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Sample records for mo ne nh

  1. Theoretical investigation of HNgNH{sub 3}{sup +} ions (Ng = He, Ne, Ar, Kr, and Xe)

    SciTech Connect (OSTI)

    Gao, Kunqi; Sheng, Li

    2015-04-14

    The equilibrium geometries, harmonic frequencies, and dissociation energies of HNgNH{sub 3}{sup +} ions (Ng = He, Ne, Ar, Kr, and Xe) were investigated using the following method: Becke-3-parameter-Lee-Yang-Parr (B3LYP), Boese-Matrin for Kinetics (BMK), second-order Mller-Plesset perturbation theory (MP2), and coupled-cluster with single and double excitations as well as perturbative inclusion of triples (CCSD(T)). The results indicate that HHeNH{sub 3}{sup +}, HArNH{sub 3}{sup +}, HKrNH{sub 3}{sup +}, and HXeNH{sub 3}{sup +} ions are metastable species that are protected from decomposition by high energy barriers, whereas the HNeNH{sub 3}{sup +} ion is unstable because of its relatively small energy barrier for decomposition. The bonding nature of noble-gas atoms in HNgNH{sub 3}{sup +} was also analyzed using the atoms in molecules approach, natural energy decomposition analysis, and natural bond orbital analysis.

  2. Effective hole extraction using MoO{sub x}-Al contact in perovskite CH{sub 3}NH{sub 3}PbI{sub 3} solar cells

    SciTech Connect (OSTI)

    Zhao, Yixin; Nardes, Alexandre M.; Zhu, Kai

    2014-05-26

    We report an 11.4%-efficient perovskite CH{sub 3}NH{sub 3}PbI{sub 3} solar cell using low-cost molybdenum oxide/aluminum (i.e., MoO{sub x}/Al) as an alternative top contact to replace noble/precious metals (e.g., Au or Ag) for extracting photogenerated holes. The device performance of perovskite solar cells using a MoO{sub x}/Al top contact is comparable to that of cells using the standard Ag top contact. Analysis of impedance spectroscopy measurements suggests that using 10-nm-thick MoO{sub x} and Al does not affect charge-recombination properties of perovskite solar cells. Using a thicker (20-nm) MoO{sub x} layer leads to a lower cell performance caused mainly by a reduced fill factor. Our results suggest that MoO{sub x}/Al is promising as a low-cost and effective hole-extraction contact for perovskite solar cells.

  3. 19Ne

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ne β+-Decay Evaluated Data Measurements 1939WH02: 19Ne. 1952SC15: 19Ne. 1954JO21: 19Ne. 1954NA29: 19Ne. 1957AL29: 19Ne. 1957PE12: 19Ne. 1958WE25: 19Ne. 1960JA12: 19Ne; measured not abstracted; deduced nuclear properties. 1960WA04: 19Ne; measured not abstracted; deduced nuclear properties. 1962EA02: 19Ne; measured not abstracted; deduced nuclear properties. 1964VA23: 19Ne; measured not abstracted; deduced nuclear properties. 1968GO10: 19Ne; measured T1/2. 1972LE33: 19Ne; measured K/β+ ratios.

  4. MO: ZL

    Office of Legacy Management (LM)

    II , --fsi2L /~YlO MO: ZL W./O -1 ;3UN 2 2 1984 DeLanr 6/W/f. NE-20 -24 Authorization for Remedial Action at the Seaway Industrial Park and Ashland 0 1 Co. (I) Sites at Tonawanda, 9 NY, and Mallinckrodt Chemical Co., St. Louis, MO Ba 1s J. LaGrone, Eianager Oak Ridge Operations Office 6/20/E We have determined that the subject sites are contaminated with residual NE-20 radioactive material as a result of the Manhattan Engineer District/Atomic ,/"/1. EnergyXommission operations at those

  5. 17Ne

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ne +-Decay Evaluated Data Measurements 1964MC16: 17Ne; measured not abstracted; deduced nuclear properties. 1966HA22: 17Ne; deduced log ft. 1967ES02: 17Ne; measured not...

  6. 18Ne

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ne β+-Decay Evaluated Data Measurements 1954GO17: 18Ne. 1961BU05: 18Ne; measured not abstracted; deduced nuclear properties. 1961EC02: 18Ne; measured not abstracted; deduced nuclear properties. 1963FR10: 18Ne; measured not abstracted; deduced nuclear properties. 1965FR09: 18Ne; measured not abstracted; deduced nuclear properties. 1968GO05: 18Ne; measured Eγ, Iγ; deduced Iβ, log ft. 18F deduced levels, branching ratios. 1970AL11: 18Ne; measured T1/2; deduced log ft, β-branching. 1970AS06,

  7. 15Ne

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ne Ground-State Decay Evaluated Data Measured Ground-State Γcm for 15Ne Adopted value: 0.59 MeV (2014WA09) Measured Mass Excess for 15Ne Adopted value: 40215 ± 69 keV (2014WA09) Measurements 2014WA09: C(17Ne, 2p)15Ne, E = 500 MeV/nucleon; measured reaction products; deduced fractional energy spectra, J, π, energy levels, atomic mass excess. 15Ne(2p); measured decay products, Ep, Ip; deduced implications for 13O + p + p system. Back to Top Back to Ground-State Decays Data Main Page Back to

  8. 16Ne

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ne Ground-State Decay Evaluated Data Measured Ground-State Γcm for 16Ne Adopted value: 122 ± 37 keV (1993TI07) Measured Mass Excess for 16Ne Adopted value: 23996 ± 20 keV (2003AU02) Measurements 1971MAXQ: 16O(π+, π-); measured particle spectra, σ. 1977HO13: 16O(π+, π-), E = 145 MeV; measured σ; deduced Q. 16Ne deduced mass excess. 1977KEZX: 20Ne(α, 8He), E = 118 MeV; measured σ. 16Ne deduced levels, mass excess. 1978BU09: 16O(π+, π-), E = 145 MeV; measured σ. 16Ne deduced mass

  9. Public Service Co of NH | Open Energy Information

    Open Energy Info (EERE)

    EversourceNH Outage Hotline: 800-662-7764 Outage Map: www.eversource.comContentgen Green Button Access: Implemented Green Button Landing Page: www.psnh.comSaveEnergyMo...

  10. Recent Results from MiniBooNE

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Results from MiniBooNE and the Future Project LBNE Christopher Mauger 18 December 2009 Los Alamos NaEonal Laboratory Outline * Overview of MiniBooNE * Recent OscillaEon Results * IntroducEon to the Next GeneraEon of Long- Baseline Experiment * SensiEvity PotenEal of LBNE * Conclusions MiniBooNE moEvated by LSND Result * MiniBooNE designed to test LSND result: 3.8σ appearance of electron anEneutrino in muon anEneutrino beam * Use the same L/E but in different energy regime - different

  11. NE-23,

    Office of Legacy Management (LM)

    t:"'. ? - ' y5 NE-23, wk$& Dr. Joseph A. Warburton Chainnan, Radiological and Toxicological Safety Board University of Nevada System DRI/ASC, P.O. Box 60220 Reno, Nevada 89506 Dear Dr. Warburton: The Department of Energy (DOE), as part of its Formerly Utilized Sites Remedial Action Program (FUSRAP), has reviewed information on the Mackay School of M ines facility at the University of Nevada, Reno, Nevada, to determine whether it contains residual radioactivity traceable to activities

  12. NE-23:

    Office of Legacy Management (LM)

    1 , : -2 rn; NE-23: 4 Whitr%; Ms. Theresa Schaffer 3315 S. Emerald Avenue Chicago, Illinois 60616 Dear Ms. Schaffer: . -. r ;-, .4r.-,. , ' P?;c \ \ ; . EC.. ., . The Department of Energy (DOE), as part of its Formerly Utilized Sites Remedial Action Program (FUSRAP), has reviewed information on the former General Services Administratlon 39th Street Werehouse, Chicago, Illincis, to determine whether it contains residual radioactivity traceable to activities conducted on behalf of the Manhattan

  13. NE-24

    Office of Legacy Management (LM)

    VW- 50 "id AU6 3 1983 NE-24 .' . _ : ' : R&D Decontamination Projects Under the Formerly Utilized Sites Remedial Actlon Program (FUSRAP) '_ F .- ,: 'J,.LaGrone, Manager . Oak Ridge Operations Office As a result of the House-Senate Conference Report and the Energy and Water Appropriations Act for FY 1984, and based on the data in the attached reports indicating radioactive contamination in excess of acceptable guidelines, the sites listed in the attachment and their respective vicinity

  14. BooNE: About BooNE

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    About BooNE General Information BooNE Collaboration BooNE Experiment BooNE vs MiniBooNE Interesting Facts Posters Virtual Tour Picture Gallery News Articles BooNE photo montage Technical Information BooNE Proposal Original BooNE proposal (30M ps) Run Plan MiniBooNE Run Plan(3.0M ps.gz) Detector TDR Technical Design Report for the MiniBooNE detector (6.1M .ps.gz) Horn TDR Technical Design Report for the MiniBooNE horn (7.5M .ps.gz) 8GeV Beam TDR Technical Design Report for the primary beam (0.4M

  15. NE-20

    Office of Legacy Management (LM)

    hi v. !&-2:. /qL lo 1 OCT 2 9 1984 NE-20 -. Authorization for Remedial Action of the Ashland 2 Site, Tonawanda, New York f! Joe LaGrone, Manager Oak Ridge Operations Office Based on the Aerial Radiological Survey (Attachment 1) and a "walk-on" radiologlcal survey (Attachment 2 , excerpted from the ORNL draft report "Ground-Level Investigation of Anomalous Gamma Radiation Levels in the Tonawanda, New York, Area," January 1980), the property identified as Ashland 2 is

  16. BooNE Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Experiment Goals of BooNE BooNE in a Nutshell Making Neutrinos Detecting Neutrinos schematic of BooNE experiment A sample event (3M animated PDF file) A cosmic ray event as displayed by the MiniBooNE detector.

  17. Mo-99

    National Nuclear Security Administration (NNSA)

    its project for domestic production of molybdenum-99 (Mo-99) without highly enriched uranium (HEU).

    Mo-99 is the parent isotope of technetium-99m, which is the most widely...

  18. BooNE: Picture Gallery

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Picture Gallery BooNE Collaboration Members of the BooNE collaboration Civil Construction Pictorial progress of BooNE civil construction work Detector Installation Pictorial...

  19. Morgan Wascko Imperial College London M.O. Wascko FNAL User's Meeting

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    from the BooNEs Morgan Wascko Imperial College London M.O. Wascko FNAL User's Meeting M. Sorel Goals of the BooNEs * MiniBooNE: Confirm or rule out LSND * SciBooNE: * Near detector measurements for MiniBooNE * Precise cross section measurements * Especially useful for T2K 2 M.O. Wascko FNAL User's Meeting Goals of the BooNEs * MiniBooNE: Confirm or rule out LSND * SciBooNE: * Near detector measurements for MiniBooNE * Precise cross section measurements * Especially useful for T2K 2 W + ν µ n p

  20. BooNE Collaboration

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Collaboration The BooNE collaboration consists of approximately sixty-five physicists from 13 institutions. While small on the scale of high energy physics experiments, BooNE thrives from the diversity of its membership. This includes scientists from national laboratories, research universities, predominantly undergraduate institutions, as well as a high school physics teacher. List of Collaborators The BooNE Collaboration The BooNE Collaboration

  1. MicroBooNE

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MicroBooNE MicroBooNE Investigating the field of high energy physics through experiments that strengthen our fundamental understanding of matter, energy, space, and time. Get Expertise Rajan Gupta (505) 667-7664 Email Bruce Carlsten (505) 667-5657 Email MicroBooNE schematic drawing Figure 1: A schematic drawing of the MicroBooNE liquid argon TPC detector. The main goals of the MicroBooNE experiment are: (1) to demonstrate the capabilities of a liquid argon TPC in the reconstruction of neutrino

  2. SciBooNE/MiniBooNE

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    particles * p separation using dEdx 2m 4m Used in K2K experiment Used in CHORUS, HARP and K2K Parts recycled from past experiments 31 SciBooNE publications * NuMu...

  3. M.O. Wascko, LSU NuInt05...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    O. Wascko, LSU NuInt05 26 September, 2005 MiniBooNE CC + CCQE Ratio M.O. Wascko, LSU J.R. Monroe, Columbia CC interactions Quasi-Elastic (CCQE) Inclusive Single +...

  4. Mo-99

    National Nuclear Security Administration (NNSA)

    NorthStar Medical Radioisotopes to further develop its technology to produce Mo-99 via neutron capture, bringing the total NNSA support to this project to the maximum of 25...

  5. MicroBooNE

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    optic transmission of the Resistive Wall Monitor (RWM) beam crossing time to transmit the signal to the detector. In the past, for MiniBooNE, this was done with an RG59 copper...

  6. BooNE: Posters

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Posters What's a Neutrino? How neutrinos fit into our understanding of the universe. Recipe for a Neutrino Beam Start with some protons... concocting the MiniBooNE beam. The...

  7. BooNE versus MiniBooNE

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    vs MiniBooNE MiniBooNE refers to the first phase of the BooNE experiment and describes the neutrino oscillation measurements that will be made with a single detector. If neutrino oscillations are observed, then MiniBooNE will be upgraded to a second detector. This 2-detector arrangement (BooNE) will fulfill the second and final stage of the experiment. The BooNE experiment sets out to definitively explore the neutrino oscillation signal reported by the Los Alamos LSND experiment. MiniBooNE

  8. 20Ne Cross Section

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    20Ne(α, X) (Current as of 02/08/2016) NSR Reaction Eα (MeV) Cross Section File X4 Dataset Date Added 1983SC17 20Ne(α, γ): deduced S-factor of capture σ 0.55 - 3.2 X4 09/15/2011 1997WI12 20Ne(α, γ): deduced primary transitions yield 1.64 - 2.65 X4 09/15/2011 1999KO34 20Ne(α, γ): γ-ray yield for the transition 1.9 - 2.8 g.s. 01/03/2012 1369 keV g.s. 10917 keV g.s., 1369 keV 11016 keV g.s. 1975KU06 20Ne(α, γ): σ 2.5 - 20 X4 09/15/2011 1968HI02 20Ne(α, γ): σ 3 - 6 X4 09/15/2011

  9. Category:Concord, NH | Open Energy Information

    Open Energy Info (EERE)

    16 files are in this category, out of 16 total. SVFullServiceRestaurant Concord NH Public Service Co of NH.png SVFullServiceRestauran... 74 KB SVHospital Concord NH Public...

  10. BooNE: Interesting Facts

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Interesting Facts About the BooNE experiment: BooNE is the only experiment to search the entire range covered by the LSND oscillation signal. First proposed in 1997, BooNE will be ready to collect data in summer, 2002. The BooNE collaboration is small by high energy physics standards, having 65 physicists from 13 instiutions. If BooNE detects a supernova, it will send an automatic signal to telescopes around the world describing its position. BooNE collaboration - click to enlarge About the

  11. 20Ne Cross Section

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    p, X) (Current as of 05152012) NSR Reaction Ep (MeV) Cross Section File X4 Dataset Date Added 1981DY03 20Ne(p, p'): for production of -rays threshold - 23 1.63-MeV -rays...

  12. NE - Nuclear Energy - Energy Conservation Plan

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    NUCLEAR ENERGY (NE) ENERGY CONSERVATION PLAN NE has heavily emphasized the use of flexiplace, both regular and situational. Since approximately 56 percent of NE staff use ...

  13. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Booster Neutrino Experiment (BooNE) Goals of BooNE BooNE in a Nutshell Making Neutrinos Detecting Neutrinos

  14. The MicroBooNE Experiment - Collaboration

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The DOE Tours MicroBooNE! - Nov. 27, 2012

  15. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Progress in Delivering Beam to MiniBooNE

  16. UPdate THE NE

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    UPdate THE NE January 2014 Edition U.S. Department of Energy's Nuclear Energy University Programs It's not every day graduate students get to meet one of nuclear energy's most important decision makers. Integrated University Program (IUP) Fellows had this opportunity at the 2013 Winter American Nuclear Society (ANS) Meeting this past November in Washington, D.C. Department of Energy Assistant Secretary for Nuclear Energy, Dr. Pete Lyons, greeted IUP Fellows in a special meeting to discuss

  17. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Picture Gallery BooNE Collaboration Members of the BooNE collaboration Civil Construction Pictorial progress of BooNE civil construction work Detector Installation Pictorial progress of MiniBooNE detector installation BooNE Scrapbook A selection from BooNE

  18. US NE MA Site Consumption

    Gasoline and Diesel Fuel Update (EIA)

    NE MA Site Consumption million Btu $0 $500 $1,000 $1,500 $2,000 $2,500 $3,000 US NE MA Expenditures dollars ALL ENERGY average per household (excl. transportation) 0 2,000 4,000 6,000 8,000 10,000 12,000 US NE MA Site Consumption kilowatthours $0 $250 $500 $750 $1,000 $1,250 $1,500 US NE MA Expenditures dollars ELECTRICITY ONLY average per household * Massachusetts households use 109 million Btu of energy per home, 22% more than the U.S. average. * The higher than average site consumption

  19. US NE MA Site Consumption

    U.S. Energy Information Administration (EIA) Indexed Site

    NE MA Site Consumption million Btu $0 $500 $1,000 $1,500 $2,000 $2,500 $3,000 US NE MA Expenditures dollars ALL ENERGY average per household (excl. transportation) 0 2,000 4,000 6,000 8,000 10,000 12,000 US NE MA Site Consumption kilowatthours $0 $250 $500 $750 $1,000 $1,250 $1,500 US NE MA Expenditures dollars ELECTRICITY ONLY average per household * Massachusetts households use 109 million Btu of energy per home, 22% more than the U.S. average. * The higher than average site consumption

  20. MiniBooNE E. D. Zimmerman

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    SciBooNE Detector TargetHorn SciBooNE constraint reduces error at MiniBooNE * Flux errors become 1-2% level: negligible for this analysis * Cross-section errors reduced, but...

  1. DOE - Office of Legacy Management -- R Brew Co - NH 01

    Office of Legacy Management (LM)

    Brew Co - NH 01 FUSRAP Considered Sites Site: R. BREW CO. (NH.01 ) Eliminated from consideration under FUSRAP Designated Name: Not Designated Alternate Name: None Location: Concord , New Hampshire NH.01-1 Evaluation Year: 1994 NH.01-2 Site Operations: Conducted vacuum furnace tests using uranium and copper billets. NH.01-1 NH.01-3 Site Disposition: Eliminated - Potential for contamination remote NH.01-2 Radioactive Materials Handled: Yes Primary Radioactive Materials Handled: Uranium NH.01-1

  2. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    vs MiniBooNE MiniBooNE is the first phase of the Booster Neutrino Experiment (BooNE); in this phase, neutrino oscillation measurements will be made with a single detector. If oscillations are observed, then MiniBooNE will be upgraded to stage two (BooNE) with a two-detector configuration. The BooNE experiment proposes to definitively explore the neutrino oscillation signal reported by the Los Alamos LSND experiment. MiniBooNE represents the first phase for the BooNE collaboration and consists of

  3. MiniBooNE Results

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Results and Follow-On Experiments W. C. LOUIS for the MiniBooNE collaboration Physics Division, Los Alamos National Laboratory, Los Alamos, NM 87545, USA E-mail: louis@lanl.gov ABSTRACT The MiniBooNE experiment at Fermilab was designed to test the LSND evi- dence for neutrino oscillations 1) . The updated MiniBooNE oscillation result in neutrino mode 2) with 6.5E20 protons on target (POT) shows no significant excess of events at higher energies (above 475 MeV), although a sizeable ex- cess

  4. A=14Ne (1981AJ01)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    1AJ01) (Not illustrated) 14Ne has not been observed. See (1976BE1V

  5. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    BooNE General Information BooNE Collaboration Booster Neutrino Experiment (BooNE) BooNE vs MiniBooNE Interesting Facts Posters Virtual Tour Picture Gallery News Articles Technical Information BooNE Proposal Original BooNE proposal (30M ps) Run Plan MiniBooNE Run Plan(3.0M ps.gz) Detector TDR Technical Design Report for the MiniBooNE detector (6.1M .ps.gz) Horn TDR Technical Design Report for the MiniBooNE horn (7.5M .ps.gz) 8GeV Beam TDR Technical Design Report for the primary beam (0.4M .ps.gz)

  6. Beyond standard model searches in the MiniBooNE experiment

    SciTech Connect (OSTI)

    Katori, Teppei; Conrad, Janet M.

    2014-08-05

    The MiniBooNE experiment has contributed substantially to beyond standard model searches in the neutrino sector. The experiment was originally designed to test the Δm2<mo>~>1eV2 region of the sterile neutrino hypothesis by observing νe(ν<mo>-mo>e) charged current quasielastic signals from a νμ(ν<mo>-mo>μ) beam. MiniBooNE observed excesses of νe and ν<mo>-mo>e candidate events in neutrino and antineutrino mode, respectively. To date, these excesses have not been explained within the neutrino standard model (νSM); the standard model extended for three massive neutrinos. Confirmation is required by future experiments such as MicroBooNE. MiniBooNE also provided an opportunity for precision studies of Lorentz violation. The results set strict limits for the first time on several parameters of the standard-model extension, the generic formalism for considering Lorentz violation. Most recently, an extension to MiniBooNE running, with a beam tuned in beam-dump mode, is being performed to search for dark sector particles. In addition, this review describes these studies, demonstrating that short baseline neutrino experiments are rich environments in new physics searches.

  7. Djurcic_MiniBooNE_PANIC2008

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MiniBooNE Neutrino Oscillation Results Neutrino Oscillation Results Zelimir Djurcic Zelimir Djurcic Physics Department Physics Department Columbia University Columbia University The Eighteenth Particle and The Eighteenth Particle and Nuclei International Conference Nuclei International Conference 9-14 November 2008, 9-14 November 2008, Eilat Eilat , ISRAEL , ISRAEL Outline Outline MiniBooNE MiniBooNE Motivation and Description Motivation and Description MiniBooNE MiniBooNE ' ' s s First First

  8. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Interesting Facts About the Booster Neutrino Experiment (BooNE): BooNE is the only experiment to search the entire range covered by the LSND oscillation signal. First proposed in 1997, BooNE has been collecting data since August 2002. The BooNE collaboration is small by high energy physics standards, comprising 75 physicists from 16 instiutions. If BooNE detects a supernova, it will send an automatic signal to telescopes around the world describing its position. BooNE collaboration - click to

  9. ICARUS/MicroBooNE

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ) ICARUS/MicroBooNE ν ( Φ 0.0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 µ ν µ ν e ν e ν

  10. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Goals of BooNE BooNE's primary goal is to investigate the neutrino oscillation signal reported by the Los Alamos Liquid Scintillator Neutrino Detector (LSND) experiment. In 1995,...

  11. A=19Ne (1978AJ03)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    78AJ03) (See Energy Level Diagrams for 19Ne) GENERAL: See (1972AJ02) and Table 19.24 Table of Energy Levels (in PDF or PS). Nuclear models: (1972EN03, 1972NE1B, 1972WE01,...

  12. MiniBooNE Nuebar Data Release

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Event Excess in the MiniBooNE Search for bar numu rightarrow bar nue Oscillations", arXiv:1007.1150 hep-ex,Phys.Rev.Lett.105,181801 (2010) The following MiniBooNE...

  13. A=14Ne (1986AJ01)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    6AJ01) (Not illustrated) 14Ne, 14Na and 14Mg have not been observed. See (1983ANZQ

  14. A=14Ne (1991AJ01)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    91AJ01) (Not illustrated) 14Ne, 14Na and 14Mg have not been observed. See (1986AN07

  15. The MicroBooNE Experiment - Collaboration

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Collaboration (*) The MicroBooNE spokespeople are Bonnie Fleming (Yale) and Sam Zeller (FNAL) (+) The MicroBooNE project manager was Gina Rameika Updated collaboration list for presentations: powerpoint pdf map collaboration photo MicroBooNE organizational chart MicroBooNE contact list (password required) (IB) = Insititutional Board representative (PD) = postdoc (GS) = graduate student (UG) = undergraduate student Laboratory for High Energy Physics, University of Bern, Switzerland Martin Auger

  16. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    collaboration Find here collaboration lists of MiniBooNE at various stages of the experiment Current MiniBooNE-darkmatter collaboration Original MiniBooNE collaboration From script reading a simple data base, last updated ~2008. from inspirehep.net Booster Neutrino Experiment FNAL-E-0898

  17. A=18Ne (1959AJ76)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    1959AJ76) (Not illustrated) Theory: See (RA57). 1. 18Ne(β+)18F Qm = 4.227 The maximum energy of the positrons is 3.2 ± 0.2 MeV, the half-life is 1.6 ± 0.2 sec: log ft = 2.9 ± 0.2 (GO54D). See also (DZ56). 2. 16O(3He, n)18Ne Qm = -2.966 See (KU53A). 3. 19F(p, 2n)18Ne Qm = -15.424 See (GO54D). 4. 20Ne(p, t)18Ne Qm = -19.812 Not reported

  18. A=17Ne (1977AJ02)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    77AJ02) (See the Isobar Diagram for 17Ne) GENERAL: See also (1971AJ02) and Table 17.20 [Table of Energy Levels] (in PDF or PS). Theory and reviews: (1971HA1Y, 1973HA77, 1973RE17, 1975BE31). Mass of 17Ne: The mass excess of 17Ne, determined from a measurement of the Q-value of 20Ne(3He, 6He)17Ne is 16.48 ± 0.05 MeV (1970ME11, 1972CE1A). Then 17Ne - 17F = 14.53 MeV and Eb for p, 3He and α are, respectively, 1.50, 6.46 and 9.05 MeV. See also (1971AJ02). 1. (a) 17Ne(β+)17F* → 16O + p Qm = 13.93

  19. Ne

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    m er of 2002, the cross sections for an 8 GeV proton beam on Be were m easured by the HARP ex perim ent at CERN. Harp Setup Intro ductio n Im po rtant s te ps s ince las t re v...

  20. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Contact BooNE Spokespersons: E898 (ν running); E944 (anti-ν and beam-dump running) Rex Tayloe rtayloe@indiana.edu (812) 855-3057 Richard Van de Water vdwater@lanl.gov (505) 695 8364 BooNE Experiment: contact-boone@fnal.gov Current Shifter: (505) 500 5511 Detector Enclosure: (630) 840 6881 or 6081 BooNE Collaborators and Associates:

  1. MiniBooNE E. D. Zimmerman

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    NNN'10 Recent Results from MiniBooNE * MiniBooNE * Neutrino cross-sections * Quasielastic and elastic scattering * Hadron production channels * Neutrino Oscillations * Antineutrino Oscillations Motivating MiniBooNE: LSND Liquid Scintillator Neutrino Detector * Stopped + beam at Los Alamos LAMPF produces e , , but no e (due to capture). * Neutron thermalizes, captures ➨2.2 MeV -ray * Look for the delayed coincidence. * Major background non-beam (measured, subtracted) * 3.8 standard dev. excess

  2. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Scrapbook Page 2 The BooNE collaboration in winter. A tour of the construction site. Working with the BooNE Horn. BooNE in the winter A tour of the construction site. A day with the Horn Janet, Bonnie, and Jen in the Tank. Janet and Bill: the early years. Bill, Richard, Jeff, and Shawn in the midst of discussion. Preparing the tubes Janet and Bill: the early days Discussion in progress The oil tanker arrives. The final stages of oil filling. The BooNE Collaboration in the summer. The oil tanker

  3. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    dominate. For MiniBooNE, the contributions from multi-pion production and deep inelastic scattering (DIS) are small. image: neutrino cross sections vs energy There are...

  4. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Civil Construction Pictures The civil construction required for the MiniBooNE experiment consists of two independent construction projects. The Detector Construction: This project...

  5. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Data Releases This page provides MiniBooNE data (histograms, error matrices, ntuples, etc) released in association with particular publications. Only the subset of MiniBooNE papers with released data are listed here. Refer to the Publications page for a complete list of MiniBooNE publications. Other MiniBooNE Data Releases: Data Released with A.A. Aguilar-Arevalo et al., "First Measurement of the Muon Antineutrino Double-Differential Charged-Current Quasielastic Cross section",

  6. The MicroBooNE Experiment - Collaboration

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MicroBooNE In the News MicroBooNE internal newletters (password protected) The Hidden Neutrino, Symmetry Magazine, 03/01/16 Booster Neutrino Beam Reaches Record Beam Intensity, Fermilab This Week, 02/02/16 MicroBooNE Sees First Accelerator-Born Neutrinos, Fermilab Today, 11/02/15 MicroBooNE Sees First Accelerator-Born Neutrinos, Symmetry Magazine, 11/02/15 Detector Finds its First Ghost Particle, Daily Mail, 11/03/15 First Evidence of Neutrinos, Daily Galaxy, 11/03/15 A Neutrino in a Haystack,

  7. The MicroBooNE Experiment - Publications

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MicroBooNE Documents and Publications Public Notes See the Public Notes Page for a list of notes with results made public by the MicroBooNE collaboration. Presentations See the Talks Page for copies of slides and posters presented at conferences and workshops. MicroBooNE DocDB Like most experiments at Fermilab, MicroBooNE uses DocDB - a documents database. Much of the contents of the DocDB are restricted to members of the collaboration, but some items are public. Use the link below to enter the

  8. MiniBooNE Pion Group

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Contents: Pion Group Home Pion Group Members Pion References Colin's Cross Section Page MiniBooNE Internal Email M. Tzanov.

  9. MiniBooNE Results / MicroBooNE Status! Eric Church, Yale University

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    at this talk?) 3 Outline MiniBooNE past results future MicroBooNE physics motivation R&D motivation status: (running is imminent) 4 The Booster...

  10. Measurement and Modeling of Spatial NH3 Storage Distributions...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Measurement and Modeling of Spatial NH3 Storage Distributions in a Commercial Small Port Cu Zeolite Urea SCR Catalyst A modified Spaci-IR technique can measure transient NH3 and ...

  11. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The BooNE collaboration consists of approximately sixty-five physicists from 13 institutions. While small on the scale of high energy physics experiments, BooNE thrives from the diversity of its membership. This includes scientists from national laboratories, research universities, predominantly undergraduate institutions, as well as a high school physics teacher. List of Collaborators

  12. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Experiment Details This page provides information on the MiniBooNE experiment. Images are linked in their own page with captions. Additional resources are the Talks, Slides and Posters page, Publications page, and Data Release page Beamline Flux Detector Cross sections Light Propagation (Optical Model) Calibration Particle Identification BooNE photo montage

  13. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    For Physicists These pages provides information (numbers, plots, details) of the MiniBooNE experiment and analysis pieces. Images are linked in their own page with captions. Additional resources are the Talks, Slides and Posters page and the Publications page Experiment Details Data Releases BooNE photo montage

  14. MiniBooNE Collaboration MiniBooNE Collaboration Yale University

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    a Neutrino Oscillation Search Progress on a Neutrino Oscillation Search at MiniBooNE at MiniBooNE B. T. Fleming for the B. T. Fleming for the MiniBooNE Collaboration MiniBooNE Collaboration Yale University Yale University The LSND experiment observed ν e appearance in a ν μ beam MiniBooNE experiment: designed to confirm or rule out the LSND result ν e appearance in a ν μ beam L=540 m (~x20 LSND) E = 800 MeV (~x20 LSND) 8 GeV protons from Fermilab Booster incident on target inside horn π's

  15. A=16Ne (1982AJ01)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    82AJ01) (See the Isobar Diagram for 16Ne) GENERAL: See also (1977AJ02) and Table 16.27 [Table of Energy Levels] (in PDF or PS). Theoretical work: (1978GU10, 1978SP1C, 1981LI1M). Reviews: (1977CE05, 1979AL1J, 1980TR1E). Mass of 16Ne: The Q-values of the 20Ne(α, 8He) and 16O(π+, π-) reactions lead to an atomic mass excess of 24.02 ± 0.04 MeV for 16Ne. 16Ne is then unbound with respect to decay into 14O + 2p by 1.43 MeV and is bound with respect to decay into 15F + p by 0.04 MeV. 1. 16O(π+,

  16. A=17Ne (1993TI07)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    93TI07) (See the Isobar Diagram for 17Ne) GENERAL: See Table Prev. Table 17.26 preview 17.26 [Table of Energy Levels] (in PDF or PS). 1. (a) 17Ne(β+)17F* → 16O + p Qm = 13.928 (b) 17Ne(β+)17F → 13N + α Qm = 8.711 (c) 17Ne(β+)17F Qm = 14.529 The half-life of 17Ne has been reported as 109.0 ± 1.0 msec (1971HA05) and 109.3 ± 0.6 msec (1988BO39): the weighted mean is 109.2 ± 0.6 and we adopt it. The decay is primarily to the proton unstable states of 17F at 4.65, 5.49, 6.04 and 8.08 MeV

  17. A=17Ne (71AJ02)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    71AJ02) (See the Isobar Diagram for 17Ne) GENERAL: See also Table 17.22 [Table of Energy Levels] (in PDF or PS). Theory: (WI64E, MA65J, MA66BB). Reviews: (BA60Q, GO60P, BA61F, GO62N, GO64J, GO66J, GO66L, MC66E, CE68A, GA69M). Mass of 17Ne: M - A, determined from the Q-value of the 20Ne(3He, 6He)17Ne reaction, is 16.479 ± 0.050 MeV (ME70E). See also (ES67). Then 17Ne - 17F = 14.53 MeV and Eb for p, 3He and α are, respectively, 1.50, 6.46 and 9.05 MeV. [Eb for an α-particle is calculated using

  18. Extraordinary selectivity of CoMo{sub 3}S{sub 13} chalcogel for C{sub 2}H{sub 6} and CO{sub 2} adsorption.

    SciTech Connect (OSTI)

    Shafaei-Fallah, M.; Rothenberger, Z.; Katsoulidis, A. P.; He, J.; Malliakas, C. D.; Kanatzidis, M. G.

    2011-11-09

    The chalcogel CoMo{sub 3}S{sub 13} is obtained from the reaction of (NH{sub 4}){sub 2}[Mo{sub 3}S{sub 13}] with cobalt acetate in solution. The chalcogel has a BET surface area of 570 m{sup 2} g{sup -1}, and pair distribution function analysis (PDF) and infrared spectroscopy indicate that the [Mo{sub 3}S{sub 13}]{sup 2-} cluster is a building block in the porous network. The CoMo{sub 3}S{sub 13} chalcogel exhibits high selectivity for separating ethane and carbon dioxide from hydrogen and methane.

  19. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    in a Nutshell BooNE will investigate the question of neutrino mass by searching for oscillations of muon neutrinos into electron neutrinos. This will be done by directing a muon neutrino beam into the MiniBooNE detector and looking for electron neutrinos. This experiment is motivated by the oscillation results reported by the LSND experiment at Los Alamos. By changing the muon neutrino beam into a muon anti-neutrino beam, BooNE can explore oscillations from muon anti-neutrinos to electron

  20. MiniBooNE Flux Data Release

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Neutrino Flux Prediction at MiniBooNE", arXiv:0806.1449 [hep-ex], Phys. Rev. D. 79, 072002 (2009) The following MiniBooNE information from the large flux paper in 2009 is made available to the public: Text files containing flux information for each neutrino species Positive horn polarity (neutrino-enhanced mode) Negative horn polarity (anti neutrino-enhanced mode) Contact Information For clarifications on how to use MiniBooNE public data or for enquiries about additional data not linked

  1. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Proceedings This page contains links to conference proceedings submitted by members of the MiniBooNE collaboration New Guidelines for Submitting Proceedings at MiniBooNE: As of June 2007, we have changed the rules on conference proceedings. Proceedings must be read by one other MiniBooNE person (besides the author) of postdoc level or above before being submitted. Proceedings should also be sent to boone-talks@fnal.gov for archiving on this website. back to Talks page Speaker Proceedings Info

  2. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The primary goal of The inside of the MiniBooNE tank is covered with 1280 photomultiplier tubes. (Courtesy: Fermilab Visual Media Services) this experiment is: To test for neutrino mass by searching for neutrino oscillations. Neutrino mass is important because it may lead us to physics beyond the Standard Model. Masses in the range accessible to MiniBooNE will expand our understanding of how the universe has evolved. The BooNE project began in 1997. The first beam induced neutrino events were

  3. About the MicroBooNE Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    About MicroBooNE The MicroBooNE collaboration is currently operating a large 170-ton liquid Argon Time Projection Chamber (LArTPC) that is located on the Booster neutrino beam line at Fermilab. The experiment will measure low energy neutrino cross sections and investigate the low energy excess events observed by the MiniBooNE experiment. The detector also serves as a next step in a phased program towards the construction of massive kiloton scale LArTPC detectors for future long-baseline neutrino

  4. Corrosion report for the U-Mo fuel concept

    SciTech Connect (OSTI)

    Henager, Jr., Charles H.; Bennett, Wendy D.; Doherty, Ann L.; Fuller, E. S.; Hardy, John S.; Omberg, Ronald P.

    2014-08-28

    The Fuel Cycle Research and Development (FCRD) program of the Office of Nuclear Energy (NE) has implemented a program to develop a Uranium-Molybdenum (U-Mo) metal fuel for Light Water Reactors (LWR)s. Uranium-Molybdenum fuel has the potential to provide superior performance based on its thermo-physical properties, which includes high thermal conductivity for less stored heat energy. With sufficient development, it may be able to provide the Light Water industry with a melt-resistant accident tolerant fuel with improved safety response. However, the corrosion of this fuel in reactor water environments needs to be further explored and optimized by additional alloying. The Pacific Northwest National Laboratory has been tasked with performing ex-reactor corrosion testing to characterize the performance of U-Mo fuel. This report documents the results of the effort to characterize and develop the U-Mo metal fuel concept for LWRs with regard to corrosion testing. The results of a simple screening test in buffered water at 30C using surface alloyed U-10Mo is documented and discussed. The screening test was used to guide the selection of several potential alloy improvements that were found and are recommended for further testing in autoclaves to simulate PWR water conditions more closely.

