprehensive investigation into the reactivity of complex, ambient aerosol particles is proposed to determine: 1) how representative laboratory investigations of heterogeneous and multi-phase processes conducted on model, simple systems are of the real atmosphere, and 2) the impact of heterogeneous and multi-phase processes on ambient particle optical properties and their ability to nucleate clouds. This work has focused on the uptake kinetics for ammonia (NH3) and dinitrogen pentoxide (N2O5). The results of these investigations will be used to directly improve the representation of heterogeneous and multi-phase processes in global climate models, by identifying the key mechanistic drivers that control the variability in the observed kinetics.

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Submitter: Turner, D. D., National Oceanic and Atmospheric Administration Area of Research: Radiation Processes Working Group(s): Radiative Processes Journal Reference: Turner DD. ...

  12. Global distribution and climate forcing of marine organic aerosol: 1. Model improvements and evaluation

    SciTech Connect (OSTI)

    Meskhidze, N.; Xu, J.; Gantt, Brett; Zhang, Yang; Nenes, Athanasios; Ghan, Steven J.; Liu, Xiaohong; Easter, Richard C.; Zaveri, Rahul A.

    2011-11-23

    Marine organic aerosol emissions have been implemented and evaluated within the National Center of Atmospheric Research (NCAR)'s Community Atmosphere Model (CAM5) with the Pacific Northwest National Laboratory's 7-mode Modal Aerosol Module (MAM-7). Emissions of marine primary organic aerosols (POA), phytoplanktonproduced isoprene- and monoterpenes-derived secondary organic aerosols (SOA) and methane sulfonate (MS{sup -}) are shown to affect surface concentrations of organic aerosols in remote marine regions. Global emissions of submicron marine POA is estimated to be 7.9 and 9.4 Tg yr{sup -1}, for the Gantt et al. (2011) and Vignati et al. (2010) emission parameterizations, respectively. Marine sources of SOA and particulate MS{sup -} (containing both sulfur and carbon atoms) contribute an additional 0.2 and 5.1 Tg yr{sup -1}, respectively. Widespread areas over productive waters of the Northern Atlantic, Northern Pacific, and the Southern Ocean show marine-source submicron organic aerosol surface concentrations of 100 ngm{sup -3}, with values up to 400 ngm{sup -3} over biologically productive areas. Comparison of long-term surface observations of water insoluble organic matter (WIOM) with POA concentrations from the two emission parameterizations shows that despite revealed discrepancies (often more than a factor of 2), both Gantt et al. (2011) and Vignati et al. (2010) formulations are able to capture the magnitude of marine organic aerosol concentrations, with the Gantt et al. (2011) parameterization attaining better seasonality. Model simulations show that the mixing state of the marine POA can impact the surface number concentration of cloud condensation nuclei (CCN). The largest increases (up to 20 %) in CCN (at a supersaturation (S) of 0.2 %) number concentration are obtained over biologically productive ocean waters when marine organic aerosol is assumed to be externally mixed with sea-salt. Assuming marine organics are internally-mixed with sea-salt provides diverse results with increases and decreases in the concentration of CCN over different parts of the ocean. The sign of the CCN change due to the addition of marine organics to seasalt aerosol is determined by the relative significance of the increase in mean modal diameter due to addition of mass, and the decrease in particle hygroscopicity due to compositional changes in marine aerosol. Based on emerging evidence for increased CCN concentration over biologically active surface ocean areas/periods, our study suggests that treatment of sea spray in global climate models (GCMs) as an internal mixture of marine organic aerosols and sea-salt will likely lead to an underestimation in CCN number concentration.

  13. Measurements of Aerosol Charge and Size Distribution for Graphite, Gold, Palladium, and Silver Nanoparticles

    SciTech Connect (OSTI)

    Simones, Matthew P.; Gutti, Veera R.; Meyer, Ryan M.; Loyalka, Sudarshan K.

    2011-11-01

    The role of charge on aerosol evolution and hence the nuclear source term has been an issue of interest, and there is a need for both experimental techniques and modeling for quantifying this role. Our focus here is on further exploration of a tandem differential mobility analyzer (TDMA) technique to simultaneously measure both the size and charge (positive, negative and neutral) dependent aerosol distributions. We have generated graphite, gold, silver, and palladium nanoparticles (aerosol) using a spark generator. We measure the electrical mobility-size distributions for these aerosols using a TDMA, and from these data we deduce the full charge-size distributions. We observe asymmetry in the particle size distributions for negative and positive charges. This asymmetry could have a bearing on the dynamics of charged aerosols, indicating that the assumption of symmetry for size distributions of negatively and positively charged particles in source term simulations may not be always appropriate. Also, the experimental technique should find applications in measurements of aerosol rate processes that are affected by both particle charge and size (e.g. coagulation, deposition, resuspension), and hence in modeling and simulation of the nuclear source term.

  14. Small-Scale Spray Releases: Additional Aerosol Test Results

    SciTech Connect (OSTI)

    Schonewill, Philip P.; Gauglitz, Phillip A.; Kimura, Marcia L.; Brown, G. N.; Mahoney, Lenna A.; Tran, Diana N.; Burns, Carolyn A.; Kurath, Dean E.

    2013-08-01

    One of the events postulated in the hazard analysis at the Waste Treatment and Immobilization Plant (WTP) and other U.S. Department of Energy (DOE) nuclear facilities is a breach in process piping that produces aerosols with droplet sizes in the respirable range. The current approach for predicting the size and concentration of aerosols produced in a spray leak involves extrapolating from correlations reported in the literature. These correlations are based on results obtained from small engineered spray nozzles using pure liquids with Newtonian fluid behavior. The narrow ranges of physical properties on which the correlations are based do not cover the wide range of slurries and viscous materials that will be processed in the WTP and across processing facilities in the DOE complex. To expand the data set upon which the WTP accident and safety analyses were based, an aerosol spray leak testing program was conducted by Pacific Northwest National Laboratory (PNNL). PNNL’s test program addressed two key technical areas to improve the WTP methodology (Larson and Allen 2010). The first technical area was to quantify the role of slurry particles in small breaches where slurry particles may plug the hole and prevent high-pressure sprays. The results from an effort to address this first technical area can be found in Mahoney et al. (2012a). The second technical area was to determine aerosol droplet size distribution and total droplet volume from prototypic breaches and fluids, including sprays from larger breaches and sprays of slurries for which literature data are largely absent. To address the second technical area, the testing program collected aerosol generation data at two scales, commonly referred to as small-scale and large-scale. The small-scale testing and resultant data are described in Mahoney et al. (2012b) and the large-scale testing and resultant data are presented in Schonewill et al. (2012). In tests at both scales, simulants were used to mimic the relevant physical properties projected for actual WTP process streams.

  15. Large-Scale Spray Releases: Additional Aerosol Test Results

    SciTech Connect (OSTI)

    Daniel, Richard C.; Gauglitz, Phillip A.; Burns, Carolyn A.; Fountain, Matthew S.; Shimskey, Rick W.; Billing, Justin M.; Bontha, Jagannadha R.; Kurath, Dean E.; Jenks, Jeromy WJ; MacFarlan, Paul J.; Mahoney, Lenna A.

    2013-08-01

    One of the events postulated in the hazard analysis for the Waste Treatment and Immobilization Plant (WTP) and other U.S. Department of Energy (DOE) nuclear facilities is a breach in process piping that produces aerosols with droplet sizes in the respirable range. The current approach for predicting the size and concentration of aerosols produced in a spray leak event involves extrapolating from correlations reported in the literature. These correlations are based on results obtained from small engineered spray nozzles using pure liquids that behave as a Newtonian fluid. The narrow ranges of physical properties on which the correlations are based do not cover the wide range of slurries and viscous materials that will be processed in the WTP and in processing facilities across the DOE complex. To expand the data set upon which the WTP accident and safety analyses were based, an aerosol spray leak testing program was conducted by Pacific Northwest National Laboratory (PNNL). PNNL’s test program addressed two key technical areas to improve the WTP methodology (Larson and Allen 2010). The first technical area was to quantify the role of slurry particles in small breaches where slurry particles may plug the hole and prevent high-pressure sprays. The results from an effort to address this first technical area can be found in Mahoney et al. (2012a). The second technical area was to determine aerosol droplet size distribution and total droplet volume from prototypic breaches and fluids, including sprays from larger breaches and sprays of slurries for which literature data are mostly absent. To address the second technical area, the testing program collected aerosol generation data at two scales, commonly referred to as small-scale and large-scale testing. The small-scale testing and resultant data are described in Mahoney et al. (2012b), and the large-scale testing and resultant data are presented in Schonewill et al. (2012). In tests at both scales, simulants were used to mimic the relevant physical properties projected for actual WTP process streams.

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Group(s): Aerosol Journal Reference: McComiskey, A, SE Schwartz, B Schmid, H Guan, ER Lewis, P Ricchiazzi, and JA Ogren. 2008. "Direct aerosol forcing: Calculation from...

  17. Final Report, The Influence of Organic-Aerosol Emissions and Aging on Regional and Global Aerosol Size Distributions and the CCN Number Budget

    SciTech Connect (OSTI)

    Donahue, Neil M.

    2015-12-23

    We conducted laboratory experiments and analyzed data on aging of organic aerosol and analysis of field data on volatility and CCN activity. With supplemental ASR funding we participated in the FLAME-IV campaign in Missoula MT in the Fall of 2012, deploying a two-chamber photochemical aging system to enable experimental exploration of photochemical aging of biomass burning emissions. Results from that campaign will lead to numerous publications, including demonstration of photochemical production of Brown Carbon (BrC) from secondary organic aerosol associated with biomass burning emissions as well as extensive characterization of the effect of photochemical aging on the overall concentrations of biomass burning organic aerosol. Excluding publications arising from the FLAME-IV campaign, project research resulted in 8 papers: [11, 5, 3, 10, 12, 4, 8, 7], including on in Nature Geoscience addressing the role of organic compounds in nanoparticle growth [11

  18. INDEPENDENT TECHNICAL ASSESSMENT OF MANAGEMENT OF STORMWATER AND WASTEWATER AT THE SEPARATIONS PROCESS RESEARCH UNIT (SPRU) DISPOSITION PROJECT, NEW YORK

    SciTech Connect (OSTI)

    Abitz, R.; Jackson, D.; Eddy-Dilek, C.

