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  1. Nepal: Energy Resources | Open Energy Information

    Open Energy Info (EERE)

    Country Profile Name Nepal Population 26,494,504 GDP Unavailable Energy Consumption 0.08 Quadrillion Btu 2-letter ISO code NP 3-letter ISO code NPL Numeric ISO...

  2. Nepal-NREL Cooperation | Open Energy Information

    Open Energy Info (EERE)

    Nepal-NREL Cooperation Jump to: navigation, search Logo: Nepal-NREL Cooperation Name Nepal-NREL Cooperation AgencyCompany Organization National Renewable Energy Laboratory...

  3. Nepal-Sectoral Climate Impacts Economic Assessment | Open Energy...

    Open Energy Info (EERE)

    Nepal-Sectoral Climate Impacts Economic Assessment (Redirected from Nepal Sectoral Climate impacts Economic Assessment) Jump to: navigation, search Name Nepal Sectoral Climate...

  4. NP Science Network Requirements

    SciTech Connect (OSTI)

    Dart, Eli; Rotman, Lauren; Tierney, Brian

    2011-08-26

    The Energy Sciences Network (ESnet) is the primary provider of network connectivity for the U.S. Department of Energy (DOE) Office of Science (SC), the single largest supporter of basic research in the physical sciences in the United States. To support SC programs, ESnet regularly updates and refreshes its understanding of the networking requirements of the instruments, facilities, scientists, and science programs it serves. This focus has helped ESnet to be a highly successful enabler of scientific discovery for over 20 years. In August 2011, ESnet and the Office of Nuclear Physics (NP), of the DOE SC, organized a workshop to characterize the networking requirements of the programs funded by NP. The requirements identified at the workshop are summarized in the Findings section, and are described in more detail in the body of the report.

  5. NP-NearFinal

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    NP / ASCR Requirements Workshop May 26 and 27, 2011 LARGE SCALE COMPUTING AND STORAGE REQUIREMENTS Nuclear Physics Large Scale Computing and Storage Requirements for Nuclear Physics i Large Scale Computing and Storage Requirements for Nuclear Physics ii DISCLAIMER This report was prepared as an account of a workshop sponsored by the U.S. Department of Energy. Neither the United States Government nor any agency thereof, nor any of their employees or officers, makes any warranty, express or

  6. Nepal-USAID Climate Activities | Open Energy Information

    Open Energy Info (EERE)

    investments to increase Nepal's use of hydropower, USAID secured funding to develop two micro-hydropower projects in the Dolpa and Taplejung districts of Nepal. The first power...

  7. Nepal-Sectoral Climate Impacts Economic Assessment | Open Energy...

    Open Energy Info (EERE)

    Nepal-Sectoral Climate Impacts Economic Assessment Jump to: navigation, search Name Nepal Sectoral Climate impacts Economic Assessment AgencyCompany Organization Climate and...

  8. Nepal-Climate Change Support Programme | Open Energy Information

    Open Energy Info (EERE)

    Nepal-Climate Change Support Programme Jump to: navigation, search Name Nepal Climate Change Support Programme AgencyCompany Organization United Kingdom Department for...

  9. Yukiko-NP-NERSCWorkshop.ppt

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    NP/NERSC Requirements Gathering Workshop Yukiko Sekine Program Manager, Facilities Division Advanced Scientific Computing Research Office of Science, DOE May 26 & 27, 2011 Advanced Scientific Computing Research Topics for Discussion * Goal and Outcome of this Workshop * Other approaches to NERSC requirements gathering * Benefits of SC/HQ-centric requirements gathering for NERSC resources in the context of Programmatic mission needs * NERSC requirements gathering workshop schedule * Past

  10. HEP/NP Requirements Review 2013

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    NP Program Offices. These requirements will serve as input to the ESnet architecture and planning processes, and will help ensure that ESnet continues to provide world-class...

  11. OpenSM Monitoring System

    Energy Science and Technology Software Center (OSTI)

    2015-04-17

    The OpenSM Monitoring System includes a collection of diagnostic and monitoring tools for use on Infiniband networks. The information this system gathers is obtained from a service, which in turn is obtained directly from the OpenSM subnet manager.

  12. Nepal-Pilot Program for Climate Resilience (PPCR) | Open Energy...

    Open Energy Info (EERE)

    Pilot Program for Climate Resilience (PPCR) Jump to: navigation, search Name Nepal-Pilot Program for Climate Resilience (PPCR) AgencyCompany Organization World Bank Sector...

  13. Nepal-GTZ Energy Efficiency Program | Open Energy Information

    Open Energy Info (EERE)

    1 GTZ is working with Nepal on integration of EE as part of the national energy strategy, development of EE measures for households. References "GTZ projects" Retrieved...

  14. HEP/NP Requirements Review 2013

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    HEP/NP Requirements Review 2013 Science Engagement Move your data Programs & Workshops Science Requirements Reviews Network Requirements Reviews Documents and Background Materials FAQ for Case Study Authors BER Requirements Review 2015 ASCR Requirements Review 2015 Previous Reviews HEP/NP Requirements Review 2013 HEP Attendees 2013 FES Requirements Review 2014 BES Requirements Review 2014 Requirements Review Reports Case Studies Contact Us Technical Assistance: 1 800-33-ESnet (Inside US) 1

  15. LITERATURE REVIEW: REDUCTION OF NP(V) TO NP (IV)-ALTERNATIVES TO FERROUS SULFAMATE

    SciTech Connect (OSTI)

    Kessinger, G.; Kyser, E.; Almond, P.

    2009-09-28

    The baseline approach to control of Np oxidation in UREX and PUREX separation processes is the reduction of Np(V) and Np(VI) to Np(IV) using ferrous sulfamate. Use of this reagent results in increased sulfur and iron concentrations in the liquid waste streams from the process. Presence of these two elements, especially sulfur, increases the complexity of the development of wasteforms for immobilizing these effluents. Investigations are underway to identify reductants that eliminate sulfur and iron from the Np reduction process. While there are a variety of chemical reductants that will reduce Np to Np(IV) in nitric acid media, the reaction rates for most are so slow that the reductants are not be feasible for use in an operating plant process. In an attempt to identify additional alternatives to ferrous sulfamate, a literature search and review was performed. Based on the results of the literature review, it is concluded that photochemical and catalytic processes should also be investigated to test the utility of these two approaches. The catalytic process could be investigated for use in conjunction with chemical oxidants to speed the reaction rates for reductants that react slowly, but would otherwise be appropriate replacements for ferrous sulfamate. The photochemical approach, which has received little attention during the past few decades, also shows promise, especially the photocatalytic approach that includes a catalyst, such as Pt supported on SiC, which can be used in tandem with an oxidant, for Np reduction.

  16. NP-MHTGR Fuel Development Program Results

    SciTech Connect (OSTI)

    Maki, John Thomas; Petti, David Andrew; Hobbins, Richard Redfield; McCardell, Richard K.; Shaber, Eric Lee; Southworth, Finis Hio

    2002-10-01

    In August 1988, the Secretary of Energy announced a strategy to acquire New Production Reactor capacity for producing tritium. The strategy involved construction of a New Production Modular High Temperature Gas-Cooled Reactor (NP-MHTGR) where the Idaho National Engineering and Environmental Laboratory (INEEL) was selected as the Management and Operations contractor for the project. Immediately after the announcement in August 1988, tritium target particle development began with the INEEL selected as the lead laboratory. Fuel particle development was initially not considered to be on a critical path for the project, therefore, the fuel development program was to run concurrently with the design effort of the NP-MHTGR.

  17. NP Budget | U.S. DOE Office of Science (SC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Budget Nuclear Physics (NP) NP Home About Organization Chart .pdf file (90KB) Staff NP Budget NP Committees of Visitors Directions Jobs Labs & Universities Nuclear Physics Related Brochures Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301)

  18. NP Committees of Visitors | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

    NSAC COV Report on NP Program .pdf file (1.8MB) NP Response to NSAC COV Report on NP .pdf file (56KB) 2010 NSAC COV Report on NP Program .pdf file (410KB) NP Response to NSAC COV ...

  19. Absolute photoneutron cross sections of Sm isotopes

    SciTech Connect (OSTI)

    Gheorghe, I.; Glodariu, T.; Utsunomiya, H.; Filipescu, D.; Nyhus, H.-T.; Renstrom, T.; Tesileanu, O.; Shima, T.; Takahisa, K.; Miyamoto, S.

    2015-02-24

    Photoneutron cross sections for seven samarium isotopes, {sup 144}Sm, {sup 147}Sm, {sup 148}Sm, {sup 149}Sm, {sup 150}Sm, {sup 152}Sm and {sup 154}Sm, have been investigated near neutron emission threshold using quasimonochromatic laser-Compton scattering γ-rays produced at the synchrotron radiation facility NewSUBARU. The results are important for nuclear astrophysics calculations and also for probing γ-ray strength functions in the vicinity of neutron threshold. Here we describe the neutron detection system and we discuss the related data analysis and the necessary method improvements for adapting the current experimental method to the working parameters of the future Gamma Beam System of Extreme Light Infrastructure - Nuclear Physics facility.

  20. Gamma beam system at ELI-NP

    SciTech Connect (OSTI)

    Ur, Calin Alexandru

    2015-02-24

    The Gamma Beam System of ELI-NP will produce brilliant, quasi-monochromatic gamma-ray beams via Inverse Compton Scattering of short laser pulses on relativistic electron beam pulses. The scattered radiation is Doppler upshifted by more than 1,000,000 times and is forward focused in a narrow, polarized, tunable, laser-like beam. The gamma-ray beam at ELI-NP will be characterized by large spectral density of about 10{sup 4} photons/s/eV, narrow bandwidth (< 0.5%) and tunable energy from 200 keV up to about 20 MeV. The Gamma Beam System is a state-of-the-art equipment employing techniques and technologies at the limits of the present-day's knowledge.

  1. Barnes_NP_Program_Office_Research_Directions_V2.pptx

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Physics (NP): Target 2017 April 29-30, 2014 Bethesda, MD Ted Barnes DOENP Program Manager, Nuclear Data & Nuclear Theory Computing NP Program Office Research Directions n.b. ...

  2. EA-165 NP Energy INC. | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Order authorizing NP Energy INC to export electric energy to Canada. EA-165 NP Energy INC. (44.4 KB) More Documents & Publications EA-162 PP&L, Inc EA-163 Duke Energy Trading and ...

  3. NP Early Career Opportunities Archives | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

    Funding Opportunities » NP Early Career Opportunities » NP Early Career Opportunities Archives Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Closed Funding Opportunity Announcements (FOAs) Closed Lab Announcements Award Search / Public Abstracts Additional Requirements and Guidance for Digital Data Management Reviews NP Early Career Opportunities NP Early Career Opportunities Archives Nuclear Science Advisory Committee (NSAC)

  4. ApplicationReadinessLunchNP.pptx

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Transitioning to NERSC-8 and Beyond --- 1 --- NP R equirements R eview April 2 9, 2 014 Harvey Wasserman What This Talk is About * NERSC w ill a nnounce t he N ERSC---8 a rchitecture soon. * This t alk c oncerns p reparaEon f or t he s ystem. * Although w e c annot d isclose t he a rchitecture f or NERSC---8, t rend f or a ll 2 015---2016 s ystems i s manycore --- 2 --- NERSC-8 Project Goals * NERSC d irectly s upports D OE's s cience m ission; w e f ocus o n the scienEfic impact of our users *

  5. Sierra/SM theory manual.

    SciTech Connect (OSTI)

    Crane, Nathan Karl

    2013-07-01

    Presented in this document are the theoretical aspects of capabilities contained in the Sierra/SM code. This manuscript serves as an ideal starting point for understanding the theoretical foundations of the code. For a comprehensive study of these capabilities, the reader is encouraged to explore the many references to scientific articles and textbooks contained in this manual. It is important to point out that some capabilities are still in development and may not be presented in this document. Further updates to this manuscript will be made as these capabilites come closer to production level.

  6. Barnes_NP_Program_Office_Research_Directions_V2.pptx

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Timothy J. Hallman Associate Director for Nuclear Physics DOE Office of Science NP-NERSC Meeting on: Large Scale Computing and Storage Requirements for Nuclear Physics (NP): Target 2017 April 29-30, 2014 Bethesda, MD Ted Barnes DOE/NP Program Manager, Nuclear Data & Nuclear Theory Computing NP Program Office Research Directions n.b. Many slides c/o T. Hallman, "NP Overview" presentation to NSAC, 4/24/2014. NSAC Meeting December 119 2013 DOE Nuclear Physics Mission Statement 2

  7. DOE-NP SBIR/STTR Exchange Meeting

    Office of Science (SC) Website

    August 9-10 2016| U.S. DOE Office of Science (SC) 9-10 2016 Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of Nuclear Science Small Business Innovation Research / Small Business Technology Transfer Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F:

  8. NP Early Career Opportunities | U.S. DOE Office of Science (SC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    NP Early Career Opportunities Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Closed Funding Opportunity Announcements (FOAs) Closed Lab Announcements Award Search / Public Abstracts Additional Requirements and Guidance for Digital Data Management Reviews NP Early Career Opportunities NP Early Career Opportunities Archives Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S.

  9. SM Environmental Technologies Pvt Ltd | Open Energy Information

    Open Energy Info (EERE)

    SM Environmental Technologies Pvt Ltd Jump to: navigation, search Name: SM Environmental Technologies Pvt. Ltd. Place: Tamil Nadu, India Sector: Biomass Product: Chennai-based...

  10. Laminin receptor specific therapeutic gold nanoparticles (198AuNP...

    Office of Scientific and Technical Information (OSTI)

    prostate cancer Citation Details In-Document Search Title: Laminin receptor specific therapeutic gold nanoparticles (198AuNP-EGCg) show efficacy in treating prostate cancer ...

  11. MHK Technologies/Neptune Proteus NP1000 | Open Energy Information

    Open Energy Info (EERE)

    Neptune Proteus NP1000.jpg Technology Profile Primary Organization Neptune Renewable Energy Ltd Project(s) where this technology is utilized *MHK ProjectsNeptune Renewable...

  12. Ferro- and antiferro-magnetism in (Np, Pu)BC

    SciTech Connect (OSTI)

    Klimczuk, T.; Kozub, A. L.; Griveau, J.-C.; Colineau, E.; Wastin, F.; Falmbigl, M.; Rogl, P.

    2015-04-01

    Two new transuranium metal boron carbides, NpBC and PuBC, have been synthesized. Rietveld refinements of powder XRD patterns of (Np,Pu)BC confirmed in both cases isotypism with the structure type of UBC. Temperature dependent magnetic susceptibility data reveal antiferromagnetic ordering for PuBC below T{sub N} = 44 K, whereas ferromagnetic ordering was found for NpBC below T{sub C} = 61 K. Heat capacity measurements prove the bulk character of the observed magnetic transition for both compounds. The total energy electronic band structure calculations support formation of the ferromagnetic ground state for NpBC and the antiferromagnetic ground state for PuBC.

  13. NP Budget | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

    Print Text Size: A A A FeedbackShare Page The following links contain NP's budget request to Congress for current and prior years: FY2017 Budget Request to Congress .pdf file ...

  14. NP Committees of Visitors | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

    The links below provide an archive of Nuclear Physics (NP) Committees of Visitors (COV) reports and responses. 2016 NSAC COV Report on NP Program .pdf file (1.4MB) NP Response to ...

  15. Conceptual Design Plan SM-43 Replacement Project

    SciTech Connect (OSTI)

    University of California, Los Alamos National Laboratory, SCC Project Office

    2000-11-01

    The Los Alamos National Laboratory Conceptual Design Plan for the SM-43 Replacement Project outlines plans for replacing the SM-43 Administration Building. Topics include the reasons that replacement is considered a necessity; the roles of the various project sponsors; and descriptions of the proposed site and facilities. Also covered in this proposal is preliminary information on the project schedule, cost estimates, acquisition strategy, risk assessment, NEPA strategy, safety strategy, and safeguards and security. Spreadsheets provide further detail on space requirements, project schedules, and cost estimates.

  16. Combined SM Higgs Limits at the Tevatron

    SciTech Connect (OSTI)

    Krumnack, N.

    2009-10-01

    We combine results from CDF and D{sup 0} on direct searches for a standard model (SM) Higgs boson (H) in p{bar p} collisions at the Fermilab Tevatron at {radical}s = 1.96 TeV. Compared to the previous Higgs Tevatron combination, more data and new channels WH {yields} {tau}{nu}b{bar b}, VH {yields} {tau}{tau}b{bar b}/jj{tau}{tau}, VH {yields} jjb{bar b}, t{bar t}H {yields} t{bar t}b{bar b} have been added. Most previously used channels have been reanalyzed to gain sensitivity. We use the latest parton distribution functions and gg {yields} H theoretical cross sections when comparing our limits to the SM predictions. With 2.0-3.6 fb{sup -1} of data analyzed at CDF, and 0.9-4.2 fb{sup -1} at D{sup 0}, the 95% C.L. upper limits on Higgs boson production are a factor of 2.5 (0.86) times the SM cross section for a Higgs boson mass of m{sub H} = 115 (165) GeV/c{sup 2}. Based on simulation, the corresponding median expected upper limits are 2.4 (1.1). The mass range excluded at 95% C.L. for a SM Higgs has been extended to 160 < m{sub H} < 170 GeV/c{sup 2}.

  17. SmAHTR-CTC Neutronic Design

    SciTech Connect (OSTI)

    Ilas, Dan; Holcomb, David Eugene; Gehin, Jess C

    2014-01-01

    Building on prior experience for the 2010 initial SmAHTR neutronic design and on 2012 neutronic design for the advanced high temperature reactor (AHTR), this paper presents the main results of the neutronic design effort for the newly re-purposed SmAHTR-CTC reactor concept. The results are obtained based on full-core simulations performed with SCALE6.1. The dimensionality of the SmAHTR design space is reduced by using constraints originating in material fabricability, fuel licensing, molten salt chemistry, thermal-hydraulic and mechanical considerations. The new design represents in many regards a substantial improvement from the neutronic performance standpoint over the 2010 SmAHTR concept. Among other results, it is shown that fuel cycle length of over 2 years or discharged fuel burnup of 40GWd/MTHM are possible with a low, 8% fuel enrichment in a once-through fuel cycle, while 8-year once-through fuel cycle lengths are possible at higher fuel enrichments.

  18. NP Committees of Visitors | U.S. DOE Office of Science (SC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Committees of Visitors Nuclear Physics (NP) NP Home About Organization Chart .pdf file (90KB) Staff NP Budget NP Committees of Visitors Directions Jobs Labs & Universities Nuclear Physics Related Brochures Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301)

  19. Method for separating actinides. [Patent application; stripping of Np from organic extractant

    DOE Patents [OSTI]

    Friedman, H.A.; Toth, L.M.

    1980-11-10

    An organic solution used for processing spent nuclear reactor fuels is contacted with an aqueous nitric acid solution to strip Np(VI), U(VI), and Pu(IV) from the organic solution into the acid solution. The acid solution is exposed to ultraviolet light, which reduces Np(VI) to Np(V) without reducing U(VI) and Pu(IV). Since the solubility of Np(V) in the organic solution is much lower than that of Np(VI), U(VI), and Pu(IV), a major part of the Np is stripped from the organic solution while leaving most of the U and Pu therein.

  20. Covariant spectator theory of np scattering: Deuteron quadrupole moment

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Gross, Franz

    2015-01-26

    The deuteron quadrupole moment is calculated using two CST model wave functions obtained from the 2007 high precision fits to np scattering data. Included in the calculation are a new class of isoscalar np interaction currents automatically generated by the nuclear force model used in these fits. The prediction for model WJC-1, with larger relativistic P-state components, is 2.5% smaller that the experiential result, in common with the inability of models prior to 2014 to predict this important quantity. However, model WJC-2, with very small P-state components, gives agreement to better than 1%, similar to the results obtained recently frommore » XEFT predictions to order N3LO.« less

  1. Covariant spectator theory of np scattering: Deuteron quadrupole moment

    SciTech Connect (OSTI)

    Gross, Franz

    2015-01-26

    The deuteron quadrupole moment is calculated using two CST model wave functions obtained from the 2007 high precision fits to np scattering data. Included in the calculation are a new class of isoscalar np interaction currents automatically generated by the nuclear force model used in these fits. The prediction for model WJC-1, with larger relativistic P-state components, is 2.5% smaller that the experiential result, in common with the inability of models prior to 2014 to predict this important quantity. However, model WJC-2, with very small P-state components, gives agreement to better than 1%, similar to the results obtained recently from XEFT predictions to order N3LO.

  2. Robust ferromagnetism in the compressed permanent magnet Sm 2...

    Office of Scientific and Technical Information (OSTI)

    Journal Article: Robust ferromagnetism in the compressed permanent magnet Sm 2 Co 17 Citation Details In-Document Search Title: Robust ferromagnetism in the compressed permanent ...

  3. Determining the 239Np(n,f) cross section using the surrogate...

    Office of Scientific and Technical Information (OSTI)

    Journal Article: Determining the 239Np(n,f) cross section using the surrogate ratio method Citation Details In-Document Search Title: Determining the 239Np(n,f) cross section using ...

  4. Np and Pu Sorption to Manganese Oxide Minerals

    SciTech Connect (OSTI)

    Zhao, P; Johnson, M R; Roberts, S K; Zavarin, M

    2005-08-30

    Manganese oxide minerals are a significant component of the fracture lining mineralogy at Yucca Mountain (Carlos et al., 1993) and within the tuff-confining unit at Yucca Flat (Prothro, 1998), Pahute Mesa (Drellack et al., 1997), and other locations at the Nevada Test Site (NTS). Radionuclide sorption to manganese oxide minerals was not included in recent Lawrence Livermore National Laboratory (LLNL) hydrologic source term (HST) models which attempt to predict the migration behavior of radionuclides away from underground nuclear tests. However, experiments performed for the Yucca Mountain Program suggest that these minerals may control much of the retardation of certain radionuclides, particularly Np and Pu (Triay et al., 1991; Duff et al., 1999). As a result, recent HST model results may significantly overpredict radionuclide transport away from underground nuclear tests. The sorption model used in HST calculations performed at LLNL includes sorption to iron oxide, calcite, zeolite, smectite, and mica minerals (Zavarin and Bruton 2004a; 2004b). For the majority of radiologic source term (RST) radionuclides, we believe that this accounts for the dominant sorption processes controlling transport. However, for the case of Np, sorption is rather weak to all but the iron and manganese oxides (Figure 1). Thus, we can expect to significantly reduce predicted Np transport by accounting for Np sorption to manganese oxides. Similarly, Pu has been shown to be predominantly associated with manganese oxides in Yucca Mountain fractured tuffs (Duff et al., 1999). Recent results on colloid-facilitated Pu transport (Kersting and Reimus, 2003) also suggest that manganese oxide coatings on fracture surfaces may compete with colloids for Pu, thus reducing the effects of colloid-facilitated Pu transport (Figure 1b). The available data suggest that it is important to incorporate Np and Pu sorption to manganese oxides in reactive transport models. However, few data are available for

  5. Nuclear Physics (NP) Homepage | U.S. DOE Office of Science (SC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    NP Home Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email Us More Information » Accelerating Innovation .pdf file (1.2MB) Nuclear Physics supports the experimental and theoretical research needed

  6. SmAHTR-CTC Neutronic Design (Conference) | SciTech Connect

    Office of Scientific and Technical Information (OSTI)

    SmAHTR-CTC Neutronic Design Citation Details In-Document Search Title: SmAHTR-CTC Neutronic Design Building on prior experience for the 2010 initial SmAHTR neutronic design and on ...

  7. Friedrich: ENERGY STAR Referral (SM18M30)

    Broader source: Energy.gov [DOE]

    DOE referred the matter of Friedrich room air conditioner model SM18M30 to the EPA for appropriate action after DOE testing showed that the model does not meet the ENERGY STAR specification.

  8. Discovery of a metastable Al20Sm4 phase

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Ye, Z.; Zhang, F.; Sun, Y.; Mendelev, M. I.; Ott, R. T.; Park, E.; Besser, M. F.; Kramer, M. J.; Ding, Z.; Wang, C. -Z.; et al

    2015-03-09

    In this study, we present an efficient genetic algorithm, integrated with experimental diffraction data, to solve a nanoscale metastable Al20Sm4 phase that evolves during crystallization of an amorphous magnetron sputtered Al90Sm10 alloy. The excellent match between calculated and experimental X-ray diffraction patterns confirms an accurate description of this metastable phase. Molecular dynamic simulations of crystal growth from the liquid phase predict the formation of disordered defects in the devitrified crystal.

  9. Pesticide use knowledge and practices: A gender differences in Nepal

    SciTech Connect (OSTI)

    Atreya, Kishor . E-mail: k.atreya@gmail.com

    2007-06-15

    It is important to understand gender difference on pesticide use knowledge, attitude and practices for identifying pesticide risks by gender and to recommend more gender-sensitive programs. However, very few studies have been conducted so far in Nepal. This study, thus, interviewed a total of 325 males and 109 females during 2005 to assess gender differences on pesticide use knowledge, attitude and practices. More than 50% females had never been to school and only <8% individuals were found trained in Integrated Pest Management (IPM). Almost all males and females did not smoke, drink and eat during pesticides application and also believed that pesticides are harmful to human health, livestock, plant diversity and their environment. However, there were gender differences on household decision on pesticides to be used (p<0.001), care of wind direction during spraying (p=0.032), prior knowledge on safety measures (p=0.016), reading and understanding of pesticides labels (p<0.001), awareness of the labels (p<0.001) and protective covers. Almost all respondents were aware of negative impacts of pesticide use on human health and environment irrespective of gender; however, females were at higher risk due to lower level of pesticide use safety and awareness. It is strongly recommended to initiate gender-sensitive educational and awareness activities, especially on pesticide use practices and safety precautions.

  10. Facile Routes to Th(IV), U(IV), and Np(IV) Phosphites and Phosphates

    SciTech Connect (OSTI)

    Villa, Eric M.; Wang, Shuao; Alekseev, Evgeny V.; Depmeier, Wulf; Albrecht-Schmitt, Thomas E.

    2011-08-05

    Three actinide(IV) phosphites and a NpIV phosphate, AnIV(HPO₃)₂(H₂O)₂ (An = Th, U, Np) and Cs[Np(H1.5PO₄)(PO₄)]₂, respectively, were synthesized using mild hydrothermal conditions. The first three phases are isotypic and were obtained using similar reaction conditions. Cs[Np(H1.5PO₄)(PO₄)]₂ was synthesized using an analogous method to that of Np(HPO₃)₂(H₂O)₂. However, this fourth phase is quite different in comparison to the other phases in both composition and structure. The structure of Cs[Np(H1.5PO₄)(PO₄)]₂ is constructed from double layers of neptunium(IV) phosphate with caesium cations in the interlayer region. In contrast, An(HPO₃)₂(H₂O)₂ (An = Th, U, Np) form dense 3D networks. The actinide contraction is detected in variety of metrics obtained from single-crystal X-ray diffraction data. Changes in the oxidation state of the neptunium starting materials yield different products.

  11. Searches for Beyond SM Higgs Boson at the Tevatron

    SciTech Connect (OSTI)

    Safonov, A.; /Texas A-M

    2006-05-01

    In the following, the authors describe preliminary results of searches for non-SM higgs bosons at the CDF and D0 experiments. Both experiments use data obtained in p{bar p} collisions at the Tevatron at {radical}s = 1.96 TeV.

  12. Combined upper limit for SM Higgs at the Tevatron

    SciTech Connect (OSTI)

    Penning, Bjorn; /Fermilab

    2009-01-01

    We combine results from CDF and D0 on direct searches for a standard model (SM) Higgs boson (H) in p{bar p} collisions at the Fermilab Tevatron at {radical}s = 1.96 TeV. Compared to the previous Higgs Tevatron combination, more data and new channels (WH {yields} {tau}{nu}b{bar b}, VH {yields} {tau}{tau}b{bar b}/jj{tau}{tau}, VH {yields} jjb{bar b}, t{bar t}H {yields} t{bar t}b{bar b}) have been added. Most previously used channels have been reanalyzed to gain sensitivity. We use the latest parton distribution functions and gg {yields} H theoretical cross sections when comparing our limits to the SM predictions. With 2.0-3.6 fb{sup -1} of data analyzed at CDF, and 0.9-4.2 fb{sup -1} at D0, the 95%C.L. upper limits on Higgs boson production are a factor of 2.5 (0.86) times the SM cross section for a Higgs boson mass of m{sub H} = 115 (165) GeV/c{sup 2}. Based on simulation, the corresponding median expected upper limits are 2.4 (1.1). The mass range excluded at 95% C.L. for a SM Higgs has been extended to 160 < m{sub H} < 170 GeV/c{sup 2}.

  13. Robust ferromagnetism in the compressed permanent magnet Sm2Co17...

    Office of Scientific and Technical Information (OSTI)

    Robust ferromagnetism in the compressed permanent magnet Sm2Co17 Citation Details In-Document Search Title: Robust ferromagnetism in the compressed permanent magnet Sm2Co17 ...

  14. Ruby and Sm:YAG fluorescence pressure gauges up to 120 GPa and...

    Office of Scientific and Technical Information (OSTI)

    Ruby and Sm:YAG fluorescence pressure gauges up to 120 GPa and 700 K Citation Details In-Document Search Title: Ruby and Sm:YAG fluorescence pressure gauges up to 120 GPa and 700 K ...

  15. Structural Deformation of Sm@C88 Under High Pressure (Journal...

    Office of Scientific and Technical Information (OSTI)

    Deformation of Sm@C88 Under HighPressure Citation Details In-Document Search Title: Structural Deformation of Sm@C88 Under High Pressure Authors: J Cui ; M Yao ; H Yang ; Z Liu ; ...

  16. Approaching isotropy in the vortex system of SmFeAs(O,F) at extreme...

    Office of Scientific and Technical Information (OSTI)

    vortex system of SmFeAs(O,F) at extreme magnetic fields Citation Details In-Document Search Title: Approaching isotropy in the vortex system of SmFeAs(O,F) at extreme magnetic ...

  17. Discovery of a meta-stable Al-Sm phase with unknown stoichiometry...

    Office of Scientific and Technical Information (OSTI)

    Discovery of a meta-stable Al-Sm phase with unknown stoichiometry using a genetic algorithm Citation Details In-Document Search Title: Discovery of a meta-stable Al-Sm phase with...

  18. NP User Facilities | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

    User Facilities at a Glance NP User Facilities Print Text Size: A A A FeedbackShare Page The Nuclear Physics program supports the following national scientific user facilities: ...

  19. Enhanced conversion efficiency in wide-bandgap GaNP solar cells...

    Office of Scientific and Technical Information (OSTI)

    Enhanced conversion efficiency in wide-bandgap GaNP solar cells Citation Details In-Document Search This content will become publicly available on October 12, 2016 Title: Enhanced...

  20. Evaluation of the exothermicity of the chemi-ionization reaction Sm + O → SmO{sup +} + e{sup −}

    SciTech Connect (OSTI)

    Cox, Richard M; Kim, JungSoo; Armentrout, P. B. E-mail: mheaven@emory.edu; Bartlett, Joshua; VanGundy, Robert A.; Heaven, Michael C. E-mail: mheaven@emory.edu; Ard, Shaun G.; Shuman, Nicholas S.; Viggiano, Albert A. E-mail: mheaven@emory.edu; Melko, Joshua J.

    2015-04-07

    The exothermicity of the chemi-ionization reaction Sm + O → SmO{sup +} + e{sup −} has been re-evaluated through the combination of several experimental methods. The thermal reactivity (300–650 K) of Sm{sup +} and SmO{sup +} with a range of species measured using a selected ion flow tube-mass spectrometer apparatus is reported and provides limits for the bond strength of SmO{sup +}, 5.661 eV ≤ D{sub 0}(Sm{sup +}-O) ≤ 6.500 eV. A more precise value is measured to be 5.72{sub 5} ± 0.07 eV, bracketed by the observed reactivity of Sm{sup +} and SmO{sup +} with several species using a guided ion beam tandem mass spectrometer (GIBMS). Combined with the established Sm ionization energy (IE), this value indicates an exothermicity of the title reaction of 0.08 ± 0.07 eV, ∼0.2 eV smaller than previous determinations. In addition, the ionization energy of SmO has been measured by resonantly enhanced two-photon ionization and pulsed-field ionization zero kinetic energy photoelectron spectroscopy to be 5.7427 ± 0.0006 eV, significantly higher than the literature value. Combined with literature bond energies of SmO, this value indicates an exothermicity of the title reaction of 0.14 ± 0.17 eV, independent from and in agreement with the GIBMS result presented here. The evaluated thermochemistry also suggests that D{sub 0}(SmO) = 5.83 ± 0.07 eV, consistent with but more precise than the literature values. Implications of these results for interpretation of chemical release experiments in the thermosphere are discussed.

  1. DOE-NP SBIR/STTR Exchange Meeting 2014 | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

    4 Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of Nuclear Science Small Business Innovation Research / Small Business Technology Transfer Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email Us More Information » Small Business

  2. DOE-NP SBIR/STTR Exchange Meeting 2015 | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

    5 Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of Nuclear Science Small Business Innovation Research / Small Business Technology Transfer Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email Us More Information » Small Business

  3. Surface state reconstruction in ion-damaged SmB?

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Wakeham, N.; Wang, Y. Q.; Fisk, Z.; Ronning, F.; Thompson, J. D.

    2015-02-01

    We have used ion-irradiation to damage the (001) surfaces of SmB? single crystals to varying depths, and have measured the resistivity as a function of temperature for each depth of damage. We observe a reduction in the residual resistivity with increasing depth of damage. Our data are consistent with a model in which the surface state is not destroyed by the ion-irradiation, but instead the damaged layer is poorly conducting and the initial surface state is reconstructed below the damage. This behavior is consistent with a surface state that is topologically protected.

  4. Variable temperature electrochemical strain microscopy of Sm-doped ceria

    SciTech Connect (OSTI)

    Jesse, Stephen; Morozovska, A. N.; Kalinin, Sergei V; Eliseev, E. A.; Yang, Nan; Doria, Sandra; Tebano, Antonello

    2013-01-01

    Variable temperature electrochemical strain microscopy has been used to study the electrochemical activity of Sm-doped ceria as a function of temperature and bias. The electrochemical strain microscopy hysteresis loops have been collected across the surface at different temperatures and the relative activity at different temperatures has been compared. The relaxation behavior of the signal at different temperatures has been also evaluated to relate kinetic process during bias induced electrochemical reactions with temperature and two different kinetic regimes have been identified. The strongly non-monotonic dependence of relaxation behavior on temperature is interpreted as evidence for water-mediated mechanisms.

  5. Approaching isotropy in the vortex system of SmFeAs(O,F) at extreme...

    Office of Scientific and Technical Information (OSTI)

    Approaching isotropy in the vortex system of SmFeAs(O,F) at extreme magnetic fields ... Sponsoring Org: NSF Country of Publication: United States Language: English Subject: ...

  6. Tunable giant magnetic anisotropy in amorphous SmCo thin films

    SciTech Connect (OSTI)

    Magnus, F.; Moubah, R.; Roos, A. H.; Kapaklis, V.; Hjoervarsson, B.; Andersson, G.; Kruk, A.; Hase, T.

    2013-04-22

    SmCo thin films have been grown by magnetron sputtering at room temperature with a composition of 2-35 at. % Sm. Films with 5 at. % or higher Sm are amorphous and smooth. A giant tunable uniaxial in-plane magnetic anisotropy is induced in the films which peaks in the composition range 11-22 at. % Sm. This cross-over behavior is not due to changes in the atomic moments but rather the local configuration changes. The excellent layer perfection combined with highly tunable magnetic properties make these films important for spintronics applications.

  7. Enhanced conversion efficiency in wide-bandgap GaNP solar cells

    SciTech Connect (OSTI)

    Sukrittanon, Supanee; Liu, Ren; Ro, Yun Goo; Pan, Janet L.; Jungjohann, Katherine Leigh; Tu, Charles W.; Dayeh, Shadi A.

    2015-10-12

    In this study, we demonstrate –2.05 eV dilute nitride GaNP solar cells on GaP substrates for potential use as the top junction in dual-junction integrated cells on Si. By adding a small amount of N into indirect-bandgap GaP, GaNP has several extremely important attributes: a direct-bandgap that is also tunable, and easily attained lattice-match with Si. Our best GaNP solar cell ([N] –1.8%, Eg –2.05 eV) achieves an efficiency of 7.9%, even in the absence of a window layer. This GaNP solar cell's efficiency is 3× higher than the most efficient GaP solar cell to date and higher than other solar cells with similar direct bandgap (InGaP, GaAsP). Through a systematic study of the structural, electrical, and optical properties of the device, efficient broadband optical absorption and enhanced solar cell performance are demonstrated.

  8. Ab initio calculation of the $$np \\to d ³$$ radiative capture process

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Beane, Silas R.; Chang, Emmanuel; Detmold, William; Orginos, Kostas; Parreño, Assumpta; Savage, Martin J.; Tiburzi, Brian C.

    2015-09-24

    In this study, lattice QCD calculations of two-nucleon systems are used to isolate the short-distance two-body electromagnetic contributions to the radiative capture processmore » $$np \\to d\\gamma$$, and the photo-disintegration processes $$\\gamma^{(\\ast)} d \\to np$$. In nuclear potential models, such contributions are described by phenomenological meson-exchange currents, while in the present work, they are determined directly from the quark and gluon interactions of QCD. Calculations of neutron-proton energy levels in multiple background magnetic fields are performed at two values of the quark masses, corresponding to pion masses of $$m_\\pi \\sim 450$$ and 806 MeV, and are combined with pionless nuclear effective field theory to determine these low-energy inelastic processes. Extrapolating to the physical pion mass, a cross section of $$\\sigma^{lqcd}(np\\to d\\gamma)=332.4({\\tiny \\begin{array}{l}+5.4 \\\\ - 4.7\\end{array}})\\ mb$$ is obtained at an incident neutron speed of $$v=2,200\\ m/s$$, consistent with the experimental value of $$\\sigma^{expt}(np \\to d\\gamma) = 334.2(0.5)\\ mb$$.« less

  9. Enhanced conversion efficiency in wide-bandgap GaNP solar cells

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Sukrittanon, Supanee; Liu, Ren; Ro, Yun Goo; Pan, Janet L.; Jungjohann, Katherine Leigh; Tu, Charles W.; Dayeh, Shadi A.

    2015-10-12

    In this study, we demonstrate –2.05 eV dilute nitride GaNP solar cells on GaP substrates for potential use as the top junction in dual-junction integrated cells on Si. By adding a small amount of N into indirect-bandgap GaP, GaNP has several extremely important attributes: a direct-bandgap that is also tunable, and easily attained lattice-match with Si. Our best GaNP solar cell ([N] –1.8%, Eg –2.05 eV) achieves an efficiency of 7.9%, even in the absence of a window layer. This GaNP solar cell's efficiency is 3× higher than the most efficient GaP solar cell to date and higher than othermore » solar cells with similar direct bandgap (InGaP, GaAsP). Through a systematic study of the structural, electrical, and optical properties of the device, efficient broadband optical absorption and enhanced solar cell performance are demonstrated.« less

  10. Am phases in the matrix of a U–Pu–Zr alloy with Np, Am, and rare-earth elements

    SciTech Connect (OSTI)

    Janney, Dawn E.; Kennedy, J. Rory; Madden, James W.; O’Holleran, Thomas P.

    2015-01-01

    Phases and microstructures in the matrix of an as-cast U-Pu-Zr alloy with 3 wt% Am, 2% Np, and 8% rare-earth elements were characterized by scanning and transmission electron microscopy. The matrix consists primarily of two phases, both of which contain Am: ζ-(U, Np, Pu, Am) (~70 at% U, 5% Np, 14% Pu, 1% Am, and 10% Zr) and δ-(U, Np, Pu, Am)Zr2 (~25% U, 2% Np, 10-15% Pu, 1-2% Am, and 55-60 at% Zr). These phases are similar to those in U-Pu-Zr alloys, although the Zr content in ζ-(U, Np, Pu, Am) is higher than that in ζ-(U, Pu) and the Zr content in δ-(U, Np, Pu, Am)Zr2 is lower than that in δ-UZr2. Nanocrystalline actinide oxides with structures similar to UO2 occurred in some areas, but may have formed by reactions with the atmosphere during sample handling. Planar features consisting of a central zone of ζ-(U, Np, Pu, Am) bracketed by zones of δ-(U, Np, Pu, Am)Zr2 bound irregular polygons ranging in size from a few micrometers to a few tens of micrometers across. The rest of the matrix consists of elongated domains of ζ-(U, Np, Pu, Am) and δ-(U, Np, Pu, Am)Zr2. Each of these domains is a few tens of nanometers across and a few hundred nanometers long. The domains display strong preferred orientations involving areas a few hundred nanometers to a few micrometers across.

  11. Post-Irradiation Examination of 237Np Targets for 238Pu Production

    SciTech Connect (OSTI)

    Morris, Robert Noel [ORNL; Baldwin, Charles A [ORNL; Hobbs, Randy W [ORNL; Schmidlin, Joshua E [ORNL

    2015-01-01

    Oak Ridge National Laboratory is recovering the US 238Pu production capability and the first step in the process has been to evaluate the performance of a 237Np target cermet pellet encased in an aluminum clad. The process proceeded in 3 steps; the first step was to irradiate capsules of single pellets composed of NpO2 and aluminum power to examine their shrinkage and gas release. These pellets were formed by compressing sintered NpO2 and aluminum powder in a die at high pressure followed by sintering in a vacuum furnace. Three temperatures were chosen for sintering the solution precipitated NpO2 power used for pellet fabrication. The second step was to irradiate partial targets composed of 8 pellets in a semi-prototypical arrangement at the two best performing sintering temperatures to determine which temperature gave a pellet that performed the best under the actual planned irradiation conditions. The third step was to irradiate ~50 pellets in an actual target configuration at design irradiation conditions to assess pellet shrinkage and gas release, target heat transfer, and dimensional stability. The higher sintering temperature appeared to offer the best performance after one cycle of irradiation by having the least shrinkage, thus keeping the heat transfer gap between the pellets and clad small minimizing the pellet operating temperature. The final result of the testing was a target that can meet the initial production goals, satisfy the reactor safety requirements, and can be fabricated in production quantities. The current focus of the program is to verify that the target can be remotely dissembled, the pellets dissolved, and the 238Pu recovered. Tests are being conducted to examine these concerns and to compare results to code predictions. Once the performance of the full length targets has been quantified, the pellet 237Np loading will be revisited to determine if it can be increased to increase 238Pu production.

  12. The reduction of Np(VI) and Pu(VI) by organic chelating agents.

    SciTech Connect (OSTI)

    Reed, D.T.; Aase, S.B.; Banaszak, J.E.

    1998-03-19

    The reduction of NpO{sup 2+} and PuO{sub 2}{sup 2+} by oxalate. citrate, and ethylenediaminetetraacetic acid (EDTA) was investigated in low ionic strength media and brines. This was done to help establish the stability of the An(VI) oxidation state in the presence of organic complexants. The stability of the An(VI) oxidation state depended on the pH and relative strength of the various oxidation state-specific complexes. At low ionic strength and pH 6, NpO{sub 2}O{sup 2+} was rapidly reduced to form NpO{sub 2}{sup +} organic complexes. At longer times, Np(IV) organic complexes were observed in the presence of citrate. PuO{sub 2}{sup 2+} was predominantly reduced to Pu{sup 4+}, resulting in the formation of organic complexes or polymeric/hydrolytic precipitates. The relative rates of reduction to the An(V) complex were EDTA > citrate > oxalate. Subsequent reduction to An(IV) complexes, however, occurred in the following order: citrate > EDTA > oxalate because of the stability of the An(V)-EDTA complex. The presence of organic complexants led to the rapid reduction of NpO{sub 2}{sup 2+} and PuO{sub 2}P{sup 2+} in G-seep brine at pHs 5 and 7. At pHs 8 and 10 in ERDA-6 brine, carbonate and hydrolytic complexes predominated and slowed down or prevented the reduction of An(VI) by the organics present.

  13. The QCD/SM Working Group: Summary Report

    SciTech Connect (OSTI)

    M. Dobbs et al.

    2004-08-05

    Among the many physics processes at TeV hadron colliders, we look most eagerly for those that display signs of the Higgs boson or of new physics. We do so however amid an abundance of processes that proceed via Standard Model (SM) and in particular Quantum Chromodynamics (QCD) interactions, and that are interesting in their own right. Good knowledge of these processes is required to help us distinguish the new from the known. Their theoretical and experimental study teaches us at the same time more about QCD/SM dynamics, and thereby enables us to further improve such distinctions. This is important because it is becoming increasingly clear that the success of finding and exploring Higgs boson physics or other New Physics at the Tevatron and LHC will depend significantly on precise understanding of QCD/SM effects for many observables. To improve predictions and deepen the study of QCD/SM signals and backgrounds was therefore the ambition for our QCD/SM working group at this Les Houches workshop. Members of the working group made significant progress towards this on a number of fronts. A variety of tools were further developed, from methods to perform higher order perturbative calculations or various types of resummation, to improvements in the modeling of underlying events and parton showers. Furthermore, various precise studies of important specific processes were conducted. A significant part of the activities in Les Houches revolved around Monte Carlo simulation of collision events. A number of contributions in this report reflect the progress made in this area. At present a large number of Monte Carlo programs exist, each written with a different purpose and employing different techniques. Discussions in Les Houches revealed the need for an accessible primer on Monte Carlo programs, featuring a listing of various codes, each with a short description, but also providing a low-level explanation of the underlying methods. This primer has now been compiled and a

  14. The QCD/SM working group: Summary report

    SciTech Connect (OSTI)

    Dobbs, Matt; Frixione, S.; Laenen, E.; De Roeck, A.; Tollefson, K.; Andersen, J.; Balazs, C.; Banfi, A.; Bernreuther, W.; Binoth, T.; Brandenburg, A.; Buttar, C.; Cao, C-H.; Cruz, A.; Dawson, I.; DelDuca, V.; Drollinger, V.; Dudko, L.; Eynck, T.; Field, R.; Grazzini, M.; Guillet, J.P.; Heinrich, G.; Huston, J.; Kauer, N.; Kidonakis, N.; Kulesza, A.; Lassila-Perini, K.; Magnea, L.; Mahmoudi, F.; Maina, E.; Maltoni, F.; Nolten, M.; Moraes, A.; Moretti, S.; Mrenna, S.; Nagy, Z.; Olness, F.; Puljak, I.; Ross, D.A.; Sabio-Vera, A.; Salam, G.P.; Sherstnev, A.; Si, Z.G.; Sjostrand, T.; Skands, P.; Thome, E.; Trocsanyi, Z.; Uwer, P.; Weinzierl, S.; Yuan, C.P.; Zanderighi,G.; Zanderighi, G.

    2004-04-09

    Among the many physics processes at TeV hadron colliders, we look most eagerly for those that display signs of the Higgs boson or of new physics. We do so however amid an abundance of processes that proceed via Standard Model (SM) and in particular Quantum Chromodynamics (QCD) interactions, and that are interesting in their own right. Good knowledge of these processes is required to help us distinguish the new from the known. Their theoretical and experimental study teaches us at the same time more about QCD/SM dynamics, and thereby enables us to further improve such distinctions. This is important because it is becoming increasingly clear that the success of finding and exploring Higgs boson physics or other New Physics at the Tevatron and LHC will depend significantly on precise understanding of QCD/SM effects for many observables. To improve predictions and deepen the study of QCD/SM signals and backgrounds was therefore the ambition for our QCD/SM working group at this Les Houches workshop. Members of the working group made significant progress towards this on a number of fronts. A variety of tools were further developed, from methods to perform higher order perturbative calculations or various types of resummation, to improvements in the modeling of underlying events and parton showers. Furthermore, various precise studies of important specific processes were conducted. A significant part of the activities in Les Houches revolved around Monte Carlo simulation of collision events. A number of contributions in this report reflect the progress made in this area. At present a large number of Monte Carlo programs exist, each written with a different purpose and employing different techniques. Discussions in Les Houches revealed the need for an accessible primer on Monte Carlo programs, featuring a listing of various codes, each with a short description, but also providing a low-level explanation of the underlying methods. This primer has now been compiled and a

  15. Investigation of crystallization of a mechanically alloyed Sm-Fe alloy

    SciTech Connect (OSTI)

    Lue, M.Q.; Wang, K.Y.; Miao, W.F.; Song, Q.H.; Sun, W.S.; Wei, W.D.; Wang, L.B. )

    1992-06-15

    The crystallization of a mechanically alloyed Sm-Fe alloy was investigated. The results show that the Sm-Fe alloy prepared by mechanical alloying consists of amorphous Sm-Fe phase and crystalline {alpha}-Fe phase. The composition of the alloy is inhomogeneous, i.e., the surface of the as-milled powder is relatively poor in iron. The crystallization process involves the long-range diffusion of iron atoms and solid state reaction. After proper crystallization, the as-milled powder transforms into a Sm{sub 2}Fe{sub 17} phase completely; no distinguishable crystalline {alpha}-Fe phase can be found. A metastable phase, which may be a Sm{sub 2}Fe{sub 17} phase with the structure of hexagonal Th{sub 2}Ni{sub 17} type, appears during the crystallization process.