  5. A=16Ne (1986AJ04)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    6AJ04) (See the Isobar Diagram for 16Ne) GENERAL: See also (1982AJ01) and Table 16.26 [Table of Energy Levels] (in PDF or PS) here. See (1981SE1B, 1983ANZQ, 1985AN28, 1985MA1X). Mass of 16Ne: The Q-values of the 20Ne(α, 8He) and 16O(π+, π-) reactions lead to atomic mass excesses of 23.93 ± 0.08 MeV (1978KE06), 23.978 ± 0.024 MeV (1983WO01) and 24.048 ± 0.045 MeV (1980BU15) [recalculated using the (1985WA02) masses for 8He, 16O and 20Ne]. The weighted mean is 23.989 ± 0.020 MeV which is

  6. A=16Ne (1993TI07)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    93TI07) (See the Isobar Diagram for 16Ne) GENERAL: See Table Prev. Table 16.29 preview 16.29 [General Table] (in PDF or PS) and Table Prev. Table 16.32 preview 16.32 [Table of Energy Levels] (in PDF or PS). Mass of 16Ne: The Q-values of the 20Ne(α, 8He) and 16O(π+, π-) reactions lead to atomic mass excesses of 23.93 ± 0.08 MeV (1978KE06), 23.978 ± 0.024 MeV (1983WO01) and 24.048 ± 0.045 MeV (1980BU15) [recalculated using the (1985WA02) masses for 8He, 16O and 20Ne]. The weighted mean is

  7. A=17Ne (1982AJ01)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    82AJ01) (See the Isobar Diagram for 17Ne) GENERAL: See (1977AJ02) and Table 17.22 [Table of Energy Levels] (in PDF or PS). Theory and reviews:(1975BE56, 1977CE05, 1978GU10, 1978WO1E, 1979BE1H). Other topics:(1981GR08). Mass of 17Ne: The mass excess adopted by (1977WA08) is 16.478 ± 0.026 MeV, based on unpublished data. We retain the mass excess 16.48 ± 0.05 MeV based on the evidence reviewed in (1977AJ02). 1. (a) 17Ne(β+)17F* → 16O + p Qm = 13.93 (b) 17Ne(β+)17F Qm = 14.53 The half-life of

  8. A=17Ne (1986AJ04)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    6AJ04) (See the Isobar Diagram for 17Ne) GENERAL: See (1982AJ01) and Table 17.20 [Table of Energy Levels] (in PDF or PS). Theory and reviews: (1983ANZQ, 1983AU1B, 1985AN28). 1. (a) 17Ne(β+)17F* → 16O + p Qm = 13.93 (b) 17Ne(β+)17F Qm = 14.53 The half-life of 17Ne is 109.0 ± 1.0 msec (1971HA05). Earlier values (see (1971AJ02)) gave a mean value of 108.0 ± 2.7 msec. The decay is primarily to the proton unstable states of 17F at 4.70, 5.52 and 6.04 MeV with Jπ = 3/2-, 3/2- and 1/2-: see

  9. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    on a beryllium target. The beam is modeled with measured mean position and angle with Gaussian smearing. MiniBooNE simulates the effects of varying the spread in the beam and...

  10. A=19Ne (1983AJ01)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    83AJ01) (See Energy Level Diagrams for 19Ne) GENERAL: See (1978AJ03) and Table 19.23 Table of Energy Levels (in PDF or PS). Nuclear models: (1978MA2H, 1978PE09, 1978PI06,...

  11. A=18Ne (1978AJ03)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    1978AJ03) (See Energy Level Diagrams for 18Ne) GENERAL: See also (1972AJ02) and Table 18.22 Table of Energy Levels (in PDF or PS). Model calculations: (1972EN03, 1974LO04)....

  12. A=19Ne (1987AJ02)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    7AJ02) (See Energy Level Diagrams for 19Ne) GENERAL: See (1983AJ01) and Table 19.21 Table of Energy Levels (in PDF or PS). Nuclear models:(1983BR29, 1983PO02). Special states:...

  13. A=18Ne (1983AJ01)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    83AJ01) (See Energy Level Diagrams for 18Ne) GENERAL: See also (1978AJ03) and Table 18.21 Table of Energy Levels (in PDF or PS). Model calculations: (1979DA15, 1979SA31,...

  14. A=18Ne (1987AJ02)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    7AJ02) (See Energy Level Diagrams for 18Ne) GENERAL: See (1983AJ01) and Table 18.22 Table of Energy Levels (in PDF or PS). Model calculations:(1982ZH01, 1983BR29, 1984SA37,...

  15. The MicroBooNE Experiment - Collaboration

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Contact MicroBooNE Spokespeople: Bonnie Fleming, Yale email: bonnie.fleming(AT)yale.edu phone: (203) 432-3235 Sam Zeller, FNAL email: gzeller(AT)fnal.gov phone: (630) 840-6879 Collaboration Members

  16. A=20Ne (72AJ02)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ) elastic scattering. It is interpreted in terms of a quasi-molecular -particle cluster model (CO69S). See also (WA65M). 18. 17O(, n)20Ne Qm 0.588 Angular...

  17. The NeXus data format

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Könnecke, Mark; Akeroyd, Frederick A.; Bernstein, Herbert J.; Brewster, Aaron S.; Campbell, Stuart I.; Clausen, Björn; Cottrell, Stephen; Hoffmann, Jens Uwe; Jemian, Pete R.; Männicke, David; et al

    2015-01-30

    NeXus is an effort by an international group of scientists to define a common data exchange and archival format for neutron, X-ray and muon experiments. NeXus is built on top of the scientific data format HDF5 and adds domain-specific rules for organizing data within HDF5 files, in addition to a dictionary of well defined domain-specific field names. The NeXus data format has two purposes. First, it defines a format that can serve as a container for all relevant data associated with a beamline. This is a very important use case. Second, it defines standards in the form of application definitionsmore » for the exchange of data between applications. NeXus provides structures for raw experimental data as well as for processed data.« less

  18. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Posters What's a Neutrino? How neutrinos fit into our understanding of the universe. Recipe for a Neutrino Beam Start with some protons... concocting the MiniBooNE beam. The...

  19. MicroBooNE Detector Move

    ScienceCinema (OSTI)

    Flemming, Bonnie; Rameika, Gina

    2014-07-15

    On Monday, June 23, 2014 the MicroBooNE detector -- a 30-ton vessel that will be used to study ghostly particles called neutrinos -- was transported three miles across the Fermilab site and gently lowered into the laboratory's Liquid-Argon Test Facility. This video documents that move, some taken with time-lapse camerad, and shows the process of getting the MicroBooNE detector to its new home.

  20. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Talks and Proceedings This page contains links to talks and proceedings about the MiniBooNE experiment presented by members of the collaboration. Password protected link to page containing future talks schedule and unassigned talks list. Password protected link to seminar schedule. Conference talks Other talks Proceedings Posters All Experimenters Meeting talks The MiniBooNE Talks Committee is Jon Link (chair), Rex Tayloe, and Morgan Wascko. Conference Talks Speaker Conference Info Material Name

  1. The MicroBooNE Experiment - Public Notes

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MicroBooNE Public Notes Page Back to the Publications Page

  2. FY17 NE Budget Request Presentation | Department of Energy

    Energy Savers [EERE]

    7 NE Budget Request Presentation FY17 NE Budget Request Presentation PDF icon FY17 NE Budget Request Presentation More Documents & Publications FY16 NE Budget Request Presentation Office of Nuclear Energy Fiscal Year 2014 Budget Request Before the House Subcommittee on Energy, Committee on Science, Space and Technology

  3. US WNC MO Site Consumption

    U.S. Energy Information Administration (EIA) Indexed Site

    WNC MO Site Consumption million Btu $0 $500 $1,000 $1,500 $2,000 $2,500 US WNC MO Expenditures dollars ALL ENERGY average per household (excl. transportation) 0 3,000 6,000 9,000 12,000 15,000 US WNC MO Site Consumption kilowatthours $0 $300 $600 $900 $1,200 $1,500 US WNC MO Expenditures dollars ELECTRICITY ONLY average per household * Missouri households consume an average of 100 million Btu per year, 12% more than the U.S. average. * Average household energy costs in Missouri are slightly less

  4. Cross section analyses in MiniBooNE and SciBooNE experiments

    SciTech Connect (OSTI)

    Katori, Teppei

    2015-05-15

    The MiniBooNE experiment (2002-2012) and the SciBooNE experiment (2007-2008) are modern high statistics neutrino experiments, and they developed many new ideas in neutrino cross section analyses. In this note, I discuss selected topics of these analyses.

  5. Mo#va#on

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    = a n i nherent l imita#ons of both: h ot & c old f usion r eac#ons: Hot (well--- d eformed r adioac1ve ac1nides ( Act.) t argets a re u sed a nd compound n ucleus i s q uite e xcited ) * a8empts o f g oing b eyond the r eac#ons A ct. + 48 Ca b y using h eavier p rojec#les l ike 50 Ti, 54 Cr, 58 Fe, a nd 64 Ni gave n o r esults s o f ar. * all h eavier a c#nides w ith Z>98 l ive t o s hort t hat o ne could p erform t arget w ith them. Cold ( magic n uclei a s t argets a re u sed w ith

  6. A=18Ne (72AJ02)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    72AJ02) (See Energy Level Diagrams for 18Ne) GENERAL: See Table 18.23 [Table of Energy Levels] (in PDF or PS). Shell and cluster model calculations:(WI57H, BE69H, BA70P, EL70D, HA70M, KA72). Electromagnetic transitions:(EL70D, HA70M). Special levels:(MI66C, KA69P, KA72). Pion reactions:(PA65F). Other theoretical calculations:(GO65E, KE66C, BA68EE, BE68V, MU68G, NE68A, VA68E, VA68L, BA69GG, GA69O, KA69P, MU69C, RA69C, SO69A, BA70, DI70F, EL70D, KA72). 1. 18Ne(β+)18F Qm = 4.447 The half-life of

  7. A=19Ne (1995TI07)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    95TI07) (See Energy Level Diagrams for 19Ne) GENERAL: See Table Prev. Table 19.26 preview 19.26 [General Table] (in PDF or PS) and Table Prev. Table 19.27 preview 19.27 [Table of Energy Levels] (in PDF or PS) here. μg.s. = -1.88542 (8) nm (1982MA39) μ0.239 = -0.740 (8) nm (1978LEZA) 1. 19Ne(β+)19F Qm = 3.238 We adopt the half-life of 19Ne suggested by (1983AD03): 17.34 ± 0.09 s. See also (1978AJ03). The decay is principally to 19Fg.s.: see Table Prev. Table 19.29 preview 19.29 (in PDF or

  8. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    FermiNews A biweekly magazine published by the Fermilab Office of Public Affairs about work and life at Fermilab. 2002: September 20, 2002 - New Neutrino Experiment at Fermilab Goes Live June 14, 2002 - Changing of the Guard: Mike Shaevitz returns to Columbia May 24, 2002 - Beam Me Up: MiniBooNE gets ready to go May 10, 2002 - Dastow 2002: 3D neutrino event simulation Mar. 29, 2002 - Exploring the Invisible Universe Jan. 18, 2002 - A Clear View: MiniBooNE's detector oil 2001: Dec. 14, 2001 -

  9. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Detector The MiniBooNE tank is 12 m diameter sphere, filled with approximately 800 tons of mineral oil, CH2, which has a density of 0.845 ± 0.001 g/cm3. 1280 PMTs provide about 10% coverage of the inner tank region, and 240 PMTs cover the outer, optically isolated "veto" region in the last 1.3 m in the tank. Most of the tubes were recovered from LSND, and are 'old' tubes, some additional ones were bought for MiniBooNE, and are 'new'; differences in the new vs the old tube function are

  10. MiniBooNE Nue Data Release

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Neutrino Appearance at the Δm2 ~1 eV2 Scale", arXiv:0704.1500 [hep-ex], Phys. Rev. Lett. 98, 231801 (2007) The following MiniBooNE information from the first oscillation paper in 2007 is made available to the public: Energy Range for Default Oscillation Fit (475 MeV - 3000 MeV reconstructed neutrino energy) ntuple file of official MiniBooNE sin2(2theta) sensitivity and upper limit curves as a function of Dm2, for a 2-neutrino muon-to-electron oscillation fit, and 90% and 3sigma confidence

  11. MiniBooNE Nuebar Data Release

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Search for Electron Anti-Neutrino Appearance at the Δm2 ~1 eV2 Scale", arXiv:0904.1958 [hep-ex], Phys. Rev. Lett. 103, 111801 (2009) The following MiniBooNE information from the 2009 nuebar appearance paper is made available to the public: Energy Range: 475 MeV - 3000 MeV reconstructed neutrino energy ntuple file of MiniBooNE sin2(2theta) sensitivity and upper limit curves as a function of Dm2, for a 2-neutrino muon-to-electron antineutrino oscillation fit, and 90% and 3sigma confidence

  12. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Milestones 2008: January 1 1E21 protons on target recorded by MiniBooNE 2007: April 10 25m absorber repaired 2006: August 23 9e16 protons delivered in a single hour (Booster champagne goal) January 18 first antineutrino beam 2004: April 26 Record week (04/19-04/26) 6.83E18 protons delivered. 2003: March 28 Record day: 9.6E17 protons delivered March 18 Record day: 8.18E17 protons delivered March 06 5.5E17 protons delivered to MiniBooNE in 1 hour. (passed the official BD 5E16 milestone) March 01

  13. MicroBooNE First Cosmic Tracks

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    First Tracks in MicroBooNE (August 6, 2015) On August 6, 2015, we started to turn on the drift high voltage in the MicroBooNE detector for the very first time. We paused at 58 kV (this is about 1/2 of our design voltage) and immediately started to see tracks across the entire TPC. Below are some of our first images of cosmic rays and UV laser tracks (last picture) recorded by the TPC! Collection plane images: And here is one of the first images of a UV laser track in the TPC. You can tell which

  14. MiniBooNE Steve Brice Fermilab

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    17 May 2006 1 MiniBooNE Steve Brice Fermilab * Oscillation Analysis * Issues of the Past Year - Normalization - Optical Model -  0 MisIDs * Summary * Future DOE Review 17 May 2006 2 MiniBooNE Goal * Search for  e appearance in a   beam at the ~0.3% level - L=540 m ~10x LSND - E~500 MeV ~10x LSND DOE Review 17 May 2006 3 Particle ID * Identify electrons (and thus candidate  e events) from characteristic hit topology * Non-neutrino background easily removed     n p W

  15. In Situ Time-Resolved Characterization of Ni-MoO2 Catalysts for the Water-Gas Shift Reaction

    SciTech Connect (OSTI)

    Wen,W.; Calderon, J.; Brito, J.; Marinkovic, N.; Hanson, J.; Rodriquez, J.

    2008-01-01

    Active catalysts for the water-gas shift (WGS, CO + H2O ? H2 + CO2) reaction were synthesized from nickel molybdates ({beta}-NiMoO4 and nH2O{center_dot}NiMoO4) as precursors, and their structural transformations were monitored using in situ time-resolved X-ray diffraction and X-ray absorption near-edge spectroscopy. In general, the nickel molybdates were not stable and underwent partial reduction in the presence of CO or CO/H2O mixtures at high temperatures. The interaction of {beta}-NiMoO4 with the WGS reactants at 500 C led to the formation of a mixture of Ni (24 nm particle size) and MoO2 (10 nm particle size). These Ni-MoO2 systems displayed good catalytic activity at 350, 400, and 500 C. At 350 and 400 C, catalytic tests revealed that the Ni-MoO2 system was much more active than isolated Ni (some activity) or isolated MoO2 (negligible activity). Thus, cooperative interactions between the admetal and oxide support were probably responsible for the high WGS activity of Ni-MoO2. In a second synthetic approach, the NiMoO4 hydrate was reduced to a mixture of metallic Ni, NiO, and amorphous molybdenum oxide by direct reaction with H2 gas at 350 C. In the first pass of the water-gas shift reaction, MoO2 appeared gradually at 500 C with a concurrent increase of the catalytic activity. For these catalysts, the particle size of Ni (4 nm) was much smaller than that of the MoO2 (13 nm). These systems were found to be much more active WGS catalysts than Cu-MoO2, which in turn is superior to commercial low-temperature Cu-ZnO catalysts.

  16. Verification of Allowable Stresses In ASME Section III Subsection NH For Grade 91 Steel & Alloy 800H

    SciTech Connect (OSTI)

    R. W. Swindeman; M. J. Swindeman; B. W. Roberts; B. E. Thurgood; D. L. Marriott

    2007-11-30

    The database for the creep-rupture of 9Cr-1Mo-V (Grade 91) steel was collected and reviewed to determine if it met the needs for recommending time-dependent strength values, S{sub t}, for coverage in ASME Section III Subsection NH (ASME III-NH) to 650 C (1200 F) and 600,000 hours. The accumulated database included over 300 tests for 1% total strain, nearly 400 tests for tertiary creep, and nearly 1700 tests to rupture. Procedures for analyzing creep and rupture data for ASME III-NH were reviewed and compared to the procedures used to develop the current allowable stress values for Gr 91 for ASME II-D. The criteria in ASME III-NH for estimating S{sub t} included the average strength for 1% total strain for times to 600,000 hours, 80% of the minimum strength for tertiary creep for times to 600,000 hours, and 67% of the minimum rupture strength values for times to 600,000 hours. Time-temperature-stress parametric formulations were selected to correlate the data and make predictions of the long-time strength. It was found that the stress corresponding to 1% total strain and the initiation of tertiary creep were not the controlling criteria over the temperature-time range of concern. It was found that small adjustments to the current values in III-NH could be introduced but that the existing values were conservative and could be retained. The existing database was found to be adequate to extend the coverage to 600,000 hours for temperatures below 650 C (1200 F).

  17. MiniBooNE Cross Sections

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Sections Group e-mail: BOONE-CROSSSECTIONS(AT)fnal.gov convenors: Alessandro Curioni (alessandro.curioni(AT)yale.edu) and Sam Zeller (gzeller(AT)fnal.gov) Cross Sections at MiniBooNE, Meetings, Reference Articles, Conferences, Useful Links Last updated on 07/19/07

  18. A=16Ne (71AJ02)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    predicts M - A 25.15 0.6 MeV (CE68A: 16Ne is then unbound with respect to breakup into 14O + 2p by 2.6 MeV. See also (GO60K, GO60P, BA61F, GO61N, GO62N, GO62O, GA64A,...

  19. A=16Ne (1977AJ02)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    predicts M - A 25.15 0.6 MeV (1968CE1A); 16Ne is then unbound with respect to breakup into 14O + 2p by 2.6 MeV: see (1971AJ02) for the earlier work. See also (1972WA07)...

  20. NE-23 Disposal of Offsite-Generated Defense Radioactive Waste...

    Office of Legacy Management (LM)

    piL +3 *3L 52. NE-23 Disposal of Offsite-Generated Defense Radioactive Waste, Ventron FUSRAP Site Jill E. Lytle, DP-12 NE-23 The Office of Remedial Action and Waste Technology has...

  1. US WNC MO Site Consumption

    Gasoline and Diesel Fuel Update (EIA)

    in the South than those in the Midwest. 0% 20% 40% 60% 80% 100% US WNC MO OtherNone Propane Electricity Natural Gas MAIN HEATING FUEL USED COOLING EQUIPMENT USED DIVISION:...

  2. FY16 NE Budget Request Presentation | Department of Energy

    Energy Savers [EERE]

    6 NE Budget Request Presentation FY16 NE Budget Request Presentation PDF icon Office of Nuclear Energy FY16 Budget Request Presentation More Documents & Publications FY17 NE Budget Request Presentation Office of Nuclear Energy Fiscal Year 2014 Budget Request FY 2016 Budget Justification

  3. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Light propagation in mineral oil Though the dominant light observed in MiniBooNE is Cherenkov light, scintillation and fluorescence (here, reabsorbed Cherenkov light re-emitted) account for about 25% of the light. We model: scintillation light (yield, decay times, spectrum), fluorescence, scattering (Rayleigh, Raman), absorption, reflection (off tank walls, PMT faces) and PMT effects (single pe charge response). External measurements Scintillation from p beam (IUCF) Scintillation from cosmic mu

  4. MicroBooNE Proposal Addendum March

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MicroBooNE Proposal Addendum March 3, 2008 H. Chen, G. de Geronimo, J. Farrell, A. Kandasamy, F. Lanni, D. Lissauer, D. Makowiecki, J. Mead, V. Radeka, S. Rescia, J. Sondericker, B. Yu Brookhaven National Laboratory, Upton, NY L. Bugel, J. M. Conrad, Z. Djurcic, V. Nguyen, M. Shaevitz, W. Willis ‡ Columbia University, New York, NY C. James, S. Pordes, G. Rameika Fermi National Accelerator Laboratory, Batavia, IL C. Bromberg, D. Edmunds Michigan State University, Lansing, MI P. Nienaber St.

  5. NE Press Releases | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Press Releases NE Press Releases RSS January 5, 2016 Energy Department selects Battelle team for a deep borehole field test in North Dakota The U.S. Department of Energy has selected a Battelle Memorial Institute-led team to drill a test borehole of over 16,000 feet into a crystalline basement rock formation near Rugby, North Dakota. December 10, 2015 Energy Department Announces New Investments in Supercritical Transformational Electric Power (STEP) Program The U.S. Department of Energy's

  6. M r. Andrew Wallo, III, NE-23

    Office of Legacy Management (LM)

    300.955 L*Enfom Plaza, S. Iv.. Washrhington. D.C. 200242174, Tekphonc (202) 7117-03.87.cdy.43 23 September 1987 M r. Andrew Wallo, III, NE-23 Division of Facility & Site Deconnnissioning Projects U.S. Department of Energy Germantown, Maryland 20545 Dear M r. Wallo: ELIMINATION RECOMMENDATION -- COLLEGES AND UNIVERSITIES The attached elimination recommendation was prepared in accordi with your suggestion during our meeting on 22 September. The reconu includes 26 colleges and universities

  7. For the MicroBooNE Collaboration IPA2013

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Status of MicroBooNE Christina Ignarra (MIT) For the MicroBooNE Collaboration IPA2013 May 14, 2013 Motivation for MicroBooNE: MiniBooNE Motivation for MiniBooNE: LSND * LSND result: Observed an appearance signal consistant with oscillations at a m 2 not consistent with known mass splittings: * A 3 rd mass splitting would solve this problem: P (ν µ → ν e ) = sin 2 2θ sin 2 (1.27∆m 2 L E ) 3 3+1 Sterile Neutrino Model l Assume one more neutrino that doesn't interact through the weak

  8. Djurcic_MiniBooNE_NuFact2010

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MiniBooNE Results Zelimir Djurcic Zelimir Djurcic Argonne National Laboratory Argonne National Laboratory NuFact2010: 12th International Workshop on Neutrino Factories, NuFact2010: 12th International Workshop on Neutrino Factories, Superbeams Superbeams and and Beta Beams Beta Beams October 20-25, 2010. Mumbai, India October 20-25, 2010. Mumbai, India Outline Outline * * MiniBooNE MiniBooNE Experiment Description Experiment Description * * MiniBooNE MiniBooNE ' ' s s Neutrino Results Neutrino

  9. The MicroBooNE Experiment - Home Page

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MicroBooNE one of the first neutrino event candidates seen in the MicroBooNE detector see more neutrino images here! see more cosmic tracks here! The MicroBooNE Experiment Located at Fermilab, the MicroBooNE collaboration is currently operating a large 170 ton Liquid Argon Time Projection Chamber (LAr TPC) that is located on the Booster neutrino beam line at Fermilab. The experiment first started collecting neutrino data in October 2015. MicroBooNE will measure low energy neutrino cross sections

  10. Public Service Co of NH | Open Energy Information

    Open Energy Info (EERE)

    800-662-7764 Outage Map: www.eversource.comContentgen Green Button Access: Implemented Green Button Landing Page: www.psnh.comSaveEnergyMo Green Button Reference Page:...

  11. MiniBooNE at All Experimenter's Meeting

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Year [2002] [2003] [2004] [2005] [2006][2007] [2008] [2009] [2010] [2011] [2012] [2014] 2014 Date Focus Speaker Every Monday @ 4:00 P.M., Curia II 09/08/14 MiniBooNE Status Report Zarko Pavlovic 08/25/14 MiniBooNE Status Report Zarko Pavlovic 08/18/14 MiniBooNE Status Report Zarko Pavlovic 08/11/14 MiniBooNE Status Report Zarko Pavlovic 08/04/14 MiniBooNE Status Report Zarko Pavlovic 07/28/14 MiniBooNE Status Report Zarko Pavlovic 07/21/14 MiniBooNE Status Report Zarko Pavlovic 07/14/14

  12. DOE - Office of Legacy Management -- St Louis Airport - MO 01

    Office of Legacy Management (LM)

    Airport - MO 01 FUSRAP Considered Sites St. Louis Airport, MO Alternate Name(s): Airport Site St. Louis Airport Storage Site (SLAPS) Former Robertson Storage Area Robertson Airport MO.01-1 MO.01-2 Location: Brown Road, Robertson, Missouri MO.01-2 Historical Operations: Stored uranium process residues containing uranium, radium, and thorium for the MED and AEC. MO.01-2 MO.01-3 MO.01-4 Eligibility Determination: Eligible MO.01-1 MO.01-7 Radiological Survey(s): Assessment Surveys MO.01-4 MO.01-5

  13. Effect of supplementation on vitamin A and zinc nutriture of children in northeast (NE) Thailand

    SciTech Connect (OSTI)

    Udomkesmalee, E.; Dhanamitta, S.; Charoenklatkul, S.; Tantipopipat, S.; Banjong, O.; Rojroongwasinkul, N.; Kramer, T.R.; Smith, J.C. Jr. USDA, Beltsville, MD )

    1991-03-11

    Previous surveys of the nutritional status of young children in NE Thailand suggested that they may benefit from vitamin A (VA) and/or zinc (Zn) supplementation. 140 children, with low plasma retinol concentrations were entered in a double-blind study. They were randomized and supplemented with either VA, Zn, VA + Zn or placebo each weekday for 6 mos. All subjects consumed their usual diet that provided adequate protein, less than recommended calories, fat, Zn and VA. Biochemical indices of VA and Zn status increased significantly. The children had adequate VA liver stores as assessed by relative dose response. Zn supplementation resulted in improvement of vision restoration time in dim light using rapid dark adaptometry. VA and Zn synergistically normalized conjunctival epithelium after a 6 mo supplementation. Data suggest that functional improvements of populations with suboptimal VA and Zn nutriture can be accomplished by supplementation with {lt}2 times of RDA of these nutrients.

  14. 1. Hallam Nuclear Power Facility, NE

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Hallam Nuclear Power Facility, NE 1969 1998 2. Piqua Nuclear Power Facility, OH 1969 1998 3. Bayo Canyon, NM 1982 1998 4. Kellex/Pierpont, NJ 1982 1998 5. University of California, CA 1982 1998 6. Acid/Pueblo Canyons, NM 1984 1999 7. Chupadera Mesa, NM 1984 1999 8. Canonsburg, PA 1986 1999 9.Shiprock, NM 1987 2000 10. Middlesex Municipal Landfill, NJ 1987 2000 11. Niagara Falls Storage Site Vicinity Properties, NY 1987 2001 12. Salt Lake City, UT 1989 2001 13. Spook, WY 1989 2001 14. National

  15. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Author Resources The following is a randomly ordered set of useful resources for people writing MiniBooNE publications:- Have a journal in mind when first putting together the paper. Each journal has LaTeX style files that can be downloaded from their web pages. There is a nice little LaTeX macro that will put line numbers by each line of your document. This makes it much easier for people to feedback comments on the paper. To use it just put \RequirePackage{lineno} just before the

  16. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Publications Goto: refereed publications , theses , related publications, proposals/TDRs. Refereed publications by the MiniBooNE Collaboration: A.A. Aguilar-Arevalo et al., Measurement of the Antineutrino Neutral-Current Elastic Differential Cross Section, arXiv:1309.7257, Phys. Rev. D91, 012004 (2015), Data Release A.A. Aguilar-Arevalo et al., First Measurement of the Muon Antineutrino Double Differential Charged Current Quasi-Elastic Cross Section, arXiv:1301.7067, Phys. Rev. D88, 032001

  17. BooNE: Booster Neutrino Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Virtual Tour This series of pages about MiniBooNE will help you understand more about the what, why, and how of our experiment. When you begin the tour, a new window will open and you can use the next and back buttons to navigate. You may exit at any time by clicking on the "X" button in the upper right hand corner of the window. Start the tour here... This tour was created by Jessica Falco in 2000 and updated by Kelly O'Hear in 2002. Jessica and Kelly were high school students who

  18. NE Blog Archive | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Blog Archive NE Blog Archive RSS December 21, 2015 The Department of Energy is working toward long-term solutions for nuclear waste storage. | Photo by <a href="https://www.flickr.com/photos/mandj98/">James Marvin Phelps</a>. Finding Long-Term Solutions for Nuclear Waste Find out how we are working with communities, tribes and states to find long-term nuclear waste storage solutions. July 15, 2015 This image of Pluto, taken by New Horizons after a 9 1/2-year journey, is our

  19. CA Mr. Andrew Wallo, III, NE-23

    Office of Legacy Management (LM)

    ?9OQ, 95.5 L'E&nt Plaza, SW.. W.ashin@.m, D.C. 20024.2174, Tekphone: (202) 488AQOO 7117-03.B7.cdy.43 23 September 1987 CA Mr. Andrew Wallo, III, NE-23 Division of Facility & Site Decommissioning Projects U.S. Oepartment of Energy Germantown, Maryland 20545 Dear Mr. Wallo: ELIMINATION RECOMMENDATION -- COLLEGES AND UNIVERSITIES zh/ ! o-01 lM!tl5 ML)!o-05 PI 77!0> The attached elimination recoannendation was prepared in accordance . -1 rlL.0~ with your suggestion during our meeting on

  20. Mr. Andrew Wallo, III, NE-23

    Office of Legacy Management (LM)

    300, 955 L'E~~MI Phm.SW.:. Washin@on. LX. 200242174, T~kphonc(202)48ll. 5 7117-03.87.cdy.43 23 September 1987 cA Mr. Andrew Wallo, III, NE-23 Division of Facility & Site Decommissioning Projects U.S. Department of Energy Germantown, Maryland 20545 Dear Mr. Wallo: ELIMINATION RECOMMENDATION -- COLLEGES AND UNIVERSITIES M/).0-05 pl 0.0% The attached elimination recommendation was prepared in accordance ML.05 with your suggestion during our meeting on 22 September. The recommendation flD.o-02

  1. Mr. Andrew Wallo, III, NE-23

    Office of Legacy Management (LM)

    9% L'Enfam Plaza, S, W.. Warhin@on, D.C. 2002ijl74j Tekphow (202) 488ddO 7117-03.87.cdy.'i3 23 September 1967 ~ s ~ Mr. Andrew Wallo, III, NE-23 Oivision of Facility & Site Decommissioning Projects U.S. Department of Energy Germantown, Maryland 20545 Dear Mr. Wallo: ELIMINATION RECOMMENDATION -- COLLEGES AND IJNIVFRSITIES , The attached elimination reconnnendation was prepar!ad in accordance with your suggestion during our meeting on 22 September! The recommendation includes 26 colleges and

  2. Mr. Andrew Wallo, III, NE-23

    Office of Legacy Management (LM)

    suite 7900,955 L%l/onr Plaza, S. W., Washingion, D.C. 20024.?174,, Telephone: (202) 488.~ Mr. Andrew Wallo, III, NE-23 Division of Facility & Site Decommissioning Projects U.S. Department of Energy Germantown, Maryland 20545 7117~03.87.dy.43 23 September 1987 I j / Dear Mr. Wallo: I ELIMINATION RECOMMENDATION -- COLLEGES AND UN&ITIES I . The attached elimination recommendation was prepared in accordance with your suggestion during our meeting on 22 September!. The recommend includes 26

  3. REPLY TO ATTN OF NE-301

    Office of Legacy Management (LM)

    N\I&?' d,' g 4 DATE. fdov 2 5 1980 REPLY TO ATTN OF NE-301 .* - memoraadu SUBJECT Remedial Action for Linde Air Products Plant, Tonawanda, New York TO W. E. Mott, EV In view of the General Counsel's reconsideration of the authority to proceed with remedial action on this site and your determination that remedial action is needed to protect the public health and safety, we will include this site in our program for remedial action. of this memorandum. Oak Ridge is requested to do so by copy I

  4. SSL Demonstration: Street Lighting, Kansas City, MO

    SciTech Connect (OSTI)

    2013-08-01

    GATEWAY program report brief summarizing an SSL street lighting demonstration at nine separate installations in Kansas City, MO.

  5. The MicroBooNE Experiment - About the Physics

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Physics Physics Goals MicroBooNE will collect neutrino interactions using the Booster Neutrino Beam at Fermilab and produce the first neutrino cross section measurements on argon in the 1 GeV energy range. MicroBooNE will also explore the currently unexplained excess of low energy electromagnetic events observed in the MiniBooNE experiment. Click here for public plots and physics distributions.

  6. The MicroBooNE Experiment - Getting Started

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Getting Started on MicroBooNE Welcome to MicroBooNE! This page is designed to help new MicroBooNE collaborators find their way around the experiment and Fermilab. Table of Contents Fermilab ID, Computing Accounts, and Required Training Visas for non-US Citizens Traveling to Fermilab Housing/Hotels Getting Around Communication within the Collaboration Software Getting Help Fermilab ID, Computing Accounts, and Required Training Badging changes for non-US visitors Whether obtaining a new Fermilab

  7. A=19Ne (1959AJ76)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    1959AJ76) (See Energy Level Diagram for 19Ne) GENERAL: See also Table 19.9 [Table of Energy Levels] (in PDF or PS). Theory: See (EL55A, RE55, RE55B, RA57, RE58). 1. 19Ne(β+)19F Qm = 3.256 The positron end point is 2.18 ± 0.03 (SC52A), 2.23 ± 0.05 (AL57), 2.24 ± 0.01 MeV (WE58B). The half-life is 17.4 ± 0.2 sec (HE59), 17.7 ± 0.1 (PE57), 18.3 ± 0.5 (AL57), 18.5 ± 0.5 (SC52A), 19 ± 1 (NA54B), 19.5 ± 1.0 (WE58B), 20.3 ± 0.5 sec (WH39). The absence of low-energy γ-rays (see 19F)

  8. Appearance Results from MiniBooNE Georgia Karagiorgi Columbia...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    with 1280 PMT's (10% photocathode) & optically isolated veto (240 PMT's) dominant beam component: (C or H nucleus) 14 Events in the MiniBooNE detector: Dominant neutrino...

  9. CA CAIOlf Mr. Andrew Wallo. III, NE-23

    Office of Legacy Management (LM)

    III, NE-23 Division of Facility & Site Decommissioning Projects U.S. Department of Energy ... Enclosure 4 to Aerospace letter subject: Status of Actions - FUSRAP Site List, dated ...

  10. Djurcic_MiniBooNE_NuFact2011

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Events Rate Flux x Cross-sections x Detector response External measurements (HARP, etc) rate constrained by neutrino data External and MiniBooNE Measurements 0 ,...

  11. A=20Ne (1983AJ01)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    3AJ01) (See Energy Level Diagrams for 20Ne) GENERAL: See also (1978AJ03) and Table 20.17 [Table of Energy Levels] (in PDF or PS). Shell model: (1977GR16, 1977HA1Z, 1977SC27, 1978AR1H, 1978CH26, 1978HA2C, 1978HE04, 1978MA2H, 1978RA1B, 1978TO07, 1979DA15, 1979EL04, 1979HA50, 1979HA59, 1979SI12, 1979WU06, 1980CA12, 1980MC1D, 1980RO11, 1980TE02, 1981ER03, 1981GR06, 1981KR1G, 1981SC12, 1982KA1K, 1982KI02). Collective, deformed and rotational models: (1977FO1E, 1977HA1Z, 1978HO1E, 1978PE09, 1978PI08,

  12. A=20Ne (1987AJ02)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    7AJ02) (See Energy Level Diagrams for 20Ne) GENERAL: See (1983AJ01) and Table 20.13 [Table of Energy Levels] (in PDF or PS). Shell model: (1978WI1B, 1982BR08, 1982FL04, 1982RA1N, 1982SH30, 1983BR29, 1983DR04, 1983DR03, 1984JA15, 1984PA04, 1984RA13, 1985AN16, 1985HA15, 1985HU08, 1985MI23, 1985MU10, 1986CH28, 1986COZZ, 1986HU1G, 1986WA1R, 1987PR01). Collective, deformed and rotational models: (1981OK02, 1982BR08, 1982RA1N, 1982RO06, 1982SC20, 1983DR04, 1983DR03, 1983LO05, 1983MA29, 1983MA68,

  13. MiniBooNE darkmatter collaboration

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MiniBooNE-DM Collaboration A.A. Aguilar-Arevalo,1 B. Batell,2 B.C. Brown,3 R. Carr,4 R. Cooper,5 P. deNiverville,6 R. Dharmapalan,7 R. Ford,3 F.G. Garcia,3 G. T. Garvey,8 J. Grange,9 W. Huelsnitz,8 I. L. de Icaza Astiz,1 R.A. Johnson,10 G. Karagiorgi,4 T. Katori,11 T. Kobilarcik,3 W. Ketchum,8 Q. Liu,8 W.C. Louis,8 C. Mariani,12 W. Marsh,3 D. McKeen,13 C.D. Moore,3 G.B. Mills,8 J. Mirabal,8 P. Nienaber,14 Z. Pavlovic,8 D. Perevalov,3 M. Pospelov,6 H. Ray,9 A. Ritz,6 B.P. Roe,15 M.H. Shaevitz,4

  14. Microsoft Word - NEAC International Subcommittee Recomendations List for NE and NE6.docx

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Nuclear Energy Advisory Committee International Subcommittee Report Recommendations Specifically NE Related December 8 th , 2013 (Prepared for the December 19 th , 2013 NEAC Meeting) Introduction There is a broad array of U.S. policy objectives in which nuclear energy plays a role, including: prevention of nuclear terrorism; nonproliferation; nuclear safety; energy security; climate change and environmental protection; and exports of American nuclear products with increased jobs to strengthen

  15. NE-23 List of California Sites NE-23 Hattie Car-well, SAN/NSQA Division

    Office of Legacy Management (LM)

    NE-23 Hattie Car-well, SAN/NSQA Division Attached for your information is the list of California sites we identified in our search of Manhattdn Engineer District records for the Formerly Utilized Sites Remedial Action Program (FUSRAP). None of the facilities listed qualified"fbr'FUSRAP:'~- The only site in California,that was included in FUSRAP was Gilman Hall on the University of California-Berkeley Campus. All California sites that are in our Surplus Facilities Management Prcgram are

  16. DOE - Office of Legacy Management -- Washington University - MO 07

    Office of Legacy Management (LM)

    Washington University - MO 07 FUSRAP Considered Sites Site: WASHINGTON UNIVERSITY (MO.07 ) Eliminated from consideration under FUSRAP Designated Name: Not Designated Alternate Name: None Location: St. Louis , Missouri MO.07-1 Evaluation Year: 1987 MO.07-1 Site Operations: Activities were limited to programs involving relatively small quantities of radionuclides and chemicals in a controlled environment. MO.07-3 MO.07-1 Site Disposition: Eliminated - Potential for contamination remote MO.07-1

  17. Neutrino Scattering Results from MiniBooNE R. Tayloe, Indiana...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Neutrino Scattering Results from MiniBooNE R. Tayloe, Indiana U. ECT workshop Trento, Italy, 1211 Outline: introduction, motivation MiniBooNE experiment MiniBooNE ...

  18. Selective Catalytic Oxidation (SCO) of NH3 to N2 for Hot Exhaust...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Oxidation (SCO) of NH3 to N2 for Hot Exhaust Treatment Selective Catalytic Oxidation (SCO) of NH3 to N2 for Hot Exhaust Treatment Investigation of a series of transition metal...

