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1

Spent fuel utilization in a compact traveling wave reactor  

SciTech Connect (OSTI)

In recent years, several innovative designs of nuclear reactors are proposed. One of them is Traveling Wave Reactor (TWR). The unique characteristic of a TWR is the capability of breeding its own fuel in the reactor. The reactor is fueled by mostly depleted, natural uranium or spent nuclear fuel and a small amount of enriched uranium to initiate the fission process. Later on in the core, the reactor gradually converts the non-fissile material into the fissile in a process like a traveling wave. In this work, a TWR with spent nuclear fuel blanket was studied. Several parameters such as reactivity coefficients, delayed neutron fraction, prompt neutron generation lifetime, and fission power, were analyzed. The discharge burnup composition was also analyzed. The calculation is performed by a continuous energy Monte Carlo code McCARD.

Hartanto, Donny; Kim, Yonghee [Korea Advanced Institute of Science and Technology 373-1 Kusong-dong, Yuseong-gu, Daejeon, 305-701 (Korea, Republic of)

2012-06-06T23:59:59.000Z

2

Economic Analysis on Direct Use of Spent Pressurized Water Reactor Fuel in CANDU Reactors - III: Spent DUPIC Fuel Disposal Cost  

SciTech Connect (OSTI)

The disposal costs of spent pressurized water reactor (PWR), Canada deuterium uranium (CANDU) reactor, and DUPIC fuels have been estimated based on available literature data and the engineering design of a spent CANDU fuel disposal facility by the Atomic Energy of Canada Limited. The cost estimation was carried out by the normalization concept of total electricity generation. Therefore, the future electricity generation scale was analyzed to evaluate the appropriate capacity of the high-level waste disposal facility in Korea, which is a key parameter of the disposal cost estimation. Based on the total electricity generation scale, it is concluded that the disposal unit costs for spent CANDU natural uranium, CANDU-DUPIC, and PWR fuels are 192.3, 388.5, and 696.5 $/kg heavy element, respectively.

Ko, Won Il; Choi, Hangbok; Roh, Gyuhong; Yang, Myung Seung [Korea Atomic Energy Research Institute (Korea, Republic of)

2001-05-15T23:59:59.000Z

3

Dry Storage of Research Reactor Spent Nuclear Fuel - 13321  

SciTech Connect (OSTI)

Spent fuel from domestic and foreign research reactors is received and stored at the Savannah River Site's L Area Material Storage (L Basin) Facility. This DOE-owned fuel consists primarily of highly enriched uranium in metal, oxide or silicide form with aluminum cladding. Upon receipt, the fuel is unloaded and transferred to basin storage awaiting final disposition. Disposition alternatives include processing via the site's H Canyon facility for uranium recovery, or packaging and shipment of the spent fuel to a waste repository. A program has been developed to provide a phased approach for dry storage of the L Basin fuel. The initial phase of the dry storage program will demonstrate loading, drying, and storage of fuel in twelve instrumented canisters to assess fuel performance. After closure, the loaded canisters are transferred to pad-mounted concrete overpacks, similar to those used for dry storage of commercial fuel. Unlike commercial spent fuel, however, the DOE fuel has high enrichment, very low to high burnup, and low decay heat. The aluminum cladding presents unique challenges due to the presence of an oxide layer that forms on the cladding surface, and corrosion degradation resulting from prolonged wet storage. The removal of free and bound water is essential to the prevention of fuel corrosion and radiolytic generation of hydrogen. The demonstration will validate models predicting pressure, temperature, gas generation, and corrosion performance, provide an engineering scale demonstration of fuel handling, drying, leak testing, and canister backfill operations, and establish 'road-ready' storage of fuel that is suitable for offsite repository shipment or retrievable for onsite processing. Implementation of the Phase I demonstration can be completed within three years. Phases II and III, leading to the de-inventory of L Basin, would require an additional 750 canisters and 6-12 years to complete. Transfer of the fuel from basin storage to dry storage requires integration with current facility operations, and selection of equipment that will allow safe operation within the constraints of existing facility conditions. Examples of such constraints that are evaluated and addressed by the dry storage program include limited basin depth, varying fuel lengths up to 4 m, (13 ft), fissile loading limits, canister closure design, post-load drying and closure of the canisters, instrument selection and installation, and movement of the canisters to storage casks. The initial pilot phase restricts the fuels to shorter length fuels that can be loaded to the canister directly underwater; subsequent phases will require use of a shielded transfer system. Removal of the canister from the basin, followed by drying, inerting, closure of the canister, and transfer of the canister to the storage cask are completed with remotely operated equipment and appropriate shielding to reduce personnel radiation exposure. (authors)

Adams, T.M.; Dunsmuir, M.D.; Leduc, D.R.; Severynse, T.F.; Sindelar, R.L. [Savannah River National Laboratory (United States)] [Savannah River National Laboratory (United States); Moore, E.N. [Moore Nuclear Energy, LLC (United States)] [Moore Nuclear Energy, LLC (United States)

2013-07-01T23:59:59.000Z

4

Foreign Research Reactor Spent Nuclear Fuel Acceptance Program  

Broader source: Energy.gov (indexed) [DOE]

Global Threat Reduction Initiative: Global Threat Reduction Initiative: U.S. Nuclear Remove Program Foreign Research Reactor Spent Nuclear Fuel (FRR SNF) Acceptance 2007 DOE TEC Meeting Chuck Messick DOE/NNSA/SRS 2 Contents * Program Objective and Policy * Program implementation status * Shipment Information * Operational Logistics * Lessons Learned * Conclusion 3 U.S. Nuclear Remove Program Objective * To play a key role in the Global Threat Reduction Remove Program supporting permanent threat reduction by accepting program eligible material. * Works in conjunction with the Global Threat Reduction Convert Program to accept program eligible material as an incentive to core conversion providing a disposition path for HEU and LEU during the life of the Acceptance Program. 4 Reasons for the Policy

5

Determining Reactor Flux from Xenon-136 and Cesium-135 in Spent Fuel  

E-Print Network [OSTI]

The ability to infer the reactor flux from spent fuel or seized fissile material would enhance the tools of nuclear forensics and nuclear nonproliferation significantly. We show that reactor flux can be inferred from the ratios of xenon-136 to xenon-134 and cesium-135 to cesium-137. If the average flux of a reactor is known, the flux inferred from measurements of spent fuel could help determine whether that spent fuel was loaded as a blanket or close to the mid-plane of the reactor. The cesium ratio also provides information on reactor shutdowns during the irradiation of fuel, which could prove valuable for identifying the reactor in question through comparisons with satellite reactor heat monitoring data. We derive analytic expressions for these correlations and compare them to experimental data and to detailed reactor burn simulations. The enrichment of the original uranium fuel affects the correlations by up to 3 percent, but only at high flux.

A. C. Hayes; Gerard Jungman

2012-05-30T23:59:59.000Z

6

The burnup dependence of light water reactor spent fuel oxidation  

SciTech Connect (OSTI)

Over the temperature range of interest for dry storage or for placement of spent fuel in a permanent repository under the conditions now being considered, UO{sub 2} is thermodynamically unstable with respect to oxidation to higher oxides. The multiple valence states of uranium allow for the accommodation of interstitial oxygen atoms in the fuel matrix. A variety of stoichiometric and nonstoichiometric phases is therefore possible as the fuel oxidizers from UO{sub 2} to higher oxides. The oxidation of UO{sub 2} has been studied extensively for over 40 years. It has been shown that spent fuel and unirradiated UO{sub 2} oxidize via different mechanisms and at different rates. The oxidation of LWR spent fuel from UO{sub 2} to UO{sub 2.4} was studied previously and is reasonably well understood. The study presented here was initiated to determine the mechanism and rate of oxidation from UO{sub 2.4} to higher oxides. During the early stages of this work, a large variability in the oxidation behavior of samples oxidized under nearly identical conditions was found. Based on previous work on the effect of dopants on UO{sub 2} oxidation and this initial variability, it was hypothesized that the substitution of fission product and actinide impurities for uranium atoms in the spent fuel matrix was the cause of the variable oxidation behavior. Since the impurity concentration is roughly proportional to the burnup of a specimen, the oxidation behavior of spent fuel was expected to be a function of both temperature and burnup. This report (1) summarizes the previous oxidation work for both unirradiated UO{sub 2} and spent fuel (Section 2.2) and presents the theoretical basis for the burnup (i.e., impurity concentration) dependence of the rate of oxidation (Sections 2.3, 2.4, and 2.5), (2) describes the experimental approach (Section 3) and results (Section 4) for the current oxidation tests on spent fuel, and (3) establishes a simple model to determine the activation energies associated with spent fuel oxidation (Section 5).

Hanson, B.D.

1998-07-01T23:59:59.000Z

7

Economic Analysis on Direct Use of Spent Pressurized Water Reactor Fuel in CANDU Reactors - I: DUPIC Fuel Fabrication Cost  

SciTech Connect (OSTI)

A preliminary conceptual design of a Direct Use of spent Pressurized water reactor (PWR) fuel In Canada deuterium uranium (CANDU) reactors (DUPIC) fuel fabrication plant was studied, which annually converts spent PWR fuel of 400 tonnes heavy element (HE) into CANDU fuel. The capital and operating costs were estimated from the viewpoint of conceptual design. Assuming that the annual discount rate is 5% during the construction (5 yr) and operation period (40 yr) and contingency is 25% of the capital cost, the levelized unit cost (LUC) of DUPIC fuel fabrication was estimated to be 616 $/kg HE, which is mostly governed by annual operation and maintenance costs that correspond to 63% of LUC. Among the operation and maintenance cost components being considered, the waste disposal cost has the dominant effect on LUC ({approx}49%). From sensitivity analyses of production capacity, discount rate, and contingency, it was found that the production capacity of the plant is the major parameter that affects the LUC.

Choi, Hangbok; Ko, Won Il; Yang, Myung Seung [Korea Atomic Energy Research Institute (Korea, Republic of)

2001-05-15T23:59:59.000Z

8

Nuclear nonproliferation: Concerns with US delays in accepting foregin research reactors` spent fuel  

SciTech Connect (OSTI)

One key US nonproliferation goal is to discourage use of highly enriched uranium fuel (HEU), which can be used to make nuclear bombs, in civilian nuclear programs worldwide. DOE`s Off-Site Fuels Policy for taking back spent HEU from foreign research reactors was allowed to expire due to environmental reasons. This report provides information on the effects of delays in renewing the Off-Site Fuels Policy on US nonproliferation goals and programs (specifically the reduced enrichment program), DOE`s efforts to renew the fuels policy, and the price to be charged to the operators of foreign reactors for DOE`s activities in taking back spent fuel.

NONE

1994-03-25T23:59:59.000Z

9

Radio-toxicity of spent fuel of the advanced heavy water reactor  

Science Journals Connector (OSTI)

......Radio-toxicity of spent fuel of the advanced heavy water reactor S. Anand * K. D. S...Mumbai 400085, India The Advanced Heavy Water Reactor (AHWR) is a new power...PHWR. INTRODUCTION The Advanced Heavy Water Reactor (AHWR)(1, 2), currently......

S. Anand; K. D. S. Singh; V. K. Sharma

2010-01-01T23:59:59.000Z

10

MANAGEMENT OF RESEARCH AND TEST REACTOR ALUMINUM SPENT NUCLEAR FUEL - A TECHNOLOGY ASSESSMENT  

SciTech Connect (OSTI)

The Department of Energy's Environmental Management (DOE-EM) Program is responsible for the receipt and storage of aluminum research reactor spent nuclear fuel or used fuel until ultimate disposition. Aluminum research reactor used fuel is currently being stored or is anticipated to be returned to the U.S. and stored at DOE-EM storage facilities at the Savannah River Site and the Idaho Nuclear Technology and Engineering Center. This paper assesses the technologies and the options for safe transportation/receipt and interim storage of aluminum research reactor spent fuel and reviews the comprehensive strategy for its management. The U.S. Department of Energy uses the Appendix A, Spent Nuclear Fuel Acceptance Criteria, to identify the physical, chemical, and isotopic characteristics of spent nuclear fuel to be returned to the United States under the Foreign Research Reactor Spent Nuclear Fuel Acceptance Program. The fuel is further evaluated for acceptance through assessments of the fuel at the foreign sites that include corrosion damage and handleability. Transport involves use of commercial shipping casks with defined leakage rates that can provide containment of the fuel, some of which are breached. Options for safe storage include wet storage and dry storage. Both options must fully address potential degradation of the aluminum during the storage period. This paper focuses on the various options for safe transport and storage with respect to technology maturity and application.

Vinson, D.

2010-07-11T23:59:59.000Z

11

In-Situ Safeguards Verification of Low Burn-up Pressurized Water Reactor Spent Fuel Assemblies  

SciTech Connect (OSTI)

A novel in-situ gross defect verification method for light water reactor spent fuel assemblies was developed and investigated by a Monte Carlo study. This particular method is particularly effective for old pressurized water reactor spent fuel assemblies that have natural uranium in their upper fuel zones. Currently there is no method or instrument that does verification of this type of spent fuel assemblies without moving the spent fuel assemblies from their storage positions. The proposed method uses a tiny neutron detector and a detector guiding system to collect neutron signals inside PWR spent fuel assemblies through guide tubes present in PWR assemblies. The data obtained in such a manner are used for gross defect verification of spent fuel assemblies. The method uses 'calibration curves' which show the expected neutron counts inside one of the guide tubes of spent fuel assemblies as a function of fuel burn-up. By examining the measured data in the 'calibration curves', the consistency of the operator's declaration is verified.

Ham, Y S; Sitaraman, S; Park, I; Kim, J; Ahn, G

2008-04-16T23:59:59.000Z

12

Fresh and Spent Nuclear Fuel Repatriation from the IRT-2000 Research Reactor Facility, Sofia, Bulgaria  

SciTech Connect (OSTI)

The IRT 2000 research reactor, operated by the Bulgarian Institute for Nuclear Research and Nuclear Energy (INRNE), safely shipped all of their Russian-origin nuclear fuel from the Republic of Bulgaria to the Russian Federation beginning in 2003 and completing in 2008. These fresh and spent fuel shipments removed all highly enriched uranium (HEU) from Bulgaria. The fresh fuel was shipped by air in December 2003 using trucks and a commercial cargo aircraft. One combined spent fuel shipment of HEU and low enriched uranium (LEU) was completed in July 2008 using high capacity VPVR/M casks transported by truck, barge, and rail. The HEU shipments were assisted by the Russian Research Reactor Fuel Return Program (RRRFR) and the LEU spent fuel shipment was funded by Bulgaria. This report describes the work, approvals, organizations, equipment, and agreements required to complete these shipments and concludes with several major lessons learned.

K. J. Allen; T. G. Apostolov; I. S. Dimitrov

2009-03-01T23:59:59.000Z

13

Spent nuclear fuel discharges from US reactors 1992  

SciTech Connect (OSTI)

This report provides current statistical data on every fuel assembly irradiated in commercial nuclear reactors operating in the United States. It also provides data on the current inventories and storage capacities of those reactors to a wide audience, including Congress, Federal and State agencies, the nuclear and electric industries and the general public. It uses data from the mandatory, ``Nuclear Fuel Data`` survey, Form RW-859 for 1992 and historical data collected by the Energy Information Administration (EIA) on previous Form RW-859 surveys. The report was prepared by the EIA under a Memorandum of Understanding with the Office of Civilian Radioactive Waste Management.

Not Available

1994-05-05T23:59:59.000Z

14

Spent Nuclear Fuel (SNF) Project Acceptance Criteria for Light Water Reactor Spent Fuel Storage System [OCRWM PER REV2  

SciTech Connect (OSTI)

As part of the decommissioning of the 324 Building Radiochemical Engineering Cells there is a need to remove commercial Light Water Reactor (LWR) spent nuclear fuel (SNF) presently stored in these hot cells. To enable fuel removal from the hot cells, the commercial LWR SNF will be packaged and shipped to the 200 Area Interim Storage Area (ISA) in a manner that satisfies site requirements for SNF interim storage. This document identifies the criteria that the 324 Building Radiochemical Engineering Cell Clean-out Project must satisfy for acceptance of the LWR SNF by the SNF Project at the 200 Area ISA. In addition to the acceptance criteria identified herein, acceptance is contingent on adherence to applicable Project Hanford Management Contract requirements and procedures in place at the time of work execution.

JOHNSON, D.M.

2000-12-20T23:59:59.000Z

15

Environmental Assessment of Urgent-Relief Acceptance of Foreign Research Reactor Spent Nuclear Fuel  

SciTech Connect (OSTI)

The Department of Energy has completed the Environmental Assessment (EA) of Urgent-Relief Acceptance of Foreign Research Reactor Spent Nuclear Fuel and issued a Finding of No Significant Impact (FONSI) for the proposed action. The EA and FONSI are enclosed for your information. The Department has decided to accept a limited number of spent nuclear fuel elements (409 elements) containing uranium that was enriched in the United States from eight research reactors in Austria, Denmark, Germany, Greece, the Netherlands, Sweden, and Switzerland. This action is necessary to maintain the viability of a major US nuclear weapons nonproliferation program to limit or eliminate the use of highly enriched uranium in civil programs. The purpose of the EA is to maintain the cooperation of the foreign research reactor operators with the nonproliferation program while a more extensive Environmental Impact Statement (EIS) is prepared on a proposed broader policy involving the acceptance of up to 15,000 foreign research reactor spent fuel elements over a 10 to 15 year period. Based on an evaluation of transport by commercial container liner or chartered vessel, five eastern seaboard ports, and truck and train modes of transporting the spent fuel overland to the Savannah River Sits, the Department has concluded that no significant impact would result from any combination of port and made of transport. In addition, no significant impacts were found from interim storage of spent fuel at the Savannah River Site.

Not Available

1994-04-01T23:59:59.000Z

16

Report to Congress on Plan for Interim Storage of Spent Nuclear Fuel from Decommissioned Reactors  

Broader source: Energy.gov (indexed) [DOE]

6 6 Report to Congress on the Demonstration of the Interim Storage of Spent Nuclear Fuel from Decommissioned Nuclear Power Reactor Sites December 2008 U.S. Department of Energy Office of Civilian Radioactive Waste Management Washington, D.C. Report to Congress on the Demonstration of the Interim Storage of Spent Nuclear Fuel The picture on the cover is the Connecticut Yankee Independent Spent Fuel Storage Installation site in Haddam, Connecticut, with 43 dry storage NRC-licensed dual-purpose (storage and transport) casks. ii Report to Congress on the Demonstration of the Interim Storage of Spent Nuclear Fuel EXECUTIVE SUMMARY The House Appropriations Committee Print that accompanied the Consolidated Appropriations Act, 2008, requests that the U.S. Department of Energy (the Department):

17

Advanced dry head-end reprocessing of light water reactor spent nuclear fuel  

SciTech Connect (OSTI)

A method for reprocessing spent nuclear fuel from a light water reactor includes the step of reacting spent nuclear fuel in a voloxidation vessel with an oxidizing gas having nitrogen dioxide and oxygen for a period sufficient to generate a solid oxidation product of the spent nuclear fuel. The reacting step includes the step of reacting, in a first zone of the voloxidation vessel, spent nuclear fuel with the oxidizing gas at a temperature ranging from 200-450.degree. C. to form an oxidized reaction product, and regenerating nitrogen dioxide, in a second zone of the voloxidation vessel, by reacting oxidizing gas comprising nitrogen monoxide and oxygen at a temperature ranging from 0-80.degree. C. The first zone and the second zone can be separate. A voloxidation system is also disclosed.

Collins, Emory D.; Delcul, Guillermo D.; Hunt, Rodney D.; Johnson, Jared A.; Spencer, Barry B.

2014-06-10T23:59:59.000Z

18

Advanced dry head-end reprocessing of light water reactor spent nuclear fuel  

DOE Patents [OSTI]

A method for reprocessing spent nuclear fuel from a light water reactor includes the step of reacting spent nuclear fuel in a voloxidation vessel with an oxidizing gas having nitrogen dioxide and oxygen for a period sufficient to generate a solid oxidation product of the spent nuclear fuel. The reacting step includes the step of reacting, in a first zone of the voloxidation vessel, spent nuclear fuel with the oxidizing gas at a temperature ranging from 200-450.degree. C. to form an oxidized reaction product, and regenerating nitrogen dioxide, in a second zone of the voloxidation vessel, by reacting oxidizing gas comprising nitrogen monoxide and oxygen at a temperature ranging from 0-80.degree. C. The first zone and the second zone can be separate. A voloxidation system is also disclosed.

Collins, Emory D; Delcul, Guillermo D; Hunt, Rodney D; Johnson, Jared A; Spencer, Barry B

2013-11-05T23:59:59.000Z

19

Pyroprocessing of Light Water Reactor Spent Fuels Based on an Electrochemical Reduction Technology  

SciTech Connect (OSTI)

A concept of pyroprocessing light water reactor (LWR) spent fuels based on an electrochemical reduction technology is proposed, and the material balance of the processing of mixed oxide (MOX) or high-burnup uranium oxide (UO{sub 2}) spent fuel is evaluated. Furthermore, a burnup analysis for metal fuel fast breeder reactors (FBRs) is conducted on low-decontamination materials recovered by pyroprocessing. In the case of processing MOX spent fuel (40 GWd/t), UO{sub 2} is separately collected for {approx}60 wt% of the spent fuel in advance of the electrochemical reduction step, and the product recovered through the rare earth (RE) removal step, which has the composition uranium:plutonium:minor actinides:fission products (FPs) = 76.4:18.4:1.7:3.5, can be applied as an ingredient of FBR metal fuel without a further decontamination process. On the other hand, the electroreduced alloy of high-burnup UO{sub 2} spent fuel (48 GWd/t) requires further decontamination of residual FPs by an additional process such as electrorefining even if RE FPs are removed from the alloy because the recovered plutonium (Pu) is accompanied by almost the same amount of FPs in addition to RE. However, the amount of treated materials in the electrorefining step is reduced to {approx}10 wt% of the total spent fuel owing to the prior UO{sub 2} recovery step. These results reveal that the application of electrochemical reduction technology to LWR spent oxide fuel is a promising concept for providing FBR metal fuel by a rationalized process.

Ohta, Hirokazu; Inoue, Tadashi; Sakamura, Yoshiharu; Kinoshita, Kensuke

2005-05-15T23:59:59.000Z

20

Radio-toxicity of spent fuel of the advanced heavy water reactor  

Science Journals Connector (OSTI)

......during their short/long term-storage is investigated in...radio-toxicity of radioactive waste is widely regarded...exchangers of the spent fuel storage bay. The decay power...VVER type reactors at long-term storage. Radiat. Prot. Dosim......

S. Anand; K. D. S. Singh; V. K. Sharma

2010-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


21

Spent Isopropanol Solution as Possible Liquid Fuel for Moving Bed Reactor in Chemical Looping Combustion  

Science Journals Connector (OSTI)

Spent Isopropanol Solution as Possible Liquid Fuel for Moving Bed Reactor in Chemical Looping Combustion ... The fuels, such as natural gas, coal, petroleum coke, and biomass combusted by CLC are frequently studied by various researchers(17, 26-31) and compared in the previous studies;(20, 33) however, only few studies on liquid fuel combustion are reported. ... Ishida, M.; Takeshita, K.; Susuki, K.; Ohba, T..Application of Fe2O3-Al2O3 composite particles as solid looping material of the chemical loop combustor Energy Fuels 2005, 19, 2514– 2518 ...

Ping-Chin Chiu; Young Ku; Hsuan-Chih Wu; Yu-Lin Kuo; Yao-Hsuan Tseng

2013-10-31T23:59:59.000Z

22

Modeling the Pyrochemical Reduction of Spent UO2 Fuel in a Pilot-Scale Reactor  

SciTech Connect (OSTI)

A kinetic model has been derived for the reduction of oxide spent nuclear fuel in a radial flow reactor. In this reaction, lithium dissolved in molten LiCl reacts with UO2 and fission product oxides to form a porous, metallic product. As the reaction proceeds, the depth of the porous layer around the exterior of each fuel particle increases. The observed rate of reaction has been found to be only dependent upon the rate of diffusion of lithium across this layer, consistent with a classic shrinking core kinetic model. This shrinking core model has been extended to predict the behavior of a hypothetical, pilot-scale reactor for oxide reduction. The design of the pilot-scale reactor includes forced flow through baskets that contain the fuel particles. The results of the modeling indicate that this is an essential feature in order to minimize the time needed to achieve full conversion of the fuel.

Steven D. Herrmann; Michael F. Simpson

2006-08-01T23:59:59.000Z

23

Summary engineering description of underwater fuel storage facility for foreign research reactor spent nuclear fuel  

SciTech Connect (OSTI)

This document is a summary description for an Underwater Fuel Storage Facility (UFSF) for foreign research reactor (FRR) spent nuclear fuel (SNF). A FRR SNF environmental Impact Statement (EIS) is being prepared and will include both wet and dry storage facilities as storage alternatives. For the UFSF presented in this document, a specific site is not chosen. This facility can be sited at any one of the five locations under consideration in the EIS. These locations are the Idaho National Engineering Laboratory, Savannah River Site, Hanford, Oak Ridge National Laboratory, and Nevada Test Site. Generic facility environmental impacts and emissions are provided in this report. A baseline fuel element is defined in Section 2.2, and the results of a fission product analysis are presented. Requirements for a storage facility have been researched and are summarized in Section 3. Section 4 describes three facility options: (1) the Centralized-UFSF, which would store the entire fuel element quantity in a single facility at a single location, (2) the Regionalized Large-UFSF, which would store 75% of the fuel element quantity in some region of the country, and (3) the Regionalized Small-UFSF, which would store 25% of the fuel element quantity, with the possibility of a number of these facilities in various regions throughout the country. The operational philosophy is presented in Section 5, and Section 6 contains a description of the equipment. Section 7 defines the utilities required for the facility. Cost estimates are discussed in Section 8, and detailed cost estimates are included. Impacts to worker safety, public safety, and the environment are discussed in Section 9. Accidental releases are presented in Section 10. Standard Environmental Impact Forms are included in Section 11.

Dahlke, H.J.; Johnson, D.A.; Rawlins, J.K.; Searle, D.K.; Wachs, G.W.

1994-10-01T23:59:59.000Z

24

Spent fuel pyroprocessing demonstration  

SciTech Connect (OSTI)

A major element of the shutdown of the US liquid metal reactor development program is managing the sodium-bonded spent metallic fuel from the Experimental Breeder Reactor-II to meet US environmental laws. Argonne National Laboratory has refurbished and equipped an existing hot cell facility for treating the spent fuel by a high-temperature electrochemical process commonly called pyroprocessing. Four products will be produced for storage and disposal. Two high-level waste forms will be produced and qualified for disposal of the fission and activation products. Uranium and transuranium alloys will be produced for storage pending a decision by the US Department of Energy on the fate of its plutonium and enriched uranium. Together these activities will demonstrate a unique electrochemical treatment technology for spent nuclear fuel. This technology potentially has significant economic and technical advantages over either conventional reprocessing or direct disposal as a high-level waste option.

McFarlane, L.F.; Lineberry, M.J.

1995-05-01T23:59:59.000Z

25

Categorization of failed and damaged spent LWR (light-water reactor) fuel currently in storage  

SciTech Connect (OSTI)

The results of a study that was jointly sponsored by the US Department of Energy and the Electric Power Research Institute are described in this report. The purpose of the study was to (1) estimate the number of failed fuel assemblies and damaged fuel assemblies (i.e., ones that have sustained mechanical or chemical damage but with fuel rod cladding that is not breached) in storage, (2) categorize those fuel assemblies, and (3) prepare this report as an authoritative, illustrated source of information on such fuel. Among the more than 45,975 spent light-water reactor fuel assemblies currently in storage in the United States, it appears that there are nearly 5000 failed or damaged fuel assemblies. 78 refs., 23 figs., 19 tabs.

Bailey, W.J.

1987-11-01T23:59:59.000Z

26

Intact and Degraded Component Criticality Calculations of N Reactors Spent Nuclear Fuel  

SciTech Connect (OSTI)

The objective of this calculation is to perform intact and degraded mode criticality evaluations of the Department of Energy's (DOE) N Reactor Spent Nuclear Fuel codisposed in a 2-Defense High-Level Waste (2-DHLW)/2-Multi-Canister Overpack (MCO) Waste Package (WP) and emplaced in a monitored geologic repository (MGR) (see Attachment I). The scope of this calculation is limited to the determination of the effective neutron multiplication factor (k{sub eff}) for both intact and degraded mode internal configurations of the codisposal waste package. This calculation will support the analysis that will be performed to demonstrate the technical viability for disposing of U-metal (N Reactor) spent nuclear fuel in the potential MGR.

L. Angers

2001-01-31T23:59:59.000Z

27

Analysis of Experimental Data for High Burnup PWR Spent Fuel Isotopic Validation - Vandellos II Reactor  

SciTech Connect (OSTI)

This report is one of the several recent NUREG/CR reports documenting benchmark-quality radiochemical assay data and the use of the data to validate computer code predictions of isotopic composition for spent nuclear fuel, to establish the uncertainty and bias associated with code predictions. The experimental data analyzed in the current report were acquired from a high-burnup fuel program coordinated by Spanish organizations. The measurements included extensive actinide and fission product data of importance to spent fuel safety applications, including burnup credit, decay heat, and radiation source terms. Six unique spent fuel samples from three uranium oxide fuel rods were analyzed. The fuel rods had a 4.5 wt % {sup 235}U initial enrichment and were irradiated in the Vandellos II pressurized water reactor operated in Spain. The burnups of the fuel samples range from 42 to 78 GWd/MTU. The measurements were used to validate the two-dimensional depletion sequence TRITON in the SCALE computer code system.

Ilas, Germina [ORNL; Gauld, Ian C [ORNL

2011-01-01T23:59:59.000Z

28

DOE/EIS-0218-SA-3: Supplement Analysis for the Foreign Research Reactor Spent Nuclear Fuel Acceptance Program (November 2004)  

Broader source: Energy.gov (indexed) [DOE]

SUPPLEMENT ANALYSIS FOR THE FOREIGN SUPPLEMENT ANALYSIS FOR THE FOREIGN RESEARCH REACTOR SPENT NUCLEAR FUEL ACCEPTANCE PROGRAM NOVEMBER 2004 DOE/EIS-0218-SA-3 U.S. Department of Energy National Nuclear Security Administration Washington, DC Final Supplement Analysis for the Foreign Research Reactor Spent Nuclear Fuel Acceptance Program Final i TABLE OF CONTENTS Page 1. Introduction.............................................................................................................................................. 1 2. Background .............................................................................................................................................. 1 3. The Proposed Action ...............................................................................................................................

29

German concept and status of the disposal of spent fuel elements from German research reactors  

SciTech Connect (OSTI)

Eight research reactors with a power {>=} 100 kW are currently being operated in the Federal Republic of Germany. These comprise three TRIGA-type reactors (power 100 kW to 250 kW), four swimming-pool reactors (power 1 MW to 10 MW) and one DIDO type reactor (power 23 MW). The German research reactors are used for neutron scattering for basic research in the field of solid state research, neutron metrology, for the fabrication of isotopes and for neutron activation analysis for medicine and biology, for investigating the influence of radiation on materials and for nuclear fuel behavior. It will be vital to continue current investigations in the future. Further operation of the German research reactors is therefore indispensable. Safe, regular disposal of the irradiated fuel elements arising now and in future operation is of primary importance. Furthermore, there are several plants with considerable quantities of spent fuel, the safe disposal of which is a matter of urgency. These include above all the VKTA facilities in Rossendorf and also the TRIGA reactors, where disposal will only be necessary upon decommissioning. The present paper report is concerned with the disposal of fuel from the German research reactors. It briefly deals with the situation in the USA since the end of 1988, describes interim solutions for current disposal requirements and then mainly concentrates on the German disposal concept currently being prepared. This concept initially envisages the long-term (25--50 years) dry interim storage of fuel elements in special containers in a central German interim store with subsequent direct final disposal without reprocessing of the irradiated fuel.

Komorowski, K. [Bundesministerium fuer Bildung Wissenschaft, Bonn (Germany); Storch, S.; Thamm, G. [Forschungszentrum Juelich GmbH (Germany)

1995-12-31T23:59:59.000Z

30

Electrolytic Reduction of Spent Light Water Reactor Fuel Bench-Scale Experiment Results  

SciTech Connect (OSTI)

A series of experiments were performed to demonstrate the electrolytic reduction of spent light water reactor fuel at bench-scale in a hot cell at the Idaho National Laboratory Materials and Fuels Complex. The process involves the conversion of oxide fuel to metal by electrolytic means, which would then enable subsequent separation and recovery of actinides via existing electrometallurgical technologies, i.e., electrorefining. Four electrolytic reduction runs were performed at bench scale using ~500 ml of molten LiCl – 1 wt% Li2O electrolyte at 650 ºC. In each run, ~50 g of crushed spent oxide fuel was loaded into a permeable stainless steel basket and immersed into the electrolyte as the cathode. A spiral wound platinum wire was immersed into the electrolyte as the anode. When a controlled electric current was conducted through the anode and cathode, the oxide fuel was reduced to metal in the basket and oxygen gas was evolved at the anode. Salt samples were extracted before and after each electrolytic reduction run and analyzed for fuel and fission product constituents. The fuel baskets following each run were sectioned and the fuel was sampled, revealing an extent of uranium oxide reduction in excess of 98%.

Steven D. Herrmann

2007-04-01T23:59:59.000Z

31

Record of Decision for the Final EIS on Proposed Nuclear Weapons Nonproliferation Policy Concerning Foreign Research Reactor Spent Nuclear Fuel  

Broader source: Energy.gov (indexed) [DOE]

5091 5091 Friday May 17, 1996 Part IV Department of Energy Record of Decision for the Final Environmental Impact Statement on a Proposed Nuclear Weapons Nonproliferation Policy Concerning Foreign Research Reactor Spent Nuclear Fuel; Notice 25092 Federal Register / Vol. 61, No. 97 / Friday, May 17, 1996 / Notices DEPARTMENT OF ENERGY Record of Decision for the Final Environmental Impact Statement on a Proposed Nuclear Weapons Nonproliferation Policy Concerning Foreign Research Reactor Spent Nuclear Fuel AGENCY: Department of Energy. ACTION: Record of decision. SUMMARY: DOE, in consultation with the Department of State, has decided to implement a new foreign research reactor spent fuel acceptance policy as specified in the Preferred Alternative contained in the Final Environmental Impact Statement on a Proposed

32

Combined cooling and purification system for nuclear reactor spent fuel pit, refueling cavity, and refueling water storage tank  

DOE Patents [OSTI]

The spent fuel pit of a pressured water reactor (PWR) nuclear power plant has sufficient coolant capacity that a safety rated cooling system is not required. A non-safety rated combined cooling and purification system with redundant branches selectively provides simultaneously cooling and purification for the spent fuel pit, the refueling cavity, and the refueling water storage tank, and transfers coolant from the refueling water storage tank to the refueling cavity without it passing through the reactor core. Skimmers on the suction piping of the combined cooling and purification system eliminate the need for separate skimmer circuits with dedicated pumps.

Corletti, Michael M. (New Kensington, PA); Lau, Louis K. (Monroeville, PA); Schulz, Terry L. (Murrysville Boro, PA)

1993-01-01T23:59:59.000Z

33

Radiation Exposures Associated with Shipments of Foreign Research Reactor Spent Nuclear Fuel  

SciTech Connect (OSTI)

Experience has shown that the analyses of marine transport of spent fuel in the Environmental Impact Statement (EIS) were conservative. It is anticipated that for most shipments. The external dose rate for the loaded transportation cask will be more in line with recent shipments. At the radiation levels associated with these shipments, we would not expect any personnel to exceed radiation exposure limits for the public. Package dose rates usually well below the regulatory limits and personnel work practices following ALARA principles are keeping human exposures to minimal levels. However, the potential for Mure shipments with external dose rates closer to the exclusive-use regulatory limit suggests that DOE should continue to provide a means to assure that individual crew members do not receive doses in excess of the public dose limits. As a minimum, the program will monitor cask dose rates and continue to implement administrative procedures that will maintain records of the dose rates associated with each shipment, the vessel used, and the crew list for the vessel. DOE will continue to include a clause in the contract for shipment of the foreign research reactor spent nuclear fuel requiring that the Mitigation Action Plan be followed.

MASSEY,CHARLES D.; MESSICK,C.E.; MUSTIN,T.

1999-11-01T23:59:59.000Z

34

Calculations of thermal-reactor spent-fuel nuclide inventories and comparisons with measurements  

SciTech Connect (OSTI)

Comparisons with integral measurements have demonstrated the accuracy of CINDER codes and libraries in calculating aggregate fission-product properties, including neutron absorption, decay power, and decay spectra. CINDER calculations have, alternatively, been used to supplement measured integral data describing fission-product decay power and decay spectra. Because of the incorporation of the extensive actinide library and the use of ENDF/B-V data, it is desirable to compare the inventory of individual nuclides obtained from tandem EPRI-CELL/CINDER-2 calculations with those determined in documented benchmark inventory measurements of spent reactor fuel. The development of the popular /sup 148/Nd burnup measurement procedure is outlined, and areas of uncertainty in it and lack of clarity in its interpretation are indicated. Six inventory samples of varying quality and completeness are examined. The power histories used in the calculations have been listed for other users.

Wilson, W.B.; LaBauve, R.J.; England, T.R.

1982-01-01T23:59:59.000Z

35

Management of Hanford Site non-defense production reactor spent nuclear fuel, Hanford Site, Richland, Washington  

SciTech Connect (OSTI)

The US Department of Energy (DOE) needs to provide radiologically, and industrially safe and cost-effective management of the non-defense production reactor spent nuclear fuel (SNF) at the Hanford Site. The proposed action would place the Hanford Site`s non-defense production reactor SNF in a radiologically- and industrially-safe, and passive storage condition pending final disposition. The proposed action would also reduce operational costs associated with storage of the non-defense production reactor SNF through consolidation of the SNF and through use of passive rather than active storage systems. Environmental, safety and health vulnerabilities associated with existing non-defense production reactor SNF storage facilities have been identified. DOE has determined that additional activities are required to consolidate non-defense production reactor SNF management activities at the Hanford Site, including cost-effective and safe interim storage, prior to final disposition, to enable deactivation of facilities where the SNF is now stored. Cost-effectiveness would be realized: through reduced operational costs associated with passive rather than active storage systems; removal of SNF from areas undergoing deactivation as part of the Hanford Site remediation effort; and eliminating the need to duplicate future transloading facilities at the 200 and 400 Areas. Radiologically- and industrially-safe storage would be enhanced through: (1) removal from aging facilities requiring substantial upgrades to continue safe storage; (2) utilization of passive rather than active storage systems for SNF; and (3) removal of SNF from some storage containers which have a limited remaining design life. No substantial increase in Hanford Site environmental impacts would be expected from the proposed action. Environmental impacts from postulated accident scenarios also were evaluated, and indicated that the risks associated with the proposed action would be small.

NONE

1997-03-01T23:59:59.000Z

36

Achieving increased spent fuel storage capacity at the High Flux Isotope Reactor (HFIR)  

SciTech Connect (OSTI)

The HFIR facility was originally designed to store approximately 25 spent cores, sufficient to allow for operational contingencies and for cooling prior to off-site shipment for reprocessing. The original capacity has now been increased to 60 positions, of which 53 are currently filled (September 1994). Additional spent cores are produced at a rate of about 10 or 11 per year. Continued HFIR operation, therefore, depends on a significant near-term expansion of the pool storage capacity, as well as on a future capability of reprocessing or other storage alternatives once the practical capacity of the pool is reached. To store the much larger inventory of spent fuel that may remain on-site under various future scenarios, the pool capacity is being increased in a phased manner through installation of a new multi-tier spent fuel rack design for higher density storage. A total of 143 positions was used for this paper as the maximum practical pool capacity without impacting operations; however, greater ultimate capacities were addressed in the supporting analyses and approval documents. This paper addresses issues related to the pool storage expansion including (1) seismic effects on the three-tier storage arrays, (2) thermal performance of the new arrays, (3) spent fuel cladding corrosion concerns related to the longer period of pool storage, and (4) impacts of increased spent fuel inventory on the pool water quality, water treatment systems, and LLLW volume.

Cook, D.H.; Chang, S.J.; Dabs, R.D.; Freels, J.D.; Morgan, K.A.; Rothrock, R.B. [Oak Ridge National Lab., TN (United States); Griess, J.C. [Griess (J.C.), Knoxville, TN (United States)

1994-12-31T23:59:59.000Z

37

HFIR spent fuel management alternatives  

SciTech Connect (OSTI)

The High Flux Isotope Reactor (HFIR) at Martin Marietta Energy Systems' Oak Ridge National Laboratory (ORNL) has been unable to ship its spent fuel to Savannah River Site (SRS) for reprocessing since 1985. The HFIR storage pools are expected to fill up in the February 1994 to February 1995 time frame. If a management altemative to existing HFIR pool storage is not identified and implemented before the HFIR pools are full, the HFIR will be forced to shut down. This study investigated several alternatives for managing the HFIR spent fuel, attempting to identify options that could be implemented before the HFIR pools are full. The options investigated were: installing a dedicated dry cask storage facility at ORNL, increasing HFIR pool storage capacity by clearing the HFIR pools of debris and either close-packing or stacking the spent fuel elements, storing the spent fuel at another ORNL pool, storing the spent fuel in one or more hot cells at ORNL, and shipping the spent fuel offsite for reprocessing or storage elsewhere.

Begovich, J.M.; Green, V.M.; Shappert, L.B.; Lotts, A.L.

1992-10-15T23:59:59.000Z

38

HFIR spent fuel management alternatives  

SciTech Connect (OSTI)

The High Flux Isotope Reactor (HFIR) at Martin Marietta Energy Systems` Oak Ridge National Laboratory (ORNL) has been unable to ship its spent fuel to Savannah River Site (SRS) for reprocessing since 1985. The HFIR storage pools are expected to fill up in the February 1994 to February 1995 time frame. If a management altemative to existing HFIR pool storage is not identified and implemented before the HFIR pools are full, the HFIR will be forced to shut down. This study investigated several alternatives for managing the HFIR spent fuel, attempting to identify options that could be implemented before the HFIR pools are full. The options investigated were: installing a dedicated dry cask storage facility at ORNL, increasing HFIR pool storage capacity by clearing the HFIR pools of debris and either close-packing or stacking the spent fuel elements, storing the spent fuel at another ORNL pool, storing the spent fuel in one or more hot cells at ORNL, and shipping the spent fuel offsite for reprocessing or storage elsewhere.

Begovich, J.M.; Green, V.M.; Shappert, L.B.; Lotts, A.L.

1992-10-15T23:59:59.000Z

39

Criticality safety assessment of a TRIGA reactor spent-fuel pool under accident conditions  

SciTech Connect (OSTI)

Additional criticality safety analysis of a pool-type storage for TRIGA spent fuel at the Jozef Stefan Institute in Ljubljana, Slovenia, is presented. Previous results have shown that subcriticality is not guaranteed for some postulated accidents (earthquake with subsequent fuel rack disintegration resulting in contact fuel pitch) under the assumption that the fuel rack is loaded with fresh 12 wt% standard fuel. To mitigate this deficiency, a study was done on replacing a certain number of fuel elements in the rack with cadmium-loaded absorber rods. The Monte Carlo computer code MCNP4A with an ENDF/B-V library and detailed three-dimensional geometrical model of the spent-fuel rack was used for this purpose. First, a minimum critical number of fuel elements was determined for contact pitch, and two possible geometries of rack disintegration were considered. Next, it was shown that subcriticality can be ensured when pitch is decreased from a rack design pitch of 8 cm to contact, if a certain number of fuel elements (8 to 20 out of 70) are replaced by absorber rods, which are uniformly mixed into the lattice. To account for the possibility that random mixing of fuel elements and absorber rods can occur during rack disintegration and result in a supercritical configuration, a probabilistic study was made to sample the probability density functions for random absorber rod lattice loadings. Results of the calculations show that reasonably low probabilities for supercriticality can be achieved (down to 10{sup {minus}6} per severe earthquake, which would result in rack disintegration and subsequent maximum possible pitch decrease) even in the case where fresh 12 wt% standard TRIGA fuel would be stored in the spent-fuel pool.

Glumac, B; Ravnik, M. [Jozef Stefan Inst., Ljubljana (Slovenia); Logar, M. [Univ. of Maribor (Slovenia). Faculty of Electrical Engineering and Computer Sciences

1997-02-01T23:59:59.000Z

40

Separation and Recovery of Uranium Metal from Spent Light Water Reactor Fuel via Electrolytic Reduction and Electrorefining  

SciTech Connect (OSTI)

A series of bench-scale experiments was performed in a hot cell at Idaho National Laboratory to demonstrate the separation and recovery of uranium metal from spent light water reactor (LWR) oxide fuel. The experiments involved crushing spent LWR fuel to particulate and separating it from its cladding. Oxide fuel particulate was then converted to metal in a series of six electrolytic reduction runs that were performed in succession with a single salt loading of molten LiCl – 1 wt% Li2O at 650 °C. Analysis of salt samples following the series of electrolytic reduction runs identified the diffusion of select fission products from the spent fuel to the molten salt electrolyte. The extents of metal oxide conversion in the post-test fuel were also quantified, including a nominal 99.7% conversion of uranium oxide to metal. Uranium metal was then separated from the reduced LWR fuel in a series of six electrorefining runs that were performed in succession with a single salt loading of molten LiCl-KCl-UCl3 at 500 °C. Analysis of salt samples following the series of electrorefining runs identified additional partitioning of fission products into the molten salt electrolyte. Analyses of the separated uranium metal were performed, and its decontamination factors were determined.

S. D. Herrmann; S. X. Li

2010-09-01T23:59:59.000Z

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


41

Development of a Safeguards Verification Method and Instrument to Detect Pin Diversion from Pressurized Water Reactor (PWR) Spent Fuel Assemblies  

SciTech Connect (OSTI)

A technical safeguards challenge has remained for decades for the IAEA to identify possible diversion of nuclear fuel pins from Light Water Reactor (LWR) spent fuel assemblies. In fact, as modern nuclear power plants are pushed to higher power levels and longer fuel cycles, fuel failures (i.e., ''leakers'') as well as the corresponding fuel assembly repairs (i.e., ''reconstitutions'') are commonplace occurrences within the industry. Fuel vendors have performed hundreds of reconstitutions in the past two decades, thus, an evolved know-how and sophisticated tools exist to disassemble irradiated fuel assemblies and replace damaged pins with dummy stainless steel or other type rods. Various attempts have been made in the past two decades to develop a technology to identify a possible diversion of pin(s) and to determine whether some pins are missing or replaced with dummy or fresh fuel pins. However, to date, there are no safeguards instruments that can detect a possible pin diversion scenario to the requirements of the IAEA. The FORK detector system [1-2] can characterize spent fuel assemblies using operator declared data, but it is not sensitive enough to detect missing pins from spent fuel assemblies. Likewise, an emission computed tomography system [3] has been used to try to detect missing pins from a spent fuel assembly, which has shown some potential for identifying possible missing pins but this capability has not yet been fully demonstrated. The use of such a device in the future would not be envisaged, especially in an inexpensive, easy to handle setting for field applications. In this article, we describe a concept and ongoing research to help develop a new safeguards instrument for the detection of pin diversions in a PWR spent fuel assembly. The proposed instrument is based on one or more very thin radiation detectors that could be inserted within the guide tubes of a Pressurized Water Reactor (PWR) assembly. Ultimately, this work could lead to the development of a detector cluster and corresponding high-precision driving system to collect radiation signatures inside PWR spent fuel assemblies. The data obtained would provide the spatial distribution of the neutron and gamma flux fields within the spent fuel assembly, while the data analysis would be used to help identify missing or replaced pins. Monte Carlo simulations have been performed to help validate this concept using a realistic 17 x 17 PWR spent fuel assembly [4-5]. The initial results of this study show that neutron profile in the guide tubes, when obtained in the presence of missing pins, can be identifiably different from the profiles obtained without missing pins, Our latest simulations have focused upon a specific type of fission chamber that could be tested for this application.

Ham, Y S; Maldonado, G I; Burdo, J; He, T

2006-10-10T23:59:59.000Z

42

Utilization of TRISO Fuel with LWR Spent Fuel in Fusion-Fission Hybrid Reactor System  

Science Journals Connector (OSTI)

HTRs use a high performance particulate TRISO fuel with ceramic multi-layer coatings due to the high burn up capability and very neutronic performance. TRISO fuel because of capable of high burn up and very neutr...

Adem Ac?r; Taner Altunok

2010-10-01T23:59:59.000Z

43

Assessment of uranium-free nitride fuels for spent fuel transmutation in fast reactor systems  

E-Print Network [OSTI]

. ....................................................................................... 18 Fig. 4. Standard PWR ¼ core model with fresh, once- and twice-burned fuel, and the location of MOX fuel assemblies with respect to original layout, 32% MOX loading................................................................................................................ 21 Fig. 5. Control rod locations......................................................................................... 21 Fig. 6. Net change of U, Pu and Am for PWR and 1/3 MOX fueled whole cores, 360 day burn...

Szakaly, Frank Joseph

2004-09-30T23:59:59.000Z

44

EIS-0015: U.S. Spent Fuel Policy  

Broader source: Energy.gov [DOE]

Subsumed DOE/EIS-0040 and DOE/EIS-0041. The Savannah River Laboratory prepared this EIS to analyze the impacts of implementing or not implementing the policy for interim storage of spent power reactor fuel. This Final EIS is a compilation of three Draft EISs and one Supplemental Draft EIS: DOE/EIS-0015-D, Storage of U.S. Spent Power Reactor Fuel; DOE/EIS-0015-DS, Storage of U.S. Spent Power Reactor Fuel - Supplement; DOE/EIS-0040-D, Storage of Foreign Spent Power Reactor Fuel; and DOE/EIS-0041-D, Charge for Spent Fuel Storage.

45

Spent fuel storage requirements 1993--2040  

SciTech Connect (OSTI)

Historical inventories of spent fuel are combined with U.S. Department of Energy (DOE) projections of future discharges from commercial nuclear reactors in the United States to provide estimates of spent fuel storage requirements through the year 2040. The needs are estimated for storage capacity beyond that presently available in the reactor storage pools. These estimates incorporate the maximum capacities within current and planned in-pool storage facilities and any planned transshipments of spent fuel to other reactors or facilities. Existing and future dry storage facilities are also discussed. The nuclear utilities provide historical data through December 1992 on the end of reactor life are based on the DOE/Energy Information Administration (EIA) estimates of future nuclear capacity, generation, and spent fuel discharges.

Not Available

1994-09-01T23:59:59.000Z

46

Nuclear Spent Fuel Program Drivers  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

was created to plan and coordinate the management of Department of Energy-owned spent nuclear fuel. It was established as a result of a 1992 decision to stop spent nuclear fuel...

47

Low-temperature rupture behavior of Zircaloy-clad pressurized water reactor spent fuel rods under dry storage conditions  

SciTech Connect (OSTI)

Creep rupture studies on five well-characterized Zircaloy-clad pressurized water reactor spent fuel rods, which were pressurized to a hoop stress of about145 MPa, were conducted for up to 2101 h at 323/sup 0/C. The conditions were chosen for limited annealing of in-reactor irradiation hardening. No cladding breaches occurred, although significant hydride agglomeration and reorientation took place in rods that cooled under stress. Observations are interpreted in terms of a conservatively modified Larson-Miller curve to provide a lower bound on permissible maximum dry-storage temperatures, assuming creep rupture as the life-limiting mechanism. If hydride reorientation can be ruled out during dry storage, 305/sup 0/C is a conservative lower bound, based on the creep-rupture mechanism, for the maximum storage temperature of rods with irradiation-hardened cladding to ensure a 100-yr cladding lifetime in an inert atmosphere. An oxidizing atmosphere reduced the lower bound on the maximum permissible storage temperature by about5/sup 0/C. While this lower bound is based on whole-rod data, other types of data on spent fuel behavior in dry storage might support a higher limit. This isothermal temperature limit does not take credit for the decreasing rod temperature during dry storage. High-temperature tests based on creep rupture as the limiting mechanism indicate that storage at temperatures between 400 and 440/sup 0/C may be feasible for rods that are annealed.

Einsiger, R.E.; Kohli, R.

1984-10-01T23:59:59.000Z

48

Spent Fuel Background Report Volume I  

SciTech Connect (OSTI)

This report is an overview of current spent nuclear fuel management in the DOE complex. Sources of information include published literature, internal DOE documents, interviews with site personnel, and information provided by individual sites. Much of the specific information on facilities and fuels was provided by the DOE sites in response to the questionnaire for data for spent fuels and facilities data bases. This information is as accurate as is currently available, but is subject to revision pending results of further data calls. Spent fuel is broadly classified into three categories: (a) production fuels, (b) special fuels, and (c) naval fuels. Production fuels, comprising about 80% of the total inventory, are those used at Hanford and Savannah River to produce nuclear materials for defense. Special fuels are those used in a wide variety of research, development, and testing activities. Special fuels include fuel from DOE and commercial reactors used in research activities at DOE sites. Naval fuels are those developed and used for nuclear-powered naval vessels and for related research and development. Given the recent DOE decision to curtail reprocessing, the topic of main concern in the management of spent fuel is its storage. Of the DOE sites that have spent nuclear fuel, the vast majority is located at three sites-Hanford, INEL, and Savannah River. Other sites with spent fuel include Oak Ridge, West Valley, Brookhaven, Argonne, Los Alamos, and Sandia. B&W NESI Lynchburg Technology Center and General Atomics are commercial facilities with DOE fuel. DOE may also receive fuel from foreign research reactors, university reactors, and other commercial and government research reactors. Most DOE spent fuel is stored in water-filled pools at the reactor facilities. Currently an engineering study is being performed to determine the feasibility of using dry storage for DOE-owned spent fuel currently stored at various facilities. Delays in opening the deep geologic repository and the decision to phase out reprocessing of production fuels are extending the need for interim storage. The report describes the basic storage conditions and the general SNF inventory at individual DOE facilities.

Abbott, D.

