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1

COLLABORATIVE RESEARCH: Study of Aerosol Sources and Processing at the GVAX Pantnagar Supersite  

SciTech Connect

This project funded the participation of scientists from seven research groups, running more than thirty instruments, in the Winter Intensive Operating Period (January-February 2012) of the Clean Air for London (ClearfLo) campaign at a rural site in Detling, UK, 45 km southeast of central London. The primary science questions for the ClearfLo Winter IOP were, 1) what is the urban increment of particulate matter (PM) and other pollutants in the greater London area, and, 2) what is the contribution of solid fuel use for home heating to wintertime PM? An additional motivation for the Detling measurements was the question of whether coatings on black carbon particles enhance absorption. The following four key accomplishments have been identified so far: 1) Chemical, physical and optical characterization of PM from local and regional sources (Figures 2, 4, 5 and 6). 2) Measurement of urban increment in particulate matter and gases in London (Figure 3). 3) Measurement of optical properties and chemical composition of coatings on black carbon containing particles indicates absorption enhancement. 4) First deployment of chemical ionization instrument (MOVI-CI-TOFMS) to measure both particle-phase and gas-phase organic acids. (See final report from Joel Thornton, University of Washington, for details.) Analysis of the large dataset acquired in Detling is ongoing and will yield further key accomplishments. These measurements of urban and rural aerosol properties will contribute to improved modeling of regional aerosol emissions, and of atmospheric aging and removal. The measurement of absorption enhancement by coatings on black carbon will contribute to improved modeling of the direct radiative properties of PM.

Worsnop, Douglas R. [Principal Investigator

2014-07-28T23:59:59.000Z

2

DOE research on atmospheric aerosols  

SciTech Connect

Atmospheric aerosols are the subject of a significant component of research within DOE`s environmental research activities, mainly under two programs within the Department`s Environmental Sciences Division, the Atmospheric Radiation Measurement (ARM) Program and the Atmospheric Chemistry Program (ACP). Research activities conducted under these programs include laboratory experiments, field measurements, and theoretical and modeling studies. The objectives and scope of these programs are briefly summarized. The ARM Program is the Department`s major research activity focusing on atmospheric processes pertinent to understanding global climate and developing the capability of predicting global climate change in response to energy related activities. The ARM approach consists mainly of testing and improving models using long-term measurements of atmospheric radiation and controlling variables at highly instrumented sites in north central Oklahoma, in the Tropical Western Pacific, and on the North Slope of Alaska. Atmospheric chemistry research within DOE addresses primarily the issue of atmospheric response to emissions from energy-generation sources. As such this program deals with the broad topic known commonly as the atmospheric source-receptor sequence. This sequence consists of all aspects of energy-related pollutants from the time they are emitted from their sources to the time they are redeposited at the Earth`s surface.

Schwartz, S.E.

1995-11-01T23:59:59.000Z

3

Researchers Model Impact of Aerosols Over California  

NLE Websites -- All DOE Office Websites (Extended Search)

Researchers Model Researchers Model Impact of Aerosols Over California Researchers Model Impact of Aerosols Over California Research may clarify the effectiveness of regional pollution controls May 28, 2013 | Tags: Climate Research, Hopper Contact: Linda Vu, lvu@lbl.gov, (510) 495-2404 LosAngelesSmogv1.jpg Smog over downtown Los Angeles. Aerosols are microscopic particles-like dust, pollen and soot-that ubiquitously float around in our atmosphere. Despite their tiny stature, these particles can have a huge impact on human health, climate and the environment. So scientists from the Pacific Northwest National Laboratory (PNNL), Colorado State University and the California Air Resources Board have set out to characterize the roles of various particles as atmospheric change agents on a regional scale.

4

ARM - Field Campaign - 2007 Cumulus Humilis Aerosol Process Study (CHAPS)  

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7 Cumulus Humilis Aerosol Process Study (CHAPS) 7 Cumulus Humilis Aerosol Process Study (CHAPS) Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : 2007 Cumulus Humilis Aerosol Process Study (CHAPS) 2007.06.04 - 2007.06.25 Lead Scientist : Carl Berkowitz For data sets, see below. Description The primary goal of this campaign was to characterize and contrast freshly emitted aerosols above, within and below fields of cumulus humilis (or fair-weather cumulus, FWC) and to use these observations to address how below-cloud and above-cloud aerosol optical and cloud nucleating properties differ downwind of a mid-size city relative to similar aerosols in air less affected by emissions. The observations from this campaign can also be used to aid in the development and evaluation of parameterizations of the

5

Aerosol Science and Technology, 41:202216, 2007 Copyright c American Association for Aerosol Research  

E-Print Network (OSTI)

processes, such as con- densation, coagulation, gas-to-particle conversion (Reid et al. 1998), and particle Aerosol size distribution is, along with particle refractive in- dex and shape, one of important

6

The Aerosol Modeling Testbed: A community tool to objectively evaluate aerosol process modules  

SciTech Connect

This study describes a new modeling paradigm that significantly advances how the third activity is conducted while also fully exploiting data and findings from the first two activities. The Aerosol Modeling Testbed (AMT) is a computational framework for the atmospheric sciences community that streamlines the process of testing and evaluating aerosol process modules over a wide range of spatial and temporal scales. The AMT consists of a fully-coupled meteorology-chemistry-aerosol model, and a suite of tools to evaluate the performance of aerosol process modules via comparison with a wide range of field measurements. The philosophy of the AMT is to systematically and objectively evaluate aerosol process modules over local to regional spatial scales that are compatible with most field campaigns measurement strategies. The performance of new treatments can then be quantified and compared to existing treatments before they are incorporated into regional and global climate models. Since the AMT is a community tool, it also provides a means of enhancing collaboration and coordination among aerosol modelers.

Fast, Jerome D.; Gustafson, William I.; Chapman, Elaine G.; Easter, Richard C.; Rishel, Jeremy P.; Zaveri, Rahul A.; Grell, Georg; Barth, Mary

2011-03-02T23:59:59.000Z

7

Representing Cloud Processing of Aerosol in Numerical Models  

SciTech Connect

The satellite imagery in Figure 1 provides dramatic examples of how aerosol influences the cloud field. Aerosol from ship exhaust can serve as nucleation centers in otherwise cloud-free regions, forming ship tracks (top image), or can enhance the reflectance/albedo in already cloudy regions. This image is a demonstration of the first indirect effect, in which changes in aerosol modulate cloud droplet radius and concentration, which influences albedo. It is thought that, through the effects it has on precipitation (drizzle), aerosol can also affect the structure and persistence of planetary boundary layer (PBL) clouds. Regions of cellular convection, or open pockets of cloudiness (bottom image) are thought to be remnants of strongly drizzling PBL clouds. Pockets of Open Cloudiness (POCs) (Stevens et al. 2005) or Albrecht's ''rifts'' are low cloud fraction regions characterized by anomalously low aerosol concentrations, implying they result from precipitation. These features may in fact be a demonstration of the second indirect effect. To accurately represent these clouds in numerical models, we have to treat the coupled cloud-aerosol system. We present the following series of mesoscale and large eddy simulation (LES) experiments to evaluate the important aspects of treating the coupled cloud-aerosol problem. 1. Drizzling and nondrizzling simulations demonstrate the effect of drizzle on a mesoscale forecast off the California coast. 2. LES experiments with explicit (bin) microphysics gauge the relative importance of the shape of the aerosol spectrum on the 3D dynamics and cloud structure. 3. Idealized mesoscale model simulations evaluate the relative roles of various processes, sources, and sinks.

Mechem, D.B.; Kogan, Y.L.

2005-03-18T23:59:59.000Z

8

Final Report for LDRD Project ''A New Era of Research in Aerosol/Cloud/Climate Interactions at LLNL''  

SciTech Connect

Observations of global temperature records seem to show less warming than predictions of global warming brought on by increasing concentrations of CO{sub 2} and other greenhouse gases. One of the reasonable explanations for this apparent inconsistency is that the increasing concentrations of anthropogenic aerosols may be partially counteracting the effects of greenhouse gases. Aerosols can scatter or absorb the solar radiation, directly change the planetary albedo. Aerosols, unlike CO{sub 2}, may also have a significant indirect effect by serving as cloud condensation nuclei (CCN). Increases in CCN can result in clouds with more but smaller droplets, enhancing the reflection of solar radiation. Aerosol direct and indirect effects are a strong function of the distributions of all aerosol types and the size distribution of the aerosol in question. However, the large spatial and temporal variabilities in the concentration, chemical characteristics, and size distribution of aerosols have made it difficult to assess the magnitude of aerosol effects on atmospheric radiation. These variabilities in aerosol characteristics as well as their effects on clouds are the leading sources of uncertainty in predicting future climate variation. Inventory studies have shown that the present-day anthropogenic emissions contribute more than half of fine particle mass primarily due to sulfate and carbonaceous aerosols derived from fossil fuel combustion and biomass burning. Parts of our earlier studies have been focused on developing an understanding of global sulfate and carbonaceous aerosol abundances and investigating their climate effects [Chuang et al., 1997; Penner et al., 1998]. We have also modeled aerosol optical properties to account for changes in the refractive indices with relative humidity and dry aerosol composition [Grant et al., 1999]. Moreover, we have developed parameterizations of cloud response to aerosol abundance for use in global models to evaluate the importance of aerosol/cloud interactions on climate forcing [Chuang and Penner, 1995]. Our research has been recognized as one of a few studies attempting to quantify the effects of anthropogenic aerosols on climate in the IPCC Third Assessment Report [IPCC, 2001]. Our previous assessments of aerosol climate effects were based on a general circulation model (NCAR CCM1) fully coupled to a global tropospheric chemistry model (GRANTOUR). Both models, however, were developed more than a decade ago. The lack of advanced physics representation and techniques in our current models limits us from further exploring the interrelationship between aerosol, cloud, and climate variation. Our objective is to move to a new era of aerosol/cloud/climate modeling at LLNL by coupling the most advanced chemistry and climate models and by incorporating an aerosol microphysics module. This modeling capability will enable us to identify and analyze the responsible processes in aerosol/cloud/climate interactions and therefore, to improve the level of scientific understanding for aerosol climate effects. This state-of-the-art coupled models will also be used to address the relative importance of anthropogenic and natural emissions in the spatial pattern of aerosol climate forcing in order to assess the potential of human induced climate change.

Chuang, C; Bergman, D J; Dignon, J E; Connell, P S

2002-01-31T23:59:59.000Z

9

ARM AOS Processing Status and Aerosol Intensive Properties VAP  

NLE Websites -- All DOE Office Websites (Extended Search)

Andrews, and P. J. Sheridan National Oceanic and Atmospheric Administration Boulder, Colorado Abstract The Atmospheric Radiation Measurement (ARM) Aerosol Observing System (AOS)...

10

The Campaign on atmospheric Aerosol REsearch network of China: CARE-China  

Science Journals Connector (OSTI)

Based on a network of field stations belonging to the Chinese Academy of Sciences (CAS), the Campaign on atmospheric Aerosol REsearch network of China (CARE-China) was recently established as the country's first monitoring network for the study ...

Yuesi Wang; Jinyuan Xin; Yuepeng Pan; Dongsheng Ji; Zirui Liu; Tianxue Wen; Yinghong Wang; Xingru Li; Yang Sun; Jie Sun; Pucai Wang; Gehui Wang; Xinming Wang; Zhiyuan Cong; Tao Song; Bo Hu; Lili Wang; Guiqian Tang; Wenkang Gao; Yuhong Guo; Hongyan Miao; Shili Tian; Lu Wang

11

Jankovic Aerosol Characterization.ppt  

NLE Websites -- All DOE Office Websites (Extended Search)

Characterization, Characterization, Aerosol Characterization, Interpretation, and Interpretation, and Application of Data Application of Data NSRC Symposium NSRC Symposium July 8, 2008 John Jankovic, CIH CIH Center for Nanophase Materials Sciences Center for Nanophase Materials Sciences Aerosol Characterization, Interpretation, and Aerosol Characterization, Interpretation, and Application of Data Application of Data Department of Energy (DOE) Nanoscale Science Research Centers (NSRC) developing Approach to Nanomaterial ES&H - The CNMS Approach * Establish Exposure Control Guideline (ECG) - Characterize Aerosol * Collect and interpret data * Assign Process to a Control Band Aerosol Particle Characterization * Size distribution (geometric mean and geometric standard deviation related to either mass, surface, or number)

12

Aerosol Science and Technology, 47:818830, 2013 Copyright C American Association for Aerosol Research  

E-Print Network (OSTI)

concentrations (mean mid October 2012; accepted 29 January 2013. This research was funded by NSF ATM-0723582 and ATM- 0919189, DOE, and thermal shifts in gas-particle partitioning. Wet deposition was estimated to be an order of magnitude

13

Aerosol Science and Technology, 47:9398, 2013 Copyright C American Association for Aerosol Research  

E-Print Network (OSTI)

and the specific surface area of the composite also increased from 122 to 146 m2 /g. Also, the intensity of the GR higher performance on methanol oxidation than a commercial 20 wt% Pt/carbon black catalyst. 1 Research Project of the Korea Institute of Geoscience and Mineral Resources funded by the Ministry

Huang, Jiaxing

14

Aerosol Science and Technology, 40:10021015, 2006 Copyright c American Association for Aerosol Research  

E-Print Network (OSTI)

Research ISSN: 0278-6826 print / 1521-7388 online DOI: 10.1080/02786820600919408 Studies of Diesel Engine, Upton, New York, USA 2 Oak Ridge National Laboratory, Oak Ridge, Tennessee, USA Diesel engine particle sources of sub 2.5 micron particles (PM2.5) and it is well known that diesel engines emit more particle

15

Photolytic processing of secondary organic aerosols dissolved in cloud droplets  

SciTech Connect

The effect of UV irradiation on the molecular composition of aqueous extracts of secondary organic aerosol (SOA) was investigated. SOA was prepared by the dark reaction of ozone and d-limonene at 0.05 - 1 ppm precursor concentrations and collected with a particle-into-liquid sampler (PILS). The PILS extracts were photolyzed by 300 - 400 nm radiation for up to 24 hours. Water-soluble SOA constituents were analyzed using high-resolution electrospray ionization mass spectrometry (HR-ESI-MS) at different stages of photolysis for all SOA precursor concentrations. Exposure to UV radiation increased the average O/C ratio and decreased the average double bond equivalent (DBE) of the dissolved SOA compounds. Oligomeric compounds were significantly reduced by photolysis relative to the monomeric compounds. Direct pH measurements showed that compounds containing carboxylic acids increased upon photolysis. Methanol reactivity analysis revealed significant photodissociation of molecules containing carbonyl groups and formation of carboxylic acids. Aldehydes, such as limononaldehyde, were almost completely removed. The removal of carbonylswas confirmed by the UV-Vis absorption spectroscopy of the SOA extracts where the absorbance in the carbonyl n??* band decreased significantly upon photolysis. The effective quantum yield (the number of carbonyls destroyed per photon absorbed) was estimated as ~ 0.03. The concentration of peroxides did not change significantly during photolysis as quantified with an iodometric test. Although organic peroxides were photolyzed, the likely end products of photolysis were smaller peroxides, including hydrogen peroxide, resulting in a no net change in the peroxide content.

Bateman, Adam P.; Nizkorodov, Serguei; Laskin, Julia; Laskin, Alexander

2011-05-26T23:59:59.000Z

16

Hospital Sterile Processing | GE Global Research  

NLE Websites -- All DOE Office Websites (Extended Search)

Researches Use of Robots for Hospital Sterile Processing GE Researches Use of Robots for Hospital Sterile Processing GE principal investigator Lynn DeRose discusses the robotic...

17

Research Unit on Biosphere -Aerosol -Cloud -Climate Interactions  

E-Print Network (OSTI)

-222. Seinfeld J., 1986: Atmospheric Chemistry and Physics of Air Pollution. Jonh Wiley and sons. New York, USA that dry deposition and surface exchange processes require a better description in atmospheric chemistry.R. and Lenschow D.H., 1983) in the modelling. Finlayson-Pitts B.J. and Pitts J.N., 1986: Atmospheric Chemistry

18

Use of the ARM Measurements of Spectral Zenith Radiance for Better Understanding of 3D Cloud-Radiation Processes & Aerosol-Cloud Interaction  

SciTech Connect

We proposed a variety of tasks centered on the following question: what can we learn about 3D cloud-radiation processes and aerosol-cloud interaction from rapid-sampling ARM measurements of spectral zenith radiance? These ARM measurements offer spectacular new and largely unexploited capabilities in both the temporal and spectral domains. Unlike most other ARM instruments, which average over many seconds or take samples many seconds apart, the new spectral zenith radiance measurements are fast enough to resolve natural time scales of cloud change and cloud boundaries as well as the transition zone between cloudy and clear areas. In the case of the shortwave spectrometer, the measurements offer high time resolution and high spectral resolution, allowing new discovery-oriented science which we intend to pursue vigorously. Research objectives are, for convenience, grouped under three themes: ? Understand radiative signature of the transition zone between cloud-free and cloudy areas using data from ARM shortwave radiometers, which has major climatic consequences in both aerosol direct and indirect effect studies. ? Provide cloud property retrievals from the ARM sites and the ARM Mobile Facility for studies of aerosol-cloud interactions. ? Assess impact of 3D cloud structures on aerosol properties using passive and active remote sensing techniques from both ARM and satellite measurements.

Alexander Marshak; Warren Wiscombe; Yuri Knyazikhin; Christine Chiu

2011-05-24T23:59:59.000Z

19

BNL | Atmospheric Systems Research  

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Atmospheric System Research is a DOE observation-based research program Atmospheric System Research is a DOE observation-based research program created to advance process-level understanding of the key interactions among aerosols, clouds, precipitation, radiation, dynamics, and thermodynamics, with the ultimate goal of reducing the uncertainty in global and regional climate simulations and projections. General areas of research at BNL under this program include studies of aerosol and cloud lifecycles, and cloud-aerosol-precipitation interactions. Contact Robert McGraw, 631.344.3086 aerosols Aerosol Life Cycle The strategic focus of the Aerosol Life Cycle research is observation-based process science-examining the properties and evolution of atmospheric aerosols. Observations come from both long-term studies conducted by the

20

Research Highlights Sorted by Research Area  

NLE Websites -- All DOE Office Websites (Extended Search)

Research Area Research Area Radiation Processes | Cloud Distributions/Characterizations | Surface Properties | General Circulation and Single Column Models/Parameterizations | Aerosol Properties | Atmospheric Thermodynamics and Vertical Structures | Clouds with Low Optical [Water] Depths (CLOWD) | Vertical Velocity | Broadband Heating Rate Profile (BBHRP) | Cloud-Aerosol-Precipitation Interactions | Cloud Processes | Aerosol Processes Radiation Processes Alexandrov, M. D. Optical Depth Measurements by Shadowband Radiometers and Their Uncertainties ARM Berg, L. Surface Summertime Radiative Forcing by Shallow Cumuli at the ARM SGP ARM Bergmann, D. The Influence of Regional Anthropogenic Emission Reductions on Aerosol Direct Radiative Forcing ASR Bhattacharya, A. Burning on the Prairies ARM

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


21

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Study Aerosol Humidity Effects Using the ARM Measurements Study Aerosol Humidity Effects Using the ARM Measurements Submitter: Li, Z., University of Maryland Area of Research: Radiation Processes Working Group(s): Aerosol Journal Reference: Jeong, M.-J., Z. Li, E. Andrews, and S.-C. Tsay (2007). Effect of aerosol humidification on the column aerosol optical thickness over the Atmospheric Radiation Measurement Southern Great Plains site, J. Geophys. Res., 112, D10202, doi:10.1029/2006JD007176. (a)-(j) Column-mean aerosol humidification factor as functions of the weighted column mean RH, . The ambient RH at one of the ten level-legs of the In-situ Aerosol Profile (IAP) measurements is replaced with RH equals 99%. Comparison of estimated column R(RH) following six different methods (M1~M6). Gray solid lines and black dashed lines are linear fit and

22

E-Print Network 3.0 - atmospheric aerosol processes Sample Search...  

NLE Websites -- All DOE Office Websites (Extended Search)

of Applied Science Collection: Environmental Sciences and Ecology 3 Arctic-Winter Climatology and Radiative Effects of Clouds and Aerosols Based on Lidar and Radar Measurements...

23

Edinburgh Research Explorer Probabilistic Programming Process Algebra  

E-Print Network (OSTI)

Edinburgh Research Explorer Probabilistic Programming Process Algebra Citation for published version: Georgoulas, A, Hillston, J, Milios, D & Sanguinetti, G 2014, 'Probabilistic Programming Process.1007/978-3-319-10696-0_21 Link: Link to publication record in Edinburgh Research Explorer Document Version: Preprint (usually

Millar, Andrew J.

24

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

"Invisible" Giants in the Sky "Invisible" Giants in the Sky Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Kassianov E, M Pekour, and J Barnard. 2012. "Aerosols in central California: Unexpectedly large contribution of coarse mode to aerosol radiative forcing." Geophysical Research Letters, 39, L20806, doi:10.1029/2012GL053469. Daily averaged values of (a, b) the direct aerosol radiative forcing (DARF) and (c, d) aerosol radiative forcing efficiency at the top-of-atmosphere calculated for the "original" aerosol optical properties (blue) and their PM1.0 (red) and PM2.5 (green) counterparts at the CARES (left) T0 and (right) T1 sites.

25

Electrically Driven Technologies for Radioactive Aerosol Abatement  

SciTech Connect

The purpose of this research project was to develop an improved understanding of how electriexecy driven processes, including electrocoalescence, acoustic agglomeration, and electric filtration, may be employed to efficiently treat problems caused by the formation of aerosols during DOE waste treatment operations. The production of aerosols during treatment and retrieval operations in radioactive waste tanks and during thermal treatment operations such as calcination presents a significant problem of cost, worker exposure, potential for release, and increased waste volume.

David W. DePaoli; Ofodike A. Ezekoye; Costas Tsouris; Valmor F. de Almeida

2003-01-28T23:59:59.000Z

26

The Joint AerosolMonsoon Experiment: A New Challenge for Monsoon Climate Research  

Science Journals Connector (OSTI)

Aerosol- and moonsoon-related droughts and floods are two of the most serious environmental hazards confronting more than 60% of the population of the world living in the Asian monsoon countries. In recent years, thanks to improved satellite and ...

K-M. Lau; S. C. Tsay; C. Hsu; M. Chin; V. Ramanathan; G-X. Wu; Z. Li; R. Sikka; B. Holben; D. Lu; H. Chen; G. Tartari; P. Koudelova; Y. Ma; J. Huang; K. Taniguchi; R. Zhang

2008-03-01T23:59:59.000Z

27

Chemistry of carbonaceous aerosols : studies of atmospheric processing and OH-initiated oxidation  

E-Print Network (OSTI)

Carbonaceous aerosols are among the most prevalent yet least understood constituents of the atmosphere, particularly in urban environments. We have performed analyses of field samples and laboratory studies to probe the ...

Johnson, Kirsten S. (Kirsten Sue)

2008-01-01T23:59:59.000Z

28

Process-model Simulations of Cloud Albedo Enhancement by Aerosols in the Arctic  

SciTech Connect

A cloud-resolving model is used to simulate the effectiveness of Arctic marine cloud brightening via injection of cloud condensation nuclei (CCN). An updated cloud microphysical scheme is employed, with prognostic CCN and cloud particle numbers in both liquid and mixed-phase marine low clouds. Injection of CCN into the marine boundary layer can delay the collapse of the boundary layer and increase low-cloud albedo. Because nearly all of the albedo effects are in the liquid phase due to the removal of ice water by snowfall when ice processes are involved, albedo increases are stronger for pure liquid clouds than mixed-phase clouds. Liquid precipitation can be suppressed by CCN injection, whereas ice precipitation (snow) is affected less; thus the effectiveness of brightening mixed-phase clouds is lower than for liquid-only clouds. CCN injection into a clean regime results in a greater albedo increase than injection into a polluted regime, consistent with current knowledge about aerosol-cloud interactions. Unlike previous studies investigating warm clouds, dynamical changes in circulation due to precipitation changes are small.

Kravitz, Benjamin S.; Wang, Hailong; Rasch, Philip J.; Morrison, H.; Solomon, Amy

2014-11-17T23:59:59.000Z

29

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Aerosols Help Clouds Warm Up Arctic Aerosols Help Clouds Warm Up Arctic Submitter: Lubin, D., National Science Foundation Area of Research: Radiation Processes Working Group(s): Radiative Processes Journal Reference: Lubin, D., and A.M. Vogelmann, 2006: A climatologically significant aerosol longwave indirect effect in the Arctic, Nature, 439, 26 January, 453-456, doi:10.1038/nature04449 In a process known as the first aerosol indirect effect, enhanced aerosol concentrations cause the droplets in a cloud to be smaller and more numerous within a cloud of fixed water amount. This study found that this process can make many clouds more opaque and emit more thermal energy to the surface. The warming of the Arctic climate and decreases in sea ice area and thickness observed over recent decades are believed to result from

30

Use of the ARM Measurement of Spectral Zenith Radiance For Better Understanding Of 3D Cloud-Radiation Processes and Aerosol-Cloud Interaction  

SciTech Connect

Our proposal focuses on cloud-radiation processes in a general 3D cloud situation, with particular emphasis on cloud optical depth and effective particle size. We also focus on zenith radiance measurements, both active and passive. The proposal has three main parts. Part One exploits the ?¢????solar-background?¢??? mode of ARM lidars to allow them to retrieve cloud optical depth not just for thin clouds but for all clouds. This also enables the study of aerosol cloud interactions with a single instrument. Part Two exploits the large number of new wavelengths offered by ARM?¢????s zenith-pointing ShortWave Spectrometer (SWS), especially during CLASIC, to develop better retrievals not only of cloud optical depth but also of cloud particle size. We also propose to take advantage of the SWS?¢???? 1 Hz sampling to study the ?¢????twilight zone?¢??? around clouds where strong aerosol-cloud interactions are taking place. Part Three involves continuing our cloud optical depth and cloud fraction retrieval research with ARM?¢????s 2NFOV instrument by, first, analyzing its data from the AMF-COPS/CLOWD deployment, and second, making our algorithms part of ARM?¢????s operational data processing.

D. Jui-Yuan Chiu

2010-10-19T23:59:59.000Z

31

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Variations of Meridional Aerosol Distribution and Solar Dimming Variations of Meridional Aerosol Distribution and Solar Dimming Download a printable PDF Submitter: Long, C. N., Pacific Northwest National Laboratory Kishcha, P., Tel-Aviv University Starobinets, B., Tel-Aviv University Kalashnikova, O., Jet Propulsion Laboratory Alpert, P., Tel-Aviv University Area of Research: Radiation Processes Working Group(s): Aerosol, Radiative Processes Journal Reference: Kishcha P, B Starobinets, O Kalashnikova, CN Long, and P Alpert. 2009. "Variations of meridional aerosol distribution and solar dimming." Journal of Geophysical Research - Atmospheres, 114, D00D14, 10.1029/2008JD010975. The distribution of four-year aerosol differences (δAOT/δFAOT) between the last four years (March 2004 - February 2008) and the first four years

32

Use of the ARM Measurements of Spectral Zenith Radiance for Better Understanding of 3D Cloud-Radiation Processes & Aerosol-Cloud Interaction  

SciTech Connect

This project focuses on cloud-radiation processes in a general three-dimensional cloud situation, with particular emphasis on cloud optical depth and effective particle size. The proposal has two main parts. Part one exploits the large number of new wavelengths offered by the Atmospheric Radiation Measurement (ARM) zenith-pointing ShortWave Spectrometer (SWS), to develop better retrievals not only of cloud optical depth but also of cloud particle size. We also take advantage of the SWS high sampling resolution to study the twilight zone around clouds where strong aerosol-cloud interactions are taking place. Part two involves continuing our cloud optical depth and cloud fraction retrieval research with ARMs 2-channel narrow vield-of-view radiometer and sunphotometer instrument by, first, analyzing its data from the ARM Mobile Facility deployments, and second, making our algorithms part of ARMs operational data processing.

Chiu, Jui-Yuan Christine [University of Reading] [University of Reading

2014-04-10T23:59:59.000Z

33

Direct measurements of marine aerosols to examine the influence of biological activity, anthropogenic emissions, and secondary processing on particle chemistry  

E-Print Network (OSTI)

from a low-speed marine diesel engine, Aerosol Sci. Tech. ,from a low-speed marine diesel engine, Aerosol Sci. Tech. ,

Gaston, Cassandra Jayne

2012-01-01T23:59:59.000Z

34

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Scale Shows True Weight of Aerosol Effects on Clouds Scale Shows True Weight of Aerosol Effects on Clouds Download a printable PDF Submitter: McComiskey, A. C., National Oceanic and Atmospheric Administration Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: McComiskey A and G Feingold. 2012. "The scale problem in quantifying aerosol indirect effects." Atmospheric Chemistry and Physics, 12, doi:10.5194/acp-12-1031-2012. Differing values: Values derived from aircraft and surface observations, which represent disaggregated data, differ from those derived from satellite-based data, which represent data aggregated at a range of levels. Currently, many climate change models treat the two types of data the same. Aerosols-tiny airborne particles from sources like pollution or desert

35

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

researchers published research in 2007 that addressed assumptions in the ability of diesel exhaust organic aerosols to mix with organic aerosols from tree evaporate. This new...

36

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

The Mixing State of Carbonaceous Aerosol Particles in Northern and Southern The Mixing State of Carbonaceous Aerosol Particles in Northern and Southern California Measured During CARES and CalNex Download a printable PDF Submitter: Zaveri, R., Pacific Northwest National Laboratory Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Cahill JF, K Suski, JH Seinfeld, RA Zaveri, and KA Prather. 2012. "The mixing state of carbonaceous aerosol particles in Northern and Southern California measured during CARES and CalNex 2010." Atmospheric Chemistry and Physics, 12, doi:10.5194/acp-12-10989-2012. The CARES campaign took place in Sacramento in order to sample the city's urban plume. Photo courtesy of Jason Tomlinson. Researchers, including DOE scientists working at Pacific Northwest National

37

ARM - Measurement - Aerosol particle size  

NLE Websites -- All DOE Office Websites (Extended Search)

particle size particle size ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol particle size Linear size (e.g. radius or diameter) of an aerosol particle. Categories Aerosols Instruments The above measurement is considered scientifically relevant for the following instruments. Refer to the datastream (netcdf) file headers of each instrument for a list of all available measurements, including those recorded for diagnostic or quality assurance purposes. Field Campaign Instruments AEROSMASSSPEC : Aerosol Mass Spectrometer CPI : Cloud Particle Imager DRI-GND : Desert Research Institute Ground-Based Aerosol Instruments DRUM-AEROSOL : Drum Aerosol Sampler AEROSOL-TOWER-EML : EML Tower based Aerosol Measurements

38

E-Print Network 3.0 - aerosol jet system Sample Search Results  

NLE Websites -- All DOE Office Websites (Extended Search)

-controlled laminar aerosol jets and their application for studying aerosol combustion processes Author(s): Shoshin Y... 2002 Times Cited: 6 48. Title: Exhaust aerosol of a...

39

aerosols | EMSL  

NLE Websites -- All DOE Office Websites (Extended Search)

aerosols aerosols Leads No leads are available at this time. Magnesium behavior and structural defects in Mg+ ion implanted silicon carbide. Abstract: As a candidate material for...

40

ARM - Measurement - Aerosol absorption  

NLE Websites -- All DOE Office Websites (Extended Search)

absorption absorption ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol absorption The process in which radiation energy is retained by aerosols. Categories Aerosols Instruments The above measurement is considered scientifically relevant for the following instruments. Refer to the datastream (netcdf) file headers of each instrument for a list of all available measurements, including those recorded for diagnostic or quality assurance purposes. ARM Instruments AOS : Aerosol Observing System CSPHOT : Cimel Sunphotometer IAP : In-situ Aerosol Profiles (Cessna Aerosol Flights) PSAP : Particle Soot Absorption Photometer PASS : Photoacoustic Soot Spectrometer External Instruments OMI : Ozone Monitoring Instrument

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


41

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Impact of Anthropogenic Emissions on Organic Aerosols During CARES Impact of Anthropogenic Emissions on Organic Aerosols During CARES Submitter: Zhang, Q., University of California, Davis Area of Research: Aerosol Processes Working Group(s): Aerosol Life Cycle Journal Reference: Setyan A, Q Zhang, M Merkel, WB Knighton, Y Sun, C Song, J Shilling, TB Onasch, S Herndon, D Worsnop, JD Fast, R Zaveri, LK Berg, A Wiedensohler, BA Flowers, MK Dubey, and R Subramanian. 2012. "Characterization of submicron particles influenced by mixed biogenic and anthropogenic emissions using high-resolution aerosol mass spectrometry: Results from CARES." Atmospheric Chemistry and Physics, 12, doi:10.5194/acp-12-8131-2012. High-resolution mass spectra (colored by ion category) and elemental ratios of the OA factors. Average contribution of ion categories to the total

42

Research towards a systematic signature discovery process  

SciTech Connect

In its most general form, a signature is a unique or distinguishing measurement, pattern, or collection of data that identifies a phenomenon (object, action, or behavior) of interest. The discovery of signatures is an important aspect of a wide range of disciplines from basic science to national security for the rapid and efficient detection and/or prediction of phenomena. Current practice in signature discovery is typically accomplished by asking domain experts to characterize and/or model individual phenomena to identify what might compose a useful signature. What is lacking is an approach that can be applied across a broad spectrum of domains and information sources to efficiently and robustly construct candidate signatures, validate their reliability, measure their quality, and overcome the challenge of detection -- all in the face of dynamic conditions, measurement obfuscation and noisy data environments. Our research has focused on the identification of common elements of signature discovery across application domains and the synthesis of those elements into a systematic process for more robust and efficient signature development. In this way, a systematic signature discovery process lays the groundwork for leveraging knowledge obtained from signatures to a particular domain or problem area, and, more generally, to problems outside that domain. This paper presents the initial results of this research by discussing a mathematical framework for representing signatures and placing that framework in the context of a systematic signature discovery process. Additionally, the basic steps of this process are described with details about the methods available to support the different stages of signature discovery, development, and deployment.

Baker, Nathan A.; Barr, Jonathan L.; Bonheyo, George T.; Joslyn, Cliff A.; Krishnaswami, Kannan; Oxley, Mark; Quadrel, Richard W.; Sego, Landon H.; Tardiff, Mark F.; Wynne, Adam S.

2013-06-04T23:59:59.000Z

43

Two-Column Aerosol Project  

NLE Websites -- All DOE Office Websites (Extended Search)

help find the answer, the Department of Energy's Atmospheric Radiation Measurement (ARM) Climate Research Facility is conducting the Two-Column Aerosol Project (TCAP) at Cape Cod...

44

BNL | Aerosol Lifecycle IOP  

NLE Websites -- All DOE Office Websites (Extended Search)

Program Program Aerosol Life Cycle IOP The primary objectives that make up the Aerosol Life Cycle IOP can be broken down into three categories: Scientific; Logistical; and GVAX preparation. Scientific Objectives The science goals are to conduct intensive aerosol observations in a region exposed to anthropogenic, biogenic, and marine emissions with atmospheric processing times depending on air mass trajectories and time of day. Take advantage of new instruments in the MAOS (e.g., SP2, HR-PTRMS, ACSM, Trace Gas Suite, PASS-3, Aethelometer, UHSAS). Within this broad umbrella are embedded three main foci: Aerosol light absorption: How does the aerosol mass absorption coefficient (absorption per unit mass of BC) vary with atmospheric processing? Do observations agree with a shell-core model?

45

The Indirect and Semi-Direct Aerosol Campaign  

SciTech Connect

Research projects like the Indirect and Semi-Direct Aerosol Campaign, or ISDAC, increase our knowledge of atmospheric aerosol particles and cloud physics.

Ghan, Steve

2014-03-24T23:59:59.000Z

46

Li et al., Aerosol and Air Quality Research, Vol. 6, No. 4, pp. 418-429, 2006 UV-Absorption-Based Measurements of Ozone and Mercury  

E-Print Network (OSTI)

interferences. For example, CMMs based on atomic absorption spectrometry (AAS) are subject to interferences of the Hg detection technique. Atomic absorption spectrometry (AAS) is one of the major techniques appliedLi et al., Aerosol and Air Quality Research, Vol. 6, No. 4, pp. 418-429, 2006 UV-Absorption

Li, Ying

47

Environmental research program: FY 1987, annual report  

SciTech Connect

This multidisciplinary research program includes fundamental and applied research in physics, chemistry, engineering, and biology, as well as research on the development of advanced methods of measurement and analysis. The Program's Annual Report contains summaries of research performed during FY 1987 in the areas of atmospheric aerosols, flue gas chemistry, combustion, membrane bioenergetics, and analytical chemistry. The main research interests of the Atmospheric Aerosol Research group concern the chemical and physical processes that occur in haze, clouds, and fogs. For their studies, the group is developing novel analytical and research methods for characterizing aerosol species. Aerosol research is performed in the laboratory and in the field. Studies of smoke emissions from fires and their possible effects on climatic change, especially as related to nuclear winter, are an example of the collaboration between the Atmospheric Aerosol Research and Combustion Research Groups.

Not Available

1988-03-01T23:59:59.000Z

48

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

the First Aerosol Indirect Effect in Shallow Cumuli Download a printable PDF Submitter: Berg, L., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working...

49

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Key Contributor to Low-Level Cloud Reflectivity Submitter: Penner, J. E., University of Michigan Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference:...

50

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Kelly, JT, CC Chuang, and AS Wexler. 2007. "Influence of dust composition on cloud droplet...

51

A Simple Apparatus for the Injection of Lithium Aerosol into the Scrape-Off Layer of Fusion Research Devices  

SciTech Connect

A simple device has been developed to deposit elemental lithium onto plasma facing components in the National Spherical Torus Experiment. Deposition is accomplished by dropping lithium powder into the plasma column. Once introduced, lithium particles quickly become entrained in scrape-off layer flow as an evaporating aerosol. Particles are delivered through a small central aperture in a computer-controlled resonating piezoelectric disk on which the powder is supported. The device has been used to deposit lithium both during discharges as well as prior to plasma breakdown. Clear improvements to plasma performance have been demonstrated. The use of this apparatus provides flexibility in the amount and timing of lithium deposition and, therefore, may benefit future fusion research devices.

D. K. Mansfield, A.L Roquemore, H. Schneider, J. Timberlake, H. Kugel, M.G. Bell and the NSTX Research Team

2010-10-11T23:59:59.000Z

52

Responsible Science: Ensuring the Integrity of the Research Process  

SciTech Connect

This is the final technical report for DE-SC0005916 Responsible Science: Ensuring the Integrity of the Research Process.

Arrison, Thomas Samuel

2014-03-31T23:59:59.000Z

53

Modeling aerosols and their interactions with shallow cumuli during the 2007 CHAPS field study  

SciTech Connect

The Weather Research and Forecasting model coupled with chemistry (WRF-Chem) is used to simulate relationships between aerosols and clouds in the vicinity of Oklahoma City during the June 2007 Cumulus Humilis Aerosol Processing Study (CHAPS). The regional scale simulation completed using 2 km horizontal grid spacing evaluates four important relationships between aerosols and shallow cumulus clouds observed during CHAPS. First, the model reproduces the trends of higher nitrate volume fractions in cloud droplet residuals compared to interstitial non-activated aerosols, as measured using the Aerosol Mass Spectrometer. Comparing simulations with cloud chemistry turned on and off, we show that nitric acid vapor uptake by cloud droplets explains the higher nitrate content of cloud droplet residuals. Second, as documented using an offline code, both aerosol water and other inorganics (OIN), which are related to dust and crustal emissions, significantly affect predicted aerosol optical properties. Reducing the OIN content of wet aerosols by 50% significantly improves agreement of model predictions with measurements of aerosol optical properties. Third, the simulated hygroscopicity of aerosols is too high as compared to their hygroscopicity derived from cloud condensation nuclei and particle size distribution measurements, indicating uncertainties associated with simulating size-dependent chemical composition and treatment of aerosol mixing state within the model. Fourth, the model reasonably represents the observations of the first aerosol indirect effect where pollutants in the vicinity of Oklahoma City increase cloud droplet number concentrations and decrease the droplet effective radius. While previous studies have often focused on cloud-aerosol interactions in stratiform and deep convective clouds, this study highlights the ability of regional-scale models to represent some of the important aspects of cloud-aerosol interactions associated with fields of short-lived shallow cumuli.

Shrivastava, ManishKumar B.; Berg, Larry K.; Fast, Jerome D.; Easter, Richard C.; Laskin, Alexander; Chapman, Elaine G.; Gustafson, William I.; Liu, Ying; Berkowitz, Carl M.

2013-02-07T23:59:59.000Z

54

10 DESIGN SCIENCE RESEARCH FOR BUSINESS PROCESS DESIGN  

E-Print Network (OSTI)

10 DESIGN SCIENCE RESEARCH FOR BUSINESS PROCESS DESIGN: Organizational Transition at Intersport strategies. This paper elaborates on experiences from a business process design effort in an action research for taking the retail chain Intersport into a new organizational state where the new process design

Paris-Sud XI, Université de

55

EM Marks Milestone at Separations Process Research Unit | Department of  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

Marks Milestone at Separations Process Research Unit Marks Milestone at Separations Process Research Unit EM Marks Milestone at Separations Process Research Unit March 7, 2013 - 12:00pm Addthis Workers construct an enclosure for Building H2 at the Separations Process Research Unit Workers construct an enclosure for Building H2 at the Separations Process Research Unit NISKAYUNA, N.Y. - EM met a major regulatory milestone at the Separations Process Research Unit (SPRU) by completing construction of enclosures and ventilation systems required for cleanup. The SPRU project at the Knolls Atomic Power Laboratory reached the milestone last week in a consent order between DOE and the U.S. Environmental Protection Agency issued pursuant to the Clean Air Act. The Department has now accomplished all the requirements of the consent order.

56

Mobile Climate Observatory for Atmospheric Aerosols in India  

NLE Websites -- All DOE Office Websites (Extended Search)

Atmospheric Aerosols in India Atmospheric Aerosols in India Nainital, India, was the site chosen for deployment of a portable climate research laboratory to study how aerosols impact clouds and energy transfer in the atmosphere. The well-being of hundreds of millions of residents in northeastern India depends on the fertile land around the Ganges River, which is fed by monsoon rains and runoff from the nearby Himalayan Mountains. Any disturbance to the monsoon rains could threaten the population. In the same region, increased industrial activities due to economic growth are releasing small aerosol particles, such as soot and dust, that absorb and scatter sunlight and thus can change cloud formation processes and the heat distribution in the atmosphere. Such changes could greatly increase or

57

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Heating Up the Arctic: Most Complete Data Set Ever Collected Helps Heating Up the Arctic: Most Complete Data Set Ever Collected Helps Scientists Understand Aerosol Download a printable PDF Submitter: Ghan, S. J., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: McFarquhar GM, S Ghan, J Verlinde, A Korolev, JW Strapp, B Schmid, JM Tomlinson, M Wolde, SD Brooks, D Cziczo, MK Dubey, JW Fan, C Flynn, I Gultepe, J Hubbe, MK Gilles, A Laskin, P Lawson, WR Leaitch, P Liu, XH Liu, D Lubin, C Mazzoleni, AM Macdonald, RC Moffet, H Morrison, M Ovchinnikov, MD Shupe, DD Turner, SC Xie, A Zelenyuk, K Bae, M Freer, and A Glen. 2011. "Indirect and Semi-Direct Aerosol Campaign: the impact of Arctic aerosols on clouds." Bulletin of the American Meteorological

58

Aerosol Cans? -Aerosol cans use a pressurized  

E-Print Network (OSTI)

? - The waste generated in the processing of images/photos contains silver. Silver is a toxic heavy metal the product. Propellants are often flammable and/or toxic. Therefore, never store aerosol cans near ignition of this pamphlet. -Carefully transfer the old paint thinner from the one gallon closable can to the 30 gallon metal

Jia, Songtao

59

Examination of the Effects of Sea Salt Aerosols on Southeast Texas Ozone and Secondary Organic Aerosol  

E-Print Network (OSTI)

of this research is to examine sea salt aerosols and their impact on polluted environments. Sea salt aerosols act as Cloud Condensation Nuclei (CCN) as well as providing a surface for heterogeneous reactions. Such reactions have implications for trace gases...

Benoit, Mark David

2013-02-06T23:59:59.000Z

60

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

The Apparent Bluing of Aerosols Near Clouds The Apparent Bluing of Aerosols Near Clouds Download a printable PDF Submitter: Marshak, A., NASA - Goddard Space Flight Center Area of Research: Radiation Processes Working Group(s): Radiative Processes Journal Reference: Marshak, A, G Wen, JA Coakley, LA Remer, NG Loeb, and RF Cahalan. 2008. "A simple model of the cloud adjacency effect and the apparent bluing of aerosols near clouds." Journal of Geophysical Research 113, D14S17, doi: 10.1029/2007JD009196. (upper panel) A schematic two-layer model of a broken cloud field and Rayleigh scatterers. (lower panel) An example of the Poisson distribution of broken cloud fields with cloud fraction Ac = 0.3 for a 10 by 10 km area. For a cloud vertical thickness of 1 km, the left lower panel has cloud

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


61

Purchase Requisition & Purchase Order Approval Process Office of Research Administration  

E-Print Network (OSTI)

Purchase Requisition & Purchase Order Approval Process Office of Research Administration Purchase are sent to the Office of Research Administration as part of the approval for setting up a Purchase Order Requisition & Purchase Order Approval Process 1. Overview Purchase Requisitions and Field Purchase orders

62

NREL: Hydrogen and Fuel Cells Research - Thermochemical Processes  

NLE Websites -- All DOE Office Websites (Extended Search)

Printable Version Printable Version Thermochemical Processes Photo of a researcher wearing a hardhat and examining a catalytic steam reformer. Catalytic steam reforming increases the overall yield of fuel gas from biomass. NREL's researchers have investigated the thermochemical conversion of renewable energy feedstocks since the lab's inception. Researchers are developing gasification and pyrolysis processes to convert biomass and its residues to hydrogen, fuels, chemicals, and power. Building on past successes, biomass is increasingly one of the best near-term options for renewable hydrogen production. Thermochemical Process R&D Research and development at NREL provides a fundamental understanding of the chemistry of biomass pyrolysis. This R&D includes stabilizing and

63

DOE - Office of Legacy Management -- Separations Process Research Unit -  

NLE Websites -- All DOE Office Websites (Extended Search)

Separations Process Research Unit - Separations Process Research Unit - 024 FUSRAP Considered Sites Site: Separations Process Research Unit (024) Designated Name: Alternate Name: Location: Evaluation Year: Site Operations: Site Disposition: Radioactive Materials Handled: Primary Radioactive Materials Handled: Radiological Survey(s): Site Status: This facility was constructed and operated by the Atomic Energy Commission as a pilot plant for developing and testing the chemical processes to extract both uranium and plutonium from irradiated fuel. Through Fiscal Year 1999 the Department of Energy's Office of Naval Reactors performed surveillance and maintenance activities. In Fiscal Year 2000, a contract was initiated to begin the characterization of the facilities. This will be

64

The Southeastern Aerosol Research and Characterization Study, Part 3: Continuous measurements of fine particulate matter mass and composition  

SciTech Connect

Deployment of continuous analyzers in the Southeastern Aerosol Research and Characterization Study (SEARCH) network began in 1998 and continues today as new technologies are developed. Measurement of fine particulate matter (PM2.5) mass is performed using a dried, 30 {sup o}C tapered element oscillating microbalance (TEOM). TEOM measurements are complemented by observations of light scattering by nephelometry. Measurements of major constituents include: (1) SO{sub 4}{sup 2-} via reduction to SO{sub 2}; (2) NH{sub 4}{sup +} and NO{sub 3}{sup -} via respective catalytic oxidation and reduction to NO, (3) black carbon (BC) by optical absorption,(4) total carbon by combustion to CO{sup 2}, and (5) organic carbon by difference between the latter two measurements. Several illustrative examples of continuous data from the SEARCH network are presented. A distinctive composite annual average diurnal pattern is observed for PM2.5 mass, nitrate, and BC, likely indicating the influence of traffic-related emissions, growth, and break up of the boundary layer and formation of ammonium nitrate. Examination of PM2.5 components indicates the need to better understand the continuous composition of the unmeasured 'other' category, because it contributes a significant fraction to total mass during periods of high PM2.5 loading. Selected episodes are presented to illustrate applications of SEARCH data. An SO{sub 2} conversion rate of 0.2%/hr is derived from an observation of a plume from a coal-fired power plant during early spring, and the importance of local, rural sources of NH{sub 3} to the formation of ammonium nitrate in particulate matter (PM) is demonstrated. 41 refs., 15 figs., 3 tabs.