  19. DOE - Office of Legacy Management -- Latty Avenue Site - MO 04

    Office of Legacy Management (LM)

    Latty Avenue Site - MO 04 FUSRAP Considered Sites Latty Avenue Site, MO Alternate Name(s): Futura Coatings Futura Chemical Company Facility Hazelwood Interim Storage Site (HISS) Former Cotter Site, Latty Avenue Properties Contemporary Metals Corp. Continental Mining and Milling MO.04-1 MO.04-2 MO.04-5 MO.04-6 MO.06-8 MO.06-11 Location: 9200 Latty Avenue, Hazelwood, Missouri MO.04-1 Historical Operations: Received, stored, and processed uranium residues for the AEC. Storage and processing were

  20. MiniBooNE Numu/Numubar Disappearance Data Release

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    A Search for muon neutrino and antineutrino disappearance in MiniBooNE", arXiv:0903.2465 [hep-ex], Phys. Rev. Lett. 103, 061802 (2009) The following MiniBooNE information from the 2009 numu and numubar disappearance paper is made available to the public: Numu Disappearance ntuple file of MiniBooNE numu 90% confidence level sensitivity as a function of Dm2, for a 2-neutrino numu -> nux ocillation fit. The file contains 141 rows, with two columns: Dm2 value in the range 0.4 < Dm2 (eV2)

  1. MiniBooNE QE Cross Section Data Release

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Neutrino Charged Current Quasielastic Double Differential Cross section", arXiv:1002:2680 [hep-ex], Phys. Rev. D81, 092005 (2010) The following MiniBooNE information from the 2010 CCQE cross section paper is made available to the public: νμ CCQE cross sections: MiniBooNE flux table of predicted MiniBooNE muon neutrino flux (Table V) flux-integrated double differential cross section (Figure 13) 1D array of bin boundaries partitioning the muon kinetic energy (top) and the cosine of the muon

  2. MiniBooNE Requires a LOT of Protons

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Requires a LOT of Protons Our goal is 1 X 10 21 to be exact! In fact the Booster has been running at record intensities for over a year now delivering protons to MiniBooNE. But for MiniBooNE we actually need more, so we continue to work with our colleagues in Accelerator Division to improve the Booster performance. More protons leads directly to better coverage of the LSND allowed regions as MiniBooNE is statistically limited. Booster Monitoring and Improvement Projects This figure shows

  3. Mo99 Production Plant Layout

    SciTech Connect (OSTI)

    Woloshun, Keith Albert; Dale, Gregory E.; Naranjo, Angela Carol

    2015-06-25

    The NorthStar Medical Technologies 99Mo production facility configuration is envisioned to be 8 accelerator pairs irradiating 7 100Mo targets (one spare accelerator pair undergoing maintenance while the other 7 pairs are irradiating targets). The required shielding in every direction for the accelerators is initially estimated to be 10 feet of concrete. With the accelerator pairs on one (ground) level and spaced with the required shielding between adjacent pairs, the only practical path for target insertion and removal while minimizing floor space is vertical. The current scheme then requires a target vertical lift of nominally 10 feet through a shield stack. It is envisioned that the lift will be directly into a hot cell where an activated target can be removed from its holder and a new target attached and lowered. The hot cell is on a rail system so that a single hot cell can service all active target locations, as well as deliver the ready targets to the separations lab. On this rail system, coupled to the hot cell, will be a helium recovery and clean-up system. All helium coolant equipment is located on the upper level near to the target removal point.

  4. Neutral Current Elastic Interactions at MiniBooNE

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Current Elastic Interactions at MiniBooNE -Ranjan Dharmapalan for the MiniBooNE collaboration NuInt '11 Dehradun, India. 2 Outline: 1. The MiniBooNE Experiment 2. Neutral current Elastic scattering (theory) 3. Neutral current Elastic scattering in MiniBooNE (expt) 4. mode results 5. First look at data 6. Future plans and conclusion 3 B o o s t e r t a r g e t a n d h o r n d e t e c t o r d i r t d e c a y r e g i o n a b s o r b e r p r i m a r y b e a m t e r t i a r y b e a m s e c o n d a r

  5. MicroBooNE Project Critical Decision Documents

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Critical Decisions for MicroBooNE Documents CD-0 Mission Need CD-1 Selection of Alternatives CD-2/3a Performance Baseline and Long Lead Procurements CD-3b Start of Construction

  6. MiniBooNE/LSND Neutrino Oscillation Results

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MiniBooNE/LSND Neutrino Oscillation Results 1 M. Sorel (IFIC - CSIC & U. Valencia) Workshop on Beyond Three Family Neutrino Oscillations May 3-4, 2011, LNGS (Italy) 1. LSND ν̅ μ →ν̅ e (1993-2001) 2. MiniBooNE ν μ →ν e (2001-2007) 3. MiniBooNE ν̅ μ →ν̅ e (2006-2010) 5. Light sterile neutrino oscillations: where we stand (2011) Outline of this talk 2 4. MiniBooNE ν μ →ν μ and ν̅ μ →ν̅ μ (2001-2011) 3 LSND ν̅ μ →ν̅ e The LSND Experiment 4 Stopped pion

  7. New Oscillation Results From MiniBooNE

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Intrinsic e 20 Background prediction Intrinsic nue External measurements - HARP p+Be for - Sanford-Wang fits to world K + K 0 data MiniBooNE data...

  8. {alpha}-cluster states in N{ne}Z nuclei

    SciTech Connect (OSTI)

    Goldberg, V. Z.; Rogachev, G. V.

    2012-10-20

    The importance of studies of {alpha}-Cluster structure in N{ne}Z light nuclei is discussed. Spin-parity assignments for the low-lying levels in {sup 10}C are suggested.

  9. High Precision Measurement of the 19Ne Lifetime

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Precision Measurement of the 19 Ne Lifetime by Leah Jacklyn Broussard Department of Physics Duke University Date: Approved: Albert Young Calvin Howell Kate Scholberg Berndt Mueller John Thomas Dissertation submitted in partial fulfillment of the requirements for the degree of Doctor of Philosophy in the Department of Physics in the Graduate School of Duke University 2012 Abstract (Nuclear physics) High Precision Measurement of the 19 Ne Lifetime by Leah Jacklyn Broussard Department of Physics

  10. DOE NE Used Fuel Disposition FY2015 Working Group Presentations

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    NE Used Fuel Disposition FY2015 Working Group Presentations http://energy.sandia.gov/energy/nuclear-energy/ne-workshops/ufd-working-group-2015/ FOLDER NAME PRESENTATION TITLE AUTHOR Tuesday, June 9, 2015 UFD WG 2015-06-09 Tue Auditorium Afternoon - 1 Quantification of Cation Sorption to Engineered Barrier Materials Under Extreme Conditions Powell UFD WG 2015-06-09 Tue Auditorium Afternoon - 1 Development and Experimental Benchmark of Simulations to Predict Used Nuclear Fuel Cladding Temperatures

  11. DOE - Office of Legacy Management -- Petrolite Corp - MO 08

    Office of Legacy Management (LM)

    Petrolite Corp - MO 08 FUSRAP Considered Sites Site: PETROLITE CORP (MO.08) Eliminated from further consideration under FUSRAP Designated Name: Not Designated Alternate Name: None Location: St. Louis , Missouri MO.08-1 Evaluation Year: 1987 MO.08-4 Site Operations: Research involving test quantities of radioactive materials. MO.08-2 Site Disposition: Eliminated - Licensed - Potential for contamination remote MO.08-3 Radioactive Materials Handled: Yes Primary Radioactive Materials Handled:

  12. Missouri Department of National Resources Energy Center Mo DNR...

    Open Energy Info (EERE)

    Department of National Resources Energy Center Mo DNR Jump to: navigation, search Name: Missouri Department of National Resources Energy Center (Mo DNR) Place: Jefferson City,...

  13. Demonstration of LED Street Lighting in Kansas City, MO (Technical...

    Office of Scientific and Technical Information (OSTI)

    Report: Demonstration of LED Street Lighting in Kansas City, MO Citation Details In-Document Search Title: Demonstration of LED Street Lighting in Kansas City, MO Nine different ...

  14. Array-type NH.sub.3 sensor

    DOE Patents [OSTI]

    West, David Lawrence; Montgomery, Frederick Charles; Armstrong, Timothy R; Warmack, Robert J

    2013-12-31

    An array-type sensor that senses NH.sub.3 includes non-Nernstian sensing elements constructed from metal and/or metal-oxide electrodes on an O.sub.2 ion conducting substrate. In one example sensor, one electrode may be made of platinum, another electrode may be made of manganese (III) oxide (Mn.sub.2O.sub.3), and another electrode may be made of tungsten trioxide (WO.sub.3). Some sensing elements may further include an electrode made of La.sub.0.6Sr.sub.0.4Co.sub.0.2Fe.sub0.8O.sub.3 and another electrode made of LaCr.sub.0.95.Mg.sub.0.05O.sub.3.

  15. Hollow-fiber gas-membrane process for removal of NH{sub 3} from solution of NH{sub 3} and CO{sub 2}

    SciTech Connect (OSTI)

    Qin, Y.; Cabral, J.M.S.; Wang, S.

    1996-07-01

    A hollow-fiber supported gas membrane process for the separation of NH{sub 3} from aqueous solutions containing both NH{sub 3} and CO{sub 2} was investigated theoretically and experimentally. A lumen laminar flow and radial diffusion model was applied to calculate the membrane wall transfer coefficient from the data stripping a single volatile component, NH{sub 3} or CO{sub 2}, from their individual aqueous solutions. Influence of the type of membranes and operating conditions on mass-transfer rate were discussed, especially the influence of the membrane transfer coefficient on the film mass-transfer coefficient in the lumen. Appropriate configurations of the hollow-fiber modules for stripping of a single component were analyzed to optimize mass transfer. To predict the stripping of NH{sub 3} from a solution containing NH{sub 3} and CO{sub 2}, a mathematical model incorporating local chemical equilibria and Nernst-Planck diffusion was developed to describe the mass transport. The models described the experimental data fairly well. The experimental results showed that the supported gas membrane process can be used to remove NH{sub 3} effectively from aqueous media containing NH{sub 3} and CO{sub 2}.

  16. Measurement and Modeling of Spatial NH3 Storage Distributions in a

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Commercial Small Port Cu Zeolite Urea SCR Catalyst | Department of Energy Modeling of Spatial NH3 Storage Distributions in a Commercial Small Port Cu Zeolite Urea SCR Catalyst Measurement and Modeling of Spatial NH3 Storage Distributions in a Commercial Small Port Cu Zeolite Urea SCR Catalyst A modified Spaci-IR technique can measure transient NH3 and NOx concentrations; data have been used to calibrate and validate an SCR model, with good agreement between experiments and simulations. PDF

  17. Release on M&O Selection Final

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Federal Services LLC, of Bethesda, Maryland) has been awarded a 1.3 billion contract for management and operating (M&O) at DOE's Waste Isolation Pilot Plant (WIPP) in Carlsbad,...

  18. Modeling Study of SCR/PGM Interactions in NH3 Slip Catalysts | Department

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    of Energy Study of SCR/PGM Interactions in NH3 Slip Catalysts Modeling Study of SCR/PGM Interactions in NH3 Slip Catalysts The focus of this research is on the optimization of NH3 slip catalyst performance by simulating the behavior of different SCR/PGM configurations. PDF icon p-19_nova.pdf More Documents & Publications Experimental and Modelling Study of the Effect of Diffusional Limitations on the NH3 SCR Activity Selective ammonia slip catalyst enabling highly efficient NOx removal

  19. Exclusive Neutrino Cross Sections From MiniBooNE

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Exclusive Neutrino Cross Sections From MiniBooNE Martin Tzanov University of Colorado PANIC 2008, 9-14 November, Eilat, ISRAEL Martin Tzanov, PANIC 2008 Neutrino Cross Sections Today * Precise knowledge needed for precise oscillation measurements. * Cross section well measured above 20 GeV. * Few measurements below 20 GeV. * 20-30 years old bubble chamber experiments (mostly H 2 , D 2 ). * Neutral current cross sections are even less understood. ν CC world data CC world data ν T2K, BooNE K2K,

  20. The MicroBooNE Experiment - At Work

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MicroBooNE at Work At Work Now The Getting Started Page holds links to help find your way around Fermilab services and prepare for working on the experiment. The MicroBooNE Contact List contains contact information for collaboration members. The Working Groups Page is a portal to these sub-sites. The Operations Page is a portal to the running detector. The Meetings Page lists the current regular meeting time slots, and also lists the collaboration meeting dates with links to the DocDB for past

  1. The MicroBooNE Experiment - Conference Talks

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Talks and Posters Once you have given a MicroBooNE presentation, please send your talk to Ben Carls so it can be archived. If you have written proceedings to accompany your talk, please upload them to the MicroBooNE DocDB and send the document number to Ben. Also, remember that conference proceedings are required by Fermilab policy to be submitted to the Fermilab Technical Publications archive. Instructions for doing that appear here. Click here for Future talks. Conference Presentations Speaker

  2. MiniBooNE Antineutrino Data Van Nguyen Columbia University

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Moriond EW 2008 Coherent NC π 0 Production in the MiniBooNE Antineutrino Data Van Nguyen Columbia University for the MiniBooNE collaboration Moriond EW 2008 2 Moriond EW 2008 At low energy, NC π 0 's can be created through resonant and coherent production:  Resonant NC π 0 production:  Coherent NC π 0 production: (Signature: π 0 which is highly forward-going) NC π 0 Production 3 Moriond EW 2008 Why study coherent NC π 0 production? ➔ NC π 0 events are the dominant bgd to osc

  3. MiniBooNE at First Physics E. D. Zimmerman

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    at First Physics E. D. Zimmerman University of Colorado NBI 2003 KEK, Tsukuba November 7, 2003 MiniBooNE at First Physics Physics motivation: LSND MiniBooNE overview ¡ Beam ¡ Detector ¡ Reconstruction and particle ID First physics results Status and near future LSND decay-at-rest neutrino source ν µ -> ν e appearance search Decay-at-rest E ν <53 MeV Baseline 30 meters Energy E<53 MeV L/E ~ 1-1.5 km/GeV . . LSND oscillation signature From µ + decay at rest: Reconstruct e + and γ

  4. SHORT-BASELINE NEUTRINO PHYSICS AT MiniBooNE E. D. Zimmerman

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    NEUTRINO PHYSICS AT MiniBooNE E. D. Zimmerman University of Colorado PANIC 2011 Cambridge, Mass. 25 July 2011 Short-Baseline Neutrino Physics at MiniBooNE * MiniBooNE * Neutrino cross-sections * Hadron production channels * Oscillation physics * Antineutrino Oscillations * MiniBooNE-SciBooNE joint result Motivating MiniBooNE: LSND Liquid Scintillator Neutrino Detector * Stopped + beam at Los Alamos LAMPF produces e , , ̅ but no ̅ e (due to capture). * Look for delayed coincidence of positron

  5. EA-1801: Granite Reliable Power Wind Park Project in Coos County, NH |

    Office of Environmental Management (EM)

    Department of Energy 01: Granite Reliable Power Wind Park Project in Coos County, NH EA-1801: Granite Reliable Power Wind Park Project in Coos County, NH June 25, 2010 EA-1801: Final Environmental Impact Granite Reliable Power Wind Project, Coos County, New Hampshire July 23, 2010 EA-1801: Finding of No Significant Impact Granite Reliable Power Wind Project, Coos County, New Hampshire

  6. Oscillations results from the MiniBooNE experiment Alexis Aguilar...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    (ICN-UNAM) SILAFAE 2010, Valparaso, Chile December 6-12, 2010 Input from HARP production data 10 and interactions MiniBooNE MiniBooNE CCQE (MB...

  7. Analysis of Neutral Current 0 Events at MiniBooNE

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Neutral Current 0 Events at MiniBooNE Colin Anderson April 14, 2008 The Experiment Analysis Outline Experiment MiniBooNE Description NC 0 Overview Analysis Selection and...

  8. Elevated Temperature Tensile Tests on DU10Mo Rolled Foils

    SciTech Connect (OSTI)

    Schulthess, Jason

    2014-09-01

    Tensile mechanical properties for uranium-10 wt.% molybdenum (U10Mo) foils are required to support modeling and qualification of new monolithic fuel plate designs. It is expected that depleted uranium-10 wt% Mo (DU10Mo) mechanical behavior is representative of the low enriched U10Mo to be used in the actual fuel plates, therefore DU-10Mo was studied to simplify material processing, handling, and testing requirements. In this report, tensile testing of DU-10Mo fuel foils prepared using four different thermomechanical processing treatments were conducted to assess the impact of foil fabrication history on resultant tensile properties.

  9. RESULTS OF THE MiniBooNE NEUTRINO OSCILLATION SEARCH E. D. Zimmerman

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    RESULTS OF THE MiniBooNE NEUTRINO OSCILLATION SEARCH E. D. Zimmerman University of Colorado American Physical Society Meeting Jacksonville, April 16, 2007 Results of the MiniBooNE Neutrino Oscillation Search * Introduction to MiniBooNE * The oscillation analysis * The initial results and their implications * The next steps MiniBooNE: E898 at Fermilab * Purpose is to test LSND with: * Higher energy * Different beam * Different oscillation signature * Different systematics * L=500 meters, E=0.5-1

  10. 2011 Annual Planning Summary for Nuclear Energy (NE) | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Nuclear Energy (NE) 2011 Annual Planning Summary for Nuclear Energy (NE) The ongoing and projected Environmental Assessments and Environmental Impact Statements for 2011 and 2012 within the Nuclear Energy (NE). PDF icon 2011 Annual Planning Summary for Nuclear Energy (NE) More Documents & Publications 2012 Annual Planning Summary for Fossil Energy, National Energy Technology Laboratory, RMOTC, and Strategic Petroleum Reserve Field Office 2011 Annual Planning Summary for NNSA Service Center

  11. Morgan Wascko Imperial College London MiniBooNE's First Neutrino Oscillation Result

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Wascko Imperial College London MiniBooNE's First Neutrino Oscillation Result Morgan Wascko CalTech Physics Research Conference 26 April, 2007 Outline * A short course in the physics of ν oscillations * What are neutrinos? Oscillations? * ν oscillation landscape * MiniBooNE * Experiment description * MiniBooNE's First Results * Neutrino Physics Big Picture * Next Steps for the Field * What has MiniBooNE told us? 2 Morgan Wascko CalTech Physics Research Conference 26 April, 2007 * Particle

  12. Application for Presidential Permit OE Docket No. PP-400 TDI- NE New

    Energy Savers [EERE]

    England Clean Power Link Project | Department of Energy NE New England Clean Power Link Project Application for Presidential Permit OE Docket No. PP-400 TDI- NE New England Clean Power Link Project Response to TDI - NE application from State Department to construct, operate, and maintain electric transmission facilities at the U.S. - Canada Border. PDF icon State Department Concurrence.pdf More Documents & Publications Application for Presidential Permit OE Docket No. PP-400 TDI-NE New

  13. Oxidation, Reduction, and Condensation of Alcohols over (MO3)3 (M=Mo, W) Nanoclusters

    SciTech Connect (OSTI)

    Fang, Zongtang; Li, Zhenjun; Kelley, Matthew S.; Kay, Bruce D.; Li, Shenggang; Hennigan, Jamie M.; Rousseau, Roger J.; Dohnalek, Zdenek; Dixon, David A.

    2014-10-02

    The reactions of deuterated methanol, ethanol, 1-propanol, 1-butanol, 2-propanol, 2-butanol and t-butanol over cyclic (MO3)3 (M = Mo, W) clusters were studied experimentally with temperature programmed desorption (TPD) and theoretically with coupled cluster CCSD(T) theory and density functional theory. The reactions of two alcohols per M3O9 cluster are required to provide agreement with experiment for D2O release, dehydrogenation and dehydration. The reaction begins with the elimination of water by proton transfers and forms an intermediate dialkoxy species which can undergo further reaction. Dehydration proceeds by a ? hydrogen transfer to a terminal M=O. Dehydrogenation takes place via an ? hydrogen transfer to an adjacent MoVI = O atom or a WVI metal center with redox involved for M = Mo and no redox for M = W. The two channels have comparable activation energies. H/D exchange to produce alcohols can take place after olefin is released or via the dialkoxy species depending on the alcohol and the cluster. The Lewis acidity of the metal center with WVI being larger than MoVI results in the increased reactivity of W3O9 over Mo3O9 for dehydrogenation and dehydration.

  14. Simulation of an Ar/NH{sub 3} low pressure magnetized direct current discharge

    SciTech Connect (OSTI)

    Li Zhi [School of Science, University of Science and Technology Liaoning, Anshan 114051 (China); School of Physics and Optoelectronic Engineering, Dalian University of Technology, Dalian 116024 (China); Zhao Zhen [School of Chemistry and Life Science, Anshan Normal University, Anshan 114007 (China); School of Chemical Engineering, University of Science and Technology Liaoning, Anshan 114051 (China); Li Xuehui [Physiccal Science and Technical College, Dalian University, Dalian 116622 (China)

    2013-01-15

    A two-dimensional fluid model has been used to investigate the properties of plasma in an Ar/NH{sub 3} low pressure magnetized direct current discharge. We compared the simulation results with the theoretical and experimental results of the other gas discharge in which the magnetic field is considered. Results that obtained using this method are in good agreement with literature. The simulation results show that the positive ammonia ion density follows the positive argon ion density. The Ar{sub 2}{sup +} density is slightly higher than the Ar{sup +} density at 100 mTorr. The largest ammonia ion is NH{sub 3}{sup +} ion, followed by NH{sub 2}{sup +}, NH{sub 4}{sup +}, and NH{sup +} ions. The contribution of NH{sup +} ions to the density of the positive ammonia ions is marginal. The influence of pressure on the plasma discharge has been studied by simulation, and the mechanisms have been discussed. The average plasma density increases as pressure increased. The plasma density appears to be more inhomogeneous than that at the lower pressure. The ratio of charge particles changed as pressure increased. The Ar{sup +} density is slightly higher than the Ar{sub 2}{sup +} density as the pressure increased. It makes NH{sub 4}{sup +} ratio increase as pressure increased. It shows that the electron temperature drops with rising pressure by numerical calculation.

  15. NH3-Selective Catalytic Reduction over Ag/Al2O3 Catalysts | Department of

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Energy -Selective Catalytic Reduction over Ag/Al2O3 Catalysts NH3-Selective Catalytic Reduction over Ag/Al2O3 Catalysts DRIFT spectroscopy used together with flow reactor experiments to investigate the role of H2 for SCR over Ag/Al2O3 PDF icon deer12_tamm.pdf More Documents & Publications Progress on Acidic Zirconia Mixed Oxides for Efficient NH3-SCR Catalysis Experimental and Modelling Study of the Effect of Diffusional Limitations on the NH3 SCR Activity Development of Optimal Catalyst

  16. Overview of DOE-NE Proliferation and Terrorism Risk Assessment

    SciTech Connect (OSTI)

    Sadasivan, Pratap

    2012-08-24

    Research objectives are: (1) Develop technologies and other solutions that can improve the reliability, sustain the safety, and extend the life of current reactors; (2) Develop improvements in the affordability of new reactors to enable nuclear energy; (3) Develop Sustainable Nuclear Fuel Cycles; and (4) Understand and minimize the risks of nuclear proliferation and terrorism. The goal is to enable the use of risk information to inform NE R&D program planning. The PTRA program supports DOE-NE's goal of using risk information to inform R&D program planning. The FY12 PTRA program is focused on terrorism risk. The program includes a mix of innovative methods that support the general practice of risk assessments, and selected applications.

  17. MICROBOONE PHYSICS Ben Carls Fermilab MicroBooNE Physics Outline

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    PHYSICS Ben Carls Fermilab MicroBooNE Physics Outline * The detector and beam - MicroBooNE TPC - Booster and NuMI beams at Fermilab * Oscillation physics - Shed light on the MiniBooNE low energy excess * Low energy neutrino cross sections * Non-accelerator topics - Supernova neutrino detection - Proton decay backgrounds 2 B. Carls, Fermilab MicroBooNE Physics MicroBooNE Detector * 60 ton fiducial volume (of 170 tons total) liquid Argon TPC * TPC consists of 3 planes of wires; vertical Y, ±60°

  18. Microsoft PowerPoint - TAUP_07_MiniBooNE.ppt

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MinibooNE Oscillation Results and Implications Mike Shaevitz Columbia University for the MiniBooNE Collaboration 2 Outline * MiniBooNE Experiment and Analysis Techniques * MiniBooNE First Oscillation Result * Going Beyond the First Result * Future Plans and Prospects 3 LSND observed a (~3.8σ) excess of⎯ν e events in a pure⎯ν μ beam: 87.9 ± 22.4 ± 6.0 events MiniBooNE was Prompted by the Positive LSND Result Oscillation Probability: ( ) (0.264 0.067 0.045)% e P μ ν ν → = ± ± The

  19. Accelerator Production Options for 99MO

    SciTech Connect (OSTI)

    Bertsche, Kirk; /SLAC

    2010-08-25

    Shortages of {sup 99}Mo, the most commonly used diagnostic medical isotope, have caused great concern and have prompted numerous suggestions for alternate production methods. A wide variety of accelerator-based approaches have been suggested. In this paper we survey and compare the various accelerator-based approaches.

  20. MOED_of_the_Italian_Republic.PDF | Department of Energy

    Office of Environmental Management (EM)

    MOED_of_the_Italian_Republic.PDF MOED_of_the_Italian_Republic.PDF PDF icon MOED_of_the_Italian_Republic.PDF More Documents & Publications Scanned_Agreement.pdf International_Agreements_January_2001_December_2004.pdf Implementing Arrangement Between DOE and METI on R&D Cooperation on Clean Energy Technology - April 2015

  1. NH3 generation over commercial Three-Way Catalysts and Lean-NOx...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    generation over commercial Three-Way Catalysts and Lean-NOx Traps NH3 generation over commercial Three-Way Catalysts and Lean-NOx Traps Research to identify most promising...

  2. NH3 generation over commercial Three-Way Catalysts and Lean-NOx Traps

    Broader source: Energy.gov [DOE]

    Research to identify most promising catalytic formulations and operation for the in-situ generation of NH3, storage on a downstream SCR catalyst, and utilized to reduce the remaining NOx

  3. Selective Catalytic Oxidation (SCO) of NH3 to N2 for Hot Exhaust Treatment

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    | Department of Energy Oxidation (SCO) of NH3 to N2 for Hot Exhaust Treatment Selective Catalytic Oxidation (SCO) of NH3 to N2 for Hot Exhaust Treatment Investigation of a series of transition metal oxides and precious metal based catalysts for ammonia selective oxidation at low temperatures PDF icon deer12_thrun.pdf More Documents & Publications Deactivation Mechanisms of Base Metal/Zeolite Urea Selective Catalytic Reduction Materials, and Development of Zeolite-Based Hydrocarbon

  4. Spatiotemporal Distribution of NOx Storage: a Factor Controlling NH3 and

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    N2O Selectivities over a Commercial LNT Catalyst | Department of Energy Spatiotemporal Distribution of NOx Storage: a Factor Controlling NH3 and N2O Selectivities over a Commercial LNT Catalyst Spatiotemporal Distribution of NOx Storage: a Factor Controlling NH3 and N2O Selectivities over a Commercial LNT Catalyst Evaluation of commercial Ba-based LNT (CLEERS benchmark catalyst; containing oxygen storage capacity) in a bench flow reactor under fast-cycling conditions, varying reductant type,

  5. Study of On-Board Ammonia (NH3) Generation for SCR Operation | Department

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    of Energy Study of On-Board Ammonia (NH3) Generation for SCR Operation Study of On-Board Ammonia (NH3) Generation for SCR Operation The feasibility of on-board ammonia generation was examined using synthesized exhaust compositions PDF icon deer09_wong.pdf More Documents & Publications On-Board Ammonia Generation Using Delphi Diesel Fuel Reformer Delphi On-board Ammonia Generation (OAG) Reductant Utilization in a LNT + SCR System

  6. Role of SrMoO{sub 4} in Sr{sub 2}MgMoO{sub 6} synthesis

    SciTech Connect (OSTI)

    Vasala, S.; Yamauchi, H.; Karppinen, M.

    2011-05-15

    Here we investigate the elemental and phase compositions during the solid-state synthesis of the promising SOFC-anode material, Sr{sub 2}MgMoO{sub 6}, and demonstrate that molybdenum does not notably evaporate under the normal synthesis conditions with temperatures up to 1200 {sup o}C due to the formation of SrMoO{sub 4} as an intermediate product at low temperatures, below 600 {sup o}C. However, partial decomposition of the Sr{sub 2}MgMoO{sub 6} phase becomes evident at the higher temperatures ({approx}1500 {sup o}C). The effect of SrMoO{sub 4} on the electrical conductivity of Sr{sub 2}MgMoO{sub 6} is evaluated by preparing a series of Sr{sub 2}MgMoO{sub 6} samples with different amounts of additional SrMoO{sub 4}. Under the reducing operation conditions of an SOFC anode the insulating SrMoO{sub 4} phase is apparently reduced to the highly conductive SrMoO{sub 3} phase. Percolation takes place with 20-30 wt% of SrMoO{sub 4} in a Sr{sub 2}MgMoO{sub 6} matrix, with a notable increase in electrical conductivity after reduction. Conductivity values of 14, 60 and 160 S/cm are determined at 800 {sup o}C in 5% H{sub 2}/Ar for the Sr{sub 2}MgMoO{sub 6} samples with 30, 40 and 50 wt% of added SrMoO{sub 4}, respectively. -- Graphical abstract: SrMoO{sub 4} is formed at low temperatures during the synthesis of Sr{sub 2}MgMoO{sub 6}, which prevents the volatilization of Mo from typical precursor mixtures of this promising SOFC anode material. SrMoO{sub 4} is insulating and it is often found as an impurity in Sr{sub 2}MgMoO{sub 6} samples. It is however readily reduced to highly conducting SrMoO{sub 3}. Composites of Sr{sub 2}MgMoO{sub 6} and SrMoO{sub 3} show increased electrical conductivities compared to pure Sr{sub 2}MgMoO{sub 6} under the reductive operation conditions of an SOFC anode. Display Omitted Highlights: {yields} Sr{sub 2}MgMoO{sub 6} is a promising SOFC anode material. {yields} During the Sr{sub 2}MgMoO{sub 6} synthesis SrMoO{sub 4} is formed at low temperatures. {yields} Formation of SrMoO{sub 4} effectively prevents volatilization of Mo at high temperatures. {yields} Insulating SrMoO{sub 4} reduces to highly conductive SrMoO{sub 3} under SOFC-anode conditions. {yields} Composites of Sr{sub 2}MgMoO{sub 6} and SrMoO{sub 3} show high electrical conductivities.

  7. Migration of Nuclear Shell Gaps Studied in the d({sup 24}Ne,p{gamma}){sup 25}Ne Reaction

    SciTech Connect (OSTI)

    Catford, W. N.; Timis, C. N.; Baldwin, T. D.; Gelletly, W.; Pain, S. D.; Lemmon, R. C.; Pucknell, V. P. E.; Warner, D. D.; Labiche, M.; Orr, N. A.; Achouri, N. L.; Chapman, R.; Amzal, N.; Burns, M.; Liang, X.; Spohr, K.; Freer, M.; Ashwood, N. I.

    2010-05-14

    The transfer of neutrons onto {sup 24}Ne has been measured using a reaccelerated radioactive beam of {sup 24}Ne to study the (d,p) reaction in inverse kinematics. The unusual raising of the first 3/2{sup +} level in {sup 25}Ne and its significance in terms of the migration of the neutron magic number from N=20 to N=16 is put on a firm footing by confirmation of this state's identity. The raised 3/2{sup +} level is observed simultaneously with the intruder negative parity 7/2{sup -} and 3/2{sup -} levels, providing evidence for the reduction in the N=20 gap. The coincident gamma-ray decays allowed the assignment of spins as well as the transferred orbital angular momentum. The excitation energy of the 3/2{sup +} state shows that the established USD shell model breaks down well within the sd model space and requires a revised treatment of the proton-neutron monopole interaction.

  8. DOE - Office of Legacy Management -- St Louis Downtown Site - MO 02

    Office of Legacy Management (LM)

    Downtown Site - MO 02 FUSRAP Considered Sites St. Louis Downtown, MO Alternate Name(s): Destrehan Street Plant Downtown Site Mallinckrodt Chemical Plant Mallinckrodt Chemical Works MO.02-1 MO.02-3 Location: 65 Destrehan Street, St. Louis, Missouri MO.02-5 Historical Operations: Conducted uranium metal and uranium oxides research, development, and production for MED and AEC. MO.02-6 MO.02-7 Eligibility Determination: Eligible MO.02-1 Radiological Survey(s): Assessment Surveys MO.02-2 MO.02-3 Site

  9. Mo-99 | National Nuclear Security Administration

    National Nuclear Security Administration (NNSA)

    Mo-99 | National Nuclear Security Administration Facebook Twitter Youtube Flickr RSS People Mission Managing the Stockpile Preventing Proliferation Powering the Nuclear Navy Emergency Response Recapitalizing Our Infrastructure Countering Nuclear Terrorism About Our Programs Our History Who We Are Our Leadership Our Locations Budget Our Operations Library Bios Congressional Testimony Fact Sheets Newsletters Press Releases Photo Gallery Jobs Apply for Our Jobs Our Jobs Working at NNSA Blog Home /

  10. MiniBooNE LowE Data Release

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Unexplained Excess of Electron-Like Events From a 1 GeV Neutrino Beam", arXiv:0812.2243 [hep-ex], Phys. Rev. Lett. 102, 101802 (2009) The following MiniBooNE information from the 2009 updated nue oscillation paper is made available to the public: Energy Range for Default Oscillation Fit (475 MeV - 3000 MeV reconstructed neutrino energy) 1D array of bin boundaries in electron neutrino reconstructed neutrino energy 1D array of observed electron neutrino candidate events per reconstructed

  11. The MicroBooNE Project - Home Page

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Project Home Project Status Reporting Project Reports Monthly Reports Quarterly Reports, pre-CD2 PMG Meetings Project Management Group meetings are held on the 2nd Wednesday of each month, at 1pm CT in the Black Hole meeting room (WH2NW). Presentation materials are posted in the MicroBooNE DocDB, private access user-name is reviewer, password on request. From the DocDB home page, select Calendar, and on the Calendar click on PMG in the appropriate day box to bring up the meeting's Event Page.

  12. MiniBooNE Nue & Nuebar Data Release 2012

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Combined Neutrino and Antineutrino fit in 200 MeV - 3000 MeV reconstructed neutrino energy range 90% sensitivity contour, 1 sigma limit contour, 90% limit contour, 99% limit contour and 3 sigma limit contour. Sensitivity and limit curves for a 2-neutrino muon-to-electron neutrino and antineutrino oscillation fit. Frequentist studies were performed to determine the proper coverage. Each file contains a set of (sin2(2theta), Dm2 ) points on a given contour. ntuple file of MiniBooNE 2-dimensional

  13. MiniBooNE Nue & Nuebar Data Release 2012

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Antineutrino mode fit in 200 MeV - 3000 MeV reconstructed neutrino energy range 90% sensitivity contour, 1 sigma limit contour, 90% limit contour and 99% limit contour. Sensitivity and limit curves for a 2-neutrino muon-to-electron antineutrino oscillation fit. Only anti-neutrinos were assumed to oscillate. Frequentist studies were performed to determine the proper coverage. Each file contains a set of (sin2(2theta), Dm2 ) points on a given contour. ntuple file of MiniBooNE 2-dimensional

  14. MiniBooNE Nue & Nuebar Data Release 2012

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Neutrino mode fit in 200 MeV - 3000 MeV reconstructed neutrino energy range 90% sensitivity contour, 1 sigma limit contour, 90% limit contour and 99% limit contour. Sensitivity and limit curves for a 2-neutrino muon-to-electron neutrino and antineutrino oscillation fit. Frequentist studies were performed to determine the proper coverage. Each file contains a set of (sin2(2theta), Dm2 ) points on a given contour. ntuple file of MiniBooNE 2-dimensional likelihood surface as a function of ( Dm2,

  15. NE-24 Unlverslty of Chicayo Remedial Action Plan

    Office of Legacy Management (LM)

    (YJ 4 tlsj .?I2 416 17 1983 NE-24 Unlverslty of Chicayo Remedial Action Plan 22&d 7 IA +-- E. I.. Keller, Director Technical Services Division Oak Ridge Operations Ufflce In response to your memorandum dated July 29, 1983, the Field Task Proposal/Agreement (FTP/A) received frw Aryonne National Laboratory (ANL) appears to be satisfactory, and this office concurs in the use of ANL to provide the decontamination effort as noted in the FTP/A. The final decontaminatton report should Include the

  16. Office of Nuclear Energy Doe/ne-0143

    Energy Savers [EERE]

    Doe/ne-0143 Table of Contents Lesson 1 - Energy Basics Lesson 2 - Electricity Basics Lesson 3 - Atoms and Isotopes Lesson 4 - Ionizing Radiation Lesson 5 - Fission, Chain Reactions Lesson 6 - Atom to Electricity Lesson 7 - Waste from Nuclear Power Plants Lesson 8 - Concerns Lesson 9 - Energy and You 1 Lesson 1 Energy Basics ENERGY BASICS What is energy? Energy is the ability to do work. But what does that really mean? You might think of work as cleaning your room, cutting the grass, or studying

  17. Idaho National Laboratory DOE-NE's National Nuclear Capability-

    Office of Environmental Management (EM)

    -2023 Idaho National Laboratory DOE-NE's National Nuclear Capability- Developing and Maintaining the INL Infrastructure TEN-YEAR SITE PLAN DOE/ID-11474 Final June 2012 Sustainable INL continues to exceed DOE goals for reduction in the use of petroleum fuels - running its entire bus fleet on biodiesel while converting 75% of its light-duty fleet to E85 fuel. The Energy Systems Laboratory (ESL), slated for completion this year, will be a state-of-the-art laboratory with high-bay lab space where

  18. CA CAIOlf Mr. Andrew Wallo. III, NE-23

    Office of Legacy Management (LM)

    kire 7900. 955 L*E,,fa,u PLUG S. W.. Washin@ on. D.C. 20024-2174, Tekphme: (202) 488-6000 7117-03.87.cdy.43 23 September 1987 CA CAIOlf Mr. Andrew Wallo. III, NE-23 Division of Facility & Site Decommissioning Projects U.S. Department of Energy Germantown, Maryland 20545 CT.05 FL .0-o/ lti.Ob id.Or Dear Mr. Wallo: In/. O-01 flA.05 ELIMINATION RECOMMENDATION -- COLLEGES AND UNIVERSITIES Mbj.o-03 I4 v.o+ The attached elimination recommendation was prepared in accordance ML.o= with your

  19. CA M r. Andrew Wallo, III, NE-23

    Office of Legacy Management (LM)

    i900,9SS L%nfam Phm, S. W.. Washington. D.C. 20024.2174, Tlkphme: (20.7) 4S.S-M)o 7117-03.87.cdy.43 23 September 1987 CA M r. Andrew Wallo, III, NE-23 Division of Facility & Site Decommissioning Projects U.S. Department of Energy Germantown, Maryland 20545 Dear M r. Wallo: ELIMINATION RECOMMENDATION -- COLLEGES AND UNIVERSITIES I - The attached elimination recommendation was prepared in accordance M1.oS with your suggestion during our meeting on 22 September. The recommendation nO.O-02

  20. CA M r. Andrew Wallo, III. NE-23

    Office of Legacy Management (LM)

    i5W 95.5 L' E&nt plom. S. W.:. Washingr on. D.C. ZOOX2i74, Tekphm: (202) 488-6OGb 7II7-03.87.cdy.43 23 September 1987. Ii CA M r. Andrew Wallo, III. NE-23 Division of Facility & Site Decommissioning Projects U.S. Department of Energy Germantown, Maryland 20545 Dear M r. Wallo: ELIMINATION RECOMMENDATION -- COLLEGES AND UNIVERSITIES pqq.0' 05 PI ;p.03- The attached elimination recommendation was prepared in accordance ,I ML.05 with your suggestion during our meeting on 22 September. The

  1. Numerical analysis of a mixture of Ar/NH{sub 3} microwave plasma chemical vapor deposition reactor

    SciTech Connect (OSTI)

    Li Zhi [School of Physics and Optoelectronic Engineering, Dalian University of Technology, Dalian 116024 (China); School of Science, University of Science and Technology Liaoning, Anshan 114051 (China); Zhao Zhen [Chemistry Department, Anshan Normal University, Anshan 114007 (China); School of Chemical Engineering, University of Science and Technology Liaoning, Anshan 114051 (China); Li Xuehui [School of Physics and Optoelectronic Engineering, Dalian University of Technology, Dalian 116024 (China); Physical Science and Technical College, Dalian University, Dalian 116622 (China)

    2012-06-01

    A two-dimensional fluid model has been used to investigate the properties of plasma in Ar/NH{sub 3} microwave electron cyclotron resonance discharge at low pressure. The electromagnetic field model solved by the three-dimensional Simpson method is coupled to a fluid plasma model. The finite difference method was employed to discrete the governing equations. 40 species (neutrals, radicals, ions, and electrons) are consisted in the model. In total, 75 electron-neutral, 43 electron-ion, 167 neutral-neutral, 129 ion-neutral, 28 ion-ion, and 90 3-body reactions are used in the model. According to the simulation, the distribution of the densities of the considered plasma species has been showed and the mechanisms of their variations have been discussed. It is found that the main neutrals (Ar*, Ar**, NH{sub 3}{sup *}, NH, H{sub 2}, NH{sub 2}, H, and N{sub 2}) are present at high densities in Ar/NH{sub 3} microwave electron cyclotron resonance discharge when the mixing ratio of Ar/NH{sub 3} is 1:1 at 20 Pa. The density of NH is more than that of NH{sub 2} atom. And NH{sub 3}{sup +} are the most important ammonia ions. But the uniformity of the space distribution of NH{sub 3}{sup +} is lower than the other ammonia ions.