    2011-06-27

    The U.S. Department of Energy (DOE) is currently evaluating the water management procedures at the Separations Process Research Unit (SPRU). The facility has three issues related to water management that require technical assistance: (1) due to a excessive rainfall event in October, 2010, contaminated water collected in basements of G2 and H2 buildings. As a result of this event, the contractor has had to collect and dispose of water offsite; (2) The failure of a sump pump at a KAPL outfall resulted in a Notice of Violation issued by the New York State Department of Environment and Conservation (NYSDEC) and subsequent Consent Order. On-site water now requires treatment and off-site disposition; and (3) stormwater infiltration has resulted in Strontium-90 levels discharged to the storm drains that exceed NR standards. The contractor has indicated that water management at SPRU requires major staff resources (at least 50 persons). The purpose of this review is to determine if the contractor's technical approach warrants the large number of staff resources and to ensure that the technical approach is compliant and in accordance with federal, state and NR requirements.

  19. Aerosol chemical vapor deposition of metal oxide films

    DOE Patents [OSTI]

    Ott, Kevin C.; Kodas, Toivo T.

    1994-01-01

    A process of preparing a film of a multicomponent metal oxide including: forming an aerosol from a solution comprised of a suitable solvent and at least two precursor compounds capable of volatilizing at temperatures lower than the decomposition temperature of said precursor compounds; passing said aerosol in combination with a suitable oxygen-containing carrier gas into a heated zone, said heated zone having a temperature sufficient to evaporate the solvent and volatilize said precursor compounds; and passing said volatilized precursor compounds against the surface of a substrate, said substrate having a sufficient temperature to decompose said volatilized precursor compounds whereby metal atoms contained within said volatilized precursor compounds are deposited as a metal oxide film upon the substrate is disclosed. In addition, a coated article comprising a multicomponent metal oxide film conforming to the surface of a substrate selected from the group consisting of silicon, magnesium oxide, yttrium-stabilized zirconium oxide, sapphire, or lanthanum gallate, said multicomponent metal oxide film characterized as having a substantially uniform thickness upon said FIELD OF THE INVENTION The present invention relates to the field of film coating deposition techniques, and more particularly to the deposition of multicomponent metal oxide films by aerosol chemical vapor deposition. This invention is the result of a contract with the Department of Energy (Contract No. W-7405-ENG-36).

  20. CARES: Carbonaceous Aerosol and Radiative Effects Study Science Plan

    SciTech Connect (OSTI)

    Zaveri, RA; Shaw, WJ; Cziczo, DJ

    2010-05-27

    Carbonaceous aerosol components, which include black carbon (BC), urban primary organic aerosols (POA), biomass burning aerosols, and secondary organic aerosols (SOA) from both urban and biogenic precursors, have been previously shown to play a major role in the direct and indirect radiative forcing of climate. The primary objective of the CARES 2010 intensive field study is to investigate the evolution of carbonaceous aerosols of different types and their effects on optical and cloud formation properties.

  1. ARM - Field Campaign - 2006 MAX-Mex-Megacity Aerosol eXperiment...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    characterization of the aerosols, on aerosol transformations including aging of the black carbon during outflow from the region, and on the effects of the megacity aerosol plume on...

  2. ARM - Research Support for International Polar Year (IPY)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Polar YearResearch Support for International Polar Year (IPY) Research Support International Polar Year Begins at ACRF with 3-week Campaign in Barrow Aerosol Affects on Clouds To...

  3. Evaluating Global Aerosol Models and Aerosol and Water Vapor Properties Near Clouds

    SciTech Connect (OSTI)

    Richard A. Ferrare; David D. Turner

    2011-09-01

    Project goals: (1) Use the routine surface and airborne measurements at the ARM SGP site, and the routine surface measurements at the NSA site, to continue our evaluations of model aerosol simulations; (2) Determine the degree to which the Raman lidar measurements of water vapor and aerosol scattering and extinction can be used to remotely characterize the aerosol humidification factor; (3) Use the high temporal resolution CARL data to examine how aerosol properties vary near clouds; and (4) Use the high temporal resolution CARL and Atmospheric Emitted Radiance Interferometer (AERI) data to quantify entrainment in optically thin continental cumulus clouds.

  4. ARM - Evaluation Product - Aerosol Modeling Testbed

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    and satellite aerosol optical depth data is included to supplement and enhance the value of the CARES data. The software that is provided in AMT extracts model output from...

  5. Long-Term Measurements of Submicrometer Aerosol

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    non-refractory submicron particulate matter (NR-PM1) including organic aerosol (OA), sulfate (SO 4 2- ), nitrate (NO 3 - ), ammonium (NH 4 + ), and chloride (Cl-). In this study,...

  6. ARM - Field Campaign - Aerosol Lidar Validation Experiment -...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsAerosol Lidar Validation Experiment - ALIVE Campaign Links ALIVE Website ARM Data Discovery Browse Data Comments? We would love to hear from you Send us a note below...

  7. ARM - Field Campaign - MASRAD: Marine Aerosol Properties

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsMASRAD: Marine Aerosol Properties Campaign Links AMF Point Reyes Website Comments? We would love to hear from you Send us a note below or call us at 1-888-ARM-DATA....

  8. Lidar techniques for chemical and aerosol air pollution studies

    SciTech Connect (OSTI)

    Hardesty, R.M.

    1993-12-31

    At the Wave Propagation Laboratory (WPL), lidar methods are being applied in several areas of air pollution research. Differential absorption lidar (DIAL) systems for measuring ozone, ethylene, and other pollutants have been recently developed. The ozone instrument profiles ozone concentration in the boundary layer and lower troposphere to study sources, sinks, and transport of ozone. A goal is to combine DIAL and Doppler lidar techniques for measurement of the vertical fluxes of ozone and other pollutants. Doppler lidars have been also used at WPL to study visibility reduction caused by aerosol pollutants at the Grand Canyon, and to investigate dispersion of hazardous emissions near the Rocky Flats nuclear plant.

  9. Biogenic Aerosols-Effects on Clouds and Climate (BAECC)

    Office of Scientific and Technical Information (OSTI)

    51 Biogenic Aerosols-Effects on Clouds and Climate (BAECC) Final Campaign Summary T Petaja D Moisseev V Sinclair E O'Connor A Manninen J Levula R Vaananen L Heikkinen M Aijala J Aalto JA Thornton March 2016 CLIMATE RESEARCH FACILITY DISCLAIMER This report was prepared as an account of work sponsored by the U.S. Government. Neither the United States nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the

  10. Aerosol remote sensing in polar regions

    SciTech Connect (OSTI)

    Tomasi, Claudio; Kokhanovsky, Alexander A.; Lupi, Angelo; Ritter, Christoph; Smirnov, Alexander; O'Neill, Norman T.; Stone, Robert S.; Holben, Brent N.; Nyeki, Stephan; Mazzola, Mauro; Lanconelli, Christian; Vitale, Vito; Stebel, Kerstin; Aaltonen, Veijo; de Leeuw, Gerrit; Rodriguez, Edith; Herber, Andreas B.; Radionov, Vladimir F.; Zielinski, Tymon; Petelski, Tomasz; Sakerin, Sergey M.; Kabanov, Dmitry M.; Xue, Yong; Mei, Linlu; Istomina, Larysa; Wagener, Richard; McArthur, Bruce; Sobolewski, Piotr S.; Kivi, Rigel; Courcoux, Yann; Larouche, Pierre; Broccardo, Stephen; Piketh, Stuart J.

    2015-01-01

    Multi-year sets of ground-based sun-photometer measurements conducted at 12 Arctic sites and 9 Antarctic sites were examined to determine daily mean values of aerosol optical thickness ?(?) at visible and near-infrared wavelengths, from which best-fit values of ngstrm's exponent ? were calculated. Analysing these data, the monthly mean values of ?(0.50 ?m) and ? and the relative frequency histograms of the daily mean values of both parameters were determined for winterspring and summerautumn in the Arctic and for austral summer in Antarctica. The Arctic and Antarctic covariance plots of the seasonal median values of ? versus ?(0.50 ?m) showed: (i) a considerable increase in ?(0.50 ?m) for the Arctic aerosol from summer to winterspring, without marked changes in ?; and (ii) a marked increase in ?(0.50 ?m) passing from the Antarctic Plateau to coastal sites, whereas ? decreased considerably due to the larger fraction of sea-salt aerosol. Good agreement was found when comparing ground-based sun-photometer measurements of ?(?) and ? at Arctic and Antarctic coastal sites with Microtops measurements conducted during numerous AERONET/MAN cruises from 2006 to 2013 in three Arctic Ocean sectors and in coastal and off-shore regions of the Southern Atlantic, Pacific, and Indian Oceans, and the Antarctic Peninsula. Lidar measurements were also examined to characterise vertical profiles of the aerosol backscattering coefficient measured throughout the year at Ny-lesund. Satellite-based MODIS, MISR, and AATSR retrievals of ?(?) over large parts of the oceanic polar regions during spring and summer were in close agreement with ship-borne and coastal ground-based sun-photometer measurements. An overview of the chemical composition of mode particles is also presented, based on in-situ measurements at Arctic and Antarctic sites. Fourteen log-normal aerosol number size-distributions were defined to represent the average features of nuclei, accumulation and coarse mode particles for Arctic haze, summer background aerosol, Asian dust and boreal forest fire smoke, and for various background austral summer aerosol types at coastal and high-altitude Antarctic sites. The main columnar aerosol optical characteristics were determined for all 14 particle modes, based on in-situ measurements of the scattering and absorption coefficients. Diurnally averaged direct aerosol-induced radiative forcing and efficiency were calculated for a set of multimodal aerosol extinction models, using various Bidirectional Reflectance Distribution Function models over vegetation-covered, oceanic and snow-covered surfaces. These gave a reliable measure of the pronounced effects of aerosols on the radiation balance of the surfaceatmosphere system over polar regions.

  11. Apparatus for sampling and characterizing aerosols

    DOE Patents [OSTI]

    Dunn, P.F.; Herceg, J.E.; Klocksieben, R.H.