Edgerton, E.S.; Hartsell, B.E.; Saylor, R.D.; Jansen, J.J.; Hansen, D.A.; Hidy, G.M. [Atmospheric Research & Analysis, Inc., Cary, NC (United States)

2006-09-15T23:59:59.000Z

65

2, 20952131, 2002 Below-cloud aerosol  

E-Print Network (OSTI)

). In addition, the understanding of wet removal processes remains crucial in local and regional pollutionACPD 2, 2095­2131, 2002 Below-cloud aerosol removal C. Andronache Title Page Abstract Introduction-cloud aerosol removal by rainfall for observed aerosol size distributions C. Andronache Boston College, Chestnut

Paris-Sud XI, Université de

66

4, 58315854, 2004 Fluorescing aerosol  

E-Print Network (OSTI)

released by combustion into the atmosphere absorbs radiation and therefore heats the climate counteracting such as polycyclic aromatic hydrocarbons sticking to the aerosol particles, or bioaerosol such as bacteria, spores) or by combustion processes (soot), or they form in situ by gas to particle conversion, like sulphate aerosol. While

Paris-Sud XI, Université de

67

Modal Bin Hybrid Model: A Surface Area Consistent, Triple Moment Sectional Method for Use in Process-oriented Modeling of Atmospheric Aerosols  

SciTech Connect

A triple moment sectional method, Modal Bin Hybrid Model (MBHM), has been developed. In addition to number and mass (volume), surface area is predicted (and preserved), which is important for gas-to-particle mass transfer and light extinction cross section. The performance of MBHM was evaluated against double moment sectional (DMS) methods with various size resolutions up to BIN256 (BINx: x is number of sections over three orders of magnitude in size, ?logD = 3/x) for simulating evolution of particles under simultaneously occurring nucleation, condensation and coagulation processes. Because MBHM gives a physically consistent form of the intra-sectional distributions, errors and biases of MBHM at BIN4-8 resolution were almost equivalent to those of DMS at BIN16-32 resolution for various important variables such as the moments Mk (k: 0, 2, 3), dMk/dt, and the number and volume of particles larger than a certain diameter. Another important feature of MBHM is that only a single bin is adequate to simulate full aerosol dynamics for particles whose size distribution can be approximated by a single lognormal mode. This flexibility is useful for process-oriented (multi category and/or mixing state) modeling: primary aerosols whose size parameters would not differ substantially in time and space can be expressed by a single or a small number of modes, whereas secondary aerosols whose size changes drastically from one to several hundred nanometers can be expressed by a number of modes. Added dimensions can be applied to MBHM to represent mixing state or photo-chemical age for aerosol mixing state studies.

Kajino, Mizuo; Easter, Richard C.; Ghan, Steven J.

2013-09-10T23:59:59.000Z

68

Edinburgh Research Explorer Processivity and Coupling in Messenger RNA Transcription  

E-Print Network (OSTI)

Edinburgh Research Explorer Processivity and Coupling in Messenger RNA Transcription Citation and processing that is not captured in the model. Methodology: In this paper, we explore the impact on the m, 'Processivity and Coupling in Messenger RNA Transcription' PLoS One, vol 5, no. 1, e8845, pp. 1-12., 10

Millar, Andrew J.

69

Super Building Insulation by CO2 Foaming Process Research Project |  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

Emerging Technologies » Super Building Insulation by CO2 Foaming Emerging Technologies » Super Building Insulation by CO2 Foaming Process Research Project Super Building Insulation by CO2 Foaming Process Research Project The Department of Energy is currently researching the development of building superinsulation through a carbon dioxide (CO2) foaming process. Project Description This project seeks to develop building super insulation through a carbon dioxide foaming process that does not use hydrofluorocarbons (HFCs), and which produces insulation with a high R-value. Project Partners Research is being undertaken between the Department of Energy and The Industrial Science & Technology Network. Project Goals The goal of this project is to develop advanced insulation without HFC, and to achieve a competitive processing cost for CO2 foaming technology.

70

Characterizing the formation of secondary organic aerosols  

SciTech Connect

Organic aerosol is an important fraction of the fine particulate matter present in the atmosphere. This organic aerosol comes from a variety of sources; primary organic aerosol emitted directly from combustion process, and secondary aerosol formed in the atmosphere from condensable vapors. This secondary organic aerosol (SOA) can result from both anthropogenic and biogenic sources. In rural areas of the United States, organic aerosols can be a significant part of the aerosol load in the atmosphere. However, the extent to which gas-phase biogenic emissions contribute to this organic load is poorly understood. Such an understanding is crucial to properly apportion the effect of anthropogenic emissions in these rural areas that are sometimes dominated by biogenic sources. To help gain insight on the effect of biogenic emissions on particle concentrations in rural areas, we have been conducting a field measurement program at the University of California Blodgett Forest Research Facility. The field location includes has been used to acquire an extensive suite of measurements resulting in a rich data set, containing a combination of aerosol, organic, and nitrogenous species concentration and meteorological data with a long time record. The field location was established in 1997 by Allen Goldstein, a professor in the Department of Environmental Science, Policy and Management at the University of California at Berkeley to study interactions between the biosphere and the atmosphere. The Goldstein group focuses on measurements of concentrations and whole ecosystem biosphere-atmosphere fluxes for volatile organic compounds (VOC's), oxygenated volatile organic compounds (OVOC's), ozone, carbon dioxide, water vapor, and energy. Another important collaborator at the Blodgett field location is Ronald Cohen, a professor in the Chemistry Department at the University of California at Berkeley. At the Blodgett field location, his group his group performs measurements of the concentrations of important gas phase nitrogen compounds. Experiments have been ongoing at the Blodgett field site since the fall of 2000, and have included portions of the summer and fall of 2001, 2002, and 2003. Analysis of both the gas and particle phase data from the year 2000 show that the particle loading at the site correlates with both biogenic precursors emitted in the forest and anthropogenic precursors advected to the site from Sacramento and the Central Valley of California. Thus the particles at the site are affected by biogenic processing of anthropogenic emissions. Size distribution measurements show that the aerosol at the site has a geometric median diameter of approximately 100 nm. On many days, in the early afternoon, growth of nuclei mode particles (<20 nm) is also observed. These growth events tend to occur on days with lower average temperatures, but are observed throughout the summer. Analysis of the size resolved data for these growth events, combined with typical measured terpene emissions, show that the particle mass measured in these nuclei mode particles could come from oxidation products of biogenic emissions, and can serve as a significant route for SOA partitioning into the particle phase. During periods of each year, the effect of emissions for forest fires can be detected at the Blodgett field location. During the summer of 2002 emissions from the Biscuit fire, a large fire located in Southwest Oregon, was detected in the aerosol data. The results show that increases in particle scattering can be directly related to increased black carbon concentration and an appearance of a larger mode in the aerosol size distribution. These results show that emissions from fires can have significant impact on visibility over large distances. The results also reinforce the view that forest fires can be a significant source of black carbon in the atmosphere, which has important climate and visibility. Continuing work with the 2002 data set, particularly the combination of the aerosol and gas phase data, will continue to provide important information o

Lunden, Melissa; Black, Douglas; Brown, Nancy

2004-02-01T23:59:59.000Z

71

Time-and size-resolved chemical composition of submicron particles in Pittsburgh: Implications for aerosol sources and processes  

E-Print Network (OSTI)

Time- and size-resolved chemical composition of submicron particles in Pittsburgh: Implications), Time- and size-resolved chemical composition of submicron particles in Pittsburgh: Implications] Atmospheric aerosols have important adverse impacts on human health [Dockery et al., 1993; Pope et al., 2002

Jimenez, Jose-Luis

72

Atomic Collision Processes in Magnetic Confinement Controlled Thermonuclear Fusion Research  

Science Journals Connector (OSTI)

This NATO Advanced Study Institute is concerned with atomic and molecular processes in controlled thermonuclear fusion research. Most of our attention will be ... and planned tokamaks, since this approach to fusion

M. R. C. McDowell

1980-01-01T23:59:59.000Z

73

Northwestern University Facility for Clean Catalytic Process Research  

SciTech Connect

Northwestern University with DOE support created a Facility for Clean Catalytic Process Research. This facility is designed to further strengthen our already strong catalysis research capabilities and thus to address these National challenges. Thus, state-of-the art instrumentation and experimentation facility was commissioned to add far greater breadth, depth, and throughput to our ability to invent, test, and understand catalysts and catalytic processes, hence to improve them via knowledge-based design and evaluation approaches.

Marks, Tobin Jay [Northwestern University

2013-05-08T23:59:59.000Z

74

DOE - Office of Legacy Management -- Processes Research Inc - OH 44  

Office of Legacy Management (LM)

Processes Research Inc - OH 44 Processes Research Inc - OH 44 FUSRAP Considered Sites Site: PROCESSES RESEARCH, INC (OH.44) Eliminated from consideration under FUSRAP Designated Name: Not Designated Alternate Name: None Location: 2905 Vernon Place , Cincinnati , Ohio OH.44-1 Evaluation Year: 1991 OH.44-2 OH.44-3 Site Operations: Research and development of machining methods during the early 1950s; no indication of involvement with radioactive materials. OH.44-1 OH.44-3 Site Disposition: Eliminated - Potential for contamination considered remote based on nature of operations at the site OH.44-2 Radioactive Materials Handled: None Indicated Primary Radioactive Materials Handled: None OH.44-3 Radiological Survey(s): No Site Status: Eliminated from consideration under FUSRAP

75

NREL: Photovoltaics Research - New Materials, Devices, and Processes for  

NLE Websites -- All DOE Office Websites (Extended Search)

New Materials, Devices, and Processes for Advanced Concepts New Materials, Devices, and Processes for Advanced Concepts Computational Science and Theory We can use high-performance computing tools in modeling and simulation studies of semiconductor and other solar materials. We also determine the performance of solar devices. Theoretical studies can help us understand underlying physical principles or predict useful chemical compositions and crystalline structures. Scientific Computing Experimental Materials Science Solid-State Theory. NREL has strong complementary research capabilities in organic photovoltaic (OPV) cells, transparent conducting oxides (TCOs), combinatorial (combi) methods, and atmospheric processing. From fundamental physical studies to applied research relating to solar industry needs, we are developing the

76

NREL: Biomass Research - Projects in Integrated Biorefinery Processes  

NLE Websites -- All DOE Office Websites (Extended Search)

Projects in Integrated Biorefinery Processes Projects in Integrated Biorefinery Processes A photo of a control room with four large computer screens. A man and a woman are looking at the screens. The Thermochemical Process Development Unit is equipped with sophisticated process monitoring and operation control systems. NREL is focused on integrating all the biomass conversion unit operations. With extensive knowledge of the individual unit operations, NREL is well-positioned to link these operations together at the mini-pilot and pilot scales. Among the integrated biorefinery projects are: Sorghum to Ethanol Research Initiative Sorghum shows promising characteristics as a feedstock for biofuel production. However, little basic research data exists. NREL is performing integrated research on sorghum by studying it at every step along the

77

E-Print Network 3.0 - aerosols harbor diverse Sample Search Results  

NLE Websites -- All DOE Office Websites (Extended Search)

Cloud & Aerosol Process Group CSDESRLNOAA Presented at: NIST... Aerosol Metrology for Climate Workshop 15th March, 2011 12;Deposition Snow Darkens and Warms BC...

78

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Lord of the Wings: Elevated Particles a Rising Star Lord of the Wings: Elevated Particles a Rising Star Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Kassianov E, C Flynn, J Redemann, B Schmid, PB Russell, and A Sinyuk. 2012. "Initial assessment of the Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR)-based aerosol retrieval: Sensitivity study." Atmosphere, 3, doi:10.3390/atmos3040495. The 4STAR instrument. The 4STAR instrument (inset) is installed through the upper hull of the PNNL G-1 research aircraft, for in-flight sun-tracking and sky light-scanning. Researchers at Pacific Northwest National Laboratory, in collaboration with colleagues at NASA Ames Research Center, developed a next-generation

79

NREL: Biomass Research - Projects in Biomass Process and Sustainability  

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Projects in Biomass Process and Sustainability Analyses Projects in Biomass Process and Sustainability Analyses Researchers at NREL use biomass process and sustainability analyses to understand the economic, technical, and global impacts of biomass conversion technologies. These analyses reveal the economic feasibility and environmental benefits of biomass technologies and are useful for government, regulators, and the private sector. NREL's Energy Analysis Office integrates and supports the energy analysis functions at NREL. Among NREL's projects in biomass process and sustainability analyses are: Life Cycle Assessment of Energy Independence and Security Act for Ethanol NREL is determining the life cycle environmental impacts of the ethanol portion of the Energy Independence and Security Act (EISA). EISA mandates

80

Research Highlight  

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First Observation-Based Estimates of Cloud-Free Aerosol Radiative Forcing First Observation-Based Estimates of Cloud-Free Aerosol Radiative Forcing Across China Download a printable PDF Submitter: Li, Z., University of Maryland Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: N/A Mean annual shortwave aerosol radiative forcing (SWARF) averaged across China. Spatial variation of the annual mean SW aerosol radiative forcing. Heavy loading of aerosols in China is widely known, but little is known about their impact on regional radiation budgets, which is often expressed as aerosol radiative forcing (ARF). Depending on their composition, aerosols can absorb a substantial amount of solar radiation, leading to a warming of the atmosphere and cooling of the surface. Many investigations have been made to characterize atmospheric aerosols and their radiative

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


81

Research Highlight  

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Aerosol Experiment Results Featured in Technical Journal Aerosol Experiment Results Featured in Technical Journal Submitter: Sheridan, P., U.S. Department of Commerce/NOAA Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Sheridan, P, W Arnott, J Ogren, E Andrews, D Atkinson, D Covert, H Moosmuller, A Petzold, B Schmid, A Strawa, R Varma, and A Virkkula. 2005. "The Reno Aerosol Optics Study: An evaluation of aerosol absorption measurement methods." Aerosol Science and Technology 39(1):1-16. This magnification shows the size of aerosol particles relative to the pore size of the filter used during one of the study's sampling runs. Aerosol particles are gaining increasing scientific attention as a key factor in climate change. Through scattering and absorption of solar radiation, or by altering cloud properties, aerosols have the potential to

82

Evidence that the spectral dependence of light absorption by aerosols is  

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Evidence that the spectral dependence of light absorption by aerosols is Evidence that the spectral dependence of light absorption by aerosols is affected by organic carbon Title Evidence that the spectral dependence of light absorption by aerosols is affected by organic carbon Publication Type Journal Article LBNL Report Number LBNL-55056 Year of Publication 2004 Authors Kirchstetter, Thomas W., Tihomir Novakov, and Peter V. Hobbs Journal Journal of Geophysical Research: Atmospheres Volume 109 Issue D21 Keywords aerosol light absorption, biomass burning, organic carbon Abstract The wavelength dependence of light absorption by aerosols collected on filters is investigated throughout the near-ultraviolet to near-infrared spectral region. Measurements were made using an optical transmission method. Aerosols produced by biomass combustion, including wood and savanna burning, and by motor vehicles, including diesel trucks, are included in the analysis. These aerosol types were distinguished by different wavelength (λ) dependences in light absorption. Light absorption by the motor vehicle aerosols exhibited relatively weak wavelength dependence; absorption varied approximately as λ-1, indicating that black carbon (BC) was the dominant absorbing aerosol component. By contrast, the biomass smoke aerosols had much stronger wavelength dependence, approximately λ-2. The stronger spectral dependence was the result of enhanced light absorption at wavelengths shorter than 600 nm and was largely reduced when much of the sample organic carbon (OC) was extracted by dissolution in acetone. This indicates that OC in addition to BC in the biomass smoke aerosols contributed significantly to measured light absorption in the ultraviolet and visible spectral regions and that OC in biomass burning aerosols may appreciably absorb solar radiation. Estimated absorption efficiencies and imaginary refractive indices are presented for the OC extracted from biomass burning samples and the BC in motor vehicle-dominated aerosol samples. The uncertainty of these constants is discussed. Overall, results of this investigation show that low-temperature, incomplete combustion processes, including biomass burning, can produce light-absorbing aerosols that exhibit much stronger spectral dependence than high-temperature combustion processes, such as diesel combustion.

83

Research Highlight  

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Spectrally Invariant Approximation Within Atmospheric Radiative Transfer Spectrally Invariant Approximation Within Atmospheric Radiative Transfer Download a printable PDF Submitter: Marshak, A., NASA - Goddard Space Flight Center Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Marshak A, Y Knyazikhin, JC Chiu, and WJ Wiscombe. 2011. "Spectrally-invariant approximation within atmospheric radiative transfer." Journal of the Atmospheric Sciences, 68(12), doi:10.1175/JAS-D-11-060.1. Ratio of reflectance Rλ plus transmittance Tλ over single scattering albedo ω0λ plotted against the sum Rλ+Tλ for two cloud optical depths: 5 and 10. The aerosol optical depth at 0.55 μm is 0.2 (rural type of aerosol). Different dots correspond to different wavelengths from 0.4 to

84

Research Highlight  

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Exploring Parameterization for Turbulent Entrainment-Mixing Processes in Exploring Parameterization for Turbulent Entrainment-Mixing Processes in Clouds Download a printable PDF Submitter: Liu, Y., Brookhaven National Laboratory Lu, C., Brookhaven National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Lu C, S Niu, S Krueger, and T Wagner. 2013. "Exploring parameterization for turbulent entrainment-mixing processes in clouds." Journal of Geophysical Research - Atmospheres, 118(1), doi:10.1029/2012JD018464. Relationships between the three microphysical measures of homogeneous mixing degree (ψ1, ψ2, ψ3) and the two transition scale numbers (NLa, NL0), respectively. The results shown here are from the EMPM simulations.

85

The Wool Industries Research Association: New Laboratories for Worsted Processing  

Science Journals Connector (OSTI)

... THE new Worsted Processing Block at Torridon, the Leeds headquarters of the Wool Industries Research Association, was opened by the Right Hon. R. G. Menzies, ... been very active in the Association's affairs since 1929, particularly in the field of scouring and combing, and also in that of finance-an impor tant aspect when new ...

H. LEMON

1961-04-22T23:59:59.000Z

86

NREL: Biomass Research - Capabilities in Biomass Process and Sustainability  

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Capabilities in Biomass Process and Sustainability Analyses Capabilities in Biomass Process and Sustainability Analyses A photo of a woman and four men, all wearing hard hats and looking into a large square bin of dried corn stover. One man is using a white scoop to pick up some of the material and another man holds some in his hand. Members of Congress visit NREL's cellulosic ethanol pilot plant. A team of NREL researchers uses biomass process and sustainability analyses to bridge the gap between research and commercial operations, which is critical for the scale-up of biomass conversion technology. Among NREL's biomass analysis capabilities are: Life cycle assessments Technoeconomic analysis Sensitivity analysis Strategic analysis. Life Cycle Assessments Conducting full life cycle assessments is important for determining the

87

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Raman Lidar Observations of Aerosol Humidification Near Clouds Raman Lidar Observations of Aerosol Humidification Near Clouds Submitter: Ferrare, R. A., NASA - Langley Research Center Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Ferrare, R., et al., Evaluation of Daytime Measurements of Aerosols and Water Vapor Made by an Operational Raman Lidar over the Southern Great Plains, J. Geophys. Res., 111, D05S08, doi:10.1029/2005JD005836, 2006. Relative humidity profiles derived from the Raman lidar during the ALIVE 2005 field experiment. Aerosol extinction profiles derived from the Raman lidar during the ALIVE 2005 field experiment. Aerosol humidification factor f(RH) from Raman lidar measured profiles of aerosol extinction and relative humidity. Upgrades to the Raman lidar at the ARM Climate Research Facility (ACRF)

88

Coal liquefaction process research quarterly report, October-December 1979  

SciTech Connect

This quarterly report summarizes the activities of Sandia's continuing program in coal liquefaction process research. The overall objectives are to: (1) provide a fundamental understanding of the chemistry of coal liquefaction; (2) determine the role of catalysts in coal liquefaction; and (3) determine the mechanism(s) of catalyst deactivation. The program is composed of three major projects: short-contact-time coal liquefaction, mineral effects, and catalyst studies. These projects are interdependent and overlap significantly.

Bickel, T.C.; Curlee, R.M.; Granoff, B.; Stohl, F.V.; Thomas, M.G.

1980-03-01T23:59:59.000Z

89

Spectro-microscopic Measurements of Carbonaceous Aerosol Aging in Central California  

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Spectro-microscopic Measurements of Carbonaceous Spectro-microscopic Measurements of Carbonaceous Aerosol Aging in Central California For original submission and image(s), see ARM Research Highlights http://www.arm.gov/science/highlights/ Research Highlight Atmospheric aerosols affect climate by scattering and absorbing sunlight and by modifying the properties of clouds. However, there are gaps in our understanding of chemical processes involving these airborne particulates, and these gaps contribute significantly to uncertainties in predicting future climate change. Developing more- accurate global climate models requires a more complete understanding of the aerosol lifecycle, from initial particle formation to loss through incorporation into precipitating clouds or dry deposition. In research published in the journal Atmospheric Chemistry and Physics, a team of

90

Oil shale, tar sand, coal research, advanced exploratory process technology, jointly sponsored research  

SciTech Connect

Progress made in five research programs is described. The subtasks in oil shale study include oil shale process studies and unconventional applications and markets for western oil shale.The tar sand study is on recycle oil pyrolysis and extraction (ROPE) process. Four tasks are described in coal research: underground coal gasification; coal combustion; integrated coal processing concepts; and sold waste management. Advanced exploratory process technology includes: advanced process concepts; advanced mitigation concepts; and oil and gas technology. Jointly sponsored research covers: organic and inorganic hazardous waste stabilization; CROW field demonstration with Bell Lumber and Pole; development and validation of a standard test method for sequential batch extraction fluid; PGI demonstration project; operation and evaluation of the CO[sub 2] HUFF-N-PUFF process; fly ash binder for unsurfaced road aggregates; solid state NMR analysis of Mesaverde group, Greater Green River Basin, tight gas sands; flow-loop testing of double-wall pipe for thermal applications; shallow oil production using horizontal wells with enhanced oil recovery techniques; NMR analysis of sample from the ocean drilling program; and menu driven access to the WDEQ hydrologic data management system.

Not Available

1992-01-01T23:59:59.000Z

91

FY 2011 Second Quarter: Demonstration of New Aerosol Measurement Verification Testbed for Present-Day Global Aerosol Simulations  

SciTech Connect

The regional-scale Weather Research and Forecasting (WRF) model is being used by a DOE Earth System Modeling (ESM) project titled Improving the Characterization of Clouds, Aerosols and the Cryosphere in Climate Models to evaluate the performance of atmospheric process modules that treat aerosols and aerosol radiative forcing in the Arctic. We are using a regional-scale modeling framework for three reasons: (1) It is easier to produce a useful comparison to observations with a high resolution model; (2) We can compare the behavior of the CAM parameterization suite with some of the more complex and computationally expensive parameterizations used in WRF; (3) we can explore the behavior of this parameterization suite at high resolution. Climate models like the Community Atmosphere Model version 5 (CAM5) being used within the Community Earth System Model (CESM) will not likely be run at mesoscale spatial resolutions (1020 km) until 510 years from now. The performance of the current suite of physics modules in CAM5 at such resolutions is not known, and current computing resources do not permit high-resolution global simulations to be performed routinely. We are taking advantage of two tools recently developed under PNNL Laboratory Directed Research and Development (LDRD) projects for this activity. The first is the Aerosol Modeling Testbed (Fast et al., 2011b), a new computational framework designed to streamline the process of testing and evaluating aerosol process modules over a range of spatial and temporal scales. The second is the CAM5 suite of physics parameterizations that have been ported into WRF so that their performance and scale dependency can be quantified at mesoscale spatial resolutions (Gustafson et al., 2010; with more publications in preparation).

Koch, D

2011-03-20T23:59:59.000Z

92

Assessing regional scale predictions of aerosols, marine stratocumulus, and their interactions during VOCALS-REx using WRF-Chem  

SciTech Connect

This study assesses the ability of the recent chemistry version (v3.3) of the Weather Research and Forecasting (WRF-Chem) model to simulate boundary layer structure, aerosols, stratocumulus clouds, and energy fluxes over the Southeast Pacific Ocean. Measurements from the VAMOS Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-REx) and satellite retrievals (i.e., products from the MODerate resolution Imaging Spectroradiometer (MODIS), Clouds and Earth's Radiant Energy System (CERES), and GOES-10) are used for this assessment. The Morrison double-moment microphysics scheme is newly coupled with interactive aerosols in the model. The 31-day (15 October-16 November 2008) WRF-Chem simulation with aerosol-cloud interactions (AERO hereafter) is also compared to a simulation (MET hereafter) with fixed cloud droplet number concentrations in the microphysics scheme and simplified cloud and aerosol treatments in the radiation scheme. The well-simulated aerosol quantities (aerosol number, mass composition and optical properties), and the inclusion of full aerosol-cloud couplings lead to significant improvements in many features of the simulated stratocumulus clouds: cloud optical properties and microphysical properties such as cloud top effective radius, cloud water path, and cloud optical thickness. In addition to accounting for the aerosol direct and semi-direct effects, these improvements feed back to the simulation of boundary-layer characteristics and energy budgets. Particularly, inclusion of interactive aerosols in AERO strengthens the temperature and humidity gradients within the capping inversion layer and lowers the marine boundary layer (MBL) depth by 130 m from that of the MET simulation. These differences are associated with weaker entrainment and stronger mean subsidence at the top of the MBL in AERO. Mean top-of-atmosphere outgoing shortwave fluxes, surface latent heat, and surface downwelling longwave fluxes are in better agreement with observations in AERO, compared to the MET simulation. Nevertheless, biases in some of the simulated meteorological quantities (e.g., MBL temperature and humidity) and aerosol quantities (e.g., underestimations of accumulation mode aerosol number) might affect simulated stratocumulus and energy fluxes over the Southeastern Pacific, and require further investigation. The well-simulated timing and outflow patterns of polluted and clean episodes demonstrate the model's ability to capture daily/synoptic scale variations of aerosol and cloud properties, and suggest that the model is suitable for studying atmospheric processes associated with pollution outflow over the ocean. The overall performance of the regional model in simulating mesoscale clouds and boundary layer properties is encouraging and suggests that reproducing gradients of aerosol and cloud droplet concentrations and coupling cloud-aerosol-radiation processes are important when simulating marine stratocumulus over the Southeast Pacific.

Yang Q.; Lee Y.; GustafsonJr., W. I.; Fast, J. D.; Wang, H.; Easter, R. C.; Morrison, H.; Chapman, E. G.; Spak, S. N.; Mena-Carrasco, M. A.

2011-12-02T23:59:59.000Z

93

Time-resolved distributions of bulk parameters, diacids, ketoacids and ?-dicarbonyls and stable carbon and nitrogen isotope ratios of TC and TN in tropical Indian aerosols: Influence of land/sea breeze and secondary processes  

Science Journals Connector (OSTI)

Abstract To better understand the photochemical production and diurnal distributions of organic and inorganic aerosols in the tropical coastal Indian atmosphere, the aerosol (TSP) samples were collected every 3h during 3031 January, 1415 February and 2829 May 2007 from Chennai and studied for total carbon (TC) and nitrogen (TN) and their stable isotope ratios (?13CTC and ?15NTN), carbonaceous components, inorganic ions, diacids, ketoacids and ?-dicarbonyls. Time-resolved distributions of bulk parameters, inorganic ions, and diacids and related compounds, except for few species, did not show any clear diurnal trend but showed peaks at 69h during all the study periods, except for the peak at 1518h on 28 May. SO42?, C2?C6 diacids, ketoacids and ?-dicarbonyls in February and on 29 May showed a diurnal trend. ?13CTC and ?15NTN stayed relatively constant during the study periods but showed 13C depletion (in January) and 15N enrichment when TC and TN peaked. Based on these results together with air mass trajectories, we found that the diurnal distributions of Chennai aerosols are mainly influenced by land/sea breeze and the aged (photochemically processed) air masses, although in situ photochemical production and nighttime chemistry of secondary aerosol species, particularly C2C4 diacids and SO42?, are significant. The characteristics of seasonal variations of carbonaceous components, and diacids and related compounds and comparisons of ?13CTC and ?15NTN of Chennai aerosols with the isotopic signatures of the point sources inferred that biofuel/biomass burning in South and Southeast Asia are the major sources of aerosols (TSP).

Chandra Mouli Pavuluri; Kimitaka Kawamura; T. Swaminathan

2015-01-01T23:59:59.000Z

94

2004 research briefs :Materials and Process Sciences Center.  

SciTech Connect

This report is the latest in a continuing series that highlights the recent technical accomplishments associated with the work being performed within the Materials and Process Sciences Center. Our research and development activities primarily address the materials-engineering needs of Sandia's Nuclear-Weapons (NW) program. In addition, we have significant efforts that support programs managed by the other laboratory business units. Our wide range of activities occurs within six thematic areas: Materials Aging and Reliability, Scientifically Engineered Materials, Materials Processing, Materials Characterization, Materials for Microsystems, and Materials Modeling and Simulation. We believe these highlights collectively demonstrate the importance that a strong materials-science base has on the ultimate success of the NW program and the overall DOE technology portfolio.

Cieslak, Michael J.

2004-01-01T23:59:59.000Z

95

Investigation of Aerosol Indirect Effects using a Cumulus Microphysics Parameterization in a Regional Climate Model  

SciTech Connect

A new Zhang and McFarlane (ZM) cumulus scheme includes a two-moment cloud microphysics parameterization for convective clouds. This allows aerosol effects to be investigated more comprehensively by linking aerosols with microphysical processes in both stratiform clouds that are explicitly resolved and convective clouds that are parameterized in climate models. This new scheme is implemented in the Weather Research and Forecasting (WRF) model, which is coupled with the physics and aerosol packages from the Community Atmospheric Model version 5 (CAM5). A test case of July 2008 during the East Asian summer monsoon is selected to evaluate the performance of the new ZM scheme and to investigate aerosol effects on monsoon precipitation. The precipitation and radiative fluxes simulated by the new ZM scheme show a better agreement with observations compared to simulations with the original ZM scheme that does not include convective cloud microphysics and aerosol convective cloud interactions. Detailed analysis suggests that an increase in detrained cloud water and ice mass by the new ZM scheme is responsible for this improvement. To investigate precipitation response to increased anthropogenic aerosols, a sensitivity experiment is performed that mimics a clean environment by reducing the primary aerosols and anthropogenic emissions to 30% of that used in the control simulation of a polluted environment. The simulated surface precipitation is reduced by 9.8% from clean to polluted environment and the reduction is less significant when microphysics processes are excluded from the cumulus clouds. Ensemble experiments with ten members under each condition (i.e., clean and polluted) indicate similar response of the monsoon precipitation to increasing aerosols.

Lim, Kyo-Sun; Fan, Jiwen; Leung, Lai-Yung R.; Ma, Po-Lun; Singh, Balwinder; Zhao, Chun; Zhang, Yang; Zhang, Guang; Song, Xiaoliang

2014-01-29T23:59:59.000Z

96

Research Highlight  

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Cloud Susceptibility Measures Potential Cloud Sensitivity to First Aerosol Cloud Susceptibility Measures Potential Cloud Sensitivity to First Aerosol Indirect Effect Download a printable PDF Submitter: Oreopoulos, L., NASA Platnick, S., NASA - Goddard Space Flight Center Area of Research: Cloud Distributions/Characterizations Working Group(s): Radiative Processes Journal Reference: Platnick, S, and L Oreopoulos. 2008. "Radiative susceptibility of cloudy atmospheres to droplet number perturbations: 1. Theoretical analysis and examples from MODIS." Journal of Geophysical Research doi:10.1029/2007JD009654, in press. Oreopoulos, L., and S. Platnick. 2008. Radiative susceptibility of cloudy atmospheres to droplet number perturbations: 2. Global analysis from MODIS, J. Geophys. Res., doi:10.1029/2007JD009655, in press. Theoretical calculations with a shortwave broadband radiative transfer

97

Research Highlight  

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Remote Sensing of Mineral Dust Using AERI Remote Sensing of Mineral Dust Using AERI Download a printable PDF Submitter: Hansell, R. A., University of California, Los Angeles Area of Research: Radiation Processes Working Group(s): Aerosol Journal Reference: Hansell R, KN Liou, SC Ou, SC Tsay, Q Ji, and JS Reid. 2008. "Remote sensing of mineral dust aerosol using AERI during the UAE2: A modeling and sensitivity study." Journal of Geophysical Research - Atmospheres, 113, D18202, doi:10.1029/2008JD010246. BT sensitivity to dust optical depth at 962 cm-1 with markers denoting locations of AERI subbands 1-17 from left to right. (a) Volz compact hexagon model spectra for four optical depths with best fit AERI spectrum. (b) Same as (a) but for a kaolinite/50% calcium carbonate mixturedust model.

98

Research Highlight  

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Measured Radiative Cooling from Reflective Roofs in India Measured Radiative Cooling from Reflective Roofs in India Download a printable PDF Submitter: Fischer, M. L., Lawrence Berkeley National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle, Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Salamanca F, S Tonse, S Menon, V Garg, KP Singh, M Naja, and ML Fischer. 2012. "Top-of-atmosphere radiative cooling with white roofs: Experimental verification and model-based evaluation." Environmental Research Letters, 7(4), 044007, doi:10.1088/1748-9326/7/4/044007. True color image of light (PW1, PW2) and unpainted tar (PD1), and concrete (PD2) roofs at the Pantnagar, India site taken on October 21, 2011. We note that the concrete roof is considerably more reflective than the tar roof

99

Research Highlight  

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Chemical Diffusivity and Viscosity of Secondary Organic Aerosols Download a printable PDF Submitter: Zelenyuk-Imre, A., Pacific Northwest National Laboratory Area of Research:...

100

Research Highlight  

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Y Qian, and JE Penner. 2012. "Constraining cloud lifetime effects of aerosols using A-Train satellite observations." Geophysical Research Letters, 39, L15709, doi: 10.1029...

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


101

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

A., Pacific Northwest National Laboratory Area of Research: Atmospheric Thermodynamics and Vertical Structures Working Group(s): Cloud-Aerosol-Precipitation Interactions...

102

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

of Maryland Sawyer, V. R., University of Maryland Area of Research: Atmospheric Thermodynamics and Vertical Structures Working Group(s): Cloud-Aerosol-Precipitation Interactions...

103

Research Highlight  

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New Insight on the Atmosphere's Tiniest Particles Download a printable PDF Submitter: Smith, J., NCAR McMurry, P. ., University of Minnesota Area of Research: Aerosol Properties...

104

E-Print Network 3.0 - advanced process research Sample Search...  

NLE Websites -- All DOE Office Websites (Extended Search)

computer science, education and scientific research aimed at helping... of the research process. Microsoft ... Source: Narasayya, Vivek - Data Management, Exploration and Mining...

105

Research Highlight  

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Aerosols Help Heat Up the Yangtze River Delta in China Aerosols Help Heat Up the Yangtze River Delta in China Download a printable PDF Submitter: Flynn, C. J., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Liu J, Z Li, Y Zheng, C Flynn, and M Cribb. 2012. "Seasonal variations of aerosol optical properties, vertical distribution and associated radiative effects in the Yangtze Delta region of China." Journal of Geophysical Research, 117, D00K38, doi:10.1029/2011JD016490. A team of scientists found that aerosols significantly alter the vertical profile of solar heating in the central Yangtze River Delta region in eastern China. Aerosols were identified from as far away as Mongolia and Siberia. These findings have considerable implications for atmospheric

106

Research Highlight  

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Invisible Giants in the Sky Invisible Giants in the Sky Download a printable PDF Submitter: Ovink, J., Pacific Northwest National Laboratory Kassianov, E., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Kassianov E, M Pekour, and J Barnard. 2012. "Aerosols in central California: Unexpectedly large contribution of coarse mode to aerosol radiative forcing." Geophysical Research Letters, 39, L20806, doi:10.1029/2012GL053469. Photo courtesy of the U.S. National Park Service Daily averaged values of (a, b) the direct aerosol radiative forcing (DARF) and (c, d) aerosol radiative forcing efficiency at the top-of-atmosphere calculated for the "original" aerosol optical properties (blue) and

107

BNL | Mobile Aerosol Observing System (MAOS)  

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Mobile Aerosol Observing System (MAOS) Mobile Aerosol Observing System (MAOS) The Mobile Aerosol Observing System (MAOS) is a platform and instrument suite for Intensive Operation Periods (IOPs) to conduct in situ measurements of aerosols and their precursors. MAOS is part of the ARM Climate Research Facility. Physically MAOS is contained in two 20' SeaTainers custom adapted to provide a sheltered laboratory environment for operators and instruments even under harsh conditions. The two structures are designated MAOS-A and MAOS-C for Aerosol and Chemistry respectively. Although independent, with separate data systems, inlets and power distribution, the two structures are normally a single operating unit. The two enclosures comprising MAOS are designed for rapid deployment. All components (except for the Radar Wind Profiler) are transported internally

108

Mass Spectral Evidence That Small Changes in Composition Caused by Oxidative Aging Processes Alter Aerosol CCN Properties  

E-Print Network (OSTI)

Mass Spectral Evidence That Small Changes in Composition Caused by Oxidative Aging Processes Alter that small changes in particle chemical composition caused by oxidation could increase the CCN activity increased cloud condensation nuclei (CCN) activity compared to their hydro- phobic counterparts. At present

109

Response of California temperature to regional anthropogenic aerosol  

NLE Websites -- All DOE Office Websites (Extended Search)

Response of California temperature to regional anthropogenic aerosol Response of California temperature to regional anthropogenic aerosol changes Title Response of California temperature to regional anthropogenic aerosol changes Publication Type Journal Article Year of Publication 2008 Authors Novakov, Tihomir, Thomas W. Kirchstetter, Surabi Menon, and Jeffery Aguiar Journal Geophysical Research Letters Volume 35 Issue 19 Abstract In this paper, we compare constructed records of concentrations of black carbon (BC) - an indicator of anthropogenic aerosols - with observed surface temperature trends in California. Annual average BC concentrations in major air basins in California significantly decreased after about 1990, coincident with an observed statewide surface temperature increase. Seasonal aerosol concentration trends are consistent with observed seasonal temperature trends. These data suggest that the reduction in anthropogenic aerosol concentrations contributed to the observed surface temperature increase. Conversely, high aerosol concentrations may lower surface temperature and partially offset the temperature increase of greenhouse gases.

110

RESEARCH ON CARBON PRODUCTS FROM COAL USING AN EXTRACTIVE PROCESS  

SciTech Connect

This report presents the results of a one-year effort directed at the exploration of the use of coal as a feedstock for a variety of industrially-relevant carbon products. The work was basically divided into three focus areas. The first area dealt with the acquisition of laboratory equipment to aid in the analysis and characterization of both the raw coal and the coal-derived feedstocks. Improvements were also made on the coal-extraction pilot plant which will now allow larger quantities of feedstock to be produced. Mass and energy balances were also performed on the pilot plant in an attempt to evaluate the scale-up potential of the process. The second focus area dealt with exploring hydrogenation conditions specifically aimed at testing several less-expensive candidate hydrogen-donor solvents. Through a process of filtration and vacuum distillation, viable pitch products were produced and evaluated. Moreover, a recycle solvent was also isolated so that the overall solvent balance in the system could be maintained. The effect of variables such as gas pressure and gas atmosphere were evaluated. The pitch product was analyzed and showed low ash content, reasonable yield, good coking value and a coke with anisotropic optical texture. A unique plot of coke yield vs. pitch softening point was discovered to be independent of reaction conditions or hydrogen-donor solvent. The third area of research centered on the investigation of alternate extraction solvents and processing conditions for the solvent extraction step. A wide variety of solvents, co-solvents and enhancement additives were tested with varying degrees of success. For the extraction of raw coal, the efficacy of the alternate solvents when compared to the benchmark solvent, N-methyl pyrrolidone, was not good. However when the same coal was partially hydrogenated prior to solvent extraction, all solvents showed excellent results even for extractions performed at room temperature. Standard analyses of the extraction products indicated that they had the requisite properties of viable carbon-product precursors.

Peter G. Stansberry; Alfred H. Stiller; John W. Zondlo; Chong Chen; Brian Bland; David Fenton

2002-03-31T23:59:59.000Z

111

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Laboratory-Measured Optical Properties of Primary Organic Aerosol for Laboratory-Measured Optical Properties of Primary Organic Aerosol for Humidities Up to 95% Download a printable PDF Submitter: Bond, T., University of Illinois, Urbana Rood, M. J., University of Illinois, Urbana Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Brem BT, FC Mena Gonzalez, SR Meyers, TC Bond, and MJ Rood. 2011. "Laboratory-measured optical properties of inorganic and organic aerosols at relative humidities up to 95%." Aerosol Science and Technology, 46(2), doi:10.1080/02786826.2011.617794. Optical properties of the nigrosin benchmark aerosol as a function of relative humidity (RH). Measured extinction (σep) and scattering (σsp) for 467 nm, 530 nm and 660 nm are shown in 1a), 1b) and 1c); calculated

112

Improved solid aerosol generator  

DOE Patents (OSTI)

An improved solid aerosol generator used to produce a gas borne stream of dry, solid particles of predetermined size and concentration. The improved solid aerosol generator nebulizes a feed solution of known concentration with a flow of preheated gas and dries the resultant wet heated aerosol in a grounded, conical heating chamber, achieving high recovery and flow rates. 2 figs.

Prescott, D.S.; Schober, R.K.; Beller, J.

1988-07-19T23:59:59.000Z

113

Investigation of the aerosol-cloud interaction using the WRF framework  

E-Print Network (OSTI)

In this dissertation, a two-moment bulk microphysical scheme with aerosol effects is developed and implemented into the Weather Research and Forecasting (WRF) model to investigate the aerosol-cloud interaction. Sensitivities of cloud properties...

Li, Guohui

2009-05-15T23:59:59.000Z

114

Understanding Brown Carbon Aerosols and Their Role in Climate Change  

NLE Websites -- All DOE Office Websites (Extended Search)

Brown Carbon Aerosols Brown Carbon Aerosols Tiny aerosol particles in the atmosphere are a possible cause of climate change. Among the many contributors to climate change are aerosols in the atmosphere. These tiny particles suspended in the air come from many sources, some natural and some man-made. Some aerosols are organic (containing carbon), while others are inorganic (such as sea salt and sulfates). Most aerosols reflect sunlight, and some also absorb it. Many of these nanoparticles have severe health effects in addition to climate effects. Human activities that produce aerosols include transportation, industry, and agriculture. Black carbon particles (a component of soot) originating from combustion processes have been known for some time to absorb sunlight and warm the

115

Sulfate aerosols and polar stratospheric cloud formation  

SciTech Connect

Before the discovery of the Antarctic ozone hole, it was generally assumed that gas-phase chemical reactions controlled the abundance of stratospheric ozone. However, the massive springtime ozone losses over Antarctica first reported by Farman et al in 1985 could not be explained on the basis of gas-phase chemistry alone. In 1986, Solomon et al suggested that chemical reactions occurring on the surfaces of polar stratospheric clouds (PSCs) could be important for the observed ozone losses. Since that time, an explosion of laboratory, field, and theoretical research in heterogeneous atmospheric chemistry has occurred. Recent work has indicated that the most important heterogeneous reaction on PSCs is ClONO[sub 2] + HCl [yields] Cl[sub 2] + HNO[sub 3]. This reaction converts inert chlorine into photochemically active Cl[sub 2]. Photolysis of Cl[sub 2] then leads to chlorine radicals capable of destroying ozone through very efficient catalytic chain reactions. New observations during the second Airborne Arctic Stratospheric Expedition found stoichiometric loss of ClONO[sub 2] and HCl in air processed by PSCs in accordance with reaction 1. Attention is turning toward understanding what kinds of aerosols form in the stratospheric, their formation mechanism, surface area, and specific chemical reactivity. Some of the latest findings, which underline the importance of aerosols, were presented at a recent National Aeronautics and Space Administration workshop in Boulder, Colorado.

Tolbert, M.A. (Univ. of Colorado, Boulder, CO (United States))

1994-04-22T23:59:59.000Z

116

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

How Aerosols Affect Cloud Properties in Arctic Mixed-Phase Stratocumulus How Aerosols Affect Cloud Properties in Arctic Mixed-Phase Stratocumulus Download a printable PDF Submitter: McFarquhar, G., University of Illinois, Urbana Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Jackson RC, GM McFarquhar, AV Korolev, ME Earle, PS Liu, RP Lawson, S Brooks, M Wolde, A Laskin, and M Freer. 2012. "The dependence of ice microphysics on aerosol concentration in arctic mixed-phase stratus clouds during ISDAC and M-PACE." Journal of Geophysical Research - Atmospheres, 117, D15207, doi:10.1029/2012JD017668. Cloud mean ice crystal concentration Nice(D ≥ 50 micrometers) versus mean aerosol concentration (NPCASP) above cloud for all 41 vertical profiles

117

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Climatology of Aerosol Optical Depth in North-Central Oklahoma: Climatology of Aerosol Optical Depth in North-Central Oklahoma: 1992-2008 Download a printable PDF Submitter: Michalsky, J. J., DOC/NOAA/OAR/ESRL Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Michalsky J, F Denn, C Flynn, G Hodges, P Kiedron, A Koontz, J Schlemmer, and SE Schwartz. 2010. "Climatology of aerosol optical depth in north-central Oklahoma: 1992-2008." Journal of Geophysical Research - Atmospheres, 115, D07203, doi: 10.1029/2009JD012197. Box plots of each complete year\'s daily averaged aerosol optical depth (AOD) at 500 nm. The dark horizontal line in each box plot is the median daily averaged AOD for the year; the top and bottom of the rectangular box spans the middle 50% of the data. The mean values for the year are plotted

118

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Direct Aerosol Forcing: Calculation from Observables and Sensitivities to Direct Aerosol Forcing: Calculation from Observables and Sensitivities to Inputs Download a printable PDF Submitter: McComiskey, A. C., National Oceanic and Atmospheric Administration Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: McComiskey, A, SE Schwartz, B Schmid, H Guan, ER Lewis, P Ricchiazzi, and JA Ogren. 2008. "Direct aerosol forcing: Calculation from observables and sensitivities to inputs." Journal of Geophysical Research 113, D09202, doi:10.1029/2007JD009170. Figure 1. The sensitivity of calculated aerosol direct radiative forcing to input parameters has been examined to determine the consequences of uncertainties in these input parameters on calculated radiative forcing and to identify areas where measurements might be most profitably improved. Input

119

Laboratory and field testing of an aerosol-based duct-sealing technology  

NLE Websites -- All DOE Office Websites (Extended Search)

Laboratory and field testing of an aerosol-based duct-sealing technology Laboratory and field testing of an aerosol-based duct-sealing technology for large commercial buildings. Title Laboratory and field testing of an aerosol-based duct-sealing technology for large commercial buildings. Publication Type Journal Article LBNL Report Number LBNL-44220 Year of Publication 2002 Authors Carrié, François Rémi, Ronnen M. Levinson, Tengfang T. Xu, Darryl J. Dickerhoff, William J. Fisk, Jennifer A. McWilliams, Mark P. Modera, and Duo Wang Journal ASHRAE Transactions Start Page Chapter Date Published January 2002 Abstract Laboratory and field experiments were performed to evaluate the feasibility of sealing leaks in commercial duct systems with an aerosol sealant. The method involves blowing an aerosol through the duct system to seal the leaks from the inside, the principle being that the aerosol particles deposit in the cracks as they try to escape under pressure. It was shown that the seals created with the current sealant material can withstand pressures far in excess of what is found in commercial-building duct systems. We also performed two field experiments in two large-commercial buildings. The ASHRAE leakage classes of the systems were reduced from 653 down to 103, and from 40 down to 3. Methods and devices specifically devised for this application proved to be very efficient at (a) increasing the sealing rate and (b) attaining state-of-the-art duct leakage classes. Additional research is needed to improve the aerosol injection and delivery processes.

120

Spectro-Microscopic Measurements of Carbonaceous Aerosol Aging in Central California  

SciTech Connect

Carbonaceous aerosols are responsible for large uncertainties in climate models, degraded visibility, and adverse health effects. The Carbonaceous Aerosols and Radiative Effects Study (CARES) was designed to study carbonaceous aerosols in the natural environment of Central Valley, California, and learn more about their atmospheric formation and aging. This paper presents results from spectro-microscopic measurements of carbonaceous particles collected during CARES at the time of pollution accumulation event (June 27-29, 2010), when in situ measurements indicated an increase in the organic carbon content of aerosols as the Sacramento urban plume aged. Computer controlled scanning electron microscopy coupled with an energy dispersive X-ray detector (CCSEM/EDX) and scanning transmission X-ray microscopy coupled with near edge X-ray absorption spectroscopy (STXM/NEXAFS) were used to probe the chemical composition and morphology of individual particles. It was found that the mass of organic carbon on individual particles increased through condensation of secondary organic aerosol. STXM/NEXAFS indicated that the number fraction of homogenous organic particles lacking inorganic inclusions (greater than ~50 nm diameter) increased with plume age as did the organic mass per particle. Comparison of the CARES spectro-microscopic data set with a similar dataset obtained in Mexico City during the MILAGRO campaign showed that individual particles in Mexico City contained twice as much carbon as those sampled during CARES. The number fraction of soot particles at the Mexico City urban site (30%) was larger than at the CARES urban site (10%) and the most aged samples from CARES contained less carbon-carbon double bonds. Differences between carbonaceous particles in Mexico City and California result from different sources, photochemical conditions, gas phase reactants, and secondary organic aerosol precursors. The detailed results provided by these spectro-microscopic measurements will allow for a comprehensive evaluation of aerosol process models used in climate research.

