National Library of Energy BETA

Sample records for neutron scattering instrumentation

  1. Elastic Incoherent Neutron Scattering, operating by varying instrumental energy resolution, Principles, Simulations and Experiments of the Resolution Elastic Neutron

    E-Print Network [OSTI]

    Doster, Wolfgang

    Elastic Incoherent Neutron Scattering, operating by varying instrumental energy resolution, Principles, Simulations and Experiments of the Resolution Elastic Neutron Scattering (RENS) by Magazu a different name "RENS" (resolution dependent elastic neutron scattering) [1-5]. Our ERS papers, first

  2. Instrumentation for Neutron Scattering at the Missouri University Research Reactor Paul F. Miceli

    E-Print Network [OSTI]

    Montfrooij, Wouter

    Instrumentation for Neutron Scattering at the Missouri University Research Reactor Paul F. Miceli Research Reactor (MURR) provides significant thermal neutron flux, which enables neutron scattering]. There are presently 5 instruments located on the beam port floor that are dedicated to neutron scattering: (1) TRIAX

  3. Instrumentation development for neutron scattering at high pressure 

    E-Print Network [OSTI]

    Fang, Junwei

    2012-11-29

    Neutron scattering at extremes of pressure is a powerful tool for studying the response of structural and magnetic properties of materials on microscopic level to applied stresses. However, experimental neutron studies ...

  4. Bragg optics computer codes for neutron scattering instrument design

    SciTech Connect (OSTI)

    Popovici, M.; Yelon, W.B.; Berliner, R.R.; Stoica, A.D.

    1997-09-01

    Computer codes for neutron crystal spectrometer design, optimization and experiment planning are described. Phase space distributions, linewidths and absolute intensities are calculated by matrix methods in an extension of the Cooper-Nathans resolution function formalism. For modeling the Bragg reflection on bent crystals the lamellar approximation is used. Optimization is done by satisfying conditions of focusing in scattering and in real space, and by numerically maximizing figures of merit. Examples for three-axis and two-axis spectrometers are given.

  5. A neutron imaging device for sample alignment in a pulsed neutron scattering instrument

    SciTech Connect (OSTI)

    Grazzi, F.; Scherillo, A.; Zoppi, M.

    2009-09-15

    A neutron-imaging device for alignment purposes has been tested on the INES beamline at ISIS, the pulsed neutron source of Rutherford Appleton Laboratory (U.K.). Its use, in conjunction with a set of movable jaws, turns out extremely useful for scattering application to complex samples where a precise and well-defined determination of the scattering volume is needed.

  6. For more information about each of these instruments go to neutrons.ornl.gov, or contact Neutron Scattering Science User Office, neutronusers@ornl.gov or

    E-Print Network [OSTI]

    -Small-Angle Neutron Scattering Instrument (USANS)* · BL-1B Nanoscale-Ordered Materials Diffractometer (NOMAD) · BL-2For more information about each of these instruments go to neutrons.ornl.gov, or contact Neutron Scattering Science User Office, neutronusers@ornl.gov or (865) 574-4600. Proposals for beam time at Oak Ridge

  7. March, 2001 Neutron Scattering Group

    E-Print Network [OSTI]

    Johnson, Peter D.

    March, 2001 Neutron Scattering Group A High Performance Hybrid Spectrometer for theA High of the instrument performance · Igor Zaliznyak · Laurence Passell OutlineOutline #12;Neutron Scattering GroupNeutron states in single crystals.single crystals. #12;Neutron Scattering GroupNeutron Scattering Group What

  8. The 40m General Purpose Small-Angle Neutron Scattering Instrument at Oak Ridge National Laboratory

    SciTech Connect (OSTI)

    Wignall, George D [ORNL; Bailey, Katherine M [ORNL; Buchanan, Michelle V [ORNL; Butler, Paul D [ORNL; Heller, William T [ORNL; Littrell, Ken [ORNL; Lynn, Gary W [ORNL; Melnichenko, Yuri B [ORNL; Myles, Dean A A [ORNL; Urban, Volker S [ORNL

    2012-01-01

    A high-flux, 40m long small-angle neutron scattering (SANS) instrument has been constructed at Oak Ridge National Laboratory (ORNL). The facility utilizes a mechanical velocity selector, pinhole collimation and a high count-rate (> 105 Hz), large-area (1m2) two-dimensional position-sensitive detector. The incident wavelength ( ), resolution ( / ), incident collimation and sample-detector distance are independently variable under computer control. The detector can translate 45cm off axis to increase the overall Q-range (< 0.001 < Q = 4 -1sin < 1 -1), where 2 is the angle of scatter. The design and characteristics of this instrument are described along with examples of scattering data to illustrate the performance.

  9. Demonstration of a novel focusing small-angle neutron scattering instrument equipped with axisymmetric mirrors

    E-Print Network [OSTI]

    Liu, Dazhi

    Small-angle neutron scattering (SANS) is the most significant neutron technique in terms of impact on science and engineering. However, the basic design of SANS facilities has not changed since the technique’s inception ...

  10. Requirements, possible alternatives & international NEUTRON SCATTERING

    E-Print Network [OSTI]

    Dimeo, Robert M.

    Requirements, possible alternatives & international NEUTRON SCATTERING DETECTORS for Rob Dimeo NIST neutron scattering instruments are the most demanding require background low #12;#12;The Helium-3 Supply Crisis ­ Alternative Techniques to Helium-3 based Detectors for Neutron Scattering Applications

  11. Neutron Scattering Group February, 2001

    E-Print Network [OSTI]

    Johnson, Peter D.

    Neutron Scattering Group February, 2001 A High Performance Instrument for the Single Crystal Igor Zaliznyak Outline #12;Neutron Scattering Group Neutron spectrometer for studies of the low-energy coherent excitations in single crystals. Common requirements for a single crystal neutron spectrometer

  12. Small-angle Neutron Scattering for Molecular Biology: Basics and Instrumentation

    SciTech Connect (OSTI)

    Heller, William T [ORNL; Littrell, Ken [ORNL

    2009-01-01

    As researchers strive to understand the interplay between the complex molecular systems that make up living cells, tools for characterizing the interactions between the various players involved have developed. Small-angle neutron scattering (SANS) plays an important role in building a molecular-level understanding of the structures of macromolecular systems that make up cells. SANS is widely applicable to the study of biological structures including, but by no means limited to, protein-protein or protein-nucleic acid complexes, lipid membranes, cellular scaffolding, and amyloid plaques. Here, we present a brief description of the technique as it is commonly applied to the study of biological systems and an overview instrumentation that is available at the various facilities around the world.

  13. Instruments | Neutron Science | ORNL

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Neutrons and Pressure Diffractometer CG-2 GP-SANS - General-Purpose Small-Angle Neutron Scattering Diffractometer 4A MR - Magnetism Reflectometer CG-3 Bio-SANS -...

  14. Neutron Scattering Tutorials | Neutron Science | ORNL

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Neutron Scattering Tutorials SHARE Neutron Scattering Tutorials The following lectures were presented at the 2011 and 2010 National School on Neutron & X-Ray Scattering. This...

  15. UNIVERSITY OF CALIFORNIA Inelastic Neutron Scattering Study of the

    E-Print Network [OSTI]

    Lawrence, Jon

    UNIVERSITY OF CALIFORNIA IRVINE Inelastic Neutron Scattering Study of the Intermediate Valence . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2.2 Inelastic Neutron Scattering . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2.2.a Neutron Scattering Instruments . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2.2.b

  16. Response to 'Comment on 'Elastic incoherent neutron scattering operating by varying instrumental energy resolution: Principle, simulations, and experiments of the resolution elastic neutron scattering (RENS)'' [Rev. Sci. Instrum. 83, 107101 (2012)

    SciTech Connect (OSTI)

    Magazu, Salvatore; Migliardo, Federica; Benedetto, Antonio [Dipartimento di Fisica, Universita di Messina, C.da Papardo n Degree-Sign 31, P.O. Box 55, Vill. S. Agata 98166 Messina (Italy)

    2012-10-15

    Recently [S. Magazu et al., Rev. Sci. Instrum. 82, 105115 (2011)] we have proposed a new method for characterizing, by neutron scattering, the dynamical properties of complex material systems, such as, the ones of interest in the biophysical field. This approach called Resolution Elastic Neutron Scattering, in short RENS, is based on the detection of the elastically scattered neutron intensity as a function of the instrumental energy resolution. By experimental, theoretical, and numerical findings, we have pointed out that an inflection point occurs in the elastic intensity when the system relaxation time approaches the instrumental energy resolution time. This approach, differently from quasi-elastic neutron scattering (QENS), gives the chance to evaluate the system relaxation times without using pre-defined models that can be wrong and/or misleading. Here, we reply to a Comment on the above-mentioned main paper in which Wuttke proposes a different approach to evaluate the above-mentioned inflection point; on this regard, it should be noticed that the existence of the inflection point, which is the main topic of our work, is not questioned and that the approach proposed by Wuttke in the Comment, although valid for a class of dynamical processes, is not applicable when different and distinct processes occur simultaneously at different time scale.

  17. Neutron scatter camera

    DOE Patents [OSTI]

    Mascarenhas, Nicholas; Marleau, Peter; Brennan, James S.; Krenz, Kevin D.

    2010-06-22

    An instrument that will directly image the fast fission neutrons from a special nuclear material source has been described. This instrument can improve the signal to background compared to non imaging neutron detection techniques by a factor given by ratio of the angular resolution window to 4.pi.. In addition to being a neutron imager, this instrument will also be an excellent neutron spectrometer, and will be able to differentiate between different types of neutron sources (e.g. fission, alpha-n, cosmic ray, and D-D or D-T fusion). Moreover, the instrument is able to pinpoint the source location.

  18. Neutron Scattering User Program | Neutron Science | ORNL

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    User Program SHARE Neutron Scattering Can Benefit Your Research Neutron scattering has applications in almost every technical and scientific field, from biology and chemistry to...

  19. Lujan Neutron Scattering Center

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    the inadvertent spread of Technetium 99 by employees and contractors at the Lujan Neutron Scattering Center August 27, 2012-The Laboratory is investigating the inadvertent...

  20. Small Angle Neutron Scattering

    SciTech Connect (OSTI)

    Urban, Volker S [ORNL

    2012-01-01

    Small Angle Neutron Scattering (SANS) probes structural details at the nanometer scale in a non-destructive way. This article gives an introduction to scientists who have no prior small-angle scattering knowledge, but who seek a technique that allows elucidating structural information in challenging situations that thwart approaches by other methods. SANS is applicable to a wide variety of materials including metals and alloys, ceramics, concrete, glasses, polymers, composites and biological materials. Isotope and magnetic interactions provide unique methods for labeling and contrast variation to highlight specific structural features of interest. In situ studies of a material s responses to temperature, pressure, shear, magnetic and electric fields, etc., are feasible as a result of the high penetrating power of neutrons. SANS provides statistical information on significant structural features averaged over the probed sample volume, and one can use SANS to quantify with high precision the structural details that are observed, for example, in electron microscopy. Neutron scattering is non-destructive; there is no need to cut specimens into thin sections, and neutrons penetrate deeply, providing information on the bulk material, free from surface effects. The basic principles of a SANS experiment are fairly simple, but the measurement, analysis and interpretation of small angle scattering data involves theoretical concepts that are unique to the technique and that are not widely known. This article includes a concise description of the basics, as well as practical know-how that is essential for a successful SANS experiment.

  1. Simulation of a D-T Neutron Source for Neutron Scattering Experiments

    E-Print Network [OSTI]

    Lou, T.P.; Ludewigt, B.A.; Vujic, J.L.; Leung, K.-N.

    2003-01-01

    T Neutron Source for Neutron Scattering Experiments T.P. Louor cold neutrons for neutron scattering experiments. Thisto simulate a neutron scattering setup and to estimate

  2. Search for: "neutron scattering" | DOE PAGES

    Office of Scientific and Technical Information (OSTI)

    neutron scattering" Find + Advanced Search Advanced Search All Fields: "neutron scattering" Title: Full Text: Bibliographic Data: Creator Author: Name Name ORCID Search...

  3. 11th LANSCE School on Neutron Scattering

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    11th LANSCE School on Neutron Scattering LANSCE 11th LANSCE School on Neutron Scattering Home Abstract Lecturers Lecturer Abstracts Hands-On Experiments Free Day About the...

  4. SciTech Connect: "neutron scattering"

    Office of Scientific and Technical Information (OSTI)

    neutron scattering" Find + Advanced Search Term Search Semantic Search Advanced Search All Fields: "neutron scattering" Semantic Semantic Term Title: Full Text: Bibliographic...

  5. BUILDING A NETWORK FOR NEUTRON SCATTERING EDUCATION

    SciTech Connect (OSTI)

    Pynn, Roger; Baker, Shenda Mary; Louca, Despo A; McGreevy, Robert L; Ekkebus, Allen E; Kszos, Lynn A; Anderson, Ian S

    2008-10-01

    In a concerted effort supported by the National Science Foundation, the Department of Commerce, and the Department of Energy, the United States is rebuilding its leadership in neutron scattering capability through a significant investment in U.S. neutron scattering user facilities and related instrumentation. These unique facilities provide opportunities in neutron scattering to a broad community of researchers from academic institutions, federal laboratories, and industry. However, neutron scattering is often considered to be a tool for 'experts only' and in order for the U.S. research community to take full advantage of these new and powerful tools, a comprehensive education and outreach program must be developed. The workshop described below is the first step in developing a national program that takes full advantage of modern education methods and leverages the existing educational capacity at universities and national facilities. During March 27-28, 2008, a workshop entitled 'Building a Network for Neutron Scattering Education' was held in Washington, D.C. The goal of the workshop was to define and design a roadmap for a comprehensive neutron scattering education program in the United States. Successful implementation of the roadmap will maximize the national intellectual capital in neutron sciences and will increase the sophistication of research questions addressed by neutron scattering at the nation's forefront facilities. (See Appendix A for the list of attendees, Appendix B for the workshop agenda, Appendix C for a list of references. Appendix D contains the results of a survey given at the workshop; Appendix E contains summaries of the contributed talks.) The workshop brought together U.S. academicians, representatives from neutron sources, scientists who have developed nontraditional educational programs, educational specialists, and managers from government agencies to create a national structure for providing ongoing neutron scattering education. A concerted effort was made to involve representatives from historically black colleges and universities (HBCUs) and minority educational institutions (MEIs). The roadmap contained herein provides the path to a national infrastructure for education of students, faculty, and professional researchers who wish to make use of national neutron scattering facilities but do not have (or do not believe they have) the educational background to do so. Education of other stakeholders, including the public, students in kindergarten through twelfth grade (K-12), and policy makers is also included. The opening sessions of the workshop provided the current status of neutron scattering education in North America, Europe, and Australia. National neutron sources have individually developed outreach and advertising programs aimed at increasing awareness among researchers of the potential applications of neutron scattering. However, because their principal mission is to carry out scientific research, their outreach efforts are necessarily self-limiting. The opening session was designed to build awareness that the individual programs need to be coupled with, and integrated into, a broader education program that addresses the complete range of experience, from the student to the experienced researcher, and the wide range of scientific disciplines covered by neutron scattering. Such a program must also take full advantage of existing educational programs and expertise at universities and expand them using modern distance learning capabilities, recognizing that the landscape of education is changing.

  6. RisR1125(EN) Neutron Scattering

    E-Print Network [OSTI]

    Risø­R­1125(EN) Neutron Scattering Studies of Modulated Magnetic Structures Steen Aagaard Sørensen investigations of the magnetic systems DyFe4Al8 and MnSi by neutron scattering and in the former case also by X and the correlations between the scattering entities of the sample. The theoretical framework of neutron scattering

  7. 10th LANSCE School on Neutron Scattering

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    10th LANSCE School on Neutron Scattering LANSCE 10th LANSCE School on Neutron Scattering Home Abstract Lecturers Hands-On Experiments Free Day About the School Sponsors FAQ's...

  8. Neutron-deuteron breakup and quasielastic scattering

    E-Print Network [OSTI]

    Ohlson, Alice Elisabeth

    2009-01-01

    Quasielastic scattering and deuteron breakup in the 200 MeV region is studied by impinging a pulsed neutron beam on a deuterium target at the Weapons Neutron Research facility at the Los Alamos Neutron Science Center. The ...

  9. Measurements of the Thermal Neutron Scattering Kernel

    E-Print Network [OSTI]

    Danon, Yaron

    Measurements of the Thermal Neutron Scattering Kernel Li (Emily) Liu, Yaron Danon, Bjorn Becker and discussions Problems and Future study Questions #12;3 M. Mattes and J. Keinert, Thermal Neutron Scattering experimental data used was from 1973-1974! M. Mattes and J. Keinert, Thermal Neutron Scattering Data

  10. Neutron Scattering Studies of Correlated Electron Systems

    E-Print Network [OSTI]

    Boothroyd, Andrew

    Neutron Scattering Studies of Correlated Electron Systems Lucy Helme Thesis submitted submitted for the Degree of Doctor of Philosophy, Trinity Term 2006 This thesis presents neutron scatteringO2, through inelastic neutron scattering studies of the crystal field transitions above and below

  11. Optimizing moderator dimensions for neutron scattering at the spallation neutron source

    SciTech Connect (OSTI)

    Zhao, J. K.; Robertson, J. L.; Herwig, Kenneth W.; Gallmeier, Franz X.; Riemer, Bernard W. [Instrument and Source Division, Spallation Neutron Source, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831 (United States)] [Instrument and Source Division, Spallation Neutron Source, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831 (United States)

    2013-12-15

    In this work, we investigate the effect of neutron moderator dimensions on the performance of neutron scattering instruments at the Spallation Neutron Source (SNS). In a recent study of the planned second target station at the SNS facility, we have found that the dimensions of a moderator play a significant role in determining its surface brightness. A smaller moderator may be significantly brighter over a smaller viewing area. One of the immediate implications of this finding is that for modern neutron scattering instrument designs, moderator dimensions and brightness have to be incorporated as an integrated optimization parameter. Here, we establish a strategy of matching neutron scattering instruments with moderators using analytical and Monte Carlo techniques. In order to simplify our treatment, we group the instruments into two broad categories: those with natural collimation and those that use neutron guide systems. For instruments using natural collimation, the optimal moderator selection depends on the size of the moderator, the sample, and the moderator brightness. The desired beam divergence only plays a role in determining the distance between sample and moderator. For instruments using neutron optical systems, the smallest moderator available that is larger than the entrance dimension of the closest optical element will perform the best (assuming, as is the case here that smaller moderators are brighter)

  12. Neutron inelastic scattering in natural Pb as a background in...

    Office of Scientific and Technical Information (OSTI)

    SCATTERING; ISOTOPES; LEAD; LEAD 206; LEAD 207; LEVELS; NEUTRONS; SCATTERING Inelastic neutron scattering on Pb isotopes can result in gamma rays near the signature endpoint...

  13. Optimizing Moderator Dimensions for Neutron Scattering at the Spallation Neutron Source

    SciTech Connect (OSTI)

    Zhao, Jinkui [ORNL; Robertson, Lee [ORNL; Herwig, Kenneth W [ORNL; Gallmeier, Franz X [ORNL; Riemer, Bernie [ORNL

    2013-01-01

    In this work, we investigate the effect of neutron moderator dimensions on the performance of neutron scattering instruments at the Spallation Neutron Source. In a recent study of the planned second target station at the Spallation Neutron Source (SNS) facility [1,2], we have found that the dimensions of a moderator play a significant role in determining its surface brightness. A smaller moderator may be significantly brighter for a smaller viewing area [4]. One of the immediate implications of this finding is that for modern neutron scattering instrument designs, moderator dimensions and brightness have to be incorporated as an integrated optimization parameter. Here, we establish a strategy of matching neutron scattering instruments with moderators using analytical and Monte Carlo techniques. In order to simplify our treatment, we group the instruments into two broad categories, those with natural collimation and those that use neutron guide systems. We found that the cross-sections of the sample and the neutron guide, respectively, are the deciding factors for choosing the moderator. Beam divergence plays no role as long as it is within the reach of practical constraints. Namely, the required divergence is not too large for the guide or sample to be located close enough to the moderator on an actual spallation source.

  14. EXPERIMENTS ON N-P SCATTERING WITH 260 MEV NEUTRONS

    E-Print Network [OSTI]

    Kelly, E.; Leith, C.; Segre, E.; Wiegand, C.

    1950-01-01

    FIG. IN MEV Mu 56 NEUTRON SCATTERING ANGLE FIG 3 Mu 57EXPERIWNTS ON N-P SCATTERING WITH 260 MEV NEUTRONS Eo Refly,EXPERIMENTS OM N-P SCATTERING WITH 260 MEV NEUTRONS E Kelly,

  15. Fully portable, highly flexible dilution refrigerator systems for neutron scattering

    E-Print Network [OSTI]

    Boyer, Edmond

    775 Fully portable, highly flexible dilution refrigerator systems for neutron scattering P. A systems developed specifically for neutron scattering environ- ments. The refrigerators are completely relatively recently however, the lowest temperatures available in almost all neutron scattering laboratories

  16. Neutron scattering Materials research for modern life Almost all of the major changes in our society, the dramatic

    E-Print Network [OSTI]

    Crowther, Paul

    Neutron scattering Materials research for modern life #12;Almost all of the major changes in our scattering experiments, materials are exposed to intense beams of neutrons inside specialised instruments that neutron scattering science contributes to our lives. Because of the collaborative nature of modern

  17. Application of Neutron Imaging and Scattering to Fluid Flow and...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Application of Neutron Imaging and Scattering to Fluid Flow and Fracture in EGS Environments Application of Neutron Imaging and Scattering to Fluid Flow and Fracture in EGS...

  18. Quasielastic Neutron Scattering Study of Water Confined in Carbon...

    Office of Scientific and Technical Information (OSTI)

    Quasielastic Neutron Scattering Study of Water Confined in Carbon Nanopores Citation Details In-Document Search Title: Quasielastic Neutron Scattering Study of Water Confined in...

  19. Neutron scattering of iron-based superconductors (Journal Article...

    Office of Scientific and Technical Information (OSTI)

    Neutron scattering of iron-based superconductors Citation Details In-Document Search Title: Neutron scattering of iron-based superconductors Low-energy spin excitations have been...

  20. Proton Angular Distribution for 90 Mev Neutron-proton Scattering

    E-Print Network [OSTI]

    Hadley, James

    2010-01-01

    recoil protons in neutron -proton scattering at 90 Mev hasFOR 90 lWEV NEUTRON-PROTON SCATTERING James Hadley, Cecil E.

  1. 2012 LANSCE Neutron Scattering School | Los Alamos National Laboratory

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    2 LANSCE Neutron Scattering School LANSCE 2012 LANSCE Neutron Scattering School Home About the School Hands-On Experiments Quick Links Application - Closed Schedule Poster...

  2. Neutron inelastic scattering in natural Pb as a background in...

    Office of Scientific and Technical Information (OSTI)

    Neutron inelastic scattering in natural Pb as a background in neutrinoless double-beta decay experiments Citation Details In-Document Search Title: Neutron inelastic scattering in...

  3. 2012 LANSCE Neutron Scattering School | Los Alamos National Laboratory

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    1 LANSCE Neutron Scattering School LANSCE 2011 LANSCE Neutron Scattering School Home NSS 2011 About the School Lecturers Hands-On Experiments Quick Links Application Schedule...

  4. International Conference on Neutron Scattering 2005 Darling Harbour. Sydney. Australia

    E-Print Network [OSTI]

    International Conference on Neutron Scattering 2005 Darling Harbour. Sydney. Australia 27 November, Hillerød, Denmark Combined application of small-angle neutron scattering and oscillatory shear

  5. A New Polyethylene Scattering Law Determined Using Inelastic Neutron Scattering

    SciTech Connect (OSTI)

    Lavelle, Christopher M [ORNL; Liu, C [Oak Ridge National Laboratory (ORNL); Stone, Matthew B [ORNL

    2013-01-01

    Monte Carlo neutron transport codes such as MCNP rely on accurate data for nuclear physics cross-sections to produce accurate results. At low energy, this takes the form of scattering laws based on the dynamic structure factor, S (Q, E). High density polyethylene (HDPE) is frequently employed as a neutron moderator at both high and low temperatures, however the only cross-sections available are for T =300 K, and the evaluation has not been updated in quite some time. In this paper we describe inelastic neutron scattering measurements on HDPE at 5 and 300 K which are used to improve the scattering law for HDPE. We describe the experimental methods, review some of the past HDPE scattering laws, and compare computations using these models to the measured S (Q, E). The total cross-section is compared to available data, and the treatment of the carbon secondary scatterer as a free gas is assessed. We also discuss the use of the measurement itself as a scattering law via the 1 phonon approximation. We show that a scattering law computed using a more detailed model for the Generalized Density of States (GDOS) compares more favorably to this experiment, suggesting that inelastic neutron scattering can play an important role in both the development and validation of new scattering laws for Monte Carlo work.

  6. Scattered neutron tomography based on a neutron transport problem 

    E-Print Network [OSTI]

    Scipolo, Vittorio

    2005-11-01

    and scattered images generated from a beam passing through an optically thick object. This inverse problem makes use of a computationally efficient, two-dimensional forward problem based on neutron transport theory that effectively calculates the detector...

  7. A workshop on enhanced national capability for neutron scattering

    SciTech Connect (OSTI)

    Hurd, Alan J [Los Alamos National Laboratory; Rhyne, James J [Los Alamos National Laboratory; Lewis, Paul S [Los Alamos National Laboratory

    2009-01-01

    This two-day workshop will engage the international neutron scattering community to vet and improve the Lujan Center Strategic Plan 2007-2013 (SP07). Sponsored by the LANL SC Program Office and the University of California, the workshop will be hosted by LANSCE Professor Sunny Sinha (UCSD). Endorsement by the Spallation Neutron Source will be requested. The discussion will focus on the role that the Lujan Center will play in the national neutron scattering landscape assuming full utilization of beamlines, a refurbished LANSCE, and a 1.4-MW SNS. Because the Lujan Strategic Plan is intended to set the stage for the Signature Facility era at LANSCE, there will be some discussion of the long-pulse spallation source at Los Alamos. Breakout groups will cover several new instrument concepts, upgrades to present instruments, expanded sample environment capabilities, and a look to the future. The workshop is in keeping with a request by BES to update the Lujan strategic plan in coordination with the SNS and the broader neutron community. Workshop invitees will be drawn from the LANSCE User Group and a broad cross section of the US, European, and Pacific Rim neutron scattering research communities.

  8. 2010 American Conference on Neutron Scattering (ACNS 2010)

    SciTech Connect (OSTI)

    Billinge, Simon

    2011-06-17

    The ACNS provides a focal point for the national neutron user community to strengthen ties within this diverse group, while at the same time promoting neutron research among colleagues in related disciplines identified as “would-be” neutron users. The American Conference on Neutron Scattering thus serves a dual role as a national user meeting and a scientific meeting. As a venue for scientific exchange, the ACNS showcases recent results and provides forums for scientific discussion of neutron research in diverse fields such as hard and soft condensed matter, liquids, biology, magnetism, engineering materials, chemical spectroscopy, crystal structure, and elementary excitations, fundamental physics and development of neutron instrumentation through a combination of invited talks, contributed talks and poster sessions. As a “super-user” meeting, the ACNS fulfills the main objectives of users' meetings previously held periodically at individual national neutron facilities, with the advantage of a larger and more diverse audience. To this end, each of the major national neutron facilities (NIST, LANSCE, HFIR and SNS) have an opportunity to exchange information and update users, and potential users, of their facility. This is also an appropriate forum for users to raise issues that relate to the facilities. For many of the national facilities, this super-user meeting should obviate the need for separate user meetings that tax the time, energy and budgets of facility staff and the users alike, at least in years when the ACNS is held. We rely upon strong participation from the national facilities. The NSSA intends that the American Conference on Neutron Scattering (ACNS) will occur approximately every two years, but not in years that coincide with the International or European Conferences on Neutron Scattering. The ACNS is to be held in association with one of the national neutron centers in a rotating sequence, with the host facility providing local organization and planning assistance. Additional logistical support is being provided this year through a partnership with the conferencing office of the Materials Research Society (MRS). The ACNS, targeting the entire potential neutron North American user community, complements the annual NIST, ANL and LANSCE neutron and scattering schools which give hands-on experience primarily to graduate students who anticipate using neutron scattering in their thesis research. The summer schools are promoted at the ACNS and represent a natural path for students to take after being inspired by the activities of the ACNS.

  9. Neutron Scattering of CeNi at the Spallation Neutron Source at...

    Office of Scientific and Technical Information (OSTI)

    Spallation Neutron Source at Oak Ridge National Laboratory: A Preliminary Report Citation Details In-Document Search Title: Neutron Scattering of CeNi at the Spallation Neutron...

  10. Neutron scattering Materials research for modern life Almost all of the major changes in our society, the dramatic

    E-Print Network [OSTI]

    Neutron scattering Materials research for modern life #12;Almost all of the major changes in our on the atomic scale, and to use this knowledge to optimise the properties or develop new materials. In neutron scattering experiments, materials are exposed to intense beams of neutrons inside specialised instruments

  11. The Neutron Scattering Society www.neutronscattering.org

    E-Print Network [OSTI]

    Chen, Sow-Hsin

    The Neutron Scattering Society of America www.neutronscattering.org Press Release, February 4, 2008 The Neutron Scattering Society of America is pleased to announce the 2008 recipients of its 3 major prizes. The Neutron Scattering Society of America (NSSA) established the Clifford G. Shull Prize in Neutron Science

  12. Neutron and X-ray Scattering Study of Magnetic Manganites

    E-Print Network [OSTI]

    Boothroyd, Andrew

    Neutron and X-ray Scattering Study of Magnetic Manganites Graeme Eoin Johnstone A Thesis submitted are performed using a variety of neutron scattering and x-ray scattering techniques. The electronic ground for analysing the results of the polarised neutron scattering experiment. There are a large number of people who

  13. Neutron scattering at high pressure D. B. McWhan

    E-Print Network [OSTI]

    Paris-Sud XI, Université de

    715 Neutron scattering at high pressure D. B. McWhan Room 1D-234, Murray Hill, New Jersey 07974, U scattering at steady-state and pulsed sources are reviewed. The pressure cells available at most neutron 10 GPa have been made. For elastic scattering, a comparison is made between neutron scattering and X

  14. AND/R: Advanced neutron diffractometer/reflectometer for investigation of thin films and multilayers for the life sciences

    E-Print Network [OSTI]

    2006-01-01

    Krueger et al. , in Neutron Scattering in Biology, edited by2006? An elastic neutron scattering instrument, the advancedadvantage offered by neutron scattering methods derives from

  15. Concepts of Neutron ScatteringConcepts of Neutron Scattering 66thth PSI Summer School on Condensed Matter ResearchPSI Summer School on Condensed Matter Research

    E-Print Network [OSTI]

    Boothroyd, Andrew

    Concepts of Neutron ScatteringConcepts of Neutron Scattering 66thth PSI Summer School on Condensed Andrew Boothroyd University of Oxford Basic features of neutron scattering Neutron diffraction Neutron on the lattice * * * #12;ScatteringScattering ``nuts and boltsnuts and bolts'' Neutrons, photons, electrons

  16. Cold neutron scattering in imperfect deuterium crystals

    E-Print Network [OSTI]

    Andrzej Adamczak

    2010-12-10

    The differential cross sections for cold neutron scattering in mosaic deuterium crystals have been calculated for various target temperatures. The theoretical results are compared with the recent experimental data for the neutron wavelengths $\\lambda\\approx$~1--9~\\AA. It is shown that the structures of observed Bragg peaks can be explained by the mosaic spread of about $3^{\\circ}$ and contributions from a~limited number of crystal orientations. Such a~crystal structure should be also taken into account in ultracold neutron upscattering due to the coherent phonon annihilation in solid deuterium.

  17. Attosecond neutron Compton scattering from protons

    E-Print Network [OSTI]

    C. Aris Chatzidimitriou-Dreismann

    2007-02-01

    The effect of "anomalous" scattering of neutrons and electrons from protons in the electron-volt energy-transfer range is considered, and related experimental results are mentioned. A recent independent confirmation of this effect with a new data analysis procedure is presented. Due to the very short characteristic scattering time, there is no well defined separation of time scales of electronic and protonic motions. An outline of a proposed theoretical interpretation is presented, which is based on the fact that scattering protons represent \\textit{open} quantum systems, thus being subject to decoherence.

  18. 2009 International Conference on Neutron Scattering (ICNS 2009)

    SciTech Connect (OSTI)

    Gopal Rao, PhD; Donna Gillespie

    2010-08-05

    The ICNS provides a focal point for the worldwide neutron user community to strengthen ties within this diverse group, while at the same time promoting neutron research among colleagues in related disciplines identified as �¢����would-be�¢��� neutron users. The International Conference on Neutron Scattering thus serves a dual role as an international user meeting and a scientific meeting. As a venue for scientific exchange, the ICNS showcases recent results and provides forums for scientific discussion of neutron research in diverse fields such as hard and soft condensed matter, liquids, biology, magnetism, engineering materials, chemical spectroscopy, crystal structure, and elementary excitations, fundamental physics and development of neutron instrumentation through a combination of invited talks, contributed talks and poster sessions. Each of the major national neutron facilities (NIST, LANSCE, ANL, HFIR and SNS), along with their international counterparts, has an opportunity to exchange information with each other and to update users, and potential users, of their facility. This is also an appropriate forum for users to raise issues that relate to the facilities.

  19. Neutrons for Catalysis: A Workshop on Neutron Scattering Techniques for Studies in Catalysis

    SciTech Connect (OSTI)

    Overbury, Steven {Steve} H; Coates, Leighton; Herwig, Kenneth W; Kidder, Michelle

    2011-10-01

    This report summarizes the Workshop on Neutron Scattering Techniques for Studies in Catalysis, held at the Spallation Neutron Source (SNS) at Oak Ridge National Laboratory (ORNL) on September 16 and 17, 2010. The goal of the Workshop was to bring experts in heterogeneous catalysis and biocatalysis together with neutron scattering experimenters to identify ways to attack new problems, especially Grand Challenge problems in catalysis, using neutron scattering. The Workshop locale was motivated by the neutron capabilities at ORNL, including the High Flux Isotope Reactor (HFIR) and the new and developing instrumentation at the SNS. Approximately 90 researchers met for 1 1/2 days with oral presentations and breakout sessions. Oral presentations were divided into five topical sessions aimed at a discussion of Grand Challenge problems in catalysis, dynamics studies, structure characterization, biocatalysis, and computational methods. Eleven internationally known invited experts spoke in these sessions. The Workshop was intended both to educate catalyst experts about the methods and possibilities of neutron methods and to educate the neutron community about the methods and scientific challenges in catalysis. Above all, it was intended to inspire new research ideas among the attendees. All attendees were asked to participate in one or more of three breakout sessions to share ideas and propose new experiments that could be performed using the ORNL neutron facilities. The Workshop was expected to lead to proposals for beam time at either the HFIR or the SNS; therefore, it was expected that each breakout session would identify a few experiments or proof-of-principle experiments and a leader who would pursue a proposal after the Workshop. Also, a refereed review article will be submitted to a prominent journal to present research and ideas illustrating the benefits and possibilities of neutron methods for catalysis research.

  20. Nitrogen Contamination in Elastic Neutron Scattering Songxue Chi,ab

    E-Print Network [OSTI]

    Lynn, Jeffrey W.

    Nitrogen Contamination in Elastic Neutron Scattering Songxue Chi,ab Jeffrey W. Lynn,a* Ying Chen a neutron scattering measurement is a contribution to the background, especially in inelastic measurements of having N2 in the sample environment system during elastic neutron scattering measurements on a single

  1. National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    15th National School on Neutron and X-ray Scattering August 10 - 24, 2013 at Argonne National of the National School on Neutron and X-ray Scattering is to educate graduate students on the utilization of major Ridge National Laboratory's Neutron Scattering Science Division. Scientific Directors: Jonathan C. Lang

  2. Thirteenth National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    Thirteenth National School on Neutron and X-ray Scattering June 11 ­ June 25, 2011 at Argonne of the National School on Neutron and X-ray Scattering is to educate graduate students on the utilization of major National Laboratory's Neutron Scattering Science Division. Scientific Directors: Jonathan C. Lang, Suzanne

  3. Neutron scattering in magnetic fields (*) W. C. Koehler

    E-Print Network [OSTI]

    Boyer, Edmond

    691 Neutron scattering in magnetic fields (*) W. C. Koehler Solid State Division, Oak Ridge. Abstract 2014 The use of magnetic fields in neutron scattering experimentation is reviewed briefly. Two of the scattering sample ; in the second the field acts on the neutron itself. Several examples are discussed

  4. Sixteenth National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    Pennycook, Steve

    Sixteenth National School on Neutron and X-ray Scattering June 14-28, 2014 at Argonne National of the National School on Neutron and X-ray Scattering is to educate graduate students on the utilization of major's Neutron Scattering Science Division. Scientific Directors: Suzanne G.E. te Velthuis, Esen Ercan Alp

  5. The Neutron Scattering Society www.neutronscattering.org

    E-Print Network [OSTI]

    Homes, Christopher C.

    The Neutron Scattering Society of America www.neutronscattering.org Press Release February 11, 2008 The Neutron Scattering Society of America is pleased to announce the election as Fellows of the Society of in application of neutron scattering to studies of surfaces and crystal field excitations as well as his

  6. National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    Pennycook, Steve

    National School on Neutron and X-ray Scattering May 30 ­ June 13, 2009 at Argonne National of the National School on Neutron and X-ray Scattering is to educate graduate students on the utilization of major National Laboratory's Neutron Scattering Science Division. Scientific Directors: Jonathan C. Lang, Suzanne

  7. Fourteenth National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    Pennycook, Steve

    Fourteenth National School on Neutron and X-ray Scattering August 12 - 25, 2012 at Argonne National of the National School on Neutron and X-ray Scattering is to educate graduate students on the utilization of major Ridge National Laboratory's Neutron Scattering Science Division. Scientific Directors: Jonathan C. Lang

  8. Neutron Scattering Society of America Purpose and New Initiatives

    E-Print Network [OSTI]

    1 Neutron Scattering Society of America (NSSA) Purpose and New Initiatives www.neutronscattering.org SNS/ANL School on Neutron and X-Ray Scattering June 2011 Visit us now on Facebook #12;2 What and provide a focal point for the neutron scattering community in the USA To identify the needs

  9. A Java-based Science Portal for Neutron Scattering Experiments

    E-Print Network [OSTI]

    Vazhkudai, Sudharshan

    A Java-based Science Portal for Neutron Scattering Experiments Sudharshan S. Vazhkudai James A scattering facility recently commissioned by the US Department of Energy (DOE). The neutron beam produced (SNS) [14] is a large-scale leading- edge neutron scattering facility that hopes to fundamen- tally

  10. TUTORIAL / ARTICLE DIDACTIQUE Neutron scattering study of the classical

    E-Print Network [OSTI]

    Ryan, Dominic

    TUTORIAL / ARTICLE DIDACTIQUE Neutron scattering study of the classical antiferromagnet MnF2: a perfect hands-on neutron scattering teaching course1 Z. Yamani, Z. Tun, and D.H. Ryan Abstract: We present of neutron scattering concepts. The nature of antiferromagnetism and the magnetic Hamiltonian in this classi

  11. ORNL Neutron Scattering School May 30 -June 5, 2009

    E-Print Network [OSTI]

    Pennycook, Steve

    ORNL Neutron Scattering School May 30 - June 5, 2009 Oak Ridge National Laboratory Oak Ridge, 2009, for the first week of the Neutron Xray Scattering School. Please be certain to bring photo for Neutron Scattering Users · Radiological Worker Training for HFIR and SNS Users In addition

  12. Twelfth National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    Pennycook, Steve

    Twelfth National School on Neutron and X-ray Scattering June 12 ­ June 26, 2010 at Argonne National of the National School on Neutron and X-ray Scattering is to educate graduate students on the utilization of major National Laboratory's Neutron Scattering Science Division. Scientific Directors: Jonathan C. Lang, Suzanne

  13. LANSCE School on Neutron Scattering: Materials at the Mesoscale

    E-Print Network [OSTI]

    1 11th LANSCE School on Neutron Scattering: Materials at the Mesoscale Lujan Center Los Alamos. Please name the applicant for admission to the 11th LANSCE School on Neutron Scattering: Last, First LANSCE School on Neutron Scattering including: drive and motivation, ability to work with others

  14. Tenth National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    Pennycook, Steve

    Tenth National School on Neutron and X-ray Scattering September 24 - October 11, 2008 at Argonne of the National School on Neutron and X-ray Scattering is to educate graduate students on the utilization of major National Laboratory's Neutron Scattering Science Division. Scientific Directors: Jonathan C. Lang, Suzanne

  15. Neutron Scattering Society of America Purpose and New Initiatives

    E-Print Network [OSTI]

    Pennycook, Steve

    1 Neutron Scattering Society of America (NSSA) Purpose and New Initiatives www.neutronscattering.org SNS/ANL School on Neutron and X-Ray Scattering June 2010 Visit us now on Facebook #12;2 What and provide a focal point for the neutron scattering community in the USA To identify the needs

  16. Dynamic neutron scattering on incoherent systems using efficient resonance spin flip techniques

    SciTech Connect (OSTI)

    Häussler, Wolfgang [Heinz Maier-Leibnitz Zentrum, Technische Universität München, D-85748 Garching, Germany and Physik-Department E21, Technische Universität München, D-85748 Garching (Germany); Kredler, Lukas [Physik-Department E21, Technische Universität München, D-85748 Garching (Germany)

    2014-05-15

    We have performed numerical ray-tracing Monte-Carlo-simulations of incoherent dynamic neutron scattering experiments. We intend to optimize the efficiency of incoherent measurements depending on the fraction of neutrons scattered without and with spin flip at the sample. In addition to conventional spin echo, we have numerically and experimentally studied oscillating intensity techniques. The results point out the advantages of these different spin echo variants and are an important prerequisite for neutron resonance spin echo instruments like RESEDA (FRM II, Munich), to choose the most efficient technique depending on the scattering vector range and the properties of the sample system under study.

  17. Current Status and Future Works of Neutron Scattering Laboratory at BATAN in Serpong

    SciTech Connect (OSTI)

    Ikram, A. [Center of Technology for Nuclear Industrial Materials, National Nuclear Energy Agency of Indonesia (BATAN) Kawasan Puspiptek Serpong, Tangerang 15314 (Indonesia)

    2008-03-17

    Current status of neutron beam instruments using neutrons produced by the Multi Purpose Research Reactor--30MWth (MPR 30, RSG GA Siwabessy) located in Serpong is presented. Description of the reactor as the neutron source is mentioned briefly. There are six neutron beam tubes coming from the beryllium reflector surrounding half of the reactor core providing neutrons in the experimental hall of the reactor (XHR). Four of them are dedicated to R and D in materials science using neutron scattering techniques. Neutron Radiography Facility (NRF), Triple Axis Spectrometer (TAS) and Residual Stress Measurement (RSM) Diffractometer are installed respectively at beam tubes S2, S4 and S6. The largest neutron beam tube (S5) is exploited to accommodate two neutron guide tubes that transfer the neutrons to a neighbouring building called neutron guide hall (NGH). There are three other neutron beam instruments installed in this building, namely Small Angle Neutron Scattering (SANS) Spectrometer (SMARTer), High Resolution SANS (HRSANS) Spectrometer and High Resolution Powder Diffractometer (HRPD). In the XHR, a Four Circle and Texture Diffractometer (FCD/TD) is attached to one of the neutron guide tubes. These seven instruments were installed to utilize the neutrons for materials science research, and recently the RSM diffractometer has shown its capabilities in identifying different amount of stress left due to different treatments of welding in fuel cladding, while the SANS spectrometer is now gaining capabilities in identifying different sizes and shapes of macromolecules in polymers as well as investigations of magnetic samples. In the mean time, non-destructive tests using the NRF is gathering more confidence from some latest real time measurements eventhough there are still some shortcomings in the components and their alignments. Future works including improvement of each facility and its components, even replacement of some parts are necessary and have to be carried out carefully. A plan for developing a neutron reflectometer at one of the neutron guide in the Neutron Guide Hall is also part of the near future activities.

  18. Total Cross Sections for Neutron Scattering

    E-Print Network [OSTI]

    C. R. Chinn; Ch. Elster; R. M. Thaler; S. P. Weppner

    1994-10-19

    Measurements of neutron total cross-sections are both extensive and extremely accurate. Although they place a strong constraint on theoretically constructed models, there are relatively few comparisons of predictions with experiment. The total cross-sections for neutron scattering from $^{16}$O and $^{40}$Ca are calculated as a function of energy from $50-700$~MeV laboratory energy with a microscopic first order optical potential derived within the framework of the Watson expansion. Although these results are already in qualitative agreement with the data, the inclusion of medium corrections to the propagator is essential to correctly predict the energy dependence given by the experiment.

  19. Neutron scattering and extra short range interactions

    E-Print Network [OSTI]

    V. V. Nesvizhevsky; G. Pignol; K. V. Protasov

    2007-11-14

    The available data on neutron scattering were analyzed to constrain a hypothetical new short-range interaction. We show that these constraints are several orders of magnitude better than those usually cited in the range between 1 pm and 5 nm. This distance range occupies an intermediate space between collider searches for strongly coupled heavy bosons and searches for new weak macroscopic forces. We emphasise the reliability of the neutron constraints in so far as they provide several independent strategies. We have identified the most promising way to improve them.

  20. Novel Boron-10-based detectors for Neutron Scattering Science

    E-Print Network [OSTI]

    Piscitelli, Francesco

    2015-01-01

    Nowadays neutron scattering science is increasing its instrumental power. Most of the neutron sources in the world are pushing the development of their technologies to be more performing. The neutron scattering development is also pushed by the European Spallation Source (ESS) in Sweden, a neutron facility which has just started construction. Concerning small area detectors (1m^2), the 3He technology, which is today cutting edge, is reaching fundamental limits in its development. Counting rate capability, spatial resolution and cost-e?ectiveness, are only a few examples of the features that must be improved to ful?fill the new requirements. On the other hand, 3He technology could still satisfy the detector requirements for large area applications (50m^2), however, because of the present 3He shortage that the world is experiencing, this is not practical anymore. The recent detector advances (the Multi-Grid and the Multi-Blade prototypes) developed in the framework of the collaboration between the Institut Laue...

  1. Timelike Compton scattering off the neutron

    E-Print Network [OSTI]

    Marie Boër; Michel Guidal; Marc Vanderhaeghen

    2015-10-10

    We study the exclusive photoproduction of an electron-positron pair on a neutron target in the Jefferson Lab energy domain. The reaction consists of two processes: the Bethe-Heitler and the Timelike Compton Scattering. The latter process provides potentially access to the Generalized Parton Distributions (GPDs) of the nucleon. We calculate all the unpolarized, single- and double-spin observables of the reaction and study their sensitivities to GPDs.

  2. Inelastic neutron scattering in valence fluctuation compounds

    SciTech Connect (OSTI)

    Jon M Lawrence

    2011-02-15

    The valence fluctuation compounds are rare earth intermetallics where hybridization of the nearly-localized 4f electrons with the conduction electrons leads to incorporation of the 4f's into the itinerant states. This hybridization slows down the conduction electrons and hence gives them a heavy effective mass, justifying application of the term 'heavy Fermion' (HF) to these materials. During the project period, we grew large single crystals of several such compounds and measured their properties using both standard thermodynamic probes and state-of-the-art inelastic neutron scattering. We obtained three main results. For the intermediate valence compounds CePd{sub 3} and YbAl{sub 3}, we showed that the scattering of neutrons by the fluctuations of the 4f magnetic moment does not have the momentum dependence expected for the itinerant heavy mass state; rather, the scattering is more typical of a localized spin fluctuation. We believe that incoherent scattering localizes the excitation. For the heavy Fermion compound Ce(Ni{sub 0.935}Pd{sub 0.065}){sub 2}Ge{sub 2}, which sits at a T = 0 critical point for transformation into an antiferromagnetic (AF) phase, we showed that the scattering from the AF fluctuations does not exhibit any of the divergences that are expected at a phase transition. We speculate that alloy disorder profoundly suppresses the growth of the fluctuating AF regions, leading to short range clusters rather than regions of infinite size. Finally, we explored the applicability of key concepts used to describe the behavior of rare earth heavy Fermions to uranium based HF compounds where the 5f electrons are itinerant as opposed to localized. We found that scaling laws relating the spin fluctuation energy measured in neutron scattering to the low temperature specific heat and susceptibility are valid for the uranium compounds, once corrections are made for AF fluctuations; however, the degeneracy of the high temperature moment is smaller than expected for rare-earth-like Hund's rule behavior, essentially because the orbital moment is suppressed for itinerant 5f electrons. We also found that the standard local-moment-based theory of the temperature dependence of the specific heat, susceptibility and neutron scattering fails badly for URu{sub 2}Zn{sub 20} and UCo{sub 2}Zn{sub 20}, even though the theory is phenomenally successful for the closely related rare earth compound YbFe{sub 2}Zn{sub 20}. Both these results highlight the distinction between the itineracy of the 5f's and the localization of the 4f's. It is our hope that these results are sufficiently significant as to stimulate deeper investigation of these compounds.

  3. ORNL study uses neutron scattering, supercomputing to demystify...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Morgan McCorkle Communications and Media Relations 865.574.7308 ORNL study uses neutron scattering, supercomputing to demystify forces at play in biofuel production This graphical...

  4. Deeply Virtual Compton Scattering off the neutron

    E-Print Network [OSTI]

    M. Mazouz; A. Camsonne; C. Muñoz Camacho; for the Jefferson Lab Hall A collaboration

    2007-12-12

    The present experiment exploits the interference between the Deeply Virtual Compton Scattering (DVCS) and the Bethe-Heitler processes to extract the imaginary part of DVCS amplitudes on the neutron and on the deuteron from the helicity-dependent D$({\\vec e},e'\\gamma)X$ cross section measured at $Q^2$=1.9 GeV$^2$ and $x_B$=0.36. We extract a linear combination of generalized parton distributions (GPDs) particularly sensitive to $E_q$, the least constrained GPD. A model dependent constraint on the contribution of the up and down quarks to the nucleon spin is deduced.

  5. Structure determination of micelle-like intermediates in amyloid ?-protein fibril assembly by using small angle neutron scattering

    E-Print Network [OSTI]

    2002-01-01

    by using small angle neutron scattering Winnie Yong †‡ ,technique of small angle neutron scattering has been used tois small angle neutron scattering (SANS). SANS experiments

  6. Enhanced reaction rates in NDP analysis with neutron scattering

    SciTech Connect (OSTI)

    Downing, R. Gregory

    2014-04-15

    Neutron depth profiling (NDP) makes accessible quantitative information on a few isotopic concentration profiles ranging from the surface into the sample a few micrometers. Because the candidate analytes for NDP are few, there is little interference encountered. Furthermore, neutrons have no charge so mixed chemical states in the sample are of no direct concern. There are a few nuclides that exhibit large probabilities for neutron scattering. The effect of neutron scattering on NDP measurements has not previously been evaluated as a basis for either enhancing the reaction rates or as a source of measurement error. Hydrogen is a common element exhibiting large neutron scattering probability found in or around sample volumes being analyzed by NDP. A systematic study was conducted to determine the degree of signal change when neutron scattering occurs during analysis. The relative signal perturbation was evaluated for materials of varied neutron scattering probability, concentration, total mass, and geometry. Signal enhancements up to 50% are observed when the hydrogen density is high and in close proximity to the region of analysis with neutron beams of sub thermal energies. Greater signal enhancements for the same neutron number density are reported for thermal neutron beams. Even adhesive tape used to position the sample produces a measureable signal enhancement. Because of the shallow volume, negligible distortion of the NDP measured profile shape is encountered from neutron scattering.

  7. X-ray and Neutron Scattering Studies of Magnetic Domain Dynamics and Spin Structures /

    E-Print Network [OSTI]

    Chen, San-Wen

    2014-01-01

    Stanley. X-ray and neutron scattering from rough surfaces.1988. [3] R. Pynn. Neutron scattering by rough surfaces at39] V. F. Sears. Neutron scattering lengths and cross

  8. Using Back-Scattering to Enhance Efficiency in Neutron Detectors

    E-Print Network [OSTI]

    Kittelmann, Thomas; Cai, Xiao Xiao; Kanaki, Kalliopi; Cooper-Jensen, Carsten P; Hall-Wilton, Richard

    2015-01-01

    The principle of using strongly scattering materials to recover efficiency in neutron detectors, via back-scattering of unconverted thermal neutrons, is discussed in general. Feasibility of the method is illustrated through Geant4-based simulations of a specific setup involving a moderator-like material placed behind a single layered boron-10 thin film gaseous detector.

  9. SANS -Small Angle Neutron Scattering Tcnica de difrao

    E-Print Network [OSTI]

    Loh, Watson

    SANS - Small Angle Neutron Scattering Técnica de difração informações sobre tamanho e forma de- Neutrons are created in the centre of the target station when the beam of high energy protons collides by evaporating nuclear particles, mainly neutrons, in all directions. Each proton produces approximately 15

  10. Investigating Neutron Polarizabilities through Compton Scattering on $^3He$

    E-Print Network [OSTI]

    Deepshikha Choudhury; Andreas Nogga; Daniel R. Phillips

    2007-06-11

    We examine manifestations of neutron electromagnetic polarizabilities in coherent Compton scattering from the Helium-3 nucleus. We calculate $\\gamma ^3He$ elastic scattering observables using chiral perturbation theory to next-to-leading order (${\\mathcal O}(e^2 Q)$). We find that the unpolarized differential cross section can be used to measure neutron electric and magnetic polarizabilities, while two double-polarization observables are sensitive to different linear combinations of the four neutron spin polarizabilities.