    1984-04-11

    Apparatus for sampling and characterizing aerosols having a wide particle size range at relatively low velocities may comprise a chamber having an inlet and an outlet, the chamber including: a plurality of vertically stacked, successive particle collection stages; each collection stage includes a separator plate and a channel guide mounted transverse to the separator plate, defining a labyrinthine flow path across the collection stage. An opening in each separator plate provides a path for the aerosols from one collection stage t

  12. Aerosol fabrication methods for monodisperse nanoparticles

    DOE Patents [OSTI]

    Jiang, Xingmao; Brinker, C Jeffrey

    2014-10-21

    Exemplary embodiments provide materials and methods for forming monodisperse particles. In one embodiment, the monodisperse particles can be formed by first spraying a nanoparticle-containing dispersion into aerosol droplets and then heating the aerosol droplets in the presence of a shell precursor to form core-shell particles. By removing either the shell layer or the nanoparticle core of the core-shell particles, monodisperse nanoparticles can be formed.

  13. Impact of aerosol size representation on modeling aerosol-cloud interactions

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Zhang, Y.; Easter, R. C.; Ghan, S. J.; Abdul-Razzak, H.

    2002-11-07

    In this study, we use a 1-D version of a climate-aerosol-chemistry model with both modal and sectional aerosol size representations to evaluate the impact of aerosol size representation on modeling aerosol-cloud interactions in shallow stratiform clouds observed during the 2nd Aerosol Characterization Experiment. Both the modal (with prognostic aerosol number and mass or prognostic aerosol number, surface area and mass, referred to as the Modal-NM and Modal-NSM) and the sectional approaches (with 12 and 36 sections) predict total number and mass for interstitial and activated particles that are generally within several percent of references from a high resolution 108-section approach.more » The modal approach with prognostic aerosol mass but diagnostic number (referred to as the Modal-M) cannot accurately predict the total particle number and surface areas, with deviations from the references ranging from 7-161%. The particle size distributions are sensitive to size representations, with normalized absolute differences of up to 12% and 37% for the 36- and 12-section approaches, and 30%, 39%, and 179% for the Modal-NSM, Modal-NM, and Modal-M, respectively. For the Modal-NSM and Modal-NM, differences from the references are primarily due to the inherent assumptions and limitations of the modal approach. In particular, they cannot resolve the abrupt size transition between the interstitial and activated aerosol fractions. For the 12- and 36-section approaches, differences are largely due to limitations of the parameterized activation for non-log-normal size distributions, plus the coarse resolution for the 12-section case. Differences are larger both with higher aerosol (i.e., less complete activation) and higher SO2 concentrations (i.e., greater modification of the initial aerosol distribution).« less

  14. WRF-Chem Simulations of Aerosols and Anthropogenic Aerosol Radiative Forcing in East Asia

    SciTech Connect (OSTI)

    Gao, Yi; Zhao, Chun; Liu, Xiaohong; Zhang, Meigen; Leung, Lai-Yung R.

    2014-08-01

    This study aims to provide a first comprehensive evaluation of WRF-Chem for modeling aerosols and anthropogenic aerosol radiative forcing (RF) over East Asia. Several numerical experiments were conducted from November 2007 to December 2008. Comparison between model results and observations shows that the model can generally reproduce the observed spatial distributions of aerosol concentration, aerosol optical depth (AOD) and single scattering albedo (SSA) from measurements at different sites, including the relatively higher aerosol concentration and AOD over East China and the relatively lower AOD over Southeast Asia, Korean, and Japan. The model also depicts the seasonal variation and transport of pollutions over East Asia. Particulate matter of 10 um or less in the aerodynamic diameter (PM10), black carbon (BC), sulfate (SO42-), nitrate (NO3-) and ammonium (NH4+) concentrations are higher in spring than other seasons in Japan due to the pollutant transport from polluted area of East Asia. AOD is high over Southwest and Central China in winter, spring and autumn and over North China in summer while is low over South China in summer due to monsoon precipitation. SSA is lowest in winter and highest in summer. The model also captures the dust events at the Zhangye site in the semi-arid region of China. Anthropogenic aerosol RF is estimated to range from -5 to -20 W m-2 over land and -20 to -40 W m-2 over ocean at the top of atmosphere (TOA), 5 to 30 W m-2 in the atmosphere (ATM) and -15 to -40 W m-2 at the bottom (BOT). The warming effect of anthropogenic aerosol in ATM results from BC aerosol while the negative aerosol RF at TOA is caused by scattering aerosols such as SO4 2-, NO3 - and NH4+. Positive BC RF at TOA compensates 40~50% of the TOA cooling associated with anthropogenic aerosol.

  15. Characterizing Aerosol Distributions and Optical Properties Using the NASA Langley High Spectral Resolution Lidar

    SciTech Connect (OSTI)

    Hostetler, Chris; Ferrare, Richard

    2013-02-14

    The objective of this project was to provide vertically and horizontally resolved data on aerosol optical properties to assess and ultimately improve how models represent these aerosol properties and their impacts on atmospheric radiation. The approach was to deploy the NASA Langley Airborne High Spectral Resolution Lidar (HSRL) and other synergistic remote sensors on DOE Atmospheric Science Research (ASR) sponsored airborne field campaigns and synergistic field campaigns sponsored by other agencies to remotely measure aerosol backscattering, extinction, and optical thickness profiles. Synergistic sensors included a nadir-viewing digital camera for context imagery, and, later in the project, the NASA Goddard Institute for Space Studies (GISS) Research Scanning Polarimeter (RSP). The information from the remote sensing instruments was used to map the horizontal and vertical distribution of aerosol properties and type. The retrieved lidar parameters include profiles of aerosol extinction, backscatter, depolarization, and optical depth. Products produced in subsequent analyses included aerosol mixed layer height, aerosol type, and the partition of aerosol optical depth by type. The lidar products provided vertical context for in situ and remote sensing measurements from other airborne and ground-based platforms employed in the field campaigns and was used to assess the predictions of transport models. Also, the measurements provide a data base for future evaluation of techniques to combine active (lidar) and passive (polarimeter) measurements in advanced retrieval schemes to remotely characterize aerosol microphysical properties. The project was initiated as a 3-year project starting 1 January 2005. It was later awarded continuation funding for another 3 years (i.e., through 31 December 2010) followed by a 1-year no-cost extension (through 31 December 2011). This project supported logistical and flight costs of the NASA sensors on a dedicated aircraft, the subsequent analysis and archival of the data, and the presentation of results in conferences, workshops, and publications. DOE ASR field campaigns supported under this project included - MAX-Mex /MILAGRO (2006) - TexAQS 2006/GoMACCS (2006) - CHAPS (2007) - RACORO (2009) - CARE/CalNex (2010) In addition, data acquired on HSRL airborne field campaigns sponsored by other agencies were used extensively to fulfill the science objectives of this project and the data acquired have been made available to other DOE ASR investigators upon request.

  16. The First Aerosol Indirect Effect: Beyond Twomey

    SciTech Connect (OSTI)

    Liu, Y.; Dunn, M.; Daum, P.

    2008-03-10

    The traditional first aerosol indirect effect or the Twomey effect involves several fundamental assumptions. Some of the assumptions (e.g., constant liquid water content) are explicitly stated in studies of the Twomey effect whereas others are only implicitly embedded in the quantitative formulation. This work focuses on examining the implicit assumptions. In particular, we will show that anthropogenic pollution not only increases aerosol loading and droplet concentrations but also alters the relative dispersions of both the aerosol and subsequent droplet size distributions. The indirect effects resulting from the two altered relative dispersions (aerosol dispersion effect and droplet dispersion effect) are likely opposite in sign and proportional in magnitude to the conventional Twomey effect. This result suggests that the outstanding problems of the Twomey effect (i.e., large uncertainty and overestimation reported in literature) may lie with violation of the constant spectral shapes of aerosol and droplet size distributions implicitly assumed in evaluation of the Twomey effect, and therefore, further progress in understanding and quantification of the first aerosol indirect effect demands moving beyond the traditional paradigm originally conceived by Twomey.

  17. Impact of aerosol on mixed-phase stratocumulus during MPACE in a mesoscale

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    model with two-moment microphysics Impact of aerosol on mixed-phase stratocumulus during MPACE in a mesoscale model with two-moment microphysics Morrison, Hugh MMM/ASP National Center for Atmospheric Research Pinto, James University of Colorado Curry, Judith Georgia Institute of Technology Category: Modeling The Penn State/NCAR mesoscale model MM5 is coupled to a new microphysics scheme to examine the impact of aerosol on mixed-phase stratocumulus during the Mixed-Phase Arctic Stratus

  18. Sources and composition of submicron organic mass in marine aerosol particles

    SciTech Connect (OSTI)

    Frossard, Amanda A.; Russell, Lynn M.; Burrows, Susannah M.; Elliott, Scott M.; Bates, Timothy S.; Quinn, Patricia K.

    2014-11-27

    Recent studies have proposed a variety of interpretations of the sources and composition of atmospheric marine aerosol particles (aMA) based on a range of physical and chemical measurements collected during open-ocean research cruises. To investigate the processes that affect marine organic particles, this study uses the characteristic functional group composition (from Fourier transform infrared (FTIR) spectroscopy) of aMAP from five ocean regions to show that: (i) The organic functional group composition of aMAP that can be identified as atmospheric primary marine (ocean-derived) aerosol (aPMA) is 65±12% hydroxyl, 21±9% alkane, 6±6% amine, and 7±8% carboxylic acid functional groups. Contributions from photochemical reactions add carboxylic acid groups (15%-25%), shipping effluent in seawater and ship emissions add additional alkane groups (up to 70%), and coastal emissions mix in alkane and carboxylic acid groups from coastal pollution sources. (ii) The organic composition of aPMA is nearly identical to model generated primary marine aerosol particles (gPMA) from bubbled seawater (55% hydroxyl, 32% alkane, and 13% amine functional groups), indicating that its overall functional group composition is the direct consequence of the organic constituents of the seawater source. (iii) While the seawater organic functional group composition was nearly invariant across all three ocean regions studied, the gPMA alkane group fraction increased with chlorophyll-a concentrations (r = 0.79). gPMA from productive seawater had a larger fraction of alkane functional groups (35%) compared to gPMA from non-productive seawater (16%), likely due to the presence of surfactants in productive seawater that stabilize the bubble film and lead to preferential drainage of the more soluble (lower alkane group fraction) organic components. gPMA has a hydroxyl group absorption peak location characteristic of monosaccharides and disaccharides, where the seawater OM hydroxyl group peak location is closer to that of polysaccharides. This may result from the larger saccharides preferentially remaining in the seawater during gPMA and aPMA production

  19. Sources and composition of submicron organic mass in marine aerosol particles

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Frossard, Amanda A.; Russell, Lynn M.; Burrows, Susannah M.; Elliott, Scott M.; Bates, Timothy S.; Quinn, Patricia K.