Moffet, Ryan C.; Rodel, Tobias; Kelly, Stephen T.; Yu, Xiao-Ying; Carroll, Gregory; Fast, Jerome D.; Zaveri, Rahul A.; Laskin, Alexander; Gilles, Mary K.

2013-10-29T23:59:59.000Z

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


121

Empirical research in business process management: introduction to the special issue  

E-Print Network (OSTI)

of BPM lies in its promise to create sustainable high-performing processes that demonstrate strategicEDITORIAL Empirical research in business process management: introduction to the special issue Jan with an introduction to Business Process Management and the challenges of empirical research in this field. We

Wieringa, Roel

122

Cloud Scavenging Effects on Aerosol Radiative and Cloud-nucleating Properties - Final Technical Report  

SciTech Connect

The optical properties of aerosol particles are the controlling factors in determining direct aerosol radiative forcing. These optical properties depend on the chemical composition and size distribution of the aerosol particles, which can change due to various processes during the particles lifetime in the atmosphere. Over the course of this project we have studied how cloud processing of atmospheric aerosol changes the aerosol optical properties. A counterflow virtual impactor was used to separate cloud drops from interstitial aerosol and parallel aerosol systems were used to measure the optical properties of the interstitial and cloud-scavenged aerosol. Specifically, aerosol light scattering, back-scattering and absorption were measured and used to derive radiatively significant parameters such as aerosol single scattering albedo and backscatter fraction for cloud-scavenged and interstitial aerosol. This data allows us to demonstrate that the radiative properties of cloud-processed aerosol can be quite different than pre-cloud aerosol. These differences can be used to improve the parameterization of aerosol forcing in climate models.

Ogren, John A.; Sheridan, Patrick S.; Andrews, Elisabeth

2009-03-05T23:59:59.000Z

123

REPRESENTING AEROSOL DYNAMICS AND PROPERTIES IN CHEMICAL TRANSPORT MODELS BY THE METHOD OF MOMENTS  

E-Print Network (OSTI)

understanding of the key processes that govern the aerosol size distribution: · Gas-to-particle conversion--conversion, suspensions of solid or liquid particles, are an important multi- phase system. Aerosols scatter and absorb retrospectively and prospectively for different emissions scenarios. Important aerosol properties and processes

124

JOURNAL OF GEOPHYSICAL RESEARCH, VOL. 102, NO. D24, PAGES 29,737-29,745, DECEMBER 26, 1997 Atmospheric aerosol and water vapor characteristics over north  

E-Print Network (OSTI)

Atmospheric aerosol and water vapor characteristics over north central Canada during BOREAS B. L. Markham, J typically0.09 and 0.34 cm, respectively.Size distributionsderivedfrom solar almucantarmeasurementsshowtheHughesSTXCorporation,Greenbelt,Maryland. 2Formerlyat HSTX/GSFC-NASA,Greenbelt,Maryland. Copyright1997by the American

125

THE EFFECTS OF FLAME TEMPERATURE, PARTICLE SIZE AND EUROPIUM DOPING CONCENTRATION ON THE PROPERTIES OF Y2O3:EU PARTICLES FORMED IN A FLAME AEROSOL PROCESS  

E-Print Network (OSTI)

ix LIST OF FIGURES FIGURE Page 1 Schematic of flame spray pyrolysis apparatus... 2 O 3 :Eu 9, 10 . A number of methods may be used to synthesize Y 2 O 3 :Eu particles, including colloidal methods 11-13 , combustion in fuel-oxidizer mixture 14 , evaporation? condensation 15, 16 , furnace spray pyrolysis 17 . Flame aerosol...

Yim, Hoon

2010-07-14T23:59:59.000Z

126

CHASER: An Innovative Satellite Mission Concept to Measure the Effects of Aerosols on Clouds and Climate  

E-Print Network (OSTI)

The formation of cloud droplets on aerosol particles, technically known as the activation of cloud condensation nuclei (CCN), is the fundamental process driving the interactions of aerosols with clouds and precipitation. ...

Rosenfeld, Daniel

127

Aerosol-Based Duct Sealing Technology  

NLE Websites -- All DOE Office Websites (Extended Search)

8 8 Aerosol-Based Duct Sealing Technology During the past five years, research has quantified the impacts of residential duct system leakage on HVAC energy consumption and peak electricity demand. A typical house with ducts located in the attic or crawlspace wastes approximately 20% of heating and cooling energy through duct leaks and draws approximately 0.5 KW more electricity during peak cooling periods. A 1991 study indicated that sealing leaks could save close to one Quadrillion Btus per year. (see also Commercializing a New Technology) Because the major cost of sealing leaks in existing air distribution systems is the labor for the location and sealing process, reducing the labor could greatly improve the cost-effectiveness of such a retrofit. Field studies of duct sealing programs performed by HVAC contractors show

128

Aerosol Best Estimate Value-Added Product  

SciTech Connect

The objective of the Aerosol Best Estimate (AEROSOLBE) value-added product (VAP) is to provide vertical profiles of aerosol extinction, single scatter albedo, asymmetry parameter, and Angstroem exponents for the atmospheric column above the Central Facility at the ARM Southern Great Plains (SGP) site. We expect that AEROSOLBE will provide nearly continuous estimates of aerosol optical properties under a range of conditions (clear, broken clouds, overcast clouds, etc.). The primary requirement of this VAP was to provide an aerosol data set as continuous as possible in both time and height for the Broadband Heating Rate Profile (BBHRP) VAP in order to provide a structure for the comprehensive assessment of our ability to model atmospheric radiative transfer for all conditions. Even though BBHRP has been completed, AEROSOLBE results are very valuable for environmental, atmospheric, and climate research.

Flynn, C; Turner, D; Koontz, A; Chand, D; Sivaraman, C

2012-07-19T23:59:59.000Z

129

Atmospheric Aerosol Chemistry Analyzer: Demonstration of feasibility  

SciTech Connect

This is the final report of a three-year, Laboratory-Directed Research and Development (LDRD) project at the Los Alamos National Laboratory (LANL). The project objective was to demonstrate the technical feasibility of an Atmospheric Aerosol Chemistry Analyzer (AACA) that will provide a continuous, real-time analysis of the elemental (major, minor and trace) composition of atmospheric aerosols. The AACA concept is based on sampling the atmospheric aerosol through a wet cyclone scrubber that produces an aqueous suspension of the particles. This suspension can then be analyzed for elemental composition by ICP/MS or collected for subsequent analysis by other methods. The key technical challenge was to develop a wet cyclone aerosol sampler suitable for respirable particles found in ambient aerosols. We adapted an ultrasonic nebulizer to a conventional, commercially available, cyclone aerosol sampler and completed collection efficiency tests for the unit, which was shown to efficiently collect particles as small as 0.2 microns. We have completed the necessary basic research and have demonstrated the feasibility of the AACA concept.

Mroz, E.J.; Olivares, J.; Kok, G.

1996-04-01T23:59:59.000Z

130

Research Needs and Priorities for Textile Process Electrification  

E-Print Network (OSTI)

," Final Report for RP1275-10, Electric Power Research Institute, Energy Management and Utilization Division, Industrial Applications Program, August, 1982. (5) Brandon, C. A. and Samfield, M., "Application of High-Temperature Hyperfiltration to Unit...

Hendrix, W. A.

1983-01-01T23:59:59.000Z

131

Climate impacts of carbonaceous and other non-sulfate aerosols: A proposed study  

SciTech Connect

In addition to sulfate aerosols, carbonaceous and other non-sulfate aerosols are potentially significant contributors to global climate change. We present evidence that strongly suggests that current assessments of the effects of aerosols on climate may be inadequate because major aerosol components, especially carbonaceous aerosols, are not included in these assessments. Although data on the properties and distributions of anthropogenic carbonaceous aerosols are insufficient to allow quantification of their climate impacts, the existing information suggests that climate forcing by this aerosol component may be significant and comparable to that by sulfate aerosols. We propose that a research program be undertaken to support a quantitative assessment of the role in climate forcing of non-sulfate, particularly carbonaceous, aerosols.

Andreae, M.O.; Crutzen, P.J. [Max Planck Institute for Chemistry, Mainz (Germany); Cofer, W.R. III; Hollande, J.M. [NASA Langley Research Center, Hampton, VA (United States). Atmospheric Sciences Division] [and others

1995-06-01T23:59:59.000Z

132

BNL | Two-Column Aerosol Program (TCAP)  

NLE Websites -- All DOE Office Websites (Extended Search)

Two-Column Aerosol Project (TCAP) Two-Column Aerosol Project (TCAP) There remain many key knowledge gaps despite advances in the scientific understanding of how aerosols and clouds evolve and affect climate. Many climatically important processes depend on particles that undergo continuous changes within a size range spanning a few nanometers to a few microns, and with compositions that consist of a variety of carbonaceous materials, soluble inorganic salts and acids and insoluble mineral dust. Primary particles, which are externally-mixed when emitted, are subject to coagulation and chemical changes associated with the condensation of semi-volatile gases to their surface resulting in a spectrum of compositions or mixing-states with a range of climate-affecting optical and hygroscopic properties. The numerical treatments of aerosol transformation

133

ARM - Measurement - Aerosol concentration  

NLE Websites -- All DOE Office Websites (Extended Search)

concentration concentration ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol concentration A measure of the amount of aerosol particles (e.g. number, mass, volume) per unit volume of air. Categories Aerosols Instruments The above measurement is considered scientifically relevant for the following instruments. Refer to the datastream (netcdf) file headers of each instrument for a list of all available measurements, including those recorded for diagnostic or quality assurance purposes. ARM Instruments AOS : Aerosol Observing System CSPHOT : Cimel Sunphotometer CPC : Condensation Particle Counter IAP : In-situ Aerosol Profiles (Cessna Aerosol Flights) TDMA : Tandem Differential Mobility Analyzer

134

Indirect and Semi-Direct Aerosol Campaign  

NLE Websites -- All DOE Office Websites (Extended Search)

Campaign Campaign For the month of April, researchers are descending on and above Barrow, Alaska, to obtain data from the atmosphere that will help them understand the impacts that aerosols have on Arctic clouds and climate. Scientists sponsored by the U.S. Department of Energy's Atmospheric Radiation Measurement (ARM) Climate Research Facility are using a heavily instrumented aircraft to collect data from the sky, while instruments based at surface sites in Barrow and Atqasuk, Alaska, are obtaining measurements from the ground. Information obtained during the Indirect and Semi-Direct Aerosol Campaign, or ISDAC, will help scientists analyze the role of aerosols in climate, and represents a key contribution to Arctic climate research during International Polar Year.

135

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

A New Method for Satellite/Surface Comparisons A New Method for Satellite/Surface Comparisons Download a printable PDF Submitter: Long, C. N., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Cloud Properties, Radiative Processes Journal Reference: Zhang Y, CN Long, WB Rossow, and EG Dutton. 2010. "Exploiting diurnal variations to evaluate the ISCCP-FD flux calculations and radiative-flux-analysis-processed surface observations from BSRN, ARM, and SURFRAD." Journal of Geophysical Research - Atmospheres, 115, D00K11, 10.1029/2009JD012812. Figure 1: Scatter plot for the column aerosol optical depth (AOD) at 550 nm, measured at the surface (PSO) and used as input for the ISCCP-FD calculations (FD) at 10 ARM/SURFRAD/BSRN stations. The robust linear regression line is also shown.

136

Development of Aerosol Models for Radiative Flux Calculations at ARM Sites: Utility of Trajectory Clustering for Characterizing Aerosol Climatology  

NLE Websites -- All DOE Office Websites (Extended Search)

Development of Aerosol Models for Radiative Flux Development of Aerosol Models for Radiative Flux Calculations at ARM Sites: Utility of Trajectory Clustering for Characterizing Aerosol Climatology E. Andrews Cooperative Institute for Research in the Environment University of Colorado Boulder, Colorado E. Andrews, J. A. Ogren, P. J. Sheridan, and J. M. Harris Climate Monitoring and Diagnostics Laboratory National Oceanic and Atmospheric Administration Boulder, Colorado P. K. Quinn Pacific Marine Environmental Laboratory National Oceanic and Atmospheric Administration Seattle, Washington Abstract The uncertainties associated with assumptions of generic aerosol properties in radiative transfer codes are unknown, which means that these uncertainties are frequently invoked when models and

137

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

New Characterization of Organic Aerosol Evolution Will Help Improve Models New Characterization of Organic Aerosol Evolution Will Help Improve Models Download a printable PDF Submitter: Jimenez, J., University of Colorado Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Jimenez JL and . et al. 2009. "Evolution of organic aerosols in the atmosphere." Science, 326, doi: 10.1126/science.1180353. Total mass concentration (in micrograms per cubic meter) and mass fractions of non-refractory inorganic species and organic components in submicrometer aerosols measured with the AMS at multiple surface locations in the Northern Hemisphere. Inset: Distributions of O:C for the OA components identified at the different sites. Relationship between O:C and hygroscopicity (k, or equivalently the

138

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Production Flux of Sea-Spray Aerosol Production Flux of Sea-Spray Aerosol Download a printable PDF Submitter: Schwartz, S. E., Brookhaven National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: de Leeuw G, EL Andreas, MD Anguelova, ER Lewis, C O'Dowd, M Schulz, and SE Schwartz. 2011. "Production flux of sea-spray aerosol." Reviews of Geophysics, 49, RG2001, doi:10.1029/2010RG000349. Lewis ER and SE Schwartz. 2004. Sea Salt Aerosol Production: Mechanisms, Methods, Measurements, and Models-A Critical Review. Washington DC: American Geophysical Union. Parameterizations of size-dependent SSA production flux evaluated for wind speed U10 = 8 m s-1. Also, central values (curves) and associated uncertainty ranges (bands) from Lewis and Schwartz (2004). Abscissa denotes

139

Carbonaceous Aerosols and Radiative...  

NLE Websites -- All DOE Office Websites (Extended Search)

and absorption of light by aerosols. At the ground sites, a new Humidigraph, a Cloud Condensation Nuclei Counter, a Scanning Mobility Particle Sizer, and an upgraded 915-MHz...

140

A balloon-borne aerosol spectrometer for high altitude low aerosol concentration measurements  

SciTech Connect

Funded by Air Force Wright Aeronautical Laboratory, a new balloon-borne high altitude aerosol spectrometer, for the measurement of cirrus cloud ice crystals, has been developed and successfully flown by Sandia National Laboratories and Radiance Research. This report (1) details the aerosol spectrometer design and construction, (2) discusses data transmission and decoding, (3) presents data collected on three Florida flights in tables and plots. 2 refs., 11 figs., 3 tabs.

Brown, G.S. (Sandia National Labs., Albuquerque, NM (USA)); Weiss, R.E. (Radiance Research, Seattle, WA (USA))

1990-08-01T23:59:59.000Z

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


141

Edinburgh Research Explorer Quantifying the implicit process flow abstraction in SBGN-PD  

E-Print Network (OSTI)

Edinburgh Research Explorer Quantifying the implicit process flow abstraction in SBGN-PD diagrams the implicit process flow abstraction in SBGN-PD diagrams with Bio-PEPA'. in Proceedings of COMPMOD 2009. ETPCS to publication record in Edinburgh Research Explorer Published In: Proceedings of COMPMOD 2009 General rights

Millar, Andrew J.

142

Aid to Education: House Group Cites Need for More Technicians, Research on Learning Process  

Science Journals Connector (OSTI)

...technical training facilities and basic research into the learning process...least until very recently, basic research in the learning process...Universitetets Institut for Teore-tisk Fysik, Blegdamsvej 17, Copen-hagen...program in steroid biochemistry theory and tech-niques, offered...

D. S. G.

1962-02-02T23:59:59.000Z

143

Final Report - Independent Verification Survey Activities at the Seperations Process Research Unit Sites, Niskayuna, New York  

SciTech Connect

The Separations Process Research Unit (SPRU) complex located on the Knolls Atomic Power Laboratory (KAPL) site in Niskayuna, New York, was constructed in the late 1940s to research the chemical separation of plutonium and uranium (Figure A-1). SPRU operated as a laboratory scale research facility between February 1950 and October 1953. The research activities ceased following the successful development of the reduction oxidation and plutonium/uranium extraction processes. The oxidation and extraction processes were subsequently developed for large scale use by the Hanford and Savannah River sites (aRc 2008a). Decommissioning of the SPRU facilities began in October 1953 and continued through the 1990s.

Evan Harpenau

2011-03-15T23:59:59.000Z

144

Wind Program Manufacturing Research Advances Processes and Reduces Costs  

Energy.gov (U.S. Department of Energy (DOE))

Knowing that reducing the overall cost of wind energy begins on the factory floor, the Wind Program supports R&D efforts and funding opportunities that integrate new designs, materials, and advanced techniques into the manufacturing process, making wind a more affordable source of renewable energy for communities nationwide.

145

Signal and Image Processing Research at the Lawrence Livermore National Laboratory  

SciTech Connect

Lawrence Livermore National Laboratory is a large, multidisciplinary institution that conducts fundamental and applied research in the physical sciences. Research programs at the Laboratory run the gamut from theoretical investigations, to modeling and simulation, to validation through experiment. Over the years, the Laboratory has developed a substantial research component in the areas of signal and image processing to support these activities. This paper surveys some of the current research in signal and image processing at the Laboratory. Of necessity, the paper does not delve deeply into any one research area, but an extensive citation list is provided for further study of the topics presented.

Roberts, R S; Poyneer, L A; Kegelmeyer, L M; Carrano, C J; Chambers, D H; Candy, J V

2009-06-29T23:59:59.000Z

146

Direct Aerosol Forcing Uncertainty  

DOE Data Explorer (OSTI)

Understanding sources of uncertainty in aerosol direct radiative forcing (DRF), the difference in a given radiative flux component with and without aerosol, is essential to quantifying changes in Earth's radiation budget. We examine the uncertainty in DRF due to measurement uncertainty in the quantities on which it depends: aerosol optical depth, single scattering albedo, asymmetry parameter, solar geometry, and surface albedo. Direct radiative forcing at the top of the atmosphere and at the surface as well as sensitivities, the changes in DRF in response to unit changes in individual aerosol or surface properties, are calculated at three locations representing distinct aerosol types and radiative environments. The uncertainty in DRF associated with a given property is computed as the product of the sensitivity and typical measurement uncertainty in the respective aerosol or surface property. Sensitivity and uncertainty values permit estimation of total uncertainty in calculated DRF and identification of properties that most limit accuracy in estimating forcing. Total uncertainties in modeled local diurnally averaged forcing range from 0.2 to 1.3 W m-2 (42 to 20%) depending on location (from tropical to polar sites), solar zenith angle, surface reflectance, aerosol type, and aerosol optical depth. The largest contributor to total uncertainty in DRF is usually single scattering albedo; however decreasing measurement uncertainties for any property would increase accuracy in DRF. Comparison of two radiative transfer models suggests the contribution of modeling error is small compared to the total uncertainty although comparable to uncertainty arising from some individual properties.

Mccomiskey, Allison

147

Knowledge Mobilization Processes During the Research Process in Two Projects: Lessons for the Leslie Harris Centre of Regional Policy and Development  

E-Print Network (OSTI)

Knowledge Mobilization Processes During the Research Process in Two Projects: Lessons......................................................................................................... 7 SECTION IV: FRAMEWORK FOR KNOWLEDGE MOBILIZATION ASSESSMENT... 10 Theoretical Framework for KMb

deYoung, Brad

148

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Hemispherical Simulations Show Impact of Aerosols on Cloud Reflectivity Hemispherical Simulations Show Impact of Aerosols on Cloud Reflectivity Submitter: Rotstayn, L., Commonwealth Scientific and Industrial Research Organization Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Rotstayn, L., and Y. Liu, Sensitivity of the First Indirect Aerosol Effect to an Increase in Cloud Droplet Spectral Dispersion with Droplet Number Concentration, Journal of Climate: Vol. 16, No. 21, pp.3476-3481, May 2003. Figure 1. Measurements of the relation between the relative dispersion of the cloud droplet spectrum and the cloud droplet number concentration (N). The lower, middle, and upper curves show the parameterizations used in the LOWER, MIDDLE, and UPPER simulations, respectively. A recent study by DOE Atmospheric Radiation Measurement (ARM) Program

149

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Micropulse Lidar-Derived Aerosol Optical Depth Climatology at ARM Sites Micropulse Lidar-Derived Aerosol Optical Depth Climatology at ARM Sites Worldwide Download a printable PDF Submitter: Kafle, D. N., University of California, Riverside Coulter, R. L., Argonne National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Kafle DN and RL Coulter. 2013. "Micropulse lidar-derived aerosol optical depth climatology at ARM sites worldwide." Journal of Geophysical Research - Atmospheres, 118(13), 10.1002/jgrd.50536. Vertical profiles of multi-year annually averaged AOD (z) at different ARM sites: SGP, NSA, TWP, GRW, and FKB. Inset plots are the profiles of corresponding relative standard deviation, Srel (z). The corresponding 1-sigma measurement errors are given in horizontal bars.

150

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Clouds Brighten Up the Sky Near Them Clouds Brighten Up the Sky Near Them Download a printable PDF Submitter: Varnai, T., University of Maryland, Baltimore County/JCEST Marshak, A., NASA - Goddard Space Flight Center Area of Research: Radiation Processes Working Group(s): Radiative Processes Journal Reference: Varnai T and A Marshak. 2009. "MODIS observations of enhanced clear sky reflectance near clouds." Geophysical Research Letters, 36, L06807, doi:10.1029/2008GL037089. Figure 1. Illustration of clouds enhancing the brightness of sky in nearby clear areas. In cloud-free areas light is scattered mainly by air molecules, but aerosols also contribute. Figure 2. Top: Average increase in MODIS clear-sky reflectivity (R) near clouds. The difference between areas near illuminated and shadowy cloud

151

Research Highlight  

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Putting the Pieces Together Putting the Pieces Together Download a printable PDF Submitter: Fan, J., Pacific Northwest National Laboratory Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle Journal Reference: Fan J, S Ghan, M Ovchinnikov, X Liu, P Rasch, and A Korolev. 2011. "Representation of arctic mixed-phase clouds and the Wegener-Bergeron-Findeisen process in climate models: Perspectives from a cloud-resolving study." Journal of Geophysical Research - Atmospheres, 116, D00T07, doi:10.1029/2010JD015375. PNNL's Arctic mixed-phase cloud research was augmented with field observations from the 2008 Indirect and Semi-Direct Aerosol Campaign (ISDAC) in Northern Alaska. Photo courtesy of A. Korolev, Environment Canada. Vertical cross sections of (a) the vertical velocity (the contour lines)

152

Research investigations in oil shale, tar sand, coal research, advanced exploratory process technology, and advanced fuels research: Volume 1 -- Base program. Final report, October 1986--September 1993  

SciTech Connect

Numerous studies have been conducted in five principal areas: oil shale, tar sand, underground coal gasification, advanced process technology, and advanced fuels research. In subsequent years, underground coal gasification was broadened to be coal research, under which several research activities were conducted that related to coal processing. The most significant change occurred in 1989 when the agreement was redefined as a Base Program and a Jointly Sponsored Research Program (JSRP). Investigations were conducted under the Base Program to determine the physical and chemical properties of materials suitable for conversion to liquid and gaseous fuels, to test and evaluate processes and innovative concepts for such conversions, to monitor and determine environmental impacts related to development of commercial-sized operations, and to evaluate methods for mitigation of potential environmental impacts. This report is divided into two volumes: Volume 1 consists of 28 summaries that describe the principal research efforts conducted under the Base Program in five topic areas. Volume 2 describes tasks performed within the JSRP. Research conducted under this agreement has resulted in technology transfer of a variety of energy-related research information. A listing of related publications and presentations is given at the end of each research topic summary. More specific and detailed information is provided in the topical reports referenced in the related publications listings.

Smith, V.E.

1994-05-01T23:59:59.000Z

153

Chemical Composition and Cloud Nucleation Ability of Marine Aerosol  

E-Print Network (OSTI)

This study is focused on the chemical composition and cloud nucleation ability of marine aerosol based on two cruise researches over Pacific Ocean and North Atlantic Ocean respectively. Implications of CLAW hypothesis and the factors influencing its...

Deng, Chunhua

2013-12-12T23:59:59.000Z

154

3, 59195976, 2003 The nitrate aerosol  

E-Print Network (OSTI)

ACPD 3, 5919­5976, 2003 The nitrate aerosol field over Europe M. Schaap et al. Title Page Abstract of Utrecht, Institute of Marine and Atmospheric Science, PO Box 80005, 3508 TA, Utrecht, The Netherlands 2, The Netherlands 3 Netherlands Energy Research Foundation (ECN), PO Box 1, 1755 LE Petten, The Netherlands 4 Joint

Paris-Sud XI, Université de

155

Emerging Issues in Nanoparticle Aerosol Science and Technology Workshop report sponsored by: NSF, Southern California Particle Center and UCLA  

E-Print Network (OSTI)

has responsibility for nuclear reactor safety which includes emissions of radioactive particles pollution sources, (2) industrial production of nanoparticle reinforcing fillers such as carbon black nanoparticle products by aerosol processes, (4) atmospheric dynamics of fractal-like nanoparticle aerosols (e

Jimenez, Jose-Luis

156

Intercomparison and evaluation of global aerosol microphysical properties among AeroCom models of a range of complexity  

E-Print Network (OSTI)

Many of the next generation of global climate models will include aerosol schemes which explicitly simulate the microphysical processes that determine the particle size distribution. These models enable aerosol optical ...

Ridley, David Andrew

157

Aerosol Retrievals under Partly Cloudy Conditions: Challenges and Perspectives  

SciTech Connect

There are lots of interesting and intriguing features of aerosols near clouds many of which can be quite engaging, as well being useful and climate-related. Exploring aerosol with the aid of the remote sensing, in situ observations and numerical modeling has piqued our curiosity and led to improve insights into the nature of aerosol and clouds and their complex relationship. This chapter conveys the outstanding issues of cloudy-sky aerosol retrievals of important climate properties and outlines their fruitful connections to other research areas such as in situ measurements and model simulations. The chapter focuses mostly on treating the inverse problems in the context of the passive satellite remote sensing and how they can improve our understanding of the cloud-aerosol interactions. The presentation includes a basis in the inverse problem theory, reviews available approaches and discusses their applications to partly cloudy situations. Potential synergy of observations and model simulations is described as well.

Kassianov, Evgueni I.; Ovchinnikov, Mikhail; Berg, Larry K.; Flynn, Connor J.

2011-06-01T23:59:59.000Z

158

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

More Like Shades of Gray: the Effects of Black Carbon in Aerosols More Like Shades of Gray: the Effects of Black Carbon in Aerosols Submitter: McComiskey, A. C., National Oceanic and Atmospheric Administration Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Cappa CD, TB Onasch, P Massoli, DR Worsnop, TS Bates, ES Cross, P Davidovits, J Hakala, KL Hayden, BT Jobson, KR Kolesar, DA Lack, BM Lerner, SM Li, D Mellon, I Nuaaman, JS Olfert, T Petaja, PK Quinn, C Song, R Subramanian, EJ Williams, and RA Zaveri. 2012. "Radiative absorption enhancements due to the mixing state of atmospheric black carbon." Science, 337(6098), doi:10.1126/science.1223447. Black to the core: Scientists are combining field and laboratory measurements to understand more about the physical properties of aerosols

159

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Simulating the Impact of Aerosols on Tropical Deep Convection Simulating the Impact of Aerosols on Tropical Deep Convection Download a printable PDF Submitter: Morrison, H. C., NCAR Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Morrison H and WW Grabowski. 2011. "Cloud-system resolving model simulations of aerosol indirect effects on tropical deep convection and its thermodynamic environment." Atmospheric Chemistry and Physics, 11(20), doi:10.5194/acp-11-10503-201. Profiles of ensemble- and horizontally averaged a) cloud water mixing ratio, b) rain mixing ratio, c) ice mixing ratio, d) cloud droplet concentration, e) rain number concentration, and f) ice number concentration, Ni, for pristine (blue), polluted (green), and highly

160

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

To Rain or Not to Rain...Aerosols May Be the Answer To Rain or Not to Rain...Aerosols May Be the Answer Download a printable PDF Submitter: Li, Z., University of Maryland Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Niu F and Z Li. 2012. "Systematic variations of cloud top temperature and precipitation rate with aerosols over the global tropics." Atmospheric Chemistry and Physics, 12, doi:10.5194/acp-12-8491-2012. Cloud-top temperature (A, C) and ice water path (B, D) as functions of AI/AOT for warm (blue dots) and cold (red dots) base mixed-phase clouds and liquid clouds (green dots) over the ocean (upper panels) and land (lower panels). The right-hand axes of (A) and (C) are for liquid clouds. Precipitation rate as a function of AI for mixed-phase (blue dots) and

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


161

A World-wide Stratospheric Aerosol Layer  

Science Journals Connector (OSTI)

...Massachusetts An aerosol layer has been identified by a stratospheric balloon and aircraft aerosol collection program. Measurements...Abstract. An aerosol layer has been identified by a stratospheric balloon and aircraft aerosol collection program. Meas-urements...

Christian E. Junge; Charles W. Chagnon; James E. Manson

1961-05-12T23:59:59.000Z

162

Development and Characterization of a Thermodenuder for Aerosol Volatility Measurements  

SciTech Connect

This SBIR Phase I project addressed the critical need for improved characterization of carbonaceous aerosol species in the atmosphere. The proposed work focused on the development of a thermodenuder (TD) system capable of systematically measuring volatility profiles of primary and secondary organic aerosol species and providing insight into the effects of absorbing and nonabsorbing organic coatings on particle absorption properties. This work provided the fundamental framework for the generation of essential information needed for improved predictions of ambient aerosol loadings and radiative properties by atmospheric chemistry models. As part of this work, Aerodyne Research, Inc. (ARI) continued to develop and test, with the final objective of commercialization, an improved thermodenuder system that can be used in series with any aerosol instrument or suite of instruments (e.g., aerosol mass spectrometers-AMS, scanning mobility particle sizers-SMPS, photoacoustic absorption spectrometers-PAS, etc.) to obtain aerosol chemical, physical, and optical properties as a function of particle volatility. In particular, we provided the proof of concept for the direct coupling of our improved TD design with a full microphysical model to obtain volatility profiles for different organic aerosol components and to allow for meaningful comparisons between different TD-derived aerosol measurements. In a TD, particles are passed through a heated zone and a denuding (activated charcoal) zone to remove semi-volatile material. Changes in particle size, number concentration, optical absorption, and chemical composition are subsequently detected with aerosol instrumentation. The aerosol volatility profiles provided by the TD will strengthen organic aerosol emission inventories, provide further insight into secondary aerosol formation mechanisms, and provide an important measure of particle absorption (including brown carbon contributions and identification, and absorption enhancements due to coatings on soot particles). The successfully completed Phase I project included construction of a prototype design for the TD with detailed physical modeling, testing with laboratory and ambient aerosol particles, and the initiation of a detailed microphysical model of the aerosol particles passing through the TD to extract vapor pressure distributions. The objective of the microphysical model is to derive vapor pressure distributions (i.e. vapor pressure ranges, including single chemical compounds, mixtures of known compounds, and complex real-world aerosols, such as SOA, and soot particles with absorbing and nonabsorbing coatings) from TD measurements of changes in particle size, mass, and chemical composition for known TD temperatures and flow rates (i.e. residence times). The proposed Phase II project was designed to optimize several TD systems for different instrument applications and to combine the hardware and modeling into a robust package for commercial sales.

Dr. Timothy Onasch

2009-09-09T23:59:59.000Z

163

Strong radiative heating due to the mixing state of black carbon in atmospheric aerosols  

Science Journals Connector (OSTI)

... The global model that I used was GATOR-GCMM, which treated gas, aerosol, radiative, meteorological and transport processes (see Supplementary ...

Mark Z. Jacobson

2001-02-08T23:59:59.000Z

164

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Critical Role of Cloud Drop Effective Radius >14 Micron Radius in Rain Critical Role of Cloud Drop Effective Radius >14 Micron Radius in Rain Initiation Download a printable PDF Submitter: Rosenfeld, D., The Hebrew University of Jerusalem Wang, H., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Rosenfeld D, H Wang, and PJ Rasch. 2012. "The roles of cloud drop effective radius and LWP in determining rain properties in marine stratocumulus." Journal of Geophysical Research - Atmospheres, 39, doi:10.1029/2012GL052028. The dependence of rain rate on cloud drop effective radius (re) near cloud top. The color scale is for the median value of column maximum rain rate in each joint bin of CWP-re (cloud liquid water path and cloud-top re).

165

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Improving the Treatment of Radiation in Climate Models Improving the Treatment of Radiation in Climate Models Download a printable PDF Submitter: Delamere, J. S., Tech-X Corporation Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle, Cloud Life Cycle Journal Reference: Delamere JS, SA Clough, VH Payne, EJ Mlawer, DD Turner, and RR Gamache. 2010. "A far-infrared radiative closure study in the Arctic: Application to water vapor." Journal of Geophysical Research - Atmospheres, 115, D17106, 10.1029/2009JD012968. The mean AERI-ER radiances for a select set of cloud-free cases at NSA in 2007 are presented in the top panel. The bottom panel presents mean spectral differences between the measurements and model calculations. The red line demonstrates the differences when using the pre-RHUBC version of

166

Research Highlight  

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Field Experiments to Improve the Treatment of Radiation in the Mid-to-Upper Field Experiments to Improve the Treatment of Radiation in the Mid-to-Upper Troposphere Download a printable PDF Submitter: Turner, D. D., National Oceanic and Atmospheric Administration Mlawer, E. J., Atmospheric & Environmental Research, Inc. Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Turner DD and EJ Mlawer. 2010. "The Radiative Heating in Underexplored Bands Campaigns (RHUBC)." Bulletin of the American Meteorological Society, 91, doi:10.1175/2010BAMS2904.1. (a) Atmospheric transmittance at 1 cm-1 resolution in the far-infrared for three atmospheres that are representative of the ARM SGP site, NSA site, and RHUBC-II site in the Chajnantor plateau (CJC). (b) The transmittance

167

Research Highlight  

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Cloud-Resolving Model (CRM) Simulations: Robust Results for Use in Climate Cloud-Resolving Model (CRM) Simulations: Robust Results for Use in Climate Model Development Download a printable PDF Submitter: Fridlind, A. M., NASA - Goddard Institute for Space Studies Smith-Mrowiec, A. A., Columbia University/NASA Goddard Institute for Space Studies Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Mrowiec AA, C Rio, AM Fridlind, AS Ackerman, AD Del Genio, OM Pauluis, AC Varble, and J Fan. 2012. "Analysis of cloud-resolving simulations of a tropical mesoscale convective system observed during TWP-ICE: Vertical fluxes and draft properties in convective and stratiform regions." Journal of Geophysical Research, 117, D19201, doi:10.1029/2012JD017759.

168

Research Highlight  

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Burning on the Prairies Burning on the Prairies Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Fischer ML, MS Torn, DP Billesbach, G Doyle, B Northup, and SC Biraud. 2012. "Carbon, water, and heat flux responses to experimental burning and drought in a tallgrass prairie." Agricultural and Forest Meteorology, 166, doi:10.1016/j.agrformet.2012.07.011. Pasture burning during the beginning of the experiment at the USDA Grazing Lands Research Laboratory in March 2005. What does it mean for the carbon cycle? The deep drought in the United States that fueled wildfires and damaged crops in 2012 has now continued well into 2013. However, long before the droughts and fires wreaked havoc, a team of

169

Research Highlight  

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Buffering of Ice Crystal Number Concentration to Ice Nucleus Abundance Buffering of Ice Crystal Number Concentration to Ice Nucleus Abundance Above Arctic Stratus Download a printable PDF Submitter: Fridlind, A. M., NASA - Goddard Institute for Space Studies Ackerman, A., NASA - Goddard Institute for Space Studies Area of Research: Cloud Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Fridlind AM, B van Diedenhoven, AS Ackerman, A Avramov, A Mrowiec, H Morrison, P Zuidema, and MD Shupe. 2012. "A FIRE-ACE/SHEBA case study of mixed-phase Arctic boundary-layer clouds: Entrainment rate limitations on rapid primary ice nucleation processes." Journal of the Atmospheric Sciences, 69(1), doi:10.1175/JAS-D-11-052.1. Observed and simulated histograms of MMCR radar reflectivity (left) and

170

Thermochemical Process Development Unit: Researching Fuels from Biomass, Bioenergy Technologies (Fact Sheet)  

NLE Websites -- All DOE Office Websites (Extended Search)

Highlights Highlights Thermochemical conversion technologies convert biomass and its residues to fuels and chemicals using gasification and pyrolysis. Gasification entails heating biomass and results in a mixture of carbon monoxide and hydrogen, known as syngas. Pyrolysis, which is heating biomass in the absence of oxygen, produces liquid pyrolysis oil. Both syngas and pyrolysis oil can be chemically converted into clean, renewable transportation fuels and chemicals. The Thermochemical Process Development Unit (TCPDU) at the National Renewable Energy Laboratory (NREL) is a unique facility dedicated to researching thermochemical processes to produce fuels from biomass. Thermochemical processes include gasification and pyrolysis-processes used to convert

171

Aerosol radiative forcing and the accuracy of satellite aerosol optical depth retrieval  

E-Print Network (OSTI)

, New Mexico, USA Michael Mishchenko Goddard Institute for Space Studies, NASA, New York, New York, USA between t = 0.1 and t = 0.8. The Department of Energy research satellite instrument, the Multispectral [Hobbs et al., 1997]. The aerosols' direct effect involves their interaction with solar and terrestrial

172

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Strong Impacts of Vertical Velocity on Cloud Microphysics and Implications Strong Impacts of Vertical Velocity on Cloud Microphysics and Implications for Aerosol Indirect Download a printable PDF Submitter: Liu, Y., Brookhaven National Laboratory Lu, C., Brookhaven National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Lu C, Y Liu, S Niu, and AM Vogelmann. 2012. "Observed impacts of vertical velocity on cloud microphysics and implications for aerosol indirect effects." Geophysical Research Letters, 39, L21808, doi:10.1029/2012GL053599. Joint probability density functions (PDF) of relative dispersion (ε) versus vertical velocity (w) along horizontal aircraft legs for each cumulus flight (date given in legend). The red lines denote weighted least

173

Research Highlight  

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Climate Warming Due to Soot and Smoke? Maybe Not. Climate Warming Due to Soot and Smoke? Maybe Not. Submitter: Penner, J. E., University of Michigan Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Penner, J.E., S.Y. Zhang, and C.C. Chuang, Soot and smoke aerosol may not warm climate, J. Geophys. Res., 108(D21), 4657, doi:10.1029/2003JD003409, 2003. New research results from the Department of Energy's Atmospheric Radiation Measurement (ARM) Program suggest that fossil fuel soot emissions and biomass smoke may actually have a negligible warming effect and, in some cases, may even result in a net cooling effect. Black carbon is the absorbing component of smoke aerosols that result from the incomplete combustion of various fuels, the most significant sources being fossil fuel

174

Long-term Statistics of Continental Cumuli: Does Aerosol Trigger Cumulus Variability?  

SciTech Connect

Atmospheric aerosols may control the formation, maintenance, and dissipation of cumuli by changing their microphysics. Recent observational and modeling results exist both in support and against strong potential impacts of aerosol [1-3]. Typically, the aerosol impact on water clouds has been investigated for regions with high aerosol loading and/or large atmospheric moisture [4]. Can we provide observational evidence of the aerosol-cloud relationship for a relatively dry continental region with low/moderate aerosol burden? To address this question, we revisit the aerosol-cloud relationship at the Atmospheric Radiation Measurement (ARM) Climate Research Facility (ACRF) Southern Great Plains (SGP) site. In comparison with highly polluted regions, the SGP site is characterized by relatively small-to-moderate aerosol loading. Also, moisture content is small-to-moderate (compared to marine and coastal regions) for the SGP site. Because cumulus clouds have important impacts on climate forcing estimations [5] and are susceptible to aerosol effects [6], we focus on fair-weather cumuli (FWC) and their association with aerosol concentration and other potentially important factors. This association is investigated using a new 8-year aerosol and cloud climatology (2000-2007) developed with collocated and coincident surface and satellite observations.

Kassianov, Evgueni I.; Berg, Larry K.; McFarlane, Sally A.; Flynn, Connor J.; Turner, David D.

2009-02-01T23:59:59.000Z

175

Geometrical Optics of Dense Aerosols  

SciTech Connect

Assembling a free-standing, sharp-edged slab of homogeneous material that is much denser than gas, but much more rare ed than a solid, is an outstanding technological challenge. The solution may lie in focusing a dense aerosol to assume this geometry. However, whereas the geometrical optics of dilute aerosols is a well-developed fi eld, the dense aerosol limit is mostly unexplored. Yet controlling the geometrical optics of dense aerosols is necessary in preparing such a material slab. Focusing dense aerosols is shown here to be possible, but the nite particle density reduces the eff ective Stokes number of the flow, a critical result for controlled focusing. __________________________________________________

Hay, Michael J.; Valeo, Ernest J.; Fisch, Nathaniel J.

2013-04-24T23:59:59.000Z

176

BNL | Aerosol, Cloud, Precipitation Interactions  

NLE Websites -- All DOE Office Websites (Extended Search)

Cloud-Aerosol-Precipitation Interactions Cloud-Aerosol-Precipitation Interactions Atmospheric aerosols exert important "indirect effects" on clouds and climate by serving as cloud condensation nuclei (CCN) and ice nuclei that affect cloud radiative and microphysical properties. For example, an increase in CCN increases the number concentration of droplets enhances cloud albedo, and suppresses precipitation that alters cloud coverage and lifetime. However, in the case of moist and strong convective clouds, increasing aerosols may increase precipitation and enhance storm development. Although aerosol-induced indirect effects on climate are believed to have a significant impact on global climate change, estimating their impact continues to be one of the most uncertain climate forcings.

177

NDE research focuses on questions such as: How do fabrication, growth, andlor processing  

E-Print Network (OSTI)

NDE research focuses on questions such as: How do fabrication, growth, andlor processing contribute-structural properties affect overall thermal, mechanical, electrical, and optical behavior? WILLIAM & MARY NDE Nondestructive Evaluation (NDE) is an interdisciplinary field of study that is concerned with the development

Lewis, Robert Michael

178

The Two-Column Aerosol Project (TCAP) Science Plan  

SciTech Connect

The Two-Column Aerosol Project (TCAP) field campaign will provide a detailed set of observations with which to (1) perform radiative and cloud condensation nuclei (CCN) closure studies, (2) evaluate a new retrieval algorithm for aerosol optical depth (AOD) in the presence of clouds using passive remote sensing, (3) extend a previously developed technique to investigate aerosol indirect effects, and (4) evaluate the performance of a detailed regional-scale model and a more parameterized global-scale model in simulating particle activation and AOD associated with the aging of anthropogenic aerosols. To meet these science objectives, the Atmospheric Radiation Measurement (ARM) Climate Research Facility will deploy the ARM Mobile Facility (AMF) and the Mobile Aerosol Observing System (MAOS) on Cape Cod, Massachusetts, for a 12-month period starting in the summer of 2012 in order to quantify aerosol properties, radiation, and cloud characteristics at a location subject to both clear and cloudy conditions, and clean and polluted conditions. These observations will be supplemented by two aircraft intensive observation periods (IOPs), one in the summer and a second in the winter. Each IOP will deploy one, and possibly two, aircraft depending on available resources. The first aircraft will be equipped with a suite of in situ instrumentation to provide measurements of aerosol optical properties, particle composition and direct-beam irradiance. The second aircraft will fly directly over the first and use a multi-wavelength high spectral resolution lidar (HSRL) and scanning polarimeter to provide continuous optical and cloud properties in the column below.

Berkowitz, CM; Berg, LK; Cziczo, DJ; Flynn, CJ; Kassianov, EI; Fast, JD; Rasch, PJ; Shilling, JE; Zaveri, RA; Zelenyuk, A; Ferrare, RA; Hostetler, CA; Cairns, B; Russell, PB; Ervens, B

2011-07-27T23:59:59.000Z

179

Continuous air monitor for alpha-emitting aerosol particles  

SciTech Connect

A new alpha Continuous Air Monitor (CAM) sampler is being developed for use in detecting the presence of alpha-emitting aerosol particles. The effort involves design, fabrication and evaluation of systems for the collection of aerosol and for the processing of data to speciate and quantify the alpha emitters of interest. At the present time we have a prototype of the aerosol sampling system and we have performed wind tunnel tests to characterize the performance of the device for different particle sizes, wind speeds, flow rates and internal design parameters. The results presented herein deal with the aerosol sampling aspects of the new CAM sampler. Work on the data processing, display and alarm functions is being done in parallel with the particle sampling work and will be reported separately at a later date. 17 refs., 5 figs., 3 tabs.

McFarland, A.R.; Ortiz, C.A. (Texas A and M Univ., College Station, TX (USA). Dept. of Mechanical Engineering); Rodgers, J.C.; Nelson, D.C. (Los Alamos National Lab., NM (USA))

1990-01-01T23:59:59.000Z

180

aerosols and climate : uncertainties  

E-Print Network (OSTI)

contributes to creating a level playing field. (BC emissions tradeble like CO2 emissions?) OUTLINE #12;size. policy measures, is even more uncertain (emissions & their chemical fingerprint are uncertain (not just aerosol emissions, not just climate impacts) OUTLINE #12;- Standardization doesn't reduce

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


181

Overview of Fiscal Year 2002 Research and Development for Savannah River Site's Salt Waste Processing Facility  

SciTech Connect

The Department of Energy's (DOE) Savannah River Site (SRS) high-level waste program is responsible for storage, treatment, and immobilization of high-level waste for disposal. The Salt Processing Program (SPP) is the salt (soluble) waste treatment portion of the SRS high-level waste effort. The overall SPP encompasses the selection, design, construction and operation of treatment technologies to prepare the salt waste feed material for the site's grout facility (Saltstone) and vitrification facility (Defense Waste Processing Facility). Major constituents that must be removed from the salt waste and sent as feed to Defense Waste Processing Facility include actinides, strontium, cesium, and entrained sludge. In fiscal year 2002 (FY02), research and development (R&D) on the actinide and strontium removal and Caustic-Side Solvent Extraction (CSSX) processes transitioned from technology development for baseline process selection to providing input for conceptual design of the Salt Waste Processing Facility. The SPP R&D focused on advancing the technical maturity, risk reduction, engineering development, and design support for DOE's engineering, procurement, and construction (EPC) contractors for the Salt Waste Processing Facility. Thus, R&D in FY02 addressed the areas of actual waste performance, process chemistry, engineering tests of equipment, and chemical and physical properties relevant to safety. All of the testing, studies, and reports were summarized and provided to the DOE to support the Salt Waste Processing Facility, which began conceptual design in September 2002.

H. D. Harmon, R. Leugemors, PNNL; S. Fink, M. Thompson, D. Walker, WSRC; P. Suggs, W. D. Clark, Jr

2003-02-26T23:59:59.000Z

182

One ARM, Two Columns and a Whole Lot of Aerosols | Department of Energy  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

ARM, Two Columns and a Whole Lot of Aerosols ARM, Two Columns and a Whole Lot of Aerosols One ARM, Two Columns and a Whole Lot of Aerosols July 25, 2012 - 5:49pm Addthis This observatory is part of an air particles research initiative at Cape Cod National Seashore in Massachusetts, and includes dozens of sophisticated instruments that take continuous ground-based measurements of clouds, aerosols, and other atmospheric properties. | Photo courtesy of the ARM Climate Research Facility. This observatory is part of an air particles research initiative at Cape Cod National Seashore in Massachusetts, and includes dozens of sophisticated instruments that take continuous ground-based measurements of clouds, aerosols, and other atmospheric properties. | Photo courtesy of the ARM Climate Research Facility.