  16. Development of interatomic potentials appropriate for simulation of devitrification of Al90Sm10 alloy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Mendelev, M. I.; Zhang, F.; Ye, Z.; Sun, Y.; Nguyen, M. C.; Wilson, S. R.; Wang, C. Z.; Ho, K. M.

    2015-04-23

    In this study, a semi-empirical potential for the Al90Sm10 alloy is presented. The potential provides satisfactory reproduction of pure Al properties, the formation energies of a set of Al–Sm crystal phases with Sm content about 10%, and the structure of the liquid Al90Sm10 alloy. During molecular dynamics simulation in which the liquid alloy is cooled at a rate of 1010 K/s, the developed potential produces a glass structure with lower ab initio energy than that produced by ab initio molecular dynamics (AIMD) itself using a typical AIMD cooling rate of 8 ∙1013 K/s. Based on these facts the developed potentialmore » should be suitable for simulations of phase transformations in the Al90Sm10 alloy.« less

  17. Dipole-dipole broadening of Rb ns-np microwave transitions

    SciTech Connect (OSTI)

    Park, Hyunwook; Tanner, P. J.; Claessens, B. J.; Shuman, E. S.; Gallagher, T. F.

    2011-08-15

    The dipole-dipole broadening of ns-np microwave transitions of cold Rb Rydberg atoms in a magneto-optical trap has been recorded for 28{<=}n{<=}51. Since the electric dipole transition matrix elements scale as n{sup 2}, a broadening rate scaling as n{sup 4} is expected and a broadening rate of 8.2x10{sup -15}n{sup 4} MHz cm{sup 3} is observed. The observed broadening is smaller than expected from a classical picture due to the spin-orbit interaction in the np atoms. The broadened resonances are asymmetric and cusp shaped, and their line shapes can be reproduced by a diatomic model which takes into account the dipole-dipole interaction, including the spin-orbit interaction, the strengths of the allowed microwave transitions, and the distribution of the atomic spacings in the trap.

  18. Positron production at extreme light infrastructure – nuclear physics (ELI-NP)

    SciTech Connect (OSTI)

    Oprisa, A. Balascuta, S. Ur, C. A.

    2015-02-24

    Applied and material physics studies with positron beams of Fermi–surfaces, defects, interfaces etc. offer excellent diagnostics tools. At ELI-NP, an intense γ beam of about 10{sup 11} photons/s with energies up to 3.5 MeV will be used to generate a positron beam via pair production in a tungsten converter target. To obtain a high intensity beam of moderated positrons the design of the positron source is of high importance. The design of a dedicated positron source at ELI–NP is being investigated based on extensive GEANT4 simulations. The goal of the simulations is to optimize the geometry of the target and the gamma beam collimation. We present here the characteristics of the positron beam obtained for different geometries of the converter target.

  19. Implementation status of the extreme light infrastructure - nuclear physics (ELI-NP) project

    SciTech Connect (OSTI)

    Gales, S. Zamfir, N. V.

    2015-02-24

    The Project Extreme Light Infrastructure (ELI) is part of the European Strategic Forum for Research Infrastructures (ESFRI) Roadmap. ELI will be built as a network of three complementary pillars at the frontier of laser technologies. The ELI-NP pillar (NP for Nuclear Physics) is under construction near Bucharest (Romania) and will develop a scientific program using two 10 PW lasers and a Compton back-scattering high-brilliance and intense gamma beam, a marriage of laser and accelerator technology at the frontier of knowledge. In the present paper, the technical description of the facility, the present status of the project as well as the science, applications and future perspectives will be discussed.

  20. MOX and MOX with 237Np/241Am Inert Fission Gas Generation Comparison in ATR

    SciTech Connect (OSTI)

    G. S. Chang; M. Robel; W. J. Carmack; D. J. Utterbeck

    2006-06-01

    The treatment of spent fuel produced in nuclear power generation is one of the most important issues to both the nuclear community and the general public. One of the viable options to long-term geological disposal of spent fuel is to extract plutonium, minor actinides (MA), and potentially long-lived fission products from the spent fuel and transmute them into short-lived or stable radionuclides in currently operating light-water reactors (LWR), thus reducing the radiological toxicity of the nuclear waste stream. One of the challenges is to demonstrate that the burnup-dependent characteristic differences between Reactor-Grade Mixed Oxide (RG-MOX) fuel and RG-MOX fuel with MA Np-237 and Am 241 are minimal, particularly, the inert gas generation rate, such that the commercial MOX fuel experience base is applicable. Under the Advanced Fuel Cycle Initiative (AFCI), developmental fuel specimens in experimental assembly LWR-2 are being tested in the northwest (NW) I-24 irradiation position of the Advanced Test Reactor (ATR). The experiment uses MOX fuel test hardware, and contains capsules with MOX fuel consisting of mixed oxide manufactured fuel using reactor grade plutonium (RG-Pu) and mixed oxide manufactured fuel using RG-Pu with added Np/Am. This study will compare the fuel neutronics depletion characteristics of Case-1 RG-MOX and Case-2 RG-MOX with Np/Am.

  1. Post-Irradiation Examination of 237Np Targets for 238Pu Production

    SciTech Connect (OSTI)

    Morris, Robert Noel; Baldwin, Charles A; Hobbs, Randy W; Schmidlin, Joshua E

    2015-01-01

    Oak Ridge National Laboratory is recovering the US 238Pu production capability and the first step in the process has been to evaluate the performance of a 237Np target cermet pellet encased in an aluminum clad. The process proceeded in 3 steps; the first step was to irradiate capsules of single pellets composed of NpO2 and aluminum power to examine their shrinkage and gas release. These pellets were formed by compressing sintered NpO2 and aluminum powder in a die at high pressure followed by sintering in a vacuum furnace. Three temperatures were chosen for sintering the solution precipitated NpO2 power used for pellet fabrication. The second step was to irradiate partial targets composed of 8 pellets in a semi-prototypical arrangement at the two best performing sintering temperatures to determine which temperature gave a pellet that performed the best under the actual planned irradiation conditions. The third step was to irradiate ~50 pellets in an actual target configuration at design irradiation conditions to assess pellet shrinkage and gas release, target heat transfer, and dimensional stability. The higher sintering temperature appeared to offer the best performance after one cycle of irradiation by having the least shrinkage, thus keeping the heat transfer gap between the pellets and clad small minimizing the pellet operating temperature. The final result of the testing was a target that can meet the initial production goals, satisfy the reactor safety requirements, and can be fabricated in production quantities. The current focus of the program is to verify that the target can be remotely dissembled, the pellets dissolved, and the 238Pu recovered. Tests are being conducted to examine these concerns and to compare results to code predictions. Once the performance of the full length targets has been quantified, the pellet 237Np loading will be revisited to determine if it can be

  2. Characterization of the Kinetics of NF3-Fluorination of NpO2

    SciTech Connect (OSTI)

    Casella, Andrew M.; Scheele, Randall D.; McNamara, Bruce K.

    2015-12-23

    The exploitation of selected actinide and fission product fluoride volatilities has long been considered as a potentially attractive compact method for recycling used nuclear fuels to avoid generating the large volumes of radioactive waste arising from aqueous reprocessing [1-7]. The most developed process uses the aggressive and hazardous fluorinating agents hydrogen fluoride (HF) and/or molecular fluorine (F2) at high temperatures to volatilize the greatest fraction of the used nuclear fuel into a single gas stream. The volatilized fluorides are subsequently separated using a series of fractionation and condensation columns to recover the valuable fuel constituents and fission products. In pursuit of a safer and less complicated approach, we investigated an alternative fluoride volatility-based process using the less hazardous fluorinating agent nitrogen trifluoride (NF3) and leveraging its less aggressive nature to selectively evolve fission product and actinide fluorides from the solid phase based on their reaction temperatures into a single recycle stream [8-15]. In this approach, successive isothermal treatments using NF3 will first evolve the more thermally susceptible used nuclear fuel constituents leaving the other constituents in the residual solids until subsequent isothermal temperature treatments cause these others to volatilize. During investigation of this process, individual neat used fuel components were treated with isothermal NF3 in an attempt to characterize the kinetics of each fluorination reaction to provide input into the design of a new volatile fluoride separations approach. In these directed investigations, complex behavior was observed between NF3 and certain solid reactants such as the actinide oxides of uranium, plutonium, and neptunium. Given the similar thermal reaction susceptibilities of neptunium oxide (NpO2) and uranium dioxide (UO2) and the importance of Np and U, we initially focused our efforts on determining the reaction

  3. Kinetic studies of the [NpO? (CO?)?]?? ion at alkaline conditions using C NMR

    SciTech Connect (OSTI)

    Panasci, Adele F.; Harley, Stephen J.; Zavarin, Mavrik; Casey, William H.

    2014-04-21

    Carbonate ligand-exchange rates on the [NpO? (CO?)?]?? ion were determined using a saturation-transfer C nuclear magnetic resonance (NMR) pulse sequence in the pH range of 8.1 ? pH ? 10.5. Over the pH range 9.3 ? pH ? 10.5, which compares most directly with previous work of Stout et al.,1 we find an average rate, activation energy, enthalpy, and entropy of k298ex = 40.6(4.3) s?, Ea =45.1(3.8) kJ mol?, ?H = 42.6(3.8) kJ mol?, and ?S = -72(13) J mol? K?, respectively. These activation parameters are similar to the Stout et al. results at pH 9.4. However, their room-temperature rate at pH 9.4, k298ex = 143(1.0) s?, is ~3 times faster than what we experimentally determined at pH 9.3: k298ex = 45.4(5.3) s?. Our rates for [NpO? (CO?)?]?? are also faster by a factor of ~3 relative to the isoelectronic [UO?(CO?)?]?? as reported by Brucher et al.2 of k298ex = 13(3) s?. Consistent with results for the [UO?(CO?)?]?? ion, we find evidence for a proton-enhanced pathway for carbonate exchange for the [NpO?(CO?)?]?? ion at pH < 9.0.

  4. AREVA NP Cr{sub 2}O{sub 3}-doped fuel development for BWRs

    SciTech Connect (OSTI)

    Delafoy, C.; Dewes, P.; Miles, T.

    2007-07-01

    The search for improvements in nuclear fuel cycle economics results in increasing demands for fuel discharged burnup and reliability, plant maneuverability and power up-rating. To achieve these objectives without any reduction of safety margins, fuel design and materials that enable enhanced performance capabilities have been developed or are under investigations. Research on fuel pellets focuses on the modification of the microstructure to increase fission product retention and pellet mechanical compliance. Currently, production of the desired large grain viscoplastic UO{sub 2} fuel microstructures has been extensively investigated by AREVA NP through the use of doping elements. This track is nowadays a worldwide working field. In this area, AREVA NP has launched the development of a new UO{sub 2} fuel pellet obtained by optimum chromium oxide doping. The purpose of this paper is first to present the current results with the AREVA NP optimized chromia doped fuel and to discuss the key advantages in terms of fuel performance for BWR applications. In particular, the development relies on ramp testing results, fuel temperature and fission gas release values acquired at high burnup and high power levels. Second, the paper focuses on the qualification process implemented by AREVA NP to assess the margins of the optimized Cr{sub 2}O{sub 3}-doped UO{sub 2} fuel towards safety criteria at high burnup and the risk of PCI failure, as well as to develop calculation tools to support design. The driving force in this qualification plan is to gain the accurate knowledge of the optimized doped fuel behavior under normal, transient and anticipated accident conditions. To support this effort, irradiation campaigns are under progress in PWR and BWR plants to cover a wide range of existing operating conditions and to anticipate future demands. Considering only the BWR part, the program has successfully run since 2005 and is designed to obtain data up to high burnup, at least 70 GWd

  5. RAPID SEPARATION METHOD FOR 237NP AND PU ISOTOPES IN LARGE SOIL SAMPLES

    SciTech Connect (OSTI)

    Maxwell, S.; Culligan, B.; Noyes, G.

    2010-07-26

    A new rapid method for the determination of {sup 237}Np and Pu isotopes in soil and sediment samples has been developed at the Savannah River Site Environmental Lab (Aiken, SC, USA) that can be used for large soil samples. The new soil method utilizes an acid leaching method, iron/titanium hydroxide precipitation, a lanthanum fluoride soil matrix removal step, and a rapid column separation process with TEVA Resin. The large soil matrix is removed easily and rapidly using this two simple precipitations with high chemical recoveries and effective removal of interferences. Vacuum box technology and rapid flow rates are used to reduce analytical time.

  6. NMR relaxation in the topological Kondo insulator SmB 6 (Journal...

    Office of Scientific and Technical Information (OSTI)

    Title: NMR relaxation in the topological Kondo insulator SmB 6 Authors: Schlottmann, P. Publication Date: 2014-10-21 OSTI Identifier: 1181567 GrantContract Number: FG02-98ER45707 ...

  7. Natural SM-like 126 GeV Higgs boson via nondecoupling D terms

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Bertuzzo, Enrico; Frugiuele, Claudia

    2016-02-16

    Accommodating both a 126 GeV mass and standard model (SM)-like couplings for the Higgs has a fine-tuning price in supersymmetric models. Examples are the minimal supersymmetric standard model, in which SM-like couplings are natural, but raising the Higgs mass to 126 GeV requires a considerable tuning, and the nonminimal supersymmetric standard model, in which the situation is reversed: the Higgs is naturally heavier, but being SM-like requires some tuning. Finally, we show that models with nondecoupling D terms alleviate this tension—a 126 GeV SM-like Higgs comes out basically with no fine-tuning cost. In addition, the analysis of the fine-tuning of the extended gaugemore » sector shows that naturalness requires the heavy gauge bosons to likely be within the reach of LHC run II.« less

  8. Perspectives for neutron and gamma spectroscopy in high power laser driven experiments at ELI-NP

    SciTech Connect (OSTI)

    Negoita, F. Gugiu, M. Petrascu, H. Petrone, C. Pietreanu, D.; Fuchs, J.; Chen, S.; Higginson, D.; Vassura, L.; Hannachi, F.; Tarisien, M.; Versteegen, M.; Antici, P.; Balabanski, D.; Balascuta, S.; Cernaianu, M.; Dancus, I.; Gales, S.; Neagu, L.; Petcu, C.; and others

    2015-02-24

    The measurement of energy spectra of neutrons and gamma rays emitted by nuclei, together with charge particles spectroscopy, are the main tools for understanding nuclear phenomena occurring also in high power laser driven experiments. However, the large number of particles emitted in a very short time, in particular the strong X-rays flash produced in laser-target interaction, impose adaptation of technique currently used in nuclear physics experiment at accelerator based facilities. These aspects are discussed (Section 1) in the context of proposed studies at high power laser system of ELI-NP. Preliminary results from two experiments performed at Titan (LLNL) and ELFIE (LULI) facilities using plastic scintillators for neutron detection (Section 2) and LaBr{sub 3}(Ce) scintillators for gamma detection (Section 3) are presented demonstrating the capabilities and the limitations of the employed methods. Possible improvements of these spectroscopic methods and their proposed implementation at ELI-NP will be discussed as well in the last section.

  9. Strong field physics and QED experiments with ELI-NP 2×10PW laser beams

    SciTech Connect (OSTI)

    Turcu, I. C. E. Balascuta, S. Negoita, F.; Jaroszynski, D.; McKenna, P.

    2015-02-24

    The ELI-NP facility will focus a 10 PW pulsed laser beam at intensities of ∼10{sup 23} W/cm{sup 2} for the first time, enabling investigation of the new physical phenomena at the interfaces of plasma, nuclear and particle physics. The electric field in the laser focus has a maximum value of ∼10{sup 15} V/m at such laser intensities. In the ELI-NP Experimental Area E6, we propose the study of Radiation Reaction, Strong Field Quantum Electrodynamics (QED) effects and resulting production of Ultra-bright Sources of Gamma-rays which could be used for nuclear activation. Two powerful, synchronized 10 PW laser beams will be focused in the E6 Interaction Chamber on either gas or solid targets. One 10 PW beam is the Pump-beam and the other is the Probe-beam. The focused Pump beam accelerates the electrons to relativistic energies. The accelerated electron bunches interact with the very high electro-magnetic field of the focused Probe beam. The layout of the experimental area E6 will be presented with several options for the experimental configurations.

  10. Covariant Spectator Theory of np scattering: Deuteron magnetic moment and form factors

    SciTech Connect (OSTI)

    Gross, Franz L.

    2014-06-01

    The deuteron magnetic moment is calculated using two model wave functions obtained from 2007 high precision fits to $np$ scattering data. Included in the calculation are a new class of isoscalar $np$ interaction currents which are automatically generated by the nuclear force model used in these fits. After normalizing the wave functions, nearly identical predictions are obtained: model WJC-1, with larger relativistic P-state components, gives 0.863(2), while model WJC-2 with very small $P$-state components gives 0.864(2) These are about 1\\% larger than the measured value of the moment, 0.857 n.m., giving a new prediction for the size of the $\\rho\\pi\\gamma$ exchange, and other purely transverse interaction currents that are largely unconstrained by the nuclear dynamics. The physical significance of these results is discussed, and general formulae for the deuteron form factors, expressed in terms of deuteron wave functions and a new class of interaction current wave functions, are given.

  11. The QCD/SM working group: Summary report

    SciTech Connect (OSTI)

    W. Giele et al.

    2004-01-12

    Quantum Chromo-Dynamics (QCD), and more generally the physics of the Standard Model (SM), enter in many ways in high energy processes at TeV Colliders, and especially in hadron colliders (the Tevatron at Fermilab and the forthcoming LHC at CERN), First of all, at hadron colliders, QCD controls the parton luminosity, which rules the production rates of any particle or system with large invariant mass and/or large transverse momentum. Accurate predictions for any signal of possible ''New Physics'' sought at hadron colliders, as well as the corresponding backgrounds, require an improvement in the control of uncertainties on the determination of PDF and of the propagation of these uncertainties in the predictions. Furthermore, to fully exploit these new types of PDF with uncertainties, uniform tools (computer interfaces, standardization of the PDF evolution codes used by the various groups fitting PDF's) need to be proposed and developed. The dynamics of colour also affects, both in normalization and shape, various observables of the signals of any possible ''New Physics'' sought at the TeV scale, such as, e.g. the production rate, or the distributions in transverse momentum of the Higgs boson. Last, but not least, QCD governs many backgrounds to the searches for this ''New Physics''. Large and important QCD corrections may come from extra hard parton emission (and the corresponding virtual corrections), involving multi-leg and/or multi-loop amplitudes. This requires complex higher order calculations, and new methods have to be designed to compute the required multi-legs and/or multi-loop corrections in a tractable form. In the case of semi-inclusive observables, logarithmically enhanced contributions coming from multiple soft and collinear gluon emission require sophisticated QCD resummation techniques. Resummation is a catch-all name for efforts to extend the predictive power of QCD by summing the large logarithmic corrections to all orders in perturbation theory. In

  12. DETERMINATION OF 237NP AND PU ISOTOPES IN LARGE SOIL SAMPLES BY INDUCTIVELY COUPLED PLASMA MASS SPECTROMETRY

    SciTech Connect (OSTI)

    Maxwell, S.

    2010-07-26

    A new method for the determination of {sup 237}Np and Pu isotopes in large soil samples has been developed that provides enhanced uranium removal to facilitate assay by inductively coupled plasma mass spectrometry (ICP-MS). This method allows rapid preconcentration and separation of plutonium and neptunium in large soil samples for the measurement of {sup 237}Np and Pu isotopes by ICP-MS. {sup 238}U can interfere with {sup 239}Pu measurement by ICP-MS as {sup 238}UH{sup +} mass overlap and {sup 237}Np via {sup 238}U peak tailing. The method provides enhanced removal of uranium by separating Pu and Np initially on TEVA Resin, then transferring Pu to DGA resin for additional purification. The decontamination factor for removal of uranium from plutonium for this method is greater than 1 x 10{sup 6}. Alpha spectrometry can also be applied so that the shorter-lived {sup 238}Pu isotope can be measured successfully. {sup 239}Pu, {sup 242}Pu and {sup 237}Np were measured by ICP-MS, while {sup 236}Pu and {sup 238}Pu were measured by alpha spectrometry.

  13. RAPID DETERMINATION OF 237 NP AND PU ISOTOPES IN WATER BY INDUCTIVELY COUPLED PLASMA MASS SPECTROMETRY AND ALPHA SPECTROMETRY

    SciTech Connect (OSTI)

    Maxwell, S.; Jones, V.; Culligan, B.; Nichols, S.; Noyes, G.

    2010-06-23

    A new method that allows rapid preconcentration and separation of plutonium and neptunium in water samples was developed for the measurement of {sup 237}Np and Pu isotopes by inductively-coupled plasma mass spectrometry (ICP-MS) and alpha spectrometry; a hybrid approach. {sup 238}U can interfere with {sup 239}Pu measurement by ICP-MS as {sup 238}UH{sup +} mass overlap and {sup 237}Np via peak tailing. The method provide enhanced removal of uranium by separating Pu and Np initially on TEVA Resin, then moving Pu to DGA resin for additional removal of uranium. The decontamination factor for uranium from Pu is almost 100,000 and the decontamination factor for U from Np is greater than 10,000. This method uses stacked extraction chromatography cartridges and vacuum box technology to facilitate rapid separations. Preconcentration is performed using a streamlined calcium phosphate precipitation method. Purified solutions are split between ICP-MS and alpha spectrometry so that long and short-lived Pu isotopes can be measured successfully. The method allows for simultaneous extraction of 20 samples (including QC samples) in 4 to 6 hours, and can also be used for emergency response. {sup 239}Pu, {sup 242}Pu and {sup 237}Np were measured by ICP-MS, while {sup 236}Pu, {sup 238}Pu, and {sup 239}Pu were measured by alpha spectrometry.

  14. Preparation and structure characterization of SmCo{sub 5}(0001) epitaxial thin films grown on Cu(111) underlayers

    SciTech Connect (OSTI)

    Ohtake, Mitsuru; Nukaga, Yuri; Futamoto, Masaaki; Kirino, Fumiyoshi

    2009-04-01

    SmCo{sub 5}(0001) epitaxial films were prepared on Cu(111) single-crystal underlayers formed on Al{sub 2}O{sub 3}(0001) substrates at 500 deg. C. The nucleation and growth mechanism of (0001)-oriented SmCo{sub 5} crystal on Cu(111) underlayer is investigated and a method to control the nucleation is proposed. The SmCo{sub 5} epitaxial thin film formed directly on Cu underlayer consists of two types of domains whose orientations are rotated around the film normal by 30 deg. each other. By introducing a thin Co seed layer on the Cu underlayer, a SmCo{sub 5}(0001) single-crystal thin film is successfully obtained. Nucleation of SmCo{sub 5} crystal on Cu underlayer seems controllable by varying the interaction between the Cu underlayer and the SmCo{sub 5} layer.

  15. Raman spectroscopy of GaP/GaNP core/shell nanowires

    SciTech Connect (OSTI)

    Dobrovolsky, A.; Chen, W. M.; Buyanova, I. A.; Sukrittanon, S.; Kuang, Y. J.; Tu, C. W.

    2014-11-10

    Raman spectroscopy is employed to characterize structural and phonon properties of GaP/GaNP core/shell nanowires (NWs) grown by molecular beam epitaxy on Si substrates. According to polarization-dependent measurements performed on single NWs, the dominant Raman modes associated with zone-center optical phonons obey selection rules in a zinc-blende lattice, confirming high crystalline quality of the NWs. Two additional modes at 360 and 397 cm{sup −1} that are specific to the NW architecture are also detected in resonant Raman spectra and are attributed to defect-activated scattering involving zone-edge transverse optical phonons and surface optical phonons, respectively. It is concluded that the formation of the involved defect states are mainly promoted during the NW growth with a high V/III ratio.

  16. A conceptual design of an electron spectrometer for ELI-NP

    SciTech Connect (OSTI)

    Balascuta, S. Turcu, I. C. E.

    2015-02-24

    We present the geometry and field parameters of an Electron Spectrometer (ES) with two dipole magnets, considered for electron energy measurements at the High Fields QED experimental area at ELI-NP. The first magnet is a 2 meter long permanent magnet, placed inside the Interaction Chamber (IC). The second magnet is a 1.5 meters long electromagnet, placed outside IC. The pulsed electron beam will be produced by the 10 PW pulsed Laser, ‘pump-beam’, focused into one meter long capillary low density plasma cell. A second 10 PW pulsed Laser, ‘probe-beam’, will interact with the relativistic electron bunch providing the strong electromagnetic field. The ES will measure the subtle changes in the electron energy spectrum as a result of the electron beam interaction with the probe-beam field.

  17. Radon emanation from giant landslides of Koefels (Tyrol, Austria) and Langtang Himal (Nepal)

    SciTech Connect (OSTI)

    Purtscheller, F.; Pirchl, T.; Sieder, G.

    1995-07-01

    The identification of extremely high indoor radon concentrations in the village Umhausen (Tyrol, Austria) initiated a scientific program to get information about the source and distribution of this noble gas. The high concentrations can not be related to U anomalies or large-scale fault zones. The nearby giant landslide of Koefels, with its highly fractured and crushed orthogneisses, are the only possible source of radon, despite the fact that the U and Ra content of the rocks is by no means exceptional. The reasons for the high emanation rates from the landslide are discussed and compared to results gained from a similar examination of the giant landslide of Langtang Himal (Nepal). The exceptional geologic situation in both cases, as well as the spatial distribution of different concentration levels, indicate that both landslides must be considered as the production sites of radon. Independent of the U and Ra contents of the rocks, the most important factors producing high emanation rates are the production of a high active surface area in circulation pathways for Rn-enriched soil air by brittle deformation due to the impact of the landslidemass. 37 refs., 4 figs., 1 tab.

  18. Impact of low-dose electron irradiation on $$n^{+}p$$ silicon strip sensors

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Adam, W.

    2015-08-28

    The response of n+p silicon strip sensors to electrons from a 90Sr source was measured using a multi-channel read-out system with 25 ns sampling time. The measurements were performed over a period of several weeks, during which the operating conditions were varied. The sensors were fabricated by Hamamatsu Photonics on 200 μm thick float-zone and magnetic-Czochralski silicon. Their pitch was 80 μm, and both p-stop and p-spray isolation of the n+ strips were studied. The electrons from the 90Sr source were collimated to a spot with a full-width-at-half-maximum of 2 mm at the sensor surface, and the dose rate inmore » the SiO2 at the maximum was about 50 Gy(SiO2)/d. After only a few hours of making measurements, significant changes in charge collection and charge sharing were observed. Annealing studies, with temperatures up to 80 °C and annealing times of 18 h showed that the changes can only be partially annealed. The observations can be qualitatively explained by the increase of the positive oxide-charge density due to the ionization of the SiO2 by the radiation from the β source. TCAD simulations of the electric field in the sensor for different oxide-charge densities and different boundary conditions at the sensor surface support this explanation. As a result, the relevance of the measurements for the design of n+p strip sensors is discussed.« less

  19. Local structure in solid solutions of stabilised zirconia with actinide dioxides (UO{sub 2}, NpO{sub 2})

    SciTech Connect (OSTI)

    Walter, Marcus; Somers, Joseph; Bouexiere, Daniel; Rothe, Joerg

    2011-04-15

    The local structure of (Zr,Lu,U)O{sub 2-x} and (Zr,Y,Np)O{sub 2-x} solid solutions has been investigated by extended X-ray absorption fine structure (EXAFS). Samples were prepared by mixing reactive (Zr,Lu)O{sub 2-x} and (Zr,Y)O{sub 2-x} precursor materials with the actinide oxide powders, respectively. Sintering at 1600 {sup o}C in Ar/H{sub 2} yields a fluorite structure with U(IV) and Np(IV). As typical for stabilised zirconia the metal-oxygen and metal-metal distances are characteristic for the different metal ions. The bond lengths increase with actinide concentration, whereas highest adaptation to the bulk stabilised zirconia structure was observed for U---O and Np---O bonds. The Zr---O bond shows only a slight increase from 2.14 A at 6 mol% actinide to 2.18 A at infinite dilution in UO{sub 2} and NpO{sub 2}. The short interatomic distance between Zr and the surrounding oxygen and metal atoms indicate a low relaxation of Zr with respect to the bulk structure, i.e. a strong Pauling behaviour. -- Graphical abstract: Metal-oxygen bond distances in (Zr,Lu,U)O{sub 2-x} solid solutions with different oxygen vacancy concentrations (Lu/Zr=1 and Lu/Zr=0.5). Display Omitted Research Highlights: {yields} EXAFS indicates high U and Np adaption to the bulk structure of stabilised zirconia. {yields} Zr---O bond length is 2.18 A at infinite Zr dilution in UO{sub 2} and NpO{sub 2}. {yields} Low relaxation (strong Pauling behaviour) of Zr explains its low solubility in UO{sub 2}.

  20. Effect of oxidation state and ionic strength on sorption of actinides (Th, U, Np, Am) to geologic media

    SciTech Connect (OSTI)

    Dittrich, Timothy M.; Richmann, Michael K.; Reed, Donald T.

    2015-10-30

    The degree of conservatism in the estimated sorption partition coefficients (Kds) used in a performance assessment model is being evaluated based on a complementary batch and column method. The main focus of this work is to investigate the role of ionic strength, solution chemistry, and oxidation state (III-VI) in actinide sorption to dolomite rock. Based on redox conditions and solution chemistry expected at the WIPP, possible actinide species include Pu(III), Pu(IV), U(IV), U(VI), Np(IV), Np(V), Am(III), and Th(IV).

  1. Magnetic properties and Fermi surface of antiferromagnetic SmCu sub 6

    SciTech Connect (OSTI)

    Onuki, Y.; Umezawa, A.; Kwok, W.K.; Crabtree, G.W. ); Nishihara, M.; Ina, K.; Yamazaki, T.; Omi, T.; Komatsubara, T. ); Maezawa, K.; Wakabayashi, S. ); Takayanagi, S. ); Wada, N. )

    1990-01-01

    We report measurements of the magnetic susceptibility, specific heat, magnetoresistance, Hall effect, and Fermi surface in SmCu{sub 6}. The susceptibility follows the Van Vleck form for Sm{sup 3+} near room temperature and shows two antiferromagnetic phase transitions at 9.6 and 5.2 K. The specific heat implies a quartet ground state for the crystal-field-split {ital J}=5/2 angular momentum state. Magnetoresistance indicates that SmCu{sub 6} contains both electron and hole carriers but is uncompensated. de Haas--van Alphen measurements show that the Fermi surface in the antiferromagnetic state consists of a network of cylinders oriented 30{degree} from the {ital b} and {ital c} axes.

  2. QuickSite{sup SM}, the Argonne expedited site characterization methodology,

    SciTech Connect (OSTI)

    Burton, J.C.; Meyer, W.T.

    1997-09-01

    Expedited site characterization (ESC), developed by Argonne National Laboratory, is an interactive, integrated process emphasizing the use of existing data of sufficient quality, multiple complementary characterization methods, and on-site decision making to optimize site investigations. The Argonne ESC is the basis for the provisional ESC standard of the ASTM (American Society for Testing and Materials). QuickSite{sup SM} is the implementation package developed by Argonne to facilitate ESC of sites contaminated with hazardous wastes. At various sites, Argonne has successfully implemented QuickSite{sup SM} and demonstrated the technical superiority of the ESC process over traditional methodologies guided by statistics and random-sampling approaches. For example, in a QuickSite{sup SM} characterization of a perched aquifer at the Pantex Plant in Texas, past data and geochemical analyses of existing wells were used to develop a model for recharge and contaminant movement. With the model as a guide, closure was achieved with minimal field work.

  3. Report on Lessons Learned from the NP 2010 Early Site Permit Program FINAL REPORT

    SciTech Connect (OSTI)

    2008-03-26

    This report provides a summary of lessons learned from the demonstration of the licensing process for three Early Site Permit (ESP) applications supported as part of the Department of Energy’s (DOE) Nuclear Power 2010 (NP 2010) program. The ESP process was established by the Nuclear Regulatory Commission (NRC) to enable completion of the site evaluation component of nuclear power plant licensing under 10 CFR Part 52 before a utility makes a decision to build a plant. Early Site Permits are valid for 10 to 20 years and can be renewed for an additional 10 to 20 years. NRC review of an ESP application addresses site safety issues, environmental protection issues, and plans for coping with emergencies. Successful completion of the ESP process will establish that a site is suitable for possible future construction and operation of a nuclear power plant. Most importantly, an ESP resolves significant site-related safety and environmental issues early in the decision process and helps achieve acceptance by the public. DOE competitively selected Dominion Nuclear Energy North Anna, LLC (Dominion); System Energy Resources, Inc. (an Entergy subsidiary); and Exelon Generation Company, LLC (Exelon) in 2002 to demonstrate the ESP process and provided cost-shared support through the NP 2010 program. Dominion pursued an ESP for the North Anna site in Virginia; System Energy Resources, Inc. pursued an ESP for the Grand Gulf site in Mississippi; and Exelon pursued an ESP for the Clinton site in Illinois. After successfully demonstrating the process, the NRC issued an ESP for Clinton on March 17, 2007; Grand Gulf on April 5, 2007; and North Anna on November 27, 2007. As with all successful projects, there are lessons to be learned from the NP 2010 early site permitting demonstration that can help improve future implementation guidance documents and regulatory review standards. In general, these lessons pertain to the effectiveness of the regulatory process, experience related to

  4. Structural, morphological and optical investigations on Sm{sup 3+} doped gadolinium oxide nanorods

    SciTech Connect (OSTI)

    Boopathi, G.; Mohan, R.; Raj, S. Gokul; Kumar, G. Ramesh

    2014-04-24

    One dimensional uniform Sm{sup 3+} doped gadolinium hydroxide nanorods have been prepared via simple co– precipitation technique at 60 °C temperature for 1 hour. The samples were calcinated at 750 °C to obtain Sm{sup 3+} doped gadolinium oxide nanorods. The 1D nanorods were then subjected to different characterization techniques to ascertain its structural stability and its morphology were investigated using high–resolution transmission electron microscopy. Photoluminescence (PL) spectrophotometry was investigated and the obtained results were discussed in detail.

  5. Discovery of a metastable Al20Sm4 phase

    SciTech Connect (OSTI)

    Ye, Z.; Zhang, F.; Sun, Y.; Mendelev, M. I.; Ott, R. T.; Park, E.; Besser, M. F.; Kramer, M. J.; Ding, Z.; Wang, C. -Z.; Ho, K. -M.

    2015-03-09

    In this study, we present an efficient genetic algorithm, integrated with experimental diffraction data, to solve a nanoscale metastable Al20Sm4 phase that evolves during crystallization of an amorphous magnetron sputtered Al90Sm10 alloy. The excellent match between calculated and experimental X-ray diffraction patterns confirms an accurate description of this metastable phase. Molecular dynamic simulations of crystal growth from the liquid phase predict the formation of disordered defects in the devitrified crystal.

  6. On the Chemistry and Physical Properties of Flux and Floating Zone Grown SmB6 Single Crystals

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Phelan, W. A.; Koohpayeh, S. M.; Cottingham, P.; Tutmaher, J. A.; Leiner, J. C.; Lumsden, M. D.; Lavelle, C. M.; Wang, X. P.; Hoffmann, C.; Siegler, M. A.; et al

    2016-02-19

    Recent theoretical and experimental findings suggest the long-known but not well understood low temperature resistance plateau of SmB6 may originate from protected surface states arising from a topologically non-trivial bulk band structure having strong Kondo hybridization. Yet others have ascribed this feature to impurities, vacancies, and surface reconstructions. Given the typical methods used to prepare SmB6 single crystals, flux and floating-zone procedures, such ascriptions should not be taken lightly. We demonstrate how compositional variations and/or observable amounts of impurities in SmB6 crystals grown using both procedures affect the physical properties. From X-ray diffraction, neutron diffraction, and X-ray computed tomography experimentsmore » we observe that natural isotope containing (SmB6) and doubly isotope enriched (154Sm11B6) crystals prepared using aluminum flux contain co-crystallized, epitaxial aluminum. Further, a large, nearly stoichiometric crystal of SmB6 was successfully grown using the float-zone technique; upon continuing the zone melting, samarium vacancies were introduced. These samarium vacancies drastically alter the resistance and plateauing magnitude of the low temperature resistance compared to stoichiometric SmB6. Finally, these results highlight that impurities and compositional variations, even at low concentrations, must be considered when collecting/analyzing physical property data of SmB6. Finally, a more accurate samarium-154 coherent neutron scattering length, 8.9(1) fm, is reported.« less

  7. Preparation and characterization of SiO?:Sm? nanotube arrays with 1.06 ?m laser antireflective property

    SciTech Connect (OSTI)

    Tan, Wei-min; Huang, Ning; Wang, Li-jun; Song, Tian-shun; Lu, Chun-hua; Wang, Liu-fang; Zhang, Jun-zhi

    2013-05-01

    SiO?: Sm? nanotube arrays with excellent antireflective property at 1.06 ?m were synthesized by a template-assisted solgel process. The molecular structure, morphology and optical properties of the fabricated SiO?:Sm? nanotube arrays were investigated by a Fourier transform infrared spectroscope (FTIR), a Scanning electron microscope (SEM), and a spectro-fluorometer, respectively. The experimental results demonstrate that the SiO?:Sm? nanotube arrays were formed via the AAO membrane during the solgel process. The remarkable antireflective characteristic of about 0.166% at 1.06 ?m was attributed to the drastic decrease of effective refraction index which enhances the matching effect between air and substrate. As well as the absorption performance of Sm? at 1.06 ?m which consumes the energies of incident light. - Graphical abstract: Directional aligned SiO?:Sm? nanotube arrays were synthesized in AAO template by solgel process, and the antiflective performance of arrays is prominent comparing to the blank AAO template. Highlights: SiO?:Sm? nanotube arrays are synthesized by a template-assisted solgel process. SiO?:Sm? nanotube arrays have remarkable antireflective properties at 1.06 ?m. The subwavelength structure results in a decrease of effective refraction index. The absorption performance of Sm? at 1.06 ?m consume the energies of incident light.

  8. Rapid fusion method for the determination of Pu, Np, and Am in large soil samples

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Maxwell, Sherrod L.; Culligan, Brian; Hutchison, Jay B.; McAlister, Daniel R.

    2015-02-14

    A new rapid sodium hydroxide fusion method for the preparation of 10-20 g soil samples has been developed by the Savannah River National Laboratory (SRNL). The method enables lower detection limits for plutonium, neptunium, and americium in environmental soil samples. The method also significantly reduces sample processing time and acid fume generation compared to traditional soil digestion techniques using hydrofluoric acid. Ten gram soil aliquots can be ashed and fused using the new method in 1-2 hours, completely dissolving samples, including refractory particles. Pu, Np and Am are separated using stacked 2mL cartridges of TEVA and DGA Resin and measuredmore » using alpha spectrometry. The method can be adapted for measurement by inductively-coupled plasma mass spectrometry (ICP-MS). Two 10 g soil aliquots of fused soil may be combined prior to chromatographic separations to further improve detection limits. Total sample preparation time, including chromatographic separations and alpha spectrometry source preparation, is less than 8 hours.« less

  9. Rapid fusion method for the determination of Pu, Np, and Am in large soil samples

    SciTech Connect (OSTI)

    Maxwell, Sherrod L.; Culligan, Brian; Hutchison, Jay B.; McAlister, Daniel R.

    2015-02-14

    A new rapid sodium hydroxide fusion method for the preparation of 10-20 g soil samples has been developed by the Savannah River National Laboratory (SRNL). The method enables lower detection limits for plutonium, neptunium, and americium in environmental soil samples. The method also significantly reduces sample processing time and acid fume generation compared to traditional soil digestion techniques using hydrofluoric acid. Ten gram soil aliquots can be ashed and fused using the new method in 1-2 hours, completely dissolving samples, including refractory particles. Pu, Np and Am are separated using stacked 2mL cartridges of TEVA and DGA Resin and measured using alpha spectrometry. The method can be adapted for measurement by inductively-coupled plasma mass spectrometry (ICP-MS). Two 10 g soil aliquots of fused soil may be combined prior to chromatographic separations to further improve detection limits. Total sample preparation time, including chromatographic separations and alpha spectrometry source preparation, is less than 8 hours.

  10. Neutrino-4 experiment on the search for a sterile neutrino at the SM-3 reactor

    SciTech Connect (OSTI)

    Serebrov, A. P. Ivochkin, V. G.; Samoylov, R. M.; Fomin, A. K.; Zinoviev, V. G.; Neustroev, P. V.; Golovtsov, V. L.; Gruzinsky, N. V.; Solovey, V. A.; Chernyi, A. V.; Zherebtsov, O. M.; Martemyanov, V. P.; Tsinoev, V. G.; Tarasenkov, V. G.; Aleshin, V. I.; Petelin, A. L.; Pavlov, S. V.; Izhutov, A. L.; Sazontov, S. A.; Ryazanov, D. K.; and others

    2015-10-15

    In view of the possibility of the existence of a sterile neutrino, test measurements of the dependence of the reactor antineutrino flux on the distance from the reactor core has been performed on SM-2 reactor with the Neutrino-2 detector model in the range of 6–11 m. Prospects of the search for reactor antineutrinos at short distances have been discussed.

  11. Correct implementation of the Argonne QuickSite{sup SM} process for preremedial site investigations

    SciTech Connect (OSTI)

    Burton, J.C.; Walker, J.L.

    1997-10-01

    Expedited site characterization (ESC), developed by Argonne National Laboratory, is an interactive, integrated process emphasizing the use of existing data of sufficient quality, multiple complementary characterization methods, and on-site decision making to optimize environmental site investigations. The Argonne ESC is the basis for the provisional ESC standard guide of the ASTM (American Society for Testing and Materials). QuickSite{sup SM} is the implementation package developed by Argonne to facilitate ESC of sites contaminated with hazardous wastes. At various sites, Argonne has successfully implemented QuickSite{sup SM} and demonstrated the technical superiority of the ESC process over traditional methodologies guided by statistics and random-sampling approaches. A key feature in the success of QuickSite{sup SM} investigations is achieving an understanding of the subsurface geologic and hydrogeologic controls and processes at a site before extensive sampling efforts begin. The QuickSite{sup SM} investigation at the Tustin Marine Corps Air Station (MCAS) in California will be used to illustrate the importance of understanding these potential controls in minimizing sampling activities and correctly predicting potential contaminant migration patterns for risk assessment.

  12. Chemical stability of highly (0001) textured Sm(CoCu){sub 5} thin films with a thin Ta capping layer

    SciTech Connect (OSTI)

    Zhao Haibao; Wang Hao; Liu Xiaoqi; Wang Jianping; Zhang Tao

    2011-04-01

    With the highest magnetocrystalline anisotropy constant (Ku) among practical magnetic materials, SmCo{sub 5} could be a very attractive candidate for future high areal density magnetic recording. However, its corrosion resistance is always a concern in recording media applications. In this paper, the chemical stability and microstructures of highly (0001) textured Sm(CoCu){sub 5} thin films with and without a 3 nm Ta capping layer were reported. For Sm(CoCu){sub 5} thin films without a capping layer, the coercivity decreases significantly (from 8kOe to 1kOe) within one month. Sm(CoCu){sub 5} thin films capped with a thin Ta layer (3 nm) behave differently. Even exposed to a laboratory environment (25 deg. C) over 3 years, the Ta-capped Sm(CoCu){sub 5} thin films are stable in terms of structural and magnetic properties, i.e., there were no changes in X-ray diffraction peaks and vibrating sample magnetometer hysteresis loops. Microstructure of Ta-capped Sm(CoCu){sub 5} thin films showed that Sm(CoCu){sub 5} formed a domelike particle assembly structure on a smooth Ru underlayer and were well covered by partially oxidized Ta capping layer, as shown by TEM cross-section micrographs. Accelerated corrosion treatment (130 deg. C, 95% relative humidity, 6 h) was performed on Ta-capped Sm(CoCu){sub 5} thin films. X-ray photoelectron spectroscopy (XPS) results showed that no Co was detected on the sample surface before the corrosion treatment, but strong XPS signals of CoOx and Co(OH)x were observed after treatment. Therefore, none of our Sm(CoCu){sub 5} thin films can pass the accelerated corrosion test. Hcp-phased CoPt-alloys are proposed as better capping materials for Sm(CoCu){sub 5} thin films in future high-density magnetic recording applications.

  13. Theory of point-defects, non-stoichiometry, and solute additions in SmCo{sub 5+x}-Sm{sub 2}Co{sub 17{minus}y} and related compounds

    SciTech Connect (OSTI)

    WELCH,D.O.

    1998-09-03

    There is considerable interest in the possibility of producing Sm-Co-based nanocomposite magnets by rapid solidification and other far-from-equilibrium processing methods. Thermodynamic and kinetic models are quite valuable in understanding and optimizing such methods. This paper describes a method of estimation, utilizing tight-binding-based bond-order interatomic interaction potentials, of the thermodynamic properties of point defects such as vacancies, interstitials, antisite defects, and solute additions in the SmCo{sub 5+x} and Sm{sub 2}Co {sub 17}-y phases and related rare-earth-transition metal compounds. Illustrative calculations for point defects in SmCo{sub 5} will be presented. The results suggest a unified model of the thermodynamic properties of the SmCo{sub 5+x} -- Sm{sub 2} Co{sub 17{minus}y} region of the phase diagram, based on the 1-5 structure and the replacement of Sm by interacting dumb-bell interstitials to form the 2-17 structure; the model is similar in nature to theories of the thermodynamics of metal hydrides.

  14. TANK 40 FINAL SB5 CHEMICAL CHARACTERIZATION RESULTS PRIOR TO NP ADDITION

    SciTech Connect (OSTI)

    Bannochie, C.; Click, D.

    2010-01-06

    A sample of Sludge Batch 5 (SB5) was pulled from Tank 40 in order to obtain radionuclide inventory analyses necessary for compliance with the Waste Acceptance Product Specifications (WAPS). This sample was also analyzed for chemical composition including noble metals. Prior to radionuclide inventory analyses, a final sample of the H-canyon Np stream will be added to bound the Np addition anticipated for Tank 40. These analyses along with the WAPS radionuclide analyses will help define the composition of the sludge in Tank 40 that is currently being fed to DWPF as SB5. At the Savannah River National Laboratory (SRNL) the 3-L Tank 40 SB5 sample was transferred from the shipping container into a 4-L high density polyethylene vessel and solids allowed to settle overnight. Supernate was then siphoned off and circulated through the shipping container to complete the transfer of the sample. Following thorough mixing of the 3-L sample, a 239 g sub-sample was removed. This sub-sample was then utilized for all subsequent analytical samples. Eight separate aliquots of the slurry were digested, four with HNO{sub 3}/HCl (aqua regia) in sealed Teflon{reg_sign} vessels and four in Na{sub 2}O{sub 2} (alkali or peroxide fusion) using Zr crucibles. Due to the use of Zr crucibles and Na in the peroxide fusions, Na and Zr cannot be determined from this preparation. Additionally, other alkali metals, such as Li and K that may be contaminants in the Na{sub 2}O{sub 2} are not determined from this preparation. Three Analytical Reference Glass - 14 (ARG-1) standards were digested along with a blank for each preparation. The ARG-1 glass allows for an assessment of the completeness of each digestion. Each aqua regia digestion and blank was diluted to 1:100 mL with deionized water and submitted to Analytical Development (AD) for inductively coupled plasma - atomic emission spectroscopy (ICPAES) analysis, inductively coupled plasma - mass spectrometry (ICP-MS) analysis of masses 81-209 and 230

  15. QCD Thermodynamics at High Temperature Peter Petreczky Large Scale Computing and Storage Requirements for Nuclear Physics (NP),

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    QCD Thermodynamics at High Temperature Peter Petreczky Large Scale Computing and Storage Requirements for Nuclear Physics (NP), Bethesda MD, April 29-30, 2014 NY Center for Computational Science 2 Defining questions of nuclear physics research in US: Nuclear Science Advisory Committee (NSAC) "The Frontiers of Nuclear Science", 2007 Long Range Plan "What are the phases of strongly interacting matter and what roles do they play in the cosmos ?" "What does QCD predict for

  16. ARCADIA{sup R} - A New Generation of Coupled Neutronics / Core Thermal- Hydraulics Code System at AREVA NP

    SciTech Connect (OSTI)

    Curca-Tivig, Florin; Merk, Stephan; Pautz, Andreas; Thareau, Sebastien

    2007-07-01

    Anticipating future needs of our customers and willing to concentrate synergies and competences existing in the company for the benefit of our customers, AREVA NP decided in 2002 to develop the next generation of coupled neutronics/ core thermal-hydraulic (TH) code systems for fuel assembly and core design calculations for both, PWR and BWR applications. The global CONVERGENCE project was born: after a feasibility study of one year (2002) and a conceptual phase of another year (2003), development was started at the beginning of 2004. The present paper introduces the CONVERGENCE project, presents the main feature of the new code system ARCADIA{sup R} and concludes on customer benefits. ARCADIA{sup R} is designed to meet AREVA NP market and customers' requirements worldwide. Besides state-of-the-art physical modeling, numerical performance and industrial functionality, the ARCADIA{sup R} system is featuring state-of-the-art software engineering. The new code system will bring a series of benefits for our customers: e.g. improved accuracy for heterogeneous cores (MOX/ UOX, Gd...), better description of nuclide chains, and access to local neutronics/ thermal-hydraulics and possibly thermal-mechanical information (3D pin by pin full core modeling). ARCADIA is a registered trademark of AREVA NP. (authors)

  17. Effect of 1-hydroxyethane-1,1-diphosphonic acid (HEDPA) on Partitioning of Np and Pu to Synthetic Boehmite

    SciTech Connect (OSTI)

    Powell, Brian A.; Rao, Linfeng; Nash, Kenneth L.