  11. Quantum Monte Carlo calculations of neutron-alpha scattering

    E-Print Network [OSTI]

    Kenneth M. Nollett; Steven C. Pieper; R. B. Wiringa; J. Carlson; G. M. Hale

    2006-12-09

    We describe a new method to treat low-energy scattering problems in few-nucleon systems, and we apply it to the five-body case of neutron-alpha scattering. The method allows precise calculations of low-lying resonances and their widths. We find that a good three-nucleon interaction is crucial to obtain an accurate description of neutron-alpha scattering.

  12. Liquid Argon Cryogenic Detector Calibration by Inelastic Scattering of Neutrons

    E-Print Network [OSTI]

    Sergey Polosatkin; Evgeny Grishnyaev; Alexander Dolgov

    2014-07-10

    A method for calibration of cryogenic liquid argon detector response to recoils with certain energy -8.2 keV - is proposed. The method utilizes a process of inelastic scattering of monoenergetic neutrons produced by fusion DD neutron generator. Features of kinematics of inelastic scattering cause sufficient (forty times) increase in count rate of useful events relative to traditional scheme exploited elastic scattering with the same recoil energy and compatible energy resolution. The benefits of the proposed scheme of calibration most well implemented with the use of tagged neutron generator as a neutron source that allows to eliminate background originated from casual coincidence of signals on cryogenic detector and additional detector of scattered neutrons.

  13. NEUTRONS AND 2 D ADSORBED PHASES. NEUTRON SCATTERING FROM 36ArAND 4HeFILMS

    E-Print Network [OSTI]

    Paris-Sud XI, Université de

    NEUTRONS AND 2 D ADSORBED PHASES. NEUTRON SCATTERING FROM 36ArAND 4HeFILMS K. CARNEIRO Physics. - The technique of neutron scattering is well established as a unique tool to investigate the details technique to physisorbed phases is quite natural. But on the other hand since neutron scattering, compared

  14. Neutron scattering studies in the actinide region. Progress report, August 1, 1992--July 31, 1993

    SciTech Connect (OSTI)

    Kegel, G.H.R.; Egan, J.J.

    1993-09-01

    This report discusses the following topics: Prompt fission neutron energy spectra for {sup 235}U and {sup 239}Pu; Two-parameter measurement of nuclear lifetimes; ``Black`` neutron detector; Data reduction techniques for neutron scattering experiments; Inelastic neutron scattering studies in {sup 197}Au; Elastic and inelastic scattering studies in {sup 239}Pu; and neutron induced defects in silicon dioxide MOS structures.

  15. The Extended Q-Range Small Angle Neutron Scattering Diffractometer at the SNS

    SciTech Connect (OSTI)

    Zhao, Jinkui [ORNL; Gao, Carrie Y [ORNL; Liu, Dazhi [ORNL

    2010-01-01

    The Extended Q-Range Small Angle Neutron Scattering Diffractometer (EQ-SANS) at the Spallation Neutron Source is designed to have wide neutron momentum transfer (Q) coverage, high neutron beam intensity, and good wavelength resolution. In addition, the design and construction of the instrument aim at achieving maximum signal to noise ratio by minimizing the background. The instrument is located on the 60Hz SNS target. It has a primary flight path of 14m. Its secondary flight path varies from ~1m to 10m. One of the key components in the primary flight path is the neutron optics, consisting of a true-curved multi channel beam bender and sections of neutron guides. The optics is optimized to reduce the neutron transport loss to a minimum, thereby maximizing the available flux on sample. It also enables the avoidance of the direct line of sight of the neutron moderator at downstream locations. The instrument has three bandwidth-limiting choppers. These choppers effectively eliminate higher frame neutrons up to ~38 from the beam. A frame overlap mirror further cleans up the beam by reflecting out neutrons whose wavelengths are longer than ~33 . The bandwidth choppers also allow a frame-skipping mode of operation, which enables the EQ-SANS diffractometer to achieve a dynamic Q-range equivalent to that of a similar machine on a 20Hz source. The two-dimensional low-angle detector, based on 3He tube technologies, offers very high counting rates and counting efficiency. Initial operations have shown that the instrument has achieved its best-in-class design requirement.

  16. LANSCE | Lujan Center | Instruments | Neutron Radiography

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantity ofkandz-cm11 Outreach Home Room NewsInformationJesse Bergkamp Graduate student Subtask2 J.N.openNeutron Radiography The

  17. Dynamic Properties of Materials: Phonons from Neutron Scattering

    E-Print Network [OSTI]

    Cope, Elizabeth Ruth

    2010-01-01

    A detailed understanding of fundamental material properties can be obtained through the study of atomic vibrations, performed experimentally with neutron scattering techniques and coupled with the two powerful new computational methodologies I have...

  18. Neutron-Scattering Evidence for a Periodically Modulated Superconducti...

    Office of Scientific and Technical Information (OSTI)

    Neutron-Scattering Evidence for a Periodically Modulated Superconducting Phase in the Underdoped Cuprate La1.905Ba0.095CuO4 Citation Details In-Document Search Title:...

  19. Can one extract the pi-neutron scattering length from pi-deuteron scattering?

    E-Print Network [OSTI]

    A. Nogga; C. Hanhart

    2005-11-02

    We give a prove of evidence that the original power counting by Weinberg can be applied to estimate the contributions of the operators contributing to the pi-deuteron scattering length. As a consequence, pi-deuteron observables can be used to extract neutron amplitudes--in case of pi-deuteron scattering this means that the pi-neutron scattering length can be extracted with high accuracy. This result is at variance with recent claims. We discuss the origin of this difference.

  20. Entangling neutrons via successive scattering from a substrate

    E-Print Network [OSTI]

    M. Avellino; S. Bose; A. J. Fisher

    2008-08-18

    This letter details a simple scheme to entangle two neutrons by successive scattering from a macroscopic sample. In zero magnetic field the entanglement falls as the sample size increases. However, by applying a field and tuning the momentum of the neutrons, one can achieve a substantial degree of entanglement irrespective of the size of the sample.

  1. Neutron-deuteron elastic scattering and three-nucleon force

    E-Print Network [OSTI]

    Chtangeev, Maxim B

    2005-01-01

    The differential cross section for neutron-deuteron elastic scattering was measured at six angles over the center-of-mass angular range 65? - 1300? and incident neutron energies 140 - 240 MeV at the LANSCE/WNR facility of ...

  2. Elastic Neutron Scattering at 96 MeV

    SciTech Connect (OSTI)

    Hildebrand, A.; Blomgren, J.; Atac, A.; Bergenwall, B.; Johansson, C.; Klug, J.; Mermod, P.; Nilsson, L.; Pomp, S.; Esterlund, M.; Dangtip, S.; Tippawan, U.; Phansuke, P.; Jonsson, O.; Renberg, P.-U.; Prokofiev, A.; Nadel-Turonski, P.; Elmgren, K.; Olsson, N.; Blideanu, V.

    2005-05-24

    A facility for detection of scattered neutrons in the energy interval 50-130 MeV, SCANDAL (SCAttered Nucleon Detection AssembLy), has recently been installed at the 20 - 180-MeV neutron beam line of The Svedberg Laboratory, Uppsala. Elastic neutron scattering from 12C, 16O, 56Fe, 89Y, and 208Pb has been studied at 96 MeV in the 10-70 deg. interval. The results from 12C and 208Pb have recently been published,6 while the data from 16O, 56Fe, and 89Y are under analysis. The achieved energy resolution, 3.7 MeV, is about an order of magnitude better than for any previous experiment above 65 MeV incident energy. The present experiment represents the highest neutron energy where the ground state has been resolved from the first excited state in neutron scattering. A novel method for normalization of the absolute scale of the cross section has been used. The estimated normalization uncertainty, 3%, is unprecedented for a neutron-induced differential cross section measurement on a nuclear target. The results are compared with modern optical model predictions, based on phenomenology or microscopic theory. Applications for these measurements are nuclear-waste incineration, single-event upsets in electronics, and fast-neutron therapy.

  3. Realization of adiabatic Aharonov-Bohm scattering with neutrons

    E-Print Network [OSTI]

    Erik Sjöqvist; Martin Almquist; Ken Mattsson; Zeynep Nilhan Gürkan; Björn Hessmo

    2015-03-08

    The adiabatic Aharonov-Bohm (AB) effect is a manifestation of the Berry phase acquired when some slow variables take a planar spin around a loop. While the effect has been observed in molecular spectroscopy, direct measurement of the topological phase shift in a scattering experiment has been elusive in the past. Here, we demonstrate an adiabatic AB effect for neutrons that scatter on a long straight current-carrying wire. We propose an experiment to verify the effect and demonstrate its feasibility by explicit simulation of the dynamics of unpolarized very slow neutrons that scatter on the wire under realistic conditions.

  4. Neutron cross section standards and instrumentation. Annual report

    SciTech Connect (OSTI)

    Wasson, O.A.

    1993-07-01

    The objective of this interagency program is to provide accurate neutron interaction measurements for the US Department of Energy nuclear programs which include waste disposal, fusion, safeguards, defense, fission, and personnel protection. These measurements are also useful to other energy programs which indirectly use the unique properties of the neutron for diagnostic and analytical purposes. The work includes the measurement of reference cross sections and related neutron data employing unique facilities and capabilities at NIST and other laboratories as required; leadership and participation in international intercomparisons and collaborations; the preservation of standard reference deposits and the development of improved neutron detectors and measurement methods. A related and essential element of the program is critical evaluation of neutron interaction data including international coordinations. Data testing of critical data for important applications is included. The program is jointly supported by the Department of Energy and the National Institute of Standards and Technology. This report from the National Institute of Standards and Technology contains a summary of the accomplishments of the Neutron Cross Section Standards and Instrumentation Project during the third year of this three-year interagency agreement. The proposed program and required budget for the following three years are also presented. The program continues the shifts in priority instituted in order to broaden the program base.

  5. Test of the consistency of various linearized semiclassical initial value time correlation functions in application to inelastic neutron scattering from liquid para-hydrogen

    E-Print Network [OSTI]

    Liu, Jian

    2008-01-01

    Theory of Thermal Neutron Scattering. (Dover Publications,S. W. Lovesey, Theory of Neutron Scattering from Condensedwith the inelastic neutron scattering experiment results.

  6. MAGNETIC NEUTRON SCATTERING. And Recent Developments in the Triple Axis Spectroscopy

    E-Print Network [OSTI]

    Johnson, Peter D.

    Chapter 1 MAGNETIC NEUTRON SCATTERING. And Recent Developments in the Triple Axis Spectroscopy Igor.................................................................................... 2 2. Neutron interaction with matter and scattering cross-section ........ 6 2.1 Basic scattering theory and differential cross-section................ 7 2.2 Neutron interactions and scattering lengths

  7. Small-Angle Neutron Scattering Studies of Charged Carboxyl-Terminated Dendrimers in Solutions

    E-Print Network [OSTI]

    Dubin, Paul D.

    Small-Angle Neutron Scattering Studies of Charged Carboxyl-Terminated Dendrimers in Solutions Q. R-angle neutron scattering was used to characterize the solution behavior of charged carboxylic acid terminated- copy,16 small-angle X-ray scattering,17 and small-angle neutron scattering (SANS),18-25 have been used

  8. Neutron and X-ray Scattering Studies of Strongly Correlated Electron Systems

    E-Print Network [OSTI]

    Boothroyd, Andrew

    Neutron and X-ray Scattering Studies of Strongly Correlated Electron Systems Russell A. Ewings 2008 #12;Abstract Neutron and X-ray Scattering Studies of Strongly Correlated Electron Systems Russell-ray scattering and neutron scattering experiments on several strongly correlated transition metal oxides

  9. hal-00154048,version1-12Jun2007 The new very small angle neutron scattering

    E-Print Network [OSTI]

    Boyer, Edmond

    hal-00154048,version1-12Jun2007 The new very small angle neutron scattering spectrometer The design and characteristics of the new very small angle neutron scattering spectrometer under construction in order to fill the gap between light scattering and classical small angle neutron scattering (SANS

  10. The Algebraic Approach to the Phase Problem for Neutron Scattering

    E-Print Network [OSTI]

    A. Cervellino; S. Ciccariello

    2004-01-27

    The algebraic approach to the phase problem for the case of X-ray scattering from an ideal crystal is extended to the case of the neutron scattering, overcoming the difficulty related to the non-positivity of the scattering density. In this way, it is proven that the atomicity is the crucial assumption while the positiveness of the scattering density only affects the method for searching the basic sets of reflections. We also report the algebraic expression of the determinants of the Karle-Hauptman matrices generated by the basic sets with the most elongated shape along one of the reciprocal crystallographic axes.

  11. Constraints on new interactions from neutron scattering experiments

    E-Print Network [OSTI]

    Yu. N. Pokotilovski

    2006-01-19

    Constraints for the constants of hypothetical Yukawa-type corrections to the Newtonian gravitational potential are obtained from analysis of neutron scattering experiments. Restrictions are obtained for the interaction range between 10^{-12} and 10^{-7} cm, where Casimir force experiments and atomic force microscopy are not sensitive. Experimental limits are obtained also for non-electromagnetic inverse power law neutron-nucleus potential. Some possibilities are discussed to strengthen these constraints.

  12. A small angle neutron scattering (SANS) experiment using very cold neutrons (VCN).

    SciTech Connect (OSTI)

    Bleuel, M.; Carpenter, J. M.; Micklich, B. J.; Geltenbort, P.; Mishima, K.; Shimizu, H. M.; Iwashita, Y.; Hirota, K.; Hino, M.; Kennedy, S. J.; Lal, J.; Inst. Laue Langevin; Neutron Science Lab.; Kyoto Univ.; Riken; Bragg Inst.

    2009-01-01

    This paper describes the results of SANS measurements of small samples using the very cold neutron (VCN) beam of the PF2 instrument at the Institut Laue Langevin (ILL), France. In addition to a classical SANS pinhole collimation, the experiment used a polarizing supermirror as a monochromator and a magnetic sextupole lens to focus the neutron beam in order to gain intensity and avoid any material in the neutron beam besides the sample.

  13. Improved di-neutron cluster model for 6He scattering

    E-Print Network [OSTI]

    A. M. Moro; K. Rusek; J. M. Arias; J. Gomez-Camacho; M. Rodriguez-Gallardo

    2007-03-01

    The structure of the three-body Borromean nucleus 6He is approximated by a two-body di-neutron cluster model. The binding energy of the 2n-\\alpha system is determined to obtain a correct description of the 2n-\\alpha coordinate, as given by a realistic three-body model calculation. The model is applied to describe the break-up effects in elastic scattering of 6He on several targets, for which experimental data exist. We show that an adequate description of the di-neutron-core degree of freedom permits a fairly accurate description of the elastic scattering of 6He on different targets.

  14. Event-Based Processing of Neutron Scattering Data

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Peterson, Peter F.; Campbell, Stuart I.; Reuter, Michael A.; Taylor, Russell J.; Zikovsky, Janik L.

    2015-09-16

    Many of the world's time-of-flight spallation neutrons sources are migrating to the recording of individual neutron events. This provides for new opportunities in data processing, the least of which is to filter the events based on correlating them with logs of sample environment and other ancillary equipment. This paper will describe techniques for processing neutron scattering data acquired in event mode that preserve event information all the way to a final spectrum, including any necessary corrections or normalizations. This results in smaller final errors, while significantly reducing processing time and memory requirements in typical experiments. Results with traditional histogramming techniquesmore »will be shown for comparison.« less

  15. Neutron scattering of CeNi at the SNS-ORNL: A preliminary report

    SciTech Connect (OSTI)

    Mirmelstein, A. [Russian Federal Nuclear Center VNIITF, Snezhinsk, Russia; Podlesnyak, Andrey A [ORNL; Kolesnikov, Alexander I [ORNL; Saporov, B. [Oak Ridge National Laboratory (ORNL); Sefat, A.S. [Oak Ridge National Laboratory (ORNL); Tobin, J. G. [Lawrence Livermore National Laboratory (LLNL)

    2014-01-01

    This is a preliminary report of a neutron scattering experiment used to investigate 4f electron behavior in Ce.

  16. Time Reversal Invariance Violation in Neutron Deuteron Scattering

    E-Print Network [OSTI]

    Young-Ho Song; Rimantas Lazauskas; Vladimir Gudkov

    2011-04-15

    Time reversal invariance violating (TRIV) effects for low energy elastic neutron deuteron scattering are calculated for meson exchange and EFT-type of TRIV potentials in a Distorted Wave Born Approximation, using realistic hadronic strong interaction wave functions, obtained by solving three-body Faddeev equations in configuration space. The relation between TRIV and parity violating observables are discussed.

  17. SPIN-DEPENDENT SCATTERING LENGTHS OF SLOW NEUTRONS WITH NUCLEI BY PSEUDOMAGNETIC MEASUREMENTS

    E-Print Network [OSTI]

    Boyer, Edmond

    L-263 SPIN-DEPENDENT SCATTERING LENGTHS OF SLOW NEUTRONS WITH NUCLEI BY PSEUDOMAGNETIC MEASUREMENTS vu par les noyaux. Abstract. - The spin-dependent scattering length of slow neutrons by the nuclei 23 can be of practical importance in many thermal neutron scattering experiments. A new method, called

  18. Spin-dependent scattering and absorption of thermal neutrons on dynamically polarized nuclei

    E-Print Network [OSTI]

    Paris-Sud XI, Université de

    957 Spin-dependent scattering and absorption of thermal neutrons on dynamically polarized nuclei H neutrons and polarized nuclei have been used to measure spin-dependent scattering lengths and absorption cross sections of slow (S-wave) neutrons on nuclei. In order to obtain those scattering lengths

  19. Molecular-dynamics study of incoherent quasielastic neutron-scattering spectra of supercooled water

    E-Print Network [OSTI]

    Sciortino, Francesco

    Molecular-dynamics study of incoherent quasielastic neutron-scattering spectra of supercooled water neutron-scattering experiments. Second, we explore the possibility of an alterna- tive method of analysis of high-resolution quasielastic neutron-scattering spectra, taking into account the slow dynamics

  20. Dynamics of Different Hydrogen Classes in -lactoglobulin: A Quasielastic Neutron Scattering Investigation

    E-Print Network [OSTI]

    Tuscia, Università Degli Studi Della

    Dynamics of Different Hydrogen Classes in -lactoglobulin: A Quasielastic Neutron Scattering investigated by means of quasielastic neutron scattering. To discriminate the possibly different dynamical- thods,11-13 molecular dynamics (MD) simulations,14 X-ray crys- tallography,15 and neutron scattering.6

  1. neutron scattering shows magnetic excitation mechanism at work in new materials.

    E-Print Network [OSTI]

    neutron scattering shows magnetic excitation mechanism at work in new materials. In 2008 dai of orNl and the university of tennes- see led early neutron scattering studies of the pnictides. dai ticks off four main things neutron scattering has revealed about superconducting iron com- pounds

  2. THE JOURNAL OF CHEMICAL PHYSICS 139, 175101 (2013) Dynamic neutron scattering from conformational dynamics. I. Theory

    E-Print Network [OSTI]

    2013-01-01

    #12;THE JOURNAL OF CHEMICAL PHYSICS 139, 175101 (2013) Dynamic neutron scattering from, a conformational dynamics theory of dynamical neutron and X-ray scattering is developed, follow- ing our previous spectroscopy (dynamic neutron scattering) probes time correlations on the sub pico- to microsec- ond timescales

  3. Effective Long-Range Attraction between Protein Molecules in Solutions Studied by Small Angle Neutron Scattering

    E-Print Network [OSTI]

    Chen, Sow-Hsin

    Neutron Scattering Yun Liu,1 Emiliano Fratini,2 Piero Baglioni,1,2 Wei-Ren Chen,1 and Sow-Hsin Chen1,* 1, Italy (Received 8 February 2005; published 8 September 2005) Small angle neutron scattering intensity neutron and x-ray scattering investigations of proteins suggest the presence of a short-range attractive

  4. Large Area Imaging Detector for Neutron Scattering Based on Boron-Rich Liquid Scintillator

    E-Print Network [OSTI]

    Large Area Imaging Detector for Neutron Scattering Based on Boron-Rich Liquid Scintillator D detector, neutron scattering, gaseous photomultiplier Pacs: 29.40.Mc, 29.40.Cs, 61.12.-q, 61.12.Ex to Nucl. Instr. & Meth. A WIS/31/02-July-DPP #12;1. Introduction Slow neutron scattering is one of the key

  5. PHYSICAL REVIEW B VOLUME 25, NUMBER 7 Neutron scattering from paramagnetic bcc 'He

    E-Print Network [OSTI]

    Glyde, Henry R.

    PHYSICAL REVIEW B VOLUME 25, NUMBER 7 Neutron scattering from paramagnetic bcc 'He 1 APRIL 1982 H is calculated using the self-consistent-phonon (SCP) theory for comparison with proposed neutron scattering excitations or critical scattering will be observable only at very small neutron energy transfers (-0.1 pev

  6. Neutron scattering evidence of a boson peak in protein hydration water Alessandro Paciaroni,1

    E-Print Network [OSTI]

    Tuscia, Università Degli Studi Della

    Neutron scattering evidence of a boson peak in protein hydration water Alessandro Paciaroni,1 Anna Viterbo, Italy Received 24 February 1999 Measurement of the low temperature neutron excess of scattering, has been detected by neutron scattering and Raman spectros- copy in a large variety of glassy systems

  7. Incompatibility of modulated checkerboard patterns with the neutron scattering resonance peak in cuprate superconductors

    E-Print Network [OSTI]

    Carlson, Erica

    Incompatibility of modulated checkerboard patterns with the neutron scattering resonance peak rotated 45° from the direction of the charge IC peaks, contrary to what is seen in neutron scattering energy response is inconsistent with neutron scattering results. In particular, the modulated

  8. THE JOURNAL OF CHEMICAL PHYSICS 139, 175102 (2013) Dynamic neutron scattering from conformational dynamics. II. Application

    E-Print Network [OSTI]

    2013-01-01

    #12;THE JOURNAL OF CHEMICAL PHYSICS 139, 175102 (2013) Dynamic neutron scattering from; accepted 12 September 2013; published online 1 November 2013) Neutron scattering experiments directly probe.1063/1.4824071] I. INTRODUCTION Dynamic neutron scattering is a direct probe of the inter- nal, conformational

  9. ELSEVIER Physica B 213&214 11995J454 458 Neutron scattering from liquid 3He

    E-Print Network [OSTI]

    Glyde, Henry R.

    ELSEVIER Physica B 213&214 11995J454 458 HIYSICA[ Neutron scattering from liquid 3He at large Abstract Neutron inelastic scattering measurements have been made on liquid 3He at 1,4 K for wave vectors to investigate the neutron inelastic scattering from liquid 3He at T = 1.4 K for wave vec- tors between 9 and 20

  10. Naysaying the Neutron Scattering Society Lawrence Cranberg, Jill Trewhella, and Henry R. Glyde

    E-Print Network [OSTI]

    Glyde, Henry R.

    Naysaying the Neutron Scattering Society Lawrence Cranberg, Jill Trewhella, and Henry R. Glyde, Austin Naysaying the Neutron Scattering Society The news story announcing the estab- lishment of the Neutron Scattering Society of America (June, page 73) raises a number of questions, and further

  11. The Neutron Scattering Society of America http:///www.neutronscattering.org

    E-Print Network [OSTI]

    The Neutron Scattering Society of America http:///www.neutronscattering.org Page 8 of 9 Dr. Claire of the Neutron Scattering Society of America (NSSA) with the citation "For pioneering a new methodology and computational chemistry" The Neutron Scattering Society of America (NSSA) established the Prize for Outstanding

  12. National School on Neutron and X-ray Scattering August 10-24, 2013

    E-Print Network [OSTI]

    Kemner, Ken

    National School on Neutron and X-ray Scattering August 10-24, 2013 Argonne National Laboratory National Laboratory 3:15 ­ 3:30 Break #12;National School on Neutron and X-ray Scattering August 10 Dinner Week 1 wrap-up Picnic #12;National School on Neutron and X-ray Scattering August 10-24, 2012 Oak

  13. Small angle neutron scattering on periodically deformed polymers A. R. Rennie

    E-Print Network [OSTI]

    Boyer, Edmond

    765 Small angle neutron scattering on periodically deformed polymers A. R. Rennie Institut für Phys-768 SEPTEMBRE 1984, 1. Introduction. Neutron scattering has proved a useful tool for the investigation of a wide time for a small angle neutron scattering spectrum is several minutes. Obser- vation on rapidly

  14. A comparison of neutron scattering studies and computer simulations of polymer melts

    E-Print Network [OSTI]

    Utah, University of

    A comparison of neutron scattering studies and computer simulations of polymer melts G.D. Smith a; in ®nal form 22 May 2000 Abstract Neutron scattering and computer simulations are powerful tools in particular. When neutron scattering studies and quan- titative atomistic molecular dynamics simulations

  15. High temperature furnaces for small and large angle neutron scattering of disordered materials

    E-Print Network [OSTI]

    Boyer, Edmond

    725 High temperature furnaces for small and large angle neutron scattering of disordered materials and small angle neutron scattering (SANS) experiments respectively. They are vacuum furnaces with a thin maintained in a tantalum box. In a neutron beam, the furnaces produce a very low scattering level (without

  16. Micellar structure from comparison of X-ray and neutron small-angle scattering

    E-Print Network [OSTI]

    Boyer, Edmond

    249 Micellar structure from comparison of X-ray and neutron small-angle scattering T. Zemb and P according to the method developed by Hayter and Penfold. Both X-ray and neutron scattering signals, or by a combination of both. It has been shown recent- ly [1, 2] that it is possible in neutron scattering studies

  17. 2015 LaCNS Neutron Scattering Seed Funding Request for White Papers

    E-Print Network [OSTI]

    pg. 1 2015 LaCNS Neutron Scattering Seed Funding Request for White Papers DEADLINE: January 12, 2015 The Louisiana Consortium for Neutron Scattering (LaCNS), a Department of Energy ­ EPSCo projects involving neutron scattering. These projects can be in any area of Materials Science

  18. Ris-PhD-7(EN) Neutron scattering studies of two-

    E-Print Network [OSTI]

    Risø-PhD-7(EN) Neutron scattering studies of two- dimensional antiferromagnetic spin fluctuations Denmark January 2005 #12;Neutron scattering studies of two-dimensional antiferromagnetic spin fluctuations Laboratory 4000 Roskilde, Denmark #12;#12;Abstract: In this thesis, neutron scattering techniques are used

  19. TTOTT Ris0-R-986(EN) A Neutron Scattering Study of Triblock

    E-Print Network [OSTI]

    TTOTT Ris0-R-986(EN) DK9800004 A Neutron Scattering Study of Triblock Copolymer Micelles Michael C. Gerstenberg Ris0 National Laboratory, Roskilde, Denmark November 1997 #12;Ris0-R-986(EN) A Neutron Scattering, Denmark November 1997 #12;Abstract The thesis describes the neutron scattering experiments performed

  20. INELASTIC NEUTRON SCATTERING SELECTION RULES OF 03B1 HgI2 M. SIESKIND

    E-Print Network [OSTI]

    Boyer, Edmond

    899 INELASTIC NEUTRON SCATTERING SELECTION RULES OF 03B1 HgI2 M. SIESKIND Laboratoire de The inelastic neutron scattering selection rules of 03B1 HgI2 in the directions 0394, 03A3 and 039B are derived Abstracts 63.20D Introduction. - Inelastic neutron scattering is a powerful technique for the determination

  1. Neutron scattering effects on fusion ion temperature measurements.

    SciTech Connect (OSTI)

    Ziegler, Lee (Bechtel/Nevada, Las Vegas, NV); Starner, Jason R.; Cooper, Gary Wayne; Ruiz, Carlos L.; Franklin, James Kenneth (Ktech Corporation, Albuquerque, NM); Casey, Daniel T.

    2006-06-01

    To support the nuclear fusion program at Sandia National Laboratories (SNL), a consistent and verifiable method to determine fusion ion temperatures needs to be developed. Since the fusion temperature directly affects the width in the spread of neutron energies produced, a measurement of the neutron energy width can yield the fusion temperature. Traditionally, the spread in neutron energies is measured by using time-of-flight to convert a spread in neutron energies at the source to a spread in time at detector. One potential obstacle to using this technique at the Z facility at SNL is the need to shield the neutron detectors from the intense bremsstrahlung produced. The shielding consists of eight inches of lead and the concern is that neutrons will scatter in the lead, artificially broaden the neutron pulse width and lead to an erroneous measurement. To address this issue, experiments were performed at the University of Rochester's Laboratory for Laser Energetics, which demonstrated that a reliable ion temperature measurement can be achieved behind eight inches of lead shielding. To further expand upon this finding, Monte Carlo N-Particle eXtended (MCNPX) was used to simulate the experimental geometric conditions and perform the neutron transport. MCNPX was able to confidently estimate results observed at the University of Rochester.

  2. Anisotropic Elastic Resonance Scattering model for the Neutron Transport equation

    SciTech Connect (OSTI)

    Mohamed Ouisloumen; Abderrafi M. Ougouag; Shadi Z. Ghrayeb

    2014-11-24

    The resonance scattering transfer cross-section has been reformulated to account for anisotropic scattering in the center-of-mass of the neutron-nucleus system. The main innovation over previous implementations is the relaxation of the ubiquitous assumption of isotropic scattering in the center-of-mass and the actual effective use of scattering angle distributions from evaluated nuclear data files in the computation of the angular moments of the resonant scattering kernels. The formulas for the high order anisotropic moments in the laboratory system are also derived. A multi-group numerical formulation is derived and implemented into a module incorporated within the NJOY nuclear data processing code. An ultra-fine energy mesh cross section library was generated using these new theoretical models and then was used for fuel assembly calculations with the PARAGON lattice physics code. The results obtained indicate a strong effect of this new model on reactivity, multi-group fluxes and isotopic inventory during depletion.

  3. Solutions for implementing time-of-flight techniques in low-angle neutron scattering, as realized on the Low-Q Diffractometer at Los Alamos

    SciTech Connect (OSTI)

    Hjelm, R.P. Jr.; Seeger, P.A.

    1992-12-01

    The implementation of small-angle (Low-momentum transfer) neutron scattering at pulsed spallation sources, using time of flight methods, has meant the introduction of some new ideas in instrument design, data acquisition, data reduction and computer management of the experiment and the data. Here we recount some of the salient aspects of solutions for implementing time of fight small-angle neutron scattering instruments at pulsed sources, as realized on the Low-Q Diffractometer, LQD, at Los Alamos. We consider, fortlier, some of the problems that are yet to be solved, and take a short excursion into the future of SANS instrumentation at pulsed sources.

  4. Small angle neutron scattering in materials science: Recent practical applications

    SciTech Connect (OSTI)

    Melnichenko, Yuri B [ORNL; Wignall, George D [ORNL

    2007-01-01

    Modern materials science and engineering relies increasingly on detailed knowledge of the structure and interactions in 'soft' and 'hard' materials, but there have been surprisingly few microscopic techniques for probing the structures of bulk samples of these substances. Small-angle neutron scattering (SANS) was first recognized in Europe as a major technique for this purpose and, over the past several decades, has been a growth area in both academic and industrial materials research to provide structural information on length scales {approx}10-1000 Angstroms (or 1-100 nm). The technique of ultrahigh resolution small-angle neutron scattering (USANS) raises the upper resolution limit for structural studies by more than two orders of magnitude and (up to {approx}30 {micro}m) and hence overlaps with light scattering and microscopy. This review illustrates the ongoing vitality of SANS and USANS in materials research via a range of current practical applications from both soft and hard matter nanostructured systems.

  5. Instrument performance study on the short and long pulse options of the second Spallation Neutron Source target station

    SciTech Connect (OSTI)

    Zhao, J. K.; Herwig, Kenneth W.; Robertson, J. L.; Gallmeier, Franz X.; Riemer, Bernard W.

    2013-10-15

    The Spallation Neutron Source (SNS) facility at the Oak Ridge National Laboratory is designed with an upgrade option for a future low repetition rate, long wavelength second target station. This second target station is intended to complement the scientific capabilities of the 1.4 MW, 60 Hz high power first target station. Two upgrade possibilities have been considered, the short and the long pulse options. In the short pulse mode, proton extraction occurs after the pulse compression in the accumulator ring. The proton pulse structure is thus the same as that for the first target station with a pulse width of ?0.7 ?s. In the long pulse mode, protons are extracted as they are produced by the linac, with no compression in the accumulator ring. The time width of the uncompressed proton pulse is ?1 ms. This difference in proton pulse structure means that neutron pulses will also be different. Neutron scattering instruments thus have to be designed and optimized very differently for these two source options which will directly impact the overall scientific capabilities of the SNS facility. In order to assess the merits of the short and long pulse target stations, we investigated a representative suit of neutron scattering instruments and evaluated their performance under each option. Our results indicate that the short pulse option will offer significantly better performance for the instruments and is the preferred choice for the SNS facility.

  6. Complete Monte Carlo Simulation of Neutron Scattering Experiments

    SciTech Connect (OSTI)

    Drosg, M.

    2011-12-13

    In the far past, it was not possible to accurately correct for the finite geometry and the finite sample size of a neutron scattering set-up. The limited calculation power of the ancient computers as well as the lack of powerful Monte Carlo codes and the limitation in the data base available then prevented a complete simulation of the actual experiment. Using e.g. the Monte Carlo neutron transport code MCNPX [1], neutron scattering experiments can be simulated almost completely with a high degree of precision using a modern PC, which has a computing power that is ten thousand times that of a super computer of the early 1970s. Thus, (better) corrections can also be obtained easily for previous published data provided that these experiments are sufficiently well documented. Better knowledge of reference data (e.g. atomic mass, relativistic correction, and monitor cross sections) further contributes to data improvement. Elastic neutron scattering experiments from liquid samples of the helium isotopes performed around 1970 at LANL happen to be very well documented. Considering that the cryogenic targets are expensive and complicated, it is certainly worthwhile to improve these data by correcting them using this comparatively straightforward method. As two thirds of all differential scattering cross section data of {sup 3}He(n,n){sup 3}He are connected to the LANL data, it became necessary to correct the dependent data measured in Karlsruhe, Germany, as well. A thorough simulation of both the LANL experiments and the Karlsruhe experiment is presented, starting from the neutron production, followed by the interaction in the air, the interaction with the cryostat structure, and finally the scattering medium itself. In addition, scattering from the hydrogen reference sample was simulated. For the LANL data, the multiple scattering corrections are smaller by a factor of five at least, making this work relevant. Even more important are the corrections to the Karlsruhe data due to the inclusion of the missing outgoing self-attenuation that amounts to up to 15%.

  7. Resonant Cyclotron Scattering and Comptonization in Neutron Star Magnetospheres

    E-Print Network [OSTI]

    Maxim Lyutikov; Fotis P. Gavriil

    2006-02-10

    Resonant cyclotron scattering of the surface radiation in the magnetospheres of neutron stars may considerably modify the emergent spectra and impede efforts to constraint neutron star properties. Resonant cyclotron scattering by a non-relativistic warm plasma in an inhomogeneous magnetic field has a number of unusual characteristics: (i) in the limit of high resonant optical depth, the cyclotron resonant layer is half opaque, in sharp contrast to the case of non-resonant scattering. (ii) The transmitted flux is on average Compton up-scattered by ~ $1+ 2 beta_T$, where $\\beta_T$ is the typical thermal velocity in units of the velocity of light; the reflected flux has on average the initial frequency. (iii) For both the transmitted and reflected fluxes the dispersion of intensity decreases with increasing optical depth. (iv) The emergent spectrum is appreciably non-Plankian while narrow spectral features produced at the surface may be erased. We derive semi-analytically modification of the surface Plankian emission due to multiple scattering between the resonant layers and apply the model to anomalous X-ray pulsar 1E 1048.1--5937. Our simple model fits just as well as the ``canonical'' magnetar spectra model of a blackbody plus power-law.

  8. Solid phases of spatially nanoconfined oxygen: A neutron scattering study

    SciTech Connect (OSTI)

    Kojda, Danny [Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, 14109 Berlin (Germany) [Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, 14109 Berlin (Germany); Freie Universität Berlin, 14195 Berlin (Germany); Wallacher, Dirk; Hofmann, Tommy, E-mail: tommy.hofmann@helmholtz-berlin.de [Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, 14109 Berlin (Germany)] [Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, 14109 Berlin (Germany); Baudoin, Simon; Hansen, Thomas [Institut Laue-Langevin, BP 156, 38042 Grenoble Cedex 9 (France)] [Institut Laue-Langevin, BP 156, 38042 Grenoble Cedex 9 (France); Huber, Patrick [Technische Universität Hamburg-Harburg, 21073 Hamburg (Germany)] [Technische Universität Hamburg-Harburg, 21073 Hamburg (Germany)

    2014-01-14

    We present a comprehensive neutron scattering study on solid oxygen spatially confined in 12 nm wide alumina nanochannels. Elastic scattering experiments reveal a structural phase sequence known from bulk oxygen. With decreasing temperature cubic ?-, orthorhombic ?- and monoclinic ?-phases are unambiguously identified in confinement. Weak antiferromagnetic ordering is observed in the confined monoclinic ?-phase. Rocking scans reveal that oxygen nanocrystals inside the tubular channels do not form an isotropic powder. Rather, they exhibit preferred orientations depending on thermal history and the very mechanisms, which guide the structural transitions.

  9. Method for improving the angular resolution of a neutron scatter camera

    DOE Patents [OSTI]

    Mascarenhas, Nicholas; Marleau, Peter; Gerling, Mark; Cooper, Robert Lee; Mrowka, Stanley; Brennan, James S.

    2012-12-25

    An instrument that will directly image the fast fission neutrons from a special nuclear material source wherein the neutron detection efficiency is increased has been described. Instead of the previous technique that uses a time-of-flight (TOF) between 2 widely spaced fixed planes of neutron detectors to measure scatter neutron kinetic energy, we now use the recoil proton energy deposited in the second of the 2 scatter planes which can now be repositioned either much closer together or further apart. However, by doubling the separation distance between the 2 planes from 20 cm to a distance of 40 cm we improved the angular resolution of the detector from about 12.degree. to about 10.degree.. A further doubling of the separation distance to 80 cm provided an addition improvement in angular resolution of the detector to about 6.degree. without adding additional detectors or ancillary electronics. The distance between planes also may be dynamically changed using a suitable common technique such as a gear- or motor-drive to toggle between the various positions. The angular resolution of this new configuration, therefore, is increased at the expanse of detection sensitivity. However, the diminished sensitivity may be acceptable for those applications where the detector is able to interrogate a particular site for an extended period.

  10. Polarized and unpolarized neutron-scattering study of the dynamical spin susceptibility of YBa2Cu3O7

    E-Print Network [OSTI]

    Aksay, Ilhan A.

    Polarized and unpolarized neutron-scattering study of the dynamical spin susceptibility of YBa2Cu3O to previous neutron- scattering data on YBa2Cu3O7 , theoretical interpretations of NMR data and current models, , is mea- sured by neutron scattering as a function of momentum q and energy . Neutron-scattering

  11. [49] INTERSUBUNIT MEASUREMENTS BY NEUTRON SCATTERING 629 ribosomal 30 S subparticle in its lateral view. The amount of the particles

    E-Print Network [OSTI]

    [49] INTERSUBUNIT MEASUREMENTS BY NEUTRON SCATTERING 629 ribosomal 30 S subparticle in its lateral Neutron Scattering By PETER B. MOOREand DONALDM. ENGELMAN Several years ago we suggested that neutron.28 " The scattering lengths are taken from G. E. Bacon, "Neutron Scattering." Oxford Univ. Press (Clarendon

  12. Accurate Development of Thermal Neutron Scattering Cross Section Libraries

    SciTech Connect (OSTI)

    Hawari, Ayman; Dunn, Michael

    2014-06-10

    The objective of this project is to develop a holistic (fundamental and accurate) approach for generating thermal neutron scattering cross section libraries for a collection of important enutron moderators and reflectors. The primary components of this approach are the physcial accuracy and completeness of the generated data libraries. Consequently, for the first time, thermal neutron scattering cross section data libraries will be generated that are based on accurate theoretical models, that are carefully benchmarked against experimental and computational data, and that contain complete covariance information that can be used in propagating the data uncertainties through the various components of the nuclear design and execution process. To achieve this objective, computational and experimental investigations will be performed on a carefully selected subset of materials that play a key role in all stages of the nuclear fuel cycle.

  13. Nucleon semimagic numbers and low-energy neutron scattering

    E-Print Network [OSTI]

    D. A. Zaikin; I. V. Surkova

    2010-04-09

    It is shown that experimental values of the cross sections of inelastic low-energy neutron scattering on even-even nuclei together with the description of these cross sections in the framework of the coupled channel optical model may be considered as a reliable method for finding nuclei with a semimagic number (or numbers) of nucleons. Some examples of the application of this method are considered.

  14. Previously, DC Magnets located at Neutron-Scattering Beamlines were commercially-manufactured superconducting magnets and limited to 17 T. A

    E-Print Network [OSTI]

    Weston, Ken

    Previously, DC Magnets located at Neutron-Scattering Beamlines were commercially, this was the first designed specifically for neutron scattering and the first to include resistive suitable for neutron scattering, diffraction and spectroscopy experiments with the neutron beam passing

  15. Total cross section of neutron-proton scattering at low energies in quark-gluon model

    E-Print Network [OSTI]

    V. A. Abramovsky; N. V. Radchenko

    2011-07-30

    We show that analysis of nonrelativistic neutron-proton scattering in a framework of relativistic QCD based quark model can give important information about QCD vacuum structure. In this model we describe total cross section of neutron-proton scattering at kinetic energies of projectile neutron from 1 eV up to 1 MeV.

  16. American Conference on Neutron Scattering M4-C4 (5:15 pm)

    E-Print Network [OSTI]

    Danon, Yaron

    50 American Conference on Neutron Scattering M4-C4 (5:15 pm) aCORN: A New MeasurementBeamlineatSnS.Inthistalk,theprinciple oftheexperiment,andthestatusofongoingR&d willbereviewedanddiscussed. M4-C6 (5:45 pm) Neutron-proton Scattering of the Electron- antineutrino Correlation Coefficient in Neutron Decay M. Leuschner (Indiana University Cyclotron

  17. NEUTRON SCATTERING SHOWS THAT CYTOCHROME b5 PENETRATES DEEPLY INTO THE LIPID BILAYER

    E-Print Network [OSTI]

    NEUTRON SCATTERING SHOWS THAT CYTOCHROME b5 PENETRATES DEEPLY INTO THE LIPID BILAYER E. P. GOGOL of a highly deuterated phospholipid. Small-angle neutron diffraction patterns were collected in a series of H to lipid vesicles using neutron small-angle scattering methods. To increase scat- tering contrast between

  18. Small angle neutron scattering (SANS) under non-equilibrium conditions R. C. Oberthr

    E-Print Network [OSTI]

    Boyer, Edmond

    663 Small angle neutron scattering (SANS) under non-equilibrium conditions R. C. Oberthür Institut with the times obtained from quasi- elastic neutron and light scattering, which yield information about neutrons aux petits angles (DNPA) pour l'étude des systèmes hors d'équi- libre thermodynamique est

  19. National School on Neutron and X-ray Scattering June 14-28, 2014

    E-Print Network [OSTI]

    Kemner, Ken

    National School on Neutron and X-ray Scattering June 14-28, 2014 Argonne National Laboratory:00 Dinner Dinner Dinner Dinner Week 1 wrap-up Picnic #12;National School on Neutron and X-ray Scattering Restaurant 9:45 - 10:45 Lecture Interaction of X-rays and Neutrons with Matter Roger Pynn University

  20. Small angle neutron scattering from single-wall carbon nanotube suspensions: evidence for isolated

    E-Print Network [OSTI]

    Wang, Howard "Hao"

    Small angle neutron scattering from single-wall carbon nanotube suspensions: evidence for isolated online: Abstract We report small angle neutron scattering (SANS) from dilute suspensions of purified University, Houghton, MI 49931, USA e NIST Center for Neutron Research, National Institute of Standards

  1. Inelastic magnetic neutron scattering in CePd{sub 3}.

    SciTech Connect (OSTI)

    Lawrence, J. M.; Fanelli, V. R.; Goremychkin, E. A.; Osborn, R.; Bauer, E. D.; McClellan, K. J.; Christianson, A. D.; Univ. of California at Irvine; LANL; ORNL

    2008-01-01

    We have performed time-of-flight neutron scattering measurements on a single crystal of the intermediate valence compound CePd{sub 3}. At 10 K, a Kondo-esque inelastic magnetic scattering peak occurs near {Delta}E = 60 meV with maximum intensity for momentum transfer Q near the (1/2, 1/2, 0) zone boundary. Spectral weight is transferred to lower energy as Q varies until at zone center the intensity at 60 meV is considerably weaker. These results are in qualitative accord with predictions of the Anderson lattice. The Q-dependence may resolve an older controversy concerning the low-temperature scattering. We discuss the relationship of these results to our recent results in YbAl{sub 3}.

  2. Chiral Three-Nucleon Interactions in Light Nuclei, Neutron-$\\alpha$ Scattering, and Neutron Matter

    E-Print Network [OSTI]

    Lynn, J E; Carlson, J; Gandolfi, S; Gezerlis, A; Schmidt, K E; Schwenk, A

    2015-01-01

    We present quantum Monte Carlo calculations of light nuclei, neutron-$\\alpha$ scattering, and neutron matter using local two- and three-nucleon (3N) interactions derived from chiral effective field theory up to next-to-next-to-leading order (N$^2$LO). The two undetermined 3N low-energy couplings are fit to the $^4$He binding energy and, for the first time, to the spin-orbit splitting in the neutron-$\\alpha$ $P$-wave phase shifts. Furthermore, we investigate different choices of local 3N operator structures and find that chiral interactions at N$^2$LO are able to simultaneously reproduce the properties of $A=4,5$ systems and of neutron matter, in contrast to commonly used phenomenological 3N interactions.

  3. Electron scattering from high-momentum neutrons in deuterium

    SciTech Connect (OSTI)

    Klimenko, A.V.; Kuhn, S.E.; Bueltmann, S.; Careccia, S.L.; Dharmawardane, K.V.; Dodge, G.E.; Guler, N.; Hyde-Wright, C.E.; Klein, A.; Tkachenko, S.; Weinstein, L.B.; Zhang, J. [Old Dominion University, Norfolk, Virginia 23529 (United States); Butuceanu, C.; Griffioen, K.A.; Baillie, N.; Fersch, R.G.; Funsten, H. [College of William and Mary, Williamsburg, Virginia 23187 (United States); Egiyan, K.S.; Asryan, G.; Dashyan, N.B. [Yerevan Physics Institute, 375036 Yerevan (Armenia)] (and others)

    2006-03-15

    We report results from an experiment measuring the semiinclusive reaction {sup 2}H(e,e{sup '}p{sub s}) in which the proton p{sub s} is moving at a large angle relative to the momentum transfer. If we assume that the proton was a spectator to the reaction taking place on the neutron in deuterium, the initial state of that neutron can be inferred. This method, known as spectator tagging, can be used to study electron scattering from high-momentum (off-shell) neutrons in deuterium. The data were taken with a 5.765 GeV electron beam on a deuterium target in Jefferson Laboratory's Hall B, using the CEBAF large acceptance spectrometer. A reduced cross section was extracted for different values of final state missing mass W*, backward proton momentum p{sup {yields}}{sub s}, and momentum transfer Q{sup 2}. The data are compared to a simple plane wave impulse approximation (PWIA) spectator model. A strong enhancement in the data observed at transverse kinematics is not reproduced by the PWIA model. This enhancement can likely be associated with the contribution of final state interactions (FSI) that were not incorporated into the model. Within the framework of the simple spectator model, a 'bound neutron structure function' F{sub 2n}{sup eff} was extracted as a function of W* and the scaling variable x* at extreme backward kinematics, where the effects of FSI appear to be smaller. For p{sub s}>0.4 GeV/c, where the neutron is far off-shell, the model overestimates the value of F{sub 2n}{sup eff} in the region of x* between 0.25 and 0.6. A dependence of the bound neutron structure function on the neutron's 'off-shell-ness' is one possible effect that can cause the observed deviation.

  4. New measurement of the scattering cross section of slow neutrons on liquid parahydrogen from neutron transmission

    E-Print Network [OSTI]

    K. B. Grammer; R. Alarcon; L. Barrón-Palos; D. Blyth; J. D. Bowman; J. Calarco; C. Crawford; K. Craycraft; D. Evans; N. Fomin; J. Fry; M. Gericke; R. C. Gillis; G. L. Greene; J. Hamblen; C. Hayes; S. Kucuker; R. Mahurin; M. Maldonado-Velázquez; E. Martin; M. McCrea; P. E. Mueller; M. Musgrave; H. Nann; S. I. Penttilä; W. M. Snow; Z. Tang; W. S. Wilburn

    2015-04-24

    Liquid hydrogen is a dense Bose fluid whose equilibrium properties are both calculable from first principles using various theoretical approaches and of interest for the understanding of a wide range of questions in many body physics. Unfortunately, the pair correlation function $g(r)$ inferred from neutron scattering measurements of the differential cross section $d\\sigma \\over d\\Omega$ from different measurements reported in the literature are inconsistent. We have measured the energy dependence of the total cross section and the scattering cross section for slow neutrons with energies between 0.43~meV and 16.1~meV on liquid hydrogen at 15.6~K (which is dominated by the parahydrogen component) using neutron transmission measurements on the hydrogen target of the NPDGamma collaboration at the Spallation Neutron Source at Oak Ridge National Laboratory. The relationship between the neutron transmission measurement we perform and the total cross section is unambiguous, and the energy range accesses length scales where the pair correlation function is rapidly varying. At 1~meV our measurement is a factor of 3 below the data from previous work. We present evidence that these previous measurements of the hydrogen cross section, which assumed that the equilibrium value for the ratio of orthohydrogen and parahydrogen has been reached in the target liquid, were in fact contaminated with an extra non-equilibrium component of orthohydrogen. Liquid parahydrogen is also a widely-used neutron moderator medium, and an accurate knowledge of its slow neutron cross section is essential for the design and optimization of intense slow neutron sources. We describe our measurements and compare them with previous work.

  5. Safety & Security Guidelines Annual U.S. National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    Safety & Security Guidelines 15th Annual U.S. National School on Neutron and X-ray Scattering-574-4600. Neutron Sciences User Programs and Outreach Office Oak Ridge National Laboratory #12;

  6. Electron Scattering From High-Momentum Neutrons in Deuterium

    E-Print Network [OSTI]

    A. V. Klimenko; S. E. Kuhn; for the CLAS collaboration

    2005-10-12

    We report results from an experiment measuring the semi-inclusive reaction $d(e,e'p_s)$ where the proton $p_s$ is moving at a large angle relative to the momentum transfer. If we assume that the proton was a spectator to the reaction taking place on the neutron in deuterium, the initial state of that neutron can be inferred. This method, known as spectator tagging, can be used to study electron scattering from high-momentum (off-shell) neutrons in deuterium. The data were taken with a 5.765 GeV electron beam on a deuterium target in Jefferson Laboratory's Hall B, using the CLAS detector. A reduced cross section was extracted for different values of final-state missing mass $W^{*}$, backward proton momentum $\\vec{p}_{s}$ and momentum transfer $Q^{2}$. The data are compared to a simple PWIA spectator model. A strong enhancement in the data observed at transverse kinematics is not reproduced by the PWIA model. This enhancement can likely be associated with the contribution of final state interactions (FSI) that were not incorporated into the model. A ``bound neutron structure function'' $F_{2n}^{eff}$ was extracted as a function of $W^{*}$ and the scaling variable $x^{*}$ at extreme backward kinematics, where effects of FSI appear to be smaller. For $p_{s}>400$ MeV/c, where the neutron is far off-shell, the model overestimates the value of $F_{2n}^{eff}$ in the region of $x^{*}$ between 0.25 and 0.6. A modification of the bound neutron structure function is one of possible effects that can cause the observed deviation.

  7. Electron Scattering From High-Momentum Neutrons in Deuterium

    SciTech Connect (OSTI)

    A.V. Klimenko; S.E. Kuhn

    2005-10-12

    We report results from an experiment measuring the semi-inclusive reaction D(e,e'p{sub s}) where the proton p{sub s} is moving at a large angle relative to the momentum transfer. If we assume that the proton was a spectator to the reaction taking place on the neutron in deuterium, the initial state of that neutron can be inferred. This method, known as spectator tagging, can be used to study electron scattering from high-momentum (off-shell) neutrons in deuterium. The data were taken with a 5.765 GeV electron beam on a deuterium target in Jefferson Laboratory's Hall B, using the CLAS detector. A reduced cross section was extracted for different values of final-state missing mass W*, backward proton momentum {rvec p}{sub s} and momentum transfer Q{sup 2}. The data are compared to a simple PWIA spectator model. A strong enhancement in the data observed at transverse kinematics is not reproduced by the PWIA model. This enhancement can likely be associated with the contribution of final state interactions (FSI) that were not incorporated into the model. A ''bound neutron structure function'' F{sub 2n}{sup eff} was extracted as a function of W* and the scaling variable x* at extreme backward kinematics, where effects of FSI appear to be smaller. For p{sub s} > 400 MeV/c, where the neutron is far off-shell, the model overestimates the value of F{sub 2n}{sup eff} in the region of x* between 0.25 and 0.6. A modification of the bound neutron structure function is one of possible effects that can cause the observed deviation.