1994-03-01T23:59:59.000Z

49

EIS-0203: Spent Nuclear Fuel Management and Idaho National Engineering  

Broader source: Energy.gov (indexed) [DOE]

EIS-0203: Spent Nuclear Fuel Management and Idaho National EIS-0203: Spent Nuclear Fuel Management and Idaho National Engineering Laboratory Environmental Restoration and Waste Management Programs EIS-0203: Spent Nuclear Fuel Management and Idaho National Engineering Laboratory Environmental Restoration and Waste Management Programs SUMMARY This EIS considers programmatic (DOE-wide) alternative approaches to safely, efficiently, and responsibly manage existing and projected quantities of spent nuclear fuel until the year 2035. This amount of time may be required to make and implement a decision on the ultimate disposition of spent nuclear fuel. DOE's spent nuclear fuel responsibilities include fuel generated by DOE production, research, and development reactors; naval reactors; university and foreign research reactors; domestic non-DOE reactors such as those at the National Institute

50

Spent Nuclear Fuel Fact Sheets  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

management needs. By coordinating common needs for research, technology development, and testing programs, the National Spent Nuclear Fuel Program is achieving cost efficiencies...

51

EQ6 Calculations for Chemical Degradation Of N Reactor (U-Metal) Spent Nuclear Fuel Waste Packages  

SciTech Connect (OSTI)

The Monitored Geologic Repository (MGR) Waste Package Department of the Civilian Radioactive Waste Management System Management & Operating Contractor (CRWMS M&O) performed calculations to provide input for disposal of spent nuclear fuel (SNF) from the N Reactor, a graphite moderated reactor at the Department of Energy's (DOE) Hanford Site (ref. 1). The N Reactor core was fueled with slightly enriched (0.947 wt% and 0.947 to 1.25 wt% {sup 235}U in Mark IV and Mark IA fuels, respectively) U-metal clad in Zircaloy-2 (Ref. 1, Sec. 3). Both types of N Reactor SNF have been considered for disposal at the proposed Yucca Mountain site. For some WPs, the outer shell and inner shell may breach (Ref. 3) allowing the influx of water. Water in the WP will moderate neutrons, increasing the likelihood of a criticality event within the WP; and the water may, in time, gradually leach the fissile components from the WP, further affecting the neutronics of the system. This study presents calculations of the long-term geochemical behavior of WPs containing two multi-canister overpacks (MCO) with either six baskets of Mark IA or five baskets of Mark IV intact N Reactor SNF rods (Ref. 1, Sec. 4) and two high-level waste (HLW) glass pour canisters (GPCs) arranged according to the codisposal concept (Ref. 4). The specific study objectives were to determine: (1) The extent to which fissile uranium will remain in the WP after corrosion/dissolution of the initial WP configuration (2) The extent to which fissile uranium will be carried out of the degraded WP by infiltrating water (such that internal criticality is no longer possible, but the possibility of external criticality may be enhanced); and (3) The nominal chemical composition for the criticality evaluations of the WP design, and to suggest the range of parametric variations for additional evaluations. The scope of this calculation, the chemical compositions (and subsequent criticality evaluations) of the simulations, is limited to time periods up to 6.35 x 10{sup 5} years. This longer time frame is closer to the one million year time horizon recently recommended by the National Academy of Sciences to the Environmental Protection Agency for performance assessment related to a nuclear repository (Ref. 5). However, it is important to note that after 100,000 years, most of the materials of interest (fissile materials) will have either been removed from the WP, reached a steady state, or been transmuted.

P. Bernot

2001-02-27T23:59:59.000Z

52

Low-temperature rupture behavior of Zircaloy clad pressurized water reactor spent fuel rods under dry storage conditions  

SciTech Connect (OSTI)

Creep rupture studies on five well-characterized Zircaloy clad pressurized water reactor spent fuel rods, which were pressurized to a hoop stress of approximately 145 MPa, were conducted for up to 2101 h at 323/sup 0/C. The conditions were chosen for limited annealing of in-reactor irradiation-hardening. No cladding breaches occurred, although significant hydride agglomeration and reorientation took place in rods that cooled under stress. Observations are interpreted in terms of a conservatively modified Larson-Miller curve to provide a lower bound on permissible maximum dry-storage temperatures, assuming creep rupture as the life-limiting mechanism. If hydride reorientation can be ruled out during dry storage, 305/sup 0/C is a conservative lower bound, based on the creep rupture mechanism, for the maximum storage temperature of rods with irradiation hardened cladding to ensure a 100-year cladding lifetime in an inert atmosphere. An oxidizing atmosphere reduces the lower bound on the maximum permissible storage temperature by approx. 5/sup 0/C. While high-temperature tests based on creep rupture as the limiting mechanism indicate that storage at temperatures between 400/sup 0/C and 440/sup 0/C may be feasible for rods which are annealed, tests to study rod performance in the 305/sup 0/ to 400/sup 0/C temperature range have not been conducted. 37 references, 10 figures, 7 tables.

Einziger, R.E.; Kohli, R.

1983-01-01T23:59:59.000Z

53

EA-0912: Urgent-Relief Acceptance of Foreign Research Reactor Spent Nuclear  

Broader source: Energy.gov (indexed) [DOE]

2: Urgent-Relief Acceptance of Foreign Research Reactor Spent 2: Urgent-Relief Acceptance of Foreign Research Reactor Spent Nuclear Fuel EA-0912: Urgent-Relief Acceptance of Foreign Research Reactor Spent Nuclear Fuel SUMMARY This EA evaluates the environmental impacts of a proposal to accept 409 spent fuel elements from eight foreign research reactors in seven European countries. The spent fuel would be shipped across the ocean in spent fuel transportation casks from the country of origin to one or more United States eastern seaboard ports. PUBLIC COMMENT OPPORTUNITIES None available at this time. DOCUMENTS AVAILABLE FOR DOWNLOAD April 22, 1994 EA-0912: Finding of No Significant Impact Urgent-Relief Acceptance of Foreign Research Reactor Spent Nuclear Fuel April 22, 1994 EA-0912: Final Environmental Assessment Urgent-Relief Acceptance of Foreign Research Reactor Spent Nuclear Fuel

54

Radio-toxicity of spent fuel of the advanced heavy water reactor  

Science Journals Connector (OSTI)

......plutonium-thorium-uranium fuel with a...of which the inventory and rate of...types (low-enriched MOX fuel for AHWR and natural uranium fuel for PHWR...input and a highly flexible and...Radioactivity The total inventory of an average-rated......

S. Anand; K. D. S. Singh; V. K. Sharma

2010-01-01T23:59:59.000Z

55

Spent fuel storage system for LMFBR fuel experiments  

SciTech Connect (OSTI)

Fuel that had been irradiated in the Argonne National Laboratory Experimental Breeder Reactor II (EBR-II) at Idaho Falls, Idaho, and examined at the Hanford Engineering Development Laboratory at Richland, Washington, was placed in long term retrievable storage utilizing a system designed at Hanford. The Spent Fuel Storage Cask system was designed for transport and storage of a large quantity of spent fuel at the Hanford 200 Area transuranic (TRU) asphalt storage pad. The entire system is designed for long term retrievable storage to allow future reprocessing of the fuel. The system was designed to meet the criticality, shielding, and thermal requirements for a maximum fuel load of four kilograms fissile. The Spent Fuel Storage Cask was built to transport and store the fuel from EBR-II on the TRU asphalt storage pad.

Seay, J.M.; Gruber, W.J.

1983-01-01T23:59:59.000Z

56

Simulated Performance of the Integrated PNAR and SINRD Detector Designed for Spent Fuel Measurements at the Fugen Reactor in Japan  

SciTech Connect (OSTI)

Objective is to investigate the use of Passive Neutron Albedo Reactivity (PNAR) and Self-Interrogation Neutron Resonance Densitometry (SINRD) to quantify fissile content in FUGEN spent fuel assemblies (FAs). Methodology used is: (1) Detector was designed using fission chambers (FCs); (2) Optimized design via MCNPX simulations; and (3) Plan to build and field test instrument in FY13. Significance was to improve safeguards verification of spent fuel assemblies in water and increase sensitivity to partial defects. MCNPX simulations were performed to optimize the design of the SINRD+PNAR detector. PNAR ratio was less sensitive to FA positioning than SINRD and SINRD ratio was more sensitive to Pu fissile mass than PNAR. Significance was that the integration of these techniques can be used to improve verification of spent fuel assemblies in water.

Lafleur, Adrienne M. [Los Alamos National Laboratory; Ulrich, Timothy J. II [Los Alamos National Laboratory; Menlove, Howard O. [Los Alamos National Laboratory; Swinhoe, Martyn T. [Los Alamos National Laboratory; Tobin, Stephen J. [Los Alamos National Laboratory; Seya, Michio [Japan Atomic Energy Agency; Bolind, Alan M. [Japan Atomic Energy Agency

2012-07-13T23:59:59.000Z

57

Spent nuclear fuel reprocessing modeling  

SciTech Connect (OSTI)

The long-term wide development of nuclear power requires new approaches towards the realization of nuclear fuel cycle, namely, closed nuclear fuel cycle (CNFC) with respect to fission materials. Plant nuclear fuel cycle (PNFC), which is in fact the reprocessing of spent nuclear fuel unloaded from the reactor and the production of new nuclear fuel (NF) at the same place together with reactor plant, can be one variant of CNFC. Developing and projecting of PNFC is a complicated high-technology innovative process that requires modern information support. One of the components of this information support is developed by the authors. This component is the programme conducting calculations for various variants of process flow sheets for reprocessing SNF and production of NF. Central in this programme is the blocks library, where the blocks contain mathematical description of separate processes and operations. The calculating programme itself has such a structure that one can configure the complex of blocks and correlations between blocks, appropriate for any given flow sheet. For the ready sequence of operations balance calculations are made of all flows, i.e. expenses, element and substance makeup, heat emission and radiation rate are determined. The programme is open and the block library can be updated. This means that more complicated and detailed models of technological processes will be added to the library basing on the results of testing processes using real equipment, in test operating mode. The development of the model for the realization of technical-economic analysis of various variants of technologic PNFC schemes and the organization of 'operator's advisor' is expected. (authors)

Tretyakova, S.; Shmidt, O.; Podymova, T.; Shadrin, A.; Tkachenko, V. [Bochvar Institute, 5 Rogova str., Moscow 123098 (Russian Federation); Makeyeva, I.; Tkachenko, V.; Verbitskaya, O.; Schultz, O.; Peshkichev, I. [Russian Federal Nuclear Center - VNIITF E.I. Zababakhin, p.o.box 245, Snezhinsk, 456770 (Russian Federation)

2013-07-01T23:59:59.000Z

58

US Spent (Used) Fuel Status, Management and Likely Directions- 12522  

SciTech Connect (OSTI)

As of 2010, the US has accumulated 65,200 MTU (42,300 MTU of PWR's; 23,000 MTU of BWR's) of spent (irradiated or used) fuel from 104 operating commercial nuclear power plants situated at 65 sites in 31 States and from previously shutdown commercial nuclear power plants. Further, the Department of Energy (DOE) has responsibility for an additional 2458 MTU of DOE-owned defense and non defense spent fuel from naval nuclear power reactors, various non-commercial test reactors and reactor demonstrations. The US has no centralized large spent fuel storage facility for either commercial spent fuel or DOE-owned spent fuel. The 65,200 MTU of US spent fuel is being safely stored by US utilities at numerous reactor sites in (wet) pools or (dry) metal or concrete casks. As of November 2010, the US had 63 'independent spent fuel storage installations' (or ISFSI's) licensed by the US Nuclear Regulatory Commission located at 57 sites in 33 states. Over 1400 casks loaded with spent fuel for dry storage are at these licensed ISFSI's; 47 sites are located at commercial reactor sites and 10 are located 'away' from a reactor (AFR's) site. DOE's small fraction of a 2458 MTU spent fuel inventory, which is not commercial spent fuel, is with the exception of 2 MTU, being stored at 4 sites in 4 States. The decades old US policy of a 'once through' fuel cycle with no recycle of spent fuel was set into a state of 'mass confusion or disruption' when the new US President Obama's administration started in early 2010 stopping the only US geologic disposal repository at the Yucca Mountain site in the State of Nevada from being developed and licensed. The practical result is that US nuclear power plant operators will have to continue to be responsible for managing and storing their own spent fuel for an indefinite period of time at many different sites in order to continue to generate electricity because there is no current US government plan, schedule or policy for taking possession of accumulated spent fuel from the utilities. There are technical solutions for continuing the safe storage of spent fuel for 100 years or more and these solutions will be implemented by the US utilities that need to keep their nuclear power plants operating while the unknown political events are played out to establish future US policy decisions that can remain in place long enough regarding accumulated spent fuel inventories to implement any new US spent fuel centralized storage or disposition policy by the US government. (author)

Jardine, Leslie J. [L. J. Jardine Services, Consultant, Dublin CA, 94568 (United States)

2012-07-01T23:59:59.000Z

59

Worker exposure for at-reactor management of spent nuclear fuel  

Science Journals Connector (OSTI)

......Impact Statement for the proposed Yucca Mountain repository(6,7); potential...a No Action Alternative in the Yucca Mountain Environmental Impact Statement...operations at reactor sites. FUNDING This research was funded by the......

Philippe F. Weck

2013-09-01T23:59:59.000Z

60

Spent Fuel Working Group report on inventory and storage of the Department`s spent nuclear fuel and other reactor irradiated nuclear materials and their environmental, safety and health vulnerabilities. Volume 3, Site team reports  

SciTech Connect (OSTI)

A self assessment was conducted of those Hanford facilities that are utilized to store Reactor Irradiated Nuclear Material, (RINM). The objective of the assessment is to identify the Hanford inventories of RINM and the ES & H concerns associated with such storage. The assessment was performed as proscribed by the Project Plan issued by the DOE Spent Fuel Working Group. The Project Plan is the plan of execution intended to complete the Secretary`s request for information relevant to the inventories and vulnerabilities of DOE storage of spent nuclear fuel. The Hanford RINM inventory, the facilities involved and the nature of the fuel stored are summarized. This table succinctly reveals the variety of the Hanford facilities involved, the variety of the types of RINM involved, and the wide range of the quantities of material involved in Hanford`s RINM storage circumstances. ES & H concerns are defined as those circumstances that have the potential, now or in the future, to lead to a criticality event, to a worker radiation exposure event, to an environmental release event, or to public announcements of such circumstances and the sensationalized reporting of the inherent risks.

Not Available

1993-11-01T23:59:59.000Z

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


61

Spent-fuel-storage alternatives  

SciTech Connect (OSTI)

The Spent Fuel Storage Alternatives meeting was a technical forum in which 37 experts from 12 states discussed storage alternatives that are available or are under development. The subject matter was divided into the following five areas: techniques for increasing fuel storage density; dry storage of spent fuel; fuel characterization and conditioning; fuel storage operating experience; and storage and transport economics. Nineteen of the 21 papers which were presented at this meeting are included in this Proceedings. These have been abstracted and indexed. (ATT)

Not Available

1980-01-01T23:59:59.000Z

62

Spent Nuclear Fuel Alternative Technology Decision Analysis  

SciTech Connect (OSTI)

The Westinghouse Savannah River Company (WSRC) made a FY98 commitment to the Department of Energy (DOE) to recommend a technology for the disposal of aluminum-based spent nuclear fuel (SNF) at the Savannah River Site (SRS). The two technologies being considered, direct co-disposal and melt and dilute, had been previously selected from a group of eleven potential SNF management technologies by the Research Reactor Spent Nuclear Fuel Task Team chartered by the DOE''s Office of Spent Fuel Management. To meet this commitment, WSRC organized the SNF Alternative Technology Program to further develop the direct co-disposal and melt and dilute technologies and ultimately provide a WSRC recommendation to DOE on a preferred SNF alternative management technology.

Shedrow, C.B.

1999-11-29T23:59:59.000Z

63

Pyrochemical Treatment of Spent Nuclear Fuel  

SciTech Connect (OSTI)

Over the last 10 years, pyrochemical treatment of spent nuclear fuel has progressed from demonstration activities to engineering-scale production operations. As part of the Advanced Fuel Cycle Initiative within the U.S. Department of Energy’s Office of Nuclear Energy, Science and Technology, pyrochemical treatment operations are being performed as part of the treatment of fuel from the Experimental Breeder Reactor II at the Idaho National Laboratory. Integral to these treatment operations are research and development activities that are focused on scaling further the technology, developing and implementing process improvements, qualifying the resulting high-level waste forms, and demonstrating the overall pyrochemical fuel cycle.

K. M. Goff; K. L. Howden; G. M. Teske; T. A. Johnson

2005-10-01T23:59:59.000Z

64

Breeder Spent Fuel Handling Program multipurpose cask design basis document  

SciTech Connect (OSTI)

The Breeder Spent Fuel Handling (BSFH) Program multipurpose cask Design Basis Document defines the performance requirements essential to the development of a legal weight truck cask to transport FFTF spent fuel from reactor to a reprocessing facility and the resultant High Level Waste (HLW) to a repository. 1 ref.

Duckett, A.J.; Sorenson, K.B.

1985-09-01T23:59:59.000Z

65

An experiment to simulate the heat transfer properties of a dry, horizontal spent nuclear fuel assembly  

E-Print Network [OSTI]

Nuclear power reactors generate highly radioactive spent fuel assemblies. Initially, the spent fuel assemblies are stored for a period of several years in an on-site storage facility to allow the radioactivity levels of ...

Lovett, Phyllis Maria

1991-01-01T23:59:59.000Z

66

Activities Related to Storage of Spent Nuclear Fuel | Department...  

Office of Environmental Management (EM)

Activities Related to Storage of Spent Nuclear Fuel Activities Related to Storage of Spent Nuclear Fuel Activities Related to Storage of Spent Nuclear Fuel More Documents &...

67

Naval Spent Fuel Rail Shipment Accident Exercise Objectives ...  

Office of Environmental Management (EM)

Naval Spent Fuel Rail Shipment Accident Exercise Objectives Naval Spent Fuel Rail Shipment Accident Exercise Objectives Naval Spent Fuel Rail Shipment Accident Exercise Objectives...

68

A case study on the influence of THM coupling on the near field safety of a spent fuel repository in sparsely fractured granite  

E-Print Network [OSTI]

geological disposal of spent CANDU fuel in Canada, a safetyhypothetical repository for spent CANDU fuel in the Canadianbuffer. The waste form: CANDU reactors in Canada are fuelled

Nguyen, T.S.

2009-01-01T23:59:59.000Z

69

Characterization plan for Hanford spent nuclear fuel  

SciTech Connect (OSTI)

Reprocessing of spent nuclear fuel (SNF) at the Hanford Site Plutonium-Uranium Extraction Plant (PUREX) was terminated in 1972. Since that time a significant quantity of N Reactor and Single-Pass Reactor SNF has been stored in the 100 Area K-East (KE) and K-West (KW) reactor basins. Approximately 80% of all US Department of Energy (DOE)-owned SNF resides at Hanford, the largest portion of which is in the water-filled KE and KW reactor basins. The basins were not designed for long-term storage of the SNF and it has become a priority to move the SNF to a more suitable location. As part of the project plan, SNF inventories will be chemically and physically characterized to provide information that will be used to resolve safety and technical issues for development of an environmentally benign and efficient extended interim storage and final disposition strategy for this defense production-reactor SNF.

Abrefah, J.; Thornton, T.A.; Thomas, L.E.; Berting, F.M.; Marschman, S.C.

1994-12-01T23:59:59.000Z

70

Spent Fuel Transportation Risk Assessment  

Broader source: Energy.gov (indexed) [DOE]

Fuel Transportation Risk Assessment Fuel Transportation Risk Assessment (SFTRA) Draft NUREG-2125 Overview for National Transportation Stakeholders Forum John Cook Division of Spent Fuel Storage and Transportation 1 SFTRA Overview Contents * Project and review teams * Purpose and goals * Basic methodology * Improvements relative to previous studies * Draft NUREG structure and format * Routine shipment analysis and results * Accident condition analysis and results * Findings and conclusions * Schedule 2 SFTRA Research and Review Teams * Sandia National Laboratory Research Team [$1.8M; 9/06-9/12] - Doug Ammerman - principal investigator - Carlos Lopez - thermal - Ruth Weiner - RADTRAN * NRC's SFTRA Technical Review Team - Gordon Bjorkman - structural

71

Comparative analysis of LWR and FBR spent fuels for nuclear forensics evaluation  

SciTech Connect (OSTI)

Some interesting issues are attributed to nuclide compositions of spent fuels from thermal reactors as well as fast reactors such as a potential to reuse as recycled fuel, and a possible capability to be manage as a fuel for destructive devices. In addition, analysis on nuclear forensics which is related to spent fuel compositions becomes one of the interesting topics to evaluate the origin and the composition of spent fuels from the spent fuel foot-prints. Spent fuel compositions of different fuel types give some typical spent fuel foot prints and can be estimated the origin of source of those spent fuel compositions. Some technics or methods have been developing based on some science and technological capability including experimental and modeling or theoretical aspects of analyses. Some foot-print of nuclear forensics will identify the typical information of spent fuel compositions such as enrichment information, burnup or irradiation time, reactor types as well as the cooling time which is related to the age of spent fuels. This paper intends to evaluate the typical spent fuel compositions of light water (LWR) and fast breeder reactors (FBR) from the view point of some foot prints of nuclear forensics. An established depletion code of ORIGEN is adopted to analyze LWR spent fuel (SF) for several burnup constants and decay times. For analyzing some spent fuel compositions of FBR, some coupling codes such as SLAROM code, JOINT and CITATION codes including JFS-3-J-3.2R as nuclear data library have been adopted. Enriched U-235 fuel composition of oxide type is used for fresh fuel of LWR and a mixed oxide fuel (MOX) for FBR fresh fuel. Those MOX fuels of FBR come from the spent fuels of LWR. Some typical spent fuels from both LWR and FBR will be compared to distinguish some typical foot-prints of SF based on nuclear forensic analysis.

Permana, Sidik; Suzuki, Mitsutoshi; Su'ud, Zaki [Department of Science and Technology for Nuclear Material Management (STNM), Japan Atomic Energy Agency (JAEA), 2-4 Shirane, Shirakata, Tokai Mura, Naka-gun, Ibaraki 319-1195 Nuclear Physics and Bio (Indonesia); Department of Science and Technology for Nuclear Material Management (STNM), Japan Atomic Energy Agency (JAEA), 2-4 Shirane, Shirakata, Tokai Mura, Naka-gun, Ibaraki 319-1195 (Japan); Nuclear Physics and Bio Physics Research Group, Department of Physics, Bandung Institute of Technology, Gedung Fisika, Jl. Ganesha 10, Bandung 40132 (Indonesia)

2012-06-06T23:59:59.000Z

72

E-Print Network 3.0 - advanced spent fuel Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

facilities should have more advanced technical monitoring... of the cycle to extract fis- sile material from the spent fuel removed from reactors. Although a complete... of...

73

Long-term management of high-level radioactive waste (HLW) and spent nuclear fuel (SNF)  

Broader source: Energy.gov [DOE]

GC-52 provides legal advice to DOE regarding the long-term management of high-level radioactive waste (HLW) and spent nuclear fuel (SNF). SNF is nuclear fuel that has been used as fuel in a reactor...

74

Spent Fuel Disposal Trust Fund (Maine)  

Broader source: Energy.gov [DOE]

Any licensee operating a nuclear power plant in this State shall establish a segregated Spent Nuclear Fuel Disposal Trust Fund in accordance with this subchapter for the eventual disposal of spent...

75

Recovery of weapon plutonium as feed material for reactor fuel  

SciTech Connect (OSTI)

This report presents preliminary considerations for recovering and converting weapon plutonium from various US weapon forms into feed material for fabrication of reactor fuel elements. An ongoing DOE study addresses the disposition of excess weapon plutonium through its use as fuel for nuclear power reactors and subsequent disposal as spent fuel. The spent fuel would have characteristics similar to those of commercial power spent fuel and could be similarly disposed of in a geologic repository.

Armantrout, G.A.; Bronson, M.A.; Choi, Jor-Shan [and others

1994-03-16T23:59:59.000Z

76

Radiological consequences of ship collisions that might occur in U.S. Ports during the shipment of foreign research reactor spent nuclear fuel to the United States in break-bulk freighters  

SciTech Connect (OSTI)

Accident source terms, source term probabilities, consequences, and risks are developed for ship collisions that might occur in U.S. ports during the shipment of spent fuel from foreign research reactors to the United States in break-bulk freighters.

Sprung, J.L.; Bespalko, S.J.; Massey, C.D.; Yoshimura, R. [Sandia National Laboratory, Albuquerque, NM (United States); Johnson, J.D. [GRAM Inc., Albuquerque, NM (United States); Reardon, P.C. [PCRT Technologies, Albuquerque, NM (United States); Ebert, M.W.; Gallagher D.W. [Science Applications International Corp., Reston, VA (United States)

1996-08-01T23:59:59.000Z

77

Loss of spent fuel pool cooling PRA: Model and results  

SciTech Connect (OSTI)

This letter report documents models for quantifying the likelihood of loss of spent fuel pool cooling; models for identifying post-boiling scenarios that lead to core damage; qualitative and quantitative results generated for a selected plant that account for plant design and operational practices; a comparison of these results and those generated from earlier studies; and a review of available data on spent fuel pool accidents. The results of this study show that for a representative two-unit boiling water reactor, the annual probability of spent fuel pool boiling is 5 {times} 10{sup {minus}5} and the annual probability of flooding associated with loss of spent fuel pool cooling scenarios is 1 {times} 10{sup {minus}3}. Qualitative arguments are provided to show that the likelihood of core damage due to spent fuel pool boiling accidents is low for most US commercial nuclear power plants. It is also shown that, depending on the design characteristics of a given plant, the likelihood of either: (a) core damage due to spent fuel pool-associated flooding, or (b) spent fuel damage due to pool dryout, may not be negligible.

Siu, N.; Khericha, S.; Conroy, S.; Beck, S.; Blackman, H.

1996-09-01T23:59:59.000Z

78

The united kingdom's changing requirements for spent fuel storage  

SciTech Connect (OSTI)

The UK is adopting an open fuel cycle, and is necessarily moving to a regime of long term storage of spent fuel, followed by geological disposal once a geological disposal facility (GDF) is available. The earliest GDF receipt date for legacy spent fuel is assumed to be 2075. The UK is set to embark on a programme of new nuclear build to maintain a nuclear energy contribution of 16 GW. Additionally, the UK are considering a significant expansion of nuclear energy in order to meet carbon reduction targets and it is plausible to foresee a scenario where up to 75 GW from nuclear power production could be deployed in the UK by the mid 21. century. Such an expansion, could lead to spent fuel storage and its disposal being a dominant issue for the UK Government, the utilities and the public. If the UK were to transition a closed fuel cycle, then spent fuel storage should become less onerous depending on the timescales. The UK has demonstrated a preference for wet storage of spent fuel on an interim basis. The UK has adopted an approach of centralised storage, but a 16 GW new build programme and any significant expansion of this may push the UK towards distributed spent fuel storage at a number of reactors station sites across the UK.

Hodgson, Z.; Hambley, D.I.; Gregg, R.; Ross, D.N. [National Nuclear Laboratory, Chadwick House, Birchwood Park, Warrington, Cheshire WA3 6AE (United Kingdom)

2013-07-01T23:59:59.000Z

79

Spent Nuclear Fuel (SNF) Project Execution Plan  

SciTech Connect (OSTI)

The Spent Nuclear Fuel (SNF) Project supports the Hanford Site Mission to cleanup the Site by providing safe, economic, environmentally sound management of Site spent nuclear fuel in a manner that reduces hazards by staging it to interim onsite storage and deactivates the 100 K Area facilities.

LEROY, P.G.

2000-11-03T23:59:59.000Z

80

TEPP - Spent Nuclear Fuel | Department of Energy  

Broader source: Energy.gov (indexed) [DOE]

- Spent Nuclear Fuel - Spent Nuclear Fuel TEPP - Spent Nuclear Fuel This scenario provides the planning instructions, guidance, and evaluation forms necessary to conduct an exercise involving a highway shipment of spent nuclear fuel. This exercise manual is one in a series of five scenarios developed by the Department of Energy Transportation Emergency Preparedness Program. Responding agencies may include several or more of the following: local municipal and county fire, police, sheriff, and Emergency Medical Services (EMS) personnel; state, local, and federal emergency response teams; emergency response contractors;and other emergency response resources that could potentially be provided by the carrier and the originating facility (shipper). Spent Nuclear Fuel.docx More Documents & Publications

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


81

2008 DOE Spent Nuclear Fuel and High Level Waste Inventory  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Management >> National Spent Nuclear Fuel INL Logo Search 2008 DOE Spent Nuclear Fuel and High Level Waste Inventory Content Goes Here Skip Navigation Links Home Newsroom About INL...

82

CASMO-2 spent-fuel-rack criticality analysis  

SciTech Connect (OSTI)

In recent years, utilities have needed to increase their spent-fuel storage capacity. Both Maine Yankee pressurized water reactor (PWR) and Vermont Yankee boiling water reactor (BWR) have increased their spent-fuel rack capacity by decreasing the canister center-to-center spacing while adding fixed poison. Licensing criticality analysis of such changes in spent-fuel rack design have been performed at Yankee Atomic Electric Co. (YAEC) using NITAWL-KENO-IV and the 123-group XSDRN library. However, KENO/Monte Carlo analysis has inherent drawbacks when applied to spent-fuel rack design and modification. These include statistical uncertainty and long computer time. In contrast, the transport theory code, CASMO-2, provides deterministic and fast criticality analysis. Also, since collapsed and transport-corrected cross sections are generated, PDQ can be used to analyze large array problems which are prohibitively expensive using KENO. In this work, the authors apply the CASMO-PDQ methodology to the Maine Yankee and Vermont Yankee high-density spent-fuel rack designs, and compare the final results against KENO.

Napolitano, D.G.; Heinrichs, D.P.; Gorski, J.P.

1986-01-01T23:59:59.000Z

83

SPENT FUEL MANAGEMENT AT THE SAVANNAH RIVER SITE  

SciTech Connect (OSTI)

Spent nuclear fuels are received from reactor sites around the world and are being stored in the L-Basin at the Savannah River Site (SRS) in Aiken, South Carolina. The predominant fuel types are research reactor fuel with aluminum-alloy cladding and aluminum-based fuel. Other fuel materials include stainless steel and Zircaloy cladding with uranium oxide fuel. Chemistry control and corrosion surveillance programs have been established and upgraded since the early 1990's to minimize corrosion degradation of the aluminum cladding materials, so as to maintain fuel integrity and minimize personnel exposure from radioactivity in the basin water. Recent activities have been initiated to support additional decades of wet storage which include fuel inspection and corrosion testing to evaluate the effects of specific water impurity species on corrosion attack.

Vormelker, P; Robert Sindelar, R; Richard Deible, R

2007-11-03T23:59:59.000Z

84

Safeguards for spent fuels: Verification problems  

SciTech Connect (OSTI)

The accumulation of large quantities of spent nuclear fuels world-wide is a serious problem for international safeguards. A number of International Atomic Energy Agency (IAEA) member states, including the US, consider spent fuel to be a material form for which safeguards cannot be terminated, even after permanent disposal in a geologic repository. Because safeguards requirements for spent fuels are different from those of conventional bulk-handling and item-accounting facilities, there is room for innovation to design a unique safeguards regime for spent fuels that satisfies the goals of the nuclear nonproliferation treaty at a reasonable cost to both the facility and the IAEA. Various strategies being pursued for long-term management of spent fuels are examined with a realistic example to illustrate the problems of verifying safeguards under the present regime. Verification of a safeguards regime for spent fuels requires a mix of standard safeguards approaches, such as quantitative verification and use of seals, with other measures that are unique to spent fuels. 17 refs.

Pillay, K.K.S.; Picard, R.R.

1991-01-01T23:59:59.000Z

85

Radiotoxicity and decay heat power of spent nuclear fuel of VVER type reactors at long-term storage  

Science Journals Connector (OSTI)

......a controllable storage facility for cooling...transferred for long-term storage. The storage...adequately handle waste radiation characteristics...type reactors at long-term storage. | Radiotoxicity...of radioactive waste (radwaste) determines......

B. R. Bergelson; A. S. Gerasimov; G. V. Tikhomirov

2005-12-20T23:59:59.000Z

86

Pyroprocessing oxide spent nuclear fuels for efficient disposal  

SciTech Connect (OSTI)

Pyrochemical processing as a means for conditioning spent nuclear fuels for disposal offers significant advantages over the direct disposal option. The advantages include reduction in high-level waste volume; conversion of most of the high-level waste to a low-level waste in which nearly all the transuranics (TRU) have been removed; and incorporation of the TRUs into a stable, highly radioactive waste form suitable for interim storage, ultimate destruction, or repository disposal. The lithium process has been under development at Argonne National Laboratory for use in pyrochemical conditioning of spent fuel for disposal. All of the process steps have been demonstrated in small-scale (0.5-kg simulated spent fuel) experiments. Engineering-scale (20-kg simulated spent fuel) demonstration of the process is underway, and small-scale experiments have been conducted with actual spent fuel from a light water reactor (LWR). The lithium process is simple, operates at relatively low temperatures, and can achieve high decontamination factors for the TRU elements. Ordinary materials, such as carbon steel, can be used for process containment.

McPheeters, C.C.; Pierce, R.D.; Mulcahey, T.P. [Argonne National Lab., IL (United States). Chemical Technology Div.

1994-12-31T23:59:59.000Z

87

Pyrochemical processing of DOE spent nuclear fuel  

SciTech Connect (OSTI)

A compact, efficient method for conditioning spent nuclear fuel is under development. This method, known as pyrochemical processing, or {open_quotes}pyroprocessing,{close_quotes} provides a separation of fission products from the actinide elements present in spent fuel and further separates pure uranium from the transuranic elements. The process can facilitate the timely and environmentally-sound treatment of the highly diverse collection of spent fuel currently in the inventory of the United States Department of Energy (DOE). The pyroprocess utilizes elevated-temperature processes to prepare spent fuel for fission product separation; that separation is accomplished by a molten salt electrorefining step that provides efficient (>99.9%) separation of transuranics. The resultant waste forms from the pyroprocess, are stable under envisioned repository environment conditions and highly leach-resistant. Treatment of any spent fuel type produces a set of common high-level waste forms, one a mineral and the other a metal alloy, that can be readily qualified for repository disposal and avoid the substantial costs that would be associated with the qualification of the numerous spent fuel types included in the DOE inventory.

Laidler, J.J.

1995-02-01T23:59:59.000Z

88

Methodology for determining criteria for storing spent fuel in air  

SciTech Connect (OSTI)

Dry storage in an air atmosphere is a method being considered for spent light water reactor (LWR) fuel as an alternative to storage in an inert gas environment. However, methods to predict fuel integrity based on oxidation behavior of the fuel first must be evaluated. The linear cumulative damage method has been proposed as a technique for defining storage criteria. Analysis of limited nonconstant temperature data on nonirradiated fuel samples indicates that this approach yields conservative results for a strictly decreasing-temperature history. On the other hand, the description of damage accumulation in terms of remaining life concepts provides a more general framework for making predictions of failure. Accordingly, a methodology for adapting remaining life concepts to UO/sub 2/ oxidation has been developed at Pacific Northwest Laboratory. Both the linear cumulative damage and the remaining life methods were used to predict oxidation results for spent fuel in which the temperature was decreased with time to simulate the temperature history in a dry storage cask. The numerical input to the methods was based on oxidation data generated with nonirradiated UO/sub 2/ pellets. The calculated maximum allowable storage temperatures are strongly dependent on the temperature-time profile and emphasize the conservatism inherent in the linear cumulative damage model. Additional nonconstant temperature data for spent fuel are needed to both validate the proposed methods and to predict temperatures applicable to actual spent fuel storage.

Reid, C.R.; Gilbert, E.R.

1986-11-01T23:59:59.000Z

89

Direct Investigations of the Immobilization of Radionuclides in the Alteration Products of Spent Nuclear Fuel  

SciTech Connect (OSTI)

Safe disposal of the nation's nuclear waste in a geological repository involves unique scientific and engineering challenges owing to the very long-lived radioactivity of the waste. The repository must retain a variety of radionuclides that have vastly different chemical characters for several thousand years. Most of the radioactivity that will be housed in the proposed repository at Yucca Mountain will be associated with spent nuclear fuel, much of which is derived from commercial reactors. DOE is custodian of approximately 8000 tons of spent nuclear fuel that is also intended for eventual disposal in a geological repository. Unlike the spent fuel from commercial reactors, the DOE fuel is diverse in composition with more than 250 varieties. Safe disposal of spent fuel requires a detailed knowledge of its long-term behavior under repository conditions, as well as the fate of radionuclides released from the spent fuel as waste containers are breached.

Peter C. Burns; Robert J. Finch; David J. Wronkiewicz

2004-12-27T23:59:59.000Z

90

DECONTAMINATION OF ZIRCALOY SPENT FUEL CLADDING HULLS  

SciTech Connect (OSTI)

The reprocessing of commercial spent nuclear fuel (SNF) generates a Zircaloy cladding hull waste which requires disposal as a high level waste in the geologic repository. The hulls are primarily contaminated with fission products and actinides from the fuel. During fuel irradiation, these contaminants are deposited in a thin layer of zirconium oxide (ZrO{sub 2}) which forms on the cladding surface at the elevated temperatures present in a nuclear reactor. Therefore, if the hulls are treated to remove the ZrO{sub 2} layer, a majority of the contamination will be removed and the hulls could potentially meet acceptance criteria for disposal as a low level waste (LLW). Discard of the hulls as a LLW would result in significant savings due to the high costs associated with geologic disposal. To assess the feasibility of decontaminating spent fuel cladding hulls, two treatment processes developed for dissolving fuels containing zirconium (Zr) metal or alloys were evaluated. Small-scale dissolution experiments were performed using the ZIRFLEX process which employs a boiling ammonium fluoride (NH{sub 4}F)/ammonium nitrate (NH{sub 4}NO{sub 3}) solution to dissolve Zr or Zircaloy cladding and a hydrofluoric acid (HF) process developed for complete dissolution of Zr-containing fuels. The feasibility experiments were performed using Zircaloy-4 metal coupons which were electrochemically oxidized to produce a thin ZrO{sub 2} layer on the surface. Once the oxide layer was in place, the ease of removing the layer using methods based on the two processes was evaluated. The ZIRFLEX and HF dissolution processes were both successful in removing a 0.2 mm (thick) oxide layer from Zircaloy-4 coupons. Although the ZIRFLEX process was effective in removing the oxide layer, two potential shortcomings were identified. The formation of ammonium hexafluorozirconate ((NH{sub 4}){sub 2}ZrF{sub 6}) on the metal surface prior to dissolution in the bulk solution could hinder the decontamination process by obstructing the removal of contamination. The thermal decomposition of this material is also undesirable if the cladding hulls are melted for volume reduction or to produce waste forms. Handling and disposal of the corrosive off-gas stream and ZrO{sub 2}-containing dross must be addressed. The stability of Zr{sup 4+} in the NHF{sub 4}/NH{sub 4}NO{sub 3} solution is also a concern. Precipitation of ammonium zirconium fluorides upon cooling of the dissolving solution was observed in the feasibility experiments. Precipitation of the solids was attributed to the high fluoride to Zr ratios used in the experiments. The solubility of Zr{sup 4+} in NH{sub 4}F solutions decreases as the free fluoride concentration increases. The removal of the ZrO{sub 2} layer from Zircaloy-4 coupons with HF showed a strong dependence on both the concentration and temperature. Very rapid dissolution of the oxide layer and significant amounts of metal was observed in experiments using HF concentrations {ge} 2.5 M. Treatment of the coupons using HF concentrations {le} 1.0 M was very effective in removing the oxide layer. The most effective conditions resulted in dissolution rates which were less than approximately 2 mg/cm{sup 2}-min. With dissolution rates in this range, uniform removal of the oxide layer was obtained and a minimal amount of Zircaloy metal was dissolved. Future HF dissolution studies should focus on the decontamination of actual spent fuel cladding hulls to determine if the treated hulls meet criteria for disposal as a LLW.

Rudisill, T; John Mickalonis, J

2006-09-27T23:59:59.000Z

91

National Report Joint Convention on the Safety of Spent Fuel...  

Office of Environmental Management (EM)

National Report Joint Convention on the Safety of Spent Fuel Management and on the Safety of Radioactive Waste Management National Report Joint Convention on the Safety of Spent...

92

Uraninite: A 2 Ga spent nuclear fuel from the natural fission reactor at Bangombe in Gabon, West Africa  

SciTech Connect (OSTI)

Uraninites from the Bangombe natural fission reactor (RZB) and normal uranium-ore occur as fine veins in the sandstone host-rock as well as altered, broken, and slightly displaced grains in an illitic matrix, and in nodules and veins of solid bitumen. Inclusions of galena, (Y,Gd)-rich phosphates, a Pb-oxide and a Ti-oxide? were observed. Uraninites just below RZB were partially altered to a uranyl-sulfate. Three generations of uraninite were identified based on their PbO-contents of 8--11.06 wt%, 6 wt% (the largest population), and a younger generation with 3 wt%. Diffusional loss of Pb is indicated by the presence of a Pb-oxide at the interface to the uraninites. The behavior of the metallic fission products, incompatible with the uraninite structure, may mimic the behavior of Pb in these uraninites. The averaged impurity-content ranges from 4.29 to 6.89 wt%, and consists mainly of SiO{sub 2}, TiO{sub 2}, ZrO{sub 2}, FeO, CaO, Al{sub 2}O{sub 3} and P{sub 2}O{sub 5}. The averaged content of Y{sub 2}O{sub 3} and the Ln`s is less than 0.78 wt% and there is a scattered positive correlation with P{sub 2}O{sub 5}. The content of Y + Ln`s is generally highest in the uraninites from RZB. Uraninite hydration and the formation of uranopelite/zippeite have caused complete loss of Y and the Ln`s. The analytical results indicate that Y and the Ln`s, which are high yield fission products, may be released from uraninite during alteration in the presence of P.

Jensen, K.A. [Aarhus Univ. (Denmark). Dept. of Earth Sciences; Ewing, R.C. [Univ. of New Mexico, Albuquerque, NM (United States). Dept. of Earth and Planetary Sciences; Gauthier-Lafaye, F. [Centre National de la Recherche Scientifique, Strasbourg (France). Centre de Geochemie de la Surface

1997-12-31T23:59:59.000Z

93

Characteristics of fuel crud and its impact on storage, handling, and shipment of spent fuel. [Fuel crud  

SciTech Connect (OSTI)

Corrosion products, called ''crud,'' form on out-of-reactor surfaces of nuclear reactor systems and are transported by reactor coolant to the core, where they deposit on external fuel-rod cladding surfaces and are activated by nuclear reactions. After discharge of spent fuel from a reactor, spallation of radioactive crud from the fuel rods could impact wet or dry storage operations, handling (including rod consolidation), and shipping. It is the purpose of this report to review earlier (1970s) and more recent (1980s) literature relating to crud, its characteristics, and any impact it has had on actual operations. Crud characteristics vary from reactor type to reactor type, reactor to reactor, fuel assembly to fuel assembly in a reactor, circumferentially and axially in an assembly, and from cycle to cycle for a specific facility. To characterize crud of pressurized-water (PWRs) and boiling-water reactors (BWRs), published information was reviewed on appearance, chemical composition, areal density and thickness, structure, adhesive strength, particle size, and radioactivity. Information was also collected on experience with crud during spent fuel wet storage, rod consolidation, transportation, and dry storage. From experience with wet storage, rod consolidation, transportation, and dry storage, it appears crud spallation can be managed effectively, posing no significant radiological problems. 44 refs., 11 figs.

Hazelton, R.F.

1987-09-01T23:59:59.000Z

94

SEU43 fuel bundle shielding analysis during spent fuel transport  

SciTech Connect (OSTI)

The basic task accomplished by the shielding calculations in a nuclear safety analysis consist in radiation doses calculation, in order to prevent any risks both for personnel protection and impact on the environment during the spent fuel manipulation, transport and storage. The paper investigates the effects induced by fuel bundle geometry modifications on the CANDU SEU spent fuel shielding analysis during transport. For this study, different CANDU-SEU43 fuel bundle projects, developed in INR Pitesti, have been considered. The spent fuel characteristics will be obtained by means of ORIGEN-S code. In order to estimate the corresponding radiation doses for different measuring points the Monte Carlo MORSE-SGC code will be used. Both codes are included in ORNL's SCALE 5 programs package. A comparison between the considered SEU43 fuel bundle projects will be also provided, with CANDU standard fuel bundle taken as reference. (authors)

Margeanu, C. A.; Ilie, P.; Olteanu, G. [Inst. for Nuclear Research Pitesti, No. 1 Campului Street, Mioveni 115400, Arges County (Romania)

2006-07-01T23:59:59.000Z

95

Management of super-grade plutonium in spent nuclear fuel  

SciTech Connect (OSTI)

This paper examines the security and safeguards implications of potential management options for DOE's sodium-bonded blanket fuel from the EBR-II and the Fermi-1 fast reactors. The EBR-II fuel appears to be unsuitable for the packaging alternative because of DOE's current safeguards requirements for plutonium. Emerging DOE requirements, National Academy of Sciences recommendations, draft waste acceptance requirements for Yucca Mountain and IAEA requirements for similar fuel also emphasize the importance of safeguards in spent fuel management. Electrometallurgical treatment would be acceptable for both fuel types. Meeting the known requirements for safeguards and security could potentially add more than $200M in cost to the packaging option for the EBR-II fuel.

McFarlane, H. F.; Benedict, R. W.

2000-03-20T23:59:59.000Z

96

Accelerator-driven transmutation of spent fuel elements  

DOE Patents [OSTI]

An apparatus and method is described for transmuting higher actinides, plutonium and selected fission products in a liquid-fuel subcritical assembly. Uranium may also be enriched, thereby providing new fuel for use in conventional nuclear power plants. An accelerator provides the additional neutrons required to perform the processes. The size of the accelerator needed to complete fuel cycle closure depends on the neutron efficiency of the supported reactors and on the neutron spectrum of the actinide transmutation apparatus. Treatment of spent fuel from light water reactors (LWRs) using uranium-based fuel will require the largest accelerator power, whereas neutron-efficient high temperature gas reactors (HTGRs) or CANDU reactors will require the smallest accelerator power, especially if thorium is introduced into the newly generated fuel according to the teachings of the present invention. Fast spectrum actinide transmutation apparatus (based on liquid-metal fuel) will take full advantage of the accelerator-produced source neutrons and provide maximum utilization of the actinide-generated fission neutrons. However, near-thermal transmutation apparatus will require lower standing

Venneri, Francesco (Los Alamos, NM); Williamson, Mark A. (Los Alamos, NM); Li, Ning (Los Alamos, NM)

2002-01-01T23:59:59.000Z

97

International Atomic Energy Agency (IAEA) activities on spent fuel management options  

SciTech Connect (OSTI)

Many countries have in the past several decades opted for storage of spent fuel for undefined periods of time. They have adopted the 'wait and see' strategy for spent fuel management. A relatively small number of countries have adopted reprocessing and use of MOX fuel as part of their strategy in spent fuel management. From the 10, 000 tonnes of heavy metal that is removed annually from nuclear reactors throughout the world, only approximately 30 % is currently being reprocessed. Continuous re-evaluation of world energy resources, announcement of the Global Nuclear Energy Partnership (GNEP) and the Russian initiative to form international nuclear centers, including reprocessing, are changing the stage for future development of nuclear energy. World energy demand is expected to more than double by 2050, and expansion of nuclear energy is a key to meeting this demand while reducing pollution and greenhouse gases. Since its foundation, the International Atomic Energy Agency (IAEA) has served as an interface between countries in exchanging information on the peaceful development of nuclear energy and at the same time guarding against proliferation of materials that could be used for nuclear weapons. The IAEA's Department of Nuclear Energy has been generating technical documents, holding meetings and conferences, and supporting technical cooperation projects to facilitate this exchange of information. This paper focuses on the current status of IAEA activities in the field of spent fuel management being carried out by the Division of Nuclear Fuel Cycle and Waste Technology. Information on those activities could be found on the web site link www.iaea.org/OurWork/ST/NE/NEFW/nfcms. To date, the IAEA has given priority in its spent fuel management activities to supporting Member States in their efforts to deal with growing accumulations of spent power reactor fuel. There is technical consensus that the present technologies for spent fuel storage, wet and dry, provide adequate protection to people and environment. As storage durations grow, the IAEA has expanded its work related to the implications of extended storage periods. Operation and maintenance of containers for storage and transport have also been investigated related to long term storage periods. In addition, as international interest in reprocessing of spent fuel increases, the IAEA continues to serve as a crossroads for sharing the latest developments in spent fuel treatment options. A Coordinated Research Project is currently addressing spent fuel performance assessment and research to evaluate long term effects of storage on spent fuel. The effect of increased burnup and mixed oxide fuels on spent fuel management is also the focus of interest as it follows the trend in optimizing the use of nuclear fuel. Implications of damaged fuel on storage and transport as well as burnup credit in spent fuel applications are areas that the IAEA is also investigating. Since spent fuel management considerations require social stability and institutional control, those aspects are taken into account in most IAEA activities. Data requirements and records management as storage durations extend were also investigated as well as the potential for regional spent fuel storage facilities. Spent fuel management activities continue to be coordinated with others in the IAEA to ensure compliance and consistency with efforts in the Department of Safety and Security and the Department of Safeguards, as well as with activities related to geologic disposal. Either disposal of radioactive waste or spent fuel will be an ultimate consideration in all spent fuel management options. Updated information on spent fuel treatment options that include fuel reprocessing as well as transmutation of minor actinides are investigated to optimize the use of nuclear fuel and minimize impact on environment. Tools for spent fuel management economics are also investigated to facilitate assessment of industrial applicability for these options. Most IAEA spent fuel management activities will ultimately be reported in o

Lovasic, Z.; Danker, W. [International Atomic Energy Agency (IAEA) Vienna (Austria)

2007-07-01T23:59:59.000Z

98

Optimization study on sample pretreatment of spent fuel storage rack  

Science Journals Connector (OSTI)

In order to evaluate radionuclide inventories as an essential item for the permanent disposal of spent fuel storage racks, chemical conditions for a sample pretreatment of a spent fuel storage rack were studied. ...

Hong-Joo Ahn; Myung-Ho Lee; Se-Chul Sohn…

2010-08-01T23:59:59.000Z

99

Description of the Canadian Particulate-Fill WastePackage (WP) System for Spent-Nuclear Fuel (SNF) and its Applicability to Ligh-Water Reactor SNF WPS with Depleted Uranium-Dioxide Fill  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

3502 3502 Chemical Technology Division DESCRIPTION OF THE CANADIAN PARTICULATE-FILL WASTE-PACKAGE (WP) SYSTEM FOR SPENT-NUCLEAR FUEL(SNF) AND ITS APPLICABILITY TO LIGHT- WATER REACTOR SNF WPS WITH DEPLETED URANIUM-DIOXIDE FILL Charles W. Forsberg Oak Ridge National Laboratory * P.O. Box 2008 Oak Ridge, Tennessee 37831-6180 Tel: (423) 574-6783 Fax: (423) 574-9512 Email: forsbergcw@ornl.gov October 20, 1997 _________________________ Managed by Lockheed Martin Energy Research Corp. under contract DE-AC05-96OR22464 for the * U.S. Department of Energy. iii CONTENTS LIST OF FIGURES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . v LIST OF TABLES . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . vii ACRONYMS . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .

100

Interim Storage of Hanford Spent Fuel & Associated Sludge  

SciTech Connect (OSTI)

The Hanford site is currently dealing with a number of types of Spent Nuclear Fuel. The route to interim dry storage for the various fuel types branches along two different paths. Fuel types such as metallic N reactor fuel and Shippingport Core 2 Blanket assemblies are being placed in approximately 4 m long canisters which are then stored in tubes below grade in a new canister storage building. Other fuels such as TRIGA{trademark} and Light Water Reactor fuel will be relocated and stored in stand-alone casks on a concrete pad. Varying degrees of sophistication are being applied with respect to the drying and/or evacuation of the fuel interim storage canisters depending on the reactivity of the fuel, the degree of damaged fuel and the previous storage environment. The characterization of sludge from the Hanford K Basins is nearly complete and canisters are being designed to store the sludge (including uranium particles from fuel element cleaning) on an interim basis.

MAKENAS, B.J.

2002-07-01T23:59:59.000Z

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


101

Spent-fuel dry-storage testing at E-MAD (March 1978-March 1982)  

SciTech Connect (OSTI)

From March 1978 through March 1982, spent fuel dry storage tests were conducted at the Engine Maintenance, Assembly and Disassembly (E-MAD) facility on the Nevada Test Site to confirm that commercial reactor spent fuel could be encapsulated and passively stored in one or more interim dry storage cell concepts. These tests were: electrically heated drywell, isolated and adjacent drywell, concrete silo, fuel assembly internal temperature measurement, and air-cooled vault. This document presents the test data and results as well as results from supporting test operations (spent fuel calorimetry and canister gas sampling).

Unterzuber, R.; Milnes, R.D.; Marinkovich, B.A.; Kubancsek, G.M.

1982-09-01T23:59:59.000Z

102

Fracture behavior of zircaloy spent-fuel cladding  

SciTech Connect (OSTI)

The Zircaloy cladding of water reactor fuel rods is susceptible to local breach-type failure, commonly known as pellet-cladding interaction (PCI) failure, during operational and off-normal power transients after the fuel has achieved a sufficiently high burnup. An optimization of power ramp procedures or fuel rod fabrication to minimize the cladding failure would result in a significant decrease in radiation exposure of plant personnel due to background and airborne radioactivity as well as an extension of core life in terms of allowable off-gas radioactivity. As part of a program to provide a better understanding of the fuel rod faiure phenomenon and to facilitate the formulation of a better failure criterion, a mechanistic study of the deformation and fracture behavior of high-burnup spent-fuel cladding is in progress under simulated PCI conditions.

Chung, H.M.; Yaggee, F.L.; Kassner, T.F.

1983-10-01T23:59:59.000Z

103

U.S. Spent Nuclear Fuel Data as of December 31, 2002  

Gasoline and Diesel Fuel Update (EIA)

Home > Nuclear > Spent Nuclear Fuel Home > Nuclear > Spent Nuclear Fuel Release Date: October 1, 2004 Next Release: Late 2010** Spent nuclear fuel data is collected by the Energy Information Administration (EIA) for the Office of Civilian Radioactive Waste Management (OCRWM). The spent nuclear fuel (SNF) data includes detailed characteristics of SNF generated by commercial U.S. nuclear power plants. From 1983 through 1995 this data was collected annually. Since 1996 this data has been collected every three years. The latest available detailed data covers all SNF discharged from commercial reactors before December 31, 2002, and is maintained in a data base by the EIA. Summary data tables from this data base may be found as indicated below. Table 1. Total U.S. Commercial Spent Nuclear Fuel Discharges, 1968 - 2002

104

Prototype spent-fuel canister design, analysis, and test  

SciTech Connect (OSTI)

Sandia National Laboratories was asked by the US Energy Research and Development Administration (now US Department of Energy) to design the spent fuel shipping cask system for the Clinch River Breeder Reactor Plant (CRBRP). As a part of this task, a canister which holds liquid sodium and the spent fuel assembly was designed, analyzed, and tested. The canister body survived the regulatory Type-B 9.1-m (30-ft) drop test with no apparent leakage. However, the commercially available metal seal used in this design leaked after the tests. This report describes the design approach, analysis, and prototype canister testing. Recommended work for completing the design, when funding is available, is included.