    2009-05-01

    The effect of 1-hydroxyethane-1,1-diphosphonic acid (HEDPA) on sorption of Np(V) and Pu(V) to synthetic boehmite ({gamma}-AlOOH) was examined a function of time and pH (between 4 to 11). Sorption of both elements in boehmite suspensions (1 M NaCl, 600 mg L{sup -1} boehmite) increased with increasing pH. Sorption edges for neptunium and plutonium occurred at approximately pH 8.0 and 6.6, respectively. After steady state partitioning was reached, HEDPA was added to the neptunium-boehmite and plutonium-boehmite suspensions. Neptunium and plutonium partitioning appears to be primarily affected by the formation of soluble Np:HEDPA and Pu:HEDPA complexes, the dissolution of boehmite promoted by HEDPA, and the precipitation of Np:HEDPA and Pu:HEDPA colloids. The results are discussed in terms of applicability of HEDPA-promoted dissolution as a waste reduction method in the treatment of sludge phases contained within high-level nuclear waste storage tanks.

  18. Synthesis and luminescent properties of spindle-like CaWO{sub 4}:Sm{sup 3+} phosphors

    SciTech Connect (OSTI)

    Tian, Yue [College of Life Science, Dalian Nationalities University, Dalian, Liaoning 116600 (China) [College of Life Science, Dalian Nationalities University, Dalian, Liaoning 116600 (China); Department of Physics, Dalian Maritime University, Dalian, Liaoning 116026 (China); Liu, Yu [Faculty of Chemical, Environmental and Biological Science and Technology, Dalian University of Technology, Dalian, Liaoning 116024 (China)] [Faculty of Chemical, Environmental and Biological Science and Technology, Dalian University of Technology, Dalian, Liaoning 116024 (China); Hua, Ruinian, E-mail: rnhua@dlnu.edu.cn [College of Life Science, Dalian Nationalities University, Dalian, Liaoning 116600 (China)] [College of Life Science, Dalian Nationalities University, Dalian, Liaoning 116600 (China); Na, Liyan [College of Life Science, Dalian Nationalities University, Dalian, Liaoning 116600 (China)] [College of Life Science, Dalian Nationalities University, Dalian, Liaoning 116600 (China); Chen, Baojiu, E-mail: chenmbj@sohu.com [Department of Physics, Dalian Maritime University, Dalian, Liaoning 116026 (China)] [Department of Physics, Dalian Maritime University, Dalian, Liaoning 116026 (China)

    2012-01-15

    Graphical abstract: In this paper, spindle-like CaWO{sub 4}:Sm{sup 3+} phosphors were prepared via a polyvinylpyrrolidone (PVP)-assisted sonochemical process. Dependence of emission intensity on Sm{sup 3+} ions concentration in the CaWO{sub 4}:Sm{sup 3+} phosphor were also calculated via a nonlinear fitting by using the formula y = ax/(1 + bx{sup c}). Highlights: Black-Right-Pointing-Pointer The samples were prepared via a PVP assisted sonochemical process. Black-Right-Pointing-Pointer The color coordinates for 1 mol% Sm{sup 3+} doped CaWO{sub 4} phosphor were calculated. Black-Right-Pointing-Pointer The D-D interaction is responsible for concentration quenching between Sm{sup 3+} ions. Black-Right-Pointing-Pointer The critical energy transfer distances (R{sub c}) were obtained. -- Abstract: Spindle-like CaWO{sub 4}:Sm{sup 3+} phosphors were prepared via a Polyvinylpyrrolidone (PVP)-assisted sonochemical process, and characterized by using X-ray diffraction (XRD), field emission scanning electron microscopy (FE-SEM) and photoluminescence spectroscopy (PL). The XRD results suggested that the prepared samples are single-phase. The FE-SEM images indicated that the prepared CaWO{sub 4}:Sm{sup 3+} phosphors are composed of many spindles with maximum average diameter of 150 nm and maximum average length of 500 nm. Under 404 nm excitation, the characteristic emissions corresponding to {sup 4}G{sub 5/2} {yields} {sup 6}H{sub J} (J = 5/2, 7/2, 9/2 and 11/2) transitions of Sm{sup 3+} in CaWO{sub 4} phosphors were observed. The color coordinates for 1 mol% Sm{sup 3+} doped CaWO{sub 4} phosphor were calculated to be (0.595, 0.404). The fluorescent concentration quenching of Sm{sup 3+} doped spindle-like phosphors was studied based on the Van Uitert's model, and it was found that the electric dipole-dipole (D-D) interaction is the dominant energy transfer mechanism between Sm{sup 3+} ions in the CaWO{sub 4}:Sm{sup 3+} phosphors. The critical energy transfer distance was

  19. Effects of substrate temperature and Cu underlayer thickness on the formation of SmCo{sub 5}(0001) epitaxial thin films

    SciTech Connect (OSTI)

    Ohtake, Mitsuru; Nukaga, Yuri; Futamoto, Masaaki; Kirino, Fumiyoshi

    2010-05-15

    SmCo{sub 5}(0001) epitaxial thin films were prepared on Cu(111) underlayers heteroepitaxially grown on Al{sub 2}O{sub 3}(0001) single-crystal substrates by molecular beam epitaxy. The effects of substrate temperature and Cu underlayer thickness on the crystallographic properties of SmCo{sub 5}(0001) epitaxial films were investigated. The Cu atoms of underlayer diffuse into the SmCo{sub 5} film and substitute the Co sites in SmCo{sub 5} structure forming an alloy compound of Sm(Co,Cu){sub 5}. The ordered phase formation is enhanced with increasing the substrate temperature and with increasing the Cu underlayer thickness. The Cu atom diffusion into the SmCo{sub 5} film is assisting the formation of Sm(Co,Cu){sub 5} ordered phase.

  20. Magnetic properties and Fermi surface of antiferromagnetic SmCu/sub 6/

    SciTech Connect (OSTI)

    Onuki, Y.; Umezawa, A.; Kwok, W.K.; Crabtree, G.W.; Nishihara, M.; Ina, K.; Yamazaki, T.; Omi, T.; Komatsubara, T.; Maezawa, K.

    1987-08-01

    We report measurements of the magnetic susceptibility, specific heat, magnetoresistance, Hall effect, and Fermi surface in SmCu/sup 6/. The susceptibility follows the Van Vleck form for Sm/sup 3 +/ near room temperature and shows two antiferromagnetic phase transitions at 9.6 K and 5.2 K. The specific heat implies a quartet ground state for the crystal field split J = 5/2 angular momentum state. Magnetoresistance indicates two conduction carriers of uncompensated electrons and holes. de Haas-van Alphen measurements show that the Fermi surface in the antiferromagnetic state consists of a network of cylinders oriented 30/degree/ from the b and c axes. 14 refs., 10 figs.

  1. 3D Torus Routing Engine Module for OFA OpenSM v. 1.0

    Energy Science and Technology Software Center (OSTI)

    2009-11-12

    This OpenFabrics Alliance (OFA) OpenSM routing engine module provides credit-loop-free routing while supporting two quality of service (QoS) levels for an InfiniBand fabric with a 3D torus topology. In addition it is able to route around multiple failed fabric links or a single failed fabric switch without introducing credit loops, and without changing path Service Level (SL) values granted before the failure.This OFA OpenSM routing engine module improves the operational characteristics of a parallel computermore » built using an InfiniBand fabric with a 3D torus topology. By providing two QoS levels, it allows system administrators to prevent application interprocess communication and file system communication from impacting each other. By providing the capability to route traffic around failed fabric components, it enables repair of failed components without impacting jobs running on the computer system.« less

  2. Brilliant Sm, Eu, Tb and Dy chiral lanthanide complexes withstrong circularly polarized luminescence

    SciTech Connect (OSTI)

    Petoud, Stephane; Muller, Gilles; Moore, Evan G.; Xu, Jide; Sokolnicki, Jurek; Riehl, James P.; Le, Uyen; Cohen, Seth M.; Raymond,Kenneth N.

    2006-07-10

    The synthesis, characterization and luminescent behavior of trivalent Sm, Eu, Dy and Tb complexes of two enantiomeric, octadentate, chiral, 2-hydroxyisophthalamide ligands are reported. These complexes are highly luminescent in solution. Functionalization of the achiral parent ligand with a chiral 1-phenylethylamine substituent on the open face of the complex in close proximity to the metal center yields complexes with strong circularly polarized luminescence (CPL) activity. This appears to be the first example of a system utilizing the same ligand architecture to sensitize four different lanthanide cations and display CPL activity. The luminescence dissymmetry factor, g{sub lum}, recorded for the Eu(III) complex is one of the highest values reported, and this is the first time the CPL effect has been demonstrated for a Sm(III) complex with a chiral ligand. The combination of high luminescence intensity with CPL activity should enable new bioanalytical applications of macromolecules in chiral environments.

  3. Di-boson production and SM SUSY Higgs searches at the Tevatron

    SciTech Connect (OSTI)

    Elvira, V.Daniel; /Fermilab

    2005-07-01

    The discovery of the Higgs boson would be a major success for the Standard Model (SM) and would provide further insights into the electroweak symmetry breaking mechanism. This report contains the latest results from the D0 and CDF Tevatron experiments on searches for the SM Higgs produced from gluon fusion with H {yields} WW, and in association with a W boson. It also includes searches for a supersymmetric Higgs in the b{bar b} and {tau}{sup +}{tau}{sup -} decay channels. The study of di-boson production at the Tevatron is important to understand backgrounds in high mass Higgs searches. It also provides a test of the SM through the measurement of the production cross section and the gauge boson self couplings. This paper includes measurements of the WW, W{gamma}, and WZ production cross sections, as well as limits on the anomalous couplings associated with the WW{gamma} and WWZ interactions. The results are based on sets of up to 320 pb{sup -1} of data collected by the D0 and CDF experiments at the {bar p}p Tevatron collider, running at a center-of-mass energy of 1.96 TeV.

  4. Ferroelectric studies of excessive Sm{sup 3+} containing perovskite PZT and pyrochlore biphase ceramics

    SciTech Connect (OSTI)

    Babu, T. Anil; Sastry, D. L.; Ramesh, K. V.; Reddy, V. Raghavendra

    2014-04-24

    Polycrystalline samples of Sm{sup 3+} modified Pb{sub 1?x} Sm{sub 2x/3} (Zr{sub 0.6}Ti{sub 0.4}) O{sub 3} (PSZT) ceramics (where x = 0.1, 0.2, 0.3, 0.4) have been prepared by a high energy ball milling technique, followed by calcination at 950C and sintering at 1150C. As x is increased more than 0.1 mole%, considerable secondary phase has been formed. This phase has been identified as pyrochlore Sm{sub 2}Ti{sub 2}O{sub 7} from its X-ray diffraction (XRD) peaks. The XRD studies also indicate that the perovskte phases of the present systems undergo a dopant induced phase transformation from rhombohedral to tetragonal strucure. All the samples exhibit diffuse but non-relaxor type ferroelectric phase transition. The results of dielectric and hysteresis studies of these materials are presented.

  5. Robust topological surface state in Kondo insulator SmB{sub 6} thin films

    SciTech Connect (OSTI)

    Yong, Jie Jiang, Yeping; Zhang, Xiaohang; Greene, Richard L.; Usanmaz, Demet; Curtarolo, Stefano; Li, Linze; Pan, Xiaoqing; Shin, Jongmoon; Takeuchi, Ichiro

    2014-12-01

    Fabrication of smooth thin films of topological insulators with true insulating bulk are extremely important for utilizing their novel properties in quantum and spintronic devices. Here, we report the growth of crystalline thin films of SmB{sub 6}, a topological Kondo insulator with true insulating bulk, by co-sputtering both SmB{sub 6} and B targets. X-ray diffraction, Raman spectroscopy, and transmission electron microscopy indicate films that are polycrystalline with a (001) preferred orientation. When cooling down, resistivity ρ shows an increase around 50 K and saturation below 10 K, consistent with the opening of the hybridization gap and surface dominated transport, respectively. The ratio ρ{sub 2K}/ρ{sub 300K} is only about two, much smaller than that of bulk, which indicates a much larger surface-to-bulk ratio. Point contact spectroscopy using a superconductor tip on SmB{sub 6} films shows both a Kondo Fano resonance and Andeev reflection, indicating an insulating Kondo lattice with metallic surface states.

  6. Effect of rare-earth doping in RCrSb3 (R = La, Pr, Sm, and Gd...

    Office of Scientific and Technical Information (OSTI)

    Journal Article: Effect of rare-earth doping in RCrSb3 (R La, Pr, Sm, and Gd) Citation Details In-Document Search ... We report on the electrical resistivity and magnetic ...

  7. Spin-glass behavior of A Fe sub 4 Al sub 8 ( A =Th,U,Np) intermetallics

    SciTech Connect (OSTI)

    Gal, J. Nuclear Research Center, 84190 Beer-Sheva Physik Department E15, Technische Universitaet Muenchen, D-8046 Garchingbei Muenchen ); Yaar, I.; Regev, D.; Fredo, S.; Shani, G.; Arbaboff, E. Nuclear Research Center, 84190 Beer-Sheva ); Potzel, W.; Aggarwal, K.; Pereda, J.A.; Kalvius, G.M. ); Litterst, F.J. Physik Department E15, Technische Universitaet Muenchen, D-8046 Garching bei Muenchen ); Schaefer, W.; Will, G. Kernforschonganlage, D-5170 Juelich )

    1990-11-01

    Combined ac- and dc-susceptibility, neutron-diffraction, and Moessbauer studies of UFe{sub 4}Al{sub 8}, NpFe{sub 4}Al{sub 8}, and ThFe{sub 4}Al{sub 8} argue for the establishment of a spin-glass (SG) state below {ital T}{sub SG}({ital B}{r arrow}0){approx}130, 120, and 110 K, respectively. The SG temperature {ital T}{sub SG}({ital B}) decreases with application of external magnetic field {ital B}. The ac susceptibility ({chi}{sub ac}) shows a sharp cusp at {ital T}{sub SG}({ital B}{approx}0). The isothermal and thermoremanent magnetization differ markedly and show temperature-dependent irreversibilities below {ital T}{sub SG}({ital B}). The Moessbauer spectra reveal onset of hyperfine splitting, indicating frozen spins below {ital T}{sub SG}(0). The neutron-diffraction studies of UFe{sub 4}Al{sub 8} and NpFe{sub 4}Al{sub 8} show that after switching off the external magnetic field greater than 3 T the U and Np momenta (2{ital a} site) are frozen parallel to the direction of the external field. We label the freezing temperature under high external fields {ital T}{sub OG}, and show that it serves as the upper limit of {ital T}{sub SG}({ital B}) with {ital T}{sub SG}({ital B}{r arrow}0){r arrow}{ital T}{sub OG}. For concentrated SG systems, {ital T}{sub SG}(0) is a reproducible value, independent of the observation time window, which indicates a true thermodynamic phase transition; the cusp in {chi}{sub ac}, however, is not necessarily a confirmation for the establishment of a SG state.

  8. High- and low-Am RE inclusion phases in a U-Np-Pu-Am-Zr alloy

    SciTech Connect (OSTI)

    Janney, Dawn E.; Madden, James W.; O'Holleran, Thomas P.; Kennedy, J. Rory

    2015-03-01

    Structural, microstructural, and microchemical data were collected from rare-earth inclusions in an as-cast U-Pu-Zr alloy with ~3 at% Am, 2% Np, and 9% rare-earth elements (La, Ce, Pr, and Nd). Two RE phases with different concentrations of Am were identified. The composition of high-Am RE inclusions is ~2-5 at% La, 15-20 % Ce, 5-10% Pr, 25-45% Nd, 1% Np, 5-10% Pu, and 10-20% Am. Some areas also have O, although this does not appear to be an essential part of the high-Am RE phase. The inclusions have a face-centered cubic structure with a lattice parameter a ~ 0.54 nm. The composition of the only low-Am RE inclusion studied in detail is ~~35-40 at% O, 40-45 % Nd, 1-2% Zr, 4-5% La, 9-10% Ce, and 6-7% Pr. This inclusion is an oxide with a crystal structure similar to the room-temperature structure of Nd2O3. Microstructural features suggest that oxidation occurred during casting, and that early crystallization of high-temperature oxides led to formation of two distinct RE phases.

  9. Magnetic property, Raman spectroscopy and crystal field analysis of Sm{sub 3+} in Sm(BrO{sub 3}){sub 3}⋅9H{sub 2}O

    SciTech Connect (OSTI)

    Mandal, J.; Chakrabarti, P. K.; Purohit, T.; Chattopadhyay, K. N.; Ghosh, M.

    2014-04-24

    Single crystals of Sm(BrO{sub 3}){sub 3}⋅9H{sub 2}O (SmBR) were grown and the principal molar susceptibility perpendicular to c-axis (χ{sub ⊥}) was measured from 300 K down to 14 K and χ{sub ‖}, the parallel susceptibility, anisotropy was measured in the temperature range of 300-120 K. A cross-over between χ{sub ‖} and χ{sub ⊥} was observed at ∼ 120 K i.e., below this temperature χ{sub |||}<χ{sub ‖}. Raman spectra of SmBR were recorded in the wave number range of 10-4000 cm{sup −1} and crystal field (CF) Stark energies were extracted from the spectra. A good theoretical simulation of the observed magnetic susceptibilities and observed CF Stark energies of Sm{sup 3+} in SmBR was achieved using the one electron crystal field (CF) interaction with D{sup 3h} site symmetry. The electronic specific heat along with the quadruple splitting and hyperfine heat capacity were calculated by using the results of CF analysis.

  10. Surface state reconstruction in ion-damaged SmB6

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Wakeham, N.; Wang, Y. Q.; Fisk, Z.; Ronning, F.; Thompson, J. D.

    2015-02-12

    We have used ion-irradiation to damage the (001) surfaces of SmB₆ single crystals to varying depths, and have measured the resistivity as a function of temperature for each depth of damage. We observe a reduction in the residual resistivity with increasing depth of damage. Our data are consistent with a model in which the surface state is not destroyed by the ion-irradiation, however instead the damaged layer is poorly conducting and the initial surface state is reconstructed below the damage. This behavior is consistent with a surface state that is topologically protected.

  11. Effect of milling time on magnetic properties and structures of bulk Sm-Co/{alpha}-(Fe, Co) nanocomposite magnets

    SciTech Connect (OSTI)

    Shen, Y.; Huang, M. Q.; Turgut, Z.; Lucas, M. S.; Michel, E.; Horwath, J. C.

    2012-04-01

    Bulk Sm-Co/{alpha}-(Fe,Co) nanocomposite magnets were fabricated by hot pressing composite powders prepared by high-energy ball milling of magnetically hard SmCo{sub 5} powder and magnetically soft Fe powder. The bulk magnets had a nanocomposite structure consisting of Sm-Co matrix (1:5 H and 1:7 H phases) and {alpha}-(Fe,Co) phases. The Fe-Co particles were distributed uniformly in the Sm-Co matrix. The milling time strongly affects the structures and the magnetic properties of the bulk magnets. Increasing milling time led to a decrease of the amount of 1:5 H phase, an increase in the phase fraction of the 1:7 H phase, and a decrease in the amount of soft phase, which resulted in an increase in magnetization and a decrease in coercivity. Scanning electron microscopy (SEM)/energy dispersive spectroscopy (EDS) analyses revealed that inter-diffusion took place between the Sm-Co matrix and Fe particles during the processing.

  12. Dipole strength in {sup 144}Sm studied via (gamma,n), (gamma,p), and (gamma,alpha) reactions

    SciTech Connect (OSTI)

    Nair, C.; Junghans, A. R.; Erhard, M.; Bemmerer, D.; Beyer, R.; Kosev, K.; Marta, M.; Rusev, G.; Schilling, K. D.; Schwengner, R.; Wagner, A.; Grosse, E.

    2010-05-15

    Photoactivation measurements on {sup 144}Sm have been performed with bremsstrahlung endpoint energies from 10.0 to 15.5 MeV at the bremsstrahlung facility of the superconducting electron accelerator ELBE of Forschungszentrum Dresden-Rossendorf. The measured activation yield for the {sup 144}Sm(gamma,n) reaction is compared with the calculated yield using cross sections from previous photoneutron experiments. The activation yields measured for all disintegration channels {sup 144}Sm(gamma,n), (gamma,p), and (gamma,alpha) are compared to the yield calculated by using Hauser-Feshbach statistical models. A new parametrization of the photon strength function is presented and the yield simulated by using the modified photon strength parameters is compared to the experimental data.

  13. Inelastic X-ray Scattering Investigations of Lattice Dynamics in SmFeAsO1-xFy Superconductors

    SciTech Connect (OSTI)

    Hill, J.P.; Le Tacon, M.; Forrest, T.R.; Ruegg, Ch.; Bosak, A.; Noffsinger, J.; Walters, A.C.; Toulemonde, P.; Palenzona, A.; Zhigadlo, N.D.; Karpinski, J.; Krisch, M.; McMorrow, D.F.

    2010-05-23

    We report measurements of the phonon density of states as measured with inelastic x-ray scattering in SmFeAsO{sub 1-x}F{sub y} powders. An unexpected strong renormalization of phonon branches around 23 meV is observed as fluorine is substituted for oxygen. Phonon dispersion measurements on SmFeAsO{sub 1-x}F{sub y} single crystals allow us to identify the 21 meV A{sub 1g} in-phase (Sm,As) and the 26 meV B{sub 1g} (Fe,O) modes to be responsible for this renormalization, and may reaveal unusual electron-phonon coupling through the spin channel in iron-based superconductors.

  14. Measurement of np elastic scattering spin-spin correlation parameters at 484, 634, and 788 MeV

    SciTech Connect (OSTI)

    Garnett, R.W.

    1989-03-01

    The spin-spin correlation parameters C/sub LL/ and C/sub SL/ were measured for np elastic scattering at the incident neutron kinetic energy of 634 MeV. Good agreement was obtained with previously measured data. Additionally, the first measurement of the correlation parameter C/sub SS/ was made at the three energies, 484, 634, and 788 MeV. It was found that the new values, in general, do not agree well with phase shift predictions. A study was carried out to determine which of the isospin-0 partial waves will be affected by this new data. It was found that the /sup 1/P/sub 1/ partial wave will be affected significantly at all three measurement energies. At 634 and 788 MeV, the /sup 3/S/sub 1/ phase shifts will also change. 29 refs., 21 figs., 16 tabs.

  15. Development of interatomic potentials appropriate for simulation of devitrification of Al90Sm10 alloy

    SciTech Connect (OSTI)

    Mendelev, M. I.; Zhang, F.; Ye, Z.; Sun, Y.; Nguyen, M. C.; Wilson, S. R.; Wang, C. Z.; Ho, K. M.

    2015-04-23

    In this study, a semi-empirical potential for the Al90Sm10 alloy is presented. The potential provides satisfactory reproduction of pure Al properties, the formation energies of a set of Al–Sm crystal phases with Sm content about 10%, and the structure of the liquid Al90Sm10 alloy. During molecular dynamics simulation in which the liquid alloy is cooled at a rate of 1010 K/s, the developed potential produces a glass structure with lower ab initio energy than that produced by ab initio molecular dynamics (AIMD) itself using a typical AIMD cooling rate of 8 ∙1013 K/s. Based on these facts the developed potential should be suitable for simulations of phase transformations in the Al90Sm10 alloy.

  16. Imaging space charge regions in Sm-doped ceria using electrochemical strain microscopy

    SciTech Connect (OSTI)

    Chen, Qian Nataly; Li, Jiangyu; Adler, Stuart B.

    2014-11-17

    Nanocrystalline ceria exhibits a total conductivity several orders of magnitude higher than microcrystalline ceria in air at high temperature. The most widely accepted theory for this enhancement (based on fitting of conductivity data to various transport and kinetic models) is that relatively immobile positively charged defects and/or impurities accumulate at the grain boundary core, leading to a counterbalancing increase in the number of mobile electrons (small polarons) within a diffuse space charge region adjacent to each grain boundary. In an effort to validate this model, we have applied electrochemical strain microscopy to image the location and relative population of mobile electrons near grain boundaries in polycrystalline Sm-doped ceria in air at 20200?C. Our results show the first direct (spatially resolved) evidence that such a diffuse space charge region does exist in ceria, and is localized to both grain boundaries and the gas-exposed surface.

  17. Probing the nuclides {sup 102}Pd, {sup 106}Cd, and {sup 144}Sm for resonant neutrinoless double-electron capture

    SciTech Connect (OSTI)

    Goncharov, M.; Blaum, K.; Eliseev, S.; Block, M.; Herfurth, F.; Minaya Ramirez, E.; Droese, C.; Schweikhard, L.; Novikov, Yu. N.; Zuber, K.

    2011-08-15

    The Q values for double-electron capture in {sup 102}Pd, {sup 106}Cd, and {sup 144}Sm have been measured by Penning-trap mass spectrometry. The results exclude at present all three nuclides from the list of suitable candidates for a search for resonant neutrinoless double-electron capture.

  18. Effect of Doping on Surface Reactivity and Conduction Mechanism in Sm-doped CeO2 Thin Films

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Yang, Nan; Belianinov, Alex; Strelcov, Evgheni; Tebano, Antonello; Daniele, Di Castro; Schlueter, Christoph; Lee, Tien-Lin; Baddorf, Arthur P.; Wisinger, Nina; Jesse, Stephen; et al

    2014-11-21

    Scanning probe microscopy measurements show irreversible surface electrochemistry in Sm-doped CeO2 thin films, which depends on humidity, temperature and doping concentration. A systematic study by electrochemical strain microscopy (ESM) in samples with two different Sm content and in several working conditions allows disclosing the microscopic mechanism underlying the difference in water adsorption and splitting with subsequent proton liberation. We measure the behavior of the hysteresis loops by changing temperature and humidity, both in standard ESM configuration and using the first order reversal curve (FORC) method. Complementing our study with spectroscopic measurements by hard x-ray photoemission spectroscopy we find that watermore » incorporation is favored until the doping with Sm is too high to allow the presence of Ce3+. The influence of doping on the surface reactivity and conduction mechanism clearly emerges from all of our experimental results. We find that at lower Sm concentration proton conduction is prevalent, featured by lower activation energy and higher mobility. Defect concentrations determine the type of the prevalent charge carrier in a doping dependent manner.« less

  19. Monte Carlo calculated TG-60 dosimetry parameters for the {beta}{sup -} emitter {sup 153}Sm brachytherapy source

    SciTech Connect (OSTI)

    Sadeghi, Mahdi; Taghdiri, Fatemeh; Hamed Hosseini, S.; Tenreiro, Claudio

    2010-10-15

    Purpose: The formalism recommended by Task Group 60 (TG-60) of the American Association of Physicists in Medicine (AAPM) is applicable for {beta} sources. Radioactive biocompatible and biodegradable {sup 153}Sm glass seed without encapsulation is a {beta}{sup -} emitter radionuclide with a short half-life and delivers a high dose rate to the tumor in the millimeter range. This study presents the results of Monte Carlo calculations of the dosimetric parameters for the {sup 153}Sm brachytherapy source. Methods: Version 5 of the (MCNP) Monte Carlo radiation transport code was used to calculate two-dimensional dose distributions around the source. The dosimetric parameters of AAPM TG-60 recommendations including the reference dose rate, the radial dose function, the anisotropy function, and the one-dimensional anisotropy function were obtained. Results: The dose rate value at the reference point was estimated to be 9.21{+-}0.6 cGy h{sup -1} {mu}Ci{sup -1}. Due to the low energy beta emitted from {sup 153}Sm sources, the dose fall-off profile is sharper than the other beta emitter sources. The calculated dosimetric parameters in this study are compared to several beta and photon emitting seeds. Conclusions: The results show the advantage of the {sup 153}Sm source in comparison with the other sources because of the rapid dose fall-off of beta ray and high dose rate at the short distances of the seed. The results would be helpful in the development of the radioactive implants using {sup 153}Sm seeds for the brachytherapy treatment.

  20. Effect of Front-Side Silver Metallization on Underlying n+-p Junction in Multicrystalline Silicon Solar Cells: Preprint

    SciTech Connect (OSTI)

    Jiang, C. S.; Li, Z. G.; Moutinho, H. R.; Liang, L.; Ionkin, A.; Al-Jassim, M. M.

    2012-06-01

    We report on the effect of front-side Ag metallization on the underlying n+-p junction of multicrystalline Si solar cells. The junction quality beneath the contacts was investigated by characterizing the uniformities of the electrostatic potential and doping concentration across the junction, using scanning Kelvin probe force microscopy and scanning capacitance microscopy. We investigated cells with a commercial Ag paste (DuPont PV159) and fired at furnace setting temperatures of 800 degrees, 840 degrees, and 930 degrees C, which results in actual cell temperatures ~100 degrees C lower than the setting temperature and the three cells being under-, optimal-, and over-fired. We found that the uniformity of the junction beneath the Ag contact was significantly degraded by the over-firing, whereas the junction retained good uniformity with the optimal- and under-fire temperatures. Further, Ag crystallites with widely distributed sizes from <100 nm to several μm were found at the Ag/Si interface of the over-fired cell. Large crystallites were imaged as protrusions into Si deeper than the junction depth. However, the junction was not broken down; instead, it was reformed on the entire front of the crystallite/Si interface. We propose a mechanism of the junction-quality degradation, based on emitter Si melting at the temperature around the Ag-Si eutectic point during firing, and subsequent recrystallization with incorporation of impurities in the Ag paste and with formation of crystallographic defects during quenching.

  1. Theoretical aspects of the magnetism in the ferromagnetic A Fe sub 2 systems ( A =U, Np, Pu, and Am)

    SciTech Connect (OSTI)

    Eriksson, O.; Johansson, B. ); Brooks, M.S.S. )

    1990-05-01

    We report on spin-polarized energy-band calculations for the cubic Laves-phase systems UFe{sub 2}, NpFe{sub 2}, PuFe{sub 2}, and AmFe{sub 2}. The calculations were performed with the local-density approximation for the exchange and correlation potential together with a term that shifts the one-electron eigenvalues and takes into account the different interelectronic repulsions for electrons with different 5{ital f} magnetic quantum numbers. The spin-orbit interaction was also included in the band Hamiltonian. Thus the parameter-free calculations incorporate Hund's first, second, and third rules. The magnetism in the first three compounds was found to be dominated by a large orbital contribution coupled antiparallel to the spin moment. In the calculations for AmFe{sub 2}, the 5{ital f} electrons were treated as core electrons. The magnetism was here found to behave very much like the magnetism of similar rare-earth Laves-phase compounds.

  2. NP Open Funding Opportunities

    Office of Science (SC) Website

    - and is the principal federal funding agency of - the Nation's research programs in high-energy physics, nuclear physics, and fusion energy sciences. en 8BF3F791-EE84-4768-BCDF-E...

  3. NP Spinoff Applications

    Office of Science (SC) Website

    of ultra-low concentrations of Krypton radioisotopes in samples of water, ice, and gas. Sun, 03 Jan 2016 12:04:19 -0500

    A state-of-the-art Atom Trap Trace Analysis (ATTA)...

  4. NP Science Highlights

    Office of Science (SC) Website

    :10px;margin-bottom:10px;'>Novel experiments measure unusual thermonuclear fusion of hydrogen with a rare oxygen isotope. Thu, 14 Jan 2016 12:08:33 -0500

    To improve our...

  5. Sm-Nd systematics of lunar ferroan anorthositic suite rocks: Constraints on lunar crust

    SciTech Connect (OSTI)

    Boyet, Maud; Carlson, Richard W.; Borg, Lars E.; Horan, Mary

    2014-09-28

    Here, we have measured Sm–Nd systematics, including the short-lived 146Sm–142Nd chronometer, in lunar ferroan anorthositic suite (FAS) whole rocks (15415, 62236, 62255, 65315, 60025). At least some members of the suite are thought to be primary crystallization products formed by plagioclase flotation during crystallization of the lunar magma ocean (LMO). Most of these samples, except 62236, have not been exposed to galactic cosmic rays for a long period and thus require minimal correction to their 142Nd isotope composition. These samples all have measured deficits in 142Nd relative to the JNdi-1 terrestrial standard in the range –45 to –21 ppm. The range is –45 to –15 ppm once the 62236 142Nd/144Nd ratio is corrected from neutron-capture effects. Analyzed FAS samples do not define a single isochron in either 146Sm–142Nd or 147Sm–143Nd systematics, suggesting that they either do not have the same crystallization age, come from different sources, or have suffered isotopic disturbance. Because the age is not known for some samples, we explore the implications of their initial isotopic compositions for crystallization ages in the first 400 Ma of solar system history, a timing interval that covers all the ages determined for the ferroan anorthositic suite whole rocks as well as different estimates for the crystallization of the LMO. 62255 has the largest deficit in initial 142Nd and does not appear to have followed the same differentiation path as the other FAS samples. The large deficit in 142Nd of FAN 62255 may suggest a crystallization age around 60–125 Ma after the beginning of solar system accretion. This result provides essential information about the age of the giant impact forming the Moon. The initial Nd isotopic compositions of FAS samples can be matched either with a bulk-Moon with chondritic Sm/Nd ratio but

  6. Sm-Nd systematics of lunar ferroan anorthositic suite rocks: Constraints on lunar crust

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Boyet, Maud; Carlson, Richard W.; Borg, Lars E.; Horan, Mary

    2014-09-28

    Here, we have measured Sm–Nd systematics, including the short-lived 146Sm–142Nd chronometer, in lunar ferroan anorthositic suite (FAS) whole rocks (15415, 62236, 62255, 65315, 60025). At least some members of the suite are thought to be primary crystallization products formed by plagioclase flotation during crystallization of the lunar magma ocean (LMO). Most of these samples, except 62236, have not been exposed to galactic cosmic rays for a long period and thus require minimal correction to their 142Nd isotope composition. These samples all have measured deficits in 142Nd relative to the JNdi-1 terrestrial standard in the range –45 to –21 ppm. Themore » range is –45 to –15 ppm once the 62236 142Nd/144Nd ratio is corrected from neutron-capture effects. Analyzed FAS samples do not define a single isochron in either 146Sm–142Nd or 147Sm–143Nd systematics, suggesting that they either do not have the same crystallization age, come from different sources, or have suffered isotopic disturbance. Because the age is not known for some samples, we explore the implications of their initial isotopic compositions for crystallization ages in the first 400 Ma of solar system history, a timing interval that covers all the ages determined for the ferroan anorthositic suite whole rocks as well as different estimates for the crystallization of the LMO. 62255 has the largest deficit in initial 142Nd and does not appear to have followed the same differentiation path as the other FAS samples. The large deficit in 142Nd of FAN 62255 may suggest a crystallization age around 60–125 Ma after the beginning of solar system accretion. This result provides essential information about the age of the giant impact forming the Moon. The initial Nd isotopic compositions of FAS samples can be matched either with a bulk-Moon with chondritic Sm/Nd ratio but enstatite-chondrite-like initial 142Nd/144Nd (e.g. 10 ppm below modern terrestrial), or a bulk-Moon with superchondritic Sm

  7. Photoluminescence properties of a new orange–red emitting Sm{sup 3+}-doped Y{sub 2}Mo{sub 4}O{sub 15} phosphor

    SciTech Connect (OSTI)

    Deng, Huajuan; Zhao, Ze; Wang, Jing; Hei, Zhoufei; Li, Mengxue; Noh, Hyeon Mi; Jeong, Jung Hyun; Yu, Ruijin

    2015-08-15

    A series of novel Y{sub 2}Mo{sub 4}O{sub 15}:xSm{sup 3+} ( (0.01 ≤ x ≤ 0.20) phosphors for white light-emitting (W-LEDs) were successfully prepared by the solid state reaction technology at 973 K for 12 h. X-ray diffraction and photoluminescence spectra were utilized to characterize the structure and luminescence properties of the as-synthesized phosphors. The emission spectra of the Y{sub 2}Mo{sub 4}O{sub 15}:Sm{sup 3+} phosphors consisted of some sharp emission peaks of Sm{sup 3+} ions centered at 565 nm, 605 nm, 650 nm, and 712 nm. The strongest one is located at 605 nm due to {sup 4}G{sub 5/2}–{sup 6}H{sub 7/2} transition of Sm{sup 3+}, generating bright orange–red light. The optimum dopant concentration of Sm{sup 3+} ions in Y{sub 2}Mo{sub 4}O{sub 15}:xSm{sup 3+} is around 5 mol% and the critical transfer distance of Sm{sup 3+} is calculated as 23.32 Å. The CIE chromaticity coordinates of the Y{sub 2}Mo{sub 4}O{sub 15}:0.05Sm{sup 3+} phosphors were located in the orange reddish region. The Y{sub 2}Mo{sub 4}O{sub 15}:Sm{sup 3+} phosphors may be potentially used as red phosphors for white light-emitting diodes. - Graphical abstract: The excitation spectrum of Y{sub 2}Mo{sub 4}O{sub 15}:Sm{sup 3+} is composed of a broad band and some sharp f–f transitions. Under 407 nm excitation, the phosphor presents some sharp emission peaks of Sm{sup 3+} ions. - Highlights: • An orange–red emitting Y{sub 2}Mo{sub 4}O{sub 15}:Sm{sup 3+} phosphor has been firstly synthesized. • Their structures, luminescent properties have also been investigated. • The optical absorption edge for the molybdate lies around 325 nm. • The CIE chromaticity coordinates were located in the orange reddish region.

  8. Ferromagnetic and paramagnetic magnetization of implanted GaN:Ho,Tb,Sm,Tm films

    SciTech Connect (OSTI)

    Maryško, M. Hejtmánek, J.; Laguta, V.; Sofer, Z.; Sedmidubský, D.; Šimek, P.; Veselý, M.; Mikulics, M.; Buchal, C.; Macková, A.; Malínský, P.; Wilhelm, R. A.

    2015-05-07

    The SQUID magnetic measurements were performed on the GaN films prepared by metal-organic vapour phase epitaxy and implanted by Tb{sup 3+}, Tm{sup 3+}, Sm{sup 3+}, and Ho{sup 3+} ions. The sapphire substrate was checked by the electron paramagnetic resonance method which showed a content of Cr{sup 3+} and Fe{sup 3+} impurities. The samples 5 × 5 mm{sup 2} were positioned in the classical straws and within an estimated accuracy of 10{sup −6 }emu, no ferromagnetic moment was detected in the temperature region of 2–300 K. The paramagnetic magnetization was studied for parallel and perpendicular orientation. In the case of GaN:Tb sample, at T = 2 K, a pronounced anisotropy with the easy axis perpendicular to the film was observed which can be explained by the lowest quasi-doublet state of the non-Kramers Tb{sup 3+} ion. The Weiss temperature deduced from the susceptibility data using the Curie-Weiss (C-W) law was found to depend substantially on the magnetic field.

  9. A Sensitivity Model (SM) approach to analyze urban development in Taiwan based on sustainability indicators

    SciTech Connect (OSTI)

    Huang Shuli Yeh Chiatsung Budd, William W. Chen Liling

    2009-02-15

    Sustainability indicators have been widely developed to monitor and assess sustainable development. They are expected to guide political decision-making based on their capability to represent states and trends of development. However, using indicators to assess the sustainability of urban strategies and policies has limitations - as they neither reflect the systemic interactions among them, nor provide normative indications in what direction they should be developed. This paper uses a semi-quantitative systematic model tool (Sensitivity Model Tools, SM) to analyze the role of urban development in Taiwan's sustainability. The results indicate that the natural environment in urban area is one of the most critical components and the urban economic production plays a highly active role in affecting Taiwan's sustainable development. The semi-quantitative simulation model integrates sustainability indicators and urban development policy to provide decision-makers with information about the impacts of their decisions on urban development. The system approach incorporated by this paper can be seen as a necessary, but not sufficient, condition for a sustainability assessment. The participatory process of expert participants for providing judgments on the relations between indicator variables is also discussed.

  10. Business Case Analysis for Replacing the Mazak 30Y Mill-Turn Machine in SM-39. Summary

    SciTech Connect (OSTI)

    Booth, Steven Richard; Dinehart, Timothy Grant; Benson, Faith Ann

    2015-03-19

    Business case studies are being looked at to support procurement of new machines and capital equipment in the SM-39 and TA-03-0102 machine shops. The first effort conducted economic analysis of replacing the Mazak 30Y Mill-Turn Machine located in SM-39. To determine the value of switching machinery, a baseline scenario was compared with a future scenario where new machinery was purchased and installed. The conditions under the two scenarios were defined via interviews with subject matter experts in terms of one-time and periodic costs. The results of the analysis were compiled in a life-cycle cost/benefit table. The costs of procuring, installing, and maintaining a new machine were balanced against the costs avoided by replacing older machinery. Productivity savings were included as a measure to show the costs avoided by being able to produce parts at a quicker and more efficient pace.

  11. Kondo Effect in 3d-host Ferromagnetic Sm1-xCexMn2Ge2

    SciTech Connect (OSTI)

    Liang,G.; Yao, Q.; Xi, H.; Mochizuki, K.; Markert, J.; Croft, M.

    2006-01-01

    Lattice, Ce L{sub 3}-edge, magnetic susceptibility, and electrical resistivity results on polycrystalline Sm{sub 1-x}Ce{sub x}Mn{sub 2}Ge{sub 2} (0 {<=} x {<=} 1) compound series are presented. The lattice parameters a and c increase almost linearly with the increase of Ce concentration x. The Ce-L{sub 3} X-ray absorption spectra indicate that the Ce in this series is nearly trivalent, and Ce valence decreases slightly with the increase of Ce concentration x. Magnetic susceptibility results indicate that the antiferromagnetic (AF) phase in the re-entrant ferromagnetic compound, SmMn{sub 2}Ge{sub 2}, is completely destroyed by merely 1.1% Ce for Sm substitution. For x > 0.011, only ferromagnetic (FM) phases exist below room temperature. It is found that in these materials Ce Kondo scattering coexists with the 3d-host FM fields and is also effectively weakened by such fields.

  12. DEGRADATION OF SM2ZR2O7 THERMAL BARRIER COATING CAUSED BY CALCIUM-MAGNESIUM-ALUMINUM-SILICON OXIDE (CMAS) DEPOSITION

    SciTech Connect (OSTI)

    Wang, Honglong; Sheng, Zhizhi; Tarwater, Emily; Zhang, Xingxing; Dasgupta, Sudip; Fergus, Jeffrey

    2015-03-16

    Rare earth zirconates are promising materials for use as thermal barrier coatings in gas turbine engines. Among the lanthanide zirconate materials, Sm2Zr2O7 with the pyrochlore structure has lower thermal conductivity and better corrosion resistance against calcium-magnesium-aluminum-silicon oxide (CMAS). In this work, after reaction with CMAS, the pyrochlore structure transforms to the cubic fluorite structure and Ca2Sm8(SiO4)6O2 forms in elongated grain.

  13. (n,2n) and (n,3n) cross sections of neutron-induced reactions on 150Sm for En from threshold to 35 MeV

    SciTech Connect (OSTI)

    Dashdorj, D; Mitchell, G; Kawano, T; Becker, J; Wu, C; Devlin, M; Fotiades, N; Nelson, R; Kunieda, S

    2009-03-16

    Cross-section measurements were made of prompt discrete {gamma}-ray production as a function of incident neutron energy (E{sub n} = 1 to 35 MeV) on a {sup 150}Sm sample fo 1550 mg/cm{sup 2} of Sm{sub 2}O{sub 3} enriched to 95.6% in {sup 150}Sm. Results are compared with enhanced Hauser-Feshbach model calculations including the pre-equilibrium reactions. Energetic neutrons were delivered by the Los Alamos Neutron Science Center facility. The prompt-reaction {gamma} rays were detected with the Compton-suppressed Germanium Array for Neutron Induced Excitations (GEANIE). Incident neutron energies were determined by the time-of-flight technique. Excitation functions for thirteen individual {gamma}-rays up to E{sub x} = 0.8 MeV in {sup 149}Sm and one {gamma}-ray transition between the first excited and ground state in {sup 148}Sm were measured. Partial {gamma}-ray cross sections were calculated using GNASH, an enhanced Hauser-Feshbach statistical nuclear reaction model code, and compared with the experimental results. The particle transmission coefficients were calculated with new systematic 'global' optical model potential parameters. The coupled-channel optical model based on the soft rotor model was employed to calculate the particle transmission coefficients. The pre-equilibrium part of the spin distribution in {sup 150}Sm was calculated using the quantum mechanical theory of Feshbach, Kerman, and Koonin (FKK) and incorporated into the GNASH reaction model code. the partial cross sections for discrete {gamma}-ray cascade paths leading to the ground state in {sup 149}Sm and {sup 148}Sm have been summed (without double counting) to estimate lower limits for reaction cross sections. These lower limits are combined with Hauser-Feshbach model calculations to deduce the reaction channel cross sections. These reaction channel cross sections agree with previously measured experimental and ENDF/B-VII evaluations.

  14. Hydrothermal synthesis and afterglow luminescence properties of hollow SnO{sub 2}:Sm{sup 3+},Zr{sup 4+} spheres for potential application in drug delivery

    SciTech Connect (OSTI)

    Feng, Pengfei; Zhang, Jiachi Qin, Qingsong; Hu, Rui; Wang, Yuhua

    2014-02-01

    Highlights: We designed a novel afterglow labeling material SnO{sub 2}:Sm{sup 3+},Zr{sup 4+} for the first time. Hollow SnO{sub 2}:Sm{sup 3+},Zr{sup 4+} spheres with afterglow were prepared by hydrothermal method. Hollow SnO{sub 2}:Sm{sup 3+},Zr{sup 4+} is a potential afterglow labeling medium for drug delivery. - Abstract: A novel afterglow labeling material SnO{sub 2}:Sm{sup 3+},Zr{sup 4+} with hollow sphere shape and intense afterglow luminescence is prepared by hydrothermal method at 180 C for the first time. The morphology and the sphere growth process of this material are investigated by scanning electron microscopy in detail. The afterglow measurement shows that this hydrothermal obtained material exhibits obvious red afterglow luminescence (550700 nm) of Sm{sup 3+} which can last for 542 s (0.32 mcd/m{sup 2}). The depth of traps in this hydrothermal obtained material is calculated to be as shallow as 0.58 eV. The results demonstrate that although it is necessary to further improve the afterglow performance of the hydrothermal derived hollow SnO{sub 2}:Sm{sup 3+},Zr{sup 4+} spheres, it still can be regarded as a potential afterglow labeling medium for drug delivery.

  15. A Linear trans -Bis(imido) Neptunium(V) Actinyl Analog: NpV (NDipp)2 ( tBu2 bipy)2Cl (Dipp = 2,6- i Pr2C6H3)

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Brown, Jessie L.; Batista, Enrique R.; Boncella, James M.; Gaunt, Andrew J.; Reilly, Sean D.; Scott, Brian L.; Tomson, Neil C.

    2015-07-22

    We present the discovery that imido analogs of actinyl dioxo cations can be extended beyond uranium into the transuranic elements. Synthesis of the Np(V) complex, Np(NDipp)2(tBu2bipy)2Cl (1), is achieved through treatment of a Np(IV) precursor with a bipyridine co-ligand and lithium-amide reagent. Complex 1 has been structurally characterized, analyzed by 1H NMR and UV/vis/NIR spectroscopies, and the electronic structure evaluated by DFT calculations.