183

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Arctic Mixed-phase Clouds Persist with Little Help from the Local Surface Arctic Mixed-phase Clouds Persist with Little Help from the Local Surface Download a printable PDF Submitter: Shupe, M., University of Colorado Area of Research: Cloud Processes Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Shupe MD, OG Persson, IM Brooks, M Tjernstrom, J Sedlar, T Mauritsen, S Sjogren, and C Leck. 2013. "Cloud and boundary layer interactions over the Arctic sea ice in late summer." Atmospheric Chemistry and Physics, 13, doi:10.5194/acp-13-9379-2013. Figure 1. Normalized profiles of (a) vertical velocity skewness and (b) variance, (c) turbulent dissipation rate, and (d) potential temperature. Black curves are all data, while red and green are for decoupled and coupled cases, respectively. Normalization is relative to the cloud top

184

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Black Carbon Reduction of Snow Albedo Black Carbon Reduction of Snow Albedo Submitter: Kirchstetter, T. W., Lawrence Berkeley National Laboratory Area of Research: Radiation Processes Working Group(s): Aerosol Life Cycle Journal Reference: Hadley OL and TW Kirchstetter. 2012. "Black carbon reduction of snow albedo." Nature Climate Change, , doi:10.1038/nclimate1433. Spectrally weighted snow albedo over the 300-2,500 nm solar spectrum: derived from our experiments (dots, 1 standard deviation) and modelled using SNICAR (shaded bands). Upper and lower boundaries of the shaded bands correspond to modelled albedo assuming BC mass absorption cross-sections, at 550 nm, of 7.5 and 15 m2/g, respectively. Climate models indicate that the reduction of surface albedo caused by black carbon contamination of snow contributes to global warming and

185

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Looking at the Full Spectrum for Water Vapor Looking at the Full Spectrum for Water Vapor Download a printable PDF Submitter: Turner, D. D., National Oceanic and Atmospheric Administration Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Mlawer EJ, VH Payne, J Moncet, JS Delamere, MJ Alvarado, and DD Tobin. 2012. "Development and recent evaluation of the MT_CKD model of continuum absorption." Philosophical Transactions of The Royal Society A, 370, doi: 10.1098/rsta.2011.0295. Radiative cooling across the full infrared spectrum: The far-infrared (the left half of the figure, from 15 to 1000 microns) plays a key role in heat transfer in the atmosphere, but scientists could not measure it, and model calculations were consequently very uncertain. Field observations from

186

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Spectral Invariant Properties of Single-Scattering Albedo for Water Spectral Invariant Properties of Single-Scattering Albedo for Water Droplets and Ice Crystals Download a printable PDF Submitter: Marshak, A., NASA - Goddard Space Flight Center Area of Research: Radiation Processes Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Marshak A, Y Knyazikhin, JC Chiu, and WJ Wiscombe. 2012. "On spectral invariance of single scattering albedo for water droplets and ice crystals at weakly absorbing wavelengths." Journal of Quantitative Spectroscopy & Radiative Transfer, 113, 715-720. The ratio of ω0λ(r)/ω0λ(r0) plotted against ω0λ(r) for four wavelengths, λ=0.86, 1.65, 2.13 and 3.75 um. An example for the aggregates ice crystal habits is shown (see Yang et al. 2000. "Parameterization of

187

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

A Tall Order: Climate Models Fall Short in Predicting African Sahel A Tall Order: Climate Models Fall Short in Predicting African Sahel Rainfall Download a printable PDF Submitter: Roehrig, R., Meteo-France CNRM/GMME/MOANA Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Roehrig R, D Bouniol, F Guichard, F Hourdin, and JL Redelsperger. 2013. "The present and future of the West African Monsoon: A process-oriented assessment of CMIP5 simulations along the AMMA transect." Journal of Climate, 26(17), doi:10.1175/jcli-d-12-00505.1. The wealth of data available from field campaigns between the Gulf of Guinea and the Sahara Desert allowed scientists to evaluate the ability of climate models to accurately predict rainfall in the area.

188

An Aerosol Condensation Model for Sulfur Trioxide  

SciTech Connect

This document describes a model for condensation of sulfuric acid aerosol given an initial concentration and/or source of gaseous sulfur trioxide (e.g. fuming from oleum). The model includes the thermochemical effects on aerosol condensation and air parcel buoyancy. Condensation is assumed to occur heterogeneously onto a preexisting background aerosol distribution. The model development is both a revisiting of research initially presented at the Fall 2001 American Geophysical Union Meeting [1] and a further extension to provide new capabilities for current atmospheric dispersion modeling efforts [2]. Sulfuric acid is one of the most widely used of all industrial chemicals. In 1992, world consumption of sulfuric acid was 145 million metric tons, with 42.4 Mt (mega-tons) consumed in the United States [10]. In 2001, of 37.5 Mt consumed in the U.S., 74% went into producing phosphate fertilizers [11]. Another significant use is in mining industries. Lawuyi and Fingas [7] estimate that, in 1996, 68% of use was for fertilizers and 5.8% was for mining. They note that H{sub 2}SO{sub 4} use has been and should continue to be very stable. In the United States, the elimination of MTBE (methyl tertiary-butyl ether) and the use of ethanol for gasoline production are further increasing the demand for petroleum alkylate. Alkylate producers have a choice of either a hydrofluoric acid or sulfuric acid process. Both processes are widely used today. Concerns, however, over the safety or potential regulation of hydrofluoric acid are likely to result in most of the growth being for the sulfuric acid process, further increasing demand [11]. The implication of sulfuric acid being a pervasive industrial chemical is that transport is also pervasive. Often, this is in the form of oleum tankers, having around 30% free sulfur trioxide. Although sulfuric acid itself is not a volatile substance, fuming sulfuric acid (referred to as oleum) is [7], the volatile product being sulfur trioxide. Sulfate aerosols and mist may form in the atmosphere on tank rupture. From chemical spill data from 1990-1996, Lawuyi02 and Fingas [7] prioritize sulfuric acid as sixth most serious. During this period, they note 155 spills totaling 13 Mt, out of a supply volume of 3700 Mt. Lawuyi and Fingas [7] summarize information on three major sulfuric acid spills. On 12 February 1984, 93 tons of sulfuric acid were spilled when 14 railroad cars derailed near MacTier, Parry Sound, Ontario. On 13 December 1978, 51 railroad cars derailed near Springhill, Nova Scotia. One car, containing 93% sulfuric acid, ruptured, spilling nearly its entire contents. In July 1993, 20 to 50 tons of fuming sulfuric acid spilled at the General Chemical Corp. plant in Richmond, California, a major industrial center near San Francisco. The release occurred when oleum was being loaded into a nonfuming acid railroad tank car that contained only a rupture disk as a safety device. The tank car was overheated and this rupture disk blew. The resulting cloud of sulfuric acid drifted northeast with prevailing winds over a number of populated areas. More than 3,000 people subsequently sought medical attention for burning eyes, coughing, headaches, and nausea. Almost all were treated and released on the day of the spill. By the day after the release, another 5,000 people had sought medical attention. The spill forced the closure of five freeways in the region as well as some Bay Area Rapid Transit System stations. Apart from corrosive toxicity, there is the additional hazard that the reactions of sulfur trioxide and sulfuric acid vapors with water are extremely exothermic [10, 11]. While the vapors are intrinsically denser than air, there is thus the likelihood of strong, warming-induced buoyancy from reactions with ambient water vapor, water-containing aerosol droplets, and wet environmental surface. Nordin [12] relates just such an occurrence following the Richmond, CA spill, with the plume observed to rise to 300 m. For all practical purposes, sulfur trioxide was the constituent released from the heated tank

Grant, K E

2008-02-07T23:59:59.000Z

189

Automated solar cell assembly teamed process research. Semiannual subcontract report, December 6, 1993--June 30, 1994  

SciTech Connect

This is the second Semiannual Technical Progress Report for the program titled `Automated Solar Cell Assembly Teamed Process Research` funded under National Renewable Energy Laboratory (NREL) subcontract No. ZAG-3-11219-01. This report describes the work done on Phase II of the program in the period from December 6, 1993 to June 30, 1994. Spire`s objective in this program is to develop high throughput (5 MW/yr) automated processes for interconnecting thin (200 {mu}m) silicon solar cells. High yield will be achieved with these fragile cells through the development of low mechanical stress and low thermal stress processes. For example, a machine vision system is being developed for cell alignment without mechanically contacting the cell edges, while a new soldering process is being developed to solder metal interconnect ribbons simultaneously to a cells` front and back contacts, eliminating one of the two heating steps normally used for soldering each cell.

Nowlan, M. [Spire Corp., Bedford, MA (United States)

1995-01-01T23:59:59.000Z

190

Aerosols in a Changing Atmosphere: From Detailed Aerosol Microphysics to  

NLE Websites -- All DOE Office Websites (Extended Search)

Aerosols in a Changing Atmosphere: From Detailed Aerosol Microphysics to Aerosols in a Changing Atmosphere: From Detailed Aerosol Microphysics to Policy Applications Speaker(s): Susanne Bauer Date: December 6, 2011 - 4:00pm Location: 90-4133 Seminar Host/Point of Contact: Surabi Menon The anthropogenic increase in aerosol concentrations since preindustrial times and its net cooling effect on the atmosphere is thought to mask some of the greenhouse gas induced warming. Although the overall effect of aerosols on solar radiation and clouds is most certainly negative, some individual forcing agents and feedbacks have positive forcing effects. Recent studies have tried to identify some of those positive forcing agents and their individual emission sectors, However, understanding the net effect of multi-source emitting sectors and the involved cloud feedbacks is

191

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Anthropogenic Aerosols: a Clearer Understanding Anthropogenic Aerosols: a Clearer Understanding Submitter: Daum, P., Brookhaven National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Liu, Y., and P. H. Daum, 2002: "Indirect warming effect from dispersion forcing," Nature 419(6872):580-581. Figure 1. Key = Green symbols: triangle - FIRE, northeastern Pacific; Crossed circles - SOCEX, Southern Ocean; Filled circle - ACE1, Southern Ocean; Blue symbols: Filled circles - ASTEX 8, northeastern Atlantic; Diamonds - SCMS 8, Florida coast; Filled triangles - Sounding 9, ASTEX; Filled squares - horizontal 9, ASTEX; Open inverted triangles - level 1; Open upright triangles - level 2; Open circles - level 3, all from southwest of San Diego 10; open diamonds - SCMS 11; stars - vertical, ASTEX

192

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Dust in the Wind... and the Clouds... and the Atmosphere Dust in the Wind... and the Clouds... and the Atmosphere Submitter: Sassen, K., University of Alaska, Fairbanks Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Sassen, K., P.J. DeMott, J.M. Propsero, and M.R. Poellot, Saharan Dust Storms and Indirect Aerosol Effects on Clouds: CRYSTAL-FACE Results, Geophys. Res. Ltt., 30(12), 1633, doi:10/1029/2003GL017371, 2003. PDL linear depolarization ratio (color scale on top) and relative returned power (in gray scale) of height versus time displays obtained on July 29, 2002, during the CRYSTAL-FACE experiment. Depicted are strong depolarizing upper tropospheric clouds (~10km), aerosols (δ ~.10 to .15) extending up to ~5.5km, and at lower right (scale adjusted to account for signal

193

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

First Measurements of Neutral Atmospheric Cluster and 1-2 Nm Particle First Measurements of Neutral Atmospheric Cluster and 1-2 Nm Particle Number Distributions During Nucleation Events Download a printable PDF Submitter: McMurry, P. ., University of Minnesota Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Jiang J, J Zhao, M Chen, J Scheckman, BJ Williams, FL Eisele, and PH McMurry. 2011. "First measurements of neutral atmospheric cluster and 1-2 nm particle number distributions during nucleation events." Aerosol Science and Technology, 45, doi:10.1080/02786826.2010.546817. Jiang J, M Chen, C Kuang, M Attoui, and PH McMurry. 2011. "Electrical mobility spectrometer using a diethylene glycol condensation particle counter for measurement of aerosol size distributions down to 1 nm."

194

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Indirect Impact of Atmospheric Aerosols on an Ensemble of Deep Convective Indirect Impact of Atmospheric Aerosols on an Ensemble of Deep Convective Clouds Download a printable PDF Submitter: Grabowski, W., NCAR Morrison, H. C., NCAR Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Grabowski WW and H Morrison. 2011. "Indirect impact of atmospheric aerosols in idealized simulations of convective-radiative quasi-equilibrium. Part II: Double-moment microphysics." Journal of Climate, 24, 1897-1912. This paper extends the previous cloud-resolving modeling study concerning the impact of cloud microphysics on convective-radiative quasi-equilibrium (CRQE) over a surface with fixed characteristics and prescribed solar input, both mimicking the mean conditions on Earth. The current study

195

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

a Cloud-Resolving Model to Identify the Role of Aerosols on Clouds a Cloud-Resolving Model to Identify the Role of Aerosols on Clouds and Precipitation Download a printable PDF Submitter: Tao, W., NASA - Goddard Space Flight Center Area of Research: Cloud Distributions/Characterizations Working Group(s): Aerosol, Cloud Modeling Journal Reference: Tao, W.-K., X. Li, A. Khain, T. Matsui, S. Lang, and J. Simpson, 2007: The role of atmospheric aerosol concentration on deep convective precipitation: Cloud-resolving model simulations. J. Geophy. Res., (accepted). Zeng, X., W.-K. Tao, S. Lang, A. Y. Hou, M. Zhang, and J. Simpson, 2007: On the sensitivity of atmospheric ensemble states to cloud microphyics in long-term cloud-resolving model simulations. J. Meteor. Soc. Jpn., (submitted). Figure 1. Dirty environment (or high CCN) enhances precipitation in a

196

Building America Webinar: Sealing of Home Enclosures with Aerosol Particles  

Energy.gov (U.S. Department of Energy (DOE))

This webinar was presented by research team Building Industry Research Alliance (BIRA), and provided information about a project that uses existing aerosol duct sealing technology to seal the entire building enclosure in order to achieve greater airtightness and energy and cost savings.

197

Quantifying the Aerosol Indirect Effect Using Ground-Based Remote Sensors and Models  

NLE Websites -- All DOE Office Websites (Extended Search)

Quantifying the Aerosol Indirect Effect Quantifying the Aerosol Indirect Effect Using Ground-Based Remote Sensors and Models G. Feingold National Oceanic and Atmospheric Administration Environmental Technology Laboratory Boulder, Colorado D. E. Lane Rutgers University Camden, New Jersey Q.-L. Min Atmospheric Sciences Research Center State University of New York Albany, New York Introduction The effect of aerosols on cloud microphysical and radiative properties (the "indirect effect") has the greatest uncertainty of all known climate-forcing mechanisms. Increases in aerosol concentrations result in higher concentrations of cloud condensation nuclei (CCN), increased cloud droplet concentrations, and smaller droplet sizes (Twomey 1974). A possible secondary effect is the suppression of rainfall.

198

ARM - Mobile Aerosol Observing System  

NLE Websites -- All DOE Office Websites (Extended Search)

FacilitiesMobile Aerosol Observing System FacilitiesMobile Aerosol Observing System AMF Information Science Architecture Baseline Instruments AMF1 AMF2 AMF3 Data Operations AMF Fact Sheet Images Contacts AMF Deployments Hyytiälä, Finland, 2014 Manacapuru, Brazil, 2014 Oliktok Point, Alaska, 2013 Los Angeles, California, to Honolulu, Hawaii, 2012 Cape Cod, Massachusetts, 2012 Gan Island, Maldives, 2011 Ganges Valley, India, 2011 Steamboat Springs, Colorado, 2010 Graciosa Island, Azores, 2009-2010 Shouxian, China, 2008 Black Forest, Germany, 2007 Niamey, Niger, 2006 Point Reyes, California, 2005 Mobile Aerosol Observing System Intensive aerosol observations conducted on the campus of Brookhaven National Laboratory on Long Island, New York, using the ARM Mobile Aerosol Observing System. Intensive aerosol observations conducted on the campus of Brookhaven

199

Aerosol Observing System (AOS) Handbook  

SciTech Connect

The Aerosol Observing System (AOS) is a suite of in situ surface measurements of aerosol optical and cloud-forming properties. The instruments measure aerosol properties that influence the earths radiative balance. The primary optical measurements are those of the aerosol scattering and absorption coefficients as a function of particle size and radiation wavelength and cloud condensation nuclei (CCN) measurements as a function of percent supersaturation. Additional measurements include those of the particle number concentration and scattering hygroscopic growth. Aerosol optical measurements are useful for calculating parameters used in radiative forcing calculations such as the aerosol single-scattering albedo, asymmetry parameter, mass scattering efficiency, and hygroscopic growth. CCN measurements are important in cloud microphysical models to predict droplet formation.

Jefferson, A

2011-01-17T23:59:59.000Z

200

Use of Aeronet Aerosol Retrievals to Calculate Clear-Sky Irradiance at the Surface  

NLE Websites -- All DOE Office Websites (Extended Search)

AERONET Aerosol Retrievals to AERONET Aerosol Retrievals to Calculate Clear-Sky Irradiance at the Surface G. L. Schuster National Aeronautics and Space Administration Langley Research Center Hampton, Virginia O. Dubovik National Aeronautics and Space Administration Goddard Space Flight Center Laboratory for Terrestrial Physics Greenbelt, Maryland Motivation The worldwide aerosol robotic network (AERONET) of ground-based radiometers was developed (in part) as a satellite validation tool (Holben et al. 1998). These sites utilize spectral sky-scanning radiometers, providing more information for aerosol retrievals than conventional sunphotometer measurements. The use of the almucantar sky radiance scans in conjunction with the aerosol optical thicknesses are the basis of the AERONET Dubovik retrievals, which provide the aerosol size

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201

Experimental study of nuclear workplace aerosol samplers  

E-Print Network (OSTI)

LITERATURE REVIEW Aerosol Losses in an Inlet . Aerosol Losses in a Transport System Aerosol Losses in CAMs Critical Flow Venturi 8 13 15 16 EXPERIMENT PROCEDURE 18 CAM Evaluation Consideration FAS Evaluation Consideration Test Protocol Mixing... Chamber Setup High Speed Aerosol Wind Tunnel Setup Low Speed Aerosol Wind Tunnel Setup Critical Flow Venturi 18 19 21 22 24 25 27 RESULTS AND DISCUSSION Page 28 Aerosol Penetration through Transport Systems and CAM Areal Uniformity Deposits...

Parulian, Antony

2012-06-07T23:59:59.000Z

202

EMSL: Science: Atmospheric Aerosol Systems  

NLE Websites -- All DOE Office Websites (Extended Search)

Atmospheric Aerosol Systems Atmospheric Aerosol Systems atmospheric logo Nighttime enhancement of nitrogen-containing organic compounds, or NOC Observed nighttime enhancement of nitrogen-containing organic compounds, or NOC, showed evidence of being formed by reactions that transform carbonyls into imines. The Atmospheric Aerosol Systems Science Theme focuses on understanding the chemistry, physics and molecular-scale dynamics of aerosols for model parameterization to improve the accuracy of climate model simulations and develop a predictive understanding of climate. By elucidating the role of natural and anthropogenic regional and global climate forcing mechanisms, EMSL can provide DOE and others with the ability to develop cost-effective strategies to monitor, control and mitigate them.

203

ARM Cloud Aerosol Precipitation Experiment  

NLE Websites -- All DOE Office Websites (Extended Search)

Satellite Observation CAS Cloud Aerosol Spectrometer CCN Cloud Condensation Nuclei CIP Cloud Imaging Probe CPC Condensation Particle Counter CSPHOT Cimel sunphotometer CVI...

204

Exploratory Research on Novel Coal Liquefaction Concept - Task 2: Evaluation of Process Steps.  

SciTech Connect

A novel direct coal liquefaction technology is being investigated in a program being conducted by CONSOL Inc. with the University of Kentucky, Center for Applied Energy Research and LDP Associates under DOE Contract DE-AC22-95PC95050. The novel concept consists of a new approach to coal liquefaction chemistry which avoids some of the inherent limitations of current high-temperature thermal liquefaction processes. The chemistry employed is based on hydride ion donation to solubilize coal at temperatures (350-400{degrees}C) significantly lower than those typically used in conventional coal liquefaction. The process concept being explored consists of two reaction stages. In the first stage, the coal is solubilized by hydride ion donation. In the second, the products are catalytically upgraded to acceptable refinery feedstocks. The program explores not only the initial solubilization step, but integration of the subsequent processing steps, including an interstage solids-separation step, to produce distillate products. A unique feature of the process concept is that many of the individual reaction steps can be decoupled, because little recycle around the liquefaction system is expected. This allows for considerable latitude in the process design. Furthermore, this has allowed for each key element in the process to be explored independently in laboratory work conducted under Task 2 of the program.

Brandes, S.D.; Winschel, R.A.

1997-05-01T23:59:59.000Z

205

Molecular Characterization of Biomass Burning Aerosols Using...  

NLE Websites -- All DOE Office Websites (Extended Search)

Biomass Burning Aerosols Using High Resolution Mass Spectrometry. Molecular Characterization of Biomass Burning Aerosols Using High Resolution Mass Spectrometry. Abstract: Chemical...

206

VERIFICATION SURVEY ACTIVITIES IN FS SURVEY UNITS 7, 8, 9, 10, 11, 13 & 14 AT THE SEPARATIONS PROCESS RESEARCH UNIT  

SciTech Connect

FINAL INTERIM REPORT VERIFICATION SURVEY ACTIVITIES IN FINAL STATUS SURVEY UNITS 7, 8, 9, 10, 11, 13 AND 14 AT THE SEPARATIONS PROCESS RESEARCH UNIT, Niskayuna, New York 0496-SR-03-0. The Separations Process Research Unit (SPRU) facilities were constructed in the late 1940s to research the chemical separation of plutonium and uranium. SPRU operated between February 1950 and October 1953. The research activities ceased following the successful development of the reduction/oxidation and plutonium/uranium extraction processes that were subsequently used by the Hanford and the Savannah River sites.

M.G. JADICK

2010-05-26T23:59:59.000Z

207

A Scalable Turbulent Mixing Aerosol Reactor for Oxide-Coated Silicon Nanoparticles  

E-Print Network (OSTI)

of Technology, 391 South Holliston Avenue, Pasadena, California 91125 A new, turbulent flow aerosol reactor. These composite nanoparticles were synthesized under clean conditions, deposited on 200 mm diameter silicon wafers aerosol technology is routinely integrated into microelectronics processing. Foremost is reluctance

Atwater, Harry

208

Currently, there is a substantial research and development effort directed toward optical signal processing and electronic signal processing for fiber-optic communications. Much of the work  

E-Print Network (OSTI)

Abstract Currently, there is a substantial research and development effort directed toward optical signal processing and electronic signal processing for fiber-optic communications. Much of the work for telecommunication services. For optical signal proc- essing, a variety of approaches are available for implementing

Wu, Shin-Tson

209

Parameterizations of Cloud Microphysics and Indirect Aerosol Effects  

SciTech Connect

1. OVERVIEW Aerosols and especially their effect on clouds are one of the key components of the climate system and the hydrological cycle [Ramanathan et al., 2001]. Yet, the aerosol effect on clouds remains largely unknown and the processes involved not well understood. A recent report published by the National Academy of Science states "The greatest uncertainty about the aerosol climate forcing - indeed, the largest of all the uncertainties about global climate forcing - is probably the indirect effect of aerosols on clouds [NRC, 2001]." The aerosol effect on clouds is often categorized into the traditional "first indirect (i.e., Twomey)" effect on the cloud droplet sizes for a constant liquid water path [Twomey, 1977] and the "semi-direct" effect on cloud coverage [e.g., Ackerman et al., 2000]. Enhanced aerosol concentrations can also suppress warm rain processes by producing a narrow droplet spectrum that inhibits collision and coalescence processes [e.g., Squires and Twomey, 1961; Warner and Twomey, 1967; Warner, 1968; Rosenfeld, 1999]. The aerosol effect on precipitation processes, also known as the second type of aerosol indirect effect [Albrecht, 1989], is even more complex, especially for mixed-phase convective clouds. Table 1 summarizes the key observational studies identifying the microphysical properties, cloud characteristics, thermodynamics and dynamics associated with cloud systems from high-aerosol continental environments. For example, atmospheric aerosol concentrations can influence cloud droplet size distributions, warm-rain process, cold-rain process, cloud-top height, the depth of the mixed phase region, and occurrence of lightning. In addition, high aerosol concentrations in urban environments could affect precipitation variability by providing an enhanced source of cloud condensation nuclei (CCN). Hypotheses have been developed to explain the effect of urban regions on convection and precipitation [van den Heever and Cotton, 2007 and Shepherd, 2005]. Recently, a detailed spectral-bin microphysical scheme was implemented into the Goddard Cumulus Ensemble (GCE) model. Atmospheric aerosols are also described using number density size-distribution functions. A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep tropical clouds in the west Pacific warm pool region and summertime convection over a mid-latitude continent with different concentrations of CCN: a low "clean" concentration and a high "dirty" concentration. The impact of atmospheric aerosol concentration on cloud and precipitation will be investigated. 2. MODEL DESCRIPTION AND CASE STUDIES 2.1 GCE MODEL The model used in this study is the 2D version of the GCE model. Modeled flow is anelastic. Second- or higher-order advection schemes can produce negative values in the solution. Thus, a Multi-dimensional Positive Definite Advection Transport Algorithm (MPDATA) has been implemented into the model. All scalar variables (potential temperature, water vapor, turbulent coefficient and all five hydrometeor classes) use forward time differencing and the MPDATA for advection. Dynamic variables, u, v and w, use a second-order accurate advection scheme and a leapfrog time integration (kinetic energy semi-conserving method). Short-wave (solar) and long-wave radiation as well as a subgrid-scale TKE turbulence scheme are also included in the model. Details of the model can be found in Tao and Simpson (1993) and Tao et al. (2003). 2.2 Microphysics (Bin Model) The formulation of the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (cloud droplets and raindrops), and six types of ice particles: pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail. Each type is described by a special size distribution function containing 33 categories (bin

Tao, Wei-Kuo [NASA/GSFC] [NASA/GSFC

2014-05-19T23:59:59.000Z

210

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Weather and Atmospheric Overview During Study of Natural and Urban Weather and Atmospheric Overview During Study of Natural and Urban Emissions (CARES) Download a printable PDF Submitter: Fast, J. ., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Fast JD, WI Gustafson, LK Berg, WJ Shaw, M Pekour, M Shrivastava, JC Barnard, RA Ferrare, CA Hostetler, JA Hair, M Erickson, BT Jobson, B Flowers, MK Dubey, S Springston, RB Pierce, L Dolislager, J Pederson, and RA Zaveri. 2012. "Transport and mixing patterns over central California during the Carbonaceous Aerosol and Radiative Effects Study (CARES)." Atmospheric Chemistry and Physics, 12, 1759-1783. Aircraft sampling flight patterns are shown over central California in this aerial overlay. Researchers collected and analyzed measurements from

211

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Wildfires Lead to More Warming Than Climate Models Predict, a New Mexico Wildfires Lead to More Warming Than Climate Models Predict, a New Mexico Fire Study Reports Download a printable PDF Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: China S, C Mazzoleni, K Gorkowski, AC Aiken, and MK Dubey. 2013. "Morphology and mixing state of individual freshly emitted wildfire carbonaceous particles." Nature Communications, 4, 2122, doi:10.1038/ncomms3122. La Conchas fire, New Mexico Analyzing fresh, carbon-rich aerosols in smoke from the largest wildfire in New Mexico (2011), scientists report large impacts of wildfires on climate. A research study, published last week in Nature Communications, has revealed that smoke from wildfires, or biomass-burning events, contains

212

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Cumuli Impact on Solar Radiation at Surface: Spectral Changes Cumuli Impact on Solar Radiation at Surface: Spectral Changes Download a printable PDF Submitter: Kassianov, E., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle, Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Kassianov E, J Barnard, LK Berg, CN Long, and C Flynn. 2011. "Shortwave spectral radiative forcing of cumulus clouds from surface observations." Geophysical Research Letters, 38, L07801, doi:10.1029/2010GL046282. Figure 1. Normalized total cloud radiative forcing and its direct and diffuse components as a function of wavelength. Typically, under cloudy conditions, radiative transfer parameterizations in climate models have been evaluated by calculating the total cloud impact on

213

Secondary Aerosol: Precursors and Formation Mechanisms. Technical Report on Grant  

SciTech Connect

This project focused on studying trace gases that participate in chemical reactions that form atmospheric aerosols. Ammonium sulfate is a major constituent of these tiny particles, and one important pathway to sulfate formation is oxidation of dissolved sulfur dioxide by hydrogen peroxide in cloud, fog and rainwater. Sulfate aerosols influence the number and size of cloud droplets, and since these factors determine cloud radiative properties, sulfate aerosols also influence climate. Peroxide measurements, in conjunction with those of other gaseous species, can used to distinguish the contribution of in-cloud reaction to new sulfate aerosol formation from gas-phase nucleation reactions. This will lead to more reliable global climate models. We constructed and tested a new 4-channel fluorescence detector for airborne detection of peroxides. We integrated the instrument on the G-1 in January, 2006 and took a test flight in anticipation of the MAX-Mex field program, where we planned to fly under pressurized conditions for the first time. We participated in the 2006 Megacity Initiative: Local and Global Research Observations (MILAGRO) - Megacity Aerosol EXperiment ?? Mexico City (MAX-Mex) field measurement campaign. Peroxide instrumentation was deployed on the DOE G-1 research aircraft based in Veracruz, and at the surface site at Tecamac University.

Weinstein-Lloyd, Judith B

2009-05-04T23:59:59.000Z

214

Aerosol Laboratory - Nuclear Engineering Division (Argonne)  

NLE Websites -- All DOE Office Websites (Extended Search)

Capabilities > Engineering Capabilities > Engineering Experimentation > Aerosol Laboratory Capabilities Engineering Experimentation Reactor Safety Experimentation Aerosol Experiments System Components Laser Applications Robots Applications Other Facilities Other Capabilities Work with Argonne Contact us For Employees Site Map Help Join us on Facebook Follow us on Twitter NE on Flickr Aerosol Laboratory The Aerosol Laboratory (AL) houses equipment to measure and record the physical parameters necessary to characterize the formation and transport of aerosols. Bookmark and Share The Aerosol Laboratory (AL) has extensive analytic and experimental capabilities to characterize the formation and transport of aerosols formed from the condensation of vapors. Computer codes have been developed to

215

Measurement and Modeling of Vertically Resolved Aerosol Optical Properties and Radiative Fluxes Over the ARM SGP Site During the May 2003 Aerosol IOP  

NLE Websites -- All DOE Office Websites (Extended Search)

Measurement and Modeling Measurement and Modeling of Vertically Resolved Aerosol Optical Properties and Radiative Fluxes Over the ARM SGP Site During the May 2003 Aerosol IOP B. Schmid and J. Redemann Bay Area Environmental Research Institute National Aeronautics and Space Administration Ames Research Center Moffett Field, California W. P. Arnott Desert Research Institute Reno, Nevada A. Bucholtz and J. Reid Naval Research Laboratory Monterey, California P. Colarco Earth System Science Interdisciplinary Center University of Maryland College Park, Maryland D. Covert and R. Elleman University of Washington Seattle, Washington J. Eilers, P. Pilewskie, and A. Strawa National Aeronautics and Space Administration Ames, Research Center Moffett Field, California R. A. Ferrare

216

A new scenario framework for climate change research: background, process, and future directions  

SciTech Connect

The scientific community is developing new integrated global, regional, and sectoral scenarios to facilitate interdisciplinary research and assessment to explore the range of possible future climates and related physical changes could pose to human and natural systems; how these could interact with social, economic, and environmental development pathways; the degree to which mitigation and adaptation policies can avoid and reduce those risks; the costs and benefits of various policy mixes; residual impacts under alternative pathways; and the relationship with sustainable development. This paper provides the background to, and process of, developing the conceptual framework for these scenarios, described in three other papers in this Special Issue (van Vuuren et al.; O'Neill et al.; Kriegler et al.). The paper also discusses research needs to further develop and apply this framework. The goal is to encourage climate change researchers from a broad range of perspectives and disciplines to work together to develop policy-relevant scenarios and explore the implications of different possible futures for the challenges and opportunities human and natural systems could face with increasing climate change.

Ebi, Kristie L.; Hallegatte, Stephane; Kram, Tom; Arnell, Nigel; Carter, Tim; Edmonds, James A.; Kriegler, Elmar; Mathur, Ritu; O'Neill, Brian; Riahi, Keywan; Winkler, Harald; Van Vuuren, Detlef; Zwickel, Timm

2014-02-01T23:59:59.000Z

217

Assessing the Effects of Anthropogenic Aerosols on Pacific Storm Track Using a Multiscale Global Climate Model  

SciTech Connect

Atmospheric aerosols impact weather and global general circulation by modifying cloud and precipitation processes, but the magnitude of cloud adjustment by aerosols remains poorly quantified and represents the largest uncertainty in estimated forcing of climate change. Here we assess the impacts of anthropogenic aerosols on the Pacific storm track using a multi-scale global aerosol-climate model (GCM). Simulations of two aerosol scenarios corresponding to the present day and pre-industrial conditions reveal long-range transport of anthropogenic aerosols across the north Pacific and large resulting changes in the aerosol optical depth, cloud droplet number concentration, and cloud and ice water paths. Shortwave and longwave cloud radiative forcing at the top of atmosphere are changed by - 2.5 and + 1.3 W m-2, respectively, by emission changes from pre-industrial to present day, and an increased cloud-top height indicates invigorated mid-latitude cyclones. The overall increased precipitation and poleward heat transport reflect intensification of the Pacific storm track by anthropogenic aerosols. Hence, this work provides for the first time a global perspective of the impacts of Asian pollution outflows from GCMs. Furthermore, our results suggest that the multi-scale modeling framework is essential in producing the aerosol invigoration effect of deep convective clouds on the global scale.

Wang, Yuan; Wang, Minghuai; Zhang, Renyi; Ghan, Steven J.; Lin, Yun; Hu, Jiaxi; Pan, Bowen; Levy, Misti; Jiang, Jonathan; Molina, Mario J.

2014-05-13T23:59:59.000Z

218

Determination of particulate lead using aerosol mass spectrometry: MILAGRO/MCMA-2006 observations  

E-Print Network (OSTI)

We report the first measurements of particulate lead (Pb) from Aerodyne Aerosol Mass Spectrometers, which were deployed in and around Mexico City during the Megacity Initiative: Local and Global Research Observations ...

Salcedo, D.

219

The Design-Build Process for the Research Support Facility (RSF), Energy Efficiency & Renewable Energy (EERE)  

NLE Websites -- All DOE Office Websites (Extended Search)

Design-Build Process for Design-Build Process for the Research Support Facility An in-depth look at how the U.S. Department of Energy and the National Renewable Energy Laboratory used a performance-based design-build contract process to build one of the most energy efficient office buildings in the world. Table of Contents The Design-Build Process for the Research Support Facility | 1 Table of Contents Executive Summary . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2 Building Features . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 7 Owner Roles and Responsibilities . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 17 Acquisition Strategy . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 19 Defining Performance Objectives . . . . . . . . . . . . . . . . . . . . . . . .

220

Cover image: Research within Pacific Northwest National Laboratory's Chemical Imaging Initiative is characterizing chemical and physical interactions of biofilms produced by microbes. This information is used to provide insight on  

E-Print Network (OSTI)

depth biofilm fermenter. #12;Douglas Ray, Ph.D. Associate Laboratory Director Fundamental, energy materials and processes, and atmospheric aerosol research. Our technical leadership of another DOE fundamental research and technology development of natural and engineered biological systems in the laboratory

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


221

Correction to Hyperspectral Aerosol Optical Depths from TCAP Flights  

SciTech Connect

In the paper Hyperspectral aerosol optical depths from TCAP flights by Y. Shinozuka et al. (Journal of Geophysical Research: Atmospheres, 118, doi:10.1002/2013JD020596, 2013), Tables 1 and 2 were published with the column heads out of order. Tables 1 and 2 are published correctly here. The publisher regrets the error.

Shinozuka, Yohei; Johnson, Roy R.; Flynn, Connor J.; Russell, P. B.; Schmid, Beat; Redemann, Jens; Dunagan, Stephen; Kluzek, Celine D.; Hubbe, John M.; Segal-Rosenheimer, Michal; Livingston, J. M.; Eck, T.; Wagener, Richard; Gregory, L.; Chand, Duli; Berg, Larry K.; Rogers, Ray; Ferrare, R. A.; Hair, John; Hostetler, Chris A.; Burton, S. P.

2014-02-16T23:59:59.000Z

222

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Aerosol Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Xu L, LM Russell, RC Somerville, and PK Quinn. 2013. "Frost flower aerosol effects on Arctic...

223

Ganges Valley Aerosol Experiment: Science and Operations Plan  

SciTech Connect

The Ganges Valley region is one of the largest and most rapidly developing sections of the Indian subcontinent. The Ganges River, which provides the region with water needed for sustaining life, is fed primarily by snow and rainfall associated with Indian summer monsoons. Impacts of changes in precipitation patterns, temperature, and the flow of the snow-fed rivers can be immense. Recent satellite-based measurements have indicated that the upper Ganges Valley has some of the highest persistently observed aerosol optical depth values. The aerosol layer covers a vast region, extending across the Indo-Gangetic Plain to the Bay of Bengal during the winter and early spring of each year. The persistent winter fog in the region is already a cause of much concern, and several studies have been proposed to understand the economic, scientific, and societal dimensions of this problem. During the INDian Ocean EXperiment (INDOEX) field studies, aerosols from this region were shown to affect cloud formation and monsoon activity over the Indian Ocean. This is one of the few regions showing a trend toward increasing surface dimming and enhanced mid-tropospheric warming. Increasing air pollution over this region could modify the radiative balance through direct, indirect, and semi-indirect effects associated with aerosols. The consequences of aerosols and associated pollution for surface insolation over the Ganges Valley and monsoons, in particular, are not well understood. The proposed field study is designed for use of (1) the ARM Mobile Facility (AMF) to measure relevant radiative, cloud, convection, and aerosol optical characteristics over mainland India during an extended period of 912 months and (2) the G-1 aircraft and surface sites to measure relevant aerosol chemical, physical, and optical characteristics in the Ganges Valley during a period of 612 weeks. The aerosols in this region have complex sources, including burning of coal, biomass, and biofuels; automobile emissions; and dust. The extended AMF deployment will enable measurements under different regimes of the climate and aerosol abundancein the wet monsoon period with low aerosol loading; in the dry, hot summer with aerosols dispersed throughout the atmospheric column; and in the cool, dry winter with aerosols confined mostly to the boundary later and mid-troposphere. Each regime, in addition, has its own distinct radiative and atmospheric dynamic drivers. The aircraft operational phase will assist in characterizing the aerosols at times when they have been observed to be at the highest concentrations. A number of agencies in India will collaborate with the proposed field study and provide support in terms of planning, aircraft measurements, and surface sites. The high concentration of aerosols in the upper Ganges Valley, together with hypotheses involving several possible mechanisms with direct impacts on the hydrologic cycle of the region, gives us a unique opportunity to generate data sets that will be useful both in understanding the processes at work and in providing answers regarding the effects of aerosols on climate in a region where the perturbation is the highest.

Kotamarthi, VR

2010-06-21T23:59:59.000Z

224

Final Project Report - ARM CLASIC CIRPAS Twin Otter Aerosol  

SciTech Connect

The NOAA/ESRL/GMD aerosol group made three types of contributions related to airborne measurements of aerosol light scattering and absorption for the Cloud and Land Surface Interaction Campaign (CLASIC) in June 2007 on the Twin Otter research airplane operated by the Center for Interdisciplinary Remotely-Piloted Aircraft Studies (CIRPAS). GMD scientists served as the instrument mentor for the integrating nephelometer and particle soot absorption photometer (PSAP) on the Twin Otter during CLASIC, and were responsible for (1) instrument checks/comparisons; (2) instrument trouble shooting/repair; and (3) data quality control (QC) and submittal to the archive.

John A. Ogren

2010-04-05T23:59:59.000Z

225

DR. DAVID J. DELENE ASSISTANT RESEARCH PROFESSOR  

E-Print Network (OSTI)

Zealand, West Africa and Saudi Arabia. RESEARCH INTERESTS: Atmospheric aerosols, cloud physics, weather: Current Research Projects Weather Modification Research in Saudi Arabia The project's goal is to access the microphysics of precipitation formation in the Saudi Arabia region. Airborne measurements of aerosol and cloud

Delene, David J.

226

Aerosols and Clouds: In Cahoots to Change Climate  

ScienceCinema (OSTI)

Key knowledge gaps persist despite advances in the scientific understanding of how aerosols and clouds evolve and affect climate. The Two-Column Aerosol Project, or TCAP, was designed to provide a detailed set of observations to tackle this area of unknowns. Led by PNNL atmospheric scientist Larry Berg, ARM's Climate Research Facility was deployed in Cape Cod, Massachusetts for the 12-month duration of TCAP, which came to a close in June 2013. "We are developing new tools to look at particle chemistry, like our mass spectrometer used in TCAP that can tell us the individual chemical composition of an aerosol," said Berg. "Then, we'll run our models and compare it with the data that we have to make sure we're getting correct answers and make sure our climate models are reflecting the best information."

Berg, Larry

2014-06-02T23:59:59.000Z

227

CARES: Carbonaceous Aerosol and Radiative Effects Study Operations Plan  

SciTech Connect

The CARES field campaign is motivated by the scientific issues described in the CARES Science Plan. The primary objectives of this field campaign are to investigate the evolution and aging of carbonaceous aerosols and their climate-affecting properties in the urban plume of Sacramento, California, a mid-size, mid-latitude city that is located upwind of a biogenic volatile organic compound (VOC) emission region. Our basic observational strategy is to make comprehensive gas, aerosol, and meteorological measurements upwind, within, and downwind of the urban area with the DOE G-1 aircraft and at strategically located ground sites so as to study the evolution of urban aerosols as they age and mix with biogenic SOA precursors. The NASA B-200 aircraft, equipped with the High Spectral Resolution Lidar (HSRL), digital camera, and the Research Scanning Polarimeter (RSP), will be flown in coordination with the G-1 to characterize the vertical and horizontal distribution of aerosols and aerosol optical properties, and to provide the vertical context for the G-1 and ground in situ measurements.

Zaveri, RA; Shaw, WJ; Cziczo, DJ

2010-07-12T23:59:59.000Z

228

The impact of biogenic carbon emissions on aerosol absorption inMexico City  

SciTech Connect

In order to determine the wavelength dependence of atmospheric aerosol absorption in the Mexico City area, the absorption angstrom exponents (AAEs) were calculated from aerosol absorption measurements at seven wavelengths obtained with a seven-channel aethalometer during two field campaigns, the Mexico City Metropolitan Area study in April 2003 (MCMA 2003) and the Megacity Initiative: Local and Global Research Observations in March 2006 (MILAGRO). The AAEs varied from 0.76 to 1.56 in 2003 and from 0.54 to 1.52 in 2006. The AAE values determined in the afternoon were consistently higher than the corresponding morning values, suggesting the photochemical formation of absorbing secondary organic aerosols (SOA) in the afternoon. The AAE values were compared to stable and radiocarbon isotopic measurements of aerosol samples collected at the same time to determine the sources of the aerosol carbon. The fraction of modern carbon (fM) in the aerosol samples, as determined from {sup 14}C analysis, showed that 70% of the carbonaceous aerosols in Mexico City were from modern sources, indicating a significant impact from biomass burning during both field campaigns. The {sup 13}C/{sup 12}C ratios of the aerosol samples illustrate the significant impact of Yucatan forest fires (C-3 plants) in 2003 and local grass fires (C-4 plants) at site T1 in 2006. A direct comparison of the fM values, stable carbon isotope ratios, and calculated aerosol AAEs suggested that the wavelength dependence of the aerosol absorption was controlled by the biogenically derived aerosol components.

Marley, N; Gaffney, J; Tackett, M J; Sturchio, N; Hearty, L; Martinez, N; Hardy, K D; Machany-Rivera, A; Guilderson, T P; MacMillan, A; Steelman, K

2009-02-24T23:59:59.000Z

229

Aerosol Processes Enabling Solar Energy Applications.  

E-Print Network (OSTI)

??Development of alternative energy sources is essential to satisfy future energy demands. While remaining fossil fuel resources may substantially meet these demands, anthropogenic carbon dioxide: (more)

An, Woo Jin

2012-01-01T23:59:59.000Z

230

Atmospheric Science Program Cumulus Humilis Aerosol Processing...  

NLE Websites -- All DOE Office Websites (Extended Search)

term used to describe the small fair weather clouds that dot the summer skies over Oklahoma. During the month of June, scientists sponsored by the U.S. Department of Energy's...

231

ARM - Surface Aerosol Observing System  

NLE Websites -- All DOE Office Websites (Extended Search)

FacilitiesSurface Aerosol Observing System FacilitiesSurface Aerosol Observing System AMF Information Science Architecture Baseline Instruments AMF1 AMF2 AMF3 Data Operations AMF Fact Sheet Images Contacts AMF Deployments Hyytiälä, Finland, 2014 Manacapuru, Brazil, 2014 Oliktok Point, Alaska, 2013 Los Angeles, California, to Honolulu, Hawaii, 2012 Cape Cod, Massachusetts, 2012 Gan Island, Maldives, 2011 Ganges Valley, India, 2011 Steamboat Springs, Colorado, 2010 Graciosa Island, Azores, 2009-2010 Shouxian, China, 2008 Black Forest, Germany, 2007 Niamey, Niger, 2006 Point Reyes, California, 2005 Surface Aerosol Observing System The ARM Mobile Facility (AMF) is equipped to quantify the interaction between clouds and aerosol particles. A counter-flow virtual impactor (CVI) is used to selectively sample cloud drops. The CVI takes advantage of the

232

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

When Pollution Gets a Whiff of Trees When Pollution Gets a Whiff of Trees Download a printable PDF Submitter: Shilling, J., Pacific Northwest National Laboratory Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Shilling JE, RA Zaveri, JD Fast, L Kleinman, M Alexander, MR Canagaratna, E Fortner, JM Hubbe, JT Jayne, A Sedlacek, A Setyan, S Springston, DR Worsnop, and Q Zhang. 2013. "Enhanced SOA formation from mixed anthropogenic and biogenic emissions during the CARES campaign." Atmospheric Chemistry and Physics, 13, doi:10.5194/acp-13-2091-2013. Organic aerosols from tree emissions increase when mixed with manmade sources, impacting the climate. It's easy to visualize particles and gases from vehicle exhaust or burning trash wafting into the atmosphere. It's harder to envision similar gases

233

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Can Ice-Nucleating Aerosols Affect Arctic Seasonal Climate? Can Ice-Nucleating Aerosols Affect Arctic Seasonal Climate? Submitter: Prenni, A. J., Colorado State University Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Properties Journal Reference: Prenni, A. J., J. Y. Harrington, M. Tjernstrom, P. J. DeMott, A. Avramov, C. N. Long, S. M. Kreidenweis, P. Q. Olsson, and J. Verlinde, (2006): Can Ice-Nucleating Aerosols Affect Arctic Seasonal Climate?, BAMS, Vol.88, Iss. 4; pg. 541-550. ACIA, 2004: Impacts of a Warming Arctic: Arctic Climate Impact Assessment. Cambridge University Press, 1020pp. Additional Key Contact: Long, C. N. , Pacific Northwest National Laboratory Figure 1. Time series for the 2-day simulation plotted over Oliktok Point for Standard IN and M-PACE IN concentrations: (a) liquid water path (g

234

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Influence of Humidified Aerosols on Lidar Depolarization Below Influence of Humidified Aerosols on Lidar Depolarization Below Ice-Precipitating Arctic Clouds Download a printable PDF Submitter: Fridlind, A. M., NASA - Goddard Institute for Space Studies van Diedenhoven, B., NASA - Goddard Institute for Space Studies Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud Life Cycle Journal Reference: van Diedenhoven B, AM Fridlind, and AS Ackerman. 2011. "Influence of humidified aerosol on lidar depolarization measurements below ice-precipitating Arctic stratus." Journal of Applied Meteorology and Climatology, 50(10), doi:10.1175/JAMC-D-11-037.1. Correlated MMCR radar reflectivities and DABUL lidar depolarizations below cloud base calculated with a reasonably low number of large, coarse-mode

235

Energy in low carbon cities and social learning: A process for defining priority research questions with UK stakeholders  

Science Journals Connector (OSTI)

Abstract City-level decision-making requires timely access to a wide range of relevant and comprehensible data and information. Although a wide range of research on energy and cities is on-going across the social, engineering and natural sciences, it cannot be taken for granted that the questions being asked and the way questions are structured reflect practitioner perspectives and requirements. This paper discusses the ways in which research questions are formed and interpreted by actors in academic research and research user communities. We also report a set of research questions produced via an initial trial of a two stage, participative process consisting of (a) a survey targeted at city-focussed practitioners in the United Kingdom (UK) with an interest in lower carbon energy futures; and (b) a workshop integrating practitioner and academic perspectives. Comparing the set of research questions identified with themes in the academic literature, we find that research and practitioner communities concur on the importance of reducing energy demand and also on a number of cross-cutting issues. However, we also find that academic research places a greater emphasis on the interfaces between the energy system and other urban systems. We conclude that the two stage, participative process followed can serve to generate and legitimate city-related research questions through collaboration between stakeholders and academic researchers.

Chris J. Martin; Peter G. Taylor; Paul Upham; Golnoush Ghiasi; Catherine S.E. Bale; Hannah James; Alice Owen; William F. Gale; Rebecca J. Slack; Simon Helmer

2014-01-01T23:59:59.000Z

236

Membrane/distillation hybrid process research and development. Final report, phase II  

SciTech Connect

This report covers work conducted under the grant awarded to BP by DOE in late 1991 entitled {open_quotes}Membrane/Distillation Hybrid Process Research and Development.{close_quotes} The program was directed towards development and commercialization of the BP process for separation of vapor phase olefins from non-olefins via facilitated transport using an aqueous facilitator. The program has come to a very successful conclusion, with formation of a partnership between BP and Stone and Webster Engineering Corporation (SWEC) to market and commercialize the technology. The focus of this report is the final portion of the program, during which engineering re-design, facilitator optimization, economic analysis, and marketing have been the primary activities. At the end of Phase II BP was looking to partner with an engineering firm to advance the selective olefin recovery (SOR) technology from the lab/demo stage to full commercialization. In August 1995 BP and SWEC reached an agreement to advance the technology by completing additional Phase III work with DOE and beginning marketing activities.

Mazanec, T.J.