Leisher, W.B.; Eakes, R.G.; Duffey, T.A.

1982-03-01T23:59:59.000Z

105

International auspices for the storage of spent nuclear fuel as a nonproliferation measure  

SciTech Connect (OSTI)

The maintenance of spent nuclear fuel from power reactors will pose problems regardless of how or when the debate over reprocessing is resolved. At present, many reactor sites contain significant buildups of spent fuel stored in holding pools, and no measure short of shutting down reactors with no remaining storage capacity will alleviate the need for away-from-reactor storage. Although the federal government has committed itself to dealing with the spent fuel problem, no solution has been reached, largely because of a debate over differing projections of storage capacity requirements. Proliferation of weapons grade nuclear material in many nations presents another pressing issue. If nations with small nuclear programs are forced to deal with their own spent fuel accumulations, they will either have to reprocess it indigenously or contract to have it reprocessed in a foreign reprocessing plant. In either case, these nations may eventually possess sufficient resources to assemble a nuclear weapon. The problem of spent fuel management demands real global solutions, and further delay in solving the problem of spent nuclear fuel accumulation, both nationally and globally, can benefit only a small class of elected officials in the short term and may inflict substantial costs on the American public, and possibly the world. (JMT)

O'Brien, J.N.

1981-10-01T23:59:59.000Z

106

CANDU core analysis with spent PWR fuel of fixed {sup 235}U and {sup 239}Pu content  

SciTech Connect (OSTI)

The direct use of spent pressurized water reactor (PWR) fuel in a CANDU (DUPIC) fuel cycle requires that the spent PWR fuel be refabricated as a DUPIC fuel to be used in a CANDU reactor that was originally designed for the natural uranium fuel. Because there is no separation of isotopes from the spent PWR fuel, the DUPIC fuel contains all the actinides and fission products as fuel constituents and, therefore, the isotopic composition changes depending on the initial and discharge conditions of PWR fuels. Such heterogeneity in fuel composition is not desirable, especially for a CANDU reactor that adopts an on-power refueling scheme, because the operational flexibility is reduced appreciably if the fuel bundles of different composition are loaded throughout the core.

Choi, Hangbok; Roh, Gyu H.; Park, J.W. [Korea Atomic Energy Research Institute, Taejon (Korea, Republic of)

1997-12-01T23:59:59.000Z

107

Spent Fuel Storage Operational Experience With Increased Crud Activities  

SciTech Connect (OSTI)

A significant part of the electricity production in Hungary is provided by 4 units of VVER 440 nuclear reactors at the Paks Nuclear Power Plant. Interim dry storage of the spent fuel assemblies that are generated during the operation of the reactors is provided in a Modular Vault Dry Storage (MVDS) facility that is located in the immediate vicinity of the Paks Nuclear Power Plant. The storage capacity of the MVDS is being continuously extended in accordance with spent the fuel production rate from the four reactors. An accident occurred at unit 2 of the Paks Nuclear Power Plant in 2003, when thirty irradiated fuel assemblies were damaged during a cleaning process. The fuel assemblies were not inside the reactor at the time of the accident, but in a separate tank within the adjacent fuel decay pool. As a result of this accident, contamination from the badly damaged fuel assemblies spread to the decay pool water and also became deposited onto the surface of (hermetic) spent fuel assemblies within the decay pool. Therefore, it was necessary to review the design basis of the MVDS and assess the effects of taking the surface contaminated spent fuel assemblies into dry storage. The contaminated hermetic assemblies were transferred from the unit 2 pool to the interim storage facility in the period between 2005 and 2007. Continuous inspection and measurement was carried out during the transfer of these fuel assemblies. On the basis of the design assessments and measurement of the results during the fuel transfer, it was shown that radiological activity values increased due to the consequences of the accident but that these levels did not compromise the release and radiation dose limits for the storage facility. The aim of this paper is to show the effect on the operation of the MVDS interim storage facility as a result of the increased activity values due to the accident that occurred in 2003, as well as to describe the measurements that were taken, and their results and experience gained. In summary: On the basis of the design assessments and measurement of the results during the fuel transfer operations, it was shown that radiological activity values increased due to the consequences of the 2003 accident but that these levels did not compromise the release and dose limits for the fuel storage facility. In the environment there was no measurable radioactivity as a result of the operation of the Paks ISFSI. The exposure of the surrounding population was calculated on measured releases and meteorological data. The calculations show negligible doses until 2004. Due to the increased surface contamination on the spent fuel assemblies the dose rate increased almost 5 times compared to the least annual value, but still less then 0.01 percent of the allowed dose restriction. (authors)

Barnabas, I. [Public Agency for Radioactive Waste, Management (PURAM) (Hungary); Eigner, T. [Paks NPP (Hungary); Gresits, I. [Technical University of Budapest (Hungary); Ordagh, M. [SOM System Llc, (Hungary)

2008-07-01T23:59:59.000Z

108

Microsoft Word - spent_fuel_nutt.doc  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Decay Heat Decay Heat When a nuclear reactor has been shut down, and nuclear fission is not occurring at a large scale, the major source of heat production will be due to the beta decay of fission fragments. At the moment of reactor shutdown the decay heat is about 6.5% of the previous core power if the reactor has had a long and steady power history. About 1 hour after shutdown, the decay heat will be about 1.5% of the previous core power. After a day, the decay heat falls to 0.4%, and after a week it falls to 0.2%. While there is a large decrease in decay heat after a reactor is shut down, the used nuclear fuel in a reactor core must be continually cooled. This is why all reactors

109

5.14 - Spent Fuel Dissolution and Reprocessing Processes  

Science Journals Connector (OSTI)

Abstract The initial motivation for the development of reprocessing technologies came from the need for obtaining pure fissile material for nuclear weapon production. The most prominent among these is the PUREX (plutonium and uranium extraction) process, still used worldwide to reprocess commercial light water reactor fuels at a few thousand tons per year scale. The fuels dissolved in nitric acid are treated with a tributyl phosphate based solvent, the extracted uranium and plutonium are further purified, and the raffinate is vitrified for a safe final disposal. Plutonium is partly recycled as mixed oxide fuel. Since the beginning of this century, a new generation of nuclear reactors is being developed in the framework of the so-called generation IV initiative. For compliance with the sustainability goals defined for the innovative reactor systems, mainly waste minimization through recycling of all actinides, and for the achievement of these goals, the corresponding fuel cycles will play a central role. The new concept of a grouped actinide separation can be derived from aqueous or pyrochemical partitioning processes. For the aqueous schemes, a direct link to PUREX is obvious, namely, with coextraction of Np. The extraction of the remaining actinides can be achieved by using specially designed solvents based on phosphine oxide or diamide molecules. A major focus is on the very challenging separation of lanthanides from the trivalent actinides. The process implementation, especially for the less developed pyrometallurgy, requires a good understanding of the extraction mechanisms. Pyro-reprocessing, where all actinides are recycled, is based on metallic fuels; they are dissolved in molten salts at around 500–900 °C and actinides are selectively recovered, either by electrorefining or by extraction into a liquid metal phase. The fuels of new generation reactors will, at least in the beginning, most likely be oxides. Thus, for pyroprocesses a head-end reduction step for oxide into metals fuels is needed. A very specific reprocessing technology, the so-called direct use of pressurized water reactor spent fuel in CANDU process, is being developed in Korea. Here, used pressurized water reactor fuel is recycled to CANDU (CANada Deuterium Uranium) reactors after a dry treatment where volatile fission products are removed.

J.-P. Glatz

2012-01-01T23:59:59.000Z

110

Transportation capabilities study of DOE-owned spent nuclear fuel  

SciTech Connect (OSTI)

This study evaluates current capabilities for transporting spent nuclear fuel owned by the US Department of Energy. Currently licensed irradiated fuel shipping packages that have the potential for shipping the spent nuclear fuel are identified and then matched against the various spent nuclear fuel types. Also included are the results of a limited investigation into other certified packages and new packages currently under development. This study is intended to support top-level planning for the disposition of the Department of Energy`s spent nuclear fuel inventory.

Clark, G.L.; Johnson, R.A.; Smith, R.W. [Packaging Technology, Inc., Tacoma, WA (United States); Abbott, D.G.; Tyacke, M.J. [Lockheed Idaho Technologies Co., Idaho Falls, ID (United States)

1994-10-01T23:59:59.000Z

111

Issues related to EM management of DOE spent nuclear fuel  

SciTech Connect (OSTI)

This document is a summary of the important issues involved in managing spent nuclear fuel (SNF) owned by the Department of Energy (DOE). Issues related to civilian SNF activities are not discussed. DOE-owned SNF is stored primarily at the Hanford Site, Idaho National Engineering Laboratory (INEL), Savannah River Site (SRS), Oak Ridge National Laboratory (ORNL), and West Valley Demonstration Project. Smaller quantities of SNF are stored at Brookhaven National Laboratory, Sandia National Laboratories, and Los Alamos National Laboratory (LANL). There is a wide variety of fuel types, including both low and high enrichment fuels from weapons production, DOE reactors, research and development programs, naval programs, and universities. Most fuel is stored in pools associated with reactor or reprocessing facilities. Smaller quantities are in dry storage. Physical conditions of the fuel range from excellent to poor or severely damaged. An issue is defined as an important question that must be answered or decision that must be made on a topic or subject relevant to achieving the complimentary objectives of (a) storing SNF in compliance with applicable regulations and orders until it can be disposed, and (b) safely disposing of DOE`s SNF. The purpose of this document is to define the issues; no recommendations are made on resolutions. As DOE`s national SNF management program is implemented, a system of issues identification, documentation, tracking, and resolution will be implemented. This document is an initial effort at issues identification. The first section of this document is an overview of issues that are common to several or all DOE facilities that manage SNF. The common issues are organized according to specific aspects of spent fuel management. This is followed by discussions of management issues that apply specifically to individual DOE facilities. The last section provides literature references.

Abbott, D.G. [EG& G Idaho, Inc., Idaho Falls, ID (United States); Abashian, M.S.; Chakraborti, S.; Roberson, K.; Meloin, J.M. [IT Corp. (United States)

1993-07-01T23:59:59.000Z

112

Nuclear Reactor Materials and Fuels  

Science Journals Connector (OSTI)

Nuclear reactor materials and fuels can be classified into six categories: Nuclear fuel materials Nuclear clad materials Nuclear coolant materials Nuclear poison materials Nuclear moderator materials

Dr. James S. Tulenko

2012-01-01T23:59:59.000Z

113

Deformation and fracture characteristics of spent Zircaloy fuel cladding  

SciTech Connect (OSTI)

For a better understanding of Zircaloy fuel-rod failure by the pellet-cladding interaction (PCI) phenomenon, a mechanistic study of deformation and fracture behavior of spent power reactor fuel cladding under simulated PCI conditions was conducted. Zircaloy-2 cladding specimens, obtained from fuel assemblies of operating power reactors, were deformed to fracture at 325/sup 0/C by internal gas pressurization in the absence of fission product simulants. Fracture characteristics and microstructures were examined via SEM, TEM, and HVEM. Numerous dislocation tangles and cell structures, observed in TEM specimens of cladding tubes that failed in a ductile manner, were consistent with SEM observations of a limited number of dimples characteristic of microvoid coalescence. A number of brittle-type failures were produced without the influence of fission product simulants. The brittle cracks occurred near the areas compressed by the Swagelok fittings of the internally pressurized tube and propagated from the outer to the inner surface. Since the outer surface was isolated and maintained under a flowing stream of pure helium, it is unlikely that the brittle-type failure was influenced by any fission product traces. SEM fractography of the brittle-type failure revealed a large area of transgranular pseudocleavage with limited areas of ductile fluting, which were similar in appearance to the surfaces produced by in-reactor PCI-type failures. A TEM evaluation of the cladding in the vicinity of the through-wall crack revealed numerous locations that contained an extensive amount of second-phase precipitate (Zr/sub 3/O). We believe that the brittle-type failures of the irradiated spent fuel cladding in the stress rupture experiments are associated with segregation of oxygen, which leads to the formation of the order structure, an immobilization of dislocations, and minimal plastic deformation in the material.

Chung, H.M.; Yaggee, F.L.

1982-09-01T23:59:59.000Z

114

Microsoft Word - spent nuclear fuel report.doc  

Broader source: Energy.gov (indexed) [DOE]

Management of Spent Nuclear Fuel Management of Spent Nuclear Fuel at the Savannah River Site DOE/IG-0727 May 2006 REPORT ON MANAGEMENT OF SPENT NUCLEAR FUEL AT THE SAVANNAH RIVER SITE TABLE OF CONTENTS Spent Nuclear Fuel Management Details of Finding 1 Recommendations 2 Comments 3 Appendices 1. Objective, Scope, and Methodology 4 2. Prior Audit Reports 5 3. Management Comments 6 SPENT NUCLEAR FUEL MANGEMENT Page 1 Details of Finding H-Canyon The Department of Energy's (Department) spent nuclear fuel Operations program at the Savannah River Site (Site) will likely require Extended H-Canyon to be maintained at least two years beyond defined operational needs. The Department committed to maintain H-Canyon operational readiness to provide a disposal path for

115

EIS-0279: Spent Nuclear Fuel Management, Aiken, South Carolina | Department  

Broader source: Energy.gov (indexed) [DOE]

79: Spent Nuclear Fuel Management, Aiken, South Carolina 79: Spent Nuclear Fuel Management, Aiken, South Carolina EIS-0279: Spent Nuclear Fuel Management, Aiken, South Carolina SUMMARY The proposed DOE action considered in this environmental impact statement (EIS) is to implement appropriate processes for the safe and efficient management of spent nuclear fuel and targets at the Savannah River Site (SRS) in Aiken County, South Carolina, including placing these materials in forms suitable for ultimate disposition. PUBLIC COMMENT OPPORTUNITIES None available at this time. DOCUMENTS AVAILABLE FOR DOWNLOAD April 5, 2013 EIS-0279: Amended Record of Decision Spent Nuclear Fuel Management at the Savannah River Site April 1, 2013 EIS-0279-SA-01: Supplement Analysis Savannah River Site Spent Nuclear Fuel Management (DOE/EIS-0279-SA-01 and

116

Naval Spent Fuel Rail Shipment Accident Exercise Objectives  

Broader source: Energy.gov (indexed) [DOE]

NAVAL SPENT FUEL RAIL SHIPMENT NAVAL SPENT FUEL RAIL SHIPMENT ACCIDENT EXERCISE OBJECTIVES * Familiarize stakeholders with the Naval spent fuel ACCIDENT EXERCISE OBJECTIVES Familiarize stakeholders with the Naval spent fuel shipping container characteristics and shipping practices * Gain understanding of how the NNPP escorts who accompany the spent fuel shipments will interact with civilian emergency services representatives g y p * Allow civilian emergency services agencies the opportunity to evaluate their response to a pp y p simulated accident * Gain understanding of how the communications links that would be activated in an accident involving a Naval spent fuel shipment would work 1 NTSF May 11 ACCIDENT EXERCISE TYPICAL TIMELINE * Conceptual/Organizational Meeting - April 6 E R T i d it t t d TYPICAL TIMELINE

117

Facts and issues of direct disposal of spent fuel; Revision 1  

SciTech Connect (OSTI)

This report reviews those facts and issues that affect the direct disposal of spent reactor fuels. It is intended as a resource document for those impacted by the current Department of Energy (DOE) guidance that calls for the cessation of fuel reprocessing. It is not intended as a study of the specific impacts (schedules and costs) to the Savannah River Site (SRS) alone. Commercial fuels, other low enriched fuels, highly enriched defense-production, research, and naval reactor fuels are included in this survey, except as prevented by rules on classification.

Parks, P.B.

1993-10-01T23:59:59.000Z

118

DOE SPENT NUCLEAR FUEL DISPOSAL CONTAINER  

SciTech Connect (OSTI)

The DOE Spent Nuclear Fuel Disposal Container (SNF DC) supports the confinement and isolation of waste within the Engineered Barrier System of the Mined Geologic Disposal System (MGDS). Disposal containers are loaded and sealed in the surface waste handling facilities, transferred to the underground through the access mains, and emplaced in emplacement drifts. The DOE Spent Nuclear Fuel Disposal Container provides long term confinement of DOE SNF waste, and withstands the loading, transfer, emplacement, and retrieval loads and environments. The DOE SNF Disposal Containers provide containment of waste for a designated period of time, and limit radionuclide release thereafter. The disposal containers maintain the waste in a designated configuration, withstand maximum handling and rockfall loads, limit the individual waste canister temperatures after emplacement. The disposal containers also limit the introduction of moderator into the disposal container during the criticality control period, resist corrosion in the expected repository environment, and provide complete or limited containment of waste in the event of an accident. Multiple disposal container designs may be needed to accommodate the expected range of DOE Spent Nuclear Fuel. The disposal container will include outer and inner barrier walls and outer and inner barrier lids. Exterior labels will identify the disposal container and contents. Differing metal barriers will support the design philosophy of defense in depth. The use of materials with different failure mechanisms prevents a single mode failure from breaching the waste package. The corrosion-resistant inner barrier and inner barrier lid will be constructed of a high-nickel alloy and the corrosion-allowance outer barrier and outer barrier lid will be made of carbon steel. The DOE Spent Nuclear Fuel Disposal Containers interface with the emplacement drift environment by transferring heat from the waste to the external environment and by protecting the DOE waste canisters and their contents from damage/degradation by the external environment. The disposal containers also interface with the SNF by limiting access of moderator and oxidizing agents to the waste. The disposal containers interface with the Ex-Container System's emplacement drift disposal container supports. The disposal containers interface with the Canister Transfer System, Waste Emplacement System, Disposal Container Handling System, and Waste Package Remediation System during loading, handling, transfer, emplacement and remediation of the disposal container.

F. Habashi

1998-06-26T23:59:59.000Z

119

Surrogate Spent Nuclear Fuel Vibration Integrity Investigation  

SciTech Connect (OSTI)

Transportation packages for spent nuclear fuel (SNF) must meet safety requirements under normal and accident conditions as specified by federal regulations. During transportation, SNF experiences unique conditions and challenges to cladding integrity due to the vibrational and impact loading encountered during road or rail shipment. ORNL has been developing testing capabilities that can be used to improve our understanding of the impacts of vibration loading on SNF integrity, especially for high burn-up SNF in normal transportation operation conditions. This information can be used to meet nuclear industry and U.S. Nuclear Regulatory Commission needs in the area of safety of SNF storage and transportation operations.

Wang, Jy-An John [ORNL; Wang, Hong [ORNL; Bevard, Bruce Balkcom [ORNL; Howard, Rob L [ORNL

2014-01-01T23:59:59.000Z

120

President Reagan Calls for a National Spent Fuel Storage Facility...  

National Nuclear Security Administration (NNSA)

Spent Fuel Storage Facility Washington, DC The Reagan Administration announces a nuclear energy policy that anticipates the establishment of a facility for the storage of...

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


121

Spent nuclear fuel project - criteria document spent nuclear fuel final safety analysis report  

SciTech Connect (OSTI)

The criteria document provides the criteria and planning guidance for developing the Spent Nuclear Fuel (SNF) Final Safety Analysis Report (FSAR). This FSAR will support the US Department of Energy, Richland Operations Office decision to authorize the procurement, installation, installation acceptance testing, startup, and operation of the SNF Project facilities (K Basins, Cold Vacuum Drying Facility, and Canister Storage Building).

MORGAN, R.G.

1999-02-23T23:59:59.000Z

122

Training implementation matrix, Spent Nuclear Fuel Project (SNFP)  

SciTech Connect (OSTI)

This Training Implementation Matrix (TIM) describes how the Spent Nuclear Fuel Project (SNFP) implements the requirements of DOE Order 5480.20A, Personnel Selection, Qualification, and Training Requirements for Reactor and Non-Reactor Nuclear Facilities. The TIM defines the application of the selection, qualification, and training requirements in DOE Order 5480.20A at the SNFP. The TIM also describes the organization, planning, and administration of the SNFP training and qualification program(s) for which DOE Order 5480.20A applies. Also included is suitable justification for exceptions taken to any requirements contained in DOE Order 5480.20A. The goal of the SNFP training and qualification program is to ensure employees are capable of performing their jobs safely and efficiently.

EATON, G.L.

2000-06-08T23:59:59.000Z

123

Licensing of spent fuel dry storage and consolidated rod storage: A Review of Issues and Experiences  

SciTech Connect (OSTI)

The results of this study, performed by Pacific Northwest Laboratory (PNL) and sponsored by the US Department of Energy (DOE), respond to the nuclear industry's recommendation that a report be prepared that collects and describes the licensing issues (and their resolutions) that confront a new applicant requesting approval from the US Nuclear Regulatory Commission (NRC) for dry storage of spent fuel or for large-scale storage of consolidated spent fuel rods in pools. The issues are identified in comments, questions, and requests from the NRC during its review of applicants' submittals. Included in the report are discussions of (1) the 18 topical reports on cask and module designs for dry storage fuel that have been submitted to the NRC, (2) the three license applications for dry storage of spent fuel at independent spent fuel storage installations (ISFSIs) that have been submitted to the NRC, and (3) the three applications (one of which was later withdrawn) for large-scale storage of consolidated fuel rods in existing spent fuel storage pools at reactors that were submitted tot he NRC. For each of the applications submitted, examples of some of the issues (and suggestions for their resolutions) are described. The issues and their resolutions are also covered in detail in an example in each of the three subject areas: (1) the application for the CASTOR V/21 dry spent fuel storage cask, (2) the application for the ISFSI for dry storage of spent fuel at Surry, and (3) the application for full-scale wet storage of consolidated spent fuel at Millstone-2. The conclusions in the report include examples of major issues that applicants have encountered. Recommendations for future applicants to follow are listed. 401 refs., 26 tabs.

Bailey, W.J.

1990-02-01T23:59:59.000Z

124

Safeguards-by-Design: Guidance for Independent Spent Fuel Dry Storage Installations (ISFSI)  

SciTech Connect (OSTI)

This document summarizes the requirements and best practices for implementing international nuclear safeguards at independent spent fuel storage installations (ISFSIs), also known as Away-from- Reactor (AFR) storage facilities. These installations may provide wet or dry storage of spent fuel, although the safeguards guidance herein focuses on dry storage facilities. In principle, the safeguards guidance applies to both wet and dry storage. The reason for focusing on dry independent spent fuel storage installations is that this is one of the fastest growing nuclear installations worldwide. Independent spent fuel storage installations are typically outside of the safeguards nuclear material balance area (MBA) of the reactor. They may be located on the reactor site, but are generally considered by the International Atomic Energy Agency (IAEA) and the State Regulator/SSAC to be a separate facility. The need for this guidance is becoming increasingly urgent as more and more nuclear power plants move their spent fuel from resident spent fuel ponds to independent spent fuel storage installations. The safeguards requirements and best practices described herein are also relevant to the design and construction of regional independent spent fuel storage installations that nuclear power plant operators are starting to consider in the absence of a national long-term geological spent fuel repository. The following document has been prepared in support of two of the three foundational pillars for implementing Safeguards-by-Design (SBD). These are: i) defining the relevant safeguards requirements, and ii) defining the best practices for meeting the requirements. This document was prepared with the design of the latest independent dry spent fuel storage installations in mind and was prepared specifically as an aid for designers of commercial nuclear facilities to help them understand the relevant international requirements that follow from a country’s safeguards agreement with the IAEA. If these requirements are understood at the earliest stages of facility design, it will help eliminate the costly retrofit of facilities that has occurred in the past to accommodate nuclear safeguards, and will help the IAEA implement nuclear safeguards worldwide, especially in countries building their first nuclear facilities. It is also hoped that this guidance document will promote discussion between the IAEA, State Regulator/SSAC, Project Design Team, and Facility Owner/Operator at an early stage to ensure that new ISFSIs will be effectively and efficiently safeguarded. This is intended to be a living document, since the international nuclear safeguards requirements may be subject to revision over time. More importantly, the practices by which the requirements are met are continuously modernized by the IAEA and facility operators for greater efficiency and cost effectiveness. As these improvements are made, it is recommended that the subject guidance document be updated and revised accordingly.

Trond Bjornard; Philip C. Durst

2012-05-01T23:59:59.000Z

125

Testing of the CANDU Spent Fuel Storage Basket Package  

SciTech Connect (OSTI)

The paper described the results of testing for a CANDU Spent Fuel Storage Basket Package Prototype intended to be used for transport and storage of the CANDU spent fuel bundles within NPP CANDU Cernavoda, Romania. The results obtained proved that the objectives of those tests were achieved

Vieru, G.

2002-02-28T23:59:59.000Z

126

RUSSIAN-ORIGIN HIGHLY ENRICHED URANIUM SPENT NUCLEAR FUEL SHIPMENT FROM BULGARIA  

SciTech Connect (OSTI)

In July 2008, the Global Threat Reduction Initiative and the IRT 2000 research reactor in Sofia, Bulgaria, operated by the Institute for Nuclear Research and Nuclear Energy (INRNE), safely shipped 6.4 kilograms of Russian origin highly enriched uranium (HEU) spent nuclear fuel (SNF) to the Russian Federation. The shipment, which resulted in the removal of all HEU from Bulgaria, was conducted by truck, barge, and rail modes of transport across two transit countries before reaching the final destination at the Production Association Mayak facility in Chelyabinsk, Russia. This paper describes the work, equipment, organizations, and approvals that were required to complete the spent fuel shipment and provides lessons learned that might assist other research reactor operators with their own spent nuclear fuel shipments.

Kelly Cummins; Igor Bolshinsky; Ken Allen; Tihomir Apostolov; Ivaylo Dimitrov

2009-07-01T23:59:59.000Z

127

Fracture behavior of high-burnup spent-fuel cladding  

SciTech Connect (OSTI)

PCI-like, brittle-type failures, characterized by pseudocleavage-plus-fluting features in the fracture surface, branching cracks, and small diametral strain, were observed to occur at 292 to 325/sup 0/C in some batches of spent power-reactor fuel-cladding tubes under internal gas-pressurization and expanding-mandrel loading conditions in which the tests were not influenced by fission product simulants. Fractographic characteristics per se do not provide evidence for a PCI failure mechanism but should be deemed only as cooroborative in nature. Evaluation of TEM thin-foil specimens, obtained from regions adjacent to the brittle-type fracture sites, characteristically revealed extensive amounts of Zr/sub 3/O precipitates and a lack of slip dislocations. The precipitation of the Zr/sub 3/O phase appears to be enhanced by a high density of irradiation-induced defects. The brittle-type failure produced in the spent-fuel cladding tubes appears to be associated with segregation of oxygen to dislocation substructures and irradiation-induced defects, which leads to the formation of an ordered zirconium-oxygen phase of Zr/sub 3/O, an immobilization of dislocations, and minimal plastic deformation in the cladding material.

Chung, H.M.; Yaggee, F.L.; Kassner, T.F.

1983-10-01T23:59:59.000Z

128

Evaluation of Radiation Impacts of Spent Nuclear Fuel Storage (SNFS-2) of Chernobyl NPP - 13495  

SciTech Connect (OSTI)

Radiation effects are estimated for the operation of a new dry storage facility for spent nuclear fuel (SNFS-2) of Chernobyl NPP RBMK reactors. It is shown that radiation exposure during normal operation, design and beyond design basis accidents are minor and meet the criteria for safe use of radiation and nuclear facilities in Ukraine. (authors)

Paskevych, Sergiy; Batiy, Valiriy; Sizov, Andriy [Institute for Safety Problems of Nuclear Power Plants, National Academy of Sciences of Ukraine, 36 a Kirova str. Chornobyl, Kiev region, 07200 (Ukraine)] [Institute for Safety Problems of Nuclear Power Plants, National Academy of Sciences of Ukraine, 36 a Kirova str. Chornobyl, Kiev region, 07200 (Ukraine); Schmieman, Eric [Battelle Memorial Institute, PO Box 999 MSIN K6-90, Richland, WA 99352 (United States)] [Battelle Memorial Institute, PO Box 999 MSIN K6-90, Richland, WA 99352 (United States)

2013-07-01T23:59:59.000Z

129

Assessment of the Fingerprinting Method for Spent Fuel Verification in MACSTOR KN-400 CANDU Dry Storage  

E-Print Network [OSTI]

The Korea Hydro and Nuclear Power has built a new modular type of dry storage facility, known as MACSTOR KN-400 at Wolsong reactor site. The building has the capacity to store up to 24000 CANDU spent fuel bundles in a 4 rows by 10 columns...

Gowthahalli Chandregowda, Nandan

2012-10-19T23:59:59.000Z

130

Safety Aspects of Wet Storage of Spent Nuclear Fuel, OAS-L-13-11  

Broader source: Energy.gov (indexed) [DOE]

Safety Aspects of Wet Storage of Safety Aspects of Wet Storage of Spent Nuclear Fuel OAS-L-13-11 July 2013 Department of Energy Washington, DC 20585 July 10, 2013 MEMORANDUM FOR THE SENIOR ADVISOR FOR ENVIRONMENTAL MANAGEMENT FROM: Daniel M. Weeber Assistant Inspector General for Audits and Administration Office of Inspector General SUBJECT: INFORMATION: Audit Report on "Safety Aspects of Wet Storage of Spent Nuclear Fuel" BACKGROUND The Department of Energy (Department) is responsible for managing and storing spent nuclear fuel (SNF) generated by weapons and research programs and recovered through nonproliferation programs. The SNF consists of irradiated reactor fuel and cut up assemblies containing uranium, thorium and/or plutonium. The Department stores 34 metric tons of heavy metal SNF primarily

131

Plutonium and Reprocessing of Spent Nuclear Fuel  

Science Journals Connector (OSTI)

...Repository for the Disposal of Spent Nuclear...Radioactive Waste at Yucca Mountain (YMP-0106...not committed funding to build...Repository for the Disposal of Spent Nuclear...Radioactive Waste at Yucca Mountain (YMP-0106, Yucca Mountain Project, North...

Frank N. von Hippel

2001-09-28T23:59:59.000Z

132

Sustainability Considerations in Spent Light-water Nuclear Fuel Retrievability  

SciTech Connect (OSTI)

This paper examines long-term cost differences between two competing Light Water Reactor (LWR) fuels: Uranium Oxide (UOX) and Mixed Uranium Oxide-Plutonium Oxide (MOX). Since these costs are calculated on a life-cycle basis, expected savings from lower future MOX fuel prices can be used to value the option of substituting MOX for UOX, including the value of maintaining access to the used UOX fuel that could be reprocessed to make MOX. The two most influential cost drivers are the price of natural uranium and the cost of reprocessing. Significant and sustained reductions in reprocessing costs and/or sustained increases in uranium prices are required to give positive value to the retrievability of Spent Nuclear Fuel. While this option has positive economic value, it might not be exercised for 50 to 200 years. Therefore, there are many years for a program during which reprocessing technology can be researched, developed, demonstrated, and deployed. Further research is required to determine whether the cost of such a program would yield positive net present value and/or increases the sustainability of LWR energy systems.

Wood, Thomas W.; Rothwell, Geoffrey

2012-01-10T23:59:59.000Z

133

SUPPLEMENT ANALYSIS OF FOREIGN RESEARCH REACTOR srENT NUCLEAR FUEL  

Broader source: Energy.gov (indexed) [DOE]

FOREIGN RESEARCH REACTOR srENT NUCLEAR FUEL FOREIGN RESEARCH REACTOR srENT NUCLEAR FUEL TRANSPORTATION ALONG OTHER THAN~. PRESENTATIVE ROUTE FROM CONCORD NAVAL WEAPO~~ STATION TO IDAHO NATIONAL ENGINEERING AND ENVIRONMENTAL LADORA TORY Introduction The Department of Energy is planning to transport foreign research reactor spent nuclear fuel by rail from the Concord Naval Weapons Station (CNWS), Concord, California, to the Idaho National Engineering and Environmental Laboratory (INEEL). The environmental analysis supporting the decision to transport, by rail or truck, foreign research reactor spent nuclear fuel from CNWS to the INEEL is contained in +he Final Environmental Impact Statement on a Proposed Nuclear Weapons Nonproliftration Policy Concerning Foreign Research Reactor

134

Fossil fuel furnace reactor  

DOE Patents [OSTI]

A fossil fuel furnace reactor is provided for simulating a continuous processing plant with a batch reactor. An internal reaction vessel contains a batch of shale oil, with the vessel having a relatively thin wall thickness for a heat transfer rate effective to simulate a process temperature history in the selected continuous processing plant. A heater jacket is disposed about the reactor vessel and defines a number of independent controllable temperature zones axially spaced along the reaction vessel. Each temperature zone can be energized to simulate a time-temperature history of process material through the continuous plant. A pressure vessel contains both the heater jacket and the reaction vessel at an operating pressure functionally selected to simulate the continuous processing plant. The process yield from the oil shale may be used as feedback information to software simulating operation of the continuous plant to provide operating parameters, i.e., temperature profiles, ambient atmosphere, operating pressure, material feed rates, etc., for simulation in the batch reactor.

Parkinson, William J. (Los Alamos, NM)

1987-01-01T23:59:59.000Z

135

Foreign experience on effects of extended dry storage on the integrity of spent nuclear fuel  

SciTech Connect (OSTI)

This report summarizes the results of a survey of foreign experience in dry storage of spent fuel from nuclear power reactors that was carried out for the US Department of Energy`s (DOE) Office of Civilian Radioactive Waste Management (OCRWM). The report reviews the mechanisms for degradation of spent fuel cladding and fuel materials in dry storage, identifies the status and plans of world-wide experience and applications, and documents the available information on the expected long-term integrity of the dry-stored spent fuel from actual foreign experience. Countries covered in this survey are: Argentina, Canada, Federal Republic of Germany (before reunification with the former East Germany), former German Democratic Republic (former East Germany), France, India, Italy, Japan, South Korea, Spain, Switzerland, United Kingdom, and the former USSR (most of these former Republics are now in the Commonwealth of Independent States [CIS]). Industrial dry storage of Magnox fuels started in 1972 in the United Kingdom; Canada began industrial dry storage of CANDU fuels in 1980. The technology for safe storage is generally considered to be developed for time periods of 30 to 100 years for LWR fuel in inert gas and for some fuels in oxidizing gases at low temperatures. Because it will probably be decades before countries will have a repository for spent fuels and high-level wastes, the plans for expanded use of dry storage have increased significantly in recent years and are expected to continue to increase in the near future.

Schneider, K.J.; Mitchell, S.J.

1992-04-01T23:59:59.000Z

136

Foreign experience on effects of extended dry storage on the integrity of spent nuclear fuel  

SciTech Connect (OSTI)

This report summarizes the results of a survey of foreign experience in dry storage of spent fuel from nuclear power reactors that was carried out for the US Department of Energy's (DOE) Office of Civilian Radioactive Waste Management (OCRWM). The report reviews the mechanisms for degradation of spent fuel cladding and fuel materials in dry storage, identifies the status and plans of world-wide experience and applications, and documents the available information on the expected long-term integrity of the dry-stored spent fuel from actual foreign experience. Countries covered in this survey are: Argentina, Canada, Federal Republic of Germany (before reunification with the former East Germany), former German Democratic Republic (former East Germany), France, India, Italy, Japan, South Korea, Spain, Switzerland, United Kingdom, and the former USSR (most of these former Republics are now in the Commonwealth of Independent States (CIS)). Industrial dry storage of Magnox fuels started in 1972 in the United Kingdom; Canada began industrial dry storage of CANDU fuels in 1980. The technology for safe storage is generally considered to be developed for time periods of 30 to 100 years for LWR fuel in inert gas and for some fuels in oxidizing gases at low temperatures. Because it will probably be decades before countries will have a repository for spent fuels and high-level wastes, the plans for expanded use of dry storage have increased significantly in recent years and are expected to continue to increase in the near future.

Schneider, K.J.; Mitchell, S.J.

1992-04-01T23:59:59.000Z

137

Dry Storage Demonstration for High-Burnup Spent Nuclear Fuel-Feasibility Study  

SciTech Connect (OSTI)

Initially, casks for dry storage of spent fuel were licensed for assembly-average burnup of about 35 GWd/MTU. Over the last two decades, the discharge burnup of fuel has increased steadily and now exceeds 45 GWd/MTU. With spent fuel burnups approaching the licensing limits (peak rod burnup of 62 GWd/MTU for pressurized water reactor fuel) and some lead test assemblies being burned beyond this limit, a need for a confirmatory dry storage demonstration program was first identified after the publication in May 1999 of the U.S. Nuclear Regulatory Commissions (NRC) Interim Staff Guidance 11 (ISG-11). With the publication in July 2002 of the second revision of ISG-11, the desirability for such a program further increased to obtain confirmatory data about the potential changes in cladding mechanical properties induced by dry storage, which would have implications to the transportation, handling, and disposal of high-burnup spent fuel. While dry storage licenses have kept pace with reactor discharge burnups, transportation licenses have not and are considered on a case by case basis. Therefore, this feasibility study was performed to examine the options available for conducting a confirmatory experimental program supporting the dry storage, transportation, and disposal of spent nuclear fuel with burnups well in excess of 45 GWd/MTU.

McKinnon, Mikal A. (BATTELLE (PACIFIC NW LAB)); Cunningham, Mitchel E. (BATTELLE (PACIFIC NW LAB))

2003-09-09T23:59:59.000Z

138

Report to Congress on Plan for Interim Storage of Spent Nuclear...  

Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

Report to Congress on Plan for Interim Storage of Spent Nuclear Fuel from Decommissioned Reactors Report to Congress on Plan for Interim Storage of Spent Nuclear Fuel from...

139

MELCOR model for an experimental 17x17 spent fuel PWR assembly.  

SciTech Connect (OSTI)

A MELCOR model has been developed to simulate a pressurized water reactor (PWR) 17 x 17 assembly in a spent fuel pool rack cell undergoing severe accident conditions. To the extent possible, the MELCOR model reflects the actual geometry, materials, and masses present in the experimental arrangement for the Sandia Fuel Project (SFP). The report presents an overview of the SFP experimental arrangement, the MELCOR model specifications, demonstration calculation results, and the input model listing.

Cardoni, Jeffrey

2010-11-01T23:59:59.000Z

140

COBRA-SFS (Spent-Fuel Storage) thermal-hydraulic analyses of the CASTOR-1C and REA 2023 BWR storage casks containing consolidated spent fuel  

SciTech Connect (OSTI)

Consolidation of spent nuclear fuel rods is being considered as one option for more efficient and compact storage of reactor spent fuel assemblies. In this concept, rods from two disassembled spent fuel assemblies will be consolidated in a space originally intended to store a single unconsolidated assembly. The thermal performance of consolidated fuel rods in dry storage, especially in multiassembly storage systems, is one of the major issues that must be addressed prior to implementation. In this study, Pacific Northwest Laboratory researchers performed thermal-hydraulic analyses for both the REA 2023 cask and the CASTOR-1C cask containing either unconsolidated or consolidated BWR spent fuel assemblies. The objective was to determine the effect of consolidating spent fuel assemblies on the temperature distributions within both types of casks. Two major conclusions resulted from this study. First, a lumping technique (combining rods and flow channels), which reduces the number of computational nodes required to model complex multiassembly geometries, could be used for both unconsolidated and consolidated rods with negligible effect on prediction accuracies. Second, with a relatively high thermal conductivity backfill gas (e.g., helium), the predicted peak fuel rod temperature in a canister of consolidated rods generating the same amount of heat as an unconsolidated assembly is essentially the same as the peak temperature in the unconsolidated assembly. In contrast, with a relatively low thermal conductivity backfill gas (e.g., nitrogen), the opposite is true and the predicted peak temperature in a consolidated canister is significantly higher than in an unconsolidated assembly. Therefore, when rods are consolidated, selection of the backfill gas is important in maintaining peak rod temperatures below allowable values for rods with relatively high decay heat generation rates.

Rector, D.R.; Cuta, J.M.; Lombardo, N.J.

1986-12-01T23:59:59.000Z

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


141

Risk and Responsibility Sharing in Nuclear Spent Fuel Management  

E-Print Network [OSTI]

With the Nuclear Waste Policy Act of 1982, the responsibility of American utilities in the long-term management of spent nuclear fuel was limited to the payment of a fee. This narrow involvement did not result in faster ...

De Roo, Guillaume

142

U.S. Spent Nuclear Fuel Data as of December 31, 1998  

Gasoline and Diesel Fuel Update (EIA)

Spent Nuclear Fuel Data, Detailed United States as of December 31, 1998 Spent nuclear fuel data is collected by the Energy Information Administration (EIA) for the Office of Civilian Radioactive Waste Management (OCRWM). The spent nuclear fuel (SNF) data includes detailed characteristics of SNF generated by commercial U.S. nuclear power plants. From 1983 through 1995 this data was collected annually. Since 1996 this data has been collected every three years. The latest available detailed data covers all SNF discharged from commercial reactors before December 31, 1998, and is maintained in a database by the EIA. Summary data tables from this database may be found as indicated below. The detailed data are available on request from Jim Finucane who can be reached at 202-287-1966 or at

143

Examining 239Pu and 240Pu Nuclear Resonance Fluorescence Measurements on Spent Fuel for Nuclear Safeguards  

E-Print Network [OSTI]

on Spent Fuel for Nuclear Safeguards Brian J. Quiter, ?resonances on nuclear safeguards measurements will be

Quiter, Brian

2013-01-01T23:59:59.000Z

144

Extraction of uranium from spent fuels using liquefied gases  

SciTech Connect (OSTI)

For reprocessing of spent nuclear fuels, a novel method to extract actinides from spent fuel using highly compressed gases, nitrogen dioxide and carbon dioxide was proposed. As a fundamental study, the nitrate conversion with liquefied nitrogen dioxide and the nitrate extraction with supercritical carbon dioxide were demonstrated by using uranium dioxide powder, uranyl nitrate and tri-n-butylphosphate complex in the present study. (authors)

Sawada, Kayo; Hirabayashi, Daisuke; Enokida, Youichi [EcoTopia Science Institute, Nagoya University, Furo-cho, Chikusa-ku, Nagoya, 464-8603 (Japan)

2007-07-01T23:59:59.000Z

145

Conditioning of spent nuclear fuel for permanent disposal  

SciTech Connect (OSTI)

A compact, efficient method for conditioning spent nuclear fuel is under development. This method, known as pyrochemical processing, or pyroprocessing, provides a separation of fission products from the actinide elements present in spent fuel and further separates pure uranium from the transuranic elements. The process can facilitate the timely and environmentally-sound treatment of the highly diverse collection of spent fuel currently in the inventory of the US Department of Energy (DOE). The pyroprocess utilizes elevated-temperature processes to prepare spent fuel for fission product separation; that separation is accomplished by a molten salt electrorefining step that provides efficient (> 99.9%) separation of transuranics. The resultant waste forms from the pyroprocess are stable under envisioned repository environment conditions and highly leach-resistant. Treatment of any spent fuel type produces a set of common high-level waste forms, one a mineral and the other a metal alloy, that can be readily qualified for repository disposal and that avoid the substantial costs that would be associated with the qualification of the numerous spent fuel types included in the DOE inventory.

Laidler, J.J. [Argonne National Lab., IL (United States). Chemical Technology Div.

1994-12-31T23:59:59.000Z

146

Conditioning of spent nuclear fuel for permanent disposal  

SciTech Connect (OSTI)

A compact, efficient method for conditioning spent nuclear fuel is under development This method, known as pyrochemical processing, or {open_quotes}pyroprocessing,{close_quotes} provides a separation of fission products from the actinide elements present in spent fuel and further separates pure uranium from the transuranic elements. The process can facilitate the timely and environmentally-sound treatment of the highly diverse collection of spent fuel currently in the inventory of the United States Department of Energy (DOE). The pyroprocess utilizes elevated-temperature processes to prepare spent fuel for fission product separation; that separation is accomplished by a molten salt electrorefining step that provides efficient (99.9%) separation of transuranics. The resultant waste forms from the pyroprocess are stable under envisioned repository environment conditions and highly leach-resistant. Treatment of any spent fuel type produces a set of common high-level waste forms, one a mineral and the other a metal alloy, that can be readily qualified for repository disposal and preclude the substantial costs that would be associated with the qualification of the numerous spent fuel types included in the DOE inventory.

Laidler, J.J.

1994-10-01T23:59:59.000Z

147

Thermal analysis for fuel handling system for sodium cooled reactor considering minor actinide-bearing metal fuel.  

SciTech Connect (OSTI)

The Advanced Burner Reactor (ABR) is one of the components of the Global Nuclear Energy Partnership (GNEP) used to close the fuel cycle. ABR is a sodium-cooled fast reactor that is used to consume transuranic elements resulting from the reprocessing of light water reactor spent nuclear fuel. ABR-1000 [1000 MW(thermal)] is a fast reactor concept created at Argonne National Laboratory to be used as a reference concept for various future trade-offs. ABR-1000 meets the GNEP goals although it uses what is considered base sodium fast reactor technology for its systems and components. One of the considerations of any fast reactor plant concept is the ability to perform fuel-handling operations with new and spent fast reactor fuel. The transmutation fuel proposed as the ABR fuel has a very little experience base, and thus, this paper investigates a fuel-handling concept and potential issues of handling fast reactor fuel containing minor actinides. In this study, two thermal analyses supporting a conceptual design study on the ABR-1000 fuel-handling system were carried out. One analysis investigated passive dry spent fuel storage, and the other analysis investigated a fresh fuel shipping cask. Passive dry storage can be made suitable for the ABR-1000 spent fuel storage with sodium-bonded metal fuel. The thermal analysis shows that spent fast reactor fuel with a decay heat of 2 kW or less can be stored passively in a helium atmosphere. The 2-kW value seems to be a reasonable and practical level, and a combination of reasonably-sized in-sodium storage followed by passive dry storage could be a candidate for spent fuel storage for the next-generation sodium-cooled reactor with sodium-bonded metal fuel. Requirements for the shipping casks for minor actinide-bearing fuel with a high decay heat level are also discussed in this paper. The shipping cask for fresh sodium-cooled-reactor fuel should be a dry type to reduce the reaction between residual moisture on fresh fuel and the sodium coolant. The cladding temperature requirement is maintained below the creep temperature limit to avoid any damage before core installation. The thermal analysis shows that a helium gas-filled cask can accommodate ABR-1000 fresh minor actinide-bearing fuel with 700-W decay heat. The above analysis results revealed the overall requirement for minor actinide-bearing metal fuel handling. The information is thought to be helpful in the design of the ABR-1000 and future sodium-cooled-reactor fuel-handling system.

Chikazawa, Y.; Grandy, C.; Nuclear Engineering Division

2009-03-01T23:59:59.000Z

148

President Reagan Calls for a National Spent Fuel Storage Facility |  

National Nuclear Security Administration (NNSA)

Reagan Calls for a National Spent Fuel Storage Facility | Reagan Calls for a National Spent Fuel Storage Facility | National Nuclear Security Administration Our Mission Managing the Stockpile Preventing Proliferation Powering the Nuclear Navy Emergency Response Recapitalizing Our Infrastructure Continuing Management Reform Countering Nuclear Terrorism About Us Our Programs Our History Who We Are Our Leadership Our Locations Budget Our Operations Media Room Congressional Testimony Fact Sheets Newsletters Press Releases Speeches Events Social Media Video Gallery Photo Gallery NNSA Archive Federal Employment Apply for Our Jobs Our Jobs Working at NNSA Blog Home > About Us > Our History > NNSA Timeline > President Reagan Calls for a National Spent ... President Reagan Calls for a National Spent Fuel Storage Facility October 08, 1981

149

Dry storage of spent nuclear fuel in UAE – Economic aspect  

Science Journals Connector (OSTI)

Abstract Cost analysis of dry storage of spent nuclear fuel (SNF) discharged from Barakah nuclear power plants in the UAE was performed using three variables: average fuel discharge rate (FD), discount rate (d), and cooling time in a spent fuel pool (Tcool). The costs of dry storage as an interim spent fuel storage option in the UAE were estimated and compared between the following two scenarios: Scenario 1 is ‘accelerated transfer of spent fuel to dry storage’ that SNF will be transferred to dry storage facilities as soon as spent fuel has been sufficiently cooled down in a pool for the dry storage; Scenario 2 is defined as ‘maximum use of spent fuel pool’ that SNF will be stored in a pool as long as possible till the amount of stored SNF in the pool reaches the capacity of the pools and, then, to be moved to dry storage. A sensitivity analysis on the costs was performed and multiple regression analysis was applied to the resulting net present values (NPVs) for Scenarios 1 and 2 and ?NPV that is difference in the net present values between the two scenarios. The results showed that \\{NPVs\\} and ?NPV could be approximately expressed by single equations with the three variables. Among the three variables, the discount rate had the largest effect on the \\{NPVs\\} of the dry storage costs. However, ?NPV was turned out to be equally sensitive to the discount rate and cooling period. Over the ranges of the variables, the additional cost for accelerated fuel transfer (Scenario 1) ranged from 86.4 to 212.9 million $. Calculated using the maximum difference (212.9 M$) between the two scenarios, the accelerated fuel transfer to dry storage could incur the additional electricity rate 8.0 × 10?5 USD/kWh, which is not considered to be significant, compared to the overall electricity generation cost.

Sara Al Saadi; Yongsun Yi

2015-01-01T23:59:59.000Z

150

Nuclear Forensics Attributing the Source of Spent Fuel Used in an RDD Event  

SciTech Connect (OSTI)

An RDD attack against the U.S. is something America needs to prepare against. If such an event occurs the ability to quickly identify the source of the radiological material used in an RDD would aid investigators in identifying the perpetrators. Spent fuel is one of the most dangerous possible radiological sources for an RDD. In this work, a forensics methodology was developed and implemented to attribute spent fuel to a source reactor. The specific attributes determined are the spent fuel burnup, age from discharge, reactor type, and initial fuel enrichment. It is shown that by analyzing the post-event material, these attributes can be determined with enough accuracy to be useful for investigators. The burnup can be found within a 5% accuracy, enrichment with a 2% accuracy, and age with a 10% accuracy. Reactor type can be determined if specific nuclides are measured. The methodology developed was implemented into a code call NEMASYS. NEMASYS is easy to use and it takes a minimum amount of time to learn its basic functions. It will process data within a few minutes and provide detailed information about the results and conclusions.

M.R. Scott

2005-06-01T23:59:59.000Z

151

Nuclear Regulatory Commission's Integrated Strategy for Spent Fuel Management  

Broader source: Energy.gov (indexed) [DOE]

NRC's NRC's Integrated Strategy for NRC s Integrated Strategy for Spent Fuel Management Earl Easton 1 U.S. Nuclear Regulatory Commission May 25, 2010 Road to Yucca Mountain * 20+ years of preparation for the licensing i review * DOE application received in June 2008 and accepted for review in September 2008 * President Obama pursues alternatives to Yucca Mountain * DOE motion to withdraw in March 2010 2 * DOE motion to withdraw in March 2010 * Blue Ribbon Commission on America's Nuclear Future 2 Growing Spent Fuel Inventory Cumulative Used Nuclear Fuel Scenarios 50,000 100,000 150,000 200,000 250,000 Metric Tons 3 - 50,000 2010 2015 2020 2025 2030 2035 2040 2045 2050 Year Reference: Crozat, March 2010 Integrated Strategy * In response to the evolving national debate on spent fuel management strategy, NRC initiated a number of actions:

152

THE ECONOMICS OF REPROCESSING vs DIRECT DISPOSAL OF SPENT NUCLEAR FUEL  

SciTech Connect (OSTI)

This report assesses the economics of reprocessing versus direct disposal of spent nuclear fuel. The breakeven uranium price at which reprocessing spent nuclear fuel from existing light-water reactors (LWRs) and recycling the resulting plutonium and uranium in LWRs would become economic is assessed, using central estimates of the costs of different elements of the nuclear fuel cycle (and other fuel cycle input parameters), for a wide range of range of potential reprocessing prices. Sensitivity analysis is performed, showing that the conclusions reached are robust across a wide range of input parameters. The contribution of direct disposal or reprocessing and recycling to electricity cost is also assessed. The choice of particular central estimates and ranges for the input parameters of the fuel cycle model is justified through a review of the relevant literature. The impact of different fuel cycle approaches on the volume needed for geologic repositories is briefly discussed, as are the issues surrounding the possibility of performing separations and transmutation on spent nuclear fuel to reduce the need for additional repositories. A similar analysis is then performed of the breakeven uranium price at which deploying fast neutron breeder reactors would become competitive compared with a once-through fuel cycle in LWRs, for a range of possible differences in capital cost between LWRs and fast neutron reactors. Sensitivity analysis is again provided, as are an analysis of the contribution to electricity cost, and a justification of the choices of central estimates and ranges for the input parameters. The equations used in the economic model are derived and explained in an appendix. Another appendix assesses the quantities of uranium likely to be recoverable worldwide in the future at a range of different possible future prices.

Matthew Bunn; Steve Fetter; John P. Holdren; Bob van der Zwaan

2003-07-01T23:59:59.000Z

153

Spent fuel sabotage aerosol test program :FY 2005-06 testing and aerosol data summary.  

SciTech Connect (OSTI)

This multinational, multi-phase spent fuel sabotage test program is quantifying the aerosol particles produced when the products of a high energy density device (HEDD) interact with and explosively particulate test rodlets that contain pellets of either surrogate materials or actual spent fuel. This program has been underway for several years. This program provides source-term data that are relevant to some sabotage scenarios in relation to spent fuel transport and storage casks, and associated risk assessments. This document focuses on an updated description of the test program and test components for all work and plans made, or revised, primarily during FY 2005 and about the first two-thirds of FY 2006. It also serves as a program status report as of the end of May 2006. We provide details on the significant findings on aerosol results and observations from the recently completed Phase 2 surrogate material tests using cerium oxide ceramic pellets in test rodlets plus non-radioactive fission product dopants. Results include: respirable fractions produced; amounts, nuclide content, and produced particle size distributions and morphology; status on determination of the spent fuel ratio, SFR (the ratio of respirable particles from real spent fuel/respirables from surrogate spent fuel, measured under closely matched test conditions, in a contained test chamber); and, measurements of enhanced volatile fission product species sorption onto respirable particles. We discuss progress and results for the first three, recently performed Phase 3 tests using depleted uranium oxide, DUO{sub 2}, test rodlets. We will also review the status of preparations and the final Phase 4 tests in this program, using short rodlets containing actual spent fuel from U.S. PWR reactors, with both high- and lower-burnup fuel. These data plus testing results and design are tailored to support and guide, follow-on computer modeling of aerosol dispersal hazards and radiological consequence assessments. This spent fuel sabotage--aerosol test program, performed primarily at Sandia National Laboratories, with support provided by both the U.S. Department of Energy and the Nuclear Regulatory Commission, had significant inputs from, and is strongly supported and coordinated by both the U.S. and international program participants in Germany, France, and the U.K., as part of the international Working Group for Sabotage Concerns of Transport and Storage Casks, WGSTSC.