  8. Neutron scattering at the high flux isotope reactor at Oak Ridge National Laboratory

    SciTech Connect (OSTI)

    Yethiraj, M.; Fernandez-Baca, J.A.

    1995-03-01

    Since its beginnings in Oak Ridge and Argonne in the late 1940`s, neutron scattering has been established as the premier tool to study matter in its various states. Since the thermal neutron wavelength is of the same order of magnitude as typical atomic spacings and because they have comparable energies to those of atomic excitations in solids, both structure and dynamics of matter can be studied via neutron scattering. The High Flux Isotope Reactor (HFIR) provides an intense source of neutrons with which to carry out these measurements. This paper summarizes the available neutron scattering facilities at the HFIR.

  9. Precision Measurement of the n-3He Incoherent Scattering Length Using Neutron Interferometry

    E-Print Network [OSTI]

    M. G. Huber; M. Arif; T. C. Black; W. C. Chen; T. R. Gentile; D. S. Hussey; D. Pushin; F. E. Wietfeldt; L. Yang

    2009-05-12

    We report the first measurement of the low-energy neutron-$^3$He incoherent scattering length using neutron interferometry: $b_i' = (-2.512\\pm 0.012{statistical}\\pm0.014{systematic})$ fm. This is in good agreement with a recent calculation using the AV18+3N potential. The neutron-$^3$He scattering lengths are important for testing and developing nuclear potential models that include three nucleon forces, effective field theories for few-body nuclear systems, and neutron scattering measurements of quantum excitations in liquid helium. This work demonstrates the first use of a polarized nuclear target in a neutron interferometer.

  10. Temperature-driven phase transformation in Y3Co: Neutron scattering...

    Office of Scientific and Technical Information (OSTI)

    Temperature-driven phase transformation in Y3Co: Neutron scattering and first-principles studies Citation Details In-Document Search Title: Temperature-driven phase transformation...

  11. Lambda-Neutron Scattering Lengths from Radiative K-minus Capture

    E-Print Network [OSTI]

    W. R. Gibbs; S. A. Coon; H. K. Han; B. F. Gibson

    2000-01-02

    Radiative capture of the K-minus by the deuteron as a reaction for measurement of the Lambda-neutron scattering lengths. The use of spin information to separate the singlet and triplet scattering lengths is treated.

  12. Parallel Computational Modelling of Inelastic Neutron Scattering in Multi-node and Multi-core Architectures 

    E-Print Network [OSTI]

    Garba, M.T.; Gonzales-Velez, H.; Roach, D.L.

    2010-11-26

    This paper examines the initial parallel implementation of SCATTER, a computationally intensive inelastic neutron scattering routine with polycrystalline averaging capability, for the General Utility Lattice Program (GULP). Of particular importance...

  13. X-ray and neutron scattering from nano-mgantic clusters | The...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-ray and neutron scattering from nano-mgantic clusters The student will participate in hands on X-ray scattering experiments on bio-inspired inorganic materials (i.e., magnetic...

  14. A system for differential neutron scattering experiments in the energy range from 0.5 to 20 MeV

    E-Print Network [OSTI]

    Danon, Yaron

    A system for differential neutron scattering experiments in the energy range from 0.5 to 20 MeV F 2010 Accepted 15 April 2010 Available online 27 May 2010 Keywords: Scattering Neutron Benchmark dependent scattered neutron distributions. Scattering measurements were performed on carbon and molybdenum

  15. Inelastic neutron and low-frequency Raman scattering in a niobium-phosphate glass for Raman gain applications

    E-Print Network [OSTI]

    Schirmacher, Walter

    Inelastic neutron and low-frequency Raman scattering in a niobium-phosphate glass for Raman gain: Raman scattering; Neutron scattering; Raman gain; Boson peak We present measurements of the vibrational, extracted from specific-heat or neutron scattering measurements [7,8]. Only very recently two of the present

  16. For more information: Neutron Scattering Science User Office, neutronusers@ornl.gov or (865) 574-4600.

    E-Print Network [OSTI]

    Pennycook, Steve

    For more information: Neutron Scattering Science User Office, neutronusers@ornl.gov or (865) 574 Cold Neutron Triple-Axis Spectrometer CallforProposals neutrons.ornl.gov Neutron Scattering Science Neutron Source (SNS) will be accepted via the web-based proposal system until 11:59 a.m. EDT, (NOON

  17. Neutron Polarisabilities from Deuteron Compton Scattering in \\chiEFT

    E-Print Network [OSTI]

    Harald W. Griesshammer

    2007-10-15

    Chiral Effective Field Theory is for photon energies up to 200 MeV the tool to accurately determine the polarisabilities of the neutron from deuteron Compton scattering. A multipole analysis reveals that dispersive effects from an explicit Delta(1232) prove in particular indispensable to understand the data at 95 MeV measured at SAL. Simple power-counting arguments derived from nuclear phenomenology lead to the correct Thomson limit and gauge invariance. At next-to-leading order, the static scalar dipole polarisabilities are extracted as identical for proton and neutron within the error-bar of available data: \\alpha^n=11.6\\pm1.5_stat\\pm0.6_Baldin, \\beta^n=3.6\\mp1.5_stat\\pm0.6_Baldin for the neutron, in units of 10^-4 fm^3, compared to \\alpha^p=11.0\\pm1.4_stat\\pm0.4_Baldin, \\beta}^p=2.8\\mp1.4_stat\\pm0.4_Baldin for the proton in the same framework. New experiments e.g. at MAXlab (Lund) will improve the statistical error-bar.

  18. Single-Volume Neutron Scatter Camera for High-Efficiency Neutron Imaging and Source Characterization. Year 2 of 3 Summary

    SciTech Connect (OSTI)

    Brubaker, Erik

    2015-10-01

    The neutron scatter camera (NSC), an imaging spectrometer for fission energy neutrons, is an established and proven detector for nuclear security applications such as weak source detection of special nuclear material (SNM), arms control treaty verification, and emergency response. Relative to competing technologies such as coded aperture imaging, time-encoded imaging, neutron time projection chamber, and various thermal neutron imagers, the NSC provides excellent event-by-event directional information for signal/background discrimination, reasonable imaging resolution, and good energy resolution. Its primary drawback is very low detection efficiency due to the requirement for neutron elastic scatters in two detector cells. We will develop a singlevolume double-scatter neutron imager, in which both neutron scatters can occur in the same large active volume. If successful, the efficiency will be dramatically increased over the current NSC cell-based geometry. If the detection efficiency approaches that of e.g. coded aperture imaging, the other inherent advantages of double-scatter imaging would make it the most attractive fast neutron detector for a wide range of security applications.

  19. Consilience: Radiocarbon, Instrumental Neutron Activation Analysis, and Litigation in the Ancestral Caddo Region 

    E-Print Network [OSTI]

    Selden, Robert Zachary

    2013-08-13

    Through the creation and analysis of databases for radiocarbon, instrumental neutron activation analysis (INAA), and law, macro-level trends are exposed that form the framework of a broader research program aimed at advancing ideas of craft...

  20. ON QUASI-ELASTIC SCATTERING OF SLOW NEUTRONS IN MOLECULAR LIQUIDS

    E-Print Network [OSTI]

    Boyer, Edmond

    L-317 ON QUASI-ELASTIC SCATTERING OF SLOW NEUTRONS IN MOLECULAR LIQUIDS M. UTSURO Research Reactor de neutrons avec élargissement par rotation moléculaire dans le liquide sont étudiés dans le cadre du du benzène liquide. Abstract. 2014 The rotational broadened quasi-elastic scattering spectrum

  1. Salt-Dependent Compaction of Di-and Trinucleosomes Studied by Small-Angle Neutron Scattering

    E-Print Network [OSTI]

    Langowski, Jörg

    Salt-Dependent Compaction of Di- and Trinucleosomes Studied by Small-Angle Neutron Scattering, Germany, and Institut Laue-Langevin Grenoble, F-38042 Grenoble, France ABSTRACT Using small-angle neutron scattering (SANS), we have measured the salt-dependent static structure factor of di- and trinucleosomes from

  2. Investigation of the tripoli porous structure by small-angle neutron scattering

    SciTech Connect (OSTI)

    Avdeev, M. V.; Blagoveshchenskii, N. M.; Garamus, V. M.; Novikov, A. G. Puchkov, A. V.

    2011-12-15

    The characteristics of the tripoli porous structure have been investigated by small-angle neutron scattering (SANS). Tripoli is a finely porous sedimentary rock formed by small spherical opal particles. Its main component is aqueous silica SiO{sub 2} {center_dot} nH{sub 2}O (80-90%). Tripoli is widely used in practice as a working medium for sorption filters and in some other commercial and construction technologies. The shape of the experimental SANS curves indicates the presence of small and large pores in tripoli. The small-pore size was estimated to be {approx}100 Angstrom-Sign . The size of large pores turned out to be beyond the range of neutron wave vector transfers Q that are available for the instrument used; however, their size was indirectly estimated to be {approx}(2000-2500) Angstrom-Sign . The pores of both groups behave as surfacetype fractal scatterers with the fractal dimension D {approx} 2.2-2.6. The densities of pores of these two groups differ by approximately three orders of magnitude ({approx}10{sup 16} and {approx}10{sup 13} cm{sup -3} for small and large pores, respectively); the fraction of large pores amounts to 70-80% of the total pore volume. The found pore characteristics (their densities, sizes, and relative volumes) are in satisfactory agreement (when a comparison is possible) with the absorption data.

  3. Membrane association of the PTEN tumor suppressor: Neutron scattering and MD simulations reveal the structure

    E-Print Network [OSTI]

    Loesche, Mathias

    Membrane association of the PTEN tumor suppressor: Neutron scattering and MD simulations reveal Engineering, Carnegie Mellon University, Pittsburgh, PA 15213, USA c NIST Center for Neutron Research Phosphatidylserine Neutron reflection Tethered bilayer lipid membranes Molecular dynamics simulations a b s t r a c

  4. Data Analysis & Visualization | Neutron Science | ORNL

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Data Analysis and Visualization As the data sets generated by the increasingly powerful neutron scattering instruments at HFIR and SNS grow ever more massive, the facilities'...

  5. Neutron Data Analysis & Visualization | More Science | ORNL

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Data Analysis and Visualization As the data sets generated by the increasingly powerful neutron scattering instruments at HFIR and SNS grow ever more massive, the facilities'...

  6. The Nature of the Surface Species Formed on Au/TiO2 during the Reaction of H2 and O2: An Inelastic Neutron Scattering Study

    E-Print Network [OSTI]

    Goodman, Wayne

    Neutron Scattering Study Chinta Sivadinarayana, Tushar V. Choudhary, Luke L. Daemen, Juergen Eckert of obvious interest for understanding this process. Vibrational spectroscopy by inelastic neutron scattering

  7. The LANSCE (Los Alamos Neutron Scattering Center) software management environment

    SciTech Connect (OSTI)

    Donahue, S.; Cort, G.

    1988-01-01

    We present the details of an innovative software management environment implemented to address life cycle support requirements at the Los Alamos Neutron Scattering Center (LANSCE). The system provides an automated configuration management framework within which all software development and maintenance activities are performed. The LANSCE environment provides a comprehensive configuration management (CM) system based upon a commercially available CM tool. The CM component ensures the integrity of all LANSCE application software, automatically performs status accounting operations, and provides a flexible automated facility for rebuilding resident software components and restoring them to the baseline. It employs high-level data structures both to enhance significantly the level of automation that can be achieved and to provide extensive, integrated support to the software development community. We discuss the software management philosophy that led to the development of the LANSCE environment on programmer productivity, system integration and software management effectiveness. 8 refs., 4 figs.

  8. J. Mol. Biol. (1975) 91, 101-120 A Neutron Scattering Study of the Distribution of Protein

    E-Print Network [OSTI]

    1975-01-01

    J. Mol. Biol. (1975) 91, 101-120 A Neutron Scattering Study of the Distribution of Protein and RNA coli have been measured by neutron scattering experiments on the intact subunit. In addition the radius, 1972; Lutter et al., 1972), and neutron scattering (Engelman & Moore, 1972; Moore et al., 1974

  9. Eur. J. Biochem. 85, 529-534 (1978) X-Ray and Neutron Small-Angle Scattering Studies

    E-Print Network [OSTI]

    1978-01-01

    Eur. J. Biochem. 85, 529-534 (1978) X-Ray and Neutron Small-Angle Scattering Studies of the Complex-ray and neutron scattering techniques. In this work, we concentrated mainly on radius of gyration analyses and a neutron scattering experiment is performed in 21-Iz0 solvent. This decrease simply reflects the fact

  10. Z .Reviews in Molecular Biotechnology 74 2000 207 231 X-ray and neutron surface scattering for studying

    E-Print Network [OSTI]

    Wong, Joyce

    Z .Reviews in Molecular Biotechnology 74 2000 207 231 X-ray and neutron surface scattering,U , Tonya L. Kuhlb , Joyce Y. Wongc , Gregory S. Smitha,1 a Manuel Lujan Jr. Neutron Scattering Center is defined as the Zratio of the number of particles neutrons or .photons elastically and specularly scattered

  11. Small angle neutron scattering study of deuterated sodium dodecylsulfate micellization in dilute poly((2edimethylamino)ethyl methacrylate) solutions

    E-Print Network [OSTI]

    Rubloff, Gary W.

    Small angle neutron scattering study of deuterated sodium dodecylsulfate micellization in dilute 2010 Keywords: Poly((2edimethylamino)ethyl methacrylate) Micelle Small angle neutron scattering a b angle neutron scattering. We found three transitions of the poly ((2edimethylamino)ethyl methacrylate

  12. HIV-1 Tat membrane interactions probed using X-ray and neutron scattering, CD spectroscopy and MD simulations

    E-Print Network [OSTI]

    Nagle, John F.

    HIV-1 Tat membrane interactions probed using X-ray and neutron scattering, CD spectroscopy and MD translocation, were provided by wide-angle X-ray scattering (WAXS) and neutron scattering. CD spectroscopy for Neutron Research, 100 Bureau Drive, Stop 6102, Gaithersburg, MD 20899, United States d CHESS, Cornell

  13. Low-frequency Vibrational Anomalies in -Lactoglobulin: Contribution of Different Hydrogen Classes Revealed by Inelastic Neutron Scattering

    E-Print Network [OSTI]

    Tuscia, Università Degli Studi Della

    Revealed by Inelastic Neutron Scattering A. Orecchini, A. Paciaroni, A. R. Bizzarri, and S. Cannistraro -lactoglobulin has been investigated by inelastic neutron scattering, on both dry and D2O-hydrated samples. Both typically accessible energy and momentum transfers, inelastic thermal neutron scattering is probably

  14. What's wrong with the field of bio-neutron scattering? 1) Not enough professional science and not enough professional scientists

    E-Print Network [OSTI]

    Doster, Wolfgang

    What's wrong with the field of bio-neutron scattering? 1) Not enough professional science a paper in this field. Anybody can do it! The most detailed analysis of bio-neutron scattering data up independent moment analysis of the neutron scattering spectrum. Up to today nobody, not even MD people, picked

  15. Quasi-differential neutron scattering from 238 U from 0.5 to 20 MeV

    E-Print Network [OSTI]

    Danon, Yaron

    Quasi-differential neutron scattering from 238 U from 0.5 to 20 MeV A.M. Daskalakis a, , R Measurement Neutron scattering Time-of-flight experiment Benchmark a b s t r a c t The Rensselaer Polytechnic scattering sample 30 m from the source. Eight liquid scintillator (EJ-301) proton recoil fast neutron

  16. Los Alamos National Laboratory | Science and people highlights from the Lujan Neutron Scattering Center at LANSCE CENTER SCIENCE & PEOPLE

    E-Print Network [OSTI]

    Los Alamos National Laboratory | Science and people highlights from the Lujan Neutron Scattering at the Lujan Neutron Scattering Center to de- termine the difference in water splitting catalytic activity be: " Local Structure of the Vacancy Disordered Fluorite Yb3 TaO7 from Neutron Total Scattering," Journal

  17. A View of Dynamics Changes in the Molten Globule-native Folding Step by Quasielastic Neutron Scattering

    E-Print Network [OSTI]

    dynamics that occur in the ®nal stages of protein folding, we have used neutron scattering to probe- lastic neutron scattering (IQNS). The IQNS results show length scale dependent, pico-second dynamics neutron scattering; a-lactalbumin*Corresponding author Introduction Proteins can form collapsed, partially

  18. PHYSICAL REVIEW B 85, 205440 (2012) Inelastic neutron scattering investigations of the quantum molecular dynamics of a H2 molecule

    E-Print Network [OSTI]

    Turro, Nicholas J.

    2012-01-01

    PHYSICAL REVIEW B 85, 205440 (2012) Inelastic neutron scattering investigations of the quantum transfer arising from the neutron scattering event has also been investigated. The -dependence spectra investigations using infrared (IR),3,13­15 inelastic neutron scattering (INS),3,16,17 and nuclear magnetic

  19. Review of Indirect Methods Used to Determine the $^1S_0$ Neutron-Neutron Scattering Length

    E-Print Network [OSTI]

    C. R. Howell

    2008-05-08

    We have determined a value for the $^1S_0$ neutron-neutron scattering length ($a_{nn}$) from high-precision measurements of time-of-flight spectra of neutrons from the $^2H(\\pi^-,n \\gamma)n$ capture reaction. The measurements were done at the Los Alamos Meson Physics Facility by the E1286 collaboration. The high spatial resolution of our gamma-ray detector enabled us to make a detailed assessment of the systematic uncertainties in our techniques. The value obtained in the present work is $a_{nn} = -18$.63 $\\pm $0.10 (statistical) $\\pm$ 0.44 (systematic) $\\pm$ 0.30 (theoretical) fm. This result is consistent with previous determinations of $a_{nn}$ from the $\\pi^-d$ capture reaction. We found that the analysis of the data with calculations that use a relativistic phase-space factor gives a more negative value for $a_{nn}$ by 0.33 fm over the analysis done using a nonrelativistic phase-space factor. Combining the present result with the previous ones from $\\pi^-d$ capture gives: $a_{nn} = - 18$.63 $\\pm$ 0.27 (expt) $\\pm$ 0.30 fm (theory). For the first time the combined statistical and systematic experimental uncertainty in $a_{nn}$ is smaller than the theoretical uncertainty and comparable to the uncertainty in the proton-proton $^1S_0$ scattering length ($a_{pp}$). This average value of $a_{nn}$ when corrected for the magnetic-moment interaction of the two neutrons becomes -18.9 $\\pm$ 0.4 fm which is 1.6 $\\pm$ 0.5 fm different from the recommended value of $a_{pp}$, thereby confirming charge symmetry breaking at the 1% confidence level.

  20. For more information: Neutron Scattering Science User Office, neutronusers@ornl.gov or (865) 574-4600.

    E-Print Network [OSTI]

    Pennycook, Steve

    For more information: Neutron Scattering Science User Office, neutronusers@ornl.gov or (865) 574 Spectrometer (ARCS) CallforProposals neutrons.ornl.gov Neutron Scattering Science - Oak Ridge National Neutron Source (SNS) will be accepted via the web-based proposal system until 11:59 a.m. EST, (NOON

  1. For more information: Neutron Scattering Science User Office, neutronusers@ornl.gov or (865) 574-4600.

    E-Print Network [OSTI]

    For more information: Neutron Scattering Science User Office, neutronusers@ornl.gov or (865) 574Proposals neutrons.ornl.gov Neutron Scattering Science - Oak Ridge National Laboratory Due March 6, 2013 #12; Neutron Source (SNS) will be accepted via the web-based proposal system until 11:59 a.m. EST, (NOON

  2. Determination of the effective parameters of proton-$^{3}$He scattering on the basis of the neutron-triton scattering data

    E-Print Network [OSTI]

    V. P. Levashev

    2008-12-22

    We have studied the relations between the neutron-triton scattering lengths and effective ranges and the corresponding quantities for the p --$^{3}$He scattering in the framework of the potential model with an effective nucleon-nucleus interaction in the form of a $\\delta $-shell potential. It is shown that the Coulomb renormalization of the pure nuclear scattering lengths does not change the relation well established for the n + $^{3}$H system between the lengths: $A^{1} scattering lengths which give preference to set I of the phase analysis performed by E.A. George et al. (2003), which corresponds to the inequality $A^{1}_{nc} scattering lengths.

  3. Neutrino Scattering in a Newly Born Neutron Star

    E-Print Network [OSTI]

    Sanjay Reddy; Madappa Prakash

    1996-10-16

    We calculate neutrino cross sections from neutral current reactions in the dense matter encountered in the evolution of a newly born neutron star. Effects of composition and of strong interactions in the deleptonization and cooling phases of the evolution are studied. The influence of the possible presence of strangeness-rich hyperons on the neutrino scattering cross sections is explored. Due to the large vector couplings of the Sigma-minus and Cascade-minus, |C_V|~2, these particles, if present in protoneutron star matter, give significant contributions to neutrino scattering. In the deleptonization phase, the presence of strangeness leads to large neutrino energies, which results in large enhancements in the cross sections compared to those in matter with nucleons only. In the cooling phase, in which matter is nearly neutrino free, the response of the Sigma-minus hyperons to thermal neutrinos is the most significant. Neutrinos couple relatively weakly to the Lambda hyperons and, hence, their contributions are significant only at high density.

  4. Neutron and light scattering studies of light-harvesting photosynthetic antenna complexes

    SciTech Connect (OSTI)

    Tang, Kuo-Hsiang [Washington Univ., St. Louis, MO (United States); Blankenship, Robert E. [Washington Univ., St. Louis, MO (United States)

    2011-06-28

    Small-angle neutron scattering (SANS) and dynamic light scattering (DLS) have been employed in studying the structural information of various biological systems, particularly in systems without high-resolution structural information available. In this report, we briefly present some principles and biological applications of neutron scattering and DLS, compare the differences in information that can be obtained with small-angle X-ray scattering (SAXS), and then report recent studies of SANS and DLS, together with other biophysical approaches, for light-harvesting antenna complexes and reaction centers of purple and green phototrophic bacteria.

  5. Micro-focused Small Angle Neutron Scattering and Imaging for Science and Engineering Using RTP--A Preliminary Study

    SciTech Connect (OSTI)

    Mohamed, Abdul Aziz; Al Rashid Megat Ahmad, Megat Harun; Md Idris, Faridah; Azman, Azraf; Jamro, Rafhayudi; Ibrahim, Mohd Rizal Mamat; Rahman, Anwar Abdul [Agensi Nuklear Malaysia, Komplek PUSPATI, Bangi, 43000 Kajang, Selangor (Malaysia)

    2010-01-05

    Malaysian Nuclear Agency's (Nuclear Malaysia) Small Angle Neutron Scattering (SANS) facility--(MYSANS)--is utilizing low flux of thermal neutron at the agency's 1 MW TRIGA reactor. As the design nature of the 8 m SANS facility can allow object resolution in the range between 5 and 80 nm to be obtained. It can be used to study alloys, ceramics and polymers in certain area of problems that relate to samples containing strong scatterers or contrast. The current SANS system at Malaysian Nuclear Agency is only capable to measure Q in limited range with a PSD (128x128) fixed at 4 m from the sample. The existing reactor hall that incorporate this MYSANS facility has a layout that prohibits the rebuilding of MYSANS therefore the position between the wavelength selector (HOPG) and sample and the PSD cannot be increased for wider Q range. The flux of the neutron at current sample holder is very low which around 10{sup 3} n/cm{sup 2}/sec. Thus it is important to rebuild the MYSANS to maximize the utilization of neutron. Over the years, the facility has undergone maintenance and some changes have been made. Modification on secondary shutter and control has been carried out to improve the safety level of the instrument. A compact micro-focus SANS method can suit this objective together with an improve cryostat system. This paper will explain some design concept and approaches in achieving higher flux and the modification needs to establish the micro-focused SANS.

  6. Your access to the Oak Ridge National Laboratory (ORNL) is approved beginning Sunday, June 20, 2010, for the second week of the Neutron X-ray Scattering School.

    E-Print Network [OSTI]

    Pennycook, Steve

    , for the second week of the Neutron X-ray Scattering School. Please be certain to bring photo identification access to the Target Facility.) · General User Access Training for Neutron Scattering Users, Neutron Scattering Science User Office Oak Ridge National Laboratory ORNL Neutron Scattering School June

  7. X-ray and neutron scattering studies of the complex compounds...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-ray and neutron scattering studies of the complex compounds Wednesday, September 25, 2013 - 1:00pm SLAC, Conference Room 137-322 Presented by Dr. Hoyoung Jang, Max Planck...

  8. Coherent neutron scattering and collective dynamics on mesoscale

    SciTech Connect (OSTI)

    Novikov, Vladimir [ORNL; Schweizer, Kenneth S [ORNL; Sokolov, Alexei P [ORNL

    2013-01-01

    By combining, and modestly extending, a variety of theoretical concepts for the dynamics of liquids in the supercooled regime, we formulate a simple analytic model for the temperature and wavevector dependent collective density fluctuation relaxation time that is measurable using coherent dynamic neutron scattering. Comparison with experiments on the ionic glass-forming liquid Ca K NO3 in the lightly supercooled regime suggests the model captures the key physics in both the local cage and mesoscopic regimes, including the unusual wavevector dependence of the collective structural relaxation time. The model is consistent with the idea that the decoupling between diffusion and viscosity is reflected in a different temperature dependence of the collective relaxation time at intermediate wavevectors and near the main (cage) peak of the static structure factor. More generally, our analysis provides support for the ideas that decoupling information and growing dynamic length scales can be at least qualitatively deduced by analyzing the collective relaxation time as a function of temperature and wavevector, and that there is a strong link between dynamic heterogeneity phenomena at the single and many particle level. Though very simple, the model can be applied to other systems, such as molecular liquids.

  9. Neutron monitoring systems including gamma thermometers and methods of calibrating nuclear instruments using gamma thermometers

    DOE Patents [OSTI]

    Moen, Stephan Craig; Meyers, Craig Glenn; Petzen, John Alexander; Foard, Adam Muhling

    2012-08-07

    A method of calibrating a nuclear instrument using a gamma thermometer may include: measuring, in the instrument, local neutron flux; generating, from the instrument, a first signal proportional to the neutron flux; measuring, in the gamma thermometer, local gamma flux; generating, from the gamma thermometer, a second signal proportional to the gamma flux; compensating the second signal; and calibrating a gain of the instrument based on the compensated second signal. Compensating the second signal may include: calculating selected yield fractions for specific groups of delayed gamma sources; calculating time constants for the specific groups; calculating a third signal that corresponds to delayed local gamma flux based on the selected yield fractions and time constants; and calculating the compensated second signal by subtracting the third signal from the second signal. The specific groups may have decay time constants greater than 5.times.10.sup.-1 seconds and less than 5.times.10.sup.5 seconds.

  10. Advances in passive neutron instruments for safeguards use

    SciTech Connect (OSTI)

    Menlove, H.O.; Krick, M.S.; Langner, D.G.; Miller, M.C.; Stewart, J.E.

    1994-02-01

    Passive neutron and other nondestructive assay techniques have been used extensively by the International Atomic Energy Agency to verify plutonium metal, powder, mixed oxide, pellets, rods, assemblies, scrap, and liquids. Normally, the coincidence counting rate is used to measure the {sup 240}Pu-effective mass and gamma-ray spectrometry or mass spectrometry is used to verify the plutonium isotopic ratios. During the past few years, the passive neutron detectors have been installed in plants and operated in the unattended/continuous mode. These radiation data with time continuity have made it possible to use the totals counting rate to monitor the movement of nuclear material. Monte Carlo computer codes have been used to optimize the detector designs for specific applications. The inventory sample counter (INVS-III) has been designed to have a higher efficiency (43%) and a larger uniform counting volume than the original INVS. Data analyses techniques have been developed, including the ``known alpha`` and ``known multiplication`` methods that depend on the sample. For scrap and other impure or poorly characterized samples, we have developed multiplicity counting, initially implemented in the plutonium scrap multiplicity counter. For large waste containers such as 200-L drums, we have developed the add-a-source technique to give accurate corrections for the waste-matrix materials. This paper summarizes recent developments in the design and application of passive neutron assay systems.

  11. Measurement of Leading Neutron Production in Deep-Inelastic Scattering at HERA

    E-Print Network [OSTI]

    H1 Collaboration

    2010-01-04

    The production of leading neutrons, where the neutron carries a large fraction x_L of the incoming proton's longitudinal momentum, is studied in deep-inelastic positron-proton scattering at HERA. The data were taken with the H1 detector in the years 2006 and 2007 and correspond to an integrated luminosity of 122 pb^{-1}. The semi-inclusive cross section is measured in the phase space defined by the photon virtuality 6 neutron transverse momentum p_T neutron structure function, F_2^{LN(3)}(Q^2,x,x_L), and the fraction of deep-inelastic scattering events containing a leading neutron are studied as a function of Q^2, x and x_L. Assuming that the pion exchange mechanism dominates leading neutron production, the data provide constraints on the shape of the pion structure function.

  12. 16th National School on Neutron and X-ray Scattering

    SciTech Connect (OSTI)

    Chakoumakos, Bryan; Achilles, Cherie; Cybulskis, Viktor; Gilbert, Ian

    2014-07-02

    Students talk about their experience at the 16th National School on Neutron and X-ray Scattering, or NXS 2014. Jointly conducted by Oak Ridge and Argonne national laboratories, NXS immerses graduate students in national user facilities to learn in a hands-on environment how to use neutrons and X-rays in their research.

  13. 16th National School on Neutron and X-ray Scattering

    ScienceCinema (OSTI)

    Chakoumakos, Bryan; Achilles, Cherie; Cybulskis, Viktor; Gilbert, Ian

    2014-07-23

    Students talk about their experience at the 16th National School on Neutron and X-ray Scattering, or NXS 2014. Jointly conducted by Oak Ridge and Argonne national laboratories, NXS immerses graduate students in national user facilities to learn in a hands-on environment how to use neutrons and X-rays in their research.

  14. The Manuel Lujan, Jr. Neutron Scattering Center LANSCE experiment reports 1989 run cycle

    SciTech Connect (OSTI)

    Hyer, D.K.; DiStravolo, M.A.

    1990-10-01

    This report contains a listing and description of experiments carried on at the LANSCE neutron scattering facility in the following areas: High Density Powder Diffraction; Neutron Powder Diffractometer, (NPD); Single Crystal Diffractometer, (SCD); Low-Q Diffractometer, (LQD); Surface Profile Analysis Reflectometer, (SPEAR); Filter Difference Spectrometer, (FDS); and Constant-Q Spectrometer.

  15. Static light scattering and small-angle neutron scattering study on aggregated recombinant gelatin in aqueous solution

    E-Print Network [OSTI]

    Sutter, Marc

    2006-10-25

    Static Light Scattering and Small-Angle Neutron Scattering Study on Aggregated Recombinant Gelatin in Aqueous Solution A. Ramzi 1, M. Sutter 2, W.E. Hennink 1, W. Jiskoot 1,2 1 Department of Pharmaceutics, UIPS, Utrecht University, The Netherlands... 2 Department of Drug Delivery Technology, LACDR, Leiden University, The Netherlands Recombinant Gelatins ? Recombinant gelatins are currently being evaluated as pharmaceutical excipients. ? Behavior of recombinant gelatins in solution is not well...

  16. Supplementary data for HIV-1 Tat membrane interaction probed using X-ray and neutron scattering, CD, and MD simulations

    E-Print Network [OSTI]

    Nagle, John F.

    1 Supplementary data for HIV-1 Tat membrane interaction probed using X-ray and neutron scattering- spacing are linearly related. Figure S3. Neutron scattering from stacks of DOPC:DOPE (3:1)/Tat, x=0 of Physics, Rensselaer Polytechnic Institute, 110 Eighth Street, Troy, NY 12180, 3 NIST Center for Neutron

  17. Anisotropic Motion and Molecular Dynamics of Cholesterol, Lanosterol, and Ergosterol in Lecithin Bilayers Studied by Quasi-elastic Neutron Scattering

    E-Print Network [OSTI]

    Brown, Michael F.

    Bilayers Studied by Quasi-elastic Neutron Scattering Emil Endress, Helmut Heller,§ He´le`ne CasaltaVised Manuscript ReceiVed June 27, 2002 ABSTRACT: Quasi-elastic neutron scattering (QENS) was employed to study of motion within the bilayer on the molecular dynamics time scale. In a recent quasi-elastic neutron

  18. Apparatus for the investigation of liquid systems in a shear gradient by small angle neutron scattering (SANS)

    E-Print Network [OSTI]

    Boyer, Edmond

    of small angle neutron scattering from fluids in a constant shear gradient. Typical systems which can angle neutron scattering experiments with liquids have given information about structural pro- perties759 Apparatus for the investigation of liquid systems in a shear gradient by small angle neutron

  19. For more information: Neutron Scattering Science User Office, neutronusers@ornl.gov or (865) 574-4600.

    E-Print Network [OSTI]

    Pennycook, Steve

    For more information: Neutron Scattering Science User Office, neutronusers@ornl.gov or (865) 574.ornl.gov Neutron Scattering Science - Oak Ridge National Laboratory Due February 26, 2014 #12; Neutron Source (SNS) will be accepted via the web-based proposal system until 11:59 a.m. EST, (NOON

  20. Salt-Dependent DNA Superhelix Diameter Studied by Small Angle Neutron Scattering Measurements and Monte Carlo Simulations

    E-Print Network [OSTI]

    Langowski, Jörg

    Salt-Dependent DNA Superhelix Diameter Studied by Small Angle Neutron Scattering Measurements-38042 Grenoble Cedex 9, France ABSTRACT Using small angle neutron scattering we have measured the static the same behavior between 10 and 100 mM salt concentration: An undulation in the scattering curve

  1. Dynamics of water in prussian blue analogues: Neutron scattering study

    SciTech Connect (OSTI)

    Sharma, V. K.; Mitra, S.; Thakur, N.; Yusuf, S. M.; Mukhopadhyay, R.; Juranyi, Fanni

    2014-07-21

    Dynamics of crystal water in Prussian blue (PB), Fe(III){sub 4}[Fe(II)(CN){sub 6}]{sub 3}.14H{sub 2}O and its analogue Prussian green (PG), ferriferricynaide, Fe(III){sub 4}[Fe(III)(CN){sub 6}]{sub 4}.16H{sub 2}O have been investigated using Quasielastic Neutron Scattering (QENS) technique. PB and its analogue compounds are important materials for their various interesting multifunctional properties. It is known that crystal water plays a crucial role towards the multifunctional properties of Prussian blue analogue compounds. Three structurally distinguishable water molecules: (i) coordinated water molecules at empty nitrogen sites, (ii) non-coordinated water molecules in the spherical cavities, and (iii) at interstitial sites exist in PB. Here spherical cavities are created due to the vacant sites of Fe(CN){sub 6} units. However, PG does not have any such vacant N or Fe(CN){sub 6} units, and only one kind of water molecules, exists only at interstitial sites. QENS experiments have been carried out on both the compounds in the temperature range of 260–360?K to elucidate the dynamical behavior of different kinds of water molecules. Dynamics is found to be much more pronounced in case of PB, compared to PG. A detailed data analysis showed that localized translational diffusion model could describe the observed data for both PB and PG systems. The average diffusion coefficient is found to be much larger in the PB than PG. The obtained domain of dynamics is found to be consistent with the geometry of the structure of the two systems. Combining the data of the two systems, a quantitative estimate of the dynamics, corresponding to the water molecules at different locations is made.

  2. Leading neutron energy and pT distributions in deep inelastic scattering and photoproduction at HERA

    E-Print Network [OSTI]

    ZEUS Collaboration; S. Chekanov

    2007-03-09

    The production of energetic neutrons in $ep$ collisions has been studied with the ZEUS detector at HERA. The neutron energy and $p_T^2$ distributions were measured with a forward neutron calorimeter and tracker in a $40 \\pb^{-1}$ sample of inclusive deep inelastic scattering (DIS) data and a $6 \\pb^{-1}$ sample of photoproduction data. The neutron yield in photoproduction is suppressed relative to DIS for the lower neutron energies and the neutrons have a steeper $p_T^2$ distribution, consistent with the expectation from absorption models. The distributions are compared to HERA measurements of leading protons. The neutron energy and transverse-momentum distributions in DIS are compared to Monte Carlo simulations and to the predictions of particle exchange models. Models of pion exchange incorporating absorption and additional secondary meson exchanges give a good description of the data.

  3. Elastic and inelastic neutron scattering cross sections for fission reactor applications

    SciTech Connect (OSTI)

    Hicks, S. F.; Combs, B.; Downes, L.; Girgis, J.; Kersting, L. J.; Lueck, C. J.; McDonough, P. J.; Schniederjan, J.; Sidwell, L.; Sigillito, A. J. [Department of Physics, University of Dallas, Irving TX 75019 (United States); Chakraborty, A.; Crider, B. P.; Kumar, A.; McEllistrem, M. T.; Peters, E. E.; Prados-Estevz, F. M. [Department of Physics and Astronomy, University of Kentucky, Lexington, KY 40506 (United States); Vanhoy, J. R.; Watts, D. [Department of Physics, United States Naval Academy, Annapolis MD 21402 (United States); Yates, S. W. [Department of Physics and Astronomy, University of Kentucky, Lexington, KY 40506 (United States) and Department of Chemistry, University of Kentucky, Lexington, KY 40506 (United States)

    2013-04-19

    Nuclear data important for the design and development of the next generation of light-water reactors and future fast reactors include neutron elastic and inelastic scattering cross sections on important structural materials, such as Fe, and on coolant materials, such as Na. These reaction probabilities are needed since neutron reactions impact fuel performance during irradiations and the overall efficiency of reactors. While neutron scattering cross sections from these materials are available for certain incident neutron energies, the fast neutron region, particularly above 2 MeV, has large gaps for which no measurements exist, or the existing uncertainties are large. Measurements have been made at the University of Kentucky Accelerator Laboratory to measure neutron scattering cross sections on both Fe and Na in the region where these gaps occur and to reduce the uncertainties on scattering from the ground state and first excited state of these nuclei. Results from measurements on Fe at incident neutron energies between 2 and 4 MeV will be presented and comparisons will be made to model calculations available from data evaluators.

  4. A study of neutron-deuteron scattering in configuration space

    E-Print Network [OSTI]

    V. M. Suslov; M. A. Braun; I. Filikhin; B. Vlahovic

    2006-10-09

    A new computational method for solving the configuration-space Faddeev equations for the breakup scattering problem has been applied to nd scattering both below and above the two-body threshold.

  5. Measurement of the Neutron Radius of 208Pb Through Parity-Violation in Electron Scattering

    E-Print Network [OSTI]

    Abrahamyan, S; Albataineh, H; Aniol, K; Armstrong, D S; Armstrong, W; Averett, T; Babineau, B; Barbieri, A; Bellini, V; Beminiwattha, R; Benesch, J; Benmokhtar, F; Bielarski, T; Boeglin, W; Camsonne, A; Canan, M; Carter, P; Cates, G D; Chen, C; Chen, J -P; Hen, O; Cusanno, F; Dalton, M M; De Leo, R; de Jager, K; Deconinck, W; Decowski, P; Deng, X; Deur, A; Dutta, D; Etile, A; Flay, D; Franklin, G B; Friend, M; Frullani, S; Fuchey, E; Garibaldi, F; Gasser, E; Gilman, R; Giusa, A; Glamazdin, A; Gomez, J; Grames, J; Gu, C; Hansen, O; Hansknecht, J; Higinbotham, D W; Holmes, R S; Holmstrom, T; Horowitz, C J; Hoskins, J; Huang, J; Hyde, C E; Itard, F; Jen, C -M; Jensen, E; Jin, G; Johnston, S; Kelleher, A; Kliakhandler, K; King, P M; Kowalski, S; Kumar, K S; Leacock, J; Leckey, J; Lee, J H; LeRose, J J; Lindgren, R; Liyanage, N; Lubinsky, N; Mammei, J; Mammoliti, F; Margaziotis, D J; Markowitz, P; McCreary, A; McNulty, D; Mercado, L; Meziani, Z -E; Michaels, R W; Mihovilovic, M; Muangma, N; Muñoz-Camacho, C; Nanda, S; Nelyubin, V; Nuruzzaman, N; Oh, Y; Palmer, A; Parno, D; Paschke, K D; Phillips, S K; Poelker, B; Pomatsalyuk, R; Posik, M; Puckett, A J R; Quinn, B; Rakhman, A; Reimer, P E; Riordan, S; Rogan, P; Ron, G; Russo, G; Saenboonruang, K; Saha, A; Sawatzky, B; Shahinyan, A; Silwal, R; Sirca, S; Slifer, K; Solvignon, P; Souder, P A; Sperduto, M L; Subedi, R; Suleiman, R; Sulkosky, V; Sutera, C M; Tobias, W A; Troth, W; Urciuoli, G M; Waidyawansa, B; Wang, D; Wexler, J; Wilson, R; Wojtsekhowski, B; Yan, X; Yao, H; Ye, Y; Ye, Z; Yim, V; Zana, L; Zhan, X; Zhang, J; Zhang, Y; Zheng, X; Zhu, P

    2012-01-01

    We report the first measurement of the parity-violating asymmetry A_PV in the elastic scattering of polarized electrons from 208Pb. A_PV is sensitive to the radius of the neutron distribution (Rn). The result A_PV = 0.656 \\pm 0.060 (stat) \\pm 0.013 (syst) corresponds to a difference between the radii of the neutron and proton distributions Rn - Rp = 0.33 +0.16 -0.18 fm and provides the first electroweak observation of the neutron skin which is expected in a heavy, neutron-rich nucleus.

  6. Measurement of the Neutron Radius of 208Pb Through Parity-Violation in Electron Scattering

    E-Print Network [OSTI]

    S. Abrahamyan; Z. Ahmed; H. Albataineh; K. Aniol; D. S. Armstrong; W. Armstrong; T. Averett; B. Babineau; A. Barbieri; V. Bellini; R. Beminiwattha; J. Benesch; F. Benmokhtar; T. Bielarski; W. Boeglin; A. Camsonne; M. Canan; P. Carter; G. D. Cates; C. Chen; J. -P. Chen; O. Hen; F. Cusanno; M. M. Dalton; R. De Leo; K. de Jager; W. Deconinck; P. Decowski; X. Deng; A. Deur; D. Dutta; A. Etile; D. Flay; G. B. Franklin; M. Friend; S. Frullani; E. Fuchey; F. Garibaldi; E. Gasser; R. Gilman; A. Giusa; A. Glamazdin; J. Gomez; J. Grames; C. Gu; O. Hansen; J. Hansknecht; D. W. Higinbotham; R. S. Holmes; T. Holmstrom; C. J. Horowitz; J. Hoskins; J. Huang; C. E. Hyde; F. Itard; C. -M. Jen; E. Jensen; G. Jin; S. Johnston; A. Kelleher; K. Kliakhandler; P. M. King; S. Kowalski; K. S. Kumar; J. Leacock; J. Leckey IV; J. H. Lee; J. J. LeRose; R. Lindgren; N. Liyanage; N. Lubinsky; J. Mammei; F. Mammoliti; D. J. Margaziotis; P. Markowitz; A. McCreary; D. McNulty; L. Mercado; Z. -E. Meziani; R. W. Michaels; M. Mihovilovic; N. Muangma; C. Muñoz-Camacho; S. Nanda; V. Nelyubin; N. Nuruzzaman; Y. Oh; A. Palmer; D. Parno; K. D. Paschke; S. K. Phillips; B. Poelker; R. Pomatsalyuk; M. Posik; A. J. R. Puckett; B. Quinn; A. Rakhman; P. E. Reimer; S. Riordan; P. Rogan; G. Ron; G. Russo; K. Saenboonruang; A. Saha; B. Sawatzky; A. Shahinyan; R. Silwal; S. Sirca; K. Slifer; P. Solvignon; P. A. Souder; M. L. Sperduto; R. Subedi; R. Suleiman; V. Sulkosky; C. M. Sutera; W. A. Tobias; W. Troth; G. M. Urciuoli; B. Waidyawansa; D. Wang; J. Wexler; R. Wilson; B. Wojtsekhowski; X. Yan; H. Yao; Y. Ye; Z. Ye; V. Yim; L. Zana; X. Zhan; J. Zhang; Y. Zhang; X. Zheng; P. Zhu

    2012-01-13

    We report the first measurement of the parity-violating asymmetry A_PV in the elastic scattering of polarized electrons from 208Pb. A_PV is sensitive to the radius of the neutron distribution (Rn). The result A_PV = 0.656 \\pm 0.060 (stat) \\pm 0.014 (syst) ppm corresponds to a difference between the radii of the neutron and proton distributions Rn - Rp = 0.33 +0.16 -0.18 fm and provides the first electroweak observation of the neutron skin which is expected in a heavy, neutron-rich nucleus.

  7. Measurement of the Neutron Radius of 208Pb Through Parity-Violation in Electron Scattering

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Abrahamyan, Sergey; Albataineh, Hisham; Aniol, Konrad; Armstrong, David; Armstrong, Whitney; Averett, Todd; Babineau, Benjamin; Barbieri, A.; Bellini, Vincenzo; Beminiwattha, Rakitha; et al

    2012-03-15

    We report the first measurement of the parity-violating asymmetry APV in the elastic scattering of polarized electrons from 208Pb. APV is sensitive to the radius of the neutron distribution (Rn). The result APV = 0.656 ± 0.060 (stat) ± 0.013 (syst) corresponds to a difference between the radii of the neutron and proton distributions Rn-Rp = 0.33-0.18+0.16 fm and provides the first electroweak observation of the neutron skin which is expected in a heavy, neutron-rich nucleus.

  8. Analyzing the Effects of Neutron Polarizabilities in Elastic Compton Scattering off ${}^3He$

    E-Print Network [OSTI]

    Deepshikha Shukla; Andreas Nogga; Daniel R. Phillips

    2008-12-01

    Motivated by the fact that a polarized ${}^3He$ nucleus behaves as an `effective' neutron target, we examine manifestations of neutron electromagnetic polarizabilities in elastic Compton scattering from the Helium-3 nucleus. We calculate both unpolarized and double-polarization observables using chiral perturbation theory to next-to-leading order (${\\mathcal O}(e^2 Q)$) at energies, $\\omega \\lsim m_{\\pi}$, where $m_{\\pi}$ is the pion mass. Our results show that the unpolarized differential cross section can be used to measure neutron electric and magnetic polarizabilities, while two double-polarization observables are sensitive to different linear combinations of the four neutron spin polarizabilities.

  9. Asterix is a reflectometer/diffractometer/grazing-incidence-SANS/SESAME-enabled-SANS spectrometer that is primarily used for experiments or neutron scattering

    E-Print Network [OSTI]

    that is primarily used for experiments or neutron scattering techniques requiring polarized neutron beams detector arm is readily configurable for polarization or energy analysis of the scattered neutron beam be translated in the horizontal and vertical directions. Neutron detector (Spin Echo Scattering Angle

  10. Structured water in polyelectrolyte dendrimers: Understanding small angle neutron scattering results through atomistic simulation

    SciTech Connect (OSTI)

    Chen, Wei-Ren [ORNL; Do, Changwoo [ORNL; Hong, Kunlun [ORNL; Liu, Emily [Rensselaer Polytechnic Institute (RPI); Liu, Yun [National Institute of Standards and Technology (NIST); Porcar, L. [National Institute of Standards and Technology (NIST); Smith, Gregory Scott [ORNL; Wu, Bin [ORNL; Egami, T [University of Tennessee, Knoxville (UTK); Smith, Sean C [ORNL

    2012-01-01

    Based on atomistic molecular dynamics (MD) simulations, the small angle neutron scattering (SANS) intensity behavior of a single generation-4 (G4) polyelectrolyte polyamidoamine (PAMAM) starburst dendrimer is investigated at different levels of molecular protonation. The SANS form factor, P(Q), and Debye autocorrelation function, (r), are calculated from the equilibrium MD trajectory based on a mathematical approach proposed in this work which provides a link between the neutron scattering experiment and MD computation. The simulations enable scattering calculations of not only the hydrocarbons, but also the contribution to the scattering length density fluctuations caused by structured, confined water within the dendrimer. Based on our computational results, we question the validity of using radius of gyration RG for microstructure characterization of a polyelectrolyte dendrimer from the scattering perspective.

  11. STUDY MAGNETIC EXCITATIONS IN DOPED TRANSITION METAL OXIDES USING INELASTIC NEUTRON SCATTERING

    SciTech Connect (OSTI)

    Dai, Pengcheng

    2014-02-18

    Understanding the interplay between magnetism and superconductivity continues to be a “hot” topic in modern condensed matter physics. The discovery of high-temperature superconductivity in iron-based materials in 2008 provided an unique opportunity to compare and contrast these materials with traditional high-Tc copper oxide superconductors. Neutron scattering plays an important role in determining the dynamical spin properties in these materials. This proposal is a continuation of previous DOE supported proposal. This report summarizes the final progress we have made over from May 2005 till Aug. 2013. Overall, we continue to carry out extensive neutron scattering experiments on Fe-based materials, focusing on understanding their magnetic properties. In addition, we have established a materials laboratory at UT that has allowed us to grow these superconductors. Because neutron scattering typically demands a large amount of samples, by growing these materials in our own laboratory, we can now pursuit neutron scattering experiments over the entire electronic phase diagram, focusing on regions of interests. The material synthesis laboratory at UT was established entirely with the support of DOE funding. This not only allowed us to carry out neutron scattering experiments, but also permit us to provide samples to other US/International collaborators for studying these materials.

  12. National School on Neutron and X-ray Scattering Oak Ridge National Laboratory June 12-26, 2010 Oak Ridge, Tennessee

    E-Print Network [OSTI]

    Pennycook, Steve

    National School on Neutron and X-ray Scattering Oak Ridge National Laboratory June 12-26, 2010 Oak:30 Lecture Inelastic Neutron Scattering B. D. Gaulin McMaster University Lecture Magnetic Scattering B. D Break Break Break Break 9:45 - 10:45 Lecture Continued Inelastic Neutron Scattering B. D. Gaulin Mc

  13. Scattering Theory When an x-ray beam (or neutron or light) passes through a material with

    E-Print Network [OSTI]

    Beaucage, Gregory

    Scattering Theory When an x-ray beam (or neutron or light) passes through a material radiation is scattered in directions that differ from that of the incident beam. Scattering arises since x of scattered radiation resulting from this process bears a direct relationship to the structure (the pattern

  14. Note: Versatile sample stick for neutron scattering experiments in high electric fields

    SciTech Connect (OSTI)

    Bartkowiak, M., E-mail: marek.bartkowiak@psi.ch [Laboratory for Developments and Methods, Paul Scherrer Institut, CH-5232 Villigen (Switzerland); White, J. S. [Laboratory for Neutron Scattering, Paul Scherrer Institut, CH-5232 Villigen (Switzerland) [Laboratory for Neutron Scattering, Paul Scherrer Institut, CH-5232 Villigen (Switzerland); Laboratory for Quantum Magnetism, Ecole Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne (Switzerland); Rønnow, H. M.; Prša, K. [Laboratory for Quantum Magnetism, Ecole Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne (Switzerland)] [Laboratory for Quantum Magnetism, Ecole Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne (Switzerland)

    2014-02-15

    We present a versatile high voltage sample stick that fits into all cryomagnets and standard cryostats at the Swiss Spallation Neutron Source, Paul Scherrer Institut, and which provides a low effort route to neutron scattering experiments that combine electric field with low temperature and magnetic field. The stick allows for voltages up to 5 kV and can be easily adapted for different scattering geometries. We discuss the design consideration and thermal behavior of the stick, and give one example to showcase the abilities of the device.

  15. Finite volume effects in low-energy neutron-deuteron scattering

    E-Print Network [OSTI]

    Alexander Rokash; Evgeny Epelbaum; Hermann Krebs; Dean Lee; Ulf-G. Meißner

    2013-08-15

    We present a lattice calculation of neutron-deuteron scattering at very low energies and investigate in detail the impact of the topological finite-volume corrections. Our calculations are carried out in the framework of pionless effective field theory at leading order in the low-energy expansion. Using lattice sizes and a lattice spacing comparable to those employed in nuclear lattice simulations, we find that the topological volume corrections must be taken into account in order to obtain correct results for the neutron-proton S-wave scattering lengths.

  16. Exact limiting relation between the structure factors in neutron and x-ray scattering

    E-Print Network [OSTI]

    V. B. Bobrov; S. A. Trigger; S. N. Skovorod'ko

    2010-07-11

    The ratio of the static matter structure factor measured in experiments on coherent X-ray scattering to the static structure factor measured in experiments on neutron scattering is considered. It is shown theoretically that this ratio in the long-wavelength limit is equal to the nucleus charge at arbitrary thermodynamic parameters of a pure substance (the system of nuclei and electrons, where interaction between particles is pure Coulomb) in a disordered equilibrium state. This result is the exact relation of the quantum statistical mechanics. The experimental verification of this relation can be done in the long wavelength X-ray and neutron experiments.

  17. Multifunction Instrument Tree (MIT) Neutron and Gamma Probe Acceptance for Beneficial Use (ABU)

    SciTech Connect (OSTI)

    CANNON, N.S.