1997-07-01T23:59:59.000Z

237

Airborne measurements of carbonaceous aerosols in southern Africa during  

NLE Websites -- All DOE Office Websites (Extended Search)

Airborne measurements of carbonaceous aerosols in southern Africa during Airborne measurements of carbonaceous aerosols in southern Africa during the dry, biomass burning season Title Airborne measurements of carbonaceous aerosols in southern Africa during the dry, biomass burning season Publication Type Journal Article LBNL Report Number LBNL-50880 Year of Publication 2003 Authors Kirchstetter, Thomas W., Tihomir Novakov, and Peter V. Hobbs Journal Journal of Geophysical Research - Atmospheres Keywords black carbon, evolved gas analysis, light absorption, organic carbon, positive sampling artifact, SAFARI Abstract Particulate matter collected aboard the University of Washington's Convair-580 research aircraft over southern Africa during the dry, biomass burning season was analyzed for total carbon, organic carbon, and black carbon contents using thermal and optical methods. Samples were collected in smoke plumes of burning savanna and in regional haze. A known artifact, produced by the adsorption of organic gases on the quartz filter substrates used to collect the particulate matter samples, comprised a significant portion of the total carbon collected. Consequently, conclusions derived from the data are greatly dependent on whether or not organic carbon concentrations are corrected for this artifact. For example, the estimated aerosol co-albedo (1 - single scattering albedo), which is a measure of aerosol absorption, of the biomass smoke samples is 60% larger using corrected organic carbon concentrations. Thus, the corrected data imply that the biomass smoke is 60% more absorbing than do the uncorrected data. The black carbon to (corrected) organic carbon mass ratio (BC/OC) of smoke plume samples (0.18±0.06) is lower than that of samples collected in the regional haze (0.25±0.08). The difference may be due to mixing of biomass smoke with background air characterized by a higher BC/OC ratio. A simple source apportionment indicates that biomass smoke contributes about three-quarters of the aerosol burden in the regional haze, while other sources (e.g., fossil fuel burning) contribute the remainder.

238

Oil shale, tar sand, coal research, advanced exploratory process technology, jointly sponsored research. Quarterly technical progress report, July--September 1992  

SciTech Connect

Progress made in five research programs is described. The subtasks in oil shale study include oil shale process studies and unconventional applications and markets for western oil shale.The tar sand study is on recycle oil pyrolysis and extraction (ROPE) process. Four tasks are described in coal research: underground coal gasification; coal combustion; integrated coal processing concepts; and sold waste management. Advanced exploratory process technology includes: advanced process concepts; advanced mitigation concepts; and oil and gas technology. Jointly sponsored research covers: organic and inorganic hazardous waste stabilization; CROW field demonstration with Bell Lumber and Pole; development and validation of a standard test method for sequential batch extraction fluid; PGI demonstration project; operation and evaluation of the CO{sub 2} HUFF-N-PUFF process; fly ash binder for unsurfaced road aggregates; solid state NMR analysis of Mesaverde group, Greater Green River Basin, tight gas sands; flow-loop testing of double-wall pipe for thermal applications; shallow oil production using horizontal wells with enhanced oil recovery techniques; NMR analysis of sample from the ocean drilling program; and menu driven access to the WDEQ hydrologic data management system.

Not Available

1992-12-31T23:59:59.000Z

239

Aerodyne Develops an Aircraft-Deployable Precision Aerosol Analyzer | U.S.  

Office of Science (SC) Website

Aerodyne Develops an Aircraft-Deployable Precision Aerosol Aerodyne Develops an Aircraft-Deployable Precision Aerosol Analyzer Small Business Innovation Research (SBIR) and Small Business Technology Transfer (STTR) SBIR/STTR Home About Funding Opportunity Announcements (FOAs) Applicant and Awardee Resources Commercialization Assistance Other Resources Awards SBIR/STTR Highlights Reporting Fraud Contact Information Small Business Innovation Research and Small Business Technology Transfer U.S. Department of Energy SC-29/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-5707 F: (301) 903-5488 E: sbir-sttr@science.doe.gov More Information » January 2013 Aerodyne Develops an Aircraft-Deployable Precision Aerosol Analyzer Aerodyne Research Inc. develops an aerosol mass spectrometer (AMS) that fills a critical need for size-resolved, quantitative chemical composition

240

Thermophoretic separation of aerosol particles from a sampled gas stream  

DOE Patents (OSTI)

This disclosure relates to separation of aerosol particles from gas samples withdrawn from within a contained atmosphere, such as containment vessels for nuclear reactors or other process equipment where remote gaseous sampling is required. It is specifically directed to separation of dense aerosols including particles of any size and at high mass loadings and high corrosivity. The United States Government has rights in this invention pursuant to Contract DE-AC06-76FF02170 between the US Department of Energy and Westinghouse Electric Corporation.

Postma, A.K.

1984-09-07T23:59:59.000Z

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


241

Thin Film Materials and Processing Techniques for a Next Generation Photovoltaic Device: Cooperative Research and Development Final Report, CRADA Number CRD-12-470  

SciTech Connect

This research extends thin film materials and processes relevant to the development and production of a next generation photovoltaic device.

van Hest, M.

2013-08-01T23:59:59.000Z

242

Transport and Mixing Patterns over Central California during the Carbonaceous Aerosol and Radiative Effects Study (CARES)  

SciTech Connect

We describe the synoptic and regional-scale meteorological conditions that affected the transport and mixing of trace gases and aerosols in the vicinity of Sacramento, California during June 2010 when the Carbonaceous Aerosol and Radiative Effects Study (CARES) was conducted. The meteorological measurements collected by various instruments deployed during the campaign and the performance of the chemistry version of the Weather Research and Forecasting model (WRF-Chem) are both discussed. WRF-Chem was run daily during the campaign to forecast the spatial and temporal variation of carbon monoxide emitted from 20 anthropogenic source regions in California to guide aircraft sampling. The model is shown to reproduce the overall circulations and boundary-layer characteristics in the region, although errors in the upslope wind speed and boundary-layer depth contribute to differences in the observed and simulated carbon monoxide. Thermally-driven upslope flows that transported pollutants from Sacramento over the foothills of the Sierra Nevada occurred every afternoon, except during three periods when the passage of mid-tropospheric troughs disrupted the regional-scales flow patterns. The meteorological conditions after the passage of the third trough were the most favorable for photochemistry and likely formation of secondary organic aerosols. Meteorological measurements and model forecasts indicate that the Sacramento pollutant plume was likely transported over a downwind site that collected trace gas and aerosol measurements during 23 periods; however, direct transport occurred during only eight of these periods. The model also showed that emissions from the San Francisco Bay area transported by intrusions of marine air contributed a large fraction of the carbon monoxide in the vicinity of Sacramento, suggesting that this source likely affects local chemistry. Contributions from other sources of pollutants, such as those in the Sacramento Valley and San Joaquin Valley, were relatively low. Aerosol layering in the free troposphere was observed during the morning by an airborne Lidar; WRF-Chem forecasts showed that mountain venting processes contributed to aged pollutants aloft in the valley atmosphere which then can be entrained into the growing boundary layer the subsequent day.

Fast, Jerome D.; Gustafson, William I.; Berg, Larry K.; Shaw, William J.; Pekour, Mikhail S.; Shrivastava, ManishKumar B.; Barnard, James C.; Ferrare, R.; Hostetler, Chris A.; Hair, John; Erickson, Matthew H.; Jobson, Tom; Flowers, Bradley; Dubey, Manvendra K.; Springston, Stephen R.; Pirce, Bradley R.; Dolislager, Leon; Pederson, J. R.; Zaveri, Rahul A.

2012-02-17T23:59:59.000Z

243

Transport and mixing patterns over Central California during the carbonaceous aerosol and radiative effects study (CARES)  

SciTech Connect

We describe the synoptic and regional-scale meteorological conditions that affected the transport and mixing of trace gases and aerosols in the vicinity of Sacramento, California during June 2010 when the Carbonaceous Aerosol and Radiative Effects Study (CARES) was conducted. The meteorological measurements collected by various instruments deployed during the campaign and the performance of the chemistry version of the Weather Research and Forecasting model (WRF-Chem) are both discussed. WRF-Chem was run daily during the campaign to forecast the spatial and temporal variation of carbon monoxide emitted from 20 anthropogenic source regions in California to guide aircraft sampling. The model is shown to reproduce the overall circulations and boundary-layer characteristics in the region, although errors in the upslope wind speed and boundary-layer depth contribute to differences in the observed and simulated carbon monoxide. Thermally-driven upslope flows that transported pollutants from Sacramento over the foothills of the Sierra Nevada occurred every afternoon, except during three periods when the passage of mid-tropospheric troughs disrupted the regional-scale flow patterns. The meteorological conditions after the passage of the third trough were the most favorable for photochemistry and likely formation of secondary organic aerosols. Meteorological measurements and model forecasts indicate that the Sacramento pollutant plume was likely transported over a downwind site that collected trace gas and aerosol measurements during 23 time periods; however, direct transport occurred during only eight of these periods. The model also showed that emissions from the San Francisco Bay area transported by intrusions of marine air contributed a large fraction of the carbon monoxide in the vicinity of Sacramento, suggesting that this source likely affects local chemistry. Contributions from other sources of pollutants, such as those in the Sacramento Valley and San Joaquin Valley, were relatively low. Aerosol layering in the free troposphere was observed during the morning by an airborne Lidar. WRF-Chem forecasts showed that mountain venting processes contributed to aged pollutants aloft in the valley atmosphere that are then entrained into the growing boundary layer the subsequent day.

Fast J. D.; Springston S.; GustafsonJr., W. I.; Berg, L. K.; Shaw, W. J.; Pekour, M.; Shrivastava, M.; Barnard, J. C.; Ferrare, R. A.; Hostetler, C. A.; Hair, J. A.; Erickson, M.; Jobson, B. T.; Flowers, B.; Dubey, M. K.; Pierce, R. B.; Dolislager, L.; Pederson, J.; Zaveri, R. A.

2012-02-17T23:59:59.000Z

244

Evolution of Asian aerosols during transpacific transport in INTEX-B  

SciTech Connect

Measurements of aerosol composition were made with an Aerodyne High Resolution Time-of-Flight Aerosol Mass Spectrometer (HR-ToF-AMS) on board the NSF/NCAR C-130 aircraft as part of the Intercontinental Chemical Transport Experiment Phase B 5 (INTEX-B) field campaign over the Eastern Pacific Ocean. The HR-ToF-AMS measurements of non-refractory submicron aerosol mass are shown to compare well with other aerosol instrumentation in the INTEX-B field study. Two case studies are described for pollution layers transported across the Pacific from the Asian continent, intercepted 34 days and 710 days downwind of Asia, respectively. Aerosol chemistry is shown to 10 be a robust tracer for air masses originating in Asia, specifically the presence of sulfate dominated aerosol is a distinguishing feature of Asian pollution layers that have been transported to the Eastern Pacific. We examine the time scales of processing for sulfate and organic aerosol in the atmosphere and show that our observations confirm a conceptual model for transpacific transport from Asia proposed by Brock et al. (2004). 15 Our observations of both sulfate and organic aerosol in aged Asian pollution layers are consistent with fast formation near the Asian continent, followed by washout during lofting and subsequent transformation during transport across the Pacific. Our observations are the first atmospheric measurements to indicate that although secondary organic aerosol (SOA) formation from pollution happens on the timescale of one day, 20 the oxidation of organic aerosol continues at longer timescales in the atmosphere. Comparisons with chemical transport models of data from the entire campaign reveal an under-prediction of SOA mass in the MOZART model, but much smaller discrepancies with the GEOS-Chem model than found in previous studies over the Western Pacific. No evidence is found to support a previous hypothesis for significant secondary 25 organic aerosol formation in the free troposphere.

Dunlea, E. J.; DeCarlo, Peter; Aiken, Allison; Kimmel, Joel; Peltier, R. E.; Weber, R. J.; Tomlinson, Jason M.; Collins, Donald R.; Shinozuka, Yohei; McNaughton, C. S.; Howell, S. G.; Clarke, A. D.; Emmons, L.; Apel, Eric; Pfister, G. G.; van Donkelaar, A.; Martin, R. V.; Millet, D. B.; Heald, C. L.; Jimenez, J. L.

2009-10-01T23:59:59.000Z

245

Association of Non-Marine Sulfate Aerosol with Sea Breeze Circulation in Tampa Bay  

Science Journals Connector (OSTI)

Peak concentrations of aerosol sulfur in Tampa, Florida may be the result of either regional-scale transformation and transport processes or local-scale transport from nearby air pollution sources. The existence of the latter has been ...

George S. Young; John W. Winchester

1980-04-01T23:59:59.000Z

246

A Satellite-Based Parameter to Monitor the Aerosol Impact on Convective Clouds  

Science Journals Connector (OSTI)

A method to monitor the aerosol impact on convective clouds using satellite data is presented. The impacts of forest fires and highly polluting megacities on cloud precipitation formation processes are quantified by the vertical extent above ...

Itamar M. Lensky; Ron Drori

2007-05-01T23:59:59.000Z

247

Sealing Ducts in Large Commercial Buildings with Aerosolized Sealant Particles  

NLE Websites -- All DOE Office Websites (Extended Search)

2414 2414 1 Sealing Ducts in Large Commercial Buildings with Aerosolized Sealant Particles M. P. Modera, O. Brzozowski ** , F. R. Carrié * , D. J. Dickerhoff, W. W. Delp, W. J. Fisk, R. Levinson, D. Wang Abstract Electricity energy savings potential by eliminating air leakage from ducts in large commercial buildings is on the order of 10 kWh/m 2 per year (1 kWh/ft 2 ). We have tested, in two large commercial buildings, a new technology that simultaneously seals duct leaks and measures effective leakage area of ducts. The technology is based upon injecting a fog of aerosolized sealant particles into a pressurized duct system. In brief, this process involves blocking all of the intentional openings in a duct system (e.g., diffusers). Therefore, when the system is pressurized, the only place for the air carrying the aerosol

248

Lognormal Size Distribution Theory for Deposition of Polydisperse Aerosol Particles  

SciTech Connect

The moments method of the lognormal size distribution theory was applied to the deposition equation of a radioactive aerosol within a liquid-metal fast breeder reactor for analysis of postulated accidents. The deposition coefficient of Crump and Seinfeld was utilized to represent the Brownian and turbulent diffusions and the gravitational sedimentation. The deposition equation was converted into a set of three ordinary differential equations. This approach takes the view point that the size distribution of an aerosol is represented by a time-dependent lognormal size distribution function during the deposition process. Numerical calculations have been performed, and the results were found to be in good agreement with the exact solution. The derived model for aerosol deposition is convenient to use in a numerical general dynamic equation solution routine based on the moments method, where nucleation, condensation, coagulation, and deposition need to be solved simultaneously.

Park, S.H.; Lee, K.W. [Kwangju Institute of Science and Technology (Korea, Republic of)

2000-07-15T23:59:59.000Z

249

MELCOR 1.8.2 assessment: Aerosol experiments ABCOVE AB5, AB6, AB7, and LACE LA2  

SciTech Connect

The MELCOR computer code has been used to model four of the large-scale aerosol behavior experiments conducted in the Containment System Test Facility (CSTF) vessel. Tests AB5, AB6 and AB7 of the ABCOVE program simulate the dry aerosol conditions during a hypothetical severe accident in an LMFBR. Test LA2 of the LACE program simulates aerosol behavior in a condensing steam environment during a postulated severe accident in an LWR with failure to isolate the containment. The comparison of code results to experimental data show that MELCOR is able to correctly predict most of the thermal-hydraulic results in the four tests. MELCOR predicts reasonably well the dry aerosol behavior of the ABCOVE tests, but significant disagreements are found in the aerosol behavior modelling for the LA2 experiment. These results tend to support some of the concerns about the MELCOR modelling of steam condensation onto aerosols expressed in previous works. During these analyses, a limitation in the MELCOR input was detected for the specification of the aerosol parameters for more than one component. A Latin Hypercube Sampling (LHS) sensitivity study of the aerosol dynamic constants is presented for test AB6. The study shows the importance of the aerosol shape factors in the aerosol deposition behavior, and reveals that MELCOR input/output processing is highly labor intensive for uncertainty and sensitivity analyses based on LHS.

Souto, F.J.; Haskin, F.E. [Univ. of New Mexico, Albuquerque, NM (United States). Dept. of Chemical and Nuclear Engineering; Kmetyk, L.N. [Sandia National Labs., Albuquerque, NM (United States)

1994-10-01T23:59:59.000Z

250

Quantifying the Uncertainties of Aerosol Indirect Effects and Impacts on Decadal-Scale Climate Variability in NCAR CAM5 and CESM1  

SciTech Connect

The main goal of this project is to systematically quantify the major uncertainties of aerosol indirect effects due to the treatment of moist turbulent processes that drive aerosol activation, cloud macrophysics and microphysics in response to anthropogenic aerosol perturbations using the CAM5/CESM1. To achieve this goal, the P.I. hired a postdoctoral research scientist (Dr. Anna Fitch) who started her work from the Nov.1st.2012. In order to achieve the project goal, the first task that the Postdoc. and the P.I. did was to quantify the role of subgrid vertical velocity variance on the activation and nucleation of cloud liquid droplets and ice crystals and its impact on the aerosol indirect effect in CAM5. First, we analyzed various LES cases (from dry stable to cloud-topped PBL) to check whether this isotropic turbulence assumption used in CAM5 is really valid. It turned out that this isotropic turbulence assumption is not universally valid. Consequently, from the analysis of LES, we derived an empirical formulation relaxing the isotropic turbulence assumption used for the CAM5 aerosol activation and ice nucleation, and implemented the empirical formulation into CAM5/CESM1, and tested in the single-column and global simulation modes, and examined how it changed aerosol indirect effects in the CAM5/CESM1. These results were reported in the poster section in the 18th Annual CESM workshop held in Breckenridge, CO during Jun.17-20.2013. While we derived an empirical formulation from the analysis of couple of LES from the first task, the general applicability of that empirical formulation was questionable, because it was obtained from the limited number of LES simulations. The second task we did was to derive a more fundamental analytical formulation relating vertical velocity variance to TKE using other information starting from basic physical principles. This was a somewhat challenging subject, but if this could be done in a successful way, it could be directly implemented into the CAM5 as a practical parameterization, and substantially contributes to achieving the project goal. Through an intensive research for about one year, we found appropriate mathematical formulation and tried to implement it into the CAM5 PBL and activation routine as a practical parameterized numerical code. During these processes, however, the Postdoc applied for another position in Sweden, Europe, and accepted a job offer there, and left NCAR in August 2014. In Sweden, Dr. Anna Fitch is still working on this subject in a part time, planning to finalize the research and to write the paper in a near future.

Park, Sungsu

2014-12-12T23:59:59.000Z

251

Direct and semi-direct aerosol effects of Southern African1 biomass burning aerosol2  

E-Print Network (OSTI)

1 Direct and semi-direct aerosol effects of Southern African1 biomass burning aerosol2 Naoko effects of biomass burning aerosols from Southern African fires9 during July-October are investigated region the overall TOA radiative effect from the23 biomass burning aerosols is almost zero due

Wood, Robert

252

ARM - Evaluation Product - Organic Aerosol Component VAP  

NLE Websites -- All DOE Office Websites (Extended Search)

ProductsOrganic Aerosol Component VAP ProductsOrganic Aerosol Component VAP Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Evaluation Product : Organic Aerosol Component VAP 2011.01.08 - 2012.03.24 Site(s) SGP General Description Organic aerosol (OA, i.e., the organic fraction of particles) accounts for 10-90% of the fine aerosol mass globally and is a key determinant of aerosol radiative forcing. But atmospheric OA is poorly characterized and its life cycle insufficiently represented in models. As a result, current models are unable to simulate OA concentrations and properties. This deficiency represents a large source of uncertainty in the quantification of aerosol direct and indirect effects and the prediction of future climate change. The Organic Aerosol Component (OACOMP) value-added product (VAP) uses

253

ARM - Field Campaign - Fall 1997 Aerosol IOP  

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Aerosol IOP Aerosol IOP Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : Fall 1997 Aerosol IOP 1997.09.15 - 1997.10.05 Lead Scientist : Stephen Schwartz For data sets, see below. Summary The Aerosol IOP was highlighted by the Gulfstream-1 aircraft flying clear-sky aerosol missions over the Central Facility to study the effect of aerosol loading on clear sky radiation fields, with weather particularly favorable for these flights during the first and third weeks of the IOP. A secondary but important goal of this IOP was to fly cloudy-sky missions over the Central Facility to study the effect of aerosol loading on cloud microphysics, and the effect of the microphysics on cloud optical properties. The Gulfstream obtained aerosol data in support of some of the

254

Reflective Aerosols and the Greenhouse Effect  

Science Journals Connector (OSTI)

The contributions of atmospheric aerosols to add to either a climate-warming effect or climate-cooling effect depend on the chemical composition of the aerosol and the local environment. The best estimation is...

Kathryn E. Kautzman

2014-07-01T23:59:59.000Z

255

Antiviral therapy with small particle aerosols  

Science Journals Connector (OSTI)

The generation and use of small particle aqueous aerosols (1.23 m aerodynamic mass median diameter, GSD=2.0 m) containing ribavirin is described. Administered via aerosol, ribavirin will be deposited rather ...

V. Knight; B. Gilbert

1988-12-01T23:59:59.000Z

256

E-Print Network 3.0 - airborne aerosol prediction Sample Search...  

NLE Websites -- All DOE Office Websites (Extended Search)

profiles of aerosol extinction and optical depth Evaluate predictions from aerosol transport... aerosol measurements. Comparison of AOT ... Source: Brookhaven National...

257

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Modified Climate Model Better Replicates Global Rainfall Modified Climate Model Better Replicates Global Rainfall Submitter: Bhattacharya, A., Pacific Northwest National Laboratory Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Song X, GJ Zhang, and JF Li. 2012. "Evaluation of microphysics parameterization for convective clouds in the NCAR Community Atmosphere Model CAM5." Journal of Climate, 25(24), doi:10.1175/JCLI-D-11-00563.1. Rainfall in the tropics. By improving an existing, sophisticated, global climate model, scientists can now simulate cloud and rainfall more accurately. Supported by the U.S. Department of Energy's Atmospheric System Research program, a research team from the Scripps Institution of Oceanography and

258

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Parameterizing the Ice Fall Speed in Climate Models: Results from TC4 and Parameterizing the Ice Fall Speed in Climate Models: Results from TC4 and ISDAC Download a printable PDF Submitter: Mitchell, D. L., Desert Research Institute Mishra, S., NOAA - Coop. Inst. for Mesoscale Meteorological Studies Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Mitchell DL, S Mishra, and RP Lawson. 2011. "Representing the ice fall speed in climate models: Results from Tropical Composition, Cloud and Climate Coupling (TC4) and the Indirect and Semi-Direct Aerosol Campaign (ISDAC)." Journal of Geophysical Research - Atmospheres, 116, D00T03, doi:10.1029/2010JD015433. Relationship between De and Vm for all tropical cirrus cloud types (solid

259

6, 93519388, 2006 Aerosol-cloud  

E-Print Network (OSTI)

ACPD 6, 9351­9388, 2006 Aerosol-cloud interaction inferred from MODIS and models G. Myhre et al Chemistry and Physics Discussions Aerosol-cloud interaction inferred from MODIS satellite data and global 6, 9351­9388, 2006 Aerosol-cloud interaction inferred from MODIS and models G. Myhre et al. Title

Paris-Sud XI, Université de

260

Laboratory Testing of Aerosol for Enclosure Air Sealing  

SciTech Connect

Space conditioning energy use can be significantly reduced by addressing uncontrolled infiltration and exfiltration through the envelope of a building. A process for improving the air tightness of a building envelope by sealing shell leaks with an aerosol sealing technology is presented. Both retrofit and new construction applications are possible through applying this process either in attics and crawlspaces or during rough-in stage.

Harrington, C.; Modera, M.

2012-05-01T23:59:59.000Z

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


261

Novel, Magnetically Fluidized-Bed Reactor Development for the Looping Process: Coal to Hydrogen Production Research and Development  

NLE Websites -- All DOE Office Websites (Extended Search)

Novel, Magnetically Fluidized-Bed Novel, Magnetically Fluidized-Bed Reactor Development for the Looping Process: Coal to Hydrogen Production Research and Development Background The U.S. Department of Energy (DOE) National Energy Technology Laboratory (NETL) is committed to improving methods for co-producing power and chemicals, fuels, and hydrogen (H2). Gasification is a process by which fuels such as coal can be used to produce synthesis gas (syngas), a mixture of H2, carbon monoxide (CO), and carbon

262

ARM - Measurement - Aerosol optical depth  

NLE Websites -- All DOE Office Websites (Extended Search)

depth depth ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol optical depth A measure of how much light aerosols prevent from passing through a column of atmosphere. Categories Aerosols Instruments The above measurement is considered scientifically relevant for the following instruments. Refer to the datastream (netcdf) file headers of each instrument for a list of all available measurements, including those recorded for diagnostic or quality assurance purposes. ARM Instruments HSRL : High Spectral Resolution Lidar MPL : Micropulse Lidar MFRSR : Multifilter Rotating Shadowband Radiometer NIMFR : Normal Incidence Multifilter Radiometer Field Campaign Instruments AOS-PMFOV : Acoustical Optical Spectrometer-Photometer with Multiple

263

ARM - Measurement - Aerosol optical properties  

NLE Websites -- All DOE Office Websites (Extended Search)

properties properties ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol optical properties The optical properties of aerosols, including asymmetry factor, phase-function, single-scattering albedo, refractive index, and backscatter fraction. Categories Aerosols Instruments The above measurement is considered scientifically relevant for the following instruments. Refer to the datastream (netcdf) file headers of each instrument for a list of all available measurements, including those recorded for diagnostic or quality assurance purposes. ARM Instruments CSPHOT : Cimel Sunphotometer NEPHELOMETER : Nephelometer Field Campaign Instruments AOS-PMFOV : Acoustical Optical Spectrometer-Photometer with Multiple

264

ARM - Measurement - Aerosol backscattered radiation  

NLE Websites -- All DOE Office Websites (Extended Search)

backscattered radiation backscattered radiation ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol backscattered radiation The scattering of radiant energy into the hemisphere of space bounded by a plane normal to the direction of the incident radiation and lying on the same side as the incident ray. Categories Aerosols Instruments The above measurement is considered scientifically relevant for the following instruments. Refer to the datastream (netcdf) file headers of each instrument for a list of all available measurements, including those recorded for diagnostic or quality assurance purposes. ARM Instruments AOS : Aerosol Observing System MPL : Micropulse Lidar NEPHELOMETER : Nephelometer

265

The LBL/AGMEF/JSU El Yunque Environmental Research Initiative  

SciTech Connect

The LBL/AGMEF/JSU Environmental Research Initiative has had several noteworthy successes. Faculty and student development is apparent. A research project involving atmospheric aerosol sampling was established at Universidad Metropolitana under Prof. Fernando Diaz. A National Science Foundation grant received to expand upon that project. Review of analyses carried out since 1986 supports the original view that El Yunque peak on the eastern end of Puerto Rico offers a unique site to study atmospheric processes relevant to current national and international concerns regarding global climate modification. Based on this review, a Puerto Rico El Yunque Intensive Summer Research Campaign is proposed. 6 refs.

Dod, R.L.; Diaz, F.; Feliu, L.; Parker, C.D.

1989-03-01T23:59:59.000Z

266

Hyperspectral Aerosol Optical Depths from TCAP Flights  

SciTech Connect

4STAR (Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research), the worlds first hyperspectral airborne tracking sunphotometer, acquired aerosol optical depths (AOD) at 1 Hz during all July 2012 flights of the Two Column Aerosol Project (TCAP). Root-mean square differences from AERONET ground-based observations were 0.01 at wavelengths between 500-1020 nm, 0.02 at 380 and 1640 nm and 0.03 at 440 nm in four clear-sky fly-over events, and similar in ground side-by-side comparisons. Changes in the above-aircraft AOD across 3-km-deep spirals were typically consistent with integrals of coincident in situ (on DOE Gulfstream 1 with 4STAR) and lidar (on NASA B200) extinction measurements within 0.01, 0.03, 0.01, 0.02, 0.02, 0.02 at 355, 450, 532, 550, 700, 1064 nm, respectively, despite atmospheric variations and combined measurement uncertainties. Finer vertical differentials of the 4STAR measurements matched the in situ ambient extinction profile within 14% for one homogeneous column. For the AOD observed between 350-1660 nm, excluding strong water vapor and oxygen absorption bands, estimated uncertainties were ~0.01 and dominated by (then) unpredictable throughput changes, up to +/-0.8%, of the fiber optic rotary joint. The favorable intercomparisons herald 4STARs spatially-resolved high-frequency hyperspectral products as a reliable tool for climate studies and satellite validation.

Shinozuka, Yohei; Johnson, Roy R.; Flynn, Connor J.; Russell, P. B.; Schmid, Beat; Redemann, Jens; Dunagan, Stephen; Kluzek, Celine D.; Hubbe, John M.; Segal-Rosenheimer, Michal; Livingston, J. M.; Eck, T.; Wagener, Richard; Gregory, L.; Chand, Duli; Berg, Larry K.; Rogers, Ray; Ferrare, R. A.; Hair, John; Hostetler, Chris A.; Burton, S. P.

2013-11-13T23:59:59.000Z

267

Research Highlights Sorted by Working Group  

NLE Websites -- All DOE Office Websites (Extended Search)

Working Group Working Group Aerosol Life Cycle | Cloud Life Cycle | Cloud-Aerosol-Precipitation Interactions | Aerosol | Cloud Modeling | Cloud Properties | Radiative Processes Aerosol Life Cycle 2013 Bhattacharya, A. Wildfires Lead to More Warming Than Climate Models Predict, a New Mexico Fire Study Reports ASR Fast, J. . Development and Validation of a Black Carbon Mixing State Resolved Three-Dimensional Model ARM ASR Gilles, M., Moffet, R. Spectro-microscopic Measurements of Carbonaceous Aerosol Aging in Central California ARM ASR Kafle, D. N., Coulter, R. L. Micropulse Lidar-Derived Aerosol Optical Depth Climatology at ARM Sites Worldwide ARM Keppel-Aleks, G. Determining the Future of CO2 Using an Earth System Model ARM Li, Z. A Mixed Bag of Aerosols over Northeastern China ARM

268

Low Cost Solar Array Project cell and module formation research area. Process research of non-CZ silicon material. Final report, November 26, 1980-September 30, 1983  

SciTech Connect

The primary objective of the work reported was to investigate high-risk, high-payoff research areas associated with the Westinghouse process for producing photovoltaic modules using non-Czochralski sheet material. These tasks were addressed: technical feasibility study of forming front and back junctions using liquid dopant techniques, liquid diffusion mask feasibility study, application studies of antireflective material using a meniscus coater, ion implantation compatibility/feasibility study, and cost analysis. (LEW)

Campbell, R.B.

1983-01-01T23:59:59.000Z

269

Sealing Ducts in Large Commercial Buildings with Aerosolized Sealant  

NLE Websites -- All DOE Office Websites (Extended Search)

Sealing Ducts in Large Commercial Buildings with Aerosolized Sealant Sealing Ducts in Large Commercial Buildings with Aerosolized Sealant Particles Title Sealing Ducts in Large Commercial Buildings with Aerosolized Sealant Particles Publication Type Journal Article LBNL Report Number LBNL-42414 Year of Publication 2001 Authors Modera, Mark P., Olivier Brzozowski, François Rémi Carrié, Darryl J. Dickerhoff, William W. Delp, William J. Fisk, Ronnen M. Levinson, and Duo Wang Journal Energy & Buildings Volume 34 Start Page Chapter Pagination 705-714 Abstract Electricity energy savings potential by eliminating air leakage from ducts in large commercial buildings is on the order of 10 kWh/m2 per year (1 kWh/ft2). We have tested, in two large commercial buildings, a new technology that simultaneously seals duct leaks and measures effective leakage area of ducts. The technology is based upon injecting a fog of aerosolized sealant particles into a pressurized duct system. In brief, this process involves blocking all of the intentional openings in a duct system (e.g., diffusers). Therefore, when the system is pressurized, the only place for the air carrying the aerosol particles to exit the system is through the leaks. The key to the technology is to keep the particles suspended within the airstream until they reach the leaks, and then to have them leave the airstream and deposit on the leak sites. The principal finding from this field study was that the aerosol technology is capable of sealing the leaks in a large commercial building duct system within a reasonable time frame. In the first building, 66% of the leakage area was sealed within 2.5 hours of injection, and in the second building 86% of the leakage area was sealed within 5 hours. We also found that the aerosol could be blown through the VAV boxes in the second building without impacting their calibrations or performance. Some remaining questions are (1) how to achieve sealing rates comparable to those experienced in smaller residential systems; and (2) what tightness level these ducts systems can be brought to by means of aerosol sealing.

270

Conclusions of the Capstone Depleted Uranium Aerosol Characterization and Risk Assessment Study  

SciTech Connect

The rationale for the Capstone Depleted Uranium (DU) Aerosol Characterization and Risk Assessment Program and its results and applications have been examined in the previous 13 articles of this special issue. This paper summarizes the results and discusses its successes and lessons learned. The robust data from the Capstone DU Aerosol Study have provided a sound basis for assessing the inhalation exposure to DU aerosols and the dose and risk to personnel in combat vehicles at the time of perforation and to those entering immediately after perforation. The Human Health Risk Assessment provided a technically sound process for evaluating chemical and radiological doses and risks from DU aerosol exposure using well-accepted biokinetic and dosimetric models innovatively applied. An independent review of the study process and results is summarized, and recommendations for possible avenues of future study by the authors and by other major reviews of DU health hazards are provided.

Parkhurst, MaryAnn; Guilmette, Raymond A.

2009-02-26T23:59:59.000Z

271

Review of models applicable to accident aerosols  

SciTech Connect

Estimations of potential airborne-particle releases are essential in safety assessments of nuclear-fuel facilities. This report is a review of aerosol behavior models that have potential applications for predicting aerosol characteristics in compartments containing accident-generated aerosol sources. Such characterization of the accident-generated aerosols is a necessary step toward estimating their eventual release in any accident scenario. Existing aerosol models can predict the size distribution, concentration, and composition of aerosols as they are acted on by ventilation, diffusion, gravity, coagulation, and other phenomena. Models developed in the fields of fluid mechanics, indoor air pollution, and nuclear-reactor accidents are reviewed with this nuclear fuel facility application in mind. The various capabilities of modeling aerosol behavior are tabulated and discussed, and recommendations are made for applying the models to problems of differing complexity.

Glissmeyer, J.A.

1983-07-01T23:59:59.000Z

272

Atmospheric Radiation Measurement (ARM) Data from Point Reyes, California for the Marine Stratus, Radiation, Aerosol, and Drizzle (MASRAD) Project  

DOE Data Explorer (OSTI)

Point Reyes National Seashore, on the California coast north of San Francisco, was the location of the first deployment of the DOE's Atmospheric Radiation Measurement (ARM) Mobile Facility (AMF). The ARM Program collaborated with the U.S. Office of Naval Research and DOE's Aerosol Science Program in the Marine Stratus, Radiation, Aerosol, and Drizzle (MASRAD) project. Their objectives were to collect data from cloud/aerosol interactions and to improve understanding of cloud organization that is often associated with patches of drizzle. Between March and September 2005, the AMF and at least two research aircraft were used to collect data.

273

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Quantifying the Impact of Dust on Ice Generation in Supercooled Stratiform Quantifying the Impact of Dust on Ice Generation in Supercooled Stratiform Clouds Download a printable PDF Submitter: Wang, Z., University of Wyoming Zhang, D., University of Wyoming Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Zhang D, Z Wang, A Heymsfield, J Fan, D Liu, and M Zhao. 2012. "Quantifying the impact of dust on heterogeneous ice generation in midlevel supercooled stratiform clouds." Journal of Geophysical Research - Atmospheres, 39, L18805, doi:10.1029/2012GL052831. An example of dusty MSSC: (a) CALIOP TAB profiles at 532nm; (b) CALIOP depolarization profiles at 532nm; (c) CloudSat CPR radar reflectivity profiles; (d) Identified dust layers and MSSC; (e) Global distribution of

274

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

CCN and Vertical Velocity Influences CCN and Vertical Velocity Influences Submitter: Hudson, J. G., Desert Research Institute Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Hudson JG and S Noble. 2013. "CCN and vertical velocity influences on droplet concentrations and supersaturations in clean and polluted stratus clouds." Journal of the Atmospheric Sciences, , . ACCEPTED. Figure 1. Effective cloud supersaturation (Seff) against CCN concentration at 1% S (N1%) for horizontal cloud penetrations, 50 for MASE and 34 for POST. Seff is the S for which nearby below cloud CCN spectra, NCCN(S), equals mean droplet concentration (Nc). Figure 2. One second droplet concentration, Nc, and vertical velocity

275

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Broadband Albedo Observations in the Southern Great Plains Broadband Albedo Observations in the Southern Great Plains Submitter: Lamb, P. J., University of Oklahoma Area of Research: Aerosol Properties Working Group(s): Aerosol Journal Reference: Journal of Applied Meteorology and Climatology, Vol. 45, 2006, pp. 210-235. Figure 1 Figure 2 Because surface reflection of solar radiation plays a fundamental role in the surface energy budget, knowledge of its spatial and temporal variability is important for understanding the weather and climate of a specific region. Research instrumentation at the U.S. Southern Great Plains site-one of three locales around the world managed by the U.S. Department of Energy's Atmospheric Radiation Measurement Program-continuously collects these types of data to help scientist investigate differences in

276

Tracing Aerosol Impacts on South Asian Monsoons | U.S. DOE Office of  

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Science Highlights » 2013 Science Highlights » 2013 » Tracing Aerosol Impacts on South Asian Monsoons Biological and Environmental Research (BER) BER Home About Research Facilities Science Highlights Searchable Archive of BER Highlights External link Benefits of BER Funding Opportunities Biological & Environmental Research Advisory Committee (BERAC) News & Resources Contact Information Biological and Environmental Research U.S. Department of Energy SC-23/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3251 F: (301) 903-5051 E: sc.ber@science.doe.gov More Information » September 2013 Tracing Aerosol Impacts on South Asian Monsoons The effect of pollution aerosols on monsoons. Print Text Size: A A A Subscribe FeedbackShare Page Click to enlarge photo. Enlarge Photo

277

Factors affecting the indoor concentrations of carbonaceous aerosols of outdoor origin  

SciTech Connect

A field study was conducted in an unoccupied single story residence in Clovis, California to provide data to address issues important to assess the indoor exposure to particles of outdoor origin. Measurements of black and organic carbonaceous aerosols were performed using a variety of methods, resulting in both near real-time measurements as well as integrated filter based measurements. Comparisons of the different measurement methods show that it is crucial to account for gas phase adsorption artifacts when measuring organic carbon (OC). Measured concentrations affected by the emissions of organic compounds sorbed to indoor surfaces imply a higher degree of infiltration of outdoor organic carbon aerosols into the indoor environment for our unoccupied house. Analysis of the indoor and outdoor data for black carbon (BC) aerosols show that, on average, the indoor concentration of black carbon aerosols behaves in a similar manner to sulfate aerosols. In contrast, organic carbon aerosols are subject to chemical transformations indoors that, for our unoccupied home, resulted in lower indoor OC concentrations than would be expected by physical loss mechanisms alone. These results show that gas to particle partitioning of organic compounds, as well as gas to surface interactions within the residence, are an important process governing the indoor concentration to OC aerosols of outdoor origin.

Lunden, Melissa M.; Kirchstetter, Thomas W.; Thatcher, Tracy L.; Hering, Susanne V.; Brown, Nancy J.

2007-06-25T23:59:59.000Z

278

X-ray Vision for Aerosol Scientists: LCLS Snapshots of Soot (Narrated)  

ScienceCinema (OSTI)

This short conceptual animation depicts how scientists can now simultaneously capture fractal morphology (structure), chemical composition and nanoscale imagery of individual aerosol particles in flight. These particles, known as "PM2.5" because they are smaller than 2.5 microns in diameter, affect climate by interacting with sunlight and impact human health by entering the lungs. The single LCLS laser pulses travel to the Atomic, Molecular and Optical Sciences (AMO) laboratory in the Near Experimental Hall. As we zoom in, we see deep inside a simplified aerosol inlet, where the complex fractal structure of the soot particles, each one completely unique, is shown. Individual soot particles are then delivered into the pulses of the LCLS beam, which destroys them. X-rays are scattered to the detector before the particle is destroyed, giving information about the morphology of the particle. Ion fragments released in the explosion are sent into a mass spectrometer, which measures their mass-to-charge ratio -- giving scientists information about the chemical composition of the particle. Many different particles are analyzed in this manner, allowing scientists to probe variations in the particles due to changes in their environment before being sent through the aerosol inlet. The final visual of aerosols emitted from a factory is representative of the goal that such LCLS aerosol dynamics experiments can provide critical feedback into modeling and understanding combustion, aerosol processes in manufacturing or aerosol effects on climate change.

None

2014-06-03T23:59:59.000Z

279

Design characteristics for facilities which process hazardous particulate  

SciTech Connect

Los Alamos National Laboratory is establishing a research and processing capability for beryllium. The unique properties of beryllium, including light weight, rigidity, thermal conductivity, heat capacity, and nuclear properties make it critical to a number of US defense and aerospace programs. Concomitant with the unique engineering properties are the health hazards associated with processing beryllium in a particulate form and the potential for worker inhalation of aerosolized beryllium. Beryllium has the lowest airborne standard for worker protection compared to all other nonradioactive metals by more than an order of magnitude. This paper describes the design characteristics of the new beryllium facility at Los Alamos as they relate to protection of the workforce. Design characteristics to be reviewed include; facility layout, support systems to minimize aerosol exposure and spread, and detailed review of the ventilation system design for general room air cleanliness and extraction of particulate at the source.

Abeln, S.P.; Creek, K.; Salisbury, S.

1998-12-01T23:59:59.000Z

280

LESSONS LEARNED IN AEROSOL MONITORING WITH THE RASA  

SciTech Connect

The Radionuclide Aerosol Sampler/Analyzer (RASA) is an automated aerosol collection and analysis system designed by Pacific Northwest National Laboratory (PNNL) in the 1990's and is deployed in several locations around the world as part of the International Monitoring System (IMS) required under the Comprehensive Nuclear-Test-Ban Treaty (CTBT). The RASA operates unattended, save for regularly scheduled maintenance, iterating samples through a three-step process on a 24-hour interval. In its 15-year history, much has been learned from the operation and maintenance of the RASA that can benefit engineering updates or future aerosol systems. On 11 March 2011, a 9.0 magnitude earthquake and tsunami rocked the eastern coast of Japan, resulting in power loss and cooling failures at the Daiichi nuclear power plants in Fukushima Prefecture. Aerosol collections were conducted with the RASA in Richland, WA. We present a summary of the lessons learned over the history of the RASA, including lessons taken from the Fukushima incident, regarding the RASA IMS stations operated by the United States.

Forrester, Joel B.; Bowyer, Ted W.; Carty, Fitz; Comes, Laura; Eslinger, Paul W.; Greenwood, Lawrence R.; Haas, Derek A.; Hayes, James C.; Kirkham, Randy R.; Lepel, Elwood A.; Litke, Kevin E.; Miley, Harry S.; Morris, Scott J.; Schrom, Brian T.; Van Davelaar, Peter; Woods, Vincent T.

2011-09-14T23:59:59.000Z

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


281

Vertical Variability of Aerosols and Water Vapor Over the Southern Great Plains  

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Vertical Variability of Aerosols and Water Vapor Vertical Variability of Aerosols and Water Vapor Over the Southern Great Plains R. A. Ferrare National Aeronautics and Space Administration Langley Research Center Hampton, Virginia D. D. Turner Pacific Northwest National Laboratory Richland, Washington M. Clayton and V. Brackett Science Applications International Corporation National Aeronautics and Space Administration Langley Research Center Hampton, Virginia T. P. Tooman and J. E. M. Goldsmith Sandia National Laboratories Livermore, California J. A. Ogren National Oceanic and Atmospheric Administration Climate Monitoring and Diagnostics Laboratory Boulder, Colorado E. Andrews Cooperative Institute for Research in Environmental Sciences University of Colorado Boulder, Colorado

282

E-Print Network 3.0 - atmospheric processes research Sample Search...  

NLE Websites -- All DOE Office Websites (Extended Search)

Roundtable Summary: , Center for Multiscale Modeling of Atmospheric Processes Colorado State University John Dunne, Ph... Exler Director, Office of Communications for...

283

Particles and People: Aerosol Movement Into and Around the Human Body  

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Particles and People: Aerosol Movement Into and Around the Human Body Particles and People: Aerosol Movement Into and Around the Human Body Speaker(s): Miriam Byrne Date: April 14, 2006 - 12:00pm Location: Bldg. 90 Miriam Byrne is a participating guest in the Airflow and Pollutant Transport Group at LBL. She is an academic member of staff in the Physics Department at the National University of Galway, Ireland. Her research interests, primarily funded by European Commission radiation protection programs, focus on the mechanisms of aerosol transport to and from human body surfaces. Over the last ten years, she has been involved in tracer aerosol experiments to determine rates of particle deposition and resuspension from skin, hair and clothing, as well as studying particle transport into skin pores and hair follicles, and contact transfer from

284

Engineering aesthetics and aesthetic ergonomics: Theoretical foundations and a dual-process research methodology  

E-Print Network (OSTI)

Engineering aesthetics and aesthetic ergonomics: Theoretical foundations and a dual, Ann Arbor, MI, 48109-2117, USA Keywords: Engineering aesthetics; Aesthetic ergonomics; Aesthetic human judgments and `educated guesses'. Whilst ergonomics and human factors researchers have made great

Liu, Yili

285

E-Print Network 3.0 - area process research Sample Search Results  

NLE Websites -- All DOE Office Websites (Extended Search)

April 2011 Together with teaching and community service, research is one of the three pillars of the University of Summary: themes and eight sub-themes that reflect areas of...

286

NCCR Digital Fabrication Innovative Building Processes in Architecture A new national research initiative  

E-Print Network (OSTI)

NCCR Digital Fabrication ­Innovative Building Processes in Architecture 14.05.2014 A new national and a resulting enhancement in the quality and sustainability of our built environment. To address the use) to investigate Digital Fabrication ­ Innovative Building Processes in Architecture. Global Challenges The rapidly

Lygeros, John

287

Overview of the 2010 Carbonaceous Aerosols and Radiative Effects Study (CARES)  

SciTech Connect

Substantial uncertainties still exist in the scientific understanding of the possible interactions between urban and natural (biogenic) emissions in the production and transformation of atmospheric aerosol and the resulting impact on climate change. The U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) program's Carbonaceous Aerosol and Radiative Effects Study (CARES) carried out in June 2010 in Central Valley, California, was a comprehensive effort designed to improve this understanding. The primary objective of the field study was to investigate the evolution of secondary organic and black carbon aerosols and their climate-related properties in the Sacramento urban plume as it was routinely transported into the forested Sierra Nevada foothills area. Urban aerosols and trace gases experienced significant physical and chemical transformations as they mixed with the reactive biogenic hydrocarbons emitted from the forest. Two heavily-instrumented ground sites - one within the Sacramento urban area and another about 40 km to the northeast in the foothills area - were set up to characterize the evolution of meteorological variables, trace gases, aerosol precursors, aerosol size, composition, and climate-related properties in freshly polluted and 'aged' urban air. On selected days, the DOE G-1 aircraft was deployed to make similar measurements upwind and across the evolving Sacramento plume in the morning and again in the afternoon. The NASA B-200 aircraft, carrying remote sensing instruments, was also deployed to characterize the vertical and horizontal distribution of aerosols and aerosol optical properties within and around the plume. This overview provides: a) the scientific background and motivation for the study, b) the operational and logistical information pertinent to the execution of the study, c) an overview of key observations and initial results from the aircraft and ground-based sampling platforms, and d) a roadmap of planned data analyses and focused modeling efforts that will facilitate the integration of new knowledge into improved representations of key aerosol processes in climate models.