Gregson, Michael Warren; Brockmann, John E.; Nolte, O. (Fraunhofer institut fur toxikologie und experimentelle Medizin, Germany); Loiseau, O. (Institut de radioprotection et de Surete Nucleaire, France); Koch, W. (Fraunhofer institut fur toxikologie und experimentelle Medizin, Germany); Molecke, Martin Alan; Autrusson, Bruno (Institut de radioprotection et de Surete Nucleaire, France); Pretzsch, Gunter Guido (Gesellschaft fur anlagen- und Reaktorsicherheit, Germany); Billone, M. C. (Argonne National Laboratory, USA); Lucero, Daniel A.; Burtseva, T. (Argonne National Laboratory, USA); Brucher, W (Gesellschaft fur anlagen- und Reaktorsicherheit, Germany); Steyskal, Michele D.

2006-10-01T23:59:59.000Z

154

Information handbook on independent spent fuel storage installations  

SciTech Connect (OSTI)

In this information handbook, the staff of the U.S. Nuclear Regulatory Commission describes (1) background information regarding the licensing and history of independent spent fuel storage installations (ISFSIs), (2) a discussion of the licensing process, (3) a description of all currently approved or certified models of dry cask storage systems (DCSSs), and (4) a description of sites currently storing spent fuel in an ISFSI. Storage of spent fuel at ISFSIs must be in accordance with the provisions of 10 CFR Part 72. The staff has provided this handbook for information purposes only. The accuracy of any information herein is not guaranteed. For verification or for more details, the reader should refer to the respective docket files for each DCSS and ISFSI site. The information in this handbook is current as of September 1, 1996.

Raddatz, M.G.; Waters, M.D.

1996-12-01T23:59:59.000Z

155

Spent fuel and radioactive waste inventories, projections, and characteristics  

SciTech Connect (OSTI)

Current inventories and characteristics of commercial spent fuels and both commercial and US Department of Energy (DOE) radioactive wastes were compiled through December 31, 1983, based on the most reliable information available from government sources and the open literature, technical reports, and direct contacts. Future waste and spent fuel to be generated over the next 37 years and characteristics of these materials are also presented, consistent with the latest DOE/Energy Information Administration (EIA) or projection of US commercial nuclear power growth and expected defense-related and private industrial and institutional activities. Materials considered, on a chapter-by-chapter basis, are: spent fuel, high-level waste, transuranic waste, low-level waste, commercial uranium mill tailings, airborne waste, remedial action waste, and decommissioning waste. For each category, current and projected inventories are given through the year 2020, and the radioactivity and thermal power are calculated, based on reported or calculated isotopic compositions. 48 figures, 107 tables.

Not Available

1984-09-01T23:59:59.000Z

156

Proliferation resistance of small modular reactors fuels  

SciTech Connect (OSTI)

In this paper the proliferation resistance of different types of Small Modular Reactors (SMRs) has been examined and classified with criteria available in the literature. In the first part of the study, the level of proliferation attractiveness of traditional low-enriched UO{sub 2} and MOX fuels to be used in SMRs based on pressurized water technology has been analyzed. On the basis of numerical simulations both cores show significant proliferation risks. Although the MOX core is less proliferation prone in comparison to the UO{sub 2} core, it still can be highly attractive for diversion or undeclared production of nuclear material. In the second part of the paper, calculations to assess the proliferation attractiveness of fuel in typical small sodium cooled fast reactor show that proliferation risks from spent fuel cannot be neglected. The core contains a highly attractive plutonium composition during the whole life cycle. Despite some aspects of the design like the sealed core that enables easy detection of unauthorized withdrawal of fissile material and enhances proliferation resistance, in case of open Non-Proliferation Treaty break-out, weapon-grade plutonium in sufficient quantities could be extracted from the reactor core.

Polidoro, F.; Parozzi, F. [RSE - Ricerca sul Sistema Energetico,Via Rubattino 54, 20134, Milano (Italy); Fassnacht, F.; Kuett, M.; Englert, M. [IANUS, Darmstadt University of Technology, Alexanderstr. 35, D-64283 Darmstadt (Germany)

2013-07-01T23:59:59.000Z

157

New Fuel Cycle and Fuel Management Options in Heavy Liquid Metal-Cooled Reactors  

Science Journals Connector (OSTI)

Technical Paper / Advances in Nuclear Fuel Management - Fuel Management of Reactors Other Than Light Water Reactors

Ehud Greenspan; Pavel Hejzlar; Hiroshi Sekimoto; Georgy Toshinsky; David Wade

158

Spent fuel dissolution studies FY 1991 to 1994  

SciTech Connect (OSTI)

Dissolution and transport as a result of groundwater flow are generally accepted as the primary mechanisms by which radionuclides from spent fuel placed in a geologic repository could be released to the biosphere. To help provide a source term for performance assessment calculations, dissolution studies on spent fuel and unirradiated uranium oxides have been conducted over the past few years at Pacific Northwest National Laboratory (PNNL) in support of the Yucca Mountain Site Characterization Project. This report describes work for fiscal years 1991 through 1994. The objectives of these studies and the associated conclusions, which were based on the limited number of tests conducted so far, are described in the following subsections.

Gray, W.J.; Wilson, C.N.

1995-12-01T23:59:59.000Z

159

Initial measurements of BN-350 spent fuel in dry storage casks using the dual slab verification detonator  

SciTech Connect (OSTI)

The Dual Slab Verification Detector (DSVD) has been developed, built, and characterized by Los Alamos National Laboratory in cooperation with the International Atomic Energy Agency (IAEA) as part of the dry storage safeguards system for the spent fuel from the BN-350 fast reactor. The detector consists of two rows of 3He tubes embedded in a slab of polyethylene which has been designed to be placed on the outer surface of the dry storage cask. By performing DSVD measurements at several different locations around the outer surface of the DUC, a signature 'fingerprint' can be established for each DUC based on the neutron flux emanating from inside the dry storage cask. The neutron fingerprint for each individual DUC will be dependent upon the spatial distribution of nuclear material within the cask, thus making it sensitive to the removal of a certain amount of material from the cask. An initial set of DSVD measurements have been performed on the first set of dry storage casks that have been loaded with canisters of spent fuel and moved onto the dry storage pad to both establish an initial fingerprint for these casks as well as to quantify systematic uncertainties associated with these measurements. The results from these measurements will be presented and compared with the expected results that were determined based on MCNPX simulations of the dry storage facility. The ability to safeguard spent nuclear fuel is strongly dependent on the technical capabilities of establishing and maintaining continuity of knowledge (COK) of the spent fuel as it is released from the reactor core and either reprocessed or packaged and stored at a storage facility. While the maintenance of COK is often done using continuous containment and surveillance (C/S) on the spent fuel, it is important that the measurement capabilities exist to re-establish the COK in the event of a significant gap in the continuous CIS by performing measurements that independently confirm the presence and content of Plutonium (Pu) in the spent fuel. The types of non-destructive assay (NDA) measurements that can be performed on the spent fuel are strongly dependent on the type of spent fuel that is being safeguarded as well as the location in which the spent fuel is being stored. The BN-350 Spent Fuel Disposition Project was initiated to improve the safeguards and security of the spent nuclear fuel from the BN-350 fast-breeder reactor and was developed cooperatively to meet the requirements of the International Atomic Energy Agency (IAEA) as well as the terms of the 1993 CTR and MPC&A Implementing Agreements. The unique characteristics of fuel from the BN-350 fast-breeder reactor have allowed for the development of an integrated safeguards measurement program to inventory, monitor, and if necessary, re-verify Pu content of the spent fuel throughout the lifetime of the project. This approach includes the development of a safeguards measurement program to establish and maintain the COK on the spent fuel during the repackaging and eventual relocation of the spent-fuel assemblies to a long-term storage site. As part of the safeguards measurement program, the Pu content of every spent-fuel assembly from the BN-350 reactor was directly measured and characterized while the spent-fuel assemblies were being stored in the spent-fuel pond at the BN-350 facility using the Spent Fuel Coincidence Counter (SFCC). Upon completion of the initial inventory of the Pu content of the individual spent-fuel assemblies, the assemblies were repackaged into welded steel canisters that were filled with inert argon gas and held either four or six individual spent-fuel assemblies depending on the type of assembly that was being packaged. This repackaging of the spent-fuel assemblies was performed in order to improve the stability of the spent-fuel assemblies for long-term storage and increase the proliferation resistance of the spent fuel. To maintain the capability of verifying the presence of the spent-fuel assemblies inside the welded steel canisters, measurements were performed on the canis

Santi, Peter Angelo [Los Alamos National Laboratory; Browne, Michael C [Los Alamos National Laboratory; Freeman, Corey R [Los Alamos National Laboratory; Parker, Robert F [Los Alamos National Laboratory; Williams, Richard B [Los Alamos National Laboratory

2010-01-01T23:59:59.000Z

160

Predictions of dry storage behavior of zircaloy clad spent fuel rods using deformation and fracture map analyses  

SciTech Connect (OSTI)

Predictions of the maximum initial allowable temperature required to achieve a 40-year life in dry storage are made for Zircaloy clad spent fuel. Maximum initial dry storage temperatures of 420/sup 0/C for 1 year fuel cladding subjected to a constant stress of 70 MPa are predicted. The technique utilized in this work is based on the deformation and fracture map methodology. Maps are presented for temperatures between 50 and 850/sup 0/C stresses between 5 and 500 MPa. These maps are combined with a life fraction rule to predict the time to rupture of Zircaloy clad spent Light Water Reactor (LWR) fuel subjected to various storage conditions.

Tarn, J.C.L.; Madsen, N.H.; Chin, B.A.

1986-03-01T23:59:59.000Z

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


161

A Parametric Study of the DUPIC Fuel Cycle to Reflect Pressurized Water Reactor Fuel Management Strategy  

SciTech Connect (OSTI)

For both pressurized water reactor (PWR) and Canada deuterium uranium (CANDU) tandem analysis, the Direct Use of spent PWR fuel In CANDU reactor (DUPIC) fuel cycle in a CANDU 6 reactor is studied using the DRAGON/DONJON chain of codes with the ENDF/B-V and ENDF/B-VI libraries. The reference feed material is a 17 x 17 French standard 900-MW(electric) PWR fuel. The PWR spent-fuel composition is obtained from two-dimensional DRAGON assembly transport and depletion calculations. After a number of years of cooling, this defines the initial fuel nuclide field in the CANDU unit cell calculations in DRAGON, where it is further depleted with the same neutron group structure. The resulting macroscopic cross sections are condensed and tabulated to be used in a full-core model of a CANDU 6 reactor to find an optimized channel fueling rate distribution on a time-average basis. Assuming equilibrium refueling conditions and a particular refueling sequence, instantaneous full-core diffusion calculations are finally performed with the DONJON code, from which both the channel power peaking factors and local parameter effects are estimated. A generic study of the DUPIC fuel cycle is carried out using the linear reactivity model for initial enrichments ranging from 3.2 to 4.5 wt% in a PWR. Because of the uneven power histories of the spent PWR assemblies, the spent PWR fuel composition is expected to differ from one assembly to the next. Uneven mixing of the powder during DUPIC fuel fabrication may lead to uncertainties in the composition of the fuel bundle and larger peaking factors in CANDU. A mixing method for reducing composition uncertainties is discussed.

Rozon, Daniel; Shen Wei [Institut de Genie Nucleaire (Canada)

2001-05-15T23:59:59.000Z

162

Plutonium and Reprocessing of Spent Nuclear Fuel  

Science Journals Connector (OSTI)

...might spawn nuclear terrorism. Less than...reprocessing plant. The U.S. nuclear-energy...current fleet of power reactors (15...operational risk of transmutation...future of nuclear power is clarified...constructed plant increased...

Frank N. von Hippel

2001-09-28T23:59:59.000Z

163

Gamma Ray Mirrors for Direct Measurement of Spent Nuclear Fuel  

SciTech Connect (OSTI)

Direct measurement of the amount of Pu and U in spent nuclear fuel represents a challenge for the safeguards community. Ideally, the characteristic gamma-ray emission lines from different isotopes provide an observable suitable for this task. However, these lines are generally lost in the fierce flux of radiation emitted by the fuel. The rates are so high that detector dead times limit measurements to only very small solid angles of the fuel. Only through the use of carefully designed view ports and long dwell times are such measurements possible. Recent advances in multilayer grazing-incidence gamma-ray optics provide one possible means of overcoming this difficulty. With a proper optical and coating design, such optics can serve as a notch filter, passing only narrow regions of the overall spectrum to a fully shielded detector that does not view the spent fuel directly. We report on the design of a mirror system and a number of experimental measurements.

Pivovaroff, Dr. Michael J. [Lawrence Livermore National Laboratory (LLNL)] [Lawrence Livermore National Laboratory (LLNL); Ziock, Klaus-Peter [ORNL] [ORNL; Harrison, Mark J [ORNL] [ORNL; Soufli, Regina [Lawrence Livermore National Laboratory (LLNL)] [Lawrence Livermore National Laboratory (LLNL)

2014-01-01T23:59:59.000Z

164

MANAGEMENT OF SPENT NUCLEAR FUEL IN FINLAND: POLICY, PAST AND PRESENT PRACTICES, PLANS FOR THE FUTURE  

Science Journals Connector (OSTI)

In Finland, about 1700 tU of spent nuclear fuel has arisen from the operation of the four nuclear power units which were commissioned in late ... 1980’s. Initially the spent fuel management policy was based on se...

E. RUOKOLA

2006-01-01T23:59:59.000Z

165

What to Expect When Readying to Move Spent Nuclear Fuel from...  

Broader source: Energy.gov (indexed) [DOE]

What to Expect When Readying to Move Spent Nuclear Fuel from Commercial Nuclear Power Plants What to Expect When Readying to Move Spent Nuclear Fuel from Commercial Nuclear Power...

166

Locations of Spent Nuclear Fuel and High-Level Radioactive Waste...  

Broader source: Energy.gov (indexed) [DOE]

Locations of Spent Nuclear Fuel and High-Level Radioactive Waste Locations of Spent Nuclear Fuel and High-Level Radioactive Waste Map of the United States of America showing the...

167

Microscopic Examination of a Corrosion Front in Spent Nuclear Fuel  

SciTech Connect (OSTI)

Spent uranium oxide nuclear fuel hosts a variety of trace chemical constituents, many of which must be sequestered from the biosphere during fuel storage and disposal. In this paper we present synchrotron x-ray absorption spectroscopy and microscopy findings that illuminate the resultant local chemistry of neptunium and plutonium within spent uranium oxide nuclear fuel before and after corrosive alteration in an air-saturated aqueous environment. We find the plutonium and neptunium in unaltered spent fuel to have a +4 oxidation state and an environment consistent with solid-solution in the UO{sub 2} matrix. During corrosion in an air-saturated aqueous environment, the uranium matrix is converted to uranyl U(VI)O{sub 2}{sup 2+} mineral assemblage that is depleted in plutonium and neptunium relative to the parent fuel. At the corrosion front interface between intact fuel and the uranyl-mineral corrosion layer, we find evidence of a thin ({approx}20 micrometer) layer that is enriched in plutonium and neptunium within a predominantly U{sup 4+} environment. Available data for the standard reduction potentials for NpO{sup 2+}/Np{sup 4+} and UO{sub 2}{sup 2+}/U{sup 4+} couples indicate that Np(IV) may not be effectively oxidized to Np(V) at the corrosion potentials of uranium dioxide spent nuclear fuel in air-saturated aqueous solutions. Neptunium is an important radionuclide in dose contribution according to performance assessment models of the proposed U. S. repository at Yucca Mountain, Nevada. A scientific understanding of how the UO{sub 2} matrix of spent nuclear fuel impacts the oxidative dissolution and reductive precipitation of neptunium is needed to predict its behavior at the fuel surface during aqueous corrosion. Neptunium would most likely be transported as aqueous Np(V) species, but for this to occur it must first be oxidized from the Np(IV) state found within the parent spent nuclear fuel [1]. In the immediate vicinity of the spent fuel's surface the redox and nucleation behavior is likely to promote/enhance nucleation of NpO{sub 2} and Np{sub 2}O{sub 5}. Alternatively, Np may be incorporated into uranyl (UO{sub 2}{sup 2+}) alteration phases [2]. In some cases, less-soluble elements such as plutonium will be enriched near the surface of the corroding fuel [3]. We have used focused synchrotron x-rays from the MRCAT beam line at the Advanced Photon Source (APS) at Argonne National Lab to examine a specimen of spent nuclear fuel that had been subject to 10 years of corrosion testing in an environment of humid air and dripping groundwater at 90 C [4]. We find evidence of a region, approximately 20 microns in thickness, enriched in plutonium and neptunium at the corrosion front that exists between the uranyl silicate alteration mineral rind and the unaltered uranium oxide fuel (Figures 1 and 2). The uranyl silicate is itself found to be depleted in these transuranic elements relative to their abundance relative to uranium in the parent fuel. This suggests a low mobility of these components owing to a resistance to oxidize further in the presence of a UO{sub 2}{sup 2+}/U{sup 4+} couple [5].

J.A> Fortner; A.J. Kropf; R.J. Finch; J.C. Cunnane

2006-06-20T23:59:59.000Z

168

Zircaloy cladding: Tough Containment for Spent Fuel Storage  

SciTech Connect (OSTI)

The present work leads us to strongly believe that if the cladding temperature is held below 425/sup 0/C then the cladding provides a significant barrier against radionuclide migration for over 1000 years. Unless some alternative benefit is identified, we feel that steps should be taken to preserve the integrity of the Zircaloy cladding - Tough Containment for Spent Fuel Storage.

Einziger, R.E.; Bosi, D.M.; Miller, A.K.

1981-01-01T23:59:59.000Z

169

Spent fuel sabotage test program, characterization of aerosol dispersal : interim final report.  

SciTech Connect (OSTI)

This multinational, multi-phase spent fuel sabotage test program is quantifying the aerosol particles produced when the products of a high energy density device (HEDD) interact with and explosively particulate test rodlets that contain pellets of either surrogate materials or actual spent fuel. This program provides source-term data that are relevant to plausible sabotage scenarios in relation to spent fuel transport and storage casks and associated risk assessments. We present details and significant results obtained from this program from 2001 through 2007. Measured aerosol results include: respirable fractions produced; amounts, nuclide content, and produced particle size distributions and morphology; measurements of volatile fission product species enhanced sorption--enrichment factors onto respirable particles; and, status on determination of the spent fuel ratio, SFR, needed for scaling studies. Emphasis is provided on recent Phase 3 tests using depleted uranium oxide pellets plus non-radioactive fission product dopants in surrogate spent fuel test rodlets, plus the latest surrogate cerium oxide results and aerosol laboratory supporting calibration work. The DUO{sub 2}, CeO{sub 2}, plus fission product dopant aerosol particle results are compared with available historical data. We also provide a status review on continuing preparations for the final Phase 4 in this program, tests using individual short rodlets containing actual spent fuel from U.S. PWR reactors, with both high- and lower-burnup fuel. The source-term data, aerosol results, and program design have been tailored to support and guide follow-on computer modeling of aerosol dispersal hazards and radiological consequence assessments. This spent fuel sabotage, aerosol test program was performed primarily at Sandia National Laboratories, with support provided by both the U.S. Department of Energy and the Nuclear Regulatory Commission. This program has significant input from, and is cooperatively supported and coordinated by both the U.S. and international program participants in Germany, France, and others, as part of the International Working Group for Sabotage Concerns of Transport and Storage Casks (WGSTSC).

Gregson, Michael Warren; Brockmann, John E.; Loiseau, Olivier (Institut de Radioprotection et de Surete Nucleaire, France); Klennert, Lindsay A.; Nolte, Oliver (Fraunhofer Institut fur Toxikologie und Experimentelle Medizin, Germany); Molecke, Martin Alan; Autrusson, Bruno A. (Institut de Radioprotection et de Surete Nucleaire, France); Koch, Wolfgang (Fraunhofer Institut fur Toxikologie und Experimentelle Medizin, Germany); Pretzsch, Gunter Guido (Gesellschaft fur Anlagen- und Reaktorsicherheit, Germany); Brucher, Wenzel (Gesellschaft fur Anlagen- und Reaktorsicherheit, Germany); Steyskal, Michele D.

2008-03-01T23:59:59.000Z

170

Ceramic-composite waste forms from the electrometallurgical treatment of spent nuclear fuel  

Science Journals Connector (OSTI)

Argonne National Laboratory is developing a method to treat spent nuclear fuel in a molten-salt electrorefiner. Glass...

C. Pereira; M. Hash; M. Lewis; M. Richmann

1997-07-01T23:59:59.000Z

171

Evaluation of Effect of Fuel Assembly Loading Patterns on Thermal and Shielding Performance of a Spent Fuel Storage/Transportation Cask  

SciTech Connect (OSTI)

The licensing of spent fuel storage casks is generally based on conservative analyses that assume a storage system being uniformly loaded with design basis fuel. The design basis fuel typically assumes a maximum assembly enrichment, maximum burn up, and minimum cooling time. These conditions set the maximum decay heat loads and radioactive source terms for the design. Recognizing that reactor spent fuel pools hold spent fuel with an array of initial enrichments, burners, and cooling times, this study was performed to evaluate the effect of load pattern on peak cladding temperature and cask surface dose rate. Based on the analysis, the authors concluded that load patterns could be used to reduce peak cladding temperatures in a cask without adversely impacting the surface dose rates.

Cuta, Judith M.; Jenquin, Urban P.; McKinnon, Mikal A.

2001-11-20T23:59:59.000Z

172

Alternate-fuel reactor studies  

SciTech Connect (OSTI)

A number of studies related to improvements and/or greater understanding of alternate-fueled reactors is presented. These studies cover the areas of non-Maxwellian distributions, materials and lifetime analysis, a /sup 3/He-breeding blanket, tritium-rich startup effects, high field magnet support, and reactor operation spanning the range from full D-T operation to operation with no tritium breeding.

Evans, K. Jr.; Ehst, D.A.; Gohar, Y.; Jung, J.; Mattas, R.F.; Turner, L.R.

1983-02-01T23:59:59.000Z

173

Further Evaluation of the Neutron Resonance Transmission Analysis (NRTA) Technique for Assaying Plutonium in Spent Fuel  

SciTech Connect (OSTI)

This is an end-of-year report (Fiscal Year (FY) 2011) for the second year of effort on a project funded by the National Nuclear Security Administration's Office of Nuclear Safeguards (NA-241). The goal of this project is to investigate the feasibility of using Neutron Resonance Transmission Analysis (NRTA) to assay plutonium in commercial light-water-reactor spent fuel. This project is part of a larger research effort within the Next-Generation Safeguards Initiative (NGSI) to evaluate methods for assaying plutonium in spent fuel, the Plutonium Assay Challenge. The second-year goals for this project included: (1) assessing the neutron source strength needed for the NRTA technique, (2) estimating count times, (3) assessing the effect of temperature on the transmitted signal, (4) estimating plutonium content in a spent fuel assembly, (5) providing a preliminary assessment of the neutron detectors, and (6) documenting this work in an end of the year report (this report). Research teams at Los Alamos National Laboratory (LANL), Lawrence Berkeley National Laboratory (LBNL), Pacific Northwest National Laboratory (PNNL), and at several universities are also working to investigate plutonium assay methods for spent-fuel safeguards. While the NRTA technique is well proven in the scientific literature for assaying individual spent fuel pins, it is a newcomer to the current NGSI efforts studying Pu assay method techniques having just started in March 2010; several analytical techniques have been under investigation within this program for two to three years or more. This report summarizes work performed over a nine month period from January-September 2011 and is to be considered a follow-on or add-on report to our previous published summary report from December 2010 (INL/EXT-10-20620).

J. W. Sterbentz; D. L. Chichester

2011-09-01T23:59:59.000Z

174

FY13 Summary Report on the Augmentation of the Spent Fuel Composition Dataset for Nuclear Forensics: SFCOMPO/NF  

SciTech Connect (OSTI)

This report documents the FY13 efforts to enhance a dataset of spent nuclear fuel isotopic composition data for use in developing intrinsic signatures for nuclear forensics. A review and collection of data from the open literature was performed in FY10. In FY11, the Spent Fuel COMPOsition (SFCOMPO) excel-based dataset for nuclear forensics (NF), SFCOMPO/NF was established and measured data for graphite production reactors, Boiling Water Reactors (BWRs) and Pressurized Water Reactors (PWRs) were added to the dataset and expanded to include a consistent set of data simulated by calculations. A test was performed to determine whether the SFCOMPO/NF dataset will be useful for the analysis and identification of reactor types from isotopic ratios observed in interdicted samples.

Brady Raap, Michaele C.; Lyons, Jennifer A.; Collins, Brian A.; Livingston, James V.

2014-03-31T23:59:59.000Z

175

Standard guide for drying behavior of spent nuclear fuel  

E-Print Network [OSTI]

1.1 This guide is organized to discuss the three major components of significance in the drying behavior of spent nuclear fuel: evaluating the need for drying, drying spent nuclear fuel, and confirmation of adequate dryness. 1.1.1 The guide addresses drying methods and their limitations in drying spent nuclear fuels that have been in storage at water pools. The guide discusses sources and forms of water that remain in SNF, its container, or both, after the drying process and discusses the importance and potential effects they may have on fuel integrity, and container materials. The effects of residual water are discussed mechanistically as a function of the container thermal and radiological environment to provide guidance on situations that may require extraordinary drying methods, specialized handling, or other treatments. 1.1.2 The basic issue in drying is to determine how dry the SNF must be in order to prevent issues with fuel retrievability, container pressurization, or container corrosion. Adequate d...

American Society for Testing and Materials. Philadelphia

2008-01-01T23:59:59.000Z

176

Proposed subcritical measurements for fresh and spent highly enriched plate type fuel assemblies  

SciTech Connect (OSTI)

A collaborative experimental research program has been established between industry and university partners to evaluate the subcritical behavior of fresh and spent highly enriched fuel assemblies at the University of Missouri Research Reactor (MURR). This proposed program will involve a series of subcritical measurements using the Oak Ridge National Laboratory (ORNL) developed {sup 252}Cf source-driven noise technique. Measurements evaluating the subcritical behavior of simple arrays of fresh MURR assemblies will be performed for evaluating the spectral effects of materials typically found in shipping casks such as lead, steel, aluminum, and boron. Also, measurements will be performed on spent assemblies to characterize physics parameters which may be useful in determining the subcritical behavior of fuels for reactivity credit of actinide burnup and fission product poisoning.

Zino, J.F.; Williamson, T.G. [Westinghouse Savannah River Company, Aiken, SC (United States); Mihalczo, J.T. [Oak Ridge National Lab., TN (United States)] [and others

1997-09-01T23:59:59.000Z

177

Uncanistered Spent Nuclear fuel Disposal Container System Description Document  

SciTech Connect (OSTI)

The Uncanistered Spent Nuclear Fuel (SNF) Disposal Container System supports the confinement and isolation of waste within the Engineered Barrier System of the Monitored Geologic Repository (MGR). Disposal containers are loaded with intact uncanistered assemblies and/or individually canistered SNF assemblies and sealed in the surface waste handling facilities, transferred to the underground through the access drifts, and emplaced in the emplacement drifts. The Uncanistered SNF Disposal Container provides long-term confinement of the commercial SNF placed inside, and withstands the loading, transfer, emplacement, and retrieval loads and environments. The Uncanistered SNF Disposal Container System provides containment of waste for a designated period of time, and limits radionuclide release. The disposal container maintains the waste in a designated configuration, withstands maximum handling and rockfall loads, limits the individual SNF assembly temperatures after emplacement, limits the introduction of moderator into the disposal container during the criticality control period, resists corrosion in the expected handling and repository environments, and provides containment of waste in the event of an accident. Multiple boiling water reactor (BWR) and pressurized water reactor (PWR) disposal container designs are needed to accommodate the expected range of spent fuel assemblies and provide long-term confinement of the commercial SNF. The disposal container will include outer and inner cylinder walls, outer cylinder lids (two on the top, one on the bottom), inner cylinder lids (one on the top, one on the bottom), and an internal metallic basket structure. Exterior labels will provide a means by which to identify the disposal container and its contents. The two metal cylinders, in combination with the cladding, Emplacement Drift System, drip shield, and natural barrier, will support the design philosophy of defense-in-depth. The use of materials with different properties prevents a single mode failure from breaching the waste package. The inner cylinder and inner cylinder lids will be constructed of stainless steel and the outer cylinder and outer cylinder lid will be made of high-nickel alloy. The basket will assist criticality control, provide structural support, and improve heat transfer. The Uncanistered SNF Disposal Container System interfaces with the emplacement drift environment and internal waste by transferring heat from the SNF to the external environment and by protecting the SFN assemblies and their contents from damage/degradation by the external environment. The system also interfaces with the SFN by limiting access of moderator and oxidizing agents of the SFN. The waste package interfaces with the Emplacement Drift System's emplacement drift pallets upon which the wasted packages are placed. The disposal container interfaces with the Assembly Transfer System, Waste Emplacement/Retrieval System, Disposal Container Handling System, and Waste Package Remediation System during loading, handling, transfer, emplacement and retrieval of the disposal container/waste package.

NONE

2000-10-12T23:59:59.000Z

178

Fate of Noble Metals during the Pyroprocessing of Spent Nuclear Fuel  

SciTech Connect (OSTI)

During the pyroprocessing of spent nuclear fuel by electrochemical techniques, fission products are separated as the fuel is oxidized at the anode and refined uranium is deposited at the cathode. Those fission products that are oxidized into the molten salt electrolyte are considered active metals while those that do not react are considered noble metals. The primary noble metals encountered during pyroprocessing are molybdenum, zirconium, ruthenium, rhodium, palladium, and technetium. Pyroprocessing of spent fuel to date has involved two distinctly different electrorefiner designs, in particular the anode to cathode configuration. For one electrorefiner, the anode and cathode collector are horizontally displaced such that uranium is transported across the electrolyte medium. As expected, the noble metal removal from the uranium during refining is very high, typically in excess of 99%. For the other electrorefiner, the anode and cathode collector are vertically collocated to maximize uranium throughput. This arrangement results in significantly less noble metals removal from the uranium during refining, typically no better than 20%. In addition to electrorefiner design, operating parameters can also influence the retention of noble metals, albeit at the cost of uranium recovery. Experiments performed to date have shown that as much as 100% of the noble metals can be retained by the cladding hulls while affecting the uranium recovery by only 6%. However, it is likely that commercial pyroprocessing of spent fuel will require the uranium recovery to be much closer to 100%. The above mentioned design and operational issues will likely be driven by the effects of noble metal contamination on fuel fabrication and performance. These effects will be presented in terms of thermal properties (expansion, conductivity, and fusion) and radioactivity considerations. Ultimately, the incorporation of minor amounts of noble metals from pyroprocessing into fast reactor metallic fuel will be shown to be of no consequence to reactor performance.

B.R. Westphal; D. Vaden; S.X. Li; G.L. Fredrickson; R.D. Mariani

2009-09-01T23:59:59.000Z

179

Accelerated Dissolution Process of the Spent Fuel (UO{sub 2}) under Repository Conditions  

SciTech Connect (OSTI)

Nowadays, nuclear energy is one of the options for developed countries in order to maintain the demand of electric energy. One of the key problems associated with kind of energy generation is the residual waste formed after a fuel cycle (spent nuclear fuel). The thermal treatment received in the reactor and there composition renders these materials very difficult to characterize and thus exhaustive studies are required to obtain knowledge that will help to build a complete, reliable and very safety underground facility. In this way, the option known as the Deep Geological Repository (DGR) is under development by each country taking part in the nuclear energy industry. The unique pathway for the migration to the biosphere of the radionuclide, actinide and lanthanides content in the spent fuel pellet (UO{sub 2}) after the closing of the deep geological repository is by a water transport phenomena. It is a fundamental question to know how much time they will spend on their trip and the first step is the rate of liberation of these radionuclides from the spent fuel pellet. In this way the matrix dissolution rate of the spent fuel pellet, which is not dependent on the specific surface area after normalization by the initial value is a key parameter to begin the performance assessment for any deep geological repository. The specific surface value is, following the Matrix Alteration Model (MAM) sensitivity analysis, one of the most important parameters controlling the radionuclides liberation. In this way, several measurements were carried out to obtain values in different conditions for different sieves of UO{sub 2} powder treated as fresh fuel. First of all, the specific surface area was measured with a multi-point isothermal procedure with N{sub 2} and Kr for both. The values obtained are presented in order to obtain a general law for the rate of evolution with the particle size. These data are part of a bigger project about the complete description of the spent fuel analogues, which are very useful for obtaining new dissolution rates for spent nuclear fuel under repository simulated conditions. (authors)

Iglesias, Eduardo; Quinones, Javier; Rodriguez, Nieves [Energy, CIEMAT, Avda. Complutense 22, Madrid, 28040 (Spain)

2008-07-01T23:59:59.000Z

180

Maximum Fuel Utilization in Advanced Fast Reactors without Actinides Separation  

E-Print Network [OSTI]

Oxford ; New York ; Oxford University Press. Fuel- Trac,Spent Fuel / Reprocessing, in Nuclear Industry Statusto Burn Non-Fissile Fuels. 2008. GA. Energy Multiplier

Heidet, Florent

2010-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


181

Integrated Data Base for 1989: Spent fuel and radioactive waste inventories, projections, and characteristics  

SciTech Connect (OSTI)

The Integrated Data Base (IDB) Program has compiled current data on inventories and characteristics of commercial spent fuel and both commercial and US government-owned radioactive wastes through December 31, 1988. These data are based on the most reliable information available from government sources, the open literature, technical reports, and direct contacts. The current projections of future waste and spent fuel to be generated through the year 2020 and characteristics of these materials are also presented. The information forecasted is consistent with the latest US Department of Energy/Energy Information Administration (DOE/EIA) projections of US commercial nuclear power growth and the expected defense-related and private industrial and institutional (I/I) activities. The radioactive materials considered, on a chapter-by-chapter basis, are spent fuel, high-level waste, transuranic waste, low-level waste, commercial uranium mill tailings, remedial action waste, commercial reactor and fuel cycle facility decommissioning waste, and mixed (hazardous and radioactive) low-level waste. For most of these categories, current and projected inventories are given through the year 2020, and the radioactivity and thermal power are calculated based on reported or estimated isotopic compositions. In addition, characteristics and current inventories are reported for miscellaneous, highly radioactive materials that may require geologic disposal. 45 figs., 119 tabs.

Not Available

1989-11-01T23:59:59.000Z

182

Integrated data base for 1990: US spent fuel and radioactive waste inventories, projections, and characteristics  

SciTech Connect (OSTI)

The Integrated Data Base (IDB) Program has compiled current data on inventories and characteristics of commercial spent fuel and both commercial and US government-owned radioactive wastes through December 31, 1989. These data are based on the most reliable information available from government sources, the open literature, technical reports, and direct contacts. The current projections of future waste and spent fuel to be generated through the year 2020 and characteristics of these materials are also presented. The information forecasted is consistent with the latest US Department of Energy/Energy Information Administration (DOE/EIA) projections of US commercial nuclear power growth and the expected DOE-related and private industrial and institutional (I/I) activities. The radioactive materials considered, on a chapter-by-chapter basis, are spent fuel, high-level waste, transuranic waste, low-level waste, commercial uranium mill tailings, environmental restoration wastes, commercial reactor and fuel cycle facility decommissioning wastes, and mixed (hazardous and radioactive) low-level waste. For most of these categories, current and projected inventories are given through the year 2020, and the radioactivity and thermal power are calculated based on reported or estimated isotopic compositions. In addition, characteristics and current inventories are reported for miscellaneous radioactive materials that may require geologic disposal. 22 refs., 48 figs., 109 tabs.

Not Available

1990-10-01T23:59:59.000Z

183

Spent-fuel pool thermal hydraulics: The evaporation question  

SciTech Connect (OSTI)

Many nuclear power plants are currently using dense fuel arrangements that increase the number of spent fuel elements stored in their spent-fuel pools (SFPs). The denser spent-fuel storage results in higher water temperatures, especially when certain event scenarios are analyzed. In some of these event scenarios, it is conservative to maximize the evaporation rate, while in other circumstances it is required to minimize the evaporation rates for conservatism. Evaporation is such a fundamental phenomenon that many branches of engineering developed various equations based on theory and experiments. The evaporation rates predicted by existing equations present a wide range of variation, especially at water temperatures >40{degrees}C. Furthermore, a study on which equations provide the highest and lowest evaporation rates has not been done until now. This study explores the sensitivity of existing evaporation equations to various parameters and recommends the limiting evaporation equations for use in the solution of SFP thermal problems. Note that the results of this study may be applicable to a much wider range of applications from irrigation ponds, cooling lakes, and liquid-waste management to calculating adequate air exchange rate for swimming pools and health spas.

Yilmaz, T.P. [Belcan Services, Lombard, IL (United States); Lai, J.C. [Public Service Electric & Gas Co., Berwick, PA (United States)

1996-12-31T23:59:59.000Z

184

EIS-0306: Treatment and Management of Sodium-Bonded Spent Nuclear Fuel |  

Broader source: Energy.gov (indexed) [DOE]

306: Treatment and Management of Sodium-Bonded Spent Nuclear 306: Treatment and Management of Sodium-Bonded Spent Nuclear Fuel EIS-0306: Treatment and Management of Sodium-Bonded Spent Nuclear Fuel Summary This EIS evaluates the potential environmental impacts of the proposed electrometallurgical treatment of DOE-owned sodium bonded spent nuclear fuel in the Fuel Conditioning Facility at Argonne National Laboratory-West (ANL-W). Public Comment Opportunities None available at this time. Documents Available for Download September 19, 2000 EIS-0306: Record of Decision Treatment and Management of Sodium-Bonded Spent Nuclear Fuel July 1, 2000 EIS-0306: Final Environmental Impact Statement Treatment and Management of Sodium-Bonded Spent Nuclear Fuel July 1, 1999 EIS-0306: Draft Environmental Impact Statement Treatment of Sodium-Bonded Spent Nuclear Fuel

185

Nuclear Waste Imaging and Spent Fuel Verification by Muon Tomography  

E-Print Network [OSTI]

This paper explores the use of cosmic ray muons to image the contents of shielded containers and detect high-Z special nuclear materials inside them. Cosmic ray muons are a naturally occurring form of radiation, are highly penetrating and exhibit large scattering angles on high Z materials. Specifically, we investigated how radiographic and tomographic techniques can be effective for non-invasive nuclear waste characterization and for nuclear material accountancy of spent fuel inside dry storage containers. We show that the tracking of individual muons, as they enter and exit a structure, can potentially improve the accuracy and availability of data on nuclear waste and the contents of Dry Storage Containers (DSC) used for spent fuel storage at CANDU plants. This could be achieved in near real time, with the potential for unattended and remotely monitored operations. We show that the expected sensitivity, in the case of the DSC, exceeds the IAEA detection target for nuclear material accountancy.

Jonkmans, G; Jewett, C; Thompson, M

2012-01-01T23:59:59.000Z

186

Method For Processing Spent (Trn,Zr)N Fuel  

DOE Patents [OSTI]

A new process for recycling spent nuclear fuels, in particular, mixed nitrides of transuranic elements and zirconium. The process consists of two electrorefiner cells in series configuration. A transuranic element such as plutonium is reduced at the cathode in the first cell, zirconium at the cathode in the second cell, and nitrogen-15 is released and captured for reuse to make transuranic and zirconium nitrides.

Miller, William E. (Naperville, IL); Richmann, Michael K. (Woodridge, IL)

2004-07-27T23:59:59.000Z

187

Machine Vision Tests for Spent Fuel Scrap Characteristics  

SciTech Connect (OSTI)

The purpose of this work is to perform a feasibility test of a Machine Vision system for potential use at the Hanford K basins during spent nuclear fuel (SNF) operations. This report documents the testing performed to establish functionality of the system including quantitative assessment of results. Fauske and Associates, Inc., which has been intimately involved in development of the SNF safety basis, has teamed with Agris-Schoen Vision Systems, experts in robotics, tele-robotics, and Machine Vision, for this work.

BERGER, W.W.

2000-04-27T23:59:59.000Z

188

SOURCE OF BURNUP VALUES FOR COMMERCIAL SPENT NUCLEAR FUEL ASSEMBLIES  

SciTech Connect (OSTI)

Waste packages are loaded with commercial spent nuclear fuel (SNF) that satisfies the minimum burnup requirements of a criticality loading curve. The burnup value assigned by the originating nuclear utility to each SNF assembly (assigned burnup) is used to load waste packages in compliance with a criticality loading curve. The burnup provided by a nuclear utility has uncertainties, so conservative calculation methods are used to characterize those uncertainties for incorporation into the criticality loading curves. Procedural safety controls ensure that the correct assembly is loaded into each waste package to prevent a misload that could create a condition affecting the safety margins. Probabilistic analyses show that procedural safety controls can minimize the chance of a misload but can not completely eliminate the possibility. Physical measurements of burnup with instrumentation in the surface facility are not necessary due to the conservative calculation methods used to produce the criticality loading curves. The reactor records assigned burnup of a commercial SNF assembly contains about two percent uncertainty, which is increased to five-percent to ensure conservatism. This five-percent uncertainty is accommodated by adjusting the criticality loading curve. Also, the record keeping methods of nuclear utilities are not uniform and the level of detail required by the NRC has varied over the last several decades. Thus, some SNF assemblies may have assigned burnups that are averages for a batch of assemblies with similar characteristics. Utilities typically have access to more detailed core-follow records that allow the batch average burnup to be changed to an assembly specific burnup. Alternatively, an additional safety margin is incorporated into the criticality loading curve to accommodate SNF assemblies with batch average burnups or greater uncertainties due to the methodology used by the nuclear utility. The utility records provide the assembly identifier, initial {sup 235}U enrichment, and time of discharge from the reactor as well as the assigned burnup, but the distribution. of burnup axially along the assembly length is not provided. The axial burnup profile is maintained within acceptable bounds by the operating conditions of the nuclear reactor and is calculated during preparations to reload a reactor, but the actual burnup profile is not measured. The axial burnup profile is important to the determination of the reactivity of a waste package, so a conservative evaluation of the calculated axial profiles for a large database of SNF has been performed. The product of the axial profile evaluation is a profile that is conservative. Thus, there is no need for physical measurement of the axial profile. The assembly identifier is legible on each SNF assembly and the utility records provide the associated characteristics of the assembly. The conservative methodologies used to determine the criticality loading curve for a waste package provide sufficient margin so that criticality safety is assured for preclosure operations even in the event of a misload. Consideration of misload effects for postclosure time periods is provided by the criticality Features, Events, and Processes (FEPs) analysis. The conservative approaches used to develop and apply the criticality loading curve are thus sufficiently robust that the utility assigned burnup is an adequate source of burnup values, and additional means of verification of assigned burnup through physical measurements are not needed.

BSC

2004-12-01T23:59:59.000Z

189

Fuel handling apparatus for a nuclear reactor  

DOE Patents [OSTI]

Fuel handling apparatus for transporting fuel elements into and out of a nuclear reactor and transporting them within the reactor vessel extends through a penetration in the side of the reactor vessel. A lateral transport device carries the fuel elements laterally within the vessel and through the opening in the side of the vessel, and a reversible lifting device raises and lowers the fuel elements. In the preferred embodiment, the lifting device is supported by a pair of pivot arms.

Hawke, Basil C. (Solana Beach, CA)

1987-01-01T23:59:59.000Z

190

Commercial Spent Nuclear Fuel Waste Package Misload Analysis  

SciTech Connect (OSTI)

The purpose of this calculation is to estimate the probability of misloading a commercial spent nuclear fuel waste package with a fuel assembly(s) that has a reactivity (i.e., enrichment and/or burnup) outside the waste package design. The waste package designs are based on the expected commercial spent nuclear fuel assemblies and previous analyses (Macheret, P. 2001, Section 4.1 and Table 1). For this calculation, a misloaded waste package is defined as a waste package that has a fuel assembly(s) loaded into it with an enrichment and/or burnup outside the waste package design. An example of this type of misload is a fuel assembly designated for the 21-PWR Control Rod waste package being incorrectly loaded into a 21-PWR Absorber Plate waste package. This constitutes a misloaded 21-PWR Absorber Plate waste package, because the reactivity (i.e., enrichment and/or burnup) of a 21-PWR Control Rod waste package fuel assembly is outside the design of a 21-PWR Absorber Plate waste package. These types of misloads (i.e., fuel assembly with enrichment and/or burnup outside waste package design) are the only types that are evaluated in this calculation. This calculation utilizes information from ''Frequency of SNF Misload for Uncanistered Fuel Waste Package'' (CRWMS M&O 1998) as the starting point. The scope of this calculation is limited to the information available. The information is based on the whole population of fuel assemblies and the whole population of waste packages, because there is no information about the arrival of the waste stream at this time. The scope of this calculation deviates from that specified in ''Technical Work Plan for: Risk and Criticality Department'' (BSC 2002a, Section 2.1.30) in that only waste package misload is evaluated. The remaining issues identified (i.e., flooding and geometry reconfiguration) will be addressed elsewhere. The intended use of the calculation is to provide information and inputs to the Preclosure Safety Analysis Department. Before using the results of this calculation, the reader is cautioned to verify that the assumptions made in this calculation regarding the waste stream, the loading process, and the staging of the spent nuclear fuel assemblies are applicable.

A. Alsaed

2005-07-28T23:59:59.000Z

191

Commercial Spent Nuclear Fuel Waste Package Misload Analysis  

SciTech Connect (OSTI)

The purpose of this calculation is to estimate the probability of misloading a commercial spent nuclear fuel waste package with a fuel assembly(s) that has a reactivity (i.e., enrichment and/or burnup) outside the waste package design. The waste package designs are based on the expected commercial spent nuclear fuel assemblies and previous analyses (Macheret, P. 2001, Section 4.1 and Table 1). For this calculation, a misloaded waste package is defined as a waste package that has a fuel assembly(s) loaded into it with an enrichment and/or burnup outside the waste package design. An example of this type of misload is a fuel assembly designated for the 21-PWR Control Rod waste package being incorrectly loaded into a 21-PWR Absorber Plate waste package. This constitutes a misloaded 21-PWR Absorber Plate waste package, because the reactivity (i.e., enrichment and/or burnup) of a 21-PWR Control Rod waste package fuel assembly is outside the design of a 21-PWR Absorber Plate waste package. These types of misloads (i.e., fuel assembly with enrichment and/or burnup outside waste package design) are the only types that are evaluated in this calculation. This calculation utilizes information from ''Frequency of SNF Misload for Uncanistered Fuel Waste Package'' (CRWMS M&O 1998) as the starting point. The scope of this calculation is limited to the information available. The information is based on the whole population of fuel assemblies and the whole population of waste packages, because there is no information about the arrival of the waste stream at this time. The scope of this calculation deviates from that specified in ''Technical Work Plan for: Risk and Criticality Department'' (BSC 2002a, Section 2.1.30) in that only waste package misload is evaluated. The remaining issues identified (i.e., flooding and geometry reconfiguration) will be addressed elsewhere. The intended use of the calculation is to provide information and inputs to the Preclosure Safety Analysis Department. Before using the results of this calculation, the reader is cautioned to verify that the assumptions made in this calculation regarding the waste stream, the loading process, and the staging of the spent nuclear fuel assemblies are applicable.

J.K. Knudson

2003-10-02T23:59:59.000Z

192

An approach to determine a defensible spent fuel ratio.  

SciTech Connect (OSTI)

Sabotage of spent nuclear fuel casks remains a concern nearly forty years after attacks against shipment casks were first analyzed and has a renewed relevance in the post-9/11 environment. A limited number of full-scale tests and supporting efforts using surrogate materials, typically depleted uranium dioxide (DUO2), have been conducted in the interim to more definitively determine the source term from these postulated events. In all the previous studies, the postulated attack of greatest interest was by a conical shape charge (CSC) that focuses the explosive energy much more efficiently than bulk explosives. However, the validity of these large-scale results remain in question due to the lack of a defensible Spent Fuel Ratio (SFR), defined as the amount of respirable aerosol generated by an attack on a mass of spent fuel compared to that of an otherwise identical DUO2 surrogate. Previous attempts to define the SFR have resulted in estimates ranging from 0.42 to 12 and include suboptimal experimental techniques and data comparisons. Different researchers have suggested using SFR values of 3 to 5.6. Sound technical arguments exist that the SFR does not exceed a value of unity. A defensible determination of the SFR in this lower range would greatly reduce the calculated risk associated with the transport and dry storage of spent nuclear fuel. Currently, Oak Ridge National Laboratory (ORNL) is in possession of several samples of spent nuclear fuel (SNF) that were used in the original SFR studies in the 1980's and were intended for use in a modern effort at Sandia National Laboratories (SNL) in the 2000's. A portion of these samples are being used for a variety of research efforts. However, the entirety of SNF samples at ORNL is scheduled for disposition at the Waste Isolation Pilot Plant (WIPP) by approximately the end of 2015. If a defensible SFR is to be determined for use in storage and transportation security analyses, the need to begin this effort is urgent in order to secure the only known available SNF samples with a clearly defined path to disposal.

Durbin, Samuel G.; Lindgren, Eric Richard

2014-03-01T23:59:59.000Z

193

E-Print Network 3.0 - advanced fissile fuel Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

will be exhausted in the foreseeable future. Spent fuel is dangerous... to the greenhouse effect. New Generation reactors to achieve the reuse of spent fuel. Fusion...

194

Spent fuel test-climax: a test of geologic storage of high-level waste in granite  

SciTech Connect (OSTI)

A test of retrievable geologic storage of spent fuel assemblies from an operating commercial nuclear reactor is underway at the Nevada Test Site (NTS) of the US Department of Energy. This generic test is located 420 m below the surface in the Climax granitic stock. Eleven canisters of spent fuel approximately 2.5 years out of reactor core (about 1.6 kW/canister thermal output) were emplaced in a storage drift along with 6 electrical simulator canisters. Two adjacent drifts contain electrical heaters, which are operated to simulate within the test array the thermal field of a large repository. Fuel was loaded during April to May 1980 and initial results of the test will be presented.

Ramspott, L.D.; Ballou, L.B.; Patrick, W.C.

1981-01-01T23:59:59.000Z

195

Actinides in metallic waste from electrometallurgical treatment of spent nuclear fuel.  

SciTech Connect (OSTI)

Argonne National Laboratory has developed a pyroprocessing-based technique for conditioning spent sodium-bonded nuclear-reactor fuel in preparation for long-term disposal. The technique produces a metallic waste form whose nominal composition is stainless steel with 15 wt.% Zr (SS-15Zr), up to {approx} 11 wt.% actinide elements (primarily uranium), and a few percent metallic fission products. Actual and simulated waste forms show similar eutectic microstructures with approximately equal proportions of iron solid solution phases and Fe-Zr intermetallics. This article reports on an analysis of simulated waste forms containing uranium, neptunium, and plutonium.

Janney, D. E.; Keiser, D. D., Jr.; Engineering Technology

2003-09-01T23:59:59.000Z

196

A Non-Proliferating Fuel Cycle: No Enrichment, Reprocessing or Accessible Spent Fuel - 12375  

SciTech Connect (OSTI)

Current fuel cycles offer a number of opportunities for access to plutonium, opportunities to create highly enriched uranium and access highly radioactive wastes to create nuclear weapons and 'dirty' bombs. The non-proliferating fuel cycle however eliminates or reduces such opportunities and access by eliminating the mining, milling and enrichment of uranium. The non-proliferating fuel cycle also reduces the production of plutonium per unit of energy created, eliminates reprocessing and the separation of plutonium from the spent fuel and the creation of a stream of high-level waste. It further simplifies the search for land based deep geologic repositories and interim storage sites for spent fuel in the USA by disposing of the spent fuel in deep sub-seabed sediments after storing the spent fuel at U.S. Navy Nuclear Shipyards that have the space and all of the necessary equipment and security already in place. The non-proliferating fuel cycle also reduces transportation risks by utilizing barges for the collection of spent fuel and transport to the Navy shipyards and specially designed ships to take the spent fuel to designated disposal sites at sea and to dispose of them there in deep sub-seabed sediments. Disposal in the sub-seabed sediments practically eliminates human intrusion. Potential disposal sites include Great Meteor East and Southern Nares Abyssal Plain. Such sites then could easily become international disposal sites since they occur in the open ocean. It also reduces the level of human exposure in case of failure because of the large physical and chemical dilution and the elimination of a major pathway to man-seawater is not potable. Of course, the recovery of uranium from sea water and the disposal of spent fuel in sub-seabed sediments must be proven on an industrial scale. All other technologies are already operating on an industrial scale. If externalities, such as reduced terrorist threats, environmental damage (including embedded emissions), long term care, reduced access to 'dirty' bomb materials, the social and political costs of siting new facilities and the psychological impact of no solution to the nuclear waste problem, were taken into account, the costs would be far lower than those of the present fuel cycle. (authors)

Parker, Frank L. [Vanderbilt University (United States)

2012-07-01T23:59:59.000Z

197

DEVELOPMENT OF METHODOLOGY AND FIELD DEPLOYABLE SAMPLING TOOLS FOR SPENT NUCLEAR FUEL INTERROGATION IN LIQUID STORAGE  

SciTech Connect (OSTI)

This project developed methodology and field deployable tools (test kits) to analyze the chemical and microbiological condition of the fuel storage medium and determine the oxide thickness on the spent fuel basin materials. The overall objective of this project was to determine the amount of time fuel has spent in a storage basin to determine if the operation of the reactor and storage basin is consistent with safeguard declarations or expectations. This project developed and validated forensic tools that can be used to predict the age and condition of spent nuclear fuels stored in liquid basins based on key physical, chemical and microbiological basin characteristics. Key parameters were identified based on a literature review, the parameters were used to design test cells for corrosion analyses, tools were purchased to analyze the key parameters, and these were used to characterize an active spent fuel basin, the Savannah River Site (SRS) L-Area basin. The key parameters identified in the literature review included chloride concentration, conductivity, and total organic carbon level. Focus was also placed on aluminum based cladding because of their application to weapons production. The literature review was helpful in identifying important parameters, but relationships between these parameters and corrosion rates were not available. Bench scale test systems were designed, operated, harvested, and analyzed to determine corrosion relationships between water parameters and water conditions, chemistry and microbiological conditions. The data from the bench scale system indicated that corrosion rates were dependent on total organic carbon levels and chloride concentrations. The highest corrosion rates were observed in test cells amended with sediment, a large microbial inoculum and an organic carbon source. A complete characterization test kit was field tested to characterize the SRS L-Area spent fuel basin. The sampling kit consisted of a TOC analyzer, a YSI multiprobe, and a thickness probe. The tools were field tested to determine their ease of use, reliability, and determine the quality of data that each tool could provide. Characterization was done over a two day period in June 2011, and confirmed that the L Area basin is a well operated facility with low corrosion potential.