  16. Surface state reconstruction in ion-damaged SmB6

    SciTech Connect (OSTI)

    Wakeham, N.; Wang, Y. Q.; Fisk, Z.; Ronning, F.; Thompson, J. D.

    2015-02-12

    We have used ion-irradiation to damage the (001) surfaces of SmB? single crystals to varying depths, and have measured the resistivity as a function of temperature for each depth of damage. We observe a reduction in the residual resistivity with increasing depth of damage. Our data are consistent with a model in which the surface state is not destroyed by the ion-irradiation, however instead the damaged layer is poorly conducting and the initial surface state is reconstructed below the damage. This behavior is consistent with a surface state that is topologically protected.

  17. Static electric dipole polarizabilities of An{sup 5+/6+} and AnO{sub 2}{sup +/2+} (An = U, Np, and Pu) ions

    SciTech Connect (OSTI)

    Parmar, Payal E-mail: kipeters@wsu.edu Peterson, Kirk A. E-mail: kipeters@wsu.edu; Clark, Aurora E. E-mail: kipeters@wsu.edu

    2014-12-21

    The parallel components of static electric dipole polarizabilities have been calculated for the lowest lying spin-orbit states of the penta- and hexavalent oxidation states of the actinides (An) U, Np, and Pu, in both their atomic and molecular diyl ion forms (An{sup 5+/6+} and AnO{sub 2}{sup +/2+}) using the numerical finite-field technique within a four-component relativistic framework. The four-component Dirac-Hartree-Fock method formed the reference for MP2 and CCSD(T) calculations, while multireference Fock space coupled-cluster (FSCC), intermediate Hamiltonian Fock space coupled-cluster (IH-FSCC) and Kramers restricted configuration interaction (KRCI) methods were used to incorporate additional electron correlation. It is observed that electron correlation has significant (?5 a.u.{sup 3}) impact upon the parallel component of the polarizabilities of the diyls. To the best of our knowledge, these quantities have not been previously reported and they can serve as reference values in the determination of various electronic and response properties (for example intermolecular forces, optical properties, etc.) relevant to the nuclear fuel cycle and material science applications. The highest quality numbers for the parallel components (?{sub zz}) of the polarizability for the lowest ? levels corresponding to the ground electronic states are (in a.u.{sup 3}) 44.15 and 41.17 for UO{sub 2}{sup +} and UO{sub 2}{sup 2+}, respectively, 45.64 and 41.42 for NpO{sub 2}{sup +} and NpO{sub 2}{sup 2+}, respectively, and 47.15 for the PuO{sub 2}{sup +} ion.

  18. THE EFFECT OF THE {sup 14}N(p, {gamma}){sup 15}O REACTION ON THE BLUE LOOPS IN INTERMEDIATE-MASS STARS

    SciTech Connect (OSTI)

    Halabi, Ghina M.; El Eid, Mounib F.; Champagne, Arthur

    2012-12-10

    We present stellar evolutionary sequences of stars in the mass range 5-12 M{sub Sun }, having solar-like initial composition. The stellar models are obtained using updated input physics, including recent rates of thermonuclear reactions. We investigate the effects of a modification of the {sup 14}N(p, {gamma}){sup 15}O reaction rate, as suggested by recent evaluations, on the formation and extension of the blue loops encountered during the evolution of the stars in the above mass range. We find that a reduced {sup 14}N(p, {gamma}){sup 15}O rate, as described in the text, has a striking impact on the physical conditions of burning and mixing during shell hydrogen burning when the blue loops are formed. In particular, we find that the efficiency of shell hydrogen burning is crucial for the formation of an extended blue loop. We show that a significantly reduced {sup 14}N(p, {gamma}){sup 15}O rate affects severely the extension of the blue loops and the time spent by the star in the blue part of the Hertzsprung-Russell diagram in the mass range 5-7 M{sub Sun} if the treatment of convection is based on the Schwarzschild criterion only. In this case, envelope overshooting helps to restore well-extended blue loops as supported by the observations of the Cepheid stars. If core overshooting is included during the core hydrogen and core helium burning phases, the loop formation and its properties depend on how this overshooting is treated for a given stellar mass range, as well as on its efficiency.

  19. Synthesis, properties and phase transitions of pyrochlore- and fluorite-like Ln{sub 2}RMO{sub 7} (Ln = Sm, Ho; R = Lu, Sc; M = Nb, Ta)

    SciTech Connect (OSTI)

    Shlyakhtina, A.V.; Belov, D.A.; Pigalskiy, K.S.; Shchegolikhin, A.N.; Kolbanev, I.V.; Karyagina, O.K.

    2014-01-01

    Graphical abstract: Temperature dependences of bulk conductivity for Sm{sub 2}ScTaO{sub 7} pyrochlore prepared at (1) 1400 °C, 20 h; and (2) 1200 °C, 40 h. - Highlights: • The phase formation of Ln{sub 2}RMO{sub 7} (Ln = Sm, Ho; R = Lu, Sc; M = Nb, Ta) at 1200–1600 °C. • The bulk conductivity and magnetic susceptibility were measured. • The bulk conductivity of Sm{sub 2}ScTaO{sub 7} has oxygen ion type at T ≥ 750 °C. • The first-order structural phase transition was observed in Sm{sub 2}ScTaO{sub 7} at ∼650–700 °C. • This phase transformation is not typical for defect fluorites. - Abstract: We have studied the new compounds with fluorite-like (Ho{sub 2}RNbO{sub 7} (R = Lu, Sc)) and pyrochlore-like (Sm{sub 2}ScTaO{sub 7}) structure as potential oxide ion conductors. The phase formation process (from 1200 to 1600 °C) and physical properties (electrical, thermo mechanical, and magnetic) for these compounds were investigated. Among the niobate materials the highest bulk conductivity is offered by the fluorite-like Ho{sub 2}ScNbO{sub 7} synthesized at 1600 °C: 3.8 × 10{sup −5} S/cm at 750 °C, whereas in Sm system the highest bulk conductivity, 7.3 × 10{sup −6} S/cm at 750 °C, is offered by the pyrochlore Sm{sub 2}ScTaO{sub 7} synthesized at 1400 °C. In Sm{sub 2}ScTaO{sub 7} pyrochlore we have observed the first-order phase transformation at ∼650–700 °C is related to rearrangement process in the oxygen sublattice of the pyrochlore structure containing B-site cations in different valence state and actually is absent in the defect fluorites. The two holmium niobates show Curie–Weiss paramagnetic behavior, with the prevalence of antiferromagnetic coupling. The magnetic susceptibility of Sm{sub 2}ScTaO{sub 7} is a weak function of temperature, corresponding to Van Vleck paramagnetism.

  20. A measurement of. Delta. sigma. sub L (np), the difference between neutron-proton total cross sections in pure longitudinal spin states

    SciTech Connect (OSTI)

    Beddo, M.E.

    1990-10-01

    A measurement off {Delta}{sigma}{sub L}(np), the difference between neutron-proton total cross sections in pure longitudinal spin states, is described. The results will help determine the isospin-zero (I = 0) scattering amplitudes, which are not well known above laboratory energies of 500 MeV, whereas the isospin-one (I = 1) amplitudes are fairly well-determined to 1 GeV. Data points were taken at the Los Alamos Meson Physics Facility (LAMPF) at Los Alamos, New Mexico, for five neutron beam energies: 484, 568, 634,720 and 788 MeV; they are the first in this energy range. Polarized neutrons were produced by charge-exchange of polarized protons on a liquid deuterium target (LD{sub 2}). Large-volume neutron counters detected the neutrons that passed through a polarized proton target. The counters subtended a range of solid angles large enough to allow extrapolation of the scattered neutrons to 0{degree}. Two modifications to the LAMPF accelerator system which were made for this work are described. They included a beam buncher,'' which modified the normal rf-time structure of the proton beam and allowed for the selection of peak-energy neutrons by time-of-flight means, and a computerized beam steering program, which reduced systematic effects due to beam motion at the LD{sub 2} target. The experimental values of {Delta}{sigma}{sub L}(np) are found to be consistent with other np data, including preliminary data from SIN and Saclay, but not with some results from Argonne which used a polarized proton beam and a polarized deuteron target. The I = 0 component was extracted from {Delta}{sigma}{sub L}(np) using existing pp data (I = 1), with the unexpected result that {Delta}{sigma}{sub L}(I = 0) was found to be essentially identical in shape to {Delta}{sigma}{sub L}(I = 1). The significance of this is not yet understood.

  1. Hydrogen passivation of nitrogen in GaNAs and GaNP alloys: How many H atoms are required for each N atom?

    SciTech Connect (OSTI)

    Buyanova, I. A.; Chen, W. M.; Izadifard, M.; Pearton, S. J.; Bihler, C.; Brandt, M. S.; Hong, Y. G.; Tu, C. W.

    2007-01-08

    Secondary ion mass spectrometry and photoluminescence are employed to evaluate the origin and efficiency of hydrogen passivation of nitrogen in GaNAs and GaNP. The hydrogen profiles are found to closely follow the N distributions, providing unambiguous evidence for their preferential binding as the dominant mechanism for neutralization of N-induced modifications in the electronic structure of the materials. Though the exact number of H atoms involved in passivation may depend on the conditions of the H treatment and the host matrixes, it is generally found that more than three H atoms are required to bind to a N atom to achieve full passivation for both alloys.

  2. Warm white light emitting ThO{sub 2}:Sm{sup 3+} nanorods: Cationic surfactant assisted reverse micellar synthesis and Photoluminescence properties

    SciTech Connect (OSTI)

    Gupta, Santosh K.; Gupta, Ruma; Natarajan, V.; Godbole, S.V.

    2014-01-01

    Graphical abstract: - Highlights: • ThO{sub 2}:Sm{sup 3+} nanoparticles have been synthesized using cationic surfactant assisted reverse micellar route. • HRTEM shows the formation of thoria nanorods. • Photoluminescence investigation shows host as well as samarium ion emission. • Time resolved fluorescence spectroscopy shows the presence of two types of samarium ion in thoria host. - Abstract: Sm{sup 3+} activated thorium oxide nanorods were synthesized by cationic surfactant assisted reverse micellar route. Phase purity, morphological and luminescent properties were investigated by X-ray diffraction, high resolution transmission electron microscopy and photoluminescence spectroscopy. Upon UV light excitation (245 nm), ThO{sub 2}:Sm{sup 3+} exhibited host emission at 447 nm, along with characteristic emission lines of Sm{sup 3+} at 569, 609, 662 and 716 nm. Lifetime spectroscopy shows the presence of two types of Sm{sup 3+} (τ = 1.1 ms and 4.9 ms) with different asymmetric ratios.

  3. Pre-Conceptual Design of a Fluoride-Salt-Cooled Small Modular Advanced High Temperature Reactor (SmAHTR)

    SciTech Connect (OSTI)

    Greene, Sherrell R; Gehin, Jess C; Holcomb, David Eugene; Carbajo, Juan J; Ilas, Dan; Cisneros, Anselmo T; Varma, Venugopal Koikal; Corwin, William R; Wilson, Dane F; Yoder Jr, Graydon L; Qualls, A L; Peretz, Fred J; Flanagan, George F; Clayton, Dwight A; Bradley, Eric Craig; Bell, Gary L; Hunn, John D; Pappano, Peter J; Cetiner, Sacit M

    2011-02-01

    This document presents the results of a study conducted at Oak Ridge National Laboratory during 2010 to explore the feasibility of small modular fluoride salt-cooled high temperature reactors (FHRs). A preliminary reactor system concept, SmATHR (for Small modular Advanced High Temperature Reactor) is described, along with an integrated high-temperature thermal energy storage or salt vault system. The SmAHTR is a 125 MWt, integral primary, liquid salt cooled, coated particle-graphite fueled, low-pressure system operating at 700 C. The system employs passive decay heat removal and two-out-of-three , 50% capacity, subsystem redundancy for critical functions. The reactor vessel is sufficiently small to be transportable on standard commercial tractor-trailer transport vehicles. Initial transient analyses indicated the transition from normal reactor operations to passive decay heat removal is accomplished in a manner that preserves robust safety margins at all times during the transient. Numerous trade studies and trade-space considerations are discussed, along with the resultant initial system concept. The current concept is not optimized. Work remains to more completely define the overall system with particular emphasis on refining the final fuel/core configuration, salt vault configuration, and integrated system dynamics and safety behavior.

  4. HETEROGENEOUS ISOTOPIC ANOMALIES OF SM AND GD IN THE NORTON COUNTY METEORITE: EVIDENCE FOR IRRADIATION FROM THE ACTIVE EARLY SUN

    SciTech Connect (OSTI)

    Hidaka, Hiroshi; Kondo, Tomoyo; Yoneda, Shigekazu

    2012-02-20

    Large and heterogeneous isotopic variations of {sup 150}Sm/{sup 149}Sm and {sup 158}Gd/{sup 157}Gd due to neutron capture reactions caused by cosmic-ray irradiation were found in chemical and mineral separates from the Norton County meteorite. The light-colored separates, consisting mainly of enstatite (Mg{sub 2}Si{sub 2}O{sub 6}), have a very large neutron fluence of 1.98 Multiplication-Sign 10{sup 17} n cm{sup -2}, which is 10 times higher than that of the whole rock. Furthermore, four chemical separates showed a large variation in neutron fluences, ranging from 1.82 Multiplication-Sign 10{sup 16} to 1.87 Multiplication-Sign 10{sup 17} n cm{sup -2}. The variable amounts of neutron fluences from a small single fragment of the Norton County meteorite cannot be simply explained by single-stage cosmic-ray irradiation in space. Rare earth element (REE) analyses revealed that the fractions with high neutron fluences have similar chemical properties to those in the early condensates in the solar system, showing depletions of Eu and Yb in their REE abundance patterns. The data provide evidence for an activity of the early Sun (T Tauri), suggesting the migration of early and intense irradiation materials into the Norton County meteorite's parent body.

  5. Preliminary laboratory study of plutonium-238 dissolution from Mound soil by means of the ACT*DE*CON{sup SM} process

    SciTech Connect (OSTI)

    Brown, K.A.; Heinrich, R.R.; Johnson, D.O.; Edgar, D.E.

    1992-04-01

    The treatment of contaminated soil presents a significant technical problem. Soil-washing and chemical-extraction methods have proven to be effective for specific applications, but a process with more comprehensive treatment properties that is both cost-effective and environmentally propitious is needed. Bradtec, Inc., has developed a process, the ACT*DE*CON{sup SM} process, that has been tested on soil contaminated with plutonium. The process effectively extracted Pu-238 after three washes, reducing the contamination levels from approximately 20 Bq/g to 1.6--1.9 Bq/g and yielding a decontamination factor ranging from 11 to 13. By using four or more ACT*DE*CON{sup SM} washes or a continuous-flow process with ACT*DE*CON{sup SM} solvents on a pilot-scale test, a target decontamination level of 0.93 Bq/g might be achievable.

  6. Preliminary laboratory study of plutonium-238 dissolution from Mound soil by means of the ACT*DE*CON sup SM process

    SciTech Connect (OSTI)

    Brown, K.A.; Heinrich, R.R.; Johnson, D.O.; Edgar, D.E. )

    1992-04-01

    The treatment of contaminated soil presents a significant technical problem. Soil-washing and chemical-extraction methods have proven to be effective for specific applications, but a process with more comprehensive treatment properties that is both cost-effective and environmentally propitious is needed. Bradtec, Inc., has developed a process, the ACT*DE*CON{sup SM} process, that has been tested on soil contaminated with plutonium. The process effectively extracted Pu-238 after three washes, reducing the contamination levels from approximately 20 Bq/g to 1.6--1.9 Bq/g and yielding a decontamination factor ranging from 11 to 13. By using four or more ACT*DE*CON{sup SM} washes or a continuous-flow process with ACT*DE*CON{sup SM} solvents on a pilot-scale test, a target decontamination level of 0.93 Bq/g might be achievable.

  7. Synthesis conditions and some properties of neptunium (IV) oxalates in which C/sub 2/O/sub 4//Np = 2. 5

    SciTech Connect (OSTI)

    Bykhovskii, D.N.; Kuz'mina, M.A.; Maksimov, V.F.; Novikov, G.S.; Smirnov, A.N.; Solntseva, L.V.

    1988-09-01

    A study was made of the formation of neptunium oxalates of the type M/sub 2/Np/sub 2//centered dot/(C/sub 2/O/sub 4/)/sub 5//centered dot/(7-9)H/sub 2/O, where M = H, NH/sub 4/, Na, K. It was found that the acid oxalate may crystallize out together with the normal hexahydrate of neptunium (IV) oxalate over a wide range of conditions, but it may be obtained in almost pure form when the initial neptunium concentration is (1-2)/centered dot/10/sup /minus/2/ M and the nitric acid concentration is above 3 M. Other salts are formed in the same conditions as the analogous thorium and uranium (IV) compounds. An analysis of the diffractograms shows the structural similarity of the acid oxalate to other salts, especially the ammonium salt. The IR spectra of the acid oxalate did not include absorption bands which could be ascribed to the bioxalate ion. The results indicate that the formula for this oxalate should be written in the form (H/sub 3/O)/sub 2/Np/sub 2/(C/sub 2/O/sub 4/)/sub 5//centered dot/7H/sub 2/O.

  8. Change in the magnetic structure of (Bi,Sm)FeO{sub 3} thin films at the morphotropic phase boundary probed by neutron diffraction

    SciTech Connect (OSTI)

    Maruyama, Shingo; Anbusathaiah, Varatharajan; Takeuchi, Ichiro; Fennell, Amy; Enderle, Mechthild; Ratcliff, William D.

    2014-11-01

    We report on the evolution of the magnetic structure of BiFeO{sub 3} thin films grown on SrTiO{sub 3} substrates as a function of Sm doping. We determined the magnetic structure using neutron diffraction. We found that as Sm increases, the magnetic structure evolves from a cycloid to a G-type antiferromagnet at the morphotropic phase boundary, where there is a large piezoelectric response due to an electric-field induced structural transition. The occurrence of the magnetic structural transition at the morphotropic phase boundary offers another route towards room temperature multiferroic devices.

  9. AREVA NP next generation fresh UO{sub 2} fuel assembly shipping cask: SCALE - CRISTAL comparisons lead to safety criticality confidence

    SciTech Connect (OSTI)

    Doucet, M.; Landrieu, M.; Montgomery, R.; O' Donnell, B.

    2007-07-01

    AREVA NP as a worldwide PWR fuel provider has to have a fleet of fresh UO{sub 2} shipping casks being agreed within a lot of countries including USA, France, Germany, Belgium, Sweden, China, and South Africa - and to accommodate foreseen EPR Nuclear Power Plants fuel buildings. To reach this target the AREVA NP Fuel Sector decided to develop an up-to-date shipping cask (so called MAP project) gathering experience feedback of the today fleet and an improved safety allowing the design to comply with international regulations (NRC and IAEA) and local Safety Authorities. Based on pre design features a safety case was set up to highlight safety margins. Criticality hypothetical accidental assumptions were defined: - Preferential flooding; - Fuel rod lattice pitch expansion for full length of fuel assemblies; - Neutron absorber penalty; -... Well known computer codes, American SCALE package and French CRISTAL package, were used to check configurations reactivity and to ensure that both codes lead to coherent results. Basic spectral calculations are based on similar algorithms with specific microscopic cross sections ENDF/BV for SCALE and JEF2.2 for CRISTAL. The main differences between the two packages is on one hand SCALE's three dimensional fuel assembly geometry is described by a pin by pin model while an homogenized fuel assembly description is used by CRISTAL and on the other hand SCALE is working with either 44 or 238 neutron energy groups while CRISTAL is with a 172 neutron energy groups. Those two computer packages rely on a wide validation process helping defining uncertainties as required by regulations in force. The shipping cask with two fuel assemblies is designed to maximize fuel isolation inside a cask and with neighboring ones even for large array configuration cases. Proven industrial products are used: - Boral{sup TM} as neutron absorber; - High density polyethylene (HDPE) or Nylon as neutron moderator; - Foam as thermal and mechanical protection. The

  10. Study of the R-(Zr,W)-(O,N) (R = Y, Nd, Sm, Gd, Yb) oxynitride system

    SciTech Connect (OSTI)

    Tessier, Franck; Maillard, Pascal; Orhan, Emmanuelle; Chevire, Francois

    2010-02-15

    The replacement of tantalum by the couple Zr/W within the RTa-O-N systems (R = Y, Nd, Sm, Gd, Yb), enables the preparation of novel oxide and oxynitride phases in the R-Zr-W-O-N system. R{sub 2}Zr{sub 2-x}W{sub x}O{sub 7+x} oxides exhibit the fluorite-type (x < 0.9) and scheelite (x {approx} 1) structures. Corresponding oxynitride compositions are of the fluorite-type and show different colors, for example in the case of ytterbium: pale yellow (x = 0.2 or 0.25), green (x = 0.5-0.8) and brown for the tungsten-rich samples (x = 0.9, 1). Photocatalytic activity measurements have been performed to investigate the overall water splitting behavior of these colored phases.

  11. Theoretical studies of strongly correlated rare-earth intermetallics RIn₃ and RSn₃ (R=Sm, Eu, and Gd)

    SciTech Connect (OSTI)

    Shafiq, M.; Ahmad, Iftikhar E-mail: dr.iftikhar@uom.edu.pk; Jalali Asadabadi, S.

    2014-09-14

    In this paper, the structural, elastic, and electronic properties of RIn₃ and RSn₃ (R = Sm, Eu, Gd) compounds have been investigated using the full potential linearized augmented plane wave plus local orbital method within the density functional theory. The structural properties are investigated using the LDA, GGA, and the band correlated LDA+U and GGA+U schemes. The lattice parameters are in good agreement with the available experimental results and the divalent state of Eu is also verified. The spin-orbit coupling is included in order to predict the correct electronic properties and splitting of 4f states of the rare earth elements is also incorporated. We calculated Bulk modulus, shear modulus, Young's modulus, anisotropic ratio, Kleinman parameters, Poisson's ratio, Lame's co-efficient, sound velocities for shear and longitudinal waves, and Debye temperature. We also predict the Cauchy pressure and B/G ratio in order to explore the ductile and brittle behaviors of these compounds.

  12. Heavy surface state in a possible topological Kondo insulator: Magnetothermoelectric transport on the (011) plane of SmB6

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Luo, Yongkang; Chen, Hua; Dai, Jianhui; Xu, Zhu -an; Thompson, J. D.

    2015-02-25

    Motivated by the high sensitivity to Fermi surface topology and scattering mechanisms in magnetothermoelectric transport, we have measured the thermopower and Nernst effect on the (011) plane of the proposed topological Kondo insulator SmB6. These experiments, together with electrical resistivity and Hall effect measurements, suggest that the (011) plane also harbors a metallic surface with an effective mass on the order of 10–102 m0. The surface and bulk conductances are well distinguished in these measurements and are categorized into metallic and nondegenerate semiconducting regimes, respectively. As a result, electronic correlations play an important role in enhancing scattering and also contributemore » to the heavy surface state.« less

  13. Spectrometric analysis of different fluorophosphate glasses doped with Sm{sup 3+} ions for reddish-orange laser emission

    SciTech Connect (OSTI)

    Babu, S. Balakrishna, A. Ratnakaram, Y. C.

    2014-04-24

    Optical properties of Sm{sup 3+} doped different fluorophosphate glasses have been synthesized and discussed. The J- O intensity parameters Ω{sub λ} (λ= 2, 4, 6) from absorption spectra have been evaluated. No sharp edges are found in the absorption spectra, which confirm amorphous nature of present glass matrices. Various radiative parameters have been obtained from luminescence spectra for excited states to corresponding {sup 4}G{sub 5/2}→{sup 6}H{sub 5/2}, {sup 6}H{sub 7/2}, {sup 6}H{sub 9/2} and {sup 6}H{sub 11/2} transitions. The nature of decay curve analysis was performed for the {sup 4}G{sub 5/2} level. These glasses are expected to give interesting application in field of optical devices.

  14. Activation energy and enthalpy of decomposition for the Fe{sub 17}Sm{sub 2} nitride

    SciTech Connect (OSTI)

    Cabral, F.A.; Gama, S.; Ribeiro, C.A.

    1997-04-01

    Decomposition studies of the Fe{sub 17}Sm{sub 2}N{sub 3} compound were done using a Calvet-type microcalorimeter and a simultaneous gravimetric and differential thermal analyzer (DTA). The results show that the decomposition has onset temperature of 570{degree}C and proceeds up to 900{degree}C, and presents only one well determined exothermic thermal event. The calorimetric measurement shows that the enthalpy associated with the decomposition is 69 kJ/mol. The activation energy of the process was also determined using the Kissinger method applied to the DTA signal. It was observed that there was only one activation energy for the decomposition process, with a value of 339 kJ/mol. {copyright} {ital 1997 American Institute of Physics.}

  15. Thermodynamic and transport properties of single crystalline RCo2Ge2 (R=Y, LaNd, SmTm)

    SciTech Connect (OSTI)

    Kong, Tai; Cunningham, Charles E.; Taufour, Valentin; Budko, Sergey L.; Buffon, Malinda L.C.; Lin, Xiao; Emmons, Heather; Canfield, Paul C.

    2014-05-01

    Single crystals of RCo2Ge2 (R=Y, LaNd, SmTm) were grown using a self-flux method and were characterized by room-temperature powder X-ray diffraction; anisotropic, temperature and field dependent magnetization; temperature and field dependent, in-plane resistivity; and specific heat measurements. In this series, the majority of the moment-bearing members order antiferromagnetically; YCo2Ge2 and LaCo2Ge2 are non-moment-bearing. Ce is trivalent in CeCo2Ge2 at high temperatures, and exhibits an enhanced electronic specific heat coefficient due to the Kondo effect at low temperatures. In addition, CeCo2Ge2 shows two low-temperature anomalies in temperature-dependent magnetization and specific heat measurements. Three members (R=TbHo) have multiple phase transitions above 1.8 K. Eu appears to be divalent with total angular momentum L =0. Both EuCo2Ge2 and GdCo2Ge2 manifest essentially isotropic paramagnetic properties consistent with J =S =7/2. Clear magnetic anisotropy for rare-earth members with finite L was observed, with ErCo2Ge2 and TmCo2Ge2 manifesting planar anisotropy and the rest members manifesting axial anisotropy. The experimentally estimated crystal electric field (CEF) parameters B 20 were calculated from the anisotropic paramagnetic ? ab and ? c values and follow a trend that agrees well with theoretical predictions. The ordering temperatures, TNTN, as well as the polycrystalline averaged paramagnetic CurieWeiss temperature, ?avg, for the heavy rare-earth members deviate from the de Gennes scaling, as the magnitude of both is the highest for Tb, which is sometimes seen for extremely axial systems. Except for SmCo2Ge2, metamagnetic transitions were observed at 1.8 K for all members that ordered antiferromagnetically.

  16. Structural and magnetic properties of Sm{sub 2?x}Mn{sub x}O{sub 3} nanoparticles

    SciTech Connect (OSTI)

    Heiba, Zein K.; Mohamed, Mohamed Bakr; Fuess, H.

    2013-10-15

    Graphical abstract: - Highlights: C-type Sm{sub 2?x}Mn{sub x}O{sub 3} (0.0 ? x ?0.20) is prepared by solgel method. A maximum solubility of x = 0.15 is confirmed by X-ray diffraction, Raman and infrared techniques. Samples with x > 0.05 exhibit weak ferromagnetic properties; for x ? 0.05 antiferromagnetic behaviors is obtained. Correlation between magnetic behaviors and structural and microstructural parameters is discussed. - Abstract: Mixed oxide Sm{sub 2?x}Mn{sub x}O{sub 3} (SMO), x = 0.0, 0.05, 0.10, 0.15 and 0.20 were synthesized by a solgel process. A single phase solid solution is formed up to x = 0.15 which confirmed by using X-ray diffraction, Raman spectroscopy and infrared techniques. Crystal structure and microstructure analyses were performed by Rietveld refinement. Preferential cationic distribution, over the two crystallographic sites 8b and 24d of space group Ia3{sup }, is found for doped samples but with different extent. The r.m.s. microstrain ??{sub L}{sup 2}?{sup 1/2} depends on composition x in a systematic way emphasizing the preferential distribution. Magnetization measurements show that samples with x ? 0.05 have antiferromagnetic behavior, while samples with x > 0.05 exhibit a weak ferromagnetic behavior with magnetic phase transformation at 15 and 16 K for x = 0.1 and x = 0.15, respectively.

  17. Crystal structure of high-Zr inclusions in an alloy containing U, Pu, Np, Am, Zr and rare-earth elements

    SciTech Connect (OSTI)

    Dawn E. Janney; James W. Madden; J. Rory Kennedy; Thomas P. O'Holleran

    2014-05-01

    Researchers commonly observe high-Zr inclusions in actinide-Zr alloys. As there is very little published data on the crystal structures of these inclusions, it has generally been assumed that the inclusions were impurity-stabilized a-Zr. However, new electron-diffraction data from two high-Zr inclusions in an alloy containing U, Pu, Np, Am, Zr, and rare-earth elements show that these inclusions are not a-Zr (which has a hexagonal structure) but instead have a face-centered cubic structure. This data is unique in that it combines single-crystal diffraction patterns and microchemical analyses from individual inclusions. More data on other high-Zr inclusions is clearly required. However, the present results suggest that caution is needed in assuming that all high-Zr inclusions in actinide-Zr alloys are a-Zr.

  18. Measurements of delayed neutron decay constants and fission yields from {sup 235}U, {sup 237}Np, {sup 241}Am, and {sup 243}Am

    SciTech Connect (OSTI)

    Saleh, H.H.; Parish, T.A.; Raman, S.; Shinohara, Nobuo

    1997-01-01

    Isotopes of the higher actinide elements are produced as a result of successive radiative capture reactions in the uranium fuel of nuclear reactors. Typically, these transuranic isotopes decay through long chains, have long half-lives, and dominate the long-term toxicity of spent reactor fuel. One of the options for high level waste management is to remove the higher actinide elements from spent fuel by chemical processing, to load them into new special fuel elements, and to transmute them by neutron-induced fission into shorter-lived fission fragments. Reactors designed to achieve high actinide fission (transmutation) rates are called actinide burners. In such reactors, the actinide wastes would constitute much of the fissionable fuel. Due to the high transuranic isotope loadings in the fuel of actinide burners, the neutronic properties of the higher actinide isotopes will have a significant effect on the criticality and safety characteristics of such reactors. While there is an extensive operational database for reactors fueled with uranium and plutonium, operating experience with fuel containing large amounts of actinide wastes is quite limited. Two important neutronic properties of actinide burner cores are their reactivity and their delayed neutron fraction. Both of these properties will be strongly influenced by the neutronic characteristics of the actinide waste isotopes. Here, delayed neutron yields and decay constants for {sup 235}U, {sup 237}Np, {sup 241}Am, and {sup 243}Am were measured at the Texas A and M University TRIGA reactor using a fast pneumatic transfer system. The detection system consisted of an array of BF{sub 3} proportional counters embedded in a polyethylene cylinder. The measured values of the total delayed neutron yield per 100 fissions from thermal neutron-induced fission of {sup 235}U, {sup 237}Np, {sup 241}Am, and {sup 243}Am were determined to be 1.59 {+-} 0.04, 1.29 {+-} 0.04, 0.49 {+-} 0.02, and 0.84 {+-} 0.04, respectively.

  19. Measurement of the {sup 237}Np(n,{gamma}) cross section from 20 meV to 500 keV with a high efficiency, highly segmented 4{pi} BaF{sub 2} detector

    SciTech Connect (OSTI)

    Esch, E.-I.; Bond, E. M.; Bredeweg, T. A.; Couture, A.; Glover, S. E.; Haight, R. C.; Jandel, M.; Kawano, T.; Mertz, A.; O'Donnell, J. M.; Rundberg, R. S.; Schwantes, J. M.; Ullmann, J. L.; Vieira, D. J.; Wilhelmy, J. B.; Wouters, J. M.; Reifarth, R.; Greife, U.; Hatarik, A. M.; Hatarik, R.

    2008-03-15

    The {sup 237}Np(n,{gamma}){sup 238}Np cross section has been measured in the neutron energy range from 20 meV to 500 keV using the DANCE array at the Los Alamos National Laboratory. This new facility allows experiments with submilligram samples and is therefore well suited to investigate isotopes with half-lives as low as a few hundred days. In this benchmark measurement, only 0.42 mg of {sup 237}Np was sufficient to determine differential cross sections relative to the well-known resonance at 0.5 eV. The thermal cross section was measured to {sigma}{sub 2200m/s}=177{+-}5 barn, {sigma}{sub kT=25.3meV}=167{+-}4 barn and the resonance integral to RI=693{+-}6 barn.

  20. La-Ce and Sm-Nd systematics of siliceous sedimentary rocks: A clue to marine environment in their deposition

    SciTech Connect (OSTI)

    Hiroshi Shimizu; Masayo Amano; Akimasa Masuda )

    1991-04-01

    La-Ce isotopic data, together with Sm-Nd isotopic data, were determined on siliceous sedimentary rocks (cherts) in order to elucidate the rare earth element (REE) character of their sources and the nature of their depositional environments. The cherts studied are a late Archean chert from the Gorge Creek Group in the Pilbara block of Western Australia, Triassic cherts from central Japan, and Cretaceous and Paleogene deep-sea cherts from the central Pacific and the Caribbean Sea. The Archean chert from the Gorge Creek Group shows chondritic Ce and Nd isotope ratios at its sedimentation age which indicate that its sources had a time-integrated chondritic REE pattern. Triassic cherts from Japan have initial Ce and Nd isotope ratios that show a direct derivation from their continental source. On the other hand, for Cretaceous and Paleogene deep-sea cherts having negative Ce anomalies in their REE patterns, two different sources for Ce and Nd are revealed from their initial Ce and Nd isotope data: Ce from long-term light-REE-depleted oceanic volcanic rocks and Nd from light-REE-enriched continental rocks. The reverse nature observed for deep-sea cherts is considered to be a reflection of their depositional environment far from a continent. These results confirm that the La-Ce isotope system is highly useful in determining the nature and cause of Ce anomalies observed in marine sedimentary rocks such as chert.

  1. Real-Space Microscopic Electrical Imaging of n+-p Junction Beneath Front-Side Ag Contact of Multicrystalline Si Solar Cells

    SciTech Connect (OSTI)

    Jiang, C. S.; Li, Z. G.; Moutinho, H. R.; Liang, L.; Ionkin, A.; Al-Jassim, M. M.

    2012-04-15

    We investigated the quality of the n+-p diffused junction beneath the front-side Ag contact of multicrystalline Si solar cells by characterizing the uniformities of electrostatic potential and doping concentration across the junction using the atomic force microscopy-based electrical imaging techniques of scanning Kelvin probe force microscopy and scanning capacitance microscopy. We found that Ag screen-printing metallization fired at the over-fire temperature significantly degrades the junction uniformity beneath the Ag contact grid, whereas metallization at the optimal- and under-fire temperatures does not cause degradation. Ag crystallites with widely distributed sizes were found at the Ag-grid/emitter-Si interface of the over-fired cell, which is associated with the junction damage beneath the Ag grid. Large crystallites protrude into Si deeper than the junction depth. However, the junction was not broken down; instead, it was reformed on the entire front of the crystallite/Si interface. We propose a mechanism of junction-quality degradation, based on emitter Si melting at the temperature around the Ag-Si eutectic point during firing, and subsequent re-crystallization with incorporation of Ag and other impurities and with formation of crystallographic defects during quenching. The effect of this junction damage on solar cell performance is discussed.

  2. A Thermodynamic Model for Acetate, Lactate, and Oxalate Complexation with Am(III), Th(IV), Np(V), and U(VI) Valid to High Ionic Strength

    SciTech Connect (OSTI)

    Bynaum, R.V.; Free, S.J.; Moore, R.C.

    1999-01-15

    The organic ligands acetate, lactate, oxalate and EDTA have been identified as components of wastes targeted for disposal in the Waste Isolation Pilot Plant (WIPP) located in Southeastern New Mexico. The presence of these ligands is of concern because complexation of the actinides with the ligands may increase dissolved actinide concentrations and impact chemical retardation during transport. The current work considers the complexation of Am(III), Th (IV), Np(V), and U(W) with two of the organic ligands, acetate and lactate, in NaCl media from dilute through high concentration. A thermodynamic model for actinide complexation with the organic ligands has been developed based on the Pitzer activity coefficient formalism and the Harvie-Moller-Weare, Felmy-Weare database for describing brine evaporite systems. The model was parameterized using first apparent stability constant data from the literature. Because of complexation of other metal ions (Fe, Mg, Ni, Pb, etc.) present in the WIPP disposal room with the organic ligands, preliminary results from model calculations indicate the organic ligands do not significantly increase dissolved actinide concentrations.

  3. Structure and magnetic properties of RE{sub 2}CuIn{sub 3} (RE=Ce, Pr, Nd, Sm and Gd)

    SciTech Connect (OSTI)

    Tyvanchuk, Yuriy B. Szytula, Andrzej; Zarzycki, Arkadiusz; Rodewald, Ute Ch.; Kalychak, Yaroslav M.; Poettgen, Rainer

    2008-12-15

    The ternary copper indides RE{sub 2}CuIn{sub 3}{identical_to}RECu{sub 0.5}In{sub 1.5} (RE=Ce, Pr, Nd, Sm and Gd) were synthesized from the elements in sealed tantalum tubes in an induction furnace. They crystallize with the CaIn{sub 2}-type structure, space group P6{sub 3}/mmc, with a statistical occupancy of copper and indium on the tetrahedral substructure. These indides show homogeneity ranges RECu{sub x}In{sub 2-x}. Single crystal structure refinements were performed for five crystals: CeCu{sub 0.66}In{sub 1.34} (a=479.90(7) pm, c=768.12(15) pm), PrCu{sub 0.52}In{sub 1.48} (a=480.23(7) pm, c=759.23(15) pm), NdCu{sub 0.53}In{sub 1.47} (a=477.51(7) pm, c=756.37(15) pm), SmCu{sub 0.46}In{sub 1.54} (a=475.31(7) pm, c=744.77(15) pm), and GdCu{sub 0.33}In{sub 1.67} (a=474.19(7), c=737.67(15) pm). Temperature-dependent susceptibility measurements show antiferromagnetic ordering at T{sub N}=4.7 K for Pr{sub 2}CuIn{sub 3} and Nd{sub 2}CuIn{sub 3} and 15 K for Sm{sub 2}CuIn{sub 3}. Fitting of the susceptibility data of the samarium compound revealed an energy gap {delta}E=39.7(7) K between the ground and the first excited levels. - Graphical abstract: The CaIn{sub 2}-type structure of Sm{sub 2}CuIn{sub 3}.

  4. Labeled nucleotide phosphate (NP) probes

    DOE Patents [OSTI]

    Korlach, Jonas; Webb, Watt W.; Levene, Michael; Turner, Stephen; Craighead, Harold G.; Foquet, Mathieu

    2009-02-03

    The present invention is directed to a method of sequencing a target nucleic acid molecule having a plurality of bases. In its principle, the temporal order of base additions during the polymerization reaction is measured on a molecule of nucleic acid, i.e. the activity of a nucleic acid polymerizing enzyme on the template nucleic acid molecule to be sequenced is followed in real time. The sequence is deduced by identifying which base is being incorporated into the growing complementary strand of the target nucleic acid by the catalytic activity of the nucleic acid polymerizing enzyme at each step in the sequence of base additions. A polymerase on the target nucleic acid molecule complex is provided in a position suitable to move along the target nucleic acid molecule and extend the oligonucleotide primer at an active site. A plurality of labelled types of nucleotide analogs are provided proximate to the active site, with each distinguishable type of nucleotide analog being complementary to a different nucleotide in the target nucleic acid sequence. The growing nucleic acid strand is extended by using the polymerase to add a nucleotide analog to the nucleic acid strand at the active site, where the nucleotide analog being added is complementary to the nucleotide of the target nucleic acid at the active site. The nucleotide analog added to the oligonucleotide primer as a result of the polymerizing step is identified. The steps of providing labelled nucleotide analogs, polymerizing the growing nucleic acid strand, and identifying the added nucleotide analog are repeated so that the nucleic acid strand is further extended and the sequence of the target nucleic acid is determined.

  5. Phase Relations and Elemental Distribution Among Co-Existing Phases in the Ceramics of the Pseudobinary System CaZrTi{sub 2}O{sub 7}-LnAlO{sub 3} (Ln= Nd, Sm)

    SciTech Connect (OSTI)

    Mikhailenko, Natalia; Stefanovsky, Sergey

    2007-07-01

    In the ceramics in series (1-x) CaZrTi{sub 2}O{sub 7} - x NdAlO{sub 3} and (1-x) CaZrTi{sub 2}O{sub 7} - x SmAlO{sub 3} (x = 0.25, 0.5 and 0.75) produced by cold pressing and sintering at 1400, 1450 and 1500 deg. C zirconolite was found to be a major phase, perovskite was an extra phase and traces of residual baddeleyite occurred. At x = 0.75 the perovskite was major phase and zirconolite and cubic oxide of fianite or tazheranite type were extra phases. Major Nd and Sm host phase at x = 0.25 was found to be zirconolite (about 65% of total Nd{sub 2}O{sub 3} and 74% of total Sm{sub 2}O{sub 3}). With the x value increasing perovskite becomes major host phase for Nd and Sm accumulating of up to about 92% of total Nd and about 72% of total Sm. As follows from SEM/EDS data Nd and Sm contents in the zirconolite may reach {approx}1 formula unit (fu). (authors)

  6. Co-operativity among defect sites in AnO2+ and An4O9 (An = U, Np or Pu)

    SciTech Connect (OSTI)

    Andersson, Anders David; Lezama Pacheco, Juan; Uberuaga, Blas P; Conradson, Steven D

    2008-01-01

    Actinide dioxides derived from the AnO{sub 2} fluorite lattice are of high technological relevance due to their application in nuclear reactor fuels. Oxidation of AnO{sub 2} compounds emerges as a central theme in fuel fabrication, reactor operation, long-term storage forms for both spent fuels and surplus weapons materials, and environmental actinide migration. In this paper, we use density functional theory calculations to study the oxidation of uranium, neptunium and plutonium dioxides, AnO{sub 2} (An = U, Np or Pu), in O{sub 2} and O{sub 2}/H{sub 2}O environments. We pay particular attention to the formation of oxygen clusters (co-operativity) in AnO{sub 2+x} and how this phenomenon govern oxidation thermodynamics and the development of ordered An{sub 4}O{sub 9} compounds. The so-called split di-interstitial, which is composed of two nearest neighbor octahedral oxygen interstitials that are distorted in such a way that they dislocate one regular fluorite lattice oxygen ion to form a cluster of triangular geometry, is predicted to be the fundamental building block of the most stable cluster configurations. We also identify how the formation of oxygen defect clusters and the degree of oxidation in AnO{sub 2+x} are both governed by the characer of the An-5f to excess O-2p charger transfer, i.e. the charge transfer to the O-2p orbitals of the interstitial-like (+x) ions, and the ability of the excess O-2p orbitals to hybridize with regular fluorite lattice ions.

  7. Theoretical analyses of (n,xn) reactions on sup 235 U, sup 238 U, sup 237 Np, and sup 239 Pu for ENDF/B-VI

    SciTech Connect (OSTI)

    Young, P.G.; Arthur, E.D.

    1991-01-01

    Theoretical analyses were performed of neutron-induced reactions on {sup 235}U, {sup 238}U, {sup 237}Np, and {sup 239}Pu between 0.01 and 20 MeV in order to calculate neutron emission cross sections and spectra for ENDF/B-VI evaluations. Coupled-channel optical model potentials were obtained for each target nucleus by fitting total, elastic, and inelastic scattering cross section data, as well as low-energy average resonance data. The resulting deformed optical model potentials were used to calculate direct (n,n{prime}) cross sections and transmission coefficients for use in Hauser-Feshbach statistical theory analyses. A fission model with multiple barrier representation, width fluctuation corrections, and preequilibrium corrections were included in the analyses. Direct cross sections for higher-lying vibrational states were calculated using DWBA theory, normalized using B(E{ell}) values determined from (d,d{prime}) and Coulomb excitation data, where available, and from systematics otherwise. Initial fission barrier parameters and transition state density enhancements appropriate to the compound systems involved were obtained from previous analyses, especially fits to charged-particle fission probability data. The parameters for the fission model were adjusted for each target system to obtain optimum agreement with direct (n,f) cross section measurements, taking account of the various multichance fission channels, that is, the different compound systems involved. The results from these analyses were used to calculate most of the neutron (n,n), (n,n{prime}), and (n,xn) cross section data in the ENDF/B/VI evaluations for the above nuclei, and all of the energy-angle correlated spectra. The deformed optical model and fission model parameterizations are described. Comparisons are given between the results of these analyses and the previous ENDF/B-V evaluations as well as with the available experimental data. 14 refs., 3 figs., 1 tab.

  8. Photocatalytic splitting of water under visible-light irradiation over the NiOx-loaded Sm{sub 2}InTaO{sub 7} with 4f-d{sup 10}-d{sup 0} configuration

    SciTech Connect (OSTI)

    Tang Xinde; Ye Hongqi; Liu Hui; Ma Chenxia; Zhao Zhi

    2010-01-15

    A new visible-light-response photocatalyst Sm{sub 2}InTaO{sub 7} with 4f-d{sup 10}-d{sup 0} configuration crystallized in a cubic system with the space group Fd3m was synthesized by a solid-state reaction method. NiOx-loaded Sm{sub 2}InTaO{sub 7} showed high photocatalytic activities for H{sub 2} evolution from pure water under visible light irradiation (lambda>400 nm). Changes in the photocatalytic activity with the calcination temperature of Sm{sub 2}InTaO{sub 7} and the amount of NiOx loaded indicated that the combination of highly crystallized Sm{sub 2}InTaO{sub 7} and a high dispersion of NiOx particles led to high photocatalytic activity. The high photocatalytic performance of NiOx-loaded Sm{sub 2}InTaO{sub 7} supported the existing view that the photocatalytic activity correlated with the lattice distortion. Density functional theory calculation indicated that strong dispersion from the hybridized In 5s 5p orbitals at the bottom of the conduction band was responsible for the high activity of photocatalyst Sm{sub 2}InTaO{sub 7}. - Graphical abstract: A new visible-light-response photocatalyst Sm{sub 2}InTaO{sub 7} with 4f-d{sup 10}-d{sup 0} configuration was developed. DFT calculation indicated that strong dispersion from the hybridized In 5s 5p orbitals was responsible for the high photocatalytic activity.

  9. Lazarus-SM

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Cloud Fraction Parameterization Using Observations and Model Data S. M. Lazarus and S. K. Krueger University of Utah, Department of Meteorology Salt Lake City, Utah A. S. Frisch National Oceanic and Atmospheric Administration Environmental Technology Laboratory Boulder, Colorado Introduction We examine an empirical cloud fraction parameterization developed by Xu and Randall (XR 1996). The XR parameterization relates the large-scale relative humidity RH and the large-scale cloud water mixing

  10. Safety Criticality Standards Using the French CRISTAL Code Package: Application to the AREVA NP UO{sub 2} Fuel Fabrication Plant

    SciTech Connect (OSTI)

    Doucet, M.; Durant Terrasson, L.; Mouton, J.

    2006-07-01

    Criticality safety evaluations implement requirements to proof of sufficient sub critical margins outside of the reactor environment for example in fuel fabrication plants. Basic criticality data (i.e., criticality standards) are used in the determination of sub critical margins for all processes involving plutonium or enriched uranium. There are several criticality international standards, e.g., ARH-600, which is one the US nuclear industry relies on. The French Nuclear Safety Authority (DGSNR and its advising body IRSN) has requested AREVA NP to review the criticality standards used for the evaluation of its Low Enriched Uranium fuel fabrication plants with CRISTAL V0, the recently updated French criticality evaluation package. Criticality safety is a concern for every phase of the fabrication process including UF{sub 6} cylinder storage, UF{sub 6}-UO{sub 2} conversion, powder storage, pelletizing, rod loading, assembly fabrication, and assembly transportation. Until 2003, the accepted criticality standards were based on the French CEA work performed in the late seventies with the APOLLO1 cell/assembly computer code. APOLLO1 is a spectral code, used for evaluating the basic characteristics of fuel assemblies for reactor physics applications, which has been enhanced to perform criticality safety calculations. Throughout the years, CRISTAL, starting with APOLLO1 and MORET 3 (a 3D Monte Carlo code), has been improved to account for the growth of its qualification database and for increasing user requirements. Today, CRISTAL V0 is an up-to-date computational tool incorporating a modern basic microscopic cross section set based on JEF2.2 and the comprehensive APOLLO2 and MORET 4 codes. APOLLO2 is well suited for criticality standards calculations as it includes a sophisticated self shielding approach, a P{sub ij} flux determination, and a 1D transport (S{sub n}) process. CRISTAL V0 is the result of more than five years of development work focusing on theoretical

  11. Investigation of cellular microstructure and enhanced coercivity in sputtered Sm{sub 2}(CoCuFeZr){sub 17} film

    SciTech Connect (OSTI)

    Bhatt, Ranu Schtz, G.; Bhatt, Pramod

    2014-03-14

    We have investigated the effect of annealing temperature on the microstructure and magnetic properties of Sm{sub 2}(CoCuFeZr){sub 17} films prepared using ion beam sputtering at room temperature. The as-deposited film shows randomly oriented polycrystalline grains and exhibits small coercivity (H{sub C}) of 0.04 T at room temperature. Post annealing of these films at 700?C under Ar atmosphere shows significant changes in the microstructure transforming it to the development of cellular growth, concomitant with enhanced coercivity up to 1.3 T. The enhanced coercivity is explained using the domain wall pinning mechanism.