    2014-11-27

    Recent studies have proposed a variety of interpretations of the sources and composition of atmospheric marine aerosol particles (aMA) based on a range of physical and chemical measurements collected during open-ocean research cruises. To investigate the processes that affect marine organic particles, this study uses the characteristic functional group composition (from Fourier transform infrared (FTIR) spectroscopy) of aMAP from five ocean regions to show that: (i) The organic functional group composition of aMAP that can be identified as atmospheric primary marine (ocean-derived) aerosol (aPMA) is 65±12% hydroxyl, 21±9% alkane, 6±6% amine, and 7±8% carboxylic acid functional groups. Contributions from photochemicalmore » reactions add carboxylic acid groups (15%-25%), shipping effluent in seawater and ship emissions add additional alkane groups (up to 70%), and coastal emissions mix in alkane and carboxylic acid groups from coastal pollution sources. (ii) The organic composition of aPMA is nearly identical to model generated primary marine aerosol particles (gPMA) from bubbled seawater (55% hydroxyl, 32% alkane, and 13% amine functional groups), indicating that its overall functional group composition is the direct consequence of the organic constituents of the seawater source. (iii) While the seawater organic functional group composition was nearly invariant across all three ocean regions studied, the gPMA alkane group fraction increased with chlorophyll-a concentrations (r = 0.79). gPMA from productive seawater had a larger fraction of alkane functional groups (35%) compared to gPMA from non-productive seawater (16%), likely due to the presence of surfactants in productive seawater that stabilize the bubble film and lead to preferential drainage of the more soluble (lower alkane group fraction) organic components. gPMA has a hydroxyl group absorption peak location characteristic of monosaccharides and disaccharides, where the seawater OM hydroxyl group peak location is closer to that of polysaccharides. This may result from the larger saccharides preferentially remaining in the seawater during gPMA and aPMA production« less

  20. NREL's Cyanobacteria Engineering Shortens Biofuel Production Process, Captures CO2 (Fact Sheet), Highlights in Research & Development, NREL (National Renewable Energy Laboratory)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The flexibility of cyanobacterial metabolism supports direct conversion of carbon dioxide (CO 2 ) to ethylene. Photosynthesis fuels growth in plants and algae, two of the primary components of biomass. Biomass, in turn, can be converted into various fuels and chemicals. NREL researchers have shortened this process by engineering one photosynthetic organism, cyanobacterium, so that it converts CO 2 directly into the target chemical ethylene, bypassing the biomass produc- tion and processing

  1. Joint federal research and development process to meet state and local needs. Part 1. Science and technology and political decision making

    SciTech Connect (OSTI)

    Wise, H F; Smith, L K; Einsweiler, R C; Jensen, D E

    1980-10-01

    This part of the handbook addresses the basic how to do it - how states and local governments can identify complex and cross-cutting issues and develop and manage scientific and technical resources in seeking policy solutions to such issues. The following subjects are discussed: background statement of the issue; the research/decision-making process; defining problems and identifying research components; research and decision-making strategies; how to identify existing knowledge or ongoing research in the area of policy concern; and managing multi-disciplinary research. The fourteen agencies involved in this effort include: US Departments of Energy, Agriculture, Transportation, Housing and Urban Development, Environmental Protection Agency, and National Science Foundation. (PSB)

  2. Investigation of warm-cloud microphysics using a multi-component cloud model: Interactive effects of the aerosol spectrum. Master's thesis

    SciTech Connect (OSTI)

    Zahn, S.G.

    1993-12-01

    Clouds, especially low, warm, boundary-layer clouds, play an important role in regulating the earth's climate due to their significant contribution to the global albedo. The radiative effects of individual clouds are controlled largely by cloud microstructure, which is itself sensitive to the concentration and spectral distribution of the atmospheric aerosol. Increases in aerosol particle concentrations from anthropogenic activity could result in increased cloud albedo and global cloudiness, increasing the amount of reflected solar radiation. However, the effects of increased aerosol particle concentrations could be offset by the presence of giant or ultragiant aerosol particles. A one-dimensional, multi-component microphysical cloud model has been used to demonstrate the effects of aerosol particle spectral variations on the microstructure of warm clouds. Simulations performed with this model demonstrate that the introduction of increased concentrations of giant aerosol particles has a destabilizing effect on the cloud microstructure. Also, it is shown that warm-cloud microphysical processes modify the aerosol particle spectrum, favoring the generation of the largest sized particles via the collision-coalescence process. These simulations provide further evidence that the effect of aerosol particles on cloud microstructure must be addressed when considering global climate forecasts.

  3. A New WRF-Chem Treatment for Studying Regional Scale Impacts of Cloud-Aerosol Interactions in Parameterized Cumuli

    SciTech Connect (OSTI)

    Berg, Larry K.; Shrivastava, ManishKumar B.; Easter, Richard C.; Fast, Jerome D.; Chapman, Elaine G.; Liu, Ying

    2015-01-01

    A new treatment of cloud-aerosol interactions within parameterized shallow and deep convection has been implemented in WRF-Chem that can be used to better understand the aerosol lifecycle over regional to synoptic scales. The modifications to the model to represent cloud-aerosol interactions include treatment of the cloud dropletnumber mixing ratio; key cloud microphysical and macrophysical parameters (including the updraft fractional area, updraft and downdraft mass fluxes, and entrainment) averaged over the population of shallow clouds, or a single deep convective cloud; and vertical transport, activation/resuspension, aqueous chemistry, and wet removal of aerosol and trace gases in warm clouds. Thesechanges have been implemented in both the WRF-Chem chemistry packages as well as the Kain-Fritsch cumulus parameterization that has been modified to better represent shallow convective clouds. Preliminary testing of the modified WRF-Chem has been completed using observations from the Cumulus Humilis Aerosol Processing Study (CHAPS) as well as a high-resolution simulation that does not include parameterized convection. The simulation results are used to investigate the impact of cloud-aerosol interactions on the regional scale transport of black carbon (BC), organic aerosol (OA), and sulfate aerosol. Based on the simulations presented here, changes in the column integrated BC can be as large as -50% when cloud-aerosol interactions are considered (due largely to wet removal), or as large as +35% for sulfate in non-precipitating conditions due to the sulfate production in the parameterized clouds. The modifications to WRF-Chem version 3.2.1 are found to account for changes in the cloud drop number concentration (CDNC) and changes in the chemical composition of cloud-drop residuals in a way that is consistent with observations collected during CHAPS. Efforts are currently underway to port the changes described here to WRF-Chem version 3.5, and it is anticipated that they will be included in a future public release of WRF-Chem.

  4. Large-Scale Spray Releases: Initial Aerosol Test Results

    SciTech Connect (OSTI)

    Schonewill, Philip P.; Gauglitz, Phillip A.; Bontha, Jagannadha R.; Daniel, Richard C.; Kurath, Dean E.; Adkins, Harold E.; Billing, Justin M.; Burns, Carolyn A.; Davis, James M.; Enderlin, Carl W.; Fischer, Christopher M.; Jenks, Jeromy WJ; Lukins, Craig D.; MacFarlan, Paul J.; Shutthanandan, Janani I.; Smith, Dennese M.

    2012-12-01

    One of the events postulated in the hazard analysis at the Waste Treatment and Immobilization Plant (WTP) and other U.S. Department of Energy (DOE) nuclear facilities is a breach in process piping that produces aerosols with droplet sizes in the respirable range. The current approach for predicting the size and concentration of aerosols produced in a spray leak involves extrapolating from correlations reported in the literature. These correlations are based on results obtained from small engineered spray nozzles using pure liquids with Newtonian fluid behavior. The narrow ranges of physical properties on which the correlations are based do not cover the wide range of slurries and viscous materials that will be processed in the WTP and across processing facilities in the DOE complex. Two key technical areas were identified where testing results were needed to improve the technical basis by reducing the uncertainty due to extrapolating existing literature results. The first technical need was to quantify the role of slurry particles in small breaches where the slurry particles may plug and result in substantially reduced, or even negligible, respirable fraction formed by high-pressure sprays. The second technical need was to determine the aerosol droplet size distribution and volume from prototypic breaches and fluids, specifically including sprays from larger breaches with slurries where data from the literature are scarce. To address these technical areas, small- and large-scale test stands were constructed and operated with simulants to determine aerosol release fractions and generation rates from a range of breach sizes and geometries. The properties of the simulants represented the range of properties expected in the WTP process streams and included water, sodium salt solutions, slurries containing boehmite or gibbsite, and a hazardous chemical simulant. The effect of anti-foam agents was assessed with most of the simulants. Orifices included round holes and rectangular slots. The round holes ranged in size from 0.2 to 4.46 mm. The slots ranged from (width × length) 0.3 × 5 to 2.74 × 76.2 mm. Most slots were oriented longitudinally along the pipe, but some were oriented circumferentially. In addition, a limited number of multi-hole test pieces were tested in an attempt to assess the impact of a more complex breach. Much of the testing was conducted at pressures of 200 and 380 psi, but some tests were conducted at 100 psi. Testing the largest postulated breaches was deemed impractical because of the large size of some of the WTP equipment. The purpose of this report is to present the experimental results and analyses for the aerosol measurements obtained in the large-scale test stand. The report includes a description of the simulants used and their properties, equipment and operations, data analysis methodology, and test results. The results of tests investigating the role of slurry particles in plugging of small breaches are reported in Mahoney et al. 2012a. The results of the aerosol measurements in the small-scale test stand are reported in Mahoney et al. (2012b).

  5. Small-Scale Spray Releases: Initial Aerosol Test Results

    SciTech Connect (OSTI)

    Mahoney, Lenna A.; Gauglitz, Phillip A.; Kimura, Marcia L.; Brown, Garrett N.; Kurath, Dean E.; Buchmiller, William C.; Smith, Dennese M.; Blanchard, Jeremy; Song, Chen; Daniel, Richard C.; Wells, Beric E.; Tran, Diana N.; Burns, Carolyn A.