  2. Demonstration Assessment of LED Roadway Lighting: NE Cully Blvd., Portland, OR

    SciTech Connect (OSTI)

    Royer, M. P.; Poplawski, M. E.; Tuenge, J. R.

    2012-08-01

    GATEWAY program report on a demonstration of LED roadway lighting on NE Cully Boulevard in Portland, OR, a residential collector road.

  3. 2014 Annual EM/NE/SC SQA Support Group Meeting | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    4 Annual EM/NE/SC SQA Support Group Meeting 2014 Annual EM/NE/SC SQA Support Group Meeting 2014 Annual EM/NE/SC SQA Support Group Meeting The 2014 Annual Face-to-Face Meeting of the Environmental Management (EM), Nuclear Energy (NE), and Science (SC) Software Quality Assurance (SQA) Support Group (SG) was held May 6-8, 2014. This meeting was hosted by the Office of Safeguards, Security and Emergency Services (OSSES) at the Savannah River Site (SRS). The Chief of Nuclear Safety (CNS) sponsors

  4. 2015 Annual EM/NE/SC SQA Support Group Meeting | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    5 Annual EM/NE/SC SQA Support Group Meeting 2015 Annual EM/NE/SC SQA Support Group Meeting 2015 Annual EM/NE/SC SQA Support Group Meeting The Chief of Nuclear Safety (CNS) formed the Environmental Management (EM), Nuclear Energy (NE), and Science (SC) Software Quality Assurance (SQA) Support Group (SG) in March 2007. The first Annual Meeting was held August 2008. The 8th Annual Meeting will be held May 11-14, 2015. This year the Annual Meeting will be hosted by EM's Office of River Protection in

  5. High-energy physics detector MicroBooNE sees first accelerator-born

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    neutrinos MicroBooNE sees first accelerator-born neutrinos High-energy physics detector MicroBooNE sees first accelerator-born neutrinos The principal purpose of the detector is to confirm or deny the existence of a hypothetical particle known as the sterile neutrino. November 2, 2015 An accelerator-born neutrino candidate, spotted with the MicroBooNE detector. Image courtesy Fermilab. An accelerator-born neutrino candidate, spotted with the MicroBooNE detector. Image courtesy Fermilab.

  6. Kaon Monitoring in MiniBooNE: The LMC Detector E. D. Zimmerman

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Kaon Monitoring in MiniBooNE: The LMC Detector E. D. Zimmerman University of Colorado NBI 2003 KEK, Tsukuba November 10, 2003 Kaon Monitoring at MiniBooNE 1) K-decay ν e background at BooNE K production estimates 2) Decay kinematics 3) The "Little Muon Counter" (LMC) Concept/Placement Civil construction/infrastructure Collimator Fiber Tracker Temporary detector Status K-decay ν e background MiniBooNE will see ~200-400 ν e from K + and K 0 L decays each year -- comparable to the

  7. 14-07-09 MicroBooNE calibrations.pptx

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    cloud disperse: Diffusion* * Charge loss due to impurities** * Signal on wires * Induction * Collection 090714 MicroBooNE Calibrations, T. Strauss 4 First we need to...

  8. MiniBooNE as realated to "Window's on the Universe"

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    "Windows on the Universe" Ray Stefanski Fermilab Blois 2009 Windows on the Universe June 22, 2009 Outline: Introduction Current Status New Results Expectations Summary June 22, 2009 Blois 2009 Windows on the Universe 2 Introduction                 : nce disappeara : appearance s experiment n oscillatio e e   MiniBooNE   SciBooNE accelerator sources stopped muons @ LANL -> LSND BNB @ FNAL -> MiniBooNE -> SciBooNE NuMI

  9. MiniBooNE's First Oscillation Result Morgan Wascko Imperial College...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    6 July, 2007 Meson Production 9 MiniBooNE Overview * External meson production data * HARP data (CERN) * Parametrisation of cross- sections * Sanford-Wang for pions * Feynman...

  10. I. Neutrino Oscillations with the MiniBooNE Experiment at FNAL...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    E QE Events Flux x Cross-section x Detector response External measurements (HARP, etc) rate constrained by neutrino data External and MiniBooNE...

  11. Application for Presidential Permit OE Docket No. PP-400 TDI-NE New England

    Energy Savers [EERE]

    Clean Power Link Project | Department of Energy New England Clean Power Link Project Application for Presidential Permit OE Docket No. PP-400 TDI-NE New England Clean Power Link Project Response for TDI-NE from Department of Defense to construct, operate, and maintain electric transmission facilities at the U.S. - Canada Border. PDF icon PP-400 TDI-NE - Response Letter from DOD.pdf More Documents & Publications Application for Presidential Permit OE Docket No. PP-400 TDI- NE New England

  12. DOE-NE Small Business Voucher Program Launched | Department of Energy

    Energy Savers [EERE]

    DOE-NE Small Business Voucher Program Launched DOE-NE Small Business Voucher Program Launched March 1, 2016 - 9:48am Addthis News Media Contact Danielle Miller, 208-569-7806 millerdc@id.doe.gov WASHINGTON - The DOE-NE Voucher Program for eligible small businesses is open for applications. As part of the Gateway for Accelerated Innovation in Nuclear (GAIN) initiative, the NE Voucher program will provide up to $2 million in this pilot year for access to expertise, knowledge, and facilities of the

  13. Photolysis of solid NH{sub 3} and NH{sub 3}-H{sub 2}O mixtures at 193 nm

    SciTech Connect (OSTI)

    Loeffler, M. J.; Baragiola, R. A.

    2010-12-07

    We have studied UV photolysis of solid ammonia and ammonia-dihydrate samples at 40 K, using infrared spectroscopy, mass spectrometry, and microgravimetry. We have shown that in the pure NH{sub 3} sample, the main species ejected are NH{sub 3}, H{sub 2}, and N{sub 2}, where the hydrogen and nitrogen increase with laser fluence. This increase in N{sub 2} ejection with laser fluence explains the increase in mass loss rate detected by a microbalance. In contrast, for the ammonia-water mixture, we see very weak signals of H{sub 2} and N{sub 2} in the mass spectrometer, consistent with the very small mass loss during the experiment and with a <5% decrease in the NH{sub 3} infrared absorption bands spectroscopy after a fluence of {approx}3 x 10{sup 19} photons/cm{sup 2}. The results imply that ammonia-ice mixtures in the outer solar system are relatively stable under solar irradiation.

  14. A Review & Assessment of Current Operating Conditions Allowable Stresses in ASME Section III Subsection NH

    SciTech Connect (OSTI)

    R. W. Swindeman

    2009-12-14

    The current operating condition allowable stresses provided in ASME Section III, Subsection NH were reviewed for consistency with the criteria used to establish the stress allowables and with the allowable stresses provided in ASME Section II, Part D. It was found that the S{sub o} values in ASME III-NH were consistent with the S values in ASME IID for the five materials of interest. However, it was found that 0.80 S{sub r} was less than S{sub o} for some temperatures for four of the materials. Only values for alloy 800H appeared to be consistent with the criteria on which S{sub o} values are established. With the intent of undertaking a more detailed evaluation of issues related to the allowable stresses in ASME III-NH, the availabilities of databases for the five materials were reviewed and augmented databases were assembled.

  15. Progress on Acidic Zirconia Mixed Oxides for Efficient NH3-SCR Catalysis |

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Department of Energy Acidic Zirconia Mixed Oxides for Efficient NH3-SCR Catalysis Progress on Acidic Zirconia Mixed Oxides for Efficient NH3-SCR Catalysis Details progress on non-zeolitic zirconia-based mixed oxides as promising new SCR catalyst materials and results of engine bench testing of full-size SCR prototype confirms Details progress on non-zeolitic zirconia-based mixed oxides as promising new SCR catalyst materials and results of engine bench testing of full-size SCR prototype

  16. Grants to Help N.H. Towns Conserve Energy | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Grants to Help N.H. Towns Conserve Energy Grants to Help N.H. Towns Conserve Energy March 19, 2010 - 4:17pm Addthis New Hampshire has a plan to lower expenses and create jobs, all while conserving energy. In all, the state has received $17.3 million in Energy Efficiency and Conservation Block Grant (EECBG) funding. Of that, $9.6 million has been sent to the New Hampshire Office of Energy and Planning (NHOEP) to launch several energy saving projects. NHOEP established a subgrant program to award

  17. Evaluation of NH3-SCR Catalyst Technology on a 250-kW Stationary Diesel

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Genset | Department of Energy NH3-SCR Catalyst Technology on a 250-kW Stationary Diesel Genset Evaluation of NH3-SCR Catalyst Technology on a 250-kW Stationary Diesel Genset 2005 Diesel Engine Emissions Reduction (DEER) Conference Presentations and Posters PDF icon 2005_deer_malyala.pdf More Documents & Publications Two Catalyst Formulations - One Solution for NOx After-treatment Systems Engine and Reactor Evaluations of HC-SCR for Diesel NOx Reduction Development of Optimal Catalyst

  18. Development of ADECS to Meet 2010 Emission Levels: Optimization of NOx, NH3

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    and Fuel Consumption Using High and Low Engine-Out NOx Calibrations | Department of Energy ADECS to Meet 2010 Emission Levels: Optimization of NOx, NH3 and Fuel Consumption Using High and Low Engine-Out NOx Calibrations Development of ADECS to Meet 2010 Emission Levels: Optimization of NOx, NH3 and Fuel Consumption Using High and Low Engine-Out NOx Calibrations Development and validation of a simple strategy-based technique using four engine parameters to minimize emissions and fuel

  19. DOE - Office of Legacy Management -- Rogers Iron Works Co - MO 10

    Office of Legacy Management (LM)

    Rogers Iron Works Co - MO 10 FUSRAP Considered Sites Site: ROGERS IRON WORKS CO. (MO.10 ) Elimination from consideration under FUSRAP Designated Name: Not Designated Alternate Name: Rogers Iron Co. MO.10-1 Location: Joplin , Missouri MO.10-1 Evaluation Year: 1990 MO.10-2 MO.10-3 Site Operations: Tested C-liner crushing methods. MO.10-1 Site Disposition: Eliminated - Potential for contamination considered remote based on limited quantities of material handled MO.10-3 MO.10-4 Radioactive Materials

  20. Demonstration of LED Street Lighting in Kansas City, MO Kinzey...

    Office of Scientific and Technical Information (OSTI)

    Street Lighting in Kansas City, MO Kinzey, Bruce R.; Royer, Michael P.; Hadjian, M.; Kauffman, Rick LED streetlighting; field illuminance measurement LED streetlighting; field...

  1. MoRu/Be multilayers for extreme ultraviolet applications

    DOE Patents [OSTI]

    Bajt, Sasa C. (Livermore, CA); Wall, Mark A. (Stockton, CA)

    2001-01-01

    High reflectance, low intrinsic roughness and low stress multilayer systems for extreme ultraviolet (EUV) lithography comprise amorphous layers MoRu and crystalline Be layers. Reflectance greater than 70% has been demonstrated for MoRu/Be multilayers with 50 bilayer pairs. Optical throughput of MoRu/Be multilayers can be 30-40% higher than that of Mo/Be multilayer coatings. The throughput can be improved using a diffusion barrier to make sharper interfaces. A capping layer on the top surface of the multilayer improves the long-term reflectance and EUV radiation stability of the multilayer by forming a very thin native oxide that is water resistant.

  2. Dynamic Structural Response and Deformations of Monolayer MoS...

    Office of Scientific and Technical Information (OSTI)

    SciTech Connect Search Results Journal Article: Dynamic Structural Response and Deformations of Monolayer MoS 2 Visualized by Femtosecond Electron Diffraction Citation Details ...

  3. Valence and metal/silicate partitioning of Mo: Implications for...

    Office of Scientific and Technical Information (OSTI)

    Valence and metalsilicate partitioning of Mo: Implications for conditions of Earth accretion and core formation Citation Details In-Document Search Title: Valence and metal...

  4. Mo Year Report Period: EIA ID NUMBER:

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Mo Year Report Period: EIA ID NUMBER: http://www.eia.gov/survey/form/eia_14/instructions.pdf Mailing Address: Secure File Transfer option available at: (e.g., PO Box, RR) https://signon.eia.doe.gov/upload/noticeoog.jsp Electronic Transmission: The PC Electronic Zip Code - Data Reporting Option (PEDRO) is available. If interested in software, call (202) 586-9659. Email form to: OOG.SURVEYS@eia.doe.gov - - - - Fax form to: (202) 586-9772 Mail form to: Oil & Gas Survey Email address: U.S.

  5. Structure and electronic properties of Cu nanoclusters supported on Mo2C(001) and MoC(001) surfaces

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Posada-Pérez, Sergio; Viñes, Francesc; Rodríguez, José A.; Illas, Francesc

    2015-09-15

    In this study, the atomic structure and electronic properties of Cun nanoclusters (n = 4, 6, 7, and 10) supported on cubic nonpolar δ-MoC(001) and orthorhombic C- or Mo-terminated polar β-Mo2C(001) surfaces have been investigated by means of periodic density functional theory based calculations. The electronic properties have been analyzed by means of the density of states, Bader charges, and electron localization function plots. The Cu nanoparticles supported on β-Mo2C(001), either Mo- or C-terminated, tend to present a two-dimensional structure whereas a three-dimensional geometry is preferred when supported on δ-MoC(001), indicating that the Mo:C ratio and the surface polarity playmore » a key role determining the structure of supported clusters. Nevertheless, calculations also reveal important differences between the C- and Mo-terminated β-Mo2C(001) supports to the point that supported Cu particles exhibit different charge states, which opens a way to control the reactivity of these potential catalysts.« less

  6. THE GENESIS SOLAR WIND CONCENTRATOR TARGET: MASS FRACTIONATION CHARACTERISED BY NE ISOTOPES

    SciTech Connect (OSTI)

    WIENS, ROGER C.; OLINGER, C.; HEBER, V.S.; REISENFELD, D.B.; BURNETT, D.S.; ALLTON, J.H.; BAUR, H.; WIECHERT, U.; WIELER, R.

    2007-01-02

    The concentrator on Genesis provides samples of increased fluences of solar wind ions for precise determination of the oxygen isotopic composition of the solar wind. The concentration process caused mass fractionation as function of the radial target position. They measured the fractionation using Ne released by UV laser ablation along two arms of the gold cross from the concentrator target to compare measured Ne with modeled Ne. The latter is based on simulations using actual conditions of the solar wind during Genesis operation. Measured Ne abundances and isotopic composition of both arms agree within uncertainties indicating a radial symmetric concentration process. Ne data reveal a maximum concentration factor of {approx} 30% at the target center and a target-wide fractionation of Ne isotopes of 3.8%/amu with monotonously decreasing {sup 20}Ne/{sup 22}Ne ratios towards the center. The experimentally determined data, in particular the isotopic fractionation, differ from the modeled data. They discuss potential reasons and propose future attempts to overcome these disagreements.

  7. DOE - Office of Legacy Management -- West Lake Landfill - MO 05

    Office of Legacy Management (LM)

    Lake Landfill - MO 05 FUSRAP Considered Sites Site: West Lake Landfill (MO.05) Designated Name: Alternate Name: Location: Evaluation Year: Site Operations: Site Disposition: Radioactive Materials Handled: Primary Radioactive Materials Handled: Radiological Survey(s): Site Status: Also see http://www.epa.gov/oerrpage/superfund/sites/npl/nar1289.htm Documents Related to West Lake Landfill

  8. Fragile structural transition in Mo3Sb7

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Yan, Jiaqiang -Q.; McGuire, Michael A; May, Andrew F; Parker, David S.; Mandrus, D. G.; Sales, Brian C.

    2015-08-10

    Mo3Sb7 single crystals lightly doped with Cr, Ru, or Te are studied in order to explore the interplay between superconductivity, magnetism, and the cubic-tetragonal structural transition. The structural transition at 53 K is extremely sensitive to Ru or Te substitution which introduces additional electrons, but robust against Cr substitution. We observed no sign of a structural transition in superconducting Mo2.91Ru0.09Sb7 and Mo3Sb6.975Te0.025. In contrast, 3 at.% Cr doping only slightly suppresses the structural transition to 48 K while leaving no trace of superconductivity above 1.8 K. Analysis of magnetic properties suggests that the interdimer interaction in Mo3Sb7 is near amorecritical value and essential for the structural transition. Futhermore, all dopants suppress the superconductivity of Mo3Sb7. The tetragonal structure is not necessary for superconductivity.less

  9. Neutrino scattering off the stable even-even Mo isotopes

    SciTech Connect (OSTI)

    Balasi, K. G.; Kosmas, T. S.; Divari, P. C. [Theoretical Physics Section, University of Ioannina, GR 45110 Ioannina (Greece)

    2009-11-09

    Inelastic neutrino-nucleus reaction cross sections are studied focusing on the neutral current processes. Particularly, we investigate the angular and initial neutrino-energy dependence of the differential and integrated cross sections for low and intermediate energies of the incoming neutrino. The nuclear wave functions for the initial and final nuclear states are constructed in the context of the quasi-particle random phase approximation (QRPA) tested on the reproducibility of the low-lying energy spectrum. The results presented here refer to the isotopes Mo{sup 92}, Mo{sup 94}, Mo{sup 96}, Mo{sup 98} and Mo{sup 100}. These isotopes could play a significant role in supernova neutrino detection in addition to their use in double-beta and neutrinoless double-beta decay experiments (e.g. MOON, NEMO III)

  10. DOE - Office of Legacy Management -- United Nuclear Corp - MO 0-03

    Office of Legacy Management (LM)

    Nuclear Corp - MO 0-03 FUSRAP Considered Sites Site: UNITED NUCLEAR CORP. (MO.0-03) Eliminated from further consideration under FUSRAP Designated Name: Not Designated Alternate Name: Mallinckrodt Chemical Works Mallinckrodt Nuclear Corporation MO.0-03-1 MO.0-03-2 Location: Hematite , Missouri MO.0-03-1 Evaluation Year: Circa 1987 MO.0-03-3 Site Operations: Commercial fuel fabrication operation. Licensed to reclaim unirradiated enriched uranium from scrap generated in fuel fabrication and fuel

  11. DOE - Office of Legacy Management -- Spencer Chemical Co - MO 0-01

    Office of Legacy Management (LM)

    MO 0-01 FUSRAP Considered Sites Site: SPENCER CHEMICAL CO. (MO.0-01) Eliminated from further consideration under FUSRAP - an AEC licensed operation Designated Name: Not Designated Alternate Name: Jayhawk Works MO.0-01-1 Location: Joplin , Missouri MO.0-01-1 Evaluation Year: 1985 MO.0-01-2 Site Operations: Processed enriched uranium (UF-6) and scrap to produce primarily uranium dioxide (UO-2) under AEC licenses. MO.0-01-3 MO.0-01-4 Site Disposition: Eliminated - No Authority MO.0-01-2 Radioactive

  12. DOE - Office of Legacy Management -- Tyson Valley Powder Farm - MO 11

    Office of Legacy Management (LM)

    Tyson Valley Powder Farm - MO 11 FUSRAP Considered Sites Site: TYSON VALLEY POWDER FARM (MO.11) Eliminated from further consideration under FUSRAP Designated Name: Not Designated Alternate Name: None Location: St. Louis County , Missouri MO.11-1 Evaluation Year: 1987 MO.11-2 Site Operations: Storage of C-Special material (residue from production of uranium metal). MO.11-1 MO.11-2 MO.11-3 Site Disposition: Eliminated - Referred to Army Corps of Engineers MO.11-2 Radioactive Materials Handled: Yes

  13. Mo-O bond doping and related-defect assisted enhancement of photoluminescence in monolayer MoS{sub 2}

    SciTech Connect (OSTI)

    Wei, Xiaoxu; Yu, Zhihao; Cheng, Ying; Yu, Linwei; Wang, Junzhuan Wang, Xinran; Shi, Yi; Hu, Fengrui; Wang, Xiaoyong; Xiao, Min

    2014-12-15

    In this work, we report a strong photoluminescence (PL) enhancement of monolayer MoS{sub 2} under different treatments. We find that by simple ambient annealing treatment in the range of 200?C to 400?C, the PL emission can be greatly enhanced by a factor up to two orders of magnitude. This enhancement can be attributed to two factors: first, the formation of Mo-O bonds during ambient exposure introduces an effective p-doping in the MoS{sub 2} layer; second, localized electrons formed around Mo-O bonds related defective sites where the electrons can be effectively localized with higher binding energy resulting in efficient radiative excitons recombination. Time resolved PL decay measurement showed that longer lifetime of the treated sample consistent with the higher quantum efficiency in PL. These results give more insights to understand the luminescence properties of the MoS{sub 2}.

  14. The Ne-to-O abundance ratio of the interstellar medium from IBEX-Lo observations

    SciTech Connect (OSTI)

    Park, J.; Kucharek, H.; Mbius, E.; Leonard, T.; Bzowski, M.; Sok?, J. M.; Kubiak, M. A.; Fuselier, S. A.; McComas, D. J.

    2014-11-01

    In this paper we report on a two-year study to estimate the Ne/O abundance ratio in the gas phase of the local interstellar cloud (LIC). Based on the first two years of observations with the Interstellar Boundary Explorer, we determined the fluxes of interstellar neutral (ISN) O and Ne atoms at the Earth's orbit in spring 2009 and 2010. A temporal variation of the Ne/O abundance ratio at the Earth's orbit could be expected due to solar cycle-related effects such as changes of ionization. However, this study shows that there is no significant change in the Ne/O ratio at the Earths orbit from 2009 to 2010. We used time-dependent survival probabilities of the ISNs to calculate the Ne/O abundance ratio at the termination shock. Then we estimated the Ne/O abundance ratio in the gas phase of the LIC with the use of filtration factors and the ionization fractions. From our analysis, the Ne/O abundance ratio in the LIC is 0.33 0.07, which is in agreement with the abundance ratio inferred from pickup-ion measurements.

  15. Level-resolved R-matrix calculations for the electron-impact excitation of Ne{sup 3+} and Ne{sup 6+}

    SciTech Connect (OSTI)

    Ludlow, J. A.; Lee, T. G.; Ballance, C. P.; Loch, S. D.; Pindzola, M. S.

    2011-08-15

    Large-scale R-matrix calculations are carried out for the electron-impact excitation of Ne{sup 3+} and Ne{sup 6+}. For Ne{sup 3+}, a 581-LSJ-level R-matrix intermediate coupling frame transformation calculation is made for excitations up to the n=4 shell. For some transitions, large effective collision strength differences are found with current 23-jKJ-level Breit-Pauli R-matrix and earlier 22-LSJ-level R-matrix jj omega (JAJOM) calculations. For Ne{sup 6+}, a 171-jKJ-level Breit-Pauli R-matrix calculation is made for excitations up to the n=5 shell. For some transitions, large effective collision strength differences are found with current 46-jKJ-level Breit-Pauli R-matrix and earlier 46-LSJ-level R-matrix JAJOM calculations. Together with existing R-matrix calculations for other ion stages, high-quality excitation data are now available for astrophysical and laboratory plasma modeling along the entire Ne isonuclear sequence.

  16. /Users/jzennamo/Desktop/ObsLimit_MiniSciBooNE_SBN_numuDis.pdf

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    µ θ 2 2 sin 3 - 10 2 - 10 1 - 10 1 ] 2 [eV 2 m ∆ 1 - 10 1 10 2 10 POT) 20 10 × POT) and T600 (6.6 21 10 × MicroBooNE (1.3 POT) 20 10 × LAr1-ND (6.6 mode, CC Events ν Stat, Flux, Cross Section Uncerts. Reconstructed Energy Efficiency µ ν 80% Shape and Rate 90% CL CL σ 3 CL σ 5 MiniBooNE + SciBooNE 90% CL

  17. An accumulator/compressor ring for Ne+ ions (Conference) | SciTech Connect

    Office of Scientific and Technical Information (OSTI)

    Conference: An accumulator/compressor ring for Ne+ ions Citation Details In-Document Search Title: An accumulator/compressor ring for Ne+ ions The primary goal of the High Energy Density Physics (HEDP) program is to create an extremely bright ion beam at low duty cycle. For example, a typical set of parameters is: (1) Particle type = Ne{sup +}; (2) Ion energy = 20.1 MeV; (3) One ion pulse = 1 {micro}C, 1 ns, 1 mm{sup 2}; and (4) Repetition rate = 1 Hz. This would give a volume density of

  18. MiniBooNE: Up and Running Morgan Wascko Morgan Wascko Louisiana State University

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Up and Running Morgan Wascko Morgan Wascko Louisiana State University Louisiana State University Morgan O. Wascko, LSU Yang Institute Conference 11 October, 2002 MiniBooNE detector at Fermi National Accelerator Lab Outline Motivation MiniBooNE Overview Physics at MiniBooNE Current Status First Data! Morgan O. Wascko, LSU Yang Institute Conference 11 October, 2002 Neutrino Oscillations The Evidence So Far ... Solar Solar ∆ ∆ m m 2 2 ~ ~ 10 10 -(4~5) -(4~5) Atmospheric Atmospheric ∆ ∆ m m

  19. WC_2000_001_CLASS_WAIVER_BETWEEN_DOE_and_EMPLOYEES_OF_THE_NE.pdf |

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Department of Energy 2000_001_CLASS_WAIVER_BETWEEN_DOE_and_EMPLOYEES_OF_THE_NE.pdf WC_2000_001_CLASS_WAIVER_BETWEEN_DOE_and_EMPLOYEES_OF_THE_NE.pdf PDF icon WC_2000_001_CLASS_WAIVER_BETWEEN_DOE_and_EMPLOYEES_OF_THE_NE.pdf More Documents & Publications Class_Waiver_W_C-2000-001.pdf WC_1994_010__CLASS_WAIVER_of_the_Governments_Patent_Rights_.pdf WC_1994_001_CLASS_WAIVER_OF_THE_Governments_Patent_Rights_i

  20. EcoCAR: The NeXt Challenge | Department of Energy

    Office of Environmental Management (EM)

    EcoCAR: The NeXt Challenge EcoCAR: The NeXt Challenge May 18, 2010 - 7:30am Addthis While most college students' experience with vehicles goes no further than the beater they picked up for a few thousand dollars, students participating in the EcoCAR: The NeXT Challenge competition get to experience the cutting-edge of driving technology. The competition, which was established by the U.S. Department of Energy and General Motors, is a three year advanced vehicle engineering contest. Yesterday, May

  1. Polystyrene/MoS{sub 2}@oleylamine nanocomposites

    SciTech Connect (OSTI)

    Altavilla, Claudia; Ciambelli, Paolo; Fedi, Filippo; Sorrentino, Andrea; Iannace, Salvatore

    2014-05-15

    The effects of adding different concentrations of MoS{sub 2}@oleylamine nano particles on the thermal and mechanical properties of polystyrene (PS) nanocomposites have been investigated. X-ray diffraction and optical microscopy were used to characterize the morphology of the resulting nanocomposites. The thermal stability of the nanocomposites has been characterized by thermogravimetric analysis. It has been found that the MoS{sub 2}@oleylamine nanoparticles have a good compatibility with the PS matrix forming homogeneous dispersion even at high concentrations. The PS/MoS{sub 2}@oleylamine nanocomposites showed enhanced thermal stability in comparison with neat polystyrene.

  2. File:USDA-CE-Production-GIFmaps-NE.pdf | Open Energy Information

    Open Energy Info (EERE)

    NE.pdf Jump to: navigation, search File File history File usage Nebraska Ethanol Plant Locations Size of this preview: 776 600 pixels. Full resolution (1,650 1,275 pixels,...

  3. Fermilab | Newsroom | Press Releases | June 24, 2014: MicroBooNE...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    jpeg images. When using these images, please credit each photo as indicated. Med Res | Hi Res The 30-ton MicroBooNE neutrino detector was transported across the Fermilab site on...

  4. ARM - Field Campaign - 2001 Philadelphia NE-OPS Air Quality Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Philadelphia NE-OPS Air Quality Experiment ARM Data Discovery Browse Data Comments? We would love to hear from you Send us a note below or call us at 1-888-ARM-DATA. Send Campaign...

  5. Application for Presidential Permit PP-400 TDI-NE - New England...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    PP-400 TDI-NE - New England Clean Power Link Project - Motion to Intervene and Comments of the Vermont Department of Public Service - August 6, 2014 Application for Presidential...

  6. 2013 Annual DOE-NE Materials Research Coordination Meeting | Department of

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Energy Annual DOE-NE Materials Research Coordination Meeting 2013 Annual DOE-NE Materials Research Coordination Meeting The Reactor Materials element of the Nuclear Energy Enabling Technologies (NEET) program conducted its FY 2013 coordination meeting as a series of four web-conferences to act as a forum for the nuclear materials research community. The purpose of this meeting was to report on current and planned nuclear materials research, identify new areas of collaboration and promote

  7. DOE/NE Sponsors a U.S. - Kazakhstan Civilian Nuclear Energy Workshop at

    Energy Savers [EERE]

    Idaho National Laboratory | Department of Energy DOE/NE Sponsors a U.S. - Kazakhstan Civilian Nuclear Energy Workshop at Idaho National Laboratory DOE/NE Sponsors a U.S. - Kazakhstan Civilian Nuclear Energy Workshop at Idaho National Laboratory February 26, 2015 - 12:48pm Addthis U.S. and Kazakhstani participants follow a briefing about modeling and simulation U.S. and Kazakhstani participants follow a briefing about modeling and simulation Kazakhstanis ask questions about computing

  8. NE & EERE Working Together: 5 Facts About the New Energy Innovation Lab at

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Idaho National Laboratory | Department of Energy NE & EERE Working Together: 5 Facts About the New Energy Innovation Lab at Idaho National Laboratory NE & EERE Working Together: 5 Facts About the New Energy Innovation Lab at Idaho National Laboratory April 24, 2014 - 5:57pm Addthis The Energy Innovation Laboratory at the Energy Department’s Idaho National Laboratory was dedicated earlier this week. The new facility enables researchers to tackle some of the most pressing

  9. Introduction to MiniBooNE and Charged Current Quasi-Elastic (CCQE) Results

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    MiniBooNE and ν μ Charged Current Quasi-Elastic (CCQE) Results Byron P. Roe University of Michigan For the MiniBooNE collaboration 2 University of Alabama Los Alamos National Laboratory Bucknell University Louisiana State University University of Cincinnati University of Michigan University of Colorado Princeton University Columbia University Saint Mary's University of Minnesota Embry Riddle University Virginia Polytechnic Institute Fermi National Accelerator Laboratory Western Illinois

  10. Application for Presidential Permit OE Docket No. PP-400 TDI-NE - New

    Energy Savers [EERE]

    England Clean Power Link Project: Federal Register Notice, Volume 79, No. 131 - July 9, 2014 | Department of Energy - New England Clean Power Link Project: Federal Register Notice, Volume 79, No. 131 - July 9, 2014 Application for Presidential Permit OE Docket No. PP-400 TDI-NE - New England Clean Power Link Project: Federal Register Notice, Volume 79, No. 131 - July 9, 2014 Application from TDI-NE to construct, operate and maintain electric transmission facilities at the U.S. - Canada

  11. Application for Presidential Permit PP-400 TDI-NE - New England Clean Power

    Energy Savers [EERE]

    Link Project - Motion to Intervene and Comments of the Vermont Department of Public Service - August 6, 2014 | Department of Energy PP-400 TDI-NE - New England Clean Power Link Project - Motion to Intervene and Comments of the Vermont Department of Public Service - August 6, 2014 Application for Presidential Permit PP-400 TDI-NE - New England Clean Power Link Project - Motion to Intervene and Comments of the Vermont Department of Public Service - August 6, 2014 The Vermont Department of

  12. DOE - Office of Legacy Management -- Hallam Nuclear Power Facility - NE 01

    Office of Legacy Management (LM)

    Hallam Nuclear Power Facility - NE 01 FUSRAP Considered Sites Site: Hallam Nuclear Power Facility (NE.01 ) Designated Name: Alternate Name: Location: Evaluation Year: Site Operations: Site Disposition: Radioactive Materials Handled: Primary Radioactive Materials Handled: Radiological Survey(s): Site Status: Also see Hallam, Nebraska, Decommissioned Reactor Site Documents Related to Hallam Nuclear Power Facility U.S. Department of Energy 2009 Annual Inspection - Hallam, Nebraska June 2009 Page 1

  13. 2015 ANNUAL DOE-NE MATERIALS RESEARCH MEETING | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    ANNUAL DOE-NE MATERIALS RESEARCH MEETING 2015 ANNUAL DOE-NE MATERIALS RESEARCH MEETING The Reactor Materials element of the Nuclear Energy Enabling Technologies (NEET) program conducted its FY 2015 coordination meeting as a series of two web-conferences to act as a forum for the nuclear materials research community. The purpose of this meeting was to report on current and planned nuclear materials research, identify new areas of collaboration and promote greater coordination among the various

  14. DOE-NE Light Water Reactor Sustainability Program and EPRI Long-Term

    Office of Environmental Management (EM)

    Operations Program - Joint Research and Development Plan | Department of Energy DOE-NE Light Water Reactor Sustainability Program and EPRI Long-Term Operations Program - Joint Research and Development Plan DOE-NE Light Water Reactor Sustainability Program and EPRI Long-Term Operations Program - Joint Research and Development Plan Nuclear power has contributed almost 20% of the total amount of electricity generated in the United States over the past two decades. High capacity factors and low

  15. COS OBSERVATIONS OF METAL LINE AND BROAD LYMAN-{alpha} ABSORPTION IN THE MULTI-PHASE O VI AND Ne VIII SYSTEM AT z = 0.20701 TOWARD HE 0226-4110

    SciTech Connect (OSTI)

    Savage, B. D. [Department of Astronomy, University of Wisconsin-Madison, 475 North Charter Street, Madison, WI 53706 (United States); Lehner, N. [Department of Physics, University of Notre Dame, 225 Nieuwland Science Hall, Notre Dame, IN 46556 (United States); Narayanan, A. [Indian Institute of Space Science and Technology, Thiruvananthapuram 695547, Kerala (India)

    2011-12-20

    Observations of the QSO HE 0226-4110 (z{sub em} = 0.495) with the Cosmic Origins Spectrograph (COS) from 1134 to 1796 A with a resolution of {approx}17 km s{sup -1} and signal-to-noise ratio (S/N) per resolution element of 20-40 are used to study the multi-phase absorption system at z = 0.20701 containing O VI and Ne VIII. The system was previously studied with lower S/N observations with Far-Ultraviolet Spectroscopic Explorer (FUSE) and Space Telescope Imaging Spectrograph (STIS). The COS observations provide more reliable measures of the H I and metal lines present in the system and reveal the clear presence of broad Ly{alpha} (BLA) absorption with b = 72(+13, -6) km s{sup -1} and log N(H I) = 13.87 {+-} 0.08. Detecting BLAs associated with warm gas absorbers is crucial for determining the temperature, metallicity, and total baryonic content of the absorbers. The BLA is probably recording the trace amount of thermally broadened H I in the collisionally ionized plasma with log T {approx} 5.7 that also produces the O VI and Ne VIII absorption. The total hydrogen column in the collisionally ionized gas, log N(H) {approx} 20.1, exceeds that in the cooler photoionized gas in the system by a factor of {approx}22. The oxygen abundance in the collisionally ionized gas is [O/H] = -0.89 {+-} 0.08 {+-} 0.07. The absorber probably occurs in the circumgalactic environment (halo) of a foreground L = 0.25L{sub *} disk galaxy with an impact parameter of 109 h{sub 70}{sup -1} kpc identified by Mulchaey and Chen.

  16. 9 Cr-- 1 Mo steel material for high temperature application

    DOE Patents [OSTI]

    Jablonski, Paul D; Alman, David; Dogan, Omer; Holcomb, Gordon; Cowen, Christopher

    2012-11-27

    One or more embodiments relates to a high-temperature, titanium alloyed, 9 Cr-1 Mo steel exhibiting improved creep strength and oxidation resistance at service temperatures up to 650.degree. C. The 9 Cr-1 Mo steel has a tempered martensite microstructure and is comprised of both large (0.5-3 .mu.m) primary titanium carbides and small (5-50 nm) secondary titanium carbides in a ratio of. from about 1:1.5 to about 1.5:1. The 9 Cr-1 Mo steel may be fabricated using exemplary austenizing, rapid cooling, and tempering steps without subsequent hot working requirements. The 9 Cr-1 Mo steel exhibits improvements in total mass gain, yield strength, and time-to-rupture over ASTM P91 and ASTM P92 at the temperature and time conditions examined.

  17. Support effects on hydrotreating activity of NiMo catalysts

    SciTech Connect (OSTI)

    Dominguez-Crespo, M.A. Arce-Estrada, E.M.; Torres-Huerta, A.M.

    2007-10-15

    The effect of the gamma alumina particle size on the catalytic activity of NiMoS{sub x} catalysts prepared by precipitation method of aluminum acetate at pH = 10 was studied. The structural characterization of the supports was measured by using XRD, pyridine FTIR-TPD and nitrogen physisorption. NiMo catalysts were characterized during the preparation steps (annealing and sulfidation) using transmission electron microscopy (TEM). Hydrogen TPR studies of the NiMo catalysts were also carried out in order to correlate their hydrogenating properties and their catalytic functionality. Catalytic tests were carried out in a pilot plant at 613, 633 and 653 K temperatures. The results showed that the rate constants of hydrodesulfurization (HDS), hydrodenitrogenation (HDN) and hydrodearomatizing (HDA) at 613-653 K decreased in the following order: A > B > C corresponding to the increase of NiMoS particle size associated to these catalysts.

  18. CO2ReMoVe | Open Energy Information

    Open Energy Info (EERE)

    of industrial, research and service organizations with experience in CO2 geological storage. References: CO2ReMoVe1 This article is a stub. You can help OpenEI by expanding...