  12. A combined Sm-Nd, Rb-Sr, and U-Pb isotopic study of Mg-suite norite 78238: Further evidence for early differentiation of the Moon

    SciTech Connect (OSTI)

    Edmunson, J; E.Borg, L; Nyquist, L E; Asmerom, Y

    2008-11-17

    Lunar Mg-suite norite 78238 was dated using the Sm-Nd, Rb-Sr, and U-Pb isotopic systems in order to constrain the age of lunar magma ocean solidification and the beginning of Mg-suite magmatism, as well as to provide a direct comparison between the three isotopic systems. The Sm-Nd isotopic system yields a crystallization age for 78238 of 4334 {+-} 37 Ma and an initial {var_epsilon}{sub Nd}{sup 143} value of -0.27 {+-} 0.74. The age-initial {var_epsilon}{sub Nd}{sup 143} (T-I) systematics of a variety of KREEP-rich samples, including 78238 and other Mg-suite rocks, KREEP basalts, and olivine cumulate NWA 773, suggest that lunar differentiation was completed by 4492 {+-} 61 Ma assuming a Chondritic Uniform Reservoir bulk composition for the Moon. The Rb-Sr isotopic systematics of 78238 were disturbed by post-crystallization processes. Nevertheless, selected data points yield two Rb-Sr isochrons. One is concordant with the Sm-Nd crystallization age, 4366 {+-} 53 Ma. The other is 4003 {+-} 95 Ma and is concordant with an Ar-Ar age for 78236. The {sup 207}Pb-{sup 206}Pb age of 4333 {+-} 59 Ma is concordant with the Sm-Nd age. The U-Pb isotopic systematics of 78238 yield linear arrays equivalent to younger ages than the Pb-Pb system, and may reflect fractionation of U and Pb during sample handling. Despite the disturbed nature of the U-Pb systems, a time-averaged {mu} ({sup 238}U/{sup 204}Pb) value of the source can be estimated at 27 {+-} 30 from the Pb-Pb isotopic systematics. Because KREEP-rich samples are likely to be derived from source regions with the highest U/Pb ratios, the relatively low {mu} value calculated for the 78238 source suggests the bulk Moon does not have an exceedingly high {mu} value.

  13. Effect of metallo-organic precursors on the synthesis of Sm-Sn pyrochlore catalysts: Application to the oxidative coupling of methane

    SciTech Connect (OSTI)

    Roger, A.C.; Petit, C.; Kiennemann, A.

    1997-04-15

    Synthesis of a series of Sm{sub 2}Sn{sub 2}O{sub 7} pyrochlore catalysts by a sol-gel-like method has been developed. The preparation from the oxides gives stoichiometric pyrochlore, unlike the result obtained when starting from chlorinated salts (SmCl{sub 3} or SnCl{sub 2}), which form tin-deficient pyrochlores. A spectroscopic study of the behavior of the starting oxides or chlorides in propionic acid, to generate a series of precursors, has been carried out, particular attention being focused on the precursors generated by SnCl{sub 2} in propionic acid using {sup 119}Sn NMR and FTIR spectroscopy. The formation of SnCl{sub 2}(C{sub 2}H{sub 5}COO){sub 2} as the main precursor is responsible for the tin deficiency observed in the pyrochlore structure. The catalytic performance in oxidative coupling of methane is directly correlated with the tin deficiency in the bulk of the pyrochlore. The work highlights the importance of controlling precisely the synthesis of the catalysts. 42 refs., 10 figs., 5 tabs.

  14. Synthesis and photoluminescence properties of Ca{sub 19}Mg{sub 2}(PO{sub 4}){sub 14}:Sm{sup 3+} red phosphor for white light emitting diodes

    SciTech Connect (OSTI)

    Zhu, Ge; Ci, Zhipeng; Shi, Yurong; Wang, Yuhua

    2014-07-01

    Highlights: • A novel red phosphor Ca{sub 19}Mg{sub 2}(PO{sub 4}){sub 14}:Sm{sup 3+} was synthesized and investigated firstly. • The structure and characteristic luminescence properties are discussed. • The excellent thermal stability was found and investigated. • It has good color saturation, the CIE is close to that of commercial Y{sub 2}O{sub 3}:Eu{sup 3+}. - Abstract: A series of Sm{sup 3+} doped Ca{sub 19}Mg{sub 2}(PO{sub 4}){sub 14} red phosphors were successfully synthesized. X-ray diffraction analysis indicates that all the samples are single phased. The luminescence property is investigated in detail by measuring their photoluminescence excitation and emission spectra. Ca{sub 19}Mg{sub 2}(PO{sub 4}){sub 14}:Sm{sup 3+} phosphors show strong absorption in 400–410 nm region, which is suitable for application in LEDs. When excited at 403 nm, Ca{sub 19}Mg{sub 2}(PO{sub 4}){sub 14}:Sm{sup 3+} phosphor can emit red emission with CIE chromaticity coordinates (0.615, 0.384). The optimal doping concentration of Sm{sup 3+} doped Ca{sub 19}Mg{sub 2}(PO{sub 4}){sub 14} is measured to be 0.02. The thermal quenching property is also measured and compared with the commercial red phosphor Y{sub 2}O{sub 3}:Eu{sup 3+} (Topstar, TXC-RIA). The results indicate Ca{sub 19}Mg{sub 2}(PO{sub 4}){sub 14}:Sm{sup 3+} phosphors have potential to serve as a red phosphor for white LEDs.

  15. Magnetic and electrical properties of LaC/sub 2/, CeC/sub 2/, PrC/sub 2/, NdC/sub 2/, and SmC/sub 2/

    SciTech Connect (OSTI)

    Sakai, T.; Adachi, G.; Yoshida, T.; Shiokawa, J.

    1981-09-15

    The electrical resistivities of the tetragonal CaC/sub 2/-type rare-earth dicarbides RC/sub 2/ (R = La, Ce, Pr, Nd, and Sm) and the magnetic susceptibilities of RC/sub 2/ (R = Pr, Nd, and Sm) are reported. The dicarbide LaC/sub 2/ becomes a superconductor at 1.6 K, which is in good agreement with literature values. The resistivity vs temperature curve of CeC/sub 2/ indicates a small hump at 30 K, and those of PrC/sub 2/ and NdC/sub 2/ show a sharp change in slope at 18 and 25 K, respectively, all verifying the antiferromagnetic transitions found by neutron diffraction. The temperature dependence of resistivity of CeC/sub 2/ was explained on the basis of the GAMMA/sub 7/ components of Ce/sup 3 +/. The compound PrC/sub 2/ becomes ferromagnetic at a zero-field Curie temperature of 7 K. This magnetic behavior differs significantly from that reported previously, suggesting an antiferromagnetic-to-ferromagnetic transition in the field of less than 700 Oe. The susceptibility of NdC/sub 2/ shows a field-independent antiferromagnetic transition at 24 K. An antiferromagnetic transition in SmC/sub 2/ was found anew at 21 K in both the resistivity and susceptibility data, exhibiting Van Vleck's Sm/sup 3 +/ characteristics. The Sm/sup 3 +/ ion in SmC/sub 2/ appears to be largely confined in the J = 5/2 ground state at about 21 K, since the paramagnetic Curie temperature reduced thereby and those of the other dicarbides can be correlated reasonably in the de Gennes factor plot.

  16. HRTEM, SAED and XRD investigations of RE{sub 4}O{sub 4}[AsO{sub 4}]Cl (RE = La, Pr, Nd, Sm, Eu, Gd)

    SciTech Connect (OSTI)

    Ben Yahia, Hamdi; Rodewald, Ute Ch.; Boulahya, Khalid; Pöttgen, Rainer

    2014-05-01

    Graphical abstract: The new compounds RE{sub 4}O{sub 4}[AsO{sub 4}]Cl (RE = La, Pr, Nd, Sm, Eu, Gd) were synthesised by solid state reaction via a salt flux route and investigated by HRTEM, SAED, and single crystal X-ray diffraction. - Highlights: • We discovered the series of RE{sub 4}O{sub 4}[AsO{sub 4}]Cl (RE = La, Pr, Nd, Sm, Eu, Gd) compounds. • The RE{sub 4}O{sub 4}[AsO{sub 4}]Cl single crystals were grown using NaCl/KCl flux. • The RE{sub 4}O{sub 4}[AsO{sub 4}]Cl structures were solved using single crystal X-ray diffraction data. • The layered RE{sub 4}O{sub 4}[AsO{sub 4}]Cl compounds were further characterized using HRTEM and SAED. • We observed an alternation of ordered-[RE{sub 4}O{sub 4}]{sup 4+} and disordered-[ClAsO{sub 4}]{sup 4–} layers. - Abstract: The new compounds RE{sub 4}O{sub 4}[AsO{sub 4}]Cl (RE = La, Pr, Nd, Sm, Eu, Gd) were synthesised by solid state reaction via a salt flux route and investigated by HRTEM, SAED, and single crystal X-ray diffraction. The samples crystallise with a tetragonal cell, space group P4{sub 2}/mnm and Z = 2. Their crystal structure consists of an alternation of [RE{sub 4}O{sub 4}]{sup 4+} and [ClAsO{sub 4}]{sup 4–} layers. The [RE{sub 4}O{sub 4}]{sup 4+} layer contains ORE{sub 4/4} tetrahedra which share common edges. The anions AsO{sub 4}{sup 3–} and Cl{sup –} are located between these layers in disordered manner. SAED and HRTEM experiments confirmed this structural model and enabled us to propose an ordered model for the [ClAsO{sub 4}]{sup 4–} layers.

  17. Synthesis and photoluminescence properties of NaLaMgWO{sub 6}:RE{sup 3+} (RE = Eu, Sm, Tb) phosphor for white LED application

    SciTech Connect (OSTI)

    Hou, Jingshan; CAS Key Laboratory of Materials for Energy Conversion, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050; College of Chemistry and Molecular Engineering, Peking University, Beijing 100871 ; Yin, Xin; College of Chemistry and Molecular Engineering, Peking University, Beijing 100871 ; Huang, Fuqiang; College of Chemistry and Molecular Engineering, Peking University, Beijing 100871 ; Jiang, Weizhong

    2012-06-15

    Highlights: ► NaLa{sub 1−x}MgWO{sub 6}:xRE{sup 3+} phosphors were synthesized by solid-state reaction method. ► Compared with Y{sub 2}O{sub 3}:Eu{sup 3+}, NaLaMgWO{sub 6}:Eu{sup 3+} performed better luminescence properties. ► The results demonstrated NaLaMgWO{sub 6} as a suitable host for RE{sup 3+}-doping. -- Abstract: Single phase of NaLa{sub 1−x}MgWO{sub 6}:xRE{sup 3+} (0 < x ≤1) (RE = Eu, Sm, Tb) phosphors were prepared by solid-state reaction method. X-ray diffraction, scanning electron microscopy, the morphology energy-dispersive X-ray spectroscopy, UV–vis diffuse reflectance spectra and photoluminescence were used to characterize the samples. Under the light excitation, NaLaMgWO{sub 6}:Eu{sup 3+}, NaLaMgWO{sub 6}:Sm{sup 3+} and NaLaMgWO{sub 6}:Tb{sup 3+}, phosphors showed the characteristic emissions of Eu{sup 3+} ({sup 5}D{sub 0} → {sup 7}F{sub 4,3,2,1}), Sm{sup 3+} ({sup 4}G{sub 5/2} → {sup 6}H{sub 5/2,7/2,9/2}), and Tb{sup 3+} ({sup 5}D{sub 4} → {sup 7}F{sub 6,5,4,3}), respectively. The intensity of the red emission for Na(La{sub 0.6}Eu{sub 0.4})MgWO{sub 6} is 2.5 times higher than that of (Y{sub 0.95}Eu{sub 0.05}){sub 2}O{sub 3} under blue light irradiation. The quantum efficiencies of the entitled phosphors excited under 394 nm and 464 nm are also investigated and compared with commercial phosphors Y{sub 2}O{sub 3}:Eu{sup 3+}, Sr{sub 2}Si{sub 5}N{sub 8}:Eu{sup 2+} and Y{sub 3}A{sub 5}G{sub 12}:Ce{sup 3+}. The results demonstrated NaLaMgWO{sub 6}:RE{sup 3+} phosphors as potential candidates for white light emitting diode pumped by UV or blue chip.

  18. This invention relates to methods of generating NP gallium nitride (GaN) across large areas (>1 cm.sup.2) with controlled pore diameters, pore density, and porosity. Also disclosed are methods of generating novel optoelectronic devices based on porous GaN. Additionally a layer transfer scheme to separate and create free-standing crystalline GaN thin layers is disclosed that enables a new device manufacturing paradigm involving substrate recycling. Other disclosed embodiments of this invention relate to fabrication of GaN based nanocrystals and the use of NP GaN electrodes for electrolysis, water splitting, or photosynthetic process applications.

    DOE Patents [OSTI]

    Zhang, Yu; Sun, Qian; Han, Jung

    2015-12-08

    This invention relates to methods of generating NP gallium nitride (GaN) across large areas (>1 cm.sup.2) with controlled pore diameters, pore density, and porosity. Also disclosed are methods of generating novel optoelectronic devices based on porous GaN. Additionally a layer transfer scheme to separate and create free-standing crystalline GaN thin layers is disclosed that enables a new device manufacturing paradigm involving substrate recycling. Other disclosed embodiments of this invention relate to fabrication of GaN based nanocrystals and the use of NP GaN electrodes for electrolysis, water splitting, or photosynthetic process applications.

  19. Sensitivity of fusion and quasi-elastic barrier distributions of {sub 16}O+{sub 144}Sm reaction on the coupling radius parameter

    SciTech Connect (OSTI)

    Zamrun, Muhammad; Usman, Ida; Variani, Viska Inda; Kassim, Hasan Abu

    2014-03-05

    We study the heavy-ion collision at sub-barrier energies of {sub 16}O+{sub 144}Sm system using full order coupled-channels formalism. We especially investigate the sensitivity of fusion and quasi-elastic barrier distributions for this system on the coupling radius parameter. We found that the coupled-channels calculations of the fusion and the quasi-elastic barrier distributions are sensitive to the coupling radius for this reaction in contrast to the fusion and quasi-elastic cross section. Our study indicates that the larger coupling radius, i.e., r{sub coup}=1.20, is required by the experimental quasi-elastic barrier distribution. However, the experimental fusion barrier distribution compulsory the small value, i.e., r{sub coup}=1.06.

  20. Raman spectroscopic studies of Nd{sub 0.75}Sm{sub 0.25}GaO{sub 3} single crystals

    SciTech Connect (OSTI)

    Nithya, R. Ravindran, T. R.; Daniel, D. J.

    2015-06-24

    Single crystals of Nd{sub 1-x}Sm{sub x}GaO{sub 3} (x= 0 and 0.25) were grown by a four mirror IR image furnace using floating zone technique. The crystals are characterized by X-ray diffraction and Raman spectroscopic measurements. NGO adopts orthorhombic structure with Pbnm symmetry and samarium substituted compound also exhibited the same structure as that of the pristine compound without secondary phases. Polarized Raman spectra are measured at ambient temperature in a back scattering geometry. Spectra exhibit low intensity first-order Raman bands. In addition, several high intensity second-order Raman bands have been observed in the frequency range 2000 to 4000 cm{sup −1}.

  1. Structural phase transition of ternary dielectric SmGdO{sub 3}: Evidence from angle dispersive x-ray diffraction and Raman spectroscopic studies

    SciTech Connect (OSTI)

    Sharma, Yogesh E-mail: satya504@gmail.com Sahoo, Satyaprakash E-mail: satya504@gmail.com Misra, Pankaj; Pavunny, Shojan P.; Katiyar, Ram S. E-mail: satya504@gmail.com; Mishra, A. K.; Dwivedi, Abhilash; Sharma, S. M.

    2015-03-07

    High-pressure synchrotron based angle dispersive x-ray diffraction (ADXRD) studies were carried out on SmGdO{sub 3} (SGO) up to 25.7 GPa at room temperature. ADXRD results indicated a reversible pressure-induced phase transition from ambient monoclinic to hexagonal phase at ∼8.9 GPa. The observed pressure-volume data were fitted with the third order Birch-Murnaghan equation of state yielding zero pressure bulk modulus B{sub 0} = 132(22) and 177(9) GPa for monoclinic (B-type) and hexagonal (A-type) phases, respectively. Pressure dependent micro-Raman spectroscopy further confirmed the monoclinic to hexagonal phase transition at about 5.24 GPa. The mode Grüneisen parameters and pressure coefficients for different Raman modes corresponding to each individual phases of SGO were calculated using pressure dependent Raman mode analysis.

  2. {sup 147}Sm(n,{alpha}) cross section measurements from 3 eV to 500 keV: Implications for explosive nucleosynthesis reaction rates

    SciTech Connect (OSTI)

    Gledenov, Yu. M.; Koehler, P. E.; Andrzejewski, J.; Guber, K. H.; Rauscher, T.

    2000-10-01

    We have measured the {sup 147}Sm(n,{alpha}) cross section from 3 eV to 500 keV. These data were used to test nuclear statistical models which must be relied on to calculate the rates for as yet unmeasurable reactions occurring in explosive nucleosynthesis scenarios. It was found that our data are in reasonably good agreement with the reaction rate predicted by an older model but that the rates predicted by two very recent models are roughly a factor of 3 different from the data (in opposite directions). A detailed analysis indicates the strong dependence on the employed optical {alpha} potentials. These results, together with counting rate estimates for future experiments indicate that (n,{alpha}) measurements will be useful for improving reaction rate predictions across the global range of masses needed for explosive nucleosynthesis calculations.

  3. Thermal conductivity of La/sub 3-x/R/sub x/S/sub 4/ R = Sm, Yb, and Eu

    SciTech Connect (OSTI)

    Kokos, G.B.

    1989-02-01

    The thermal diffusivity values of La/sub 2.7/Eu/sub 0.3/S/sub 4/, La/sub 2.2/Eu/sub 0.8/S/sub 4/, La/sub 2.7/Sm/sub 0.3/S/sub 4/, La/sub 2.3/Sm/sub 0.7/S/sub 4/, La/sub 2.7/Yb/sub 0.2/S/sub 4/, and La/sub 2.2/Yb/sub 0.7/S/sub 4/ were measured by the flash diffusivity method from 400/degree/C to 1000/degree/C. These values ranged from .007 cm/sup 2//s to .018 cm/sup 2//s. The thermal conductivities of the ternary rare earth sulfides were calculated from the thermal diffusivity data and ranged from 10.7 mW/cm/degree/C to 31.6 mW/cm/degree/C. The thermal diffusivity values of three thermal conductivity standards (armco iron, NBS graphite, and NBS austenitic stainless steel) obtained using the flash diffusivity apparatus agreed with the accepted values within a deviation of +-10%. Of the ternary rare earth sulfides measured, La/sub 2.2/Eu/sub 0.8/S/sub 4/ had the highest figure of merit at 1000/degree/C of .525. All these samples had an oxysulfide present at the grain boundaries which degraded their high temperature thermoelectric performance. 56 refs., 12 figs., 7 tabs.

  4. MEASUREMENT OF THE AVERAGE ENERGY AND MULTIPLICITY OF PROMPT-FISSION-NEUTRONS FROM 238U(n,f) AND 237 Np(n,f) FROM 1 TO 200 MeV.

    SciTech Connect (OSTI)

    TAIEB,J.; GRANIER, T.; ETHVIGNOT, T.; DEVLIN, M.; HAIGHT, R.C.; NELSON, R.O.; ODONNELL, J.M.; ROCHMAN, D.

    2007-06-28

    Taking advantage of the neutron source of the LANCSE, it has been possible to obtain a measure of the velocity distribution and the number of prompt-neutrons emitted in the neutron-induced fission of {sup 238}U and {sup 237}Np over a broad incident neutron energy range. The mean kinetic energy was extracted and is shown as the function of the incident-neutron energy. We confirm here the observation, for both reactions, of a dip around the second chance fission which is explained by the lower kinetic energy of the pre-fission neutrons. Such a observation is reproduced by Los Alamos model as implemented at Bruyeres le Chatel and by the Maslov model. As far as the neutron multiplicity is concerned, a similar dip is observed. However, such a behavior is not present in data measured by other groups.

  5. High Schottky barrier at grain boundaries observed in Na{sub 1/2}Sm{sub 1/2}Cu{sub 3}Ti{sub 4}O{sub 12} ceramics

    SciTech Connect (OSTI)

    Somphan, Weeraya; Thongbai, Prasit; Yamwong, Teerapon; Maensiri, Santi

    2013-10-15

    Graphical abstract: - Highlights: NSCTO exhibits a high ?? of 7.08.4 10{sup 3} and low tan ? of 0.0300.041. NSCTO exhibits a high E{sub b} of ?2208 V cm{sup ?1} and large ? of 15.6. Giant ?? response is attributed to the electrically heterogeneous microstructure. High ?{sub b} values at grain boundaries are found to be 0.9250.964 eV. Formation of a potential barrier at grain boundaries is caused by Schottky effect. - Abstract: The dielectric properties and nonlinear currentvoltage characteristics of Na{sub 1/2}Sm{sub 1/2}Cu{sub 3}Ti{sub 4}O{sub 12} ceramics prepared by a conventional solid state reaction method were investigated. Na{sub 1/2}Sm{sub 1/2}Cu{sub 3}Ti{sub 4}O{sub 12} ceramics exhibited a high dielectric permittivity of 7.08.4 10{sup 3} and low loss tangent (tan ??0.0300.041). Non-Ohmic properties with a high breakdown voltage of ?2208 V cm{sup ?1} and large nonlinear coefficient of 15.6 were observed in Na{sub 1/2}Sm{sub 1/2}Cu{sub 3}Ti{sub 4}O{sub 12} ceramics. Using complex impedance analysis, Na{sub 1/2}Sm{sub 1/2}Cu{sub 3}Ti{sub 4}O{sub 12} ceramics were shown to be electrically heterogeneous consisting of semiconducting grains and insulating grain boundaries. Giant dielectric properties were described based on the electrically heterogeneous microstructure. X-ray photoelectron spectroscopy analysis suggested that the semiconductive nature of grains may be related to the presence of Cu{sup +} and Ti{sup 3+}. The formation of an electrostatic potential barrier at the grain boundaries of Na{sub 1/2}Sm{sub 1/2}Cu{sub 3}Ti{sub 4}O{sub 12} ceramics was suggested to be caused by the Schottky effect. Interestingly, high electrostatic potential barriers at grain boundaries in Na{sub 1/2}Sm{sub 1/2}Cu{sub 3}Ti{sub 4}O{sub 12} ceramics were calculated and found to be 0.9250.964 eV.

  6. Structure, thermodynamic, and magnetic properties of Ln[sub 4]PdO[sub 7] with Ln = La, Nd, Sm, Eu, and Gd

    SciTech Connect (OSTI)

    Andersson, M.; Grins, J.; Nygren, M. (Stockholm Univ. (Sweden))

    1999-09-01

    The structure of Nd[sub 4]PdO[sub 7] has been determined and refined using the Rietveld method and combined CuK[alpha][sub 1] X-ray and neutron powder data in space group P[bar 1] with unit cell a = 15.972(2), b = 7.1927(7), c = 6.9160(6) [angstrom], [alpha] = 96.299(4), [beta] = 131.643(3), [gamma] = 121.438(3)[degree], V = 353.83(6) [angstrom][sup 3] and Z = 2, to R[sub F] = 2.0% (neutron data) and R[sub F] = 6.2% (X-ray data). The structure is closely related to the monoclinic La[sub 4]PdO[sub 7] structure and exhibits Nd atoms coordinated by seven O atoms and Pd atoms coordinated by a square of O atoms. Isolated chains of trans-corner-sharing PdO[sub 4] squares are straight in the La[sub 4]PdO[sub 7] structure and staggered in the Nd[sub 4]PdO[sub 7] structure. Electron and X-ray powder diffraction data show that Ln[sub 4]PdO[sub 7] with Ln = Sm, Eu, and Gd is isostructural with Nd[sub 4]PdO[sub 7]. The enthalpies of dissolution of Ln[sub 4]PdO[sub 7] (Ln = La, Nd) in 1.000 M HCl have been measured with an in-house built calorimeter, and from these values the enthalpies of formation for the compounds have been calculated. The decomposition temperatures of Ln[sub 4]PdO[sub 7] with Ln = La and Nd in oxygen have been determined by thermogravimetric measurements and found to decrease from 1645 [+-] 10 K for La[sub 4]PdO[sub 7] to 1540 [+-] 10 K for Nd[sub 4]PdO[sub 7]. Using these data, an Ellingham diagram has been constructed assuming temperature-independent [Delta]H[sub f][degree] and [Delta]S[sub f][degree]. The magnetic susceptibilities of Ln[sub 4]PdO[sub 7] with Ln = La, Nd, Sm, Eu, Gd, recorded in the temperature range 10--320 K, were found to be in agreement with the expected ones for noninteracting Ln[sup 3+] ions.

  7. A Linear trans -Bis(imido) Neptunium(V) Actinyl Analog: NpV (NDipp)2 ( tBu2 bipy)2Cl (Dipp = 2,6- i Pr2C6H3)

    SciTech Connect (OSTI)

    Brown, Jessie L.; Batista, Enrique R.; Boncella, James M.; Gaunt, Andrew J.; Reilly, Sean D.; Scott, Brian L.; Tomson, Neil C.

    2015-07-22

    We present the discovery that imido analogs of actinyl dioxo cations can be extended beyond uranium into the transuranic elements. Synthesis of the Np(V) complex, Np(NDipp)2(tBu2bipy)2Cl (1), is achieved through treatment of a Np(IV) precursor with a bipyridine co-ligand and lithium-amide reagent. Complex 1 has been structurally characterized, analyzed by 1H NMR and UV/vis/NIR spectroscopies, and the electronic structure evaluated by DFT calculations.

  8. Status of ITER task T213 collaborative irradiation screening experiment on Cu/SS joints in the Russian Federation SM-2-reactor

    SciTech Connect (OSTI)

    Edwards, D.J.; Fabritsiev, S.A.; Pokrovsky, A.S.; Zinkle, S.J.

    1996-04-01

    Specimen fabrication is underway for an irradiation screening experiment planned to start in January 1996 in the SM-2 reactor in Dimitrovgrad, Russia. The purpose of the experiment is to evaluate the effects of neutron irradiation at ITER-relevant temperatures on the bond integrity performance of Cu/SS and Be/Cu joints, as well as to further investigate the base metal properties of irradiated copper alloys. Specimens from each of the four ITER parties (U.S., EU, japan, and RF) will be irradiated to a dose of {approx}0.2 dpa at two different temperatures, 150 and 300{degrees}C. The specimens will consist of Cu/SS and Be/Cu joints in several different geometries, as well as a large number of specimens from the base materials. Fracture toughness data on base metal and Cu/SS bonded specimens will be obtained from specimens supplied by the U.S. Due to lack of material, the Be/Cu specimens supplied by the U.S will only be irradiated as TEM disks.

  9. Two-dimensional electron liquid at the (111) SmTiO{sub 3}/SrTiO{sub 3} interface

    SciTech Connect (OSTI)

    Raghavan, Santosh; Zhang, Jack Y.; Stemmer, Susanne

    2015-03-30

    Similar to (001) interfaces, a high carrier density, two-dimensional electron liquid (2DEL) is expected to form at (111) RTiO{sub 3}/SrTiO{sub 3} interfaces (R is a trivalent rare earth ion). In this study, epitaxial SmTiO{sub 3} layers were grown on (111) SrTiO{sub 3} surfaces using hybrid molecular beam epitaxy. We report on electrical transport measurements and characterize the carrier densities in the 2DEL and the carrier mobilities at these interfaces. The carrier density is in reasonable agreement with the expected carrier density of ∼2 × 10{sup 14 }cm{sup −2}. Mobility-limiting mechanisms are analyzed and compared with those of (001) interfaces. Collectively, the results indicate that (111) 2DELs are less confined than those at (001) interfaces. These 2DELs should allow for the study of the phenomena induced by the unique topology of the electron system at (111) interfaces.

  10. Multiple temperature-induced magnetization reversals in SmCr{sub 1−x}Fe{sub x}O{sub 3} system

    SciTech Connect (OSTI)

    Yin, L.H.; Liu, Y.; Tan, S.G.; Zhao, B.C.; Dai, J.M.; Song, W.H.; Sun, Y.P.

    2013-10-15

    Graphical abstract: - Highlights: • Multiple temperature-induced magnetization reversals were observed in x = 0.1. • Coexistence of normal and inverse magnetocaloric effects was observed. • A reasonable model was proposed to explain the magnetization reversals. - Abstract: The structural and magnetic properties of the SmCr{sub 1−x}Fe{sub x}O{sub 3} (0 ≤ x ≤ 0.5) system have been investigated. Multiple temperature-induced magnetization reversals were observed in x = 0.1. The high-temperature magnetization reversal is due to the special spin structure, in which the net canted moment of the Cr-rich regions and the net moment of the Fe–Cr ordered regions orient in opposite direction; while the low temperature one can be ascribed to the spin reorientation. The sample with x = 0.5 exhibits the highest compensation temperature. Coexistence of normal and inverse magnetocaloric effects was observed in all doped samples. Potential applications in magnetic refrigeration based constant temperature bath near room temperature (∼286 K) have been demonstrated.

  11. Nanocrystalline Sm{sub 0.5}Sr{sub 0.5}CoO{sub 3−δ} synthesized using a chelating route for use in IT-SOFC cathodes: Microstructure, surface chemistry and electrical conductivity

    SciTech Connect (OSTI)

    Scurtu, Rares; Somacescu, Simona; Calderon-Moreno, Jose Maria; Culita, Daniela; Bulimestru, Ion; Popa, Nelea; Gulea, Aurelian; Osiceanu, Petre

    2014-02-15

    Nanocrystalline Sm{sub 0.5}Sr{sub 0.5}CoO{sub 3−δ} powders were synthesized by a chelating route using different polyfunctional H{sub x}APC acids (APC=aminopolycarboxylate; x=3, 4, 5). Different homologous aminopolycarboxylic acids, namely nitrilotriacetic (H{sub 3}nta), ethylenediaminetetraacetic (H{sub 4}edta), 1,2-cyclohexanediaminetetracetic (H{sub 4}cdta) and diethylenetriaminepentaacetic (H{sub 5}dtpa) acid, were used as chelating agents to combine Sm, Sr, Co elements into a perovskite structure. The effects of the chelating agents on the crystalline structure, porosity, surface chemistry and electrical properties were investigated. The electrical properties of the perovskite-type materials emphasized that their conductivities in the temperature range of interest (600–800 °C) depend on the nature of the precursors as well as on the presence of a residual Co oxide phase as shown by XRD and XPS analysis. The surface chemistry and the surface stoichiometries were determined by XPS revealing a complex chemical behavior of Sr that exhibits a peculiar “surface phase” and “bulk phase” chemistry within the detected volume (<10 nm). - Graphical abstract: Synthesis of nanocrystalline Sm{sub 0.5}Sr{sub 0.5}CoO{sub 3−δ} powders by a chelating route and the investigation of the microstructure, surface chemistry and electrical properties. Display Omitted - Highlights: • Nanocrystalline Sm{sub 0.5}Sr{sub 0.5}CoO{sub 3−δ} obtained by a chelating synthesis route. • Cubic perovskite structures with crystallite sizes ∼23±2 nm. • The porous nature revealed by N{sub 2} adsorption/desorption (BET). • The surface chemistry and the surface stoichiometries highlighted by XPS. • A complex chemical behavior of Sr exhibits a peculiar “surface phase” and “bulk phase” chemistry.

  12. Preparation and thermophysical properties of (Sm{sub 1?x}Er{sub x}){sub 2}Ce{sub 2}O{sub 7} oxides for thermal barrier coatings

    SciTech Connect (OSTI)

    Xiaoge, Chen; Shusen, Yang; Hongsong, Zhang; Gang, Li; Zhenjun, Li.; Bo, Ren; Xudan, Dang; Haoming, Zhang; An, Tang

    2014-03-01

    Graphical abstract: - Highlights: These ceramic materials with fluorite structure were synthesized. Defect points lead to their lower thermal conductivities. The lower ionic radius of Er{sup 3+} ion leads to the reduction of thermal expansion coefficient of (Sm{sub 1?x}Er{sub x}){sub 2}Ce{sub 2}O{sub 7} oxides. - Abstract: (Sm{sub 1?x}Er{sub x}){sub 2}Ce{sub 2}O{sub 7} ceramics were synthesized by solgel method and sintered at 1600 C for 10 h in air. The influence of Er{sub 2}O{sub 3}-substitution on the phase structure and thermophysical properties of Sm{sub 2}Ce{sub 2}O{sub 7} was investigated. The phase structures of these ceramics were identified by X-ray diffraction showing that all synthesized ceramics have fluorite-type structure. The measurements for thermophysical properties of these ceramics show that their thermal conductivities and thermal expansion coefficients remarkably decreased through Er-substitution. However, the thermal expansion coefficients were higher than that of YSZ and their thermal conductivities were much lower than that of 8YSZ. The excellent thermophysical property implies that these solid solutions are potential materials for the ceramics layer in thermal barrier coatings.

  13. Preparation, characterization, magnetic susceptibility (Eu, Gd and Sm) and XPS studies of Ln{sub 2}ZrTiO{sub 7} (Ln=La, Eu, Dy and Gd)

    SciTech Connect (OSTI)

    Vijaya Kumar, B.; Velchuri, Radha; Rama Devi, V.; Sreedhar, B.; Prasad, G.; Jaya Prakash, D.; Kanagaraj, M.; Arumugam, S.; Vithal, M.

    2011-02-15

    Bulk and nanosized pyrochlore materials Ln{sub 2}ZrTiO{sub 7} (Ln=La, Eu, Dy, Gd and Sm) have been prepared by the sol-gel method. All the samples were characterized by powder X-ray diffraction, Raman and X-ray photoelectron spectroscopy. Magnetic susceptibility ({chi}) measurements of Gd{sub 2}ZrTiO{sub 7}, Sm{sub 2}ZrTiO{sub 7} and Eu{sub 2}ZrTiO{sub 7} were carried out by vibrating sample magnetometer in the temperature range 2-320 K. The variation of {chi}{sup -1} (or {chi}) with temperature of Gd{sub 2}ZrTiO{sub 7}, Sm{sub 2}ZrTiO{sub 7} and Eu{sub 2}ZrTiO{sub 7} follows the Curie law, intermediate formula and the Curie-Weiss law, respectively. From the linear portion of {chi}T vs. T{sup -1} plot of Eu{sub 2}ZrTiO{sub 7} from 2 to 15 K, the classical nearest neighbor exchange (J{sup cl}) and dipolar interactions (D{sub nn}) are obtained. The XPS of Ln{sub 2}ZrTiO{sub 7} (Ln=La, Eu, Dy and Gd) gave characteristic peaks for Ln, Ti, Zr and O. The satellite peaks are observed only for 3d La of La{sub 2}ZrTiO{sub 7}. -- Graphical abstract: Sm{sub 2}ZrTiO{sub 7} does not follow the Curie or the Curie-Weiss law. The effective magnetic moment is found to be 0.768 BM (at 300 K), which is smaller than the free ion moment 1.3-1.4 BM. Display Omitted Research Highlights: {yields} Bulk and nano Ln{sub 2}ZrTiO{sub 7} (Ln=La, Eu, Dy, Gd and Sm) have been prepared by the sol-gel method. {yields} The broad Raman lines are attributed to cation disorder and small crystallite size. {yields} XPS of Ln{sub 2}ZrTiO{sub 7} exhibit characteristic X-ray photoelectron spectral features. {yields} Magnetic moment of Gd{sub 2}ZrTiO{sub 7} is obtained from magnetic susceptibility and ESR spectra.

  14. The RELi{sub x}Sn{sub 2} (RE=La–Nd, Sm, and Gd; 0≤x<1) series revisited. Synthesis, crystal chemistry, and magnetic susceptibilities

    SciTech Connect (OSTI)

    Makongo, Julien P.A.; Suen, Nian-Tzu; Guo, Shengping; Saha, Shanta; Greene, Richard; Paglione, Johnpierre; Bobev, Svilen

    2014-03-15

    This study is concerned with the ternary compounds RELi{sub x}Sn{sub 2} (RE=La–Nd, Sm, and Gd; 0≤x<1), which have been previously thought to be the stoichiometric RELiSn{sub 2} phases. These materials crystallize with the base-centered orthorhombic space group Cmcm (No. 63), and can be formally assigned with the CeNiSi{sub 2} structure type (Pearson symbol oC16). Our systematic single-crystal X-ray diffraction studies revealed substantial Li-deficiencies in all cases, with SmSn{sub 2} (space group Cmmm, ZrGa{sub 2} structure type, Pearson symbol oC12) and GdSn{sub 2} (space group Cmcm, ZrSi{sub 2} structure type, Pearson symbol oC12) being completely lithium-free. The structure refinements also uncovered positional disorder on the Sn site neighboring the vacancies. The Sn-disorder and the Li-deficiency correlate, and vary monotonically with the decreased size of the rare-earth atoms in the order RE=La–Nd. The SmSn{sub 2} and GdSn{sub 2} structures are devoid of any disorder. Temperature-dependent studies of the magnetic response of the title compounds are also presented and discussed. -- Graphical abstract: RELi{sub x}Sn{sub 2} (RE=La–Nd, 0≤x<1) crystallize in a defect variants of the CeNiSi{sub 2} structure type (a). The Sn-disorder and the Li-deficiency correlate, and vary monotonically with the decreased size of the rare-earth atoms in the order RE=La–Nd. The SmSn{sub 2} (b) and GdSn{sub 2} (c) structures are devoid of any disorder. Highlights: • The crystal structures of the RELi{sub x}Sn{sub 2} (RE=La–Nd, 0≤x<1) compounds are revised using single-crystal X-ray diffraction data. • The structure is a filled derivative of the ZrSi{sub 2} structure type or defect variant of the CeNiSi{sub 2} structure type. • SmSn{sub 2} is isotypic with the ZrGa{sub 2} structure, while RESn{sub 2} (RE=Gd–Lu) are isotypic with the ZrSi{sub 2} structure.

  15. Combined effect of chemical pressure and valence electron concentration through the electron-deficient Li substitution on the RE{sub 4}LiGe{sub 4} (RE=La, Ce, Pr, and Sm) system

    SciTech Connect (OSTI)

    Nam, Gnu; Jeon, Jieun; Kim, Youngjo; Kwon Kang, Sung; Ahn, Kyunghan; You, Tae-Soo

    2013-09-15

    Four members of the RE{sub 4}LiGe{sub 4} (RE=La, Ce, Pr, and Sm) system have been prepared by high-temperature reaction method and characterized by X-ray diffractions. All compounds crystallize in the orthorhombic Gd{sub 5}Si{sub 4}-type structure (space group Pnma, Pearson code oP16) with bonding interactions for interslab Ge{sub 2} dimers. The Li substitution for rare-earth elements in the RE{sub 4}LiGe{sub 4} system leads to a combined effect of the increased chemical pressure and the decreased valance electron concentration (VEC), which eventually results in the structure transformation from the Sm{sub 5}Ge{sub 4}-type with all broken interslab Ge–Ge bond for the parental RE{sub 5}Ge{sub 4} to the Gd{sub 5}Si{sub 4}-type structure for the ternary RE{sub 4}LiGe{sub 4} (RE=La, Ce, Pr, and Sm) system. Site-preference between rare-earth metals and Li is proven to generate energetically the most favorable atomic arrangements according to coloring-problem, and the rationale is provided using both the size-factor and the electronic-factor related, respectively, to site-volume and electronegativity as well as QVAL values. Tight-binding, linear-muffin-tin-orbital (TB-LMTO) calculations are performed to investigate electronic densities of states (DOS) and crystal orbital Hamilton population (COHP) curves. The influence of reduced VEC for chemical bonding including the formation of interslab Ge{sub 2} dimers is also discussed. The magnetic property measurements prove that the non-magnetic Li substitution leads to the ferromagnetic (FM)-like ground state for Ce{sub 4}LiGe{sub 4} and the co-existence of antiferromagntic (AFM) and FM ground states for Sm{sub 4}LiGe{sub 4}. - Graphical abstract: Reported is a combined effect of the chemical pressure and the reduced VEC caused by the smaller monovalent non-magnetic Li substitution for the larger trivalent magnetic rare-earth metals in the RE{sub 4}LiGe{sub 4} (RE=La, Ce, Pr, and Sm) system. This results in the structure

  16. Enhanced exchange bias effect in size modulated Sm{sub 0.5}Ca{sub 0.5}MnO{sub 3} phase separated manganite

    SciTech Connect (OSTI)

    Giri, S. K.; Nath, T. K.; Yusuf, S. M.; Mukadam, M. D.

    2014-03-07

    The effect of grain size modulation on exchange bias effect in CE-type antiferromagnetic Sm{sub 0.5}Ca{sub 0.5}MnO{sub 3} phase separated manganite is reported here. With the reduction of particle size, ferromagnetic clusters are found to form in the charge ordered antiferromagnetic matrix and gradually become larger. The horizontal and vertical shifts of the magnetic hysteresis loops in the field cooled magnetization process clearly indicate the size dependent exchange bias effect and it can be tuned with the reduction of particle sizes. The values of exchange bias parameter, i.e., exchange bias field (H{sub E}), coercivity (H{sub C}), remanence asymmetry (M{sub E}), and magnetic coercivity (M{sub C}) are found to depend strongly on the particle size. The variations of H{sub E} follow non-monotonic dependencies with reduction in particle size and show maximum (1205 Oe) at particle size of 150 nm at T = 5 K, which can be ascribed due to the changes in uncompensated surface spins. The values of H{sub E} and M{sub E} are found to decrease exponentially with increasing temperature below the spin- or cluster-glass like freezing temperature. The spin relaxation model has been employed for analysis of large magnetic training effect. The linear relationship between H{sub E} and M{sub E} further confirms the role of uncompensated surface spins. In view of spintronics application of manganites, the present observation of large exchange bias shift in this half-doped manganite may have great technological importance.

  17. FES BER HEP NP BES ASCR

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    December 2015 NERSC Science Highlights Science Highlights December 2015 Chemistry Simula'ons run at NERSC lead to the predic'on of a new phase of superionic ice, a special form of ice that could exist on Uranus and Neptune (Roberto Car , Princeton U., Nature Comm.) Fusion Energy 3D simula'ons run at NERSC help gain new insights into fusion plasma behavior that will improve the ability to stabilize a tokamak reactor (S. Jardin , Princeton Plasma Physics Lab, Phys. Rev. Lett.) High Energy &

  18. FES BER HEP NP BES ASCR

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    September 2015 NERSC Science Highlights NERSC Science Highlights September 2015 Fusion Energy 3D simula*ons yield new insights into why plasma in a Tokamak fusion reactor fails to reach required temperatures (R. Davidson/E. Belova , PPPL) Renewable Energy Ensemble simula*ons of flow through geothermal fracture networks improve reliability & economics of renewable geothermal energy. (Melior Innovations Inc.) Geophysics 3D scan of Earth's interior connects plumes of hot rock rising through the

  19. Lignin Valorization-final-sm

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Discovering effective methods of depolymerizing lignin will improve economics of biorefineries and create a renewable resource for chemicals Biofuels: Increasing the Value of Lignin Lignin Valorization Current lignocellulose biomass conversion to biofuels requires the breakdown of lignin to liberate sugars that can be converted into advanced fuels. The process results in a significant amount of lignin waste product that could be utilized for other byproducts improving the economics for

  20. Lignin Valorization-final-sm

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    renewable resource for chemicals Biofuels: Increasing the Value of Lignin Lignin Valorization Current lignocellulose biomass conversion to biofuels requires the breakdown of lignin ...

  1. Poster09sm.pdf

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

  2. Synchrotron X-ray diffraction and Raman spectroscopy of Ln{sub 3}NbO{sub 7} (Ln=La, Pr, Nd, Sm-Lu) ceramics obtained by molten-salt synthesis

    SciTech Connect (OSTI)

    Siqueira, K.P.F.; Soares, J.C.; Granado, E.; Bittar, E.M.; Paula, A.M. de; Moreira, R.L.; Dias, A.

    2014-01-15

    Ln{sub 3}NbO{sub 7} (Ln=La, Pr, Nd, Sm, Eu, Gd, Tb, Dy, Ho, Er, Tm, Yb, and Lu) ceramics were obtained by molten-salt synthesis and their structures were systematically investigated by synchrotron X-ray diffraction (SXRD), second harmonic generation (SHG) and Raman spectroscopy. It was observed that ceramics with the largest ionic radii (La, Pr, Nd) crystallized into the Pmcn space group, while the ceramics with intermediate ionic radii (Sm-Gd) exhibited a different crystal structure belonging to the Ccmm space group. For this last group of ceramics, this result was corroborated by SHG and Raman scattering and ruled out any possibility for the non-centrosymmetric C 222{sub 1} space group, solving a recent controversy in the literature. Finally, according to SXRD, Tb-Lu containing samples exhibited an average defect fluorite structure (Fm3{sup ¯}m space group). Nonetheless, broad scattering at forbidden Bragg reflections indicates the presence of short-range domains with lower symmetry. Vibrational spectroscopy showed the presence of six Raman-active modes, inconsistent with the average cubic fluorite structure, and in line with the existence of lower-symmetry nano-domains immersed in the average fluorite structure of these ceramics. - Graphical abstract: Raman spectrum for Sm{sub 3}NbO{sub 7} ceramics showing their 27 phonon modes adjusted through Lorentzian lines. According to synchrotron X-ray diffraction and Raman scattering, this material belongs to the space group Cmcm. Display Omitted - Highlights: • Ln{sub 3}NbO{sub 7} ceramics were obtained by molten-salt synthesis. • SXRD, SHG and Raman scattering confirmed orthorhombic and cubic structures. • Ccmm instead of C222{sub 1} is the correct structure for Sm–Gd ceramics. • Pmcn space group was confirmed for La-, Pr- and Nd-based ceramics. • For Tb–Lu ceramics, ordered domains of a pyrochlore structure were observed.

  3. Preparation and spectroscopic properties of rare-earth (RE) (RE = Sm, Eu, Tb, Dy, Tm)-activated K{sub 2}LnZr(PO{sub 4}){sub 3} (Ln = Y, La, Gd and Lu) phosphate in vacuum ultraviolet region

    SciTech Connect (OSTI)

    Zhang, Zhi-Jun; Lin, Xiao; Graduate School of Chinese Academy of Science, Beijing, 100039 ; Zhao, Jing-Tai; Zhang, Guo-Bin

    2013-02-15

    Graphical abstract: Display Omitted Highlights: ? We report the VUV spectroscopic properties of rare-earth ions in K{sub 2}LnZr(PO{sub 4}){sub 3}. ? The O{sup 2?}-Eu{sup 3+} charge transfer bands at about 220 nm have been observed. ? The 4f5d spin-allowed and spin-forbidden transitions of Tb{sup 3+} have been observed. ? There is energy transfer between the host and rare-earth activators. -- Abstract: Rare earth (RE = Sm, Eu, Tb, Dy and Tm)-activated K{sub 2}LnZr(PO{sub 4}){sub 3} (Ln = Y, La, Gd and Lu) have been synthesized by solid-state reaction method, and their vacuum ultraviolet (VUV) excitation luminescent characteristics have been investigated. The band in the wavelength range of 130157 nm and the other one range from 155 to 216 nm with the maximum at about 187 nm in the VUV excitation spectra of these compounds are attributed to the host lattice absorption and OZr charge transfer transition, respectively. The charge transfer bands (CTB) of O{sup 2?}-Sm{sup 3+}, O{sup 2?}-Dy{sup 3+} and O{sup 2?}-Tm{sup 3+}, in Sm{sup 3+}, Dy{sup 3+} and Tm{sup 3+}-activated samples, have not been obviously observed probably because the 2p electrons of oxygen are tightly bound to the zirconium ion in the host lattice. For Eu{sup 3+}-activated samples, the relatively weak O{sup 2?}-Eu{sup 3+} CTB at about 220 nm is observed. And for Tb{sup 3+}-activated samples, the bands at 223 and 258 nm are related to the 4f-5d spin-allowed and spin-forbidden transitions of Tb{sup 3+}, respectively. It is observed that there is energy transfer between the host lattice and the luminescent activators (e.g. Eu{sup 3+}, Tb{sup 3+}). From the standpoint of luminescent efficiency, color purity and chemical stability, K{sub 2}GdZr(PO{sub 4}){sub 3}:Sm{sup 3+}, Eu{sup 3+}, Tb{sup 3+} are attractive candidates for novel yellow, red, green-emitting PDP phosphors.