Berry, T.; Milliken, C.; Martinez-Rodriguez, M.; Hathcock, D.; Heitkamp, M.

2012-06-04T23:59:59.000Z

198

EIS-0245: Management of Spent Fuel from the K Basins at the Hanford Site -  

Broader source: Energy.gov (indexed) [DOE]

245: Management of Spent Fuel from the K Basins at the Hanford 245: Management of Spent Fuel from the K Basins at the Hanford Site - Supplement Analysis, Richland, Washington EIS-0245: Management of Spent Fuel from the K Basins at the Hanford Site - Supplement Analysis, Richland, Washington Overview Overview to be provided. Public Comment Opportunities No public comment opportunities available at this time. Documents Available for Download August 15, 2011 EIS-0245-SA-03: Supplement Analysis Management of Spent Nuclear Fuel from the K Basins at the Hanford Site, Richland, Washington August 1, 2001 EIS-0245-SA-02: Supplement Analysis Management of Spent Nuclear Fuel from the K Basins at the Hanford Site, Richland, Washington August 1, 1998 EIS-0245-SA-01: Supplement Analysis Management of Spent Nuclear Fuel from the K Basins at the Hanford Site,

199

EM Safely and Efficiently Manages Spent Nuclear Fuel | Department of Energy  

Broader source: Energy.gov (indexed) [DOE]

Services » Waste Management » Nuclear Materials & Waste » EM Services » Waste Management » Nuclear Materials & Waste » EM Safely and Efficiently Manages Spent Nuclear Fuel EM Safely and Efficiently Manages Spent Nuclear Fuel Dry storage casks at Idaho National Laboratory can safely house spent nuclear fuel for decades. Dry storage casks at Idaho National Laboratory can safely house spent nuclear fuel for decades. EM's mission is to safely and efficiently manage its spent nuclear fuel and prepare it for disposal in a geologic repository. Previously, the Office of Environmental Management's (EM) mission had included the safe and efficient management of its spent nuclear fuel (SNF) and preparation for its disposal in a geologic repository. However, in May 2009, the planned geologic repository at Yucca Mountain was cancelled. The

200

National Report Joint Convention on the Safety of Spent Fuel Management and  

Broader source: Energy.gov (indexed) [DOE]

National Report Joint Convention on the Safety of Spent Fuel National Report Joint Convention on the Safety of Spent Fuel Management and on the Safety of Radioactive Waste Management National Report Joint Convention on the Safety of Spent Fuel Management and on the Safety of Radioactive Waste Management This is the first National Report prepared under the terms of the Joint Convention on the Safety of Spent Fuel Management and on the Safety of Radioactive Waste Managementi hereafter referred to as the "Joint Convention". This report satisfies the requirements of the Joint Convention for reporting on the status of safety at spent fuel and radioactive waste management facilities within the United States of America (U.S.). National Report Joint Convention on the Safety of Spent Fuel Management and on the Safety of Radioactive Waste Management - May 2003

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


201

DECONTAMINATION OF ZIRCALOY CLADDING HULLS FROM SPENT NUCLEAR FUEL  

SciTech Connect (OSTI)

The feasibility of decontaminating spent fuel cladding hulls using hydrofluoric acid (HF) was investigated as part of the Global Energy Nuclear Partnership (GNEP) Separations Campaign. The concentrations of the fission product and transuranic (TRU) isotopes in the decontaminated hulls were compared to the limits for determining the low level waste (LLW) classification in the United States (US). The {sup 90}Sr and {sup 137}Cs concentrations met the disposal criteria for a Class C LLW; although, in a number of experiments the criteria for disposal as a Class B LLW were met. The TRU concentration in the hulls generally exceeded the Class C LLW limit by at least an order of magnitude. The concentration decreased sharply as the initial 30-40 {micro}m of the cladding hull surface were removed. At depths beyond this point, the TRU activity remained relatively constant, well above the Class C limit. Reprocessing of spent nuclear fuel generates a cladding waste which would likely require disposal as a Greater than Class C LLW in the US. If the cladding hulls could be treated to remove a majority of the actinide and fission product contamination, the hulls could potentially meet acceptance criteria for disposal as a LLW or allow recycle of the Zr metal. Discard of the hulls as a LLW would result in significant cost savings compared to disposal as a Greater than Class C waste which currently has no disposition path. During fuel irradiation and reprocessing, radioactive materials are produced and deposited in the Zircaloy cladding. Due to short depths of penetration, the majority of the fission products and actinide elements are located in the ZrO{sub 2} layer which forms on the surface of the cladding during fuel irradiation. Therefore, if the oxide layer is removed, the majority of the contamination should also be removed. It is very difficult, if not impossible to remove all of the activity from spent fuel cladding since traces of U and Th in the unirradiated Zircaloy adsorb neutrons generating higher actinides in the bulk material. During fuel irradiation, {sup 92}Zr is also converted to radioactive {sup 93}Zr by neutron adsorption. Methods for decontaminating and conditioning irradiated Zircaloy cladding hulls have been investigated in Europe, Japan, and the US during the last 35 years; however, a method to decontaminate the hulls to an activity level which meets US acceptance criteria for disposal as a LLW was not deployed on a commercial scale. The feasibility of decontaminating spent fuel cladding hulls was investigated as part of the GNEP Separations Campaign. Small-scale experiments were used to demonstrate the removal of the ZrO{sub 2} layer from Zircaloy coupons using dilute solutions ({le}1.0 M) of HF. The most effective conditions resulted in dissolution rates which were less than approximately 2 mg/cm{sup 2}-min. With dissolution rates in this range, uniform removal of the oxide layer was obtained and a minimal amount of Zircaloy metal was dissolved. To test the HF decontamination process, experiments were subsequently performed using actual spent fuel cladding hulls. Decontamination experiments were performed to measure the fission product and actinide concentrations as a function of the depth of the surface removed from the cladding hull. The experimental methods used to perform these experiments and a discussion of the results and observations are presented in the following sections.

Rudisill, T.

2010-09-29T23:59:59.000Z

202

Spent Fuel and Waste Management Activities for Cleanout of the 105 F Fuel Storage Basin at Hanford  

SciTech Connect (OSTI)

Clean-out of the F Reactor fuel storage basin (FSB) by the Environmental Restoration Contractor (ERC) is an element of the FSB decontamination and decommissioning and is required to complete interim safe storage (ISS) of the F Reactor. Following reactor shutdown and in preparation for a deactivation layaway action in 1970, the water level in the F Reactor FSB was reduced to approximately 0.6 m (2 ft) over the floor. Basin components and other miscellaneous items were left or placed in the FSB. The item placement was performed with a sense of finality, and no attempt was made to place the items in an orderly manner. The F Reactor FSB was then filled to grade level with 6 m (20 ft) of local surface material (essentially a fine sand). The reactor FSB backfill cleanout involves the potential removal of spent nuclear fuel (SNF) that may have been left in the basin unintentionally. Based on previous cleanout of four water-filled FSBs with similar designs (i.e., the B, C, D, and DR FSBs in the 1980s), it was estimated that up to five SNF elements could be discovered in the F Reactor FSB (1). In reality, a total of 10 SNF elements have been found in the first 25% of the F Reactor FSB excavation. This paper discusses the technical and programmatic challenges of performing this decommissioning effort with some of the controls needed for SNF management. The paper also highlights how many various technologies were married into a complete package to address the issue at hand and show how no one tool could be used to complete the job; but by combining the use of multiple tools, progress is being made.

Morton, M. R.; Rodovsky, T. J.; Day, R. S.

2002-02-25T23:59:59.000Z

203

Corrosion of Spent Nuclear Fuel: The Long-Term Assessment  

SciTech Connect (OSTI)

Spent nuclear fuel, essentially U{sub 2}, accounts for over 95% of the total radioactivity of all of the radioactive wastes in the United States that require disposal, disposition or remediation. The UO{sub 2} in SNF is not stable under oxiding conditions and may also be altered under reducing conditions. The alteration of SNF results in the formation of new uranium phases that can cause the release or retardation of actinide and fission product radionuclides. Over the long term, and depending on the extent to which the secondary uranium phases incorporate fission products and actinides, these alteration phases become the near-field source term.

Rodney C. Ewing

2004-10-07T23:59:59.000Z

204

Test protocol for aluminum based spent nuclear fuel  

SciTech Connect (OSTI)

Aluminum based spent nuclear fuel (Al-SNF) will be treated and then stored in a geological repository. A series of corrosion tests, including coupon, galvanic, and electrochemical, were performed to measure the effects of degradation on U-Al alloys, which simulated various Al-SNF forms. The test solutions were variants of a J-13 well water chemistry. As part of the degradation characteristics, the dissolution of uranium, which is the primary radionuclide, was measured. The degradation and dissolution were changed by the type of water chemistry and the temperature. The alloy composition and fabrication were not significant variables.

Mickalonis, J.I.; Wiersma, B.J.

1999-07-01T23:59:59.000Z

205

Closure mechanism and method for spent nuclear fuel canisters  

DOE Patents [OSTI]

A canister is provided for storing, transporting, and/or disposing of spent nuclear fuel. The canister includes a canister shell, a top shield plug disposed within the canister, and a leak-tight closure arrangement. The closure arrangement includes a shear ring which forms a containment boundary of the canister, and which is welded to the canister shell and top shield plug. An outer seal plate, forming an outer seal, is disposed above the shear ring and is welded to the shield plug and the canister.

Doman, Marvin J. (Monroeville, PA)

2004-11-23T23:59:59.000Z

206

Production of metal waste forms from spent fuel treatment  

SciTech Connect (OSTI)

Treatment of spent nuclear fuel at Argonne National Laboratory consists of a pyroprocessing scheme in which the development of suitable waste forms is being advanced. Of the two waste forms being proposed, metal and mineral, the production of the metal waste form utilizes induction melting to stabilize the waste product. Alloying of metallic nuclear materials by induction melting has long been an Argonne strength and thus, the transition to metallic waste processing seems compatible. A test program is being initiated to coalesce the production of the metal waste forms with current induction melting capabilities.

Westphal, B.R.; Keiser, D.D.; Rigg, R.H.; Laug, D.V.

1995-02-01T23:59:59.000Z

207

Corrosion Minimization for Research Reactor Fuel  

SciTech Connect (OSTI)

Existing university research reactors are being converted to use low-enriched uranium fue to eliminate the use of highly-enriched uranium. These conversions require increases in fuel loading that will result in the use of elements with more fuel plates, resulting in a net decrease in the water annulus between fuel plates. The proposed decrease in the water annulus raises questions about the requirements and stability of the surface hydroxide on the aluminum fuel cladding and the potential for runaway corrosion resulting in fuel over-temperature incidents. The Nuclear Regulatory Commission (NRC), as regulator for these university reactors, must ensure that proposed fuel modifications will not result in any increased risk or hazard to the reactor operators or the public. This document reviews the characteristics and behavior of aluminum hydroxides, analyzes the drivers for fuel plate corrosion, reviews relevant historical incidents, and provides recommendations on fuel design, surface treatment, and reactor operational practices to avoid corrosion issues.

Eric Shaber; Gerard Hofman

2005-06-01T23:59:59.000Z

208

Rethinking the light water reactor fuel cycle  

E-Print Network [OSTI]

The once through nuclear fuel cycle adopted by the majority of countries with operating commercial power reactors imposes a number of concerns. The radioactive waste created in the once through nuclear fuel cycle has to ...

Shwageraus, Evgeni, 1973-

2004-01-01T23:59:59.000Z

209

FOREIGN ASSISTANCE FOR HANDLING SPENT NUCLEAR NAVAL FUEL IN RUSSIA: SETTING PRIORITIESi  

Science Journals Connector (OSTI)

For Russia's foreign partners, prioritizing tasks related to spent fuel management first involves identifying urgent needs, potential bottlenecks or gaps in assistance programs, safety and security issues, and...

C. CHUEN

2006-01-01T23:59:59.000Z

210

Kinematics and thermodynamics across a propagating non-stoichiometric oxidation phase front in spent fuel grains  

SciTech Connect (OSTI)

Spent fuel contains mixtures, alloy and compound, but are dominated by U and O except for some UO{sub 2} fuels with burnable poisons (gadolinia in BWR rods), the other elements evolve during reactor operation from neutron reaction and fission + fission decay events. Due to decay, chemical composition and activity of spent fuel will continue to evolve after removal from reactors. During the time interval with significant radioactivity levels relevant for a geological repository, it is important to develop models for potential chemical responses in spent fuel and potential degradation of repository. One such potential impact is the oxidation of spent fuel, which results in initial phase change of UO{sub 2} lattice to U{sub 4}O{sub 9} and the next phase change is probably to U{sub 3}O{sub 8} although it has not been observed yet below 200C. The U{sub 4}O{sub 9} lattice is nonstoichiometric with a O/U weight ratio at 2.4. Preliminary indications are that the UO{sub 2} has a O/U of 2. 4 at the time just before it transforms into the U{sub 4}O{sub 9} phase. In the oxygen weight gain versus time response, a plateau appears as the O/U approaches 2.4. Part of this plateau is due to geometrical effects of a U{sub 4}O{sub 9} phase change front propagating into UO{sub 2} grain volumes; however, this may indicate a metastable phase change delay kinetics or a diffusional related delay time until the oxygen density can satisfy stoichiometry and energy conditions for phase changes. Experimental data show a front of U{sub 4}O{sub 9} lattice structure propagating into grains of the UO{sub 2} lattice. To describe this spatially inhomogenous oxidation phase transition, as well as the expected U{sub 3}O{sub 8} phase transition from the U{sub 4}O{sub 9} lattice, lattice models are developed and spatially discontinuous kinematic and energetic expressions are derived. 9 refs.

Stout, R.B.; Kansa, E.J.; Wijesinghe, A.M.

1993-09-01T23:59:59.000Z

211

Non-Proliferative, Thorium-Based, Core and Fuel Cycle for Pressurized Water Reactors  

SciTech Connect (OSTI)

Two of the major barriers to the expansion of worldwide adoption of nuclear power are related to proliferation potential of the nuclear fuel cycle and issues associated with the final disposal of spent fuel. The Radkowsky Thorium Fuel (RTF) concept proposed by Professor A. Radkowsky offers a partial solution to these problems. The main idea of the concept is the utilization of the seed-blanket unit (SBU) fuel assembly geometry which is a direct replacement for a 'conventional' assembly in either a Russian pressurized water reactor (VVER-1000) or a Western pressurized water reactor (PWR). The seed-blanket fuel assembly consists of a fissile (U) zone, known as seed, and a fertile (Th) zone known as blanket. The separation of fissile and fertile allows separate fuel management schemes for the thorium part of the fuel (a subcritical 'blanket') and the 'driving' part of the core (a supercritical 'seed'). The design objective for the blanket is an efficient generation and in-situ fissioning of the U233 isotope, while the design objective for the seed is to supply neutrons to the blanket in a most economic way, i.e. with minimal investment of natural uranium. The introduction of thorium as a fertile component in the nuclear fuel cycle significantly reduces the quantity of plutonium production and modifies its isotopic composition, reducing the overall proliferation potential of the fuel cycle. Thorium based spent fuel also contains fewer higher actinides, hence reducing the long-term radioactivity of the spent fuel. The analyses show that the RTF core can satisfy the requirements of fuel cycle length, and the safety margins of conventional pressurized water reactors. The coefficients of reactivity are comparable to currently operating VVER's/PWR's. The major feature of the RTF cycle is related to the total amount of spent fuel discharged for each cycle from the reactor core. The fuel management scheme adopted for RTF core designs allows a significant decrease in the amount of discharged spent fuel, for a given energy production, compared with standard VVER/PWR. The total Pu production rate of RTF cycles is only 30 % of standard reactor. In addition, the isotopic compositions of the RTF's and standard reactor grade Pu are markedly different due to the very high burnup accumulated by the RTF spent fuel.

Todosow M.; Todosow M.; Raitses, G. (BNL) Galperin, A. (Ben Gurion University)

2009-07-12T23:59:59.000Z

212

On the Criticality Safety of Transuranic Sodium Fast Reactor Fuel Transport Casks  

SciTech Connect (OSTI)

This work addresses the neutronic performance and criticality safety issues of transport casks for fuel pertaining to low conversion ratio sodium cooled fast reactors, conventionally known as Advanced Burner Reactors. The criticality of a one, three, seven and 19-assembly cask capacity is presented. Both dry “helium” and flooded “water” filled casks are considered. No credit for fuel burnup or fission products was assumed. As many as possible of the conservatisms used in licensing light water reactor universal transport casks were incorporated into this SFR cask criticality design and analysis. It was found that at 7-assemblies or more, adding moderator to the SFR cask increases criticality margin. Also, removal of MAs from the fuel increases criticality margin of dry casks and takes a slight amount of margin away for wet casks. Assuming credit for borated fuel tube liners, this design analysis suggests that as many as 19 assemblies can be loaded in a cask if limited purely by criticality safety. If no credit for boron is assumed, the cask could possibly hold seven assemblies if low conversion ratio fast reactor grade fuel and not breeder reactor grade fuel is assumed. The analysis showed that there is a need for new cask designs for fast reactors spent fuel transportation. There is a potential of modifying existing transportation cask design as the starting point for fast reactor spent fuel transportation.

Samuel Bays; Ayodeji Alajo

2010-05-01T23:59:59.000Z

213

Radioactive Waste Management: Study of Spent Fuel Dissolution Rates in Geological Storage Using Dosimetry Modeling and Experimental Verification  

SciTech Connect (OSTI)

This research will provide improved predictions into the mechanisms and effects of radiolysis on spent nuclear fuel dissolution in a geological respository through accurate dosimetry modeling of the dose to water, mechanistic chemistry modeling of the resulting radiolytic reactions and confirmatory experimental measurements. This work will combine effort by the Nuclear Science and Engineering Institute (NSEI) and the Missouri University Research Reactor (MURR) at the University of Missouri-Columbia, and the expertise and facilities at the Pacific Northwest National Laboratory (PNNL).

Brady Hansen; William Miller

2011-10-28T23:59:59.000Z

214

The behaviour of transuranic mixed oxide fuel in a Candu-900 reactor  

SciTech Connect (OSTI)

The production of transuranic actinide fuels for use in current thermal reactors provides a useful intermediary step in closing the nuclear fuel cycle. Extraction of actinides reduces the longevity, radiation and heat loads of spent material. The burning of transuranic fuels in current reactors for a limited amount of cycles reduces the infrastructure demand for fast reactors and provides an effective synergy that can result in a reduction of as much as 95% of spent fuel waste while reducing the fast reactor infrastructure needed by a factor of almost 13.5 [1]. This paper examines the features of actinide mixed oxide fuel, TRUMOX, in a CANDU{sup R}* nuclear reactor. The actinide concentrations used were based on extraction from 30 year cooled spent fuel and mixed with natural uranium in 3.1 wt% actinide MOX fuel. Full lattice cell modeling was performed using the WIMS-AECL code, super-cell calculations were analyzed in DRAGON and full core analysis was executed in the RFSP 2-group diffusion code. A time-average full core model was produced and analyzed for reactor coefficients, reactivity device worth and online fuelling impacts. The standard CANDU operational limits were maintained throughout operations. The TRUMOX fuel design achieved a burnup of 27.36 MWd/kg HE. A full TRUMOX fuelled CANDU was shown to operate within acceptable limits and provided a viable intermediary step for burning actinides. The recycling, reprocessing and reuse of spent fuels produces a much more sustainable and efficient nuclear fuel cycle. (authors)

Morreale, A. C.; Ball, M. R.; Novog, D. R.; Luxat, J. C. [Dept. of Engineering Physics, McMaster Univ., 1280 Main St. W, Hamilton, ON (Canada)

2012-07-01T23:59:59.000Z

215

Drop Testing of DOE Spent Nuclear Fuel Canisters  

SciTech Connect (OSTI)

The National Spent Nuclear Fuel Program (NSNFP) at the Idaho National Engineering and Environmental Laboratory INEEL) prepared four representative Department of Energy DOE) spent nuclear fuel (SNF) canisters for the purpose of drop testing. The first two canisters represented a modified 24- inch diameter standardized DOE SNF canister and the second two canisters represented the Hanford Multi-Canister Overpack MCO). The modified canisters and internals were constructed and assembled at the INEEL. The MCO internal weights were fabricated at the INEEL and assembled into two MCOs at Hanford and later shipped to the INEEL for drop test preparation. Drop testing of these four canisters was completed in August 2004 at Sandia National Laboratories. The modified canisters were dropped from 30 feet onto a flat, essentially unyielding surface, with the canisters oriented at 45 degrees and 70 degrees off-vertical at impact. One representative MCO was dropped from 23 feet onto the same flat surface, oriented vertically at impact. The second representative MCO was dropped onto the flat surface from 2 feet oriented at 60 degrees off-vertical. These drop heights and orientations were chosen to meet or exceed the Yucca Mountain repository drop criteria. This paper discusses the comparison of deformations between the actual dropped canisters and those predicted by pre-drop and limited post-drop finite element evaluations performed using ABAQUS/Explicit. Post-drop containment of all four canisters, demonstrated by way of helium leak testing, is also discussed.

S. D. Snow; D. K. Morton; T. E. Rahl; R. K. Blandford; T. J. Hill

2005-07-01T23:59:59.000Z

216

Integrated Data Base for 1992: US spent fuel and radioactive waste inventories, projections, and characteristics  

SciTech Connect (OSTI)

The Integrated Data Base (IDB) Program has compiled current data on inventories and characteristics of commercial spent fuel and both commercial and US government-owned radioactive wastes through December 31, 1991. These data are based on the most reliable information available from government sources, the open literature, technical reports, and direct contacts. The information forecasted is consistent with the latest US Department of Energy/Energy Information Administration (DOE/EIA) projections of US commercial nuclear power growth and the expected DOE-related and private industrial and institutional (I/I) activities. The radioactive materials considered, on a chapter-by-chapter basis, are spent nuclear fuel, high-level waste, transuranic waste, low-level waste, commercial uranium mill tailings, environmental restoration wastes, commercial reactor and fuel cycle facility decommissioning wastes, and mixed (hazardous and radioactive) low-level waste. For most of these categories, current and projected inventories are given through the year 2030, and the radioactivity and thermal power are calculated based on reported or estimated isotopic compositions. In addition, characteristics and current inventories are reported for miscellaneous radioactive materials that may require geologic disposal.

Not Available

1992-10-01T23:59:59.000Z

217

Strategic Minimization of High Level Waste from Pyroprocessing of Spent Nuclear Fuel  

SciTech Connect (OSTI)

The pyroprocessing of spent nuclear fuel results in two high-level waste streams--ceramic and metal waste. Ceramic waste contains active metal fission product-loaded salt from the electrorefining, while the metal waste contains cladding hulls and undissolved noble metals. While pyroprocessing was successfully demonstrated for treatment of spent fuel from Experimental Breeder Reactor-II in 1999, it was done so without a specific objective to minimize high-level waste generation. The ceramic waste process uses “throw-away” technology that is not optimized with respect to volume of waste generated. In looking past treatment of EBR-II fuel, it is critical to minimize waste generation for technology developed under the Global Nuclear Energy Partnership (GNEP). While the metal waste cannot be readily reduced, there are viable routes towards minimizing the ceramic waste. Fission products that generate high amounts of heat, such as Cs and Sr, can be separated from other active metal fission products and placed into short-term, shallow disposal. The remaining active metal fission products can be concentrated into the ceramic waste form using an ion exchange process. It has been estimated that ion exchange can reduce ceramic high-level waste quantities by as much as a factor of 3 relative to throw-away technology.

Simpson, Michael F.; Benedict, Robert W.

2007-09-01T23:59:59.000Z

218

Electrolysis cell for reprocessing plutonium reactor fuel  

DOE Patents [OSTI]

An electrolytic cell for refining a mixture of metals including spent fuel containing U and Pu contaminated with other metals is claimed. The cell includes a metallic pot containing a metallic pool as one anode at a lower level, a fused salt as the electrolyte at an intermediate level and a cathode and an anode basket in spaced-apart positions in the electrolyte with the cathode and anode being retractable to positions above the electrolyte during which spent fuel may be added to the anode basket. The anode basket is extendable into the lower pool to dissolve at least some metallic contaminants; the anode basket contains the spent fuel acting as a second anode when in the electrolyte.

Miller, W.E.; Steindler, M.J.; Burris, L.

1985-01-04T23:59:59.000Z

219

Impact of PWR spent fuel variations on TRU-fueled VHTRS  

E-Print Network [OSTI]

of legacy spent fuel that is given in the Yucca Mountain Safety Assessment Report. Chapter III discusses the details of the study. The concluding study was accomplished through the use of ORNL SCALE5.1 code system. The detailed whole-core 3-D models were...

Alajo, Ayodeji Babatunde

2009-05-15T23:59:59.000Z

220

Plasma processing of spent nuclear fuel by two-frequency ion cyclotron resonance heating  

Science Journals Connector (OSTI)

A previously developed method for analyzing the plasma processing of spent nuclear fuel is generalized to a plasma containing multicharged fuel ions. In such a plasma, ion cyclotron resonance heating of nuclear a...

A. V. Timofeev

2009-11-01T23:59:59.000Z

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


221

Corrosion property of 9Cr-ODS steel in nitric acid solution for spent nuclear fuel reprocessing  

SciTech Connect (OSTI)

Corrosion tests of oxide dispersion strengthened with 9% Cr (9Cr-ODS) steel, which is one of the desirable materials for cladding tube of sodium-cooled fast reactors, in pure nitric acid solution, spent FBR fuel solution, and its simulated solution were performed to understand the corrosion behavior in a spent nuclear fuel reprocessing. In this study, the 9Cr-ODS steel with lower effective chromium content was evaluated to understand the corrosion behavior conservatively. As results, the tube-type specimens of the 9Cr-ODS steels suffered severe weight loss owing to active dissolution at the beginning of the immersion test in pure nitric acid solution in the range from 1 to 3.5 M. In contrast, the weight loss was decreased and they showed a stable corrosion in the higher nitric acid concentration, the dissolved FBR fuel solution, and its simulated solution by passivation. The corrosion rates of the 9Cr-ODS steel in the dissolved FBR fuel solution and its simulated solution were 1-2 mm/y and showed good agreement with each other. The passivation was caused by the shift of corrosion potential to noble side owing to increase in nitric acid concentration or oxidative ions in the dissolved FBR fuel solution and the simulated spent fuel solution. (authors)

Takeuchi, M.; Koizumi, T. [Japan Atomic Energy Agency, Tokai-mura, Naka-gun, Ibaraki 319-1195 (Japan); Inoue, M.; Koyama, S.I. [Japan Atomic Energy Agency, Oarai-machi, Higashi-ibaraki-gun, Ibaraki 311-1393 (Japan)

2013-07-01T23:59:59.000Z

222

Second National Report for the Joint Convention on the Safety of Spent Fuel  

Broader source: Energy.gov (indexed) [DOE]

Second National Report for the Joint Convention on the Safety of Second National Report for the Joint Convention on the Safety of Spent Fuel Management and on the Safety of Radioactive Waste Management Second National Report for the Joint Convention on the Safety of Spent Fuel Management and on the Safety of Radioactive Waste Management This second National Report updates the first National Report published on May 3, 2003, under the terms of the Joint Convention on the Safety of Spent Fuel Management and on the Safety of Radioactive Waste Management (Joint Convention). This report satisfies the requirements of the Joint Convention for reporting on the status of safety at spent fuel (SF) and radioactive waste management facilities within the United States of America (U.S.). Second National Report for the Joint Convention on the Safety of Spent Fuel

223

Simulated nuclear reactor fuel assembly  

DOE Patents [OSTI]

An apparatus for electrically simulating a nuclear reactor fuel assembly. It includes a heater assembly having a top end and a bottom end and a plurality of concentric heater tubes having electrical circuitry connected to a power source, and radially spaced from each other. An outer target tube and an inner target tube is concentric with the heater tubes and with each other, and the outer target tube surrounds and is radially spaced from the heater tubes. The inner target tube is surrounded by and radially spaced from the heater tubes and outer target tube. The top of the assembly is generally open to allow for the electrical power connection to the heater tubes, and the bottom of the assembly includes means for completing the electrical circuitry in the heater tubes to provide electrical resistance heating to simulate the power profile in a nuclear reactor. The embedded conductor elements in each heater tube is split into two halves for a substantial portion of its length and provided with electrical isolation such that each half of the conductor is joined at one end and is not joined at the other end.

Berta, V.T.

1993-04-06T23:59:59.000Z

224

Behavior of Spent Nuclear Fuel in Water Pool Storage  

Office of Scientific and Technical Information (OSTI)

Behavior of Spent Nuclear Behavior of Spent Nuclear Fuel in Water Pool Storage A. 0; Johnson, jr. , I ..: . Prepared Cor the Energy Research and Development Administration under Contract EY-76-C-06-1830 ---- Pat t i ~ < N ~ ~ r ~ t b w t ~ - ! I , ~ I ~ ~ ~ I . I I ~ ) ~ I I ~ ~ N O T I C E T€& - was prepad pnpn4. m w n t of w k spon-d by the Unitd S t . & ) C a u n m ~ (*WU ij*. M t e d $tam w the Wqy R e s e w & a d Ohrsropmcnt ~dmhirmlion, nor m y d thair ewhew,,nq Pny @fw a n t r ~ ~ t 0 ~ 1 , s ~ k m r i t r i l t t q r , ~ , m r tWf ernpfQw, r(tLltm any wartany, s x p r e s or kWld,= w w aAql -9 . o r r w p a m l ~ ~ t y for e~ o r uodruincvr of any infomutim, 9 F p d + d - , or repratants that -would nat 1 d - e privately owned rfghas. ,i PAQFIC NORTHWEST UBORATORY operated b ;"' SArnLLE ' fw the E M R m RESEARCH AND DEVELOPMENT ADMINISTRAT1QN Wk.Cwfraa rv-76c-ts-is38

225

Radionuclide release rates from spent fuel for performance assessment modeling  

SciTech Connect (OSTI)

In a scenario of aqueous transport from a high-level radioactive waste repository, the concentration of radionuclides in water in contact with the waste constitutes the source term for transport models, and as such represents a fundamental component of all performance assessment models. Many laboratory experiments have been done to characterize release rates and understand processes influencing radionuclide release rates from irradiated nuclear fuel. Natural analogues of these waste forms have been studied to obtain information regarding the long-term stability of potential waste forms in complex natural systems. This information from diverse sources must be brought together to develop and defend methods used to define source terms for performance assessment models. In this manuscript examples of measures of radionuclide release rates from spent nuclear fuel or analogues of nuclear fuel are presented. Each example represents a very different approach to obtaining a numerical measure and each has its limitations. There is no way to obtain an unambiguous measure of this or any parameter used in performance assessment codes for evaluating the effects of processes operative over many millennia. The examples are intended to suggest by example that in the absence of the ability to evaluate accuracy and precision, consistency of a broadly based set of data can be used as circumstantial evidence to defend the choice of parameters used in performance assessments.

Curtis, D.B.

1994-11-01T23:59:59.000Z

226

Spent nuclear fuel policies in historical perspective: An international comparison  

Science Journals Connector (OSTI)

The purpose of this article is to explain why the world's nuclear power countries differ from each other with respect to their spent nuclear fuel (SNF) policies. The emergence and evolution of three principal SNF approaches are analyzed: direct disposal, reprocessing and SNF export. Five broad explanatory factors are identified and discussed in relation to the observed differences in policy outcomes: military ambitions and non-proliferation, technological culture, political culture and civil society, geological conditions, and energy policy. SNF policy outcomes can generally be seen to result from a complex interaction between these broad factors, but it is also possible to discern a number of important patterns. To the extent that the five factors may undergo far-reaching changes in the future, the historical experience of how they have shaped SNF policies also give a hint of possible future directions in SNF policymaking around the world.

Per Högselius

2009-01-01T23:59:59.000Z

227

Present experience of NRI REZ with preparation of spent nuclear fuel shipment to Russian Federation  

SciTech Connect (OSTI)

The Nuclear Research Institute Rez plc (NRI) jointed the Russian Research Reactor Fuel Return (RRRFR) programme under the US-Russian Global Threat Reduction Initiative (GTRI) initiative and started the preparation of the spent nuclear fuel (SNF) shipment from the LVR-15 research reactor back to the Russian Federation (RF). The transport of 16 SKODA VPVR/M casks with EK-10, IRT-2M 80 %, and IRT-2M 36% fuel types is planned for the autumn of 2007. The paper describes the experience gained so far during the preparatory works for the SNF shipment (facility equipment modification, cask licenses) and the actual preparation of the SNF for transport, in particular its checking, repacking in a hot cell, loading into the VPVR/M casks, drying, manipulation, completion of the transport documentation, etc., including its transport to the SNF storage facility at the NRI before it is shipped to the RF. The paper also briefly describes a regulatory framework for these activities with a focus on legislative and methodological aspects of the return of vitrified waste back to the Czech Republic. (author)

Svitak, F.; Broz, V.; Hrehor, M.; Marek, M.; Novosad, P.; Podlaha, J.; Rychecky, J. [Nuclear Research Institute Rez plc, Husinec 130, CZ-25068 (Czech Republic)

2008-07-15T23:59:59.000Z

228

US Department of Energy Storage of Spent Fuel and High Level Waste  

SciTech Connect (OSTI)

ABSTRACT This paper provides an overview of the Department of Energy's (DOE) spent nuclear fuel (SNF) and high level waste (HLW) storage management. Like commercial reactor fuel, DOE's SNF and HLW were destined for the Yucca Mountain repository. In March 2010, the DOE filed a motion with the Nuclear Regulatory Commission (NRC) to withdraw the license application for the repository at Yucca Mountain. A new repository is now decades away. The default for the commercial and DOE research reactor fuel and HLW is on-site storage for the foreseeable future. Though the motion to withdraw the license application and delay opening of a repository signals extended storage, DOE's immediate plans for management of its SNF and HLW remain the same as before Yucca Mountain was designated as the repository, though it has expanded its research and development efforts to ensure safe extended storage. This paper outlines some of the proposed research that DOE is conducting and will use to enhance its storage systems and facilities.

Sandra M Birk

2010-10-01T23:59:59.000Z

229

Assessment of Nuclear Resonance Fluorescence for Spent Nuclear Fuel Assay  

SciTech Connect (OSTI)

In nuclear resonance fluorescence (NRF) measurements, resonances are excited by an external photon beam leading to the emission of gamma rays with specific energies that are characteristic of the emitting isotope. NRF promises the unique capability of directly quantifying a specific isotope without the need for unfolding the combined responses of several fissile isotopes as is required in other measurement techniques. We have analyzed the potential of NRF as a non-destructive analysis technique for quantitative measurements of Pu isotopes in spent nuclear fuel (SNF). Given the low concentrations of 239Pu in SNF and its small integrated NRF cross sections, the main challenge in achieving precise and accurate measurements lies in accruing sufficient counting statistics in a reasonable measurement time. Using analytical modeling, and simulations with the radiation transport code MCNPX that has been experimentally tested recently, the backscatter and transmission methods were quantitatively studied for differing photon sources and radiation detector types. Resonant photon count rates and measurement times were estimated for a range of photon source and detection parameters, which were used to determine photon source and gamma-ray detector requirements. The results indicate that systems based on a bremsstrahlung source and present detector technology are not practical for high-precision measurements of 239Pu in SNF. Measurements that achieve the desired uncertainties within hour-long measurements will either require stronger resonances, which may be expressed by other Pu isotopes, or require quasi-monoenergetic photon sources with intensities that are approximately two orders of magnitude higher than those currently being designed or proposed.This work is part of a larger effort sponsored by the Next Generation Safeguards Initiative to develop an integrated instrument, comprised of individual NDA techniques with complementary features, that is fully capable of determining Pu mass in spent fuel assemblies.

Quiter, Brian; Ludewigt, Bernhard; Ambers, Scott

2011-06-30T23:59:59.000Z

230

Roles and effects of pyroprocessing for spent nuclear fuel management in South Korea  

Science Journals Connector (OSTI)

Abstract Republic of Korea (ROK) changed its spent nuclear fuel policy from the once-through usage and direct disposal to a total system approach that includes pyroprocessing, sodium-cooled fast reactors, and a two-tier geological repository to achieve a breakthrough for domestic deadlock situation and thus enable sustainable utilization of nuclear power, but caused disagreement in the bilateral negotiation with the United States (US) for the Nuclear Cooperation Agreement. Analysis has revealed that this shift is effective to make a breakthrough for domestic deadlock because it augments variety of technological options, with which more reversible decision-making process can be conducted to accommodate broad public needs. A trade-off has been explored first by deriving four engineering options from the ROK's system concept and then by comparing their performance from six viewpoints. The option including separation of high-heat emitting radionuclides by the electrolytic reduction process has been recommended. This option should be modified as exogenous and endogenous situations change in future. It is imperative for ROK to integrate a public-participatory decision-making process that works in concert with technology development. US can verify that ROK's motivation is not deviating from successful spent fuel management by checking if a transparent process with public participation is conducted.

Joonhong Ahn

2014-01-01T23:59:59.000Z

231

The Need for Confirmatory Experiments on the Radioactive Source Term from Potential Sabotage of Spent Nuclear Fuel Casks  

SciTech Connect (OSTI)

A technical review is presented of experiment activities and state of knowledge on air-borne, radiation source terms resulting from explosive sabotage attacks on spent reactor fuel subassemblies in shielded casks. Current assumptions about the behavior of irradiated fuel are largely based on a limited number of experimental results involving unirradiated, depleted uranium dioxide ''surrogate'' fuel. The behavior of irradiated nuclear fuel subjected to explosive conditions could be different from the behavior of the surrogate fuel, depending on the assumptions made by the evaluator. Available data indicate that these potential differences could result in errors, and possible orders-of-magnitude overestimates of aerosol dispersion and potential health effects from sabotage attacks. Furthermore, it is suggested that the current assumptions used in arriving at existing regulations for the transportation and storage of spent fuel in the U.S. are overly conservative. This, in turn, has led to potentially higher-than-needed operating expenses for those activities. A confirmatory experimental program is needed to develop a realistic correlation between source terms of irradiated fuel and unirradiated fuel. The motivations for performing the confirmatory experimental program are also presented.

PHILBIN, JEFFREY S.; HOOVER, MARK D.; NEWTON, GEORGE J.

2002-04-01T23:59:59.000Z

232

The integral fast reactor fuel cycle  

SciTech Connect (OSTI)

The liquid-metal reactor (LMR) has the potential to extend the uranium resource by a factor of 50 to 100 over current commercial light water reactors (LWRs). In the integral fast reactor (IFR) development program, the entire reactor system - reactor, fuel cycle, and waste process - is being developed and optimized at the same time as a single integral entity. A key feature of the IFR concept is the metallic fuel. The lead irradiation tests on the new U-Pu-Zr metallic fuel in the Experimental Breeder Reactor II have surpassed 185000 MWd/t burnup, and its high burnup capability has now been fully demonstrated. The metallic fuel also allows a radically improved fuel cycle technology. Pyroprocessing, which utilizes high temperatures and molten salt and molten metal solvents, can be advantageously utilized for processing metal fuels because the product is metal suitable for fabrication into new fuel elements. Direct production of a metal product avoids expensive and cumbersome chemical conversion steps that would result from use of the conventional Purex solvent extraction process. The key step in the IFR process is electrorefining, which provides for recovery of the valuable fuel constituents, uranium and plutonium, and for removal of fission products. A notable feature of the IFR process is that the actinide elements accompany plutonium through the process. This results in a major advantage in the high-level waste management.

Chang, Y.I. (Argonne National Lab., IL (United States))

1990-01-01T23:59:59.000Z

233

Measurement of Spent Fuel Assemblies - Overview of the Status of the Technology for Initiating Discussion at NATIONAL RESEARCH CENTRE KURCHATOV INSTITUTE June 2013  

SciTech Connect (OSTI)

This presentation provides an overview of the status of the technology for the measurement of the fissile material content of spent nuclear reactor fuel. The emphasis is on how the needs of the U.S. Nuclear Regulatory Commission and the International Atomic Energy Agency are met by the available technology and what more needs to be done in this area.

SISKIND B.; N /A

2013-06-03T23:59:59.000Z

234

Development of alternate extractant systems for fast reactor fuel cycle  

SciTech Connect (OSTI)

Due to the limitations of TBP in processing of high burn-up, Pu-rich fast reactor fuels, there is a need to develop alternate extractants for fast reactor fuel processing. In this context, our Centre has been examining the suitability of alternate tri-alkyl phosphates. Third phase formation in the extraction of Th(IV) by TBP, tri-n-amyl phosphate (TAP) and tri-2-methyl-butyl phosphate (T2MBP) from nitric acid media has been investigated under various conditions to derive conclusions on their application for extraction of Pu at macro levels. The chemical and radiolytic degradation of tri-n-amyl-phosphate (TAP) diluted in normal paraffin hydrocarbon (NPH) in the presence of nitric acid has been investigated by the measurement of plutonium retention in organic phase. The potential application of room temperature ionic liquids (RTILs) for reprocessing of spent nuclear fuel has been explored. Extraction of uranium (VI) and palladium (II) from nitric acid medium by commercially available RTIL and tri-n-butyl phosphate solution in RTIL have been studied and the feasibility of electrodeposition of uranium as uranium oxide (UO{sub 2}) and palladium (II) as metallic palladium from the loaded organic phase have been demonstrated. This paper describes results of the above studies and discusses the suitability of the systems for fast reactor fuel reprocessing. (authors)

Vasudeva Rao, P.R.; Suresh, A.; Venkatesan, K.A.; Srinivasan, T.G.; Raj, Baldev [Indira Gandhi Centre for Atomic Research, Kalpakkam - 603 102 (India)

2007-07-01T23:59:59.000Z

235

Determining Plutonium Mass in Spent Fuel with Nondestructive Assay Techniques -- Preliminary Modeling Results Emphasizing Integration among Techniques  

E-Print Network [OSTI]

Based Spent Fuel Analysis Safeguards Strategy Assessment,”on International Safeguards: Addressing VerificationNuclear Fuel,” European Safeguards R&D Association, Vilnius,

Tobin, S. J.

2010-01-01T23:59:59.000Z

236

Expert System analysis of non-fuel assembly hardware and spent fuel disassembly hardware: Its generation and recommended disposal  

SciTech Connect (OSTI)

Almost all of the effort being expended on radioactive waste disposal in the United States is being focused on the disposal of spent Nuclear Fuel, with little consideration for other areas that will have to be disposed of in the same facilities. one area of radioactive waste that has not been addressed adequately because it is considered a secondary part of the waste issue is the disposal of the various Non-Fuel Bearing Components of the reactor core. These hardware components fall somewhat arbitrarily into two categories: Non-Fuel Assembly (NFA) hardware and Spent Fuel Disassembly (SFD) hardware. This work provides a detailed examination of the generation and disposal of NFA hardware and SFD hardware by the nuclear utilities of the United States as it relates to the Civilian Radioactive Waste Management Program. All available sources of data on NFA and SFD hardware are analyzed with particular emphasis given to the Characteristics Data Base developed by Oak Ridge National Laboratory and the characterization work performed by Pacific Northwest Laboratories and Rochester Gas & Electric. An Expert System developed as a portion of this work is used to assist in the prediction of quantities of NFA hardware and SFD hardware that will be generated by the United States` utilities. Finally, the hardware waste management practices of the United Kingdom, France, Germany, Sweden, and Japan are studied for possible application to the disposal of domestic hardware wastes. As a result of this work, a general classification scheme for NFA and SFD hardware was developed. Only NFA and SFD hardware constructed of zircaloy and experiencing a burnup of less than 70,000 MWD/MTIHM and PWR control rods constructed of stainless steel are considered Low-Level Waste. All other hardware is classified as Greater-ThanClass-C waste.

Williamson, D.A.

1991-12-31T23:59:59.000Z

237

Plasma processing of spent nuclear fuel by two-frequency ion cyclotron resonance heating  

SciTech Connect (OSTI)

A previously developed method for analyzing the plasma processing of spent nuclear fuel is generalized to a plasma containing multicharged fuel ions. In such a plasma, ion cyclotron resonance heating of nuclear ash ions should be carried out in two monochromatic RF fields of different frequencies, provided that the fraction of {xi} multicharged ions is small, {xi} {<=} 0.1, a condition that substantially restricts the productivity of systems for processing spent nuclear fuel. Ways of overcoming this difficulty are discussed.

Timofeev, A. V. [Russian Research Centre Kurchatov Institute, Nuclear Fusion Institute (Russian Federation)

2009-11-15T23:59:59.000Z

238

Characterization of LWR spent fuel MCC-approved testing material-ATM-101  

SciTech Connect (OSTI)

The characterization data, obtained to date, for Materials Characterization Center (MCC) Approved Testing Materials (ATM)-101, spent fuel from H.B. Robinson, Unit 2, Assembly BO-5, are described. ATM-101 consists of 27 equal-length segments from nine fuel rods. Characterizations provided for ATM-101 include, (1) reactor, assembly, and fuel rod descriptions, (2) Assembly BO-5 irradiation history, (3) a description of unusual incidents that occurred to the rods, (4) fission gas release measurements, (5) results of ceramography/metallography examinations, (6) fuel burnup measurement results and correlations, (7) results of gamma scanning, (8) calculated values of the radionuclide inventory, and (9) results of a radionuclide chemical overcheck. Calculations for and measurement of radial distributions of selected radionuclides are planned. A description of pertinent results from other studies on sibling rods from Assembly BO-5 is also included. The distribution of ATM-101 to date is described along with characterization results on specially processed material. It is intended that this report be revised and updated as additional characterization data become available. 6 references, 23 figures, 19 tables.

Barner, J.O.

1984-06-01T23:59:59.000Z

239

Technology development program for Idaho Chemical Processing Plant spent fuel and waste management  

SciTech Connect (OSTI)

Acidic high-level radioactive waste (HLW) resulting from fuel reprocessing at the Idaho Chemical Processing Plant (ICPP) for the U.S. Department of Energy (DOE) has been solidified to a calcine since 1963 and stored in stainless steel bins enclosed by concrete vaults. Several different types of unprocessed irradiated DOE-owned fuels are also in storage at the ICPP. In April, 1992, DOE announced that spent fuel would no longer be reprocessed to recover enriched uranium and called for a shutdown of the reprocessing facilities at the ICPP. A new Spent Fuel and HLW Technology Development program was subsequently initiated to develop technologies for immobilizing ICPP spent fuels and HLW for disposal, in accordance with the Nuclear Waste Policy Act. The Program elements include Systems Analysis, Graphite Fuel Disposal, Other Spent Fuel Disposal, Sodium-Bearing Liquid Waste Processing, Calcine Immobilization, and Metal Recycle/Waste Minimization. This paper presents an overview of the ICPP radioactive wastes and current spent fuels, and describes the Spent Fuel and HLW Technology program in more detail.

Ermold, L.F.; Knecht, D.A.; Hogg, G.W.; Olson, A.L.

1993-08-01T23:59:59.000Z

240

Water Chemistry Control System for Recovery of Damaged and Degraded Spent Fuel  

SciTech Connect (OSTI)

The International Atomic Energy Agency (IAEA) and the government of Serbia have led the project cosponsored by the U.S, Russia, European Commission, and others to repackage and repatriate approximately 8000 spent fuel elements from the RA reactor fuel storage basins at the VIN?A Institute of Nuclear Sciences to Russia for reprocessing. The repackaging and transportation activities were implemented by a Russian consortium which includes the Sosny Company, Tekhsnabeksport (TENEX) and Mayak Production Association. High activity of the water of the fuel storage basin posed serious risk and challenges to the fuel removal from storage containers and repackaging for transportation. The risk centered on personnel exposure, even above the basin water, due to the high water activity levels caused by Cs-137 leached from fuel elements with failed cladding. A team of engineers from the U.S. DOE-NNSA's Global Threat Reduction Initiative, the Vinca Institute, and the IAEA performed the design, development, and deployment of a compact underwater water chemistry control system (WCCS) to remove the Cs-137 from the basin water and enable personnel safety above the basin water for repackaging operations. Key elements of the WCCS system included filters, multiple columns containing an inorganic sorbent, submersible pumps and flow meters. All system components were designed to be remotely serviceable and replaceable. The system was assembled and successfully deployed at the Vinca basin to support the fuel removal and repackaging activities. Following the successful operations, the Cs-137 is now safely contained and consolidated on the zeolite sorbent used in the columns of the WCCS, and the fuel has been removed from the basins. This paper reviews the functional requirements, design, and deployment of the WCCS.

Sindelar, R.; Fisher, D.; Thomas, J.

2011-02-18T23:59:59.000Z

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


241

13 - Generation IV reactor designs, operation and fuel cycle  

Science Journals Connector (OSTI)

Abstract: This chapter looks at Generation IV nuclear reactors, such as the very high-temperature reactor (VHTR), the supercritical water reactor (SCWR), the molten salt reactor (MSR), the sodium-cooled fast reactor (SFR), the lead-cooled fast reactor (LFR) and the gas-cooled fast reactor (GFR). Reactor designs and fuel cycles are also described.

N. Cerullo; G. Lomonaco

2012-01-01T23:59:59.000Z

242

Interim report spent nuclear fuel retrieval system fuel handling development testing  

SciTech Connect (OSTI)

Fuel handling development testing was performed in support of the Fuel Retrieval System (FRS) Sub-Project at the Hanford Site. The project will retrieve spent nuclear fuel, clean and remove fuel from canisters, repackage fuel into baskets, and load fuel into a multi-canister overpack (MCO) for vacuum drying and interim dry storage. The FRS is required to retrieve basin fuel canisters, clean fuel elements sufficiently of uranium corrosion products (or sludge), empty fuel from canisters, sort debris and scrap from whole elements, and repackage fuel in baskets in preparation for MCO loading. The purpose of fuel handling development testing was to examine the systems ability to accomplish mission activities, optimization of equipment layouts for initial process definition, identification of special needs/tools, verification of required design changes to support performance specification development, and validation of estimated activity times/throughput. The test program was set up to accomplish this purpose through cold development testing using simulated and prototype equipment; cold demonstration testing using vendor expertise and systems; and graphical computer modeling to confirm feasibility and throughput. To test the fuel handling process, a test mockup that represented the process table was fabricated and installed. The test mockup included a Schilling HV series manipulator that was prototypic of the Schilling Hydra manipulator. The process table mockup included the tipping station, sorting area, disassembly and inspection zones, fuel staging areas, and basket loading stations. The test results clearly indicate that the Schilling Hydra arm cannot effectively perform the fuel handling tasks required unless it is attached to some device that can impart vertical translation, azimuth rotation, and X-Y translation. Other test results indicate the importance of camera locations and capabilities, and of the jaw and end effector tool design. 5 refs., 35 figs., 3 tabs.

Ketner, G.L.; Meeuwsen, P.V.; Potter, J.D.; Smalley, J.T.; Baker, C.P.; Jaquish, W.R.

1997-06-01T23:59:59.000Z

243

Evaluation of transuranium isotopes inventory for Candu/ACR standard and SEU spent fuel and the possibility to transmute them  

SciTech Connect (OSTI)

Available in abstract form only. Full text of publication follows: The main disadvantage of nuclear energy is the quantity of long lived radioactive waste produced in a NPP. Transmutation could be one of the solutions to reduce it. Waste transmutation will require a suitable deployment of techniques for spent fuel reprocessing. At present, reprocessing is done by aqueous methods that are very efficient for Pu separation (up to 99.9%). For transmutation applications, new partitioning processes must be developed for minor actinides separation from the high level waste. Although these processes are still very much at the research stage, industrial scale-up will result in the deployment of new, more specific separation techniques for transmutation applications. Partitioning and Transmutation (P and T) techniques could contribute to reduce the radioactive inventory and its associated radio-toxicity. Scientists are looking for ways to drastically reduce both the mass and the radio-toxicity of the nuclear waste to be stored in a deep geological repository, and to reduce the time needed to reach the radioactivity level of the raw material originally used to produce energy. The first stage in the transmutation process is the isotopes inventory formed in the spent fuel. In this paper is made an intercomparison evaluation using WIMS 5B.12 and ORIGEN computer codes. Using these two codes, there is evaluated the isotopes released by a fuel standard from a Candu reactor. Moreover, there is simulated an inventory released by a Candu-SEU reactor and an ACR reactor. (authors)

Ghizdeanu, Elena Nineta; Pavelescu, Alexandru [University Politehnica of Bucharest - Faculty of Power Engineering, 313 Splaiul Independentei, RO-060042, Bucharest 6 (Romania); Balaceanu, Victoria [Institute for Nuclear Research, Campului Str., 1, Mioveni P.O. Box 78, 0300 Pitesti (Romania)

2007-07-01T23:59:59.000Z

244

Integrated Data Base for 1991: US spent fuel and radioactive waste inventories, projections, and characteristics. [Contains glossary  

SciTech Connect (OSTI)

The Integrated Data Base (IDB) Program has compiled current data on inventories and characteristics of commercial spent fuel and both commercial and US government-owned radioactive wastes through December 31, 1990. These data are based on the most reliable information available form government sources, the open literature, technical reports, and direct contacts. The current projections of future waste and spent fuel to be generated generally through the year 2020 and characteristics of these materials are also presented. The information forecasted is consistent with the latest US Department of Energy/Energy Information Administration (DOE/EIA) projections of US commercial nuclear power growth and the expected DOE-related and private industrial and institutional (I/I) activities. The radioactive materials considered are spent fuel, high-level waste, transuranic waste, low-level waste, commercial uranium mill tailings, environmental restoration wastes, commercial reactor and fuel cycle facility decommissioning wastes, and mixed (hazardous and radioactive) low-level waste. For most of these categories, current and projected inventories are given through the year 2020, and the radioactivity and thermal power are calculated based on reported or estimated isotopic compositions. In addition, characteristics and current inventories are reported for miscellaneous radioactive materials that may require geologic disposal. 160 refs., 61 figs., 142 tabs.