  19. Structural Insights into FeMo Cofactor Biosynthesis

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    a catalytic component and a specific reductase, which, in the standard system, are referred to as the MoFe protein and the Fe protein. At the active site of the...

  20. Co-Mo Electric Cooperative- Energy Efficiency Rebate Program

    Broader source: Energy.gov [DOE]

    Co-Mo Electric Cooperative provides rebates to its residential and commercial members who install air source, dual fuel, and/or geothermal heat pumps, and certain energy efficient appliances. Heat...

  1. Ethanol Conversion on Cyclic (MO3)3 (M = Mo, W) Clusters

    SciTech Connect (OSTI)

    Li, Zhenjun; Fang, Zongtang; Kelley, Matthew S.; Kay, Bruce D.; Rousseau, Roger J.; Dohnalek, Zdenek; Dixon, David A.

    2014-03-06

    Oxides of molybdenum and tungsten are an important class of catalytic materials with applications ranging from isomerization of alkanes and alkenes, partial oxidation of alcohols, selective reduction of nitric oxide and metathesis of alkeness.[1-10] While many studies have focused on the structure - function relationships, the nature of high catalytic activity is still being extensively investigated. There is a general agreement that the activity of supported MOx (M = W, Mo) catalysts is correlated with the presence of acidic sites, where the catalytic activity is strongly affected by the type of oxide support, delocalization of electron density, structures of tungsten oxide domains and presence of protons

  2. Microstructures in rapidly solidified Ni-Mo alloys

    SciTech Connect (OSTI)

    Jayaraman, N.; Tewari, S.N.; Hemker, K.J.; Glasgow, T.K.

    1985-01-01

    Ni-Mo alloys of compositions ranging from pure Ni to Ni-40 at % Mo were rapidly solidified by chill block melt spinning in vacuum and were examined by optical metallography, x-ray diffraction and transmission electron microscopy. Rapid solidification resulted in an extension of molybdenum solubility in nickel from 28 to 37.5 at %. A number of different phases and microstructures were seen at different depths (solidification conditions) from the quenched surface of the melt spun ribbons.

  3. DOE - Office of Legacy Management -- Medart Co - MO 09

    Office of Legacy Management (LM)

    Medart Co - MO 09 FUSRAP Considered Sites Site: MEDART CO. (MO.09 ) Eliminated from consideration under FUSRAP - Facility believed to be torn down and the original site built over Designated Name: Not Designated Alternate Name: None Location: 180 Potomoc Street , St. Louis , Missouri MA.09-4 Evaluation Year: Circa 1990 MA.09-3 Site Operations: Conducted test machining operations on uranium bar stock during the early 1950s. MA.09-2 Site Disposition: Eliminated - Potential for contamination

  4. DOE - Office of Legacy Management -- St Louis University - MO 0-02

    Office of Legacy Management (LM)

    University - MO 0-02 FUSRAP Considered Sites Site: ST. LOUIS UNIVERSITY (MO.0-02) Eliminated from consideration under FUSRAP - As of 1987 the facility operated under an NRC license Designated Name: Not Designated Alternate Name: None Location: St. Louis , Missouri MO.0-02-1 Evaluation Year: 1987 MO.0-02-1 Site Operations: Performed research activities involving small quantities of radioactive materials in a controlled environment. MO.0-02-1 Site Disposition: Eliminated - No Authority - Potential

  5. Structural transitions of ternary imide Li{sub 2}Mg(NH){sub 2} for hydrogen storage

    SciTech Connect (OSTI)

    Liang, C.; Gao, M. X.; Pan, H. G. Liu, Y. F.

    2014-08-25

    Phase transitions and energetic properties of Li{sub 2}Mg(NH){sub 2} with different crystal structures are investigated by experiments and first-principles calculations. The Li{sub 2}Mg(NH){sub 2} with the primitive cubic and orthorhombic structure is obtained by dynamically dehydrogenating a Mg(NH{sub 2}){sub 2}-2LiH mixture up to 280?C under an initial vacuum and 9.0?bars H{sub 2}, respectively. It is found that the obtained orthorhombic Li{sub 2}Mg(NH){sub 2} is converted to a primitive cubic structure as the dehydrogenation temperature is further increased to 400?C or performed by a 36?h of high-energetic ball milling. Moreover, the primitive cubic phase can be converted to an orthorhombic phase after heating at 280?C under 9.0?bars H{sub 2} for 1?h. Thermodynamic calculations show that the orthorhombic phase is the ground state structure of Li{sub 2}Mg(NH){sub 2}. The mechanism for phase transitions of Li{sub 2}Mg(NH){sub 2} is also discussed from the angle of energy.

  6. Coated U(Mo) Fuel: As-Fabricated Microstructures

    SciTech Connect (OSTI)

    Emmanuel Perez; Dennis D. Keiser, Jr.; Ann Leenaers; Sven Van den Berghe; Tom Wiencek

    2014-04-01

    As part of the development of low-enriched uranium fuels, fuel plates have recently been tested in the BR-2 reactor as part of the SELENIUM experiment. These fuel plates contained fuel particles with either Si or ZrN thin film coating (up to 1 m thickness) around the U-7Mo fuel particles. In order to best understand irradiation performance, it is important to determine the starting microstructure that can be observed in as-fabricated fuel plates. To this end, detailed microstructural characterization was performed on ZrN and Si-coated U-7Mo powder in samples taken from AA6061-clad fuel plates fabricated at 500C. Of interest was the condition of the thin film coatings after fabrication at a relatively high temperature. Both scanning electron microscopy and transmission electron microscopy were employed. The ZrN thin film coating was observed to consist of columns comprised of very fine ZrN grains. Relatively large amounts of porosity could be found in some areas of the thin film, along with an enrichment of oxygen around each of the the ZrN columns. In the case of the pure Si thin film coating sample, a (U,Mo,Al,Si) interaction layer was observed around the U-7Mo particles. Apparently, the Si reacted with the U-7Mo and Al matrix during fuel plate fabrication at 500C to form this layer. The microstructure of the formed layer is very similar to those that form in U-7Mo versus Al-Si alloy diffusion couples annealed at higher temperatures and as-fabricated U-7Mo dispersion fuel plates with Al-Si alloy matrix fabricated at 500C.

  7. Effects of reactant rotational excitations on H{sub 2} + NH{sub 2} → H + NH{sub 3} reactivity

    SciTech Connect (OSTI)

    Song, Hongwei; Guo, Hua

    2014-12-28

    Rotational mode specificity of the title reaction is examined using an initial state selected time-dependent wave packet method on an accurate ab initio based global potential energy surface. This penta-atomic reaction presents an ideal system to test several dynamical approximations, which might be useful for future quantum dynamics studies of polyatomic reactions, particularly with rotationally excited reactants. The first approximation involves a seven-dimensional (7D) model in which the two non-reactive N–H bonds are fixed at their equilibrium geometry. The second is the centrifugal sudden (CS) approximation within the 7D model. Finally, the J-shifting (JS) model is tested, again with the fixed N–H bonds. The spectator-bond approximation works very well in the energy range studied, while the centrifugal sudden and J-shifting integral cross sections (ICSs) agree satisfactorily with the coupled-channel counterparts in the low collision energy range, but deviate at the high energies. The calculated integral cross sections indicate that the rotational excitation of H{sub 2} somewhat inhibits the reaction while the rotational excitations of NH{sub 2} have little effect. These findings are compared with the predictions of the sudden vector projection model. Finally, a simple model is proposed to predict rotational mode specificity using K-averaged reaction probabilities.

  8. Beyond standard model searches in the MiniBooNE experiment

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Katori, Teppei; Conrad, Janet M.

    2014-08-05

    Tmore » he MiniBooNE experiment has contributed substantially to beyond standard model searches in the neutrino sector. he experiment was originally designed to test the Δm2~1eV2 region of the sterile neutrino hypothesis by observing νe(ν-e) charged current quasielastic signals from a νμ(ν-μ) beam. MiniBooNE observed excesses of νe and ν-e candidate events in neutrino and antineutrino mode, respectively. o date, these excesses have not been explained within the neutrino standard model (νSM); the standard model extended for three massive neutrinos. Confirmation is required by future experiments such as MicroBooNE. MiniBooNE also provided an opportunity for precision studies of Lorentz violation. he results set strict limits for the first time on several parameters of the standard-model extension, the generic formalism for considering Lorentz violation. Most recently, an extension to MiniBooNE running, with a beam tuned in beam-dump mode, is being performed to search for dark sector particles. In addition, this review describes these studies, demonstrating that short baseline neutrino experiments are rich environments in new physics searches.« less

  9. Ligand Bridging-Angle-Driven Assembly of Molecular Architectures Based on Quadruply Bonded Mo-Mo Dimers

    SciTech Connect (OSTI)

    Li, Jian-Rong; Yakovenko, Andrey A; Lu, Weigang; Timmons, Daren J; Zhuang, Wenjuan; Yuan, Daqiang; Zhou, Hong-Cai

    2010-12-15

    A systematic exploration of the assembly of Mo?(O?C-)?-based metalorganic molecular architectures structurally controlled by the bridging angles of rigid organic linkers has been performed. Twelve bridging dicarboxylate ligands were designed to be of different sizes with bridging angles of 0, 60, 90, and 120 while incorporating a variety of nonbridging functional groups, and these ligands were used as linkers. These dicarboxylate linkers assemble with quadruply bonded MoMo clusters acting as nodes to give 13 molecular architectures, termed metalorganic polygons/polyhedra with metal cluster node arrangements of a linear shape, triangle, octahedron, and cuboctahedron/anti-cuboctahedron. The syntheses of these complexes have been optimized and their structures determined by single-crystal X-ray diffraction. The results have shown that the shape and size of the resulting molecular architecture can be controlled by tuning the bridging angle and size of the linker, respectively. Functionalization of the linker can adjust the solubility of the ensuing molecular assembly but has little or no effect on the geometry of the product. Preliminary gas adsorption, spectroscopic, and electrochemical properties of selected members were also studied. The present work is trying to enrich metal-containing supramolecular chemistry through the inclusion of well-characterized quadruply bonded MoMo units into the structures, which can widen the prospect of additional electronic functionality, thereby leading to novel properties.

  10. F-5 U.S. Energy Information Administration | Annual Energy Outlook...

    Annual Energy Outlook [U.S. Energy Information Administration (EIA)]

    Figure F4. Oil and Gas Supply Model Regions Atlantic WA MT WY ID NV UT CO AZ NM TX OK IA KS MO IL IN KY TN MS AL FL GA SC NC WV PA NJ MD DE NY CT ME RI MA NH VA WI MI OH NE...

  11. ARM - Field Campaign - 1996 NARSTO Northeast Field Study (NARSTO-NE)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    6 NARSTO Northeast Field Study (NARSTO-NE) ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : 1996 NARSTO Northeast Field Study (NARSTO-NE) 1996.07.01 - 1996.07.28 Lead Scientist : Larry Kleinman For data sets, see below. Abstract The DOE G-1 aircraft was deployed in the New York City metropolitan area as part of the North American Research Strategy for Tropospheric Ozone-Northeast effort to determine the

  12. MiniBooNE Charged Current Charged Pion Cross Section Data Release

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Muon Neutrino-Induced Charged-Current Charged Pion Production Cross Sections on Mineral Oil at Enu~1 GeV", arXiv:1011.3572 [hep-ex], submitted to Phys. Rev. D. The following MiniBooNE information for the 2010 CC π+ cross section paper is made available to the public. Tables A root file containing histograms of all of the cross section results in the paper can be found here. A text file of the cross section results can be found here. The MiniBooNE muon neutrino flux distribution can be

  13. Microsoft PowerPoint - Oxford_MiniBooNE_and_SterileNus.ppt

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Oxford Seminar June 23, 2004 * Extensions to the Neutrino Standard Model: Sterile Neutrinos * MiniBooNE: Status and Prospects * Future Directions if MiniBooNE Sees Oscillations 2 Theoretical Prejudices before 1995 * Natural scale for ∆m 2 ~ 10 - 100 eV 2 since needed to explain dark matter * Oscillation mixing angles must be small like the quark mixing angles * Solar neutrino oscillations must be small mixing angle MSW solution because it is "cool" * Atmospheric neutrino anomaly must

  14. Numerical Analysis of Parasitic Crossing Compensation with Wires in DA$\\Phi$NE

    SciTech Connect (OSTI)

    Valishev, A.; Shatilov, D.; Milardi, C.; Zobov, M.

    2015-06-24

    Current-bearing wire compensators were successfully used in the 2005-2006 run of the DAΦNE collider to mitigate the detrimental effects of parasitic beam-beam interactions. A marked improvement of the positron beam lifetime was observed in machine operation with the KLOE detector. In view of the possible application of wire beam-beam compensators for the High Luminosity LHC upgrade, we revisit the DAΦNE experiments. We use an improved model of the accelerator with the goal to validate the modern simulation tools and provide valuable input for the LHC upgrade project.

  15. LICENSE HISTORY MO.8 Petrolite Corporation, St. Louis

    Office of Legacy Management (LM)

    LICENSE HISTORY MO.8 Petrolite Corporation, St. Louis 07,16/93 l See attached Document and Pile Sumnary for MO.8 l License History: l 24-10452-01, 30-051175, 08/13/79. Loose H-3, I-131, P-32. l 24-10452-1, 10/30/64. K66 R. R. Annand et al Multiple. . 70-621, 12-15-61, SNM license for 0.5 kg. of U-235, 93% enriched as a fuel loading and star-up ~curce for Webster Groves, Missouri reactor. l Discussion: Historical documents for this site are limited. The only information available on work done

  16. Policy Flash 2013-71 AL 2013-11 NON M&O CONTRACTOR BUSINESS SYSTEMS...

    Energy Savers [EERE]

    Policy Flash 2013-71 AL 2013-11 NON M&O CONTRACTOR BUSINESS SYSTEMS CLAUSES FOR SECTION H Policy Flash 2013-71 AL 2013-11 NON M&O CONTRACTOR BUSINESS SYSTEMS CLAUSES FOR SECTION H...

  17. Solution-based thermodynamic modeling of the Ni-Al-Mo system...

    Office of Scientific and Technical Information (OSTI)

    as (Al,Mo,Ni)0.75(Al,Mo,Ni)0.25. Thus, -fcc and -Ni3Al are modeled with a single Gibbs free energy function with appropriate treatment of the chemical ordering contribution. ...

  18. The thermal decomposition of NH{sub 2}OH and subsequent reactions : ab initio transition state theory and reflected shock tube experiments.

    SciTech Connect (OSTI)

    Klippenstein, S. J.; Harding, L. B.; Ruscic, B.; Sivaramakrishnan, R.; Srinivasan, N. K.; Su, M.-C.; Michael, J. V.; Chemical Sciences and Engineering Division; Sonoma State Univ.

    2009-01-01

    Primary and secondary reactions involved in the thermal decomposition of NH{sub 2}OH are studied with a combination of shock tube experiments and transition state theory based theoretical kinetics. This coupled theory and experiment study demonstrates the utility of NH{sub 2}OH as a high temperature source of OH radicals. The reflected shock technique is employed in the determination of OH radical time profiles via multipass electronic absorption spectrometry. O-atoms are searched for with atomic resonance absorption spectrometry. The experiments provide a direct measurement of the rate coefficient, k{sub 1}, for the thermal decomposition of NH{sub 2}OH. Secondary rate measurements are obtained for the NH{sub 2} + OH (5a) and NH{sub 2}OH + OH (6a) abstraction reactions. The experimental data are obtained for temperatures in the range from 1355 to 1889 K and are well represented by the respective rate expressions: log[k/(cm{sup 3} molecule{sup -1} s{sup -1})] = (?10.12 {+-} 0.20) + (?6793 {+-} 317 K/T) (k{sub 1}); log[k/(cm{sup 3} molecule{sup -1} s{sup -1})] = (?10.00 {+-} 0.06) + (?879 {+-} 101 K/T) (k{sub 5a}); log[k/(cm{sup 3} molecule{sup -1} s{sup -1})] = (?9.75 {+-} 0.08) + (?1248 {+-} 123 K/T) (k{sub 6a}). Theoretical predictions are made for these rate coefficients as well for the reactions of NH{sub 2}OH + NH{sub 2}, NH{sub 2}OH + NH, NH + OH, NH{sub 2} + NH{sub 2}, NH{sub 2} + NH, and NH + NH, each of which could be of secondary importance in NH{sub 2}OH thermal decomposition. The theoretical analyses employ a combination of ab initio transition state theory and master equation simulations. Comparisons between theory and experiment are made where possible. Modest adjustments of predicted barrier heights (i.e., by 2 kcal/mol or less) generally yield good agreement between theory and experiment. The rate coefficients obtained here should be of utility in modeling NO{sub x} in various combustion environments.

  19. Domestic production of medical isotope Mo-99 moves a step closer

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Domestic production of medical isotope Mo-99 Domestic production of medical isotope Mo-99 moves a step closer Irradiated uranium fuel has been recycled and reused for molybdenum-99 (Mo-99) production, with virtually no losses in Mo-99 yields or uranium recovery. May 13, 2013 From left, Los Alamos scientists Roy Copping, Sean Reilly, and Daniel Rios. Copping examines the Buchi Multivapor P-12 Evaporator, and Reilly and Rios are at the Agilent Technologies Cary 60 UV-Vis Spectrometer. From left,

  20. NNSA Awards Mo-99 Cooperative Agreement to General Atomics | National

    National Nuclear Security Administration (NNSA)

    Nuclear Security Administration Mo-99 Cooperative Agreement to General Atomics | National Nuclear Security Administration Facebook Twitter Youtube Flickr RSS People Mission Managing the Stockpile Preventing Proliferation Powering the Nuclear Navy Emergency Response Recapitalizing Our Infrastructure Countering Nuclear Terrorism About Our Programs Our History Who We Are Our Leadership Our Locations Budget Our Operations Library Bios Congressional Testimony Fact Sheets Newsletters Press

  1. Simulation of Crab Waist Collisions In DA$\\Phi$NE With KLOE-2 Interaction Region

    SciTech Connect (OSTI)

    Zobov, M.; Drago, A.; Gallo, A.; Milardi, C.; Shatilov, D.; Valishev, A.

    2015-06-24

    After the successful completion of the SIDDHARTA experiment run with crab waist collisions, the electron-positron collider DAΦNE has started routine operations for the KLOE-2 detector. The new interaction region also exploits the crab waist collision scheme, but features certain complications including the experimental detector solenoid, compensating anti-solenoids, and tilted quadrupole magnets. We have performed simulations of the beam-beam collisions in the collider taking into account the real DAΦNE nonlinear lattice. In particular, we have evaluated the effect of crab waist sextupoles and beam-beam interactions on the DAΦNE dynamical aperture and energy acceptance, and estimated the luminosity that can be potentially achieved with and without crab waist sextupoles in the present working conditions. A numerical analysis has been performed in order to propose possible steps for further luminosity increase in DAΦNE such as a better working point choice, crab sextupole strength optimization, correction of the phase advance between the sextupoles and the interaction region. The proposed change of the e- ring working point was implemented and resulted in a significant performance increase.

  2. Tuning magnetism of monolayer MoS{sub 2} by doping vacancy and applying strain

    SciTech Connect (OSTI)

    Zheng, Huiling; Yang, Baishun; Han, Ruilin; Du, Xiaobo; Yan, Yu; Wang, Dingdi

    2014-03-31

    In view of important role of inducing and manipulating the magnetism in two-dimensional materials for the development of low-dimensional spintronic devices, the influences of strain on electronic structure and magnetic properties of commonly observed vacancies doped monolayer MoS{sub 2} are investigated using first-principles calculations. It is shown that unstrained V{sub S}, V{sub S2}, and V{sub MoS3} doped monolayer MoS{sub 2} systems are nonmagnetic, while the ground state of unstrained V{sub MoS6} doped system is magnetic and the magnetic moment is contributed mainly by six Mo atoms around V{sub MoS6}. In particular, tensile strain can induce magnetic moments in V{sub S}, V{sub S2}, and V{sub MoS3} doped monolayer MoS{sub 2} due to the breaking of Mo–Mo metallic bonds around the vacancies, while the magnetization induced by V{sub MoS6} can be effectively manipulated by equibiaxial strain due to the change of Mo–Mo metallic bonds around V{sub MoS6} under strains.

  3. Defects Engineered Monolayer MoS2 for Improved Hydrogen Evolution Reaction

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Ye, Gonglan; Gong, Yongji; Lin, Junhao; Li, Bo; He, Yongmin; Pantelides, Sokrates T.; Zhou, Wu; Vajtai, Robert; Ajayan, Pulickel M.

    2016-01-13

    MoS2 is a promising, low-cost material for electrochemical hydrogen production due to its high activity and stability during the reaction. Our work represents an easy method to increase the hydrogen production in electrochemical reaction of MoS2 via defect engineering, and helps to understand the catalytic properties of MoS2.

  4. Increasing biogas yield of rural biogas digester by addition of NH/sub 4/HCO/sub 3/

    SciTech Connect (OSTI)

    Sun, G.C.; Chen, G.Q.; Chen, M.; Liu, K.X.; Zhou, S.Y.

    1983-12-01

    By addition of 0.3% NH/sub 4/HCO/sub 3/ instead of animal manure into rural biogas digester in which the rotted rice straw was the major feedstock, the biogas yield doubled in comparison with the check digester (0.1 m/sup 3//m/sup 3//d) and the fertility of NH/sub 4/HCO/sub 3/ did not decrease because of biogas fermentation. Many digesters have been built in China. But, owing to the problems of improper management, unsuitable influent mixing, etc., neither digesters nor feedstock were fully utilized. In order to solve these problems, adding NH/sub 4/HCO/sub 3/ into digester instead of animal manure was tried. Its results showed that the suitable C/N ratio of influent mixing was obtained, the fertility of effluent went up, and biogas producing rate increased. The concentration of NH/sub 4/HCO/sub 3/ is 0.2-0.6%, but the optimal is 0.3%.

  5. Update and Improve Subsection NH –– Alternative Simplified Creep-Fatigue Design Methods

    SciTech Connect (OSTI)

    Tai Asayama

    2009-10-26

    This report described the results of investigation on Task 10 of DOE/ASME Materials NGNP/Generation IV Project based on a contract between ASME Standards Technology, LLC (ASME ST-LLC) and Japan Atomic Energy Agency (JAEA). Task 10 is to Update and Improve Subsection NH -- Alternative Simplified Creep-Fatigue Design Methods. Five newly proposed promising creep-fatigue evaluation methods were investigated. Those are (1) modified ductility exhaustion method, (2) strain range separation method, (3) approach for pressure vessel application, (4) hybrid method of time fraction and ductility exhaustion, and (5) simplified model test approach. The outlines of those methods are presented first, and predictability of experimental results of these methods is demonstrated using the creep-fatigue data collected in previous Tasks 3 and 5. All the methods (except the simplified model test approach which is not ready for application) predicted experimental results fairly accurately. On the other hand, predicted creep-fatigue life in long-term regions showed considerable differences among the methodologies. These differences come from the concepts each method is based on. All the new methods investigated in this report have advantages over the currently employed time fraction rule and offer technical insights that should be thought much of in the improvement of creep-fatigue evaluation procedures. The main points of the modified ductility exhaustion method, the strain range separation method, the approach for pressure vessel application and the hybrid method can be reflected in the improvement of the current time fraction rule. The simplified mode test approach would offer a whole new advantage including robustness and simplicity which are definitely attractive but this approach is yet to be validated for implementation at this point. Therefore, this report recommends the following two steps as a course of improvement of NH based on newly proposed creep-fatigue evaluation methodologies. The first step is to modify the current approach by incorporating the partial advantages the new method offer, and the second step is to replace the current method by the simplified test approach when it has become technically mature enough. The recommendations are basically in line with the work scope of the Task Force on Creep-Fatigue of the Subgroup on Elevated Temperature Design of the Standards Committee of the ASME Boiler and Pressure Vessel Committee Section III.

  6. Thermal transport properties of metal/MoS{sub 2} interfaces from first principles

    SciTech Connect (OSTI)

    Mao, Rui; Kong, Byoung Don; Kim, Ki Wook, E-mail: kwk@ncsu.edu [Department of Electrical and Computer Engineering, North Carolina State University, Raleigh, North Carolina 27695-7911 (United States)

    2014-07-21

    Thermal transport properties at the metal/MoS{sub 2} interfaces are analyzed by using an atomistic phonon transport model based on the Landauer formalism and first-principles calculations. The considered structures include chemisorbed Sc(0001)/MoS{sub 2} and Ru(0001)/MoS{sub 2}, physisorbed Au(111)/MoS{sub 2}, as well as Pd(111)/MoS{sub 2} with intermediate characteristics. Calculated results illustrate a distinctive dependence of thermal transfer on the details of interfacial microstructures. More specifically, the chemisorbed case with a stronger bonding exhibits a generally smaller interfacial thermal resistance than the physisorbed. Comparison between metal/MoS{sub 2} and metal/graphene systems suggests that metal/MoS{sub 2} is significantly more resistive. Further examination of lattice dynamics identifies the presence of multiple distinct atomic planes and bonding patterns at the interface as the key origins of the observed large thermal resistance.

  7. Strategic Plan for Nuclear Energy -- Knowledge Base for Advanced Modeling and Simulation (NE-KAMS)

    SciTech Connect (OSTI)

    Kimberlyn C. Mousseau

    2011-10-01

    The Nuclear Energy Computational Fluid Dynamics Advanced Modeling and Simulation (NE-CAMS) system is being developed at the Idaho National Laboratory (INL) in collaboration with Bettis Laboratory, Sandia National Laboratory (SNL), Argonne National Laboratory (ANL), Utah State University (USU), and other interested parties with the objective of developing and implementing a comprehensive and readily accessible data and information management system for computational fluid dynamics (CFD) verification and validation (V&V) in support of nuclear energy systems design and safety analysis. The two key objectives of the NE-CAMS effort are to identify, collect, assess, store and maintain high resolution and high quality experimental data and related expert knowledge (metadata) for use in CFD V&V assessments specific to the nuclear energy field and to establish a working relationship with the U.S. Nuclear Regulatory Commission (NRC) to develop a CFD V&V database, including benchmark cases, that addresses and supports the associated NRC regulations and policies on the use of CFD analysis. In particular, the NE-CAMS system will support the Department of Energy Office of Nuclear Energy Advanced Modeling and Simulation (NEAMS) Program, which aims to develop and deploy advanced modeling and simulation methods and computational tools for reliable numerical simulation of nuclear reactor systems for design and safety analysis. Primary NE-CAMS Elements There are four primary elements of the NE-CAMS knowledge base designed to support computer modeling and simulation in the nuclear energy arena as listed below. Element 1. The database will contain experimental data that can be used for CFD validation that is relevant to nuclear reactor and plant processes, particularly those important to the nuclear industry and the NRC. Element 2. Qualification standards for data evaluation and classification will be incorporated and applied such that validation data sets will result in well-defined, well-characterized data. Element 3. Standards will be established for the design and operation of experiments for the generation of new validation data sets that are to be submitted to NE-CAMS that addresses the completeness and characterization of the dataset. Element 4. Standards will be developed for performing verification and validation (V&V) to establish confidence levels in CFD analyses of nuclear reactor processes; such processes will be acceptable and recognized by both CFD experts and the NRC.

  8. Undercooled and rapidly quenched Ni-Mo alloys

    SciTech Connect (OSTI)

    Tewari, S.N.; Glasgow, T.K.

    1986-01-01

    Hypoeutectic, eutectic, and hypereutectic nickel-molybdenum alloys were rapidly solidified by both bulk undercooling and melt spinning techniques. Alloys were undercooled in both electromagnetic levitation and differential thermal analysis equipment. The rate of recalescence depended upon the degree of initial undercooling and the nature (faceted or nonfaceted) of the primary nucleating phase. Alloy melts were observed to undercool more in the presence of primary Beta (NiMo intermetallic) phase than in gamma (fcc solid solution) phase. Melt spinning resulted in an extension of molybdenum solid solubility in gamma nickel, from 28 to 37.5 at % Mo. Although the microstructures observed by undercooling and melt spinning were similar the microsegregation pattern across the gamma dendries was different. The range of microstructures evolved was analyzed in terms of the nature of the primary phase to nucleate, its subsequent dendritic growth, coarsening and fragmentation, and final solidification of interfenderitic liquid.

  9. IRRADIATION PERFORMANCE OF U-Mo MONOLITHIC FUEL

    SciTech Connect (OSTI)

    M.K. Meyer; J. Gan; J.-F. Jue; D.D. Keiser; E. Perez; A. Robinson; D.M. Wachs; N. Woolstenhulme; G.L. Hofman; Y.-S. Kim

    2014-04-01

    High-performance research reactors require fuel that operates at high specific power to high fission density, but at relatively low temperatures. Research reactor fuels are designed for efficient heat rejection, and are composed of assemblies of thin-plates clad in aluminum alloy. The development of low-enriched fuels to replace high-enriched fuels for these reactors requires a substantially increased uranium density in the fuel to offset the decrease in enrichment. Very few fuel phases have been identified that have the required combination of very-high uranium density and stable fuel behavior at high burnup. UMo alloys represent the best known tradeoff in these properties. Testing of aluminum matrix U-Mo aluminum matrix dispersion fuel revealed a pattern of breakaway swelling behavior at intermediate burnup, related to the formation of a molybdenum stabilized high aluminum intermetallic phase that forms during irradiation. In the case of monolithic fuel, this issue was addressed by eliminating, as much as possible, the interfacial area between U-Mo and aluminum. Based on scoping irradiation test data, a fuel plate system composed of solid U-10Mo fuel meat, a zirconium diffusion barrier, and Al6061 cladding was selected for development. Developmental testing of this fuel system indicates that it meets core criteria for fuel qualification, including stable and predictable swelling behavior, mechanical integrity to high burnup, and geometric stability. In addition, the fuel exhibits robust behavior during power-cooling mismatch events under irradiation at high power.

  10. Microsoft PowerPoint - NOW2004_MiniBooNE.ppt

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    NOW2004 Workshop * Extensions to the Neutrino Standard Model: Sterile Neutrinos * MiniBooNE: Status and Prospects * Future Directions if MiniBooNE Sees Oscillations 2 Three Signal Regions * LSND ∆m 2 = 0.1 - 10 eV 2 , small mixing * Atmospheric ∆m 2 = 2.5×10 -3 eV 2 , large mixing * Solar ∆m 2 = 8.2×10 -5 eV 2 , large mixing ∆m 13 ∆m 12 ∆m 23 2 2 2 ( ) 1 sin 2 sin (1.27 / ) P m L E α α ν ν θ → = - ∆ 2 2 2 2 2 2 21 32 31 Three distinct neutrino oscillation signals, with For

  11. Microsoft Word - MicroBooNE CD-1 appr.docx

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    1 Approve Alternative Selection and Cost Range of the Large Liquid Argon Detector for Neutrino Physics (MicroBooNE) Project at the Fermi National Accelerator Laboratory Office of High Energy Physics Office of Science Purpose The purpose of this paper is to document the review and approval by the Office of Science Energy Systems Acquisition Advisory Board-equivalent for Critical Decision 1 (CD-1) "Approve Alternative Selection and Cost Range" for the Large Liquid Argon Detector for

  12. NE-23 Elimination of the Chupadera Mesa and Los Alamos County Industrial Waste

    Office of Legacy Management (LM)

    AM? 2 2 1986 NE-23 Elimination of the Chupadera Mesa and Los Alamos County Industrial Waste Line Sites from Further Consideration for FUSRAP Inclusion Carlos E. Garcia, Director Environmental Safety and Health Division Albuquerque Operations Office The enclosed material is being provided to you to document the final actions taken under the Department's Formerly Utilized Sites Remedial Action Program (FUSRAP) for the Chupadera Mesa area and the Los Alamos County Industrial Waste Lines, New

  13. Application for Presidential Permit OE Docket No. PP-400 TDI-NE - New

    Energy Savers [EERE]

    England Clean Power Link Project - Comments and Motion to Intervene of Conservation Law Foundation | Department of Energy Project - Comments and Motion to Intervene of Conservation Law Foundation Application for Presidential Permit OE Docket No. PP-400 TDI-NE - New England Clean Power Link Project - Comments and Motion to Intervene of Conservation Law Foundation Conservation Law Foundation (CLF) provides the following comments and Motion to Intervene regarding the Application by TDI-New

  14. Application for Presidential Permit OE Docket No. PP-400 TDI-NE - New

    Energy Savers [EERE]

    England Clean Power Link Project: Motion to Intervene of The Northeast Power Coordinating Council, Inc. | Department of Energy Project: Motion to Intervene of The Northeast Power Coordinating Council, Inc. Application for Presidential Permit OE Docket No. PP-400 TDI-NE - New England Clean Power Link Project: Motion to Intervene of The Northeast Power Coordinating Council, Inc. Northeast Power Coordinating Council, Inc. (NPCC) submits its Motion to Intervene the New England Clean Power Link

  15. Application for Presidential Permit OE Docket No. PP-400 TDI-NE New England

    Energy Savers [EERE]

    Clean Power Link Project: Notice of Intent to Prepare an Environmental Impact Statement: Federal Register Notice, Volume 79, No. 165, August 26, 2014 | Department of Energy New England Clean Power Link Project: Notice of Intent to Prepare an Environmental Impact Statement: Federal Register Notice, Volume 79, No. 165, August 26, 2014 Application for Presidential Permit OE Docket No. PP-400 TDI-NE New England Clean Power Link Project: Notice of Intent to Prepare an Environmental Impact

  16. ENERGY MEASUREMENTS GROUP EG&G SURVEY REPORT NE-F-003

    Office of Legacy Management (LM)

    * * * * * * * * * ~n~EGc.G ENERGY MEASUREMENTS GROUP EG&G SURVEY REPORT NE-F-003 FEBRUARY 1983 THE REMOTE SENSING LABORATORY OF THE UNITED STATES DEPARTMENT OF ENERGY AN AERIAL RADIOLOGICAL SURVEY OF AN AREA SURROUNDING THE FORMER MIDDLESEX SAMPLING PLANT IN MIDDLESEX, NEW JERSEY DATE OF SURVEY: MAY 1978 DISCLAIMER This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of

  17. NE-24 R&D Decontamination Projects Under the Formerly Utilized Sites Remedial

    Office of Legacy Management (LM)

    " _ ,' ,:.' : NE-24 R&D Decontamination Projects Under the Formerly Utilized Sites Remedial Action Program (FUSRAP) '. * * ,~~'.'J.' L.aGrone, Manager Oak Ridge Operations O fffce As a result of the House-Senate Conference Report and the Energy and W a ter Appropriations Act for FY 1984, and based on the data in the attached reports indicating radioactive contamination In excess of acceptable guidelines, the sites listed In the attachment and their respectfve vicinity properties

  18. Single Phase Melt Processed Powellite (Ba,Ca) MoO{sub 4} For The Immobilization Of Mo-Rich Nuclear Waste

    SciTech Connect (OSTI)

    Brinkman, Kyle; Marra, James; Fox, Kevin; Reppert, Jason; Crum, Jarrod; Tang, Ming

    2012-09-17

    Crystalline and glass composite materials are currently being investigated for the immobilization of combined High Level Waste (HLW) streams resulting from potential commercial fuel reprocessing scenarios. Several of these potential waste streams contain elevated levels of transition metal elements such as molybdenum (Mo). Molybdenum has limited solubility in typical silicate glasses used for nuclear waste immobilization. Under certain chemical and controlled cooling conditions, a powellite (Ba,Ca)MoO{sub 4} crystalline structure can be formed by reaction with alkaline earth elements. In this study, single phase BaMoO{sub 4} and CaMoO{sub 4} were formed from carbonate and oxide precursors demonstrating the viability of Mo incorporation into glass, crystalline or glass composite materials by a melt and crystallization process. X-ray diffraction, photoluminescence, and Raman spectroscopy indicated a long range ordered crystalline structure. In-situ electron irradiation studies indicated that both CaMoO{sub 4} and BaMoO{sub 4} powellite phases exhibit radiation stability up to 1000 years at anticipated doses with a crystalline to amorphous transition observed after 1 X 10{sup 13} Gy. Aqueous durability determined from product consistency tests (PCT) showed low normalized release rates for Ba, Ca, and Mo (<0.05 g/m{sup 2}).

  19. Synthesis, characterization and optical properties of NH{sub 4}Dy(PO{sub 3}){sub 4}

    SciTech Connect (OSTI)

    Chemingui, S.; Ferhi, M. Horchani-Naifer, K.; Férid, M.

    2014-09-15

    Polycrystalline powders of NH{sub 4}Dy(PO{sub 3}){sub 4} polyphosphate have been grown by the flux method. This compound was found to be isotopic with NH{sub 4}Ce(PO{sub 3}){sub 4} and RbHo(PO{sub 3}){sub 4}. It crystallizes in the monoclinic space group P2{sub 1/n} with unit cell parameters a=10.474(6) Å, b=9.011(4) Å, c=10.947(7) Å and β=106.64(3)°. The title compound has been transformed to triphosphate Dy(PO{sub 3}){sub 3} after calcination at 800 °C. Powder X-ray diffraction, infrared and Raman spectroscopies and the differential thermal analysis have been used to identify these materials. The spectroscopic properties have been investigated through absorption, excitation, emission spectra and decay curves of Dy{sup 3+} ion in both compounds at room temperature. The emission spectra show the characteristic emission bands of Dy{sup 3+} in the two compounds, before and after calcination. The integrated emission intensity ratios of the yellow to blue (I{sub Y}/I{sub B}) transitions and the chromaticity properties have been determined from emission spectra. The decay curves are found to be double-exponential. The non-exponential behavior of the decay rates was related to the resonant energy transfer as well as cross-relaxation between the donor and acceptor Dy{sup 3+} ions. The determined properties have been discussed as function of crystal structure of both compounds. They reveal that NH{sub 4}Dy(PO{sub 3}){sub 4} is promising for white light generation but Dy(PO{sub 3}){sub 3} is potential candidates in field emission display (FED) and plasma display panel (PDP) devices. - Graphical abstract: The CIE color coordinate diagrams showing the chromatic coordinates of Dy{sup 3+} luminescence in NH{sub 4}Dy(PO{sub 3}){sub 4} and Dy(PO{sub 3}){sub 3}. - Highlights: • The polycrystalline powders of NH{sub 4}Dy(PO{sub 3}){sub 4} and Dy(PO{sub 3}){sub 3} are synthesized. • The obtained powders are characterized. • The spectroscopic properties of Dy{sup 3+} ion are investigated. • Results are discussed as function of crystal structure and chemical composition. • The usefulness of NH{sub 4}Dy(PO{sub 3}){sub 4} and Dy(PO{sub 3}){sub 3} in optical devices is revealed.