Zaveri, Rahul A.; Shaw, William J.; Cziczo, D. J.; Schmid, Beat; Ferrare, R.; Alexander, M. L.; Alexandrov, Mikhail; Alvarez, R. J.; Arnott, W. P.; Atkinson, D.; Baidar, Sunil; Banta, Robert M.; Barnard, James C.; Beranek, Josef; Berg, Larry K.; Brechtel, Fred J.; Brewer, W. A.; Cahill, John F.; Cairns, Brian; Cappa, Christopher D.; Chand, Duli; China, Swarup; Comstock, Jennifer M.; Dubey, Manvendra K.; Easter, Richard C.; Erickson, Matthew H.; Fast, Jerome D.; Floerchinger, Cody; Flowers, B. A.; Fortner, Edward; Gaffney, Jeffrey S.; Gilles, Mary K.; Gorkowski, K.; Gustafson, William I.; Gyawali, Madhu S.; Hair, John; Hardesty, Michael; Harworth, J. W.; Herndon, Scott C.; Hiranuma, Naruki; Hostetler, Chris A.; Hubbe, John M.; Jayne, J. T.; Jeong, H.; Jobson, Bertram T.; Kassianov, Evgueni I.; Kleinman, L. I.; Kluzek, Celine D.; Knighton, B.; Kolesar, K. R.; Kuang, Chongai; Kubatova, A.; Langford, A. O.; Laskin, Alexander; Laulainen, Nels S.; Marchbanks, R. D.; Mazzoleni, Claudio; Mei, F.; Moffet, Ryan C.; Nelson, Danny A.; Obland, Michael; Oetjen, Hilke; Onasch, Timothy B.; Ortega, Ivan; Ottaviani, M.; Pekour, Mikhail S.; Prather, Kimberly A.; Radney, J. G.; Rogers, Ray; Sandberg, S. P.; Sedlacek, Art; Senff, Christoph; Senum, Gunar; Setyan, Ari; Shilling, John E.; Shrivastava, ManishKumar B.; Song, Chen; Springston, S. R.; Subramanian, R.; Suski, Kaitlyn; Tomlinson, Jason M.; Volkamer, Rainer M.; Wallace, Hoyt A.; Wang, J.; Weickmann, A. M.; Worsnop, Douglas R.; Yu, Xiao-Ying; Zelenyuk, Alla; Zhang, Qi

2012-08-22T23:59:59.000Z

288

Multi-year Satellite and Surface Observations of AOD in support of Two-Column Aerosol Project (TCAP) Field Campaign  

SciTech Connect

We use combined multi-year measurements from the surface and space for assessing the spatial and temporal distribution of aerosol properties within a large (~400x400 km) region centered on Cape Cod, Massachusetts, along the East Coast of the United States. The ground-based Aerosol Robotic Network (AERONET) measurements at Marthas Vineyard Coastal Observatory (MVCO) site and Moderate Resolution Imaging Spectrometer (MODIS) sensors on board the Terra and Aqua satellites provide horizontal and temporal variations of aerosol optical depth, while the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) offers the altitudes of aerosol-layers. The combined ground-based and satellite measurements indicated several interesting features among which were the large differences in the aerosol properties observed in July and February. We applied the climatology of aerosol properties for designing the Two-Column Aerosol Project (TCAP), which is supported by the U.S. Department of Energys (DOEs) Atmospheric Radiation Measurement (ARM) Program. The TCAP field campaign involves 12-month deployment (started July 1, 2012) of the ground-based ARM Mobile Facility (AMF) and Mobile Aerosol Observing System (MAOS) on Cape Cod and complimentary aerosol observations from two research aircraft: the DOE Gulfstream-1 (G-1) and the National Aeronautics and Space Administration (NASA) B200 King Air. Using results from the coordinated G-1 and B200 flights during the recent (July, 2012) Intensive Observation Period, we demonstrated that the G-1 in situ measurements and B200 active remote sensing can provide complementary information on the temporal and spatial changes of the aerosol properties off the coast of North America.

Kassianov, Evgueni I.; Chand, Duli; Berg, Larry K.; Fast, Jerome D.; Tomlinson, Jason M.; Ferrare, R.; Hostetler, Chris A.; Hair, John

2012-11-01T23:59:59.000Z

289

ARM - Research Highlights  

NLE Websites -- All DOE Office Websites (Extended Search)

CenterResearch Highlights CenterResearch Highlights Media Contact Lynne Roeder lynne-dot-roeder-at-pnnl-dot-gov @armnewsteam Field Notes Blog Topics Field Notes89 AGU 3 AMIE 10 ARM Aerial Facility 2 ARM Mobile Facility 1 6 ARM Mobile Facility 2 47 BAECC 1 BBOP 4 MAGIC 12 MC3E 17 SGP 2 STORMVEX 29 TCAP 3 Search News Search Blog News Center All Categories What's this? Social Media Guidance News Center All Categories Features and Releases Facility News Field Notes Blog feed Events feed Employment Research Highlights Data Announcements Education News Archive What's this? Social Media Guidance Research Highlights Research Highlights Archive » Forecast Calls for Better Models: Examining the Core Components of Arctic Clouds to Clear Their Influence on Climate Jan 07, 2014 Predicting how atmospheric aerosols influence cloud formation and the resulting feedback to climate is a challenge that limits the accuracy of atmospheric models. This is especially true in the Arctic, where mixed-phase (both ice- and liquid-based) clouds are frequently observed, but the processes that determine their composition are poorly understood. To obtain a closer look [...]

290

ARM Climate Research Facility Annual Report 2005  

SciTech Connect

Through the ARM Program, the DOE funded the development of several highly instrumented ground stations for studying cloud formation processes and their influence on radiative transfer, and for measuring other parameters that determine the radiative properties of the atmosphere. This scientific infrastructure, and resultant data archive, is a valuable national and international asset for advancing scientific knowledge of Earth systems. In fiscal year (FY) 2003, the DOE designated ARM sites as a national scientific user facility: the ARM Climate Research (ACRF). The ACRF has enormous potential to contribute to a wide range interdisciplinary science in areas such as meteorology, atmospheric aerosols, hydrology, biogeochemical cycling, and satellite validation, to name only a few.

J. Voyles

2005-12-31T23:59:59.000Z

291

Aerosol Resuspension Model for MELCOR for Fusion and Very High Temperature Reactor Applications  

SciTech Connect

Dust is generated in fusion reactors from plasma erosion of plasma facing components within the reactors vacuum vessel (VV) during reactor operation. This dust collects in cooler regions on interior surfaces of the VV. Because this dust can be radioactive, toxic, and/or chemically reactive, it poses a safety concern, especially if mobilized by the process of resuspension during an accident and then transported as an aerosol though out the reactor confinement building, and possibly released to the environment. A computer code used at the Idaho National Laboratory (INL) to model aerosol transport for safety consequence analysis is the MELCOR code. A primary reason for selecting MELCOR for this application is its aerosol transport capabilities. The INL Fusion Safety Program (FSP) organization has made fusion specific modifications to MELCOR. Recent modifications include the implementation of aerosol resuspension models in MELCOR 1.8.5 for Fusion. This paper presents the resuspension models adopted and the initial benchmarking of these models.

B.J. Merrill

2011-01-01T23:59:59.000Z

292

RESEARCH AND DEVELOPMENT OF AN INTEGRAL SEPARATOR FOR A CENTRIFUGAL GAS PROCESSING FACILITY  

SciTech Connect

A COMPACT GAS PROCESSING DEVICE WAS INVESTIGATED TO INCREASE GAS PRODUCTION FROM REMOTE, PREVIOUSLY UN-ECONOMIC RESOURCES. THE UNIT WAS TESTED ON AIR AND WATER AND WITH NATURAL GAS AND LIQUID. RESULTS ARE REPORTED WITH RECOMMENDATIONS FOR FUTURE WORK.

LANCE HAYS

2007-02-27T23:59:59.000Z

293

Research on the evolvement of morphology of coking coal during the coking process  

Science Journals Connector (OSTI)

Abstract The evolvement of morphology and structure of the coal with different metamorphic degrees during coking process in the vertical furnace was investigated by infrared Image detector. Moreover, the temperature distribution in the radial direction and the crack formation were also studied in heating process. The results show that the amount of crack and the shrinkage level of char decrease with the coal rank rising. In addition, the initial temperature of crack formation for char increases with the coal rank rising.

Xiangyun Zhong; Shiyong Wu; Yang Liu; Zhenning Zhao; Yaru Zhang; Jinfeng Bai; Jun Xu; Bai Xi

2013-01-01T23:59:59.000Z

294

Photoacoustic optical properties at UV, VIS, and near IR wavelengths for laboratory generated and winter time ambient urban aerosols  

SciTech Connect

We present the laboratory and ambient photoacoustic (PA) measurement of aerosol light absorption coefficients at ultraviolet wavelength (i.e., 355 nm) and compare with measurements at 405, 532, 870, and 1047 nm. Simultaneous measurements of aerosol light scattering coefficients were achieved by the integrating reciprocal nephelometer within the PA's acoustic resonator. Absorption and scattering measurements were carried out for various laboratory generated aerosols, including salt, incense, and kerosene soot to evaluate the instrument calibration and gain insight on the spectral dependence of aerosol light absorption and scattering. Ambient measurements were obtained in Reno, Nevada, between 18 December 2009 and 18 January 2010. The measurement period included days with and without strong ground level temperature inversions, corresponding to highly polluted (freshly emitted aerosols) and relatively clean (aged aerosols) conditions. Particulate matter (PM) concentrations were measured and analyzed with other tracers of traffic emissions. The temperature inversion episodes caused very high concentration of PM{sub 2.5} and PM{sub 10} (particulate matter with aerodynamic diameters less than 2.5 {mu}m and 10 {mu}m, respectively) and gaseous pollutants: carbon monoxide (CO), nitric oxide (NO), and nitrogen dioxide (NO{sub 2}). The diurnal change of absorption and scattering coefficients during the polluted (inversion) days increased approximately by a factor of two for all wavelengths compared to the clean days. The spectral variation in aerosol absorption coefficients indicated a significant amount of absorbing aerosol from traffic emissions and residential wood burning. The analysis of single scattering albedo (SSA), Angstrom exponent of absorption (AEA), and Angstrom exponent of scattering (AES) for clean and polluted days provides evidences that the aerosol aging and coating process is suppressed by strong temperature inversion under cloudy conditions. In general, measured UV absorption coefficients were found to be much larger for biomass burning aerosol than for typical ambient aerosols.

Gyawali, Madhu S.; Arnott, W. Patrick; Zaveri, Rahul A.; Song, Chen; Moosmuller, H.; Liu, Li; Mishchenko, M.; Chen, L-W A.; Green, M.; Watson, J. G.; Chow, J. C.

2012-03-08T23:59:59.000Z

295

ARM - PI Product - Direct Aerosol Forcing Uncertainty  

NLE Websites -- All DOE Office Websites (Extended Search)

ProductsDirect Aerosol Forcing Uncertainty ProductsDirect Aerosol Forcing Uncertainty Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send PI Product : Direct Aerosol Forcing Uncertainty Site(s) NSA SGP TWP General Description Understanding sources of uncertainty in aerosol direct radiative forcing (DRF), the difference in a given radiative flux component with and without aerosol, is essential to quantifying changes in Earth's radiation budget. We examine the uncertainty in DRF due to measurement uncertainty in the quantities on which it depends: aerosol optical depth, single scattering albedo, asymmetry parameter, solar geometry, and surface albedo. Direct radiative forcing at the top of the atmosphere and at the surface as well as sensitivities, the changes in DRF in response to unit changes in

296

ARM - Field Campaign - Two-Column Aerosol Project (TCAP)  

NLE Websites -- All DOE Office Websites (Extended Search)

govCampaignsTwo-Column Aerosol Project (TCAP) govCampaignsTwo-Column Aerosol Project (TCAP) Campaign Links TCAP website Related Campaigns Two-Column Aerosol Project (TCAP): Field Evaluation of Real-time Cloud OD Sensor TWST 2013.04.15, Scott, AMF Two-Column Aerosol Project (TCAP): Winter Aerosol Effects on Cloud Formation 2013.02.04, Cziczo, AMF Two-Column Aerosol Project (TCAP): CU GMAX-DOAS Deployment 2012.07.15, Volkamer, AMF Two-Column Aerosol Project (TCAP): Aerosol Light Extinction Measurements 2012.07.15, Dubey, AMF Two-Column Aerosol Project (TCAP): Aerial Campaign 2012.07.07, Berg, AAF Two-Column Aerosol Project (TCAP): Aerodynamic Particle Sizer 2012.07.01, Berg, AMF Two-Column Aerosol Project (TCAP): KASPRR Engineering Tests 2012.07.01, Mead, AMF Two-Column Aerosol Project (TCAP): Airborne HSRL and RSP Measurements

297

Observations of Secondary Organic Aerosol Production and Soot Aging under Atmospheric Conditions Using a Novel Environmental Aerosol Chamber  

E-Print Network (OSTI)

, heterogeneous surface reactions, cloud processing, and gas-to-particle partitioning through the formation of secondary organic aerosol (SOA) by organic gases (Pankow 1994). Moreover, SOA has been linked to adverse health effects as they typically contain... 1985; Ng et al. 2006; Presto et al. 2005; Saathoff et al. 2003). Such classes include cycloalkenes, aromatic hydrocarbons, and terpenes, most of which are cyclic compounds. When these compounds undergo atmospheric oxidation, 3 they produce first-generation...

Glen, Crystal

2012-02-14T23:59:59.000Z

298

Direct and semidirect aerosol effects of southern African biomass burning aerosol  

E-Print Network (OSTI)

Direct and semidirect aerosol effects of southern African biomass burning aerosol Naoko Sakaeda,1 2011; published 21 June 2011. [1] Direct and semidirect radiative effects of biomass burning aerosols static stability. Over the entire region the overall TOA radiative effect from the biomass burning

Wood, Robert

299

Regional variation of organic functional groups in aerosol particles on four U.S. east coast platforms during the International Consortium for  

E-Print Network (OSTI)

and secondary organic aerosol (SOA) formation. SOA can be formed by condensation of species produced by gas aerosol samples were collected during the International Consortium for Atmospheric Research on Transport) spectroscopy at all four sampling platforms. The ratio of molar concentrations of carbonyl C=O to saturated

300

Separating Cloud Forming Nuclei from Interstitial Aerosol  

SciTech Connect

It has become important to characterize the physicochemical properties of aerosol that have initiated the warm and ice clouds. The data is urgently needed to better represent the aerosol-cloud interaction mechanisms in the climate models. The laboratory and in-situ techniques to separate precisely the aerosol particles that act as cloud condensation nuclei (CCN) and ice nuclei (IN), termed as cloud nuclei (CN) henceforth, have become imperative in studying aerosol effects on clouds and the environment. This review summarizes these techniques, design considerations, associated artifacts and challenges, and briefly discusses the need for improved designs to expand the CN measurement database.

Kulkarni, Gourihar R.

2012-09-12T23:59:59.000Z

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


301

Carbonaceous Aerosol Study Using Advanced Particle Instrumentation  

E-Print Network (OSTI)

particles from the combustion of biomass fuels. Environ.range transport of biomass combustion aerosols. Environ.during the open combustion of biomass in the laboratory, J.

Qi, Li

2010-01-01T23:59:59.000Z

302

Salt Processing at the Savannah River Site: Results of Technology Down-Selection and Research and Development to Support New Salt Waste Processing Facility  

SciTech Connect

The Department of Energy's (DOE) Savannah River Site (SRS) high-level waste (HLW) program is responsible for storage, treatment, and immobilization of HLW for disposal. The Salt Processing Project (SPP) is the salt waste (water-soluble) treatment portion of this effort. The overall SPP encompasses the selection, design, construction, and operation of technologies to prepare the salt-waste feed material for immobilization at the site's Saltstone Production Facility (SPF) and vitrification facility (Defense Waste Processing Facility [DWPF]). Major constituents that must be removed from the salt waste and sent as feed to DWPF include cesium (Cs), strontium (Sr), and actinides. In April 2000, the DOE Deputy Secretary for Project Completion (EM-40) established the SRS Salt Processing Project Technical Working Group (TWG) to manage technology development of treatment alternatives for SRS high-level salt wastes. The separation alternatives investigated included three candidate Cs-removal processes selected, as well as actinide and Sr removal that are also required as a part of each process. The candidate Cs-removal processes are: crystalline Silicotitanate Non-Elutable Ion Exchange (CST); caustic Side Solvent Extraction (CSSX); and small Tank Tetraphenylborate Precipitation (STTP). The Tanks Focus Area was asked to assist DOE by managing the SPP research and development (R&D), revising roadmaps, and developing down-selection criteria. The down-selection decision process focused its analysis on three levels: (a) identification of goals that the selected technology should achieve, (b) selection criteria that are a measure of performance of the goal, and (c) criteria scoring and weighting for each technology alternative. After identifying the goals and criteria, the TWG analyzed R&D results and engineering data and scored the technology alternatives versus the criteria. Based their analysis and scoring, the TWG recommended CSSX as the preferred alternative. This recommendation was formalized in July 2001 when DOE published the Savannah River Site Salt Processing Alternatives Final Supplemental Environmental Impact Statement (SEIS) and was finalized in the DOE Record of Decision issued in October 2001.

Lang, K.; Gerdes, K.; Picha, K.; Spader, W.; McCullough, J.; Reynolds, J.; Morin, J. P.; Harmon, H. D.

2002-02-26T23:59:59.000Z

303

Comparative Analysis of Urban Atmospheric Aerosol by Particle...  

NLE Websites -- All DOE Office Websites (Extended Search)

Analysis of Urban Atmospheric Aerosol by Particle-Induced X-ray Emission (PIXE), Proton Elastic Scattering Analysis Comparative Analysis of Urban Atmospheric Aerosol by...

304

The Two-Column Aerosol Project Definitions TCAP Educational  

NLE Websites -- All DOE Office Websites (Extended Search)

What's the big deal about aerosols? The Two-Column Aerosol Project Definitions TCAP Educational Outreach Activity About ARM: The Atmospheric Radiation Measurement (ARM) Climate...

305

Reduction in biomass burning aerosol light absorption upon humidificat...  

NLE Websites -- All DOE Office Websites (Extended Search)

in biomass burning aerosol light absorption upon humidification: Roles of inorganically-induced hygroscopicity, Reduction in biomass burning aerosol light absorption upon...

306

Overview of the COPS Aerosol and Cloud Microphysics (ACM) Subgroup...  

NLE Websites -- All DOE Office Websites (Extended Search)

properties of orographically induced clouds and how do these depend on dynamics, thermodynamics, and aerosol microphysics? * What is the role of aerosols and changing cloud...

307

Molecular Chemistry of Organic Aerosols Through the Application...  

NLE Websites -- All DOE Office Websites (Extended Search)

Chemistry of Organic Aerosols Through the Application of High Resolution Mass Spectrometry. Molecular Chemistry of Organic Aerosols Through the Application of High Resolution Mass...

308

Optical, physical, and chemical properties of springtime aerosol...  

NLE Websites -- All DOE Office Websites (Extended Search)

Optical, physical, and chemical properties of springtime aerosol over Barrow Alaska in 2008. Optical, physical, and chemical properties of springtime aerosol over Barrow Alaska in...

309

REVISED FINAL REPORT INDEPENDENT VERIFICATION SURVEY ACTIVITIES AT THE SEPARATIONS PROCESS RESEARCH UNIT SITES, NISKAYUNA, NEW YORK DCN 0496-SR-06-1  

SciTech Connect

The Separations Process Research Unit (SPRU) complex located on the Knolls Atomic Power Laboratory (KAPL) site in Niskayuna, New York, was constructed in the late 1940s to research the chemical separation of plutonium and uranium (Figure A-1). SPRU operated as a laboratory scale research facility between February 1950 and October 1953. The research activities ceased following the successful development of the reduction oxidation and plutonium/uranium extraction processes. The oxidation and extraction processes were subsequently developed for large scale use by the Hanford and Savannah River sites (aRc 2008a). Decommissioning of the SPRU facilities began in October 1953 and continued through the 1990s.

Evan Harpenau

2011-10-10T23:59:59.000Z

310

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Modeled Compared to Measured O:C and H:C Elemental Ratios of Secondary Modeled Compared to Measured O:C and H:C Elemental Ratios of Secondary Organic Material Download a printable PDF Submitter: Martin, S., Pierce Hall School of Engineering and Applied Sciences Area of Research: Aerosol Properties Working Group(s): Aerosol Life Cycle Journal Reference: Chen Q, Y Liu, N Donahue, J Shilling, and S Martin. 2011. "Particle-phase chemistry of secondary organic material: modeled compared to measured O:C and H:C elemental ratios provide constraints." Environmental Science & Technology, , 10.1021/es104398s. Figure 1. Measurements and predictions. The first row shows particle mass yields at 298 K. The second row shows the modeled and measured particle-average O:C and H:C ratios for increasing particle mass concentrations.

311

Research Highlight  

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aerosols), the Azores (sea-salt aerosols, local pollution from airport traffic, and long-range transport from Europe), the Black Forest in Germany (agricultural and forested...

312

Observations of the first aerosol indirect effect in shallow cumuli  

SciTech Connect

Data from the Cumulus Humilis Aerosol Processing Study (CHAPS) are used to estimate the impact of both aerosol indirect effects and cloud dynamics on the microphysical and optical properties of shallow cumuli observed in the vicinity of Oklahoma City, Oklahoma. Not surprisingly, we find that the amount of light scattered by the clouds is dominated by their liquid water content (LWC), which in turn is driven by cloud dynamics. However, removing the effect of cloud dynamics by examining the scattering normalized by LWC shows a strong sensitivity of scattering to pollutant loading. These results suggest that even moderately sized cities, like Oklahoma City, can have a measureable impact on the optical properties of shallow cumuli.

Berg, Larry K.; Berkowitz, Carl M.; Barnard, James C.; Senum, Gunar; Springston, Stephen R.

2011-02-08T23:59:59.000Z

313

Global distribution and climate forcing of marine organic aerosol: 1. Model improvements and evaluation  

SciTech Connect

Marine organic aerosol emissions have been implemented and evaluated within the National Center of Atmospheric Research (NCAR)'s Community Atmosphere Model (CAM5) with the Pacific Northwest National Laboratory's 7-mode Modal Aerosol Module (MAM-7). Emissions of marine primary organic aerosols (POA), phytoplanktonproduced isoprene- and monoterpenes-derived secondary organic aerosols (SOA) and methane sulfonate (MS{sup -}) are shown to affect surface concentrations of organic aerosols in remote marine regions. Global emissions of submicron marine POA is estimated to be 7.9 and 9.4 Tg yr{sup -1}, for the Gantt et al. (2011) and Vignati et al. (2010) emission parameterizations, respectively. Marine sources of SOA and particulate MS{sup -} (containing both sulfur and carbon atoms) contribute an additional 0.2 and 5.1 Tg yr{sup -1}, respectively. Widespread areas over productive waters of the Northern Atlantic, Northern Pacific, and the Southern Ocean show marine-source submicron organic aerosol surface concentrations of 100 ngm{sup -3}, with values up to 400 ngm{sup -3} over biologically productive areas. Comparison of long-term surface observations of water insoluble organic matter (WIOM) with POA concentrations from the two emission parameterizations shows that despite revealed discrepancies (often more than a factor of 2), both Gantt et al. (2011) and Vignati et al. (2010) formulations are able to capture the magnitude of marine organic aerosol concentrations, with the Gantt et al. (2011) parameterization attaining better seasonality. Model simulations show that the mixing state of the marine POA can impact the surface number concentration of cloud condensation nuclei (CCN). The largest increases (up to 20 %) in CCN (at a supersaturation (S) of 0.2 %) number concentration are obtained over biologically productive ocean waters when marine organic aerosol is assumed to be externally mixed with sea-salt. Assuming marine organics are internally-mixed with sea-salt provides diverse results with increases and decreases in the concentration of CCN over different parts of the ocean. The sign of the CCN change due to the addition of marine organics to seasalt aerosol is determined by the relative significance of the increase in mean modal diameter due to addition of mass, and the decrease in particle hygroscopicity due to compositional changes in marine aerosol. Based on emerging evidence for increased CCN concentration over biologically active surface ocean areas/periods, our study suggests that treatment of sea spray in global climate models (GCMs) as an internal mixture of marine organic aerosols and sea-salt will likely lead to an underestimation in CCN number concentration.

Meskhidze, N.; Xu, J.; Gantt, Brett; Zhang, Yang; Nenes, Athanasios; Ghan, Steven J.; Liu, Xiaohong; Easter, Richard C.; Zaveri, Rahul A.

2011-11-23T23:59:59.000Z

314

Generation of concentration density maxima of small dispersive coal dust particles in horizontal iodine air filter at air-dust aerosol blow  

E-Print Network (OSTI)

The spatial distributions of the small dispersive coal dust particles with the nano and micro sizes in the granular filtering medium with the cylindrical coal granules in the absorber in the horizontal iodine air filter during its long term operation at the nuclear power plant are researched. It is shown that the concentration density maxima of the small dispersive coal dust particles appear in the granular filtering medium with the cylindrical coal absorbent granules in the horizontal iodine air filter at an action by the air dust aerosol blow. The comparison of the measured aerodynamic resistances of the horizontal and vertical iodine air filters is conducted. The main conclusion is that the magnitude of the aerodynamic resistance of the horizontal iodine air filters is much smaller in comparison with the magnitude of the aerodynamic resistance of the vertical iodine air filters at the same loads of the air dust aerosol volumes. It is explained that the direction of the air dust aerosol blow and the direction of the gravitation force in the horizontal iodine air filter are orthogonal, hence the effective accumulation of the small dispersive coal dust particles takes place at the bottom of absorber in the horizontal iodine air filter. It is found that the air dust aerosol stream flow in the horizontal iodine air filter is not limited by the appearing structures, made of the precipitated small dispersive coal dust particles, in distinction from the vertical iodine air filter, in the process of long term operation of the iodine air filters at the nuclear power plant.

I. M. Neklyudov; O. P. Ledenyov; L. I. Fedorova; P. Ya. Poltinin

2013-06-11T23:59:59.000Z

315

Measurements of Aerosol Charge and Size Distribution for Graphite, Gold, Palladium, and Silver Nanoparticles  

SciTech Connect

The role of charge on aerosol evolution and hence the nuclear source term has been an issue of interest, and there is a need for both experimental techniques and modeling for quantifying this role. Our focus here is on further exploration of a tandem differential mobility analyzer (TDMA) technique to simultaneously measure both the size and charge (positive, negative and neutral) dependent aerosol distributions. We have generated graphite, gold, silver, and palladium nanoparticles (aerosol) using a spark generator. We measure the electrical mobility-size distributions for these aerosols using a TDMA, and from these data we deduce the full charge-size distributions. We observe asymmetry in the particle size distributions for negative and positive charges. This asymmetry could have a bearing on the dynamics of charged aerosols, indicating that the assumption of symmetry for size distributions of negatively and positively charged particles in source term simulations may not be always appropriate. Also, the experimental technique should find applications in measurements of aerosol rate processes that are affected by both particle charge and size (e.g. coagulation, deposition, resuspension), and hence in modeling and simulation of the nuclear source term.

Simones, Matthew P.; Gutti, Veera R.; Meyer, Ryan M.; Loyalka, Sudarshan K.

2011-11-01T23:59:59.000Z

316

PARAGON - An Integrated Approach for Characterizing Aerosol Climate Impacts and Environmental Interactions  

SciTech Connect

Aerosols exert myriad influences on the Earth?s environment and climate and on human health. The complexity of aerosol-related processes requires that information gathered to improve our understanding of climate change must originate from multiple sources, and that effective strategies for data integration need to be established. Currently, the aerosol community lacks the necessary tools and infrastructure to reap maximum scientific benefit from a vast array of observed and modeled data. Spatial and temporal sampling differences among a diverse set of sensors, nonuniform data qualities, aerosol mesoscale variabilities, and difficulties in separating cloud effects are some of the challenges that need to be addressed. A sustained, long-term program also requires maintaining consistently well-understood accuracies as measurement approaches evolve and improve. Achieving a comprehensive understanding of how aerosol physical, chemical, and radiative processes impact the Earth system can only be achieved through a multidisciplinary, interagency, and international initiative capable of dealing with these issues. A systematic approach, capitalizing on modern measurement and modeling techniques, geospatial statistics methodologies, and high-performance information technologies can provide the necessary machinery to support this objective. We outline a framework for integrating and interpreting observations and models and establishing an accurate, consistent and cohesive long-term record, following a strategy whereby information and tools of progressively greater sophistication are incorporated as problems of increasing complexity are tackled. This concept is named the Progressive Aerosol Retrieval and Assimilation Global Observing Network (PARAGON). To encompass the breadth of effort required, we present a set of recommendations dealing with data interoperability, integration, synergy, summarization and mining, model evaluation, calibration and validation, augmentation of surface and in situ measurements, advances in passive and active remote sensing, and design of satellite missions. Without an initiative of this nature, the scientific and policy communities will continue to struggle with understanding the quantitative impact of complex aerosol processes on regional and global climate change and air quality.

Diner, David J.; Ackerman, Thomas P.; Anderson, Theodore L.; Bosenberg, Jens; Braverman, Amy J.; Charlson, Robert J.; Collins, William D.; Davies, Roger; Holben, B. N.; Hostetler, Chris A.; Kahn, Ralph A.; Martonchik, John V.; Menzies, Robert T.; Miller, Mark A.; Ogren, J. A.; Penner, Joyce E.; Rasch, P; Schwartz, Stephen E.; Seinfeld, John H.; Stephens, Graeme L.; Torres, Omar; Travis, Larry D.; Wielicki, Bruce A.; Yu, Bin

2004-10-01T23:59:59.000Z

317

HIAPER Pole-to-Pole Observations (HIPPO): fine-grained, global-scale measurements of climatically important atmospheric gases and aerosols  

Science Journals Connector (OSTI)

...emissions to human activity or natural processes, in a variety...new features of trace gas and aerosol emissions...surface fluxes of trace gases and aerosols. 2. HIAPER...sensor drift. The quantum cascade laser spectrometer (QCLS...CO2 sensor using an IR gas analyser (IRGA), which...

2011-01-01T23:59:59.000Z

318

A multilayered analysis of energy security research and the energy supply process  

Science Journals Connector (OSTI)

Abstract After the Fukushima nuclear disaster, a reassessment of the energy system is needed in order to include such aspects as human security and resilience. More open and careful discussions are needed concerning the various risks and uncertainties of future energy options, both in Japan and globally. In this paper, we aim to offer a fundamental basis for discourse on energy security by analyzing the status and trends in academic publications on that issue. Our bibliometrics analysis indicates that research has shifted from promoting strategies for ensuring the self-sufficiency of the primary energy to diversification of the secondary energy supply chain by introducing energy networks consisting of an infrastructure established through international coordination. In the literature, the concept of energy security is ambiguous and allows for multiple interpretations. Our results illustrate the existence of highly multidisciplinary topics within energy security, which can be categorized into four perspectives: geopolitical, economic, policy related, and technological.

Eriko Kiriyama; Yuya Kajikawa

2014-01-01T23:59:59.000Z

319

The Opposed Migration Aerosol Classifier (OMAC)  

NLE Websites -- All DOE Office Websites (Extended Search)

The Opposed Migration Aerosol Classifier (OMAC) The Opposed Migration Aerosol Classifier (OMAC) Speaker(s): Harmony Gates Date: February 22, 2007 - 12:00pm Location: 90-4133 Seminar Host/Point of Contact: Melissa Lunden A new differential mobility classifier will be described. The instrument classifies aerosol particles in a channel flow between porous (or screen) electrodes. The aerosol enters the channel parallel to the porous electrodes, while a larger, particle-free cross-flow enters through one of the porous electrode. A potential difference between electrodes causes the charged aerosol particles to migrate upstream against the cross-flow. Only particles whose upward migration velocity balances the cross flow will be transmitted along the path of the classifier. Simulations of the OMAC show that it should give the same resolution at the traditional

320

Thermophoresis and its thermal parameters for aerosol collection  

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Thermophoresis and its thermal parameters for aerosol collection Thermophoresis and its thermal parameters for aerosol collection Title Thermophoresis and its thermal parameters for aerosol collection Publication Type Journal Article Year of Publication 2007 Authors Huang, Zhuo, Michael G. Apte, and Lara A. Gundel Journal U.S. Department of Energy Journal of Undergraduate Research Volume 7 Pagination 37-42 Abstract The particle collection effi ciency of a prototype environmental tobacco smoke (ETS) sampler based on the use of thermophoresis is determined by optimizing the operational voltage that determines its thermal gradient. This sampler's heating element was made of three sets of thermophoretic (TP) wires 25µm in diameter suspended across a channel cut in a printed circuit board and mounted with collection surfaces on both sides. The separation between the heating element and the room temperature collection surface was determined in a numerical simulation based on the Brock-Talbot model. Other thermal parameters of this TP ETS sampler were predicted by the Brock-Talbot model for TP deposition. From the normalized results the optimal collection ratio was expressed in terms of operational voltage and fi lter mass. Prior to the Brock-Talbot model simulation for this sampler, 1.0V was used arbitrarily. The operational voltage was raised

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321

Environmental research on a modified in situ oil shale task process. Progress report  

SciTech Connect

This report summarizes the progress of the US Department of Energy's Oil Shale Task Force in its research program at the Occidental Oil Shale, Inc. facility at Logan Wash, Colorado. More specifically, the Task Force obtained samples from Retort 3E and Retort 6 and submitted these samples to a variety of analyses. The samples collected included: crude oil (Retort 6); light oil (Retort 6); product water (Retort 6); boiler blowdown (Retort 6); makeup water (Retort 6); mine sump water; groundwater; water from Retorts 1 through 5; retort gas (Retort 6); mine air; mine dust; and spent shale core (Retort 3E). The locations of the sampling points and methods used for collection and storage are discussed in Chapter 2 (Characterization). These samples were then distributed to the various laboratories and universities participating in the Task Force. For convenience in organizing the data, it is useful to group the work into three categories: Characterization, Leaching, and Health Effects. While many samples still have not been analyzed and much of the data remains to be interpreted, there are some preliminary conclusions the Task Force feels will be helpful in defining future needs and establishing priorities. It is important to note that drilling agents other than water were used in the recovery of the core from Retort 3E. These agents have been analyzed (see Table 12 in Chapter 2) for several constituents of interest. As a result some of the analyses of this core sample and leachates must be considered tentative.

Not Available

1980-05-01T23:59:59.000Z

322

Global observations of desert dust and biomass burning aerosols  

E-Print Network (OSTI)

Global observations of desert dust and biomass burning aerosols Martin de Graaf KNMI #12; Outline · Absorbing Aerosol Index - Theory · Absorbing Aerosol Index - Reality · Biomass burning.6 Biomass burning over Angola, 09 Sep. 2004 Absorbing Aerosol Index PMD image #12;biomass burning ocean

Graaf, Martin de

323

Studying trends in biomass burning aerosol using the Absorbing Aerosol Index derived from GOME, SCIAMACHY, and GOME-2  

E-Print Network (OSTI)

Studying trends in biomass burning aerosol using the Absorbing Aerosol Index derived from GOME the resulting time series, we use tropospheric NO2 data as a reference in the regions dominated by biomass sensitive to desert dust aerosols (DDA) and biomass burning aerosols (BBA). See Figure 1. The AAI

Tilstra, Gijsbert

324

E-Print Network 3.0 - aerosol chemical composition Sample Search...  

NLE Websites -- All DOE Office Websites (Extended Search)

Aerosol on Clouds Summary: chemical composition and mixing stateTime-Resolved Aerosol Collector CCSEMEDX (ASP) Single particle... Sizer CCN spectrum Aerosol absorptionDRI...

325

E-Print Network 3.0 - aerosol number distributions Sample Search...  

NLE Websites -- All DOE Office Websites (Extended Search)

inorganic composition PILS-IC Summary: 3563 nephelometers Aerosol number concentration CNC (TSI 3010, 3025) Aerosol size distribution DMA... and APS Non-volatile aerosol size...

326

Indirect and Semi-Direct Aerosol Campaign: The Impact of Arctic...  

NLE Websites -- All DOE Office Websites (Extended Search)

Aerosol Campaign: The Impact of Arctic Aerosols on Clouds . Abstract: A comprehensive dataset of microphysical and radiative properties of aerosols and clouds in the arctic...

327

E-Print Network 3.0 - application research reactor Sample Search...  

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Nuclear Technologies 28 Research Aptitude Problem 1 Scavenging of aerosol particles by ice crystals Summary: strategies that would be required to operate these reactor systems....

328

Nano-DESI Source for OA Samples Analyses. EMSL Research and Capability...  

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Nano-DESI Source for OA Samples Analyses. EMSL Research and Capability Development Proposals Development of Novel Approaches for Analysis of Secondary Organic Aerosols Using High...

329

PHASE II CALDERON PROCESS TO PRODUCE DIRECT REDUCED IRON RESEARCH AND DEVELOPMENT PROJECT  

SciTech Connect

The commercialization path of the Calderon technology for making a feedstock for steelmaking with assistance from DOE initially focused on making coke and work was done which proved that the Calderon technology is capable of making good coke for hard driving blast furnaces. U.S. Steel which participated in such demonstration felt that the Calderon technology would be more meaningful in lowering the costs of making steel by adapting it to the making of iron--thus obviating the need for coke. U.S. Steel and Calderon teamed up to jointly work together to demonstrate that the Calderon technology will produce in a closed system iron units from iron concentrate (ore) and coal competitively by eliminating pelletizing, sintering, coking and blast furnace operation. If such process steps could be eliminated, a huge reduction in polluting emissions and greenhouse gases (including CO{sub 2}) relating to steelmaking would ensue. Such reduction will restructure the steel industry away from the very energy-intensive steelmaking steps currently practiced and drastically reduce costs of making steel. The development of a technology to lower U.S. steelmaking costs and become globally competitive is a priority of major importance. Therefore, the development work which Calderon is conducting presently under this Agreement with the U.S. Department of Energy becomes more crucial than ever. During the 3rd quarter of 2005 which the present report covers, virtually all the effort to advance the Calderon technology to make iron units was concentrated towards forming a team with a steelmaker who needs both iron units in the form of hot metal and a substitute for natural gas (SNG), both being major contributors to higher costs in steelmaking. Calderon felt that a very good candidate would be Steel Dynamics (SDI) by virtue that it operates a rotary hearth facility in Butler, Indiana that uses large amounts of natural gas to reduce briquettes made from ore and coal that they subsequently melt in a submerged arc furnace that is a large consumer of electric power. This facility is operated as a division of SDI under the name of Iron Dynamics (IDI). It is no secret that IDI has had and still has a great number of operational problems, including high cost for natural gas.

Albert Calderon

2005-10-14T23:59:59.000Z

330

CARES: Carbonaceous Aerosol and Radiative Effects Study Science Plan  

SciTech Connect

Carbonaceous aerosol components, which include black carbon (BC), urban primary organic aerosols (POA), biomass burning aerosols, and secondary organic aerosols (SOA) from both urban and biogenic precursors, have been previously shown to play a major role in the direct and indirect radiative forcing of climate. The primary objective of the CARES 2010 intensive field study is to investigate the evolution of carbonaceous aerosols of different types and their effects on optical and cloud formation properties.

Zaveri, RA; Shaw, WJ; Cziczo, DJ

2010-05-27T23:59:59.000Z

331

Carbon-Specific Analysis of Humic-like Substances in Atmospheric Aerosol and Precipitation Samples  

Science Journals Connector (OSTI)

6-9 This means that HULIS have an impact on the hygroscopicity and the cloud condensation nuclei formation potential of the atmospheric aerosol and are, therefore, of climatic relevance. ... Journal of Geophysical Research, [Atmospheres] (2000), 105 (D16), 20697-20706 CODEN: JGRDE3 ISSN:. ... solvents, and recovery from spiked rain water, were included. ...

Andreas Limbeck; Markus Handler; Bernhard Neuberger; Barbara Klatzer; Hans Puxbaum

2005-10-11T23:59:59.000Z

332

Capstone Depleted Uranium Aerosols: Generation and Characterization  

SciTech Connect

In a study designed to provide an improved scientific basis for assessing possible health effects from inhaling depleted uranium (DU) aerosols, a series of DU penetrators was fired at an Abrams tank and a Bradley fighting vehicle. A robust sampling system was designed to collect aerosols in this difficult environment and continuously monitor the sampler flow rates. Aerosols collected were analyzed for uranium concentration and particle size distribution as a function of time. They were also analyzed for uranium oxide phases, particle morphology, and dissolution in vitro. The resulting data provide input useful in human health risk assessments.

Parkhurst, MaryAnn; Szrom, Fran; Guilmette, Ray; Holmes, Tom; Cheng, Yung-Sung; Kenoyer, Judson L.; Collins, John W.; Sanderson, T. Ellory; Fliszar, Richard W.; Gold, Kenneth; Beckman, John C.; Long, Julie

2004-10-19T23:59:59.000Z

333

Sources and Composition of Submicron Organic Mass in Marine Aerosol Particles  

Recent studies have proposed a variety of interpretations of the sources and composition of atmospheric marine aerosol particles (aMAP) based on a range of physical and chemical measurements collected during open-ocean research cruises. To investigate the processes that affect marine organic particles, this study uses the characteristic functional group composition (from Fourier transform infrared (FTIR) spectroscopy) of aMAP from five ocean regions to show that: (i) The organic functional group composition of aMAP that can be identified as atmospheric primary marine (ocean-derived) aerosol (aPMA) is 6512% hydroxyl, 219% alkane, 66% amine, and 78% carboxylic acid functional groups. Contributions from photochemical reactions add carboxylic acid groups (15%-25%), shipping effluent in seawater and ship emissions add additional alkane groups (up to 70%), and coastal emissions mix in alkane and carboxylic acid groups from coastal pollution sources. (ii) The organic composition of aPMA is nearly identical to model generated primary marine aerosol particles (gPMA) from bubbled seawater (55% hydroxyl, 32% alkane, and 13% amine functional groups), indicating that its overall functional group composition is the direct consequence of the organic constituents of the seawater source. (iii) While the seawater organic functional group composition was nearly invariant across all three ocean regions studied, the gPMA alkane group fraction increased with chlorophyll-a concentrations (r = 0.79). gPMA from productive seawater had a larger fraction of alkane functional groups (35%) compared to gPMA from non-productive seawater (16%), likely due to the presence of surfactants in productive seawater that stabilize the bubble film and lead to preferential drainage of the more soluble (lower alkane group fraction) organic components. gPMA has a hydroxyl group absorption peak location characteristic of monosaccharides and disaccharides, where the seawater OM hydroxyl group peak location is closer to that of polysaccharides. This may result from the larger saccharides preferentially remaining in the seawater during gPMA and aPMA production

Frossard, Amanda; Russell, Lynn; Burrows, Susannah M.; Elliott, Scott; Bates, Timothy S.; Quinn, P. K.

2014-11-27T23:59:59.000Z

334

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Optical Properties of the 1997 TWP Smoke Event Submitter: Spinhirne, J., University of Arizona Area of Research: Radiation Processes Working Group(s): Radiative Processes Journal...

335

Evaluating WRF-Chem aerosol indirect effects in Southeast Pacific marine stratocumulus during VOCALS-REx  

SciTech Connect

We evaluate a regional-scale simulation with the WRF-Chem model for the VAMOS (Variability of the American Monsoon Systems) Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-REx), which sampled the Southeast Pacific's persistent stratocumulus deck. Evaluation of VOCALS-REx ship-based and aircraft observations focuses on analyzing how aerosol loading affects marine boundary layer (MBL) dynamics and cloud microphysics. We compare local time series and campaign averaged longitudinal gradients, and highlight differences in model simulations with (W) and without wet (NW) deposition processes. The higher aerosol loadings in the NW case produce considerable changes in MBL dynamics and cloud microphysics, in accordance with the established conceptual model of aerosol indirect effects. These include increase in cloud albedo, increase in MBL and cloud heights, drizzle suppression, increase in liquid water content, and increase in cloud lifetime. Moreover, better statistical representation of aerosol mass and number concentration improves model fidelity in reproducing observed spatial and temporal variability in cloud properties, including top and base height, droplet concentration, water content, rain rate, optical depth (COD) and liquid water path (LWP). Together, these help to quantify confidence in WRF-Chem's modeled aerosol-cloud interactions, while identifying structural and parametric uncertainties including: irreversibility in rain wet removal; overestimation of marine DMS and sea salt emissions and accelerated aqueous sulfate conversion. Our findings suggest that WRF-Chem simulates marine cloud-aerosol interactions at a level sufficient for applications in forecasting weather and air quality and studying aerosol climate forcing, including the reliability required for policy analysis and geo-engineering applications.

Saide, Pablo; Spak, S. N.; Carmichael, Gregory; Mena-Carrasco, M. A.; Yang, Qing; Howell, S. G.; Leon, Dolislager; Snider, Jefferson R.; Bandy, Alan R.; Collett, Jeffrey L.; Benedict, K. B.; de Szoeke, S.; Hawkins, Lisa; Allen, Grant; Crawford, I.; Crosier, J.; Springston, S. R.

2012-03-30T23:59:59.000Z

336

Improving Bulk Microphysics Parameterizations in Simulations of Aerosol Effects  

SciTech Connect

To improve the microphysical parameterizations for simulations of the aerosol indirect effect (AIE) in regional and global climate models, a double-moment bulk microphysical scheme presently implemented in the Weather Research and Forecasting (WRF) model is modified and the results are compared against atmospheric observations and simulations produced by a spectral bin microphysical scheme (SBM). Rather than using prescribed aerosols as in the original bulk scheme (Bulk-OR), a prognostic doublemoment aerosol representation is introduced to predict both the aerosol number concentration and mass mixing ratio (Bulk-2M). The impacts of the parameterizations of diffusional growth and autoconversion and the selection of the embryonic raindrop radius on the performance of the bulk microphysical scheme are also evaluated. Sensitivity modeling experiments are performed for two distinct cloud regimes, maritime warm stratocumulus clouds (SC) over southeast Pacific Ocean from the VOCALS project and continental deep convective clouds (DCC) in the southeast of China from the Department of Energy/ARM Mobile Facility (DOE/AMF) - China field campaign. The results from Bulk-2M exhibit a much better agreement in the cloud number concentration and effective droplet radius in both the SC and DCC cases with those from SBM and field measurements than those from Bulk-OR. In the SC case particularly, Bulk-2M reproduces the observed drizzle precipitation, which is largely inhibited in Bulk-OR. Bulk-2M predicts enhanced precipitation and invigorated convection with increased aerosol loading in the DCC case, consistent with the SBM simulation, while Bulk-OR predicts the opposite behaviors. Sensitivity experiments using four different types of autoconversion schemes reveal that the autoconversion parameterization is crucial in determining the raindrop number, mass concentration, and drizzle formation for warm 2 stratocumulus clouds. An embryonic raindrop size of 40 ?m is determined as a more realistic setting in the autoconversion parameterization. The saturation adjustment employed in calculating condensation/evaporation in the bulk scheme is identified as the main factor responsible for the large discrepancies in predicting cloud water in the SC case, suggesting that an explicit calculation of diffusion growth with predicted supersaturation is necessary for further improvements of the bulk microphysics scheme. Lastly, a larger rain evaporation rate below cloud is found in the bulk scheme in comparison to the SBM simulation, which could contribute to a lower surface precipitation in the bulk scheme.

Wang, Yuan; Fan, Jiwen; Zhang, Renyi; Leung, Lai-Yung R.; Franklin, Charmaine N.

2013-06-05T23:59:59.000Z

337

Development of a Fast Time-Resolved Aerosol Collector (Fast TRAC)  

NLE Websites -- All DOE Office Websites (Extended Search)

Yu Yu & James Cowin PNNL Fast Time-Resolved Aerosol Collector ......Fast TRAC...... Xiao-Ying Yu, Ali Hashim, Martin Iedema, and James Cowin Atmospheric Sciences, Chemical Sciences Pacific Northwest National Laboratory Richland, WA Research is supported by NOAA & DOE. *Patent Pending Xiao-Ying Yu & James Cowin PNNL Cloud Microstructures ≤ 1 m Want to know the aerosols at this resolution Aircraft flies at 150 m/s Need time resolution 1 m/150 m/s = 6 ms (!!!!!) Xiao-Ying Yu & James Cowin PNNL What is TRAC? - Time-Resolved Aerosol Collector * Uses an impactor * ~ 600 TEM samples * Flow rate: 1 l/min * Time resolution: ≥ 1 min* * Applications: Off-line analysis: - particle hygroscopicity, morphology, composition.. (6.5 in) 3 , 7 lb, 12 V, 8 W 0% 20% 40% 60%

338

Effective Radius of Cloud Droplets by Ground-Based Remote Sensing: Relationships to Aerosol?  

NLE Websites -- All DOE Office Websites (Extended Search)

Effective Radius of Cloud Droplets by Ground-Based Effective Radius of Cloud Droplets by Ground-Based Remote Sensing: Relationships to Aerosol? B.-G. Kim, S. E. Schwartz, and M. A. Miller Environmental Sciences Department Brookhaven National Laboratory Upton, New York Q.-L. Min Atmospheric Science Research Center State University of New York Albany, New York Introduction Aerosol Indirect Effect Increases in anthropogenic sources of cloud condensation nuclei can increase cloud albedo by increasing the concentration and reducing the size of cloud droplets, usually referred to as the indirect effect of aerosol on climate (Twomey 1977). However, the magnitudes of the various kinds of indirect forcing are particularly uncertain, because they involve subtle changes in cloud radiative properties and lifetimes

339

Development of Dual-Air-Assistant Atomizing Nozzle to Apply Aerosol-Sealing  

NLE Websites -- All DOE Office Websites (Extended Search)

Development of Dual-Air-Assistant Atomizing Nozzle to Apply Aerosol-Sealing Development of Dual-Air-Assistant Atomizing Nozzle to Apply Aerosol-Sealing Technology in Air Duct Systems Speaker(s): Alan Ropers Date: July 8, 2002 - 12:00pm Location: Bldg. 90 An Aerosol-sealing Technology was developed by LBNL to seal leaks in Air Duct Systems (ADS). The firm AEROSEAL already commercializes this technology for residential ADS. The current goal of our research at the Laboratory is to apply this technology to large commercial ADS. That means to develop a new kind of injector called "Compact Injector". So far, the injector that is used is a nozzle from the Schlick-Dusen firm. Results in terms of sealing rate are satisfactory, but this nozzle quickly clogs up with sealant particles. There are two reasons for the clogging problem: the

340

Southern hemisphere tropospheric aerosol microphysics  

SciTech Connect

Aerosol particle size distribution data have been obtained in the southern hemisphere from approximately 4{degree}S to 44{degree}S and between ground level and 6 km, in the vicinity of eastern Australia. The relative shape of the free-tropospheric size distribution for particles with radii larger than approximately 0.04 {mu}m was found to be remarkably stable with time, altitude, and location for the autumn-winter periods considered. This was despite some large concentration changes which were found to be typical of the southeastern Australian coastal region. The majority of free-troposphere large particles were found to have sulfuric acid or lightly ammoniated sulfate morphology. Large particles in the boundary layer almost exclusively had a sea-salt morphology.