Not Available

1991-10-01T23:59:59.000Z

245

Integrated Data Base for 1991: US spent fuel and radioactive waste inventories, projections, and characteristics. Revision 7  

SciTech Connect (OSTI)

The Integrated Data Base (IDB) Program has compiled current data on inventories and characteristics of commercial spent fuel and both commercial and US government-owned radioactive wastes through December 31, 1990. These data are based on the most reliable information available form government sources, the open literature, technical reports, and direct contacts. The current projections of future waste and spent fuel to be generated generally through the year 2020 and characteristics of these materials are also presented. The information forecasted is consistent with the latest US Department of Energy/Energy Information Administration (DOE/EIA) projections of US commercial nuclear power growth and the expected DOE-related and private industrial and institutional (I/I) activities. The radioactive materials considered are spent fuel, high-level waste, transuranic waste, low-level waste, commercial uranium mill tailings, environmental restoration wastes, commercial reactor and fuel cycle facility decommissioning wastes, and mixed (hazardous and radioactive) low-level waste. For most of these categories, current and projected inventories are given through the year 2020, and the radioactivity and thermal power are calculated based on reported or estimated isotopic compositions. In addition, characteristics and current inventories are reported for miscellaneous radioactive materials that may require geologic disposal. 160 refs., 61 figs., 142 tabs.

Not Available

1991-10-01T23:59:59.000Z

246

Measurements on spent-fuel assemblies at Arkansas Nuclear One using the Fork system. Final report, January 1995  

SciTech Connect (OSTI)

The Fork measurement system has been used to examine spent-fuel assemblies at the two reactors of Arkansas Nuclear One, operated by Entergy Operations, Inc. The Unit 1 reactor is a Babcock and Wilcox (B and W) design, and the Unit 2 reactor is a Combustion Engineering (CE) design. The neutron and gamma-ray emissions from individual spent-fuel assemblies were measured in the storage pools by raising each assembly pathway out of the storage rack and performing a measurement near the center of the assembly. The overall accuracy of the measurements after corrections is about 2%. Thirty-four assemblies were examined at Unit 1, and forty-one assemblies at Unit 2. The average deviation of the burnup measurements from the calibration was 3.0% at Unit 1 and 3.5% at Unit 2, indicating 2 to 3% random variation among the reactor records. There was no indication of clearly anomalous assemblies. Axial Scans of the variation in neutron and gamma ray emission were obtained by collecting data at several locations along the length of three assemblies at Unit 2. Two of these assemblies were nonstandard in that each contained a small neutron source. The sources were detected by the axial scans. The test program was a cooperative effort involving Sandia National Laboratories, Los Alamos National Laboratory, Entergy Operations, Inc., the Electric Power Research Institute, and the Office of Civilian Radioactive Waste Management of the US Department of Energy.

Ewing, R.I.; Bronowski, D.R. [Sandia National Labs., Albuquerque, NM (United States); Bosler, G.E.; Siebelist, R. [Los Alamos National Lab., NM (United States); Priore, J.; Hansford, C.H.; Sullivan, S. [Entergy Operations, Inc., Russellville, AR (United States). Arkansas Nuclear One

1997-03-01T23:59:59.000Z

247

The breeder reactor: a fossil fuel viewpoint  

Science Journals Connector (OSTI)

... elegant and simple: to generate electricity and, at the same time, to produce additional fuel from the uranium discarded by the existing thermal reactor system. Without the breeder reactor, ... seems likely that the role of nuclear energy will begin to be constrained by the price and availability of uranium at about the turn of the century. There is, however ...

David Merrick

1976-12-16T23:59:59.000Z

248

Department of Energy Programmatic Spent Nuclear Fuel Management and Idaho National Engineering Laboratory Environmental Restoration and Waste Management Programs Draft Environmental Impact Statement. Volume 1, Appendix D, Part B: Naval spent nuclear fuel management  

SciTech Connect (OSTI)

This volume contains the following attachments: transportation of Naval spent nuclear fuel; description of Naval spent nuclear receipt and handling at the Expended Core Facility at the Idaho National Engineering Laboratory; comparison of storage in new water pools versus dry container storage; description of storage of Naval spent nuclear fuel at servicing locations; description of receipt, handling, and examination of Naval spent nuclear fuel at alternate DOE facilities; analysis of normal operations and accident conditions; and comparison of the Naval spent nuclear fuel storage environmental assessment and this environmental impact statement.

Not Available

1994-06-01T23:59:59.000Z

249

Dosimetry Modeling for Predicting Radiolytic Production at the Spent Fuel - Water Interface  

SciTech Connect (OSTI)

Modeling of the alpha, beta, and gamma dose from spent fuel as a function of particle size and fuel to water ratio was examined. These doses will be combined with modeling of G values and interactions to determine the concentration of various species formed at the fuel water interface and their affect on dissolution rates.

Miller, William H.; Kline, Amanda J.; Hanson, Brady D.

2006-04-30T23:59:59.000Z

250

Refinishing contamination floors in Spent Nuclear Fuels storage basins  

SciTech Connect (OSTI)

The floors of the K Basins at the Hanford Site are refinished to make decontamination easier if spills occur as the spent nuclear fuel (SNF) is being unloaded from the basins for shipment to dry storage. Without removing the contaminated existing coating, the basin floors are to be coated with an epoxy coating material selected on the basis of the results of field tests of several paint products. The floor refinishing activities must be reviewed by a management review board to ensure that work can be performed in a controlled manner. Major documents prepared for management board review include a report on maintaining radiation exposure as low as reasonably achievable, a waste management plan, and reports on hazard classification and unreviewed safety questions. To protect personnel working in the radiation zone, Operational Health Physics prescribed the required minimum protective methods and devices in the radiological work permit. Also, industrial hygiene safety must be analyzed to establish respirator requirements for persons working in the basins. The procedure and requirements for the refinishing work are detailed in a work package approved by all safety engineers. After the refinishing work is completed, waste materials generated from the refinishing work must be disposed of according to the waste management plan.

Huang, F.F.; Moore, F.W.

1997-07-11T23:59:59.000Z

251

Multi-Detector Analysis System for Spent Nuclear Fuel Characterization  

SciTech Connect (OSTI)

The Spent Nuclear Fuel (SNF) Non-Destructive Analysis (NDA) program at INEEL is developing a system to characterize SNF for fissile mass, radiation source term, and fissile isotopic content. The system is based on the integration of the Fission Assay Tomography System (FATS) and the Gamma-Neutron Analysis Technique (GNAT) developed under programs supported by the DOE Office of Non-proliferation and National Security. Both FATS and GNAT were developed as separate systems to provide information on the location of special nuclear material in weapons configuration (FATS role), and to measure isotopic ratios of fissile material to determine if the material was from a weapon (GNAT role). FATS is capable of not only determining the presence and location of fissile material but also the quantity of fissile material present to within 50%. GNAT determines the ratios of the fissile and fissionable material by coincidence methods that allow the two prompt (immediately) produced fission fragments to be identified. Therefore, from the combination of FATS and GNAT, MDAS is able to measure the fissile material, radiation source term, and fissile isotopics content.

Reber, Edward Lawrence; Aryaeinejad, Rahmat; Cole, Jerald Donald; Drigert, Mark William; Jewell, James Keith; Egger, Ann Elizabeth; Cordes, Gail Adele

1999-09-01T23:59:59.000Z

252

Deployment evaluation methodology for the electrometallurgical treatment of DOE-EM spent nuclear fuel  

SciTech Connect (OSTI)

Part of the Department of Energy (DOE) spent nuclear fuel (SNF) inventory may require some type of treatment to meet acceptance criteria at various disposition sites. The current focus for much of this spent nuclear fuel is the electrometallurgical treatment process under development at Argonne National Laboratory. Potential flowsheets for this treatment process are presented. Deployment of the process for the treatment of the spent nuclear fuel requires evaluation to determine the spent nuclear fuel program need for treatment and compatibility of the spent nuclear fuel with the process. The evaluation of need includes considerations of cost, technical feasibility, process material disposition, and schedule to treat a proposed fuel. A siting evaluation methodology has been developed to account for these variables. A work breakdown structure is proposed to gather life-cycle cost information to allow evaluation of alternative siting strategies on a similar basis. The evaluation methodology, while created specifically for the electrometallurgical evaluation, has been written such that it could be applied to any potential treatment process that is a disposition option for spent nuclear fuel. Future work to complete the evaluation of the process for electrometallurgical treatment is discussed.

Dahl, C.A.; Adams, J.P.; Ramer, R.J.

1998-07-01T23:59:59.000Z

253

A Blueprint for GNEP Advanced Burner Reactor Startup Fuel Fabrication Facility  

SciTech Connect (OSTI)

The purpose of this article is to identify the requirements and issues associated with design of GNEP Advanced Burner Reactor Fuel Facility. The report was prepared in support of providing data for preparation of a NEPA Environmental Impact Statement in support the U. S. Department of Energy (DOE) Global Nuclear Energy Partnership (GNEP). One of the GNEP objectives was to reduce the inventory of long lived actinide from the light water reactor (LWR) spent fuel. The LWR spent fuel contains Plutonium (Pu) -239 and other transuranics (TRU) such as Americium-241. One of the options is to transmute or burn these actinides in fast neutron spectra as well as generate the electricity. A sodium-cooled Advanced Recycling Reactor (ARR) concept was proposed to achieve this goal. However, fuel with relatively high TRU content has not been used in the fast reactor. To demonstrate the utilization of TRU fuel in a fast reactor, an Advanced Burner Reactor (ABR) prototype of ARR was proposed, which would necessarily be started up using weapons grade (WG) Pu fuel. The WG Pu is distinguished by relatively highest proportions of Pu-239 and lesser amount of other actinides. The WG Pu was assumed to be used as the startup fuel along with TRU fuel in lead test assemblies. Because such fuel is not currently being produced in the US, a new facility (or new capability in an existing facility) was being considered for fabrication of WG Pu fuel for the ABR. It was estimated that the facility will provide the startup fuel for 10-15 years and would take 3 to 5 years to construct.

S. Khericha

2010-12-01T23:59:59.000Z

254

Uranium to Electricity: The Chemistry of the Nuclear Fuel Cycle  

Science Journals Connector (OSTI)

The nuclear fuel cycle consists of a series of industrial processes that produce fuel for the production of electricity in nuclear reactors, use the fuel to generate electricity, and subsequently manage the spent reactor fuel. While the physics and ...

Frank A. Settle

2009-03-01T23:59:59.000Z

255

FATE Unified Modeling Method for Spent Nuclear Fuel and Sludge Processing, Shipping and Storage - 13405  

SciTech Connect (OSTI)

A unified modeling method applicable to the processing, shipping, and storage of spent nuclear fuel and sludge has been incrementally developed, validated, and applied over a period of about 15 years at the US DOE Hanford site. The software, FATE{sup TM}, provides a consistent framework for a wide dynamic range of common DOE and commercial fuel and waste applications. It has been used during the design phase, for safety and licensing calculations, and offers a graded approach to complex modeling problems encountered at DOE facilities and abroad (e.g., Sellafield). FATE has also been used for commercial power plant evaluations including reactor building fire modeling for fire PRA, evaluation of hydrogen release, transport, and flammability for post-Fukushima vulnerability assessment, and drying of commercial oxide fuel. FATE comprises an integrated set of models for fluid flow, aerosol and contamination release, transport, and deposition, thermal response including chemical reactions, and evaluation of fire and explosion hazards. It is one of few software tools that combine both source term and thermal-hydraulic capability. Practical examples are described below, with consideration of appropriate model complexity and validation. (authors)

Plys, Martin; Burelbach, James; Lee, Sung Jin; Apthorpe, Robert [Fauske and Associates, LLC, 16W070 83rd St., Burr Ridge, IL, 60527 (United States)] [Fauske and Associates, LLC, 16W070 83rd St., Burr Ridge, IL, 60527 (United States)

2013-07-01T23:59:59.000Z

256

Fourth National Report for the Joint Convention on the Safety of Spent Fuel  

Broader source: Energy.gov (indexed) [DOE]

Fourth National Report for the Joint Convention on the Safety of Fourth National Report for the Joint Convention on the Safety of Spent Fuel Management and on the Safety of Radioactive Waste Management Fourth National Report for the Joint Convention on the Safety of Spent Fuel Management and on the Safety of Radioactive Waste Management This Fourth United States of America (U.S.) National Report updates the Third Report published in October 2008, under the terms of the Joint Convention on the Safety of Spent Fuel Management and on the Safety of Radioactive Waste Management (Joint Convention). This report reflects developments in the U.S. through June 2011. This report satisfies the requirements of the Joint Convention for reporting on the status of safety at spent fuel and radioactive waste management facilities within the U.S.

257

Third National Report for the Joint Convention on the Safety of Spent Fuel  

Broader source: Energy.gov (indexed) [DOE]

Third National Report for the Joint Convention on the Safety of Third National Report for the Joint Convention on the Safety of Spent Fuel Management and on the Safety of Radioactive Waste Management Third National Report for the Joint Convention on the Safety of Spent Fuel Management and on the Safety of Radioactive Waste Management This Third United States National Report updates the second National Report published in October 2005, under the terms of the Joint Convention on the Safety of Spent Fuel Management and on the Safety of Radioactive Waste Management 1(Joint Convention). This report reflects developments in the United States through September 2008. This report satisfies the requirements of the Joint Convention for reporting on the status of safety at spent fuel and radioactive waste management facilities within

258

EM Prepares Report for Convention on Safety of Spent Fuel and Radioactive Waste Management  

Broader source: Energy.gov [DOE]

WASHINGTON, D.C. – EM supported DOE in its role as the lead technical agency to produce a report recently for the Joint Convention on the Safety of Spent Fuel Management and on the Safety of Radioactive Waste Management.

259

Stainless steel-zirconium waste forms from the treatment of spent nuclear fuel  

Science Journals Connector (OSTI)

Stainless steel-zirconium waste-form alloys have been developed for the disposal of metallic wastes recovered from spent nuclear fuel using the electrometallurgical process developed by Argonne National Laborator...

S. M. McDeavitt; D. P. Abraham; J. Y. Park; D. D. Keiser

1997-07-01T23:59:59.000Z

260

Preoperational Environmental Survey for the Spent Nuclear Fuel (SNF) Project Facilities  

SciTech Connect (OSTI)

This document represents the report for environmental sampling of soil, vegetation, litter, cryptograms, and small mammals at the Spent Nuclear Fuel Project facilities located in 100 K and 200 East Areas in support of the preoperational environmental survey.

MITCHELL, R.M.

2000-09-28T23:59:59.000Z

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


261

EA-1117: Management of Spent Nuclear Fuel on the Oak Ridge Reservation, Oak Ridge, Tennessee  

Broader source: Energy.gov [DOE]

This EA evaluates the environmental impacts of the proposal for the management of spent nuclear fuel on the U.S. Department of Energy's Oak Ridge Reservation to implement the preferred alternative...

262

Spent nuclear fuel and residential property values: the influence of proximity, visual cues and public information  

Science Journals Connector (OSTI)

...This article examines whether public knowledge of spent fuel storage at nuclear power plants, and any ... that may have occurred, affect the sale price of single-family residential properties. We present ... m...

David E. Clark; Tim Allison

1999-10-01T23:59:59.000Z

263

Direct conversion of surplus fissile materials, spent nuclear fuel, and other materials to high-level-waste glass  

SciTech Connect (OSTI)

With the end of the cold war the United States, Russia, and other countries have excess plutonium and other materials from the reductions in inventories of nuclear weapons. The United States Academy of Sciences (NAS) has recommended that these surplus fissile materials (SFMs) be processed so they are no more accessible than plutonium in spent nuclear fuel (SNF). This spent fuel standard, if adopted worldwide, would prevent rapid recovery of SFMs for the manufacture of nuclear weapons. The NAS recommended investigation of three sets of options for disposition of SFMs while meeting the spent fuel standard: (1) incorporate SFMs with highly radioactive materials and dispose of as waste, (2) partly burn the SFMs in reactors with conversion of the SFMs to SNF for disposal, and (3) dispose of the SFMs in deep boreholes. The US Government is investigating these options for SFM disposition. A new method for the disposition of SFMs is described herein: the simultaneous conversion of SFMs, SNF, and other highly radioactive materials into high-level-waste (HLW) glass. The SFMs include plutonium, neptinium, americium, and {sup 233}U. The primary SFM is plutonium. The preferred SNF is degraded SNF, which may require processing before it can be accepted by a geological repository for disposal.

Forsberg, C.W.; Elam, K.R.

1995-01-31T23:59:59.000Z

264

Electrolytic recovery of reactor metal fuel  

DOE Patents [OSTI]

This invention is comprised of a new electrolytic process and apparatus using sodium, cerium or a similar metal in an alloy or within a sodium beta or beta-alumina sodium ion conductor to electrolytically displace each of the spent fuel metals except for Cesium and strontium on a selective basis from the electrolyte to an inert metal cathode. Each of the metals can be deposited separately. An electrolytic transfer of spent fuel into the electrolyte includes a sodium or cerium salt in the electrolyte with sodium or cerium alloy being deposited on the cathode during the transfer of the metals from the spent fuel. The cathode with the deposit of sodium or cerium alloy is then changed to an anode and the reverse transfer is carried out on a selective basis with each metal being deposited separately at the cathode. The result is that the sodium or cerium needed for the process is regenerated in the first step and no additional source of these reactants is required.

Miller, W.E.; Tomczuk, Z.

1993-02-03T23:59:59.000Z

265

Estimation of the Transportation Risks for the Spent Fuel in Korea for Various Transportation Scenarios  

SciTech Connect (OSTI)

According to the long term management strategy for spent fuels in Korea, they will be transported from the spent fuel pools in each nuclear power plant to the central interim storage facility (CISF) which is to start operation in 2016. Therefore, we have to determine the safe and economical logistics for the transportation of these spent fuels by considering their transportation risks and costs. In this study, we developed four transportation scenarios by considering the type of transportation casks and transport means in order to suggest safe and economical transportation logistics for the spent fuels in Korea. Also, we estimated and compared the transportation risks for these four transportation scenarios. From the results of this study, we found that these four transportation scenarios for spent fuels have a very low radiological risk activity with a manageable safety and health consequences. The results of this study can be used as basic data for the development of safe and economical logistics for a transportation of the spent fuels in Korea by considering the transportation costs for the four scenarios which will be needed in the near future. (authors)

Jongtae, Jeong; Cho, D.K.; Choi, H.J.; Choi, J.W. [Korea Atomic Energy Research Institute, Yuseong, Daejeon (Korea, Republic of)

2008-07-01T23:59:59.000Z

266

MELCOR Model of the Spent Fuel Pool of Fukushima Dai-ichi Unit 4  

SciTech Connect (OSTI)

Unit 4 of the Fukushima Dai-ichi Nuclear Power Plant suffered a hydrogen explosion at 6:00 am on March 15, 2011, exactly 3.64 days after the earthquake hit the plant and the off-site power was lost. The earthquake occurred on March 11 at 2:47 pm. Since the reactor of this Unit 4 was defueled on November 29, 2010, and all its fuel was stored in the spent fuel pool (SFP4), it was first believed that the explosion was caused by hydrogen generated by the spent fuel, in particular, by the recently discharged core. The hypothetical scenario was: power was lost, cooling to the SFP4 water was lost, pool water heated/boiled, water level decreased, fuel was uncovered, hot Zircaloy reacted with steam, hydrogen was generated and accumulated above the pool, and the explosion occurred. Recent analyses of the radioisotopes present in the water of the SFP4 and underwater video indicated that this scenario did not occur - the fuel in this pool was not damaged and was never uncovered the hydrogen of the explosion was apparently generated in Unit 3 and transported through exhaust ducts that shared the same chimney with Unit 4. This paper will try to answer the following questions: Could that hypothetical scenario in the SFP4 had occurred? Could the spent fuel in the SPF4 generate enough hydrogen to produce the explosion that occurred 3.64 days after the earthquake? Given the magnitude of the explosion, it was estimated that at least 150 kg of hydrogen had to be generated. As part of the investigations of this accident, MELCOR models of the SFP4 were prepared and a series of calculations were completed. The latest version of MELCOR, version 2.1 (Ref. 1), was employed in these calculations. The spent fuel pool option for BWR fuel was selected in MELCOR. The MELCOR model of the SFP4 consists of a total of 1535 fuel assemblies out of which 548 assemblies are from the core defueled on Nov. 29, 2010, 783 assemblies are older assemblies, and 204 are new/fresh assemblies. The total decay heat of the fuel in the pool was, at the time of the accident, 2.284 MWt, of which 1.872 MWt were from the 548 assemblies of the last core discharged and 0.412 MWt were from the older 783 assemblies. These decay heat values were calculated at Oak Ridge National Laboratory using the ORIGEN2.2 code (Ref. 2) - they agree with values reported elsewhere (Ref. 3). The pool dimensions are 9.9 m x 12.2 m x 11.8 m (height), and with the water level at 11.5 m, the pool volume is 1389 m3, of which only 1240 m3 is water, as some volume is taken by the fuel and by the fuel racks. The initial water temperature of the SFP4 was assumed to be 301 K. The fuel racks are made of an aluminum alloy but are modeled in MELCOR with stainless steel and B4C. MELCOR calculations were completed for different initial water levels: 11.5 m (pool almost full, water is only 0.3 m below the top rim), 4.4577 m (top of the racks), 4.2 m, and 4.026 m (top of the active fuel). A calculation was also completed for a rapid loss of water due to a leak at the bottom of the pool, with the fuel rapidly uncovered and oxidized in air. Results of these calculations are shown in the enclosed Table I. The calculation with the initial water level at 11.5 m (full pool) takes 11 days for the water to boil down to the top of the fuel racks, 11.5 days for the fuel to be uncovered, 14.65 days to generate 150 kg of hydrogen and 19 days for the pool to be completely dry. The calculation with the initial water level at 4.4577 m, takes 1.1 days to uncover the fuel and 4.17 days to generate 150 kg of hydrogen. The calculation with the initial water level at 4.02 m takes 3.63 days to generate 150 kg of hydrogen this is exactly the time when the actual explosion occurred in Unit 4. Finally, fuel oxidation in air after the pool drained the water in 20 minutes, generates only 10 kg of hydrogen this is because very little steam is available and Zircaloy (Zr) oxidation with the oxygen of the air does not generate hydrogen. MELCOR calculated water levels and hydrogen generated in the SFP4 as a function of time for initial water le

Carbajo, Juan J [ORNL] [ORNL

2012-01-01T23:59:59.000Z

267

CONTAINMENT ANALYSIS METHODOLOGY FOR TRANSPORT OF BREACHED CLAD ALUMINUM SPENT FUEL  

SciTech Connect (OSTI)

Aluminum-clad, aluminum-based spent nuclear fuel (Al-SNF) from foreign and domestic research reactors (FRR/DRR) is being shipped to the Savannah River Site and placed in interim storage in a water basin. To enter the United States, a cask with loaded fuel must be certified to comply with the requirements in the Title 10 of the U.S. Code of Federal Regulations, Part 71. The requirements include demonstration of containment of the cask with its contents under normal and accident conditions. Many Al-SNF assemblies have suffered corrosion degradation in storage in poor quality water, and many of the fuel assemblies are 'failed' or have through-clad damage. A methodology was developed to evaluate containment of Al-SNF even with severe cladding breaches for transport in standard casks. The containment analysis methodology for Al-SNF is in accordance with the methodology provided in ANSI N14.5 and adopted by the U. S. Nuclear Regulatory Commission in NUREG/CR-6487 to meet the requirements of 10CFR71. The technical bases for the inputs and assumptions are specific to the attributes and characteristics of Al-SNF received from basin and dry storage systems and its subsequent performance under normal and postulated accident shipping conditions. The results of the calculations for a specific case of a cask loaded with breached fuel show that the fuel can be transported in standard shipping casks and maintained within the allowable release rates under normal and accident conditions. A sensitivity analysis has been conducted to evaluate the effects of modifying assumptions and to assess options for fuel at conditions that are not bounded by the present analysis. These options would include one or more of the following: reduce the fuel loading; increase fuel cooling time; reduce the degree of conservatism in the bounding assumptions; or measure the actual leak rate of the cask system. That is, containment analysis for alternative inputs at fuel-specific conditions and at cask-loading-specific conditions could be performed to demonstrate that release is within the allowable leak rates of the cask.

Vinson, D.

2010-07-11T23:59:59.000Z

268

Assessing the Feasibility of Using Neutron Resonance Transmission Analysis (NRTA) for Assaying Plutonium in Spent Fuel Assemblies  

SciTech Connect (OSTI)

Neutron resonance transmission analysis (NRTA) is an active-interrogation nondestructive assay (NDA) technique capable of assaying spent nuclear fuel to determine plutonium content. Prior experimental work has definitively shown the technique capable of assaying plutonium isotope composition in spent-fuel pins to a precision of approximately 3%, with a spatial resolution of a few millimeters. As a Grand Challenge to investigate NDA options for assaying spent fuel assemblies (SFAs) in the commercial fuel cycle, Idaho National Laboratory has explored the feasibility of using NRTA to assay plutonium in a whole SFA. The goal is to achieve a Pu assay precision of 1%. The NRTA technique uses low-energy neutrons from 0.1-40 eV, at the bottom end of the actinide-resonance range, in a time-of-flight arrangement. Isotopic composition is determined by relating absorption of the incident neutrons to the macroscopic cross-section of the actinides of interest in the material, and then using this information to determine the areal density of the isotopes in the SFA. The neutrons used for NRTA are produced using a pulsed, accelerator-based neutron source. Distinguishable resonances exist for both the plutonium (239,240,241,242Pu) and uranium (235,236,238U) isotopes of interest in spent fuel. Additionally, in this energy range resonances exists for six important fission products (99Tc, 103Rh, 131Xe, 133Cs, 145Nd, and 152Sm) which provide additional information to support spent fuel plutonium assay determinations. Based on extensive modeling of the problem using Monte Carlo-based simulation codes, our preliminary results suggest that by rotating an SFA to acquire four symmetric views, sufficient neutron transmission can be achieved to assay a SFA. In this approach multiple scan information for the same pins may also be unfolded to potentially allow the determination of plutonium for sub-regions of the assembly. For a 17 ? 17 pressurized water reactor SFA, a simplistic preliminary analysis indicates the mass of 239Pu may be determined with a precision on the order of 5%, without the need for operator-supplied fuel information or operational histories. This paper will present our work to date on this topic, indicate our preliminary findings for a conceptual assay approach, discuss resilience against spoofing, and outline our future plans for evaluating the NRTA technique for SFA plutonium determination.

D. L. Chichester; J. W. Sterbentz

2012-07-01T23:59:59.000Z

269

EIS-0250: Geologic Repository for the Disposal of Spent Nuclear Fuel and  

Broader source: Energy.gov (indexed) [DOE]

EIS-0250: Geologic Repository for the Disposal of Spent Nuclear EIS-0250: Geologic Repository for the Disposal of Spent Nuclear Fuel and High-Level Radioactive Waste at Yucca Mountain, Nye County, Nevada EIS-0250: Geologic Repository for the Disposal of Spent Nuclear Fuel and High-Level Radioactive Waste at Yucca Mountain, Nye County, Nevada Summary This EIS analyzes DOE's proposed action to construct, operate, monitor, and eventually close a geologic repository at Yucca Mountain for the disposal of spent nuclear fuel and high-level radioactive waste. The EIS evaluates not only impacts from constructing, operating, monitoring, and closing a repository, but also from transporting the materials from 72 commercial and 4 DOE sites to the Yucca Mountain repository site in Nye County, Nevada. Public Comment Opportunities

270

Compatibility Analysis on Existing Reactivity Devices in CANDU 6 Reactors for DUPIC Fuel Cycle  

SciTech Connect (OSTI)

The performance of reactivity devices for a Canada deuterium uranium (CANDU) 6 reactor loaded with Direct Use of Spent Pressurized Water Reactor Fuel In CANDU reactors (DUPIC) fuel is assessed. The reactivity devices studied are the zone controller units, the adjuster rods, and the mechanical control absorbers. For the zone controller system, the bulk reactivity control, spatial power control, and damping capability for spatial oscillation are investigated. For the adjusters, the xenon override, restart after a poison-out, shim operation, and power step-back capabilities are confirmed. The mechanical control absorber is assessed for the function of compensating temperature reactivity feedback following a power reduction. This study shows that the current reactivity device system of a CANDU 6 reactor is compatible with DUPIC fuel for normal and transient operations.

Jeong, Chang-Joon; Choi, Hangbok [Korea Atomic Energy Research Institute (Korea, Republic of)

2000-03-15T23:59:59.000Z

271

Nuclear reactors and the nuclear fuel cycle  

SciTech Connect (OSTI)

According to the author, the first sustained nuclear fission chain reaction was not at the University of Chicago, but at the Oklo site in the African country of Gabon. Proof of this phenomenon is provided by mass spectrometric and analytical chemical measurements by French scientists. The U.S. experience in developing power-producing reactors and their related fuel and fuel cycles is discussed.

Pearlman, H

1989-11-01T23:59:59.000Z

272

Spent fuel sabotage aerosol ratio program : FY 2004 test and data summary.  

SciTech Connect (OSTI)

This multinational, multi-phase spent fuel sabotage test program is quantifying the aerosol particles produced when the products of a high energy density device (HEDD) interact with and explosively particulate test rodlets that contain pellets of either surrogate materials or actual spent fuel. This program has been underway for several years. This program provides data that are relevant to some sabotage scenarios in relation to spent fuel transport and storage casks, and associated risk assessments. The program also provides significant technical and political benefits in international cooperation. We are quantifying the Spent Fuel Ratio (SFR), the ratio of the aerosol particles released from HEDD-impacted actual spent fuel to the aerosol particles produced from surrogate materials, measured under closely matched test conditions, in a contained test chamber. In addition, we are measuring the amounts, nuclide content, size distribution of the released aerosol materials, and enhanced sorption of volatile fission product nuclides onto specific aerosol particle size fractions. These data are the input for follow-on modeling studies to quantify respirable hazards, associated radiological risk assessments, vulnerability assessments, and potential cask physical protection design modifications. This document includes an updated description of the test program and test components for all work and plans made, or revised, during FY 2004. It also serves as a program status report as of the end of FY 2004. All available test results, observations, and aerosol analyses plus interpretations--primarily for surrogate material Phase 2 tests, series 2/5A through 2/9B, using cerium oxide sintered ceramic pellets are included. Advanced plans and progress are described for upcoming tests with unirradiated, depleted uranium oxide and actual spent fuel test rodlets. This spent fuel sabotage--aerosol test program is coordinated with the international Working Group for Sabotage Concerns of Transport and Storage Casks (WGSTSC) and supported by both the U.S. Department of Energy and the Nuclear Regulatory Commission.

Brucher, Wenzel (Gesellschaft fur Anlagen- und Reaktorsicherheit, Germany); Koch, Wolfgang (Fraunhofer Institut fur Toxikologie und Experimentelle Medizin, Germany); Pretzsch, Gunter Guido (Gesellschaft fur Anlagen- und Reaktorsicherheit, Germany); Loiseau, Olivier (Institut de Radioprotection et de Surete Nucleaire, France); Mo, Tin (U.S. Nuclear Regulatory Commission, Washington, DC); Billone, Michael C. (Argonne National Laboratory, Argonne, IL); Autrusson, Bruno A. (Institut de Radioprotection et de Surete Nucleaire, France); Young, F. I. (U.S. Nuclear Regulatory Commission, Washington, DC); Coats, Richard Lee; Burtseva, Tatiana (Argonne National Laboratory, Argonne, IL); Luna, Robert Earl; Dickey, Roy R.; Sorenson, Ken Bryce; Nolte, Oliver (Fraunhofer Institut fur Toxikologie und Experimentelle Medizin, Germany); Thompson, Nancy Slater (U.S. Department of Energy, Washington, DC); Hibbs, Russell S. (U.S. Department of Energy, Washington, DC); Gregson, Michael Warren; Lange, Florentin (Gesellschaft fur Anlagen- und Reaktorsicherheit, Germany); Molecke, Martin Alan; Tsai, Han-Chung (Argonne National Laboratory, Argonne, IL)

2005-07-01T23:59:59.000Z

273

Hydrogen Storage by Boron?Nitrogen Heterocycles: A Simple Route for Spent Fuel Regeneration  

Science Journals Connector (OSTI)

We describe a new hydrogen storage platform based on well-defined BN heterocyle materials. Specifically, we demonstrate that regeneration of the spent fuel back to the charged fuel can be accomplished using molecular H2 and H?/H+ sources. Crystallographic ...

Patrick G. Campbell; Lev N. Zakharov; Daniel J. Grant; David A. Dixon; Shih-Yuan Liu

2010-02-19T23:59:59.000Z

274

Recovery of minor actinides from spent fuel using TPEN-immobilized gels  

SciTech Connect (OSTI)

A series of separation experiments was performed in order to study the recovery process for minor actinides (MAs), such as americium (Am) and curium (Cm), from the actual spent fuel by using an extraction chromatographic technique. N,N,N',N'-tetrakis-(4-propenyloxy-2-pyridylmethyl) ethylenediamine (TPPEN) is an N,N,N',N'-tetrakis (2-pyridylmethyl) ethylenediamine (TPEN) analogue consisting of an incorporated pyridine ring that acts as not only a ligand but also as a site for polymerization and crosslinking of the gel. The TPPEN and N-isopropylacrylamide (NIPA) were dissolved into dimethylformamide (DMF, Wako Co., Ltd.) and a silica beads polymer, and then TTPEN was immobilized chemically in a polymer gel (so called TPEN-gel). Mixed oxide (MOX) fuel, which was highly irradiated up to 119 GWD/MTM in the experimental fast reactor Joyo, was used as a reference spent fuel. First, uranium (U) and plutonium (Pu) were separated from the irradiated fuel using an ion-exchange method, and then, the platinum group elements were removed by CMPO to leave a mixed solution of MAs and lanthanides. The 3 mol% TPPEN-gel was packed with as an extraction column (CV: 1 ml) and then rinsed by 0.1 M NaNO{sub 3}(pH 4.0) for pH adjustment. After washing the column by 0.01 M NaNO{sub 3} (pH 4.0), Eu was detected and the recovery rate reached 93%. The MAs were then recovered by changing the eluent to 0.01 M NaNO{sub 3} (pH 2.0), and the recovery rate of Am was 48 %. The 10 mol% TPPEN-gel was used to improve adsorption coefficient of Am and a condition of eluent temperature was changed in order to confirm the temperature swing effect on TPEN-gel for MA. More than 90% Eu was detected in the eluent after washing with 0.01 M NaNO{sub 3} (pH 3.5) at 5 Celsius degrees. Americium was backwardly detected and eluted continuously during the same condition. After removal of Eu, the eluent temperature was changed to 32 Celsius degrees, then Am was detected (pH 3.0). Finally remained Am could be stripped from TPPEN-gel by changing the pH of the eluent to 2.0. These results These results prove that the proposed recovery process for MAs is a potential candidate for future reprocessing methods based on the extraction chromatographic technique. (authors)

Koyama, S.; Suto, M.; Ohbayashi, H. [Oarai Research and Development Center, Japan Atomic Energy Agency, Oarai (Japan); Oaki, H. [Solutions Research Organization, Tokyo Institute of Technology, Tokyo (Japan); Takeshita, K. [Research Laboratory for Nuclear Reactors, Tokyo Institute of Technology, Tokyo (Japan)

2013-07-01T23:59:59.000Z

275

Simplified Reference Electrode for Electrorefining of Spent Nuclear Fuel in High Temperature Molten Salt  

SciTech Connect (OSTI)

Pyrochemical processing plays an important role in development of proliferation- resistant nuclear fuel cycles. At the Idaho National Laboratory (INL), a pyrochemical process has been implemented for the treatment of spent fuel from the Experimental Breeder Reactor II (EBR-II) in the last decade. Electrorefining in a high temperature molten salt is considered a signature or central technology in pyroprocessing fuel cycles. Separation of actinides from fission products is being demonstrated by electrorefining the spent fuel in a molten UCl3-LiCl-KCl electrolyte in two engineering scale electrorefiners (ERs). The electrorefining process is current controlled. The reference electrode provides process information through monitoring of the voltage difference between the reference and the anode and cathode electrodes. This information is essential for monitoring the reactions occurring at the electrodes, investigating separation efficiency, controlling the process rate, and determining the process end-point. The original reference electrode has provided good life expectancy and signal stability, but is not easily replaceable. The reference electrode used a vycor-glass ion-permeable membrane containing a high purity silver wire with one end positioned in ~2 grams of LiCl/KCl salt electrolyte with a low concentration (~1%) AgCl. It was, however, a complex assembly requiring specialized skill and talent to fabricate. The construction involved multiple small pieces, glass joints, ceramic to glass joints, and ceramic to metal joints all assembled in a high purity inert gas environment. As original electrodes reached end-of-life it was uncertain if the skills and knowledge were readily available to successfully fabricate replacements. Experimental work has been conducted to identify a simpler electrode design while retaining the needed long life and signal stability. This improved design, based on an ion-permeable membrane of mullite has been completed. Use of the silver wire and electrolyte composition remains the same. The resulting design maximizes the use of commercial components and can be fabricated with commonly available skills. This has resulted in a significant reduction of effort and cost to fabricate replacements. The piece count requiring assembly in a high purity glove box atmosphere has been reduced by over half and all specialized joints have been eliminated. The new design has been tested in a lab scale electrorefiner and has also been successfully scaled up and installed in the engineering scale electrorefiners.

Kim Davies; Shelly X Li

2007-09-01T23:59:59.000Z

276

Criticality safety considerations in the geologic disposal of spent nuclear fuel assemblies  

SciTech Connect (OSTI)

Features of geologic disposal which hamper the demonstration that criticality cannot occur therein include possible changes of shape and form, intrusion of water as a neutron moderator, and selective leaching of spent fuel constituents. If the criticality safety of spent fuel disposal depends on burnup, independent measurements verifying the burnup should be performed prior to disposal. The status of nondestructive analysis method which might provide such verification is discussed. Calculations were performed to assess the potential for increasing the allowed size of a spent fuel disposal canister if potential water intrusion were limited by close-packing the enclosed rods. Several factors were identified which severely limited the potential of this application. The theoretical limit of hexagonal close-packing cannot be achieved due to fuel rod bowing. It is concluded that disposal canisters should be sized on the basis of assumed optimum moderation. Several topics for additional research were identified during this limited study.

Gore, B.F.; McNair, G.W.; Heaberlin, S.W.

1980-05-01T23:59:59.000Z

277

Spent Fuel and High-Level Waste Requirements (Maine) | Department of Energy  

Broader source: Energy.gov (indexed) [DOE]

Spent Fuel and High-Level Waste Requirements (Maine) Spent Fuel and High-Level Waste Requirements (Maine) Spent Fuel and High-Level Waste Requirements (Maine) < Back Eligibility Agricultural Commercial Construction Fed. Government Fuel Distributor General Public/Consumer Industrial Installer/Contractor Institutional Investor-Owned Utility Local Government Low-Income Residential Multi-Family Residential Municipal/Public Utility Nonprofit Residential Retail Supplier Rural Electric Cooperative Schools State/Provincial Govt Systems Integrator Transportation Tribal Government Utility Program Info State Maine Program Type Safety and Operational Guidelines Provider Public Utilities Commission All proposed nuclear power generation facilities must be certified by the Public Utilities Commission under this statute prior to construction and

278

Parametric Analysis of PWR Spent Fuel Depletion Parameters for Long-Term-Disposal Criticality Safety  

SciTech Connect (OSTI)

Utilization of burnup credit in criticality safety analysis for long-term disposal of spent nuclear fuel allows improved design efficiency and reduced cost due to the large mass of fissile material that will be present in the repository. Burnup-credit calculations are based on depletion calculations that provide a conservative estimate of spent fuel contents (in terms of criticality potential), followed by criticality calculations to assess the value of the effective neutron multiplication factor (k(sub)eff) for the a spent fuel cask or a fuel configuration under a variety of probabilistically derived events. In order to ensure that the depletion calculation is conservative, it is necessary to both qualify and quantify assumptions that can be made in depletion models.

DeHart, M.D.

1999-08-01T23:59:59.000Z

279

Calculation Method for the Projection of Future Spent Nuclear Fuel Discharges  

SciTech Connect (OSTI)

This report describes the calculation method developed for the projection of future utility spent nuclear fuel (SNF) discharges in regard to their timing, quantity, burnup, and initial enrichment. This projection method complements the utility-supplied RW-859 data on historic discharges and short-term projections of SNF discharges by providing long-term projections that complete the total life cycle of discharges for each of the current U.S. nuclear power reactors. The method was initially developed in mid-1999 to update the SNF discharge projection associated with the 1995 RW-859 utility survey (CRWMS M&O 1996). and was further developed as described in Rev. 00 of this report (CRWMS M&O 2001a). Primary input to the projection of SNF discharges is the utility projection of the next five discharges from each nuclear unit, which is provided via the revised final version of the Energy Information Administration (EIA) 1998 RW-859 utility survey (EIA 2000a). The projection calculation method is implemented via a set of Excel 97 spreadsheets. These calculations provide the interface between receipt of the utility five-discharge projections that are provided in the RW-859 survey, and the delivery of projected life-cycle SNF discharge quantities and characteristics in the format requisite for performing logistics analysis to support design of the Civilian Radioactive Waste Management System (CRWMS). Calculation method improvements described in this report include the addition of a reactor-specific maximum enrichment-based discharge burnup limit. This limit is the consequence of the enrichment limit, currently 5 percent. which is imposed as a Nuclear Regulatory Commission (NRC) license condition on nuclear fuel fabrication plants. In addition, the calculation method now includes the capability for projecting future nuclear plant power upratings, consistent with many such recent plant uprates and the prospect of additional future uprates. Finally. this report summarizes the results of the 2002 Reference SNF Discharge Projection.

B. McLeod

2002-02-28T23:59:59.000Z

280

Verification of plutonium content in spent fuel assemblies using neutron self-interrogation  

SciTech Connect (OSTI)

The large amounts of plutonium in reactor spent fuel assemblies has led to increased research directed toward the measurement of the plutonium for safeguards verification. The high levels of fission product gamma-ray activity and curium neutron backgrounds have made the plutonium measurement difficult. We have developed a new technique that can directly measure both the {sup 235}U concentration and the plutonium fissile concentration using the intrinsic neutron emission fronl the curium in the fuel assembly. The passive neutron albedo reactivity (PNAR) method has been described previously where the curium neutrons are moderated in the surrounding water and reflect back into the fuel assembly to induce fissions in the fissile material in the assembly. The cadmium (Cd) ratio is used to separate the spontaneous fission source neutrons from the reflected thermal neutron fission reactions. This method can measure the sum of the {sup 235}U and the plutonium fissile mass, but not the separate components. Our new differential die-away self-interrogation method (DDSI) can be used to separate the {sup 235}U from the {sup 239}Pu. The method has been applied to both fuel rods and full assemblies. For fuel rods the epi-thermal neutron reflection method filters the reflected neutrons through thin Cd filters so that the reflected neutrons are from the epi-cadmium energy region. The neutron fission energy response in the epi-cadmium region is distinctly different for {sup 235}U and {sup 239}Pu. We are able to measure the difference between {sup 235}U and {sup 239}Pu by sampling the neutron induced fission rate as a function of time and multiplicity after the initial fission neutron is detected. We measure the neutron fission rate using list-mode data collection that stores the time correlations between all of the counts. The computer software can select from the data base the time correlations that include singles, doubles, and triples. The die-away time for the doubles distribution is distinctly different for {sup 235}U and {sup 239}Pu. The {sup 239}Pu has a higher fission cross-section in the epi-cadmium neutron region and larger induced fission moments than {sup 235}U, so the measured die-away time can provide the relative amounts of {sup 239}Pu and {sup 235}U. This paper will present the Monte Carlo simulations for the detector and sample configurations for both fuel pins and full fuel assemblies.

Menlove, Howard O [Los Alamos National Laboratory; Menlove, Apencer H [Los Alamos National Laboratory; Tobin, Stephen J [Los Alamos National Laboratory

2009-01-01T23:59:59.000Z

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281

PLUTONIUM METALLIC FUELS FOR FAST REACTORS  

SciTech Connect (OSTI)

Early interest in metallic plutonium fuels for fast reactors led to much research on plutonium alloy systems including binary solid solutions with the addition of aluminum, gallium, or zirconium and low-melting eutectic alloys with iron and nickel or cobalt. There was also interest in ternaries of these elements with plutonium and cerium. The solid solution and eutectic alloys have most unusual properties, including negative thermal expansion in some solid-solution alloys and the highest viscosity known for liquid metals in the Pu-Fe system. Although metallic fuels have many potential advantages over ceramic fuels, the early attempts were unsuccessful because these fuels suffered from high swelling rates during burn up and high smearing densities. The liquid metal fuels experienced excessive corrosion. Subsequent work on higher-melting U-PuZr metallic fuels was much more promising. In light of the recent rebirth of interest in fast reactors, we review some of the key properties of the early fuels and discuss the challenges presented by the ternary alloys.

STAN, MARIUS [Los Alamos National Laboratory; HECKER, SIEGFRIED S. [Los Alamos National Laboratory

2007-02-07T23:59:59.000Z

282

Comparison of selected foreign plans and practices for spent fuel and high-level waste management  

SciTech Connect (OSTI)

This report describes the major parameters for management of spent nuclear fuel and high-level radioactive wastes in selected foreign countries as of December 1989 and compares them with those in the United States. The foreign countries included in this study are Belgium, Canada, France, the Federal Republic of Germany, Japan, Sweden, Switzerland, and the United Kingdom. All the countries are planning for disposal of spent fuel and/or high-level wastes in deep geologic repositories. Most countries (except Canada and Sweden) plan to reprocess their spent fuel and vitrify the resultant high-level liquid wastes; in comparison, the US plans direct disposal of spent fuel. The US is planning to use a container for spent fuel as the primary engineered barrier. The US has the most developed repository concept and has one of the earliest scheduled repository startup dates. The repository environment presently being considered in the US is unique, being located in tuff above the water table. The US also has the most prescriptive regulations and performance requirements for the repository system and its components. 135 refs., 8 tabs.

Schneider, K.J.; Mitchell, S.J.; Lakey, L.T.; Johnson, A.B. Jr.; Hazelton, R.F.; Bradley, D.J.

1990-04-01T23:59:59.000Z

283

Natural Fueling of a Tokamak Fusion Reactor  

E-Print Network [OSTI]

A natural fueling mechanism that helps to maintain the main core deuterium and tritium (DT) density profiles in a tokamak fusion reactor is discussed. In H-mode plasmas dominated by ion- temperature gradient (ITG) driven turbulence, cold DT ions near the edge will naturally pinch radially inward towards the core. This mechanism is due to the quasi-neutral heat flux dominated nature of ITG turbulence and still applies when trapped and passing kinetic electron effects are included. Fueling using shallow pellet injection or supersonic gas jets is augmented by an inward pinch of could DT fuel. The natural fueling mechanism is demonstrated using the three-dimensional toroidal electromagnetic gyrokinetic turbulence code GEM and is analyzed using quasilinear theory. Profiles similar to those used for conservative ITER transport modeling that have a completely flat density profile are examined and it is found that natural fueling actually reduces the linear growth rates and energy transport.

Wan, Weigang; Chen, Yang; Perkins, Francis W

2009-01-01T23:59:59.000Z

284

Head-end process for the reprocessing of HTGR spent fuel  

SciTech Connect (OSTI)

The reprocessing of HTGR spent fuels is in favor of the sustainable development of nuclear energy to realize the maximal use of nuclear resource and the minimum disposal of nuclear waste. The head-end of HTGR spent fuels reprocessing is different from that of the LWR spent fuels reprocessing because of the difference of spent fuel structure. The dismantling of the graphite spent fuel element and the highly effective dissolution of fuel kernel is the most difficult process in the head end of the reprocessing. Recently, some work on the head-end has been done in China. First, the electrochemical method with nitrate salt as electrolyte was studied to disintegrate the graphite matrix from HTGR fuel elements and release the coated fuel particles, to provide an option for the head-end technology of reprocessing. The results show that the graphite matrix can be effectively separated from the coated particle without any damage to the SiC layer. Secondly, the microwave-assisted heating was applied to dissolve the UO{sub 2} kernel from the crashed coated fuel particles. The ceramic UO{sub 2} as the solute has a good ability to absorb the microwave energy. The results of UO{sub 2} kernel dissolution from crushed coated particles by microwave heating show that the total dissolution percentage of UO{sub 2} is more than 99.99% after 3 times cross-flow dissolution with the following parameters: 8 mol/L HNO{sub 3}, temperature 100 Celsius degrees, initial ratio of solid to liquid 1.2 g/ml. (authors)

Chen, J.; Wen, M. [Institute of Nuclear and New Energy Technology, Tsinghua University, Bejing 10084 (China)

2013-07-01T23:59:59.000Z

285

Comparative Fuel Cycle Analysis of Critical and Subcritical Fast Reactor Transmutation Systems  

SciTech Connect (OSTI)

Fuel cycle analyses are performed to evaluate the impacts of further transmutation of spent nuclear fuel on high-level and low-level waste mass flows into repositories, on the composition and toxicity of the high-level waste, on the capacity of high-level waste repositories, and on the proliferation resistance of the high-level waste. Storage intact of light water reactor (LWR) spent nuclear fuel, a single recycle in a LWR of the plutonium as mixed-oxide fuel, and the repeated recycle of the transuranics in critical and subcritical fast reactors are compared with the focus on the waste management performance of these systems. Other considerations such as cost and technological challenges were beyond the scope of this study. The overall conclusion of the studies is that repeated recycling of the transuranics from spent nuclear fuel would significantly increase the capacity of high-level waste repositories per unit of nuclear energy produced, significantly increase the nuclear energy production per unit mass of uranium ore mined, significantly reduce the radiotoxicity of the waste streams per unit of nuclear energy produced, and significantly enhance the proliferation resistance of the material stored in high-level waste repositories.

Hoffman, Edward A.; Stacey, Weston M. [Georgia Institute of Technology (United States)

2003-10-15T23:59:59.000Z

286

Development of a techno-economic model to optimization DOE spent nuclear fuel disposition  

SciTech Connect (OSTI)

The purpose of the National Spent Nuclear Fuel (NSNF) Program conducted by Lockheed Martin Idaho Technology Co. (LMITCO) at the Idaho National Engineering and Environmental Laboratory (INEEL) is to evaluate what to do with the spent nuclear fuel (SNF) in the Department of Energy (DOE) complex. Final disposition of the SNF may require that the fuel be treated to minimize material concerns. The treatments may range from electrometallurgical treatment and chemical dissolution to engineering controls. Treatment options and treatment locations will depend on the fuel type and the current locations of the fuel. One of the first steps associated with selecting one or more sites for treating the SNF in the DOE complex is to determine the cost of each option. An economic analysis will assist in determining which fuel treatment alternative attains the optimum disposition of SNF at the lowest possible cost to the government and the public. For this study, a set of questions was developed for the electrometallurgical treatment process for fuels at several locations. The set of questions addresses all issues associated with the design, construction, and operation of a production facility. A matrix table was developed to determine questions applicable to various fuel treatment options. A work breakdown structure (WBS) was developed to identify a treatment process and costs from initial design to shipment of treatment products to final disposition. Costs will be applied to determine the life-cycle cost of each option. This technique can also be applied to other treatment techniques for treating spent nuclear fuel.

Ramer, R.J.; Plum, M.M.; Adams, J.P.; Dahl, C.A.

1997-11-01T23:59:59.000Z

287

Spent fuel and radioactive waste inventories, projections, and characteristics. Revision 1  

SciTech Connect (OSTI)

Current inventories and characteristics of commercial spent fuels and both commercial and US Department of Energy (DOE) radioactive wastes were compiled through December 31, 1984, based on the most reliable information available from government sources and the open literature, technical reports, and direct contacts. Future waste and spent fuel to be generated through the year 2020 and characteristics of these materials are also presented. The information forecasted is consistent with the expected defense-related and private industrial and institutional activities and the latest DOE/Energy Information Administration (EIA) projections of US commercial nuclear power growth. Materials considered, on a chapter-by-chapter basis, are: spent fuel, high-level waste, transuranic waste, low-level waste, commercial uranium mill tailings, remedial action waste, and decommissioning waste. For each category, current and projected inventories are given through the year 2020, and the radioactivity and thermal power are calculated, based on reported or calculated isotopic compositions.

Not Available

1985-12-01T23:59:59.000Z

288

Integrated data base for 1993: US spent fuel and radioactive waste inventories, projections, and characteristics. Revision 9  

SciTech Connect (OSTI)

The Integrated Data Base (IDB) Program has compiled historic data on inventories and characteristics of both commercial and DOE spent fuel; also, commercial and U.S. government-owned radioactive wastes through December 31, 1992. These data are based on the most reliable information available from government sources, the open literature, technical reports, and direct contacts. The information forecasted is consistent with the latest U.S. Department of Energy/Energy Information Administration (DOE/EIA) projections of U.S. commercial nuclear power growth and the expected DOE-related and private industrial and institutional (I/I) activities. The radioactive materials considered, on a chapter-by-chapter basis, are spent nuclear fuel, high-level waste (HLW), transuranic (TRU), waste, low-level waste (LLW), commercial uranium mill tailings, environmental restoration wastes, commercial reactor and fuel-cycle facility decommissioning wastes, and mixed (hazardous and radioactive) LLW. For most of these categories, current and projected inventories are given through the calendar-year (CY) 2030, and the radioactivity and thermal power are calculated based on reported or estimated isotopic compositions. In addition, characteristics and current inventories are reported for miscellaneous radioactive materials that may require geologic disposal.