  20. MCViNE- An object oriented Monte Carlo neutron ray tracing simulation package

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Lin, J. Y. Y.; Smith, Hillary L.; Granroth, Garrett E.; Abernathy, Douglas L.; Lumsden, Mark D.; Winn, Barry L.; Aczel, Adam A.; Aivazis, Michael; Fultz, Brent

    2015-11-28

    MCViNE (Monte-Carlo VIrtual Neutron Experiment) is an open-source Monte Carlo (MC) neutron ray-tracing software for performing computer modeling and simulations that mirror real neutron scattering experiments. We exploited the close similarity between how instrument components are designed and operated and how such components can be modeled in software. For example we used object oriented programming concepts for representing neutron scatterers and detector systems, and recursive algorithms for implementing multiple scattering. Combining these features together in MCViNE allows one to handle sophisticated neutron scattering problems in modern instruments, including, for example, neutron detection by complex detector systems, and single and multiplemore » scattering events in a variety of samples and sample environments. In addition, MCViNE can use simulation components from linear-chain-based MC ray tracing packages which facilitates porting instrument models from those codes. Furthermore it allows for components written solely in Python, which expedites prototyping of new components. These developments have enabled detailed simulations of neutron scattering experiments, with non-trivial samples, for time-of-flight inelastic instruments at the Spallation Neutron Source. Examples of such simulations for powder and single-crystal samples with various scattering kernels, including kernels for phonon and magnon scattering, are presented. As a result, with simulations that closely reproduce experimental results, scattering mechanisms can be turned on and off to determine how they contribute to the measured scattering intensities, improving our understanding of the underlying physics.« less

  1. Possible shape coexistence and magnetic dipole transitions in {sup 17}C and {sup 21}Ne

    SciTech Connect (OSTI)

    Sagawa, H.; Zhou, X. R.; Suzuki, Toshio; Yoshida, N.

    2008-10-15

    Magnetic dipole (M1) transitions of N=11 nuclei {sup 17}C and {sup 21}Ne are investigated by using shell model and deformed Skyrme Hartree-Fock + blocked BCS wave functions. Shell model calculations predict well observed energy spectra and magnetic dipole transitions in {sup 21}Ne, while the results are rather poor to predict these observables in {sup 17}C. In the deformed HF calculations, the ground states of the two nuclei are shown to have large prolate deformations close to {beta}{sub 2}=0.4. It is also pointed out that the first K{sup {pi}}=1/2{sup +} state in {sup 21}Ne is prolately deformed, while the first K{sup {pi}}=1/2{sup +} state in {sup 17}C is predicted to have a large oblate deformation close to the ground state in energy, We point out that the experimentally observed large hindrance of the M1 transition between I{sup {pi}}=1/2{sup +} and 3/2{sup +} in {sup 17}C can be attributed to a shape coexistence near the ground state of {sup 17}C.

  2. Comparison of GiBUU calculations with MiniBooNE pion production data

    SciTech Connect (OSTI)

    Lalakulich, O.; Mosel, U.

    2015-05-15

    Background: Neutrino-induced pion production can give important informationon the axial coupling to nucleon resonances. Furthermore, pion production represents a major background to quasielastic-like events. one pion production data from the MiniBooNE in charged current neutrino scattering in mineral oil appeared higher than expected within conventional theoretical approaches. Purpose: We aim to investigate which model parameters affect the calculated cross section and how they do this. Method: The Giessen BoltzmannUehlingUhlenbeck (GiBUU) model is used for an investigation of neutrino-nucleus reactions. Results: Presented are integrated and differential cross sections for 1?{sup +} and 1?{sup 0} production before and after final state interactions in comparison with the MiniBooNE data. Conclusions: For the MiniBooNE flux all processes (QE, 1?-background, ?, higher resonance production, DIS) contribute to the observed final state with one pion of a given charge. The uncertainty in elementary pion production cross sections leads to a corresponding uncertainty in the nuclear cross sections. Final state interactions change the shape of the muon-related observables only slightly, but they significantly change the shape of pion distributions.

  3. RELAP5 assessment using semiscale SBLOCA test S-NH-1. International Agreement Report

    SciTech Connect (OSTI)

    Lee, E.J.; Chung, B.D.; Kim, H.J.

    1993-06-01

    2-inch cold leg break test S-NH-1, conducted at the 1/1705 volume scaled facility Semiscale was analyzed using RELAP5/MOD2 Cycle 36.04 and MOD3 Version 5m5. Loss of HPIS was assumed, and reactor trip occurred on a low PZR pressure signal (13.1 MPa), and pumps began an unpowered coastdown on SI signal (12.5 MPa). The system was recovered by opening ADV`s when the PCT became higher than 811 K. Accumulator was finally injected into the system when the primary system pressure was less than 4.0 MPa. The experiment was terminated when the pressure reached the LPIS actuation set point RELAP5/MOD2 analysis demonstrated its capability to predict, with a sufficient accuracy, the main phenomena occurring in the depressurization transient, both from a qualitative and quantitative points of view. Nevertheless, several differences were noted regarding the break flow rate and inventory distribution due to deficiencies in two-phase choked flow model, horizontal stratification interfacial drag, and a CCFL model. The main reason for the core to remain nearly fully covered with the liquid was the under-prediction of the break flow by the code. Several sensitivity calculations were tried using the MOD2 to improve the results by using the different options of break flow modeling (downward, homogeneous, and area increase). The break area compensating concept based on ``the integrated break flow matching`` gave the best results than downward junction and homogeneous options. And the MOD3 showed improvement in predicting a CCFL in SG and a heatup in the core.

  4. Strategic Plan for Nuclear Energy -- Knowledge Base for Advanced Modeling and Simulation (NE-KAMS)

    SciTech Connect (OSTI)

    Rich Johnson; Kimberlyn C. Mousseau; Hyung Lee

    2011-09-01

    NE-KAMS knowledge base will assist computational analysts, physics model developers, experimentalists, nuclear reactor designers, and federal regulators by: (1) Establishing accepted standards, requirements and best practices for V&V and UQ of computational models and simulations, (2) Establishing accepted standards and procedures for qualifying and classifying experimental and numerical benchmark data, (3) Providing readily accessible databases for nuclear energy related experimental and numerical benchmark data that can be used in V&V assessments and computational methods development, (4) Providing a searchable knowledge base of information, documents and data on V&V and UQ, and (5) Providing web-enabled applications, tools and utilities for V&V and UQ activities, data assessment and processing, and information and data searches. From its inception, NE-KAMS will directly support nuclear energy research, development and demonstration programs within the U.S. Department of Energy (DOE), including the Consortium for Advanced Simulation of Light Water Reactors (CASL), the Nuclear Energy Advanced Modeling and Simulation (NEAMS), the Light Water Reactor Sustainability (LWRS), the Small Modular Reactors (SMR), and the Next Generation Nuclear Power Plant (NGNP) programs. These programs all involve computational modeling and simulation (M&S) of nuclear reactor systems, components and processes, and it is envisioned that NE-KAMS will help to coordinate and facilitate collaboration and sharing of resources and expertise for V&V and UQ across these programs. In addition, from the outset, NE-KAMS will support the use of computational M&S in the nuclear industry by developing guidelines and recommended practices aimed at quantifying the uncertainty and assessing the applicability of existing analysis models and methods. The NE-KAMS effort will initially focus on supporting the use of computational fluid dynamics (CFD) and thermal hydraulics (T/H) analysis for M&S of nuclear reactor systems, components and processes, and will later expand to include materials, fuel system performance and other areas of M&S as time and funding allow.

  5. Capacitive deionization of NH{sub 4}CIO{sub 4} solutions with carbon aerogel electrodes. Revision 1

    SciTech Connect (OSTI)

    Farmer, J.C.; Fix, D.V.; Mack, G.V.; Pekala, R.W.; Poco, J.F.

    1996-01-01

    A process for capacitive deionization of water with a stack of carbon aerogel electrodes was developed. Unlike ion exchange, one of the more conventional deionization processes, no chemicals are required for regeneration of the system; electricity is used instead. An aqueous solution of NH{sub 4}ClO{sub 4} is pumped through the electrochemical cell. After polarization, NH{sub 4}{sup +} and ClO{sub 4}{sup -} ions are removed from the water by the imposed electric field and trapped in the extensive cathodic and anodic double layers. Thsi process produces one stream of purified water and a second stream of concentrate. Effects of cell voltage, salt concentration, and cycling on electrosorption capacity were studied and results reported.

  6. A reaction mechanism for titanium nitride CVD from TiCl{sub 4} and NH{sub 3}

    SciTech Connect (OSTI)

    Larson, R.S.; Allendorf, M.D.

    1995-12-01

    A gas-phase and surface reaction mechanism for the CVD of TiN from TiCl{sub 4} and NH{sub 3} is proposed. The only gas-phase process is complex formation, which can compete with deposition. The surface mechanism postulates the stepwise elimination of Cl and H atoms from TiCl{sub 4} and NH{sub 3}, respectively, to form solid TiN and gaseous HCl. The mechanism also accounts for the change in oxidation state of Ti by allowing for liberation of N{sub 2}. Provided that the surface composition is at steady state, the stoichiometry of the overall reaction is reproduced exactly. In addition, the global kinetic law predicted by the mechanism is successfully fit to new deposition data from a rotating disk reactor and is shown to be consistent with literature results.

  7. NOIlVUlSININdV NOIlVWdOdNI AOd3N3 ACTO3NH

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    NOIlVUlSININdV NOIlVWdOdNI AOd3N3 ACTO3NH 0661 This publication may be purchased from the Superintendent of Documents, U.S. Government Printing Office. Purchasing in formation for this or other Energy Information Administration (EIA) publications may be obtained from the Government Printing Office or ElA's National Energy Information Center. Questions on energy statistics should be directed to the Center by mail, telephone, or telecommunications device for the hearing impaired. Addresses,

  8. High-temperature phase transformation and topochemical nature in ferroelastic (NH{sub 4}){sub 2}SO{sub 4}

    SciTech Connect (OSTI)

    Lee, Kwang-Sei; Oh, In-Hwan; Ko, Jae-Hyeon

    2014-04-01

    The electrical conductivity of ferroelastic ammonium sulfate (NH{sub 4}){sub 2}SO{sub 4} revealed an anomaly at around 130 C (=403 K, T{sub P}) on heating with large and irreversible thermal hysteresis through thermal cycle. Ferroelastic domain walls and surface morphology of (NH{sub 4}){sub 2}SO{sub 4} were investigated by hot-stage polarizing microscopy. Structural phase transition from an orthorhombic ferroelastic phase to a hexagonal paraelastic phase was not identified at T{sub P} upon heating. On further heating above T{sub P}, microscopic spots appeared and grew on the crystal surface, suggesting that the high-temperature anomaly at T{sub P} was an indication of an onset of thermal decomposition controlled by topochemical factors. The increase of electrical conductivity above T{sub P} was attributed to proton migration. - Graphical abstract: Surface morphology of the (100) face of (NH{sub 4}){sub 2}SO{sub 4} on heating, showing chemical reaction at the surface. - Highlights: We investigate the high-temperature phase transformation of ammonium sulfate. The increasing conductivity upon heating is attributed to proton migration. Structural phase transition from orthorhombic to hexagonal phase is not confirmed. High-temperature anomaly is related to an onset of thermal decomposition. The nature of the high-temperature anomaly is topochemical controlled by defects.

  9. 18Ne

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

  10. 19Ne

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

  11. 20Ne

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

  12. NE-24

    Office of Legacy Management (LM)

    the Bureau of Hines Site at Albany, Oregon, for Remedial Action Under the Formerly Utilized Sites Remedial Action Program I L@ _I' J.-La&one, Manager Oak Ridge Operations Office Based on the data in the attached draft reports, it has been determined that the subject site is contaminated with residual radioactive material ' as a result of Manhattan Engineer District/Atomic Energy Commission operations P * at this site. The contamination is in excess of the acceptable guidelines and warrants

  13. NE-23

    Office of Legacy Management (LM)

    4:00 p.m., Monday through Friday (except Federal holidays), at the DOE Public Document Room located in Room lE-190 of the Forrestal Building, 1000 Independence Avenue, S.W.,...

  14. Electrocatalytic Hydrogen Production by [Ni(7PPh2NH)2]2+: Removing the Distinction Between Endo- and Exo- Protonation Sites

    SciTech Connect (OSTI)

    Brown, Houston JS; Wiese, Stefan; Roberts, John A.; Bullock, R. Morris; Helm, Monte L.

    2015-04-03

    A new Ni(II) complex, [Ni(7PPh2NH)2]2+ (7PPh2NH = 3,6-triphenyl-1-aza-3,6-diphosphacycloheptane) has been synthesized, and its electrochemical properties are reported. The 7PPh2NH ligand features an NH, ensuring properly positioned protonated amine groups (NH+) for electrocatalysis, regardless of whether protonation occurs exo- or endo- to the metal center. The compound is an electrocatalyst for H2 production in the presence of organic acids (pKa range 1013 in CH3CN) with turnover frequencies ranging from 160770 s-1 at overpotentials between 320470 mV, as measured at the half peak potential of the catalytic wave. In stark contrast to [Ni(PR2NR'2)2]2+ and other [Ni(7PPh2NR')]2+ complexes, catalytic turnover frequencies for H2 production by [Ni(7PPh2NH)2]2+ do not show catalytic rate enhancement upon the addition of H2O. This finding supports the assertion that [Ni(7PPh2NH)2]2+ eliminates the distinction between the endo- and exo-protonation isomers. This research was supported as part of the Center for Molecular Electrocatalysis, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy.

  15. Domestic production of medical isotope Mo-99 moves a step closer

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    partners, including Morgridge Institute for Research-SHINE Medical Technologies (MIR-SHINE), which proposes to use a particle accelerator to produce Mo-99 from a mildly...

  16. Experimental activities supporting commercial U.S. accelerator production of 99-Mo

    SciTech Connect (OSTI)

    Dale, Gregory E [Los Alamos National Laboratory; Chemerisov, Sergey D [ANL; Vandegrift, George F [ANL

    2010-01-01

    {sup 99m}Tc, the daughter product of {sup 99}Mo, is the most commonly used radioisotope for nuclear medicine in the U.S. Experiments are being performed at Los Alamos National Laboratory and Argonne National Laboratory to demonstrate production of {sup 99}Mo using accelerators. The {sup 100}Mo({gamma},n){sup 99}Mo reaction in an enriched {sup 100}Mo target is currently under investigation. Three scaled low-power production experiments using a 20-MeV electron linac at Argonne have been performed to date. Two of these experiments used natural Mo targets and produced a total of 613 {mu}C of {sup 99}Mo. The third experiment used an enriched {sup 100}Mo target and produced 10.5 mCi of {sup 99}Mo. Following irradiation the targets were dissolved and the low specific activity solution was processed through an ARSII generator from NorthStar Medical Radioisotopes. Yields of {sup 99m}Tc >95% have been observed.

  17. Conceptual design of a new homogeneous reactor for medical radioisotope Mo-99/Tc-99m production

    SciTech Connect (OSTI)

    Liem, Peng Hong [Nippon Advanced Information Service (NAIS Co., Inc.) Scientific Computational Division, 416 Muramatsu, Tokaimura, Ibaraki (Japan); Tran, Hoai Nam [Chalmers University of Technology, Dept. of Applied Physics, Div. of Nuclear Engineering, SE-412 96 Gothenburg (Sweden); Sembiring, Tagor Malem [National Nuclear Energy Agency (BATAN), Center for Reactor Technology and Nuclear Safety, Kawasan Puspiptek, Serpong, Tangerang Selatan, Banten (Indonesia); Arbie, Bakri [PT MOTAB Technology, Kedoya Elok Plaza Blok DA 12, Jl. Panjang, Kebun Jeruk, Jakarta Barat (Indonesia)

    2014-09-30

    To partly solve the global and regional shortages of Mo-99 supply, a conceptual design of a nitrate-fuel-solution based homogeneous reactor dedicated for Mo-99/Tc-99m medical radioisotope production is proposed. The modified LEU Cintichem process for Mo-99 extraction which has been licensed and demonstrated commercially for decades by BATAN is taken into account as a key design consideration. The design characteristics and main parameters are identified and the advantageous aspects are shown by comparing with the BATAN's existing Mo-99 supply chain which uses a heterogeneous reactor (RSG GAS multipurpose reactor)

  18. Solution-based thermodynamic modeling of the Ni-Al-Mo system using

    Office of Scientific and Technical Information (OSTI)

    first-principles calculations (Journal Article) | SciTech Connect Solution-based thermodynamic modeling of the Ni-Al-Mo system using first-principles calculations Citation Details In-Document Search Title: Solution-based thermodynamic modeling of the Ni-Al-Mo system using first-principles calculations A solution-based thermodynamic description of the ternary Ni-Al-Mo system is developed here, incorporating first-principles calculations and reported modeling of the binary Ni-Al, Ni-Mo and

  19. Synthesis of molybdenum disulfide (MoS{sub 2}) for lithium ion battery applications

    SciTech Connect (OSTI)

    Feng Chuanqi; Ma Jun; Li Hua; Zeng Rong; Guo Zaiping; Liu Huakun

    2009-09-15

    This paper reports the use of a rheological phase reaction method for preparing MoS{sub 2} nanoflakes. The characterization by powder X-ray diffraction indicated that MoS{sub 2} had been formed. High resolution electron microscopy observation revealed that the as-prepared MoS{sub 2} nanoflakes had started to curve and partly form MoS{sub 2} nanotubes. The lithium intercalation/de-intercalation behavior of as-prepared MoS{sub 2} nanoflake electrode was also investigated. It was found that the MoS{sub 2} nanoflake electrode exhibited higher specific capacity, with very high cycling stability, compared to MoS{sub 2} nanoparticle electrode. The possible reasons for the high electrochemical performance of the nanoflakes electrodes are also discussed. The outstanding electrochemical properties of MoS{sub 2} nanoflakes obtained by this method make it possible for MoS{sub 2} to be used as a promising anode material.

  20. Mechanically Activated Combustion Synthesis of MoSi2-Based Composites

    SciTech Connect (OSTI)

    Shafirovich, Evgeny

    2015-09-30

    The thermal efficiency of gas-turbine power plants could be dramatically increased by the development of new structural materials based on molybdenum silicides and borosilicides, which can operate at temperatures higher than 1300 °C with no need for cooling. A major challenge, however, is to simultaneously achieve high oxidation resistance and acceptable mechanical properties at high temperatures. One approach is based on the fabrication of MoSi2-Mo5Si3 composites that combine high oxidation resistance of MoSi2 and good mechanical properties of Mo5Si3. Another approach involves the addition of boron to Mo-rich silicides for improving their oxidation resistance through the formation of a borosilicate surface layer. In particular, materials based on Mo5SiB2 phase are promising materials that offer favorable combinations of high temperature mechanical properties and oxidation resistance. However, the synthesis of Mo-Si-B multi-phase alloys is difficult because of their extremely high melting temperatures. Mechanical alloying has been considered as a promising method, but it requires long milling times, leading to large energy consumption and contamination of the product by grinding media. In the reported work, MoSi2-Mo5Si3 composites and several materials based on Mo5SiB2 phase have been obtained by mechanically activated self-propagating high-temperature synthesis (MASHS). Short-term milling of Mo/Si mixture in a planetary mill has enabled a self-sustained propagation of the combustion front over the mixture pellet, leading to the formation of MoSi2-T1 composites. Combustion of Mo/Si/B mixtures for the formation of T2 phase becomes possible if the composition is designed for the addition of more exothermic reactions leading to the formation of MoB, TiC, or TiB2. Upon ignition, Mo/Si/B and Mo/Si/B/Ti mixtures exhibited spin combustion, but the products were porous, contained undesired secondary phases, and had low oxidation resistance. It has been shown that use of SHS compaction (quasi-isostatic pressing after combustion) significantly improves oxidation resistance of the obtained MoSi2-Mo5Si3 composites. The “chemical oven” technique has been successfully employed to fabricate low-porous Mo5SiB2–TiC, Mo5SiB2–TiB2, and Mo–Mo5SiB2–Mo3Si materials. Among them, Mo5SiB2–TiB2 material possesses good mechanical properties and simultaneously exhibits excellent oxidation resistance at temperatures up to 1500 °C.

  1. Recovery of Mo/Si multilayer coated optical substrates

    DOE Patents [OSTI]

    Baker, S.L.; Vernon, S.P.; Stearns, D.G.

    1997-12-16

    Mo/Si multilayers are removed from superpolished ZERODUR and fused silica substrates with a dry etching process that, under suitable processing conditions, produces negligible change in either the substrate surface figure or surface roughness. The two step dry etching process removes SiO{sub 2} overlayer with a fluroine-containing gas and then moves molybdenum and silicon multilayers with a chlorine-containing gas. Full recovery of the initial normal incidence extreme ultra-violet (EUV) reflectance response has been demonstrated on reprocessed substrates. 5 figs.

  2. Recovery of Mo/Si multilayer coated optical substrates

    DOE Patents [OSTI]

    Baker, Sherry L.; Vernon, Stephen P.; Stearns, Daniel G.

    1997-12-16

    Mo/Si multilayers are removed from superpolished ZERODUR and fused silica substrates with a dry etching process that, under suitable processing conditions, produces negligible change in either the substrate surface figure or surface roughness. The two step dry etching process removes SiO.sub.2 overlayer with a fluroine-containing gas and then moves molybdenum and silicon multilayers with a chlorine-containing gas. Full recovery of the initial normal incidence extreme ultra-violet (EUV) reflectance response has been demonstrated on reprocessed substrates.

  3. Microsoft Word - chapter FeCrMo_ver2.doc

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Reference on Hydrogen Compatibility of Materials Low-Alloy Ferritic Steels: Tempered Fe-Cr-Mo Alloys (code 1211) Prepared by: B.P. Somerday, Sandia National Laboratories Editors C. San Marchi B.P. Somerday Sandia National Laboratories This report may be updated and revised periodically in response to the needs of the technical community; up-to-date versions can be requested from the editors at the address given below or downloaded at http://www.ca.sandia.gov/matlsTechRef/ . The success of this

  4. Greenfield Alternative Study LEU-Mo Fuel Fabrication Facility

    SciTech Connect (OSTI)

    Washington Division of URS

    2008-07-01

    This report provides the initial “first look” of the design of the Greenfield Alternative of the Fuel Fabrication Capability (FFC); a facility to be built at a Greenfield DOE National Laboratory site. The FFC is designed to fabricate LEU-Mo monolithic fuel for the 5 US High Performance Research Reactors (HPRRs). This report provides a pre-conceptual design of the site, facility, process and equipment systems of the FFC; along with a preliminary hazards evaluation, risk assessment as well as the ROM cost and schedule estimate.

  5. Characterization of modified 9 Cr-1 Mo steel extruded pipe

    SciTech Connect (OSTI)

    Sikka, V.K.; Hart, M.D.

    1985-04-01

    The fabrication of hot-extruded pipe of modified 9 Cr-1 Mo steel at Cameron Iron Works is described. The report also deals with the tempering response; tensile, Charpy impact, and creep properties; and microstructure of the hot-extruded pipe. The tensile properties of the pipe are compared with the average and average -1.65 standard error of estimate curves for various product forms of several commercial heats of this alloy. The creep-rupture properties are compared with the average curve for various product forms of the commercial heats.

  6. d::;":,",:::,, ST. LOUIS.7. MO,

    Office of Legacy Management (LM)

    i ,' ~CKRODT CHEMICAL d::;":,",:::,, ST. LOUIS.7. MO, PiARCH 14, ,jq;ll MR. H. L. PRICE, GIRECTOR ,.' , . . DIVISION OF LICENSING AND F~EG~~LATION ,... L.' S. ATOMIC ' ENERGY COMMISSION :' ;._ hASHINGT0N 25, D. c. T> "-VW-; PEAR P;R. FRICE: PURSUANT To THE PROVISIONS OF 10 CF? FART 20, PARAGRAPH 2O-.lO3, (4 (31, THE NUCLEAR DIVISI:IN, COMMERC I AL ~PERAT I ONS DF MALL- INCKRODT ' CHEMICAL b:ORKS WOULD LIKE TO MAKE.APPLlCATlON FOR A MODIFICATION TO LICENSE NO. SNPI 33 TO INCLUDE

  7. DOE/NNSA - MoD Certification Form

    Office of Environmental Management (EM)

    14 (01/2014) UNITED STATES DEPARTMENT OF ENERGY NATIONAL NUCLEAR SECURITY ADMINISTRATION UNITED KINGDOM MINISTRY OF DEFENCE DOE or MoD CERTIFICATION * Select as applicable SECTION I - DOE/NNSA MARK QUALITY MATERIAL This material has been accepted by the DOE/NNSA or inspected and accepted by DOE/NNSA contractor(s) authorized to acquire such material and is of like quality to that used in DOE/NNSA weapons or in support thereof. (Note: Application of UK Stamp is by DOE/NNSA only) Signature: Date:

  8. Time-Resolved XAFS Spectroscopic Studies of B-H and N-H Oxidative Addition to Transition Metal Catalysts Relevant to Hydrogen Storage

    SciTech Connect (OSTI)

    Bitterwolf, Thomas E.

    2014-12-09

    Successful catalytic dehydrogenation of aminoborane, H3NBH3, prompted questions as to the potential role of N-H oxidative addition in the mechanisms of these processes. N-H oxidative addition reactions are rare, and in all cases appear to involve initial dative bonding to the metal by the amine lone pairs followed by transfer of a proton to the basic metal. Aminoborane and its trimethylborane derivative block this mechanism and, in principle, should permit authentic N-H oxidative attrition to occur. Extensive experimental work failed to confirm this hypothesis. In all cases either B-H complexation or oxidative addition of solvent C-H bonds dominate the chemistry.

  9. A Pyrrolyl-based Triazolophane: A Macrocyclic Receptor With CH and NH Donor Groups That Exhibits a Preference for Pyrophosphate Anions

    SciTech Connect (OSTI)

    Sessler, Jonathan L.; Cia, Jiajia; Gong, Han-Yuan; Yang, Xiauping; Arambula, Jonathan F.; Hay, Benjamin

    2010-01-01

    A pyrrolyl-based triazolophane, incorporating CH and NH donor groups, acts as a receptor for the pyrophosphate anion in chloroform solution. It shows selectivity for this trianion, followed by HSO{sub 4}{sup -} > H{sub 2}PO{sub 4}{sup -} > Cl{sup -} > Br{sup -} (all as the corresponding tetrabutylammonium salts), with NH-anion interactions being more important than CH-anion interactions. In the solid state, the receptor binds the pyrophosphate anion in a clip-like slot via NH and CH hydrogen bonds.

  10. MiniBooNE Charged Current Neutral Pion Cross Section Data Release

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Muon Neutrino Induced Charged Current Neutral Pion Cross Sections on Mineral Oil at Enu=0.5-2.0 GeV" , arXiv:1010.3264 [hep-ex] The following MiniBooNE information for the 2010 CC π0 cross section paper is made available to the public. Each of the following tables contains: The bin boundaries and units. The central-value measurement or prediction with its units and multiplicative factor. The statistical uncertainty per bin of each measurement with its units and multiplicative factor. The

  11. Microsoft Word - MicroBooNE CD-3b appr.docx

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    3b Approve Start of Full Construction of the Micro Booster Neutrino Project at the Fermi National Accelerator Laboratory Office of High Energy Physics Office of Science A. Purpose The purpose of this document is to record the review and approval by the Office of Science Energy Systems Acquisition Advisory Board-equivalent for Critical Decision (CD) 3b "Approve Start of Full Construction" for the Micro Booster Neutrino (MicroBooNE) Project at the Fermi National Accelerator Laboratory

  12. MiniBooNE H. A. Tanaka Princeton University Neutrino Factory 2004 Osaka, Japan

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    H. A. Tanaka Princeton University Neutrino Factory 2004 Osaka, Japan The MiniBooNE Collaboration University of Alabama: Y.Liu, I.Stancu Bucknell University: S.Koutsoliotas University of Cincinnati: E.Hawker, R.A.Johnson, J.L.Raaf University of Colorado: T.Hart, R.H.Nelson, M.Wilking, E.D.Zimmerman Columbia University: A.A.Aguilar-Arevalo, L.Bugel, J.M.Conrad, J.Link, J.Monroe, D.Schmitz, M.H.Shaevitz, M.Sorel, G.P.Zeller Embry Riddle Aeronautical University: D.Smith Fermi National Accelerator

  13. DOE-NE Proliferation and Terrorism Risk Assessment: FY12 Plans Update

    SciTech Connect (OSTI)

    Sadasivan, Pratap

    2012-06-21

    This presentation provides background information on FY12 plans for the DOE Office of Nuclear Energy Proliferation and Terrorism Risk Assessment program. Program plans, organization, and individual project elements are described. Research objectives are: (1) Develop technologies and other solutions that can improve the reliability, sustain the safety, and extend the life of current reactors; (2) Develop improvements in the affordability of new reactors to enable nuclear energy; (3) Develop Sustainable Nuclear Fuel Cycles; and (4) Understand and minimize the risks of nuclear proliferation and terrorism - Goal is to enable the use of risk information to inform NE R&D program planning.

  14. HIA 2015 DOE Zero Energy Ready Home Case Study: Charles Thomas Homes, Anna Model, Omaha, NE

    Energy Savers [EERE]

    Thomas Homes Anna Model Omaha, NE DOE ZERO ENERGY READY HOME(tm) The U.S. Department of Energy invites home builders across the country to meet the extraordinary levels of excellence and quality specified in DOE's Zero Energy Ready Home program (formerly known as Challenge Home). Every DOE Zero Energy Ready Home starts with ENERGY STAR Certified Homes Version 3.0 for an energy-efficient home built on a solid foundation of building science research. Advanced technologies are designed in to give

  15. DOE-NE-STD-1004-92; Root Cause Analysis Guidance Document

    Office of Environmental Management (EM)

    NE-STD-1004-92 DOE GUIDELINE ROOT CAUSE ANALYSIS GUIDANCE DOCUMENT February 1992 U.S. Department of Energy Office of Nuclear Energy Office of Nuclear Safety Policy and Standards Washington, D.C. 20585 ii ABSTRACT DOE Order 5000.3A, "Occurrence Reporting and Processing of Operations Information," investigation and reporting of occurrences (including the performance of root cause analysis) requires the and the selection, implementation, and follow-up of corrective actions. The level of

  16. Characterization of U-Mo Foils for AFIP-7

    SciTech Connect (OSTI)

    Edwards, Danny J.; Ermi, Ruby M.; Schemer-Kohrn, Alan L.; Overman, Nicole R.; Henager, Charles H.; Burkes, Douglas; Senor, David J.

    2012-11-07

    Twelve AFIP in-process foil samples, fabricated by either Y-12 or LANL, were shipped from LANL to PNNL for potential characterization using optical and scanning electron microscopy techniques. Of these twelve, nine different conditions were examined to one degree or another using both techniques. For this report a complete description of the results are provided for one archive foil from each source of material, and one unirradiated piece of a foil of each source that was irradiated in the Advanced Test Reactor. Additional data from two other LANL conditions are summarized in very brief form in an appendix. The characterization revealed that all four characterized conditions contained a cold worked microstructure to different degrees. The Y-12 foils exhibited a higher degree of cold working compared to the LANL foils, as evidenced by the highly elongated and obscure U-Mo grain structure present in each foil. The longitudinal orientations for both of the Y-12 foils possesses a highly laminar appearance with such a distorted grain structure that it was very difficult to even offer a range of grain sizes. The U-Mo grain structure of the LANL foils, by comparison, consisted of a more easily discernible grain structure with a mix of equiaxed and elongated grains. Both materials have an inhomogenous grain structure in that all of the characterized foils possess abnormally coarse grains.

  17. New Generation of MoSx Based Solid Lubricant Coatings: Recent Developments and Applications

    SciTech Connect (OSTI)

    Haider, Julfikar; Hashmi, M. S. J.

    2011-01-17

    In recent times, there is a growing interest in applying Molybdenum disulphide (MoS{sub x}) solid lubricant coatings on components to improve the tribological performance (i.e. lower friction coefficient and wear rate). The tribological performance of MoS{sub x} coating is strongly dependent on coating properties and tribological environment. MoS{sub x} coatings are highly successful in certain applications such as in space/vacuum technology, but its effectiveness is questioned in other terrestrial applications such as in cutting tool industry due to its lower hardness and poor oxidation resistance leading to shorter life. In order to circumvent this drawback, the paper identifies that current research is being concentrated on developing MoS{sub x} based coatings using three different approaches: (1) Metal or compound addition in MoS{sub x} coating (2)MoS{sub x} layer on hard coating and (3)MoS{sub x} addition in hard coating matrix. Although the primary objective is same in all three cases, the third approach is considered to be more effective in improving the tribological properties of the coating. Finally, the potential applications of MoS{sub x} based coatings in different industrial sectors have been briefly outlined.

  18. Photoionization-pumped, Ne II, x-ray laser studies project. Final report

    SciTech Connect (OSTI)

    Richardson, M.C.; Hagelstein, P.L.; Eckart, M.J.; Forsyth, J.M.; Gerrassimenko, M.; Soures, J.M.

    1984-01-01

    The energetics of this pumping scheme are shown. Short-pulse (50 to 100 ps) laser irradiation of an appropriate x-ray flashlamp medium generates broad-band emission in the range of 300 to 800 eV which preferentially photoionizes Ne to the /sup 2/S state of Ne II creating an inversion at approximately 27 eV. Although this approach does not depend on precise spectral overlap between the x-ray pump radiation and the medium to be pumped, it does require that the x-ray medium remain un-ionized prior to photoionization by the soft x-ray emission. Well-controlled focus conditions are required to ensure that the x-ray medium is not subjected to electron or x-ray preheat prior to irradiation by the soft x-ray source. The magnitude of the population inversion is predicted to be critically dependent upon rapid photoionization of the two states; therefore, ultra-short pulse irradiation of the laser flashlamps is required.

  19. OZONE PRODUCTION IN THE PHILADELPHIA URBAN AREA DURING NE-OPS 99.

    SciTech Connect (OSTI)

    KLEINMAN,L.I.; DAUM,P.H.; BRECHTEL,F.; LEE,Y.N.; NUNNERMACKER,L.J.; SPRINGSTON,S.R.; WEINSTEIN-LLOYD,J.

    2001-10-01

    As part of the 1999 NARSTO Northeast Oxidant and Particulate Study (NE-OPS) field campaign, the DOE G-1 aircraft sampled trace gases and aerosols in and around the Philadelphia metropolitan area. Twenty research flights were conducted between July 25 and August 11. The overall goals of these flights were to obtain a mechanistic understanding of O{sub 3} production; to characterize the spatial and temporal behavior of photo-oxidants and aerosols; and to study the evolution of aerosol size distributions, including the process of new particle formation. Within the NE-OPS program, other groups provided additional trace gas, aerosol, and meteorological observations using aircraft, balloon, remote sensing, and surface based instruments (Phillbrick et al., 2000). In this article we provide an overview of the G-1 observations related to O{sub 3} production, focusing on the vertical distribution of pollutants. Ozone production rates are calculated using a box model that is constrained by observed trace gas concentrations. Highest O{sub 3} concentrations were observed on July 31, which we present as a case study. On that day, O{sub 3} concentrations above the 1-hour 120 ppb standard were observed downwind of Philadelphia and also in the plume of a single industrial facility located on the Delaware River south of the city.

  20. Wave packet and statistical quantum calculations for the He + NeH{sup +} → HeH{sup +} + Ne reaction on the ground electronic state

    SciTech Connect (OSTI)

    Koner, Debasish; Panda, Aditya N.; Barrios, Lizandra; González-Lezana, Tomás

    2014-09-21

    A real wave packet based time-dependent method and a statistical quantum method have been used to study the He + NeH{sup +} (v, j) reaction with the reactant in various ro-vibrational states, on a recently calculated ab initio ground state potential energy surface. Both the wave packet and statistical quantum calculations were carried out within the centrifugal sudden approximation as well as using the exact Hamiltonian. Quantum reaction probabilities exhibit dense oscillatory pattern for smaller total angular momentum values, which is a signature of resonances in a complex forming mechanism for the title reaction. Significant differences, found between exact and approximate quantum reaction cross sections, highlight the importance of inclusion of Coriolis coupling in the calculations. Statistical results are in fairly good agreement with the exact quantum results, for ground ro-vibrational states of the reactant. Vibrational excitation greatly enhances the reaction cross sections, whereas rotational excitation has relatively small effect on the reaction. The nature of the reaction cross section curves is dependent on the initial vibrational state of the reactant and is typical of a late barrier type potential energy profile.

  1. Photo-oxidation method using MoS2 nanocluster materials

    DOE Patents [OSTI]

    Wilcoxon, Jess P. (Albuquerque, NM)

    2001-01-01

    A method of photo-oxidizing a hydrocarbon compound is provided by dispersing MoS.sub.2 nanoclusters in a solvent containing a hydrocarbon compound contaminant to form a stable solution mixture and irradiating the mixture to photo-oxide the hydrocarbon compound. Hydrocarbon compounds of interest include aromatic hydrocarbon and chlorinated hydrocarbons. MoS.sub.2 nanoclusters with an average diameter less than approximately 10 nanometers are shown to be effective in decomposing potentially toxic aromatic and chlorinated hydrocarbons, such as phenol, pentachlorophenol, chlorinated biphenols, and chloroform, into relatively non-toxic compounds. The irradiation can occur by exposing the MoS.sub.2 nanoclusters and hydrocarbon compound mixture with visible light. The MoS.sub.2 nanoclusters can be introduced to the toxic hydrocarbons as either a MoS.sub.2 solution or deposited on a support material.

  2. Synthesis and characterization of model MgO supported catalyst with Pt-Mo interactions.

    SciTech Connect (OSTI)

    Alexeev, O.; Kawi, S.; Gates, B.C. [Univ. of California, Davis, CA (United States)] [Univ. of California, Davis, CA (United States); Shelef, M. [Ford Motor Co., Dearborn, MI (United States)] [Ford Motor Co., Dearborn, MI (United States)

    1996-01-04

    MgO supported platinum and platinum-molybdenum catalysts were prepared from organometallic precursors and charaterized structurally to determine how the nature of the bimetallic precursors and the treatment conditions affected the interaction between the two metals. Samples were prepared from [PtCl{sub 2}(PhCN){sub 2}], [PtCl{sub 2}(PhCN){sub 2}] + [Mo(CO){sub 6}], and [C@Pt[Mo(CO){sub 3}(C{sub 5}H{sub 5})]{sub 2}(PhCN){sub 2}] BC@ characterized by infrared and extended X-ray absorption fine structure (EXAFS) spectroscopies, tranmission electron microscopy, and chemisorption of H{sub 2}, CO, and O{sub 2}. The samples were treated in H{sub 2} at 400{degree}C prior to most of the characterizatons. Incorporation of Mo reduced the chemisorption of CO and of H{sub 2}. EXAFS spectra measured at the Pt L{sub III} edge and at the Mo K edge showed substantial Pt-Mo contributions with a Pt-Mo cordination number of about 2 and an average distance of 2.63 A for the sample prepared from [C@Pt[Mo(CO){sub 3}(C{sub 5}H{sub 5})]{sub 2}(PhCN){sub 2}] BC@. In constract, no significant Pt-Mo contribution was observed for the sample prepared from [PtCl{sub 2}(PhCN){sub 2}]+ [Mo(CO){sub 6}]. Electron micrographs and EXAFS results show that interaction between Pt and Mo ions in the former sample helped to maintain the platinum in a highly dispersed form, with supported platinum clusters being smaller than about 10 A. 53 refs., 9 figs., 9 tabs.