    2012-11-01

    One of the events postulated in the hazard analysis at the Waste Treatment and Immobilization Plant (WTP) and other U.S. Department of Energy (DOE) nuclear facilities is a breach in process piping that produces aerosols with droplet sizes in the respirable range. The current approach for predicting the size and concentration of aerosols produced in a spray leak involves extrapolating from correlations reported in the literature. These correlations are based on results obtained from small engineered spray nozzles using pure liquids with Newtonian fluid behavior. The narrow ranges of physical properties on which the correlations are based do not cover the wide range of slurries and viscous materials that will be processed in the WTP and across processing facilities in the DOE complex. Two key technical areas were identified where testing results were needed to improve the technical basis by reducing the uncertainty due to extrapolating existing literature results. The first technical need was to quantify the role of slurry particles in small breaches where the slurry particles may plug and result in substantially reduced, or even negligible, respirable fraction formed by high-pressure sprays. The second technical need was to determine the aerosol droplet size distribution and volume from prototypic breaches and fluids, specifically including sprays from larger breaches with slurries where data from the literature are scarce. To address these technical areas, small- and large-scale test stands were constructed and operated with simulants to determine aerosol release fractions and generation rates from a range of breach sizes and geometries. The properties of the simulants represented the range of properties expected in the WTP process streams and included water, sodium salt solutions, slurries containing boehmite or gibbsite, and a hazardous chemical simulant. The effect of anti-foam agents was assessed with most of the simulants. Orifices included round holes and rectangular slots. The round holes ranged in size from 0.2 to 4.46 mm. The slots ranged from (width × length) 0.3 × 5 to 2.74 × 76.2 mm. Most slots were oriented longitudinally along the pipe, but some were oriented circumferentially. In addition, a limited number of multi-hole test pieces were tested in an attempt to assess the impact of a more complex breach. Much of the testing was conducted at pressures of 200 and 380 psi, but some tests were conducted at 100 psi. Testing the largest postulated breaches was deemed impractical because of the large size of some of the WTP equipment. This report presents the experimental results and analyses for the aerosol measurements obtained in the small-scale test stand. It includes a description of the simulants used and their properties, equipment and operations, data analysis methodologies, and test results. The results of tests investigating the role of slurry particles in plugging small breaches are reported in Mahoney et al. (2012). The results of the aerosol measurements in the large-scale test stand are reported in Schonewill et al. (2012) along with an analysis of the combined results from both test scales.

  6. Small-Scale Spray Releases: Initial Aerosol Test Results

    SciTech Connect (OSTI)

    Mahoney, Lenna A.; Gauglitz, Phillip A.; Kimura, Marcia L.; Brown, Garrett N.; Kurath, Dean E.; Buchmiller, William C.; Smith, Dennese M.; Blanchard, Jeremy; Song, Chen; Daniel, Richard C.; Wells, Beric E.; Tran, Diana N.; Burns, Carolyn A.

    2013-05-29

    One of the events postulated in the hazard analysis at the Waste Treatment and Immobilization Plant (WTP) and other U.S. Department of Energy (DOE) nuclear facilities is a breach in process piping that produces aerosols with droplet sizes in the respirable range. The current approach for predicting the size and concentration of aerosols produced in a spray leak involves extrapolating from correlations reported in the literature. These correlations are based on results obtained from small engineered spray nozzles using pure liquids with Newtonian fluid behavior. The narrow ranges of physical properties on which the correlations are based do not cover the wide range of slurries and viscous materials that will be processed in the WTP and across processing facilities in the DOE complex. Two key technical areas were identified where testing results were needed to improve the technical basis by reducing the uncertainty due to extrapolating existing literature results. The first technical need was to quantify the role of slurry particles in small breaches where the slurry particles may plug and result in substantially reduced, or even negligible, respirable fraction formed by high-pressure sprays. The second technical need was to determine the aerosol droplet size distribution and volume from prototypic breaches and fluids, specifically including sprays from larger breaches with slurries where data from the literature are scarce. To address these technical areas, small- and large-scale test stands were constructed and operated with simulants to determine aerosol release fractions and net generation rates from a range of breach sizes and geometries. The properties of the simulants represented the range of properties expected in the WTP process streams and included water, sodium salt solutions, slurries containing boehmite or gibbsite, and a hazardous chemical simulant. The effect of antifoam agents was assessed with most of the simulants. Orifices included round holes and rectangular slots. For the combination of both test stands, the round holes ranged in size from 0.2 to 4.46 mm. The slots ranged from (width × length) 0.3 × 5 to 2.74 × 76.2 mm. Most slots were oriented longitudinally along the pipe, but some were oriented circumferentially. In addition, a limited number of multi-hole test pieces were tested in an attempt to assess the impact of a more complex breach. Much of the testing was conducted at pressures of 200 and 380 psi, but some tests were conducted at 100 psi. Testing the largest postulated breaches was deemed impractical because of the much larger flow rates and equipment that would be required. This report presents the experimental results and analyses for the aerosol measurements obtained in the small-scale test stand. It includes a description of the simulants used and their properties, equipment and operations, data analysis methodologies, and test results. The results of tests investigating the role of slurry particles in plugging small breaches are reported in Mahoney et al. (2012). The results of the aerosol measurements in the large-scale test stand are reported in Schonewill et al. (2012) along with an analysis of the combined results from both test scales.

  7. Reducing Plug and Process Loads for a Large Scale, Low Energy Office Building: NREL's Research Support Facility; Preprint

    SciTech Connect (OSTI)

    Lobato, C.; Pless, S.; Sheppy, M.; Torcellini, P.

    2011-02-01

    This paper documents the design and operational plug and process load energy efficiency measures needed to allow a large scale office building to reach ultra high efficiency building goals. The appendices of this document contain a wealth of documentation pertaining to plug and process load design in the RSF, including a list of equipment was selected for use.

  8. A Prototyping Environment for Research on Human-Machine Interfaces in Process Control: Use of Microsoft WPF for Microworld and Distributed Control System Development

    SciTech Connect (OSTI)

    Roger Lew; Ronald L. Boring; Thomas A. Ulrich

    2014-08-01

    Operators of critical processes, such as nuclear power production, must contend with highly complex systems, procedures, and regulations. Developing human-machine interfaces (HMIs) that better support operators is a high priority for ensuring the safe and reliable operation of critical processes. Human factors engineering (HFE) provides a rich and mature set of tools for evaluating the performance of HMIs, but the set of tools for developing and designing HMIs is still in its infancy. Here we propose that Microsoft Windows Presentation Foundation (WPF) is well suited for many roles in the research and development of HMIs for process control.

  9. Wave like signatures in aerosol optical depth and associated radiative impacts over the central Himalayan region

    SciTech Connect (OSTI)

    Shukla, K. K.; Phanikumar, D. V.; Kumar, Niranjan; Reddy, Kishore; Kotamarthi, Veerabhadra R.; Newsom, Rob K.; Ouarda, Taha B.

    2015-10-01

    In this study, we present a case study on 16 October 2011 to show the first observational evidence of the influence of short period gravity waves in aerosol transport during daytime over the central Himalayan region. The Doppler lidar data has been utilized to address the daytime boundary layer evolution and related aerosol dynamics over the site. Mixing layer height is estimated by wavelet covariance transform method and found to be ~ 0.7 km, AGL. Aerosol optical depth observations during daytime revealed an asymmetry showing clear enhancement during afternoon hours as compared to forenoon. Interestingly, Fourier and wavelet analysis of vertical velocity and attenuated backscatter showed similar 50-90 min short period gravity wave signatures during afternoon hours. Moreover, our observations showed that gravity waves are dominant within the boundary layer implying that the daytime boundary layer dynamics is playing a vital role in transporting the aerosols from surface to the top of the boundary layer. Similar modulations are also evident in surface parameters like temperature, relative humidity and wind speed indicating these waves are associated with the dynamical aspects over Himalayan region. Finally, time evolution of range-23 height indicator snapshots during daytime showed strong upward velocities especially during afternoon hours implying that convective processes through short period gravity waves plays a significant role in transporting aerosols from the nearby valley region to boundary layer top over the site. These observations also establish the importance of wave induced daytime convective boundary layer dynamics in the lower Himalayan region.

  10. Process Design and Economics for the Conversion of Lignocellulosic Biomass to High Octane Gasoline: Thermochemical Research Pathway with Indirect Gasification and Methanol Intermediate

    SciTech Connect (OSTI)

    Tan, Eric; Talmadge, M.; Dutta, Abhijit; Hensley, Jesse; Schaidle, Josh; Biddy, Mary J.; Humbird, David; Snowden-Swan, Lesley J.; Ross, Jeff; Sexton, Danielle; Yap, Raymond; Lukas, John

    2015-03-01

    The U.S. Department of Energy (DOE) promotes research for enabling cost-competitive liquid fuels production from lignocellulosic biomass feedstocks. The research is geared to advance the state of technology (SOT) of biomass feedstock supply and logistics, conversion, and overall system sustainability. As part of their involvement in this program, the National Renewable Energy Laboratory (NREL) and the Pacific Northwest National Laboratory (PNNL) investigate the economics of conversion pathways through the development of conceptual biorefinery process models. This report describes in detail one potential conversion process for the production of high octane gasoline blendstock via indirect liquefaction (IDL). The steps involve the conversion of biomass to syngas via indirect gasification followed by gas cleanup and catalytic syngas conversion to a methanol intermediate; methanol is then further catalytically converted to high octane hydrocarbons. The conversion process model leverages technologies previously advanced by research funded by the Bioenergy Technologies Office (BETO) and demonstrated in 2012 with the production of mixed alcohols from biomass. Biomass-derived syngas cleanup via tar and hydrocarbons reforming was one of the key technology advancements as part of that research. The process described in this report evaluates a new technology area with downstream utilization of clean biomass-syngas for the production of high octane hydrocarbon products through a methanol intermediate, i.e., dehydration of methanol to dimethyl ether (DME) which subsequently undergoes homologation to high octane hydrocarbon products.

  11. Process Design and Economics for the Conversion of Lignocellulosic Biomass to Hydrocarbon Fuels. Thermochemical Research Pathways with In Situ and Ex Situ Upgrading of Fast Pyrolysis Vapors

    SciTech Connect (OSTI)

    Dutta, Abhijit; Sahir, Asad; Tan, Eric; Humbird, David; Snowden-Swan, Lesley J.; Meyer, Pimphan; Ross, Jeff; Sexton, Danielle; Yap, Raymond; Lukas, John Lukas

    2015-03-01

    This report was developed as part of the U.S. Department of Energy’s Bioenergy Technologies Office’s efforts to enable the development of technologies for the production of infrastructurecompatible, cost-competitive liquid hydrocarbon fuels from biomass. Specifically, this report details two conceptual designs based on projected product yields and quality improvements via catalyst development and process integration. It is expected that these research improvements will be made within the 2022 timeframe. The two conversion pathways detailed are (1) in situ and (2) ex situ upgrading of vapors produced from the fast pyrolysis of biomass. While the base case conceptual designs and underlying assumptions outline performance metrics for feasibility, it should be noted that these are only two of many other possibilities in this area of research. Other promising process design options emerging from the research will be considered for future techno-economic analysis.