Klein, J.A.; Storch, S.N.; Ashline, R.C. [and others

1994-03-01T23:59:59.000Z

289

Integrated Data Base report--1993: U.S. spent nuclear fuel and radioactive waste inventories, projections, and characteristics. Revision 10  

SciTech Connect (OSTI)

The Integrated Data Base Program has compiled historic data on inventories and characteristics of both commercial and DOE spent nuclear fuel; also, commercial and US government-owned radioactive wastes through December 31, 1993. These data are based on the most reliable information available from government sources, the open literature, technical reports, and direct contacts. The information forecasted is consistent with the latest US Department of Energy/Energy Information Administration projections of US commercial nuclear power growth and the expected DOE-related and private industrial and institutional activities. The radioactive materials considered, on a chapter-by-chapter basis, are spent nuclear fuel, high-level waste, transuranic waste, low-level waste, commercial uranium mill tailings, DOE Environmental Restoration Program wastes, commercial reactor and fuel-cycle facility decommissioning wastes, and mixed (hazardous and radioactive) low-level waste. For most of these categories, current and projected inventories are given the calendar-year 2030, and the radioactivity and thermal power are calculated based on reported or estimated isotopic compositions. In addition, characteristics and current inventories are reported for miscellaneous radioactive materials that may require geologic disposal. 256 refs., 38 figs., 141 tabs.

Not Available

1994-12-01T23:59:59.000Z

290

Effects of an oxidizing atmosphere in a spent fuel packaging facility  

SciTech Connect (OSTI)

Sufficient oxidation of spent fuel can cause a cladding breach to propagate, resulting in dispersion of fuel particulates and gaseous radionuclides. The literature for spent fuel oxidation in storage and disposal programs was reviewed to evaluate the effect of an oxidizing atmosphere in a preclosure packaging facility on (1) physical condition of the fuel and (2) operations in the facility. Effects such as cladding breach propagation, cladding oxidation, rod dilation, fuel dispersal, {sup 14}C and {sup 85}Kr release, and crud release were evaluated. The impact of these effects, due to oxidation, upon a spent fuel handling facility is generally predicted to be less than the impact of similar effects due to fuel rod breached during handling in an inert-atmosphere facility. Preliminary temperature limits of 240{degree}C and 227{degree}C for a 2-week or 4-week handling period and 175{degree}C for 2-year lag storage would prevent breach propagation and fuel dispersal. Additional data that are needed to support the assumptions in this analysis or complete the database were identified.

Einziger, R.E.

1991-09-01T23:59:59.000Z

291

An overview of measurement methods for special nuclear material in spent nuclear fuel  

SciTech Connect (OSTI)

Summary results from a survey of nondestructive assay measurement methods applicable to the measurement of the special nuclear material content of spent nuclear fuel are described. The role of nuclear materials measurements in the domestic and international safeguarding of spent nuclear fuel in the United States' federal waste management system has yet to be determined. An understanding of the characteristics and capabilities of the potentially applicable measurement systems should provide valuable information to the developers of the safeguards approaches for the monitored retrievable storage and final disposal systems. The discussion focuses on the general characteristics of the identified direct and indirect measurement methods. 3 refs., 1 tab.

Moran, B.W.; Reich, W.J.

1989-07-01T23:59:59.000Z

292

Retention of neptunium in uranyl alteration phases formed during spent fuel corrosion  

SciTech Connect (OSTI)

Uranyl oxide hydrate phases are known to form during contact of oxide spent nuclear fuel with water under oxidizing conditions; however, less is known about the fate of fission and neutron capture products during this alteration. We describe, the first time, evidence that neptunium can become incorporated into the uranyl secondary phase, dehydrated schoepite (UO{sub 3}{lg_bullet}0.8H{sub 2}O). Based on the long-term durability of natural schoepite, the retention of neptunium in this alteration phase may be significant during spent fuel corrosion in an unsaturated geologic repository.

Buck, E.C.; Finch, R.J.; Finn, P.A.; Bates, J.K.

1997-10-01T23:59:59.000Z

293

COBRA-SFS predictions of single assembly spent fuel heat transfer data  

SciTech Connect (OSTI)

The study reported here is one of several efforts to evaluate and qualify the COBRA-SFS computer code for use in spent fuel storage system thermal analysis. The ability of COBRA-SFS to predict the thermal response of two single assembly spent fuel heat transfer tests was investigated through comparisons of predictions with experimental test data. From these comparisons, conclusions regarding the computational treatment of the physical phenomena occurring within a storage system can be made. This objective was successfully accomplished as reasonable agreement between predictions and data were obtained for the 21 individual test cases of the two experiments.

Lombardo, N.J.; Michener, T.E.; Wheeler, C.L.; Rector, D.R.

1986-04-01T23:59:59.000Z

294

Performance assessment for the geological disposal of Deep Burn spent fuel using TTBX  

SciTech Connect (OSTI)

The behavior of Deep Burn Modular High Temperature Reactor Spent Fuel (DBSF) is investigated in the Yucca Mountain geological repository (YMR) with respect to the annual dose (Sv/yr) delivered to the Reasonably Maximally Exposed Individual (RMEI) from the transport of radionuclides released from the graphite waste matrix. Transport calculations are performed with a novel computer code, TTBX which is capable of modeling transport pathways that pass through heterogeneous geological formations. TTBX is a multi-region extension of the existing single region TTB transport code. Overall the peak annual dose received by the RMEI is seen to be four orders of magnitude lower than the regulatory threshold for exposure, even under pessimistic scenarios. A number of factors contribute to the favorable performance of DBSF. A reduction of one order of magnitude in the peak annual dose received by the RMEI is observed for every order of magnitude increase in the waste matrix lifetime, highlighting the importance of the waste matrix durability and suggesting graphite's utility as a potential waste matrix for the disposal of high-level waste. Furthermore, we see that by incorporating a higher fidelity far-field model the peak annual dose calculated to be received by the RMEI is reduced by two orders of magnitude. By accounting for the heterogeneities of the far field we have simultaneously removed unnecessary conservatisms and improved the fidelity of the transport model. (authors)

Van den Akker, B.P.; Ahn, J. [Department of Nuclear Engineering, University of California, Berkeley, CA 94720 (United States)

2013-07-01T23:59:59.000Z

295

Summary of Preliminary Criticality Analysis for Peach Bottom Fuel in the DOE Standardized Spent Nuclear Fuel Canister  

SciTech Connect (OSTI)

The Department of Energy's (DOE's) National Spent Nuclear Fuel Program is developing a standardized set of canisters for DOE spent nuclear fuel (SNF). These canisters will be used for DOE SNF handling, interim storage, transportation, and disposal in the national repository. Several fuels are being examined in conjunction with the DOE SNF canisters. This report summarizes the preliminary criticality safety analysis that addresses general fissile loading limits for Peach Bottom graphite fuel in the DOE SNF canister. The canister is considered both alone and inside the 5-HLW/DOE Long Spent Fuel Co-disposal Waste Package, and in intact and degraded conditions. Results are appropriate for a single DOE SNF canister. Specific facilities, equipment, canister internal structures, and scenarios for handling, storage, and transportation have not yet been defined and are not evaluated in this analysis. The analysis assumes that the DOE SNF canister is designed so that it maintains reasonable geometric integrity. Parameters important to the results are the canister outer diameter, inner diameter, and wall thickness. These parameters are assumed to have nominal dimensions of 45.7-cm (18.0-in.), 43.815-cm (17.25-in), and 0.953-cm (0.375-in.), respectively. Based on the analysis results, the recommended fissile loading for the DOE SNF canister is 13 Peach Bottom fuel elements if no internal steel is present, and 15 Peach Bottom fuel elements if credit is taken for internal steel.

Henrikson, D.J.

1999-09-01T23:59:59.000Z

296

REGIONAL BINNING FOR CONTINUED STORAGE OF SPENT NUCLEAR FUEL AND HIGH-LEVEL WASTES  

SciTech Connect (OSTI)

In the Continued Storage Analysis Report (CSAR) (Reference 1), DOE decided to analyze the environmental consequences of continuing to store the commercial spent nuclear fuel (SNF) at 72 commercial nuclear power sites and DOE-owned spent nuclear fuel and high-level waste at five Department of Energy sites by region rather than by individual site. This analysis assumes that three commercial facilities pairs--Salem and Hope Creek, Fitzpatrick and Nine-Mile Point, and Dresden and Moms--share common storage due to their proximity to each other. The five regions selected for this analysis are shown on Figure 1. Regions 1, 2, and 3 are the same as those used by the Nuclear Regulatory Commission in their regulatory oversight of commercial power reactors. NRC Region 4 was subdivided into two regions to more appropriately define the two different climates that exist in NRC Region 4. A single hypothetical site in each region was assumed to store all the SNF and HLW in that region. Such a site does not exist and has no geographic location but is a mathematical construct for analytical purposes. To ensure that the calculated results for the regional analyses reflect appropriate inventory, facility and material degradation, and radionuclide transport, the waste inventories, engineered barriers, and environmental conditions for the hypothetical sites were developed from data for each of the existing sites within the given region. Weighting criteria to account for the amount and types of SNF and HLW at each site were used in the development of the environmental data for the regional site, such that the results of the analyses for the hypothetical site were representative of the sum of the results of each actual site if they had been modeled independently. This report defines the actual site data used in development of this hypothetical site, shows how the individual site data was weighted to develop the regional site, and provides the weighted data used in the CSAR analysis. It is divided into Part 1 that defines time-dependent releases from each regional site, Part 2 that defines transport conditions through the groundwater, and Part 3 that defines transport through surface water and populations using the surface waters for drinking.

W. Lee Poe, Jr

1998-10-01T23:59:59.000Z

297

TOPICAL REPORT ON ACTINIDE-ONLY BURNUP CREDIT FOR PWR SPENT NUCLEAR FUEL PACKAGES  

SciTech Connect (OSTI)

A methodology for performing and applying nuclear criticality safety calculations, for PWR spent nuclear fuel (SNF) packages with actinide-only burnup credit, is described. The changes in the U-234, U-235, U-236, U-238, Pu-238, Pu-239, Pu-240, Pu-241, Pu-242, and Am-241 concentration with burnup are used in burnup credit criticality analyses. No credit for fission product neutron absorbers is taken. The methodology consists of five major steps. (1) Validate a computer code system to calculate isotopic concentrations of SNF created during burnup in the reactor core and subsequent decay. A set of chemical assay benchmarks is presented for this purpose as well as a method for assessing the calculational bias and uncertainty, and conservative correction factors for each isotope. (2) Validate a computer code system to predict the subcritical multiplication factor, k{sub eff}, of a spent nuclear fuel package. Fifty-seven UO{sub 2}, UO{sub 2}/Gd{sub 2}O{sub 3}, and UO{sub 2}/PuO{sub 2} critical experiments have been selected to cover anticipated conditions of SNF. The method uses an upper safety limit on k{sub eff} (which can be a function of the trending parameters) such that the biased k{sub eff}, when increased for the uncertainty is less than 0.95. (3) Establish bounding conditions for the isotopic concentration and criticality calculations. Three bounding axial profiles have been established to assure the ''end effect'' is accounted for conservatively. (4) Use the validated codes and bounding conditions to generate package loading criteria (burnup credit loading curves). Burnup credit loading curves show the minimum burnup required for a given initial enrichment. The utility burnup record is compared to this requirement after the utility accounts for the uncertainty in its record. Separate curves may be generated for each assembly design, various minimum cooling times and burnable absorber histories. (5) Verify that SNF assemblies meet the package loading criteria and confirm proper assembly selection prior to loading. A measurement of the average assembly burnup is required and that measurement must be within 10% of the utility burnup record for the assembly to be accepted. The measurement device must be accurate to within 10%. Each step is described in detail for use with any computer code system and is then demonstrated with the SCALE 4.2 computer code package using 27BURNUPLIB cross sections.

DOE

1997-04-01T23:59:59.000Z

298

Final Report - Spent Nuclear Fuel Retrieval System Manipulator System Cold Validation Testing  

SciTech Connect (OSTI)

Manipulator system cold validation testing (CVT) was performed in support of the Fuel Retrieval System (FRS) Sub-Project, a subtask of the Spent Nuclear Fuel Project at the Hanford Site in Richland, Washington. The FRS will be used to retrieve and repackage K-Basin Spent Nuclear Fuel (SNF) currently stored in old K-Plant storage basins. The FRS is required to retrieve full fuel canisters from the basin; clean the fuel elements inside the canister to remove excessive uranium corrosion products (or sludge); remove the contents from the canisters; and sort the resulting debris, scrap, and fuel for repackaging. The fuel elements and scrap will be collected in fuel storage and scrap baskets in preparation for loading into a multi canister overpack (MCO), while the debris is loaded into a debris bin and disposed of as solid waste. The FRS is composed of three major subsystems. The Manipulator Subsystem provides remote handling of fuel, scrap, and debris; the In-Pool Equipment subsystem performs cleaning of fuel and provides a work surface for handling materials; and the Remote Viewing Subsystem provides for remote viewing of the work area by operators. There are two complete and identical FRS systems, one to be installed in the K-West basin and one to be installed in the K-East basin. Another partial system will be installed in a cold test facility to provide for operator training.

D.R. Jackson; G.R. Kiebel

1999-08-24T23:59:59.000Z

299

SPENT NUCLEAR FUEL STORAGE BASIN WATER CHEMISTRY: ELECTROCHEMICAL EVALUATION OF ALUMINUM CORROSION  

SciTech Connect (OSTI)

The factors affecting the optimal water chemistry of the Savannah River Site spent fuel storage basin must be determines in order to optimize facility efficiency, minimize fuel corrosion, and reduce overall environmental impact from long term spent nuclear fuel storage at the Savannah River Site. The Savannah River National Laboratory is using statistically designed experiments to study the effects of NO{sub 3}{sup -}, SO{sub 4}{sup 2-}, and Cl{sup -} concentrations on alloys commonly used not only as fuel cladding, but also as rack construction materials The results of cyclic polarization pitting and corrosion experiments on samples of Al 6061 and 1100 alloys will be used to construct a predictive model of the basin corrosion and its dependence on the species in the basin. The basin chemistry model and corrosion will be discussed in terms of optimized water chemistry envelope and minimization of cladding corrosion.

Hathcock, D

2007-10-30T23:59:59.000Z

300

A method for determining the spent-fuel contribution to transport cask containment requirements  

SciTech Connect (OSTI)

This report examines containment requirements for spent-fuel transport containers that are transported under normal and hypothetical accident conditions. A methodology is described that estimates the probability of rod failure and the quantity of radioactive material released from breached rods. This methodology characterizes the dynamic environment of the cask and its contents and deterministically models the peak stresses that are induced in spent-fuel cladding by the mechanical and thermal dynamic environments. The peak stresses are evaluated in relation to probabilistic failure criteria for generated or preexisting ductile tearing and material fractures at cracks partially through the wall in fuel rods. Activity concentrations in the cask cavity are predicted from estimates of the fraction of gases, volatiles, and fuel fines that are released when the rod cladding is breached. Containment requirements based on the source term are calculated in terms of maximum permissible volumetric leak rates from the cask. Calculations are included for representative cask designs.

Sanders, T.L.; Seager, K.D. [Sandia National Labs., Albuquerque, NM (United States); Rashid, Y.R.; Barrett, P.R. [ANATECH Research Corp., La Jolla, CA (United States); Malinauskas, A.P. [Oak Ridge National Lab., TN (United States); Einziger, R.E. [Pacific Northwest Lab., Richland, WA (United States); Jordan, H. [EG and G Rocky Flats, Inc., Golden, CO (United States). Rocky Flats Plant; Duffey, T.A.; Sutherland, S.H. [APTEK, Inc., Colorado Springs, CO (United States); Reardon, P.C. [GRAM, Inc., Albuquerque, NM (United States)

1992-11-01T23:59:59.000Z

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


301

Chemical Effects at the Reaction Front in Corroding Spent Nuclear Fuel  

SciTech Connect (OSTI)

Performance assessment models of the U. S. repository at Yucca Mountain, Nevada suggest that neptunium from spent nuclear fuel is a potentially important dose contributor. A scientific understanding of how the UO{sub 2} matrix of spent nuclear fuel impacts the oxidative dissolution and reductive precipitation of Np is needed to predict the behavior of Np at the fuel surface during aqueous corrosion. Neptunium would most likely be transported as aqueous Np(V) species, but for this to occur it must first be oxidized from the Np(IV) state found within the parent spent nuclear fuel. In this paper we present synchrotron X-ray absorption spectroscopy and microscopy findings that illuminate the resultant local chemistry of neptunium and plutonium within uranium oxide spent nuclear fuel before and after corrosive alteration in an air-saturated aqueous environment. We find the Pu and Np in unaltered spent fuel to have a +4 oxidation state and an environment consistent with solid-solution in the UO{sub 2} matrix. During corrosion in an air-saturated aqueous environment, the uranium matrix is converted to uranyl (UO{sub 2}{sup 2+}) mineral assemblage that is depleted in Np and Pu relative to the parent fuel. The transition from U(IV) in the fuel to a fully U(VI) character across the corrosion front is not sharp, but occurs over a transition zone of {approx} 50 micrometers. We find evidence of a thin ({approx} 20 micrometer) layer that is enriched in Pu and Np within a predominantly U(IV) environment on the fuel side of the transition zone. These experimental observations are consistent with available data for the standard reduction potentials for NpO{sub 2}{sup +}/Np{sup 4+} and UO{sub 2}{sup 2+}/U{sup 4+} couples, which indicate that Np(IV) may not be effectively oxidized to Np(V) at the corrosion potential of uranium dioxide spent nuclear fuel in air-saturated aqueous solutions. (authors)

Fortner, Jeffrey A.; Kropf, A. Jeremy; Jerden, James L.; Cunnane, James C. [Chemical Engineering, Argonne National Laboratory, CMT/205, 9700 S. Cass Avenue, Argonne, IL, 60439 (United States)

2007-07-01T23:59:59.000Z

302

Literature on fabrication of tungsten for application in pyrochemical processing of spent nuclear fuels  

SciTech Connect (OSTI)

The pyrochemical processing of nuclear fuels requires crucibles, stirrers, and transfer tubing that will withstand the temperature and the chemical attack from molten salts and metals used in the process. This report summarizes the literature that pertains to fabrication (joining, chemical vapor deposition, plasma spraying, forming, and spinning) is the main theme. This report also summarizes a sampling of literature on molbdenum and the work previously performed at Argonne National Laboratory on other container materials used for pyrochemical processing of spent nuclear fuels.

Edstrom, C.M.; Phillips, A.G.; Johnson, L.D.; Corle, R.R.

1980-10-11T23:59:59.000Z

303

A numerical investigation of natural convection heat transfer within horizontal spent-fuel assemblies  

SciTech Connect (OSTI)

A numerical investigation of natural convection heat transfer is carried out for a single, horizontal, spent-fuel assembly in an environment typical of spent-fuel transportation systems as well as some dry storage/disposal scenarios. The objective is to predict computationally the convective heat transfer trends for horizontal spent fuel and to compare the results to data taken in a supporting experimental effort. The predicted data consist of thermal and flow fields throughout the assembly for a wide range of Rayleigh number, as well as numerically obtained Nusselt-number data that are correlated as a function of Rayleigh number. Both laminar and turbulent approaches are examined for a Boussinesq fluid with Pr = 0.7. The data predict the existence of a conduction-dominated regime, a transition regime, and a convection regime. Compared with the laminar approach, a significant improvement in the predicted Nusselt number is obtained for large Rayleigh numbers when a turbulence model is employed. This lends additional support to the experimental evidence that a transition to turbulent flow occurs for Rayleigh numbers greater than 10{sup 7}. Overall, the numerically predicted heat transfer trends compare well with previously obtained experimental data, and the computed assembly Nusselt numbers generally reside within the range of experimental uncertainty. The predicted thermal and flow fields further provide a numerical flow visualization capability that enhances the understanding of natural convection in horizontal spent fuel and allows improved physical interpretation of the experimental data.

Canaan, R.E. [Lawrence Livermore National Lab., CA (United States); Klein, D.E. [Univ. of Texas System, Austin, TX (United States)

1998-08-01T23:59:59.000Z

304

Author's personal copy Cost analysis of the US spent nuclear fuel reprocessing facility  

E-Print Network [OSTI]

of this, a 1987 amendment to the US Nuclear Waste Policy Act mandates the Secretary of Energy to report on a site for a second repository by 2010 (Nuclear Waste Policy Amendments Act, 1987). HoweverAuthor's personal copy Cost analysis of the US spent nuclear fuel reprocessing facility E

Deinert, Mark

305

Review of the natural circulation effect in the Vermont Yankee spent-fuel pool  

SciTech Connect (OSTI)

A 7429-node, three-dimensional computer model of the Vermont Yankee spent-fuel pool was set up and run using the porous media model of the TEMPEST computer code. The results of this analysis show that natural circulation is sufficient to ensure adequate cooling, regardless of the loading pattern used or the orientation of the cooling system discharge nozzle.

Wheeler, C.L.

1988-01-01T23:59:59.000Z

306

Differential die-away technique for determination of the fissile contents in spent fuel assembly  

SciTech Connect (OSTI)

Monte Carlo simulations were performed for the differential die-away (DDA) technique to quantify its capability to measure the fissile contents in spent fuel assemblies of 64 different cases in terms of initial enrichment, burnup, and cooling time. The DDA count rate varies according to the contents of fissile isotopes such as {sup 235}U, {sup 239}Pu, and {sup 241}Pu contained in the spent fuel assembly. The effective {sup 239}Pu concept was introduced to quantify the total fissile mass of spent fuel by weighting the relative signal contributions of {sup 235}U and {sup 241}Pu compared to that of {sup 239}Pu. The Monte Carlo simulation results show that the count rate of the DDA instrument for a spent fuel assembly of 4% initial enrichment, 45 GWD/MTU burnup, and 5 year cooling time is {approx} 9.8 x 10{sup 4} counts per second (c/s) with the 100-Hz repeated interrogation pattern of 0 to 10 {micro}s interrogation, 0.2 ms to 1 ms counting time, and 1 x 10{sup 9} n/s neutron source. The {sup 244}Cm neutron background count rate for this counting time scheme is {approx} 1 x 10{sup 4} c/s, and thus the signal to background ratio is {approx}10.

Lee, Tachoon [Los Alamos National Laboratory; Menlove, Howard O [Los Alamos National Laboratory; Swinhoe, Nartyn T [Los Alamos National Laboratory; Tobin, Stephen J [Los Alamos National Laboratory

2010-01-01T23:59:59.000Z

307

Regulatory Perspective on Potential Fuel Reconfiguration and Its Implication to High Burnup Spent Fuel Storage and Transportation - 13042  

SciTech Connect (OSTI)

The recent experiments conducted by Argonne National Laboratory on high burnup fuel cladding material property show that the ductile to brittle transition temperature of high burnup fuel cladding is dependent on: (1) cladding material, (2) irradiation conditions, and (3) drying-storage histories (stress at maximum temperature) [1]. The experiment results also show that the ductile to brittle temperature increases as the fuel burnup increases. These results indicate that the current knowledge in cladding material property is insufficient to determine the structural performance of the cladding of high burnup fuel after it has been stored in a dry cask storage system for some time. The uncertainties in material property and the elevated ductile to brittle transition temperature impose a challenge to the storage cask and transportation packaging designs because the cask designs may not be able to rely on the structural integrity of the fuel assembly for control of fissile material, radiation source, and decay heat source distributions. The fuel may reconfigure during further storage and/or the subsequent transportation conditions. In addition, the fraction of radioactive materials available for release from spent fuel under normal condition of storage and transport may also change. The spent fuel storage and/or transportation packaging vendors, spent fuel shippers, and the regulator may need to consider this possible fuel reconfiguration and its impact on the packages' ability to meet the safety requirements of Part 72 and Part 71 of Title 10 of the Code of Federal Regulations. The United States Nuclear Regulatory Commission (NRC) is working with the scientists at Oak Ridge National Laboratory (ORNL) to assess the impact of fuel reconfiguration on the safety of the dry storage systems and transportation packages. The NRC Division of Spent Fuel Storage and Transportation has formed a task force to work on the safety and regulatory concerns in relevance to high burnup fuel storage and transportation. This paper discusses the staff's preliminary considerations on the safety implication of fuel reconfiguration with respect to nuclear safety (subcriticality control), radiation shielding, containment, the performance of the thermal functions of the packages, and the retrievability of the contents from regulatory perspective. (authors)

Li, Zhian; Rahimi, Meraj; Tang, David; Aissa, Mourad; Flaganan, Michelle [U.S. Nuclear Regulatory Commission - NRC, Washington, DC 20555-0001 (United States)] [U.S. Nuclear Regulatory Commission - NRC, Washington, DC 20555-0001 (United States); Wagner, John C. [Oak Ridge National Laboratory (United States)] [Oak Ridge National Laboratory (United States)

2013-07-01T23:59:59.000Z

308

Deep Burn: Development of Transuranic Fuel for High-Temperature Helium-Cooled Reactors- Monthly Highlights September 2010  

SciTech Connect (OSTI)

The DB Program monthly highlights report for August 2010, ORNL/TM-2010/184, was distributed to program participants by email on September 17. This report discusses: (1) Core and Fuel Analysis - (a) Core Design Optimization in the HTR (high temperature helium-cooled reactor) Prismatic Design (Logos), (b) Core Design Optimization in the HTR Pebble Bed Design (INL), (c) Microfuel analysis for the DB HTR (INL, GA, Logos); (2) Spent Fuel Management - (a) TRISO (tri-structural isotropic) repository behavior (UNLV), (b) Repository performance of TRISO fuel (UCB); (3) Fuel Cycle Integration of the HTR (high temperature helium-cooled reactor) - Synergy with other reactor fuel cycles (GA, Logos); (4) TRU (transuranic elements) HTR Fuel Qualification - (a) Thermochemical Modeling, (b) Actinide and Fission Product Transport, (c) Radiation Damage and Properties; (5) HTR Spent Fuel Recycle - (a) TRU Kernel Development (ORNL), (b) Coating Development (ORNL), (c) Characterization Development and Support, (d) ZrC Properties and Handbook; and (6) HTR Fuel Recycle - (a) Graphite Recycle (ORNL), (b) Aqueous Reprocessing, (c) Pyrochemical Reprocessing METROX (metal recovery from oxide fuel) Process Development (ANL).

Snead, Lance Lewis [ORNL; Besmann, Theodore M [ORNL; Collins, Emory D [ORNL; Bell, Gary L [ORNL

2010-10-01T23:59:59.000Z

309

Development of a Techno-Economic Model to Optimize DOE Spent Nuclear Fuel Disposition  

SciTech Connect (OSTI)

The National Spent Nuclear Fuel (NSNF) Program is evaluating final disposition of spent nuclear fuel (SNE) in the Department of Energy (DOE) complex. Final disposition of SNF may require that the fuel be treated to minimize material concerns. The treatments may range from electrometallurgical treatment (EMT) and chemical dissolution to engineering controls. Treatment options and treatment locations will depend on fuel type and location of the fuel. One of the first steps associated with selecting one or more sites for treating SNF in the DOE complex is to determine the cost of each option. An economic analysis will assist in determining which fuel treatment alternative attains the optimum disposition of SNF at the lowest possible cost to the government and the public. For this study, a set of questions was developed for the EMT process for fuels at several locations. The set of questions addresses all issues associated with design, construction, and operation of a production facility. A matrix table was developed to determine questions applicable to various fuel treatment options. A work breakdown structure (WBS) was developed to identify a treatment process and costs from initial design to shipment of treatment products to final disposition. Costs can be applied to determine the life cycle cost of each option. This technique can also be applied to other treatment techniques for treating SNF.

Ramer, R. J.; Plum, M. M.; Adams, J. P.; Dahl, C. A.

1998-02-01T23:59:59.000Z

310

Spent fuel sabotage test program, characterization of aerosol dispersal : technical review and analysis supplement.  

SciTech Connect (OSTI)

This project seeks to provide vital data required to assess the consequences of a terrorist attack on a spent fuel transportation cask. One such attack scenario involves the use of conical shaped charges (CSC), which are capable of damaging a spent fuel transportation cask. In the event of such an attack, the amount of radioactivity that may be released as respirable aerosols is not known with great certainty. Research to date has focused on measuring the aerosol release from single short surrogate fuel rodlets subjected to attack by a small CSC device in various aerosol chamber designs. The last series of three experiments tested surrogate fuel rodlets made with depleted uranium oxide ceramic pellets in a specially designed double chamber aerosol containment apparatus. This robust testing apparatus was designed to prevent any radioactive release and allow high level radioactive waste disposal of the entire apparatus following testing of actual spent fuel rodlets as proposed. DOE and Sandia reviews of the project to date identified a number of issues. The purpose of this supplemental report is to address and document the DOE review comments and to resolve the issues identified in the Sandia technical review.

Durbin, Samuel G.; Lindgren, Eric Richard

2009-07-01T23:59:59.000Z

311

Advanced Gas Reactor Fuel Program's TRISO Particle Fuel Sets A New World  

Broader source: Energy.gov (indexed) [DOE]

Advanced Gas Reactor Fuel Program's TRISO Particle Fuel Sets A New Advanced Gas Reactor Fuel Program's TRISO Particle Fuel Sets A New World Record For Irradiation Performance Advanced Gas Reactor Fuel Program's TRISO Particle Fuel Sets A New World Record For Irradiation Performance November 16, 2009 - 1:12pm Addthis As part of the Office of Nuclear Energy's Next Generation Nuclear Plant (NGNP) Program, the Advanced Gas Reactor (AGR) Fuel Development Program has achieved a new international record for irradiation testing of next-generation particle fuel for use in high temperature gas reactors (HTGRs). The AGR Fuel Development Program was initiated by the Department of Energy in 2002 to develop the advanced fabrication and characterization technologies, and provide irradiation and safety performance data required to license TRISO particle fuel for the NGNP and future HTGRs. The AGR

312

Optimizing Treatment Performance of Microbial Fuel Cells by Reactor Staging  

Science Journals Connector (OSTI)

Optimizing Treatment Performance of Microbial Fuel Cells by Reactor Staging ... Multi-unit optimization is a recently proposed method that uses multiple similar units to optimize process performance. ...

Roberto P. Pinto; Boris Tartakovsky; Michel Perrier; Bala Srinivasan

2010-08-18T23:59:59.000Z

313

Development of Technical Nuclear Forensics for Spent Research Reactor Fuel  

E-Print Network [OSTI]

time. The over prediction of cooling time and comparison of different burnup recon- struction isotope results are indicator signatures of extended shutdown or time away from power. Due to dynamic operation in time and function, detailed power his... Burnup From Models of Various Levels of Detail. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 38 3.10 Simulated Assembly Neptunium and Plutonium Mass Results . . . . . . 39 3.11 Simulated Assembly Plutonium Isotopic Results...

Sternat, Matthew Ryan 1982-

2012-11-20T23:59:59.000Z

314

Plutonium recovery from spent reactor fuel by uranium displacement  

DOE Patents [OSTI]

A process is described for separating uranium values and transuranic values from fission products containing rare earth values when the values are contained together in a molten chloride salt electrolyte. A molten chloride salt electrolyte with a first ratio of plutonium chloride to uranium chloride is contacted with both a solid cathode and an anode having values of uranium and fission products including plutonium. A voltage is applied across the anode and cathode electrolytically to transfer uranium and plutonium from the anode to the electrolyte while uranium values in the electrolyte electrolytically deposit as uranium metal on the solid cathode in an amount equal to the uranium and plutonium transferred from the anode causing the electrolyte to have a second ratio of plutonium chloride to uranium chloride. Then the solid cathode with the uranium metal deposited thereon is removed and molten cadmium having uranium dissolved therein is brought into contact with the electrolyte resulting in chemical transfer of plutonium values from the electrolyte to the molten cadmium and transfer of uranium values from the molten cadmium to the electrolyte until the first ratio of plutonium chloride to uranium chloride is reestablished.

Ackerman, J.P.

1992-03-17T23:59:59.000Z

315

Fuel assembly transfer basket for pool type nuclear reactor vessels  

DOE Patents [OSTI]

A fuel assembly transfer basket for a pool type, liquid metal cooled nuclear reactor having a side access loading and unloading port for receiving and relinquishing fuel assemblies during transfer.

Fanning, Alan W. (San Jose, CA); Ramsour, Nicholas L. (San Jose, CA)

1991-01-01T23:59:59.000Z

316

Equipment concepts for dry intercask transfer of spent fuel  

SciTech Connect (OSTI)

This report documents the results of a study of preconceptual design and analysis of four intercask transfer concepts. The four concepts are: a large shielded cylindrical turntable that contains an integral fuel handling machine (turntable concept); a shielded fuel handling machine under which shipping and storage casks are moved horizontally (shuttle concept); a small hot cell containing equipment for transferring fuel between shipping and storage casks (that enter and leave the cell on carts) in a bifurcated trench (trench concept); and a large hot cell, shielded by an earthen berm, that houses equipment for handling fuel between casks that enter and leave the cell on a single cart (igloo concept). The casks considered in this study are most of the transport casks currently operable in the USA, and the storage casks designated REA-2023 and GNS Castor-V. Exclusive of basic services assumed to be provided at the host site, the design and capital costs are estimated to range from $9 to $13 million. The portion of capital costs for portable equipment (for potential later use at another site) was estimated to range from 70% to 98%, depending on the concept. Increasing portability from a range of 70 to 90% to 98% adds $2 to 4 million to the capital costs. Operating costs are estimated at about $2 million/year for all concepts. Implementation times range from about 18 months for the more conventional systems to 40 months for the more unique systems. Times and costs for relocation to another site are 10 to 14 months and about $1 million, plus shipping costs and costs of new construction at the new site. All concepts have estimated capacities for fuel transfer at least equal to the criterion set for this study. Only the hot cell concepts have capability for recanning or repair of canisters. Some development is believed to be required for the turntable and shuttle concepts, but none for the other two concepts.

Schneider, K.J.

1983-07-01T23:59:59.000Z

317

Nuclear-fuel-cycle risk assessment: descriptions of representative non-reactor facilities. Sections 1-14  

SciTech Connect (OSTI)

The Fuel Cycle Risk Assessment Program was initiated to provide risk assessment methods for assistance in the regulatory process for nuclear fuel cycle facilities other than reactors. This report, the first from the program, defines and describes fuel cycle elements that are being considered in the program. One type of facility (and in some cases two) is described that is representative of each element of the fuel cycle. The descriptions are based on real industrial-scale facilities that are current state-of-the-art, or on conceptual facilities where none now exist. Each representative fuel cycle facility is assumed to be located on the appropriate one of four hypothetical but representative sites described. The fuel cycles considered are for Light Water Reactors with once-through flow of spent fuel, and with plutonium and uranium recycle. Representative facilities for the following fuel cycle elements are described for uranium (or uranium plus plutonium where appropriate): mining, milling, conversion, enrichment, fuel fabrication, mixed-oxide fuel refabrication, fuel reprocessing, spent fuel storage, high-level waste storage, transuranic waste storage, spent fuel and high-level and transuranic waste disposal, low-level and intermediate-level waste disposal, and transportation. For each representative facility the description includes: mainline process, effluent processing and waste management, facility and hardware description, safety-related information and potential alternative concepts for that fuel cycle element. The emphasis of the descriptive material is on safety-related information. This includes: operating and maintenance requirements, input/output of major materials, identification and inventories of hazardous materials (particularly radioactive materials), unit operations involved, potential accident driving forces, containment and shielding, and degree of hands-on operation.

Schneider, K.J.

1982-09-01T23:59:59.000Z

318

Nuclear reactor fuel rod attachment system  

DOE Patents [OSTI]

A reusable system for removably attaching a nuclear reactor fuel rod (12) to a support member (14). A locking cap (22) is secured to the fuel rod (12) and a locking strip (24) is fastened to the support member (14). The locking cap (22) has two opposing fingers (24a and 24b) shaped to form a socket having a body portion (26). The locking strip has an extension (36) shaped to rigidly attach to the socket's body portion (26). The locking cap's fingers are resiliently deflectable. For attachment, the locking cap (22) is longitudinally pushed onto the locking strip (24) causing the extension (36) to temporarily deflect open the fingers (24a and 24b) to engage the socket's body portion (26). For removal, the process is reversed.

Christiansen, David W. (Kennewick, WA)

1982-01-01T23:59:59.000Z

319

Environmental Statements, Availability, Etc., Programmatic Spent Nuclear Fuel Management and Idaho National Engineering Laboratory Environmental Restoration and Waste Management Programs  

Broader source: Energy.gov (indexed) [DOE]

8679 8679 Thursday June 1, 1995 Part III Department of Energy Environmental Statements, Availability, Etc.; Programmatic Spent Nuclear Fuel Management and Idaho National Engineering Laboratory Environmental Restoration and Waste Management Programs: Notice 28680 Federal Register / Vol. 60, No. 105 / Thursday, June 1, 1995 / Notices DEPARTMENT OF ENERGY Programmatic Spent Nuclear Fuel Management and Idaho National Engineering Laboratory Environmental Restoration and Waste Management Programs AGENCY: Department of Energy. ACTION: Record of decision. SUMMARY: The Department of Energy has issued a Record of Decision on Programmatic Spent Nuclear Fuel Management and Idaho National Engineering Laboratory Environmental Restoration and Waste Management Programs. The Record of Decision includes a Department-wide decision to

320

Non-destructive assay of spent nuclear fuel using passive neutron Albedo reactivity  

SciTech Connect (OSTI)

Passive Neutron Albedo Reactivity (PNAR) is one of fourteen techniques that has been researched and evaluated to form part of a comprehensive and integrated detection system for the non-destructive assay (NDA) of spent nuclear fuel. PNAR implemented with {sup 3}He tubes for neutron detection (PNAR-{sup 3}He) is the measurement of time correlated neutrons from a spent fuel assembly with and without a Cadmium (Cd) layer surrounding the assembly. PNAR utilizes the self-interrogation of the fuel via reflection of neutrons born in the fuel assembly back in to the fuel assembly. The neutrons originate primarily from spontaneous fission events within the fuel itself (Curium-244) but are amplified by multiplication. The presence and removal of the Cd provides two measurement conditions with different neutron energy spectra and therefore different interrogating neutron characteristics. Cd has a high cross-section of absorption for slow neutrons and therefore greatly reduces the low energy (thermal) neutron fluence rate returning. The ratios of the Singles, Doubles and Triples count rates obtained in each case are known as the Cd ratios, which are related to fissile content. A potential safeguards application for which PNAR-{sup 3}He is particularly suited is 'fingerprinting'. Fingerprinting could function as an alternative to plutonium (Pu) mass determination; providing confidence that material was not diverted during transport between sites. PNAR-{sup 3}He has six primary NDA signatures: Singles, Doubles and Triples count rates measured with two energy spectra at both shipping and receiving sites. This is to uniquely identify the fuel assembly, and confirm no changes have taken place during transport. Changes may indicate all attempt to divert material for example. Here, the physics of the PNAR-{sup 3}He concept will be explained, alongside a discussion on the development of a prototypical PNAR-{sup 3}He instrument using simulation. The capabilities and performance of the conceptual instrument will be summarized, in the context of (a) quantifying Pu mass in spent fuel assemblies and (b) detecting pin diversion (through a discrepancy between declared and measured properties of the fuel assembly) when the instrument is deployed. These quantitative capabilities are complementary to the 'fingerprinting' capability which is part of ensuring continuity of knowledge and custody of spent nuclear fuel.

Evans, L G [Los Alamos National Laboratory; Schear, M A [Los Alamos National Laboratory; Croft, S [Los Alamos National Laboratory; Tobin, S J [Los Alamos National Laboratory; Swinhoe, M T [Los Alamos National Laboratory; Menlove, H O [Los Alamos National Laboratory

2010-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


321

The Chemistry os Spent Nuclear Fuel From X-Ray Absorption Spectroscopy  

SciTech Connect (OSTI)

Present and future nuclear fuel cycles will require an understanding of the complex chemistry of trace fission products and transuranium actinides in spent nuclear fuel (SNF). Because of the unique analytical challenges presented by SNF to the materials scientist, many of its fundamental physical and chemical properties remain poorly understood, especially on the microscopic scale. Such an understanding of the chemical states of radionuclides in SNF would benefit development of technologies for fuel monitoring, fuel performance improvement and modeling, fuel reprocessing, and spent fuel storage and disposal. We have recently demonstrated the use of synchrotron x-ray absorption spectroscopy (XAS) to examine crystal chemical properties of actinides and fission products in extracted specimens of SNF. Information obtained includes oxidation state, chemical bond coordination, and quantitative elemental concentration and distribution. We have also used XAS in a scanning mode to obtain x-ray spectral micrographs with resolution approaching 1 micron. A brief overview of the technique will be presented, along with findings on uranium, plutonium, neptunium, technetium, and molybdenum in commercial PWR SNF specimens.

F.A. Fortner; A.J. Kropf; J.C. Cunnane

2006-09-21T23:59:59.000Z

322

Melted and Granulated Depleted Uranium Dioxide for Use in Containers for Spent Nuclear Fuel  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Melted and Granulated Depleted Uranium Dioxide for Use in Containers for Spent Nuclear Fuel Melted and Granulated Depleted Uranium Dioxide for Use in Containers for Spent Nuclear Fuel Vitaly T. Gotovchikov a , Victor A. Seredenko a , Valentin V. Shatalov a , Vladimir N. Kaplenkov a , Alexander S. Shulgin a , Vladimir K. Saranchin a , Michail A. Borik a∗ , Charles W. Forsberg b , All-Russian Research Institute of Chemical Technology (ARRICT) 33, Kashirskoe ave., Moscow, Russia, 115409, E-mail: chem.conv@ru.net Oak Ridge National Laboratory (ORNL) Bethel Wall Road, P.O. Box 2008, MS-6165, Oak Ridge, TN, USA, 37831 Abstract - Induction cold crucible melters (ICCM) have the potential to be a very-low-cost high-throughput method for the production of DUO 2 for SNF casks. The proposed work would develop these melters for this specific application. If a

323

Non-Destructive Spent Fuel Characterization with Semi-Conducting Gallium Arsinde Neutron Imaging Arrays  

SciTech Connect (OSTI)

High resistivity bulk grown GaAs has been used to produce thermal neutron imaging devices for use in neutron radiography and characterizing burnup in spent fuel. The basic scheme utilizes a portable Sb/Be source for monoenergetic (24 keV) neutron radiation source coupled to an Fe filter with a radiation hard B-coated pixellated GaAs detector array as the primary neutron detector. The coated neutron detectors have been tested for efficiency and radiation hardness in order to determine their fitness for the harsh environments imposed by spent fuel. Theoretical and experimental results are presented, showing detector radiation hardness, expected detection efficiency and the spatial resolution from such a scheme. A variety of advanced neutron detector designs have been explored, with experimental results achieving 13% thermal neutron detection efficiency while projecting the possibility of over 30% thermal neutron detection efficiency.

Douglas S. McGregor; Holly K. Gersch; Jeffrey D. Sanders; John C. Lee; Mark D. Hammig; Michael R. Hartman; Yong Hong Yang; Raymond T. Klann; Brian Van Der Elzen; John T. Lindsay; Philip A. Simpson

2002-01-30T23:59:59.000Z

324

Long-term kinetic effects and colloid formations in dissolution of LWR spent fuels  

SciTech Connect (OSTI)

This report evaluates continuous dissolution and colloid formation during spent-fuel performance under repository conditions in high-level waste disposal. Various observations suggest that reprecipitated layers formed on spent-fuel surfaces may not be protective. This situation may lead to continuous dissolution of highly soluble radionuclides such as C-14, Cl-36, Tc-99, I-129, and Cs-135. However, the diffusion limits of various species involved may retard dissolution significantly. For low-solubility actinides such as Pu-(239+240) or Am-(241+243), various processes regarding colloid formation have been analyzed. The processes analyzed are condensation, dispersion, and sorption. Colloid formation may lead to significant releases of low-solubility actinides. However, because there are only limited data available on matrix dissolution, colloid formation, and solubility limits, many uncertainties still exist. These uncertainties must be addressed before the significance of radionuclide releases can be determined. 118 refs.

Ahn, T.M.

1996-11-01T23:59:59.000Z

325

On the Development of a Distillation Process for the Electrometallurgical Treatment of Irradiated Spent Nuclear Fuel  

SciTech Connect (OSTI)

As part of the spent fuel treatment program at the Idaho National Laboratory, a vacuum distillation process is being employed for the recovery of actinide products following an electrorefining process. Separation of the actinide products from a molten salt electrolyte and cadmium is achieved by a batch operation called cathode processing. A cathode processor has been designed and developed to efficiently remove the process chemicals and consolidate the actinide products for further processing. This paper describes the fundamentals of cathode processing, the evolution of the equipment design, the operation and efficiency of the equipment, and recent developments at the cathode processor. In addition, challenges encountered during the processing of irradiated spent nuclear fuel in the cathode processor will be discussed.

B.R. Westphal; K.C. Marsden; J.C. Price; D.V. Laug

2008-04-01T23:59:59.000Z

326

High Temperature Reactor (HTR) Deep Burn Core and Fuel Analysis: Design Selection for the Prismatic Block Reactor  

SciTech Connect (OSTI)

The Deep Burn (DB) Project is a U.S. Department of Energy sponsored feasibility study of Transuranic Management using high burnup fuel in the high temperature helium cooled reactor (HTR). The DB Project consists of seven tasks: project management, core and fuel analysis, spent fuel management, fuel cycle integration, TRU fuel modeling, TRU fuel qualification, and HTR fuel recycle. In the Phase II of the Project, we conducted nuclear analysis of TRU destruction/utilization in the HTR prismatic block design (Task 2.1), deep burn fuel/TRISO microanalysis (Task 2.3), and synergy with fast reactors (Task 4.2). The Task 2.1 covers the core physics design, thermo-hydraulic CFD analysis, and the thermofluid and safety analysis (low pressure conduction cooling, LPCC) of the HTR prismatic block design. The Task 2.3 covers the analysis of the structural behavior of TRISO fuel containing TRU at very high burnup level, i.e. exceeding 50% of FIMA. The Task 4.2 includes the self-cleaning HTR based on recycle of HTR-generated TRU in the same HTR. Chapter IV contains the design and analysis results of the 600MWth DB-HTR core physics with the cycle length, the average discharged burnup, heavy metal and plutonium consumptions, radial and axial power distributions, temperature reactivity coefficients. Also, it contains the analysis results of the 450MWth DB-HTR core physics and the analysis of the decay heat of a TRU loaded DB-HTR core. The evaluation of the hot spot fuel temperature of the fuel block in the DB-HTR (Deep-Burn High Temperature Reactor) core under full operating power conditions are described in Chapter V. The investigated designs are the 600MWth and 460MWth DB-HTRs. In Chapter VI, the thermo-fluid and safety of the 600MWth DB-HTRs has been analyzed to investigate a thermal-fluid design performance at the steady state and a passive safety performance during an LPCC event. Chapter VII describes the analysis results of the TRISO fuel microanalysis of the 600MWth and 450MWth DB-HTRs. The TRISO fuel microanalysis covers the gas pressure buildup in a coated fuel particle including helium production, the thermo-mechanical behavior of a CFP, the failure probabilities of CFPs, the temperature distribution in a CPF, and the fission product (FP) transport in a CFP and a graphite. In Chapter VIII, it contains the core design and analysis of sodium cooled fast reactor (SFR) with deep burn HTR reactor. It considers a synergistic combination of the DB-MHR and an SFR burner for a safe and efficient transmutation of the TRUs from LWRs. Chapter IX describes the design and analysis results of the self-cleaning (or self-recycling) HTR core. The analysis is considered zero and 5-year cooling time of the spent LWR fuels.

Francesco Venneri; Chang-Keun Jo; Jae-Man Noh; Yonghee Kim; Claudio Filippone; Jonghwa Chang; Chris Hamilton; Young-Min Kim; Ji-Su Jun; Moon-Sung Cho; Hong-Sik Lim; MIchael A. Pope; Abderrafi M. Ougouag; Vincent Descotes; Brian Boer

2010-09-01T23:59:59.000Z

327

Examination of Zircaloy-clad spent fuel after extended pool storage  

SciTech Connect (OSTI)

This report presents the results from metallurgical examinations of Zircaloy-clad fuel rods from two bundles (0551 and 0074) of Shippingport PWR Core 1 blanket fuel after extended water storage. Both bundles were exposed to water in the reactor from late 1957 until discharge. The estimated average burnups were 346 GJ/kgU (4000 MWd/MTU) for bundle 0551 and 1550 GJ/kgU (18,000 MWd/MTU) for bundle 0074. Fuel rods from bundle 0551 were stored in deionized water for nearly 21 yr prior to examination in 1980, representing the world's oldest pool-stored Zircaloy-clad fuel. Bundle 0074 has been stored in deionized water since reactor discharge in 1964. Data from the current metallurgical examinations enable a direct assessment of extended pool storage effects because the metallurgical condition of similar fuel rods was investigated and documented soon after reactor discharge. Data from current and past examinations were compared, and no significant degradation of the Zircaloy cladding was indicated after almost 21 yr in water storage. The cladding dimensions and mechanical properties, fission gas release, hydrogen contents of the cladding, and external oxide film thicknesses that were measured during the current examinations were all within the range of measurements made on fuel bundles soon after reactor discharge. The appearance of the external surfaces and the microstructures of the fuel and cladding were also similar to those reported previously. In addition, no evidence of accelerated corrosion or hydride redistribution in the cladding was observed.

Bradley, E.R.; Bailey, W.J.; Johnson, A.B. Jr.; Lowry, L.M.

1981-09-01T23:59:59.000Z

328

Hazard Evaluation for Storage of Spent Nuclear Fuel (SNF) Sludge at the Solid Waste Treatment Facility  

SciTech Connect (OSTI)

As part of the Spent Nuclear Fuel (SNF) storage basin clean-up project, sludge that has accumulated in the K Basins due to corrosion of damaged irradiated N Reactor will be loaded into containers and placed in interim storage. The Hanford Site Treatment Complex (T Plant) has been identified as the location where the sludge will be stored until final disposition of the material occurs. Long term storage of sludge from the K Basin fuel storage facilities requires identification and analysis of potential accidents involving sludge storage in T Plant. This report is prepared as the initial step in the safety assurance process described in DOE Order 5480.23, Nuclear Safety Analysis Reports and HNF-PRO-704, Hazards and Accident Analysis Process. This report documents the evaluation of potential hazards and off-normal events associated with sludge storage activities. This information will be used in subsequent safety analyses, design, and operations procedure development to ensure safe storage. The hazards evaluation for the storage of SNF sludge in T-Plant used the Hazards and Operability Analysis (HazOp) method. The hazard evaluation identified 42 potential hazardous conditions. No hazardous conditions involving hazardous/toxic chemical concerns were identified. Of the 42 items identified in the HazOp study, eight were determined to have potential for onsite worker consequences. No items with potential offsite consequences were identified in the HazOp study. Hazardous conditions with potential onsite worker or offsite consequences are candidates for quantitative consequence analysis. The hazardous conditions with potential onsite worker consequences were grouped into two event categories, Container failure due to overpressure - internal to T Plant, and Spill of multiple containers. The two event categories will be developed into accident scenarios that will be quantitatively analyzed to determine release consequences. A third category, Container failure due to overpressure--external to T Plant, was included for completeness but is not within the scope of the hazards evaluation. Container failures external to T Plant will be addressed as part of the transportation analysis. This document describes the HazOp analysis performed for the activities associated with the storage of SNF sludge in the T Plant.

SCHULTZ, M.V.

2000-08-22T23:59:59.000Z

329

Comparative analyses of spent nuclear fuel transport modal options: Transport options under existing site constraints  

SciTech Connect (OSTI)

The movement of nuclear waste can be accomplished by various transport modal options involving different types of vehicles, transport casks, transport routes, and intermediate intermodal transfer facilities. A series of systems studies are required to evaluate modal/intermodal spent fuel transportation options in a consistent fashion. This report provides total life-cycle cost and life-cycle dose estimates for a series of transport modal options under existing site constraints. 14 refs., 7 figs., 28 tabs.

Brentlinger, L.A.; Hofmann, P.L.; Peterson, R.W.

1989-08-01T23:59:59.000Z

330

Annual Radiological Environmental Monitoring Program Report for the Fort St. Vrain Independent Spent Fuel Storage Installation  

SciTech Connect (OSTI)

This report presents the results of the 2001 Radiological Environmental Monitoring Program conducted in accordance with 10 CFR 72.44 for the Fort St. Vrain Independent Spent Fuel Storage Installation. A description of the facility and the monitoring program is provided. The results of monitoring the predominant radiation exposure pathway, direct and scattered radiation exposure, indicate the facility operation has not contributed to any increase in the estimated maximum potential dose commitment to the general public.

Hall, Gregory Graham; Newkirk, Jay Ronald; Borst, Frederick Jon

2002-02-01T23:59:59.000Z

331

Annual Radiological Environmental Monitoring Program Report for the Fort St. Vrain Independent Spent Fuel Storage Installation  

SciTech Connect (OSTI)

This report presents the results of the 2002 Radiological Environmental Monitoring Program conducted in accordance with 10 CFR 72.44 for the Fort St. Vrain Independent Spent Fuel Storage Installation. A description of the facility and the monitoring program is provided. The results of monitoring the predominant radiation exposure pathway, direct and scattered radiation exposure, indicate the facility operation has not contributed to any increase in the estimated maximum potential dose commitment to the general public.

Jay R. Newkirk; Frederick J. Borst; Gregory G. Hall

2003-02-01T23:59:59.000Z

332

A comparison of spent fuel assembly control instruments: The Cadarache PYTHON and the Los Alamos Fork  

SciTech Connect (OSTI)

Devices to monitor spent fuel assemblies while stored under water with nondestructive assay methods, have been developed in France and in the United States. Both devices are designed to verify operator's declared values of exposures and cooling-time but the applications and thus the designs of the systems differ. A study, whose results are presented in this paper, has been conducted to compare the features and the performances of the two instruments. 4 refs., 9 figs.

Bignan, G.; Capsie, J.; Romeyer-Dherbey, J. (CEA Centre d'Etudes Nucleaires de Cadarache, 13 - Saint-Paul-lez-Durance (France). Direction des Reacteurs Nucleaires); Rinard, P. (Los Alamos National Lab., NM (United States))

1991-01-01T23:59:59.000Z

333

K Basin spent nuclear fuel hot conditioning system functions {ampersand} requirements  

SciTech Connect (OSTI)

The purpose of this F{ampersand}R document is to establish the functional requirements baseline for the Spent Nuclear Fuel Hot Conditioning System (HCS) subproject. This F{ampersand}R documents the: -mission of the HCS, -evolution of the technical baseline leading to the HCS, -functions that must be performed to accomplish the HCS mission, -requirements basis allocated to the HCS mission and functions, -identification and definition of interfaces between the HCS and other SNF subprojects.

Miska, C.R., Westinghouse Hanford

1996-07-08T23:59:59.000Z

334

End-to-end calculation of the radiation characteristics of VVER-1000 spent fuel assemblies  

SciTech Connect (OSTI)

The results of end-to-end calculation of the radiation characteristics of VVER-1000 spent nuclear fuel are presented. Details of formation of neutron and gamma-radiation sources are analyzed. Distributed sources of different types of radiation are considered. A comparative analysis of calculated radiation characteristics is performed with the use of nuclear data from different ENDF/B and EAF files and ANSI/ANS and ICRP standards.