  3. QSO ABSORPTION SYSTEMS DETECTED IN Ne VIII: HIGH-METALLICITY CLOUDS WITH A LARGE EFFECTIVE CROSS SECTION

    SciTech Connect (OSTI)

    Meiring, J. D.; Tripp, T. M. [Department of Astronomy, University of Massachusetts, Amherst, MA 01003 (United States)] [Department of Astronomy, University of Massachusetts, Amherst, MA 01003 (United States); Werk, J. K.; Prochaska, J. X. [University of California Observatories-Lick Observatory, UC Santa Cruz, CA 95064 (United States)] [University of California Observatories-Lick Observatory, UC Santa Cruz, CA 95064 (United States); Howk, J. C. [Department of Physics, University of Notre Dame, 225 Nieuwland Science Hall, Notre Dame, IN 46556 (United States)] [Department of Physics, University of Notre Dame, 225 Nieuwland Science Hall, Notre Dame, IN 46556 (United States); Jenkins, E. B. [Princeton University Observatory, Peyton Hall, Ivy Lane, Princeton, NJ 08544 (United States)] [Princeton University Observatory, Peyton Hall, Ivy Lane, Princeton, NJ 08544 (United States); Lehner, N.; Sembach, K. R. [Space Telescope Science Institute, 3700 San Martin Drive, Baltimore, MD 21218 (United States)] [Space Telescope Science Institute, 3700 San Martin Drive, Baltimore, MD 21218 (United States)

    2013-04-10

    Using high-resolution, high signal-to-noise ultraviolet spectra of the z{sub em} = 0.9754 quasar PG1148+549 obtained with the Cosmic Origins Spectrograph (COS) on the Hubble Space Telescope, we study the physical conditions and abundances of Ne VIII+O VI absorption line systems at z{sub abs} = 0.68381, 0.70152, 0.72478. In addition to Ne VIII and O VI, absorption lines from multiple ionization stages of oxygen (O II, O III, O IV) are detected and are well aligned with the more highly ionized species. We show that these absorbers are multiphase systems including hot gas (T Almost-Equal-To 10{sup 5.7} K) that produces Ne VIII and O VI, and the gas metallicity of the cool phase ranges from Z = 0.3 Z{sub Sun} to supersolar. The cool ( Almost-Equal-To 10{sup 4} K) phases have densities n{sub H} Almost-Equal-To 10{sup -4} cm{sup -3} and small sizes (<4 kpc); these cool clouds are likely to expand and dissipate, and the Ne VIII may be within a transition layer between the cool gas and a surrounding, much hotter medium. The Ne VIII redshift density, dN/dz{approx}7{sup +7}{sub -3}, requires a large number of these clouds for every L > 0.1 L* galaxy and a large effective absorption cross section ({approx}> 100 kpc), and indeed, we find a star-forming {approx}L {sup *} galaxy at the redshift of the z{sub abs} = 0.72478 system, at an impact parameter of 217 kpc. Multiphase absorbers like these Ne VIII systems are likely to be an important reservoir of baryons and metals in the circumgalactic media of galaxies.

  4. Observational results of a multi-telescope campaign in search of interstellar urea [(NH{sub 2}){sub 2}CO

    SciTech Connect (OSTI)

    Remijan, Anthony J.; Snyder, Lewis E.; Kuo, Hsin-Lun; Looney, Leslie W.; Friedel, Douglas N.; McGuire, Brett A.; Golubiatnikov, G. Yu; Lovas, Frank J.; Ilyushin, V. V.; Alekseev, E. A.; Dyubko, S. F.; McCall, Benjamin J.; Hollis, Jan M.

    2014-03-10

    In this paper, we present the results of an observational search for gas phase urea [(NH{sub 2}){sub 2}CO] observed toward the Sgr B2(N-LMH) region. We show data covering urea transitions from ?100 GHz to 250 GHz from five different observational facilities: the Berkeley-Illinois-Maryland-Association (BIMA) Array, the Combined Array for Research in Millimeter-wave Astronomy (CARMA), the NRAO 12 m telescope, the IRAM 30 m telescope, and the Swedish-ESO Submillimeter Telescope (SEST). The results show that the features ascribed to urea can be reproduced across the entire observed bandwidth and all facilities by best-fit column density, temperature, and source size parameters which vary by less than a factor of two between observations merely by adjusting for telescope-specific parameters. Interferometric observations show that the emission arising from these transitions is cospatial and compact, consistent with the derived source sizes and emission from a single species. Despite this evidence, the spectral complexity of both (NH{sub 2}){sub 2}CO and of Sgr B2(N) makes the definitive identification of this molecule challenging. We present observational spectra, laboratory data, and models, and discuss our results in the context of a possible molecular detection of urea.

  5. Surface Structures of Cubo-octahedral Pt-Mo Catalyst Nanoparticles from Monte Carlo Simulations

    SciTech Connect (OSTI)

    Wang, Guofeng; Van Hove, M.A.; Ross, P.N.; Baskes, M.I.

    2005-03-31

    The surface structures of cubo-octahedral Pt-Mo nanoparticles have been investigated using the Monte Carlo method and modified embedded atom method potentials that we developed for Pt-Mo alloys. The cubo-octahedral Pt-Mo nanoparticles are constructed with disordered fcc configurations, with sizes from 2.5 to 5.0 nm, and with Pt concentrations from 60 to 90 at. percent. The equilibrium Pt-Mo nanoparticle configurations were generated through Monte Carlo simulations allowing both atomic displacements and element exchanges at 600 K. We predict that the Pt atoms weakly segregate to the surfaces of such nanoparticles. The Pt concentrations in the surface are calculated to be 5 to 14 at. percent higher than the Pt concentrations of the nanoparticles. Moreover, the Pt atoms preferentially segregate to the facet sites of the surface, while the Pt and Mo atoms tend to alternate along the edges and vertices of these nanoparticles. We found that decreasing the size or increasing the Pt concentration leads to higher Pt concentrations but fewer Pt-Mo pairs in the Pt-Mo nanoparticle surfaces.

  6. MiniBooNE NC 1π0 Cross Section Data Release

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    νμ and ν̅μ induced neutral current single π0 production cross sections on mineral oil at Eν~O(1 GeV)", arXiv:0911.2063 [hep-ex], Phys. Rev. D81, 013005 (2010) The following MiniBooNE information from the 2009 NC 1π0 cross section paper is made available to the public: Neutrino Mode Running νμ NC 1π0 pπ0 Differential Cross Section 1D array of bin boundaries partitioning the momentum of the π0 1D array of the value of the differential cross section in each bin in units of 10-40

  7. Test of ''Crab-Waist'' Collisions at the DA{Phi}NE {Phi} Factory

    SciTech Connect (OSTI)

    Zobov, M.; Alesini, D.; Biagini, M. E.; Biscari, C.; Bocci, A.; Boni, R.; Boscolo, M.; Bossi, F.; Buonomo, B.; Clozza, A.; Delle Monache, G. O.; Demma, T.; Di Pasquale, E.; Di Pirro, G.; Drago, A.; Gallo, A.; Ghigo, A.; Guiducci, S.; Ligi, C.; Marcellini, F.

    2010-04-30

    The electron-positron collider DA{Phi}NE, the Italian {Phi} factory, has been recently upgraded in order to implement an innovative collision scheme based on large crossing angle, small beam sizes at the crossing point, and compensation of beam-beam interaction by means of sextupole pairs creating a ''crab-waist'' configuration in the interaction region. Experimental tests of the novel scheme exhibited an increase by a factor of 3 in the peak luminosity of the collider with respect to the performances reached before the upgrade. In this Letter we present the new collision scheme, discuss its advantages, describe the hardware modifications realized for the upgrade, and report the results of the experimental tests carried out during commissioning of the machine in the new configuration and standard operation for the users.

  8. Distributed Production of Radionuclide Mo-99 Charles A. Gentile, Adam B.

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Cohen and George Ascione | Princeton Plasma Physics Lab Distributed Production of Radionuclide Mo-99 Charles A. Gentile, Adam B. Cohen and George Ascione This invention is for the production of Technetium-99m (Tc-99m), a widely used medical isotope in a distributed and in-situ fashion. Tc-99m results when Molybdenum 99 (Mo-99) decays. Mo-99 is typically produced in a nuclear reactor, but it can be produced from naturally occurring Molybdenum 100 or from Molybdenum 98 using either neutrons or

  9. Unusual defect physics in CH{sub 3}NH{sub 3}PbI{sub 3} perovskite solar cell absorber

    SciTech Connect (OSTI)

    Yin, Wan-Jian Shi, Tingting; Yan, Yanfa

    2014-02-10

    Thin-film solar cells based on Methylammonium triiodideplumbate (CH{sub 3}NH{sub 3}PbI{sub 3}) halide perovskites have recently shown remarkable performance. First-principle calculations show that CH{sub 3}NH{sub 3}PbI{sub 3} has unusual defect physics: (i) Different from common p-type thin-film solar cell absorbers, it exhibits flexible conductivity from good p-type, intrinsic to good n-type depending on the growth conditions; (ii) Dominant intrinsic defects create only shallow levels, which partially explain the long electron-hole diffusion length and high open-circuit voltage in solar cell. The unusual defect properties can be attributed to the strong Pb lone-pair s orbital and I p orbital antibonding coupling and the high ionicity of CH{sub 3}NH{sub 3}PbI{sub 3}.

  10. Monolayers of MoS{sub 2} as an oxidation protective nanocoating material

    SciTech Connect (OSTI)

    Sen, H. Sener; Sahin, H.; Peeters, F. M.; Durgun, E.

    2014-08-28

    First-principle calculations are employed to investigate the interaction of oxygen with ideal and defective MoS{sub 2} monolayers. Our calculations show that while oxygen atoms are strongly bound on top of sulfur atoms, the oxygen molecule only weakly interacts with the surface. The penetration of oxygen atoms and molecules through a defect-free MoS{sub 2} monolayer is prevented by a very high diffusion barrier indicating that MoS{sub 2} can serve as a protective layer for oxidation. The analysis is extended to WS{sub 2} and similar coating characteristics are obtained. Our calculations indicate that ideal and continuous MoS{sub 2} and WS{sub 2} monolayers can improve the oxidation and corrosion-resistance of the covered surface and can be considered as an efficient nanocoating material.

  11. Microscopic origin of low frequency noise in MoS{sub 2} field-effect transistors

    SciTech Connect (OSTI)

    Ghatak, Subhamoy; Jain, Manish; Ghosh, Arindam; Mukherjee, Sumanta; Sarma, D. D.

    2014-09-01

    We report measurement of low frequency 1/f noise in molybdenum di-sulphide (MoS{sub 2}) field-effect transistors in multiple device configurations including MoS{sub 2} on silicon dioxide as well as MoS{sub 2}-hexagonal boron nitride (hBN) heterostructures. All as-fabricated devices show similar magnitude of noise with number fluctuation as the dominant mechanism at high temperatures and density, although the calculated density of traps is two orders of magnitude higher than that at the SiO{sub 2} interface. Measurements on the heterostructure devices with vacuum annealing and dual gated configuration reveals that along with the channel, metal-MoS{sub 2} contacts also play a significant role in determining noise magnitude in these devices.

  12. File:USDA-CE-Production-GIFmaps-MO.pdf | Open Energy Information

    Open Energy Info (EERE)

    MO.pdf Jump to: navigation, search File File history File usage Missouri Ethanol Plant Locations Size of this preview: 776 600 pixels. Full resolution (1,650 1,275 pixels,...

  13. Substrate interactions with suspended and supported monolayer MoS2: Angle-resolved photoemission spectroscopy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Jin, Wencan; Yeh, Po -Chun; Zaki, Nader; Zhang, Datong; Liou, Jonathan T.; Dadap, Jerry I.; Barinov, Alexey; Yablonskikh, Mikhail; Sadowski, Jerzy T.; Sutter, Peter; et al

    2015-03-17

    We report the directly measured electronic structure of exfoliated monolayer molybdenum disulfide (MoS₂) using micrometer-scale angle-resolved photoemission spectroscopy. Measurements of both suspended and supported monolayer MoS₂ elucidate the effects of interaction with a substrate. Thus, a suggested relaxation of the in-plane lattice constant is found for both suspended and supported monolayer MoS₂ crystals. For suspended MoS₂, a careful investigation of the measured uppermost valence band gives an effective mass at Γ¯ and Κ¯ of 2.00m₀ and 0.43m₀, respectively. We also measure an increase in the band linewidth from the midpoint of Γ¯Κ¯ to the vicinity of Κ¯ and briefly discussmore » its possible origin.« less

  14. DE-EM-0001971 WIPP M&O J-8 PART III - LIST OF DOCUMENTS, EXHIBITS...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    8 PART III - LIST OF DOCUMENTS, EXHIBITS AND OTHER ATTACHMENTS SECTION J ATTACHMENT C: DRAFT PERFORMANCE EVALUATION AND MEASUREMENT PLAN (PEMP) DE-EM-0001971 WIPP M&O J-9 Draft...

  15. Electrochemical Testing of Ni-Cr-Mo-Gd Alloys

    SciTech Connect (OSTI)

    T. E. Lister; R. E. Mizia; H. Tian

    2005-10-01

    The waste package site recommendation design specified a boron-containing stainless steel, Neutronit 976/978, for fabrication of the internal baskets that will be used as a corrosion-resistant neutron-absorbing material. Recent corrosion test results gave higher-than-expected corrosion rates for this material. The material callout for these components has been changed to a Ni-Cr-Mo-Gd alloy (ASTM-B 932-04, UNS N06464) that is being developed at the Idaho National Laboratory. This report discusses the results of initial corrosion testing of this material in simulated in-package environments that could contact the fuel baskets after breach of the waste package outer barrier. The corrosion test matrix was executed using the potentiodynamic and potentiostatic electrochemical test techniques. The alloy performance shows low rates of general corrosion after initial removal of a gadolinium-rich second phase that intersects the surface. The high halide-containing test solutions exhibited greater tendencies toward initiation of crevice corrosion.

  16. Thermo-physical Properties of DU-10 wt.% Mo Alloys

    SciTech Connect (OSTI)

    Douglas E. Burkes; Cynthia A. Papesch; Andrew P. Maddison; Thomas Hartmann; Francine J. Rice

    2010-08-01

    Low-enriched uranium alloyed with 10 wt% molybdenum is under consideration by the Global Threat Reduction Initiative reactor convert program as a very high density fuel to enable the conversion of high-performance research reactors away from highly-enriched uranium fuels. As with any fuel development program, the thermophysical properties of the fuel as a function of temperature are extremely important and must be well characterized in order to effectively model and predict fuel behavior under normal and off-normal irradiation conditions. For the alloy system under investigation, there is a lack of thermophysical property data, and in most cases, the data is relatively inconsistent and lacks sufficient explanation. Available literature on this alloy system comes mainly from studies done during the 1960s and 1970s, and often does not include sufficient information on fabrication history or conditions to draw conclusions for the current application. The current paper has investigated specific heat capacity, coefficient of linear thermal expansion, density, and thermal diffusivity that were then used to calculate alloy thermal conductivity as a function of temperature. The data obtained from this investigation was compared to available literature on similar U-Mo alloys, and in most cases are in good agreement.

  17. Rotationally Commensurate Growth of MoS[subscript 2] on Epitaxial Graphene

    Office of Scientific and Technical Information (OSTI)

    (Journal Article) | SciTech Connect SciTech Connect Search Results Journal Article: Rotationally Commensurate Growth of MoS[subscript 2] on Epitaxial Graphene Citation Details In-Document Search Title: Rotationally Commensurate Growth of MoS[subscript 2] on Epitaxial Graphene Authors: Liu, Xiaolong ; Balla, Itamar ; Bergeron, Hadallia ; Campbell, Gavin P. ; Bedzyk, Michael J. ; Hersam, Mark C. [1] + Show Author Affiliations NWU Publication Date: 2016-03-04 OSTI Identifier: 1240188 Resource

  18. Demonstration of LED Street Lighting in Kansas City, MO (Technical Report)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    | SciTech Connect Demonstration of LED Street Lighting in Kansas City, MO Citation Details In-Document Search Title: Demonstration of LED Street Lighting in Kansas City, MO Nine different streetlighting products were installed on various streets in Kansas City, Missouri during February, 2011, to evaluate their performance relative to the incumbent high-pressure sodium (HPS) lighting. The applications investigated included 100 W, 150 W, 250 W, and 400 W HPS installations. Initial measurements

  19. DOE - Office of Legacy Management -- Weldon Spring Chemical Co - MO 03

    Office of Legacy Management (LM)

    Weldon Spring Chemical Co - MO 03 FUSRAP Considered Sites Site: Weldon Spring Chemical Co. (MO.03) Designated Name: Alternate Name: Location: Evaluation Year: Site Operations: Site Disposition: Radioactive Materials Handled: Primary Radioactive Materials Handled: Radiological Survey(s): Site Status: Also see Weldon Spring, Missouri, Site Documents Related to Weldon Spring Chemical Co. Summary of Work Session - Focus Area: Monitoring and Maintenance. Summary of Weldon Spring Long-Term Stewardship

  20. Solvent extraction of Li+, H3O+ and NH4+ into nitrobenzene by using sodium dicarbollylcobaltate and calix[4]arene-bis(t-octylbenzo-18-crown-6)

    SciTech Connect (OSTI)

    Makrlik, Emanuel; Selucky, P.; Vanura, Petr; Moyer, Bruce A

    2013-01-01

    From extraction experiments and c-activity measurements, the exchange extraction constants corresponding to the general equilibrium M+ (aq) + NaL+ (nb) , ML+ (nb) + Na+ (aq) taking place in the two-phase water nitrobenzene system (M+ = Li+, H3O+, NH+4; L = calix[4]arene-bis(t-octylbenzo-18-crown-6); aq = aqueous phase, nb = nitrobenzene phase) were evaluated. Furthermore, the stability constants of the ML+ complexes in nitrobenzene saturated with water were calculated; they were found to increase in the following cation order: zH3O+ < Li+ < NH+4.

  1. Microstructures and properties of CH{sub 3}NH{sub 3}PbI{sub 3?x}Cl{sub x} hybrid solar cells

    SciTech Connect (OSTI)

    Suzuki, Kohei E-mail: oku@mat.usp.ac.jp; Suzuki, Atsushi E-mail: oku@mat.usp.ac.jp; Zushi, Masahito E-mail: oku@mat.usp.ac.jp; Oku, Takeo E-mail: oku@mat.usp.ac.jp

    2015-02-27

    Halide-perovskite CH{sub 3}NH{sub 3}PbI{sub 3} was produced on mesoporous TiO{sub 2} layer by spin-coating a precursor solution of PbCl{sub 2} and CH{sub 3}NH{sub 3}I in dimethylformamide. The role of the annealing process and chlorine (Cl) doping for the perovskite-phase formation was investigated. It was found that crystallization of the perovskite materials was stimulated by the annealing process, and that longer annealing time is necessary for the Cl-doped perovskite compared with that of non-doped perovskite phase.

  2. High reflectance and low stress Mo2C/Be multilayers

    DOE Patents [OSTI]

    Bajt, Sasa (Livermore, CA); Barbee, Jr., Troy W. (Palo Alto, CA)

    2001-01-01

    A material for extreme ultraviolet (EUV) multilayers that will reflect at about 11.3 nm, have a high reflectance, low stress, and high thermal and radiation stability. The material consists of alternating layers of Mo.sub.2 C and Be deposited by DC magnetron sputtering on a substrate, such as silicon. In one example a Mo.sub.2 C/Be multilayer gave 65.2% reflectance at 11.25 nm measured at 5 degrees off normal incidence angle, and consisted of 70 bilayers with a deposition period of 5.78 nm, and was deposited at 0.83 mTorr argon (Ar) sputtering pressure, with the first and last layers being Be. The stress of the multilayer is tensile and only +88 MPa, compared to +330 MPa of a Mo/Be multilayers of the same thickness. The Mo.sub.2 C/Be multilayer was capped with carbon which produced an increase in reflectivity of about 7% over a similar multilayer with no carbon capping material, thus raising the reflectivity from 58.3% to over 65%. The multilayers were formed using either Mo.sub.2 C or Be as the first and last layers, and initial testing has shown the formation of beryllium carbide at the interfaces between the layers which both stabilizes and has a smoothing effect, and appear to be smoother than the interfaces in Mo/Be multilayers.

  3. Stability of precipitate phases in Fe-rich Fe-Cr-Ni-Mo alloys

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Yang, Ying; Tan, Lizhen; Busby, Jeremy T

    2015-01-01

    Understanding the stability of precipitate phases in the Fe-rich Fe-Cr-Ni-Mo alloys is critical to the alloy design and application of Mo-containing Austenitic steels. Coupled with thermodynamic modeling, stability of the and phases in two Fe-Cr-Ni-Mo alloys were investigated at 1000, 850 and 700 C for different annealing time. The morphologies, compositions and crystal structures of the matrix and precipitate phases were carefully examined by Scanning Electron Microscopy, Electron Probe Microanalysis, X-ray diffraction and Transmission Electron Microscopy. Two key findings resulted from this work. One is that the phase is stable at high temperature and transformed into the phase at lowmoretemperature. The other is that both the and phases have large solubilites of Cr, Mo and Ni, among which the Mo solubility has a major role on the relative stability of the precipitate phases. The developed thermodynamic models were then applied to evaluating the Mo effect on the stability of precipitate phases in AISI 316 and NF709 alloys.less

  4. Thermal stability of intermetallic phases in Fe-rich Fe-Cr-Ni-Mo alloys

    SciTech Connect (OSTI)

    Yang, Ying; Tan, Lizhen; Busby, Jeremy T.

    2015-06-12

    Understanding the stability of precipitate phases in the Fe-rich Fe-Cr-Ni-Mo alloys is critical to the alloy design and application of Mo-containing Austenitic steels. Coupled with thermodynamic modeling, stability of the chi and Laves phases in two Fe-Cr-Ni-Mo alloys were investigated at 1000, 850 and 700 °C for different annealing time. The morphologies, compositions and crystal structures of the matrix and precipitate phases were carefully examined by Scanning Electron Microscopy, Electron Probe Microanalysis, X-ray diffraction and Transmission Electron Microscopy. The two key findings resulted from this work. One is that the chi phase is stable at high temperature and transformed into the Laves phase at low temperature. The other is that both the chi and Laves phases have large solubilites of Cr, Mo and Ni, among which the Mo solubility has a major role on the relative stability of the precipitate phases. The developed thermodynamic models were then applied to evaluating the Mo effect on the stability of precipitate phases in AISI 316 and NF709 alloys.

  5. Thermal stability of intermetallic phases in Fe-rich Fe-Cr-Ni-Mo alloys

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Yang, Ying; Tan, Lizhen; Busby, Jeremy T.

    2015-06-12

    Understanding the stability of precipitate phases in the Fe-rich Fe-Cr-Ni-Mo alloys is critical to the alloy design and application of Mo-containing Austenitic steels. Coupled with thermodynamic modeling, stability of the chi and Laves phases in two Fe-Cr-Ni-Mo alloys were investigated at 1000, 850 and 700 °C for different annealing time. The morphologies, compositions and crystal structures of the matrix and precipitate phases were carefully examined by Scanning Electron Microscopy, Electron Probe Microanalysis, X-ray diffraction and Transmission Electron Microscopy. The two key findings resulted from this work. One is that the chi phase is stable at high temperature and transformed intomore » the Laves phase at low temperature. The other is that both the chi and Laves phases have large solubilites of Cr, Mo and Ni, among which the Mo solubility has a major role on the relative stability of the precipitate phases. The developed thermodynamic models were then applied to evaluating the Mo effect on the stability of precipitate phases in AISI 316 and NF709 alloys.« less

  6. Effects of thermal treatment on the co-rolled U-Mo fuel foils

    SciTech Connect (OSTI)

    Dennis D. Keiser, Jr.; Tammy L. Trowbridge; Cynthia R. Breckenridge; Brady L. Mackowiak; Glenn A. Moore; Barry H. Rabin; Mitchell K. Meyer

    2014-11-01

    A monolithic fuel type is being developed to convert US high performance research and test reactors such as Advanced Test Reactor (ATR) at Idaho National Laboratory from highly enriched uranium (HEU) to low-enriched uranium (LEU). The interaction between the cladding and the U-Mo fuel meat during fuel fabrication and irradiation is known to have negative impacts on fuel performance, such as mechanical integrity and dimensional stability. In order to eliminate/minimize the direct interaction between cladding and fuel meat, a thin zirconium diffusion barrier was introduced between the cladding and U-Mo fuel meat through a co-rolling process. A complex interface between the zirconium and U-Mo was developed during the co-rolling process. A predictable interface between zirconium and U-Mo is critical to achieve good fuel performance since the interfaces can be the weakest link in the monolithic fuel system. A post co-rolling annealing treatment is expected to create a well-controlled interface between zirconium and U-Mo. A systematic study utilizing post co-rolling annealing treatment has been carried out. Based on microscopy results, the impacts of the annealing treatment on the interface between zirconium and U-Mo will be presented and an optima annealing treatment schedule will be suggested. The effects of the annealing treatment on the fuel performance will also be discussed.

  7. MoS{sub 2} nanotube exfoliation as new synthesis pathway to molybdenum blue

    SciTech Connect (OSTI)

    Visic, B.; Gunde, M. Klanjsek; Kovac, J.; Iskra, I.; Jelenc, J.; Remskar, M.; Centre of Excellence Namaste, Jamova cesta 39, SI-1000 Ljubljana

    2013-02-15

    Graphical abstract: . Display Omitted Highlights: ? New synthesis approach to obtaining molybdenum blue via exfoliated MoS{sub 2} nanotubes. ? Material is prone to self assembly and is stable in high vacuum. ? Molecules are as small as 2 nm and their clusters are up to tens of nanometers. ? Change in absorption and oxidation states from the precursor MoS{sub 2}. -- Abstract: Molybdenum blue-type materials are usually obtained by partially reducing Mo{sup VI+} in acidic solutions, while in the presented method it is formed in ethanol solution of exfoliated MoS{sub 2} nanotubes, where the MoS{sub 2} flakes are the preferential location for their growth. Material was investigated by means of scanning electron and atomic force microscopy, showing the structure and self assembly, while also confirming that it is stable in high vacuum with molecules as small as 1.6 nm and the agglomerates of few tens of nanometres. The ultravioletvisible and photoelectron spectrometry show the change in absorption properties and oxidation states from MoS{sub 2} structure to molybdenum blue, while the presence of sulphur suggests that this is a new type of molybdenum blue material.

  8. Demonstration Assessment of LED Roadway Lighting: NE Cully Boulevard Portland, OR

    SciTech Connect (OSTI)

    Royer, Michael P.; Poplawski, Michael E.; Tuenge, Jason R.

    2012-06-29

    A new roadway lighting demonstration project was initiated in late 2010, which was planned in conjunction with other upgrades to NE Cully Boulevard, a residential collector road in the northeast area of Portland, OR. With the NE Cully Boulevard project, the Portland Bureau of Transportation hoped to demonstrate different light source technologies and different luminaires side-by-side. This report documents the initial performance of six different newly installed luminaires, including three LED products, one induction product, one ceramic metal halide product, and one high-pressure sodium (HPS) product that represented the baseline solution. It includes reported, calculated, and measured performance; evaluates the economic feasibility of each of the alternative luminaires; and documents user feedback collected from a group of local Illuminating Engineering Society (IES) members that toured the site. This report does not contain any long-term performance evaluations or laboratory measurements of luminaire performance. Although not all of the installed products performed equally, the alternative luminaires generally offered higher efficacy, more appropriate luminous intensity distributions, and favorable color quality when compared to the baseline HPS luminaire. However, some products did not provide sufficient illumination to all areas—vehicular drive lanes, bicycle lanes, and sidewalks—or would likely fail to meet design criteria over the life of the installation due to expected depreciation in lumen output. While the overall performance of the alternative luminaires was generally better than the baseline HPS luminaire, cost remains a significant barrier to widespread adoption. Based on the cost of the small quantity of luminaires purchased for this demonstration, the shortest calculated payback period for one of the alternative luminaire types was 17.3 years. The luminaire prices were notably higher than typical prices for currently available luminaires purchased in larger quantities. At prices that are more typical, the payback would be less than 10 years. In addition to the demonstration luminaires, a networked control system was installed for additional evaluation and demonstration purposes. The capability of control system to measure luminaire input power was explored in this study. A more exhaustive demonstration and evaluation of the control system will be the subject of future GATEWAY report(s).

  9. Microstructure evolution of Li uptake/removal in MoO{sub 2}@C nanoparticles with high lithium storage performance

    SciTech Connect (OSTI)

    Liu, Yulong; Zhang, Hong; Ouyang, Pan; Chen, Wenhao [School of Materials Science and Engineering, Central South University, Changsha 410083 (China); Li, Zhicheng, E-mail: zhchli@mail.csu.edu.cn [School of Materials Science and Engineering, Central South University, Changsha 410083 (China); State Key Laboratory of Powder Metallurgy, Central South University, Changsha 410083 (China)

    2014-02-01

    Highlights: The carbon-coated MoO{sub 2} (MoO{sub 2}@C) ultra fine nanoparticles are synthesized by one-pot hydrothermal method. MoO{sub 2}@C nanoparticles have high specific capacity, excellent cycling performance and rate performance. Phase transformations for lithium ion uptake/removal are examined carefully by TEM. Phase transformations are highly reversible during the redox process. - Abstract: A facile one pot strategy of a hydrothermal methodology was applied to synthesize the carbon coated MoO{sub 2} (MoO{sub 2}@C) nanostructured particles, which are composed of ultra fine nanoparticles with homogeneous carbon coating about several nanometers. As an electrode in lithium ion batteries, the MoO{sub 2}@C shows a high specific capacity and reversible capacity (730 mA h g{sup ?1} after 60 cycles). Microstructure investigations, by using a high resolution transmission electron microscopy, of the MoO{sub 2}@C based electrodes employed at various states during the first discharge/charge cycle were conducted to elucidate the lithium ion uptake/removal mechanism and cycling behavior. In the lithium uptake process, the original MoO{sub 2} phase transfers into Li{sub 0.98}MoO{sub 2} through an addition type reaction, and then nanosized metallic Mo emerges as a result of a conversion reaction. In turn, Mo could be oxidized to the intermediate Li{sub 0.98}MoO{sub 2} before converting to hyperfine MoO{sub 2} phase on upcoming lithium removal process.

  10. Proposal of a new generation of Laser Beacon for time calibration in the KM3NeT neutrino telescope

    SciTech Connect (OSTI)

    Real, Diego [IFIC, Instituto de Fsica Corpuscular, CSIC-Universidad de Valencia, C Collaboration: KM3NeT Collaboration

    2014-11-18

    The KM3NeT collaboration aims at the construction of a multi-km3 high-energy neutrino telescope in the Mediterranean Sea consisting of a matrix of pressure resistant glass spheres holding each a set (31) of small area photomultipliers. The main motivation of the telescope is to observe cosmic neutrinos through the Cherenkov light induced in sea water by charged particles produced in neutrino interactions with the surrounding medium. A relative time calibration between photomultipliers of the order of 1 ns is required to achieve an optimal performance. To this end, several time calibration subsystems have been developed. In this article, the proposal of a last generation Laser Beacon, to be used in KM3NeT and developed to measure and monitor the relative time offsets between photomultipliers, is presented.

  11. High Level Requirements for the Nuclear Energy -- Knowledge Base for Advanced Modeling and Simulation (NE-KAMS)

    SciTech Connect (OSTI)

    Rich Johnson; Hyung Lee; Kimberlyn C. Mousseau

    2011-09-01

    The US Department of Energy, Office of Nuclear Energy (DOE-NE), has been tasked with the important mission of ensuring that nuclear energy remains a compelling and viable energy source in the U.S. The motivations behind this mission include cost-effectively meeting the expected increases in the power needs of the country, reducing carbon emissions and reducing dependence on foreign energy sources. In the near term, to ensure that nuclear power remains a key element of U.S. energy strategy and portfolio, the DOE-NE will be working with the nuclear industry to support safe and efficient operations of existing nuclear power plants. In the long term, to meet the increasing energy needs of the U.S., the DOE-NE will be investing in research and development (R&D) and working in concert with the nuclear industry to build and deploy new, safer and more efficient nuclear power plants. The safe and efficient operations of existing nuclear power plants and designing, licensing and deploying new reactor designs, however, will require focused R&D programs as well as the extensive use and leveraging of advanced modeling and simulation (M&S). M&S will play a key role in ensuring safe and efficient operations of existing and new nuclear reactors. The DOE-NE has been actively developing and promoting the use of advanced M&S in reactor design and analysis through its R&D programs, e.g., the Nuclear Energy Advanced Modeling and Simulation (NEAMS) and Consortium for Advanced Simulation of Light Water Reactors (CASL) programs. Also, nuclear reactor vendors are already using CFD and CSM, for design, analysis, and licensing. However, these M&S tools cannot be used with confidence for nuclear reactor applications unless accompanied and supported by verification and validation (V&V) and uncertainty quantification (UQ) processes and procedures which provide quantitative measures of uncertainty for specific applications. The Nuclear Energy Knowledge base for Advanced Modeling and Simulation (NE-KAMS) is being developed at the Idaho National Laboratory in conjunction with Bettis Laboratory, Sandia National Laboratories, Argonne National Laboratory, Utah State University and others with the objective of establishing a comprehensive and web-accessible knowledge base that will provide technical services and resources for V&V and UQ of M&S in nuclear energy sciences and engineering. The knowledge base will serve as an important resource for technical exchange and collaboration that will enable credible and reliable computational models and simulations for application to nuclear reactor design, analysis and licensing. NE-KAMS will serve as a valuable resource for the nuclear industry, academia, the national laboratories, the U.S. Nuclear Regulatory Commission (NRC) and the public and will help ensure the safe, economical and reliable operation of existing and future nuclear reactors. From its inception, NE-KAMS will directly support nuclear energy research, development and demonstration programs within the U.S. Department of Energy (DOE), including the CASL, NEAMS, Light Water Reactor Sustainability (LWRS), Small Modular Reactors (SMR), and Next Generation Nuclear Power Plant (NGNP) programs. These programs all involve M&S of nuclear reactor systems, components and processes, and it is envisioned that NE-KAMS will help to coordinate and facilitate collaboration and sharing of resources and expertise for V&V and UQ across these programs.

  12. Doping against the native propensity of MoS₂: Degenerate hole doping by cation substitution

    SciTech Connect (OSTI)

    Suh, Joonki; Park, Tae-Eon; Lin, Der-Yuh; Fu, Deyi; Park, Joonsuk; Jung, Hee Joon; Chen, Yabin; Ko, Changhyun; Jang, Chaun; Sun, Yinghui; Sinclair, Robert; Chang, Joonyeon; Tongay, Sefaattin; Wu, Junqiao

    2014-12-10

    Layered transition metal dichalcogenides (TMDs) draw much attention as the key semiconducting material for two-dimensional electrical, optoelectronic, and spintronic devices. For most of these applications, both n- and p-type materials are needed to form junctions and support bipolar carrier conduction. However, typically only one type of doping is stable for a particular TMD. For example, molybdenum disulfide (MoS₂) is natively an n-type presumably due to omnipresent electron-donating sulfur vacancies, and stable/controllable p-type doping has not been achieved. The lack of p-type doping hampers the development of charge-splitting p–n junctions of MoS₂, as well as limits carrier conduction to spin-degenerate conduction bands instead of the more interesting, spin-polarized valence bands. Traditionally, extrinsic p-type doping in TMDs has been approached with surface adsorption or intercalation of electron-accepting molecules. However, practically stable doping requires substitution of host atoms with dopants where the doping is secured by covalent bonding. In this work, we demonstrate stable p-type conduction in MoS₂ by substitutional niobium (Nb) doping, leading to a degenerate hole density of ~3 × 10¹⁹ cm⁻³. Structural and X-ray techniques reveal that the Nb atoms are indeed substitutionally incorporated into MoS₂ by replacing the Mo cations in the host lattice. van der Waals p–n homojunctions based on vertically stacked MoS₂ layers are fabricated, which enable gate-tunable current rectification. A wide range of microelectronic, optoelectronic, and spintronic devices can be envisioned from the demonstrated substitutional bipolar doping of MoS₂. From the miscibility of dopants with the host, it is also expected that the synthesis technique demonstrated here can be generally extended to other TMDs for doping against their native unipolar propensity.

  13. MCNPX-CINDER'90 Simulation of Photonuclear Mo-99 Production Experiments

    SciTech Connect (OSTI)

    Kelsey, Charles T. IV [Los Alamos National Laboratory; Chemerizov, Sergey D. [Argonne National Laboratory; Dale, Gregory E. [Los Alamos National Laboratory; Harvey, James T. [NorthStar Medical Radioisotopes; Tkac, Peter [Argonne National Laboratory; Vandegrift, George R III [Argonne National Laboratory

    2011-01-01

    The MCNPX and CINDER'90 codes were used to support design of experiments investigating Mo-99 production with a 20-MeV electron beam. Bremsstrahlung photons produced by the electron beam interacting with the target drive the desired Mo-100({gamma},n)Mo-99 reaction, as well as many undesired reactions important to accurate prediction of radiation hazards. MCNPX is a radiation transport code and CINDER'90 is a transmutation code. They are routinely used together for accelerator activation calculations. Low energy neutron fluxes and production rates for nonneutron and high energy neutron induced reactions computed using MCNPX are inputs to CINDER'90. CINDER'90 presently has only a neutron reaction cross section library up to 25 MeV and normally the other reaction rates come from MCNPX physics models. For this work MCNPX photon flux tallies modified by energy response functions prepared from evaluated photonuclear cross section data were used to tally the reaction rates for CINDER'90 input. The cross section evaluations do not provide isomer to ground state yield ratios so a spin based approximation was used. Post irradiation dose rates were calculated using MCNPX with CINDER'90 produced decay photon spectra. The sensitivity of radionuclide activities and dose rates to beam parameters including energy, position, and profile, as well as underlying isomer assumptions, was investigated. Three experimental production targets were irradiated, two natural Mo and one Mo-100 enriched. Natural Mo foils upstream of the targets were used to analyze beam position and profile by exposing Gafchromic film to the foils after each irradiation. Activation and dose rate calculations were rerun after the experiments using measured beam parameters for comparison with measured Mo-99 activities and dose rates.

  14. Rotational and angular distributions of NO products from NO-Rg(Rg = He, Ne, Ar) complex photodissociation

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Heather L. Holmes-Ross; Hall, Gregory E.; Valenti, Rebecca J.; Yu, Hua -Gen; Lawrance, Warren D.

    2016-01-29

    In this study, we present the results of an investigation into the rotational and angular distributions of the NO A~ state fragment following photodissociation of the NO-He, NO-Ne and NO-Ar van der Waals complexed excited via the A~ ← X~ transition. For each complex the dissociation is probed for several values of Ea, the available energy above the dissociation threshold.

  15. REP&V TO ATTNJF: NE-23 SUWECC Commercial Facilities Used by National Lead Company of Ohio in Support

    Office of Legacy Management (LM)

    REP&V TO ATTNJF: NE-23 SUWECC Commercial Facilities Used by National Lead Company of Ohio in Support 'of FMPC Operations TO: Robert E. Lynch Procuresnent and CorXracts Division, AD-42 Oak Ridge Operations Office The Division of Facility and Site Decormnissioning Projects (DFSP) is responsible for managing the Department's Formerly Utilized Sites Remedial Action Program (FUSRAP). The purposes of FUSRAP are (1) to identify facilities formerly operated for or by the Manhattan Engineer District

  16. A measurement of the neutral current neutrino-nucleon elastic cross section at MiniBooNE

    SciTech Connect (OSTI)

    Cox, David Christopher; /Indiana U.