  12. Externally pressurized porous cylinder for multiple surface aerosol generation and method of generation

    DOE Patents [OSTI]

    Apel, C.T.; Layman, L.R.; Gallimore, D.L.

    1988-05-10

    A nebulizer is described for generating aerosol having small droplet sizes and high efficiency at low sample introduction rates. The nebulizer has a cylindrical gas permeable active surface. A sleeve is disposed around the cylinder and gas is provided from the sleeve to the interior of the cylinder formed by the active surface. In operation, a liquid is provided to the inside of the gas permeable surface. The gas contacts the wetted surface and forms small bubbles which burst to form an aerosol. Those bubbles which are large are carried by momentum to another part of the cylinder where they are renebulized. This process continues until the entire sample is nebulized into aerosol sized droplets. 2 figs.

  13. Aerosol characterization study using multi-spectrum remote sensing measurement techniques.

    SciTech Connect (OSTI)

    Glen, Crystal Chanea; Sanchez, Andres L.; Lucero, Gabriel Anthony; Schmitt, Randal L.; Johnson, Mark S.; Tezak, Matthew Stephen; Servantes, Brandon Lee

    2013-09-01

    A unique aerosol flow chamber coupled with a bistatic LIDAR system was implemented to measure the optical scattering cross sections and depolarization ratio of common atmospheric particulates. Each of seven particle types (ammonium sulfate, ammonium nitrate, sodium chloride, potassium chloride, black carbon and Arizona road dust) was aged by three anthropogenically relevant mechanisms: 1. Sulfuric acid deposition, 2. Toluene ozonolysis reactions, and 3. m-Xylene ozonolysis reactions. The results of pure particle scattering properties were compared with their aged equivalents. Results show that as most particles age under industrial plume conditions, their scattering cross sections are similar to pure black carbon, which has significant impacts to our understanding of aerosol impacts on climate. In addition, evidence emerges that suggest chloride-containing aerosols are chemically altered during the organic aging process. Here we present the direct measured scattering cross section and depolarization ratios for pure and aged atmospheric particulates.

  14. Automated solar cell assembly teamed process research. Semiannual subcontract report, 7 January 1993--30 June 1993

    SciTech Connect (OSTI)

    Nowlan, M.J.; Hogan, S.J.; Darkazalli, G.; Breen, W.F.; Murach, J.M.; Sutherland, S.F.

    1994-02-01

    This report describes work done under Phase 3A of the PVMaT project to address problems that are generic to the photovoltaics (PV) industry. Crystalline silicon solar cells were used in the majority of all terrestrial power modules shipped in 1992. Spire`s analysis in Phase 1 of the PVMaT project indicated that the use of thin ({le}200-{mu}m) silicon cells can substantially reduce module manufacturing costs, provided that processing yields remain as high as they are now for processing standard thickness cells. Because present solar cell tabbing and interconnecting processes have unacceptably high yield losses with such thin cells, the objective of this Phase 3A subcontract is to use Spire`s light soldering technology and experience in designing and fabricating solar cell tabbing and interconnecting equipment to develop high yield throughput, fully automated processes for tabbing and interconnecting thin cells.

  15. Automated solar cell assembly team process research. Annual subcontract report, 1 January 1993--31 December 1993

    SciTech Connect (OSTI)

    Nowlan, M.J.; Hogan, S.J.; Darkazalli, G.; Breen, W.F.; Murach, J.M.; Sutherland, S.F.; Patterson, J.S.

    1994-06-01

    This report describes work done under the Photovoltaic Manufacturing Technology (PVMaT) project, Phase 3A, which addresses problems that are generic to the photovoltaic (PV) industry. Spire`s objective during Phase 3A was to use its light soldering technology and experience to design and fabricate solar cell tabbing and interconnecting equipment to develop new, high-yield, high-throughput, fully automated processes for tabbing and interconnecting thin cells. Areas that were addressed include processing rates, process control, yield, throughput, material utilization efficiency, and increased use of automation. Spire teamed with Solec International, a PV module manufacturer, and the University of Massachusetts at Lowell`s Center for Productivity Enhancement (CPE), automation specialists, who are lower-tier subcontractors. A number of other PV manufacturers, including Siemens Solar, Mobil Solar, Solar Web, and Texas instruments, agreed to evaluate the processes developed under this program.

  16. Radiance Research Particle Soot/Absorption Photometer Instrument Handbook

    Office of Scientific and Technical Information (OSTI)

    (Technical Report) | SciTech Connect Radiance Research Particle Soot/Absorption Photometer Instrument Handbook Citation Details In-Document Search Title: Radiance Research Particle Soot/Absorption Photometer Instrument Handbook Radiance Research PSAPs as described in this Handbook are deployed in the second ARM Mobile Facility (AMF2) Aerosol Observing System (AOS), the third ARM Mobile Facility (AMF3) AOS, ENA AOS and Mobile Aerosol Observing System (MAOS)-A. An earlier version of the PSAP

  17. Chemical Composition and Sources of Coastal Marine Aerosol Particles during the 2008 VOCALS-REx Campaign

    SciTech Connect (OSTI)

    Lee, Y.- N.; Springston, S.; Jayne, John T.; Wang, Jian; Hubbe, John M.; Senum, Gunnar I.; Kleinman, Lawrence I.; Daum, Peter H.

    2014-05-23

    The chemical composition of aerosol particles (Dp 1.5 ?m) was measured over the southeast Pacific Ocean during the VAMOS (Variability of the American Monsoon Systems) Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-Rex) between 16 October and 15 November 2008 using the US Department of Energy (DOE) G-1 aircraft. The objective of these flights was to gain an understanding of the sources and evolution of these aerosols, and of how they interact with the marine stratus cloud layer that prevails in this region of the globe. Our measurements showed that the marine boundary layer (MBL) aerosol mass was dominated by non-sea-salt SO2?4, followed by Na+, Cl?, Org (total organics), NH+4 , and NO?3 , in decreasing order of importance; CH3SO?3 (MSA), Ca2+, and K+ rarely exceeded their limits of detection. Aerosols were strongly acidic with a NH+4 to SO2?4 equivalents ratio typically < 0.3. Sea-salt aerosol (SSA) particles, represented by NaCl, exhibited Cl? deficits caused by both HNO3 and H2SO4, but for the most part were externally mixed with particles, mainly SO2?4. SSA contributed only a small fraction of the total accumulation mode particle number concentration. It was inferred that all aerosol species (except SSA) were of predominantly continental origin because of their strong land-to-sea concentration gradient. Comparison of relative changes in median values suggests that (1) an oceanic source of NH3 is present between 72 W and 76 W, (2) additional organic aerosols from biomass burns or biogenic precursors were emitted from coastal regions south of 31 S, with possible cloud processing, and (3) free tropospheric (FT) contributions to MBL gas and aerosol concentrations were negligible. The very low levels of CH3SO?3 observed as well as the correlation between SO2?4 and NO?3 (which is thought primarily anthropogenic) suggest a limited contribution of DMS to SO2?4 aerosol production during VOCALS.

  18. Aerosol climate effects and air quality impacts from 1980 to 2030

    SciTech Connect (OSTI)

    Menon, Surabi; Menon, Surabi; Unger, Nadine; Koch, Dorothy; Francis, Jennifer; Garrett, Tim; Sednev, Igor; Shindell, Drew; Streets, David

    2007-11-26

    We investigate aerosol effects on climate for 1980, 1995 (meant to reflect present-day) and 2030 using the NASA Goddard Institute for Space Studies climate model coupled to an on-line aerosol source and transport model with interactive oxidant and aerosol chemistry. Aerosols simulated include sulfates, organic matter (OM), black carbon (BC), sea-salt and dust and additionally, the amount of tropospheric ozone is calculated, allowing us to estimate both changes to air quality and climate for different time periods and emission amounts. We include both the direct aerosol effect and indirect aerosol effects for liquid-phase clouds. Future changes for the 2030 A1B scenario are examined, focusing on the Arctic and Asia, since changes are pronounced in these regions. Our results for the different time periods include both emission changes and physical climate changes. We find that the aerosol indirect effect (AIE) has a large impact on photochemical processing, decreasing ozone amount and ozone forcing, especially for the future (2030-1995). Ozone forcings increase from 0 to 0.12 Wm{sup -2} and the total aerosol forcing increases from -0.10 Wm{sup -2} to -0.94 Wm{sup -2} (AIE increases from -0.13 to -0.68 Wm{sup -2}) for 1995-1980 versus 2030-1995. Over the Arctic we find that compared to ozone and the direct aerosol effect, the AIE contributes the most to net radiative flux changes. The AIE, calculated for 1995-1980, is positive (1.0 Wm{sup -2}), but the magnitude decreases (-0.3Wm{sup -2}) considerably for the future scenario. Over Asia, we evaluate the role of biofuel and transportation-based emissions (for BC and OM) via a scenario (2030A) that includes a projected increase (factor of two) in biofuel and transport-based emissions for 2030 A1B over Asia. Projected changes from present-day due to the 2030A emissions versus 2030 A1B are a factor of 4 decrease in summertime precipitation in Asia. Our results are sensitive to emissions used. Uncertainty in present-day emissions suggest that future climate projections warrant particular scrutiny.

  19. Aerosol beam-focus laser-induced plasma spectrometer device

    DOE Patents [OSTI]

    Cheng, Meng-Dawn

    2002-01-01

    An apparatus for detecting elements in an aerosol includes an aerosol beam focuser for concentrating aerosol into an aerosol beam; a laser for directing a laser beam into the aerosol beam to form a plasma; a detection device that detects a wavelength of a light emission caused by the formation of the plasma. The detection device can be a spectrometer having at least one grating and a gated intensified charge-coupled device. The apparatus may also include a processor that correlates the wavelength of the light emission caused by the formation of the plasma with an identity of an element that corresponds to the wavelength. Furthermore, the apparatus can also include an aerosol generator for forming an aerosol beam from bulk materials. A method for detecting elements in an aerosol is also disclosed.