Gras, J.L. (Commonwealth Scientific and Industrial Research Organization, Aspendale (Australia))

1991-03-20T23:59:59.000Z

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


341

Retrieval of Intensive Aerosol Properties from MFRSR observations: Partly Cloudy Cases  

SciTech Connect

An approach for the obtaining column intensive aerosol properties, namely the single scattering albedo (SSA) and asymmetry parameter (ASP), from the Multi-Filter Rotating Shadowband Radiometer (MFRSR) spectral observations under partly cloudy conditions is described. The approach involves the MFRSR-based aerosol retrieval for clear-sky periods and an interpolation of the retrieved column aerosol properties for cloudy periods. The observed weak diurnal variability of SSA and ASP at the surface and the close association of the surface intensive aerosol properties with their column counterparts form the basis of such interpolation. The approach is evaluated by calculating the corresponding clear-sky total, direct and diffuse fluxes at five wavelengths (415, 500, 615, 673 and 870 nm) and compare them with the observed fluxes. The aerosol properties provided by this approach are applied for (i) an examination of the statistical relationship between spectral (visible spectral range) and broadband values of the total normalized cloud radiative forcing and (ii) an estimation of the fractional sky cover. Data collected during 13 days with single-layer cumulus clouds observed at U.S. Department of Energy Atmospheric Radiation Measurement (ARM) Climate Research Facility (ACRF) Southern Great Plains (SGP) site during summer 2007 are applied to illustrate the performance and application of this approach.

Kassianov, Evgueni I.; Barnard, James C.; Berg, Larry K.; Flynn, Connor J.; Long, Charles N.

2010-09-30T23:59:59.000Z

342

Composition and Reactions of Atmospheric Aerosol Particles  

NLE Websites -- All DOE Office Websites (Extended Search)

Composition and Reactions of Composition and Reactions of Atmospheric Aerosol Particles Composition and Reactions of Atmospheric Aerosol Particles Print Wednesday, 29 June 2005 00:00 Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused particle growth while changing organic composition by 13 to 24% per day, an oxidation rate significantly slower than is currently used in atmospheric models. Since oxidation has a strong effect on particle lifetime in the atmosphere, these results will help climate scientists refine the computer models used to predict climate change.

343

ARM - Measurement - Aerosol particle size distribution  

NLE Websites -- All DOE Office Websites (Extended Search)

particle size distribution particle size distribution ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Aerosol particle size distribution The number of aerosol particles present in any given volume of air within a specificied size range Categories Aerosols Instruments The above measurement is considered scientifically relevant for the following instruments. Refer to the datastream (netcdf) file headers of each instrument for a list of all available measurements, including those recorded for diagnostic or quality assurance purposes. ARM Instruments SMPS : Scanning mobility particle sizer TDMA : Tandem Differential Mobility Analyzer UHSAS : Ultra-High Sensitivity Aerosol Spectrometer Field Campaign Instruments

344

Composition and Reactions of Atmospheric Aerosol Particles  

NLE Websites -- All DOE Office Websites (Extended Search)

Composition and Reactions of Atmospheric Aerosol Particles Print Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused particle growth while changing organic composition by 13 to 24% per day, an oxidation rate significantly slower than is currently used in atmospheric models. Since oxidation has a strong effect on particle lifetime in the atmosphere, these results will help climate scientists refine the computer models used to predict climate change.

345

NASA's Aerosol-Cloud-Ecosystems (ACE) Mission  

Science Journals Connector (OSTI)

Plans for NASAs Aerosol-Cloud-Ecosystem (ACE) mission is described. Recommended by Earth Science Decadal Survey in 2007, ACE is nominally planned for a 2021 launch. ACE is...

Starr, David O'C

346

Composition and Reactions of Atmospheric Aerosol Particles  

NLE Websites -- All DOE Office Websites (Extended Search)

Composition and Reactions of Atmospheric Aerosol Particles Print Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused particle growth while changing organic composition by 13 to 24% per day, an oxidation rate significantly slower than is currently used in atmospheric models. Since oxidation has a strong effect on particle lifetime in the atmosphere, these results will help climate scientists refine the computer models used to predict climate change.

347

ARM - Field Campaign - Aerosol Life Cycle IOP at BNL  

NLE Websites -- All DOE Office Websites (Extended Search)

govCampaignsAerosol Life Cycle IOP at BNL govCampaignsAerosol Life Cycle IOP at BNL Campaign Links Images Wiki 2011 ASR STM Presentation: Sedlacek 2011 ASR STM Presentation: Springston 2010 ASR Fall Meeting: Sedlacek News, June 14, 2011: Next-generation Aerosol-sampling Stations to Head for India Related Campaigns Aerosol Life Cycle: Chemical Ionization Mass Spectrometer - CIMS 2011.07.10, Lee, OSC Aerosol Life Cycle: HR-ToF-AMS 2011.06.15, Zhang, OSC Aerosol Life Cycle: ARM Mobile Facility 2 Aerosol Observing System 2011.06.15, Sedlacek, OSC Aerosol Life Cycle: UV-APS and Nano-SMPS 2011.06.10, Hallar, OSC Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : Aerosol Life Cycle IOP at BNL 2011.06.01 - 2011.08.31 Lead Scientist : Arthur Sedlacek For data sets, see below.

348

ARM - Publications: Science Team Meeting Documents: A decade long aerosol  

NLE Websites -- All DOE Office Websites (Extended Search)

A decade long aerosol and cloud statistics and aerosol indirect effect at A decade long aerosol and cloud statistics and aerosol indirect effect at the ARM SGP site Min, Qilong State University of New York at Albany Duan, Minzheng State University of New York at Albany Harrison, Lee State University of New York Joseph, Everette Howard University Twelve-year data of MFRSR and MWR have been used to derive aerosol and cloud optical properties at the ARM SGP. Diurnal, monthly, seasonal and interannual variability of aerosol (optical depth and Angstrom coefficient) and cloud (optical depth and effective radius) have been analyzed. We specially focused on aerosol-cloud interactions. We found a signature of indirect aerosol effect for summer data: increased aerosol index has a statistically-significant anti-correlation with mean effective radius. No

349

DETERMINATION OF RADIAL MOMENTS OF AN AEROSOL  

NLE Websites -- All DOE Office Websites (Extended Search)

DETERMINATION OF RADIAL MOMENTS OF AN AEROSOL DETERMINATION OF RADIAL MOMENTS OF AN AEROSOL SIZE DISTRIBUTION FROM MEASUREMENTS OF LIGHT TRANSMITTANCE AND SCATTERING Ernie R. Lewis and Stephen E. Schwartz Brookhaven National Laboratory, Upton, NY 11933 ses@bnl.gov elewis@bnl.gov MOMENTS FROM MEASUREMENTS As each of the measured quantities is linear in the size distribution dn/dr, it is possible to construct linear combinations of measurements that yield

350

Aerosol fabrication methods for monodisperse nanoparticles  

DOE Patents (OSTI)

Exemplary embodiments provide materials and methods for forming monodisperse particles. In one embodiment, the monodisperse particles can be formed by first spraying a nanoparticle-containing dispersion into aerosol droplets and then heating the aerosol droplets in the presence of a shell precursor to form core-shell particles. By removing either the shell layer or the nanoparticle core of the core-shell particles, monodisperse nanoparticles can be formed.

Jiang, Xingmao; Brinker, C Jeffrey

2014-10-21T23:59:59.000Z

351

Development of plutonium aerosol fractionation system  

E-Print Network (OSTI)

DEVELOPMENT OF A PLUTONIUM AEROSOL FRACTIONATION SYSTEM A Thesis by MALLA R. MEKALA Submitted to the Office of Graduate Studies of Texas A&M University in partial fulfillment of the requirements for the degree of MASTER OF SCIENCE August... 1993 Major Subject: Mechanical Engineering DEVELOPMENT OP A PLUTONIUM AEROSOL FRACTIONATION SYSTEM A Thesis by MALLA R. MEKALA Approved as to style and content by: A. R. McFarland (Chair of Committee) N. K. Anand (Mer toer) (', & C. B...

Mekala, Malla R.

1993-01-01T23:59:59.000Z

352

Rapid Solar-thermal Dissociation of Natural Gas in an Aerosol Flow Reactor  

E-Print Network (OSTI)

/or hydrogen powered fuel cell vehicles could help to mitigate the energy supply and environmental problems black production. For solar-thermal processing, where carbon black is sold, fossil energy usageRapid Solar-thermal Dissociation of Natural Gas in an Aerosol Flow Reactor Jaimee Dahl a , Karen

353

Atmospheric aerosols versus greenhouse gases in the twenty-first century  

Science Journals Connector (OSTI)

...energy-yielding combustion process, and its...sensible to latent heat flux over land...carbon-a tracer of combustion and pollution in...obtained by merging data from several satellite...aerosols by biogenic hydrocarbon oxidation. J...estimated from satellite data. Geophys. Res...

2007-01-01T23:59:59.000Z

354

Techniques and Methods Used to Determine the Aerosol Best Estimate Value-Added Product at SGP Central Facility  

NLE Websites -- All DOE Office Websites (Extended Search)

Determine the Aerosol Best Estimate Value-Added Product at SGP Central Facility C. Sivaraman, D. D. Turner, and C. J. Flynn Pacific Northwest National Laboratory Richland, Washington Objective Profiles of aerosol optical properties are needed for radiative closure exercises such as the broadband heating rate profile (BBHRP) project (Mlawer et al. 2002) and the Shortwave Quality Measurement Experiment (QME). Retrieving cloud microphysical properties using radiation measurements in the shortwave, such as the spectral retrieval technique described in Daniel et al. (2002), also require the optical properties of the aerosols so that they can be accounted for in the retrieval process. The objective of the aerosol best estimate (ABE) value-added procedure (VAP) is to provide profiles of

355

Protecting Vulnerable Research Subjects in Critical Care Trials: Enhancing the Informed Consent Process and Recommendations for Safeguards  

Science Journals Connector (OSTI)

Although critically ill patients represent a vulnerable group of individuals, guidelines in research ethics assert that ethically acceptable research may proceed with such vulnerable subjects if additional safeguards

Henry Silverman

2011-04-01T23:59:59.000Z

356

Physical features of small disperse coal dust fraction transportation and structurization processes in iodine air filters of absorption type in ventilation systems at nuclear power plants  

E-Print Network (OSTI)

The research on the physical features of transportation and structurization processes by the air-dust aerosol in the granular filtering medium with the cylindrical coal adsorbent granules in an air filter of the adsorption type in the heating ventilation and cooling (HVAC) system at the nuclear power plant is completed. The physical origins of the coal dust masses distribution along the absorber with the granular filtering medium with the cylindrical coal granules during the air-dust aerosol intake process in the near the surface layer of absorber are researched. The quantitative technical characteristics of air filtering elements, which have to be considered during the optimization of air filters designs for the application in the ventilation systems at the nuclear power plants, are obtained.

Ledenyov, Oleg P; Poltinin, P Ya; Fedorova, L I

2012-01-01T23:59:59.000Z

357

Formation of carbon allotrope aerosol by colliding plasmas in an inertial fusion reactor  

Science Journals Connector (OSTI)

Along with repeated implosions, the interior of an inertial fusion target chamber is exposed to short pulses of high-energy x-ray, unburned DT-fuel particles, He-ash and pellet debris. As a result, chamber wall materials are subjected to ablation, emitting particles in the plasma state. Ablated particles will either be re-deposited elsewhere or collide with each other, perhaps in the centre-of-symmetry region of the chamber volume. Colliding ablation plasma particles can lead to the formation of clusters to grow into aerosol, possibly floating thereafter, which can deteriorate the subsequent implosion performance via laser scattering, etc. In a laboratory-scale YAG laser setup, the formation of nano-scale aerosol has been demonstrated in vacuum at irradiation power densities of the orders of 10810Wcm?2 at 10Hz, each 6ns long, simulating the high-repetition rate inertial fusion reactor situation. Interestingly, carbon aerosol formation has been observed in the form of fullerene onion, nano- and micro-tubes when laser-ablated plasma plumes of carbon collide with each other. In contrast, colliding plasma plumes of metals tend to generate aerosol in the form of droplets under identical laser irradiation conditions. An atomic and molecular reaction model is proposed to interpret the process of carbon allotrope aerosol formation.

Y. Hirooka; H. Sato; K. Ishihara; T. Yabuuchi; K.A. Tanaka

2014-01-01T23:59:59.000Z

358

E-Print Network 3.0 - aerosol microphysical characteristics Sample...  

NLE Websites -- All DOE Office Websites (Extended Search)

new particle formation, aerosol microphysical evolution, three-dimensional transport, and wet... of aerosol microphysical properties. Some of ... Source: Brookhaven...

359

E-Print Network 3.0 - aerosol chemical vapor Sample Search Results  

NLE Websites -- All DOE Office Websites (Extended Search)

chemical and microphysical properties influence aerosol optical properties and radiative effects... distribution of aerosol extensive and intensive properties will aid ......

360

Small-Scale Spray Releases: Initial Aerosol Test Results  

SciTech Connect

One of the events postulated in the hazard analysis at the Waste Treatment and Immobilization Plant (WTP) and other U.S. Department of Energy (DOE) nuclear facilities is a breach in process piping that produces aerosols with droplet sizes in the respirable range. The current approach for predicting the size and concentration of aerosols produced in a spray leak involves extrapolating from correlations reported in the literature. These correlations are based on results obtained from small engineered spray nozzles using pure liquids with Newtonian fluid behavior. The narrow ranges of physical properties on which the correlations are based do not cover the wide range of slurries and viscous materials that will be processed in the WTP and across processing facilities in the DOE complex. Two key technical areas were identified where testing results were needed to improve the technical basis by reducing the uncertainty due to extrapolating existing literature results. The first technical need was to quantify the role of slurry particles in small breaches where the slurry particles may plug and result in substantially reduced, or even negligible, respirable fraction formed by high-pressure sprays. The second technical need was to determine the aerosol droplet size distribution and volume from prototypic breaches and fluids, specifically including sprays from larger breaches with slurries where data from the literature are scarce. To address these technical areas, small- and large-scale test stands were constructed and operated with simulants to determine aerosol release fractions and generation rates from a range of breach sizes and geometries. The properties of the simulants represented the range of properties expected in the WTP process streams and included water, sodium salt solutions, slurries containing boehmite or gibbsite, and a hazardous chemical simulant. The effect of anti-foam agents was assessed with most of the simulants. Orifices included round holes and rectangular slots. The round holes ranged in size from 0.2 to 4.46 mm. The slots ranged from (width length) 0.3 5 to 2.74 76.2 mm. Most slots were oriented longitudinally along the pipe, but some were oriented circumferentially. In addition, a limited number of multi-hole test pieces were tested in an attempt to assess the impact of a more complex breach. Much of the testing was conducted at pressures of 200 and 380 psi, but some tests were conducted at 100 psi. Testing the largest postulated breaches was deemed impractical because of the large size of some of the WTP equipment. This report presents the experimental results and analyses for the aerosol measurements obtained in the small-scale test stand. It includes a description of the simulants used and their properties, equipment and operations, data analysis methodologies, and test results. The results of tests investigating the role of slurry particles in plugging small breaches are reported in Mahoney et al. (2012). The results of the aerosol measurements in the large-scale test stand are reported in Schonewill et al. (2012) along with an analysis of the combined results from both test scales.

Mahoney, Lenna A.; Gauglitz, Phillip A.; Kimura, Marcia L.; Brown, Garrett N.; Kurath, Dean E.; Buchmiller, William C.; Smith, Dennese M.; Blanchard, Jeremy; Song, Chen; Daniel, Richard C.; Wells, Beric E.; Tran, Diana N.; Burns, Carolyn A.

2012-11-01T23:59:59.000Z

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


361

Small-Scale Spray Releases: Initial Aerosol Test Results  

SciTech Connect

One of the events postulated in the hazard analysis at the Waste Treatment and Immobilization Plant (WTP) and other U.S. Department of Energy (DOE) nuclear facilities is a breach in process piping that produces aerosols with droplet sizes in the respirable range. The current approach for predicting the size and concentration of aerosols produced in a spray leak involves extrapolating from correlations reported in the literature. These correlations are based on results obtained from small engineered spray nozzles using pure liquids with Newtonian fluid behavior. The narrow ranges of physical properties on which the correlations are based do not cover the wide range of slurries and viscous materials that will be processed in the WTP and across processing facilities in the DOE complex. Two key technical areas were identified where testing results were needed to improve the technical basis by reducing the uncertainty due to extrapolating existing literature results. The first technical need was to quantify the role of slurry particles in small breaches where the slurry particles may plug and result in substantially reduced, or even negligible, respirable fraction formed by high-pressure sprays. The second technical need was to determine the aerosol droplet size distribution and volume from prototypic breaches and fluids, specifically including sprays from larger breaches with slurries where data from the literature are scarce. To address these technical areas, small- and large-scale test stands were constructed and operated with simulants to determine aerosol release fractions and net generation rates from a range of breach sizes and geometries. The properties of the simulants represented the range of properties expected in the WTP process streams and included water, sodium salt solutions, slurries containing boehmite or gibbsite, and a hazardous chemical simulant. The effect of antifoam agents was assessed with most of the simulants. Orifices included round holes and rectangular slots. For the combination of both test stands, the round holes ranged in size from 0.2 to 4.46 mm. The slots ranged from (width length) 0.3 5 to 2.74 76.2 mm. Most slots were oriented longitudinally along the pipe, but some were oriented circumferentially. In addition, a limited number of multi-hole test pieces were tested in an attempt to assess the impact of a more complex breach. Much of the testing was conducted at pressures of 200 and 380 psi, but some tests were conducted at 100 psi. Testing the largest postulated breaches was deemed impractical because of the much larger flow rates and equipment that would be required. This report presents the experimental results and analyses for the aerosol measurements obtained in the small-scale test stand. It includes a description of the simulants used and their properties, equipment and operations, data analysis methodologies, and test results. The results of tests investigating the role of slurry particles in plugging small breaches are reported in Mahoney et al. (2012). The results of the aerosol measurements in the large-scale test stand are reported in Schonewill et al. (2012) along with an analysis of the combined results from both test scales.

Mahoney, Lenna A.; Gauglitz, Phillip A.; Kimura, Marcia L.; Brown, Garrett N.; Kurath, Dean E.; Buchmiller, William C.; Smith, Dennese M.; Blanchard, Jeremy; Song, Chen; Daniel, Richard C.; Wells, Beric E.; Tran, Diana N.; Burns, Carolyn A.

2013-05-29T23:59:59.000Z

362

Large-Scale Spray Releases: Initial Aerosol Test Results  

SciTech Connect

One of the events postulated in the hazard analysis at the Waste Treatment and Immobilization Plant (WTP) and other U.S. Department of Energy (DOE) nuclear facilities is a breach in process piping that produces aerosols with droplet sizes in the respirable range. The current approach for predicting the size and concentration of aerosols produced in a spray leak involves extrapolating from correlations reported in the literature. These correlations are based on results obtained from small engineered spray nozzles using pure liquids with Newtonian fluid behavior. The narrow ranges of physical properties on which the correlations are based do not cover the wide range of slurries and viscous materials that will be processed in the WTP and across processing facilities in the DOE complex. Two key technical areas were identified where testing results were needed to improve the technical basis by reducing the uncertainty due to extrapolating existing literature results. The first technical need was to quantify the role of slurry particles in small breaches where the slurry particles may plug and result in substantially reduced, or even negligible, respirable fraction formed by high-pressure sprays. The second technical need was to determine the aerosol droplet size distribution and volume from prototypic breaches and fluids, specifically including sprays from larger breaches with slurries where data from the literature are scarce. To address these technical areas, small- and large-scale test stands were constructed and operated with simulants to determine aerosol release fractions and generation rates from a range of breach sizes and geometries. The properties of the simulants represented the range of properties expected in the WTP process streams and included water, sodium salt solutions, slurries containing boehmite or gibbsite, and a hazardous chemical simulant. The effect of anti-foam agents was assessed with most of the simulants. Orifices included round holes and rectangular slots. The round holes ranged in size from 0.2 to 4.46 mm. The slots ranged from (width length) 0.3 5 to 2.74 76.2 mm. Most slots were oriented longitudinally along the pipe, but some were oriented circumferentially. In addition, a limited number of multi-hole test pieces were tested in an attempt to assess the impact of a more complex breach. Much of the testing was conducted at pressures of 200 and 380 psi, but some tests were conducted at 100 psi. Testing the largest postulated breaches was deemed impractical because of the large size of some of the WTP equipment. The purpose of this report is to present the experimental results and analyses for the aerosol measurements obtained in the large-scale test stand. The report includes a description of the simulants used and their properties, equipment and operations, data analysis methodology, and test results. The results of tests investigating the role of slurry particles in plugging of small breaches are reported in Mahoney et al. 2012a. The results of the aerosol measurements in the small-scale test stand are reported in Mahoney et al. (2012b).

Schonewill, Philip P.; Gauglitz, Phillip A.; Bontha, Jagannadha R.; Daniel, Richard C.; Kurath, Dean E.; Adkins, Harold E.; Billing, Justin M.; Burns, Carolyn A.; Davis, James M.; Enderlin, Carl W.; Fischer, Christopher M.; Jenks, Jeromy WJ; Lukins, Craig D.; MacFarlan, Paul J.; Shutthanandan, Janani I.; Smith, Dennese M.

2012-12-01T23:59:59.000Z

363

Active Spectral Nephelometry in Studies of the Condensational Activity of Submicron Aerosol  

NLE Websites -- All DOE Office Websites (Extended Search)

Active Spectral Nephelometry in Studies of the Active Spectral Nephelometry in Studies of the Condensational Activity of Submicron Aerosol M. V. Panchenko, S. A. Terpugova, and V. S. Kozlov Institute of Atmospheric Optics Russian Academy of Sciences Tomsk, Russia M. A. Sviridenkov A. M. Obukhov Institute of Atmospheric Physics Russian Academy of Sciences Moscow, Russia A. S. Kozlov Institute of Chemical Kinetics and Combustion Russian Academy of Sciences Novosibirsk, Russia Introduction Water vapor condensation and evaporation are among the main processes of the atmospheric aerosol transformation essentially affecting its optical and radiative characteristics. Most of the known methods for investigating the aerosol condensation activity are based on measurements of only the changes in the

364

Chemical Composition and Sources of Coastal Marine Aerosol Particles during the 2008 VOCALS-REx Campaign  

SciTech Connect

The chemical composition of aerosol particles (Dp 1.5 ?m) was measured over the southeast Pacific Ocean during the VAMOS (Variability of the American Monsoon Systems) Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-Rex) between 16 October and 15 November 2008 using the US Department of Energy (DOE) G-1 aircraft. The objective of these flights was to gain an understanding of the sources and evolution of these aerosols, and of how they interact with the marine stratus cloud layer that prevails in this region of the globe. Our measurements showed that the marine boundary layer (MBL) aerosol mass was dominated by non-sea-salt SO2?4, followed by Na+, Cl?, Org (total organics), NH+4 , and NO?3 , in decreasing order of importance; CH3SO?3 (MSA), Ca2+, and K+ rarely exceeded their limits of detection. Aerosols were strongly acidic with a NH+4 to SO2?4 equivalents ratio typically < 0.3. Sea-salt aerosol (SSA) particles, represented by NaCl, exhibited Cl? deficits caused by both HNO3 and H2SO4, but for the most part were externally mixed with particles, mainly SO2?4. SSA contributed only a small fraction of the total accumulation mode particle number concentration. It was inferred that all aerosol species (except SSA) were of predominantly continental origin because of their strong land-to-sea concentration gradient. Comparison of relative changes in median values suggests that (1) an oceanic source of NH3 is present between 72 W and 76 W, (2) additional organic aerosols from biomass burns or biogenic precursors were emitted from coastal regions south of 31 S, with possible cloud processing, and (3) free tropospheric (FT) contributions to MBL gas and aerosol concentrations were negligible. The very low levels of CH3SO?3 observed as well as the correlation between SO2?4 and NO?3 (which is thought primarily anthropogenic) suggest a limited contribution of DMS to SO2?4 aerosol production during VOCALS.

Lee, Y.- N.; Springston, S.; Jayne, John T.; Wang, Jian; Hubbe, John M.; Senum, Gunnar I.; Kleinman, Lawrence I.; Daum, Peter H.

2014-05-23T23:59:59.000Z

365

Study of Mechanisms of Aerosol Indirect Effects on Glaciated Clouds: Progress during the Project Final Technical Report  

SciTech Connect

This 3-year project has studied how aerosol pollution influences glaciated clouds. The tool applied has been an 'aerosol-cloud model'. It is a type of Cloud-System Resolving Model (CSRM) modified to include 2-moment bulk microphysics and 7 aerosol species, as described by Phillips et al. (2009, 2013). The study has been done by, first, improving the model and then performing sensitivity studies with validated simulations of a couple of observed cases from ARM. These are namely the Tropical Warm Pool International Cloud Experiment (TWP-ICE) over the tropical west Pacific and the Cloud and Land Surface Interaction Campaign (CLASIC) over Oklahoma. During the project, sensitivity tests with the model showed that in continental clouds, extra liquid aerosols (soluble aerosol material) from pollution inhibited warm rain processes for precipitation production. This promoted homogeneous freezing of cloud droplets and aerosols. Mass and number concentrations of cloud-ice particles were boosted. The mean sizes of cloud-ice particles were reduced by the pollution. Hence, the lifetime of glaciated clouds, especially ice-only clouds, was augmented due to inhibition of sedimentation and ice-ice aggregation. Latent heat released from extra homogeneous freezing invigorated convective updrafts, and raised their maximum cloud-tops, when aerosol pollution was included. In the particular cases simulated in the project, the aerosol indirect effect of glaciated clouds was twice than of (warm) water clouds. This was because glaciated clouds are higher in the troposphere than water clouds and have the first interaction with incoming solar radiation. Ice-only clouds caused solar cooling by becoming more extensive as a result of aerosol pollution. This 'lifetime indirect effect' of ice-only clouds was due to higher numbers of homogeneously nucleated ice crystals causing a reduction in their mean size, slowing the ice-crystal process of snow production and slowing sedimentation. In addition to the known indirect effects (glaciation, riming and thermodynamic), new indirect effects were discovered and quantified due to responses of sedimentation, aggregation and coalescence in glaciated clouds to changing aerosol conditions. In summary, the change in horizontal extent of the glaciated clouds ('lifetime indirect effects'), especially of ice-only clouds, was seen to be of higher importance in regulating aerosol indirect effects than changes in cloud properties ('cloud albedo indirect effects').

Phillips, Vaughan T. J.

2013-10-18T23:59:59.000Z

366

he Impact of Primary Marine Aerosol on Atmospheric Chemistry, Radiation and Climate: A CCSM Model Development Study  

SciTech Connect

This project examined the potential large-scale influence of marine aerosol cycling on atmospheric chemistry, physics and radiative transfer. Measurements indicate that the size-dependent generation of marine aerosols by wind waves at the ocean surface and the subsequent production and cycling of halogen-radicals are important but poorly constrained processes that influence climate regionally and globally. A reliable capacity to examine the role of marine aerosol in the global-scale atmospheric system requires that the important size-resolved chemical processes be treated explicitly. But the treatment of multiphase chemistry across the breadth of chemical scenarios encountered throughout the atmosphere is sensitive to the initial conditions and the precision of the solution method. This study examined this sensitivity, constrained it using high-resolution laboratory and field measurements, and deployed it in a coupled chemical-microphysical 3-D atmosphere model. First, laboratory measurements of fresh, unreacted marine aerosol were used to formulate a sea-state based marine aerosol source parameterization that captured the initial organic, inorganic, and physical conditions of the aerosol population. Second, a multiphase chemical mechanism, solved using the Max Planck Institute for Chemistry??s MECCA (Module Efficiently Calculating the Chemistry of the Atmosphere) system, was benchmarked across a broad set of observed chemical and physical conditions in the marine atmosphere. Using these results, the mechanism was systematically reduced to maximize computational speed. Finally, the mechanism was coupled to the 3-mode modal aerosol version of the NCAR Community Atmosphere Model (CAM v3.6.33). Decadal-scale simulations with CAM v.3.6.33, were run both with and without reactive-halogen chemistry and with and without explicit treatment of particulate organic carbon in the marine aerosol source function. Simulated results were interpreted (1) to evaluate influences of marine aerosol production on the microphysical properties of aerosol populations and clouds over the ocean and the corresponding direct and indirect effects on radiative transfer; (2) atmospheric burdens of reactive halogen species and their impacts on O3, NOx, OH, DMS, and particulate non-sea-salt SO42-; and (3) the global production and influences of marine-derived particulate organic carbon. The model reproduced major characteristics of the marine aerosol system and demonstrated the potential sensitivity of global, decadal-scale climate metrics to multiphase marine-derived components of Earth??s troposphere. Due to the combined computational burden of the coupled system, the currently available computational resources were the limiting factor preventing the adequate statistical analysis of the overall impact that multiphase chemistry might have on climate-scale radiative transfer and climate.

Keene, William C. [University of Virginia] [University of Virginia; Long, Michael S. [University of Virginia] [University of Virginia

2013-05-20T23:59:59.000Z

367

ARM Aerosol Working Group Meeting  

NLE Websites -- All DOE Office Websites (Extended Search)

and MFRSR Measurements ARM STM 2008 Norfolk, VA Connor Flynn 1 , Annette Koontz 1 , Anne Jefferson 2 , Jim Barnard 1 , Sally McFarlane 1 1 Pacific Northwest National Laboratory 2 CIRES, University of Colorado, Boulder Progress towards ARM DOE 2008 Performance Metric 3 & 4 * Produce and make available new continuous time series of aerosol total column depth, based on results from the AMF deployment in Niger, Africa. * Produce and make available new continuous time series of retrieved dust properties, based on results from the AMF deployment in Niger, Africa. 0 100 200 300 400 0 20 40 60 80 100 ITF movement and surface RH % RH day of year (2006) 0 100 200 300 400 0 50 100 150 200 250 300 350 day of year wind direction (N = 0, E = 90) 2 4 6 8 10 12 14 Wind speed m/s 0 100 200 300 1.4 1.6 1.8 2 MFRSR Vo for filter2, Niamey

368

ARM - Field Campaign - Carbonaceous Aerosol and Radiative Effects Study  

NLE Websites -- All DOE Office Websites (Extended Search)

govCampaignsCarbonaceous Aerosol and Radiative Effects Study (CARES) govCampaignsCarbonaceous Aerosol and Radiative Effects Study (CARES) Campaign Links CARES Website Related Campaigns Carbonaceous Aerosol and Radiation Effects Study (CARES) - Surface Meteorological Sounding 2010.05.26, Zaveri, OSC Carbonaceous Aerosol and Radiation Effects Study (CARES) Photo-Acoustic Aerosol Light Absorption and Scattering 2010.05.26, Arnott, OSC Carbonaceous Aerosol and Radiative Effects Study (CARES): SMPS & CCN counter deployment during CARES/Cal-NEx 2010.05.04, Wang, OSC Carbonaceous Aerosol and Radiative Effects Study (CARES) Ground Based Instruments 2010.04.01, Cziczo, OSC Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : Carbonaceous Aerosol and Radiative Effects Study (CARES)

369

Distinguishing Aerosol Impacts on Climate over the Past Century  

Science Journals Connector (OSTI)

Aerosol direct (DE), indirect (IE), and black carbonsnow albedo (BAE) effects on climate between 1890 and 1995 are compared using equilibrium aerosolclimate simulations in the Goddard Institute for Space Studies General Circulation Model ...

Dorothy Koch; Surabi Menon; Anthony Del Genio; Reto Ruedy; Igor Alienov; Gavin A. Schmidt

2009-05-01T23:59:59.000Z

370

Atmospheric Aerosol Optical Properties in the Persian Gulf  

Science Journals Connector (OSTI)

Aerosol optical depth measurements over Bahrain acquired through the ground-based Aerosol Robotic Network (AERONET) are analyzed. Optical depths obtained from ground-based sun/sky radiometers showed a pronounced temporal trend, with a maximum ...

Alexander Smirnov; Brent N. Holben; Oleg Dubovik; Norm T. O'Neill; Thomas F. Eck; Douglas L. Westphal; Andreas K. Goroch; Christophe Pietras; Ilya Slutsker

2002-02-01T23:59:59.000Z

371

Modeling aerosol growth by aqueous chemistry in nonprecipitating stratiform cloud  

SciTech Connect

A new microphysics module based on a two-dimensional (2D) joint size distribution function representing both interstitial and cloud particles is developed and applied to studying aerosol processing in non-precipitating stratocumulus clouds. The module is implemented in a three-dimensional dynamical framework of a large-eddy simulation (LES) model and in a trajectory ensemble model (TEM). Both models are used to study the modification of sulfate aerosol by the activation - aqueous chemistry - resuspension cycle in shallow marine stratocumulus clouds. The effect of particle mixing and different size-distribution representations on modeled aerosol processing are studied in a comparison of the LES and TEM simulations with the identical microphysics treatment exposes and a comparison of TEM simulations with a 2D fixed and moving bin microphysics. Particle mixing which is represented in LES and neglected in the TEM leads to the mean relative per particle dry mass change in the TEM simulations being about 30% lower than in analogous subsample of LES domain. Particles in the final LES spectrum are mixed in from different parcels, some of which have experienced longer in-cloud residence times than the TEM parcels, all of which originated in the subcloud layer, have. The mean relative per particle dry mass change differs by 14% between TEM simulations with fixed and moving bin microphysics. Finally, the TEM model with the moving bin microphysics is used to evaluate assumptions about liquid water mass partitioning among activated cloud condensation nuclei (CCN) of different dry sizes. These assumptions are used in large-scale models to map the bulk aqueous chemistry sulfate production, which is largely proportional to the liquid water mass, to the changes in aerosol size distribution. It is shown that the commonly used assumptions that the droplet mass is independent of CCN size or that the droplet mass is proportional to the CCN size to the third power do not perform well in the considered case. The explicitly predicted water partitioning indicates that the mean mass of droplets participating in the models aqueous chemistry calculations is proportional to the dry CCN size.

Ovchinnikov, Mikhail; Easter, Richard C.

2010-07-29T23:59:59.000Z

372

Assessing regional scale predictions of aerosols, marine stratocumulus, and their interactions during VOCALS-REx using WRF-Chem  

SciTech Connect

In the recent chemistry version (v3.3) of the Weather Research and Forecasting (WRF-Chem) model, we have coupled the Morrison double-moment microphysics scheme with interactive aerosols so that full two-way aerosol-cloud interactions are included in simulations. We have used this new WRF-Chem functionality in a study focused on assessing predictions of aerosols, marine stratocumulus clouds, and their interactions over the Southeast Pacific using measurements from the VAMOS Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-REx) and satellite retrievals. This study also serves as a detailed analysis of our WRF-Chem simulations contributed to the VOCALS model Assessment (VOCA) project. The WRF-Chem 31-day (October 15-November 16, 2008) simulation with aerosol-cloud interactions (AERO hereafter) is also compared to a simulation (MET hereafter) with fixed cloud droplet number concentrations assumed by the default in Morrison microphysics scheme with no interactive aerosols. The well-predicted aerosol properties such as number, mass composition, and optical depth lead to significant improvements in many features of the predicted stratocumulus clouds: cloud optical properties and microphysical properties such as cloud top effective radius, cloud water path, and cloud optical thickness, and cloud macrostructure such as cloud depth and cloud base height. These improvements in addition to the aerosol direct and semi-direct effects, in turn, feed back to the prediction of boundary-layer characteristics and energy budgets. Particularly, inclusion of interactive aerosols in AERO strengths temperature and humidity gradients within capping inversion layer and lowers the MBL depth by 150 m from that of the MET simulation. Mean top-of-the-atmosphere outgoing shortwave fluxes, surface latent heat, and surface downwelling longwave fluxes are in better agreement with observations in AERO, compared to the MET simulation. Nevertheless, biases in some of the simulated meteorological quantities (e.g., MBL temperature and humidity over the remote ocean) and aerosol quantities (e.g., overestimations of supermicron sea salt mass) might affect simulated stratocumulus and energy fluxes over the SEP, and require further investigations. Although not perfect, the overall performance of the regional model in simulating mesoscale aerosol-cloud interactions is encouraging and suggests that the inclusion of spatially varying aerosol characteristics is important when simulating marine stratocumulus over the southeastern Pacific.

Yang, Qing; Gustafson, William I.; Fast, Jerome D.; Wang, Hailong; Easter, Richard C.; Morrison, H.; Lee, Y.- N.; Chapman, Elaine G.; Spak, S. N.; Mena-Carrasco, M. A.

2011-12-02T23:59:59.000Z

373

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Ice Heating Up Cold Clouds Ice Heating Up Cold Clouds Download a printable PDF Submitter: Ovchinnikov, M., Pacific Northwest National Laboratory Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Ovchinnikov M, A Korolev, and J Fan. 2011. "Effects of ice number concentration on dynamics of a shallow mixed-phase stratiform cloud." Journal of Geophysical Research - Atmospheres, 116, D00T06, doi:10.1029/2011JD015888. The mighty cloud ice crystal appears deceptively delicate but has the power to tip the balance between ice and water in Arctic clouds. This image of an ice crystal was obtained from a Cloud Particle Imager during ISDAC. The imager was mounted on aircraft flying through clouds at a speed of 100 m/s.

374

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Minimalist Approach to Modeling Complex Arctic Clouds Minimalist Approach to Modeling Complex Arctic Clouds Download a printable PDF Submitter: Shaw, R. A., Michigan Technological University - Physics Department Area of Research: Cloud-Aerosol-Precipitation Interactions Working Group(s): Cloud Life Cycle Journal Reference: Yang F, M Ovchinnikov, and RV Shaw. 2013. "Minimalist model of ice microphysics in mixed-phase stratiform clouds." Geophysical Research Letters, 40(14), doi:10.1002/grl.50700. Nordic winter landscape. Mixed-phase stratiform clouds are common features in the Arctic environment. They contain a mix of ice and "supercooled" water that, despite the freezing temperatures, remains in liquid form. Scientists aren't sure why these clouds exist in the Arctic for long periods of time, even while steadily losing ice particles through precipitation.

375

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Understanding Ice Formation in Arctic Mixed-Phase Boundary-Layer Clouds Understanding Ice Formation in Arctic Mixed-Phase Boundary-Layer Clouds During ISDAC Download a printable PDF Submitter: Ackerman, A., NASA - Goddard Institute for Space Studies Fridlind, A. M., NASA - Goddard Institute for Space Studies Area of Research: Cloud Distributions/Characterizations Working Group(s): Cloud-Aerosol-Precipitation Interactions Journal Reference: Avramov A, AS Ackerman, AM Fridlind, B van Diedenhoven, G Botta, K Aydin, J Verlinde, KV Alexei, W Strapp, GM McFarquhar, R Jackson, SD Brooks, A Glen, and M Wolde. 2011. "Towards ice formation closure in Arctic mixed-phase boundary layer clouds during ISDAC." Journal of Geophysical Research - Atmospheres, 116, D00T08, doi:10.1029/2011JD015910. Ice number size distributions as simulated (dendrites in red, aggregates in

376

Spring, 2009 ACS Process Spectroscopy/Society for Applied Spectroscopy Meeting Topic: Discussion of current research into insitu chemical sensors  

E-Print Network (OSTI)

: Discussion of current research into insitu chemical sensors Speaker: Dr. Karl Booksh, University in chemometrics and sensor research. He was previously the codirector of Arizona Applied Nanosensors. Abstract: The theme of the Booksh research group is the development of insitu chemical sensors

Taber, Douglass

377

Emission-Induced Nonlinearities in the Global Aerosol System: Results from the ECHAM5-HAM Aerosol-Climate Model  

Science Journals Connector (OSTI)

In a series of simulations with the global ECHAM5-HAM aerosol-climate model, the response to changes in anthropogenic emissions is analyzed. Traditionally, additivity is assumed in the assessment of the aerosol climate impact, as the underlying ...

Philip Stier; Johann Feichter; Silvia Kloster; Elisabetta Vignati; Julian Wilson

2006-08-01T23:59:59.000Z

378

Toward a Minimal Representation of Aerosols in Climate Models: Comparative Decomposition of Aerosol Direct, Semidirect, and Indirect Radiative Forcing  

Science Journals Connector (OSTI)

The authors have decomposed the anthropogenic aerosol radiative forcing into direct contributions from each aerosol species to the planetary energy balance through absorption and scattering of solar radiation, indirect effects of anthropogenic ...

S. J. Ghan; X. Liu; R. C. Easter; R. Zaveri; P. J. Rasch; J.-H. Yoon; B. Eaton

2012-10-01T23:59:59.000Z

379

Nonequilibrium atmospheric secondary organic aerosol formation and growth  

Science Journals Connector (OSTI)

...Mexico City area are shown...inorganic atmospheric aerosols...2005 ) A large organic aerosol source...photochemical and thermal studies of...Characteristic Group FrequenciesTables and...particle thermal speed...phase-equilibrium in the atmospheric system: Aerosol...Support, Non-U.S...Determination by plasma-based...implications for atmospheric chemistry...2002) A thermal disso-ciation...

Vronique Perraud; Emily A. Bruns; Michael J. Ezell; Stanley N. Johnson; Yong Yu; M. Lizabeth Alexander; Alla Zelenyuk; Dan Imre; Wayne L. Chang; Donald Dabdub; James F. Pankow; Barbara J. Finlayson-Pitts

2012-01-01T23:59:59.000Z

380

Organic and Inorganic Aerosol Below-Cloud Scavenging by  

E-Print Network (OSTI)

concentrations, with an average gravimetric PM1.0 of 8.2 ( 1.6 µg m-3 and an average Fourier transform infrared-rinsing behavior was unaffected by source type. The aerosol OM was hydrophilic throughout the sampling period the description of aerosol lifetimes in global models. Introduction Wet and dry deposition of aerosol particles

Russell, Lynn

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


381

Project of Aerosol Optical Depth Change in South America  

E-Print Network (OSTI)

AerosolDepth Brazil Bolivia French Guiana Suriname Guyana Venezuela Colombia Ecuador Peru Chile Argentina Suriname Guyana Venezuela Colombia Ecuador Peru Chile Argentina Paraguay Uruguay #12;Statistics of Aerosol M ean D ec 01 to 06 Mean Month AerosolDepth Brazil Bolivia French Guiana Suriname Guyana Venezuela

Frank, Thomas D.

382

DO AEROSOLS CHANGE CLOUD COVER AND AFFECT CLIMATE?  

E-Print Network (OSTI)

AS SEEN FROM SPACE Fire plumes from southern Mexico transported north into Gulf of Mexico. #12;CLOUD IPCC AR4 (2007) 3210-1-2 Forcing, W m-2 CO2 CH4 CFCs N2O Long Lived Greenhouse Gases Tropospheric;AEROSOL INFLUENCES ON CLIMATE AND CLIMATE CHANGE #12;DMS #12;AEROSOL IN MEXICO CITY BASIN #12;AEROSOL

Schwartz, Stephen E.

383

Process to make core-shell structured nanoparticles  

DOE Patents (OSTI)

Disclosed is a process for making a composite material that contains core-shell structured nanoparticles. The process includes providing a precursor in the form of a powder a liquid and/or a vapor of a liquid that contains a core material and a shell material, and suspending the precursor in an aerosol gas to produce an aerosol containing the precursor. In addition, the process includes providing a plasma that has a hot zone and passing the aerosol through the hot zone of the plasma. As the aerosol passes through the hot zone of the plasma, at least part of the core material and at least part of the shell material in the aerosol is vaporized. Vapor that contains the core material and the shell material that has been vaporized is removed from the hot zone of the plasma and allowed to condense into core-shell structured nanoparticles.

Luhrs, Claudia; Phillips, Jonathan; Richard, Monique N

2014-01-07T23:59:59.000Z

384

Physicochemical Characterization of Capstone Depleted Uranium Aerosols II: Particle Size Distributions as a Function of Time  

SciTech Connect

The Capstone Depleted Uranium (DU) Aerosol Study, which generated and characterized aerosols containing depleted uranium from perforation of armored vehicles with large-caliber DU penetrators, incorporated a sampling protocol to evaluated particle size distributions. Aerosol particle size distribution is an important parameter that influences aerosol transport and deposition processes as well as the dosimetry of the inhaled particles. These aerosols were collected on cascade impactor substrates using a pre-established time sequence following the firing event to analyze the uranium concentration and particle size of the aerosols as a function of time. The impactor substrates were analyzed using beta spectrometry, and the derived uranium content of each served as input to the evaluation of particle size distributions. Activity median aerodynamic diameters (AMADs) of the particle size distributions were evaluated using unimodal and bimodal models. The particle size data from the impactor measurements was quite variable. Most size distributions measured in the test based on activity had bimodal size distributions with a small particle size mode in the range of between 0.2 and 1.2 um and a large size mode between 2 and 15 um. In general, the evolution of particle size over time showed an overall decrease of average particle size from AMADs of 5 to 10 um shortly after perforation to around 1 um at the end of the 2-hr sampling period. The AMADs generally decreased over time because of settling. Additionally, the median diameter of the larger size mode decreased with time. These results were used to estimate the dosimetry of inhaled DU particles.

Cheng, Yung-Sung; Kenoyer, Judson L.; Guilmette, Raymond A.; Parkhurst, MaryAnn

2009-03-01T23:59:59.000Z

385

7, 469497, 2007 Segregated aerosol  

E-Print Network (OSTI)

are normally fine (e.g. combustion processes, biomass burning and fossil25 fuel combustion). 470 #12;ACPD 7

Paris-Sud XI, Université de

386

Aerodynamic Focusing Of High-Density Aerosols  

SciTech Connect

High-density micron-sized particle aerosols might form the basis for a number of applications in which a material target with a particular shape might be quickly ionized to form a cylindrical or sheet shaped plasma. A simple experimental device was built in order to study the properties of high-density aerosol focusing for 1#22; m silica spheres. Preliminary results recover previous findings on aerodynamic focusing at low densities. At higher densities, it is demonstrated that the focusing properties change in a way which is consistent with a density dependent Stokes number.

Ruiz, D. E.; Fisch, Nathaniel

2014-02-24T23:59:59.000Z

387

An investigation of the sub-grid variability of trace gases and aerosols for global climate modeling  

SciTech Connect

One fundamental property and limitation of grid based models is their inability to identify spatial details smaller than the grid cell size. While decades of work have gone into developing sub-grid treatments for clouds and land surface processes in climate models, the quantitative understanding of sub-grid processes and variability for aerosols and their precursors is much poorer. In this study, WRF-Chem is used to simulate the trace gases and aerosols over central Mexico during the 2006 MILAGRO field campaign, with multiple spatial resolutions and emission/terrain scenarios. Our analysis focuses on quantifying the sub-grid variability (SGV) of trace gases and aerosols within a typical global climate model grid cell, i.e. 75x75 km2. Our results suggest that a simulation with 3-km horizontal grid spacing adequately reproduces the overall transport and mixing of trace gases and aerosols downwind of Mexico City, while 75-km horizontal grid spacing is insufficient to represent local emission and terrain-induced flows along the mountain ridge, subsequently affecting the transport and mixing of plumes from nearby sources. Therefore, the coarse model grid cell average may not correctly represent aerosol properties measured over polluted areas. Probability density functions (PDFs) for trace gases and aerosols show that secondary trace gases and aerosols, such as O3, sulfate, ammonium, and nitrate, are more likely to have a relatively uniform probability distribution (i.e. smaller SGV) over a narrow range of concentration values. Mostly inert and long-lived trace gases and aerosols, such as CO and BC, are more likely to have broad and skewed distributions (i.e. larger SGV) over polluted regions. Over remote areas, all trace gases and aerosols are more uniformly distributed compared to polluted areas. Both CO and O3 SGV vertical profiles are nearly constant within the PBL during daytime, indicating that trace gases are very efficiently transported and mixed vertically by turbulence. But, simulated horizontal variability indicates that trace gases and aerosols are not well mixed horizontally in the PBL. During nighttime the SGV for trace gases is maximum at the surface, and quickly decreases with height. Unlike the trace gases, the SGV of BC and secondary aerosols reaches a maximum at the PBL top during the day. The SGV decreases with distance away from the polluted urban area, has a more rapid decrease for long-lived trace gases and aerosols than for secondary ones, and is greater during daytime than nighttime. The SGV of trace gases and aerosols is generally larger than for meteorological quantities. Emissions can account for up to 50% of the SGV over urban areas such as Mexico City during daytime for less-reactive trace gases and aerosols, such as CO and BC. The impact of emission spatial variability on SGV decays with altitude in the PBL and is insignificant in the free troposphere. The emission variability affects SGV more significantly during daytime (rather than nighttime) and over urban (rather than rural or remote) areas. The terrain, through its impact on meteorological fields such as wind and the PBL structure, affects dispersion and transport of trace gases and aerosols and their SGV.