    1999-08-08

    The multifunction instrument tree (MIT) probe program has been developed to modify existing Liquid Observation Well (LOW) neutron and gamma probes for use in the validation shafts of the two MITs installed in Tank 241-SY-101. One of the program objectives is that the modified MIT probes be completely compatible with the existing LOW van instrumentation and procedures. The major program objective is to produce neutron and gamma scans from Tank 241-SY-101 that would assist in evaluating waste feature structure and elevation. The MIT probe program is described in greater detail in the engineering task plan (HNF-3322). In accordance with the engineering task plan, a test plan (HNF-3595) was written, reduced diameter (allowing insertion into the MIT validation tube) neutron and gamma probes were acquired, an acceptance and operational test procedure (HNF-3838) was written, acceptance and operational testing of the MIT probes was performed, and a report of these test results (HNF-4369) has been issued. A number of neutron and gamma probe scans have been obtained from the Tank 241-SY-101 MITs, starting on February 8, 1999, in cooperation with Operations. Now that the MIT probes are fully demonstrated, this document transfers ownership of these probes to Operations, utilizing the final acceptance for beneficial use (ABU) form that follows in Section 3.0.

  18. Elastic neutron scattering at 96 MeV from {sup 12}C and {sup 208}Pb

    SciTech Connect (OSTI)

    Klug, J.; Blomgren, J.; Atac, A.; Bergenwall, B.; Hildebrand, A.; Johansson, C.; Mermod, P.; Pomp, S.; Tippawan, U.; Nilsson, L.; Elmgren, K.; Olsson, N.; Jonsson, O.; Prokofiev, A.V.; Renberg, P.-U.; Nadel-Turonski, P.; Dangtip, S.; Phansuke, P.; Oesterlund, M.; Le Brun, C.

    2003-12-01

    A facility for detection of scattered neutrons in the energy interval 50-130 MeV, SCANDAL, has recently been installed at the 20-180 MeV neutron beam line of the The Svedberg Laboratory, Uppsala. Elastic neutron scattering from {sup 12}C and {sup 208}Pb has been studied at 96 MeV in the 10 deg. -70 deg. interval. The achieved energy resolution, 3.7 MeV, is about an order of magnitude better than for any previous experiment above 65 MeV incident energy. The present experiment represents the highest neutron energy where the ground state has been resolved from the first excited state in neutron scattering. A novel method for normalization of the absolute scale of the cross section has been used. The estimated normalization uncertainty, 3%, is unprecedented for a neutron-induced differential cross section measurement on a nuclear target. The results are compared with modern optical model predictions based on phenomenology or microscopic nuclear theory.

  19. Study on generating of thermal neutron scattering cross sections for LiH

    SciTech Connect (OSTI)

    Wang, L.; Jiang, X.; Zhao, Z.; Chen, L. [Northwest Institute of Nuclear Technology, Xi'an 710024 (China)

    2013-07-01

    LiH is designated as a promising moderator and shielding material because of its low density, high melting point and large fraction of H atoms. However, lack of the thermal neutron cross sections of LiH makes numerical calculation deviate from experimental data to some extent. As a result, it is necessary to study LiH thermal kernel effect. The phonon property of LiH has been investigated by first-principles calculations using the plane-wave pseudo potential method with CASTEP code. The scattering law and the thermal neutron scattering cross sections for Li and H have been generated using this distribution. The results have been compared with zirconium hydride data. The GASKET and NJOY/LEAPR codes have been used in the calculation of scattering law, whose results have been compared with the reference; the discrepancy mainly comes from phonon spectrums and its expansion. LEAPR had the capability to compute scattering through larger energy and momentum transfers than GASKET did. By studying LiH phonon spectrum and constructing the model of LiH thermal kernel and scattering matrix, the ACE format LiH thermal neutron cross sections for MCNP software could be made and used for reactor Neutronics calculation. (authors)

  20. Meausrement of the Neutron Radius of {sup 208}Pb Through Parity Violation in Electron Scattering

    SciTech Connect (OSTI)

    Saenboonruang, Kiadtisak [Virginia U., JLAB

    2013-05-31

    In contrast to the nuclear charge densities, which have been accurately measured with electron scattering, the knowledge of neutron densities still lack precision. Previous model-dependent hadron experiments suggest the difference between the neutron radius, R{sub n}, of a heavy nucleus and the proton radius, R{sub p}, to be in the order of several percent. To accurately obtain the difference, R{sub n}-R{sub p}, which is essentially a neutron skin, the Jefferson Lab Lead ({sup 208}Pb) Radius Experiment (PREX) measured the parity-violating electroweak asymmetry in the elastic scattering of polarized electrons from {sup 208}Pb at an energy of 1.06 GeV and a scattering angle of 5{degrees}#14;. Since Z{sup 0} boson couples mainly to neutrons, this asymmetry provides a clean measurement of R{sub n} with respect to R{sub p}. PREX was conducted at the Jefferson lab experimental Hall A, from March to June 2010. The experiment collected a final data sample of 2x#2;10{sup 7} helicity-window quadruplets. The measured parity-violating electroweak asymmetry A{sub PV} = 0.656 {+-}#6; 0.060 (stat) {+-}#6; 0.014 (syst) ppm corresponds to a difference between the radii of the neutron and proton distributions, R{sub n}-R{sub p} = 0.33{sup +0.16}{sub -0.18} fm and provides the #12;first electroweak observation of the neutron skin as expected in a heavy, neutron-rich nucleus. The value of the neutron radius of {sup 208}Pb has important implications for models of nuclear structure and their application in atomic physics and astrophysics such as atomic parity non-conservation (PNC) and neutron stars.

  1. Is there an Ay problem in low-energy neutron-proton scattering?

    E-Print Network [OSTI]

    Franz Gross; Alfred Stadler

    2008-08-21

    We calculate Ay in neutron-proton scattering for the interactions models WJC-1 and WJC-2 in the Covariant Spectator Theory. We find that the recent 12 MeV measurements performed at TUNL are in better agreement with our results than with the Nijmegen Phase Shift Analysis of 1993, and after reviewing the low-energy data, conclude that there is no Ay problem in low-energy np scattering.

  2. International Conference on Surface X-ray and Neutron Scattering (SXNS-11)

    SciTech Connect (OSTI)

    Michael J. Bedzyk

    2011-06-17

    The 11th International Surface X-ray and Neutron Scattering (SXNS) Conference was held on July 13-17, 2010, on the Northwestern University (NU) campus, in Evanston Illinois and hosted by the NU Materials Research Science and Engineering Center. This biennial conference brought together a community of 164 attendees from 16 countries. The field now makes use of a broad range of new experimental capabilities that have been made possible through the development of increasingly brilliant X-ray and neutron sources around the world, including third generation synchrotron sources, neutron reactor and spallation sources, as well as the recent development of X-ray lasers.

  3. New opportunities for quasielastic and inelastic neutron scattering at steady-state sources using mechanical selection of the incident and final neutron energy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Mamantov, Eugene

    2015-06-12

    We propose a modification of the neutron wide-angle velocity selector (WAVES) device that enables inelastic (in particular, quasielastic) scattering measurements not relying on the neutron time-of-flight. The proposed device is highly suitable for a steady-state neutron source, somewhat similar to a triple-axis spectrometer, but with simultaneous selection of the incident and final neutron energy over a broad range of scattering momentum transfer. Both the incident and final neutron velocities are defined by the WAVES geometry and rotation frequency. The variable energy transfer is achieved through the natural variation of the velocity of the transmitted neutrons as a function of themore »scattering angle component out of the equatorial plane.« less

  4. Proton Angular Distribution for 90 Mev Neutron-proton Scattering

    E-Print Network [OSTI]

    Hadley, James

    2010-01-01

    3, 1947 The angular distribution of the recoil protons inneutron -proton scattering at 90 Mev has been measured forNO. W ..7405-Eng 48 PROTON .ANGULAR DISTRIBUTION FOR 90 lWEV

  5. Small Angle Neutron Scattering Study of Conformation of Oligo(ethylene glycol)-Grafted Polystyrene in Dilute Solutions: Effect of the Backbone Length

    E-Print Network [OSTI]

    Small Angle Neutron Scattering Study of Conformation of Oligo(ethylene glycol)- Grafted Polystyrene Fengjun Hua,2 Kunlun Hong,2 and Jimmy W. Mays2 1Neutron Scattering Sciences Division, ORNL 2Center

  6. Molecular structures of fluid phase phosphatidylglycerol bilayers as determined by small angle neutron and X-ray scattering

    E-Print Network [OSTI]

    Nagle, John F.

    neutron and X-ray scattering Jianjun Pan a, , Frederick A. Heberle a , Stephanie Tristram-Nagle b Matter Division, Neutron Sciences Directorate, Oak Ridge National Laboratory, Oak Ridge, TN 378316100 Institute for Neutron Sciences, Oak Ridge National Laboratory, Oak Ridge, TN 378316453, USA e Canadian

  7. For more information: Neutron Scattering Science User Office, neutronusers@ornl.gov or (865) 574-4600.

    E-Print Network [OSTI]

    For more information: Neutron Scattering Science User Office, neutronusers@ornl.gov or (865) 574 Neutron Source (SNS) will be accepted via the web-based proposal system until 11:59 a.m. EST, (NOON. Information and instructions To learn more about submitting a proposal for beam time, go to http://neutrons

  8. The role of CP violating scatterings in baryogenesis—case study of the neutron portal

    SciTech Connect (OSTI)

    Baldes, Iason; Bell, Nicole F.; Millar, Alexander; Volkas, Raymond R.; Petraki, Kalliopi E-mail: n.bell@unimelb.edu.au E-mail: kpetraki@nikhef.nl

    2014-11-01

    Many baryogenesis scenarios invoke the charge parity (CP) violating out-of-equilibrium decay of a heavy particle in order to explain the baryon asymmetry. Such scenarios will in general also allow CP violating scatterings. We study the effect of these CP violating scatterings on the final asymmetry in a neutron portal scenario. We solve the Boltzmann equations governing the evolution of the baryon number numerically and show that the CP violating scatterings play a dominant role in a significant portion of the parameter space.

  9. Nanoscale structure in AgSbTe2 determined by diffuse elastic neutron scattering

    SciTech Connect (OSTI)

    Specht, Eliot D [ORNL; Ma, Jie [ORNL; Delaire, Olivier A [ORNL; Budai, John D [ORNL; May, Andrew F [ORNL; Karapetrova, Evguenia A. [Argonne National Laboratory (ANL)

    2015-01-01

    Diffuse elastic neutron scattering measurements confirm that AgSbTe2 has a hierarchical structure, with defects on length scales from nanometers to microns. While scattering from mesoscale structure is consistent with previously-proposed structures in which Ag and Sb order on a NaCl lattice, more diffuse scattering from nanoscale structure suggests a structural rearrangement in which hexagonal layers form a combination of (ABC), (ABA), and (AAB) stacking sequences. The AgCrSe2 structure is the best-fitting model for the local atomic arrangements.

  10. Re-evaluation of Neutron-4He Elastic Scattering Data near 20 MeV

    E-Print Network [OSTI]

    M. Drosg; R. Avalos Ortiz; B. Hoop

    2012-10-02

    Measured differential elastic scattering cross sections of 17.71-, 20.97-, and 23.72-MeV neutrons from liquid helium-4 were re-evaluated and corrected for sample size and multiple scattering effects by means of a Monte Carlo technique implemented in a more recent code (MCNPX). Results indicate that earlier corrections via a code, MAGGIE-2, overestimated the size of multiple scattering effects by an order of magnitude. The corrected differential cross sections and Legendre coefficients obtained by least-squares fits are given.

  11. The role of CP violating scatterings in baryogenesis - case study of the neutron portal

    E-Print Network [OSTI]

    Iason Baldes; Nicole F. Bell; Alexander Millar; Kalliopi Petraki; Raymond R. Volkas

    2014-11-28

    Many baryogenesis scenarios invoke the charge parity (CP) violating out-of-equilibrium decay of a heavy particle in order to explain the baryon asymmetry. Such scenarios will in general also allow CP violating scatterings. We study the effect of these CP violating scatterings on the final asymmetry in a neutron portal scenario. We solve the Boltzmann equations governing the evolution of the baryon number numerically and show that the CP violating scatterings play a dominant role in a significant portion of the parameter space.

  12. SANS (small angle neutron scattering) measurement of deuterium-dislocation correlation in palladium

    SciTech Connect (OSTI)

    Heuser, B.J.; Summerfield, G.C.; King, J.S. ); Epperson, J.E. )

    1989-11-01

    Small angle neutron scattering (SANS) measurements have been made on deformed polycrystal palladium samples with and without deuterium dissolved in the solution phase ({alpha}) at room temperature. Concentrations were held constant during SANS experiments by an equilibrium gas pressure cell. The difference scattering cross section for the same sample with and without deuterium loading has a 1/Q behavior (Q=4{pi}/{lambda} sin{theta}/2) at intermediate values of Q. At very low values of Q the dependence is much stronger than 1/Q. The 1/Q behavior is attributed to deuterium trapping close to long dislocation cores forming rod-like scattering structures.

  13. Small-Angle Neutron Scattering Studies of a-Si:H and a-Si:D

    SciTech Connect (OSTI)

    Williamson, D. L.; Marr, D. W. M.; Nelson, B. P.; Iwaniczko, E.; Yang, J.; Yan, B.; Guha, S.

    2000-01-01

    The heterogeneity of hydrogen and deuterium on the nanometer scale has been probed by samll-angle neutron scattering (SANS) from a-Si:H and a-Si:D films. Films were depsoited by two techniques, plasma-enhanced chemical vapor deposition (PECVD) and hot-wire chemical vapor deposition (HWCVD) using conditions that yield high quality films and devices.

  14. Time-independent one-speed neutron transport equation with anisotropic scattering in absorbing media

    SciTech Connect (OSTI)

    Hangelbroek, R. J.

    1980-06-01

    This report treats the time-independent, one-speed neutron transport equation with anisotropic scattering in absorbing media. For nuclear gain operators existence and uniqueness of solutions to the half-space and finite-slab problems are proved in L/sub 2/-space. The formulas needed for explicit calculations are derived by the use of perturbation theory techniques.

  15. Low-Energy Neutron-Oxygen Scattering Derived from 2-Body Forces 

    E-Print Network [OSTI]

    Mackella, A. D.; Reading, John F.; Kerman, A. K.

    1971-01-01

    was installed in the irradiation cell of the Texas A&M University Nuclear Science Center Reactor (NSCR). By increasing the thickness of the lead-bismuth alloy, the neutron spectra were shifted into lower energies by the scattering interactions of fast...

  16. Time-reversal invariance violation measurement using polarized neutron scattering from polarized xenon

    E-Print Network [OSTI]

    Pinghan Chu

    2014-03-06

    We proposed to use polarized neutrons scattering from a hyperpolarized 131Xe gaseous target in order to measure time-reversal violation effect in baryon processes with nucleons. This article provides a brief introduction, historical review, and possible methods to construct a hyperpolarized 131Xe gaseous target.

  17. Quasi-Differential Neutron Scattering in Zirconium from 0.5 to 20 MeV

    E-Print Network [OSTI]

    Danon, Yaron

    in the evaluated libraries at energies between 10 and 20 MeV. For all energies and angles, the investigated nuclear,V' r V! ~Ref. 1!. This term represents the contribution from neutrons scatter- ing from energy E not always agree with each other across the energy range of interest in nuclear reactor analysis. To help

  18. Scattering of 64 eV to 3 keV Neutrons from Polyethylene and Graphite and the Coherence Length Problem

    E-Print Network [OSTI]

    Danon, Yaron

    Scattering of 64 eV to 3 keV Neutrons from Polyethylene and Graphite and the Coherence Length 12180, USA (Received 31 August 2005; published 8 February 2006) We measured the neutron scattering by the neutron coherence length. The scattered intensity ratios were found to conform to conventional

  19. Role of Counterion Concentration in Determining Micelle Aggregation: Evaluation of the Combination of Constraints from Small-Angle Neutron Scattering, Electron Paramagnetic

    E-Print Network [OSTI]

    Bales, Barney

    of Constraints from Small-Angle Neutron Scattering, Electron Paramagnetic Resonance, and Time 91330-8268 ReceiVed: October 17, 2003; In Final Form: January 22, 2004 Small-angle neutron scattering. Introduction Small-angle neutron scattering (SANS) has evolved into a very powerful technique for studying

  20. National School on Neutron and X-ray Scattering Building 223 Auditorium, Room B002 September 24 -October 11, 2008 Argonne National Laboratory

    E-Print Network [OSTI]

    Pennycook, Steve

    National School on Neutron and X-ray Scattering Building 223 Auditorium, Room B002 September 24 (HFIR) Neutron Scattering Science Division Oak Ridge Laboratory 10:15 - 10:30 Break 9:30 - 9:45 Break 10 School on Neutron and X-ray Scattering Building 8600, Main Lobby September 24 - October 11, 2008 Oak

  1. Inelastic neutron scattering spectrum of H2@C60 and its temperature dependence decoded using rigorous quantum calculations and a new

    E-Print Network [OSTI]

    Turro, Nicholas J.

    Inelastic neutron scattering spectrum of H2@C60 and its temperature dependence decoded using://jcp.aip.org/about/rights_and_permissions #12;THE JOURNAL OF CHEMICAL PHYSICS 139, 064309 (2013) Inelastic neutron scattering spectrum of H2@C60 quantum cal- culations of the inelastic neutron scattering (INS) spectra of this prototypical endohedral

  2. The Lujan Center is a national user facility funded by Basic Energy Sciences of the Department of Energy which o ers capability for basic and applied neutron scattering

    E-Print Network [OSTI]

    of Energy which o ers capability for basic and applied neutron scattering relevant to national security are the domain of the low-Q scattering intrument, LQD. These well-established neutron techniques probe long Matter, Local Structure, and Nanomaterials The Lujan Neutron Scattering Center encompasses a set

  3. Week 2 AGENDA: National School on Neutron and X-ray Scattering page 1 of 5 Oak Ridge National Laboratory [9/30/08

    E-Print Network [OSTI]

    Pennycook, Steve

    Week 2 AGENDA: National School on Neutron and X-ray Scattering page 1 of 5 Oak Ridge National Ridge National Laboratory Dean Myles, Director ORNL Neutron Scattering Science Division 1 GROUPS [A,B,C,D,E,F,G,H,I] Iran Thomas Auditorium Lecture Inelastic Neutron Scattering R. Osborn, ANL ALL

  4. JOURNAL DE PHYSIQUE Colloque C4, supplment au n" 4, Tome 40, avril 1979, page C4-142 Magnetic neutron scattering on intermetallic uranium compounds (*)

    E-Print Network [OSTI]

    Paris-Sud XI, Université de

    neutron scattering on intermetallic uranium compounds (*) M. Loewenhaupt (f ), S. Horn (**), F. Steglich.- Abstract. -- We report on inelastic neutron scattering experiments performed in the temperature range 5 K quasielastic line. Using thermal neutrons, no inelastic contributions to the magnetic scattering could

  5. Large volume high-pressure cell for inelastic neutron scattering W. Wang, D. A. Sokolov, A. D. Huxley, and K. V. Kamenev

    E-Print Network [OSTI]

    Hall, Christopher

    Large volume high-pressure cell for inelastic neutron scattering W. Wang, D. A. Sokolov, A. D for inelastic neutron scattering measurements of quantum fluids and solids Rev. Sci. Instrum. 84, 015101 (2013) TOF-SEMSANS--Time-of-flight spin-echo modulated small-angle neutron scattering J. Appl. Phys. 112

  6. Neutron Scattering Science User Office, neutronusers@ornl.gov or (865) 574-4600. Proposals for beam time at Oak Ridge National Laboratory's High Flux Isotope Reactor (HFIR)

    E-Print Network [OSTI]

    Pennycook, Steve

    Neutron Scattering Science User Office, neutronusers@ornl.gov or (865) 574-4600. Proposals for beam Wildgruber, wildgrubercu@ornl.gov. VISION CallforProposals neutrons.ornl.gov Neutron Scattering Science - Oak time at Oak Ridge National Laboratory's High Flux Isotope Reactor (HFIR) and Spallation Neutron Source

  7. Importance of Compton scattering to radiation spectra of isolated neutron stars

    E-Print Network [OSTI]

    V. Suleimanov; K. Werner

    2006-12-22

    Model atmospheres of isolated neutron stars with low magnetic field are calculated with Compton scattering taking into account. Models with effective temperatures 1, 3 and 5 MK, with two values of surface gravity log(g)g = 13.9 and 14.3), and different chemical compositions are calculated. Radiation spectra computed with Compton scattering are softer than the computed with Thomson scattering at high energies (E > 5 keV) for hot (T_eff > 1 MK) atmospheres with hydrogen-helium composition. Compton scattering is more significant to hydrogen models with low surface gravity. The emergent spectra of the hottest (T_eff > 3 MK) model atmospheres can be described by diluted blackbody spectra with hardness factors ~ 1.6 - 1.9. Compton scattering is less important for models with solar abundance of heavy elements.

  8. A wave-mechanical model of incoherent neutron scattering II. Role of the momentum transfer

    E-Print Network [OSTI]

    Frauenfelder, Hans; Fenimore, Paul W

    2015-01-01

    We recently introduced a wave-mechanical model for quasi-elastic neutron scattering (QENS) in proteins. We call the model ELM for "Energy Landscape Model". We postulate that the spectrum of the scattered neutrons consists of lines of natural width shifted from the center by fluctuations. ELM is based on two facts: Neutrons are wave packets; proteins have low-lying substates that form the free-energy landscape (FEL). Experiments suggest that the wave packets are a few hundred micrometers long. The interaction between the neutron and a proton in the protein takes place during the transit of the wave packet. The wave packet exerts the force $F(t) = dQ(t)/dt$ on the protein moiety, a part of the protein surrounding the struck proton. $Q(t)$ is the wave vector (momentum) transferred by the neutron wave packet to the proton during the transit. The ensuing energy is stored in the energy landscape and returned to the neutron as the wave packet exits. Kinetic energy thus is changed into potential energy and back. The ...

  9. Comparison of discrete and continuous thermal neutron scattering treatments in MCNP5

    SciTech Connect (OSTI)

    Pavlou, A. T. [Univ. of Michigan, Dept. of Nuclear Engineering and Radiological Sciences, 2355 Bonisteel Boulevard, Ann Arbor, MI 48109 (United States); Brown, F. B. [Los Alamos National Laboratory, Monte Carlo Codes Group, MS A143, PO Box 1663, Los Alamos, NM 87545 (United States); Martin, W. R. [Univ. of Michigan, Dept. of Nuclear Engineering and Radiological Sciences, 2355 Bonisteel Boulevard, Ann Arbor, MI 48109 (United States); Kiedrowski, B. C. [Los Alamos National Laboratory, Monte Carlo Codes Group, MS A143, PO Box 1663, Los Alamos, NM 87545 (United States)

    2012-07-01

    The standard discrete thermal neutron S({alpha},{beta}) scattering treatment in MCNP5 is compared with a continuous S({alpha},{beta}) scattering treatment using a criticality suite of 119 benchmark cases and ENDF/B-VII.0 nuclear data. In the analysis, six bound isotopes are considered: beryllium metal, graphite, hydrogen in water, hydrogen in polyethylene, beryllium in beryllium oxide and oxygen in beryllium oxide. Overall, there are only small changes in the eigenvalue (k{sub eff}) between discrete and continuous treatments. In the comparison of 64 cases that utilize S({alpha},{beta}) scattering, 62 agreed at the 95% confidence level, and the 2 cases with differences larger than 3 {sigma} agreed within 1 {sigma} when more neutrons were run in the calculations. The results indicate that the changes in eigenvalue between continuous and discrete treatments are random, small, and well within the uncertainty of measured data for reactor criticality experiments. (authors)

  10. Diffusion Processes in Water on Oxide Surfaces: Quasielastic Neutron Scattering Study of Hydration Water in Rutile Nano-Powder

    SciTech Connect (OSTI)

    Chu, Xiang-Qiang [ORNL; Ehlers, Georg [ORNL; Mamontov, Eugene [ORNL; Podlesnyak, Andrey A [ORNL; Wang, Wei [ORNL; Wesolowski, David J [ORNL

    2011-01-01

    Quasielastic neutron scattering (QENS) was used to investigate the diffusion dynamics of hydration water on the surface of rutile (TiO{sub 2}) nanopowder. The dynamics measurements utilizing two inelastic instruments, a backscattering spectrometer and a disk chopper spectrometer, probed the fast, intermediate, and slow motions of the water molecules on the time scale of picoseconds to more than a nanosecond. We employed a model-independent analysis of the data collected at each value of the scattering momentum transfer to investigate the temperature dependence of several diffusion components. All of the probed components were present in the studied temperature range of 230-320 K, providing, at a first sight, no evidence of discontinuity in the hydration water dynamics. However, a qualitative change in the elastic scattering between 240 and 250 K suggested a surface freezing-melting transition, when the motions that were localized at lower temperatures became delocalized at higher temperatures. On the basis of our previous molecular dynamics simulations of this system, we argue that interpretation of QENS data from such a complex interfacial system requires at least qualitative input from simulations, particularly when comparing results from spectrometers with very different energy resolutions and dynamic ranges.

  11. Neutron Scattering Investigation of Phonon Scattering Rates in Ag1-xSb1+xTe2+x (x = 0, 0.1, and 0.2)

    SciTech Connect (OSTI)

    Abernathy, Douglas L [ORNL; Budai, John D [ORNL; Delaire, Olivier A [ORNL; Ehlers, Georg [ORNL; Hong, Tao [ORNL; Karapetrova, Evguenia A. [Argonne National Laboratory (ANL); Ma, Jie [ORNL; May, Andrew F [ORNL; McGuire, Michael A [ORNL; Specht, Eliot D [ORNL

    2014-01-01

    The phonon dispersions and scattering rates of the thermoelectric material AgSbTe$_{2}$ were measured as a function of temperature with inelastic neutron scattering. The results show that phonon scattering rates are large and weakly dependent on temperature. The lattice thermal conductivity was calculated from the measured phonon lifetimes and group velocities, providing good agreement with bulk transport measurements. The measured phonon scattering rates and their temperature dependence are compared with models of phonon scattering by anharmonicity and point defect. We find that these processes cannot account for the large total phonon scattering rates observed, and their lack of temperature dependence. Neutron and synchrotron diffraction measurements on single crystals revealed an extensive nanostructure from cation ordering, which is likely responsible for the strong phonon scattering.

  12. Optimizing Neutron Thermal Scattering Effects in very High Temperature Reactors. Final Report

    SciTech Connect (OSTI)

    Hawari, Ayman; Ougouag, Abderrafi

    2014-07-08

    This project aims to develop a holistic understanding of the phenomenon of neutron thermalization in the VHTR. Neutron thermalization is dependent on the type and structure of the moderating material. The fact that the moderator (and reflector) in the VHTR is a solid material will introduce new and interesting considerations that do not apply in other (e.g. light water) reactors. The moderator structure is expected to undergo radiation induced changes as the irradiation (or burnup) history progresses. In this case, the induced changes in structure will have a direct impact on many properties including the neutronic behavior. This can be easily anticipated if one recognizes the dependence of neutron thermalization on the scattering law of the moderator. For the pebble bed reactor, it is anticipated that the moderating behavior can be tailored, e.g. using moderators that consist of composite materials, which could allow improved optimization of the moderator-to-fuel ratio.

  13. Discrimination of gamma rays due to inelastic neutron scattering in AGATA

    E-Print Network [OSTI]

    A. Ataç; A. Ka?ka?; S. Akkoyun; M. ?enyi?it; T. Hüyük; S. O. Kara; J. Nyberg

    2009-06-10

    Possibilities of discriminating neutrons and gamma rays in the AGATA gamma-ray tracking spectrometer have been investigated with the aim of reducing the background due to inelastic scattering of neutrons in the high-purity germanium crystals. This background may become a serious problem especially in experiments with neutron-rich radioactive ion beams. Simulations using the Geant4 toolkit and a tracking program based on the forward tracking algorithm were carried out by emitting neutrons and gamma rays from the center of AGATA. Three different methods were developed and tested in order to find 'fingerprints' of the neutron interaction points in the detectors. In a simulation with simultaneous emission of six neutrons with energies in the range 1-5 MeV and ten gamma rays with energies between 150 and 1450 keV, the peak-to-background ratio at a gamma-ray energy of 1.0 MeV was improved by a factor of 2.4 after neutron rejection with a reduction of the photopeak efficiency at 1.0 MeV of only a factor of 1.25.

  14. Texas Instruments TPS7H1101-SP Fast Neutron Irradiation Results

    E-Print Network [OSTI]

    The ATLAS collaboration

    2015-01-01

    Texas Instruments’s TPS7H1101-SP is an ultra low drop-out voltage regulator that operates under a wide range of input voltages - 1.5 to 7V. It can operate under a load of at most 3A and is radiation qualified by Texas Instruments for Total Ionizing Dose (TID) effects and Single Event Effects (SEE). For the application of the TPS7H1101-SP on the Front End Boards (FEBs) of the New Small Wheel (NSW) of the ATLAS detector, we study its susceptibility to a third kind of radiation effect -displacement damage- and present its performance in fast neutrons up to a dose of 6 x 10$^{14}$ 1MeVNE/cm$^{2}$.

  15. Importance of Compton scattering for radiation spectra of isolated neutron stars with weak magnetic fields

    E-Print Network [OSTI]

    V. Suleimanov; K. Werner

    2007-02-15

    Emergent model spectra of neutron star atmospheres are widely used to fit the observed soft X-ray spectra of different types of isolated neutron stars. We investigate the effect of Compton scattering on the emergent spectra of hot (T_eff > 10^6 K) isolated neutron stars with weak magnetic fields. In order to compute model atmospheres in hydrostatic and radiative equilibrium we solve the radiation transfer equation with the Kompaneets operator. We calculate a set of models with effective temperatures in the range 1 - 5 * 10^6 K, with two values of surface gravity (log g = 13.9 and 14.3) and different chemical compositions. Radiation spectra computed with Compton scattering are softer than those computed without Compton scattering at high energies (E > 5 keV) for light elements (H or He) model atmospheres. The Compton effect is more significant in H model atmospheres and models with low surface gravity. The emergent spectra of the hottest (T_eff > 3 * 10^6 K) model atmospheres can be described by diluted blackbody spectra with hardness factors ~ 1.6 - 1.9. Compton scattering is less important in models with solar abundance of heavy elements.

  16. Neutrino pair emission due to scattering of electrons off fluxoids in superfluid neutron star cores

    E-Print Network [OSTI]

    A. D. Kaminker; D. G. Yakovlev; P. Haensel

    1997-02-18

    We study the emission of neutrinos, resulting from the scattering of electrons off magnetic flux tubes (fluxoids) in the neutron star cores with superfluid (superconducting) protons. In the absence of proton superfluidity (T> T_{cp}), this process transforms into the well known electron synchrotron emission of neutrino pairs in a locally uniform magnetic field B, with the neutrino energy loss rate Q proportional to B^2 T^5. For temperatures T not much below T_{cp}, the synchrotron regime (Q \\propto T^5) persists and the emissivity Q can be amplified by several orders of magnitude due to the appearance of the fluxoids and associated enhancement of the field within them. For lower T, the synchrotron regime transforms into the bremsstrahlung regime (Q \\propto T^6) similar to the ordinary neutrino-pair bremsstrahlung of electrons which scatter off atomic nuclei. We calculate Q numerically and represent our results through a suitable analytic fit. In addition, we estimate the emissivities of two other neutrino-production mechanisms which are usually neglected -- neutrino-pair bremsstrahlung processes due to electron-proton and electron-electron collisions. We show that the electron-fluxoid and electron-electron scattering can provide the main neutrino production mechanisms in the neutron star cores with highly superfluid protons and neutrons at T scattering is significant if the initial, locally uniform magnetic field B > 10^{13} G.

  17. Three-dimensional magnetic spin-echo small-angle neutron scattering and neutron depolarization: A comparison

    SciTech Connect (OSTI)

    Rekveldt, M. Theo; Dijk, Niels H. van; Grigoriev, Serguei V.; Kraan, Wicher H.; Bouwman, Wim G. [Department of Radiation, Radionuclides and Reactors, Faculty of Applied Sciences, Delft University of Technology, 2629 JB Delft (Netherlands); Petersburg Nuclear Physics Institute, 188300 Gatchina, St-Petersburg District (Russian Federation); Department of Radiation, Radionuclides and Reactors, Faculty of Applied Sciences, Delft University of Technology, 2629 JB Delft (Netherlands)

    2006-07-15

    The recently developed magnetic spin-echo small-angle neutron scattering (SANS) technique provides unique information about the distance correlation of the local vector magnetization as a function of the spin-echo length within a magnetic material. The technique probes the magnetic correlations on a length scale from 10 nm up to 10 {mu}m within the bulk of a magnetic material by evaluating the Larmor precession of a polarized neutron beam in a spin-echo setup. The characteristics of the spin-echo SANS technique are discussed and compared to those of the more conventional neutron depolarization technique. Both of these techniques probe the average size of the magnetic inhomogeneities and the local magnetic texture. The magnetic spin-echo SANS technique gives information on the size distribution of these magnetic inhomogeneities perpendicular to the beam and, in principle, independent on the local magnetic induction. This information is not accessible by the neutron depolarization technique that gives the average size parallel to the beam multiplied with the square of the local magnetic induction. The basic possibilities of the magnetic spin-echo SANS technique are demonstrated by experiments on samples with a strong magnetic texture.

  18. Review of the Lujan neutron scattering center: basic energy sciences prereport February 2009

    SciTech Connect (OSTI)

    Hurd, Alan J; Rhyne, James J; Lewis, Paul S

    2009-01-01

    The Lujan Neutron Scattering Center (Lujan Center) at LANSCE is a designated National User Facility for neutron scattering and nuclear physics studies with pulsed beams of moderated neutrons (cold, thermal, and epithermal). As one of five experimental areas at the Los Alamos Neutron Science Center (LANSCE), the Lujan Center hosts engineers, scientists, and students from around the world. The Lujan Center consists of Experimental Room (ER) 1 (ERl) built by the Laboratory in 1977, ER2 built by the Office of Basic Energy Sciences (BES) in 1989, and the Office Building (622) also built by BES in 1989, along with a chem-bio lab, a shop, and other out-buildings. According to a 1996 Memorandum of Agreement (MOA) between the Defense Programs (DP) Office of the National Nuclear Security Agency (NNSA) and the Office of Science (SC, then the Office of Energy Research), the Lujan Center flight paths were transferred from DP to SC, including those in ERI. That MOA was updated in 2001. Under the MOA, NNSA-DP delivers neutron beam to the windows of the target crypt, outside of which BES becomes the 'landlord.' The leveraging nature of the Lujan Center on the LANSCE accelerator is a substantial annual leverage to the $11 M BES operating fund worth approximately $56 M operating cost of the linear accelerator (LINAC)-in beam delivery.

  19. Analysis of C-S-H gel and cement paste by small-angle neutron scattering

    SciTech Connect (OSTI)

    Allen, Andrew J. [Materials Science and Engineering Laboratory, NIST, Gaithersburg, MD 20899 (United States)]. E-mail: andrew.allen@nist.gov; Thomas, Jeffrey J. [Department of Civil and Environmental Engineering, Northwestern University, Evanston, IL 60208 (United States)]. E-mail: jthomas@northwestern.edu

    2007-03-15

    The role of small-angle X-ray and neutron scattering (SAXS and SANS) in the characterization of cement is briefly reviewed. The unique information obtainable from SANS analysis of C-S-H gel in hydrating cement is compared with that obtainable by other neutron methods. Implications for the nature of C-S-H gel, as detected by SANS, are considered in relation to current models. Finally, the application of the SANS method to cement paste is demonstrated by analyzing the effects of calcium chloride acceleration and sucrose retardation on the resulting hydrated microstructure.

  20. Mantid - Data Analysis and Visualization Package for Neutron Scattering and $\\mu SR$ Experiments

    SciTech Connect (OSTI)

    Arnold, Owen; Bilheux, Jean-Christophe; Borreguero Calvo, Jose M; Buts, Alex; Campbell, Stuart I; Doucet, Mathieu; Draper, Nicholas J; Ferraz Leal, Ricardo F; Gigg, Martyn; Lynch, Vickie E; Mikkelson, Dennis J; Mikkelson, Ruth L; Miller, Ross G; Perring, Toby G; Peterson, Peter F; Ren, Shelly; Reuter, Michael A; Savici, Andrei T; Taylor, Jonathan W; Taylor, Russell J; Zhou, Wenduo; Zikovsky, Janik L

    2014-11-01

    The Mantid framework is a software solution developed for the analysis and visualization of neutron scattering and muon spin measurements. The framework is jointly developed by a large team of software engineers and scientists at the ISIS Neutron and Muon Facility and the Oak Ridge National Laboratory. The objective of the development is to improve software quality, both in terms of performance and ease of use, for the the user community of large scale facilities. The functionality and novel design aspects of the framework are described.

  1. A wave-mechanical model of incoherent neutron scattering II. Role of the momentum transfer

    E-Print Network [OSTI]

    Hans Frauenfelder; Robert D. Young; Paul W. Fenimore

    2015-08-20

    We recently introduced a wave-mechanical model for quasi-elastic neutron scattering (QENS) in proteins. We call the model ELM for "Energy Landscape Model". We postulate that the spectrum of the scattered neutrons consists of lines of natural width shifted from the center by fluctuations. ELM is based on two facts: Neutrons are wave packets; proteins have low-lying substates that form the free-energy landscape (FEL). Experiments suggest that the wave packets are a few hundred micrometers long. The interaction between the neutron and a proton in the protein takes place during the transit of the wave packet. The wave packet exerts the force $F(t) = dQ(t)/dt$ on the protein moiety, a part of the protein surrounding the struck proton. $Q(t)$ is the wave vector (momentum) transferred by the neutron wave packet to the proton during the transit. The ensuing energy is stored in the energy landscape and returned to the neutron as the wave packet exits. Kinetic energy thus is changed into potential energy and back. The interaction energy is proportional to $Q$, not to $Q^2$. To develop and check the ELM, we use published work on dehydrated proteins after reversing improper normalizations. In such proteins only vibrations are active and the effects caused by the neutron momentum can be studied undisturbed by external fluctuations. ELM has predictive power. For example it quantitatively predicts the observed inelastic incoherent fraction $S(Q, T)$ over a broad range of temperature and momentum $Q$ with one coefficient if $S(0, T)$ is known.

  2. Influence of the Environment Fluctuations on Incoherent Neutron Scattering Functions

    E-Print Network [OSTI]

    D. J. Bicout

    2001-04-09

    In extending the conventional dynamic models, we consider a simple model to account for the environment fluctuations of particle atoms in a protein system and derive the elastic incoherent structure factor (EISF) and the incoherent scattering correlation function C(Q,t) for both the jump dynamics between sites with fluctuating site interspacing and for the diffusion inside a fluctuating sphere. We find that the EISF of the system (or the normalized elastic intensity) is equal to that in the absence of fluctuations averaged over the distribution of site interspacing or sphere radius a. The scattering correlation function is $C(Q,t)=\\sum_{n} \\psi(t)$, where the average is taken over the Q-dependent effective distribution of relaxation rates \\lambda_n(a) and \\psi(t) is the correlation function of the length a. When \\psi(t)=1, the relaxation of C(Q,t) is exponential for the jump dynamics between sites (since \\lambda_n(a) is independent of a) while it is nonexponential for diffusion inside a sphere.

  3. Quantum correlations in bulk properties of solids obtained from neutron scattering

    E-Print Network [OSTI]

    Ben-Qiong Liu; Lian-Ao Wu; Guo-Mo Zeng; Jian-Ming Song; Wei Luo; Yang Lei; Guang-Ai Sun; Bo Chen; Shu-Ming Peng

    2014-07-02

    We demonstrate that inelastic neutron scattering technique can be used to indirectly detect and measure the macroscopic quantum correlations quantified by both entanglement and discord in a quantum magnetic material, VODPO4 . 1D2O. The amount of quantum correlations is obtained 2 by analyzing the neutron scattering data of magnetic excitations in isolated V4+ spin dimers. Our quantitative analysis shows that the critical temperature of this material can reach as high as Tc = 82.5 K, where quantum entanglement drops to zero. Significantly, quantum discord can even survive at Tc = 300 K and may be used in room temperature quantum devices. Taking into account the spin-orbit (SO) coupling, we also predict theoretically that entanglement can be significantly enhanced and the critical temperature Tc increases with the strength of spin-orbit coupling.

  4. Dynamic behavior of hydration water in calcium-silicate-hydrate gel: A quasielastic neutron scattering spectroscopy investigation

    E-Print Network [OSTI]

    Li, Hua

    The translational dynamics of hydration water confined in calcium-silicate-hydrate (C-S-H) gel was studied by quasielastic neutron scattering spectroscopy in the temperature range from 280 to 230 K. The stretch exponent ...

  5. Studies of liquid-liquid phase transition and critical phenomena in supercooled confined water by neutron scattering

    E-Print Network [OSTI]

    Liu, Dazhi, Ph. D. Massachusetts Institute of Technology

    2008-01-01

    Small angle neutron scattering (SANS) is used to measure the density of water contained in 1-D cylindrical pores of a mesoporous silica material MCM-41-S. By being able to suppress the homogenous nucleation process inside ...

  6. Neutron Scattering Studies of Vortex Matter in Type-II Superconductors

    SciTech Connect (OSTI)

    Xinsheng Ling

    2012-02-02

    The proposed program is an experimental study of the fundamental properties of Abrikosov vortex matter in type-II superconductors. Most superconducting materials used in applications such as MRI are type II and their transport properties are determined by the interplay between random pinning, interaction and thermal fluctuation effects in the vortex state. Given the technological importance of these materials, a fundamental understanding of the vortex matter is necessary. The vortex lines in type-II superconductors also form a useful model system for fundamental studies of a number of important issues in condensed matter physics, such as the presence of a symmetry-breaking phase transition in the presence of random pinning. Recent advances in neutron scattering facilities such as the major upgrade of the NIST cold source and the Spallation Neutron Source are providing unprecedented opportunities in addressing some of the longstanding issues in vortex physics. The core component of the proposed program is to use small angle neutron scattering and Bitter decoration experiments to provide the most stringent test of the Bragg glass theory by measuring the structure factor in both the real and reciprocal spaces. The proposed experiments include a neutron reflectometry experiment to measure the precise Q-dependence of the structure factor of the vortex lattice in the Bragg glass state. A second set of SANS experiments will be on a shear-strained Nb single crystal for testing a recently proposed theory of the stability of Bragg glass. The objective is to artificially create a set of parallel grain boundaries into a Nb single crystal and use SANS to measure the vortex matter diffraction pattern as a function of the changing angle between the applied magnetic field to the grain boundaries. The intrinsic merits of the proposed work are a new fundamental understanding of type-II superconductors on which superconducting technology is based, and a firm understanding of phases and phase transitions in condensed matter systems with random pinning. The broader impact of the program includes the training of future generation of neutron scientists, and further development of neutron scattering and complementary techniques for studies of superconducting materials. The graduate and undergraduate students participating in this project will learn the state-of-the-art neutron scattering techniques, acquire a wide range of materials research experiences, and participate in the frontier research of superconductivity. This should best prepare the students for future careers in academia, industry, or government.

  7. Structure and dynamics of cadmium telluride studied by x-ray and inelastic neutron scattering

    SciTech Connect (OSTI)

    Niedziela, J. L., E-mail: niedzielajl@ornl.gov [Instrument and Source Division, Neutron Sciences Directorate, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831 (United States); Stone, M. B., E-mail: stonemb@ornl.gov [Quantum Condensed Matter Division, Neutron Sciences Directorate, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831 (United States)

    2014-09-08

    We present a combined study of density functional theory, x-ray diffraction, and inelastic neutron scattering examining the temperature dependent structure and lattice dynamics of commercially available cadmium telluride. A subtle change in the structure is evinced near 80?K, which manifests also in the measured phonon density of states. There is no change to the long-range ordered structure. The implications of the change in relation to structural defects are discussed.

  8. Structure and dynamics of cadmium telluride studied by x-ray and inelastic neutron scattering

    SciTech Connect (OSTI)

    Niedziela, Jennifer L [ORNL; Stone, Matthew B [ORNL

    2014-01-01

    We present a combined study of density functional theory, x-ray diffraction, and inelastic neutron scattering examining the temperature dependent structure and lattice dynamics of commercially available cadmium telluride. A subtle change in the structure is evinced near 80~K, which manifests also in the measured phonon density of states. There is no change to the long-range ordered structure. The implications of the change in relation to structural defects are discussed.

  9. Low-energy neutron-12C analyzing powers: Results from a multichannel algebraic scattering theory

    E-Print Network [OSTI]

    J. P. Svenne; K. Amos; S. Karataglidis; D. van der Knijff; L. Canton; G. Pisent

    2005-10-29

    Analyzing powers in low-energy neutron scattering from 12C are calculated in an algebraic momentum-space coupled-channel formalism (MCAS). The results are compared with recently obtained experimental data. The channel-coupling potentials have been defined previously to reproduce the total cross section and sub-threshold bound states of the compound system. Without further adjustment, good agreement with data for the analyzing powers is obtained.

  10. Recent developments in neutron-proton scattering with Lattice Effective Field Theory

    E-Print Network [OSTI]

    Jose Manuel Alarcón

    2015-11-15

    In this contribution, we show some recent progress in the study of neutron-proton scattering with Nuclear Lattice Effective Field Theory (NLEFT). We present preliminary studies of both, the uncertainties in the $np$ phase shifts extracted with NLEFT, and the lattice spacing dependence in the transfer matrix formalism. Such investigations have not been performed before in the literature, and will be relevant for Monte Carlo simulations of nuclear structure with NLEFT.

  11. Recent developments in neutron-proton scattering with Lattice Effective Field Theory

    E-Print Network [OSTI]

    Alarcón, Jose Manuel

    2015-01-01

    In this contribution, we show some recent progress in the study of neutron-proton scattering with Nuclear Lattice Effective Field Theory (NLEFT). We present preliminary studies of both, the uncertainties in the $np$ phase shifts extracted with NLEFT, and the lattice spacing dependence in the transfer matrix formalism. Such investigations have not been performed before in the literature, and will be relevant for Monte Carlo simulations of nuclear structure with NLEFT.

  12. Evidence for Narrow N*(1685) Resonance in Quasifree Compton Scattering on the Neutron

    E-Print Network [OSTI]

    V. Kuznetsov; M. V. Polyakov; V. Bellini; T. Boiko; S. Chebotarev; H. S. Dho; G. Gervino; F. Ghio; A. Giusa; A. Kim; W. Kim; F. Mammoliti; E. Milman; A. Ni; I. A. Perevalova; C. Randieri; G. Russo; M. L. Sperduto; C. M. Sutera; A. N. Vall

    2011-02-21

    The first study of quasi-free Compton scattering on the neutron in the energy range of $E_{\\gamma}=0.75 - 1.5$ GeV is presented. The data reveals a narrow peak at $W\\sim 1.685$ GeV. This result, being considered in conjunction with the recent evidence for a narrow structure at $W\\sim 1.68$GeV in the $\\eta$ photoproduction on the neutron, suggests the existence of a new nucleon resonance with unusual properties: the mass $M\\sim 1.685$GeV, the narrow width $\\Gamma \\leq 30$MeV, and the much stronger photoexcitation on the neutron than on the proton.

  13. Neutrino-nucleus coherent scattering as a probe of neutron density distributions

    E-Print Network [OSTI]

    Kelly Patton; Jonathan Engel; Gail C. McLaughlin; Nicolas Schunck

    2012-07-03

    Neutrino-nucleus coherent elastic scattering provides a theoretically appealing way to measure the neutron part of nuclear form factors. Using an expansion of form factors into moments, we show that neutrinos from stopped pions can probe not only the second moment of the form factor (the neutron radius) but also the fourth moment. Using simple Monte Carlo techniques for argon, germanium, and xenon detectors of 3.5 tonnes, 1.5 tonnes, and 300 kg, respectively, we show that the neutron radii can be found with an uncertainty of a few percent when near a neutrino flux of $3\\times10^{7}$ neutrinos/cm$^{2}$/s. If the normalization of the neutrino flux is known independently, one can determine the moments accurately enough to discriminate among the predictions of various nuclear energy functionals.

  14. Polarized Deep Inelastic Scattering Off the "Neutron" From Gauge/String Duality

    E-Print Network [OSTI]

    Jian-Hua Gao; Zong-Gang Mou

    2010-05-25

    We investigate deep inelastic scattering off the polarized "neutron" using gauge/string duality. The "neutron" corresponds to a supergravity mode of the neutral dilatino. Through introducing the Pauli interaction term into the action in $\\textrm{AdS}_{5}$ space, we calculate the polarized deep inelastic structure functions of the "neutron" in supergravity approximation at large t' Hooft coupling $\\lambda$ and finite $x$ with $\\lambda^{-1/2}\\ll xneutron" are power suppressed at the same order as the ones of the "proton." Especially, we find the Burkhardt-Cottingham-like sum rule, which is satisfied in the work by Gao and Xiao, is broken due to the Pauli interaction term. We also illustrate how such a Pauli interaction term can arise naturally from higher dimensional fermion-graviton coupling through the usual Kaluza-Klein reduction.

  15. Pore accessibility by methane and carbon dioxide in coal as determined by neutron scattering

    SciTech Connect (OSTI)

    He, Lilin [ORNL; Melnichenko, Yuri B [ORNL; Mastalerz, Maria [Indiana Geological Survey; Sakurovs, Richard [ORNL; Radlinski, Andrzej Pawell [ORNL; Blach, Tomasz P [ORNL

    2012-01-01

    Contrast-matching ultrasmall-angle neutron scattering (USANS) and small-angle neutron scattering (SANS) techniques were used for the first time to determine both the total pore volume and the fraction of the pore volume that is inaccessible to deuterated methane, CD{sub 4}, in four bituminous coals in the range of pore sizes between {approx}10 {angstrom} and {approx}5 {micro}m. Two samples originated from the Illinois Basin in the U.S.A., and the other two samples were commercial Australian bituminous coals from the Bowen Basin. The total and inaccessible porosity were determined in each coal using both Porod invariant and the polydisperse spherical particle (PDSP) model analysis of the scattering data acquired from coals both in vacuum and at the pressure of CD{sub 4}, at which the scattering length density of the pore-saturating fluid is equal to that of the solid coal matrix (zero average contrast pressure). The total porosity of the coals studied ranged from 7 to 13%, and the volume of pores inaccessible to CD{sub 4} varied from {approx}13 to {approx}36% of the total pore volume. The volume fraction of inaccessible pores shows no correlation with the maceral composition; however, it increases with a decreasing total pore volume. In situ measurements of the structure of one coal saturated with CO{sub 2} and CD{sub 4} were conducted as a function of the pressure in the range of 1-400 bar. The neutron scattering intensity from small pores with radii less than 35 {angstrom} in this coal increased sharply immediately after the fluid injection for both gases, which demonstrates strong condensation and densification of the invading subcritical CO{sub 2} and supercritical methane in small pores.

  16. Cross sections for neutron-deuteron elastic scattering in the energy range 135–250 MeV

    E-Print Network [OSTI]

    Ertan, E.

    We report new measurements of the neutron-deuteron elastic scattering cross section at energies from 135 to 250 MeV and center-of-mass angles from 80[degrees] to 130[degrees]. Cross sections for neutron-proton elastic ...

  17. Neutron and X-ray Scattering Techniques have proved so successful in condensed matter studies that a wide variety of sample environments have been developed in consquence. Many

    E-Print Network [OSTI]

    Boyer, Edmond

    Foreword Neutron and X-ray Scattering Techniques have proved so successful in condensed matter whose function is to develop and optimise the techniques appropriate to neutron scattering. Since other neutron and X-ray research centres have similar technical support groups, it was felt timely to unité

  18. Characterization of porous materials using combined small-angle X-ray and neutron scattering techniques

    SciTech Connect (OSTI)

    Hu, Naiping; Borkar, Neha; Kohls, Doug; Schaefer, Dale W. (UCIN)

    2014-09-24

    A combination of ultra small angle X-ray scattering (USAXS) and ultra small angle neutron scattering (USANS) is used to characterize porous materials. The analysis methods yield quantitative information, including the mean skeletal chord length, mean pore chord length, skeletal density, and composition. A mixed cellulose ester (MCE) membrane with a manufacturer-labeled pore size of 0.1 {mu}m was used as a model to elucidate the specifics of the method. Four approaches describing four specific scenarios (different known parameters and form of the scattering data) are compared. Pore chords determined using all four approaches are in good agreement with the scanning electron microscopy estimates but are larger than the manufacturer's nominal pore size. Our approach also gives the average chord of the skeletal solid (struts) of the membrane, which is also consistent for all four approaches. Combined data from USAXS and USANS gives the skeletal density and the strut composition.

  19. Coherent deeply virtual Compton scattering off 3He and neutron generalized parton distributions

    E-Print Network [OSTI]

    Matteo Rinaldi; Sergio Scopetta

    2014-06-18

    It has been recently proposed to study coherent deeply virtual Compton scattering (DVCS) off 3He nuclei to access neutron generalized parton distributions (GPDs). In particular, it has been shown that, in Impulse Approximation (IA) and at low momentum transfer, the sum of the quark helicity conserving GPDs of 3He, H and E, is dominated by the neutron contribution. This peculiar result makes the 3He target very promising to access the neutron information. We present here the IA calculation of the spin dependent GPD tilde-H of 3He. Also for this quantity the neutron contribution is found to be the dominant one, at low momentum transfer. The known forward limit of the IA calculation of tilde-H, yielding the polarized parton distributions of 3He, is correctly recovered. The extraction of the neutron information could be anyway non trivial, so that a procedure, able to take into account the nuclear effects encoded in the IA analysis, is proposed. These calculations, essential for the evaluation of the coherent DVCS cross section asymmetries, which depend on the GPDs H, E and tilde-H, represent a crucial step for planning possible experiments at Jefferson Lab.