  20. Apparatus for rapid measurement of aerosol bulk chemical composition

    DOE Patents [OSTI]

    Lee, Yin-Nan E.; Weber, Rodney J.; Orsini, Douglas

    2006-04-18

    An apparatus for continuous on-line measurement of chemical composition of aerosol particles with a fast time resolution is provided. The apparatus includes an enhanced particle size magnifier for producing activated aerosol particles and an enhanced collection device which collects the activated aerosol particles into a liquid stream for quantitative analysis by analytical means. Methods for on-line measurement of chemical composition of aerosol particles are also provided, the method including exposing aerosol carrying sample air to hot saturated steam thereby forming activated aerosol particles; collecting the activated aerosol particles by a collection device for delivery as a jet stream onto an impaction surface; and flushing off the activated aerosol particles from the impaction surface into a liquid stream for delivery of the collected liquid stream to an analytical instrument for quantitative measurement.

  1. Apparatus for rapid measurement of aerosol bulk chemical composition

    DOE Patents [OSTI]

    Lee, Yin-Nan E.; Weber, Rodney J.

    2003-01-01

    An apparatus and method for continuous on-line measurement of chemical composition of aerosol particles with a fast time resolution are provided. The apparatus includes a modified particle size magnifier for producing activated aerosol particles and a collection device which collects the activated aerosol particles into a liquid stream for quantitative analysis by analytical methods. The method provided for on-line measurement of chemical composition of aerosol particles includes exposing aerosol carrying sample air to hot saturated steam thereby forming activated aerosol particles; collecting the activated aerosol particles by a collection device for delivery as a jet stream onto an impaction surface; flushing off the activated aerosol particles from the impaction surface into a liquid stream for delivery of the collected liquid stream to an analytical instrument for quantitative measurement.

  2. Biogenic Aerosols„Effects on Clouds and Climate (BAECC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Biogenic Aerosols-Effects on Clouds and Climate (BAECC) Final Campaign Summary T Petj ... DOESC-ARM-15-051 Biogenic Aerosols-Effects on Clouds and Climate (BAECC) Final Campaign ...

  3. ARM - Field Campaign - Two-Column Aerosol Project (TCAP): Aerial...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsTwo-Column Aerosol Project (TCAP): Aerial Campaign ARM Data Discovery Browse Data Related Campaigns Two-Column Aerosol Project (TCAP) 2012.07.01, Berg, AMF Comments? We...

  4. ARM - Field Campaign - Two-Column Aerosol Project (TCAP)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Browse Data Related Campaigns Two-Column Aerosol Project (TCAP): Field Evaluation of Real-time Cloud OD Sensor TWST 2013.04.15, Scott, AMF Two-Column Aerosol Project (TCAP): Winter ...

  5. ARM - Publications: Science Team Meeting Documents: Aerosol Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ice cloud formation at unusually warm temperatures and low ice supersaturations (via deposition nucleation) involving transported Asian dust layers (as will be reported in Nature)...

  6. Vertical Variability of Aerosols and Water Vapor Over the Southern Great Plains

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Vertical Variability of Aerosols and Water Vapor Over the Southern Great Plains R. A. Ferrare National Aeronautics and Space Administration Langley Research Center Hampton, Virginia D. D. Turner Pacific Northwest National Laboratory Richland, Washington M. Clayton and V. Brackett Science Applications International Corporation National Aeronautics and Space Administration Langley Research Center Hampton, Virginia T. P. Tooman and J. E. M. Goldsmith Sandia National Laboratories Livermore,

  7. Aerodyne Develops an Aircraft-Deployable Precision Aerosol Analyzer | U.S.

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    DOE Office of Science (SC) Aerodyne Develops an Aircraft-Deployable Precision Aerosol Analyzer Small Business Innovation Research (SBIR) and Small Business Technology Transfer (STTR) SBIR/STTR Home About Funding Opportunity Announcements (FOAs) Applicant and Awardee Resources Commercialization Assistance Other Resources Awards SBIR/STTR Highlights Reporting Fraud Contact Information Small Business Innovation Research and Small Business Technology Transfer U.S. Department of Energy

  8. he Impact of Primary Marine Aerosol on Atmospheric Chemistry, Radiation and Climate: A CCSM Model Development Study

    SciTech Connect (OSTI)

    Keene, William C.; Long, Michael S.

    2013-05-20

    This project examined the potential large-scale influence of marine aerosol cycling on atmospheric chemistry, physics and radiative transfer. Measurements indicate that the size-dependent generation of marine aerosols by wind waves at the ocean surface and the subsequent production and cycling of halogen-radicals are important but poorly constrained processes that influence climate regionally and globally. A reliable capacity to examine the role of marine aerosol in the global-scale atmospheric system requires that the important size-resolved chemical processes be treated explicitly. But the treatment of multiphase chemistry across the breadth of chemical scenarios encountered throughout the atmosphere is sensitive to the initial conditions and the precision of the solution method. This study examined this sensitivity, constrained it using high-resolution laboratory and field measurements, and deployed it in a coupled chemical-microphysical 3-D atmosphere model. First, laboratory measurements of fresh, unreacted marine aerosol were used to formulate a sea-state based marine aerosol source parameterization that captured the initial organic, inorganic, and physical conditions of the aerosol population. Second, a multiphase chemical mechanism, solved using the Max Planck Institute for Chemistry??s MECCA (Module Efficiently Calculating the Chemistry of the Atmosphere) system, was benchmarked across a broad set of observed chemical and physical conditions in the marine atmosphere. Using these results, the mechanism was systematically reduced to maximize computational speed. Finally, the mechanism was coupled to the 3-mode modal aerosol version of the NCAR Community Atmosphere Model (CAM v3.6.33). Decadal-scale simulations with CAM v.3.6.33, were run both with and without reactive-halogen chemistry and with and without explicit treatment of particulate organic carbon in the marine aerosol source function. Simulated results were interpreted (1) to evaluate influences of marine aerosol production on the microphysical properties of aerosol populations and clouds over the ocean and the corresponding direct and indirect effects on radiative transfer; (2) atmospheric burdens of reactive halogen species and their impacts on O3, NOx, OH, DMS, and particulate non-sea-salt SO42-; and (3) the global production and influences of marine-derived particulate organic carbon. The model reproduced major characteristics of the marine aerosol system and demonstrated the potential sensitivity of global, decadal-scale climate metrics to multiphase marine-derived components of Earth??s troposphere. Due to the combined computational burden of the coupled system, the currently available computational resources were the limiting factor preventing the adequate statistical analysis of the overall impact that multiphase chemistry might have on climate-scale radiative transfer and climate.

  9. Study of Mechanisms of Aerosol Indirect Effects on Glaciated Clouds: Progress during the Project Final Technical Report

    SciTech Connect (OSTI)

    2013-10-18

    This 3-year project has studied how aerosol pollution influences glaciated clouds. The tool applied has been an 'aerosol-cloud model'. It is a type of Cloud-System Resolving Model (CSRM) modified to include 2-moment bulk microphysics and 7 aerosol species, as described by Phillips et al. (2009, 2013). The study has been done by, first, improving the model and then performing sensitivity studies with validated simulations of a couple of observed cases from ARM. These are namely the Tropical Warm Pool International Cloud Experiment (TWP-ICE) over the tropical west Pacific and the Cloud and Land Surface Interaction Campaign (CLASIC) over Oklahoma. During the project, sensitivity tests with the model showed that in continental clouds, extra liquid aerosols (soluble aerosol material) from pollution inhibited warm rain processes for precipitation production. This promoted homogeneous freezing of cloud droplets and aerosols. Mass and number concentrations of cloud-ice particles were boosted. The mean sizes of cloud-ice particles were reduced by the pollution. Hence, the lifetime of glaciated clouds, especially ice-only clouds, was augmented due to inhibition of sedimentation and ice-ice aggregation. Latent heat released from extra homogeneous freezing invigorated convective updrafts, and raised their maximum cloud-tops, when aerosol pollution was included. In the particular cases simulated in the project, the aerosol indirect effect of glaciated clouds was twice than of (warm) water clouds. This was because glaciated clouds are higher in the troposphere than water clouds and have the first interaction with incoming solar radiation. Ice-only clouds caused solar cooling by becoming more extensive as a result of aerosol pollution. This 'lifetime indirect effect' of ice-only clouds was due to higher numbers of homogeneously nucleated ice crystals causing a reduction in their mean size, slowing the ice-crystal process of snow production and slowing sedimentation. In addition to the known indirect effects (glaciation, riming and thermodynamic), new indirect effects were discovered and quantified due to responses of sedimentation, aggregation and coalescence in glaciated clouds to changing aerosol conditions. In summary, the change in horizontal extent of the glaciated clouds ('lifetime indirect effects'), especially of ice-only clouds, was seen to be of higher importance in regulating aerosol indirect effects than changes in cloud properties ('cloud albedo indirect effects').

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Liljegren, J. C., Argonne National Laboratory Area of Research: Atmospheric Thermodynamics and Vertical Structures Working Group(s): Cloud Properties, Radiative Processes...

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    of MBL Cloud Properties over the Azores Download a printable PDF Submitter: Dong, X., University of North Dakota Area of Research: Radiation Processes Working Group(s): Cloud...

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    a printable PDF Submitter: de Boer, G., University of Colorado, BoulderCIRES Area of Research: Radiation Processes Working Group(s): Cloud Life Cycle Journal Reference: de...

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    to improve the representation of the autoconversion process in atmospheric models. This research also reveals major deficiencies of existing empirical schemes (see the figure)....

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Turner, D. D., National Oceanic and Atmospheric Administration Area of Research: Radiation Processes Working Group(s): Cloud Life Cycle Journal Reference: Paine SN, DD Turner, ...

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    "Roobik" Is Part of the Answer, Not a Puzzle Submitter: Turner, D. D., National Oceanic and Atmospheric Administration Area of Research: Radiation Processes Working Group(s): ...

  16. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Turner, D. D., National Oceanic and Atmospheric Administration Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle Journal Reference: Shupe MD, DD Turner, VP ...

  17. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Complexity of Arctic Clouds Download a printable PDF Submitter: Shupe, M., University of Colorado Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle Journal...