Linge, I. I.; Mitenkova, E. F., E-mail: mit@ibrae.ac.ru; Novikov, N. V. [Russian Academy of Sciences, Nuclear Safety Institute (Russian Federation)

2012-12-15T23:59:59.000Z

335

Spent nuclear fuel as a waste form for geologic disposal: Assessment and recommendations on data and modeling needs  

SciTech Connect (OSTI)

This study assesses the status of knowledge pertinent to evaluating the behavior of spent nuclear fuel as a waste form in geologic disposal systems and provides background information that can be used by the DOE to address the information needs that pertain to compliance with applicable standards and regulations. To achieve this objective, applicable federal regulations were reviewed, expected disposal environments were described, the status of spent-fuel modeling was summarized, and information regarding the characteristics and behavior of spent fuel was compiled. This compiled information was then evaluated from a performance modeling perspective to identify further information needs. A number of recommendations were made concerning information still needed to enhance understanding of spent-fuel behavior as a waste form in geologic repositories. 335 refs., 22 figs., 44 tabs.

Van Luik, A.E.; Apted, M.J.; Bailey, W.J.; Haberman, J.H.; Shade, J.S.; Guenther, R.E.; Serne, R.J.; Gilbert, E.R.; Peters, R.; Williford, R.E.

1987-09-01T23:59:59.000Z

336

Evaluation of fission product worth margins in PWR spent nuclear fuel burnup credit calculations.  

SciTech Connect (OSTI)

Current criticality safety calculations for the transportation of irradiated LWR fuel make the very conservative assumption that the fuel is fresh. This results in a very substantial overprediction of the actual k{sub eff} of the transportation casks; in certain cases, this decreases the amount of spent fuel which can be loaded in a cask, and increases the cost of transporting the spent fuel to the repository. Accounting for the change of reactivity due to fuel depletion is usually referred to as ''burnup credit.'' The US DOE is currently funding a program aimed at establishing an actinide only burnup credit methodology (in this case, the calculated reactivity takes into account the buildup or depletion of a limited number of actinides). This work is undergoing NRC review. While this methodology is being validated on a significant experimental basis, it implicitly relies on additional margins: in particular, the absorption of neutrons by certain actinides and by all fission products is not taken into account. This provides an important additional margin and helps guarantee that the methodology is conservative provided these neglected absorption are known with reasonable accuracy. This report establishes the accuracy of fission product absorption rate calculations: (1) the analysis of European fission product worth experiments demonstrates that fission product cross-sections available in the US provide very good predictions of fission product worth; (2) this is confirmed by a direct comparison of European and US cross section evaluations; (3) accuracy of Spent Nuclear Fuel (SNF) fission product content predictions is established in a recent ORNL report where several SNF isotopic assays are analyzed; and (4) these data are then combined to establish in a conservative manner the fraction of the predicted total fission product absorption which can be guaranteed based on available experimental data.

Blomquist, R.N.; Finck, P.J.; Jammes, C.; Stenberg, C.G.

1999-02-17T23:59:59.000Z

337

Probable leaching mechanisms for UO/sub 2/ and spent fuel  

SciTech Connect (OSTI)

The oxidation and dissolution mechanisms for UO/sub 2/ and spent fuel will be quite similar based on this preliminary work with electrochemical leaching of UO/sub 2/ and spent fuel. In solutions containing oxygen or other oxidizing species, the UO/sub 2/ surface will be rapidly oxidized and dissolved following the transformation of uranium from U(IV) to U(VI). The hydrolysis of dissolved uranyl ions forms solid UO/sub 3/ hydrates or related complex compounds deposited onto the UO/sub 2/ surface, or other surfaces, as thin or thick coatings. Depending on the pH, temperature, and time, the various kinds of porosity and the mechanical properties of the hydrate coatings will control the dissolution rate. The effects of radiation, in terms of generation of H/sub 2/O/sub 2/, will enhance the dissolution kinetics. Electrochemical methods may be useful for determining the surface conditions, dissolution rate, and accelerated dissolution behavior for NO/sub 2/ and spent fuel. Electrochemial methods can rapidly generate much information in terms of dissolution rate and surface film properties - such as thickness, porosity, and oxidation state - in-situ during the leaching process.

Wang, R.; Katayama, Y.B.

1980-01-01T23:59:59.000Z

338

Integrated data base for 1986: spent fuel and radioactive waste inventories, projections, and characteristics. Revision 2  

SciTech Connect (OSTI)

The Integrated Data Base (IDB) Program has compiled current data on inventories and characteristics of commercial spent fuel and both commercial and US Department of Energy (DOE) radioactive wastes through December 31, 1985, based on the most reliable information available from government sources, the open literature, technical reports, and direct contacts. Current projections of future waste and spent fuel to be generated through the year 2020 and characteristics of these materials are also presented. The information forecasted is consistent with the expected defense-related and private industrial and institutional activities and the latest DOE/Energy Information Administration (EIA) projections of US commercial nuclear power growth. The materials considered, on a chapter-by-chapter basis, are: spent fuel, high-level waste, transuranic waste, low-level waste, commercial uranium mill tailings, remedial action waste, and decommissioning waste. For each category, current and projected inventories are given through the year 2020, and the radioactivity and thermal power are calculated based on reported or calculated isotopic compositions.

Not Available

1986-09-01T23:59:59.000Z

339

Integrated data base for 1988: Spent fuel and radioactive waste inventories, projections, and characteristics  

SciTech Connect (OSTI)

The Integrated Data Base (IDB) Program has compiled current data on inventories and characteristics of commercial spent fuel and both commercial and US government-owned radioactive wastes through December 31, 1987. These data are based on the most reliable information available from government sources, the open literature, technical reports, and direct contacts. The current projections of future waste and spent fuel to be generated through the year 2020 and characteristics of these materials are also presented. The information forecasted is consistent with the latest US Department of Energy/Energy Information Administration (DOE/EIA) projections of US commercial nuclear power growth and the expected defense-related and private industrial and institutional (I/I) activities. The radioactive materials considered, on a chapter-by-chapter basis are: spent fuel, high-level waste, transuranic waste, low-level waste, commercial uranium mill tailings, remedial action waste, and decommissioning waste. For each category, current and projected inventories are given through the year 2020, and the radioactivity and thermal power are calculated based on reported or estimated isotopic compositions. In addition, characteristics and current inventories are reportd for miscellaneous, highly radioactive materials that may require geologic disposal. 89 refs., 46 figs., 104 tabs.

Not Available

1988-09-01T23:59:59.000Z

340

Integrated data base for 1987: Spent fuel and radioactive waste inventories, projections, and characteristics  

SciTech Connect (OSTI)

The Integrated Data Base (IDB) Program has compiled current data on inventories and characteristics of commercial spent fuel and both commercial and US government-owned radioactive wastes through December 31, 1986. These data are based on the most reliable information available from government sources, the open literature, technical reports, and direct contacts. Current projections of future waste and spent fuel to be generated through the year 2020 and characteristics of these materials are also presented. The information forecasted is consistent with the latest US Department of Energy/Energy Information Administration projections of US commercial nuclear power growth and the expected defense-related and private industrial and institutional activities. The radioactive materials considered, on a chapter-by-chapter basis, are spent fuel, high-level waste, transuranic waste, low-level waste, commercial uranium mill tailings, remedial action waste, and decommissioning waste. For each category, current and projected inventories are given through the year 2020, and the radioactivity and thermal power are calculated based on reported or estimated isotopic compositions. In addition, characteristics and current inventories are reported for miscellaneous, highly radioactive materials that may require geologic disposal. 82 refs., 57 figs., 121 tabs.

Not Available

1987-09-01T23:59:59.000Z

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


341

Dry halide method for separating the components of spent nuclear fuels  

DOE Patents [OSTI]

The invention is a nonaqueous, single method for processing multiple spent nuclear fuel types by separating the fission- and transuranic products from the nonradioactive and fissile uranium product. The invention has four major operations: exposing the spent fuels to chlorine gas at temperatures preferably greater than 1200.degree. C. to form volatile metal chlorides; removal of the fission product chlorides, transuranic product chlorides, and any nickel chloride and chromium chloride in a molten salt scrubber at approximately 400.degree. C.; fractional condensation of the remaining volatile chlorides at temperatures ranging from 164.degree. C. to 2.degree. C.; and regeneration and recovery of the transferred spent molten salt by vacuum distillation. The residual fission products, transuranic products, and nickel- and chromium chlorides are converted to fluorides or oxides for vitrification. The method offers the significant advantages of a single, compact process that is applicable to most of the diverse nuclear fuels, minimizes secondary wastes, segregates fissile uranium from the high level wastes to resolve potential criticality concerns, segregates nonradioactive wastes from the high level wastes for volume reduction, and produces a common waste form glass or glass-ceramic.

Christian, Jerry Dale (Idaho Falls, ID); Thomas, Thomas Russell (Rigby, ID); Kessinger, Glen F. (Idaho Falls, ID)

1998-01-01T23:59:59.000Z

342

Spent Nuclear Fuel Project technical baseline document. Fiscal year 1995: Volume 1, Baseline description  

SciTech Connect (OSTI)

This document is a revision to WHC-SD-SNF-SD-002, and is issued to support the individual projects that make up the Spent Nuclear Fuel Project in the lower-tier functions, requirements, interfaces, and technical baseline items. It presents results of engineering analyses since Sept. 1994. The mission of the SNFP on the Hanford site is to provide safety, economic, environmentally sound management of Hanford SNF in a manner that stages it to final disposition. This particularly involves K Basin fuel, although other SNF is involved also.

Womack, J.C. [Westinghouse Hanford Co., Richland, WA (United States); Cramond, R. [TRW (United States); Paedon, R.J. [SAIC (United States)] [and others

1995-03-13T23:59:59.000Z

343

ALARA Analysis for Shippingport Pressurized Water Reactor Core 2 Fuel Storage in the Canister Storage Building (CSB)  

E-Print Network [OSTI]

The addition of Shippingport Pressurized Water Reactor (PWR) Core 2 Blanket Fuel Assembly storage in the Canister Storage Building (CSB) will increase the total cumulative CSB personnel exposure from receipt and handling activities. The loaded Shippingport Spent Fuel Canisters (SSFCs) used for the Shippingport fuel have a higher external dose rate. Assuming an MCO handling rate of 170 per year (K East and K West concurrent operation), 24-hr CSB operation, and nominal SSFC loading, all work crew personnel will have a cumulative annual exposure of less than the 1,000 mrem limit.

Lewis, M E

2000-01-01T23:59:59.000Z

344

High Performance Fuel Desing for Next Generation Pressurized Water Reactors  

SciTech Connect (OSTI)

The use of internally and externally cooled annular fule rods for high power density Pressurized Water Reactors is assessed. The assessment included steady state and transient thermal conditions, neutronic and fuel management requirements, mechanical vibration issues, fuel performance issues, fuel fabrication methods and econmic assessment. The investigation was donducted by a team from MIT, Westinghouse, Gamma Engineering, Framatome ANP, and AECL. The analyses led to the conclusion that raising the power density by 50% may be possible with this advanced fuel. Even at the 150% power level, the fuel temperature would be a few hundred degrees lower than the current fuel temperatre. Significant economic and safety advantages can be obtained by using this fuel in new reactors. Switching to this type of fuel for existing reactors would yield safety advantages, but the economic return is dependent on the duration of plant shutdown to accommodate higher power production. The main feasiblity issue for the high power performance appears to be the potential for uneven splitting of heat flux between the inner and outer fuel surfaces due to premature closure of the outer fuel-cladding gap. This could be overcome by using a very narrow gap for the inner fuel surface and/or the spraying of a crushable zirconium oxide film at the fuel pellet outer surface. An alternative fuel manufacturing approach using vobropacking was also investigated but appears to yield lower than desirable fuel density.

Mujid S. Kazimi; Pavel Hejzlar

2006-01-31T23:59:59.000Z

345

PROTEUS - Simulation Toolset for Reactor Physics and Fuel Cycle Analysis  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Simulation Toolset for Simulation Toolset for Reactor Physics and Fuel Cycle Analysis PROTEUS Faster and more accurate neutronics calculations enable optimum reactor design... Argonne National Laboratory's powerful reactor physics toolset, PROTEUS, empowers users to create optimal reactor designs quickly, reliably and accurately. ...Reducing costs for designers of fast spectrum reactors. PROTEUS' long history of validation provides confidence in predictive simulations Argonne's simulation tools have more than 30 years of validation history against numerous experiments and measurements. The tools within PROTEUS work together, using the same interface files for easier integration of calculations. Multi-group Fast Reactor Cross Section Processing: MC 2 -3 No other fast spectrum multigroup generation tool

346

CORROSION OF ALUMINUM CLAD SPENT NUCLEAR FUEL IN THE 70 TON CASK DURING TRANSFER FROM L AREA TO H-CANYON  

SciTech Connect (OSTI)

Aluminum-clad spent nuclear fuel will be transported for processing in the 70-ton nuclear fuel element cask from L Basin to H-canyon. During transport these fuels would be expected to experience high temperature aqueous corrosion from the residual L Basin water that will be present in the cask. Cladding corrosion losses during transport were calculated for material test reactor (MTR) and high flux isotope reactors (HFIR) fuels using literature and site information on aqueous corrosion at a range of time/temperature conditions. Calculations of the cladding corrosion loss were based on Arrhenius relationships developed for aluminum alloys typical of cladding material with the primary assumption that an adherent passive film does not form to retard the initial corrosion rate. For MTR fuels a cladding thickness loss of 33 % was found after 1 year in the cask with a maximum temperature of 260 {degrees}C. HFIR fuels showed a thickness loss of only 6% after 1 year at a maximum temperature of 180 {degrees}C. These losses are not expected to impact the overall confinement function of the aluminum cladding.

Mickalonis, J.

2014-06-01T23:59:59.000Z

347

Reactor Physics and Fuel Cycle Analysis - Nuclear Engineering Division  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Analysis Analysis Capabilities Nuclear Systems Modeling and Design Analysis Reactor Physics and Fuel Cycle Analysis Overview Current Projects Software Nuclear Plant Dynamics and Safety Nuclear Data Program Advanced Reactor Development Nuclear Waste Form and Repository Performance Modeling Nuclear Energy Systems Design and Development Other Capabilities Work with Argonne Contact us For Employees Site Map Help Join us on Facebook Follow us on Twitter NE on Flickr Reactor Physics and Fuel Cycle Analysis Bookmark and Share Reactor physics and fuel cycle analysis is a core competency of the Nuclear Engineering (NE) Division. The Division has played a major role in the design and analysis of advanced reactors, particularly liquid-metal-cooled reactors. NE researchers have concentrated on developing computer codes for

348

Spent Nuclear Fuel Self-Induced XRF to Predict Pu to U Content  

E-Print Network [OSTI]

area of interest, would improve input accountability and shipper/receiver differences. XRF measurements were made on individual PWR fuel rods with varying fuel ages and final burn-ups at Oak Ridge National Laboratory (ORNL) in July 2008 and January... Committee NRF Nuclear Resonance Fluorescence viii ORNL Oak Ridge National Laboratory Pu Plutonium PUREX Plutonium and Uranium Recovery by Extraction PWR Pressurized Water Reactor RPP Reprocessing Plant SNM Special Nuclear Material...

Stafford, Alissa Sarah

2010-10-12T23:59:59.000Z

349

Spent nuclear fuel characterization for a bounding reference assembly for the receiving basin for off-site fuel  

SciTech Connect (OSTI)

The Basis for Interim Operation (BIO) for the Receiving Basin for Off-Site Fuel (RBOF) facility at the Department of Energy (DOE) Savannah River Site (SRS) nuclear materials production complex, developed in accordance with draft DOE-STD-0019-93, required a hazard categorization for the safety analysis section as outlined in DOE-STD-1027-92. The RBOF facility was thus established as a Category-2 facility (having potential for significant on-site consequences from a radiological release) as defined in DOE 5480.23. Given the wide diversity of spent nuclear fuel stored in the RBOF facility, which made a detailed assessment of the total nuclear inventory virtually impossible, the categorization required a conservative calculation based on the concept of a hypothetical, bounding reference fuel assembly integrated over the total capacity of the facility. This scheme not only was simple but also precluded a potential delay in the completion of the BIO.

Kahook, S.D.; Garrett, R.L.; Canas, L.R.; Beckum, M.J. [Westinghouse Savannah River, Aiken, SC (United States)

1995-07-01T23:59:59.000Z

350

Probabilistic assessment of spent fuel shipping cask response to severe transportation accident conditions. Report summary  

SciTech Connect (OSTI)

The licensing of commercial nuclear spent shipping casks in the United States is regulated by 10CFR71. In order to be licensed, casks must be designed not to fail under hypothetical test conditions specified in Appendix B of this regulation. Questions have been raised about the suitability of these tests in simulating actual transportation accident conditions. Our study addresses the adequacy of current regulations by comparing real-world accident conditions with regulatory test specifications using more complete accident statistics and more sophisticated structural analyses than have been used in studies to date. Our objective is to evaluate the protection provided by current regulations against severe accident conditions for commercial spent nuclear fuel casks that are transported by truck or rail. The complete spectrum of truck and rail accidents will be reviewed in order to determine the frequency (or infrequency) of cask failures during transportation accidents. 3 references, 1 figure.

Fischer, L.E.; Kimura, C.Y.; Witte, M.C.

1985-01-01T23:59:59.000Z

351

Use of Integrated Decay Heat Limits to Facilitate Spent Nuclear Fuel Loading to Yucca Mountain  

SciTech Connect (OSTI)

As an alternative to the use of the linear loading or areal power density (APD) concept, using integrated decay heat limits based on the use of mountain-scale heat transfer analysis is considered to represent the thermal impact from the deposited spent nuclear fuel (SNF) to the Yucca Mountain repository. Two different integrated decay heat limits were derived to represent both the short-term (up to 50 years from the time of repository closure) and the long-term decay heat effect (up to 1500 years from the time of repository closure). The derived limits were found to appropriately represent the drift wall temperature limit (200 deg. C) and the midway between adjacent drifts temperature limit (96 deg. C) as long as used fuel is uniformly loaded into the mountain. These limits can be a useful practical guide to facilitate the loading of used fuel into Yucca Mountain. (authors)

Li, Jun; Yim, Man-Sung; McNelis, David [Department of Nuclear Engineering, North Carolina State University (United States); Piet, Steven [Idaho National Laboratory (United States)

2007-07-01T23:59:59.000Z

352

Potential application of Zircaloy chemical embrittlement to volume reduction of spent-fuel cladding  

SciTech Connect (OSTI)

Embrittlement of Zircaloy fuel cladding tubes by corrosion media was studied from the viewpoint of its applicability to spent-fuel reprocessing. The results from irradiated as well as unirradiated tubes are summarized as follows: (1) when iodine was employed as the solute, the use of methanol as the solvent caused significant embrittlement of the Zircaloy; (2) for the iodine-methanol solution, the embrittlement increased with the iodine content but saturated at 1 wt%; (3) a water content of up to 10 vol% in the iodine-methanol solution did not decrease the extent of embrittlement; (4) fracture was of the grain-boundary type, and a fuel cladding tube irradiated to [approximately] 35GWd/t showed the same embrittlement behavior as an unirradiated one.

Nakatsuka, Masafumi (Nippon Nuclear Fuel Development Co., Ltd., Ibaraki (Japan))

1993-09-01T23:59:59.000Z

353

Modular Pebble Bed Reactor High Temperature Gas Reactor  

E-Print Network [OSTI]

Modular Pebble Bed Reactor High Temperature Gas Reactor Andrew C Kadak Massachusetts Institute For 1150 MW Combined Heat and Power Station Oil Refinery Hydrogen Production Desalinization Plant VHTR/Graphite Discrimination system Damaged Sphere ContainerGraphiteReturn FuelReturn Fresh Fuel Container Spent Fuel Tank #12

354

Comments on Americium Volatilization during Fuel Fabrication for Fast Reactors  

SciTech Connect (OSTI)

The physical processes relevant to the fabrication of metallic and ceramic nuclear fuels are analyzed, with attention to recycling of fuels containing U, Pu, and minor volatile actinides for the use in fast reactors. This analysis is relevant to the development of a process model that can be used for the numerical simulation and prediction of the spatial distribution of composition in the fuel, an important factor in fuel performance.

Sabau, Adrian S [ORNL; Ohriner, Evan Keith [ORNL

2008-01-01T23:59:59.000Z

355

Foreign programs for the storage of spent nuclear power plant fuels, high-level waste canisters and transuranic wastes  

SciTech Connect (OSTI)

The various national programs for developing and applying technology for the interim storage of spent fuel, high-level radioactive waste, and TRU wastes are summarized. Primary emphasis of the report is on dry storage techniques for uranium dioxide fuels, but data are also provided concerning pool storage.

Harmon, K.M.; Johnson, A.B. Jr.

1984-04-01T23:59:59.000Z

356

Evaluation of Options for Permanent Geologic Disposal of Spent NuclearFuel and High-Level Radioactive Waste  

Broader source: Energy.gov [DOE]

[In Support of a Comprehensive National Nuclear Fuel Cycle Strategy, Volumes I and II (Appendices)] This study provides a technical basis for informing policy decisions regarding strategies for the management and permanent disposal of spent nuclear fuel (SNF) and high-level radioactive waste (HLW) in the United States requiring geologic isolation.

357

Developments of Spent Nuclear Fuel Pyroprocessing Technology at Idaho National Laboratory  

SciTech Connect (OSTI)

This paper summarizes research in used fuel pyroprocessing that has been published by Idaho National Laboratory over the last decade. It includes work done both on treatment of Experimental Breeder Reactor-II and development of advanced technology for potential scale-up and commercialization. Collaborations with universities and other laboratories is included in the cited work.

Michael F. Simpson

2012-03-01T23:59:59.000Z

358

Analysis of dose consequences arising from the release of spent nuclear fuel from dry storage casks.  

SciTech Connect (OSTI)

The resulting dose consequences from releases of spent nuclear fuel (SNF) residing in a dry storage casks are examined parametrically. The dose consequences are characterized by developing dose versus distance curves using simplified bounding assumptions. The dispersion calculations are performed using the MELCOR Accident Consequence Code System (MACCS2) code. Constant weather and generic system parameters were chosen to ensure that the results in this report are comparable with each other and to determine the relative impact on dose of each variable. Actual analyses of site releases would need to accommodate local weather and geographic data. These calculations assume a range of fuel burnups, release fractions (RFs), three exposure scenarios (2 hrs and evacuate, 2 hrs and shelter, and 24 hrs exposure), two meteorological conditions (D-4 and F-2), and three release heights (ground level - 1 meter (m), 10 m, and 100 m). This information was developed to support a policy paper being developed by U.S. Nuclear Regulatory Commission (NRC) staff on an independent spent fuel storage installation (ISFSI) and monitored retrievable storage installation (MRS) security rulemaking.

Durbin, Samuel G.; Morrow, Charles W.

2013-01-01T23:59:59.000Z

359

Realization of the German Concept for Interim Storage of Spent Nuclear Fuel - Current Situation and Prospects  

SciTech Connect (OSTI)

The German government has determined a phase out of nuclear power. With respect to the management of spent fuel it was decided to terminate transports to reprocessing plants by 2005 and to set up interim storage facilities on power plant sites. This paper gives an overview of the German concept for spent fuel management focused on the new on-site interim storage concept and the applied interim storage facilities. Since the end of the year 1998, the utilities have applied for permission of on-site interim storage in 13 storage facilities and 5 storage areas; one application for the interim storage facility Stade was withdrawn due to the planned final shut down of Stade nuclear power plant in autumn 2003. In 2001 and 2002, 3 on-site storage areas and 2 on-site storage facilities for spent fuel were licensed by the Federal Office for Radiation Protection (BfS). A main task in 2002 and 2003 has been the examination of the safety and security of the planned interim storage facilities and the verification of the licensing prerequisites. In the aftermath of September 11, 2001, BfS has also examined the attack with a big passenger airplane. Up to now, these aircraft crash analyses have been performed for three on-site interim storage facilities; the fundamental results will be presented. It is the objective of BfS to conclude the licensing procedures for the applied on-site interim storage facilities in 2003. With an assumed construction period for the storage buildings of about two years, the on-site interim storage facilities could then be available in the year 2005.

Thomauske, B. R.

2003-02-25T23:59:59.000Z

360

Effects of spent fuel types on offsite consequences of hypothetical accidents  

SciTech Connect (OSTI)

Argonne National Laboratory (ANL) conducts experimental work on the development of waste forms suitable for several types of spent fuel at its facility on the Idaho National Engineering and Environmental Laboratory (INEEL) located 48 km West of Idaho Falls, ID. The objective of this paper is to compare the offsite radiological consequences of hypothetical accidents involving the various types of spent nuclear fuel handled in nonreactor nuclear facilities. The highest offsite total effective dose equivalents (TEDEs) are estimated at a receptor located about 5 km SSE of ANL facilities. Criticality safety considerations limit the amount of enriched uranium and plutonium that could be at risk in any given scenario. Heat generated by decay of fission products and actinides does not limit the masses of spent fuel within any given operation because the minimum time elapsed since fissions occurred in any form is at least five years. At cooling times of this magnitude, fewer than ten radionuclides account for 99% of the projected TEDE at offsite receptors for any credible accident. Elimination of all but the most important nuclides allows rapid assessments of offsite doses with little loss of accuracy. Since the ARF (airborne release fraction), RF (respirable fraction), LPF (leak path fraction) and atmospheric dilution factor ({chi}/Q) can vary by orders of magnitude, it is not productive to consider nuclides that contribute less than a few percent of the total dose. Therefore, only {sup 134}Cs, {sup 137}Cs-{sup 137m}Ba, and the actinides significantly influence the offsite radiological consequences of severe accidents. Even using highly conservative assumptions in estimating radiological consequences, they remain well below current Department of Energy guidelines for highly unlikely accidents.

Courtney, J. C.; Dwight, C. C.; Lehto, M. A.

2000-02-18T23:59:59.000Z

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


361

Research on Spent Fuel Storage and Transportation in CRIEPI (Part 2 Concrete Cask Storage)  

SciTech Connect (OSTI)

Concrete cask storage has been implemented in the world. At a later stage of storage period, the containment of the canister may deteriorate due to stress corrosion cracking phenomena in a salty air environment. High resistant stainless steels against SCC have been tested as compared with normal stainless steel. Taking account of the limited time-length of environment with certain level of humidity and temperature range, the high resistant stainless steels will survive from SCC damage. In addition, the adhesion of salt from salty environment on the canister surface will be further limited with respect to the canister temperature and angle of the canister surface against the salty air flow in the concrete cask. Optional countermeasure against SCC with respect to salty air environment has been studied. Devices consisting of various water trays to trap salty particles from the salty air were designed to be attached at the air inlet for natural cooling of the cask storage building. Efficiency for trapping salty particles was evaluated. Inspection of canister surface was carried out using an optical camera inserted from the air outlet through the annulus of a concrete cask that has stored real spent fuel for more than 15 years. The camera image revealed no gross degradation on the surface of the canister. Seismic response of a full-scale concrete cask with simulated spent fuel assemblies has been demonstrated. The cask did not tip over, but laterally moved by the earthquake motion. Stress generated on the surface of the spent fuel assemblies during the earthquake motion were within the elastic region.

Koji Shirai; Jyunichi Tani; Taku Arai; Masumi Watatu; Hirofumi Takeda; Toshiari Saegusa; Philip L. Winston

2008-10-01T23:59:59.000Z

362

Experience With Damaged Spent Nuclear Fuel at U.S. DOE Facilities  

SciTech Connect (OSTI)

This report summarizes some of the challenges encountered and solutions implemented to ensure safe storage and handling of damaged spent nuclear fuels (SNF). It includes a brief summary of some SNF storage environments and resulting SNF degradation, experience with handling and repackaging significantly degraded SNFs, and the associated lessons learned. This work provides useful insight and resolutions to many engineering challenges facing SNF handling and storage facilities. The context of this report is taken from a report produced at Idaho National Laboratory and further detailed information, such as equipment design and usage, can be found in the appendices to that report. (authors)

Carlsen, Brett; Fillmore, Denzel; Woolstenhulme, Eric [Idaho National Laboratory, P.O. Box 1625 Idaho Falls, ID 83415 (United States); McCormack, Roger L. [Fluor Hanford Site, Richland, Wash. (United States); Sindelar, Robert; Spieker, Timothy [Savannah River National Laboratory, Savannah River Site Aiken, SC 29808 (United States)

2006-07-01T23:59:59.000Z

363

What are Spent Nuclear Fuel and High-Level Radioactive Waste ?  

SciTech Connect (OSTI)

Spent nuclear fuel and high-level radioactive waste are materials from nuclear power plants and government defense programs. These materials contain highly radioactive elements, such as cesium, strontium, technetium, and neptunium. Some of these elements will remain radioactive for a few years, while others will be radioactive for millions of years. Exposure to such radioactive materials can cause human health problems. Scientists worldwide agree that the safest way to manage these materials is to dispose of them deep underground in what is called a geologic repository.

DOE

2002-12-01T23:59:59.000Z

364

Considerations for increasing unit 1 spent fuel pool capacity at the Laguna Verde station  

SciTech Connect (OSTI)

To increase the spent fuel storage capacity at the Laguna Verde Station in a safe and economical manner and assure a continuous operation of the first Mexican Nuclear Plant, Comision Federal de Electricidad (CFE), the Nation's Utility, seeked alternatives considering the overall world situation, the safety and licensing aspects, as well as the economics and the extent of the nuclear program of Mexico. This paper describes the alternatives considered, their evaluation and how the decision taken by CFE in this field, provides the Laguna Verde Station with a maximum of 37 years storage capacity plus full core reserve.

Vera, A. (Comision Federal de Electricidad, Veracruz, Ver. (Mexico))

1992-01-01T23:59:59.000Z

365

A practical strategy for reducing the future security risk of United States spent nuclear fuel  

SciTech Connect (OSTI)

Depletion calculations show that advanced oxide (AOX) fuels can be used in existing light water reactors (LWRs) to achieve and maintain virtually any desired level of US (US) reactor-grade plutonium (R-Pu) inventory. AOX fuels are composed of a neutronically inert matrix loaded with R-Pu and erbium. A 1/2 core load of 100% nonfertile, 7w% R-Pu AOX and 3.9 w% UO{sub 2} has a net total plutonium ({sup TOT}Pu) destruction rate of 310 kg/yr. The 20% residual {sup TOT}Pu in discharged AOX contains > 55% {sup 242}Pu making it unattractive for nuclear explosive use. A three-phase fuel-cycle development program sequentially loading 60 LWRs with 100% mixed oxide, 50% AOX with a nonfertile component displacing only some of the {sup 238}U, and 50% AOX, which is 100% nonfertile, could reduce the US plutonium inventory to near zero by 2050.

Chodak, P. III; Buksa, J.J. [Los Alamos National Lab., NM (United States). Nuclear Systems Design and Analysis Group

1997-06-01T23:59:59.000Z

366

TEST SYSTEM FOR EVALUATING SPENT NUCLEAR FUEL BENDING STIFFNESS AND VIBRATION INTEGRITY  

SciTech Connect (OSTI)

Transportation packages for spent nuclear fuel (SNF) must meet safety requirements specified by federal regulations. For normal conditions of transport, vibration loads incident to transport must be considered. This is particularly relevant for high-burnup fuel (>45 GWd/MTU). As the burnup of the fuel increases, a number of changes occur that may affect the performance of the fuel and cladding in storage and during transportation. The mechanical properties of high-burnup de-fueled cladding have been previously studied by subjecting defueled cladding tubes to longitudinal (axial) tensile tests, ring-stretch tests, ring-compression tests, and biaxial tube burst tests. The objective of this study is to investigate the mechanical properties and behavior of both the cladding and the fuel in it under vibration/cyclic loads similar to the sustained vibration loads experienced during normal transport. The vibration loads to SNF rods during transportation can be characterized by dynamic, cyclic, bending loads. The transient vibration signals in a specified transport environment can be analyzed, and frequency, amplitude and phase components can be identified. The methodology being implemented is a novel approach to study the vibration integrity of actual SNF rod segments through testing and evaluating the fatigue performance of SNF rods at defined frequencies. Oak Ridge National Laboratory (ORNL) has developed a bending fatigue system to evaluate the response of the SNF rods to vibration loads. A three-point deflection measurement technique using linear variable differential transformers is used to characterize the bending rod curvature, and electromagnetic force linear motors are used as the driving system for mechanical loading. ORNL plans to use the test system in a hot cell for SNF vibration testing on high burnup, irradiated fuel to evaluate the pellet-clad interaction and bonding on the effective lifetime of fuel-clad structure bending fatigue performance. Technical challenges include pure bending implementation, remote installation and detachment of the SNF test specimen, test specimen deformation measurement, and identification of a driving system suitable for use in a hot cell. Surrogate test specimens have been used to calibrate the test setup and conduct systematic cyclic tests. The calibration and systematic cyclic tests have been used to identify test protocol issues prior to implementation in the hot cell. In addition, cyclic hardening in unidirectional bending and softening in reverse bending were observed in the surrogate test specimens. The interface bonding between the surrogate clad and pellets was found to impact the bending response of the surrogate rods; confirming this behavior in the actual spent fuel segments will be an important aspect of the hot cell test implementation,

Wang, Jy-An John [ORNL] [ORNL; Wang, Hong [ORNL] [ORNL; Bevard, Bruce Balkcom [ORNL] [ORNL; Howard, Rob L [ORNL] [ORNL; Flanagan, Michelle [U.S. Nuclear Regulatory Commission] [U.S. Nuclear Regulatory Commission

2013-01-01T23:59:59.000Z

367

EIS-0251: Department of the Navy Final Environmental Impact Statement for a Container System for the Management of Naval Spent Nuclear Fuel (November 1996)  

Broader source: Energy.gov [DOE]

This Final Environmental Impact Statement addresses six general alternative systems for the loading, storage, transport, and possible disposal of naval spent nuclear fuel following examination.

368

Monte Carlo simulations of a differential die-away instrument for determination of fissile content in spent fuel assemblies  

SciTech Connect (OSTI)

The differential die-away (DDA) technique has been simulated by using the MCNPX code to quantify its capability to measure the fissile content in spent fuel assemblies, For 64 different spent fuel cases of various initial enrichment, burnup and cooling time, the count rate and signal to background ratios of the DDA system were obtained, where neutron backgrounds are mainly coming from the {sup 244}Cm of the spent fuel. To quantify the total fissile mass of spent fuel, a concept of the effective {sup 239}Pu mass was introduced by weighting the relative contribution to the signal of {sup 235}U and {sup 241}Pu compared to {sup 239}Pu and the calibration curves of DDA count rate vs. {sup 239}Pu{sub eff} were obtained by using the MCNPX code. With a deuterium-tritium (DT) neutron generator of 10{sup 9} n/s strength, signal to background ratios of sufficient magnitude are acquired for a DDA system with the spent fuel assembly in water.

Lee, Taehoon [Los Alamos National Laboratory; Menlove, Howard O [Los Alamos National Laboratory; Swinhoe, Martyn T [Los Alamos National Laboratory; Tobin, Stephen J [Los Alamos National Laboratory

2010-01-01T23:59:59.000Z

369

E-Print Network 3.0 - advanced reactors part Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

emit to the environment significant quantities of heat, contributing... to the greenhouse effect. New Generation reactors to achieve the reuse of spent fuel. Fusion...

370

E-Print Network 3.0 - advanced reactor development Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

emit to the environment significant quantities of heat, contributing... to the greenhouse effect. New Generation reactors to achieve the reuse of spent fuel. Fusion...

371

E-Print Network 3.0 - advanced reactor technology Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

advanced countries like France, Canada, the USA. Expansion... to the greenhouse effect. New Generation reactors to achieve the reuse of spent fuel. Fusion...

372

E-Print Network 3.0 - automobile exhaust reactors Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

emit to the environment significant quantities of heat, contributing... to the greenhouse effect. New Generation reactors to achieve the reuse of spent fuel. Fusion...

373

E-Print Network 3.0 - afrri-triga reactor facility Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

emit to the environment significant quantities of heat, contributing... to the greenhouse effect. New Generation reactors to achieve the reuse of spent fuel. Fusion...

374

E-Print Network 3.0 - advanced reactors advanced Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

emit to the environment significant quantities of heat, contributing... to the greenhouse effect. New Generation reactors to achieve the reuse of spent fuel. Fusion...

375

Advanced Test Reactor Tour  

SciTech Connect (OSTI)

The Advanced Test Reactor at Idaho National Laboratory is the foremost nuclear materials test reactor in the world. This virtual tour describes the reactor, how experiments are conducted, and how spent nuclear fuel is handled and stored. For more information about INL research, visit http://www.facebook.com/idahonationallaboratory.

Miley, Don

2011-01-01T23:59:59.000Z

376

Advanced Test Reactor Tour  

ScienceCinema (OSTI)

The Advanced Test Reactor at Idaho National Laboratory is the foremost nuclear materials test reactor in the world. This virtual tour describes the reactor, how experiments are conducted, and how spent nuclear fuel is handled and stored. For more information about INL research, visit http://www.facebook.com/idahonationallaboratory.

Miley, Don

2013-05-28T23:59:59.000Z

377

Analysis of Transuranic Mixed Oxide Fuel in a CANDU Nuclear Reactor.  

E-Print Network [OSTI]

?? The reprocessing of spent fuel is a key component in reducing the end waste from nuclear power plant operations and creating a sustainable closed… (more)

Morreale, Andrew C

2013-01-01T23:59:59.000Z

378

Experimental Investigation of Burnup Credit for Safe Transport, Storage, and Disposal of Spent Nuclear Fuel  

SciTech Connect (OSTI)

This report describes criticality benchmark experiments containing rhodium that were conducted as part of a Department of Energy Nuclear Energy Research Initiative project. Rhodium is an important fission product absorber. A capability to perform critical experiments with low-enriched uranium fuel was established as part of the project. Ten critical experiments, some containing rhodium and others without, were conducted. The experiments were performed in such a way that the effects of the rhodium could be accurately isolated. The use of the experimental results to test neutronics codes is demonstrated by example for two Monte Carlo codes. These comparisons indicate that the codes predict the behavior of the rhodium in the critical systems within the experimental uncertainties. The results from this project, coupled with the results of follow-on experiments that investigate other fission products, can be used to quantify and reduce the conservatism of spent nuclear fuel safety analyses while still providing the necessary level of safety.

Harms, Gary A.; Helmick, Paul H.; Ford, John T.; Walker, Sharon A.; Berry, Donald T.; Pickard, Paul S.

2004-04-01T23:59:59.000Z

379

Container for reprocessing and permanent storage of spent nuclear fuel assemblies  

DOE Patents [OSTI]

A single canister process container is described for reprocessing and permanent storage of spent nuclear fuel assemblies comprising zirconium-based cladding and fuel, which process container comprises a collapsible container, having side walls that are made of a high temperature alloy and an array of collapsible support means wherein the container is capable of withstanding temperature necessary to oxidize the zirconium-based cladding and having sufficient ductility to maintain integrity when collapsed under pressure. The support means is also capable of maintaining its integrity at a temperature necessary to oxidize the zirconium-based cladding. The process container also has means to introduce and remove fluids to and from the container. 10 figs.

Forsberg, C.W.

1992-03-24T23:59:59.000Z

380

Centrifugal microfluidic platform for radiochemistry: Potentialities for the chemical analysis of nuclear spent fuels  

Science Journals Connector (OSTI)

Abstract The use of a centrifugal microfluidic platform is for the first time reported as an alternative to classical chromatographic procedures for radiochemistry. The original design of the microfluidic platform has been thought to fasten and simplify the prototyping process with the use of a circular platform integrating four rectangular microchips made of thermoplastic. The microchips, dedicated to anion-exchange chromatographic separations, integrate a localized monolithic stationary phase as well as injection and collection reservoirs. The results presented here were obtained with a simplified simulated nuclear spent fuel sample composed of non-radioactive isotopes of Europium and Uranium, in proportion usually found for uranium oxide nuclear spent fuel. While keeping the analytical results consistent with the conventional procedure (extraction yield for Europium of ?97%), the use of the centrifugal microfluidic platform allowed to reduce the volume of liquid needed by a factor of ?250. Thanks to their unique “easy-to-use” features, centrifugal microfluidic platforms are potential successful candidates for the downscaling of chromatographic separation of radioactive samples (automation, multiplexing, easy integration in glove-boxes environment and low cost of maintenance).

Anthony Bruchet; Vélan Taniga; Stéphanie Descroix; Laurent Malaquin; Florence Goutelard; Clarisse Mariet

2013-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "reactor spent fuel" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


381

Fusion solution to dispose of spent nuclear fuel, transuranic elements, and highly enriched uranium  

Science Journals Connector (OSTI)

The disposal of the nuclear spent fuel, the transuranic elements, and the highly enriched uranium represents a major problem under investigation by the international scientific community to identify the most promising solutions. The investigation of this paper focused on achieving the top rated solution for the problem, the elimination goal, which requires complete elimination for the transuranic elements or the highly enriched uranium, and the long-lived fission products. To achieve this goal, fusion blankets with liquid carrier, molten salts or liquid metal eutectics, for the transuranic elements and the uranium isotopes are utilized. The generated energy from the fusion blankets is used to provide revenue for the system. The long-lived fission products are fabricated into fission product targets for transmutation utilizing the neutron leakage from the fusion blankets. This paper investigated the fusion blanket designs for small fusion devices and the system requirements for such application. The results show that 334 MW of fusion power from D–T plasma for 30 years with an availability factor of 0.75 can dispose of the 70,000 tons of the U.S. inventory of spent nuclear fuel generated up to the year 2015. In addition, this fusion solution eliminates the need for a geological repository site, which is a major advantage. Meanwhile, such utilization of the fusion power will provide an excellent opportunity to develop fusion energy for the future.

Yousry Gohar

2001-01-01T23:59:59.000Z

382

Consideration of critically when directly disposing highly enriched spent nuclear fuel in unsaturated tuff: Bounding estimates  

SciTech Connect (OSTI)

This report presents one of 2 approaches (bounding calculations) which were used in a 1994 study to examine the possibility of a criticality in a repository. Bounding probabilities, although rough, point to the difficulty of creating conditions under which a critical mass could be assembled (container corrosion, separation of neutron absorbers from fissile material, collapse or precipitation of fissile material) and how significant the geochemical and hydrologic phenomena are. The study could not conceive of a mechanism consistent with conditions under which an atomic explosion could occur. Should a criticality occur in or near a container in the future, boundary consequence calculations showed that fissions from one critical event (<10{sup 20} fissions, if similar to aqueous and metal accidents and experiments) are quite small compared to the amount of fissions represented by the spent fuel itself. If it is assumed that the containers necessary to hold the highly enriched spent fuel went critical once per day for 1 million years, creating an energy release of about 10{sup 20} fissions, the number of fissions equals about 10{sup 28}, which corresponds to only 1% of the fission inventory in a repository containing 70,000 metric tons of heavy metal, the expected size for the proposed repository at Yucca Mountain, Nevada.

Rechard, R.P.; Tierney, M.S.; Sanchez, L.C.; Martell, M.-A.

1996-05-01T23:59:59.000Z

383

Electrorefining process and apparatus for recovery of uranium and a mixture of uranium and plutonium from spent fuels  

DOE Patents [OSTI]

An electrorefining process and apparatus for the recovery of uranium and a mixture of uranium and plutonium from spent fuels is disclosed using an electrolytic cell having a lower molten cadmium pool containing spent nuclear fuel, an intermediate electrolyte pool, an anode basket containing spent fuels, two cathodes and electrical power means connected to the anode basket, cathodes and lower molten cadmium pool for providing electrical power to the cell. Using this cell, additional amounts of uranium and plutonium from the anode basket are dissolved in the lower molten cadmium pool, and then purified uranium is electrolytically transported and deposited on a first molten cadmium cathode. Subsequently, a mixture of uranium and plutonium is electrotransported and deposited on a second cathode. 3 figs.

Ackerman, J.P.; Miller, W.E.

1987-11-05T23:59:59.000Z

384

Electrorefining process and apparatus for recovery of uranium and a mixture of uranium and plutonium from spent fuels  

DOE Patents [OSTI]

An electrorefining process and apparatus for the recovery of uranium and a mixture of uranium and plutonium from spent fuel using an electrolytic cell having a lower molten cadmium pool containing spent nuclear fuel, an intermediate electrolyte pool, an anode basket containing spent fuel, and two cathodes, the first cathode composed of either a solid alloy or molten cadmium and the second cathode composed of molten cadmium. Using this cell, additional amounts of uranium and plutonium from the anode basket are dissolved in the lower molten cadmium pool, and then substantially pure uranium is electrolytically transported and deposited on the first alloy or molten cadmium cathode. Subsequently, a mixture of uranium and plutonium is electrotransported and deposited on the second molten cadmium cathode.

Ackerman, John P. (Downers Grove, IL); Miller, William E. (Naperville, IL)

1989-01-01T23:59:59.000Z

385

RISKIND: A computer program for calculating radiological consequences and health risks from transportation of spent nuclear fuel  

SciTech Connect (OSTI)

This report presents the technical details of RISIUND, a computer code designed to estimate potential radiological consequences and health risks to individuals and the collective population from exposures associated with the transportation of spent nuclear fuel. RISKIND is a user-friendly, semiinteractive program that can be run on an IBM or equivalent personal computer. The program language is FORTRAN-77. Several models are included in RISKIND that have been tailored to calculate the exposure to individuals under various incident-free and accident conditions. The incidentfree models assess exposures from both gamma and neutron radiation and can account for different cask designs. The accident models include accidental release, atmospheric transport, and the environmental pathways of radionuclides from spent fuels; these models also assess health risks to individuals and the collective population. The models are supported by databases that are specific to spent nuclear fuels and include a radionudide inventory and dose conversion factors.

Yuan, Y.C. [Square Y, Orchard Park, NY (United States); Chen, S.Y.; LePoire, D.J. [Argonne National Lab., IL (United States). Environmental Assessment and Information Sciences Div.; Rothman, R. [USDOE Idaho Field Office, Idaho Falls, ID (United States)

1993-02-01T23:59:59.000Z

386

COBRA-SFS (Spent Fuel Storage): A thermal-hydraulic analysis computer code: Volume 2, User's manual  

SciTech Connect (OSTI)

COBRA-SFS (Spent Fuel Storage) is a general thermal-hydraulic analysis computer code used to predict temperatures and velocities in a wide variety of systems. The code was refined and specialized for spent fuel storage system analyses for the US Department of Energy's Commercial Spent Fuel Management Program. The finite-volume equations governing mass, momentum, and energy conservation are written for an incompressible, single-phase fluid. The flow equations model a wide range of conditions including natural circulation. The energy equations include the effects of solid and fluid conduction, natural convection, and thermal radiation. The COBRA-SFS code is structured to perform both steady-state and transient calculations; however, the transient capability has not yet been validated. This volume contains the input instructions for COBRA-SFS and an auxiliary radiation exchange factor code, RADX-1. It is intended to aid the user in becoming familiar with the capabilities and modeling conventions of the code.

Rector, D.R.; Cuta, J.M.; Lombardo, N.J.; Michener, T.E.; Wheeler, C.L.

1986-11-01T23:59:59.000Z

387

Measurement and analysis of gamma-rays emitted from spent nuclear fuel above 3 MeV  

SciTech Connect (OSTI)

The Next Generation Safeguard Initiative (NGSI) includes an effort to determine the mass content of fissile isotopes contained within spent fuel through the spectroscopy of high-energy delayed gamma rays. Studies being performed indicate the primary difficulty is the ability to detect the desired signal in the presence of the intense background associated with spent fuel fission products. An enabling technology for this application is high-resolution high-purity germanium (HPGe) detectors capable of operating efficiently in at extremely high count rates. This presentation will describe the prospects of high-rate germanium detectors and delayed-gamma techniques, primarily discussing the efforts to merge these into a unique and viable system for measuring spent fuel.

Rodriguez, Douglas C. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Anderson, Elaina R. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); State Univ. of New York at Stony Brook, NY (United States); Anderson, Kevin K. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Campbell, Luke W. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Fast, James E. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Jarman, Kenneth D. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Kulisek, Jonathan A. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Orton, Christopher R. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Runkle, Robert C. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Stave, Sean [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

2013-08-28T23:59:59.000Z

388

COBRA-SFS (Spent Fuel Storage): A thermal-hydraulic analysis computer code: Volume 1, Mathematical models and solution method  

SciTech Connect (OSTI)

COBRA-SFS (Spent Fuel Storage) is a general thermal-hydraulic analysis computer code used to predict temperatures and velocities in a wide variety of systems. The code was refined and specialized for spent fuel storage system analyses for the US Department of Energy's Commercial Spent Fuel Management Program. The finite-volume equations governing mass, momentum, and energy conservation are written for an incompressible, single-phase fluid. The flow equations model a wide range of conditions including natural circulation. The energy equations include the effects of solid and fluid conduction, natural convection, and thermal radiation. The COBRA-SFS code is structured to perform both steady-state and transient calculations: however, the transient capability has not yet been validated. This volume describes the finite-volume equations and the method used to solve these equations. It is directed toward the user who is interested in gaining a more complete understanding of these methods.

Rector, D.R.; Wheeler, C.L.; Lombardo, N.J.

1986-11-01T23:59:59.000Z

389

COBRA-SFS thermal analysis of a sealed storage cask for the Monitored Retrievable Storage of spent fuel  

SciTech Connect (OSTI)

The COBRA-SFS (Spent Fuel Storage) computer code was used to predict temperature distributions in a concrete Sealed Storage Cask (SSC). This cask was designed for the Department of Energy in the Monitored Retrievable Storage (MRS) program for storage of spent fuel from commercial power operations. Analytical results were obtained for nominal operation of the SSC with spent fuel from 36 PWR fuel assemblies consolidated in 12 cylindrical canisters. Each canister generates 1650 W of thermal power. A parametric study was performed to assess the effects on cask thermal performance of thermal conductivity of the concrete, the fin material, and the amount of radial reinforcing steel bars (rebar). Seven different cases were modeled. The results of the COBRA-SFS analysis of the current cask design predict that the peak fuel cladding temperature in the SSC will not exceed the 37/sup 0/C design limit for the maximum spent fuel load of 19.8 kW and a maximum expected ambient temperature of 37.8/sup 0/C (100/sup 0/F). The results of the parametric analyses illustrate the importance of material selection and design optimization with regard to the SSC thermal performance.

Rector, D.R.; Wheeler, C.L.

1986-01-01T23:59:59.000Z

390

Parameter Selection for Department of Energy Spent Nuclear Fuel to be Used in the Yucca Mountain License Application  

SciTech Connect (OSTI)

This report contains the chemical, physical, and radiological parameters that were chosen to represent the U.S. Department of Energy spent nuclear fuel in the Yucca Mountain license application. It also contains the selected packaging requirements for the various fuel types and the criticality controls that were used. The data are reported for representative fuels and bounding fuels in groups of fuels that were selected for the analysis. The justification for the selection of each parameter is given. The data reported were not generated under any quality assurance program.

D. L. Fillmore

2003-10-01T23:59:59.000Z

391

Nuclear reactor vessel fuel thermal insulating barrier  

DOE Patents [OSTI]

The reactor vessel of a nuclear reactor installation which is suspended from the cold leg nozzles in a reactor cavity is provided with a lower thermal insulating barrier spaced from the reactor vessel that has a hemispherical lower section that increases in volume from the center line of the reactor to the outer extent of the diameter of the thermal insulating barrier and smoothly transitions up the side walls of the vessel. The space between the thermal insulating harrier and the reactor vessel forms a chamber which can be flooded with cooling water through passive valving to directly cool the reactor vessel in the event of a severe accident. The passive inlet valve for the cooling water includes a buoyant door that is normally maintained sealed under its own weight and floats open when the cavity is Hooded. Passively opening steam vents are also provided.

Keegan, C. Patrick; Scobel, James H.; Wright, Richard F.

2013-03-19T23:59:59.000Z

392

Removal plan for Shippingport pressurized water reactor core 2 blanket fuel assemblies form T plant to the canister storage building  

SciTech Connect (OSTI)

This document presents the current strategy and path forward for removal of the Shippingport Pressurized Water Reactor Core 2 blanket fuel assemblies from their existing storage configuration (wet storage within the T Plant canyon) and transport to the Canister Storage Building (designed and managed by the Spent Nuclear Fuel. Division). The removal plan identifies all processes, equipment, facility interfaces, and documentation (safety, permitting, procedures, etc.) required to facilitate the PWR Core 2 assembly removal (from T Plant), transport (to the Canister storage Building), and storage to the Canister Storage Building. The plan also provides schedules, associated milestones, and cost estimates for all handling activities.

Lata

1996-09-26T23:59:59.000Z

393

Characterization of the neutron source term and multiplicity of a spent fuel assembly in support of NSDA safeguards of spent nuclear fuel  

SciTech Connect (OSTI)

The gross neutron signal (GNS) is being considered as part of a fingerprinting or neutron balance approach to safeguards of spent nuclear fuel (SNF). Because the GNS is composed of many derivative components, understanding the time-dependent contribution of these derivative components is crucial to gauging the limitations of these approaches. The major components of the GNS are ({alpha}, n), spontaneous fission (SF), and multiplication neutrons. A methodology was developed to link MCNPX burnup output files to SOURCES4C input files for the purpose of automatically generating both the ({alpha}, n) and SF signals. Additional linking capabilities were developed to write MCNPX multiplication input files using the data obtained from the SOURCES4C output files. In this paper, the following are presented: (1) the relative contributions by source nuclide to the ({alpha}, n) signal as a function of initial enrichment/burnup/cooling time; (2) the relative contributions by source nuclide to the SF signal as a function of initial enrichment/burnup/cooling time; (3) the relative contributions by reaction type ({alpha},n vs. SF) to the GNS; and (4) the multiplication of the GNS as a function of initial enrichment/burnup/cooling time/counting environment. By developing these technologies to characterize the GNS, we can better evaluate the viability of the GNS fingerprint and neutron balance concepts for SNF.

Richard, Joshua G [Los Alamos National Laboratory; Fensin, Michael L [Los Alamos National Laboratory; Tobin, Stephen J [Los Alamos National Laboratory; Swinhoe, Martyn T [Los Alamos National Laboratory; Menlove, Howard O [Los Alamos National Laboratory; Baciak, James [UNIV OF FL.