  20. Differential Die-Away Instrument: Report on Fuel Assembly Mock-up Measurements with Neutron Generator

    SciTech Connect (OSTI)

    Goodsell, Alison Victoria; Swinhoe, Martyn Thomas; Henzl, Vladimir; Rael, Carlos D.; Desimone, David J.

    2014-09-18

    Fresh fuel experiments for the differential die-away (DDA) project were performed using a DT neutron generator, a 15x15 PWR fuel assembly, and nine 3He detectors in a water tank inside of a shielded cell at Los Alamos National Laboratory (LANL). Eight different fuel enrichments were created using low enriched (LEU) and depleted uranium (DU) dioxide fuel rods. A list-mode data acquisition system recorded the time-dependent signal and analysis of the DDA signal die-away time was performed. The die-away time depended on the amount of fissile material in the fuel assembly and the position of the detector. These experiments were performed in support of the spent nuclear fuel Next Generation Safeguards Initiative DDA project. Lessons learned from the fresh fuel DDA instrument experiments and simulations will provide useful information to the spent fuel project.

  1. Cross sections for neutron-deuteron elastic scattering in the energy range 135-250 MeV

    E-Print Network [OSTI]

    E. Ertan; T. Akdogan; M. B. Chtangeev; W. A. Franklin; P. A. M. Gram; M. A. Kovash; J. L. Matthews; M. Yuly

    2012-11-22

    We report new measurements of the neutron-deuteron elastic scattering cross section at energies from 135 to 250 MeV and center-of-mass angles from $80^\\circ$ to $130^\\circ$. Cross sections for neutron-proton elastic scattering were also measured with the same experimental setup for normalization purposes. Our $nd$ cross section results are compared with predictions based on Faddeev calculations including three-nucleon forces, and with cross sections measured with charged particle and neutron beams at comparable energies.

  2. Proton elastic scattering from tin isotopes at 295 MeV and systematic change of neutron density distributions

    E-Print Network [OSTI]

    S. Terashima; H. Sakaguchi; H. Takeda; T. Ishikawa; M. Itoh; T. Kawabata; T. Murakami; M. Uchida; Y. Yasuda; M. Yosoi; J. Zenihiro; H. P. Yoshida; T. Noro; T. Ishida; S. Asaji; T. Yonemura

    2008-02-02

    Cross sections and analyzing powers for proton elastic scattering from $^{116,118,120,122,124}$Sn at 295 MeV have been measured for a momentum transfer of up to about 3.5 fm$^{-1}$ to deduce systematic changes of the neutron density distribution. We tuned the relativistic Love-Franey interaction to explain the proton elastic scattering of a nucleus whose density distribution is well known. Then, we applied this interaction to deduce the neutron density distributions of tin isotopes. The result of our analysis shows the clear systematic behavior of a gradual increase in the neutron skin thickness of tin isotopes with mass number.

  3. Neutron Scattering of CeNi at the Spallation Neutron Source at Oak Ridge

    Office of Scientific and Technical Information (OSTI)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantity of NaturalDukeWakefieldSulfateSciTech Connect Nanomechanical switch for| SciTech Connect NeutronSciTech(Conference)

  4. Structure of spontaneously formed solid-electrolyte interphase on lithiated graphite determined using small-angle neutron scattering

    SciTech Connect (OSTI)

    Sacci, Robert L [ORNL; Banuelos, Jose Leo [ORNL; Veith, Gabriel M [ORNL; Littrell, Ken [ORNL; Cheng, Yongqiang [ORNL; Wildgruber, Christoph U [ORNL; Jones, Lacy L [ORNL; Ramirez-Cuesta, Anibal J [ORNL; Rother, Gernot [ORNL; Dudney, Nancy J [ORNL

    2015-01-01

    We report the first small-angle neutron scattering of a chemically formed solid-electrolyte interphase from LixC6 reacting with ethylene carbonate/dimethyl carbon solvent. This provides a different and perhaps simpler view of SEI formation than the usual electrochemically-driven reaction. We show that an organic layer coats the graphite particles filling in micro-pores and is polymeric in nature being 1-3 nm thick. We used inelastic neutron scattering to probe the chemistry, and we found that the SEI showed similar inelastic scattering to polyethylene oxide.

  5. The theory of compact and efficient circular-pore MCP neutron collimators

    E-Print Network [OSTI]

    Tremsin, A S; Feller, W B

    2006-01-01

    frequently used in neutron scattering experiments and aregeometric imperfections, neutron scattering and small anglecollimator for the neutron Brillouin scattering spectrometer

  6. Low Resolution Structure and Dynamics of a Colicin-Receptor Complex Determined by Neutron Scattering

    SciTech Connect (OSTI)

    Clifton, Luke A; Johnson, Christopher L; Solovyova, Alexandra; Callow, Phil; Weiss, Kevin L; Ridley, Helen; Le Brun, Anton P; Kinane, Christian; Webster, John; Holt, Stephen A; Lakey, Jeremy H

    2012-01-01

    Proteins that translocate across cell membranes need to overcome a significant hydrophobic barrier. This is usually accomplished via specialized protein complexes, which provide a polar transmembrane pore. Exceptions to this include bacterial toxins, which insert into and cross the lipid bilayer itself. We are studying the mechanism by which large antibacterial proteins enter Escherichia coli via specific outer membrane proteins. Here we describe the use of neutron scattering to investigate the interaction of colicin N with its outer membrane receptor protein OmpF. The positions of lipids, colicin N, and OmpF were separately resolved within complex structures by the use of selective deuteration. Neutron reflectivity showed, in real time, that OmpF mediates the insertion of colicin N into lipid monolayers. This data were complemented by Brewster Angle Microscopy images, which showed a lateral association of OmpF in the presence of colicin N. Small angle neutron scattering experiments then defined the three-dimensional structure of the colicin N-OmpF complex. This revealed that colicin N unfolds and binds to the OmpF-lipid interface. The implications of this unfolding step for colicin translocation across membranes are discussed.

  7. Gravitational waves from a test particle scattered by a neutron star: Axial mode case

    E-Print Network [OSTI]

    Kazuhiro Tominaga; Motoyuki Saijo; Kei-ichi Maeda

    1999-09-20

    Using a metric perturbation method, we study gravitational waves from a test particle scattered by a spherically symmetric relativistic star. We calculate the energy spectrum and the waveform of gravitational waves for axial modes. Since metric perturbations in axial modes do not couple to the matter fluid of the star, emitted waves for a normal neutron star show only one peak in the spectrum, which corresponds to the orbital frequency at the turning point, where the gravitational field is strongest. However, for an ultracompact star (the radius $R \\lesssim 3M$), another type of resonant periodic peak appears in the spectrum. This is just because of an excitation by a scattered particle of axial quasinormal modes, which were found by Chandrasekhar and Ferrari. This excitation comes from the existence of the potential minimum inside of a star. We also find for an ultracompact star many small periodic peaks at the frequency region beyond the maximum of the potential, which would be due to a resonance of two waves reflected by two potential barriers (Regge-Wheeler type and one at the center of the star). Such resonant peaks appear neither for a normal neutron star nor for a Schwarzschild black hole. Consequently, even if we analyze the energy spectrum of gravitational waves only for axial modes, it would be possible to distinguish between an ultracompact star and a normal neutron star (or a Schwarzschild black hole).

  8. Instrument and method for focusing x rays, gamma rays, and neutrons

    DOE Patents [OSTI]

    Smither, R.K.

    1982-03-25

    A crystal-diffraction instrument or diffraction-grating instrument is described with an improved crystalline structure or grating spacing structure having a face for receiving a beam of photons or neutrons and diffraction planar spacing or grating spacing along that face with the spacing increasing progressively along the face to provide a decreasing Bragg diffraction angle for a monochromatic radiation and thereby increasing the usable area and acceptance angle. The increased planar spacing for the diffraction crystal is provided by the use of a temperature differential across the line structures with different compositions, by an individual crystalline structure with a varying composition and thereby a changing planar spacing along its face, and by combinations of these techniques. The increased diffraction grating element spacing is generated during the fabrication of the diffraction grating by controlling the cutting tool that is cutting the grooves or controlling the laser beam, electron beam, or ion beam that is exposing the resist layer, etc. It is also possible to vary this variation in grating spacing by applying a thermal gradient to the diffraction grating in much the same manner as is done in the crystal-diffraction case.

  9. Search for Anomalous Scattering of keV Neutrons from H2O-D2O Mixtures R. Moreh,1,2,* R. C. Block,2

    E-Print Network [OSTI]

    Danon, Yaron

    Search for Anomalous Scattering of keV Neutrons from H2O-D2O Mixtures R. Moreh,1,2,* R. C. Block,2 (Received 20 January 2005; published 12 May 2005) We measured the neutron scattering intensities from pure Linac and the final energy of the scattered neutrons was fixed at 24.3 keV using a 20 cm thick pure iron

  10. Neutron Transmission, Capture, and Scattering Measurements at the Gaerttner LINAC Center Y. Danon, L. Liu, E.J. Blain, A.M. Daskalakis, B.J. McDermott, K. Ramic, C.R. Wendorff

    E-Print Network [OSTI]

    Danon, Yaron

    Neutron Transmission, Capture, and Scattering Measurements at the Gaerttner LINAC Center Y. Danon . As the energy of the neutrons increases to the keV region neutron resonance scattering becomes dominant compared to capture, and scattered neutrons can penetrate the 10 B4C liner of the NaI capture detector and get

  11. Quasi-Differential Neutron Scattering Measurements of 238 A.M. Daskalakis, R.M. Bahran, E.J. Blain, B.J. McDermott, S. Piela, and Y. Danon

    E-Print Network [OSTI]

    Danon, Yaron

    Quasi-Differential Neutron Scattering Measurements of 238 U A.M. Daskalakis, R.M. Bahran, E between evaluations through the energy-angle distribution of neutrons from scattering and fission of 238 U using the Rensselaer Polytechnic Institute (RPI) neutron scattering system. Differential neutron

  12. Neutrino-Pair Emission due to Electron-Phonon Scattering in a Neutron Star Crust

    E-Print Network [OSTI]

    D. G. Yakovlev; A. D. Kaminker

    1996-04-19

    Neutrino-pair bremsstrahlung radiation is considered due to electron--phonon scattering of degenerate, relativistic electrons in a lattice of spherical atomic nuclei in a neutron star crust. The neutrino energy generation rate is calculated taking into account exact spectrum of phonons, the Debye--Waller factor, and the nuclear form--factor in the density range from $10^7$~g~cm$^{-3}$ to $10^{14}$~g~cm$^{-3}$ at arbitrary nuclear composition for body-centered-cubic and face-centered-cubic Coulomb crystals. The results are fitted by a unified analytic expression. A comparison is given of the neutrino bremsstrahlung energy losses in a neutron star crust composed of ground state and accreted matter, in the solid and liquid phases.

  13. Exploration of deeply virtual Compton scattering on the neutron in the Hall A of Jefferson Laboratory

    SciTech Connect (OSTI)

    Malek Mazouz

    2006-12-08

    Generalized Parton Distributions (GPDs) are universal functions which provide a comprehensive description of hadron properties in terms of quarks and gluons. Deeply Virtual Compton Scattering (DVCS) is the simplest hard exclusive process involving GPDs. In particular, the DVCS on the neutron is mostly sensitive to E, the less constrained GPD, wich allows to access to the quark angular momentum. The first dedicated DVCS experiment on the neutron ran in the Hall A of Jefferson Lab in fall 2004. The high luminosity of the experiment and the resulting background rate recquired specific devices which are decribed in this document. The analysis methods and the experiment results, leading to preliminary constraints on the GPD E, are presented.

  14. X-ray and neutron scattering studies of the Rb?MnF? and Cu?â??õxMgx̳GeO? in an external magnetic field

    E-Print Network [OSTI]

    Christianson, Rebecca J. (Rebecca Jean), 1973-

    2001-01-01

    This thesis presents results of two scattering studies of low dimensional magnetic materials. The first is a neutron scattering study of Rb2MnF4, a nearly ideal two-dimensional square lattice Heisenberg antiferromagnet ...

  15. Study of Nano-Precipitates Using Small-Angle Neutron Scattering

    SciTech Connect (OSTI)

    Chen, Wei-Ren [ORNL

    2008-01-01

    Small-Angle-Neutron-Scattering (SANS) experiments were performed on a Ni-based nano-precipitate strengthened superalloy. A theoretical model for SANS absolute intensity distribution, I(Q), was developed to extract the structural properties. During the deformation process, a change in the morphology of precipitates was discovered. However, the average inter-precipitate distance and the average volume of precipitate were found to remain invariant. This microstructural information resolved by SANS is in good agreement with the results obtained from the quantitative transmission-electron-microscopy (TEM) image analysis.

  16. Deeply virtual Compton scattering on longitudinally polarized protons and neutrons at CLAS

    E-Print Network [OSTI]

    Silvia Niccolai; for the CLAS Collaboration

    2012-07-13

    This paper focuses on a measurement of deeply virtual Compton scattering (DVCS) performed at Jefferson Lab using a nearly-6-GeV polarized electron beam, two longitudinally polarized (via DNP) solid targets of protons (NH3) and deuterons (ND3) and the CEBAF Large Acceptance Spectrometer. Here, preliminary results for target-spin asymmetries and double (beam-target) asymmetries for proton DVCS, as well as a very preliminary extraction of beam-spin asymmetry for neutron DVCS, are presented and linked to Generalized Parton Distributions.

  17. Neutron Scattering Study on spin dynamics in superconducting (TlRb)2Fe4Se5

    SciTech Connect (OSTI)

    Chi, Songxue [ORNL; Ye, Feng [ORNL; Bao, Wei [Renmin University of China; Fang, Dr. Minghu [Zhejiang University; Wang, H.D. [Zhejiang University; Dong, C.H. [Zhejiang University; Savici, Andrei T [ORNL; Granroth, Garrett E [ORNL; Stone, Matthew B [ORNL; Fishman, Randy Scott [ORNL

    2013-01-01

    Spin dynamics in superconducting (Tl,Rb)2Fe4Se5 was investigated using the inelastic neutron scattering technique. Spin wave branches that span an energy range from 6.5 to 209 meV are success- fully described by a Heisenberg model whose dominant interactions include only the in-plane nearest (J1 and J0 1) and next nearest neighbor (J2 and J0 2) exchange terms within and between the tetramer spin blocks, respectively. These exchange constants, experimentally determined in this work, would crucially constrain the diverse theoretical viewpoints on magnetism and superconductivity in the Fe-based materials.

  18. Observation of spin-wave dispersion in Nd-Fe-B magnets using neutron Brillouin scattering

    SciTech Connect (OSTI)

    Ono, K. Inami, N.; Saito, K.; Takeichi, Y.; Kawana, D.; Yokoo, T.; Itoh, S.; Yano, M.; Shoji, T.; Manabe, A.; Kato, A.; Kaneko, Y.

    2014-05-07

    The low-energy spin-wave dispersion in polycrystalline Nd-Fe-B magnets was observed using neutron Brillouin scattering (NBS). Low-energy spin-wave excitations for the lowest acoustic spin-wave mode were clearly observed. From the spin-wave dispersion, we were able to determine the spin-wave stiffness constant D{sub sw} (100.0?±?4.9?meV.Å{sup 2}) and the exchange stiffness constant A (6.6 ± 0.3 pJ/m)

  19. Synthesis and characterization of nanophase zirconia : reverse micelle method and neutron scattering study.

    SciTech Connect (OSTI)

    Li, X.

    1998-11-23

    Zirconia is an important transition-metal oxide for catalytic applications. It has been widely used in automotive exhaust treatment, methanol synthesis, isomerization, alkylation, etc. [1]. Nanophase materials have unique physiochemical properties such as quantum size effects, high surface area, uniform morphology, narrow size distribution, and improvement of sintering rates[2]. Microemulsion method provides the means for controlling the microenvironment under which specific chemical reactions may occur in favoring the formation of homogeneous, nanometer-size particles. In this paper, we report the synthesis of nanophase zirconia and the characterization of the microemulsions as well as the powders by small- and wide-angle neutron scattering techniques.

  20. JOURNAL DE PHYSIQUE Colloque C2, suppl&mentau n o3, Tome 40, mars 1979,page C2-666 ?~OSSBAUE%SCATTERING AND NEUTRON SCATTEZINS ON L I Q U I D GLYCEROL

    E-Print Network [OSTI]

    Boyer, Edmond

    the temperature range, a high regolution neutron-scattering experiment was performed. There the q-range extended is obtained from the width and intensity of the quasielastic scattering. The neutron scattering experiment 0.7 A-' up to 3.5 A-' while for neutron scattering q was between 1 0.2 I-' and 2 A

  1. Neutron-Proton Scattering in the Context of the $d^*$(2380) Resonance

    E-Print Network [OSTI]

    P. Adlarson; W. Augustyniak; W. Bardan; M. Bashkanov; F. S. Bergmann; M. Ber?owski; H. Bhatt; M. Büscher; H. Calén; I. Ciepa?; H. Clement; D. Coderre; E. Czerwi?ski; K. Demmich; E. Doroshkevich; R. Engels; A. Erven; W. Erven; W. Eyrich; P. Fedorets; K. Föhl; K. Fransson; F. Goldenbaum; P. Goslawski; A. Goswami; K. Grigoryev; C. --O. Gullström; F. Hauenstein; L. Heijkenskjöld; V. Hejny; M. Hodana; B. Höistad; N. Hüsken; A. Jany; B. R. Jany; L. Jarczyk; T. Johansson; B. Kamys; G. Kemmerling; F. A. Khan; A. Khoukaz; D. A. Kirillov; S. Kistryn; H. Kleines; B. K?os; M. Krapp; W. Krzemie?; P. Kulessa; A. Kup??; K. Lalwani; D. Lersch; B. Lorentz; A. Magiera; R. Maier; P. Marciniewski; B. Maria?ski; M. Mikirtychiants; H. --P. Morsch; P. Moskal; H. Ohm; I. Ozerianska; E. Perez del Rio; N. M. Piskunov; P. Podkopa?; D. Prasuhn; A. Pricking; D. Pszczel; K. Pysz; A. Pyszniak; C. F. Redmer; J. Ritman; A. Roy; Z. Rudy; S. Sawant; S. Schadmand; T. Sefzick; V. Serdyuk; R. Siudak; T. Skorodko; M. Skurzok; J. Smyrski; V. Sopov; R. Stassen; J. Stepaniak; E. Stephan; G. Sterzenbach; H. Stockhorst; H. Ströher; A. Szczurek; A. Täschner; A. Trzci?ski; R. Varma; G. J. Wagner; M. Wolke; A. Wro?ska; P. Wüstner; P. Wurm; A. Yamamoto; L. Yurev; J. Zabierowski; M. J. Zieli?ski; A. Zink; J. Z?oma?czuk; P. {?}upra?ski; M. {?}urek; R. L. Workman; W. J. Briscoe; I. I. Strakovsky

    2014-08-21

    New data on quasifree polarized neutron-proton scattering, in the region of the recently observed $d^*$ resonance structure, have been obtained by exclusive and kinematically complete high-statistics measurements with WASA at COSY. This paper details the determination of the beam polarization, checks of the quasifree character of the scattering process, on all obtained $A_y$ angular distributions and on the new partial-wave analysis, which includes the new data producing a resonance pole in the $^3D_3$-$^3G_3$ coupled partial waves at ($2380\\pm10 - i40\\pm5$) MeV -- in accordance with the $d^*$ dibaryon resonance hypothesis. The effect of the new partial-wave solution on the description of total and differential cross section data as well as specific combinations of spin-correlation and spin-transfer observables available from COSY-ANKE measurements at $T_d$ = 2.27 GeV is discussed.

  2. Patchy worm-like micelles: solution structure studied by small-angle neutron scattering

    E-Print Network [OSTI]

    S. Rosenfeldt; F. Luedel; C. Schulreich; T. Hellweg; A. Radulescu; J. Schmelz; H. Schmalz; L. Harnau

    2012-09-20

    Triblock terpolymers exhibit a rich self-organization behavior including the formation of fascinating cylindrical core-shell structures with a phase separated corona. After crystallization-induced self-assembly of polystryrene-(block)-polyethylene-(block)-poly(methyl methacrylate) triblock terpolymers (abbreviated as SEMs = Styrene-Ethylene-Methacrylates) from solution, worm-like core-shell micelles with a patchy corona of polystryrene and poly(methyl methacrylate) were observed by transmission electron microscopy. However, the solution structure is still a matter of debate. Here, we present a method to distinguish in-situ between a Janus-type (two faced) and a patchy (multiple compartments) configuration of the corona. To discriminate between both models the scattering intensity must be determined mainly by one corona compartment. Contrast variation in small-angle neutron scattering enables us to focus on one compartment of the SEMs. The results validate the existence of the patchy structure also in solution.

  3. Recent Applications of Small-angle Neutron Scattering in Strongly Interacting Soft-condensed Matter

    SciTech Connect (OSTI)

    Wignall, George D [ORNL; Melnichenko, Yuri B [ORNL

    2005-01-01

    Before the application of small-angle neutron scattering (SANS) to the study of polymer structure, chain conformation studies were limited to light and small-angle x-ray scattering techniques, usually conducted in dilute solution owing to the difficulties of separating the inter- and intrachain contributions to the structure. The unique role of neutron scattering in soft condensed matter arises from the difference in the coherent scattering length between deuterium (b{sub D} = 0.67 x 10{sup -12} cm) and hydrogen (b{sub H} = -0.37 x 10{sup -12} cm), which results in a marked difference in scattering power (contrast) between molecules synthesized from normal (hydrogeneous) and deuterated monomer units. Thus, deuterium labelling techniques may be used to 'stain' molecules and make them 'visible' in the condensed state and other crowded environments, such as concentrated solutions of overlapping chains. For over two decades, SANS has proved to be a powerful tool for studies of structure-property relationships in polymeric systems and has made it possible to extract unique information about their size, shape, conformational changes and molecular associations. These applications are now so numerous that an exhaustive review of the field is no longer practical, so the authors propose to focus on the use of SANS for studies of strongly interacting soft matter systems. This paper will therefore discuss basic theory and practical aspects of the technique and will attempt to explain the physics of scattering with the minimum of unnecessary detail and mathematical rigour. Examples will be given to demonstrate the power of SANS and to show how it has helped to unveil universal aspects of the behaviour of macromolecules in such apparently diverse systems as polymer solutions, blends, polyelectrolytes and supercritical mixtures. The aim of the authors is to aid potential users who have a general scientific background, but no specialist knowledge of scattering, to understand the potential of the technique and, if they so choose, to apply it to provide new information in areas of their own particular research interests.

  4. Quark Structure of the Nucleon and Angular Asymmetry of Proton-Neutron Hard Elastic Scattering

    E-Print Network [OSTI]

    Carlos G. Granados; Misak M. Sargsian

    2009-07-29

    We investigate an asymmetry in the angular distribution of hard elastic proton-neutron scattering with respect to 90deg center of mass scattering angle. We demonstrate that the magnitude of the angular asymmetry is related to the helicity-isospin symmetry of the quark wave function of the nucleon. Our estimate of the asymmetry within the quark-interchange model of hard scattering demonstrates that the quark wave function of a nucleon based on the exact SU(6) symmetry predicts an angular asymmetry opposite to that of experimental observations. On the other hand the quark wave function based on the diquark picture of the nucleon produces an asymmetry consistent with the data. Comparison with the data allowed us to extract the relative sign and the magnitude of the vector and scalar diquark components of the quark wave function of the nucleon. These two quantities are essential in constraining QCD models of a nucleon. Overall, our conclusion is that the angular asymmetry of a hard elastic scattering of baryons provides a new venue in probing quark-gluon structure of baryons and should be considered as an important observable in constraining the theoretical models.

  5. Small-angle neutron scattering measurement of deuterium trapping at dislocations and grain boundaries in palladium

    SciTech Connect (OSTI)

    Heuser, B.J.

    1991-01-01

    Small angle neutron scattering measurements have been performed on deformed single and polycrystalline palladium with and without deuterium dissolved in the solution phase at room temperature. The purpose of these experiments was to directly measure the spatial distribution of trapped deuterium at dislocations in the deformed metal. The net scattering cross section for the same smaple with and without deuterium shows a behavior expected from deuterium correlation with dislocations froming rod-like scattering structures. The measured cross sections indicate the trapped deuterium is within 2 to 3 Burgers vectors of the dislocation core. On average 1 to 3 deuterons per {angstrom} are trapped at the dislocations in the deformed samples. The measurements also indicate the straight, rod-like correlation geometry extends on average 50 to 100 {angstrom} along the dislocations. Dislocation densities on the order of 5 {times} 10{sup 11} cm/cm{sup 3} were found for all samples investigated. Net scattering from a well annealed polycrystalline palladium sample exhibiting a behavior expected from spherical shells has been observed. This net scattering is attributed to deuterium trapping at grain boundaries in the polycrystalline sample. net scattering in excess of that expected from deuterium correlated at dislocations was also observed in a deformed polycrystalline measurement. This too is attributed to deuterium trapping at grain boundaries. The dislocation substructure of the deformed palladium samples was characterized by transmission electron microscopy (TEM). This analysis illustrated the cellular arrangement that evolved in palladium during cold working. The presence of MnO particles also was confirmed by TEM analysis.

  6. Faddeev calculation for breakup neutron-deuteron scattering at 14.1 MeV lab energy

    E-Print Network [OSTI]

    V M Suslov; I Filikhin; B Vlahovic; M A Braun; I Slaus

    2013-04-03

    A new computational method for solving the nucleon-deuteron breakup scattering problem has been applied to study the inelastic neutron-deuteron scattering on the basis of the configuration-space Faddeev equations. This method is based on the spline-decomposition in the angular variable and on a generalization of the Numerov method for the hyperradius. The Merkuriev-Gignoux-Laverne approach has been generalized for arbitrary nucleon-nucleon potentials and with an arbitrary number of partial waves. Neutron-deuteron observables at the incident nucleon energy 14.1 MeV have been calculated using the charge-independent AV14 nucleon-nucleon potential. Results have been compared with those of other authors and with experimental neutron-deuteron scattering data.

  7. Equilibrium Structure of a Triblock Copolymer System Revealed by Mesoscale Simulation and Neutron Scattering

    SciTech Connect (OSTI)

    Do, Changwoo [ORNL] [ORNL; Chen, Wei-Ren [ORNL] [ORNL; Hong, Kunlun [ORNL] [ORNL; Smith, Gregory Scott [ORNL] [ORNL

    2013-01-01

    We have performed both mesoscale simulations and neutron scattering experiments on Pluronic L62, a poly(ethylene oxide)-poly(propylene oxide)-poly(ethylene oxide) (PEO-PPO-PEO) triblock copolymer system in aqueous solution. The influence of simulation variables such PEO/PPO block ratio, interaction parameters, and coarse-graining methods is extensively investigated by covering all permutations of parameters found in the literatures. Upon increasing the polymer weight fraction from 50 wt% to 90 wt%, the equilibrium structure of the isotropic, reverse micellar, bicontinuous, worm-like micelle network, and lamellar phases are respectively predicted from the simulation depending on the choices of simulation parameters. Small angle neutron scattering (SANS) measurements show that the same polymer systems exhibit the spherical micellar, lamellar, and reverse micellar phases with the increase of the copolymer concentration at room temperature. Detailed structural analysis and comparison with simulations suggest that one of the simulation parameter sets can provide reasonable agreement with the experimentally observed structures.

  8. Neutron Scattering Facility for Characterization of CRESST and EURECA Detectors at mK Temperatures

    E-Print Network [OSTI]

    J. -C. Lanfranchi; C. Ciemniak; C. Coppi; F. von Feilitzsch; A. Gütlein; H. Hagn; C. Isaila; J. Jochum; M. Kimmerle; S. Pfister; W. Potzel; W. Rau; S. Roth; K. Rottler; C. Sailer; S. Scholl; I. Usherov; W. Westphal

    2008-10-01

    CRESST (Cryogenic Rare Event Search with Superconducting Thermometers) is an experiment located at the Gran Sasso underground laboratory and aimed at the direct detection of dark matter in the form of WIMPs. The setup has just completed a one year commissioning run in 2007 and is presently starting a physics run with an increased target mass. Scintillating $\\mathrm{CaWO_4}$ single crystals, operated at temperatures of a few millikelvin, are used as target to detect the tiny nuclear recoil induced by a WIMP. The powerful background identification and rejection of $\\alpha$, e$^{-}$ and $\\gamma$ events is realized via the simultaneous measurement of a phonon and a scintillation signal generated in the $\\mathrm{CaWO_4}$ crystal. However, neutrons could still be misidentified as a WIMP signature. Therefore, a detailed understanding of the individual recoil behaviour in terms of phonon generation and scintillation light emission due to scattering on Ca, O or W nuclei, respectively, is mandatory. The only setup which allows to perform such measurements at the operating temperature of the CRESST detectors has been installed at the Maier-Leibnitz-Accelerator Laboratory in Garching and is presently being commissioned. The design of this neutron scattering facility is such that it can also be used for other target materials, e.g. $\\mathrm{ZnWO_4}$, $\\mathrm{PbWO_4}$ and others as foreseen in the framework of the future multitarget tonne-scale experiment EURECA (European Underground Rare Event Calorimeter Array).

  9. Solvent contribution to the stability of a physical gel characterized by quasi-elastic neutron scattering

    E-Print Network [OSTI]

    Sylvie Spagnoli; Isabelle Morfin; Miguel A. Gonzalez; Pierre Carcabal; Marie Plazanet

    2015-02-05

    The dynamics of a physical gel, namely the Low Molecular Mass Organic Gelator {\\textit Methyl-4,6-O-benzylidene-$\\alpha$ -D-mannopyranoside ($\\alpha$-manno)} in water and toluene are probed by neutron scattering. Using high gelator concentrations, we were able to determine, on a timescale from a few ps to 1 ns, the number of solvent molecules that are immobilised by the rigid network formed by the gelators. We found that only few toluene molecules per gelator participate to the network which is formed by hydrogen bonding between the gelators' sugar moieties. In water, however, the interactions leading to the gel formations are weaker, involving dipolar, hydrophobic or $\\pi-\\pi$ interactions and hydrogen bonds are formed between the gelators and the surrounding water. Therefore, around 10 to 14 water molecules per gelator are immobilised by the presence of the network. This study shows that neutron scattering can give valuable information about the behaviour of solvent confined in a molecular gel.

  10. Development and Validation of Temperature Dependent Thermal Neutron Scattering Laws for Applications and Safety Implications in Generation IV Reactor Designs

    SciTech Connect (OSTI)

    Ayman Hawari

    2008-06-20

    The overall obljectives of this project are to critically review the currently used thermal neutron scattering laws for various moderators as a function of temperature, select as well documented and representative set of experimental data sensitive to the neutron spectra to generate a data base of benchmarks, update models and models parameters by introducing new developments in thermalization theory and condensed matter physics into various computational approaches in establishing the scattering laws, benchmark the results against the experimentatl set. In the case of graphite, a validation experiment is performed by observing nutron slowing down as a function of temperatures equal to or greater than room temperature.

  11. Characterization of Sol-gel Encapsulated Proteins using Small-angle Neutron Scattering

    SciTech Connect (OSTI)

    Luo, Guangming [ORNL; Zhang, Qiu [ORNL; Del Castillo, Alexis Rae [ORNL; Urban, Volker S [ORNL; O'Neill, Hugh Michael [ORNL

    2009-01-01

    Entrapment of biomolecules in silica-derived sol-gels has grown into a vibrant area of research since it was originally demonstrated. However, accessing the consequences of entrapment on biomolecules and the gel structure remains a major challenge in characterizing these biohybrid materials. We present the first demonstration that it is possible with small-angle neutron scattering (SANS) to study the conformation of dilute proteins that are entrapped in transparent and dense sol-gels. Using deuterium-labeled green fluorescent protein (GFP) and SANS with contrast variation, we demonstrate that the scattering signatures of the sol-gel and the protein can be separated. Analysis of the scattering curves of the sol-gels using a mass-fractal model shows that the size of the colloidal silica particles and the fractal dimensions of the gels were similar in the absence and presence of protein, demonstrating that GFP did not influence the reaction pathway for the formation of the gel. The major structural difference in the gels was that the pore size was increased 2-fold in the presence of the protein. At the contrast match point for silica, the scattering signal from GFP inside the gel became distinguishable over a wide q range. Simulated scattering curves representing a monomer, end-to-end dimer, and parallel dimer of the protein were calculated and compared to the experimental data. Our results show that the most likely structure of GFP is that of an end-to-end dimer. This approach can be readily applied and holds great potential for the structural characterization of complex biohybrid and other materials.

  12. Inelastic neutron scattering study of hydrogen in d8-THF/D2O ice clathrate Kimberly T. Tait,a

    E-Print Network [OSTI]

    Downs, Robert T.

    materials is of considerable interest from the per- spective of hydrogen storage for a future hydrogen fuelInelastic neutron scattering study of hydrogen in d8-THF/D2O ice clathrate Kimberly T. Tait,a Frans October 2007 In situ neutron inelastic scattering experiments on hydrogen adsorbed into a fully deutrated

  13. Investigation of Three-Body Force Effects in Neutron-Deuteron Scattering at 95 MeV

    SciTech Connect (OSTI)

    Mermod, P.; Blomgren, J.; Bergenwall, B.; Hildebrand, A.; Johansson, C.; Klug, J.; Oesterlund, M.; Pomp, S.; Nilsson, L.; Olsson, N.; Tippawan, U.; Jonsson, O.; Prokofiev, A.; Renberg, P.-U.; Nadel-Turonski, P.; Maeda, Y.; Sakai, H.; Tamii, A.

    2005-05-24

    We have measured the neutron-deuteron (nd) elastic-scattering differential cross section at 95 MeV incident neutron energy, using both the Medley and the SCANDAL setups at TSL in Uppsala. The full angular distribution was covered by detecting recoil deuterons from thin CD2 targets, and the result was normalized to the neutron-proton (np) cross section. Recent theories predict that three-nucleon (3N) force effects, if present, would affect the cross section in the minimum region by about 30%. The results are compared with theoretical calculations and are well described if 3N forces are included.

  14. Monte Carlo and analytical model predictions of leakage neutron exposures from passively scattered proton therapy

    SciTech Connect (OSTI)

    Pérez-Andújar, Angélica [Department of Radiation Physics, Unit 1202, The University of Texas MD Anderson Cancer Center, 1515 Holcombe Boulevard, Houston, Texas 77030 (United States)] [Department of Radiation Physics, Unit 1202, The University of Texas MD Anderson Cancer Center, 1515 Holcombe Boulevard, Houston, Texas 77030 (United States); Zhang, Rui; Newhauser, Wayne [Department of Radiation Physics, Unit 1202, The University of Texas MD Anderson Cancer Center, 1515 Holcombe Boulevard, Houston, Texas 77030 and The University of Texas Graduate School of Biomedical Sciences at Houston, 6767 Bertner Avenue, Houston, Texas 77030 (United States)] [Department of Radiation Physics, Unit 1202, The University of Texas MD Anderson Cancer Center, 1515 Holcombe Boulevard, Houston, Texas 77030 and The University of Texas Graduate School of Biomedical Sciences at Houston, 6767 Bertner Avenue, Houston, Texas 77030 (United States)

    2013-12-15

    Purpose: Stray neutron radiation is of concern after radiation therapy, especially in children, because of the high risk it might carry for secondary cancers. Several previous studies predicted the stray neutron exposure from proton therapy, mostly using Monte Carlo simulations. Promising attempts to develop analytical models have also been reported, but these were limited to only a few proton beam energies. The purpose of this study was to develop an analytical model to predict leakage neutron equivalent dose from passively scattered proton beams in the 100-250-MeV interval.Methods: To develop and validate the analytical model, the authors used values of equivalent dose per therapeutic absorbed dose (H/D) predicted with Monte Carlo simulations. The authors also characterized the behavior of the mean neutron radiation-weighting factor, w{sub R}, as a function of depth in a water phantom and distance from the beam central axis.Results: The simulated and analytical predictions agreed well. On average, the percentage difference between the analytical model and the Monte Carlo simulations was 10% for the energies and positions studied. The authors found that w{sub R} was highest at the shallowest depth and decreased with depth until around 10 cm, where it started to increase slowly with depth. This was consistent among all energies.Conclusion: Simple analytical methods are promising alternatives to complex and slow Monte Carlo simulations to predict H/D values. The authors' results also provide improved understanding of the behavior of w{sub R} which strongly depends on depth, but is nearly independent of lateral distance from the beam central axis.

  15. Characterization of the Neutron Detector Upgrade to the GP-SANS and BIO-SANS Instruments at HFIR

    SciTech Connect (OSTI)

    Berry, Kevin D [ORNL; Bailey, Katherine M [ORNL; Beal, Justin D [ORNL; Diawara, Yacouba [ORNL; Funk, Loren L [ORNL; Hicks, J Steve [ORNL; Jones, Amy Black [ORNL; Littrell, Ken [ORNL; Summers, Randy [ORNL; Urban, Volker S [ORNL; Vandergriff, David H [ORNL; Johnson, Nathan [GE Energy Services; Bradley, Brandon [GE Energy Services

    2012-01-01

    Over the past year, new 1 m x 1 m neutron detectors have been installed at both the General Purpose SANS (GP-SANS) and the Bio-SANS instruments at HFIR, each intended as an upgrade to provide improved high rate capability. This paper presents the results of characterization studies performed in the detector test laboratory, including position resolution, linearity and background, as well as a preliminary look at high count rate performance.

  16. Measurement of cross sections for inelastic cold-neutron scattering in metals and polymers by the method of (n, {gamma}) analysis

    SciTech Connect (OSTI)

    Arzumanov, S. S.; Bondarenko, L. N.; Geltenbort, P.; Morozov, V. I.; Panin, Yu. N.; Chernyavsky, S. M.

    2008-11-15

    The results obtained by measuring the cross sections for the inelastic scattering of very cold neutrons for a number of metals and polymers by the method of a neutron-irradiation analysis are presented. The method is based on simultaneously measuring events of inelastic scattering and neutron capture in the sample under investigation via recording gamma radiation with a semiconductor germanium detector. Neutron capture by a nucleus of the sample is accompanied by the prompt radiation of gamma rays having a known spectrum. Upon inelastic scattering, a neutron acquires thermal energy. Upon leaving the sample, this neutron is absorbed in a special converter that contains the isotope {sup 10}B. The capture of the neutron by a {sup 10}B nucleus is followed by the emission of a 477-keV gamma ray. The probabilities of capture and inelastic scattering are proportional to the respective neutron-interaction cross sections, and the ratio of the recorded detector counts corresponding to events of the two types does not depend on the spectrum of the incident flux of very cold neutrons or on the trajectory of neutron motion in the sample. The sought inelastic-scattering cross section at a fixed sample temperature is calculated by using this ratio and the known cross section for neutron capture by the sample isotope having a known gamma-radiation spectrum.

  17. Small Angle X-ray Scattering (SAXS) Laboratory Learning Experiences

    E-Print Network [OSTI]

    Meagher, Mary

    .A. & Svergun D.I. (1987). Structure Analysis by Small-Angle X-Ray and Neutron Scattering. NY: Plenum PressSmall Angle X-ray Scattering (SAXS) Laboratory Learning Experiences o - Use of small angle X-ray scattering instrumentation o - Programs that you will use SAXS (BRUKER AXS) PRIMUS (Konarev, Volkov, Koch

  18. NEUTRON INTERFEROMETRY Neutron Interferometry

    E-Print Network [OSTI]

    Jeanjean, Louis

    #12;NEUTRON INTERFEROMETRY #12;#12;Neutron Interferometry Lessons in Experimental Quantum Mechanics of the modern quantum mechanical literature. Neutron interferometry is a mature technique in experimental of many isotopes is given in Chapter 3. Very accurate measurements of the neutron scattering lengths

  19. Test of the consistency of various linearized semiclassical initial value time correlation functions in application to inelastic neutron scattering

    E-Print Network [OSTI]

    Miller, William H.

    -IVR is approximate. Some of the correlation functions involve only linear operators, and others involve nonlinearTest of the consistency of various linearized semiclassical initial value time correlation functions in application to inelastic neutron scattering from liquid para-hydrogen Jian Liua and William H

  20. Bending elasticity of a curved amphiphilic film decorated anchored copolymers: a small angle neutron scattering study

    E-Print Network [OSTI]

    Jacqueline Appell; Christian Ligoure; Gregoire Porte

    2004-06-30

    Microemulsion droplets (oil in water stabilized by a surfactant film) are progressively decorated with increasing amounts of poly ethylene- oxide (PEO) chains anchored in the film by the short aliphatic chain grafted at one end of the PEO chain . The evolution of the bending elasticity of the surfactant film with increasing decoration is deduced from the evolution in size and polydispersity of the droplets as reflected by small angle neutron scattering. The optimum curvature radius decreases while the bending rigidity modulus remains practically constant. The experimental results compare well with the predictions of a model developed for the bending properties of a curved film decorated by non-adsorbing polymer chains, which takes into account, the finite curvature of the film and the free diffusion of the chains on the film.

  1. Inelastic Neutron-Scattering Measurements of a Three-Dimensional Spin Resonance in the FeAs-Based BaFe1:9Ni0:1As2 Superconductor

    E-Print Network [OSTI]

    Hu, Jiangping

    Inelastic Neutron-Scattering Measurements of a Three-Dimensional Spin Resonance in the Fe, Purdue University, West Lafayette, Indiana 47907, USA 5 Neutron Scattering Science Division, Oak Ridge 2009) We use inelastic neutron scattering to study magnetic excitations of the Fe

  2. Inelastic neutron scattering of a quantum translator-rotator encapsulated in a closed fullerene cage: Isotope effects and translation-rotation coupling in H2@C60 and HD@C60

    E-Print Network [OSTI]

    Turro, Nicholas J.

    Inelastic neutron scattering of a quantum translator-rotator encapsulated in a closed fullerene, New York 10027, USA Received 1 July 2010; published 20 August 2010 We report an inelastic neutron-scattering inelastic neutron scattering INS ,6 and specific heat7 inves- tigations have recently been reported

  3. Nuclear Instruments and Methods in Physics Research A 562 (2006) 401406 Generating a multi-line neutron beam using an electron

    E-Print Network [OSTI]

    Danon, Yaron

    2006-01-01

    Nuclear Instruments and Methods in Physics Research A 562 (2006) 401­406 Generating a multi-line neutron beam using an electron Linac and a U-filter R. Moreha,b,Ã, R.C. Blockb , Y. Danonb a Physics with the steady-state filtered neutron beams obtained using nuclear reactors [1­4]. The filter materials used

  4. Ultracold neutron production and up-scattering in superfluid helium between 1.1 K and 2.4 K

    E-Print Network [OSTI]

    K. K. H. Leung; S. Ivanov; F. M. Piegsa; M. Simson; O. Zimmer

    2015-07-27

    Ultracold neutrons (UCNs) were produced in a 4 liter volume of superfluid helium using the PF1B cold neutron beam facility at the Institut Laue-Langevin and then extracted to a detector at room temperature. With a converter temperature of 1.08 K the number of accumulated UCNs was counted to be $91,\\!700 \\pm 300$. From this, we derive a volumetric UCN production rate of $(6.9 \\pm 1.7)\\,\\mathrm{cm^{-3}\\,s^{-1}}$, which includes a correction for losses in the converter during UCN extraction caused by a short storage time, but not accounting for UCN transport and detection efficiencies. The up-scattering rate of UCNs due to excitations in the superfluid was studied by scanning the temperature between 1.2-2.4 K. Using the temperature-dependent UCN production rate calculated from inelastic neutron scattering data in the analysis, the only UCN up-scattering process found to be present was from two-phonon scattering. Our analysis rules out contributions from the other scattering processes to $\\lesssim 10\\%$ of their predicted levels.

  5. Ultracold neutron production and up-scattering in superfluid helium between 1.1 K and 2.4 K

    E-Print Network [OSTI]

    Leung, K K H; Piegsa, F M; Simson, M; Zimmer, O

    2015-01-01

    Ultracold neutrons (UCNs) were produced in a 4 liter volume of superfluid helium using the PF1B cold neutron beam facility at the Institut Laue-Langevin and then extracted to a detector at room temperature. With a converter temperature of 1.08 K the number of accumulated UCNs was counted to be $91,\\!700 \\pm 300$. From this, we derive a volumetric UCN production rate of $(6.9 \\pm 1.7)\\,\\mathrm{cm^{-3}\\,s^{-1}}$, which includes a correction for losses in the converter during UCN extraction caused by a short storage time, but not accounting for UCN transport and detection efficiencies. The up-scattering rate of UCNs due to excitations in the superfluid was studied by scanning the temperature between 1.2-2.4 K. Using the temperature-dependent UCN production rate calculated from inelastic neutron scattering data in the analysis, the only UCN up-scattering process found to be present was from two-phonon scattering. Our analysis rules out contributions from the other scattering processes to $\\lesssim 10\\%$ of their ...

  6. Small-angle Neutron Scattering and Contrast Variation: A Powerful Combination for Studying Biological Structures

    SciTech Connect (OSTI)

    Heller, William T [ORNL

    2010-01-01

    The use of small-angle scattering (SAS) in the biological sciences continues to increase, driven as much by the need to study increasingly complex systems that are often resistant to crystallization or are too large for NMR as by the availability of user facilities and advancements in the modelling of biological structures from SAS data. SAS, whether with neutrons (SANS) or X-rays (SAXS), is a structural probe of length scales ranging from 10 to 10,000 {angstrom}. When applied to biological complexes in dilute solution, it provides size and shape information that can be used to produce structural models that can provide insight into function. SANS enables the use of contrast-variation methods through the unique interaction of neutrons with hydrogen and its isotope deuterium. SANS with contrast variation enables the visualization of components within multisubunit complexes, making it a powerful tool for probing protein-protein and protein-nucleic acid complexes, as well as the interaction of proteins with lipids and detergents.

  7. Neutron–proton effective mass splitting in neutron-rich matter at normal density from analyzing nucleon–nucleus scattering data within an isospin dependent optical model

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Li, Xiao -Hua; Guo, Wen -Jun; Li, Bao -An; Chen, Lie -Wen; Fattoyev, Farrukh J.; Newton, William G.

    2015-04-01

    The neutron–proton effective mass splitting in asymmetric nucleonic matter of isospin asymmetry ? and normal density is found to be m*n-p?(m*n – m*p)/m = (0.41 ± 0.15)? from analyzing globally 1088 sets of reaction and angular differential cross sections of proton elastic scattering on 130 targets with beam energies from 0.783 MeV to 200 MeV, and 1161 sets of data of neutron elastic scattering on 104 targets with beam energies from 0.05 MeV to 200 MeV within an isospin dependent non-relativistic optical potential model. It sets a useful reference for testing model predictions on the momentum dependence of the nucleonmore »isovector potential necessary for understanding novel structures and reactions of rare isotopes.« less

  8. Molecular dynamics and neutron scattering study of the dependence of polyelectrolyte dendrimer conformation on counterion behavior

    SciTech Connect (OSTI)

    Chen, Wei-Ren [ORNL; Do, Changwoo [ORNL; Egami, T [University of Tennessee, Knoxville (UTK); Hong, Kunlun [ORNL; Li, Xin [ORNL; Liu, Emily [Rensselaer Polytechnic Institute (RPI); Liu, Yun [National Institute of Standards and Technology (NIST); Porcar, L. [National Institute of Standards and Technology (NIST); Smith, Gregory Scott [ORNL; Smith, Sean C [ORNL; Wu, Bin [ORNL

    2012-01-01

    Atomistic molecular dynamics (MD) simulations and contrast variation small angle neutron scattering (SANS) technique have been used to investigate the generation-5 (G5) polyelectrolyte polyamidoamine (PAMAM) starburst dendrimer with respect to its conformational dependence on counterion behavior at different levels of molecular charge. Satisfactory agreement is seen between the simulated results, such as the excess intra-dendrimer scattering length density (SLD) distribution and hydration level, and their experimental counterparts. The conformational evolution of charged dendrimer appears to be highly dependent on the association behavior of counterion. We explore the nature of the distribution of counterions around charged amines and qualitatively account for its sensitivity to the counterion valency on the difference of excess free energy. Moreover, via extending the concept of electrical double layer for compact charged colloids, we define an effective radius of charged dendrimer based on the spatial distribution of counterions in its vicinity. Within the same framework, the correlation between the strength of intra-dendrimer electrostatic repulsion and counterion valency and dynamics is also addressed.

  9. A New On-the-Fly Sampling Method for Incoherent Inelastic Thermal Neutron Scattering Data in MCNP6

    SciTech Connect (OSTI)

    Pavlou, Andrew Theodore; Brown, Forrest B.; Ji, Wei

    2014-09-02

    At thermal energies, the scattering of neutrons in a system is complicated by the comparable velocities of the neutron and target, resulting in competing upscattering and downscattering events. The neutron wavelength is also similar in size to the target's interatomic spacing making the scattering process a quantum mechanical problem. Because of the complicated nature of scattering at low energies, the thermal data files in ACE format used in continuous-energy Monte Carlo codes are quite large { on the order of megabytes for a single temperature and material. In this paper, a new storage and sampling method is introduced that is orders of magnitude less in size and is used to sample scattering parameters at any temperature on-the-fly. In addition to the reduction in storage, the need to pre-generate thermal scattering data tables at fine temperatures has been eliminated. This is advantageous for multiphysics simulations which may involve temperatures not known in advance. A new module was written for MCNP6 that bypasses the current S(?,?) table lookup in favor of the new format. The new on-the-fly sampling method was tested for graphite for two benchmark problems at ten temperatures: 1) an eigenvalue test with a fuel compact of uranium oxycarbide fuel homogenized into a graphite matrix, 2) a surface current test with a \\broomstick" problem with a monoenergetic point source. The largest eigenvalue difference was 152pcm for T= 1200K. For the temperatures and incident energies chosen for the broomstick problem, the secondary neutron spectrum showed good agreement with the traditional S(?,?) sampling method. These preliminary results show that sampling thermal scattering data on-the-fly is a viable option to eliminate both the storage burden of keeping thermal data at discrete temperatures and the need to know temperatures before simulation runtime.

  10. Periodic magnetic fieldas a polarized and focusing thermal neutron spectrometer and monochromator

    E-Print Network [OSTI]

    2010-01-01

    Carlile, Experimental Neutron Scattering ?Oxford Universitysmall angle neutron scattering, and neutron absorptionbirefringent to neutrons, and uses scattering length b F in

  11. Characterization of a Thermo Scientific D711 D-T Neutron Generator Located in a Low-Scatter Facility

    SciTech Connect (OSTI)

    Hayes, John W.; Finn, Erin C.; Greenwood, Lawrence R.; Wittman, Richard S.

    2014-03-21

    A dosimetry experiment used to measure the neutron flux and spectrum of a D-T neutron generator is presented. The D-T generator at Pacific Northwest National Laboratory is installed in the middle of a large room to minimize scatter of neutrons back to the sample. The efficacy of maintaining a pure fast neutron field for the sample is investigated. Twenty-one positions within 13 cm of the neutron source contained foils or wires of Fe, Ni, Al with additional Au, and In monitors at some locations. Spectral adjustment of the neutron flux at each position based on measured reaction rates and theoretical Monte Carlo calculations show that at least 99.1% of the spectrum lies above 110 keV for all measured positions, and neutrons above 14 MeV can account for as much as 91% at locations along the axis of the generator and close to the source. The 14 MeV component drops to 77% in radial positions far from the source. The largest total flux observed was 8.29E+08 n/cm2-s (±1.4%) in the center of the cooling cap, although additional experiments have shown this value could be as high as 1.20E+09 n/cm2-s.

  12. Fast, Quantitative, and Nondestructive Evaluation on Hydrided LWR Fuel Cladding by Small Angle Incoherent Neutron Scattering of Hydrogen

    SciTech Connect (OSTI)

    Yan, Yong; Qian, Shuo; Littrell, Ken; Parish, Chad M; Plummer, Lee K

    2015-01-01

    A non-destructive neutron scattering method to precisely measure the uptake of hydrogen and the distribution of hydride precipitates in light water reactor (LWR) fuel cladding was developed. Zircaloy-4 cladding used in commercial LWRs was used to produce hydrided specimens. The hydriding apparatus consists of a closed stainless steel vessel that contains Zr alloy specimens and hydrogen gas. Following hydrogen charging, the hydrogen content of the hydrided specimens was measured using the vacuum hot extraction method, by which the samples with desired hydrogen concentration were selected for the neutron study. Optical microscopy shows that our hydriding procedure results in uniform distribution of circumferential hydrides across the wall. Small angle neutron incoherent scattering was performed in the High Flux Isotope Reactor at Oak Ridge National Laboratory. Our study demonstrates that the hydrogen in commercial Zircaloy-4 cladding can be measured very accurately in minutes by this nondestructive method over a wide range of hydrogen concentrations from a very small amount ( 20 ppm) to over 1000 ppm. The hydrogen distribution in a tube sample was obtained by scaling the neutron scattering rate with a factor determined by a calibration process using standard, destructive direct chemical analysis methods on the specimens. This scale factor can be used in future tests with unknown hydrogen concentrations, thus providing a nondestructive method for absolute hydrogen concentration determination.