  4. Anisotropic magnetization and transport properties of RAgSb{sub 2} (R=Y, La-Nd, Sm, Gd-Tm)

    SciTech Connect (OSTI)

    Myers, Kenneth D.

    1999-11-08

    This study of the RAgSb{sub 2} series of compounds arose as part of an investigation of rare earth intermetallic compounds containing antimony with the rare earth in a position with tetragonal point symmetry. Materials with the rare earth in a position with tetragonal point symmetry frequently manifest strong anisotropies and rich complexity in the magnetic properties, and yet are simple enough to analyze. Antimony containing intermetallic compounds commonly possess low carrier densities and have only recently been the subject of study. Large single grain crystals were grown of the RAgSb{sub 2} (R=Y, La-Nd, Sm, Gd-Tm) series of compounds out of a high temperature solution. This method of crystal growth, commonly known as flux growth is a versatile method which takes advantage of the decreasing solubility of the target compound with decreasing temperature. Overall, the results of the crystal growth were impressive with the synthesis of single crystals of LaAgSb{sub 2} approaching one gram. However, the sample yield diminishes as the rare earth elements become smaller and heavier. Consequently, no crystals could be grown with R=Yb or Lu. Furthermore, EuAgSb{sub 2} could not be synthesized, likely due to the divalency of the Eu ion. For most of the RAgSb{sub 2} compounds, strong magnetic anisotropies are created by the crystal electric field splitting of the Hund's rule ground state. This splitting confines the local moments to lie in the basal plane (easy plane) for the majority of the members of the series. Exceptions to this include ErAgSb{sub 2} and TmAgSb{sub 2}, which have moments along the c-axis (easy axis) and CeAgSb{sub 2}, which at intermediate temperatures has an easy plane, but exchange coupling at low temperatures is anisotropic with an easy axis. Additional anisotropy is also observed within the basal plane of DyAgSb{sub 2}, where the moments are restricted to align along one of the {l_angle}110{r_angle} axes. Most of the RAgSb{sub 2} compounds

  5. Bright reddish-orange emission and good piezoelectric properties of Sm{sub 2}O{sub 3}-modified (K{sub 0.5}Na{sub 0.5})NbO{sub 3}-based lead-free piezoelectric ceramics

    SciTech Connect (OSTI)

    Hao, Jigong; Xu, Zhijun Chu, Ruiqing; Li, Wei; Du, Juan

    2015-05-21

    Reddish orange-emitting 0.948(K{sub 0.5}Na{sub 0.5})NbO{sub 3}-0.052LiSbO{sub 3}-xmol%Sm{sub 2}O{sub 3} (KNN-5.2LS-xSm{sub 2}O{sub 3}) lead-free piezoelectric ceramics with good piezoelectric properties were fabricated in this study, and the photoluminescence and electrical properties of the ceramics were systematically studied. Results showed that Sm{sub 2}O{sub 3} substitution into KNN-5.2LS induces a phase transition from the coexistence of orthorhombic and tetragonal phases to a pseudocubic phase and shifts the polymorphic phase transition (PPT) to below room temperature. The temperature stability and fatigue resistance of the modified ceramics were significantly improved by Sm{sub 2}O{sub 3} substitution. The KNN-5.2LS ceramic with 0.4 mol. % Sm{sub 2}O{sub 3} exhibited temperature-independent properties (25–150 °C), fatigue-free behavior (up to 10{sup 6} cycles), and good piezoelectric properties (d{sub 33}{sup * }= 230 pm/V, d{sub 33} = 176 pC/N, k{sub p} = 35%). Studies on the photoluminescence properties of the samples showed strong reddish-orange emission upon blue light excitation; these emission intensities were strongly dependent on the doping concentration and sintering temperature. The 0.4 mol. % Sm{sub 2}O{sub 3}-modified sample exhibited temperature responses over a wide temperature range of 10–443 K. The maximum sensing sensitivity of the sample was 7.5 × 10{sup −4} K at 293 K, at which point PPT occurred. A relatively long decay lifetime τ of 1.27–1.40 ms and a large quantum yield η of 0.17–0.19 were obtained from the Sm-modified samples. These results suggest that the KNN-5.2LS-xSm{sub 2}O{sub 3} system presents multifunctional properties and significant technological potential in novel multifunctional devices.

  6. CaO-MgO-Al2O3-SiO2 (CMAS) corrosion of Gd2Zr2O7 and Sm2Zr2O7

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Wang, Honglong; Bakal, Ahmet; Zhang, Xingxing; Tarwater, Emily; Sheng, Zhizhi; Fergus, Jeffrey W.

    2016-08-08

    Ceramic thermal barrier coatings are applied to superalloys used in gas turbine engineering to increase the operating temperature and the energy conversion efficiency. However, dust consisting of CaO-MgO-Al2O3-SiO2 (CMAS) from the air can be injected into the engines and corrode the thermal barrier coatings. Lanthanide zirconates are promising materials in thermal barrier coatings due to their low thermal conductivities, good phase stability and good corrosion resistance. However, the corrosion resistance mechanism of CMAS on lanthanide zirconates is still not clearly understood. In this work, the corrosion mechanism of Gd2Zr2O7 and Sm2Zr2O7 in CMAS is studied. Here, the results show thatmore » the CMAS can easily react with lanthanide zirconate thermal barrier coatings to form a dense layer, which can resist further corrosion« less

  7. DC current induced metal-insulator transition in epitaxial Sm{sub 0.6}Nd{sub 0.4}NiO{sub 3}/LaAlO{sub 3} thin film

    SciTech Connect (OSTI)

    Huang, Haoliang; CAS Key Laboratory of Materials for Energy Conversion, Department of Materials Science and Engineering, University of Science and Technology of China, Hefei, Anhui 230026 ; Luo, Zhenlin Yang, Yuanjun; Yang, Mengmeng; Wang, Haibo; Hu, Sixia; Bao, Jun; National Synchrotron Radiation Laboratory and School of Nuclear Science and Technology, University of Science and Technology of China, Hefei, Anhui 230026 ; Yun, Yu; Meng, Dechao; Lu, Yalin; Gao, Chen; CAS Key Laboratory of Materials for Energy Conversion, Department of Materials Science and Engineering, University of Science and Technology of China, Hefei, Anhui 230026; National Synchrotron Radiation Laboratory and School of Nuclear Science and Technology, University of Science and Technology of China, Hefei, Anhui 230026

    2014-05-15

    The metal-insulator transition (MIT) in strong correlated electron materials can be induced by external perturbation in forms of thermal, electrical, optical, or magnetic fields. We report on the DC current induced MIT in epitaxial Sm{sub 0.6}Nd{sub 0.4}NiO{sub 3} (SNNO) thin film deposited by pulsed laser deposition on (001)-LaAlO{sub 3} substrate. It was found that the MIT in SNNO film not only can be triggered by thermal, but also can be induced by DC current. The T{sub MI} of SNNO film decreases from 282 K to 200 K with the DC current density increasing from 0.003 × 10{sup 9} A•m{sup −2} to 4.9 × 10{sup 9} A•m{sup −2}. Based on the resistivity curves measured at different temperatures, the MIT phase diagram has been successfully constructed.

  8. Structural and electrical transport properties of La{sub 0.8}Sm{sub 0.05}K{sub 0.15}MnO{sub 3} manganites

    SciTech Connect (OSTI)

    Shaikh, M. W.; Mansuri, I.; Varshney, Dinesh

    2014-04-24

    Polycrystalline sample of single-phase La{sub 0.8}Sm{sub 0.05}K{sub 0.15}MnO{sub 3} perovskite compound have been synthesized by solid-state reaction route. X-ray diffraction patterns accompanied by Rietveldrefined crystal structure parameters reveal the rhombohedral structure with space group R 3C. Electrical resistivity infers transition from metallic to insulator phase at 537 K. The application of magnetic field of 8 T, suppresses the resistivity. The metallic resistivity is retraced by considering electronphonon, electronelectron and electron-spin-fluctuation interactions while insulating behaviour is analysed with small polaron conduction model.

  9. Heavy surface state in a possible topological Kondo insulator: Magnetothermoelectric transport on the (011) plane of SmB6

    SciTech Connect (OSTI)

    Luo, Yongkang; Chen, Hua; Dai, Jianhui; Xu, Zhu -an; Thompson, J. D.

    2015-02-25

    Motivated by the high sensitivity to Fermi surface topology and scattering mechanisms in magnetothermoelectric transport, we have measured the thermopower and Nernst effect on the (011) plane of the proposed topological Kondo insulator SmB6. These experiments, together with electrical resistivity and Hall effect measurements, suggest that the (011) plane also harbors a metallic surface with an effective mass on the order of 10–102 m0. The surface and bulk conductances are well distinguished in these measurements and are categorized into metallic and nondegenerate semiconducting regimes, respectively. As a result, electronic correlations play an important role in enhancing scattering and also contribute to the heavy surface state.

  10. New rare-earth metal germanides with bismuth substitution. Synthesis, structural variations, and magnetism of the RE[Bi{sub x}Ge{sub 1-x}]{sub 2} (RE=Y, Pr, Nd, Sm, Gd-Tm, Lu) compounds

    SciTech Connect (OSTI)

    Zhang, Jiliang; Hmiel, Benjamin; Antonelli, Anthony; Tobash, Paul H.; Bobev, Svilen; Saha, Shanta; Kirshenbaum, Kevin; Greene, Richard L.; Paglione, Johnpierre

    2012-12-15

    Single-crystals of the novel rare-earth metal-bismuth digermanides with idealized formula RE[Bi{sub x}Ge{sub 1-x}]{sub 2} (RE=Y, Pr, Nd, Sm, Gd-Tm, Lu; x<0.16(1)) have been obtained using the Bi-flux technique. Their structures have been established by single-crystal X-ray diffraction; they can be divided into three classes, closely related to the ZrSi{sub 2} structure with the space group Cmcm (no. 63). The structural relationship and the variations with the type of the rare-earth metal have been explored and discussed. Temperature-dependent magnetization measurements on the single-crystals reveal magnetic behavior, which have been rationalized based on the mean-field theory. At cryogenic temperatures, the localized 4f electrons in most of the compounds exhibit antiferromagnetic ordering, mediated by the conduction electrons via Ruderman-Kittel-Kasuya-Yosida (RKKY) exchange interactions. - Graphical abstract: This paper details the synthesis and the structural characterization of an extended series of rare-earth metal-bismuth-germanides RE[Bi{sub x}Ge{sub 1-x}]{sub 2} (RE=Y, Pr-Sm, Gd-Tm, Lu). They crystallize with the same extended symmetry (space group Cmcm), but with three distinct structures, which are closely related. Magnetization measurements show low-temperature antiferromagnetic ordering. RE[Bi{sub x}Ge{sub 1-x}]{sub 2} are the first compounds between these elements. Highlights: Black-Right-Pointing-Pointer RE[Bi{sub x}Ge{sub 1-x}]{sub 2} (RE=rare-earth metal) are the first compounds of the respective elements. Black-Right-Pointing-Pointer Their structures are closely related. Black-Right-Pointing-Pointer Three structures can be distinguished based on the packing of the REGe{sub 6} triangular prisms. Black-Right-Pointing-Pointer All compounds show low-temperature antiferromagnetic ordering.

  11. Structural and Magnetothermal Properties of Compounds: Yb5SixGe4-x,Sm5SixGe4-x, EuO, and Eu3O4

    SciTech Connect (OSTI)

    Kyunghan Ahn

    2007-05-09

    The family of R{sub 5}Si{sub x}Ge{sub 4-x} alloys demonstrates a variety of unique physical phenomena related to magneto-structural transitions associated with reversible breaking and reforming of specific bonds that can be controlled by numerous external parameters such as chemical composition, magnetic field, temperature, and pressure. Therefore, R{sub 5}Si{sub x}Ge{sub 4-x} systems have been extensively studied to uncover the mechanism of the extraordinary magneto-responsive properties including the giant magnetoresistance (GMR) and colossal magnetostriction, as well as giant magnetocaloric effect (GMCE). Until now, more than a half of possible R{sub 5}Si{sub x}Ge{sub 4-x} pseudobinary systems have been completely or partially investigated with respect to their crystallography and phase relationships (R = La, Pr, Nd, Gd, Tb, Dy, Er, Lu, Y). Still, there are other R{sub 5}Si{sub x}Ge{sub 4-x} systems (R = Ce, Sm, Ho, Tm, and Yb) that are not studied yet. Here, we report on phase relationships and structural, magnetic, and thermodynamic properties in the Yb{sub 5}Si{sub x}Ge{sub 4-x} and Sm{sub 5}Si{sub x}Ge{sub 4-x} pseudobinary systems, which may exhibit mixed valence states. The crystallography, phase relationships, and physical properties of Yb{sub 5}Si{sub x}Ge{sub 4-x} alloys with 0 {le} x {le} 4 have been examined by using single crystal and powder x-ray diffraction at room temperature, and dc magnetization and heat capacity measurements between 1.8 K and 400 K in magnetic fields ranging from 0 to 7 T. Unlike the majority of R{sub 5}Si{sub x}Ge{sub 4-x} systems studied to date, where R is the rare earth metal, all Yb-based germanide-silicides with the 5:4 stoichiometry crystallize in the same Gd{sub 5}Si{sub 4}-type structure. The magnetic properties of Yb{sub 5}Si{sub x}Ge{sub 4-x} materials are nearly composition-independent, reflecting the persistence of the same crystal structure over the whole range of x from 0 to 4. Both the crystallographic and

  12. Hydrogen in polar intermetallics: Syntheses and structures of the ternary Ca5Bi3D0.93, Yb5Bi3Hx, and Sm5Bi3H~1 by powder neutron or single crystal X-ray diffraction

    SciTech Connect (OSTI)

    Leon-Escamilla, E. Alejandro; Dervenagas, Panagiotis; Stasis, Constantine; Corbett, John D.

    2010-01-01

    The syntheses of the title compounds are described in detail. Structural characterizations from refinements of single crystal X-ray diffraction data for Yb{sub 5}Bi{sub 3}H{sub x} and Sm{sub 5}Bi{sub 3}H{sub 1} and of powder neutron diffraction data for Ca{sub 5}Bi{sub 3}D{sub 0.93(3)} are reported. These confirm that all three crystallize with the heavy atom structure type of {beta}-Yb{sub 5}Sb{sub 3}, and the third gives the first proof that the deuterium lies in the center of nominal calcium tetrahedra, isostructural with the Ca{sub 5}Sb{sub 3}F-type structure. These Ca and Yb phases are particularly stable with respect to dissociation to Mn{sub 5}Si{sub 3}-type product plus H{sub 2}. Some contradictions in the literature regarding Yb{sub 5}Sb{sub 3} and Yb{sub 5}Sb{sub 3}H{sub x} phases are considered in terms of adventitious hydrogen impurities that are generated during reactions in fused silica containers at elevated temperatures.

  13. An investigation of low temperature electronic phase arrest in Sm{sub 0.55}Sr{sub 0.45}MnO{sub 3} phase separated manganite

    SciTech Connect (OSTI)

    Giri, S. K. Nath, T. K.

    2014-02-07

    The temperature dependence of electronic-transport and magneto-transport of polycrystalline Sm{sub 0.55}Sr{sub 0.45}MnO{sub 3} manganite at low temperatures has been investigated in detail. The low temperature resistivity data show a distinct minimum in the resistivity versus temperature plots for all fields. The low temperature resistivity upturn below this minimum has been fitted to an expression, which includes three terms, namely, residual resistivity, inelastic scattering, and electron-electron (e-e) interaction or Kondo effects. It has been found that the dominating mechanism is e-e interaction. The resistivity of the sample shows strong dependence on the magnetic fieldtemperature history. The electronic-transport property clearly confirms that the electronic phase of the sample gets arrested to a low resistive state during field cooling and cannot return to its original state even after the magnetic field is removed. The magnetoresistance of the sample also shows a strong irreversibility with respect to the sweeping of the magnetic field between its highest positive and negative values. Moreover, the resistivity of the sample is found to be time dependent. All the observed phenomena have been explained through the phase separation scenario and kinetic arrest of electronic phase.

  14. Performances of YBaCo1.4Cu0.6O5+δ–Ce0.8Sm0.2O1.9 composite cathodes for intermediate-temperature solid oxide fuel cells

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Wang, Lizhong; Peng, Lu; Hu, Michael Z.; Lü, Shiquan; Meng, Xiangwei; Yu, Bo; Wei, Maobin; Fan, Hougang; Yang, Lili

    2015-08-20

    In this paper, the electrochemical properties of YBaCo1.4Cu0.6O5+δ–xCe0.8Sm0.2O1.9 (YBCC–xSDC, x=20, 30, 40, 50 wt%) have been investigated for the potential application in intermediate-temperature solid oxide fuel cells (IT-SOFCs). No chemical reactions between YBCC cathode and SDC electrolyte, and YBCC and La0.9Sr0.1Ga0.8Mg0.2O3-δ (LSGM) occur. The thermal expansion coefficient (TEC) of YBCC cathode decreases with SDC addition. The TEC of YBCC–30SDC cathode is 13.60×10–6 K-1 from 30 to 850 °C in air and it exhibits the best electrochemical performance among the YBCC–xSDC cathodes. The polarization resistance (Rp) of YBCC–30SDC is 0.027 Ω cm2 at 850 °C, 0.044 Ω cm2 at 800 °Cmore » and 0.075 Ω cm2 at 750 °C. The maximum power density value of electrolyte-based cell with YBCC–30SDC cathode is 662, 483 and 319 mW cm-2 at 850, 800 and 750 °C, respectively. Finally, preliminary results indicate that YBCC–30SDC is especially promising as a cathode for IT-SOFCs.« less

  15. Synthesis of nanocrystalline REBO{sub 3} (RE=Y, Nd, Sm, Eu, Gd, Ho) and YBO{sub 3}:Eu using a borohydride-based solution precursor route

    SciTech Connect (OSTI)

    Henkes, Amanda E.; Schaak, Raymond E.

    2008-12-15

    A solution precursor route has been used to synthesize a series of nanocrystalline rare-earth borates. Amorphous precursor powders are precipitated during an aqueous reaction between RE{sup 3+} and NaBH{sub 4}, and the isolated powders can be annealed in air at 700 deg. C to form YBO{sub 3}, NdBO{sub 3}, SmBO{sub 3}, EuBO{sub 3}, GdBO{sub 3}, and HoBO{sub 3}. YBO{sub 3}:Eu formed using this strategy shows red-orange emission properties that are similar to high-quality nanocrystals prepared by other methods. The materials have been characterized by FTIR spectroscopy, powder XRD, SEM, DSC, UV-Vis fluorimetry, and TEM with EDS and element mapping. - Graphical abstract: Amorphous nanoscopic precursor powders are formed through the aqueous reaction of RE{sup 3+} with NaBH{sub 4}. Once isolated, the powders can be annealed at 700 deg. C in air to form a series of nanocrystalline REBO{sub 3} orthoborates. Nanocrystalline YBO{sub 3}:Eu formed using this strategy shows red-orange emission properties when excited with UV light.

  16. Advanced Enzymes and Mixtures-final-sm

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    biorefinery conditions lowers conversion costs of lignocellulosic biomass to biofuel Genes are synthesized and expressed in an appropriate expression host, typically in E. Coli. ...

  17. Variable temperature electrochemical strain microscopy of Sm...

    Office of Scientific and Technical Information (OSTI)

    Sponsoring Org: SC USDOE - Office of Science (SC) Country of Publication: United States Language: English Subject: Solid-oxide fuel cells (SOFC); Electrochemical Strain Microscopy ...

  18. LANFILGAS(sm) process. Technology spotlight report

    SciTech Connect (OSTI)

    1995-08-01

    The United States is facing a garbage crisis. Several areas of the country have already run out of landfill space, and recent studies indicate that many other areas will be experiencing the same problem with the next ten years. Institute of Gas Technology (IGT) has patented an advanced biogasification technology called LANFILGAS that accelerates the stabilization of landfills through anaerobic composting and recovers the methane gas for its energy value. Anaerobic composting, or digestion, is a natural process that takes place in every landfill. It is generally uncontrolled, however, and can take up to 30 years to stabilize a landfill.

  19. Recycling & Reuse of BOF - BOP SM Slags

    SciTech Connect (OSTI)

    2002-01-01

    New Technologies and Methodologies May Allow Value-Added Utilization of Steelmaking Slag Thus Reducing Waste and Use of Landfills, and Saving Energy.

  20. Advanced Enzymes and Mixtures-final-sm

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    enzyme mixtures to meet biorefinery conditions lowers conversion costs of lignocellulosic biomass to biofuel Genes are synthesized and expressed in an appropriate expression host, typically in E. Coli. Each enzyme is screened for activity across a range of temperatures, pH and biorefinery relevant conditions. An enzyme mixture developed by Sandia researchers that functions optimally at 70 °C and 20% of the ionic liquid 1-ethyl-3-methylimidazolium acetate. Biofuels: Advanced Enzymes and Mixtures

  1. Syntheses, structure and rare earth metal photoluminescence of new and known isostructural A{sub 2}Mo{sub 4}Sb{sub 2}O{sub 18} (A=Ce, Pr, Sm, Eu, Gd, Tb, Dy, Ho, Er, Tm, Yb, Lu) compounds

    SciTech Connect (OSTI)

    Mohitkar, Shrikant A.; Kalpana, G.; Vidyasagar, K.

    2011-04-15

    Nine new A{sub 2}Mo{sub 4}Sb{sub 2}O{sub 18} (A=Ce, Pr, Eu, Tb, Ho, Er, Tm, Yb, Lu) compounds have been synthesized by solid-state reactions. They are isostructural with six reported analogues of yttrium and other lanthanides and the monoclinic unit cell parameters of all fifteen of them vary linearly with the size of A{sup 3+} ion. Single crystal X-ray structures of eight A{sub 2}Mo{sub 4}Sb{sub 2}O{sub 18} (A=Ce, Pr, Eu, Gd, Tb, Ho, Er, Tm) compounds have been determined. Neat A{sub 2}Mo{sub 4}Sb{sub 2}O{sub 18} (A=Pr, Sm, Eu, Tb, Dy, Ho, Er, Tm) compounds exhibit characteristic rare earth metal photoluminescence. -- Graphical abstract: Among the fifteen isostructural A{sub 2}Mo{sub 4}Sb{sub 2}O{sub 18} (A=rare earth metal) molybdoantimonites, eight (A=Pr, Sm, Eu, Tb, Dy, Ho, Er, Tm) compounds exhibit neat characteristic lanthanide photoluminescence in the 200-800 nm range at room temperature. Display Omitted Research highlights: {yields} Syntheses of nine new A{sub 2}Mo{sub 4}Sb{sub 2}O{sub 18} (A=Ce, Pr, Eu, Tb, Ho, Er, Tm, Yb, Lu) compounds. {yields} X-ray structures of eight A{sub 2}Mo{sub 4}Sb{sub 2}O{sub 18} (A=Ce, Pr, Eu, Gd, Tb, Ho, Er, Tm) compounds. {yields} Photoluminescence of neat A{sub 2}Mo{sub 4}Sb{sub 2}O{sub 18} (A=Pr, Sm, Eu, Tb, Dy, Ho, Er, Tm) compounds.

  2. NP2010: An Assessment and Outlook for Nuclear Physics

    SciTech Connect (OSTI)

    Lancaster, James

    2014-05-22

    This grant provided partial support for the National Research Council’s (NRC) decadal survey of nuclear physics. This is part of NRC’s larger effort to assess and discuss the outlook for different fields in physics and astronomy, Physics 2010, which takes place approximately every ten years. A report has been prepared as a result of the study that is intended to inform those who are interested about the current status of research in this area and to help guide future developments of the field. A pdf version of the report is available for download, for free, at http://www.nap.edu/catalog.php?record_id=13438. Among the principal conclusions reached in the report are that the nuclear physics program in the United States has been especially well managed, principally through a recurring long-range planning process conducted by the community, and that current opportunities developed pursuant to that planning process should be exploited. In the section entitled “Building the Foundation for the Future,” the report notes that attention needs to be paid to certain elements that are essential to the continued vitality of the field. These include ensuring that education and research at universities remain a focus for funding and that a plan be developed to ensure that forefront-computing resources, including exascale capabilities when developed, be made available to nuclear science researchers. The report also notes that nimbleness is essential for the United States to remain competitive in a rapidly expanding international nuclear physics arena and that streamlined and flexible procedures should be developed for initiating and managing smaller-scale nuclear science projects.

  3. FES BER HEP NP BES ASCR NERSC Science Highlights

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    March 2016 Science Highlights March 2016 Energy & Environment Simula'ons support findings that migra'on of liquids and gases due to fracking have not had a widespread impact on drinking water. (Moridis , LBNL, Water Resources Research) Climate Researchers have reduced the 'me needed to detect important features in large climate datasets from years to hours. (O'Brien, LBNL. Env. Sci. & Tech) High Energy Physics New tools handle increasingly large datasets produced by ATLAS experiments at

  4. Microsoft Word - TSA _NP Boilerplate- revised 7-29-13

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    including any subsequent amendment. A. The Sponsor shall advance the following amount in United States dollars (U.S.) at the time shown below: , Upon execution...

  5. 24052_NP_ESnet_Cover_150_v3

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Network Requirements Report of the Nuclear Physics Network Requirements Workshop Conducted ... the University of California. 3 Nuclear Physics Network Requirements Office of Nuclear ...

  6. High power femtosecond lasers at ELI-NP

    SciTech Connect (OSTI)

    Dabu, Razvan

    2015-02-24

    Specifications of the high power laser system (HPLS) designed for nuclear physics experiments are presented. Configuration of the 2 × 10 PW femtosecond laser system is described. In order to reach the required laser beam parameters, advanced laser techniques are proposed for the HPLS: parametric amplification and cross-polarized wave generation for the intensity contrast improvement and spectral broadening, acousto-optic programmable filters to compensate for spectral phase dispersion, optical filters for spectrum management, combined methods for transversal laser suppression.

  7. Future directions of accelerator-based NP and HEP facilities

    SciTech Connect (OSTI)

    Roser, T.

    2011-07-24

    Progress in particle and nuclear physics has been closely connected to the progress in accelerator technologies - a connection that is highly beneficial to both fields. This paper presents a review of the present and future facilities and accelerator technologies that will push the frontiers of high-energy particle interactions and high intensity secondary particle beams.

  8. NP2017-DRAFT-FINALJan05WithNumber

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ... S cientific C omputing C enter ( NERSC) Editors Richard A . ... and the use of nuclei to search for evidence o f n ew p ... experimental results in terms of our current ...

  9. FES BER HEP NP BES ASCR NERSC Science Highlights

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    detail. (Saye, LBNL, Science Advances) High Energy Physics Model confirms existence of an ... Brown-Dwarf Companion to Accre*ng White Dwarf HEP PI: E. Baron (Univ. of Oklahoma) ...

  10. Net Power Technology NP Holdings or NPH | Open Energy Information

    Open Energy Info (EERE)

    Holdings or NPH) Place: Chanchun, Jilin Province, China Sector: Efficiency, Renewable Energy Product: China-based company, focused on electricity storage systems based on...

  11. 27264_ESNet_HEP_NP_Cover_final3_102113

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ... With ESnet's knowledge and experience, these local partnerships made possible the Eastern ... Russia, Saudi Arabia, Slovenia, Spain, Taiwan, Thailand, Turkey, Ukraine, and Vietnam. ...

  12. Phase evolution studies in CaZrTi{sub 2}O{sub 7}−RE{sub 2}Ti{sub 2}O{sub 7} (RE = Nd{sup 3+}, Sm{sup 3+}) system: Futuristic ceramic host matrices for nuclear waste immobilization

    SciTech Connect (OSTI)

    Jafar, M. Achary, S. N. Tyagi, A. K.

    2014-04-24

    Series of compositions with general stoichiometry as Ca{sub 1−x}Zr{sub 1−x}RE{sub 2x}Ti{sub 2}O{sub 7} (RE = Nd{sup 3+}, Sm{sup 3+}) were prepared by solid state reaction and characterized by powder x-ray diffraction technique to unravel the phase fields in the title systems. The phase fields in CaZrTi{sub 2}O{sub 7−}Nd{sub 2}Ti{sub 2}O{sub 7} and CaZrTi{sub 2}O{sub 7−}Sm{sub 2}Ti{sub 2}O{sub 7} systems differed significantly at the rareearth rich regions. The common phase fields like zirconolite-2M, zirconolite-4M, cubic perovskite are observed at the zirconolite rich regions of both systems. Depending on the structure of RE{sub 2}Ti{sub 2}O{sub 7} phase, the cubic pyrochlore or monoclinic RE{sub 2}Ti{sub 2}O{sub 7} phases are observed in the studied system. The observed phase fields in these two systems indicate ionic radius of the rare-earth ion has a dominating role in the phase relations. Further details of the phases and their homogeneity are explained in the text of the manuscript.

  13. Improvement in J{sub c} performance below liquid nitrogen temperature for SmBa{sub 2}Cu{sub 3}O{sub y} superconducting films with BaHfO{sub 3} nano-rods controlled by low-temperature growth

    SciTech Connect (OSTI)

    Miura, S. Yoshida, Y.; Ichino, Y.; Xu, Q.; Matsumoto, K.; Ichinose, A.; Awaji, S.

    2016-01-01

    For use in high-magnetic-field coil-based applications, the critical current density (J{sub c}) of REBa{sub 2}Cu{sub 3}O{sub y} (REBCO, where RE = rare earth) coated conductors must be isotropically improved, with respect to the direction of the magnetic field; these improvements must be realized at the operating conditions of these applications. In this study, improvement of the J{sub c} for various applied directions of magnetic field was achieved by controlling the morphology of the BaHfO{sub 3} (BHO) nano-rods in a SmBCO film. We fabricated the 3.0 vol. % BHO-doped SmBCO film at a low growth temperature of 720 °C, by using a seed layer technique (T{sub s} = 720 °C film). The low-temperature growth resulted in a morphological change in the BHO nano-rods. In fact, a high number density of (3.1 ± 0.1) × 10{sup 3} μm{sup −2} of small (diameter: 4 ± 1 nm), discontinuous nano-rods that grew in various directions, was obtained. In J{sub c} measurements, the J{sub c} of the T{sub s} = 720 °C film in all directions of the applied magnetic field was higher than that of the non-doped SmBCO film. The J{sub c}{sup min} (6.4 MA/cm{sup 2}) of the former was more than 6 times higher than that (1.0 MA/cm{sup 2}) of the latter at 40 K, under 3 T. The aforementioned results indicated that the discontinuous BHO nano-rods, which occurred with a high number density, exerted a 3D-like flux pinning at the measurement conditions considered. Moreover, at 4.2 K and under 17 T, a flux pinning force density of 1.6 TN/m{sup 3} was realized; this value was comparable to the highest value recorded, to date.

  14. Size and charge effects of dopant M on the unit-cell parameters of monoclinic zirconia solid solutions Zr{sub 0.98}M{sub 0.02}O{sub 2{minus}{delta}} (M = Ce, La, Nd, Sm, Y, Er, Yb, Sc, Mg, Ca)

    SciTech Connect (OSTI)

    Yashima, Masatomo; Kakihana, Masato; Yoshimura, Masahiro; Hirose, Teruo; Suzuki, Yasuo

    1997-01-01

    The crystal structure of monoclinic phase [P2{sub 1}/c, Z = 4] has been refined by the Rietveld analysis of X-ray powder diffraction data to study the size and charge effects of dopant M{sup n+} on the unit-cell parameters of monoclinic ZrO{sub 2}-2 mol% MO{sub n/2} solid solutions (n = 4 for M = Ce; n = 3 for M = La, Nd, Sm, Y, Er, Yb, Sc; and n = 2 for M = Mg and Ca). For trivalent dopant (n = 3), the unit-cell parameters a{sub m}, b{sub m}, c{sub m} and unit-cell volume increase and {beta}{sub m} decreases with an increase of dopant size. Unit-cell volume increases with increasing of dopant charge n.

  15. Nepal-Climate and Carbon Unit | Open Energy Information

    Open Energy Info (EERE)

    and capacity in renewable energy dissemination and create linkages with climate resilience and low-carbon growth that builds on SNV's core strengths of developing localised RE...

  16. Microsoft Word - Nepal_10km_solar_country_report.doc

    Open Energy Info (EERE)

    of 5x5 km. Figure 1: The solar irradiance data is derived from Meteosat a 0 (red circle) and at 63 East (orange circle). The brightened area marks the quantitatively...

  17. Alternate Energy Promotion Centre, Nepal Alternate Energy Promotion...

    Open Energy Info (EERE)

    rate of SHS dissemination is around 16,000 per annum. A typical SHS system has 40 Wp of solar panel with BOS (balance of system) sized adequately for 3 autonomy days. Important...

  18. Nepal-UNEP Green Economy Advisory Services | Open Energy Information

    Open Energy Info (EERE)

    the Middle East, including the following: Armenia, Azerbaijan, Barbados, Burkina Faso, China, Egypt, Ghana, Indonesia, Jordan, Kenya, Korea, Mali, Mexico, Moldova, Mongolia,...

  19. Nepal-Climate Finance Readiness Programme | Open Energy Information

    Open Energy Info (EERE)

    support from the German Federal Ministry for the Environment, Nature Conservation and Nuclear Safety (BMU). The Programme will prepare developing countries to effectively and...

  20. Nepal-Low Emissions Asian Development (LEAD) Program | Open Energy...

    Open Energy Info (EERE)

    the growth of greenhouse gas emissions. The LEAD program supports and enhances country-led development programs, plans, and policies, and complements efforts of other...

  1. Nepal-DLR Resource Assessments | Open Energy Information

    Open Energy Info (EERE)

    Area Renewable Energy Topics Background analysis, Resource assessment Resource Type Softwaremodeling tools, Dataset, Maps Website http:www.dlr.dettdesktopde Program Start...

  2. The emergence of magnetic properties in (Pb{sub 0.845}Sm{sub 0.08}Fe{sub 0.035})(Ti{sub 0.98}Mn{sub 0.02})O{sub 3} and (Pb{sub 0.88}Nd{sub 0.08})(Ti{sub 0.98}Mn{sub 0.02})O{sub 3} perovskite ceramics

    SciTech Connect (OSTI)

    Craciun, F.; Dimitriu, E.; Grigoras, M.; Lupu, N.; Vasile, B. S.; Cernea, M.

    2014-08-21

    The emergence of magnetic properties and quadratic magnetoelectric coupling in a material with outstanding ferroelectric properties has been pursued. Thus, the multiferroicity driven by the substitution of rare earth R{sup 3+} ions (R = Sm, Nd) on the A-site of PbTiO{sub 3} perovskite ceramics has been investigated. In some samples, a transition element with large ionic radius, like Fe{sup 2+}, has been also added on the A site. Polycrystalline ceramic samples with composition (Pb{sub 1-3x/2-y}R{sub x}Fe{sub y}) (Ti{sub 0.98}Mn{sub 0.02})O{sub 3} (R = Sm; x = 0.08, y = 0.035) and (Pb{sub 1−3x/2}R{sub x})(Ti{sub 0.98}Mn{sub 0.02})O{sub 3} (R = Nd, x = 0.08) have been prepared by conventional solid state ceramic processing, starting from reagent grade oxide powders. X-ray diffraction analysis confirmed the obtaining of a crystalline phase with tetragonal P4 mm symmetry. Transmission electron microscopy and high resolution transmission electron microscopy investigations have been carried out in order to analyze the local structure. Temperature dependence of dielectric permittivity revealed a strong anomaly at the temperature T{sub c} of the paraelectric-ferroelectric phase transition. Transition temperature values depend on the R ion type and are lower than in pure lead titanate by 80–100 K. A broad anomaly of dielectric permittivity is found below 140–180 K, where magnetization also increases due to the quadratic magnetoelectric coupling between ferroelectric and magnetic states. For the (Pb{sub 0.845}Sm{sub 0.08}Fe{sub 0.035})(Ti{sub 0.98}Mn{sub 0.02})O{sub 3} composition, the piezoelectric charge coefficient at room temperature was d{sub 31} ∼−6.5 pC/N and the remanent magnetization M{sub r} at room temperature was about 0.1 emu/g.

  3. Performances of YBaCo1.4Cu0.6O5+δ–Ce0.8Sm0.2O1.9 composite cathodes for intermediate-temperature solid oxide fuel cells

    SciTech Connect (OSTI)

    Wang, Lizhong; Peng, Lu; Hu, Michael Z.; Lü, Shiquan; Meng, Xiangwei; Yu, Bo; Wei, Maobin; Fan, Hougang; Yang, Lili

    2015-08-20

    In this paper, the electrochemical properties of YBaCo1.4Cu0.6O5+δ–xCe0.8Sm0.2O1.9 (YBCC–xSDC, x=20, 30, 40, 50 wt%) have been investigated for the potential application in intermediate-temperature solid oxide fuel cells (IT-SOFCs). No chemical reactions between YBCC cathode and SDC electrolyte, and YBCC and La0.9Sr0.1Ga0.8Mg0.2O3-δ (LSGM) occur. The thermal expansion coefficient (TEC) of YBCC cathode decreases with SDC addition. The TEC of YBCC–30SDC cathode is 13.60×10–6 K-1 from 30 to 850 °C in air and it exhibits the best electrochemical performance among the YBCC–xSDC cathodes. The polarization resistance (Rp) of YBCC–30SDC is 0.027 Ω cm2 at 850 °C, 0.044 Ω cm2 at 800 °C and 0.075 Ω cm2 at 750 °C. The maximum power density value of electrolyte-based cell with YBCC–30SDC cathode is 662, 483 and 319 mW cm-2 at 850, 800 and 750 °C, respectively. Finally, preliminary results indicate that YBCC–30SDC is especially promising as a cathode for IT-SOFCs.

  4. An Introduction to Architectural Surety(SM) Education

    SciTech Connect (OSTI)

    Matalucci, R.V.; Miyoshi, D.S.

    1998-09-01

    This report describes the Sandia activities in the developing field management approach to enhancing National Laboratories (Sandia) educational outreach of architectural and infrastructure surety, a risk the safety, security, and reliability of facilities, systems, and structures. It begins with a description of the field of architectural and infrastmcture surety, including Sandia's historical expertise and experience in nuclear weapons surety. An overview of the 1996 Sandia Workshop on Architectural SuretysM is then provided to reference the initiation of the various activities. This workshop established the need for a surety education program at the University level and recommended that Sandia develop the course material as soon as possible. Technical material was assembled and the course was offered at the University of New Mexico (UNM) during the 1997 spring semester. The bulk of this report accordingly summarizes the lecture material presented in this pioneering graduate-level course on Infrastructure Surety in the Civil Engineering Department at UNM. This groundbreaking class presented subject matter developed by experts from Sandia, and included additional information from guest lecturers from academia, government, and industry. Also included in this report are summaries of the term projects developed by the graduate students, an overview of the 1997 International Conference on Architectural Suretp: Assuring the Performance of Buildings and Injiastruchwes (co-sponsored by Sandia, the American Institute of Architects, and the American Society of Civil Engineers), and recommendations for further course work development. The U.S. Department of Energy provides support to this emerging field of architectural and infrastructure surety and recognizes its broad application to developing government, industry, and professional standards in the national interest.

  5. Whole Turf Algae to biofuels-final-sm

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Whole Turf Algae Polyculture Biofuels The production and conversion of whole turf algae polyculture maximizes fuels, chemicals and nutrients New Approach to Algal Biomass Production Sandia National Laboratories in partnership with the Smithsonian Institute and HydroMentia are pursuing the affordable, scalable and sustainable production of biofuels from benthic algal polyculture turf biomass. The highly productive, easily harvested and dewatered algae is a promising new alternative for achieving

  6. Whole Turf Algae to biofuels-final-sm

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Whole Turf Algae Polyculture Biofuels The production and conversion of whole turf algae ... and sustainable production of biofuels from benthic algal polyculture turf biomass. ...

  7. R{sup 2}-inflation with conformal SM Higgs field

    SciTech Connect (OSTI)

    Gorbunov, Dmitry; Tokareva, Anna E-mail: tokareva@ms2.inr.ac.ru

    2013-12-01

    We introduce conformal coupling of the Standard Model Higgs field to gravity and discuss the subsequent modification of R{sup 2}-inflation. The main observation is a lower temperature of reheating which happens mostly through scalaron decays into gluons due to the conformal (trace) anomaly. This modifies all predictions of the original R{sup 2}-inflation. To the next-to-leading order in slow roll parameters we calculate amplitudes and indices of scalar and tensor perturbations produced at inflation. The results are compared to the next-to-leading order predictions of R{sup 2}-inflation with minimally coupled Higgs field and of Higgs-inflation. We discuss additional features in gravity wave signal that may help to distinguish the proposed variant of R{sup 2}-inflation. Remarkably, the features are expected in the region available for study at future experiments like BBO and DECIGO. Finally, we check that (meta)stability of electroweak vacuum in the cosmological model is consistent with recent results of searches for the Higgs boson at LHC.

  8. Increasing Sugar Yields with IL-final-sm

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    a feedstock agnostic ionic liquid pretreatment process that: Agriculture Waste Woody Biomass Mixed Feedstocks Municipal Solid Waste (MSW) Biofuels Program Contact: Blake...

  9. Real Time Diagnostics for Algae-final-sm

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Real-time Monitoring And Diagnostics Detecting pathogens and predators to quickly recover ... Real-time Monitoring With Online Algal Reflectance Monitor System Researchers have ...

  10. The SM and NLO Multileg Working Group: Summary Report

    SciTech Connect (OSTI)

    Andersen, J.R.; Archibald, J.; Badger, S.; Ball, R.D.; Bevilacqua, G.; Bierenbaum, I.; Binoth, T.; Boudjema, F.; Boughezal, R.; Bredenstein, A.; Britto, R.; Campanelli, M.; Campbell, J.; Carminati, L.; Chachamis, G.; Ciulli, V.; Cullen, G.; Czakon, M.; Del Debbio, L.; Denner, A.; Dissertori, G.; /Edinburgh U. /Zurich, ETH /Michigan State U. /CAFPE, Granada /CERN /Durham U., IPPP /DESY, Zeuthen /Democritos Nucl. Res. Ctr. /Valencia U., IFIC /Annecy, LAPTH /Zurich U. /KEK, Tsukuba /Saclay, SPhT /University Coll. London /Fermilab /INFN, Milan /Milan U. /PSI, Villigen /Florence U. /INFN, Florence /RWTH Aachen U.

    2012-04-10

    After years of waiting, and after six Les Houches workshops, the era of LHC running is finally upon us, albeit at a lower initial center-of-mass energy than originally planned. Thus, there has been a great sense of anticipation from both the experimental and theoretical communities. The last two years, in particular, have seen great productivity in the area of multi-parton calculations at leading order (LO), next-to-leading order (NLO) and next-to-next-to-leading order (NNLO), and this productivity is reflected in the proceedings of the NLM group. Both religions, Feynmanians and Unitarians, as well as agnostic experimenters, were well-represented in both the discussions at Les Houches, and in the contributions to the write-up. Next-to-leading order (NLO) is the first order at which the normalization, and in some cases the shape, of perturbative cross sections can be considered reliable. This can be especially true when probing extreme kinematic regions, as for example with boosted Higgs searches considered in several of the contributions to this writeup. A full understanding for both standard model and beyond the standard model physics at the LHC requires the development of fast, reliable programs for the calculation of multi-parton final states at NLO. There have been many advances in the development of NLO techniques, standardization and automation for such processes and this is reflected in the contributions to the first section of this writeup. Many calculations have previously been performed with the aid of semi-numerical techniques. Such techniques, although retaining the desired accuracy, lead to codes which are slow to run. Advances in the calculation of compact analytic expressions for Higgs + 2 jets have resulted in the development of much faster codes, which extend the phenomenology that can be conducted, as well as making the code available to the public for the first time. A prioritized list of NLO cross sections was assembled at Les Houches in 2005 and added to in 2007. This list includes cross sections which are experimentally important, and which are theoretically feasible (if difficult) to calculate. Basically all 2-3 cross sections of interest have been calculated, with the frontier now extending to 2 {yields} 4 calculations. Often these calculations exist only as private codes. Since 2007, two additional calculations have been completed: t{bar t}b{bar b} and W+3 jets, reflecting the advance of the NLO technology to 2 {yields} 4 processes. In addition, the cross section for b{bar b}b{bar b} has been calculated for the q{bar q} initial state with the gg initial state calculation in progress. Final states of such complexity usually lead to multi-scale problems, and the correct choice of scales to use can be problematic not only at LO, but also at NLO. The size of the higher order corrections and of the residual scale dependence at NLOcan depend strongly on whether the considered cross section is inclusive, or whether a jet veto cut has been applied. Depending on the process, dramatically different behavior can be observed upon the application of a jet veto. There is a trade-off between suppressing the NLO cross section and increasing the perturbative uncertainty, with application of a jet veto sometimes destroying the cancellation between infra-red logs of real and virtual origin, and sometimes just suppressing large (and very scale-sensitive) tree-level contributions. So far, there is no general rule predicting the type of behavior to be expected, but this is an important matter for further investigation. From the experimental side, an addition to the above wish-list that will be crucial is the determination of the accuracy to which each of the calculations needs to be known. This is clearly related to the experimental accuracy at which the cross sections can be measured at the LHC, and can determine, for example, for what processes it may be necessary to calculate electo-weak corrections, in addition to the higher order QCD corrections. On the theoretical side, it would also be interesting to categorize the impact of a jet veto on the size and stability of each of the NLO cross sections. The technology does exist to carry out a calculation for W/Z production at NNLO (QCD) and at NLO (EW). This process was placed on the wish-list in 2007 and it is unfortunate that the combined calculation has not yet been carried out, as this precision benchmark will be very useful and important at the LHC.

  11. The QCD/SM working group: A Summary report

    SciTech Connect (OSTI)

    Alekhin, S.; Balazs, C.; Ball, R.; Binoth, T.; Boos, E.; Botje, M.; Cacciari, M.; Catani, S.; Del Duca, V.; Dobbs, M.; Ellis, S.D.; Field, R.; deFlorian, D.; Forte, S.; Gardi, E.; Gehrmann, T.; Gehrmann-De Riddler, A.; Giele, W.; Glover, E.W.N.; Grazzini, M.; Guillet, J.-Ph.; HeinRich, G.; Huston, J.; Hinchliffe, I.; Llyin, V.; Kanzaki, J.; Kato, K.; Kersevan, B.; Kidonakis, N.; Kulesza, A.; Kurihara, Y.; Laenen, E.; Lassila-Perini, K.; Lonnblad, L.; Magnea, L.; Mangano, M.; Mazumudar, K.; Moch, S.; Mrenna, S.; Nadolsky, P.; Nason, P.; Olness, F.; Paige, F.; Puljak, I.; Pumplin, J.; Richter-Was, E.; Salam, G.; Scalise, R.; Seymour, M.; Sjostrand, T.; Sterman, G.; Monnesmann, M.; Tournefier, E.; Vogelsang, W.; Vogt, A.; Vogt, R.; Webber, B.; Yuan, C.-P.; Zeppenfeld, D.

    2002-04-01

    This report documents the results obtained by the Working Group on Quantum Chromodynamics and the Standard Model for the Workshop ''Physics at TeV Colliders,'' Les Houches, France, 26 May - 6 June 2003. After a Monte Guide description, the first contributions report on progress in describing multiple interactions, important for the LHC, and underlying events. An announcement of a Monte Carlo database, under construction, is then followed by a number of contributions improving parton shower descriptions. Subsequently, a large number of contributions address resummations in various forms, after which follow studies of QCD effects in pion pair, top quark pair and photon pair plus jet production. After a study of electroweak corrections to hadronic precision observables, the report ends by presenting recent progress in methods to compute finite order corrections at one-loop with many legs, and at two-loop.