Qian, Yun; Gustafson, William I.; Fast, Jerome D.

2010-07-29T23:59:59.000Z

388

Atmospheric Science and Climate Research [EVS Program Area]  

NLE Websites -- All DOE Office Websites (Extended Search)

Atmospheric Science and Climate Research Atmospheric Science and Climate Research EVS research, combined with portable, high-performance climate and weather applications, offers a unique look at the complexities of a dynamic planet. In an ever-changing, dynamic climate, we measure, model, and analyze atmospheric processes that are vital to understanding our planet. Our measurement capabilities range from remote sensing and surface meteorology instruments to instrumentation designed to quantify the land-atmosphere exchange of energy, water, and greenhouse gases. Modeling capabilities begin with regional-scale climate, air quality, and aerosol modeling and extend to global chemical transport models, general circulation models of the atmosphere, models of the biosphere, and coupled Earth system models.

389

A Prototyping Environment for Research on Human-Machine Interfaces in Process Control: Use of Microsoft WPF for Microworld and Distributed Control System Development  

SciTech Connect

Operators of critical processes, such as nuclear power production, must contend with highly complex systems, procedures, and regulations. Developing human-machine interfaces (HMIs) that better support operators is a high priority for ensuring the safe and reliable operation of critical processes. Human factors engineering (HFE) provides a rich and mature set of tools for evaluating the performance of HMIs, but the set of tools for developing and designing HMIs is still in its infancy. Here we propose that Microsoft Windows Presentation Foundation (WPF) is well suited for many roles in the research and development of HMIs for process control.

Roger Lew; Ronald L. Boring; Thomas A. Ulrich

2014-08-01T23:59:59.000Z

390

Everything in Its Place: Researchers Identify Brain Cells Used to Categorize Findings Shed Light on the Brain Processes Behind Learning and Memory  

E-Print Network (OSTI)

Everything in Its Place: Researchers Identify Brain Cells Used to Categorize Images Findings Shed Light on the Brain Processes Behind Learning and Memory Boston, MA-August 27,2006-Socks in the sock in youth. But what parts of the brain are used to encode such categories as socks, shirts, or any other

Freedman, David J.

391

High-School Projects at the Laboratory for Laser Energetics (2011) Brandon Avila (Allendale Columbia) researched Natural Language Processing (NLP) for extracting information from LLE  

E-Print Network (OSTI)

Columbia) researched Natural Language Processing (NLP) for extracting information from LLE documentation generator (MTG) for the OMEGA Laser System on a state-of- the-art programmable logic device as a replacement for the previous MTG that uses 20-year-old discrete-circuit technology. The MTG synchronizes all the triggers

Portman, Douglas

392

Post-genomic science: cross-disciplinary and large-scale collaborative research and its organizational and technological challenges for the scientific research process  

Science Journals Connector (OSTI)

...organizations will have to consider the reform of academic funding and reward...Proc. HealthGrid, Studies in Health Technology and Informatics 112...behalf of the Subcommittee of the Health and Environmental Research Advisory...gender and divisions of infant care. Soc. Probl. 43, 219-234...

2006-01-01T23:59:59.000Z

393

Near real time vapor detection and enhancement using aerosol adsorption  

SciTech Connect

A vapor sample detection method where the vapor sample contains vapor and ambient air and surrounding natural background particles. The vapor sample detection method includes the steps of generating a supply of aerosol that have a particular effective median particle size, mixing the aerosol with the vapor sample forming aerosol and adsorbed vapor suspended in an air stream, impacting the suspended aerosol and adsorbed vapor upon a reflecting element, alternatively directing infrared light to the impacted aerosol and adsorbed vapor, detecting and analyzing the alternatively directed infrared light in essentially real time using a spectrometer and a microcomputer and identifying the vapor sample.

Novick, Vincent J.; Johnson, Stanley A.

1997-12-01T23:59:59.000Z

394

Technical Note: Estimating Aerosol Effects on Cloud Radiative Forcing  

SciTech Connect

Estimating anthropogenic aerosol effects on the planetary energy balance through the aerosol influence on clouds using the difference in cloud radiative forcing from simulations with and without anthropogenic emissions produces estimates that are positively biased. A more representative method is suggested using the difference in cloud radiative forcing calculated with aerosol radiative effects neglected. The method also yields an aerosol radiative forcing decomposition that includes a term quantifying the impact of changes in surface albedo. The method requires only two additional diagnostic calculations: the whole-sky and clear-sky top-of-atmosphere radiative flux with aerosol radiative effects neglected.

Ghan, Steven J.

2013-10-09T23:59:59.000Z

395

Near real time vapor detection and enhancement using aerosol adsorption  

DOE Patents (OSTI)

A vapor sample detection method is described where the vapor sample contains vapor and ambient air and surrounding natural background particles. The vapor sample detection method includes the steps of generating a supply of aerosol that have a particular effective median particle size, mixing the aerosol with the vapor sample forming aerosol and adsorbed vapor suspended in an air stream, impacting the suspended aerosol and adsorbed vapor upon a reflecting element, alternatively directing infrared light to the impacted aerosol and adsorbed vapor, detecting and analyzing the alternatively directed infrared light in essentially real time using a spectrometer and a microcomputer and identifying the vapor sample. 13 figs.

Novick, V.J.; Johnson, S.A.

1999-08-03T23:59:59.000Z

396

Near real time vapor detection and enhancement using aerosol adsorption  

DOE Patents (OSTI)

A vapor sample detection method where the vapor sample contains vapor and ambient air and surrounding natural background particles. The vapor sample detection method includes the steps of generating a supply of aerosol that have a particular effective median particle size, mixing the aerosol with the vapor sample forming aerosol and adsorbed vapor suspended in an air stream, impacting the suspended aerosol and adsorbed vapor upon a reflecting element, alternatively directing infrared light to the impacted aerosol and adsorbed vapor, detecting and analyzing the alternatively directed infrared light in essentially real time using a spectrometer and a microcomputer and identifying the vapor sample.

Novick, Vincent J. (Downers Grove, IL); Johnson, Stanley A. (Countryside, IL)

1999-01-01T23:59:59.000Z

397

Aerosol Science and Technology, 46:13131327, 2012 Copyright C American Association for Aerosol Research  

E-Print Network (OSTI)

High-Resolution Time-of-Flight Mass Spectrometer Coupled to a Micro Orifice Volatilization Impactor) high- resolution time-of-flight mass spectrometer (ToFMS) coupled to a micro-orifice volatilization = 5000 above m/Q 250 Th) and mass accuracy (±20 ppm) enabling estimation of compound elemental

Jimenez, Jose-Luis

398

Aerosol Science and Technology, 44:11401145, 2010 Copyright American Association for Aerosol Research  

E-Print Network (OSTI)

application in fuel cells and sensors involving adsorp- tion and dissociation of hydrogen, oxygen, and various. Activated carbon, car- bon nanotubes (CNTs), carbon nanosheets, and silica (SiO2) gel have often been

Huang, Jiaxing

399

Aerosol Science and Technology, 46:309315, 2012 Copyright C American Association for Aerosol Research  

E-Print Network (OSTI)

- cursors are of fundamental and practical interest in the study of gas-to-particle conversion, and play an important role in diverse fields including nanomaterials synthesis, nanoparticle health effects

400

Processing Research snd Development of Green Polymer Nanoclay Composites Containing a Polyhydroxybutyrate, Vinyl Acetates, and Modified Montmorillonite Clay.  

E-Print Network (OSTI)

??The purpose of this research was to determine the feasibility of direct melt-blending (intercalation) montmorillonite nanoclay to polyhydroxybutyrate along with vinyl acetate, at different weight (more)

McKirahan, James N. Jr.

2013-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


401

Proceedings of the 2009 Industrial Engineering Research Conference Technology Assessment for an Inventory Management Process in a  

E-Print Network (OSTI)

, short shelf lives, and a large number of stock keeping units (SKUs). The processes used to track for an Inventory Management Process in a Hospital Unit Angelica Burbano, Behlul Saka, Ronald Rardin, Manuel process in a hospital unit. In particular we will refer to implantable devices within a catheterization

Rossetti, Manuel D.

402

Aerosol analysis for the regional air pollution study. Final report  

SciTech Connect

The design and operation of an aerosol sampling and analysis program implemented during the 1975 to 1977 St. Louis Regional Air Pollution Study is described. A network of ten samplers were operated at selected sites in the St. Louis area and the total mass and elemental composition of the collected particulates were determined. Sampling periods of 2 to 24 hours were employed. The samplers were capable of collecting aerosol particles in two distinct size ranges corresponding to fine (< 2.4 ..mu..m diameter) and coarse (> 2.4 ..mu..m diameter) particles. This unique feature allowed the separation of the particulate samples into two distinct fractions with differing chemical origins and health effects. The analysis methods were also newly developed for use in the St. Louis RAPS study. Total particulate mass was measured by a beta-particle attenuation method in which a precision of +- 5 ..mu..m/cm/sup 2/ could be obtained in a one minute measurement time. Elemental compositions of the samples were determined using an energy dispersive x-ray fluorescence method in which detectable limits of 5 ng/cm/sup 2/ or less were routinely achieved for elements ranging in atomic number from Al to Pb. The advantages of these analytical methods over more conventional techniques arise from the ability to automate the measurements. During the course of the two year study, a total of more than 35,000 individual samples were processed and a total of 28 concentrations measured for each sample.

Jaklevic, J.M.; Gatti, R.C.; Goulding, F.S.; Loo, B.W.; Thompson, A.C.

1980-05-01T23:59:59.000Z

403

Aerosol chemical vapor deposition of metal oxide films  

DOE Patents (OSTI)

A process of preparing a film of a multicomponent metal oxide including: forming an aerosol from a solution comprised of a suitable solvent and at least two precursor compounds capable of volatilizing at temperatures lower than the decomposition temperature of said precursor compounds; passing said aerosol in combination with a suitable oxygen-containing carrier gas into a heated zone, said heated zone having a temperature sufficient to evaporate the solvent and volatilize said precursor compounds; and passing said volatilized precursor compounds against the surface of a substrate, said substrate having a sufficient temperature to decompose said volatilized precursor compounds whereby metal atoms contained within said volatilized precursor compounds are deposited as a metal oxide film upon the substrate is disclosed. In addition, a coated article comprising a multicomponent metal oxide film conforming to the surface of a substrate selected from the group consisting of silicon, magnesium oxide, yttrium-stabilized zirconium oxide, sapphire, or lanthanum gallate, said multicomponent metal oxide film characterized as having a substantially uniform thickness upon said substrate.

Ott, K.C.; Kodas, T.T.

1994-01-11T23:59:59.000Z

404

How do A-train Sensors Intercompare in the Retrieval of Above-Cloud Aerosol Optical Depth? A Case Study-based Assessment  

SciTech Connect

We inter-compare the above-cloud aerosol optical depth (ACAOD) of biomass burning plumes retrieved from different A-train sensors, i.e., MODIS, CALIOP, POLDER, and OMI. These sensors have shown independent capabilities to detect and retrieve aerosol loading above marine boundary layer clouds--a kind of situation often found over the Southeast Atlantic Ocean during dry burning season. A systematic one-to-one comparison reveals that, in general, all passive sensors and CALIOP-based research methods derive comparable ACAOD with differences mostly within 0.2 over homogeneous cloud fields. The 532-nm ACAOD retrieved by CALIOP operational algorithm is largely underestimated; however, its 1064-nm AOD when converted to 500 nm shows closer agreement to the passive sensors. Given the different types of sensor measurements processed with different algorithms, the close agreement between them is encouraging. Due to lack of adequate direct measurements above cloud, the validation of satellite-based ACAOD retrievals remains an open challenge. The inter-satellite comparison, however, can be useful for the relative evaluation and consistency check.

Jethva, H. T.; Torres, O.; Waquet, F.; Chand, Duli; Hu, Yong X.

2014-01-16T23:59:59.000Z

405

Spent fuel sabotage test program, characterization of aerosol dispersal : technical review and analysis supplement.  

SciTech Connect

This project seeks to provide vital data required to assess the consequences of a terrorist attack on a spent fuel transportation cask. One such attack scenario involves the use of conical shaped charges (CSC), which are capable of damaging a spent fuel transportation cask. In the event of such an attack, the amount of radioactivity that may be released as respirable aerosols is not known with great certainty. Research to date has focused on measuring the aerosol release from single short surrogate fuel rodlets subjected to attack by a small CSC device in various aerosol chamber designs. The last series of three experiments tested surrogate fuel rodlets made with depleted uranium oxide ceramic pellets in a specially designed double chamber aerosol containment apparatus. This robust testing apparatus was designed to prevent any radioactive release and allow high level radioactive waste disposal of the entire apparatus following testing of actual spent fuel rodlets as proposed. DOE and Sandia reviews of the project to date identified a number of issues. The purpose of this supplemental report is to address and document the DOE review comments and to resolve the issues identified in the Sandia technical review.

Durbin, Samuel G.; Lindgren, Eric Richard

2009-07-01T23:59:59.000Z

406

Custom data support for the FAst -physics System Testbed and Research (FASTER) Project  

SciTech Connect

The multi-institution FAst -physics System Testbed and Research (FASTER) project, funded by the DOE Earth System Modeling program, aims to evaluate and improve the parameterizations of fast processes (those involving clouds, precipitation and aerosols) in global climate models, using a combination of numerical prediction models, single column models, cloud resolving models, large-eddy simulations, full global climate model output and ARM active and passive remote sensing and in-situ data. This poster presents the Custom Data Support effort for the FASTER project. The effort will provide tailored datasets, statistics, best estimates and quality control data, as needed and defined by FASTER participants, for use in evaluating and improving parameterizations of fast processes in GCMs. The data support will include custom gridding and averaging, for the model of interest, using high time resolution and pixel level data from continuous ARM observations and complementary datasets. In addition to the FASTER team, these datasets will be made available to the ARM Science Team. Initial efforts with respect to data product development, priorities, availability and distribution are summarized here with an emphasis on cloud, atmospheric state and aerosol properties as observed during the Spring 2000 Cloud IOP and the Spring 2003 Aerosol IOP at the ARM Southern Great Plains site.

Toto, T.; Jensen, M.; Vogelmann, A.; Wagener, R.; Liu, Y.; Lin, W.

2010-03-15T23:59:59.000Z

407

Source Apportionment of Carbonaceous Aerosols using  

E-Print Network (OSTI)

are different than the collection of particles from water Filtration has high efficiency for all sizes Size Condensation Nuclei (CCN) Human health Carbonaceous aerosol implicated as important for toxicity and adverse of particulate matter Again, agreement between these two approaches would give a high level of confidence

Einat, Aharonov

408

Photophoretic levitation of engineered aerosols for geoengineering  

Science Journals Connector (OSTI)

...W. Keith Energy and Environmental...space-based solar scattering...The salient advantage of sulfate aerosols...instrument. Disadvantages of sulfates...concentrating solar power systems...higher energy than molecules...solving the energy balance equation...ratio of solar-spectrum to thermal-spectrum...two of the disadvantages of stratospheric...

David W. Keith

2010-01-01T23:59:59.000Z

409

Modeling Semivolatile Organic Aerosol Mass Emissions from  

E-Print Network (OSTI)

in diluted diesel and wood combustion exhaust are interpreted using a two-component absorptive with dilution of both wood smoke and diesel exhaust can be described by two lumped compounds in roughly equal. Introduction Sources of organic aerosol such as diesel engines and wood stoves emit semivolatile organic

Stanier, Charlie

410

ADEPT. aerosol deposition in cylindrical pipes  

SciTech Connect

ADEPT calculates the deposition of aerosols in straight cylindrical pipes during turbulent air flow. Aerosol deposition is calculated in a time-dependent manner based on empirical correlations for turbulent flow in pipes. The calculated deposition during a single time interval is cumulative with that of previous time intervals and results in a decreasing inner diameter of the pipe. The calculated deposition is assumed uniform over the length of the pipe. The entering aerosol distribution is specified by the user in the form of a log-normal distribution of accumulated mass versus particle size and may be time dependent. Entering flow conditions are also specified by the user and may also be time dependent. For simplicity and generality, the geometry implicit in the program is that of a cylindrical pipe with no bends or fittings. The flow is turbulent and monodirectional; only one set of inlet conditions may be applied at a given time. The flow parameters are not calculated along the length of pipe; therefore, the dynamic behavior of the aerosol within the pipe as well as the effects of reentrainment cannot be determined explicitly. A typical problem requires 2 minutes of CPU time.

Fazekas, P.; Tewarson, S.C (Burns and Roe, Oradell, NJ (United States))

1985-01-01T23:59:59.000Z

411

ADEPT. Aerosol Deposition in Cylindrical Pipes  

SciTech Connect

ADEPT calculates the deposition of aerosols in straight cylindrical pipes during turbulent air flow. Aerosol deposition is calculated in a time-dependent manner based on empirical correlations for turbulent flow in pipes. The calculated deposition during a single time interval is cumulative with that of previous time intervals and results in a decreasing inner diameter of the pipe. The calculated deposition is assumed uniform over the length of the pipe. The entering aerosol distribution is specified by the user in the form of a log-normal distribution of accumulated mass versus particle size and may be time dependent. Entering flow conditions are also specified by the user and may also be time dependent. For simplicity and generality, the geometry implicit in the program is that of a cylindrical pipe with no bends or fittings. The flow is turbulent and monodirectional; only one set of inlet conditions may be applied at a given time. The flow parameters are not calculated along the length of pipe; therefore, the dynamic behavior of the aerosol within the pipe as well as the effects of reentrainment cannot be determined explicitly. A typical problem requires 2 minutes of CPU time.

Fazekas, P.; Tewarson, S.C [Burns and Roe, Oradell, NJ (United States)

1985-01-01T23:59:59.000Z

412

8, 14571503, 2008 The aerosol  

E-Print Network (OSTI)

: comparison to near surface in situ and sunphotometer measurements V. Matthias GKSS Research Center, Institute: 18 December 2007 ­ Published: 29 January 2008 Correspondence to: V. Matthias (volker.matthias@gkss

Paris-Sud XI, Université de

413

Single-scattering properties of tri-axial ellipsoidal mineral dust aerosols: A database for application to radiative transfer calculations  

E-Print Network (OSTI)

Single-scattering properties of tri-axial ellipsoidal mineral dust aerosols: A database Applications and Research, Camp Spring, MD 20746, USA a r t i c l e i n f o Article history: Received 14 Optical properties Database a b s t r a c t This paper presents a user-friendly database software package

Liou, K. N.

414

FY 2010 Fourth Quarter Report: Evaluation of the Dependency of Drizzle Formation on Aerosol Properties  

SciTech Connect

Metric for Quarter 4: Report results of implementation of composite parameterization in single-column model (SCM) to explore the dependency of drizzle formation on aerosol properties. To better represent VOCALS conditions during a test flight, the Liu-Duam-McGraw (LDM) drizzle parameterization is implemented in the high-resolution Weather Research and Forecasting (WRF) model, as well as in the single-column Community Atmosphere Model (CAM), to explore this dependency.

Lin, W; McGraw, R; Liu, Y; Wang, J; Vogelmann, A; Daum, PH

2010-10-01T23:59:59.000Z

415

Ultrafine aerosol diffusion charging: an improved interaction potential for metallic particles  

E-Print Network (OSTI)

appreciation to my committee chairman Dr. W. H. Marlow for his guidance and encouragement for the entire duration of the work. He stimulated my interest in aerosol research via, the radon charging problem. He also provided the materials and support needed...' correction 39 11 Collision rate vs. diameter of particle, using Marlow's correction CHAPTER I INTRODUCTION I. l Introduction In recent years, the radiological dose to humans from airborne radioactivity associ- ated with naturally occurring radon has...

Zhu, Xiaowei, d 1963-

2012-06-07T23:59:59.000Z

416

Preparation of ferric-sulfide-based catalysts using an aerosol technique  

SciTech Connect

Iron sulfides are used as catalysts for direct coal liquefaction. They are reasonably active, cheap, and environmentally benign. This permits their use as once-through, non-regenerated catalysts. Our work in this area is based on the products of disproportionation of ferric sulfide, produced in sufficiently small particle sizes. The small particle sizes have been produced by in-situ impregnation or by using an aerosol reactor. This talk will concentrate on the aerosol process. The resulting particles have been characterized and used as catalysts for coal liquefaction. The effects of precursor solution concentration and the pressure and temperature in the aerosol reactor on the performance of the catalysts have been noted. We have recently investigated the effect of adding small amounts of a second metal to the catalyst. Multi-metal catalysts prepared to date with the aerosol technique include Fe-Cu-S and Fe-Zn-S, each with 10% additive, and Fe-Cu-Zn-S, with 10% Cu and 5% Zn.

Stiller, A.H.; Dadyburjor, D.B.; Stinespring, C.D. [West Virginia Univ., Morgantown, WV (United States)] [and others

1995-12-01T23:59:59.000Z

417

Stable carbon fractionation in size-segregated aerosol particles produced by controlled biomass burning  

Science Journals Connector (OSTI)

Abstract Six different biomass fuel types (wood pellets, sunflower stalk pellets, straw pellets, buckwheat shells, mixed biomass waste pellets, and grain screenings) and wastewater sludge pellets were burned under controlled conditions to determine the effect of the biomass type on the emitted particulate matter mass and stable carbon isotope composition of bulk and size-segregated particles. Aerosol particles were sampled using the total suspended particle (TSP) sampler and a micro-orifice uniform deposit impactor (MOUDI). The results demonstrated that particle emissions were dominated by the submicron particles (size <1m) in all biomass types. However, significant differences in emissions of submicron particles and their dominant sizes were found between different biomass fuels. The isotopic fractionation between aerosol particles and original biomass material varied from ?0.940.23 to 1.120.16. The largest negative fractionation ?0.940.23 was obtained for the wood pellet fuel type while the largest positive isotopic fractionation (1.120.16) was observed during the grain screenings combustion. The carbon isotope composition of MOUDI samples compared very well with the isotope composition of TSP samples indicating consistency of the results. The measurements of the stable carbon isotope ratio in size-segregated aerosol particles suggested that combustion processes could strongly affect isotopic fractionation in aerosol particles of different sizes thereby potentially affecting an interpretation of ambient atmospheric observations.

A. Garbaras; A. Masalaite; I. Garbariene; D. Ceburnis; E. Krugly; V. Remeikis; E. Puida; K. Kvietkus; D. Martuzevicius

2015-01-01T23:59:59.000Z

418

Feasibility of Ceramic Membranes in Lignocellulosic Processing: Cooperative Research and Development Final Report, CRADA number CRD-06-00198  

SciTech Connect

NREL will conduct field trials in their biomass process pilot plant using CeraMem developmental membranes and system supplied by CeraMem.

Schell, D. J.

2010-07-01T23:59:59.000Z

419

Direct and semidirect aerosol effects of Southern African biomass burning aerosol  

SciTech Connect

The direct and semi-direct radiative effects of biomass burning aerosols from Southern African fires during July-October are investigated using 20 year runs of the Community Atmospheric Model (CAM) coupled to a slab ocean model. The aerosol optical depth is constrained using observations in clear skies from MODIS and for aerosol layers above clouds from CALIPSO. Over the ocean, where the absorbing biomass burning aerosol layers are primarily located above cloud, negative top of atmosphere (TOA) semi-direct radiative effects associated with increased low cloud cover dominate over a weaker positive all-sky direct radiative effect (DRE). In contrast, over the land where the aerosols are often below or within cloud layers, reductions in cloud liquid water path (LWP) lead to a positive semi-direct radiative effect that dominates over a near-zero DRE. Over the ocean, the cloud response can be understood as a response to increased lower tropospheric stability (LTS) which is caused both by aerosol absorptive warming in overlying layers and surface cooling in response to direct aerosol forcing. The ocean cloud changes are robust to changes in the cloud parameterization (removal of the hard-wired dependence of clouds on LTS), suggesting that they are physically realistic. Over land where cloud cover changes are minimal, decreased LWP is consistent with weaker convection driven by increased static stability. Over the entire region the overall TOA radiative effect from the biomass burning aerosols is almost zero due to opposing effects over the land and ocean. However, the surface forcing is strongly negative requiring a reduction in precipitation. This is primarily realized through reductions in convective precipitation on both the southern and northern flanks of the convective precipitation region spanning the equatorial rainforest and the ITCZ in the southern Sahel. The changes are consistent with the low-level aerosol forced cooling pattern. The results highlight the importance of semi-direct radiative effects and precipitation responses for determining the climatic effects of aerosols in the African region.

Sakaeda, Naoko; Wood, Robert; Rasch, Philip J.

2011-06-21T23:59:59.000Z

420

Lidar Investigation of Tropical Nocturnal Boundary Layer Aerosols and Cloud Macrophysics  

SciTech Connect

Observational evidence of two-way association between nocturnal boundary layer aerosols and cloud macrophysical properties under different meteorological conditions is reported in this paper. The study has been conducted during 2008-09 employing a high space-time resolution polarimetric micro-pulse lidar over a tropical urban station in India. Firstly, the study highlights the crucial role of boundary layer aerosols and background meteorology on the formation and structure of low-level stratiform clouds in the backdrop of different atmospheric stability conditions. Turbulent mixing induced by the wind shear at the station, which is associated with a complex terrain, is found to play a pivotal role in the formation and structural evolution of nocturnal boundary layer clouds. Secondly, it is shown that the trapping of energy in the form of outgoing terrestrial radiation by the overlying low-level clouds can enhance the aerosol mixing height associated with the nocturnal boundary layer. To substantiate this, the long-wave heating associated with cloud capping has been quantitatively estimated in an indirect way by employing an Advanced Research Weather Research and Forecasting (WRF-ARW) model version 2.2 developed by National Center for Atmospheric Research (NCAR), Colorado, USA, and supplementary data sets; and differentiated against other heating mechanisms. The present investigation as well establishes the potential of lidar remote-sensing technique in exploring some of the intriguing aspects of the cloud-environment relationship.

Manoj, M. G.; Devara, PC S.; Taraphdar, Sourav

2013-10-01T23:59:59.000Z

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


421

UNDERSTANDING THE INFLUENCES OF ATMOSPHERIC AEROSOLS ON CLIMATE AND CLIMATE CHANGE  

E-Print Network (OSTI)

.ecd.bnl.gov/steve BOB BRAWDY / AP #12;OVERVIEW Aerosol influences on climate and climate change Earth's energy balance remarks #12;DMS #12;AEROSOL IN MEXICO CITY BASIN #12;AEROSOL IN MEXICO CITY BASIN Light scattering by aerosols decreases absorption of solar radiation. #12;AEROSOLS AS SEEN FROM SPACE Fire plumes from southern

Schwartz, Stephen E.

422

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Determining the Future of CO2 Using an Earth System Model Determining the Future of CO2 Using an Earth System Model Download a printable PDF Submitter: Keppel-Aleks, G., University of Michigan Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Aerosol Life Cycle Journal Reference: Keppel-Aleks G, JT Randerson, K Lindsay, BB Stephens, JK Moore, SC Doney, PE Thornton, NM Mahowald, FM Hoffman, C Sweeney, PP Tans, PO Wennberg, and SC Wofsy. 2013. "Atmospheric carbon dioxide variability in the Community Earth System Model: evaluation and transient dynamics during the twentieth and twenty-first centuries." Journal of Climate, 26(13), doi:10.1175/JCLI-D-12-00589.1. How models, such as the Community Earth System Model, simulate the amount of CO2 in the atmosphere will likely hold the key to monitoring climate

423

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Estimating the Ice Crystal Enhancement Factor in the Tropics Estimating the Ice Crystal Enhancement Factor in the Tropics Download a printable PDF Submitter: Zeng, X., NASA - Goddard Space Flight Center Tao, W., NASA - Goddard Space Flight Center Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Cloud Life Cycle, Cloud-Aerosol-Precipitation Interactions Journal Reference: Zeng X, W Tao, T Matsui, S Xie, S Lang, M Zhang, DO Starr, and X Li. 2011. "Estimating the ice crystal enhancement factor in the tropics." Journal of the Atmospheric Sciences, 68(7), doi:10.1175/2011JAS3550.1. Figure 1. Twenty-day mean vertical profiles of IWC from the ARM-SGP observations and the three simulations using low, moderate, and high ice crystal concentrations, respectively. Figure 2. Eight-day mean vertical profiles of IWC from the TWP-ICE

424

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

General Formulation for Representing Cloud-to-Rain Transition in General Formulation for Representing Cloud-to-Rain Transition in Atmospheric Models Submitter: Liu, Y., Brookhaven National Laboratory Area of Research: General Circulation and Single Column Models/Parameterizations Working Group(s): Aerosol, Cloud Modeling, Cloud Properties Journal Reference: Liu, Y., P. H. Daum, R. McGraw, M. Miller, and S. Niu, 2007: Theoretical formulation for autoconversion rate of cloud droplet concentration. Geophys. Res. Lett., 34, L116821, doi:10.1029/2007GL030389 Figure 1. The typical drop radius r* as a function of the volume-mean radius r3 derived from the new theoretical formulation. Note that a constant r* corresponds to the commonly used assumption that the autoconversion rate for droplet concentration is linearly proportional to

425

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

Cotton-Ball Clouds Contained Download a printable PDF Submitter: Berg, L., Pacific Northwest National Laboratory Area of Research: Cloud Processes Working Group(s): Cloud Life...

426

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

a Modified Scheme for Shallow Convection with CuP Download a printable PDF Submitter: Berg, L., Pacific Northwest National Laboratory Area of Research: Cloud Processes Working...

427

Research Highlight  

NLE Websites -- All DOE Office Websites (Extended Search)

MBL Cloud Properties Derived from the Azores-AMF Observations Submitter: Dong, X., University of North Dakota Area of Research: Cloud Processes Working Group(s):...

428

EVALUATION OF AEROSOL EMISSIONS DOWNSTREAM OF AN AMMONIA-BASED SO2 SCRUBBER  

SciTech Connect

Depending on the size and type of boiler, the 1990 Clean Air Act Amendments required specific reductions in SO{sub 2} emissions from coal-fired electric utilities. To meet these requirements, SO{sub 2} reduction strategies have included installing scrubbing technology, switching to a more expensive low-sulfur coal, or purchasing SO{sub 2} allowances. It is expected that over the next 10 years there will be an increase in the price of low-sulfur coals, but that higher-sulfur coal costs will remain the same. Technologies must be strongly considered that allow the use of high-sulfur fuels while at the same time meeting current and future SO{sub 2} emission limits. One such technology is the ammonia based flue gas desulfurization (FGD) (NH{sub 3}-based FGD) system manufactured by Marsulex Environmental Technologies (MET). The MET scrubber is a patented NH{sub 3}-based FGD process that efficiently converts SO{sub 2} (>95%) into a fertilizer product, ammonium sulfate ([NH{sub 4}]{sub 2}SO{sub 4}). A point of concern for the MET technology, as well as other FGD systems, is the emission of sulfuric acid/SO{sub 3} aerosols that could result in increased opacity at the stack. This is a direct result of firing high-sulfur fuels that naturally generate more SO{sub 3} than do low-sulfur coals. SO{sub 3} is formed during the coal combustion process. SO{sub 3} is converted to gaseous H{sub 2}SO{sub 4} by homogeneous condensation, leading to a submicron acid fume that is very difficult to capture in a dry electrostatic precipitator (ESP). The condensed acid can also combine with the fly ash in the duct and scale the duct wall, potentially resulting in corrosion of both metallic and nonmetallic surfaces. Therefore, SO{sub 3} in flue gas can have a significant impact on the performance of coal-fired utility boilers, air heaters, and ESPs. In addition to corrosion problems, excess SO{sub 3} emissions can result in plume opacity problems. Thus the Energy & Environmental Research Center (EERC) was contracted by MET and the U.S. Department of Energy (DOE) to evaluate the potential of a wet ESP for reducing SO{sub 3} emissions. The work consisted of pilot-scale tests using the EERC's slagging furnace system (SFS) to determine the effectiveness of a wet ESP to control SO{sub 3}/H{sub 2}SO{sub 4} aerosol emissions in conjunction with a dry ESP and MET's NH{sub 3}-based FGD. Because these compounds are in the form of fine particles, it is speculated that a relatively small, highly efficient wet ESP following the MET scrubber would remove these fine aerosol particles. The performance target for the wet ESP was a particulate mass collection efficiency of >90%; this level of performance would likely ensure a stack opacity of <10%.

Dennis L. Laudal

2002-04-01T23:59:59.000Z

429

Proposal Process  

NLE Websites -- All DOE Office Websites (Extended Search)

Testbed Results Current Testbed Research Proposal Process Terms and Conditions Dark Fiber Testbed Performance (perfSONAR) Software & Tools Development Partnerships...

430

Reducing Plug and Process Loads for a Large Scale, Low Energy Office Building: NREL's Research Support Facility; Preprint  

SciTech Connect

This paper documents the design and operational plug and process load energy efficiency measures needed to allow a large scale office building to reach ultra high efficiency building goals. The appendices of this document contain a wealth of documentation pertaining to plug and process load design in the RSF, including a list of equipment was selected for use.

Lobato, C.; Pless, S.; Sheppy, M.; Torcellini, P.

2011-02-01T23:59:59.000Z

431

Photolytic Processes  

Energy.gov (U.S. Department of Energy (DOE))

Photolytic processes use the energy in sunlight to separate water into hydrogen and oxygen. These processes are in the very early stages of research but offer long-term potential for sustainable...

432

Research Unit on Biosphere -Aerosol -Cloud -Climate Interactions  

E-Print Network (OSTI)

of nitrogen fluxes from deep- water entrainment and it seems that higher values can be expected from of the Kattegat Strait. For shorter time- scales like one-year the deep-water entrainement flux is around 30 mg N conducted in the framework of the MEAD (Marine Effects of Atmospheric Deposition) project. METHODS

433

ATMOSPHERIC AEROSOL RESEARCH ANNUAL REPORT 1975-76  

E-Print Network (OSTI)

of a) soot particles from propane-benzene combustion in air;tempera downstream from a propane Photoelectron spectraand carbon (Is) regions of propane soot particles produced

Novakov, T.

2010-01-01T23:59:59.000Z

434

8, 80918118, 2008 Aerosol source  

E-Print Network (OSTI)

and markers are discussed. 1 Introduction Biomass combustion is a major global source of particulate matter for Materials Testing and Research, Laboratory for Internal Combustion Engines, 8600 Duebendorf, Switzerland Discussion Abstract Residential wood combustion has only recently been recognized as a major contributor

Paris-Sud XI, Université de

435

Indirect radiative forcing by ion-mediated nucleation of aerosol  

SciTech Connect

A clear understanding of particle formation mechanisms is critical for assessing aerosol indirect radiative forcing and associated climate feedback processes. Recent studies reveal the importance of ion-mediated nucleation (IMN) in generating new particles and cloud condensation nuclei (CCN) in the atmosphere. Here we implement for the first time a physically based treatment of IMN into the Community Atmosphere Model version 5. Our simulations show that, compared to globally averaged results based on binary homogeneous nucleation (BHN), the presence of ionization (i.e., IMN) halves H2SO4 column burden, but increases the column integrated nucleation rate by around one order of magnitude, total particle number burden by a factor of ~ 3, CCN burden by ~ 10% (at 0.2% supersaturation) to 65% (at 1.0% supersaturation), and cloud droplet number burden by ~ 18%. Compared to BHN, IMN increases cloud liquid water path by 7.5%, decreases precipitation by 1.1%, and increases total cloud cover by 1.9%. This leads to an increase of total shortwave cloud radiative forcing by 3.67 W/m2 (more negative) and longwave cloud forcing by 1.78 W/m2 (more positive), resulting in a -1.9 W/m2 net change in cloud radiative forcing associated with IMN. The significant impacts of ionization on global aerosol formation, CCN abundance, and cloud radiative forcing may provide an important physical mechanism linking the global energy balance to various processes affecting atmospheric ionization, which should be properly represented in climate models.

Yu, Fangqun; Luo, Gan; Liu, Xiaohong; Easter, Richard C.; Ma, Xiaoyan; Ghan, Steven J.

2012-12-03T23:59:59.000Z

436

ARM - Field Campaign - Biogenic Aerosols - Effects on Clouds and Climate:  

NLE Websites -- All DOE Office Websites (Extended Search)

govCampaignsBiogenic Aerosols - Effects on Clouds and Climate: govCampaignsBiogenic Aerosols - Effects on Clouds and Climate: FIGAERO-ToF-CIMS Instrument in Hyytiala with AMF-2 Related Campaigns Biogenic Aerosols- Effects on Clouds and Climate 2014.02.01, Petäjä, AMF Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : Biogenic Aerosols - Effects on Clouds and Climate: FIGAERO-ToF-CIMS Instrument in Hyytiala with AMF-2 2014.04.01 - 2014.06.01 Lead Scientist : Joel Thornton Description The ultimate goal of this work is to connect field and laboratory observations of organic aerosol chemical and physical properties during the nascent growth stage to the diurnal and vertical distributions of aerosol abundance measured over the boreal forest by the ARM Mobile Facility 2

437

Aerosol Modeling at LLNL - Our capability, results, and perspective  

NLE Websites -- All DOE Office Websites (Extended Search)

Aerosol Indirect Effects to Cloud Aerosol Indirect Effects to Cloud Parameterizations in Short-Range Weather Forecasts with CAM3 Over the Southern Great Plains during May 2003 IOP Lawrence Livermore National Laboratory This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 Catherine Chuang, James Boyle Shaocheng Xie and James Kelly LLNL-POST-401948 March 11, 2008 Why are aerosol/cloud interactions important? The greatest uncertainty in the assessment of radiative forcing arises from the interactions of aerosols with clouds. Radiative forcing of climate between 1750 and 2005 (IPCC, 2007) Sources of uncertainty Emissions Gas to particle conversion Aerosol size distribution Linkage between aerosols

438

AEROgui: A graphical user interface for the optical properties of aerosols  

Science Journals Connector (OSTI)

Atmospheric aerosols have an uncertain effect on climate, and serious impact on human health. The uncertainty in the aerosols role on climate has several sources. First, aerosols present a great spatial and temporal variability. The spatial variability ...

R. Pedrs; J.L. Gmez-Amo; C.R. Marcos; M.P. Utrillas; S. Ganda; F. Tena; J.A. Martinez Lozano

439

Tropospheric Aerosol Optical Thickness from the GOCART Model and Comparisons with Satellite and Sun Photometer Measurements  

Science Journals Connector (OSTI)

The Georgia Institute of TechnologyGoddard Global Ozone Chemistry Aerosol Radiation and Transport (GOCART) model is used to simulate the aerosol optical thickness ? for major types of tropospheric aerosols including sulfate, dust, organic carbon ...

Mian Chin; Paul Ginoux; Stefan Kinne; Omar Torres; Brent N. Holben; Bryan N. Duncan; Randall V. Martin; Jennifer A. Logan; Akiko Higurashi; Teruyuki Nakajima

2002-02-01T23:59:59.000Z

440

Retrieval of ozone and nitrogen dioxide concentrations from Stratospheric Aerosol and Gas Experiment III (SAGE III)  

E-Print Network (OSTI)

Retrieval of ozone and nitrogen dioxide concentrations from Stratospheric Aerosol and Gas extinction. We retrieve ozone and nitrogen dioxide number densities and aerosol extinction from transmission), Retrieval of ozone and nitrogen dioxide concentrations from Stratospheric Aerosol and Gas Experiment III

Note: This page contains sample records for the topic "research aerosol processes" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


441

Aerosol climate effects and air quality impacts from 1980 to 2030  

E-Print Network (OSTI)

Aerosol climate e?ects and air quality impacts from 1980 toAerosol climate e?ects and air quality impacts from 1980 toAerosol climate e?ects and air quality impacts from 1980 to

Menon, Surabi

2008-01-01T23:59:59.000Z

442

Statistical analysis of aerosol species, trace gasses, and meteorology in Chicago  

E-Print Network (OSTI)

possible pollutant sources. Keywords Atmospheric aerosols . Canonical correlation analysis . Chicago air pollution studies involve collection and anal- ysis of atmospheric aerosols and concurrent meteorol- ogy) and principal component analysis (PCA) were applied to atmospheric aerosol and trace gas concentrations

O'Brien, Timothy E.

443

Priorities for In-situ Aerosol Measurements  

NLE Websites -- All DOE Office Websites (Extended Search)

Priorities for In-situ Priorities for In-situ Aerosol Measurements Parameters * Aerosol light absorption coefficient - spectral, including UV, vis, and IR - as f(RH), and at ambient RH * Phase function - or relevant integral properties (how many?) * Ice nuclei * Scattering vs. RH, for RH>90% * CCN, as f(S, D p ) * Size distribution * Chemical composition - for determining climate forcing, vs. radiative effect Calibration * Number concentration * Size and shape * Light absorption reference method Characterization * Accuracy and precision - need well-understood error bars * Algorithm comparisons * Closure studies * Facilities for method testing - aircraft time Methods * Inlets - shattering/splashing - location on airplane - passing efficiency - inletless analyzers/samplers * Packaging - modular/portable "pods" for multiple a/c

444

Aerosol and graphitic carbon content of snow  

SciTech Connect

Snow samples from southern New Mexico, west Texas, Antarctica, and Greenland were analyzed for aerosol and graphitic carbon. Graphitic carbon contents were found to be between 2.2 and 25 ..mu..g L/sup -1/ of snow meltwater; water-insoluble aerosol content varied between 0.62 and 8.5 mg L/sup -1/. For comparison, two samples of Camp Century, Greenland, ice core, having approximate ages of 4,000 and 6,000 years, were also analyzed. Ice core graphitic carbon contents were found to be 2.5 and 1.1 ..mu..g L/sup -1/. copyrightAmerican Geophysical Union 1987

Chy-acute-accentlek, P.; Srivastava, V.; Cahenzli, L.; Pinnick, R.G.; Dod, R.L.; Novakov, T.; Cook, T.L.; Hinds, B.D.

1987-08-20T23:59:59.000Z

445

U.S. and Portugal Sign Agreement for Climate Research Collaboration |  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

Portugal Sign Agreement for Climate Research Collaboration Portugal Sign Agreement for Climate Research Collaboration U.S. and Portugal Sign Agreement for Climate Research Collaboration March 27, 2009 - 12:00am Addthis WASHINGTON, DC - The United States signed an agreement with Portugal today to launch the installation of a portable climate observatory on Graciosa Island in the Azores. The mobile observatory will obtain measurements of cloud and aerosol properties from the island's marine environment for 20 months, beginning in May. The measurements are expected to greatly enhance scientific understanding of the microscopic processes that occur in low-level marine clouds, and will be used to test and improve climate models. The portable observatory, or Atmospheric Radiation Measurement (ARM) Mobile Facility, is part of U.S. Department of Energy (DOE) ARM Climate Research

446

On The Importance of Organic Oxygen for Understanding Organic Aerosol  

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On The Importance of Organic Oxygen for Understanding Organic Aerosol On The Importance of Organic Oxygen for Understanding Organic Aerosol Particles Title On The Importance of Organic Oxygen for Understanding Organic Aerosol Particles Publication Type Journal Article Year of Publication 2006 Authors Pang, Yanbo, B. J. Turpin, and Lara A. Gundel Journal Journal of Aerosol Science and Technology Volume 40 Start Page Chapter Pagination 128-133 Abstract This study shows how aerosol organic oxygen data could provide new and independent information about organic aerosol mass, aqueous solubility of organic aerosols, formation of secondary organic aerosol (SOA) and the relative contributions of anthropogenic and biogenic sources. For more than two decades atmospheric aerosol organic mass concentration has usually been estimated by multiplying the measured carbon content by an assumed organic mass (OM)-to-organic carbon (OC ) factor of 1.4. However, this factor can vary from 1.0 to 2.5 depending on location. This great uncertainty about aerosol organic mass limits our understanding of the influence of organic aerosol on climate, visibility and health.New examination of organic aerosol speciation data shows that the oxygen content is the key factor responsible for the observed range in the OM-to-OC factor. When organic oxygen content is excluded, the ratio of non-oxygen organic mass to carbon mass varies very little across different environments (1.12 to 1.14). The non-oxygen-OM-to-non-oxygen OC factor for all studied sites (urban and non-urban) is 1.13± 0.02. The uncertainty becomes an order of magnitude smaller than the uncertainty in the best current estimates of organic mass to organic carbon ratios (1.6± 0.2 for urban and 2.1± 0.2 for non-urban areas). When aerosol organic oxygen data become available, organic aerosol mass can be quite accurately estimated using just OC and organic oxygen (OO) without the need to know whether the aerosol is fresh or aged. In addition, aerosol organic oxygen data will aid prediction of water solubility since compounds with OO-to-OC higher than 0.4 have water solubilities higher than 1g per 100 g water

447

Aerosol generation and entrainment model for cough simulations.  

E-Print Network (OSTI)

??The airborne transmission of diseases is of great concern to the public health community. The possible spread of infectious disease by aerosols is of particular (more)

Ersahin, Cem.

2007-01-01T23:59:59.000Z

448

Method of Preparing Super-Concentrated Jets From Dense Aerosol...  

NLE Websites -- All DOE Office Websites (Extended Search)

Michael J. Hay, Ernest J. Valeo, and Nathaniel J. Fisch This is improvement in aerodynamic focusing of dilute aerosol suspensions. All previous work on this subject has...

449

ARM - Field Campaign - Pajarito Aerosol Coupling to Ecosystems...  

NLE Websites -- All DOE Office Websites (Extended Search)

properties during the winter-spring transition. Opportunity to investigate fire and automobile emission interactions with biogenic aerosols will also harnessed MAOS will be...

450

Heavy Duty Diesel Engine Exhaust Aerosol Particle and Ion Measurements  

Science Journals Connector (OSTI)

Heavy Duty Diesel Engine Exhaust Aerosol Particle and Ion Measurements ... diesel engines have received increasing attention due to their potential health effects. ...

Tero Lhde; Topi Rnkk; Annele Virtanen; Tanja J. Schuck; Liisa Pirjola; Kaarle Hmeri; Markku Kulmala; Frank Arnold; Dieter Rothe; Jorma Keskinen

2008-12-09T23:59:59.000Z

451

Raman Lidar Measurements of Aerosols and Water Vapor During the...  

NLE Websites -- All DOE Office Websites (Extended Search)

modifications reduced but could not eliminate these adverse effects. The Raman lidar water vapor (aerosol extinction) measurements produced by these modified algorithms were,...

452

aerosol influenza transmission: Topics by E-print Network  

NLE Websites -- All DOE Office Websites (Extended Search)

and Information Sciences Websites Summary: . In preliminary work, we used artificial neural networks (ANNs) to construct global aerosol predictors by learningIntegration...

453

E-Print Network 3.0 - aerosol particle size Sample Search Results  

NLE Websites -- All DOE Office Websites (Extended Search)

Summary: of aerosol over many orders-of-magnitude of particle size range, from subcritical clusters on the molecular... to modeling aerosol dynamics under conditions of new...

454

E-Print Network 3.0 - aerosol modeling decadal Sample Search...  

NLE Websites -- All DOE Office Websites (Extended Search)

Geosciences 8 Absorbing aerosols and pre-summer monsoon hydroclimate variability over the Indian subcontinent: The challenge in investigating links Summary: in the aerosol-monsoon...

455

E-Print Network 3.0 - aerosol radiative forcing Sample Search...  

NLE Websites -- All DOE Office Websites (Extended Search)

No. DE- Summary: : WHY MEASUREMENTS ALONE CANNOT QUANTIFY AEROSOL RADIATIVE FORCING OF CLIMATE CHANGE Stephen E. Schwartz... of radiative forcing of climate change by aerosols,...

456

E-Print Network 3.0 - aerosols nanometriques application Sample...  

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is studying how aerosol particles affect everything from Summary: of aerosol particles on climate change, public health, and renewable energy applications. In particular, he......

457

E-Print Network 3.0 - aerosol lung inhalation Sample Search Results  

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aerosolized by means... is aerosolized upon inhalation by utilizing the ... Source: Groningen, Rijksuniversiteit - Centre for Ecological and Evolutionary Studies, Department of...

458

E-Print Network 3.0 - aerosol condensation model Sample Search...  

NLE Websites -- All DOE Office Websites (Extended Search)

Applied Science Collection: Environmental Sciences and Ecology 8 DETERMINING AEROSOL RADIATIVE FORCING AT ARM SITES Summary: OF AEROSOL DIRECT FORCING By linear model and by...

459

E-Print Network 3.0 - aerosol code comparisons Sample Search...  

NLE Websites -- All DOE Office Websites (Extended Search)

and Ecology 4 Estimates of global radiative forcing derived from the GlobAEROSOL dataset Summary: -sky direct aerosol radiative forcing. The Edwards and Slingo (1996)...

460

Aerosol-Cloud-Precipitation Interactions in the Trade Wind Boundary Layer.  

E-Print Network (OSTI)

??This dissertation includes an overview of aerosol, cloud, and precipitation properties associated with shallow marine cumulus clouds observed during the Barbados Aerosol Cloud Experiment (BACEX, (more)

Jung, Eunsil

2012-01-01T23:59:59.000Z

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