  13. Neutron interferometric measurement of the scattering length difference between the triplet and singlet states of n-$^3$He

    E-Print Network [OSTI]

    M. G. Huber; M. Arif; W. C. Chen; T. R. Gentile; D. S. Hussey; T. C. Black; D. A. Pushin; C. B. Shahi; F. E. Wietfeldt; L. Yang

    2014-09-30

    We report a determination of the n-$^3$He scattering length difference $\\Delta b^{\\prime} = b_{1}^{\\prime}-b_{0}^{\\prime} = $ ($-5.411$ $\\pm$ $0.031$ (statistical) $\\pm$ $0.039$ (systematic)) fm between the triplet and singlet states using a neutron interferometer. This revises our previous result $\\Delta b^{\\prime} = $ (-5.610 $\\pm$ $0.027$ (statistical) $\\pm$ $0.032$ (systematic) fm obtained using the same technique in 2008. This revision is due to a re-analysis of the 2008 experiment that includes a more robust treatment of the phase shift caused by magnetic field gradients near the $^3$He cell. Furthermore, we more than doubled our original data set from 2008 by acquiring six months of additional data in 2013. Both the new data set and a re-analysis of the older data are in good agreement. Scattering lengths of low Z isotopes are valued for use in few-body nuclear effective field theories, provide important tests of modern nuclear potential models and in the case of $^3$He aid in the interpretation of neutron scattering from quantum liquids. The difference $\\Delta b^{\\prime}$ was determined by measuring the relative phase shift between two incident neutron polarizations caused by the spin-dependent interaction with a polarized $^3$He target. The target $^3$He gas was sealed inside a small, flat windowed glass cell that was placed in one beam path of the interferometer. The relaxation of $^3$He polarization was monitored continuously with neutron transmission measurements. The neutron polarization and spin flipper efficiency were determined separately using $^3$He analyzers and two different polarimetry analysis methods. A summary of the measured scattering lengths for n-$^3$He with a comparison to nucleon interaction models is given.

  14. Thermal Neutron Computed Tomography of Soil Water and Plant Roots

    E-Print Network [OSTI]

    Leanne G. Tumlinson; Hungyuan Liu; Wendy K. Silk; Jan W. Hopmans

    2007-01-01

    caused by increased neutron scattering with an increase inof beam hardening and neutron scattering could be correctedof beam hardening or neutron scattering and backscattering

  15. Instrumentation development for magneto-transport and neutron scattering measurements at high pressure and low temperature 

    E-Print Network [OSTI]

    Wang, Weiwei

    2013-07-01

    High pressure, high magnetic field and low temperature techniques are required to investigate magnetic transitions and quantum critical behaviour in different ferromagnetic materials to elucidate how novel forms of ...

  16. Neutron scattering in molecular liquids: Influence of orientational degrees of freedom and the prepeak in a fragile glass former

    E-Print Network [OSTI]

    Christoph Theis; Rolf Schilling

    1998-08-07

    The intermediate scattering function S(q,t) for neutron scattering is expanded with respect to a complete set of correlation functions which describe the dynamical correlations in a molecular liquid. For the static ns-structure factor S(q) of a system of diatomic molecules the results of the expansion are compared with the exact results from a MD-imulation and it is shown that the Sears-expansion, which is commonly used to interpret such data, fails in the supercooled regime. The representation for S(q) is used to draw conclusions about the q-dependence and especially the origin of the prepeak.

  17. Quark-Model Baryon-Baryon Interaction Applied to the Neutron-Deuteron Scattering (II) Polalization Observables of the Elastic Scattering

    E-Print Network [OSTI]

    Kenji Fukukawa; Yoshikazu Fujiwara

    2011-02-15

    The neutron-deuteron (nd) scattering is solved in the Faddeev formalism, employing the energy-independent version of the quark-model baryon-baryon interaction fss2. The differential cross sections and the spin polarization of the elastic scattering up to the neutron incident energy $E_n=65$ MeV are well reproduced without reinforcing fss2 with the three-body force. The vector analyzing-power of the neutron, $A_y(\\theta)$, in the energy region $E_n$ < 25 MeV is largely improved in comparison with the predictions by the meson-exchange potentials, thus yielding a partial solution of the long-standing $A_y$-puzzle owing to the nonlocality of the short-range repulsion produced by the quark-model baryon-baryon interaction. The large Coulomb effect in the vector and tensor analyzing-powers in $E_n$ < 10 MeV is also analyzed based on the Vincent and Phatak method and recent detailed studies by other authors.

  18. Structural formation of huntingtin-like aggregates probed by small-angle neutron scattering

    SciTech Connect (OSTI)

    Stanley, Christopher B [ORNL; Perevozchikova, Tatiana [ORNL; Berthelier-Jung, Valerie M [ORNL

    2011-01-01

    In several neurodegenerative disorders, including Huntington s disease (HD), aspects concerning the earliest of protein structures that form along the aggregation pathway have increasingly gained attention since these particular species are likely to be neurotoxic. We used time-resolved small-angle neutron scattering (SANS) to probe in solution these transient structures formed by peptides having the N-terminal sequence context of mutant huntingtin (Htt) exon 1. We obtained snapshots of the formed aggregates as the kinetic reaction ensued to yield quantitative information on their size and mass. At the early stage, small precursor species with an initial radius of gyration (Rg) of 16.1 5.9 and average mass of a dimer to trimer were monitored. Structural growth was treated as two modes with a transition from three-dimensional early aggregate formation to two-dimensional fibril growth and association. Our SANS results on the internal structure of the mature fibrils demonstrate loose packing with about 1 peptide per 4.75 -sheet repeat distance, which is shown to be quantitatively consistent with a -helix model. This research provides new insights into the structures forming along the pathway of Htt exon 1 aggregation and should assist in determining the role that precursors play in neuronal toxicity.

  19. Using Small-Angle Neutron Scattering to Detect Nanoscopic Lipid Domains

    SciTech Connect (OSTI)

    Pan, Jianjun [ORNL; Heberle, Frederick A [ORNL; Petruzielo, Robin S [Cornell University; Katsaras, John [ORNL

    2013-01-01

    The cell plasma membrane is a complex system, which is thought to be capable of exhibiting non-random lateral organization. Studies of live cells and model membranes have yielded mechanisms responsible for the formation, growth, and maintenance of nanoscopic heterogeneities, although the existence and mechanisms that give rise to these heterogeneities remain controversial. Small-angle neutron scattering (SANS) is a tool ideally suited to interrogate lateral heterogeneity in model membranes, primarily due to its unique spatial resolution (i.e., "5 100 nm) and its ability to resolve structure with minimal perturbation to the membrane. In this review we examine several methods used to analyze the SANS signal arising from freely suspended unilamellar vesicles containing lateral heterogeneity. Specifically, we discuss an analytical model for a single, round domain on a spherical vesicle. We then discuss a numerical method that uses Monte Carlo simulation to describe systems with multiple domains and/or more complicated morphologies. Also discussed are several model-independent approaches that are sensitive to membrane heterogeneity. The review concludes with several recent applications of SANS to the study of membrane raft mixtures.

  20. Multi-component modeling of quasielastic neutron scattering from phospholipid membranes

    SciTech Connect (OSTI)

    Wanderlingh, U. D’Angelo, G.; Branca, C.; Trimarchi, A.; Rifici, S.; Finocchiaro, D.; Conti Nibali, V.; Crupi, C.; Ollivier, J.; Middendorf, H. D.

    2014-05-07

    We investigated molecular motions in the 0.3–350 ps time range of D{sub 2}O-hydrated bilayers of 1-palmitoyl-oleoyl-sn-glycero-phosphocholine and 1,2-dimyristoyl-sn-glycero-phosphocholine in the liquid phase by quasielastic neutron scattering. Model analysis of sets of spectra covering scale lengths from 4.8 to 30 Å revealed the presence of three types of motion taking place on well-separated time scales: (i) slow diffusion of the whole phospholipid molecules in a confined cylindrical region; (ii) conformational motion of the phospholipid chains; and (iii) fast uniaxial rotation of the hydrogen atoms around their carbon atoms. Based on theoretical models for the hydrogen dynamics in phospholipids, the spatial extent of these motions was analysed in detail and the results were compared with existing literature data. The complex dynamics of protons was described in terms of elemental dynamical processes involving different parts of the phospholipid chain on whose motions the hydrogen atoms ride.

  1. Soluble Hydrogen-bonding Interpolymer Complexes in Water: A Small-Angle Neutron Scattering Study

    E-Print Network [OSTI]

    Maria Sotiropoulou; Julian Oberdisse; Georgios Staikos

    2006-04-03

    The hydrogen-bonding interpolymer complexation between poly(acrylic acid) (PAA) and the poly(N,N-dimethylacrylamide) (PDMAM) side chains of the negatively charged graft copolymer poly(acrylic acid-co-2-acrylamido-2-methyl-1-propane sulfonic acid)-graft-poly(N, N dimethylacrylamide) (P(AA-co-AMPSA)-g-PDMAM), containing 48 wt % of PDMAM, and shortly designated as G48, has been studied by small-angle neutron scattering in aqueous solution. Complexation occurs at low pH (pH < 3.75), resulting in the formation of negatively charged colloidal particles, consisting of PAA/PDMAM hydrogen-bonding interpolymer complexes, whose radius is estimated to be around 165 A. As these particles involve more than five graft copolymer chains, they act as stickers between the anionic chains of the graft copolymer backbone. This can explain the characteristic thickening observed in past rheological measurements with these mixtures in the semidilute solution, with decreasing pH. We have also examined the influence of pH and PAA molecular weight on the formation of these nanoparticles.

  2. Can the Neutron Polarizabilities Be Determined from a Deuteron Compton Scattering Experiment?

    E-Print Network [OSTI]

    Jonathan Karakowski; Gerald A. Miller

    1999-01-06

    A calculation of deuteron Compton scattering using non-relativistic diagrammatic perturbation theory is presented, with the primary motivation of investigating the feasibility of determining the neutron polarizabilities from this type of experiment. This calculation is expected to be valid for energies below 100 MeV. Previous theoretical and experimental estimates for the polarizabilities are given. All diagrams are calculated by expanding the photon wavefunctions into partial waves and using realistic deuteron wavefunctions. The Green's function for the intermediate state in the dispersive states is determined numerically. Pion-exchange, relativistic, and recoil corrections are also included. The low-energy theorem is shown to be satisfied. The relative effects of the different terms as well as their effects on the determinations of the polarizabilities are discussed at energies of 49, 69, and 95 MeV. The cross-section is dominated by the seagull, polarizability, and electromagnetic multipole interactions. Relativistic and pion-exchange terms are also important, while recoil corrections and multipoles of L=2 and greater are negligible. The calculation provides a reasonable description of the experimental data points at 49 and 69 MeV, except for the point at the greatest angle. The polarizabilities are difficult to determine at these energies due to the size of the experimental error bars. No data has been published at 95 MeV but a more accurate determination of the polarizabilities is likely at this higher energy. Detailed calculations for all terms can be found in the appendices.

  3. Measurement Of Neutron Radius In Lead By Parity Violating Scattering Flash ADC DAQ

    SciTech Connect (OSTI)

    Ahmed, Zafar

    2012-06-01

    This dissertation reports the experiment PREx, a parity violation experiment which is designed to measure the neutron radius in {sup 208}Pb. PREx is performed in hall A of Thomas Jefferson National Accelerator Facility from March 19th to June 21st. Longitudionally polarized electrons at energy 1 GeV scattered at and angle of {theta}{sub lab} = 5.8 {degrees} from the Lead target. Beam corrected pairty violaing counting rate asymmetry is (A{sub corr} = 594 ± 50(stat) ± 9(syst))ppb at Q{sup 2} = 0.009068GeV {sup 2}. This dissertation also presents the details of Flash ADC Data Acquisition(FADC DAQ) system for Moller polarimetry in Hall A of Thomas Jefferson National Accelerator Facility. The Moller polarimeter measures the beam polarization to high precision to meet the specification of the PREx(Lead radius experiment). The FADC DAQ is part of the upgrade of Moller polarimetery to reduce the systematic error for PREx. The hardware setup and the results of the FADC DAQ analysis are presented

  4. Structure of water in mesoporous organosilica by calorimetry and inelastic neutron scattering

    SciTech Connect (OSTI)

    Levy, Esthy [Institute of Nanotechnology Bar-Ilan University, Ramat-Gan, Israel; Kolesnikov, Alexander I [ORNL; Li, Jichen [University of Manchester, UK; Mastai, Yitzhak [Institute of Nanotechnology Bar-Ilan University, Ramat-Gan, Israel

    2009-01-01

    In this paper, we describe the preparation of mesoporous organosilica samples with hydrophilic or hydrophobic organic functionality inside the silica channel. We synthesized mesoporous organosilica of identical pore sizes based on two different organic surface functionality namely hydrophobic (based on octyltriethoxysilane OTES) and hydrophilic (3-aminopropyltriethoxysilane ATES) and MCM-41 was used as a reference system. The structure of water/ice in those porous silica samples have been investigated over a range temperatures by differential scanning calorimetry (DSC) and inelastic neutron scattering (INS). INS study revealed that water confined in hydrophobic mesoporous organosilica shows vibrational behavior strongly different than bulk water. It consists of two states: water with strong and weak hydrogen bonds (with ratio 1:2.65, respectively), compared to ice-Ih. The corresponding O-O distances in these water states are 2.67 and 2.87 ?, which strongly differ compared to ice-Ih (2.76 ?). INS spectra for water in hydrophilic mesoporous organosilica ATES show behavior similar to bulk water, but with greater degree of disorder.

  5. Status report on the analysis of inelastic neutron scattering from carbon, iron, yttrium and lead at 96 MeV

    E-Print Network [OSTI]

    C. Gustavsson; C. Hellesen; S. Pomp; A. Öhrn; J. Blomgren; U. Tippawan

    2013-03-27

    This work is part of an effort to provide more experimental data for the (n,n'x) reaction. The experiments were carried out at The Svedberg Laboratory in Uppsala, Sweden, at the quasi-mono-energetic neutron beam of 96 MeV, before the facility was upgraded in 2004. Using an extended data analysis of data primarily intended for measuring elastic neutron scattering only, it was found to be possible to extract information on the inelastic scattering from several nuclei. In the preliminary data analysis, an iterative forward-folding technique was applied, in which a physically reasonable trial spectrum was folded with the response function of the detector system and the output was compared to the experimental data. As a result, double-differential cross sections and angular distributions of inelastic neutron scattering from 12-C, 56-Fe, 89-Y and 208-Pb could be obtained. In this paper, a status update on the efforts to improve the description of the detector response function is given.

  6. MCViNE -- An object oriented Monte Carlo neutron ray tracing simulation package

    E-Print Network [OSTI]

    Lin, Jiao Y Y; Granroth, Garrett E; Abernathy, Douglas L; Lumsden, Mark D; Winn, Barry; Aczel, Adam A; Aivazis, Michael; Fultz, Brent

    2015-01-01

    MCViNE (Monte-Carlo VIrtual Neutron Experiment) is a versatile Monte Carlo (MC) neutron ray-tracing program that provides researchers with tools for performing computer modeling and simulations that mirror real neutron scattering experiments. By adopting modern software engineering practices such as using composite and visitor design patterns for representing and accessing neutron scatterers, and using recursive algorithms for multiple scattering, MCViNE is flexible enough to handle sophisticated neutron scattering problems including, for example, neutron detection by complex detector systems, and single and multiple scattering events in a variety of samples and sample environments. In addition, MCViNE can take advantage of simulation components in linear-chain-based MC ray tracing packages widely used in instrument design and optimization, as well as NumPy-based components that make prototypes useful and easy to develop. These developments have enabled us to carry out detailed simulations of neutron scatteri...

  7. The investigation of spices by use of instrumental neutron activation analysis 

    E-Print Network [OSTI]

    Wise, Jatara Rob

    2008-10-10

    .0072 null nullnullnull 5.9E-22 barns ? 7.1E+12 neutrons cm -2 s -1 null nullnullnull 46080 seconds null nullnullnullnull 0.0555 ? 2.8E-08 s -1 expected counts 541 counts expected activity 4.3E-06 ?Ci g -1 The above calculation...

  8. Dynamics of a globular protein and its hydration water studied by neutron scattering and MD simulations

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Chen, Sow-Hsin; Lagi, Marco; Chu, Xiang-qiang; Zhang, Yang; Kim, Chansoo; Faraone, Antonio; Fratini, Emiliano; Baglioni, Piero

    2010-01-01

    This review article describes our neutron scattering experiments made in the past four years for the understanding of the single-particle (hydrogen atom) dynamics of a protein and its hydration water and the strong coupling between them. We found that the key to this strong coupling is the existence of a fragile-to-strong dynamic crossover (FSC) phenomenon occurring at aroundTL= 225±5 K in the hydration water. On lowering of the temperature toward FSC, the structure of hydration water makes a transition from predominantly the high density form (HDL), a more fluid state, to predominantly the low density form (LDL), a less fluidmore »state, derived from the existence of a liquid–liquid critical point at an elevated pressure. We show experimentally that this sudden switch in the mobility of hydration water on Lysozyme, B-DNA and RNA triggers the dynamic transition, at a temperatureTD= 220 K, for these biopolymers. In the glassy state, belowTD, the biopolymers lose their vital conformational flexibility resulting in a substantial diminishing of their biological functions. We also performed molecular dynamics (MD) simulations on a realistic model of hydrated lysozyme powder, which confirms the existence of the FSC and the hydration level dependence of the FSC temperature. Furthermore, we show a striking feature in the short time relaxation (?-relaxation) of protein dynamics, which is the logarithmic decay spanning 3 decades (from ps to ns). The long time?-relaxation shows instead a diffusive behavior, which supports the liquid-like motions of protein constituents. We then discuss our recent high-resolution X-ray inelastic scattering studies of globular proteins, Lysozyme and Bovine Serum Albumin. We were able to measure the dispersion relations of collective, intra-protein phonon-like excitations in these proteins for the first time. We found that the phonon energies show a marked softening and at the same time their population increases substantially in a certain wave vector range when temperature crosses over theTD. Thus the increase of biological activities aboveTDhas positive correlation with activation of slower and large amplitude collective motions of a protein.« less

  9. New Measurement of Compton Scattering from the Deuteron and an Improved Extraction of the Neutron Electromagnetic Polarizabilities

    E-Print Network [OSTI]

    L. S. Myers; J. R. M. Annand; J. Brudvik; G. Feldman; K. G. Fissum; H. W. Grießhammer; K. Hansen; S. S. Henshaw; L. Isaksson; R. Jebali; M. A. Kovash; M. Lundin; J. A. McGovern; D. G. Middleton; A. M. Nathan; D. R. Phillips; B. Schröder; S. C. Stave

    2014-11-13

    The electromagnetic polarizabilities of the nucleon are fundamental properties that describe its response to external electric and magnetic fields. They can be extracted from Compton-scattering data --- and have been, with good accuracy, in the case of the proton. In contradistinction, information for the neutron requires the use of Compton scattering from nuclear targets. Here we report a new measurement of elastic photon scattering from deuterium using quasimonoenergetic tagged photons at the MAX IV Laboratory in Lund, Sweden. These first new data in more than a decade effectively double the world dataset. Their energy range overlaps with previous experiments and extends it by 20 MeV to higher energies. An analysis using Chiral Effective Field Theory with dynamical \\Delta(1232) degrees of freedom shows the data are consistent with and within the world dataset. After demonstrating that the fit is consistent with the Baldin sum rule, extracting values for the isoscalar nucleon polarizabilities and combining them with a recent result for the proton, we obtain the neutron polarizabilities as \\alpha_n = [11.55 +/- 1.25(stat) +/- 0.2(BSR) +/- 0.8(th)] X 10^{-4} fm^3 and \\beta_n = [3.65 -/+ 1.25(stat) +/- 0.2(BSR) -/+ 0.8(th)] X 10^{-4} fm3, with \\chi^2 = 45.2 for 44 degrees of freedom.

  10. Polarized neutron scattering investigation of excitations at low momentum transfer in liquid Ga: The mystery continues

    E-Print Network [OSTI]

    Montfrooij, Wouter

    Neutron Beam Center, Chalk River Laboratories, Chalk River KOJ 1JO, Ontario, Canada a b s t r a c ta r t i

  11. X-ray magnetic circular dichroism and small angle neutron scattering studies of thiol capped gold nanoparticles.

    SciTech Connect (OSTI)

    de la Venta, J.; Bouzas, V.; Pucci, A.; Laguna-Marco, M. A.; Haskel, D.; te Velthuis, S. G. E; Hoffmann, A.; Lal, J.; Bleuel, M.; Ruggeri, G.; de Julian Fernandez, C.; Garcia, M. A.; Univ.Complutense de Madrid; Inst. de Magnetismo Aplicado; Univ. of Pisa; Lab. di Magnetismo Molecolare

    2009-01-01

    X-ray magnetic circular dichroism (XMCD) and Small Angle Neutron Scattering (SANS) measurements were performed on thiol capped Au nanoparticles (NPs) embedded into polyethylene. An XMCD signal of 0.8 {center_dot} 10{sup -4} was found at the Au L{sub 3} edge of thiol capped Au NPs embedded in a polyethylene matrix for which Superconducting Quantum Interference Device (SQUID) magnetometry yielded a saturation magnetization, M{sub s}, of 0.06 emu/g{sub Au}. SANS measurements showed that the 3.2 nm average-diameter nanoparticles are 28% polydispersed, but no detectable SANS magnetic signal was found with the resolution and sensitivity accessible with the neutron experiment. A comparison with previous experiments carried out on Au NPs and multilayers, yield to different values between XMCD signals and magnetization measured by SQUID magnetometer. We discuss the origin of those differences.

  12. X-ray magnetic circular dichroism and small angle neutron scattering study of thiol capped gold nanoparticles.

    SciTech Connect (OSTI)

    de la Venta, J.; Bouzas, V.; Pucci, A.; Laguna-Marco, M. A.; Haskel, D.; Pinel, E. F.; te Velthuis, S. G. E.; Hoffmann, A.; Lal, J.; Bleuel, M.; Ruggeri, G.; de Julian, C.; Garcia, M. A.; Univ. Complutense de Madrid; Inst. de Magnetismo Aplicado UCM; Univ. Pisa; Univ. di Padova

    2009-11-01

    X-ray magnetic circular dichroism (XMCD) and Small Angle Neutron Scattering (SANS) measurements were performed on thiol capped Au nanoparticles (NPs) embedded into polyethylene. An XMCD signal of 0.8 {center_dot} 10{sup -4} was found at the Au L{sub 3} edge of thiol capped Au NPs embedded in a polyethylene matrix for which Superconducting Quantum Interference Device (SQUID) magnetometry yielded a saturation magnetization, M{sub s}, of 0.06 emu/g{sub Au}. SANS measurements showed that the 3.2 nm average-diameter nanoparticles are 28% polydispersed, but no detectable SANS magnetic signal was found with the resolution and sensitivity accessible with the neutron experiment. A comparison with previous experiments carried out on Au NPs and multilayers, yield to different values between XMCD signals and magnetization measured by SQUID magnetometer. We discuss the origin of those differences.

  13. Comments to the problem of experimental determination of the neutron-electron scattering length and its theoretical interpretation

    E-Print Network [OSTI]

    A. B. Popov; T. Yu. Tretyakova

    2008-12-30

    We discuss the experimental data on the n,e-scattering length bne and the values of mean square charge radius of the neutron obtained from them. It is shown that the accumulated during the last 50 years most significant experimental estimates of the bne are not contradictory and lead to the average value =-0.1178+-0.0037 fm^2. Assuming that all the authors have underestimated the errors of their measurements by a factor of 1.7, the combined fit of all available experimental data would lead to Chi^2~1 per degree of freedom. Different modern theoretical predictions of are considered. They are found to be in a good agreement with the obtained experimental value . However the existing theoretical description of the structure of neutron does not provide a value of with a sufficient accuracy.

  14. Neutron Sources for Standard-Based Testing

    SciTech Connect (OSTI)

    Radev, Radoslav; McLean, Thomas

    2014-11-10

    The DHS TC Standards and the consensus ANSI Standards use 252Cf as the neutron source for performance testing because its energy spectrum is similar to the 235U and 239Pu fission sources used in nuclear weapons. An emission rate of 20,000 ± 20% neutrons per second is used for testing of the radiological requirements both in the ANSI standards and the TCS. Determination of the accurate neutron emission rate of the test source is important for maintaining consistency and agreement between testing results obtained at different testing facilities. Several characteristics in the manufacture and the decay of the source need to be understood and accounted for in order to make an accurate measurement of the performance of the neutron detection instrument. Additionally, neutron response characteristics of the particular instrument need to be known and taken into account as well as neutron scattering in the testing environment.

  15. Nano-crystal growth in cordierite glass ceramics studied with X-ray scattering

    E-Print Network [OSTI]

    Bras, Wim

    2010-01-01

    By Small-Angle Neutron-Scattering, Electron-Paramagneticphases.. Small angle neutron scattering (SANS) experimentsand Small Angle Neutron Scattering (SANS) on some of the

  16. Investigation of coercivity mechanism in hot deformed Nd-Fe-B permanent magnets by small-angle neutron scattering

    SciTech Connect (OSTI)

    Yano, M., E-mail: masao-yano-aa@mail.toyota.co.jp; Manabe, A.; Shoji, T.; Kato, A. [Advanced Material Engineering Division, Toyota Motor Corporation, Susono 410-1193 (Japan); Ono, K. [High Energy Accelerator Research Organization (KEK), Tsukuba 305-0801 (Japan); Harada, M. [Toyota Central R and D Labs, Inc., Aichi 480-1192 (Japan); Kohlbrecher, J. [Laboratory for Neutron Scattering, Paul Scherrer Institut, 5232 Villigen PSI (Switzerland)

    2014-05-07

    The magnetic reversal behaviors of single domain sized Nd-Fe-B permanent magnets, with and without isolation between the Nd{sub 2}Fe{sub 14}B grains, was clarified using small-angle neutron scattering (SANS). The SANS patterns obtained arose from changes in the magnetic domains and were analyzed using the Teubner–Stray model, a phenomenological correlation length model, to quantify the periodicity and morphology of the magnetic domains. The results indicated that the magnetic reversal evolved with the magnetic domains that had similar sized grains. The grain isolation enabled us to realize the reversals of single domains.

  17. An effective long-range attraction between protein molecules in solutions studied by small angle neutron scattering

    E-Print Network [OSTI]

    Yun Liu; Emiliano Fratini; Piero Baglioni; Wei-Ren Chen; Sow-Hsin Chen

    2005-08-05

    Small angle neutron scattering intensity distributions taken from cytochrome C and lysozyme protein solutions show a rising intensity at very small wave vector, Q, which can be interpreted in terms of the presence of a weak long-range attraction between protein molecules. This interaction has a range several times that of the diameter of the protein molecule, much greater than the range of the screened electrostatic repulsion. We show evidence that this long-range attraction is closely related to the type of anion present and ion concentration in the solution.

  18. Differential Die-Away Instrument: Report on Neutron Detector Recovery Performance and Proposed Improvements

    SciTech Connect (OSTI)

    Goodsell, Alison Victoria; Swinhoe, Martyn Thomas; Henzl, Vladimir; Ianakiev, Kiril Dimitrov; Iliev, Metodi; Rael, Carlos D.; Desimone, David J.

    2014-09-22

    Four helium-3 (3He) detector/preamplifier packages (¾”/KM200, DDSI/PDT-A111, DDA/PDT-A111, and DDA/PDT10A) were experimentally tested to determine the deadtime effects at different DT neutron generator output settings. At very high count rates, the ¾”/KM200 package performed best. At high count rates, the ¾”/KM200 and the DDSI/PDT-A111 packages performed very well, with the DDSI/PDT-A111 operating with slightly higher efficiency. All of the packages performed similarly at mid to low count rates. Proposed improvements include using a fast recovery LANL-made dual channel preamplifier, testing smaller diameter 3He tubes, and further investigating quench gases.

  19. Effect of heat treatment on pore structure in nano-crystalline NiO: A small angle neutron scattering study

    SciTech Connect (OSTI)

    Bahadur, J. [Solid State Physics Division, Bhabha Atomic Research Centre, Mumbai 400085 (India)], E-mail: jbahadur@barc.gov.in; Sen, D.; Mazumder, S. [Solid State Physics Division, Bhabha Atomic Research Centre, Mumbai 400085 (India); Ramanathan, S. [Materials Science Division, Bhabha Atomic Research Centre, Mumbai 400085 (India)

    2008-05-15

    Nano-crystalline nickel oxide powder was synthesized by a precipitation route. Powder samples were heat treated at 300, 600 and 900 deg. C, and pore structure evolution was followed by small angle neutron scattering (SANS) technique. SANS measurements were carried out also on pelleted samples in order to study the modifications of pore morphology due to heat treatment. SANS data reveal scattering from pores at two different length scales. The pore structure at various heat treatment temperatures does not follow any scaling behavior. - Graphical abstract: SEM micrograph shows the microstructure of the nano-crystalline NiO. An average agglomerate size of {approx}1 {mu}m is evident from SEM and LS. SANS profiles for the samples heat treated at 300, 600 and 900 deg. C, respectively, are shown. A significant variation in the profile shape due to the modification in the intra-agglomerate pore structure under heat treatment is visible.

  20. Phonon self-energy and origin of anomalous neutron scattering spectra in SnTe and PbTe thermoelectrics

    SciTech Connect (OSTI)

    Li, Chen [ORNL] [ORNL; Ma, Jie [ORNL] [ORNL; May, Andrew F [ORNL] [ORNL; Cao, Huibo [ORNL] [ORNL; Christianson, Andrew D [ORNL] [ORNL; Ehlers, Georg [ORNL] [ORNL; Singh, David J [ORNL] [ORNL; Sales, Brian C [ORNL] [ORNL; Delaire, Olivier A [ORNL] [ORNL

    2014-01-01

    The anharmonic lattice dynamics of rock-salt thermoelectric compounds SnTe and PbTe are investigated with inelastic neutron scattering (INS) and first-principles calculations. The experiments show that, surprisingly, although SnTe is closer to the ferroelectric instability, phonon spectra in PbTe exhibit a more anharmonic character. This behavior is reproduced in first-principles calculations of the temperature-dependent phonon self-energy. Our simulations reveal how the nesting of phonon dispersions induces prominent features in the self-energy, which account for the measured INS spectra and their temperature dependence. We establish that the phase-space for three-phonon scattering processes, rather than just the proximity to the lattice instability, is the mechanism determining the complex spectrum of the transverse-optical ferroelectric mode.

  1. A Survey of Students from the National School on Neutron and X-ray Scattering: Communication Habits and Preferences

    SciTech Connect (OSTI)

    Bryant, Rebecca [Bryant Research, LLC

    2010-12-01

    Oak Ridge National Laboratory (ORNL) offers the scientific community unique access to two types of world-class neutron sources at a single site - the Spallation Neutron Source (SNS) and the High Flux Isotope Reactor (HFIR). The 85-MW HFIR provides one of the highest steady-state neutron fluxes of any research reactor in the world. And the SNS is one of the world's most intense pulse neutron beams. Management of these resources is the responsibility of the Neutron Sciences Directorate (NScD). NScD started conducting the National School on Neutron and X-ray Scattering (NXS) in conjunction with the Advanced Photon Source (APS) at Argonne National Laboratory in 2007. This survey was conducted to determine the most effective ways to reach students with information about what SNS and HFIR offer the scientific community, including content and communication vehicles. The emphasis is on gaining insights into compelling messages and the most effective channels, e.g., Web sites and social media, for communicating with students about neutron science The survey was conducted in two phases using a classic qualitative investigation to confirm language and content followed by a survey designed to quantify issues, assumptions, and working hypotheses. Phase I consisted of a focus group in late June 2010 with students attending NXS. The primary intent of the group was to inform development of an online survey. Phase two consisted of an online survey that was developed and pre-tested in July 2010 and launched on August 9, 2010 and remained in the field until September 9, 2010. The survey achieved an overall response rate of 48% for a total of 157 completions. The objective of this study is to determine the most effective ways to reach students with information about what SNS and HFIR offer the scientific community, including content and communication vehicles. The emphasis is on gaining insights into compelling messages and the most effective channels, e.g., Web sites, social media, for communicating with students about neutron science.

  2. Measurement of the structure function of the nearly free neutron using spectator tagging in inelastic $^2$H(e, e'p)X scattering with CLAS

    E-Print Network [OSTI]

    S. Tkachenko; N. Baillie; S. E. Kuhn; J. Zhang; J. Arrington; P. Bosted; S. Bültmann; M. E. Christy; D. Dutta; R. Ent; H. Fenker; K. A. Griffioen; M. Ispiryan; N. Kalantarians; C. E. Keppel; W. Melnitchouk; V. Tvaskis; K. P. Adhikari; M. Aghasyan; M. J. Amaryan; S. Anefalos Pereira; H. Avakian; J. Ball; N. A. Baltzell; M. Battaglieri; I. Bedlinskiy; A. S. Biselli; W. J. Briscoe; W. K. Brooks; V. D. Burkert; D. S. Carman; A. Celentano; S. Chandavar; G. Charles; P. L. Cole; M. Contalbrigo; O. Cortes; V. Crede; A. D'Angelo; N. Dashyan; R. De Vita; E. De Sanctis; A. Deur; C. Djalali; G. E. Dodge; D. Doughty; R. Dupre; H. Egiyan; A. El Alaoui; L. El Fassi; L. Elouadrhiri; P. Eugenio; G. Fedotov; J. A. Fleming; B. Garillon; N. Gevorgyan; Y. Ghandilyan; G. P. Gilfoyle; K. L. Giovanetti; F. X. Girod; J. T. Goetz; E. Golovatch; R. W. Gothe; M. Guidal; L. Guo; K. Hafidi; H. Hakobyan; C. Hanretty; N. Harrison; M. Hattawy; K. Hicks; D. Ho; M. Holtrop; C . E. Hyde; Y. Ilieva; D. G. Ireland; B. S. Ishkhanov; H. S. Jo; D. Keller; M. Khandaker; A. Kim; W. Kim; P. M. King; A. Klein; F. J. Klein; S. Koirala; V. Kubarovsky; S. V. Kuleshov; P. Lenisa; S. Lewis; K. Livingston; H. Lu; M. MacCormick; I. J. D. MacGregor; N. Markov; M. Mayer; B. McKinnon; T. Mineeva; M. Mirazita; V. Mokeev; R. A. Montgomery; H. Moutarde; C. Munoz Camacho; P. Nadel-Turonski; S. Niccolai; G. Niculescu; I. Niculescu; M. Osipenko; L. L. Pappalardo; R. Paremuzyan; K. Park; E. Pasyuk; J. J. Phillips; S. Pisano; O. Pogorelko; S. Pozdniakov; J. W. Price; S. Procureur; D. Protopopescu; A. J . R. Puckett; D. Rimal; M. Ripani; A. Rizzo; G. Rosner; P. Rossi; P. Roy; F. Sabatié; D. Schott; R. A. Schumacher; E. Seder; I. Senderovich; Y. G. Sharabian; A. Simonyan; G. D. Smith; D. I. Sober; D. Sokhan; S. Stepanyan; S. S. Stepanyan; S. Strauch; W. Tang; M. Ungaro; A. V. Vlassov; H. Voskanyan; E. Voutier; N. K. Walford; D. Watts; X. Wei; L. B. Weinstein; M. H. Wood; L. Zana; I. Zonta

    2014-10-03

    Much less is known about neutron structure than that of the proton due to the absence of free neutron targets. Neutron information is usually extracted from data on nuclear targets such as deuterium, requiring corrections for nuclear binding and nucleon off-shell effects. These corrections are model dependent and have significant uncertainties, especially for large values of the Bjorken scaling variable x. The Barely Off-shell Nucleon Structure (BONuS) experiment at Jefferson Lab measured the inelastic electron deuteron scattering cross section, tagging spectator protons in coincidence with the scattered electrons. This method reduces nuclear binding uncertainties significantly and has allowed for the first time a (nearly) model independent extraction of the neutron structure function. A novel compact radial time projection chamber was built to detect protons with momentum between 70 and 150 MeV/c. For the extraction of the free neutron structure function $F_{2n}$, spectator protons at backward angle and with momenta below 100 MeV/c were selected, ensuring that the scattering took place on a nearly free neutron. The scattered electrons were detected with Jefferson Lab's CLAS spectrometer. The extracted neutron structure function $F_{2n}$ and its ratio to the deuteron structure function $F_{2d}$ are presented in both the resonance and deep inelastic regions. The dependence of the cross section on the spectator proton momentum and angle is investigated, and tests of the spectator mechanism for different kinematics are performed. Our data set can be used to study neutron resonance excitations, test quark hadron duality in the neutron, develop more precise parametrizations of structure functions, as well as investigate binding effects (including possible mechanisms for the nuclear EMC effect) and provide a first glimpse of the asymptotic behavior of d/u as x goes to 1.

  3. SMALL-ANGLE NEUTRON SCATTERING CHARACTERIZATION OF THE STRUCTURE OF NANOPOROUS CARBONS FOR ENERGY-RELATED APPLICATIONS

    SciTech Connect (OSTI)

    He, Lilin [ORNL; Mavila Chathoth, Suresh [ORNL; Melnichenko, Yuri B [ORNL; Presser, Volker [Drexel University; Mcdonough, John [Drexel University; Gogotsi, Yury G. [Drexel University

    2011-01-01

    We used small-angle neutron scattering (SANS) and neutron contrast variation to study the structure of four nanoporouscarbons prepared by thermo-chemical etching of titanium carbide TiC in chlorine at 300, 400, 600, and 800 C with pore diameters ranging between -4 and -11 {angstrom}. SANS patterns were obtained from dry samples and samples saturated with deuterium oxide (D{sub 2}O) in order to delineate origin of the power law scattering in the low Q domain as well as to evaluate pore accessibility for D{sub 2}O molecules. SANS cross section of all samples was fitted to Debye-Anderson-Brumberger (DAB), DAB-Kirste-Porod models as well as to the Guinier and modified Guinier formulae for cylindrical objects, which allowed for evaluating the radii of gyration as well as the radii and lengths of the pores under cylindrical shape approximation. SANS data from D{sub 2}O-saturated samples indicate that strong upturn in the low Q limit usually observed in the scattering patterns from microporous carbon powders is due to the scattering from outer surface of the powder particles. Micropores are only partially filled with D{sub 2}O molecules due to geometrical constraints and or partial hydrophobicity of the carbon matrix. Structural parameters of the dry carbons obtained using SANS are compared with the results of the gas sorption measurements and the values agree for carbide-derived carbons (CDCs) obtained at high chlorination temperatures (>600 C). For lower chlorination temperatures, pore radii obtained from gas sorption overestimate the actual pore size as calculated from SANS for two reasons: inaccessible small pores are present and the model-dependent fitting based on density functional theory models assumes non-spherical pores, whereas SANS clearly indicates that the pore shape in microporous CDC obtained at low chlorination temperatures is nearly spherical.

  4. Anharmonic lattice dynamics of Ag2O studied by inelastic neutron scattering and first-principles molecular dynamics simulations

    SciTech Connect (OSTI)

    Lan, Tian [California Institute of Technology, Pasadena] [California Institute of Technology, Pasadena; Li, Chen [ORNL] [ORNL; Niedziela, Jennifer L [ORNL] [ORNL; Smith, Hillary [California Institute of Technology, Pasadena] [California Institute of Technology, Pasadena; Abernathy, Douglas L [ORNL] [ORNL; Rossman, George [California Institute of Technology, Pasadena] [California Institute of Technology, Pasadena; Fultz, B. [California Institute of Technology, Pasadena] [California Institute of Technology, Pasadena

    2014-01-01

    Inelastic neutron scattering measurements on silver oxide (Ag2O) with the cuprite structure were performed at temperatures from 40 to 400 K, and Fourier transform far-infrared spectra were measured from 100 to 300 K. The measured phonon densities of states and the infrared spectra showed unusually large energy shifts with temperature, and large linewidth broadenings. First principles molecular dynamics (MD) calculations were performed at various temperatures, successfully accounting for the negative thermal expansion (NTE) and local dynamics. Using the Fourier-transformed velocity autocorrelation method, the MD calculations reproduced the large anharmonic effects of Ag2O, and were in excellent agreement with the neutron scattering data. The quasiharmonic approximation (QHA) was less successful in accounting for much of the phonon behavior. The QHA could account for some of the NTE below 250 K, although not at higher temperatures. Strong anharmonic effects were found for both phonons and for the NTE. The lifetime broadenings of Ag2O were explained by anharmonic perturbation theory, which showed rich interactions between the Ag-dominated modes and the O-dominated modes in both up- and down-conversion processes.

  5. Adsorption of Supercritical CO2 in Aeroglass Studied by Small--Angle Neutron Scattering and Neutron Transmission Techniques

    SciTech Connect (OSTI)

    Melnichenko, Yuri B [ORNL; Wignall, George D [ORNL; Cole, David R [ORNL; Frielinghaus, H. [Forschungszentrum Julich, Julich, Germany

    2006-01-01

    Small-angle neutron scattering (SANS) has been used to study the adsorption behavior of supercritical carbon dioxide (CO{sub 2}) in porous Vycor glass and silica aerogels. Measurements were performed along two isotherms (T = 35 and 80 C) as a function of pressure (P) ranging from atmospheric up to 25 MPa, which corresponds to the bulk fluid densities ranging from {rho}CO{sub 2} - 0 to 0.9 g/cm{sup 3}. The intensity of scattering from CO{sub 2}-saturated Vycor porous glass can be described by a two-phase model which suggests that CO{sub 2} does not adsorb on the pore walls and fills the pore space uniformly. In CO{sub 2}-saturated aerogels an adsorbed phase is formed with a density substantially higher that of the bulk fluid, and neutron transmission data were used to monitor the excess adsorption at different pressures. The results indicate that adsorption of CO{sub 2} is significantly stronger in aerogels than in activated carbons, zeolites, and xerogels due to the extremely high porosity and optimum pore size of these materials. SANS data revealed the existence of a compressed adsorbed phase with the average density - 1.07 g/cm{sup 3}, close to the density corresponding to closely packed van der Waals volume of CO{sub 2}. A three-phase model [W. L. Wu, Polymer 23, 1907 (1982)] was used to estimate the volume fraction {phi}{sub 3} of the adsorbed phase as a function of the fluid density, and gave {phi}{sub 3} - 0.78 in the maximum adsorption regime around {rho}CO{sub 2} - 0.374 g/cm{sup 3}. The results presented in this work demonstrate the utility of SANS combined with the transmission measurements to study the adsorption of supercritical fluids in porous materials.

  6. Secondary neutron spectrum from 250-MeV passively scattered proton therapy: Measurement with an extended-range Bonner sphere system

    SciTech Connect (OSTI)

    Howell, Rebecca M.; Burgett, E. A.

    2014-09-15

    Purpose: Secondary neutrons are an unavoidable consequence of proton therapy. While the neutron dose is low compared to the primary proton dose, its presence and contribution to the patient dose is nonetheless important. The most detailed information on neutrons includes an evaluation of the neutron spectrum. However, the vast majority of the literature that has reported secondary neutron spectra in proton therapy is based on computational methods rather than measurements. This is largely due to the inherent limitations in the majority of neutron detectors, which are either not suitable for spectral measurements or have limited response at energies greater than 20 MeV. Therefore, the primary objective of the present study was to measure a secondary neutron spectrum from a proton therapy beam using a spectrometer that is sensitive to neutron energies over the entire neutron energy spectrum. Methods: The authors measured the secondary neutron spectrum from a 250-MeV passively scattered proton beam in air at a distance of 100 cm laterally from isocenter using an extended-range Bonner sphere (ERBS) measurement system. Ambient dose equivalent H*(10) was calculated using measured fluence and fluence-to-ambient dose equivalent conversion coefficients. Results: The neutron fluence spectrum had a high-energy direct neutron peak, an evaporation peak, a thermal peak, and an intermediate energy continuum between the thermal and evaporation peaks. The H*(10) was dominated by the neutrons in the evaporation peak because of both their high abundance and the large quality conversion coefficients in that energy interval. The H*(10) 100 cm laterally from isocenter was 1.6 mSv per proton Gy (to isocenter). Approximately 35% of the dose equivalent was from neutrons with energies ?20?MeV. Conclusions: The authors measured a neutron spectrum for external neutrons generated by a 250-MeV proton beam using an ERBS measurement system that was sensitive to neutrons over the entire energy range being measured, i.e., thermal to 250 MeV. The authors used the neutron fluence spectrum to demonstrate experimentally the contribution of neutrons with different energies to the total dose equivalent and in particular the contribution of high-energy neutrons (?20 MeV). These are valuable reference data that can be directly compared with Monte Carlo and experimental data in the literature.

  7. Neutron inelastic scattering and reactions in natural Pb as a background in neutrinoless double-beta-decay experiments

    E-Print Network [OSTI]

    V. E. Guiseppe; M. Devlin; S. R. Elliott; N. Fotiades; A. Hime; D. -M. Mei; R. O. Nelson; D. V. Perepelitsa

    2009-09-24

    Inelastic neutron scattering and reactions on Pb isotopes can result in gamma rays near the signature endpoint energy in a number of double-beta decay isotopes. In particular, there are gamma-ray transitions in Pb-206,207,208 that might produce energy deposits at the 76-Ge Q value in Ge detectors used for double-beta decay searches. The levels that produce these gamma rays can be excited by (n,n'gamma) or (n,xngamma) reactions, but the cross sections are small and previously unmeasured. This work uses the pulsed neutron beam at the Los Alamos Neutron Science Center to directly measure reactions of interest to double-beta decay experiments. The cross section on natural Pb to produce the 2041-keV gamma ray from Pb-206 is measured to be 3.6 +/- 0.7 (stat.) +/- 0.3 (syst.) mb at ~9.6 MeV. The cross section on natural Pb to produce the 3062-keV gamma ray from Pb-207 and Pb-208 is measured to be 3.9 +/- 0.8 (stat.) +/- 0.4 (syst.) mb at the same energy. We report cross sections or place upper limits on the cross sections for exciting some other levels in Pb that have transition energies corresponding to Q value in other double-beta decay isotopes.

  8. Scattering Density Profile Model of POPG Bilayers as Determined by Molecular Dynamics Simulations and Small-Angle Neutron and X-ray Scattering Experiments

    SciTech Connect (OSTI)

    Kucerka, Norbert [Canadian Neutron Beam Centre and Comelius University (Slovakia); Holland, B [University of Guelph; Gray, C.G [University of Guelph; Tomberli, B [Brandon University; Katsaras, John [ORNL

    2012-01-01

    We combine molecular dynamics (MD) simulations and experiment, both small-angle neutron (SANS) and small-angle X-ray scattering (SAXS), to determine the precise structure of bilayers composed of 1-palmitoyl-2-oleoyl-sn-glycero-3-phosphatidylglycerol (POPG), a lipid commonly encountered in bacterial membranes. Experiment and simulation are used to develop a one-dimensional scattering density profile (SDP) model suitable for the analysis of experimental data. The joint refinement of such data (i.e., SANS and SAXS) results in the area per lipid that is then used in the fixed-area simulations. In the final step, the direct comparison of simulated-to-experimental data gives rise to the detailed structure of POPG bilayers. From these studies we conclude that POPG s molecular area is 66.0 +/- 1.3 ^2, its overall bilayer thickness is 36.7 +/- 0.7 , and its hydrocarbon region thickness is 27.9 ( 0.6 , assuming a simulated value of 1203 ^3 for the total lipid volume.

  9. Structural and magnetic properties of transition metal substituted BaFe{sub 2}As{sub 2} compounds studied by x-ray and neutron scattering

    SciTech Connect (OSTI)

    Kim, Min Gyu [Ames Laboratory

    2012-08-28

    The purpose of my dissertation is to understand the structural and magnetic properties of the newly discovered FeAs-based superconductors and the interconnection between superconductivity, antiferromagnetism, and structure. X-ray and neutron scattering techniques are powerful tools to directly observe the structure and magnetism in this system. I used both xray and neutron scattering techniques on di#11;erent transition substituted BaFe2As2 compounds in order to investigate the substitution dependence of structural and magnetic transitions and try to understand the connections between them.

  10. Instrument performance on the short and long pulse second SNS target stations

    SciTech Connect (OSTI)

    Zhao, Jinkui [ORNL; Herwig, Kenneth W [ORNL; Robertson, Lee [ORNL; Gallmeier, Franz X [ORNL; Riemer, Bernie [ORNL

    2013-01-01

    In this work, we investigate the effect of neutron moderator dimensions on the performance of neutron scattering instruments at the Spallation Neutron Source. In a recent study of the planned second target station at the Spallation Neutron Source (SNS) facility [1,2], we have found that the dimensions of a moderator play a significant role in determining its surface brightness. A smaller moderator may be significantly brighter for a smaller viewing area [4]. One of the immediate implications of this finding is that for modern neutron scattering instrument designs, moderator dimensions and brightness have to be incorporated as an integrated optimization parameter. Here, we establish a strategy of matching neutron scattering instruments with moderators using analytical and Monte Carlo techniques. In order to simplify our treatment, we group the instruments into two broad categories, those with natural collimation and those that use neutron guide systems. We found that the cross-sections of the sample and the neutron guide, respectively, are the deciding factors for choosing the moderator. Beam divergence plays no role as long as it is within the reach of practical constraints. Namely, the required divergence is not too large for the guide or sample to be located close enough to the moderator on an actual spallation source.

  11. Measuring the Noble Metal and Iodine Composition of Extracted Noble Metal Phase from Spent Nuclear Fuel Using Instrumental Neutron Activation Analysis

    SciTech Connect (OSTI)

    Palomares, R. I.; Dayman, Kenneth J.; Landsberger, Sheldon; Biegalski, Steven R.; Soderquist, Chuck Z.; Casella, Amanda J.; Brady Raap, Michaele C.; Schwantes, Jon M.

    2015-04-01

    Mass quantities of noble metal and iodine nuclides in the metallic noble metal phase extracted from spent fuel are measured using instrumental neutron activation analysis (NAA). Nuclide presence is predicted using fission yield analysis, and mass quantification is derived from standard gamma spectroscopy and radionuclide decay analysis. The nuclide compositions of noble metal phase derived from two dissolution methods, UO2 fuel dissolved in nitric acid and UO2 fuel dissolved in ammonium-carbonate and hydrogen-peroxide solution, are compared. Lastly, the implications of the rapid analytic speed of instrumental NAA are discussed in relation to potential nuclear forensics applications.

  12. Fast neutron scattering on Gallium target at 14.8 MeV

    E-Print Network [OSTI]

    R. Han; R. Wada; Z. Chen; Y. Nie; X. Liu; S. Zhang; P. Ren; B. Jia; G. Tian; F. Luo; W. Lin; J. Liu; F. Shi; M. Huang; X. Ruan; J. Ren; Z. Zhou; H. Huang; J. Bao; K. Zhang; B. Hu

    2014-11-03

    Benchmarking of evaluated nuclear data libraries was performed for $\\sim 14.8$ MeV neutrons on Gallium targets. The experiments were performed at China Institute of Atomic Energy(CIAE). Solid samples of natural Gallium (3.2 cm and 6.4 cm thick) were bombarded by $\\sim 14.8$ MeV neutrons and leakage neutron energy spectra were measured at 60$^{\\circ}$ and 120$^{\\circ}$. The measured spectra are rather well reproduced by MCNP-4C simulations with the CENDL-3.1, ENDF/B-VII and JENDL-4.0 evaluated nuclear data libraries, except for the inelastic contributions around $E_{n} = 10-13$ MeV. All three libraries significantly underestimate the inelastic contributions. The inelastic contributions are further studied, using the Talys simulation code and the experimental spectra are reproduced reasonably well in the whole energy range by the Talys calculation, including the inelastic contributions.

  13. Scattering of particles by neutron stars: Time-evolutions for axial perturbations

    E-Print Network [OSTI]

    V. Ferrari; K. D. Kokkotas

    2000-08-23

    The excitation of the axial quasi-normal modes of a relativistic star by scattered particles is studied by evolving the time dependent perturbation equations. This work is the first step towards the understanding of more complicated perturbative processes, like the capture or the scattering of particles by rotating stars. In addition, it may serve as a test for the results of the full nonlinear evolution of binary systems.

  14. Lipid Bilayer Structure Determined by the Simultaneous Analysis of Neutron and X-Ray Scattering Data

    E-Print Network [OSTI]

    Nagle, John F.

    Jackson,** and John Katsaras*yyzz *Canadian Neutron Beam Centre, National Research Council, Chalk River River Laboratories, Chalk River, Ontario K0J 1J0, Canada; **National Institute of Standards; { Department of Chemistry, Wabash College, Crawfordsville, Indiana 47933; k Atomic Energy of Canada, Chalk

  15. Binary and ternary cluster integrals of polymer segments as determined by small angle neutron scattering

    E-Print Network [OSTI]

    Paris-Sud XI, Université de

    -ku, Tokyo, Japan E. Wada, K. Kurita, H. Hiramatsu and H. Fukuro College of Science and Technology, NihonL-171 Binary and ternary cluster integrals of polymer segments as determined by small angle neutron integrals of polymer segments in these semi-dilute, poor solvent, solutions. In the present note we show

  16. Dipolar structures in magnetite ferrofluids studied with small-angle neutron scattering with and without applied magnetic field

    SciTech Connect (OSTI)

    Klokkenburg, M.; Erne, B. H.; Petukhov, A. V.; Philipse, A. P. [Van 't Hoff Laboratory for Physical and Colloid Chemistry, Debye Institute, Utrecht University, Padualaan 8, 3584 CH Utrecht (Netherlands); Wiedenmann, A. [Hahn-Meitner-Institut Berlin, Department SF3, Glienickerstrasse 100, D-14109 Berlin (Germany)

    2007-05-15

    Field-induced structure formation in a ferrofluid with well-defined magnetite nanoparticles with a permanent magnetic dipole moment was studied with small-angle neutron scattering (SANS) as a function of the magnetic interactions. The interactions were tuned by adjusting the size of the well-defined, single-magnetic-domain magnetite (Fe{sub 3}O{sub 4}) particles and by applying an external magnetic field. For decreasing particle dipole moments, the data show a progressive distortion of the hexagonal symmetry, resulting from the formation of magnetic sheets. The SANS data show qualitative agreement with recent cryogenic transmission electron microscopy results obtained in 2D [Klokkenburg et al., Phys. Rev. Lett. 97, 185702 (2006)] on the same ferrofluids.