  12. Increasing Sugar Yields with IL-final-sm

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ionic Liquid Processing Increasing sugar yields from diverse biomass feedstock with ionic liquid processing and cultivation of renewable ionic liquids Liberating Sugars from Biomass Lignocellulose, one of the most abundant plants on Earth, has the potential to displace a substantial portion of the fossil fuels currently consumed within the transportation sector. Converting lignocellulose to biofuels requires the disruption of the lignin-carbohydrate complex within the plant and conversion into

  13. Real Time Diagnostics for Algae-final-sm

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Real-time Monitoring And Diagnostics Detecting pathogens and predators to quickly recover from pond crashes Algal Pond Crash Detection Sandia National Laboratories is developing a suite of complementary technologies to help the emerging algae industry detect and quickly recover from algal pond crashes, an obstacle to large-scale algae cultivation for biofuels. Because of the way algae is grown and produced in most algal ponds, they are prone to attack by fungi, rotifers, viruses or other

  14. The Fastmet[sup SM] direct reduction process

    SciTech Connect (OSTI)

    Lepinski, J.A.

    1993-01-01

    The Fastmet Process offers a simple and economical approach to producing direct reduced iron (DRI). It combines conventional equipment into a reliable ironmaking system. The process is ideally suited for processing U.S. iron oxide concentrates and coals. High iron yields are achievable due to the inherent ability to recycle in-plant fines and dust. Very low residence time of material in the rotary hearth furnace allows rapid adjustment of process parameters and minimal production loss from process upsets. Environmental impact is minimal. The paper gives a description of the process, then describes the economics, test facilities, test results, and scale-up.

  15. Synthesis, structure, and physical properties of [Sm(C{sub 6}NO{sub 2}H{sub 5}){sub 3}(H{sub 2}O){sub 2}]{sub 2n}.(H{sub 5}O{sub 2}){sub n}(ZnCl{sub 5}){sub n}(ZnCl{sub 4}){sub 2n}.(H{sub 2}O){sub 2n} with unprecedented ZnCl{sub 5}{sup 3-} species

    SciTech Connect (OSTI)

    Xie Yiming Chen Wentong; Wu Jihuai

    2008-08-15

    A novel bimetallic 4f-3d metal-isonicotinic acid inorganic-organic hybrid complex [Sm(C{sub 6}NO{sub 2}H{sub 5}){sub 3}(H{sub 2}O){sub 2}]{sub 2n}.(H{sub 5}O{sub 2}){sub n}(ZnCl{sub 5}){sub n}(ZnCl{sub 4}){sub 2n}.(H{sub 2}O){sub 2n} (1) has been synthesized via hydrothermal reaction and structurally characterized by single-crystal X-ray diffraction. Complex 1 is characteristic of a one-dimensional polycationic chain-like structure and unprecedented ZnCl{sub 5}{sup 3-} species. Photoluminescent investigation reveals that the title complex displays interesting emissions in a wide region. Optical absorption spectra of 1 reveal the presence of an optical gap of 3.59 eV. - Graphical abstract: A novel bimetallic 4f-3d metal-isonicotinic acid inorganic-organic hybrid complex was synthesized. It is characteristic of a one-dimensional polycationic chain-like structure. Photoluminescent investigation reveals that the title complex displays interesting emissions in a wide region. Optical absorption spectra of 1 reveal the presence of a wide optical bandgap.

  16. Electronic Spectra and Excited States of Neptunyl and Its [NpO...

    Office of Scientific and Technical Information (OSTI)

    obtain a copy of this journal article from the publisher. Find in Google Scholar Find in Google Scholar Search WorldCat Search WorldCat to find libraries that may hold this journal

  17. Impact of low-dose electron irradiation on $n^{+}p$ silicon strip sensors

    SciTech Connect (OSTI)

    Adam, W.

    2015-08-28

    The response of n+p silicon strip sensors to electrons from a 90Sr source was measured using a multi-channel read-out system with 25 ns sampling time. The measurements were performed over a period of several weeks, during which the operating conditions were varied. The sensors were fabricated by Hamamatsu Photonics on 200 μm thick float-zone and magnetic-Czochralski silicon. Their pitch was 80 μm, and both p-stop and p-spray isolation of the n+ strips were studied. The electrons from the 90Sr source were collimated to a spot with a full-width-at-half-maximum of 2 mm at the sensor surface, and the dose rate in the SiO2 at the maximum was about 50 Gy(SiO2)/d. After only a few hours of making measurements, significant changes in charge collection and charge sharing were observed. Annealing studies, with temperatures up to 80 °C and annealing times of 18 h showed that the changes can only be partially annealed. The observations can be qualitatively explained by the increase of the positive oxide-charge density due to the ionization of the SiO2 by the radiation from the β source. TCAD simulations of the electric field in the sensor for different oxide-charge densities and different boundary conditions at the sensor surface support this explanation. As a result, the relevance of the measurements for the design of n+p strip sensors is discussed.

  18. Microsoft Word - ZnSe_NP_AMI_R2-jh_jz[1].docx

    Office of Scientific and Technical Information (OSTI)

    ... DE-AC05-00OR22750 and DE-AC02-05CH11231, respectively. References 16 (1) Ithurria, S.; Tessier, M. D.; Mahler, B.; Lobo, R. P. S. M.; Dubertret, B.; Efros, A. L. Colloidal ...

  19. Measurements of plutonium, 237Np, and 137Cs in the BCR 482 lichen reference material

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Lavelle, Kevin B.; Miller, Jeffrey L.; Hanson, Susan K.; Connick, William B.; Spitz, Henry B.; Glover, Samuel E.; Oldham, Warren J.

    2015-10-01

    Select anthropogenic radionuclides were measured in lichen reference material, BCR 482. This material was originally collected in Axalp, Switzerland in 1991 and is composed of the epiphytic lichen Pseudevernia furfuracea. Samples from three separate bottles of BCR 482 were analyzed for uranium, neptunium, and plutonium isotopes by inductively coupled plasma mass spectrometry (ICP-MS) and analyzed for cesium-137 by gamma-ray spectrometry. The isotopic composition of the radionuclides measured in BCR 482 suggests contributions from both global fallout resulting from historical nuclear weapons testing and more volatile materials released following the Chernobyl accident.

  20. NP Early Career Opportunities Archives | U.S. DOE Office of Science...

    Office of Science (SC) Website

    ... the elastic scattering power of the QGP to test theoretical calculations based on QCD and ... Coordination of data analysis and simulations efforts as well as studies with test ...

  1. Materials Data on NpCo2 (SG:227) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2015-03-09

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  2. Materials Data on Np(SiNi)2 (SG:139) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2014-07-09

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  3. Materials Data on Np(CrSi)2 (SG:139) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  4. Materials Data on NpC (SG:225) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  5. Kootenai River Nutrient Dosing System and N-P Consumption: Year 2008.

    SciTech Connect (OSTI)

    Holderman, Charles

    2009-02-19

    In early 2006 we designed and built low energy consumption, pump-operated system, for dosing of the liquid nutrient in the summer 2006 season. This operated successfully, and the system was used again during the 2007 and 2008 seasons for dosing. During the early winter period, 2008, laboratory tests were made of the liquid nutrient pump system, and it was noted that small amounts of air were being entrained on the suction side of the pump, during conditions when the inlet pressure was low. It was believed that this was the cause of diurnal fluctuations in the flow supplied, characteristic of the 2007 year flow data. Replacement of '0' rings on the inlet side of the pumps was the solution to this problem, and when tested in the field during the summer season, the flow supplied was found to be stable. A decision was made by the IKERT committee at the meeting of 20th to 21st May 2008 (held in Coeur d'Alene, Idaho) to use an injection flow rate of liquid fertilizer (polyammonium phosphate 10-34-0) to achieve a target phosphorus concentration of 3.0 {micro}g/L, after complete mixing in the river. This target concentration was the same as that used in 2006 and 2007. The proposed starting date was as early as possible in June 2008. Plans were made to measure the dosing flow in three ways. Two of the three methods of flow measurement (1 and 2 below) are inter-dependent. These were: (1) Direct measurement of flow rate by diverting dosing flow into a 1000 mL volume standard flask. The flow rate was computed by dividing the flask volume by the time required to fill the flask. This was done a few times only during the summer period. (2) Adjusting the flow rate reading of the Gamma dosing pump using the 'calibration' function to achieve agreement with the flow rate computed by method 1 above. (3) Direct measurement by electrical signal from conductive fluid passing through a magnetic field (Seametrics meter, as used in previous years). Values were recorded every 4 minutes by a data-logger. This instrument has been shown to be reliable, and in agreement with method 1 to within the expected uncertainty (within 2%). Liquid nutrients were delivered to the site in late May, and system testing was done the same day. High concentrations of suspended sediment in the water column, as indicated by shallow Secchi depth readings, were present in the river in the last part of May, into June. A plan was made to delay the start up of nutrient addition to a date later than 1st June, because the aquatic productivity was almost certainly to be compromised by insufficient light availability. Daily monitoring of Secchi depths was done, showing declining turbidity in early June. A decision was made to start the system on 15th June, by which time conditions were good.

  6. Microsoft Word - 9-3-14 Vehicle Utilization At Rocky Mountain NP Final_edited.docx

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    MIS-14-32720 AVTA Federal Fleet PEV Readiness Data Logging and Characterization Study for the National Park Service: Rocky Mountain National Park Stephen Schey Jim Francfort Ian Nienhueser July 2014 DISCLAIMER This information was prepared as an account of work sponsored by an agency of the U.S. Government. Neither the U.S. Government nor any agency thereof, nor any of their employees, makes any warranty, expressed or implied, or assumes any legal liability or responsibility for the accuracy,

  7. Benefits of NP | U.S. DOE Office of Science (SC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Information Resources » Hydropower Basics » Benefits of Hydropower Benefits of Hydropower Benefits of Hydropower Water power offers a number of advantages to the communities that they serve. Below are just some of the benefits that hydropower has over other methods of providing energy. Advantages of Hydropower: Hydropower is fueled by water, so it's a clean fuel source, meaning it won't pollute the air like power plants that burn fossil fuels, such as coal or natural gas. Hydroelectric power

  8. Materials Data on NpCo2 (SG:227) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  9. Materials Data on NpOs2 (SG:227) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2015-02-09

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  10. Nepal-Program for Scaling Up Renewable Energy in Low Income Countries...

    Open Energy Info (EERE)

    number of low income countries for energy efficiency, renewable energy and access to modern sustainable energy. The SREP stimulates economic growth through the scaled-up...

  11. From Nepal to JLab â€" One Scientist's Journey (Daily Press) |

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Work | Department of Energy From Mind to Marketplace: SunShot Incubator's Latest Protégés Get to Work From Mind to Marketplace: SunShot Incubator's Latest Protégés Get to Work October 22, 2013 - 1:00pm Addthis Workers from Clean Power Research review a software platform that aims to lower the costs associated with connecting distributed solar electricity generation to the grid. The platform is one of several projects funded through the Energy Department’s SunShot Incubator Program,

  12. Assess institutional frameworks for LEDS for land-use sector...

    Open Energy Info (EERE)

    Energy in Low Income Countries (SREP) Nepal-Sectoral Climate Impacts Economic Assessment Nepal-UNEP Green Economy Advisory Services Nicaragua-Joint Programme on Resource...

  13. Preclosure seismic design methodology for a geologic repository at Yucca Mountain. Topical report YMP/TR-003-NP

    SciTech Connect (OSTI)

    1996-10-01

    This topical report describes the methodology and criteria that the U.S. Department of Energy (DOE) proposes to use for preclosure seismic design of structures, systems, and components (SSCs) of the proposed geologic repository operations area that are important to safety. Title 10 of the Code of Federal Regulations, Part 60 (10 CFR 60), Disposal of High-Level Radioactive Wastes in Geologic Repositories, states that for a license to be issued for operation of a high-level waste repository, the U.S. Nuclear Regulatory Commission (NRC) must find that the facility will not constitute an unreasonable risk to the health and safety of the public. Section 60.131 (b)(1) requires that SSCs important to safety be designed so that natural phenomena and environmental conditions anticipated at the geologic repository operations area will not interfere with necessary safety functions. Among the natural phenomena specifically identified in the regulation as requiring safety consideration are the hazards of ground shaking and fault displacement due to earthquakes.

  14. Microsoft PowerPoint - McDonald+Planas Highlight_LG_NP-1-1 [Read-Only]

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Achievement The mechanism of CO 2 adsorption in the amine-func onalized metal-organic framework mmen- Mg 2 (dobpdc) was characterized by quantum-chemical calculations. Significance and Impact The unusual 1:1 (amine:CO 2 ) stoichiometry was rationalized. Reactivity within the MOFs environment can be better understood. Research Details - Two fragment models were designed to account for the different interactions occurring in the periodic structure. - The reaction path was followed by

  15. S.M. Stoller Corporation and US Department of Energy PINELLAS...

    Office of Legacy Management (LM)

    Stoller Corporation and US Department of Energy PINELLAS ENVIRONMENTAL RESTORATION ... to a "stack effect" induced by building heating (electrical, gas furnace, or solar). ...

  16. Revised calibration of the Sm:SrB{sub 4}O{sub 7} pressure sensor...

    Office of Scientific and Technical Information (OSTI)

    Subject: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 71 CLASSICAL ... DEPENDENCE; PRESSURE RANGE GIGA PA; SAMARIUM COMPOUNDS; SENSORS; STRONTIUM COMPOUNDS; ...

  17. Materials Data on Sm2Hf2O7 (SG:227) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  18. Materials Data on Sm2CdS4 (SG:122) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  19. Materials Data on SmCd2 (SG:191) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  20. Materials Data on Sm2CdSe4 (SG:122) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  1. Materials Data on Ca(Sm2Se3)4 (SG:9) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2015-04-10

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  2. Microsoft PowerPoint - ARM07_3sm.ppt [Compatibility Mode

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    period. Once a model has been obtained, intrinsic measures of the surface albedo and reflectance b d d f ill i ti diti temporal, and angular scales. This project is using ARM...

  3. Materials Data on SmSF (SG:129) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  4. Materials Data on Sr(SmS2)2 (SG:122) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  5. Materials Data on Sr(SmSe2)2 (SG:122) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  6. Materials Data on LiSm2IrO6 (SG:14) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2015-02-09

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  7. 2014 VissionMissionGoals poster_SM Size.pdf

    Office of Environmental Management (EM)

    Human Reliability Program Workshop Agenda 2014 Human Reliability Program Workshop Agenda September 17-19, 2014 2014 DOE Human Reliability Program Workshop And Webinar Agenda DOE National Training Center Albuquerque, New Mexico 2014 DOE HRP Workshop Agenda (96.79 KB) More Documents & Publications Memorandum, Clarification of Requirements for Certification in Title 10 Code of Federal Regulations Part 712, Human Reliability Program INSPECTION REPORT: DOE/IG-0919 Response to several FOIA

  8. Materials Data on Sm3Rh2 (SG:148) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  9. Materials Data on SmNi5 (SG:191) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  10. Robust topological surface state in Kondo insulator SmB{sub 6...

    Office of Scientific and Technical Information (OSTI)

    X-ray diffraction, Raman spectroscopy, and transmission electron microscopy indicate films ... THIN FILMS; TRANSMISSION ELECTRON MICROSCOPY; X-RAY DIFFRACTION Word Cloud More Like ...

  11. Materials Data on Ca(SmS2)2 (SG:122) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  12. Materials Data on SmCo2 (SG:227) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2015-03-09

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  13. Materials Data on Ba2SmReO6 (SG:225) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2015-03-24

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  14. Materials Data on BaSm2FeS5 (SG:140) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2015-03-08

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  15. Materials Data on La5SmS8 (SG:82) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2015-04-10

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  16. Materials Data on Sm2Be2GeO7 (SG:113) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  17. Materials Data on SmBPd3 (SG:221) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2015-02-09

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  18. Materials Data on SmB2Ru3 (SG:191) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  19. Materials Data on SmPd (SG:63) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2015-02-09

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  20. Materials Data on Sm(GePd)2 (SG:139) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  1. Materials Data on Sm(GaPd)2 (SG:139) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  2. Materials Data on SmPd3 (SG:221) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  3. Present Limits on the Precision of SM Predictions for Jet Energies

    SciTech Connect (OSTI)

    Paramonov, A.A.; Canelli, F.; D'Onofrio, M.; Frisch, H.J.; Mrenna, S.; /Fermilab

    2010-08-01

    We investigate the impact of theoretical uncertainties on the accuracy of measurements involving hadronic jets. The analysis is performed using events with a Z boson and a single jet observed in p{bar p} collisions at {radical}s = 1.96 TeV in 4.6 fb{sup -1} of data from the Collider Detector at Fermilab (CDF). The transverse momenta (p{sub T}) of the jet and the boson should balance each other due to momentum conservation in the plane transverse to the direction of the p and {bar p} beams. We evaluate the dependence of the measured p{sub T}-balance on theoretical uncertainties associated with initial and final state radiation, choice of renormalization and factorization scales, parton distribution functions, jet-parton matching, calculations of matrix elements, and parton showering. We find that the uncertainty caused by parton showering at large angles is the largest amongst the listed uncertainties. The proposed method can be re-applied at the LHC experiments to investigate and evaluate the uncertainties on the predicted jet energies. The distributions produced at the CDF environment are intended for comparison to those from modern event generators and new tunes of parton showering.

  4. MERCURY REMOVAL FROM DOE SOLID MIXED WASTE USING THE GEMEP(sm) TECHNOLOGY

    SciTech Connect (OSTI)

    1999-03-01

    Under the sponsorship of the Federal Energy Technology Center (FETC), Metcalf and Eddy (M and E), in association with General Electric Corporate Research and Development Center (GE-CRD), Colorado Minerals Research Institute (CMRI), and Oak Ridge National Laboratory (ORNL), conducted laboratory-scale and bench-scale tests of the General Electric Mercury Extraction Process technology on two mercury-contaminated mixed solid wastes from U. S. Department of Energy sites: sediment from the East Fork of Poplar Creek, Oak Ridge (samples supplied by Oak Ridge National Laboratory), and drummed soils from Idaho National Environmental and Engineering Laboratory (INEEL). Fluorescent lamps provided by GE-CRD were also studied. The GEMEP technology, invented and patented by the General Electric Company, uses an extraction solution composed of aqueous potassium iodide plus iodine to remove mercury from soils and other wastes. The extraction solution is regenerated by chemical oxidation and reused, after the solubilized mercury is removed from solution by reducing it to the metallic state. The results of the laboratory- and bench-scale testing conducted for this project included: (1) GEMEP extraction tests to optimize extraction conditions and determine the extent of co-extraction of radionuclides; (2) pre-screening (pre-segregation) tests to determine if initial separation steps could be used effectively to reduce the volume of material needing GEMEP extraction; and (3) demonstration of the complete extraction, mercury recovery, and iodine recovery and regeneration process (known as locked-cycle testing).

  5. Materials Data on Sm4S3N2 (SG:12) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  6. Materials Data on Sm2S3 (SG:122) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  7. Microsoft Word - Sellers_1_5_7_07sm.doc

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    2007 United States Department of Energy Idaho Operations Office Idaho Falls, ID 83415 DOE Video DOE-Idaho Manager Beth Sellers Looks at Year of Accomplishment at INL May 7, 2007 The Idaho National Laboratory Site has gone through tremendous change over the past two years as we have refocused the missions and how they are to be accomplished. We welcomed the former Argonne Area Office staff and the Radiological Environmental Sciences Laboratory into the Idaho Operations Office family. We split one

  8. Materials Data on Sm2TeO2 (SG:139) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  9. Robust ferromagnetism in the compressed permanent magnet Sm2Co17...

    Office of Scientific and Technical Information (OSTI)

    Resource Type: Journal Article Resource Relation: Journal Name: Physical Review B, vol. 104408, no. 10, September 8, 2014, pp. 104408 Research Org: Lawrence Livermore...

  10. Environmental Cleanup of the East Tennessee Technology Park Year One - Execution with Certainty SM - 13120

    SciTech Connect (OSTI)

    Schubert, A.L.

    2013-07-01

    On August 1, 2011, URS - CH2M Oak Ridge LLC (UCOR) began its five-year, $1.4 billion cleanup of the East Tennessee Technology Park (ETTP), located on the U.S. Department of Energy's (DOE) Oak Ridge Reservation in Tennessee. UCOR will close out cleanup operations that began in 1998 under a previous contract. When the Contract Base scope of work [1] is completed in 2016, the K-25 gaseous diffusion building will have been demolished and all waste dispositioned, demolition will have started on the K-27 gaseous diffusion building, all contact-handled and remote-handled transuranic waste in inventory (approximately 500 cubic meters) will have been transferred to the Transuranic Waste Processing Center, previously designated 'No-Path-To-Disposition Waste' will have been dispositioned to the extent possible, and UCOR will have managed DOE Office of Environmental Management (EM)- owned facilities at ETTP, Oak Ridge National Laboratory (ORNL), and the Y-12 National Security Complex in a safe and cost-effective manner. Since assuming its responsibilities as the ETTP cleanup contractor, UCOR has completed its life-cycle Performance Measurement Baseline; received its Earned Value Management System (EVMS) certification; advanced the deactivation and demolition (D and D) of the K-25 gaseous diffusion building; recovered and completed the Tank W-1A and K-1070-B Burial Ground remediation projects; characterized, packaged, and shipped contact-handled transuranic waste to the Transuranic Waste Processing Center; disposed of more than 90,000 cubic yards of cleanup waste while managing the Environmental Management Waste Management Facility (EMWMF); and provided operations, surveillance, and maintenance activities at DOE EM facilities at ETTP, ORNL, and the Y-12 National Security Complex. Project performance as of December 31, 2012 has been excellent: - Cost Performance Index - 1.06; - Schedule Performance Index - 1.02. At the same time, since safety is the foundation of all cleanup work, UCOR's safety record goes hand in hand with its excellent project performance. Through calendar year 2012, UCOR's recordable injury rate was 0.33, and the company has worked close to 4 million hours without a lost work day injury. UCOR's safety record is one of the best in the DOE EM Complex. This performance was due, in large part, to the people and processes URS and CH2M HILL, the parent companies of UCOR, brought to the project. Key approaches included: - Selected and deployed experienced staff in key leadership positions throughout the organization; - Approached 'Transition' as the 'true' beginning of the cleanup project - kicking off a number of project initiatives such as Partnering, PMB development, D and D Plan execution, etc. - Established a project baseline for performance measurement and obtained EVMS certification in record time; - Determined material differences and changed conditions that warranted contract change - then quickly addressed these changes with the DOE client; - Aligned the project and the contract within one year - also done in record time; - Implemented Safety Trained Supervisor and Safety Conscious Work Environment Programs, and kicked off the pursuit of certification under DOE's Voluntary Protection Program. (authors)

  11. Materials Data on SmMg2Ag (SG:225) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2015-02-09

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  12. Materials Data on Sm5Sb3H (SG:193) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2015-04-29

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  13. Technical Basis Agreement Document for UGTA CAU 99 RM/SM

    National Nuclear Security Administration (NNSA)

    D.L. Finnegan, J.L. Thompson, C.M. Miller, P.L. Baca, L.F. Olivas, C.G. Geoffrion, D.K. Smith, W. Goishi, B.K. Esser, J.W. Meadows, N. Namboodiri, J.F. Wild. 2001. Nevada Test Site...

  14. Ternary rare earth-lanthanide sulfides. [Re = Eu, Sm or Yb

    DOE Patents [OSTI]

    Takeshita, Takuo; Gschneidner, K.A. Jr.; Beaudry, B.J.

    1986-03-06

    Disclosed is a new ternary rare earth sulfur compound having the formula La/sub 3-x/M/sub x/S/sub 4/, where M is europium, samarium, or ytterbium, with x = 0.15 to 0.8. The compound has good high-temperature thermoelectric properties and exhibits long-term structural stability up to 1000/sup 0/C.

  15. Materials Data on SmCo2 (SG:227) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  16. Kondo Breakdown and Quantum Oscillations in SmB 6 (Journal Article...

    Office of Scientific and Technical Information (OSTI)

    Journal Name: Physical Review Letters Additional Journal Information: Journal Volume: 116; ... Language: English Word Cloud More Like This Free Publicly Accessible Full Text This ...

  17. Materials Data on LiSm2OsO6 (SG:14) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  18. Materials Data on Sm2Te4O11 (SG:15) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  19. Materials Data on SmOF (SG:216) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  20. Materials Data on Sm2F (SG:8) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  1. Materials Data on Sm(SbTe2)2 (SG:122) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2015-04-10

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  2. Materials Data on Sm(BiTe2)2 (SG:122) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2015-04-15

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  3. Materials Data on SmTe (SG:225) by Materials Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  4. Concordant plutonium-241-americium-241 dating of environmental samples: results from forest fire ash

    SciTech Connect (OSTI)

    Goldstein, Steven J; Oldham, Warren J; Murrell, Michael T; Katzman, Danny

    2010-12-07

    We have measured the Pu, {sup 237}Np, {sup 241}Am, and {sup 151}Sm isotopic systematics for a set of forest fire ash samples from various locations in the western U.S. including Montana, Wyoming, Idaho, and New Mexico. The goal of this study is to develop a concordant {sup 241}Pu (t{sub 1/2} = 14.4 y)-{sup 241}Am dating method for environmental collections. Environmental samples often contain mixtures of components including global fallout. There are a number of approaches for subtracting the global fallout component for such samples. One approach is to use {sup 242}/{sup 239}Pu as a normalizing isotope ratio in a three-isotope plot, where this ratio for the nonglobal fallout component can be estimated or assumed to be small. This study investigates a new, complementary method of normalization using the long-lived fission product, {sup 151}Sm (t{sub 1/2} = 90 y). We find that forest fire ash concentrates actinides and fission products with {approx}1E10 atoms {sup 239}Pu/g and {approx}1E8 atoms {sup 151}Sm/g, allowing us to measure these nuclides by mass spectrometric (MIC-TIMS) and radiometric (liquid scintillation counting) methods. The forest fire ash samples are characterized by a western U.S. regional isotopic signature representing varying mixtures of global fallout with a local component from atmospheric testing of nuclear weapons at the Nevada Test Site (NTS). Our results also show that {sup 151}Sm is well correlated with the Pu nuclides in the forest fire ash, suggesting that these nuclides have similar geochemical behavior in the environment. Results of this correlation indicate that the {sup 151}Sm/{sup 239}Pu atom ratio for global fallout is {approx}0.164, in agreement with an independent estimate of 0.165 based on {sup 137}Cs fission yields for atmospheric weapons tests at the NTS. {sup 241}Pu-{sup 241}Am dating of the non-global fallout component in the forest fire ash samples yield ages in the late 1950's-early 1960's, consistent with a peak in NTS

  5. Asian Development Outlook 2010 | Open Energy Information

    Open Energy Info (EERE)

    Turkmenistan, Uzbekistan, China, South Korea, Mongolia, Afghanistan, Bangladesh, Bhutan, India, Maldives, Pakistan, Sri Lanka, Nepal, Cambodia, Indonesia, Malaysia, Laos, Vietnam,...

  6. Two-Dimensional Measurement of n+-p Asymmetrical Junctions in Multicrystalline Silicon Solar Cells using AFM-Based Electrical Techniques with Nanometer Resolution

    SciTech Connect (OSTI)

    Jiang, C. S.; Heath, J. T.; Moutinho, H. R.; Li, J. V.; Al-Jassim, M. M.

    2011-01-01

    Lateral inhomogeneities of modern solar cells demand direct electrical imaging with nanometer resolution. We show that atomic force microscopy (AFM)-based electrical techniques provide unique junction characterizations, giving a two-dimensional determination of junction locations. Two AFM-based techniques, scanning capacitance microscopy/spectroscopy (SCM/SCS) and scanning Kelvin probe force microscopy (SKPFM), were significantly improved and applied to the junction characterizations of multicrystalline silicon (mc-Si) cells. The SCS spectra were taken pixel by pixel by precisely controlling the tip positions in the junction area. The spectra reveal distinctive features that depend closely on the position relative to the electrical junction, which allows us to indentify the electrical junction location. In addition, SKPFM directly probes the built-in potential over the junction area modified by the surface band bending, which allows us to deduce the metallurgical junction location by identifying a peak of the electric field. Our results demonstrate resolutions of 10-40 nm, depending on the techniques (SCS or SKPFM). These direct electrical measurements with nanometer resolution and intrinsic two-dimensional capability are well suited for investigating the junction distribution of solar cells with lateral inhomogeneities.

  7. Two-Dimensional Measurement of n+-p Asymmetrical Junctions in Multicrystalline Silicon Solar Cells Using AFM-Based Electrical Techniques with Nanometer Resolution: Preprint

    SciTech Connect (OSTI)

    Jiang, C. S.; Moutinho, H. R.; Li, J. V.; Al-Jassim, M. M.; Heath, J. T.

    2011-07-01

    Lateral inhomogeneities of modern solar cells demand direct electrical imaging with nanometer resolution. We show that atomic force microscopy (AFM)-based electrical techniques provide unique junction characterizations, giving a two-dimensional determination of junction locations. Two AFM-based techniques, scanning capacitance microscopy/spectroscopy (SCM/SCS) and scanning Kelvin probe force microscopy (SKPFM), were significantly improved and applied to the junction characterizations of multicrystalline silicon (mc-Si) cells. The SCS spectra were taken pixel by pixel by precisely controlling the tip positions in the junction area. The spectra reveal distinctive features that depend closely on the position relative to the electrical junction, which allows us to indentify the electrical junction location. In addition, SKPFM directly probes the built-in potential over the junction area modified by the surface band bending, which allows us to deduce the metallurgical junction location by identifying a peak of the electric field. Our results demonstrate resolutions of 10-40 nm, depending on the techniques (SCS or SKPFM). These direct electrical measurements with nanometer resolution and intrinsic two-dimensional capability are well suited for investigating the junction distribution of solar cells with lateral inhomogeneities.

  8. Neutronics Simulations of 237Np Targets to Support Safety-Basis and 238Pu Production Assessment Efforts at the High Flux Isotope Reactor

    SciTech Connect (OSTI)

    Chandler, David; Ellis, Ronald James

    2015-01-01

    Fueled by two highly enriched uranium-bearing fuel elements surrounded by a large concentric ring of beryllium reflector, the High Flux Isotope Reactor (HFIR) provides one of the highest neutron fluxes in the world and is used to produce unique isotopes like plutonium-238. The National Aeronautics and Space Administration use radioisotope thermoelectric generators powered by 238Pu for deep-space missions. As part of the US Department of Energy s task to reestablish the domestic production of 238Pu, a technology demonstration sub-project has been initiated to establish a new 238Pu supply chain. HFIR safety-basis neutronics calculations are being performed to ensure the target irradiations have no adverse impacts on reactor performance and to calculate data required as input to follow-on thermal-structural, thermal-hydraulic and radionuclide/dose analyses. Plutonium-238 production assessments are being performed to estimate the amount of 238Pu that can be produced in HFIR s permanent beryllium reflector. It is estimated that a total of 0.96 1.12 kg 238Pu (~1.28 1.49 kg PuO2 at 85% 238Pu/Pu purity) could be produced per year in HFIR s permanent beryllium reflector irradiation facilities if they are all utilized.

  9. Measurements of plutonium, 237Np, and 137Cs in the BCR 482 lichen reference material

    SciTech Connect (OSTI)

    Lavelle, Kevin B.; Miller, Jeffrey L.; Hanson, Susan K.; Connick, William B.; Spitz, Henry B.; Glover, Samuel E.; Oldham, Warren J.

    2015-10-01

    Select anthropogenic radionuclides were measured in lichen reference material, BCR 482. This material was originally collected in Axalp, Switzerland in 1991 and is composed of the epiphytic lichen Pseudevernia furfuracea. Samples from three separate bottles of BCR 482 were analyzed for uranium, neptunium, and plutonium isotopes by inductively coupled plasma mass spectrometry (ICP-MS) and analyzed for cesium-137 by gamma-ray spectrometry. The isotopic composition of the radionuclides measured in BCR 482 suggests contributions from both global fallout resulting from historical nuclear weapons testing and more volatile materials released following the Chernobyl accident.

  10. Searches for new physics in the tt-bar events at CDF

    SciTech Connect (OSTI)

    Loginov, Andrey; /Yale U.

    2009-01-01

    The authors review the latest results on searches for physics beyond the Standard Model in the top quark sector at CDF Run II in a data sample with integrated luminosity up to 2.8 fb{sup -1}. Since its discovery, the top quark has appeared to be a very special object. It is distinguished by its large mass ({approx} 170 GeV) close to the scale of electroweak symmetry breaking (EWSB), and a Yukawa coupling surprisingly close to one (0.98). Is the top quark mass generated by the Higgs mechanism as the Standard Model (SM) predicts, or does it play a more fundamental role in the EWSB? How would physics beyond the standard model (SM) affect top quark properties? Searches for new physics (NP) should provide answers to the many open questions left by the SM. In these proceedings they present the latest CDF results on the searches for exotic decay modes of the top quark, as well as the production and decay of new particles into final states with a top quark pair. The analyses of the Run II data are performed with approximately 30 times the statistics of the Run I top quark discovery.

  11. Low dose rectal inoculation of rhesus macaques by SIV smE660 or SIVmac251 recapitulates

    SciTech Connect (OSTI)

    Hraber, Peter; Giorgi, Elena E; Keele, Brandon; Li, Hui; Learn, Gerald

    2008-01-01

    We recently developed a novel strategy to identify transmitted HIV-1 genomes in acutely infected humans using single-genome amplification and a model of random virus evolution. Here, we used this approach to determine the molecular features of simian immunodeficiency virus (SIV) transmission in 18 experimentally infected Indian rhesus macaques. Animals were inoculated intrarectally (i.r.) or intravenously (i.v.) with stocks of SIVmac251 or SIVsmE660 that exhibited sequence diversity typical of early-chronic HIV-1 infection. 987 full-length SIV env sequences (median of 48 per animal) were determined from plasma virion RNA 1--5 wk after infection. i.r. inoculation was followed by productive infection by one or a few viruses (median 1; range 1--5) that diversified randomly with near starlike phylogeny and a Poisson distribution of mutations. Consensus viral sequences from ramp-up and peak viremia were identical to viruses found in the inocula or differed from them by only one or a few nucleotides, providing direct evidence that early plasma viral sequences coalesce to transmitted/founder viruses. i.v. infection was >2,000-fold more efficient than i.r. infection, and viruses transmitted by either route represented the full genetic spectra of the inocula. These findings identify key similarities in mucosal transmission and early diversification between SIV and HIV-1, and thus validate the SIV-macaque mucosal infection model for HIV-1 vaccine and microbicide research.

  12. Effect of rare-earth doping in RCrSb3 (R = La, Pr, Sm, and Gd...

    Office of Scientific and Technical Information (OSTI)

    Alloying on the rare-earth site varies the de Gennes factor, DG (g-1)sup 2J(J+1), and dTsub C1d(DG) -2K, while dTsub C2d(DG) 5K. These ordering temperatures are found ...

  13. Materials Data on BaSm4Si3SeO12 (SG:173) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2014-11-02

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  14. Materials Data on Sr2SmCu3(PbO4)2 (SG:123) by Materials Project

    SciTech Connect (OSTI)

    Kristin Persson

    2015-02-19

    Computed materials data using density functional theory calculations. These calculations determine the electronic structure of bulk materials by solving approximations to the Schrodinger equation. For more information, see https://materialsproject.org/docs/calculations

  15. Extension of Studies with 3M Empore TM and Selentec MAG *SEP SM Technologies for Improved Radionuclide Field Sampling

    SciTech Connect (OSTI)

    Beals, D.M.; Bibler, J.P.; Brooks, D.A.

    1996-07-10

    The Savannah River Technology Center is evaluating new field sampling methodologies to more easily determine concentrations of radionuclides in aqueous systems. One methodology studied makes use of 3M EmporeTM disks. The disks are composed of selective resins embedded in a Teflon support. The disks remove the ion of interest from aqueous solutions when the solution is passed through the disk. The disk can then be counted directly to quantify the isotope of interest. Four types of disks were studied during this work: for the extraction of technetium (two types), cesium, plutonium, and strontium. A sampler has been developed for automated, unattended, in situ use of the EmporeTM disks.

  16. Final Technical Report for Collaborative Research: CRI-EaSM Multiscale Modeling Aerosol Indirect Effects on Decadal Timescales

    SciTech Connect (OSTI)

    Park, Sungsu

    2015-11-29

    Originally, the main role of the P.I. (Sungsu Park) in this project was to improve the treatment of cloud microphysics in the CAM5 shallow and deep convection scheme. During the progress of the project, however, the main research theme was changed to develop a new unified convection scheme (so called, UNICON) with the permission of the program manager.

  17. Leptonic B Decays at BaBar

    SciTech Connect (OSTI)

    Monorchio, Diego; /INFN, Naples /Naples U.

    2011-09-13

    The authors will present the most recent results on leptonic B decays B{sup {+-}(0)} {yields} K*{sup {+-}(0)} {nu}{bar {nu}} and B{sup {+-}} {yields} {mu}{sup {+-}}{nu}, based on the data collected by the BaBar detector at PEP-II, an asymmetric e{sup +}e{sup -} collider at the center of mass energy of the {Upsilon}(4S) resonance. Rare B decays have always been a standard probe for New Physics (NP) searches. The very low Standard Model (SM) rate of these decays often make them unaccessible with the present experimental datasets, unless NP effects enhance the rate up to the current experimental sensitivity. Moreover, as NP effects can modify the decay kinematic, particular attention must be payed in order to perform a model independent analysis. A B-Factory provides an unique environment where to investigate these processes. The high number of B{bar B} pairs produced by a B-Factory often allows to approach the needed experimental sensitivity. Moreover, the clean environment and the closed kinematic of the initial state enable to obtaining a very pure sample where to look for these decays.

  18. Leptonic B Decays at BaBar

    SciTech Connect (OSTI)

    Baracchini, Elisabetta; /Rome U. /INFN, Rome

    2011-11-10

    We will present the most recent results on leptonic B decays B{sup {+-}(0)} {yields} K*{sup {+-}(0)}{nu}{bar {nu}} and B{sup {+-}} {yields} {mu}{sup {+-}}{nu}, based on the data collected by the BaBar detector at PEP-II, an asymmetric e{sup +}e{sup -} collider at the center of mass energy of the {Upsilon}(4S) resonance. Rare B decays have always been a standard probe for New Physics (NP) searches. The very low Standard Model (SM) rate of these decays often make them unaccessible with the present experimental datasets, unless NP effects enhance the rate up to the current experimental sensitivity. Moreover, as NP effects can modify the decay kinematic, particular attention must be paid in order to perform a model independent analysis. A B-Factory provides an unique environment to investigate these processes. The high number of B{bar B} pairs produced by a B-Factory often allows to approach the needed experimental sensitivity. Moreover, the clean environment and the closed kinematic of the initial state enable to obtaining a very pure sample where to look for these decays.

  19. Nuclear Resonance Fluorescence at MIT | U.S. DOE Office of Science...

    Office of Science (SC) Website

    Resonance Fluorescence at MIT Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of Nuclear Science Applications of Nuclear Science ...

  20. Superconducting laser photocathode RF gun at BNL | U.S. DOE Office...

    Office of Science (SC) Website

    Superconducting laser photocathode RF gun at BNL Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of Nuclear Science ...

  1. Biomedical Instrumentation and Imaging at TJNAF | U.S. DOE Office...

    Office of Science (SC) Website

    Biomedical Instrumentation and Imaging at TJNAF Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of Nuclear Science ...

  2. Neutron Detectors for Detection of Nuclear Materials at LANL...

    Office of Science (SC) Website

    Neutron Detectors for Detection of Nuclear Materials at LANL Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of Nuclear ...

  3. Diamond Amplified Photocathode at BNL | U.S. DOE Office of Science...

    Office of Science (SC) Website

    Diamond Amplified Photocathode at BNL Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of Nuclear Science Applications of ...

  4. High Power Superconducting Continuous Wave Linacs for Protons...

    Office of Science (SC) Website

    Power Superconducting Continuous Wave Linacs for Protons and Heavy-Ions Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of ...

  5. Documentation - Laboratory for Laser Energetics

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Replace PLC Backup Batteries (S-SM-P-225) Reprogram Neuron Module (S-SM-P-226) Check and Balance Video Inputs (S-SM-P-227) Laser Bay Structure Grounding (S-SM-P-228) Laser Bay ...

  6. Documentation - Laboratory for Laser Energetics

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Clean Non-Cleanroom Floors (S-SM-P-346) Tacky Mats (S-SM-P-348) Clean Overhead Crane (S-SM-P-355) Clean Target Bay Elevator (S-SM-P-356) Clean Target Bay Stairwell ...

  7. 2.3.1.11: Low-Energy Magnetic-Field Separation using Magnetic...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    (Brotzman) 23 May 2013 Abbreviations HC: hydrocarbon SN: superparamagnetic nanoparticles NP: nanoparticle NA: nanostructured adsorbent D: diameter (NP) ALD: ...

  8. Radionuclide-Chelating Agent Complexes in Low-Level Radioactive Decontamination Waste; Stability, Adsorption and Transport Potential

    SciTech Connect (OSTI)

    Serne, R. Jeffrey; Cantrell, Cantrell J.; Lindenmeier, Clark W.; Owen, Antionette T.; Kutnyakov, Igor V.; Orr, Robert D.; Felmy, Andrew R.

    2002-02-01

    Speciation calculations were done to determine whether organic complexants facilitate transport of radionuclides leached from waste buried in soils. EDTA readily mobilizes divalent transition metals and moderately impacts trivalent actinides. Picolinate readily mobilizes only Ni2+ and Co2+. These speciation predictions ignore the influence of soil adsorption and biodegradation that break apart the complexes. In adsorption studies, picolinate concentrations have to be >10-4 M to lower the adsorption of Ni and Co. For Sm(III), Th(IV), Np(V), U(VI), and Pu, the picolinate concentration must be >10-3 M before adsorption decreases. EDTA forms strong complexes with divalent transition metals and can stop adsorption of Ni and Co when EDTA solution concentrations are 10-5 M. EDTA complexes with Np(V), U(VI), and Pu are much weaker; EDTA concentrations would have to be >10-3 M to adversely effects non-transition metal/radionuclide adsorption. Most picolinate and ETDA-metal complexes appear to readily dissociate during interactions with soils. The enhanced migration of radionuclide-organic complexes may be limited to a few unique conditions. We recommend that mixtures of metal/radionuclides and EDTA should not be solidified or co-disposed with high pH materials such as cement. For weaker binding organic complexants, such as picolinate, citrate and oxalate, co-disposal of decontamination wastes and concrete should be acceptable.

  9. Forest Carbon Partnership Facility | Open Energy Information

    Open Energy Info (EERE)

    Madagascar, Mexico, Moldova, Mozambique, Nepal, Nicaragua, Panama, Papua New Guinea, Paraguay, Peru, Republic of the Congo, Suriname, Tanzania, Thailand, Uganda, Vanuatu, Vietnam...

  10. WWS_LorrieC157L_0915

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ireland Italy Japan Kenya Latvia Lesotho Libya Lithuania Madagascar Malawi Malaysia Mauritius Mexico Mozambique Nepal The Netherlands New Zealand Nicaragua Nigeria Norway ...

  11. WorldWide Science.org

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Libya Lithuania Madagascar Malawi Malaysia Mauritius Mexico Mozambique Nepal The Netherlands New Zealand Nicaragua Nigeria Norway Philippines Poland Portugal Russia Rwanda Saudi ...

  12. Annual Energy Outlook 2015 - Appendix A

    Gasoline and Diesel Fuel Update (EIA)

    ... Myanmar (Burma), Nauru, Nepal, New Caledonia, Niue, North Korea, Pakistan, Papua New Guinea, Philippines, Samoa, Singapore, Solomon Islands, Sri Lanka, Taiwan, Thailand, ...

  13. Lotus Energy Pvt Ltd | Open Energy Information

    Open Energy Info (EERE)

    to: navigation, search Name: Lotus Energy Pvt. Ltd. Place: Kathmandu, Nepal Sector: Solar Product: Complete turnkey projects from assessment and design to manufacture, installation...

  14. Climate and Development Knowledge Network (CDKN) | Open Energy...

    Open Energy Info (EERE)

    Mozambique-Accrediation of NIE Nepal-Sectoral Climate Impacts Economic Assessment Pakistan-Technical Assistance to PDMA Punjab in Incorporating Climate Compatibility...

  15. File:Nepalmetst 223.pdf | Open Energy Information

    Open Energy Info (EERE)

    usage Meteorology: map of Nepal selected meteorological stations and elevation from NREL Size of this preview: 776 600 pixels. Full resolution (1,650 1,275 pixels,...

  16. File:NREL-asia-tilt.pdf | Open Energy Information

    Open Energy Info (EERE)

    Countries Bhutan, China, Nepal, Mongolia, India, North Korea, South Korea, Vietnam, Laos, Thailand, Cambodia, Philippines, Bangladesh UN Region Southern Asia, Eastern Asia,...

  17. File:NREL-asia-dir.pdf | Open Energy Information

    Open Energy Info (EERE)

    Countries Bhutan, China, Nepal, Mongolia, India, North Korea, South Korea, Vietnam, Laos, Thailand, Cambodia, Philippines, Bangladesh UN Region Southern Asia, Eastern Asia,...

  18. File:NREL-asia-glo.pdf | Open Energy Information

    Open Energy Info (EERE)

    Countries Bhutan, China, Nepal, Mongolia, India, North Korea, South Korea, Vietnam, Laos, Thailand, Cambodia, Philippines, Bangladesh UN Region Southern Asia, Eastern Asia,...

  19. LEDSGP/events/2013workshop/participants | Open Energy Information

    Open Energy Info (EERE)

    and Planning ) Awafo, Edward (Ghana Energy Center of the Kwame Nkrumah University of Science and Technology) Bahadur KC, Lava (Nepal Ministry of Science, Technology and...

  20. 2011 - 12 | Jefferson Lab

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    - 12 Dec 2011 Sun, 2011-12-04 00:00 From Nepal to JLab â€" One Scientist's Journey

  1. File:SWERA-252.pdf | Open Energy Information

    Open Energy Info (EERE)

    1,275 pixels, file size: 243 KB, MIME type: applicationpdf) Title Monthly Average Solar Resource for 2-axis tracking concentrating collectors for Nepal. Description Solar:...

  2. Geospatial Toolkit | Open Energy Information

    Open Energy Info (EERE)

    Ghana, Guatemala, Honduras, India, Nepal, Nicaragua, Oaxaca, Pakistan, Sri Lanka, Turkey Cost: Free Southern Asia, Southern Asia, Southern Asia, South America, Eastern Asia,...

  3. Technique development for uiper critical field studies of SmFeAs(O,F) in the 300T single turn system

    SciTech Connect (OSTI)

    Mcdonald, Ross D [Los Alamos National Laboratory; Balakirev, F. F. [Los Alamos National Laboratory; Altarawneh, M. M. [Los Alamos National Laboratory; Betts, J [Los Alamos National Laboratory; Mielke, C. H. [Los Alamos National Laboratory; Moll, Philip Jw [ETH ZURICH; Zhigadlo, N D [ETH ZURICH; Karpinski, J [ETH ZURICH; Batlogg, B. [ETH ZURICH

    2011-01-14

    In high temperature superconductors, such as the most recent class of iron pnictides, extremely high upper critical fields H{sub c2} are common. The determination of H{sub c2}(T) is crucial to understand the detailed nature of the superconductor, in particular H{sub c2}(T = 0K) is of great interest. It is not only related to fundamental properties of the system, it is furthermore of great importance for materials science, as it is the ultimate limit of applicability of this superconductor in high field applications. However, this important quantity can only be estimated by extrapolation, as H{sub c2}(T = 0K) well exceeds hundreds of Tesla in optimally doped SillFeAs(O,F). We are developing methods to measure Ha(T) in direct transport in the extreme magnetic fields generated by the LANL single turn magnet.

  4. ARPES study of the evolution of band structure and charge density wave properties in RTe3 ( R=Y , La, Ce, Sm, Gd, Tb, and Dy)

    SciTech Connect (OSTI)

    Hussain, Zahid; Brouet, Veronique; Yang, Wanli; Zhou, Xingjiang; Hussain, Zahid; Moore, R.G.; He, R.; Lu, D. H.; Shen, Z.X.; Laverock, J.; Dugdale, S.B.; Ru, N.; Fisher, R.