  18. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Get Organized Download a printable PDF Submitter: Del Genio, A. D., National Aeronautics and Space Administration Area of Research: Cloud Processes Working Group(s): Cloud...

  19. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    National Laboratory Long, C. N., NOAA Global Monitoring DivisionCIRES Area of Research: Radiation Processes Working Group(s): Cloud Life Cycle Journal Reference: Riihimaki...

  20. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    National Laboratory Ronfeld, D., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Cloud Properties Journal Reference: NA The...

  1. Potential Aerosol Indirect Effects on Atmospheric Circulation and Radiative

    Office of Scientific and Technical Information (OSTI)

    Forcing through Deep Convection (Journal Article) | SciTech Connect Potential Aerosol Indirect Effects on Atmospheric Circulation and Radiative Forcing through Deep Convection Citation Details In-Document Search Title: Potential Aerosol Indirect Effects on Atmospheric Circulation and Radiative Forcing through Deep Convection Aerosol indirect effects, i.e., the interactions of aerosols with clouds by serving as cloud condensation nuclei (CCN) or ice nuclei (IN), constitute the largest

  2. Direct Aerosol Forcing: Calculation from Observables and Sensitivities to

    Office of Scientific and Technical Information (OSTI)

    Inputs (Journal Article) | SciTech Connect Direct Aerosol Forcing: Calculation from Observables and Sensitivities to Inputs Citation Details In-Document Search Title: Direct Aerosol Forcing: Calculation from Observables and Sensitivities to Inputs Understanding sources of uncertainty in aerosol direct radiative forcing (DRF), the difference in a given radiative flux component with and without aerosol, is essential to quantifying changes in Earth's radiation budget. We examine the uncertainty

  3. Pajarito Aerosol Couplings to Ecosystems (PACE) Field Campaign Report

    Office of Scientific and Technical Information (OSTI)

    (Technical Report) | SciTech Connect Pajarito Aerosol Couplings to Ecosystems (PACE) Field Campaign Report Citation Details In-Document Search Title: Pajarito Aerosol Couplings to Ecosystems (PACE) Field Campaign Report Laboratory (LANL) worked on the Pajarito Aerosol Couplings to Ecosystems (PACE) intensive operational period (IOP). PACE's primary goal was to demonstrate routine Mobile Aerosol Observing System (MAOS) field operations and improve instrumental and operational performance.

  4. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Download a printable PDF Submitter: Turner, D. D., National Oceanic and Atmospheric ... Working Group(s): Aerosol Life Cycle, Cloud Life Cycle Journal Reference: Turner DD, EJ ...

  5. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Download a printable PDF Submitter: Turner, D. D., National Oceanic and Atmospheric ... Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Turner DD ...

  6. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Submitter: Turner, D. D., National Oceanic and Atmospheric Administration Area of ... Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Turner DD ...

  7. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Mixing State of Carbonaceous Aerosol Particles in Northern and Southern California ... particles in Northern and Southern California measured during CARES and CalNex 2010." ...

  8. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Aerosols Help Heat Up the Yangtze River Delta in China Download a printable PDF Submitter: ... distribution and associated radiative effects in the Yangtze Delta region of China." ...

  9. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Mixed Bag of Aerosols over Northeastern China Download a printable PDF Submitter: Li, Z., ... over northeastern China: Vertical profiles and the influence of weather on air quality." ...

  10. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Measured Parameterization of Fire Aerosol Single Scattering Albedo Using Combustion Efficiency Download a printable PDF Submitter: Dubey, M. K., Los Alamos National Laboratory Area...

  11. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Yang F, M Ovchinnikov, and RA Shaw. 2014. "Microphysical consequences of the spatial...

  12. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Cloud-Aerosol-Precipitation Interactions Journal Reference: Qian Y, MY Huang, B Yang, and LK Berg. 2013. "A modeling study of irrigation effects on surface fluxes and...

  13. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Chemical Diffusivity and Viscosity of Secondary Organic Aerosols Download a printable PDF ... determination of chemical diffusion within secondary organic zerosol particles." ...

  14. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    organic aerosol and size distribution dynamics: Representing effects of volatility, phase state, and particle-phase reaction." Atmospheric Chemistry and Physics, 14, doi:10.5194...

  15. Research Highlight

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    rates, and changes to liquid droplet nucleation and growth rates. Freezing point depression resulting from soluble material associated with aerosol particles was demonstrated...

  16. ARM Cloud Aerosol Precipitation Experiment (ACAPEX) Science Plan

    SciTech Connect (OSTI)

    Leung, L. R.; Prather, K.; Ralph, R.; Rosenfeld, D.; Spackman, R.; DeMott, P.; Fairall, C.; Fan, J.; Hagos, S.; Hughes, M.; Long, C.; Rutledge, S.; Waliser, D.; Wang, H.

    2014-09-01

    The western U.S. receives precipitation predominantly during the cold season when storms approach from the Pacific Ocean. The snowpack that accumulates during winter storms provides about 70-90% of water supply for the region. Understanding and modeling the fundamental processes that govern the large precipitation variability and extremes in the western U.S. is a critical test for the ability of climate models to predict the regional water cycle, including floods and droughts. Two elements of significant importance in predicting precipitation variability in the western U.S. are atmospheric rivers and aerosols. Atmospheric rivers (ARs) are narrow bands of enhanced water vapor associated with the warm sector of extratropical cyclones over the Pacific and Atlantic oceans. Because of the large lower-tropospheric water vapor content, strong atmospheric winds and neutral moist static stability, some ARs can produce heavy precipitation by orographic enhancement during landfall on the U.S. West Coast. While ARs are responsible for a large fraction of heavy precipitation in that region during winter, much of the rest of the orographic precipitation occurs in post-frontal clouds, which are typically quite shallow, with tops just high enough to pass the mountain barrier. Such clouds are inherently quite susceptible to aerosol effects on both warm rain and ice precipitation-forming processes.

  17. Design and construction of coal/biomass to liquids (CBTL) process development unit (PDU) at the University of Kentucky Center for Applied Energy Research (CAER)

    SciTech Connect (OSTI)

    Placido, Andrew; Liu, Kunlei; Challman, Don; Andrews, Rodney; Jacques, David

    2015-10-30

    This report describes a first phase of a project to design, construct and commission an integrated coal/biomass-to-liquids facility at a capacity of 1 bbl. /day at the University of Kentucky Center for Applied Energy Research (UK-CAER) – specifically for construction of the building and upstream process units for feed handling, gasification, and gas cleaning, conditioning and compression. The deliverables from the operation of this pilot plant [when fully equipped with the downstream process units] will be firstly the liquid FT products and finished fuels which are of interest to UK-CAER’s academic, government and industrial research partners. The facility will produce research quantities of FT liquids and finished fuels for subsequent Fuel Quality Testing, Performance and Acceptability. Moreover, the facility is expected to be employed for a range of research and investigations related to: Feed Preparation, Characteristics and Quality; Coal and Biomass Gasification; Gas Clean-up/ Conditioning; Gas Conversion by FT Synthesis; Product Work-up and Refining; Systems Analysis and Integration; and Scale-up and Demonstration. Environmental Considerations - particularly how to manage and reduce carbon dioxide emissions from CBTL facilities and from use of the fuels - will be a primary research objectives. Such a facility has required significant lead time for environmental review, architectural/building construction, and EPC services. UK, with DOE support, has advanced the facility in several important ways. These include: a formal EA/FONSI, and permits and approvals; construction of a building; selection of a range of technologies and vendors; and completion of the upstream process units. The results of this project are the FEED and detailed engineering studies, the alternate configurations and the as-built plant - its equipment and capabilities for future research and demonstration and its adaptability for re-purposing to meet other needs. These are described in some detail in this report, along with lessons learned.

  18. Research & Development of Materials/Processing Methods for Continuous Fiber Ceramic Composites (CFCC) Phase 2 Final Report.

    SciTech Connect (OSTI)

    Szweda, A.

    2001-01-01

    The Department of Energy's Continuous Fiber Ceramic Composites (CFCC) Initiative that begun in 1992 has led the way for Industry, Academia, and Government to carry out a 10 year R&D plan to develop CFCCs for these industrial applications. In Phase II of this program, Dow Corning has led a team of OEM's, composite fabricators, and Government Laboratories to develop polymer derived CFCC materials and processes for selected industrial applications. During this phase, Dow Corning carried extensive process development and representative component demonstration activities on gas turbine components, chemical pump components and heat treatment furnace components.

  19. Aerosol can puncture device test report

    SciTech Connect (OSTI)

    Leist, K.J.

    1994-10-01

    This test report documents the evaluation of an aerosol can puncture device to replace a system currently identified for use in the WRAP-1 facility. The new system is based upon a commercially available puncture device, as recommended by WHC Fire Protection. With modifications found necessary through the testing program, the Aerosol Can Puncture Device was found able to puncture and drain aerosol cans without incident. Modifications include the addition of a secondary collection bottle and the modification of the can puncture needle. In the course of testing, a variety of absorbents were tested to determine their performance in immobilizing drained fluids. The visibility of the puncture with Non-Destructive Examination techniques were also reviewed.

  20. Aerosol Properties from Multi-spectral and Multi-angular Aircraft 4STAR Observations: Expected Advantages and Challenges

    SciTech Connect (OSTI)

    Kassianov, Evgueni I.; Flynn, Connor J.; Redemann, Jens; Schmid, Beat; Russell, P. B.; Sinyuk, Alexander

    2012-11-01

    The airborne Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR) is developed to retrieve aerosol microphysical and optical properties from multi-angular and multi-spectral measurements of sky radiance and direct-beam sun transmittance. The necessarily compact design of the 4STAR may cause noticeable apparent enhancement of sky radiance at small scattering angles. We assess the sensitivity of expected 4STAR-based aerosol retrieval to such enhancement by applying the operational AERONET retrieval code and constructed synthetic 4STARlike data. Also, we assess the sensitivity of the broadband fluxes and the direct aerosol radiative forcing to uncertainties in aerosol retrievals associated with the sky radiance enhancement. Our sensitivity study results suggest that the 4STARbased aerosol retrieval has limitations in obtaining detailed information on particle size distribution and scattering phase function. However, these limitations have small impact on the retrieved bulk optical parameters, such as the asymmetry factor (up to 4%, or 0.02) and single-scattering albedo (up to 2%, or 0.02), and the calculated direct aerosol radiative forcing (up to 6%, or 2 Wm-2).