  17. Structural Investigation of PAMAM Dendrimers in Aqueous Solutions Using Small-Angle Neutron Scattering: Effect of Generation

    SciTech Connect (OSTI)

    Chen, Wei-Ren [ORNL

    2008-01-01

    We investigate a series of poly(amidoamine) starburst dendrimers (PAMAM) of different generations in acidic, aqueous solutions using small-angle neutron scattering (SANS). While the overall molecular size is found to be practically unaffected by a pD change, a strong generational dependence of counterion association is revealed. Upon increasing the dendrimer generation, the effective charge obtained from our SANS experiments only shows a small increase in contrast to the nearly exponential increase predicted by a recent atomic simulation. We also find that with the same degree of molecular protonation the specific counterion association, which is defined as the ratio of bound chloride anions to positively charged amines in solutions, is larger for higher-generation PAMAM dendrimer. The associated counterion density also increases upon increasing generation number.

  18. Probing the Room Temperature Spatial Distribution of Hydrogen in Nanoporous Carbon by Use of Small-Angle Neutron Scattering

    SciTech Connect (OSTI)

    Tsao, Cheng-Si [Massachusetts Institute of Technology (MIT); Li, Mingda [ORNL; Zhang, Yang [ORNL; Leao, Juscelino B [ORNL; Chiang, Wei-Shan [ORNL; Chung, Tsui-Yun [Institute of Nuclear Energy Research, Taiwan; Tzeng, Yi-Ren [Institute of Nuclear Energy Research, Taiwan; Chen, Sow-hsin H [ORNL

    2010-01-01

    The spatial distribution of hydrogen physically adsorbed in a nanoporous carbon at room temperature (RT) as a function of H2 gas pressure is investigated for the first time using small-angle neutron scattering (SANS). A hierarchical pore structure consisting of micropores and a fractal mesopore network of the used activated carbon is also studied to correlate the relationship between the spatial distribution of hydrogen and the pore confinement. The cylinder-like cluster of aggregated hydrogen is formed and is confined in the disklike micropore. The evolution of spatial structures of adsorbed hydrogen with hydrogen pressure is elucidated. A direct experimental observation of the spatial distribution and the behavior of hydrogen adsorbed in the porous materials at RT is still scarce to date. The analysis results obtained by SANS provide new information for the future investigations of the RT storage mechanism of hydrogen in the nanoporous materials developed for the purpose of on-board hydrogen storage.

  19. Small-Angle Neutron Scattering study of solubilization of tributyl phosphate in aqueous solutions of L64 Pluronic triblock copolymers

    E-Print Network [OSTI]

    Jeremy Causse; Julian Oberdisse; Jacques Jestin; Serge Lagerge

    2010-12-04

    We have studied the solubilization behaviour of tributylphosphate (TBP) in aqueous solutions of L64-Pluronics, using light and small angle neutron scattering (SANS). Varying the temperature and the oil-content, the system presents a non trivial phase behaviour. In particular, at 308K, a first solubilization followed by an emulsification failure and a resolubilization is found. We have measured the microstructure by SANS and characterized the microemulsion droplet core-size, corona-thickness, polydispersity, and interactions. It is shown that at low oil content, the system is made of small swollen micelles. After the phase separation, the resolubilization is carried by larger oil droplets decorated by copolymer. From specific surface measurements at large angles, a surprising change in surfactant conformation is found to accompany this morphological evolution which is also supported by previous results obtained from 1H NMR experiments. In independent measurements, our structural modelling is confirmed using contrast-variation SANS.

  20. Microemulsion nanocomposites: phase diagram, rheology and structure using a combined small angle neutron scattering and reverse Monte Carlo approach

    E-Print Network [OSTI]

    Nicolas Puech; Serge Mora; Ty Phou; Gregoire Porte; Jacques Jestin; Julian Oberdisse

    2010-12-04

    The effect of silica nanoparticles on transient microemulsion networks made of microemulsion droplets and telechelic copolymer molecules in water is studied, as a function of droplet size and concentration, amount of copolymer, and nanoparticle volume fraction. The phase diagram is found to be affected, and in particular the percolation threshold characterized by rheology is shifted upon addition of nanoparticles, suggesting participation of the particles in the network. This leads to a peculiar reinforcement behaviour of such microemulsion nanocomposites, the silica influencing both the modulus and the relaxation time. The reinforcement is modelled based on nanoparticles connected to the network via droplet adsorption. Contrast-variation Small Angle Neutron Scattering coupled to a reverse Monte Carlo approach is used to analyse the microstructure. The rather surprising intensity curves are shown to be in good agreement with the adsorption of droplets on the nanoparticle surface.

  1. Q-dependence of the inelastic neutron scattering cross section for molecular spin clusters with high molecular symmetry

    E-Print Network [OSTI]

    O. Waldmann

    2003-04-21

    For powder samples of polynuclear metal complexes the dependence of the inelastic neutron scattering intensity on the momentum transfer Q is known to be described by a combination of so called interference terms. They reflect the interplay between the geometrical structure of the compound and the spatial properties of the wave functions involved in the transition. In this work, it is shown that the Q-dependence is strongly interrelated with the molecular symmetry of molecular nanomagnets, and, if the molecular symmetry is high enough, is actually completely determined by it. A general formalism connecting spatial symmetry and interference terms is developed. The arguments are detailed for cyclic spin clusters, as experimentally realized by e.g. the octanuclear molecular wheel Cr8, and the star like tetranuclear cluster Fe4.

  2. Electric dipole response of 208Pb from proton inelastic scattering: constraints on neutron skin thickness and symmetry energy

    E-Print Network [OSTI]

    A. Tamii; P. von Neumann-Cosel; I. Poltoratska

    2013-10-02

    The electric dipole (E1) response of 208Pb has been precisely determined by measuring Coulomb excitation induced by proton scattering at very forward angles. The electric dipole polarizability, defined as inverse energy-weighted sum rule of the E1 strength, has been extracted as 20.1+-0.6 fm^3. The data can be used to constrain the neutron skin thickness of 208Pb to 0.168(+-0.009)_expt(+-0.013)_theo(+-0.021)_est fm, where the subscript "expt" refers to the experimental uncertainty, "theor" to the theoretical confidence band and "est" to the uncertainty associated with the estimation of the symmetry energy at the saturation density. In addition, a constraint band has been extracted in the plane of the symmetry energy (J) and its slope parameter (L) at the saturation density.

  3. VOLUME 75, NUMBER 2 P H Y S I C A L R E V I E W L E T T E R S 10 JULY 1995 Phonon and Magnetic Neutron Scattering at 41 meV in YBa2Cu3O7

    E-Print Network [OSTI]

    Aksay, Ilhan A.

    Neutron Scattering at 41 meV in YBa2Cu3O7 Hung Fai Fong, B. Keimer, and P. W. Anderson Department is the generalized magnetic susceptibility whose imaginary part x00 q, v is measur- able by neutron scattering. Below to be of mag- netic origin in polarized neutron scattering experiments by Mook et al. [2]. (We quote the in

  4. Polarized inelastic neutron scattering of the partially ordered Tb2Sn2O7 K. C. Rule,1 G. Ehlers,2 J. R. Stewart,3 A. L. Cornelius,4 P. P. Deen,3 Y. Qiu,5,6 C. R. Wiebe,7,8 J. A. Janik,7 H. D. Zhou,7

    E-Print Network [OSTI]

    Weston, Ken

    Polarized inelastic neutron scattering of the partially ordered Tb2Sn2O7 K. C. Rule,1 G. Ehlers,2 J 17 August 2007; published 21 December 2007 We present inelastic neutron scattering results neutron scattering, susceptibility, and specific heat techniques have shown that below 0.87 K Tb2Sn2O7

  5. A Measurement of the neutron electric form factor at very large momentum transfer using polaried electrions scattering from a polarized helium-3 target

    SciTech Connect (OSTI)

    Aidan Kelleher

    2010-10-01

    Knowledge of the electric and magnetic elastic form factors of the nucleon is essential for an understanding of nucleon structure. Of the form factors, the electric form factor of the neutron has been measured over the smallest range in Q{sup 2} and with the lowest precision. Jefferson Lab experiment 02-013 used a novel new polarized {sup 3}He target to nearly double the range of momentum transfer in which the neutron form factor has been studied and to measure it with much higher precision. Polarized electrons were scattered off this target, and both the scattered electron and neutron were detected. G{sup n}{sub E} was measured to be 0.0242 ± 0.0020(stat) ± 0.0061(sys) and 0.0247 ± 0.0029(stat) ± 0.0031(sys) at Q{sup 2} = 1.7 and 2.5 GeV{sup 2}, respectively.

  6. SU-E-T-591: Measurement and Monte Carlo Simulation of Stray Neutrons in Passive Scattering Proton Therapy: Needs and Challenges

    SciTech Connect (OSTI)

    Farah, J; Bonfrate, A; Donadille, L; Dubourg, N; Lacoste, V; Martinetti, F; Sayah, R; Trompier, F; Clairand, I [IRSN - Institute for Radiological Protection and Nuclear Safety, Fontenay-aux-roses (France); Caresana, M [Politecnico di Milano, Milano (Italy); Delacroix, S; Nauraye, C [Institut Curie - Centre de Protontherapie d Orsay, Orsay (France); Herault, J [Centre Antoine Lacassagne, Nice (France); Piau, S; Vabre, I [Institut de Physique Nucleaire d Orsay, Orsay (France)

    2014-06-01

    Purpose: Measure stray radiation inside a passive scattering proton therapy facility, compare values to Monte Carlo (MC) simulations and identify the actual needs and challenges. Methods: Measurements and MC simulations were considered to acknowledge neutron exposure associated with 75 MeV ocular or 180 MeV intracranial passively scattered proton treatments. First, using a specifically-designed high sensitivity Bonner Sphere system, neutron spectra were measured at different positions inside the treatment rooms. Next, measurement-based mapping of neutron ambient dose equivalent was fulfilled using several TEPCs and rem-meters. Finally, photon and neutron organ doses were measured using TLDs, RPLs and PADCs set inside anthropomorphic phantoms (Rando, 1 and 5-years-old CIRS). All measurements were also simulated with MCNPX to investigate the efficiency of MC models in predicting stray neutrons considering different nuclear cross sections and models. Results: Knowledge of the neutron fluence and energy distribution inside a proton therapy room is critical for stray radiation dosimetry. However, as spectrometry unfolding is initiated using a MC guess spectrum and suffers from algorithmic limits a 20% spectrometry uncertainty is expected. H*(10) mapping with TEPCs and rem-meters showed a good agreement between the detectors. Differences within measurement uncertainty (10–15%) were observed and are inherent to the energy, fluence and directional response of each detector. For a typical ocular and intracranial treatment respectively, neutron doses outside the clinical target volume of 0.4 and 11 mGy were measured inside the Rando phantom. Photon doses were 2–10 times lower depending on organs position. High uncertainties (40%) are inherent to TLDs and PADCs measurements due to the need for neutron spectra at detector position. Finally, stray neutrons prediction with MC simulations proved to be extremely dependent on proton beam energy and the used nuclear models and cross sections. Conclusion: This work highlights measurement and simulation limits for ion therapy radiation protection applications.

  7. Small-angle neutron scattering reveals the assembly mode and oligomeric architecture of TET, a large, dodecameric aminopeptidase

    SciTech Connect (OSTI)

    Appolaire, Alexandre; Girard, Eric; Colombo, Matteo; Durá, M. Asunción [Université Grenoble Alpes, IBS, 38044 Grenoble (France); CNRS, IBS, 38044 Grenoble (France); CEA, IBS, 38044 Grenoble (France); Moulin, Martine; Härtlein, Michael [Institut Laue–Langevin, 38042 Grenoble CEDEX 9 (France); Franzetti, Bruno [Université Grenoble Alpes, IBS, 38044 Grenoble (France); CNRS, IBS, 38044 Grenoble (France); CEA, IBS, 38044 Grenoble (France); Gabel, Frank, E-mail: frank.gabel@ibs.fr [Université Grenoble Alpes, IBS, 38044 Grenoble (France); CNRS, IBS, 38044 Grenoble (France); CEA, IBS, 38044 Grenoble (France); Institut Laue–Langevin, 38042 Grenoble CEDEX 9 (France)

    2014-11-01

    The present work illustrates that small-angle neutron scattering, deuteration and contrast variation, combined with in vitro particle reconstruction, constitutes a very efficient approach to determine subunit architectures in large, symmetric protein complexes. In the case of the 468 kDa heterododecameric TET peptidase machine, it was demonstrated that the assembly of the 12 subunits is a highly controlled process and represents a way to optimize the catalytic efficiency of the enzyme. The specific self-association of proteins into oligomeric complexes is a common phenomenon in biological systems to optimize and regulate their function. However, de novo structure determination of these important complexes is often very challenging for atomic-resolution techniques. Furthermore, in the case of homo-oligomeric complexes, or complexes with very similar building blocks, the respective positions of subunits and their assembly pathways are difficult to determine using many structural biology techniques. Here, an elegant and powerful approach based on small-angle neutron scattering is applied, in combination with deuterium labelling and contrast variation, to elucidate the oligomeric organization of the quaternary structure and the assembly pathways of 468 kDa, hetero-oligomeric and symmetric Pyrococcus horikoshii TET2–TET3 aminopeptidase complexes. The results reveal that the topology of the PhTET2 and PhTET3 dimeric building blocks within the complexes is not casual but rather suggests that their quaternary arrangement optimizes the catalytic efficiency towards peptide substrates. This approach bears important potential for the determination of quaternary structures and assembly pathways of large oligomeric and symmetric complexes in biological systems.

  8. The quantum nature of the OH stretching mode in ice and water probed by neutron scattering experiments

    SciTech Connect (OSTI)

    Senesi, Roberto; Flammini, Davide; Kolesnikov, Alexander I; Murray, Eamonn D.; Galli, Giulia; Andreani, Carla

    2013-01-01

    The OH stretching vibrational spectrum of water was measured in a wide range of temperatures across the triple point, 269 K < T < 296 K, using Inelastic Neutron Scattering (INS). The hydrogen projected density of states and the proton mean kinetic energy, _OH, were determined for the first time within the framework of a harmonic description of the proton dynamics. We found that in the liquid the value of _OH is nearly constant as a function of T, indicating that quantum effects on the OH stretching frequency are weakly dependent on temperature. In the case of ice, ab initio electronic structure calculations, using non-local van der Waals functionals, provided _OH values in agreement with INS experiments. We also found that the ratio of the stretching (_OH) to the total (_exp) kinetic energy, obtained from the present measurements, increases in going from ice, where hydrogen bonding is the strongest, to the liquid at ambient conditions and then to the vapour phase, where hydrogen bonding is the weakest. The same ratio was also derived from the combination of previous deep inelastic neutron scattering data, which does not rely upon the harmonic approximation, and the present measurements. We found that the ratio of stretching to the total kinetic energy shows a minimum in the metastable liquid phase. This finding suggests that the strength of intermolecular interactions increases in the supercooled phase, with respect to that in ice, contrary to the accepted view that supercooled water exhibits weaker hydrogen bonding than ice.

  9. Determination of Low-Energy Parameters of Neutron--Proton Scattering on the Basis of Modern Experimental Data from Partial-Wave Analyses

    E-Print Network [OSTI]

    V. A. Babenko; N. M. Petrov

    2007-04-08

    The triplet and singlet low-energy parameters in the effective-range expansion for neutron--proton scattering are determined by using the latest experimental data on respective phase shifts from the SAID nucleon--nucleon database. The results differ markedly from the analogous parameters obtained on the basis of the phase shifts of the Nijmegen group and contradict the parameter values that are presently used as experimental ones. The values found with the aid of the phase shifts from the SAID nucleon--nucleon database for the total cross section for the scattering of zero-energy neutrons by protons, $\\sigma_{0}=20.426 $b, and the neutron--proton coherent scattering length, $f=-3.755 $fm, agree perfectly with the experimental cross-section values obtained by Houk, $\\sigma_{0}=20.436\\pm 0.023 $b, and experimental scattering-length values obtained by Houk and Wilson, $f=-3.756\\pm 0.009 $fm, but they contradict cross-section values of $\\sigma_{0}=20.491\\pm 0.014 $b according to Dilg and coherent-scattering-length values of $f=-3.7409\\pm 0.0011 $fm according to Koester and Nistler.

  10. Nanosecond molecular relaxations in lipid bilayers studied by high energy resolution neutron scattering and in-situ diffraction

    E-Print Network [OSTI]

    Maikel C. Rheinstädter; Tilo Seydel; Tim Salditt

    2006-07-20

    We report a high energy-resolution neutron backscattering study to investigate slow motions on nanosecond time scales in highly oriented solid supported phospholipid bilayers of the model system DMPC -d54 (deuterated 1,2-dimyristoyl-sn-glycero-3-phoshatidylcholine), hydrated with heavy water. Wave vector resolved quasi-elastic neutron scattering (QENS) is used to determine relaxation times $\\tau$, which can be associated with different molecular components, i.e., the lipid acyl chains and the interstitial water molecules in the different phases of the model membrane system. The inelastic data are complemented both by energy resolved and energy integrated in-situ diffraction. From a combined analysis of the inelastic data in the energy and time domain, the respective character of the relaxation, i.e., the exponent of the exponential decay is also determined. From this analysis we quantify two relaxation processes. We associate the fast relaxation with translational diffusion of lipid and water molecules while the slow process likely stems from collective dynamics.

  11. FINAL REPORT: DOE CONTRACT NUMBER FG0205ER64026 Biological Neutron Scattering: A Collaboration with the Oak Ridge Center for Structural Molecular Biology

    SciTech Connect (OSTI)

    Jill Trewhella

    2011-01-12

    The overarching goal of this project was to promote applications of small-angle scattering in structural molecular biology by providing model examples of cutting edge applications that demonstrate the unique capabilities and potential of the DOE national user facilities at Oak Ridge, especially the newly commissioned BioSANS. The approach taken was three-fold: (1) to engage in high impact collaborative research projects that would benefit from small-angle neutron scattering to both demonstrate the power of the technique while expanding the potential user community; (2) to provide access to scattering facilities established at the University of Utah to as broad a set of researchers as possible to increase the expertise in small-angle scattering generally; and (3) to develop new methods and tools for small-angle scattering. To these ends, three major research collaborations were pursued that resulted in a significant body of published work where neutron scattering and contrast variation played a major role. These major collaborations involved studies of protein complexes involved in (1) bacterial transcription regulation and adaptive response (a DOE/BER priority area); (2) regulation of cardiac muscle; and (3) neuronal disorders. In addition, to broaden the impact of the project, smaller collaborative efforts were supported that used either small-angle X-ray or neutron scattering. Finally, the DOE supported facilities at the University of Utah were made available to researchers on a service basis and a number of independent groups took advantage of this opportunity. In all of this work, there was an emphasis on the training of students and post docs in scattering techniques, and a set of publications (a book chapter, a review, and an encyclopedia article) were produced to guide the non-specialist potential user of scattering techniques in successful applications of the techniques. We also developed a suite of user friendly web-based computational tools currently being accessed world-wide by researchers as an aid in neutron scattering data interpretation. In all, these collaborative projects and resulted in 29 original refereed journal articles published between 2005 and 2010 and engaged groups from at least 14 Universities (10 US, 4 international) and 3 National Laboratories (2 US, 1 international). An important final initiative from this project was to begin a process for international community agreement on a set of standards for the publication of biomolecular small-angle scattering data. This initiative is being championed with the International Union of Crystallography and has engaged a number of Journal Editors and is a very important step in the maturing of this now burgeoning field.

  12. The new Cold Neutron Chopper Spectrometer at the Spallation Neutron Source -- Design and Performance

    SciTech Connect (OSTI)

    Ehlers, Georg; Podlesnyak, Andrey A.; Niedziela, Jennifer L.; Iverson, Erik B.; Sokol, Paul E.

    2011-01-01

    The design and performance of the new cold neutron chopper spectrometer (CNCS) at the Spallation Neutron Source in Oak Ridge are described. CNCS is a direct-geometry inelastic time-of-flight spectrometer, designed essentially to cover the same energy and momentum transfer ranges as IN5 at ILL, LET at ISIS, DCS at NIST, TOFTOF at FRM-II, AMATERAS at J-PARC, PHAROS at LANSCE, and NEAT at HZB, at similar energy resolution. Measured values of key figures such as neutron flux at sample position and energy resolution are compared between measurements and ray tracing Monte Carlo simulations, and good agreement (better than 20% of absolute numbers) has been achieved. The instrument performs very well in the cold and thermal neutron energy ranges, and promises to become a workhorse for the neutron scattering community for quasielastic and inelastic scattering experiments.

  13. The new cold neutron chopper spectrometer at the Spallation Neutron Source: Design and performance

    SciTech Connect (OSTI)

    Ehlers, G.; Podlesnyak, A. A.; Niedziela, J. L.; Iverson, E. B.; Sokol, P. E.

    2011-08-15

    The design and performance of the new cold neutron chopper spectrometer (CNCS) at the Spallation Neutron Source in Oak Ridge are described. CNCS is a direct-geometry inelastic time-of-flight spectrometer, designed essentially to cover the same energy and momentum transfer ranges as IN5 at ILL, LET at ISIS, DCS at NIST, TOFTOF at FRM-II, AMATERAS at J-PARC, PHAROS at LANSCE, and NEAT at HZB, at similar energy resolution. Measured values of key figures such as neutron flux at sample position and energy resolution are compared between measurements and ray tracing Monte Carlo simulations, and good agreement (better than 20% of absolute numbers) has been achieved. The instrument performs very well in the cold and thermal neutron energy ranges, and promises to become a workhorse for the neutron scattering community for quasielastic and inelastic scattering experiments.

  14. The structure of Sindbis virus produced from vertebrate and invertabrate hosts determined by small angle neutron scattering

    SciTech Connect (OSTI)

    He, Lilin [ORNL; Piper, Amanda [North Carolina State University; Meilleur, Flora [ORNL; Myles, Dean A A [ORNL; Hernandez, Raquel [North Carolina State University; Brown, Dennis [North Carolina State University; Heller, William T [ORNL

    2010-01-01

    The complex natural cycle of vectored viruses that transition between host species, such as between insects and mammals, makes understanding the full life cycle of the virus an incredibly complex problem. Sindbis virus, an arbovirus and prototypic alphavirus having an inner protein shell and an outer glycoprotein coat separated by a lipid membrane, is one example of a vectored virus that transitions between vertebrate and insect hosts. While evidence of host-specific differences in Sindbis virus has been observed, no work has been performed to characterize the impact of the host species on the structure of the virus. Here, we report the first study of the structural differences between Sindbis viruses grown in mammalian and insect cells, which were determined by small-angle neutron scattering (SANS), a nondestructive technique that did not decrease the infectivity of the Sindbis virus particles studied. The scattering data and modeling showed that, while the radial position of the lipid bilayer did not change significantly, it was possible to conclude that it did have significantly more cholesterol when the virus was grown in mammalian cells. Additionally, the outer protein coat was found to be more extended in the mammalian Sindbis virus. The SANS data also demonstrated that the RNA and nucleocapsid protein share a closer interaction in the mammalian-cell-grown virus than in the virus from insect cells.

  15. Conformational effect on small angle neutron scattering behavior of interacting polyelectrolyte solutions: a perspective of integral equation theory

    SciTech Connect (OSTI)

    Chen, Wei-Ren [ORNL; Do, Changwoo [ORNL; Hong, Kunlun [ORNL; Liu, Yun [National Institute of Standards and Technology (NIST); Porcar, L. [National Institute of Standards and Technology (NIST); Shew, Chwen-Yang [City University of New York (CUNY); Smith, Greg [ORNL

    2012-01-01

    We present small angle neutron scattering (SANS) measurements of deuterium oxide (D2O) solutions of linear and star sodium poly(styrene sulfonate) (NaPSS) as a function of polyelectrolyte concentration. Emphasis is on understanding the dependence of their SANS coherent scattering cross section I(Q) on the molecular architecture of single polyelectrolyte. The key finding is that for a given concentration, star polyelectrolytes exhibit more pronounced characteristic peaks in I(Q), and the position of the first peak occurs at a smaller Q compared to their linear counterparts. Based on a model of integral equation theory, we first compare the SANS experimental I(Q) of salt free polyelectrolyte solutions with that predicted theoretically. Having seen their satisfactory qualitative agreement, the dependence of counterion association behavior on polyelectrolyte geometry and concentration is further explored. Our predictions reveal that the ionic environment of polyelectrolyte exhibits a strong dependence on polyelectrolyte geometry at lower polyelectrolyte concentration. However, when both linear and star polyelectrolytes exceed their overlap concentrations, the spatial distribution of counterion is found to be essentially insensitive to polyelectrolyte geometry due to the steric effect.

  16. Atomic dynamics in molten AlCu alloys of different compositions and at different temperatures by cold neutron scattering

    SciTech Connect (OSTI)

    Dahlborg, U. [University of Rouen; Besser, M. [Ames Laboratory; Kramer, Matthew J. [Ames Laboratory; Morris, J. R. [Oak Ridge National Laboratory; Calvo-Dahlborg, M. [University of Rouen

    2013-12-21

    The atomic motions in molten Al1?xCux (x=0.10, 0.171 and 0.25) around the eutectic composition (x=0.171) were studied by cold neutron inelastic scattering at three different temperatures (973 K, 1173 K and 1373 K). An alloy of eutectic composition containing the 63Cu isotope was also studied. Self-diffusion coefficients for the Cu ions were determined from the width of quasielastic peaks and were found to decrease slightly with increasing Cu concentration. Longitudinal current correlation functions Jl(Q,E) exhibit at all temperatures and at all compositions a shoulder at energies below 10 meV and one main maximum at higher energies. These features can be interpreted in terms of excitations of acoustic and optic nature. The shape of Jl(Q,E) is sensitive to composition, being considerably more structured for larger Cu content. This can be coupled to the existence of a prepeak in the measured zeroth moment of dynamic scattering function indicating an increased chemical ordering with increasing Cu concentration for all temperatures. Indications for an existence of a liquid–liquid phase transition are presented.

  17. Format requirements of thermal neutron scattering data in a nuclear data format to succeed the ENDF format

    SciTech Connect (OSTI)

    Brown, D. [Brookhaven National Lab. (BNL), Upton, NY (United States)

    2014-03-31

    In November 2012, the Working Party on Evaluation Cooperation Subgroup 38 (WPEC-SG38) began with the task of developing a nuclear data format and supporting infrastructure to replace the now nearly 50 year old ENDF format. The first step in this process is to develop requirements for the new format and infrastructure. In this talk, I will review the status of ENDF's Thermal Scattering Law (TSL) formats as well as support for this data in the GND format (from which the new format is expected to evolve). Finally, I hope to begin a dialog with members of the thermal neutron scattering community so that their data needs can be accurately and easily accommodated by the new format and tools, as captured by the requirements document. During this discussion, we must keep in mind that the new tools and format must; Support what is in existing data files; Support new things we want to put in data files; and Be flexible enough for us to adapt it to future unanticipated challenges.

  18. In-Situ Observation of Solid Electrolyte Interphase Formation in Ordered Mesoporous Hard Carbon by Small-Angle Neutron Scattering

    SciTech Connect (OSTI)

    Bridges, Craig A [ORNL; Paranthaman, Mariappan Parans [ORNL; Sun, Xiao-Guang [ORNL; Zhao, Jinkui [ORNL; Dai, Sheng [ORNL

    2012-01-01

    The aim of this work was to better understand the electrochemical processes occurring during the cycling of a lithium-ion half-cell containing ordered mesoporous hard carbon using time-resolved in situ small-angle neutron scattering (SANS). Utilizing electrolytes containing mixtures of deuterated (2H) and non-deuterated (1H) carbonates, we have addressed the challenging task of monitoring the formation and evolution of the solid-electrolyte interphase (SEI) layer. An evolution occurs in the SEI layer during discharge from a composition dominated by a higher scattering length density (SLD) lithium salt, to a lower SLD lithium salt for the ethylene carbonate/dimethyl carbonate (EC/DMC) mixture employed. By comparing half-cells containing different solvent deuteration levels, we show that it is possible to observe both SEI formation and lithium intercalation occurring concurrently at the low voltage region in which lithium intercalates into the hard carbon. These results demonstrate that SANS can be employed to monitor complicated electrochemical processes occurring in rechargeable batteries, in a manner that simultaneously provides information on the composition and microstructure of the electrode.

  19. Scattering

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

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  20. Scattering

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantity ofkandz-cm11 Outreach Home RoomPreservation ofAlbuquerque| Stanford Synchrotron Radiation LightsourceScattering

  1. Digenetic Changes in Macro- to Nano-Scale Porosity in the St. Peter Sandstone:L An (Ultra) Small Angle Neutron Scattering and Backscattered Electron Imagining Analysis

    SciTech Connect (OSTI)

    Anovitz, Lawrence {Larry} M [ORNL; Cole, David [Ohio State University; Rother, Gernot [ORNL; Allard Jr, Lawrence Frederick [ORNL; Jackson, Andrew [NIST Center for Neutron Research (NCRN), Gaithersburg, MD; Littrell, Ken [ORNL

    2013-01-01

    Small- and Ultra-Small Angle Neutron Scattering (SANS and USANS) provide powerful tools for quantitative analysis of porous rocks, yielding bulk statistical information over a wide range of length scales. This study utilized (U)SANS to characterize shallowly buried quartz arenites from the St. Peter Sandstone. Backscattered electron imaging was also used to extend the data to larger scales. These samples contain significant volumes of large-scale porosity, modified by quartz overgrowths, and neutron scattering results show significant sub-micron porosity. While previous scattering data from sandstones suggest scattering is dominated by surface fractal behavior over many orders of magnitude, careful analysis of our data shows both fractal and pseudo-fractal behavior. The scattering curves are composed of subtle steps, modeled as polydispersed assemblages of pores with log-normal distributions. However, in some samples an additional surface-fractal overprint is present, while in others there is no such structure, and scattering can be explained by summation of non-fractal structures. Combined with our work on other rock-types, these data suggest that microporosity is more prevalent, and may play a much more important role than previously thought in fluid/rock interactions.

  2. Forward-angle neutron-proton scattering at 96 MeV

    SciTech Connect (OSTI)

    Johansson, C.; Blomgren, J.; Atac, A.; Bergenwall, B.; Hildebrand, A.; Klug, J.; Mermod, P.; Pomp, S.; Oesterlund, M.; Dangtip, S.; Tippawan, U.; Elmgren, K.; Jonsson, O.; Prokofiev, A.V.; Renberg, P.-U.; Nadel-Turonski, P.; Nilsson, L.; Olsson, N.

    2005-02-01

    The differential np scattering cross section has been measured at 96 MeV in the angular range {theta}{sub c.m.}=20 deg. -76 deg. Together with an earlier data set at the same energy, covering the angles {theta}{sub c.m.}=74 deg. -180 deg., a new data set has been formed in the angular range {theta}{sub c.m.}=20 deg. - 180 deg. This extended data set has been normalized to the experimental total np cross section, resulting in a renormalization of the earlier data of 0.7%, which is well within the reported normalization uncertainty for that experiment. A novel normalization technique has been investigated. The results on forward np scattering are in reasonable agreement with theory models and partial wave analyses and have been compared with data from the literature.

  3. The Manuel Lujan, Jr. Neutron Scattering Center, LANSCE experiment reports: 1990 Run Cycle

    SciTech Connect (OSTI)

    DiStravolo, M.A.

    1991-10-01

    This year was the third in which LANSCE ran a formal user program. A call for proposals was issued before the scheduled run cycles, and experiment proposals were submitted by scientists from universities, industry, and other research facilities around the world. An external program advisory committee, which LANSCE shares with the Intense Pulsed Neutron Source (IPNS), Argonne National Laboratory examined the proposals and made recommendations. At LANSCE, neutrons are produced by spallation when a pulsed, 800-MeV proton beam impinges on a tungsten target. The proton pulses are provided by the Clinton P. Anderson Meson Physics Facility (LAMPF) accelerator and an associated Proton Storage Ring (PSR), which can alter the intensity, time structure, and repetition rate of the pulses. The LAMPF protons of Line D are shared between the LANSCE target and the Weapons Neutron Research facility, which results in LANSCE spectrometers being available to external users for unclassified research about 80% of each six-month LAMPF run cycle. Measurements of interest to the Los Alamos National Laboratory may also be performed and may occupy up to an additional 20% of the available beam time. These experiments are reviewed by an internal program advisory committee. One hundred thirty-four proposals were submitted for unclassified research and twelve proposals for research of a programmatic nature to the Laboratory. Our definition of beam availability is when the proton current from the PSR exceeds 50% of the planned value. The PSR ran at 65{mu}A current (average) at 20 Hz for most of 1990. All of the scheduled experiments were performed and experiments in support of the LANSCE research program were accomplished during the discretionary periods.

  4. Scintillation efficiency of liquid argon in low energy neutron-argon scattering

    E-Print Network [OSTI]

    Creus, W; Amsler, C; Ferella, A D; Rochet, J; Scotto-Lavina, L; Walter, M

    2015-01-01

    Experiments searching for weak interacting massive particles with noble gases such as liquid argon require very low detection thresholds for nuclear recoils. A determination of the scintillation efficiency is crucial to quantify the response of the detector at low energy. We report the results obtained with a small liquid argon cell using a monoenergetic neutron beam produced by a deuterium-deuterium fusion source. The light yield relative to electrons was measured for six argon recoil energies between 11 and 120 keV at zero electric drift field.

  5. Neutron Scattering of CeNi at the SNS-ORNL: A Preliminary Report

    Office of Scientific and Technical Information (OSTI)

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  6. Neutron scattering of CeNi at the SNS-ORNL: A preliminary report

    Office of Scientific and Technical Information (OSTI)

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  7. Neutron Scattering Facilities | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

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  8. Neutron scattering from myelin revisited: bilayer asymmetry and water-exchange kinetics

    SciTech Connect (OSTI)

    Denninger, Andrew R. [Boston College, Chestnut Hill, MA 02467 (United States); Demé, Bruno; Cristiglio, Viviana [Institut Laue–Langevin (ILL), CS 20156, F-38042 Grenoble CEDEX 9 (France); LeDuc, Géraldine [European Synchrotron Radiation Facility (ESRF), CS 40220, F-38043 Grenoble CEDEX 9 (France); Feller, W. Bruce [NOVA Scientific Inc., Sturbridge, MA 01566 (United States); Kirschner, Daniel A., E-mail: kirschnd@bc.edu [Boston College, Chestnut Hill, MA 02467 (United States)

    2014-12-01

    The structure of internodal myelin in the rodent central and peripheral nervous systems has been determined using neutron diffraction. The kinetics of water exchange in these tissues is also described. Rapid nerve conduction in the central and peripheral nervous systems (CNS and PNS, respectively) of higher vertebrates is brought about by the ensheathment of axons with myelin, a lipid-rich, multilamellar assembly of membranes. The ability of myelin to electrically insulate depends on the regular stacking of these plasma membranes and on the presence of a number of specialized membrane-protein assemblies in the sheath, including the radial component, Schmidt–Lanterman incisures and the axo–glial junctions of the paranodal loops. The disruption of this fine-structure is the basis for many demyelinating neuropathies in the CNS and PNS. Understanding the processes that govern myelin biogenesis, maintenance and destabilization requires knowledge of myelin structure; however, the tight packing of internodal myelin and the complexity of its junctional specializations make myelin a challenging target for comprehensive structural analysis. This paper describes an examination of myelin from the CNS and PNS using neutron diffraction. This investigation revealed the dimensions of the bilayers and aqueous spaces of myelin, asymmetry between the cytoplasmic and extracellular leaflets of the membrane, and the distribution of water and exchangeable hydrogen in internodal multilamellar myelin. It also uncovered differences between CNS and PNS myelin in their water-exchange kinetics.

  9. Transport of thermal neutrons in D/sub 2/O in the temperature Range 5 to 60/sup 0/C based on a new scattering kernel

    SciTech Connect (OSTI)

    Bansal, R.M.; Kothari, L.S.; Tewari, S.P.

    1980-10-01

    A new scattering kernel for heavy water has been proposed. The kernel takes into account the chemical binding energy effects and also includes the rotational and intramolecular vibrational modes. Using this scattering kernel, various neutron transport processes in the temperature range 5 to 60/sup 0/C have been studied and compared with the corresponding experimental results. The calculated results include total neutron scattering cross section at 20/sup 0/C; asymptotic decay of neutron pulses in the temperature range 5 to 60/sup 0/C and temperature variation of the diffusion coefficient and diffusion cooling coefficient; timedependent spectra inside finite-sized assemblies of heavy water at 20 and 43.3/sup 0/C thermalization time; and diffusion length and space-dependent study in pure and poisoned assemblies of heavy water. The calculated results are in good agreement with the experimental results. At some places notable differences are observed between the results obtained using our scattering kernel and those based on the Honeck kernel.

  10. High-energy magnetic excitations in overdoped La 2 - x Sr x CuO 4 studied by neutron and resonant inelastic x-ray scattering

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Wakimoto, S.; Ishii, K.; Kimura, H.; Fujita, M.; Dellea, G.; Kummer, K.; Braicovich, L.; Ghiringhelli, G.; Debeer-Schmitt, L. M.; Granroth, G. E.

    2015-05-21

    We have performed neutron inelastic scattering and resonant inelastic x-ray scattering (RIXS) at the Cu-L? edge to study high-energy magnetic excitations at energy transfers of more than 100 meV for overdoped La2-xSrxCuO? with x=0.25 (Tc=15 K) and x=0.30 (nonsuperconducting) using identical single-crystal samples for the two techniques. From constant-energy slices of neutron-scattering cross sections, we have identified magnetic excitations up to ~250 meV for x=0.25. Although the width in the momentum direction is large, the peak positions along the (?,?) direction agree with the dispersion relation of the spin wave in the nondoped La?CuO? (LCO), which is consistent with themore »previous RIXS results of cuprate superconductors. Using RIXS at the Cu-L? edge, we have measured the dispersion relations of the so-called paramagnon mode along both (?,?) and (?,0) directions. Although in both directions the neutron and RIXS data connect with each other and the paramagnon along (?,0) agrees well with the LCO spin-wave dispersion, the paramagnon in the (?,?) direction probed by RIXS appears to be less dispersive and the excitation energy is lower than the spin wave of LCO near (?/2,?/2). Thus, our results indicate consistency between neutron inelastic scattering and RIXS, and elucidate the entire magnetic excitation in the (?,?) direction by the complementary use of two probes. The polarization dependence of the RIXS profiles indicates that appreciable charge excitations exist in the same energy range of magnetic excitations, reflecting the itinerant character of the overdoped sample. A possible anisotropy in the charge excitation intensity might explain the apparent differences in the paramagnon dispersion in the (?,?) direction as detected by the x-ray scattering.« less

  11. High-energy magnetic excitations in overdoped La 2 - x Sr x CuO 4 studied by neutron and resonant inelastic x-ray scattering

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Wakimoto, S.; Ishii, K.; Kimura, H.; Fujita, M.; Dellea, G.; Kummer, K.; Braicovich, L.; Ghiringhelli, G.; Debeer-Schmitt, L. M.; Granroth, G. E.

    2015-05-01

    We have performed neutron inelastic scattering and resonant inelastic x-ray scattering (RIXS) at the Cu-L? edge to study high-energy magnetic excitations at energy transfers of more than 100 meV for overdoped La2-xSrxCuO? with x=0.25 (Tc=15 K) and x=0.30 (nonsuperconducting) using identical single-crystal samples for the two techniques. From constant-energy slices of neutron-scattering cross sections, we have identified magnetic excitations up to ~250 meV for x=0.25. Although the width in the momentum direction is large, the peak positions along the (?,?) direction agree with the dispersion relation of the spin wave in the nondoped La?CuO? (LCO), which is consistent with the previous RIXS results of cuprate superconductors. Using RIXS at the Cu-L? edge, we have measured the dispersion relations of the so-called paramagnon mode along both (?,?) and (?,0) directions. Although in both directions the neutron and RIXS data connect with each other and the paramagnon along (?,0) agrees well with the LCO spin-wave dispersion, the paramagnon in the (?,?) direction probed by RIXS appears to be less dispersive and the excitation energy is lower than the spin wave of LCO near (?/2,?/2). Thus, our results indicate consistency between neutron inelastic scattering and RIXS, and elucidate the entire magnetic excitation in the (?,?) direction by the complementary use of two probes. The polarization dependence of the RIXS profiles indicates that appreciable charge excitations exist in the same energy range of magnetic excitations, reflecting the itinerant character of the overdoped sample. A possible anisotropy in the charge excitation intensity might explain the apparent differences in the paramagnon dispersion in the (?,?) direction as detected by the x-ray scattering.

  12. New insights into water bonding during early tricalcium silicate hydration with quasielastic neutron scattering

    SciTech Connect (OSTI)

    Gutberlet, T., E-mail: gutberlet@cbm.bv.tum.de [Centre for Building Materials (CBM), Technische Universität München, Baumbachstraße 7, 81245 Munich (Germany); Hilbig, H.; Beddoe, R.E. [Centre for Building Materials (CBM), Technische Universität München, Baumbachstraße 7, 81245 Munich (Germany)] [Centre for Building Materials (CBM), Technische Universität München, Baumbachstraße 7, 81245 Munich (Germany); Lohstroh, W. [Forschungs-Neutronenquelle Heinz Maier-Leibnitz (FRM II), Technische Universität München, Lichtenbergstraße 1, 85748 Garching (Germany)] [Forschungs-Neutronenquelle Heinz Maier-Leibnitz (FRM II), Technische Universität München, Lichtenbergstraße 1, 85748 Garching (Germany)

    2013-09-15

    New information on the water bonding during the first 36 h of hydration of tricalcium silicate was obtained using the high neutron flux at the sample position of the time-of-flight spectrometer (TOFTOF), FRM II in Garching, Germany, together with {sup 29}Si NMR and X-ray diffraction measurements. A rapid increase in the amount of constrained water was observed at the beginning of the induction period. This is attributed to the formation of an early C-S-H with a large specific surface area (around 800 m{sup 2}/g). During subsequent hydration, the amount of constrained water, as given by the total surface area of the hydration products, is controlled by (a) the formation of new metastable early C-S-H which increases total surface area and (b) polymerisation processes which reduce total surface area. The relative contribution of these processes varies during hydration.

  13. Magnetic Transitions in Iron Porphyrin Halides by Inelastic Neutron Scattering and Ab-initio Studies of Zero-Field Splittings

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Stavretis, Shelby E.; Atanasov, Mihail; Podlesnyak, Andrey A.; Hunter, Seth C.; Neese, Frank; Xue, Zi-Ling

    2015-10-02

    Zero-field splitting (ZFS) parameters of nondeuterated metalloporphyrins [Fe(TPP)X] (X = F, Br, I; H2TPP = tetraphenylporphyrin) are determined by inelastic neutron scattering (INS). The ZFS values are D = 4.49(9) cm–1 for tetragonal polycrystalline [Fe(TPP)F], and D = 8.8(2) cm–1, E = 0.1(2) cm–1 and D = 13.4(6) cm–1, E = 0.3(6) cm–1 for monoclinic polycrystalline [Fe(TPP)Br] and [Fe(TPP)I], respectively. Along with our recent report of the ZFS value of D = 6.33(8) cm–1 for tetragonal polycrystalline [Fe(TPP)Cl], these data provide a rare, complete determination of ZFS parameters in a metalloporphyrin halide series. The electronic structure of [Fe(TPP)X] (X =more »F, Cl, Br, I) has been studied by multireference ab initio methods: the complete active space self-consistent field (CASSCF) and the N-electron valence perturbation theory (NEVPT2) with the aim of exploring the origin of the large and positive zero-field splitting D of the 6A1 ground state. D was calculated from wave functions of the electronic multiplets spanned by the d5 configuration of Fe(III) along with spin–orbit coupling accounted for by quasi degenerate perturbation theory. Results reproduce trends of D from inelastic neutron scattering data increasing in the order from F, Cl, Br, to I. A mapping of energy eigenvalues and eigenfunctions of the S = 3/2 excited states on ligand field theory was used to characterize the ?- and ?-antibonding effects decreasing from F to I. This is in agreement with similar results deduced from ab initio calculations on CrX63- complexes and also with the spectrochemical series showing a decrease of the ligand field in the same directions. A correlation is found between the increase of D and decrease of the ?- and ?-antibonding energies e?X (? = ?, ?) in the series from X = F to I. Analysis of this correlation using second-order perturbation theory expressions in terms of angular overlap parameters rationalizes the experimentally deduced trend. Furthermore, D parameters from CASSCF and NEVPT2 results have been calibrated against those from the INS data, yielding a predictive power of these approaches. Methods to improve the quantitative agreement between ab initio calculated and experimental D and spectroscopic transitions for high-spin Fe(III) complexes are proposed.« less

  14. Local Structure of La1-xSrxCoO3 determined from EXAFS and neutron PDF studies

    E-Print Network [OSTI]

    Sundaram, N.

    2009-01-01

    60439, USA and Lujan Neutron Scattering Center, Los Alamos31] at the Lujan Neutron Scattering Cen- ter, LANL. Data at

  15. Neutron Science Research Areas | ORNL

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Home | Science & Discovery | Neutron Science | Research Areas SHARE Research Areas Neutron scattering research at ORNL covers four broad research areas: biology and soft...

  16. Conformation of Oligo(Ethylene Glycol) grafted Poly(Norbornene) in solutions: A Small Angle Neutron Scattering Study

    SciTech Connect (OSTI)

    Cheng, Gang [ORNL; Melnichenko, Yuri B [ORNL; Hua, Fengjun [ORNL; Hong, Kunlun [ORNL; Wignall, George D [ORNL; Hammouda, B. [National Institute of Standards and Technology (NIST); Mays, Jimmy [ORNL

    2008-01-01

    The structure of thermo sensitive poly(methoxyoligo(ethylene glycol) norbornenyl esters) homopolymers in dilute solution was investigated by Small Angle Neutron Scattering (SANS). The homopolymers consist of a polynorbornene (PNB) backbone with a degree of polymerization (DP) of 50, and each backbone monomer has a grafted Ethylene Glycol (EG) side chain with an average DP of 6.6. The hydrophobic backbone and hydrophilic side chains interact differently with solvents depending on their polarity, which makes the conformation very sensitive to the solvent quality. The polymer conformation was studied in two solvents, d-toluene and D2O, with the aim of understanding the influence of solvent/polymer interactions on the resulting structures. It was found that in a 0.5 wt. % solution in d-toluene the polymers assume wormlike chains and gradually contract with increasing polymer concentration. In a 0.5 wt. % solution in D2O, the polymers are partially contracted at room temperature and their conformation can be described by the form factor of a rigid cylinder. The volume of the cylinder shows no concentration dependence. Furthermore, the polymers in D2O collapse at higher temperatures due to decreasing solubility of the side chains in water.

  17. Structural Evolution of Polylactide Molecular Bottlebrushes: Kinetics Study by Size Exclusion Chromatography, Small Angle Neutron Scattering and Simulations

    SciTech Connect (OSTI)

    Pickel, Deanna L [ORNL; Kilbey, II, S Michael [ORNL; Uhrig, David [ORNL; Hong, Kunlun [ORNL; Carrillo, Jan-Michael Y [ORNL; Sumpter, Bobby G [ORNL; Ahn, Suk-Kyun [ORNL; Han, Youngkyu [ORNL; Kim, Dr. Tae-Hwan [Korea Atomic Energy Research Institute; Smith, Gregory Scott [ORNL; Do, Changwoo [ORNL

    2014-01-01

    Structural evolution from poly(lactide) (PLA) macromonomer to resultant PLA molecular bottlebrush during ring opening metathesis polymerization (ROMP) was investigated for the first time by combining size exclusion chromatography (SEC), small-angle neutron scattering (SANS) and coarse-grained molecular dynamics (CG-MD) simulations. Multiple aliquots were collected at various reaction times during ROMP, and subsequently analyzed by SEC and SANS. The two complementary techniques enable the understanding of systematic changes in conversion, molecular weight and dispersity as well as structural details of PLA molecular bottlebrushes. CG-MD simulation not only predicts the experimental observations, but it also provides further insight into the analysis and interpretation of data obtained in SEC and SANS experiments. We find that PLA molecular bottlebrushes undergo three conformational transitions with increasing conversion (i.e., increasing the backbone length): (1) from an elongated to a globular shape due to longer side chain at lower conversion, (2) from a globular to an elongated shape at intermediate conversion caused by excluded volume of PLA side chain, and (3) the saturation of contour length at higher conversion due to chain transfer reactions.

  18. Growth Kinetics of Lipid-Based Nanodiscs to Unilamellar Vesicles: A Time-Resolved Small Angle Neutron Scattering (SANS) Study

    SciTech Connect (OSTI)

    Mahabir, Suanne [University of Western Ontario, The; Small, Darcy [University of Western Ontario, The; Li, Ming [University of Connecticut, Storrs; Wan, Wankei [University of Western Ontario, The; Kucerka, Norbert [Canadian Neutron Beam Centre and Comelius University (Slovakia); Littrell, Ken [ORNL; Katsaras, John [ORNL; Nieh, Mu-Ping [University of Connecticut, Storrs

    2013-01-01

    Mixtures of dimyristoyl-phosphatidylcholine (DMPC), dimyristoyl-phosphatidylglycerol (DMPG) and dihexanoylphosphatidylcholine (DHPC) in aqueous solutions spontaneously form monodisperse, bilayered nanodiscs (also known as bicelles ) at or below the melting transition temperature of DMPC (TM ~23 C). In dilute systems above the main transition temperature TM of DMPC, bicelles coalesce (increasing their diameter) and eventually self-fold into unilamellar vesicles (ULVs). Time resolved small angle neutron scattering was used to study the growth kinetics of nanodiscs below and equal to TM over a period of hours as a function of temperature at two lipid concentrations in presence or absence of NaCl salt. Bicelles seem to undergo a sudden initial growth phase with increased temperature, which is then followed by a slower reaction-limited growth phase that depends on ionic strength, lipid concentration and temperature. The bicelle interaction energy was derived from the colloidal theory of Derjaguin and Landau, and Verwey and Overbeek (DLVO). While the calculated total energy between discs is attractive and proportional to their growth rate, a more detailed mechanism is proposed to describe the mechanism of disc coalescence. After annealing at low temperature (low-T), samples were heated to 50 C in order to promote the formation of ULVs. Although the low-T annealing of samples has only a marginal effect on the mean size of end-state ULVs, it does affect their polydispersity, which increases with increased T, presumably driven by the entropy of the system.

  19. Monitoring phase behavior of hydrogen confined in carbon nanopores by in-situ small angle neutron scattering technique

    SciTech Connect (OSTI)

    Zhang, Hongxin [ORNL; He, Lilin [ORNL; Melnichenko, Yuri B [ORNL; Contescu, Cristian I [ORNL; Gallego, Nidia C [ORNL

    2012-01-01

    We report on the use of in-situ small angle neutron scattering (SANS) technique to study the phase behavior of hydrogen confined in narrow pores of ultramicroporous carbon (UMC) with a very large surface area (2630 m2/g) and pore volume (1.3 cm3/g). The effect of pore size and pressure on hydrogen adsorbed on UMC at room temperature and pressures up to ~200 bar were investigated. In a previous experiment, we have measured the density of adsorbed H2 gas in the nanopores and mesopores of polyfurfuryl alcohol-derived activated carbon (PFAC) by SANS techniques. Here, a comparative SANS study between the UMC and PFAC was conducted in order to further investigate the densification of H2 as a function of pore size and pressure. Initial results suggest that the density of confined H2 in both UMC and PFAC is considerably higher than that of the bulk hydrogen gas. The density is systematically higher in the narrow pores and decreases with increasing pore size. These results clearly demonstrate the advantage of adsorptive storage over compressed gas storage and emphasize the greater efficiency of micropores over mesopores in the adsorption process, which can be used to guide the development of new carbon adsorbents tailored for maximum H2 storage capacities at near-ambient temperatures.

  20. Early stages of spinodal decomposition in Fe–Cr resolved by in-situ small-angle neutron scattering

    SciTech Connect (OSTI)

    Hörnqvist, M. Thuvander, M.; Steuwer, A.; King, S.; Odqvist, J.; Hedström, P.