    2008-01-16

    We present a detailed angle-resolved photoemission spectroscopy (ARPES) investigation of the RTe3 family, which sets this system as an ideal"textbook" example for the formation of a nesting driven charge density wave (CDW). This family indeed exhibits the full range of phenomena that can be associated to CDWinstabilities, from the opening of large gaps on the best nested parts of Fermi surface (up to 0.4 eV), to the existence of residual metallic pockets. ARPES is the best suited technique to characterize these features, thanks to its unique ability to resolve the electronic structure in k space. An additional advantage of RTe3 is that theband structure can be very accurately described by a simple two dimensional tight-binding (TB) model, which allows one to understand and easily reproduce many characteristics of the CDW. In this paper, we first establish the main features of the electronic structure by comparing our ARPES measurements with the linear muffin-tinorbital band calculations. We use this to define the validity and limits of the TB model. We then present a complete description of the CDW properties and of their strong evolution as a function of R. Using simple models, we are able to reproduce perfectly the evolution of gaps in k space, the evolution of the CDW wave vector with R, and the shape of the residual metallic pockets. Finally, we give an estimation of the CDWinteraction parameters and find that the change in the electronic density of states n (EF), due to lattice expansion when different R ions are inserted, has the correct order of magnitude to explain the evolution of the CDW properties.

  5. Evaluation Data of a High Temperature COTS Flash Memory Module (TI SM28VLT32) for Use in Geothermal Electronics Packages

    SciTech Connect (OSTI)

    Cashion, Avery

    2014-08-29

    The accompanying raw data is composslection. Each file is 3 columns and tab-delimited with the first column being the data address, the second column being the first byte of the data, and the third column being the second byte of the data.

  6. Documentation - Laboratory for Laser Energetics

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Laser Bay Optics Inspect and Document Laser Rod Condition (S-SM-P-198) Inspect and Clean Beam Splitter Optics (S-SM-P-199) Inspect and Clean Spatial Filter Optics (S-SM-P-200) ...

  7. Documentation - Laboratory for Laser Energetics

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ... Crane Procedures Inspect and Grease Gantry Crane (S-SM-P-101) Gantry Crane Contract Service (S-SM-P-102) Inspect and Grease Hydraulic Floor Crane (S-SM-P-103) Inspect and Grease ...

  8. Documentation - Laboratory for Laser Energetics

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Module Windows (S-SM-P-180) SSA Laser Disk Inspection (S-SM-P-181) Inspect Structure & CraneWinch Assemblies (S-SM-P-182) Cooling System Procedures Cooling Subsystem Vendor ...

  9. Libopensmskummeeplug

    Energy Science and Technology Software Center (OSTI)

    2007-08-30

    A library plugin which utilizes the OpenSM evernt plugin interface to capture data from the OpenSM and passes it to the Skummee monitoring system.

  10. Energy Department Awards Small Business Contract for Legacy Management...

    Office of Environmental Management (EM)

    Small Business Contract for Legacy Management Work to S.M. Stoller Corporation Energy Department Awards Small Business Contract for Legacy Management Work to S.M. Stoller ...

  11. JOURNAL OF L A T E X CLASS FILES, VOL.

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Current Contribution of a Single Phase DQ-Controlled Inverter Javier Alvidrez, Member, IEEE, Satish Ranade, SM, IEEE, Stephen Bukowski, Member, IEEE, Sukumar Brahma, SM, IEEE,...

  12. Nuclear Wallet Cards at BNL | U.S. DOE Office of Science (SC...

    Office of Science (SC) Website

    Data Center, BNL Developed in: 2000-current Result of NP research: DOE-NP nuclear data program Application currently being supported by: DOE-NP Impactbenefit to spin-off ...

  13. Global Nuclear Energy Initiative at LBNL | U.S. DOE Office of...

    Office of Science (SC) Website

    Global Nuclear Energy Initiative at LBNL Nuclear Physics (NP) NP Home About Research ... Contact Information Nuclear Physics U.S. Department of Energy SC-26Germantown Building ...

  14. High Current Energy Recovery Linac at BNL | U.S. DOE Office of...

    Office of Science (SC) Website

    Current Energy Recovery Linac at BNL Nuclear Physics (NP) NP Home About Research ... Contact Information Nuclear Physics U.S. Department of Energy SC-26Germantown Building ...

  15. SOLID-STATE LIGHTING BUILDING TECHNOLOGIES OFFICE Solid-State...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    ... Dow Corning * Four patent applications filed Eastman Kodak * Device Containing Non-Blinking Quantum Dots NP, PCT * Doped Nanoparticle-Based Semiconductor Junction NP, PCT * Ex-Situ ...

  16. 9.5.1.9: Hydrocyclone Separation of Targeted Biochemical Intermediates...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    ... May 2013 1.2 Adsorbent Separation Approach Unique synthesis process: magnetic nanoparticles (NP) X Colloidal method - Solid-state reaction Assembly of magnetic NP - ...

  17. NSAC Long Range Plan 2007 Subcommittee White Papers | U.S. DOE...

    Office of Science (SC) Website

    Science Advisory Committee (NSAC) NSAC Home Meetings Members ChargesReports Charter .pdf file (78KB) NP Committees of Visitors Federal Advisory Committees NP Home Charges...

  18. File:SWERA-253.pdf | Open Energy Information

    Open Energy Info (EERE)

    File File history File usage Solar: monthly and annual average global horizontal (GHI) GIS data at 40km resolution for Nepal from NREL Size of this preview: 776 600 pixels....

  19. File:SWERA-254.pdf | Open Energy Information

    Open Energy Info (EERE)

    to: navigation, search File File history File usage Solar: monthly and annual latitude tilt horizontal GIS data at 40km resolution for Nepal from NREL Size of this preview: 776 ...

  20. RusSUNHydro | Open Energy Information

    Open Energy Info (EERE)

    JSC RusHydro (RTS: HYDR) and India's investment firm Sun Group have set up the joint venture RusSUNHydro to work on hydroelectric projects across India, Nepal and...

  1. Closed Lab Announcements | U.S. DOE Office of Science (SC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Lab Announcements Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Closed Funding Opportunity Announcements (FOAs) Closed Lab Announcements Award Search / Public Abstracts Additional Requirements and Guidance for Digital Data Management Reviews NP Early Career Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000

  2. Synthesis and characterization of compounds Sr{sub 2}{ital RM}Cu{sub 2}O{sub 8{minus}{delta}} ({ital R}=Pr, Nd, Sm, Eu, Gd; {ital M}=Nb, Ta)

    SciTech Connect (OSTI)

    Vybornov, M.; Perthold, W.; Michor, H.; Holubar, T.; Hilscher, G.; Rogl, P.; Fischer, P.; Divis, M.

    1995-07-01

    Although traces of superconductivity ({lt}0.2%) have been detected in Ba{sub 2}La{ital M}{sub 1{minus}{ital x}}W{sub {ital x}}Cu{sub 2}O{sub 8{minus}{delta}} ({ital x}{similar_to}0.3,{ital M}=Nb,Ta) below 30 K, the superconducting impurity phase could not be resolved. The antiferromagnetic (AF) order of the rare-earth sublattice in this {ital R}-2112 system (e.g., {ital T}{sub {ital N}}{sup Gd}=2.18 K) appears to be similar to that of the {ital R}Ba{sub 2}Cu{sub 3}O{sub 7{minus}{delta}} series (e.g., {ital T}{sub {ital N}}{sup Gd}=2.29 K); however, the exceptional high AF order of Pr in Pr-123 (with 17 K) is reduced to below 2.3 K for Sr{sub 2}Pr{ital M} Cu{sub 2}O{sub 8{minus}{delta}}. The temperature and field dependence of the specific heat and the susceptibility is discussed in terms of crystal field splitting derived from the {ital R}Ba{sub 2}Cu{sub 3}O{sub 7{minus}{delta}} compounds. Overall crystal field splitting in the title compounds is comparable with that of the {ital R}-123 compounds.

  3. Local Map | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

    About » Directions » Local Map Nuclear Physics (NP) NP Home About Organization Chart .pdf file (89KB) Staff NP Budget NP Committees of Visitors Directions Local Map Jobs Labs & Universities Nuclear Physics Related Brochures Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC

  4. About | U.S. DOE Office of Science (SC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    About Nuclear Physics (NP) NP Home About Organization Chart .pdf file (90KB) Staff NP Budget NP Committees of Visitors Directions Jobs Labs & Universities Nuclear Physics Related Brochures Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301)

  5. Jobs | U.S. DOE Office of Science (SC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Jobs Nuclear Physics (NP) NP Home About Organization Chart .pdf file (90KB) Staff NP Budget NP Committees of Visitors Directions Jobs Labs & Universities Nuclear Physics Related Brochures Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301)

  6. Staff | U.S. DOE Office of Science (SC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    About » Staff Nuclear Physics (NP) NP Home About Organization Chart .pdf file (90KB) Staff NP Budget NP Committees of Visitors Directions Jobs Labs & Universities Nuclear Physics Related Brochures Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F:

  7. Sulfur mustard primes human neutrophils for increased degranulation and stimulates cytokine release via TRPM2/p38 MAPK signaling

    SciTech Connect (OSTI)

    Ham, Hwa-Yong; Hong, Chang-Won; Lee, Si-Nae; Kwon, Min-Soo; Kim, Yeon-Ja; Song, Dong-Keun

    2012-01-01

    Sulfur mustard (2,2′-bis-chloroethyl-sulfide; SM) has been a military threat since the World War I. The emerging threat of bioterrorism makes SM a major threat not only to military but also to civilian world. SM injury elicits an inflammatory response characterized by infiltration of neutrophils. Although SM was reported to prime neutrophils, the mechanism has not been identified yet. In the present study, we investigated the mechanism of SM-induced priming in human neutrophils. SM increased [Ca{sup 2+}]{sub i} in human neutrophils in a concentration-dependent fashion. Transient receptor potential melastatin (TRPM) 2 inhibitors (clotrimazole, econazole and flufenamic acid) and silencing of TRPM2 by shRNA attenuated SM-induced [Ca{sup 2+}]{sub i} increase. SM primed degranulation of azurophil and specific granules in response to activation by fMLP as previously reported. SB203580, an inhibitor of p38 MAPK, inhibited SM-induced priming. Neither PD98057, an ERK inhibitor, nor SP600215, a JNK inhibitor, inhibited SM-induced priming. In addition, SM enhanced phosphorylation of NF-kB p65 and release of TNF-α, interleukin (IL)-6 and IL-8. SB203580 inhibited SM-induced NF-kB phosphorylation and cytokine release. These results suggest the involvement of TRPM2/p38 MAPK pathway in SM-induced priming and cytokines release in neutrophils. -- Highlights: ► SM increased [Ca{sup 2+}]{sub i} in human neutrophils through TPRM2-mediated calcium influx. ► SM primed degranulation of azurophil and specific granules. ► SM enhanced p38 MAPK and NF-κB p65 phosphorylation in human neutrophils. ► SM enhanced release of TNF-α, interleukin (IL)-6 and IL-8 from human neutrophils. ► SB203580 inhibited SM-induced priming, NF-κB p65 phosphorylation and cytokine release.

  8. Documentation - Laboratory for Laser Energetics

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    2 - Laser Amplifiers Volume X Subsystem and Component Maintenance Index and Cycle Schedule (S-AB-P-017) Rod Amplifier Procedures Rod Inspection (S-SM-P-162) Camshaft Assembly (S-SM-P-164) Rod Module (S-SM-P-166) Rod Module O-Rings (S-SM-P-167) Rod Jacket (S-SM-P-168) Pump Module (S-SM-P-169) Inspect and Clean Rod Face (S-AB-P-234) Remove and Replace Rod Amplifier Tube Extender (S-AB-P-238) Remove and Replace Rod Pump Module (S-AB-P-235) 4w Probe Amplifier Mechanical Inspection (S-AB-P-549)

  9. An intrinsically disordered peptide from Ebola virus VP35 controls viral RNA synthesis by modulating nucleoprotein-RNA interactions

    SciTech Connect (OSTI)

    Leung, Daisy  W.; Borek, Dominika; Luthra, Priya; Binning, Jennifer  M.; Anantpadma, Manu; Liu, Gai; Harvey, Ian B.; Su, Zhaoming; Endlich-Frazier, Ariel; Pan, Juanli; Shabman, Reed  S.; Chiu, Wah; Davey, Robert  A.; Otwinowski, Zbyszek; Basler, Christopher  F.; Amarasinghe, Gaya  K.

    2015-04-01

    During viral RNA synthesis, Ebola virus (EBOV) nucleoprotein (NP) alternates between an RNA-template-bound form and a template-free form to provide the viral polymerase access to the RNA template. In addition, newly synthesized NP must be prevented from indiscriminately binding to noncognate RNAs. Here, we investigate the molecular bases for these critical processes. We identify an intrinsically disordered peptide derived from EBOV VP35 (NPBP, residues 20–48) that binds NP with high affinity and specificity, inhibits NP oligomerization, and releases RNA from NP-RNA complexes in vitro. The structure of the NPBP/ΔNPNTD complex, solved to 3.7 Å resolution, reveals how NPBP peptide occludes a large surface area that is important for NP-NP and NP-RNA interactions and for viral RNA synthesis. Together, our results identify a highly conserved viral interface that is important for EBOV replication and can be targeted for therapeutic development.

  10. ELIFE07322 1..3

    Office of Scientific and Technical Information (OSTI)

    ... 2 of 3 LI FE Insight Metagenomics | Social behavior and the microbiome LaxS, Smith DP, Hampton-Marcell J, Owens SM, Handley KM, Scott NM, Gibbons SM, Larsen P, Shogan BD, ...

  11. Interaction Driven Subgap Spin Exciton in the Kondo Insulator...

    Office of Scientific and Technical Information (OSTI)

    Interaction Driven Subgap Spin Exciton in the Kondo Insulator SmB 6 Title: Interaction Driven Subgap Spin Exciton in the Kondo Insulator SmB 6 Authors: Fuhrman, W. T. ; Leiner, J. ...

  12. ARM - Datastreams - amc

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    interval V battvoltmin ( time ) Average bulk soil electrical conductivity sensor 1 dSm ec1 ( time ) Average bulk soil electrical conductivity sensor 1 dSm ec1avg ( ...

  13. Microsoft Word - S05767_PostClosureInspRpt.doc

    Office of Legacy Management (LM)

    U.S. Department of Energy Post-Closure Inspection & Monitoring Report for CAU 417 October 2009 Doc. No. S05767 Page B-1 Table 1. UC-1 Monument Elevations and Subsidence Elevation at Top of Monument a,b Subsidence (m) Date SM-1 N 6,430,874.2869 E 539,588.2339 SM-2 N 6,430,863.3239 E 539,644.8195 SM-3 N 6,430,855.2553 E 539,684.3327 SM-4 N 6,430,849.7763 E 539,715.7991 SM-5 N 6,430,852.0243 E 539,585.4651 SM-6 N 6,430,841.7590 E 539,641.4674 SM-7 N 6,430,834.5289 E 539,680.5243 SM-8 N

  14. Chemical Quantification of Atomic-Scale EDS Maps under Thin Specimen...

    Office of Scientific and Technical Information (OSTI)

    Furthermore, the method developed by this work is applied to study a Sm-doped STO thin film and antiphase boundaries present within the STO film. We find that Sm atoms...

  15. In-gap collective mode spectrum of the topological Kondo insulator...

    Office of Scientific and Technical Information (OSTI)

    In-gap collective mode spectrum of the topological Kondo insulator SmB 6 Title: In-gap collective mode spectrum of the topological Kondo insulator SmB 6 Authors: Fuhrman, W. T. ; ...

  16. Documentation - Laboratory for Laser Energetics

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ... Output Quality Procedures Output ShearCollimation Check (at A-Splitter) (S-SM-P-045) Fiducial Procedures UV Fiducial Fiber Output Energy Measurement (S-SM-P-051) Weekly UV ...

  17. Widget:AnchorIcon | Open Energy Information

    Open Energy Info (EERE)

    iconv4 help-1 iconv4 image-1 iconv4 map-1 iconv4 presentation-1 iconv4 tool-1 iconv4 video-1 iconv4 website-1 iconv4 article-1-sm iconv4 dataset-1-sm iconv4 definition-1-sm...

  18. Ion Sources for High Energy Ion Implantation at BNL | U.S. DOE...

    Office of Science (SC) Website

    Ion Sources for High Energy Ion Implantation at BNL Nuclear Physics (NP) NP Home About ... Contact Information Nuclear Physics U.S. Department of Energy SC-26Germantown Building ...

  19. Sleuthing the Fate of Water in Ancient Aquifers and Ice Cores...

    Office of Science (SC) Website

    Sleuthing the Fate of Water in Ancient Aquifers and Ice Cores Nuclear Physics (NP) NP Home ... Sleuthing the Fate of Water in Ancient Aquifers and Ice Cores Precision analytical ...

  20. Streamlined Approach for Environmental Restoration Plan for Corrective Action Unit 107: Low Impact Soil Sites, Nevada Test Site, Nevada

    SciTech Connect (OSTI)

    NSTec Environmental Restoration

    2009-03-31

    This Streamlined Approach for Environmental Restoration Plan covers activities associated with Corrective Action Unit (CAU) 107 of the Federal Facility Agreement and Consent Order (1996 [as amended February 2008]). CAU 107 consists of the following Corrective Action Sites (CASs) located in Areas 1, 2, 3, 4, 5, 9, 10, and 18 of the Nevada Test Site. {sm_bullet} CAS 01-23-02, Atmospheric Test Site - High Alt{sm_bullet} CAS 02-23-02, Contaminated Areas (2){sm_bullet} CAS 02-23-03, Contaminated Berm{sm_bullet} CAS 02-23-10, Gourd-Amber Contamination Area{sm_bullet} CAS 02-23-11, Sappho Contamination Area{sm_bullet} CAS 02-23-12, Scuttle Contamination Area{sm_bullet} CAS 03-23-24, Seaweed B Contamination Area{sm_bullet} CAS 03-23-27, Adze Contamination Area{sm_bullet} CAS 03-23-28, Manzanas Contamination Area{sm_bullet} CAS 03-23-29, Truchas-Chamisal Contamination Area{sm_bullet} CAS 04-23-02, Atmospheric Test Site T4-a{sm_bullet} CAS 05-23-06, Atmospheric Test Site{sm_bullet} CAS 09-23-06, Mound of Contaminated Soil{sm_bullet} CAS 10-23-04, Atmospheric Test Site M-10{sm_bullet} CAS 18-23-02, U-18d Crater (Sulky) Based on historical documentation, personnel interviews, site process knowledge, site visits, photographs, engineering drawings, field screening, analytical results, and the results of data quality objectives process (Section 3.0), closure in place with administrative controls or no further action will be implemented for CAU 107.

  1. 2008 Workshop on The Nation's Needs for Isotopes: Present and Future |

    Office of Science (SC) Website

    U.S. DOE Office of Science (SC) 08 Workshop on The Nation's Needs for Isotopes: Present and Future Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources NP Workforce Survey Results .pdf file (182KB) Links News Archives Databases Reports Workshops Nuclear Physics Related Brochures and Videos Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown

  2. 2012 Workshop on Isotope Federal Supply and Demand | U.S. DOE Office of

    Office of Science (SC) Website

    Science (SC) 2 Workshop on Isotope Federal Supply and Demand Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources NP Workforce Survey Results .pdf file (182KB) Links News Archives Databases Reports Workshops Nuclear Physics Related Brochures and Videos Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW

  3. 2013 Workshop on Isotope Federal Supply and Demand | U.S. DOE Office of

    Office of Science (SC) Website

    Science (SC) 3 Workshop on Isotope Federal Supply and Demand Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources NP Workforce Survey Results .pdf file (182KB) Links News Archives Databases Reports Workshops Nuclear Physics Related Brochures and Videos Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW

  4. 2014 Workshop on Isotope Federal Supply and Demand | U.S. DOE Office of

    Office of Science (SC) Website

    Science (SC) 4 Workshop on Isotope Federal Supply and Demand Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources NP Workforce Survey Results .pdf file (182KB) Links News Archives Databases Reports Workshops Nuclear Physics Related Brochures and Videos Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW

  5. 2015 Workshop on Isotope Federal Supply and Demand | U.S. DOE Office of

    Office of Science (SC) Website

    Science (SC) 5 Workshop on Isotope Federal Supply and Demand Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources NP Workforce Survey Results .pdf file (182KB) Links News Archives Databases Reports Workshops Nuclear Physics Related Brochures and Videos Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW

  6. Agenda | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

    2 Workshop on Isotope Federal Supply and Demand » Agenda Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources NP Workforce Survey Results .pdf file (182KB) Links News Archives Databases Reports Workshops Nuclear Physics Related Brochures and Videos Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC

  7. Agenda/Presentations | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

    3 Workshop on Isotope Federal Supply and Demand » Agenda/Presentations Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources NP Workforce Survey Results .pdf file (182KB) Links News Archives Databases Reports Workshops Nuclear Physics Related Brochures and Videos Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW

  8. Agenda/Presentations | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

    4 Workshop on Isotope Federal Supply and Demand » Agenda/Presentations Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources NP Workforce Survey Results .pdf file (182KB) Links News Archives Databases Reports Workshops Nuclear Physics Related Brochures and Videos Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW

  9. Agenda/Presentations | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

    5 Workshop on Isotope Federal Supply and Demand » Agenda/Presentations Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources NP Workforce Survey Results .pdf file (182KB) Links News Archives Databases Reports Workshops Nuclear Physics Related Brochures and Videos Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW

  10. Full Program | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

    Agenda / Presentations Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources NP Workforce Survey Results .pdf file (182KB) Links News Archives Databases Reports Workshops Nuclear Physics Related Brochures and Videos Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301)

  11. Working Group Presentations | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

    Working Group Presentations Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources NP Workforce Survey Results .pdf file (182KB) Links News Archives Databases Reports Workshops Nuclear Physics Related Brochures and Videos Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F:

  12. Archives | U.S. DOE Office of Science (SC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    News Archives Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources NP Workforce Survey Results .pdf file (182KB) Links News Archives Databases Reports Workshops Nuclear Physics Related Brochures and Videos Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833

  13. Reports | U.S. DOE Office of Science (SC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Reports Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources NP Workforce Survey Results .pdf file (182KB) Links News Archives Databases Reports Workshops Nuclear Physics Related Brochures and Videos Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email

  14. Closed Funding Opportunity Announcements (FOAs) | U.S. DOE Office of

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Science (SC) Funding Opportunity Announcements (FOAs) Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Closed Funding Opportunity Announcements (FOAs) Closed Lab Announcements Award Search / Public Abstracts Additional Requirements and Guidance for Digital Data Management Reviews NP Early Career Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy

  15. Relativistic Heavy Ion Collider (RHIC) | U.S. DOE Office of Science (SC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Relativistic Heavy Ion Collider (RHIC) Nuclear Physics (NP) NP Home About Research Facilities User Facilities Argonne Tandem Linac Accelerator System (ATLAS) Continuous Electron Beam Accelerator Facility (CEBAF) Relativistic Heavy Ion Collider (RHIC) Project Development Isotope Program Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown

  16. Continuous Electron Beam Accelerator Facility (CEBAF) | U.S. DOE Office of

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Science (SC) Continuous Electron Beam Accelerator Facility (CEBAF) Nuclear Physics (NP) NP Home About Research Facilities User Facilities Argonne Tandem Linac Accelerator System (ATLAS) Continuous Electron Beam Accelerator Facility (CEBAF) Relativistic Heavy Ion Collider (RHIC) Project Development Isotope Program Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department

  17. Oxidation behaviour of uranium and neptunium in stabilised zirconia

    SciTech Connect (OSTI)

    Walter, Marcus; Somers, Joseph; Bouexiere, Daniel; Gaczynski, Piotr; Brendebach, Boris

    2009-12-15

    Yttria stabilised zirconia (YSZ) based (Zr,Y,U)O{sub 2-x} and (Zr,Y,Np)O{sub 2-x} solid solutions with 6 and 20 mol% actinide were prepared with Y/Zr ratios ranging from 0.2 to 2.0 to investigate uranium and neptunium oxidation behaviour depending on the oxygen vacancies in the defect fluorite lattice. Sintering at 1600 deg. C in Ar/H{sub 2} yields a cubic, fluorite-type structure with U(IV) and Np(IV). Annealing (Zr,Y,U)O{sub 2-x} with Y/Zr=0.2 at 800 deg. C in air results in a tetragonal phase, whereas (Zr,Y,U)O{sub 2-x} with higher Y/Zr ratios and (Zr,Y,Np)O{sub 2-x} retain the cubic structure. XANES and O/M measurements indicate mixed U(V)-U(VI) and Np(IV)-Np(V) oxidation states after oxidation. Based on X-ray diffraction, O/M and EXAFS measurements, different oxidation mechanisms are identified for U- and Np-doped stabilised zirconia. In contrast to U, excess oxygen vacancies are needed to oxidise Np in (Zr,Y,Np)O{sub 2-x} as the oxidation process competes with Zr for oxygen vacancies. As a consequence, U(VI) and Np(V) can only be obtained in stabilised zirconia with Y/Zr=1 but not in YSZ with Y/Zr=0.2. - Graphical abstract: The O/U ratio in oxidised (Zr,Y,U)O{sub 2-x} depends on the Y/U ratio, whereas O/Np in (Zr,Y,Np)O{sub 2-x} correlates with the Y/(Zr+Np) ratio. This indicates that both Zr and Np compete for oxygen vacancies, which hinders the Np oxidation at low Y/Zr ratios. Display Omitted

  18. CRC handbook of agricultural energy potential of developing countries

    SciTech Connect (OSTI)

    Duke, J.A.

    1986-01-01

    The contents of this book are: Introduction; Kenya; Korea (Republic of); Lesotho; Liberia; Malagasy; Malawi; Mali; Mauritania; Mexico, Mozambique, Nepal; Nicaragua; Niger; Nigeria; Pakistan; Panama; Paraguay; Peru; Philippines; Rwanda; Senegal; Sierra Leone; Somalia; Sri Lanka; Sudana; Surinam; Swaziland; Tanzania; Thailand; Togo; Uganda; Uruguay; Venezuela; Zaire; Zambia; Appendix I. Conventional and Energetic Yields; Appendix II, Phytomass Files; and References.

  19. The arsenides LnPd{sub 3}As{sub 2} (Ln = La-Nd, Sm, Gd) and structure refinement of CePd{sub 2-x}As{sub 2} with the ThCr{sub 2}Si{sub 2} structure

    SciTech Connect (OSTI)

    Quebe, P.; Jeitschko, W.

    1995-02-15

    The title compounds were prepared in well-crystallized form by annealing the corresponding binary arsenides in a NaCl/KCl flux. The compounds LnPd{sub 3}As{sub 2} crystallize with a new monoclinic structure type, which was determined from single-crystal X-ray data of GdPd{sub 3}As{sub 2}: C2/m, a = 1656.3(6) pm, b = 404.6(2) pm, c = 993.7(4) pm, {beta} = 107.85(2){degrees}, Z = 6, R = 0.025 for 1728 structure factors and 58 variable parameters. These arsenides belong to a large structural family with a metal to metalloid ratio of 2:1. Somewhat unusual features in the structure of GdPd{sub 3}As{sub 2} are the (distorted) octahedral coordination of one gadolinium site and the square-planar coordination of arsenic atoms around two palladium sites. All of these, however, are also observed for the corresponding atoms in the previously reported, closely related structure of Th{sub 5}Fe{sub 19}P{sub 12}. CePd{sub 2-x}As{sub 2} has the tetragonal ThCr{sub 2}Si{sub 2} structure (a = 425.1(2) pm, c = 1026.1(6)pm, R = 0.023 for 244 F values and 11 variables) with an As-As distance of 247.1(1) pm. The refinement of the occupancy parameter of the palladium position resulted in a value of 87.9(2)% corresponding to the formula CePd{sub 1.758(4)}As{sub 2}. It is argued that the formation of these defects reduces antibonding (destabilizing) Pd-Pd interactions.

  20. Monodisperse and core-shell structured SiO{sub 2}-Lu{sub 2}O{sub 3}:Ln{sup 3+} (Ln=Eu, Tb, Dy, Sm, Er, Ho, and Tm) spherical particles: A facile synthesis and luminescent properties

    SciTech Connect (OSTI)

    Xu, Zhenhe; Feng, Bin; Bian, Shasha; Liu, Tao; Wang, Mingli; Gao, Yu; Sun, Di; Gao, Xin; Sun, Yaguang

    2012-12-15

    The core-shell structured SiO{sub 2}-Lu{sub 2}O{sub 3}:Ln{sup 3+} particles were realized by coating the Lu{sub 2}O{sub 3}:Ln{sup 3+} phosphors onto the surface of non-aggregated, monodisperse and spherical SiO{sub 2} particles by the Pechini sol-gel method. The as-synthesized products were characterized by X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FT-IR), energy-dispersive X-ray (EDX) spectra, scanning electron microscopy (SEM), transmission electron microscopy (TEM), high-resolution transmission electron microscopy (HRTEM), photolumiminescence (PL), and low-voltage cathodoluminescence (CL). The results indicate that the 800 Degree-Sign C annealed sample consists of crystalline Lu{sub 2}O{sub 3} shells and amorphous SiO{sub 2} cores, in spherical shape with a narrow size distribution. The as-obtained particles show strong light emission with different colors corresponding to different Ln{sup 3+} ions under ultraviolet-visible light excitation and low-voltage electron beams excitation, which have potential applications in fluorescent lamps and field emission displays. - Graphical Abstract: Representative SEM and TEM images of the core-shell structured SiO{sub 2}-Lu{sub 2}O{sub 3}:Eu{sup 3+} particles; CIE chromaticity diagram showing the emission colors for SiO{sub 2}-Lu{sub 2}O{sub 3}:Ln{sup 3+}; Multicolor emissions of SiO{sub 2}-Lu{sub 2}O{sub 3}:Ln{sup 3+} particles. Highlights: Black-Right-Pointing-Pointer The core-shell particles were realized by coating the phosphors onto the surface of SiO{sub 2} particles. Black-Right-Pointing-Pointer The sample consists of crystalline Lu{sub 2}O{sub 3} shells and amorphous SiO{sub 2} cores. Black-Right-Pointing-Pointer The particles show different light emission colors corresponding to Ln{sup 3+} ions. Black-Right-Pointing-Pointer They have potential applications in fluorescent lamps and field emission displays.

  1. Measurement of the $WZ\\rightarrow \\ell\

    SciTech Connect (OSTI)

    Abazov, Victor Mukhamedovich; Abbott, Braden Keim; Abolins, Maris A.; Acharya, Bannanje Sripath; Adams, Mark Raymond; Adams, Todd; Alexeev, Guennadi D.; Alkhazov, Georgiy D.; Alton, Andrew K.; Alverson, George O.; Alves, Gilvan Augusto

    2010-06-01

    The standard model (SM) of particle physics has been extensively tested in the past three decades and is found to be in excellent agreement with experimental observations. It is widely assumed, however, that the SM is only a low energy approximation of a more general theory. Therefore, any significant deviation from the SM predictions yields information on the nature of a more fundamental theory. Production of WZ pairs is the least studied diboson process within the SM, as it is a charged final state and can only be produced at hadron colliders. A detailed study of this process probes the electroweak sector of the SM. In addition, searches for new phenomena in the production of heavy gauge boson pairs are interesting, as many extensions of the SM predict 1-4 additional heavy gauge bosons that can decay into a WZ boson pairs.

  2. Therapeutic potential of a non-steroidal bifunctional anti-inflammatory and anti-cholinergic agent against skin injury induced by sulfur mustard

    SciTech Connect (OSTI)

    Chang, Yoke-Chen; Wang, James D.; Hahn, Rita A.; Gordon, Marion K.; Joseph, Laurie B.; Heck, Diane E.; Heindel, Ned D.; Young, Sherri C.; Sinko, Patrick J.; Casillas, Robert P.; Laskin, Jeffrey D.; Laskin, Debra L.; Gerecke, Donald R.

    2014-10-15

    Sulfur mustard (bis(2-chloroethyl) sulfide, SM) is a highly reactive bifunctional alkylating agent inducing edema, inflammation, and the formation of fluid-filled blisters in the skin. Medical countermeasures against SM-induced cutaneous injury have yet to be established. In the present studies, we tested a novel, bifunctional anti-inflammatory prodrug (NDH 4338) designed to target cyclooxygenase 2 (COX2), an enzyme that generates inflammatory eicosanoids, and acetylcholinesterase, an enzyme mediating activation of cholinergic inflammatory pathways in a model of SM-induced skin injury. Adult SKH-1 hairless male mice were exposed to SM using a dorsal skin vapor cup model. NDH 4338 was applied topically to the skin 24, 48, and 72 h post-SM exposure. After 96 h, SM was found to induce skin injury characterized by edema, epidermal hyperplasia, loss of the differentiation marker, keratin 10 (K10), upregulation of the skin wound marker keratin 6 (K6), disruption of the basement membrane anchoring protein laminin 322, and increased expression of epidermal COX2. NDH 4338 post-treatment reduced SM-induced dermal edema and enhanced skin re-epithelialization. This was associated with a reduction in COX2 expression, increased K10 expression in the suprabasal epidermis, and reduced expression of K6. NDH 4338 also restored basement membrane integrity, as evidenced by continuous expression of laminin 332 at the dermal–epidermal junction. Taken together, these data indicate that a bifunctional anti-inflammatory prodrug stimulates repair of SM induced skin injury and may be useful as a medical countermeasure. - Highlights: • Bifunctional anti-inflammatory prodrug (NDH4338) tested on SM exposed mouse skin • The prodrug NDH4338 was designed to target COX2 and acetylcholinesterase. • The application of NDH4338 improved cutaneous wound repair after SM induced injury. • NDH4338 treatment demonstrated a reduction in COX2 expression on SM injured skin. • Changes of skin repair

  3. Aluminoborosilicate glasses codoped with rare-earth elements as radiation-protective covers for solar cells

    SciTech Connect (OSTI)

    Malchukova, E. V. Abramov, A. S.; Nepomnyashchikh, A. I.; Terukov, E. I.

    2015-06-15

    The radiation hardness of aluminoborosilicate glasses codoped with rare-earth ions of Sm, Gd or Sm, Eu in various ratios is studied. The effect of codoping and β irradiation at a dose of 10{sup 9} Gr on the optical transmission and electron paramagnetic resonance spectra is examined. It is found that the introduction of Sm and Gd codopants in a 1 : 1 ratio reduces the number of radiation defects and raises the transmission of irradiated glasses in the visible spectral range.

  4. E

    Office of Scientific and Technical Information (OSTI)

    ... crystalline orientation (A81.4"). The oriented growth presently precludes a unique determination of the Co-Sm phase ... orientations suggesting domain formation a t low fields. ...

  5. Heavy surface state in a possible topological Kondo insulator...

    Office of Scientific and Technical Information (OSTI)

    Heavy surface state in a possible topological Kondo insulator: Magnetothermoelectric transport on the (011) plane of SmB 6 This content will become publicly available on February...

  6. Documentation - Laboratory for Laser Energetics

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    5 - Optomechanical Front Matter - Maintenance Index & Schedules (S-OM-P-030) Subsystem ... HEDVAC Procedures HEDVAC System Maintenance (S-SM-P-331) HEDVAC Pump Maintenance ...

  7. 8.0 FACILITY DISPOSITION PROCESS

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    facility transition, surveillance and maintenance (S&M), and disposition phase activities. ... handling and processing, storage, maintenance, administrative, or support activities ...

  8. Decision Support Tool for Prioritization of Resources Dedicated...

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    Dedicated to Surveillance and Maintenance Activities Challenge The Department of ... are transferred to surveillance and maintenance (S&M), maintenance budgets are reduced ...

  9. Search for: All records | SciTech Connect

    Office of Scientific and Technical Information (OSTI)

    ... Point contact spectroscopy using a superconductor tip on SmBsub 6 films shows both a Kondo Fano resonance and Andeev reflection, indicating an insulating Kondo lattice with ...

  10. 85-GAL DRUM AND NUCFIL-007LS FILTERS

    SciTech Connect (OSTI)

    JB WOODBURY

    2009-06-30

    {sm_bullet} 55-gallon drums were overpacked into 85-gallon drums {sm_bullet} ANucFiI-007LS long-stem filter was installed- NucFiI certified the use of NucFiI-007LS filters in 8S-gallon drums as DOT 7AType A - Wood wedges were used during the tests to center and . stabilize the inner 55-gallon drums {sm_bullet} During inspection, afew filters were found to be loose, canted, and/or with RTV seals broken - No contamination or loss of container integrity {sm_bullet} Discovered in November 2008 U.

  11. International Hydropower Association | Open Energy Information

    Open Energy Info (EERE)

    International Hydropower Association Place: United Kingdom Zip: SM1 4JH Sector: Hydro Product: The International Hydropower Association is a non-governmental mutual association of...

  12. Search for: All records | SciTech Connect

    Office of Scientific and Technical Information (OSTI)

    Filter by Author Ballaran, Tiziana Boffa (2) Kurnosov, Alexander (2) Berkowski, Marek (1) ... Ballaran, Tiziana Boffa ; Kurnosov, Alexander ; Trots, Dmytro December 2013 The Sm:YAG ...

  13. Energy Department Awards Small Business Contract for Legacy Management Work

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    to S.M. Stoller Corporation | Department of Energy Small Business Contract for Legacy Management Work to S.M. Stoller Corporation Energy Department Awards Small Business Contract for Legacy Management Work to S.M. Stoller Corporation July 2, 2007 - 2:54pm Addthis WASHINGTON, DC - The U.S. Department of Energy (DOE) today announced the award of a prime contract for the Department's Office of Legacy Management (LM) Support Services work to S.M. Stoller Corporation for surveillance and

  14. Preliminary Estimates of Combined Heat and Power Greenhouse GasAbatement Potential for California in 2020

    SciTech Connect (OSTI)

    Firestone, Ryan; Ling, Frank; Marnay, Chris; Hamachi LaCommare,Kristina

    2007-07-31

    The objective of this scoping project is to help the California Energy Commission's (CEC) Public Interest Energy Research (PIER) Program determine where it should make investments in research to support combined heat and power (CHP) deployment. Specifically, this project will: {sm_bullet} Determine what impact CHP might have in reducing greenhouse gas (GHG) emissions, {sm_bullet} Determine which CHP strategies might encourage the most attractive early adoption, {sm_bullet} Identify the regulatory and technological barriers to the most attractive CHP strategies, and {sm_bullet} Make recommendations to the PIER program as to research that is needed to support the most attractive CHP strategies.

  15. ORNL/CP-97155 Instantaneous Reactive Power and Power Factor of

    Office of Scientific and Technical Information (OSTI)

    ... cos@ - Components for Power Quality Control and Continuous Diagnostics," Paper ... 98SM202. 3 John S. Hsu, "Induction Motor Field Efficiency Evaluation Using ...

  16. Search for: All records | SciTech Connect

    Office of Scientific and Technical Information (OSTI)

    Eva (4) Toro, Natalia (4) Alves, Daniele S.M. (3) Arvanitaki, Asimina (3) Harrison, Sarah (3) Horn, Bart (3) Izaguirre, Eder (3) Tomasiello, Alessandro (3) Trivedi,...

  17. Evaluation of methods for measuring relative permeability of...

    Office of Scientific and Technical Information (OSTI)

    Dept.; Howarth, S.M. Sandia National Labs., Albuquerque, NM (United States) 05 NUCLEAR FUELS; WIPP; RESERVOIR ROCK; ANHYDRITE; PERMEABILITY; MEASURING METHODS; SITE...

  18. WindStor Power Co WPC | Open Energy Information

    Open Energy Info (EERE)

    Michigan Zip: 48114 Sector: Wind energy Product: Focused on manufacture of WindStor(SM) wind turbine. Coordinates: 50.865669, 4.62993 Show Map Loading map......

  19. http://www.em.doe.gov/Pages/groundwaterReport.aspx?plumeCode...

    Office of Environmental Management (EM)

    Plume) Remediation Contractor: SM Stoller Corp Report Last Updated: 2009 Contaminants Halogenated VOCsSVOCs Present? Yes VOC Name Concentration (ppb) Regulatory Driver Cleanup...

  20. The Secretary of Energy Advisory Board (SEAB) Task Force on Technology...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Maloney, CH2M Hill Gerald Boyd, SM Stoller Corporation * SEAB Member DESIGNATED FEDERAL OFFICIAL: Corey Williams-Allen, Deputy Director, Office of Secretaral Boards and Councils

  1. http://www.em.doe.gov/Pages/groundwaterReport.aspx?plumeCode...

    Office of Environmental Management (EM)

    Legacy Management Plume Name: Chemical Plant (Quarry) Remediation Contractor: SM Stoller ... by naturally occurring chemical reduction process and absorption onto aquifer materials. ...

  2. San Marino: Energy Resources | Open Energy Information

    Open Energy Info (EERE)

    Country Profile Name San Marino Population 32,576 GDP Unavailable Energy Consumption Quadrillion Btu 2-letter ISO code SM 3-letter ISO code SMR Numeric ISO code...

  3. ENDF/B-VII.1 Nuclear Data for Science and Technology: Cross Sections, Covariances, Fission Product Yields and Decay Data

    SciTech Connect (OSTI)

    G. Palmiotti

    2011-12-01

    The ENDF/B-VII.1 library is our latest recommended evaluated nuclear data file for use in nuclear science and technology applications, and incorporates advances made in the five years since the release of ENDF/B-VII.0. These advances focus on neutron cross sections, covariances, fission product yields and decay data, and represent work by the US Cross Section Evaluation Working Group (CSEWG) in nuclear data evaluation that utilizes developments in nuclear theory, modeling, simulation, and experiment. The principal advances in the new library are: (1) An increase in the breadth of neutron reaction cross section coverage, extending from 393 nuclides to 418 nuclides; (2) Covariance uncertainty data for 185 of the most important nuclides, as documented in companion papers in this edition; (3) R-matrix analyses of neutron reactions on light nuclei, including isotopes of He, Li, and Be; (4) Resonance parameter analyses at lower energies and statistical high energy reactions at higher energies for isotopes of F, Cl, K, Ti, V, Mn, Cr, Ni, Zr and W; (5) Modifications to thermal neutron reactions on fission products (isotopes of Mo, Tc, Rh, Ag, Cs, Nd, Sm, Eu) and neutron absorber materials (Cd, Gd); (6) Improved minor actinide evaluations for isotopes of U, Np, Pu, and Am (we are not making changes to the major actinides 235,238U and 239Pu at this point, except for delayed neutron data, and instead we intend to update them after a further period of research in experiment and theory), and our adoption of JENDL-4.0 evaluations for isotopes of Cm, Bk, Cf, Es, Fm, and some other minor actinides; (7) Fission energy release evaluations; (8) Fission product yield advances for fission-spectrum neutrons and 14 MeV neutrons incident on 239Pu; and (9) A new Decay Data sublibrary. Integral validation testing of the ENDF/B-VII.1 library is provided for a variety of quantities: For nuclear criticality, the VII.1 library maintains the generally-good performance seen for VII.0 for a wide

  4. News and Resources | U.S. DOE Office of Science (SC)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    News and Resources Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email Us More Information » News and Resources Print Text Size: A A A FeedbackShare Page The address you entered is no longer valid.

  5. Encapsulation of Gold Nanoparticles in a DNA Origami Cage

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    Encapsulation of Gold Nanoparticles in a DNA Origami Cage Authors: Zhao, Z., Jacovetty, E. L., Liu, Y., and Yan, H. Title: Encapsulation of Gold Nanoparticles in a DNA Origami Cage Source: Angewandte Chemie International Edition Year: 2011 Volume: 50 Pages: 2041-2044 ABSTRACT: A critical challenge in nanoparticle (NP) surface functionalization is to label the NP surface with a single copy of a functional group or to display multiple, unique molecules on the NP surface with control of the

  6. Facilities | U.S. DOE Office of Science (SC)

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    Facilities Nuclear Physics (NP) NP Home About Research Facilities User Facilities Project Development Isotope Program Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email Us More Information » Facilities Print Text Size: A A A FeedbackShare

  7. Ripples Ruffle Primordial Plasma | U.S. DOE Office of Science (SC)

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    Ripples Ruffle Primordial Plasma Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email Us More Information » 11.01.15 Ripples Ruffle Primordial Plasma RHIC physicists discover key evidence for a

  8. 2013 | U.S. DOE Office of Science (SC)

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    3 Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email Us More Information » Science Highlights 2013 Print Text Size: A A A FeedbackShare Page Filter by Performer Or press Esc Key to close. close

  9. 2014 | U.S. DOE Office of Science (SC)

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    4 Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email Us More Information » Science Highlights 2014 Print Text Size: A A A FeedbackShare Page Filter by Performer Or press Esc Key to close. close

  10. 2015 | U.S. DOE Office of Science (SC)

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    5 Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email Us More Information » Science Highlights 2015 Print Text Size: A A A FeedbackShare Page Filter by Performer Or press Esc Key to close. close

  11. Applications of Nuclear Science Archives | U.S. DOE Office of Science (SC)

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    Applications of Nuclear Science » Applications of Nuclear Science Archives Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of Nuclear Science Applications of Nuclear Science Archives Small Business Innovation Research / Small Business Technology Transfer Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence

  12. European Labs | U.S. DOE Office of Science (SC)

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    European Labs Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of Nuclear Science Small Business Innovation Research / Small Business Technology Transfer Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email Us More Information »

  13. Isotope Related Reports | U.S. DOE Office of Science (SC)

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    Isotope Related Reports Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email Us More Information » Isotope Development & Production for Research and Applications (IDPRA) Isotope Related Reports

  14. Nidc Orgchart | U.S. DOE Office of Science (SC)

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    Nidc Orgchart Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email Us More Information » Isotope Development & Production for Research and Applications (IDPRA) Nidc Orgchart Print Text Size: A A

  15. SBIR STTR Exchange Meeting 2011 | U.S. DOE Office of Science (SC)

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    Meeting 2011 Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of Nuclear Science Small Business Innovation Research / Small Business Technology Transfer Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email Us More Information » Small

  16. SBIR STTR Exchange Mtg 2010 | U.S. DOE Office of Science (SC)

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  17. SBIR STTR Exchange Mtg 2013 Presentations | U.S. DOE Office of Science (SC)

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  18. SBIR/STTR Exchange Meeting August 6-7, 2014 | U.S. DOE Office of Science

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  19. SBIR/STTR Exchange Meeting August 6-7, 2015 | U.S. DOE Office of Science

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  20. SBIR/STTR Exchange Meeting November 6-7, 2013 | U.S. DOE Office of Science

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    (SC) November 6-7, 2013 Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of Nuclear Science Small Business Innovation Research / Small Business Technology Transfer Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email Us More

  1. Small Business Innovation Research/Small Business Technology Transfer

    Office of Science (SC) Website

    Meeting August, 9-10, 2016 | U.S. DOE Office of Science (SC) Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of Nuclear Science Small Business Innovation Research / Small Business Technology Transfer Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F:

  2. Supply and Demand of Helium-3| U.S. DOE Office of Science (SC)

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    Supply and Demand of Helium-3 Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E: Email Us More Information » Isotope Development & Production for Research and Applications (IDPRA) Supply and Demand

  3. sbir sttr exchange mtg 2012 | U.S. DOE Office of Science (SC)

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    SBIR/STTR Exchange Meeting October 1-2, 2012 Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of Nuclear Science Small Business Innovation Research / Small Business Technology Transfer Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000 Independence Ave., SW Washington, DC 20585 P: (301) 903-3613 F: (301) 903-3833 E:

  4. Accelerator Mass Spectrometry | U.S. DOE Office of Science (SC)

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  5. Accelerators for Testing Radiation Tolerances of Electronics at TAMU | U.S.

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  6. Atom Trap Trace Analysis at ANL | U.S. DOE Office of Science (SC)

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  7. Awake Animal Imaging at BNL | U.S. DOE Office of Science (SC)

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  8. Basic Research for an Era of Nuclear Energy at LBNL, LLNL, AND LANL | U.S.

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  9. Beryllium-7 Implantation in Plastics for Prosthesis Wear Studies | U.S. DOE

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  10. Biomedical Instrumentation and Imaging at TJNAF | U.S. DOE Office of

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  11. Boron-Nitride (BN) Nanotubes (BNNT) at TJNAF| U.S. DOE Office of Science

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  12. Carbon Nanotubes and Nano-Structure Manufacturing at TJNAF | U.S. DOE

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    Office of Science (SC) Carbon Nanotubes and Nano-Structure Manufacturing at TJNAF Nuclear Physics (NP) NP Home About Research Facilities Science Highlights Benefits of NP Applications of Nuclear Science Applications of Nuclear Science Archives Small Business Innovation Research / Small Business Technology Transfer Funding Opportunities Nuclear Science Advisory Committee (NSAC) Community Resources Contact Information Nuclear Physics U.S. Department of Energy SC-26/Germantown Building 1000

  13. Cyclotrons to Make Neutrons & Radioactive Targets for SBSS at LBNL | U.S.

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