    2015-02-09

    In-situ, time-resolved small-angle neutron scattering (SANS) investigations of the early stages of the spinodal decomposition process in Fe–35Cr were performed at 773 and 798?K. The kinetics of the decomposition, both in terms of characteristic distance and peak intensity, followed a power-law behaviour from the start of the heat treatment (a?{sup ?}=?0.10–0.11 and a??=?0.67–0.86). Furthermore, the method allows tracking of the high–Q slope, which is a sensitive measure of the early stages of decomposition. Ex-situ SANS and atom probe tomography were used to verify the results from the in-situ investigations. Finally, the in-situ measurement of the evolution of the characteristic distance at 773?K was compared with the predictions from the Cahn-Hilliard-Cook model, which showed good agreement with the experimental data (a?{sup ?}=?0.12–0.20 depending on the assumed mobility)

  1. Swollen Micelles Plus Hydrophobically Modified Hydrosoluble Polymers in Aqueous Solutions: Decoration Versus Bridging. a Small Angle Neutron Scattering Study

    E-Print Network [OSTI]

    Mohammed Filali; Raymond Aznar; Mattias Svenson; Gregoire Porte; Jacqueline Appell

    2004-10-12

    In this paper we examine the effective interactions introduced between the droplets of an oil in water microemulsion upon progressive addition of hydrophobically modified water soluble poly(ethylene oxide)-PEO using essentially small angle neutron scattering. To discuss the relative importance of decoration and bridging of the droplets we compare analogous samples with addition of a PEO grafted at both extremities with hydrophobic C12H 25 chains (PEO-2m) or addition of a PEO grafted at one extremity only with a C12H 25 chain (PEO-m). PEO-m or PEO-2m adsorb onto the droplets via their hydrophobic extremities and the droplets are found to retain their form and size upon addition of up to 40 hydrophobic C12H 25 chains per droplet. When the volume fraction of droplets is less than about 10%, the effective interactions introduced by PEO-m or PEO-2m are found to be very different: PEO-m introduces a repulsive interaction while PEO-2m introduces an effective attractive interaction. This attractive interaction leads to an associative phase separation in the range of low volume fraction when a sufficient amount of PEO-2m is added.

  2. Neutron detector

    DOE Patents [OSTI]

    Stephan, Andrew C. (Knoxville, TN); Jardret; Vincent D. (Powell, TN)

    2011-04-05

    A neutron detector has a volume of neutron moderating material and a plurality of individual neutron sensing elements dispersed at selected locations throughout the moderator, and particularly arranged so that some of the detecting elements are closer to the surface of the moderator assembly and others are more deeply embedded. The arrangement captures some thermalized neutrons that might otherwise be scattered away from a single, centrally located detector element. Different geometrical arrangements may be used while preserving its fundamental characteristics. Different types of neutron sensing elements may be used, which may operate on any of a number of physical principles to perform the function of sensing a neutron, either by a capture or a scattering reaction, and converting that reaction to a detectable signal. High detection efficiency, an ability to acquire spectral information, and directional sensitivity may be obtained.

  3. Anomalous dynamics of aqueous solutions of di-propylene glycol methylether confined in MCM-41 by quasielastic neutron scattering

    SciTech Connect (OSTI)

    Swenson, Jan Elamin, Khalid; Chen, Guo; Lohstroh, Wiebke; Sakai, Victoria Garcia

    2014-12-07

    The molecular dynamics of solutions of di-propylene glycol methylether (2PGME) and H{sub 2}O (or D{sub 2}O) confined in 28 Å pores of MCM-41 have been studied by quasielastic neutron scattering and differential scanning calorimetry over the concentration range 0–90 wt.% water. This system is of particular interest due to its pronounced non-monotonic concentration dependent dynamics of 2PGME in the corresponding bulk system, showing the important role of hydrogen bonding for the dynamics. In this study we have elucidated how this non-monotonic concentration dependence is affected by the confined geometry. The results show that this behaviour is maintained in the confinement, but the slowest diffusive dynamics of 2PGME is now observed at a considerably higher water concentration; at 75 wt.% water in MCM-41 compared to 30 wt.% water in the corresponding bulk system. This difference can be explained by an improper mixing of the two confined liquids. The results suggest that water up to a concentration of about 20 wt.% is used to hydrate the hydrophilic hydroxyl surface groups of the silica pores, and that it is only at higher water contents the water becomes partly mixed with 2PGME. Hence, due to this partial micro-phase separation of the two liquids larger, and thereby slower relaxing, structural entities of hydrogen bonded water and 2PGME molecules can only be formed at higher water contents than in the bulk system. However, the Q-dependence is unchanged with confinement, showing that the nature of the molecular motions is preserved. Thus, there is no indication of localization of the dynamics at length scales of less than 20 Å. The dynamics of both water and 2PGME is strongly dominated by translational diffusion at a temperature of 280 K.

  4. Neutron Scattering Studies of Liquid on or Confined in Nano- and Mesoporous Carbons, Including Carbide-Derived Carbons

    SciTech Connect (OSTI)

    Wesolowski, David J

    2014-07-01

    This project involved the synthesis of microporous graphitic-carbon powders with subnanometer average pore size, and very narrow pore size distributions, and the use of these materials in experimental studies of pore-fluid structure and dynamics. Samples of carbide-derived carbon powder, synthesized by extraction of the metal cations from TiC by a high temperature chlorination process, followed by high temperature vacuum annealing, were prepared by Ranjan Dash and his associates at CRADA partner Y-Carbon, Inc. The resulting material had average pore sizes ranging from 5 to 8 . These powders were used in two experiments conducted by researchers involved in the Energy Frontier Research Center Directed by David J. Wesolowski at ORNL, the Fluid Interface Reactions, Structures and Transport (FIRST) Center. FIRST-funded researchers at Drexel University collaborated with scientists at the Paul Scherrer Institute, Switzerland, to measure the expansion and contraction of the microporous carbon particles during charging and discharging of supercapactor electrodes composed of these particles (Hantell et al., 2011, Electrochemistry Communications, v. 13, pp. 1221-1224.) in an electrolyte composed of tetraethylammonium tetrafluoroborate dissolved in acetonitrile. In the second experiment, researchers at Oak Ridge National Laboratory and Drexel University conducted quasielastic neutron scattering studies of the diffusional dynamics of water imbibed into the micropores of the same material (Chathoth et al., 2011, EuroPhysics Journal, v. 95, pp. 56001/1-6). These studies helped to establish the role of pores approaching the size of the solvent and dissolved ions in altering diffusional dynamics, ion transport and physical response of conducting substrates to ion desolvation and entry into subnamometer pores.

  5. Design of a backscatter 14-MeV neutron time-of-flight spectrometer for experiments at ITER

    SciTech Connect (OSTI)

    Dzysiuk, N.; Hellesen, C.; Conroy, S.; Ericsson, G.; Hjalmarsson, A.; Skiba, M. [Div. Applied Nuclear Physics, Dept. Physics and Astronomy, Uppsala University, Box 516, Uppsala, 751 20 (Sweden)

    2014-08-21

    Neutron energy spectrometry diagnostics play an important role in present-day experiments related to fusion energy research. Measurements and thorough analysis of the neutron emission from the fusion plasma give information on a number of basic fusion performance quantities, on the condition of the neutron source and plasma behavior. Here we discuss the backscatter Time-of-Flight (bTOF) spectrometer concept as a possible instrument for performing high resolution measurements of 14 MeV neutrons. The instrument is based on two sets of scintillators, a first scatterer exposed to a collimated neutron beam and a second detector set placed in the backward direction. The scintillators of the first set are enriched in deuterium to achieve neutron backscattering. The energy resolution and efficiency of a bTOF instrument have been determined for various geometrical configurations. A preliminary design of optimal geometry for the two scintillator sets has been obtained by Monte Carlo simulations based on the MCNPX code.

  6. A radial collimator for a time-of-flight neutron spectrometer

    SciTech Connect (OSTI)

    Stone, M. B.; Abernathy, D. L. [Quantum Condensed Matter Science Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831 (United States); Niedziela, J. L.; Loguillo, M. J.; Overbay, M. A. [Instrument and Source Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831 (United States)

    2014-08-15

    We have engineered and installed a radial collimator for use in the scattered beam of a neutron time-of-flight spectrometer at a spallation neutron source. The radial collimator may be used with both thermal and epithermal neutrons, reducing the detected scattering intensity due to material outside of the sample region substantially. The collimator is located inside of the sample chamber of the instrument, which routinely cycles between atmospheric conditions and cryogenic vacuum. The oscillation and support mechanism of the collimator allow it to be removed from use without breaking vacuum. We describe here the design and characterization of this radial collimator.

  7. Laboratory performances of the solar multichannel resonant scattering spectrometer prototype of the GOLF-New Generation instrument

    E-Print Network [OSTI]

    S. Turck-Chieze; P. H. Carton; S. Mathur; J. -C. Barriere; P. Daniel-Thomas; C. Lahonde-Hamdoun; R. Granelli; D. Loiseau; F. Nunio; Y. Piret; J. M. Robillot

    2008-06-21

    This article quickly summarizes the performances and results of the GOLF/SoHO resonant spectrometer, thus justifying to go a step further. We then recall the characteristics of the multichannel resonant GOLF-NG spectrometer and present the first successful performances of the laboratory tests on the prototype and also the limitations of this first technological instrument. Scientific questions and an observation strategy are discussed.

  8. Small-angle neutron scattering measurements of hydrogen and deuterium trapping at dislocations in deformed single-crystalline Pd at low temperature

    SciTech Connect (OSTI)

    Heuser, Brent J. [University of Illinois, Urbana-Champaign; JU, H. S. [University of Illinois, Urbana-Champaign

    2011-01-01

    Small-angle neutron scattering (SANS) measurements of hydrogen and deuterium trapped at dislocation defects in deformed single-crystalline Pd have been performed at 15, 100, and 200 K at total interstitial solute concentrations of order 10 3. This work supports recent incoherent inelastic neutron scattering measurements of the vibrational density of states of trapped hydrogen under similar concentration-temperature conditions [Heuser et al., Phys. Rev. B 78, 214101 (2008)]. The measured net absolute macroscopic differential scattering cross sections have been fitted with a cylindrical form factor representing solute-decorated dislocation line segments. Generally, very little difference in the measured cross sections was observed with temperature for a given solute type, while a significant change was observed between hydrogen- and deuterium-loaded samples. The latter difference is understood within a cross-section model that takes into account the local lattice dilatation associated with solute segregation at dislocations. The application of the model cross section to the net PdH0.0013 SANS response yields an effective trapping radius of R 10 A and dislocation density of d 1010 cm 2. Analysis of the SANS response allowed the local trapped solute concentration ( 0.5 [H]/[Pd]) and volumetric dilatation (/ 1.1) to be determined with the constraint that the system locally satisfies the known lattice expansion of Pd hydride (i.e., Vegard s law).

  9. Neutrostriction in Neutron stars

    E-Print Network [OSTI]

    V. K. Ignatovich

    2006-06-29

    It is demonstrated that not only gravity, but also neutrostriction forces due to optical potential created by coherent elastic neutron-neutron scattering can hold a neutron star together. The latter forces can be stronger than gravitational ones. The effect of these forces on mass, radius and structure of the neutron star is estimated.

  10. Neutron Optics Optimization for the SNS EQ-SANS Diffractometer

    SciTech Connect (OSTI)

    Zhao, Jinkui [ORNL

    2011-01-01

    The extended Q-range small angle neutron scattering (EQ-SANS) diffractometer at the Spallation Neutron Source has recently been completed. Initial commissioning has shown that it has achieved its high intensity, low background, and wide dynamic range design goals. One of the key components that enable these performances is its neutron optics, which are extensively optimized using analytical and Monte Carlo methods. The EQ-SANS optics consist of a curved multichannel beam bender and sections of straight neutron guides on both ends of the bender. The bender and the guide are made of float glass coated with supermirror multilayers. The function of the optics is to ensure low instrument background by avoiding the direct line of sight of the neutron moderator at downstream locations, while transporting thermal and cold neutrons to the sample with maximum efficiency. In this work, the optimization of the EQ-SANS optics is presented.

  11. Analytical Calculation of the Neutrons Spectrum for Direct Measurement of N-N Scattering at Pulsed Reactor Yaguar

    E-Print Network [OSTI]

    V. K. Ignatovich

    2008-06-23

    Analytical calculation of a single neutron detector counts per YAGUAR reactor pulse is presented and comparison with coincidence scheme is given.

  12. Neutron-Scattering Evidence for a Periodically Modulated Superconducting Phase in the Underdoped Cuprate La1.905Ba0.095CuO4

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Xu, Zhijun [Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Mater Physics and Materials Science Dept.; Stock, C. [National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States). Center for Neutron Research; Chi, Songxue [National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States). Center for Neutron Research; Kolesnikov, A. I. [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Chemical and Engineering Materials Div.; Xu, Guangyong I. [Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Mater Physics and Materials Science Dept.; Gu, Genda [Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Mater Physics and Materials Science Dept.; Tranquada, J. M. [Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Mater Physics and Materials Science Dept.

    2014-10-01

    The role of antiferromagnetic spin correlations in high-temperature superconductors remains a matter of debate. We present inelastic neutron-scattering evidence that gapless spin fluctuations coexist with superconductivity in La1.905Ba0.095CuO4. Furthermore, we observe that both the low-energy magnetic spectral weight and the spin incommensurability are enhanced with the onset of superconducting correlations. We propose that the coexistence occurs through intertwining of spatial modulations of the pair wave function and the antiferromagnetic correlations. This proposal is also directly relevant to sufficiently underdoped La2-xSrxCuO4 and YBa2Cu3O6+x.

  13. Neutron-scattering evidence for a periodically modulated superconducting phase in the underdoped cuprate La1.905Ba0.095CuO4

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Xu, Zhijun; Stock, C.; Chi, Songxue; Kolesnikov, A. I.; Xu, Guangyong I.; Gu, Genda; Tranquada, J. M.

    2014-10-01

    The role of antiferromagnetic spin correlations in high-temperature superconductors remains a matter of debate. We present inelastic neutron-scattering evidence that gapless spin fluctuations coexist with superconductivity in La1.905Ba0.095CuO4. Furthermore, we observe that both the low-energy magnetic spectral weight and the spin incommensurability are enhanced with the onset of superconducting correlations. We propose that the coexistence occurs through intertwining of spatial modulations of the pair wave function and the antiferromagnetic correlations. This proposal is also directly relevant to sufficiently underdoped La2-xSrxCuO4 and YBa2Cu3O6+x.

  14. A portable hydro-thermo-mechanical loading cell for in-situ small angle neutron scattering studies of proton exchange membranes

    SciTech Connect (OSTI)

    Yu, Dunji [ORNL; An, Ke [ORNL; Gao, Carrie Y [ORNL; Heller, William T [ORNL; Chen, Xu [Tianjin UNiversity, China

    2013-01-01

    A portable hydro-thermo-mechanical loading cell has been designed to enable in-situ small angle neutron scattering (SANS) studies of proton exchange membranes (PEM) under immersed tensile loadings at different temperatures. The cell consists of three main parts as follows: a letter-paper-size motor-driven mechanical load frame, a SANS friendly reservoir that provides stable immersed and thermal sample conditions, and a data acquisition & control system. The ex-situ tensile tests of Nafion 212 membranes demonstrated a satisfactory thermo-mechanical testing performance of the cell for either dry or immersed conditions at elevated temperatures. The in-situ SANS tensile measurements on the Nafion 212 membranes immersed in D2O at 70oC proved the feasibility and capability of the cell for small angle scattering study on deformation behaviors of PEM and other polymer materials under hydro-thermo-mechanical loading.

  15. Neutron scattering studies of the H2a-H2b and (H3-H4)/sub 2/ histone complexes

    SciTech Connect (OSTI)

    Carlson, R.D.

    1982-01-01

    Neutron scattering experiments have shown that both the (H3-H4)/sub 2/ and H2a-H2b histone complexes are quite asymmetric in solution. The (H3-H4)/sub 2/ tetramer is an oblate or flattened structure, with a radius of gyration almost as large as that of the core octamer. If the tetramer is primarily globular, it must have an axial ratio of about 1:5. It is more likely, however, that this asymmetry results in part from N-terminal arms that extend outward approximately within the major plane of the particle. If this is the case, less asymmetric models for the globular part of the tetramer, including a dislocated disk, can be made consistent with the scattering data. The H2a-H2b dimer, on the other hand, is an elongated structure. 48 references, 12 figures, 1 table.

  16. Lujan Neutron Scattering Center

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power Administration would likeUniverseIMPACTThousandReport) | SciTech Connect Lower-Energyresponds to

  17. Neutron Science | ORNL

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    User Office User Program Manager Laura Morris Edwards 865.574.2966 ORNL study uses neutron scattering, supercomputing to demystify forces at play in biofuel production Full...

  18. Neutron rich nuclei and neutron stars

    E-Print Network [OSTI]

    C. J. Horowitz

    2013-03-01

    The PREX experiment at Jefferson Laboratory measures the neutron radius of 208Pb with parity violating electron scattering in a way that is free from most strong interaction uncertainties. The 208Pb radius has important implications for neutron rich matter and the structure of neutron stars. We present first PREX results, describe future plans, and discuss a follow on measurement of the neutron radius of 48Ca. We review radio and X-ray observations of neutron star masses and radii. These constrain the equation of state (pressure versus density) of neutron rich matter. We present a new energy functional that is simultaneously fit to both nuclear and neutron star properties. In this approach, neutron star masses and radii constrain the energy of neutron matter. This avoids having to rely on model dependent microscopic calculations of neutron matter. The functional is then used to predict the location of the drip lines and the properties of very neutron rich heavy nuclei.

  19. Measurement of porosity in a composite high explosive as a function of pressing conditions by ultra-small-angle neutron scattering with contrast variation

    SciTech Connect (OSTI)

    Mang, Joseph Thomas; Hjelm, Rex P; Francois, Elizabeth G

    2009-01-01

    We have used ultra-small-angle neutron scattering (USANS) with contrast variation to measure the porosity (voids and binder-filled regions) in a composite high explosive, PBX 9501, formulated with a deuterated binder. Little is known about the microstructure of pressed PBX 9501 parts and thus how it is affected by processing. Here, we explore the effect of varying the pressing intensity on the PBX 9501 microstructure. Disk-shaped samples of PBX 9501 were die-pressed with applied pressures ranging between 10,000 and 29,000 psi at 90 C. Five samples were prepared at each pressure that differed in the fraction of deuterated binder, facilitating variation of the neutron scattering length density contrast ({Delta}{rho}) and thus, the resolution of microstructural details. The sample composition was determined by calculation of the Porod Invariant as a function of {Delta}{rho} and compared with compositional estimates obtained from the bulk sample density. Structural modeling of the USANS data, at different levels of contrast, assuming both spherical and cylindrical morphologies, allowed the mean size and size distribution of voids and binder-filled regions to be determined. A decrease in the mean diameter of binder-filled regions was found with increasing pressing intensity, while the mean void diameter showed no significant change.

  20. Science Education Programs | Neutron Science | ORNL

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Scattering Tutorials Kids' Corner NScD Careers Supporting Organizations Neutron Science Home | Science & Discovery | Neutron Science | Science and Education SHARE Inspiring...

  1. Synchrotron X-ray Scattering Studies of Rapidly Evolving Nanoscale Interfacial Systems /

    E-Print Network [OSTI]

    Dai, Yeling

    2013-01-01

    Stanley. X-ray and neutron scattering from rough surfaces.Stanley. X-ray and neutron scattering from rough surfaces.grazing incidence x-ray and neutron scattering from ordered

  2. Analysis of Order Formation in Block Copolymer Thin Films Using Resonant Soft X-Ray Scattering

    E-Print Network [OSTI]

    Virgili, Justin M.; Tao, Yuefei; Kortright, Jeffrey B.; Balsara, Nitash P.; Segalman, Rachel A.

    2006-01-01

    Methods of X-Ray and Neutron Scattering in Polymer Science.µ t for X-ray and neutron scattering experiments is unity;18 In classical scattering of light, X-rays or neutrons the

  3. X-ray scattering studies of structure and dynamics of surfaces and interfaces of polymeric liquids

    E-Print Network [OSTI]

    Jiang, Zhang

    2007-01-01

    Evanescent X-ray and Neutron Scattering. Springer-Verlag,Methods of X-ray and neutron scattering in polymer science.Stanley. X-ray and neutron scattering from rough surfaces.

  4. Neutron and X-ray experiments at high temperature P. Aldebert (*)

    E-Print Network [OSTI]

    Boyer, Edmond

    neutron scattering have appeared as power- ful tools to get information, mainly structural temperature scattering devices compared to X-rays. At the present time thermal neutron high flux reactors be investigated by neutron scattering.

  5. Small-Angle Neutron Scattering and Electron Microscopy Study of the Wet and Dry High-Temperature Oxidation of Alumina- and Chromia- Forming Stainless Steels

    SciTech Connect (OSTI)

    Rother, Gernot [ORNL; Keiser, James R [ORNL; Brady, Michael P [ORNL; Unocic, Kinga A [ORNL; Anovitz, Lawrence {Larry} M [ORNL; Littrell, Ken [ORNL; Meisner, Roberta Ann [ORNL; Santella, Michael L [ORNL; Wesolowski, David J [ORNL; Cole, David R [ORNL

    2012-01-01

    Foils of T347 stainless steel and a developmental alumina-forming austenitic (AFA) stainless steel were oxidized at 800 C in dry air, air with 10% H2O, and air with 10% D2O. The T347 foils exhibited a transition to rapid Fe-base oxide formation between 24 and 72 h of exposure in H2O and D2O, but exhibited protective Cr-rich oxide formation in dry air. In contrast, only thin, protective Al-rich oxide surfaces were observed for the AFA alloy foils under all conditions studied. Changes in the small angle neutron scattering (SANS) signal were observed for the T347 stainless steel as a function of oxidation time in dry air, attributed to oxide grain growth and porosity formation/partial scale detachment associated with spinel phase at the scale/gas interface. For the AFA alloy, only minor changes in scattering as a result of oxidation time were observed. For both T347 and AFA, similar scattering was observed in dry and wet air (H2O and D2O) exposure. This finding indicates that water vapor exposure did not induce significant morphological changes in the oxide scales (such as increased porosity) in the 5-300 nm size regime accessed by SANS.

  6. Ferroelectric nanoscale domains and the 905 K phase transition in SrSnO{sub 3}: A neutron total-scattering study

    SciTech Connect (OSTI)

    Goodwin, Andrew L.; Redfern, Simon A. T.; Dove, Martin T.; Keen, David A.; Tucker, Matthew G.

    2007-11-01

    The 905 K Pnma-Imma phase transition in SrSnO{sub 3} is studied here using a combination of variable-temperature neutron total scattering together with the reverse Monte Carlo (RMC) refinement method. The real-space RMC configurations obtained are analyzed in terms of bond distance and bond-angle distributions, and a geometric algebra approach is used to quantify the associated octahedral-tilting distributions. What emerges from this analysis is that the transition is displacive in nature, in contrast to the results of a recent average-structure investigation in which an order-disorder model was proposed [E. H. Mountstevens et al., Phys. Rev. B 71, 220102(R) (2005)]. Three-dimensional diffuse scattering patterns calculated from the same RMC configurations reveal the existence of an additional disorder mechanism which persists across the Pnma-Imma transition. The ''reflection conditions'' of this diffuse scattering, together with displacement correlation calculations, point to the existence of ferroelectric nanoscale domains within the configurations, which are found to extend across planar regions of approximately 10-15 A ring in diameter.

  7. Characterization of a Thermo Scientific D711 D-T Neutron Generator Located in a Low-Scatter Facility

    SciTech Connect (OSTI)

    Hayes, John W.; Finn, Erin C.; Greenwood, Lawrence R.; Wittman, Richard S.

    2014-03-21

    Pacific Northwest National Laboratory (PNNL) purchased and installed a D711 D-T neutron generator (“D-T”) from Thermo Scientific in August 2011. The D-T nominally produces 14 MeV neutrons which are important for research in matters of national security. Fast neutrons provide the capability of harnessing threshold reactions for the production of rare isotopes, which are of interest to radiochemistry groups at PNNL concerned with validating radioanalytical techniques for the separation of these isotopes. Rare fission product isotopes from fast fission of 235U, 238U, and 239Pu are also desired to further develop these techniques. Experiments with 14 MeV neutrons are also of interest because nuclear data for fast fission has not been researched as extensively as it has been for thermal fission. Analyses of these applications require first that the source spectrum be well characterized. Neutron fluences in Fe, Ni, Al, In, and Au were measured in 21 locations near the generator head. STAYSL PNNL and MCNP codes were used to produce flux spectra based on experimental fluences.

  8. Application of small-angle neutron scattering to the study of forces between magnetically chained monodisperse ferrofluid emulsion droplets

    SciTech Connect (OSTI)

    Jain, Dr Nirmesh [University of Sydney, Australia] [University of Sydney, Australia; Liu, Dr C K [Institute of Materials research and Engineering, A-STAR, Singapore] [Institute of Materials research and Engineering, A-STAR, Singapore; Hawkett, Dr B. S. [University of Sydney, Australia] [University of Sydney, Australia; Warr, G. G. [University of Sydney, Australia] [University of Sydney, Australia; Hamilton, William A [ORNL] [ORNL

    2014-01-01

    The optical magnetic chaining technique (MCT) developed by Leal-Calderon, Bibette and co-workers in the 1990 s allows precise measurements of force profiles between droplets in monodisperse ferrofluid emulsions. However, the method lacks an in-situ determination of droplet size and therefore requires the combination of separately acquired measurements of droplet chain periodicity versus an applied magnetic field from optical Bragg scattering and droplet diameter inferred from dynamic light scattering (DLS) to recover surface force-distance profiles between the colloidal particles. Compound refractive lens (CRL) focussed small-angle scattering (SANS) MCT should result in more consistent measurements of droplet size (form factor measurements in the absence of field) and droplet chaining period (from structure factor peaks when the magnetic field is applied); and, with access to shorter length scales, extend force measurements to closer approaches than possible by optical measurements. We report on CRL-SANS measurements of monodisperse ferrofluid emulsion droplets aligned in straight chains by an applied field perpendicular to the incident beam direction. Analysis of the scattering from the closely spaced droplets required algorithms that carefully treated resolution and its effect on mean scattering vector magnitudes in order to determine droplet size and chain periods to sufficient accuracy. At lower applied fields scattering patterns indicate structural correlations transverse to the magnetic field direction due to the formation of intermediate structures in early chain growth.

  9. PHYSICAL REVIEW C 86, 024612 (2012) Neutrino-nucleus coherent scattering as a probe of neutron density distributions

    E-Print Network [OSTI]

    Engel, Jonathan

    2012-01-01

    provides a theoretically appealing way to measure the neutron part of nuclear form factors. Using an expansion of form factors into moments, we show that neutrinos from stopped pi- ons can probe not only of various nuclear energy functionals. DOI: 10.1103/PhysRevC.86.024612 PACS number(s): 25.30.Pt, 21.10.Gv, 21

  10. A high resolution neutron scattering study of Tb2Mo2O7: A geometrically frustrated and disorder-free spin glass

    SciTech Connect (OSTI)

    Ehlers, Georg; Gardner, Jason; Qiu, Y.; Rule, K; Greedan, John E; Stewart, John Ross; Fouquet, Peter; Cornelius, A. L.; Adriano, Cris; Pagliuso, P G

    2010-01-01

    Neutron scattering, muon spin relaxation, and de susceptibility studies have been carried out on polycrystalline Tb{sub 2}Ti{sub 2}O{sub 7}, a pyrochlore antiferromagnet in which the Tb{sup 3+} moments reside on a network of corner-sharing tetrahedra. Unlike other geometrically frustrated systems, Tb{sub 2}Ti{sub 2}O{sub 7} remains paramagnetic down to {approx}0.07 K, rather than ordering into a conventional Neel or spin-glass-like state, despite the fact that short-range antiferromagnetic correlations (AFC) develop at {approx}50 K. At the first AFC wave vector, its low-lying, relatively flat magnetic excitation spectrum softens partially below 30 K.

  11. Level crossings and zero-field splitting in the {Cr8}-cubane spin-cluster studied using inelastic neutron scattering and magnetization

    SciTech Connect (OSTI)

    Vaknin, D.; Garlea, Vasile O; Demmel, F.; Mamontov, Eugene; Nojiri, H; Martin, Catalin; Chiorescu, Irinel; Qiu, Y.; Luban, M.; Kogerler, P.; Fielden, J.; Engelhardt, L; Rainey, C

    2010-01-01

    Inelastic neutron scattering (INS) in variable magnetic field and high-field magnetization measurements in the millikelvin temperature range were performed to gain insight into the low-energy magnetic excitation spectrum and the field-induced level crossings in the molecular spin cluster {Cr8}-cubane. These complementary techniques provide consistent estimates of the lowest level-crossing field. The overall features of the experimental data are explained using an isotropic Heisenberg model, based on three distinct exchange interactions linking the eight CrIII paramagnetic centers (spins s = 3/2), that is supplemented with a relatively large molecular magnetic anisotropy term for the lowest S = 1 multiplet. It is noted that the existence of the anisotropy is clearly evident from the magnetic field dependence of the excitations in the INS measurements, while the magnetization measurements are not sensitive to its effects.

  12. Structural evolution across the insulator-metal transition in oxygen-deficient BaTiO3-? studied using neutron total scattering and Rietveld analysis

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Jeong, I.-K.; Lee, Seunghun; Jeong, Se-Young; Won, C. J.; Hur, N.; Llobet, A.

    2011-08-01

    Oxygen-deficient BaTiO3-? exhibits an insulator-metal transition with increasing ?. We performed neutron total scattering measurements to study structural evolution across an insulator-metal transition in BaTiO3-?. Despite its significant impact on resistivity, slight oxygen reduction (?=0.09) caused only a small disturbance on the local doublet splitting of Ti-O bond. This finding implies that local polarization is well preserved under marginal electric conduction. In the highly oxygen-deficient metallic state (?=0.25), however, doublet splitting of the Ti-O bond became smeared. The smearing of the local Ti-O doublet is complemented with long-range structural analysis and demonstrates that the metallic conduction in the highly oxygen-reducedmore »BaTiO3-? is due to the appearance of nonferroelectric cubic lattice.« less

  13. Negative Thermal Expansion in ZrW{sub 2}O{sub 8}: Mechanisms, Rigid Unit Modes, and Neutron Total Scattering

    SciTech Connect (OSTI)

    Tucker, Matthew G. [Department of Earth Sciences, University of Cambridge, Downing Street, Cambridge CB2 3EQ (United Kingdom); ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot, Oxon OX11 0QX (United Kingdom); Goodwin, Andrew L.; Dove, Martin T. [Department of Earth Sciences, University of Cambridge, Downing Street, Cambridge CB2 3EQ (United Kingdom); Keen, David A. [Physics Department, Oxford University, Clarendon Laboratory, Parks Road, Oxford OX1 3PU (United Kingdom); ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot, Oxon OX11 0QX (United Kingdom); Wells, Stephen A. [Biological Physics, Bateman Physical Sciences Building, Arizona State University, Tempe, Arizona 85287-1504 (United States); Evans, John S.O. [Department of Chemistry, University Science Laboratories, South Road, Durham DH1 3LE (United Kingdom)

    2005-12-16

    The local structure of the low-temperature ordered phase of the negative thermal expansion (NTE) material ZrW{sub 2}O{sub 8} has been investigated by reverse Monte Carlo (RMC) modeling of neutron total scattering data. We obtain, for the first time, quantitative measurements of the extent to which the WO{sub 4} and ZrO{sub 6} polyhedra move as rigid units, and we show that these values are consistent with the predictions of rigid unit mode theory. We suggest that rigid unit modes are associated with the NTE. Our results do not support a recent interpretation of x-ray-absorption fine structure spectroscopy data in terms of a larger rigid structural component involving the Zr-O-W linkage.

  14. Neutron scattering evidence for isolated spin-1/2 ladders in (C5D12N)2CuBr4

    SciTech Connect (OSTI)

    Savici, Andrei T [ORNL; Granroth, Garrett E [ORNL; Broholm, Collin L [ORNL; Pajerowski, Daniel M. [University of Florida, Gainesville; Brown, Craig [National Institute of Standards and Technology (NIST); Talham, Daniel R. [University of Florida, Gainesville; Meisel, Mark W. [University of Florida, Gainesville; Schmidt, K. P. [Technische Universit Dortmund, Germany; Uhrig, G. S. [Technische Universit Dortmund, Germany; Nagler, Stephen E [ORNL

    2009-01-01

    Inelastic neutron scattering was used to determine the spin Hamiltonian for the singlet ground state system (C5D12N)2CuBr4 (BPCB). A 2-leg spin 1/2 ladder model, with J? = 1:084 0:005 meV and Jk = 0:321 0:008 meV, accurately describes the data. The experimental limit on the inter-ladder exchange constant is jJ0j 0.005 meV, and the limit on diagonal, intra-ladder exchange is jJF j 0.1 meV. The experimental ratios of intra-ladder bond energies are consistent with the predictions of continuous unitary transformations calculations.

  15. Structural evolution across the insulator-metal transition in oxygen-deficient BaTiO3-? studied using neutron total scattering and Rietveld analysis

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Jeong, I.-K.; Lee, Seunghun; Jeong, Se-Young; Won, C. J.; Hur, N.; Llobet, A.

    2011-08-01

    Oxygen-deficient BaTiO3-? exhibits an insulator-metal transition with increasing ?. We performed neutron total scattering measurements to study structural evolution across an insulator-metal transition in BaTiO3-?. Despite its significant impact on resistivity, slight oxygen reduction (?=0.09) caused only a small disturbance on the local doublet splitting of Ti-O bond. This finding implies that local polarization is well preserved under marginal electric conduction. In the highly oxygen-deficient metallic state (?=0.25), however, doublet splitting of the Ti-O bond became smeared. The smearing of the local Ti-O doublet is complemented with long-range structural analysis and demonstrates that the metallic conduction in the highly oxygen-reduced BaTiO3-? is due to the appearance of nonferroelectric cubic lattice.

  16. Nuclear Instruments and Methods in Physics Research A 566 (2006) 598608 The number distribution of neutrons and gamma photons generated in a

    E-Print Network [OSTI]

    Pázsit, Imre

    2006-01-01

    of neutrons and gamma photons generated in a multiplying sample Andreas Enqvista,�, Imre Pa´ zsita , Sara is an analytical derivation of the full probability distribution of the number of neutrons and photons generated. With the introduction of a modified factorial moment of the number of neutrons and gamma photons generated in fission

  17. Models to analyze small-angle neutron scattering from unilamellar lipid vesicles Norbert Kucerka* and John F. Nagle

    E-Print Network [OSTI]

    Nagle, John F.

    (bending modulus and compressibility modulus) for the liquid crystal array [2]. The second approach-angle scattering has been employed to study the structure of lipid bilayers in unilamellar vesicles. This paper to lipid bilayer structure that is the subject of this paper studies samples composed of unilamel- lar

  18. Pulsed-neutron monochromator

    DOE Patents [OSTI]

    Mook, H.A. Jr.

    1984-01-01

    In one aspect, the invention is an improved pulsed-neutron monochromator of the vibrated-crystal type. The monochromator is designed to provide neutron pulses which are characterized both by short duration and high density. A row of neutron-reflecting crystals is disposed in a neutron beam to reflect neutrons onto a common target. The crystals in the row define progressively larger neutron-scattering angles and are vibrated sequentially in descending order with respect to the size of their scattering angles, thus generating neutron pulses which arrive simultaneously at the target. Transducers are coupled to one end of the crystals to vibrate them in an essentially non-resonant mode. The transducers propagate transverse waves in the crystal which progress longitudinally therein. The waves are absorbed at the undriven ends of the crystals by damping material mounted thereon. In another aspect, the invention is a method for generating neutron pulses characterized by high intensity and short duration.

  19. Pulsed-neutron monochromator

    DOE Patents [OSTI]

    Mook, Jr., Herbert A. (Oak Ridge, TN)

    1985-01-01

    In one aspect, the invention is an improved pulsed-neutron monochromator of the vibrated-crystal type. The monochromator is designed to provide neutron pulses which are characterized both by short duration and high density. A row of neutron-reflecting crystals is disposed in a neutron beam to reflect neutrons onto a common target. The crystals in the row define progressively larger neutron-scattering angles and are vibrated sequentially in descending order with respect to the size of their scattering angles, thus generating neutron pulses which arrive simultaneously at the target. Transducers are coupled to one end of the crystals to vibrate them in an essentially non-resonant mode. The transducers propagate transverse waves in the crystal which progress longitudinally therein. The wave are absorbed at the undriven ends of the crystals by damping material mounted thereon. In another aspect, the invention is a method for generating neutron pulses characterized by high intensity and short duration.

  20. Quark-model Baryon-Baryon Interaction Applied to the Neutron-Deuteron Scattering. I Noyes-Kowalski Approach to the AGS Equations

    E-Print Network [OSTI]

    Yoshikazu Fujiwara; Kenji Fukukawa

    2011-02-15

    We solve the neutron-deuteron (nd) scattering in the Faddeev formalism, employing the NN sector of the quark-model baryon-baryon interaction fss2. The energy-dependence of the NN interaction, inherent to the resonating-group formulation of the quark-model baryon-baryon interaction, is eliminated by the standard off-shell transformation utilizing the normalization kernel of two-cluster systems. An extra nonlocality originating from this procedure is very important to reproduce all the nd scattering observables below E_n Green function is shown in detail, which is based on the spline function method originally developed by the Bochum-Krakow group. The predicted elastic differnetial cross sections reproduce the observed deep cross section minima at E_n=35-65 MeV and $\\theta_{c.m}=130^{\\circ}-135^{\\circ}$, which is consitent with the nearly correct triton binding energy predicted by fss2 without the three-body force.

  1. Neutron Science | More Science | ORNL

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ORNL's long history of neutron science began in the 1940s with the pioneering neutron scattering studies of Ernest Wollan and Clifford Shull. Shull was co-recipient of...

  2. Multiple-Input Data Acquisition System (MIDAS) for Measuring the Carbon Content in Soil Using Inelastic Neutron Scattering

    SciTech Connect (OSTI)

    Warburton, William K.

    2014-01-24

    This report describes work funder under STTR grants Phase I and II and carried out jointly by XIA LLC and Brookhaven National Laboratory (BNL). The project goal was to develop a mobile nuclear activation analysis instrument that could be towed behind a tractor to document soil carbon levels in agricultural lands for carbon credit certification. XIA developed large NaI(Tl) detectors with integrated digital pulse processors controlled over USB 2.0 and delivered 16 of these units to BNL for integration into the prototype instrument, together with the necessary software to calibrate them and collect data. For reasons that are unknown to XIA, the BNL participants never completed the prototype vehicle, performed system integration, or carried out the proposed qualification and field tests, leaving the project incomplete.

  3. Raw neutron scattering data for strain measurement of hydraulically loaded granite and marble samples in triaxial stress state

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Polsky, Yarom

    This entry contains raw data files from experiments performed on the Vulcan beamline at the Spallation Neutron Source at Oak Ridge National Laboratory using a pressure cell. Cylindrical granite and marble samples were subjected to confining pressures of either 0 psi or approximately 2500 psi and internal pressures of either 0 psi, 1500 psi or 2500 psi through a blind axial hole at the center of one end of the sample. The sample diameters were 1.5" and the sample lengths were 6". The blind hole was 0.25" in diameter and 3" deep. One set of experiments measured strains at points located circumferentially around the center of the sample with identical radii to determine if there was strain variability (this would not be expected for a homogeneous material based on the symmetry of loading). Another set of experiments measured load variation across the radius of the sample at a fixed axial and circumferential location. Raw neutron diffraction intensity files and experimental parameter descriptions are included.

  4. Raw neutron scattering data for strain measurement of hydraulically loaded granite and marble samples in triaxial stress state

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Polsky, Yarom

    2014-05-23

    This entry contains raw data files from experiments performed on the Vulcan beamline at the Spallation Neutron Source at Oak Ridge National Laboratory using a pressure cell. Cylindrical granite and marble samples were subjected to confining pressures of either 0 psi or approximately 2500 psi and internal pressures of either 0 psi, 1500 psi or 2500 psi through a blind axial hole at the center of one end of the sample. The sample diameters were 1.5" and the sample lengths were 6". The blind hole was 0.25" in diameter and 3" deep. One set of experiments measured strains at points located circumferentially around the center of the sample with identical radii to determine if there was strain variability (this would not be expected for a homogeneous material based on the symmetry of loading). Another set of experiments measured load variation across the radius of the sample at a fixed axial and circumferential location. Raw neutron diffraction intensity files and experimental parameter descriptions are included.

  5. The Neutron Science TeraGrid Gateway, a TeraGrid Science Gateway to Support the Spallation Neutron Source

    E-Print Network [OSTI]

    Vazhkudai, Sudharshan

    by a service oriented architecture for functional implementation. KEY WORDS: Portal, Neutron Scattering, TeraGrid, Science Gateway, Service Architecture, Grid 1. INTRODUCTION Neutron Science: Neutron scattering is used, earth science, and fundamental physics [3]. As a diagnostic tool, neutron scattering provides unique

  6. Supporting Organizations | Neutron Science | ORNL

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    materials. The user community takes advantage of division-supported capabilities of neutron scattering for measurements over wide ranges of experimental and operating...

  7. Neutron Science Laboratory The Neutron Science Laboratory (NSL) has been playing

    E-Print Network [OSTI]

    Katsumoto, Shingo

    Neutron Science Laboratory The Neutron Science Laboratory (NSL) has been playing a central role in neutron scattering activities in Japan since 1961 by performing its own research programs as well as providing a strong general user program for the university- owned various neutron scattering spectrometers

  8. Paul Langan to lead ORNL's Neutron Sciences Directorate | ornl...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    science activities, which include two leading DOE Office of Science user facilities for neutron scattering analysis: The Spallation Neutron Source (SNS) and the High Flux Isotope...

  9. Neutrons provide new insights into human cell behavior

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    institutions, are breaking new ground in cellular biology through the application of neutron-scattering techniques. "Neutrons have advantages over other imaging probes, such...

  10. Small-angle neutron scattering study of magnetic ordering and inhomogeneity across the martensitic phase transformation in Ni50–xCoxMn??Sn?? alloys

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Bhatti, Kanwal Preet; El-Khatib, S.; Srivastava, Vijay; James, R. D.; Leighton, C.

    2012-04-27

    The Heusler-derived multiferroic alloy Ni50–xCoxMn??Sn?? has recently been shown to exhibit, at just above room temperature, a highly reversible martensitic phase transformation with an unusually large magnetization change. In this work the nature of the magnetic ordering above and below this transformation has been studied in detail in the critical composition range x = 6–8 via temperature-dependent (5–600 K) magnetometry and small-angle neutron scattering (SANS). We observe fairly typical paramagnetic to long-range-ordered ferromagnetic phase transitions on cooling to 420–430 K, with the expected critical spin fluctuations, followed by first-order martensitic phase transformations to a nonferromagnetic state below 360–390 K. Themore »static magnetization reveals complex magnetism in this low-temperature nonferromagnetic phase, including a Langevin-like field dependence, distinct spin freezing near 60 K, and significant exchange bias effects, consistent with superparamagnetic blocking of ferromagnetic clusters of nanoscopic dimensions. We demonstrate that these spin clusters, whose existence has been hypothesized in a variety of martensitic alloys exhibiting competition between ferromagnetic and antiferromagnetic exchange interactions, can be directly observed by SANS. The scattering data are consistent with a liquidlike spatial distribution of interacting magnetic clusters with a mean center-to-center spacing of 12 nm. Considering the behavior of the superparmagnetism, cooling-field and temperature-dependent exchange bias, and magnetic SANS, we discuss in detail the physical form and origin of these spin clusters, their intercluster interactions, the nature of the ground-state magnetic ordering in the martensitic phase, and the implications for our understanding of such alloy systems.« less

  11. Solution Structure of an Amyloid-Forming Protein During Photoinitiated Hexamer-Dodecamer Transitions Revealed Through Small-Angle Neutron Scattering

    SciTech Connect (OSTI)

    Hamill,A.; Wang, S.; Lee, Jr., C.

    2007-01-01

    Shape-reconstruction analysis applied to small angle neutron scattering (SANS) data is used to determine the in vitro conformations of {alpha}-chymotrypsin oligomers that form as a result of partial unfolding with a photoresponsive surfactant. In the presence of the photoactive surfactant under visible light, the native oligomers (dimers or compact hexamers) rearrange into expanded corkscrew-like hexamers. Converting the surfactant to the photopassive form with UV light illumination causes the hexamers to laterally aggregate and intertwine into dodecamers with elongated, twisted conformations containing cross-sectional dimensions similar to amyloid protofilaments. Secondary-structure measurements with FT-IR indicate that this photoinduced hexamer-to-dodecamer association occurs through intermolecular {beta} sheets stabilized with hydrogen bonds, similar to amyloid formation. Traditional structural characterization techniques such as X-ray crystallography and NMR are not easily amenable to the study of these non-native protein conformations; however, SANS is ideally suited to the study of these associated intermediates, providing direct observation of the mechanism of oligomeric formation in an amyloid-forming protein. Combined with photoinitiated hexamer-to-dodecamer associations in the presence of the photoresponsive surfactant, this study could provide unique insight into the amyloidosis disease pathway, as well as novel disease treatment strategies.

  12. Characterization of nanostructured zirconia prepared by hydrolysis and reverse micelle synthesis by small-angle neutron and X-ray scattering

    SciTech Connect (OSTI)

    Thiyagarajan, P.; Li, X.; Littrell, K.; Seifert, S.; Csencsits, R.; Loong, C.

    1999-12-07

    Low temperature techniques such as hydrolysis and reverse micelle syntheses provide the opportunity to determine the relationship between the structural properties and preparation conditions of zirconia powders as well as to tailor their physicochemical properties. The authors have performed small-angle neutron and synchrotron X-ray scattering (SANS and SAXS) experiments to study the nucleation and organization of zirconia nanoparticles via different preparation routes. First, the formation of reverse micelles in individual and mixed solutions of (ZrOCl{sub 2}+D{sub 2}O)/AOT/C{sub 6}D{sub 5}CD{sub 3}, and (NH{sub 4}OH+H{sub 2}O)/AOT/C{sub 6}D{sub 5}CD{sub 3} systems at water/AOT molar ratio of 20 was characterized. Second, the aggregation of zirconia gels obtained from the reaction of the reverse micelle solutions after heat treatments was studied. Third, the nanostructure of zirconia powders prepared by the reverse micelle method is compared with the corresponding powders prepared by hydrolysis after different heat treatments.

  13. Nuclear Instruments and Methods in Physics Research A 432 (1999) 403}409 Measurement of the thermal and fast neutron #ux in a research

    E-Print Network [OSTI]

    Pázsit, Imre

    1999-01-01

    the neutron converter material to measure neu- trons of various energies, such as fast, thermal and epithermal positions, such as between the fuel plates of an MTR-type reactor. At the same time, its sensitive volume

  14. LIGHT SCATTERING STUDIES OF SILICA AEROGELS

    E-Print Network [OSTI]

    Hunt, A.J.

    2010-01-01

    van de Hulst, H.C. , Light Scattering by Small Particles,A New Polarization-Modulated Light Scattering Instrument,"and interpretation of light scattering effects in aerogels.

  15. Canonical quantum potential scattering theory

    E-Print Network [OSTI]

    M. S. Hussein; W. Li; S. Wuester

    2008-07-13

    A new formulation of potential scattering in quantum mechanics is developed using a close structural analogy between partial waves and the classical dynamics of many non-interacting fields. Using a canonical formalism we find non-linear first-order differential equations for the low energy scattering parameters like scattering length and effective range. They significantly simplify typical calculations, as we illustrate for atom-atom and neutron-nucleus scattering systems. A generalization to charged particle scattering is also possible.

  16. Neutron-deuteron breakup reaction as a tool for studying neutron-neutron interactions

    SciTech Connect (OSTI)

    Konobeevski, E. S., E-mail: konobeev@inr.ru; Zuyev, S. V.; Mordovskoy, M. V.; Potashev, S. I.; Sharapov, I. M. [Russian Academy of Sciences, Institute for Nuclear Research (Russian Federation)] [Russian Academy of Sciences, Institute for Nuclear Research (Russian Federation)

    2013-11-15

    An analysis of the most recent data on the reaction nd {yields} pnn revealed a serious discrepancy between theoretical predictions and cross sections measured for this reaction in various configurations where the role of neutron-neutron interactions is important. In view of this, it seems necessary both to develop theoretical approaches and to obtain new experimental data. For this purpose, a setup for studying the neutron-deuteron breakup reaction was created at the Institute for Nuclear Research on the basis of the neutron beam in the RADEX channel and deuterium targets. This facility makes it possible to perform experiments over a broad region of primary-neutron energies (10-60 MeV) and in various (final-state interaction, quasifree scattering, and spatial-star) configurations. Preliminary results of the respective experiment were obtained for configurations of final-state neutron-neutron interaction and quasifree neutron-neutron scattering.

  17. Neutron Detection Efficiency of the

    E-Print Network [OSTI]

    Gilfoyle, Jerry

    Neutron Detection Efficiency of the CLAS12 Detector M. Moog and G. Gilfoyle University Of Richmond - Department of Physics Software We simulated the neutron detection efficiency of the forward time of flight scintillators for quasielastic electron-neutron scattering using a series of software packages. Elastic

  18. Applications of compact accelerator-driven neutron sources: An updated assessment from the perspective of materials research in Italy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Andreani, C.; Anderson, I. S.; Carpenter, J. M.; Festa, G.; Gorini, G.; Loong, C. -K.; Senesi, R.

    2014-12-24

    In 2005 the International Atomic Energy Agency (IAEA) in Vienna published a report [1] on ‘Development Opportunities of Small and Medium Scale Accelerator Driven Neutron Sources’ which summarized the prospect of smaller sources in supporting the large spallation neutron sources for materials characterization and instrumentation, a theme advocated by Bauer, Clausen, Mank, and Mulhauser in previous publications [2-4]. In 2010 the Union for Compact Accelerator-driven Neutron Sources (UCANS) was established [5], galvanizing cross-disciplinary collaborations on new source and neutronics development and expanded applications based on both slow-neutron scattering and other neutron-matter interactions of neutron energies ranging from 10?? to 10²more »MeV [6]. Here, we first cover the recent development of ongoing and prospective projects of compact accelerator-driven neutron sources (CANS) but concentrate on prospective accelerators currently proposed in Italy. Two active R&D topics, irradiation effects on electronics and cultural heritage studies, are chosen to illustrate the impact of state-of-the-art CANS on these programs with respect to the characteristics and complementarity of the accelerator and neutronics systems as well as instrumentation development.« less

  19. Applications of compact accelerator-driven neutron sources: An updated assessment from the perspective of materials research in Italy

    SciTech Connect (OSTI)

    Andreani, C. [Università degli studi di Roma Tor Vergata Centre NAST, Rome (Italy); Anderson, I. S. [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Carpenter, J. M. [Argonne National Lab. (ANL), Argonne, IL (United States); Festa, G. [Università degli studi di Roma Tor Vergata Centre NAST, Rome (Italy); Gorini, G. [Universita' degli Studi di Milano - Bicocca, Milano (Italy); Loong, C. -K. [Università degli studi di Roma Tor Vergata Centre NAST, Rome (Italy); Senesi, R. [Università degli studi di Roma Tor Vergata Centre NAST, Rome (Italy)

    2014-12-24

    In 2005 the International Atomic Energy Agency (IAEA) in Vienna published a report [1] on ‘Development Opportunities of Small and Medium Scale Accelerator Driven Neutron Sources’ which summarized the prospect of smaller sources in supporting the large spallation neutron sources for materials characterization and instrumentation, a theme advocated by Bauer, Clausen, Mank, and Mulhauser in previous publications [2-4]. In 2010 the Union for Compact Accelerator-driven Neutron Sources (UCANS) was established [5], galvanizing cross-disciplinary collaborations on new source and neutronics development and expanded applications based on both slow-neutron scattering and other neutron-matter interactions of neutron energies ranging from 10?? to 10² MeV [6]. Here, we first cover the recent development of ongoing and prospective projects of compact accelerator-driven neutron sources (CANS) but concentrate on prospective accelerators currently proposed in Italy. Two active R&D topics, irradiation effects on electronics and cultural heritage studies, are chosen to illustrate the impact of state-of-the-art CANS on these programs with respect to the characteristics and complementarity of the accelerator and neutronics systems as well as instrumentation development.

  20. Structure Transition in PSS/Lysozyme Complexes: A Chain-Conformation-Driven Process, as Directly Seen by Small Angle Neutron Scattering

    E-Print Network [OSTI]

    Jérémie Gummel; Fabrice Cousin; François Boué

    2009-03-30

    Measurements of chain conformation in proteins/polyelectrolytes complexes (lysozyme and PSSNa) show that the crossover observed between an open structure -a chain network crosslinked by the proteins, and a globular one - dense globules of ~ 10 nm aggregated in a fractal way, results from a conformation modification prior to the transition. Before showing this, we have widened the parameters range for the observation of the transition. We had shown before that the two structures can be formed depending on chain length (for a given [PSS]/[lysozyme] ratio): gel for large chains, globules for short chains. We show here that the crossover between these two regimes can also be reached as a function of chains concentration or salinity of the buffer. Since all these crossover parameters act on chains overlapping concentration c*, we reinforce the idea of a transition from the dilute to the semi-dilute regime, but c* is shifted compared to pure PSS solutions. In order to understand this, we have measured by SANS the conformation of a single chain of PSS in presence of proteins within the complexes. This is achieved by a specific labeling trick where we take advantage of the fact that lysozyme and hydrogenated PSS chains have the same neutron scattering length density. In the gel structure, the PSS chains keep a wormlike structure as in pure solutions, but their persistence length is strongly reduced, from 50 {\\AA} without proteins to 20 {\\AA} in average with lysozyme. With this value of 20 {\\AA}, we calculate new overlapping thresholds (concentration, mass, ionic strength) in agreement with observed ones. In a second stage, after the globular structure is formed, the PSS chains get a third conformation, no longer wormlike, but more collapsed, within the globules.