    2008-02-01

    The neutral current neutrino-nucleon elastic interaction {nu} N {yields} {nu} N is a fundamental process of the weak interaction ideally suited for characterizing the structure of the nucleon neutral weak current. This process comprises {approx}18% of neutrino events in the neutrino oscillation experiment, MiniBooNE, ranking it as the experiment's third largest process. Using {approx}10% of MiniBooNE's available neutrino data, a sample of these events were identified and analyzed to determine the differential cross section as a function of the momentum transfer of the interaction, Q{sup 2}. This is the first measurement of a differential cross section with MiniBooNE data. From this analysis, a value for the nucleon axial mass M{sub A} was extracted to be 1.34 {+-} 0.25 GeV consistent with previous measurements. The integrated cross section for the Q{sup 2} range 0.189 {yields} 1.13 GeV{sup 2} was calculated to be (8.8 {+-} 0.6(stat) {+-} 0.2(syst)) x 10{sup -40} cm{sup 2}.

  17. Demonstration of isotype GaN/AlN/GaN heterobarrier diodes by NH{sub 3}-molecular beam epitaxy

    SciTech Connect (OSTI)

    Fireman, Micha N.; Browne, David A.; Mazumder, Baishakhi; Speck, James S.; Mishra, Umesh K.

    2015-05-18

    The results of vertical transport through nitride heterobarrier structures grown by ammonia molecular beam epitaxy are presented. Structures are designed with binary layers to avoid the effects of random alloy fluctuations in ternary nitride barriers. The unintentional incorporation of Ga in the AlN growth is investigated by atom probe tomography and is shown to be strongly dependent on both the NH{sub 3} flowrate and substrate temperature growth parameters. Once nominally pure AlN layer growth conditions are achieved, structures consisting of unintentionally doped (UID) GaN spacer layers adjacent to a nominally pure AlN are grown between two layers of n+ GaN, from which isotype diodes are fabricated. Varying the design parameters of AlN layer thickness, UID spacer layer thickness, and threading dislocation density show marked effects on the vertical transport characteristics of these structures. The lack of significant temperature dependence, coupled with Fowler-Nordheim and/or Milliken-Lauritsen analysis, point to a prevalently tunneling field emission mechanism through the AlN barrier. Once flatband conditions in the UID layer are achieved, electrons leave the barrier with significant energy. This transport mechanism is of great interest for applications in hot electron structures.

  18. Density Functional Studies of Stoichiometric Surfaces of Orthorhombic Hybrid Perovskite CH3NH3PbI3

    SciTech Connect (OSTI)

    Wang, Yun; Huang, Jingsong; Sumpter, Bobby G; Zhang, Haimin; Liu, Porun; Yang, Huagui; Zhao, Huijun

    2015-01-01

    Organic/inorganic hybrid perovskite materials are highly attractive for dye-sensitized solar cells as demonstrated by their rapid advances in energy conversion efficiency. In this work, the structures, energetics, and electronic properties for a range of stoichiometric surfaces of the orthorhombic perovskite CH3NH3PbI3 are theoretically studied using density functional theory. Various possible spatially and constitutionally isomeric surfaces are considered by diversifying the spatial orientations and connectivities of surface Pb-I bonds. The comparison of the surface energies for the most stable configurations identified for various surfaces shows that the stabilities of stoichiometric surfaces are mainly dictated by the coordination numbers of surface atoms, which are directly correlated with the numbers of broken bonds. Additionally, Coulombic interactions between I anions and organic countercations on the surface also contribute to the stabilization. Electronic properties are compared between the most stable (100) surface and the bulk phase, showing generally similar features except for the lifted band degeneracy and the enhanced bandgap energy for the surface. These studies on the stoichiometric surfaces serve as the first step toward gaining a fundamental understanding of the interfacial properties in the current structural design of perovskite based solar cells, in order to achieve further breakthroughs in solar conversion efficiencies.

  19. The efficiency limit of CH{sub 3}NH{sub 3}PbI{sub 3} perovskite solar cells

    SciTech Connect (OSTI)

    Sha, Wei E. I.; Ren, Xingang; Chen, Luzhou; Choy, Wallace C. H.

    2015-06-01

    With the consideration of photon recycling effect, the efficiency limit of methylammonium lead iodide (CH{sub 3}NH{sub 3}PbI{sub 3}) perovskite solar cells is predicted by a detailed balance model. To obtain convincing predictions, both AM 1.5 spectrum of Sun and experimentally measured complex refractive index of perovskite material are employed in the detailed balance model. The roles of light trapping and angular restriction in improving the maximal output power of thin-film perovskite solar cells are also clarified. The efficiency limit of perovskite cells (without the angular restriction) is about 31%, which approaches to Shockley-Queisser limit (33%) achievable by gallium arsenide (GaAs) cells. Moreover, the Shockley-Queisser limit could be reached with a 200?nm-thick perovskite solar cell, through integrating a wavelength-dependent angular-restriction design with a textured light-trapping structure. Additionally, the influence of the trap-assisted nonradiative recombination on the device efficiency is investigated. The work is fundamentally important to high-performance perovskite photovoltaics.

  20. Method for the production of .sup.99m Tc compositions from .sup.99 Mo-containing materials

    DOE Patents [OSTI]

    Bennett, Ralph G. (Idaho Falls, ID); Christian, Jerry D. (Idaho Falls, ID); Grover, S. Blaine (Idaho Falls, ID); Petti, David A. (Idaho Falls, ID); Terry, William K. (Idaho Falls, ID); Yoon, Woo Y. (Idaho Falls, ID)

    1998-01-01

    An improved method for producing .sup.99m Tc compositions from .sup.99 Mo compounds. .sup.100 Mo metal or .sup.100 MoO.sub.3 is irradiated with photons in a particle (electron) accelerator to ultimately produce .sup.99 MoO.sub.3. This composition is then heated in a reaction chamber to form a pool of molten .sup.99 MoO.sub.3 with an optimum depth of 0.5-5 mm. A gaseous mixture thereafter evolves from the molten .sup.99 MoO.sub.3 which contains vaporized .sup.99 MoO.sub.3, vaporized .sup.99m TcO.sub.3, and vaporized .sup.99m TcO.sub.2. This mixture is then combined with an oxidizing gas (O.sub.2(g)) to generate a gaseous stream containing vaporized .sup.99m Tc.sub.2 O.sub.7 and vaporized .sup.99 MoO.sub.3. Next, the gaseous stream is cooled in a primary condensation stage in the reaction chamber to remove vaporized .sup.99 MoO.sub.3. Cooling is undertaken at a specially-controlled rate to achieve maximum separation efficiency. The gaseous stream is then cooled in a sequential secondary condensation stage to convert vaporized .sup.99m Tc.sub.2 O.sub.7 into a condensed .sup.99m Tc-containing reaction product which is collected.

  1. Method for the production of {sup 99m}Tc compositions from {sup 99}Mo-containing materials

    DOE Patents [OSTI]

    Bennett, R.G.; Christian, J.D.; Grover, S.B.; Petti, D.A.; Terry, W.K.; Yoon, W.Y.

    1998-09-01

    An improved method is described for producing {sup 99m}Tc compositions from {sup 99}Mo compounds. {sup 100}Mo metal or {sup 100}MoO{sub 3} is irradiated with photons in a particle (electron) accelerator to ultimately produce {sup 99}MoO{sub 3}. This composition is then heated in a reaction chamber to form a pool of molten {sup 99}MoO{sub 3} with an optimum depth of 0.5--5 mm. A gaseous mixture thereafter evolves from the molten {sup 99}MoO{sub 3} which contains vaporized {sup 99}MoO{sub 3}, vaporized {sup 99m}TcO{sub 3}, and vaporized {sup 99m}TcO{sub 2}. This mixture is then combined with an oxidizing gas (O{sub 2(g)}) to generate a gaseous stream containing vaporized {sup 99m}Tc{sub 2}O{sub 7} and vaporized {sup 99}MoO{sub 3}. Next, the gaseous stream is cooled in a primary condensation stage in the reaction chamber to remove vaporized {sup 99}MoO{sub 3}. Cooling is undertaken at a specially-controlled rate to achieve maximum separation efficiency. The gaseous stream is then cooled in a sequential secondary condensation stage to convert vaporized {sup 99m}Tc{sub 2}O{sub 7} into a condensed {sup 99m}Tc-containing reaction product which is collected. 1 fig.

  2. Surface oxidation energetics and kinetics on MoS{sub 2} monolayer

    SciTech Connect (OSTI)

    KC, Santosh; Longo, Roberto C.; Wallace, Robert M.; Cho, Kyeongjae

    2015-04-07

    In this work, surface oxidation of monolayer MoS{sub 2} (one of the representative semiconductors in transition-metal dichalcogenides) has been investigated using density functional theory method. Oxygen interaction with MoS{sub 2} shows that, thermodynamically, the surface tends to be oxidized. However, the dissociative absorption of molecular oxygen on the MoS{sub 2} surface is kinetically limited due to the large energy barrier at low temperature. This finding elucidates the air stability of MoS{sub 2} surface in the atmosphere. Furthermore, the presence of defects significantly alters the surface stability and adsorption mechanisms. The electronic properties of the oxidized surface have been examined as a function of oxygen adsorption and coverage as well as substitutional impurities. Our results on energetics and kinetics of oxygen interaction with the MoS{sub 2} monolayer are useful for the understanding of surface oxidation, air stability, and electronic properties of transition-metal dichalcogenides at the atomic scale.

  3. TEM Characterization of High Burn-up Microstructure of U-7Mo Alloy

    SciTech Connect (OSTI)

    Jian Gan; Brandon Miller; Dennis Keiser; Adam Robinson; James Madden; Pavel Medvedev; Daniel Wachs

    2014-04-01

    As an essential part of global nuclear non-proliferation effort, the RERTR program is developing low enriched U-Mo fuels (< 20% U-235) for use in research and test reactors that currently employ highly enriched uranium fuels. One type of fuel being developed is a dispersion fuel plate comprised of U-7Mo particles dispersed in Al alloy matrix. Recent TEM characterizations of the ATR irradiated U-7Mo dispersion fuel plates include the samples with a local fission densities of 4.5, 5.2, 5.6 and 6.3 E+21 fissions/cm3 and irradiation temperatures of 101-136?C. The development of the irradiated microstructure of the U-7Mo fuel particles consists of fission gas bubble superlattice, large gas bubbles, solid fission product precipitates and their association to the large gas bubbles, grain subdivision to tens or hundreds of nanometer size, collapse of bubble superlattice, and amorphisation. This presentation will describe the observed microstructures specifically focusing on the U-7Mo fuel particles. The impact of the observed microstructure on the fuel performance and the comparison of the relevant features with that of the high burn-up UO2 fuels will be discussed.

  4. FeAl and Mo-Si-B Intermetallic Coatings Prepared by Thermal Spraying

    SciTech Connect (OSTI)

    Totemeier, T.C.; Wright, R.N.; Swank, W.D.

    2003-04-22

    FeAl and Mo-Si-B intermetallic coatings for elevated temperature environmental resistance were prepared using high-velocity oxy-fuel (HVOF) and air plasma spray (APS) techniques. For both coating types, the effect of coating parameters (spray particle velocity and temperature) on the microstructure and physical properties of the coatings was assessed. Fe-24Al (wt.%) coatings were prepared using HVOF thermal spraying at spray particle velocities varying from 540 m/s to 700 m/s. Mo-13.4Si-2.6B coatings were prepared using APS at particle velocities of 180 and 350 m/s. Residual stresses in the HVOF FeAl coatings were compressive, while stresses in the APS Mo-Si-B coatings were tensile. In both cases, residual stresses became more compressive with increasing spray particle velocity due to increased peening imparted by the spray particles. The hardness and elastic moduli of FeAl coatings also increased with increasing particle velocity, again due to an increased peening effect. For Mo-Si-B coatings, plasma spraying at 180 m/s resulted in significant oxidation of the spray particles and conversion of the T1 phase into amorphous silica and {alpha}-Mo. The T1 phase was retained after spraying at 350 m/s.

  5. Fragile structural transition in Mo3Sb7

    SciTech Connect (OSTI)

    Yan, Jiaqiang -Q.; McGuire, Michael A; May, Andrew F; Parker, David S.; Mandrus, D. G.; Sales, Brian C.

    2015-08-10

    Mo3Sb7 single crystals lightly doped with Cr, Ru, or Te are studied in order to explore the interplay between superconductivity, magnetism, and the cubic-tetragonal structural transition. The structural transition at 53 K is extremely sensitive to Ru or Te substitution which introduces additional electrons, but robust against Cr substitution. We observed no sign of a structural transition in superconducting Mo2.91Ru0.09Sb7 and Mo3Sb6.975Te0.025. In contrast, 3 at.% Cr doping only slightly suppresses the structural transition to 48 K while leaving no trace of superconductivity above 1.8 K. Analysis of magnetic properties suggests that the interdimer interaction in Mo3Sb7 is near a critical value and essential for the structural transition. Futhermore, all dopants suppress the superconductivity of Mo3Sb7. The tetragonal structure is not necessary for superconductivity.

  6. Monte Carlo calculations for reference dosimetry of electron beams with the PTW Roos and NE2571 ion chambers

    SciTech Connect (OSTI)

    Muir, B. R. Rogers, D. W. O.

    2013-12-15

    Purpose: To investigate recommendations for reference dosimetry of electron beams and gradient effects for the NE2571 chamber and to provide beam quality conversion factors using Monte Carlo simulations of the PTW Roos and NE2571 ion chambers. Methods: The EGSnrc code system is used to calculate the absorbed dose-to-water and the dose to the gas in fully modeled ion chambers as a function of depth in water. Electron beams are modeled using realistic accelerator simulations as well as beams modeled as collimated point sources from realistic electron beam spectra or monoenergetic electrons. Beam quality conversion factors are calculated with ratios of the doses to water and to the air in the ion chamber in electron beams and a cobalt-60 reference field. The overall ion chamber correction factor is studied using calculations of water-to-air stopping power ratios. Results: The use of an effective point of measurement shift of 1.55 mm from the front face of the PTW Roos chamber, which places the point of measurement inside the chamber cavity, minimizes the difference betweenR{sub 50}, the beam quality specifier, calculated from chamber simulations compared to that obtained using depth-dose calculations in water. A similar shift minimizes the variation of the overall ion chamber correction factor with depth to the practical range and reduces the root-mean-square deviation of a fit to calculated beam quality conversion factors at the reference depth as a function of R{sub 50}. Similarly, an upstream shift of 0.34 r{sub cav} allows a more accurate determination of R{sub 50} from NE2571 chamber calculations and reduces the variation of the overall ion chamber correction factor with depth. The determination of the gradient correction using a shift of 0.22 r{sub cav} optimizes the root-mean-square deviation of a fit to calculated beam quality conversion factors if all beams investigated are considered. However, if only clinical beams are considered, a good fit to results for beam quality conversion factors is obtained without explicitly correcting for gradient effects. The inadequacy of R{sub 50} to uniquely specify beam quality for the accurate selection of k{sub Q} factors is discussed. Systematic uncertainties in beam quality conversion factors are analyzed for the NE2571 chamber and amount to between 0.4% and 1.2% depending on assumptions used. Conclusions: The calculated beam quality conversion factors for the PTW Roos chamber obtained here are in good agreement with literature data. These results characterize the use of an NE2571 ion chamber for reference dosimetry of electron beams even in low-energy beams.

  7. Thermal stability of fission gas bubble superlattice in irradiated U10Mo fuel

    SciTech Connect (OSTI)

    Gan, J.; Keiser, D. D.; Miller, B. D.; Robinson, A. B.; Wachs, D. M.; Meyer, M. K.

    2015-09-01

    To investigate the thermal stability of the fission gas bubble superlattice, a key microstructural feature in both irradiated U-7Mo dispersion and U-10Mo monolithic fuel plates, a FIB-TEM sample of the irradiated U-10Mo fuel with a local fission density of 3.51021 fissions/cm3 was used for an in-situ heating TEM experiment. The temperature of the heating holder was raised at a ramp rate of approximately 10 C/min up to ~700 C, kept at that temperature for about 34 min, continued to 850 C with a reduced rate of 5 C/min. The result shows a high thermal stability of the fission gas bubble superlattice. The implication of this observation on the fuel microstructural evolution and performance under irradiation is discussed.

  8. Observation of localized states in atomically thin MoS{sub 2} field effect transistor

    SciTech Connect (OSTI)

    Ghatak, Subhamoy; Pal, Atindra Nath; Ghosh, Arindam

    2013-12-04

    We present electrical transport and low frequency (1/f) noise measurements on mechanically exfoliated single, bi and trilayer MoS{sub 2}-based FET devices on Si/SiO{sub 2} substrate. We find that the electronic states in MoS{sub 2} are localized at low temperatures (T) and conduction happens through variable range hopping (VRH). A steep increase of 1/f noise with decreasing T, typical for localized regime was observed in all of our devices. From gate voltage dependence of noise, we find that the noise power is inversely proportional to square of the number density (? 1/n{sup 2}) for a wide range of T, indicating number density fluctuations to be the dominant source of 1/f noise in these MoS{sub 2} FETs.

  9. Controlling the metal to semiconductor transition of MoS2 and WS2 in solution

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Chou, Stanley Shihyao; Yi-Kai Huang; Kim, Jaemyung; Kaehr, Bryan James; Foley, Brian M.; Lu, Ping; Conner Dykstra; Hopkins, Patrick E.; Brinker, C. Jeffrey; Jiaxing Huang; et al

    2015-01-22

    Lithiation-exfoliation produces single to few-layered MoS2 and WS2 sheets dispersible in water. However, the process transforms them from the pristine semiconducting 2H phase to a distorted metallic phase. Recovery of the semiconducting properties typically involves heating of the chemically exfoliated sheets at elevated temperatures. Therefore, it has been largely limited to sheets deposited on solid substrates. We report the dispersion of chemically exfoliated MoS2 sheets in high boiling point organic solvents enabled by surface functionalization and the controllable recovery of their semiconducting properties directly in solution. Ultimately, this process connects the scalability of chemical exfoliation with the simplicity of solutionmore » processing, enabling a facile method for tuning the metal to semiconductor transitions of MoS2 and WS2 within a liquid medium.« less

  10. Electronic and magnetic properties of Mo doped graphene; full potential approach

    SciTech Connect (OSTI)

    Thakur, Jyoti Kashyap, Manish K.; Singh, Mukhtiyar; Saini, Hardev S.

    2015-05-15

    The electronic and magnetic properties of Pristine and Mo doped Graphene have been calculated using WIEN2k implementation of full potential linearized augmented plane wave (FPLAPW) method based on Density Functional Theory (DFT). The exchange and correlation (XC) effects were taken into account by generalized gradient approximation (GGA). The calculated results show that Mo doping creates magnetism in Graphene by shifting the energy levels at E{sub F} and opens up a channel for Graphene to be used in real nanoscale device applications. The unpaired d-electrons of Mo atom are responsible for induced magnetism in Graphene. Magnetic ordering created in Graphene in this way makes it suitable for recording media, magnetic sensors, magnetic inks and spintronic devices.

  11. Highly conducting SrMoO{sub 3} thin films for microwave applications

    SciTech Connect (OSTI)

    Radetinac, Aldin Mani, Arzhang; Ziegler, Jrgen; Alff, Lambert; Komissinskiy, Philipp; Melnyk, Sergiy; Nikfalazar, Mohammad; Zheng, Yuliang; Jakoby, Rolf

    2014-09-15

    We have measured the microwave resistance of highly conducting perovskite oxide SrMoO{sub 3} thin film coplanar waveguides. The epitaxial SrMoO{sub 3} thin films were grown by pulsed laser deposition and showed low mosaicity and smooth surfaces with a root mean square roughness below 0.3?nm. Layer-by-layer growth could be achieved for film thicknesses up to 400?nm as monitored by reflection high-energy electron diffraction and confirmed by X-ray diffraction. We obtained a constant microwave resistivity of 29???cm between 0.1 and 20?GHz by refining the frequency dependence of the transmission coefficients. Our result shows that SrMoO{sub 3} is a viable candidate as a highly conducting electrode material for all-oxide microwave electronic devices.

  12. Exciton-dominant electroluminescence from a diode of monolayer MoS{sub 2}

    SciTech Connect (OSTI)

    Ye, Yu; Ye, Ziliang; Gharghi, Majid; Zhu, Hanyu; Wang, Yuan; Zhao, Mervin; Yin, Xiaobo; Zhang, Xiang

    2014-05-12

    In two-dimensional monolayer MoS{sub 2}, excitons dominate the absorption and emission properties. However, the low electroluminescent efficiency and signal-to-noise ratio limit our understanding of the excitonic behavior of electroluminescence. Here, we study the microscopic origin of the electroluminescence from a diode of monolayer MoS{sub 2} fabricated on a heavily p-type doped silicon substrate. Direct and bound-exciton related recombination processes are identified from the electroluminescence. At a high electron-hole pair injection rate, Auger recombination of the exciton-exciton annihilation of the bound exciton emission is observed at room temperature. Moreover, the efficient electrical injection demonstrated here allows for the observation of a higher energy exciton peak of 2.255?eV in the monolayer MoS{sub 2} diode, attributed to the excited exciton state of a direct-exciton transition.

  13. Two-step growth of two-dimensional WSe2/MoSe2 heterostructures

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Gong, Yongji; Lei, Sidong; Lou, Jun; Liu, Zheng; Vajtai, Robert; Zhou, Wu; Ajayan, Pullikel M.

    2015-08-03

    Two dimensional (2D) materials have attracted great attention due to their unique properties and atomic thickness. Although various 2D materials have been successfully synthesized with different optical and electrical properties, a strategy for fabricating 2D heterostructures must be developed in order to construct more complicated devices for practical applications. Here we demonstrate for the first time a two-step chemical vapor deposition (CVD) method for growing transition-metal dichalcogenide (TMD) heterostructures, where MoSe2 was synthesized first and followed by an epitaxial growth of WSe2 on the edge and on the top surface of MoSe2. Compared to previously reported one-step growth methods, thismore » two-step growth has the capability of spatial and size control of each 2D component, leading to much larger (up to 169 μm) heterostructure size, and cross-contamination can be effectively minimized. Furthermore, this two-step growth produces well-defined 2H and 3R stacking in the WSe2/MoSe2 bilayer regions and much sharper in-plane interfaces than the previously reported MoSe2/WSe2 heterojunctions obtained from one-step growth methods. The resultant heterostructures with WSe2/MoSe2 bilayer and the exposed MoSe2 monolayer display rectification characteristics of a p-n junction, as revealed by optoelectronic tests, and an internal quantum efficiency of 91% when functioning as a photodetector. As a result, a photovoltaic effect without any external gates was observed, showing incident photon to converted electron (IPCE) efficiencies of approximately 0.12%, providing application potential in electronics and energy harvesting.« less

  14. Thermal aging modeling and validation on the Mo containing Fe-Cr-Ni alloys

    SciTech Connect (OSTI)

    Yang, Ying; Tan, Lizhen; Busby, Jeremy T.

    2015-04-01

    Thermodynamics of intermetallic phases in Fe-rich Fe-Cr-Ni-Mo alloys is critical knowledge to understand thermal aging effect on the phase stability of Mo-containing austenitic steels, which subsequently facilitates alloy design/improvement and degradation mitigation of these materials for reactor applications. Among the intermetallic phases, Chi (χ), Laves, and Sigma (σ) are often of concern because of their tendency to cause embrittlement of the materials. The focus of this study is thermal stability of the Chi and Laves phases as they were less studied compared to the Sigma phase. Coupled with thermodynamic modeling, thermal stability of intermetallic phases in Mo containing Fe-Cr-Ni alloys was investigated at 1000, 850 and 700 C for different annealing times. The morphologies, compositions and crystal structures of the precipitates of the intermetallic phases were carefully examined by scanning electron microscopy, electron probe microanalysis, X-ray diffraction, and transmission electron microscopy. Three key findings resulted from this study. First, the Chi phase is stable at high temperature, and with decreasing temperature it transforms into the Laves phase that is stable at low temperature. Secondly, Cr, Mo, Ni are soluble in both the Chi and Laves phases, with the solubility of Mo playing a major role in the relative stability of the intermetallic phases. Thirdly, in situ transformation from Chi phase to Laves phase was directly observed, which increased the local strain field, generated dislocations in the intermetallic phases, and altered the precipitate phase orientation relationship with the austenitic matrix. The thermodynamic models that were developed and validated were then applied to evaluating the effect of Mo on the thermal stability of intermetallic phases in type 316 and NF709 stainless steels.

  15. Electrical and photovoltaic characteristics of MoS{sub 2}/Si p-n junctions

    SciTech Connect (OSTI)

    Hao, Lanzhong Liu, Yunjie Gao, Wei; Han, Zhide; Xue, Qingzhong; Zeng, Huizhong; Wu, Zhipeng; Zhu, Jun; Zhang, Wanli

    2015-03-21

    Bulk-like molybdenum disulfide (MoS{sub 2}) thin films were deposited on the surface of p-type Si substrates using dc magnetron sputtering technique and MoS{sub 2}/Si p-n junctions were formed. The vibrating modes of E{sup 1}{sub 2g} and A{sub 1g} were observed from the Raman spectrum of the MoS{sub 2} films. The current density versus voltage (J-V) characteristics of the junction were investigated. A typical J-V rectifying effect with a turn-on voltage of 0.2?V was shown. In different voltage range, the electrical transporting of the junction was dominated by diffusion current and recombination current, respectively. Under the light illumination of 15?mW?cm{sup ?2}, the p-n junction exhibited obvious photovoltaic characteristics with a short-circuit current density of 3.2?mA?cm{sup ?2} and open-circuit voltage of 0.14?V. The fill factor and energy conversion efficiency were 42.4% and 1.3%, respectively. According to the determination of the Fermi-energy level (?4.65?eV) and energy-band gap (?1.45?eV) of the MoS{sub 2} films by capacitance-voltage curve and ultraviolet-visible transmission spectra, the mechanisms of the electrical and photovoltaic characteristics were discussed in terms of the energy-band structure of the MoS{sub 2}/Si p-n junctions. The results hold the promise for the integration of MoS{sub 2} thin films with commercially available Si-based electronics in high-efficient photovoltaic devices.

  16. Rapid first-cycle lithiation strategy for enhanced performance of Li-MoS2

    Office of Scientific and Technical Information (OSTI)

    batteries as identified by in situ studies. (Journal Article) | SciTech Connect Rapid first-cycle lithiation strategy for enhanced performance of Li-MoS2 batteries as identified by in situ studies. Citation Details In-Document Search Title: Rapid first-cycle lithiation strategy for enhanced performance of Li-MoS2 batteries as identified by in situ studies. Abstract not provided. Authors: Jiayu Wan ; Wenzhong Bao ; Yang Liu ; Jiaqi Dai ; Fei Shen ; Lihui Zhou ; Xinghan Cai ; Dan Urban ;

  17. Neutrino-nucleus scattering of {sup 95,97}Mo and {sup 116}Cd

    SciTech Connect (OSTI)

    Ydrefors, E.; Almosly, W.; Suhonen, J.

    2013-12-30

    Accurate knowledge about the nuclear responses to supernova neutrinos for relevant nuclear targets is important both for neutrino detection and for astrophysical applications. In this paper we discuss the cross sections for the charged-current neutrino-nucleus scatterings off {sup 95,97}Mo and {sup 116}Cd. The microscopic quasiparticle-phonon model is adopted for the odd-even nuclei {sup 95,97}Mo. In the case of {sup 116}Cd we present cross sections both for the Bonn one-boson-exchange potential and self-consistent calculations based on modern Skyrme interactions.

  18. Valence and metal/silicate partitioning of Mo: Implications for conditions

    Office of Scientific and Technical Information (OSTI)

    of Earth accretion and core formation (Journal Article) | SciTech Connect SciTech Connect Search Results Journal Article: Valence and metal/silicate partitioning of Mo: Implications for conditions of Earth accretion and core formation Citation Details In-Document Search Title: Valence and metal/silicate partitioning of Mo: Implications for conditions of Earth accretion and core formation Authors: Righter, K. ; Danielson, L.R. ; Pando, K.M. ; Shofner, G.A. ; Sutton, S.R. ; Newville, M. ; Lee,

  19. Site-dependent free energy barrier for proton reduction on MoS2 edges

    Office of Scientific and Technical Information (OSTI)

    (Journal Article) | SciTech Connect Site-dependent free energy barrier for proton reduction on MoS2 edges Citation Details In-Document Search Title: Site-dependent free energy barrier for proton reduction on MoS2 edges Authors: Choi, W ; Wood, B C ; Schwegler, E ; Ogitsu, T Publication Date: 2013-05-30 OSTI Identifier: 1113397 Report Number(s): LLNL-JRNL-639087 DOE Contract Number: W-7405-ENG-48 Resource Type: Journal Article Resource Relation: Journal Name: Journal of Physical Chemistry C,

  20. Primary arm spacing in chill block melt spun Ni-Mo alloys

    SciTech Connect (OSTI)

    Tewari, S.N.; Glasgow, T.K.

    1986-01-01

    Chill block melt spun ribbons of Ni-Mo binary alloys containing 8.0 to 41.8 wt % Mo have been prepared under carefully controlled processing conditions. The growth velocity has been determined as a function of distance from the quench surface from the observed ribbon thickness dependence on the melt puddle residence time. Primary arm spacings measured at the midribbon thickness locations show a dependence on growth velocity and alloy composition which is expected from dendritic growth models for binary alloys directionally solidified in a positive temperature gradient.

  1. Single-layer MoS{sub 2} roughness and sliding friction quenching by interaction with atomically flat substrates

    SciTech Connect (OSTI)

    Quereda, J.; Castellanos-Gomez, A.; Agrat, N.; Rubio-Bollinger, G.

    2014-08-04

    We experimentally study the surface roughness and the lateral friction force in single-layer MoS{sub 2} crystals deposited on different substrates: SiO{sub 2}, mica, and hexagonal boron nitride (h-BN). Roughness and sliding friction measurements are performed by atomic force microscopy. We find a strong dependence of the MoS{sub 2} roughness on the underlying substrate material, being h-BN the substrate which better preserves the flatness of the MoS{sub 2} crystal. The lateral friction also lowers as the roughness decreases, and attains its lowest value for MoS{sub 2} flakes on h-BN substrates. However, it is still higher than for the surface of a bulk MoS{sub 2} crystal, which we attribute to the deformation of the flake due to competing tip-to-flake and flake-to-substrate interactions.

  2. High blue-near ultraviolet photodiode response of vertically stacked graphene-MoS{sub 2}-metal heterostructures

    SciTech Connect (OSTI)

    Wi, Sungjin; Chen, Mikai; Nam, Hongsuk; Liu, Amy C.; Meyhofer, Edgar; Liang, Xiaogan

    2014-06-09

    We present a study on the photodiode response of vertically stacked graphene/MoS{sub 2}/metal heterostructures in which MoS{sub 2} layers are doped with various plasma species. In comparison with undoped heterostructures, such doped ones exhibit significantly improved quantum efficiencies in both photovoltaic and photoconductive modes. This indicates that plasma-doping-induced built-in potentials play an important role in photocurrent generation. As compared to indium-tin-oxide/ MoS{sub 2}/metal structures, the presented graphene/MoS{sub 2}/metal heterostructures exhibit greatly enhanced quantum efficiencies in the blue-near ultraviolet region, which is attributed to the low density of recombination centers at graphene/MoS{sub 2} heterojunctions. This work advances the knowledge for making photo-response devices based on layered materials.

  3. Modeling of plasma chemistry in an atmospheric pressure Ar/NH{sub 3} cylindrical dielectric barrier discharge described using the one-dimensional fluid model

    SciTech Connect (OSTI)

    Li Zhi [School of Science, University of Science and Technology Liaoning, Anshan 114051 (China); School of Physics and Optoelectronic Engineering, Dalian University of Technology, Dalian 116024 (China); Zhao Zhen [School of Chemistry and Life Science, Anshan Normal University, Anshan 114007 (China); School of Chemical Engineering, University of Science and Technology Liaoning, Anshan 114051 (China); Li Xuehui [Physical Science and Technical College, Dalian University, Dalian 116622 (China)

    2013-01-15

    The keynote of our research is to study the gas phase chemistry in an atmospheric pressure Ar/NH{sub 3} cylindrical dielectric barrier discharge, which is very important to produce the iron-nitride magnetic fluid. For this purpose, a home-made one dimensional fluid model with the Scharfetter-Gummel method has been developed. The equations solved are the particle balances, assuming a drift-diffusion approximation for the fluxes, and the electron energy equation. The self-consistent electric field is obtained by the simultaneous solution of Poisson's equation. The simulations were carried out for the different ammonia concentrations (2%, 3.5%, and 7%), at a voltage of 1 kV, and a driving frequency of 20 kHz. It concluded that the major ion products of Ar are Ar{sup +} and Ar{sub 2}{sup +}. Ar{sup +} is the most important positive ions, followed by Ar{sub 2}{sup +}. It is shown that the NH{sup +} density is smaller than that of the other ammonia ions. The density of NH{sub 4}{sup +} is more than that of the other ammonia ions when the ammonia concentration increased. The diffuse mode can be established after the discharge was ignited, and the mode changes to filamentary mode with an increase in ammonia concentration.

  4. The Origin and Coupling Mechanism of the Magnetoelectric Effect in TM Cl 2 -4SC(NH 2 ) 2 ( TM = Ni and Co)

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Mun, Eundeok; Wilcox, Jason; Manson, Jamie L.; Scott, Brian; Tobash, Paul; Zapf, Vivien S.

    2014-01-01

    Most research on multiferroics and magnetoelectric effects to date has focused on inorganic oxides. Molecule-based materials are a relatively new field in which to search for magnetoelectric multiferroics and to explore new coupling mechanisms between electric and magnetic order. We present magnetoelectric behavior in NiCl 2 -4SC(NH 2 ) 2 (DTN) and CoCl 2 -4SC(NH 2 ) 2 (DTC). These compounds form tetragonal structures where the transition metal ion (Ni or Co) is surrounded by four electrically polar thiourea molecules [SC(NH 2 ) 2 ]. By tracking the magnetic and electric properties of these compounds as a function ofmore » magnetic field, we gain insights into the coupling mechanism by observing that, in DTN, the electric polarization tracks the magnetic ordering, whereas in DTC it does not. For DTN, all electrically polar thiourea molecules tilt in the same direction along the c -axis, breaking spatial-inversion symmetry, whereas, for DTC, two thiourea molecules tilt up and two tilt down with respect to c -axis, perfectly canceling the net electrical polarization. Thus, the magnetoelectric coupling mechanism in DTN is likely a magnetostrictive adjustment of the thiourea molecule orientation in response to magnetic order.« less

  5. Electron-hole diffusion lengths >175 μm in solution-grown CH3NH3PbI3 single crystals

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Dong, Qingfeng; Fang, Yanjun; Shao, Yuchuan; Mulligan, Padhraic; Qiu, Jie; Cao, Lei; Huang, Jinsong

    2015-02-27

    Long, balanced electron and hole diffusion lengths greater than 100 nanometers in the polycrystalline organolead trihalide compound CH3NH3PbI3 are critical for highly efficient perovskite solar cells. We found that the diffusion lengths in CH3NH3PbI3 single crystals grown by a solution-growth method can exceed 175 micrometers under 1 sun (100 mW cm–2) illumination and exceed 3 millimeters under weak light for both electrons and holes. The internal quantum efficiencies approach 100% in 3-millimeter-thick single-crystal perovskite solar cells under weak light. These long diffusion lengths result from greater carrier mobility, longer lifetime, and much smaller trap densities in the single crystals thanmore » in polycrystalline thin films. As a result, the long carrier diffusion lengths enabled the use of CH3NH3PbI3 in radiation sensing and energy harvesting through the gammavoltaic effect, with an efficiency of 3.9% measured with an intense cesium-137 source.« less

  6. Electron-hole diffusion lengths >175 μm in solution-grown CH3NH3PbI3 single crystals

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Dong, Qingfeng; Fang, Yanjun; Shao, Yuchuan; Mulligan, Padhraic; Qiu, Jie; Cao, Lei; Huang, Jinsong

    2015-02-27

    Long, balanced electron and hole diffusion lengths greater than 100 nanometers in the polycrystalline organolead trihalide compound CH3NH3PbI3 are critical for highly efficient perovskite solar cells. We found that the diffusion lengths in CH3NH3PbI3 single crystals grown by a solution-growth method can exceed 175 micrometers under 1 sun (100 mW cm–2) illumination and exceed 3 millimeters under weak light for both electrons and holes. The internal quantum efficiencies approach 100% in 3-millimeter-thick single-crystal perovskite solar cells under weak light. These long diffusion lengths result from greater carrier mobility, longer lifetime, and much smaller trap densities in the single crystals thanmore »in polycrystalline thin films. As a result, the long carrier diffusion lengths enabled the use of CH3NH3PbI3 in radiation sensing and energy harvesting through the gammavoltaic effect, with an efficiency of 3.9% measured with an intense cesium-137 source.« less

  7. Angular momentum exchange by gravitational torques and infall in the circumbinary disk of the protostellar system L1551 NE

    SciTech Connect (OSTI)

    Takakuwa, Shigehisa; Ho, Paul T. P. [Academia Sinica Institute of Astronomy and Astrophysics, P.O. Box 23-141, Taipei 10617, Taiwan (China); Saito, Masao [Joint ALMA Observatory, Ave. Alonso de Cordova 3107, Vitacura, Santiago (Chile); Saigo, Kazuya [ALMA Project Office, National Astronomical Observatory of Japan, Osawa 2-21-1, Mitaka, Tokyo 181-8588 (Japan); Matsumoto, Tomoaki [Faculty of Humanity and Environment, Hosei University, Chiyoda-ku, Tokyo 102-8160 (Japan); Lim, Jeremy [Department of Physics, University of Hong Kong, Pokfulam Road (Hong Kong); Hanawa, Tomoyuki, E-mail: takakuwa@asiaa.sinica.edu.tw [Center for Frontier Science, Chiba University, Inage-ku, Chiba 263-8522 (Japan)

    2014-11-20

    We report an ALMA observation of the Class I binary protostellar system L1551 NE in the 0.9 mm continuum, C{sup 18}O (3-2), and {sup 13}CO (3-2) lines at a ?1.6 times higher resolution and a ?6 times higher sensitivity than those of our previous SubMillimeter Array (SMA) observations, which revealed a r ? 300 AU scale circumbinary disk in Keplerian rotation. The 0.9 mm continuum shows two opposing U-shaped brightenings in the circumbinary disk and exhibits a depression between the circumbinary disk and the circumstellar disk of the primary protostar. The molecular lines trace non-axisymmetric deviations from Keplerian rotation in the circumbinary disk at higher velocities relative to the systemic velocity, where our previous SMA observations could not detect the lines. In addition, we detect inward motion along the minor axis of the circumbinary disk. To explain the newly observed features, we performed a numerical simulation of gas orbits in a Roche potential tailored to the inferred properties of L1551 NE. The observed U-shaped dust features coincide with locations where gravitational torques from the central binary system are predicted to impart angular momentum to the circumbinary disk, producing shocks and hence density enhancements seen as a pair of spiral arms. The observed inward gas motion coincides with locations where angular momentum is predicted to be lowered by the gravitational torques. The good agreement between our observation and model indicates that gravitational torques from the binary stars constitute the primary driver for exchanging angular momentum so as to permit infall through the circumbinary disk of L1551 NE.

  8. Quantum dynamics of solid Ne upon photo-excitation of a NO impurity: A Gaussian wave packet approach

    SciTech Connect (OSTI)

    Unn-Toc, W.; Meier, C.; Halberstadt, N.; Uranga-Pina, Ll.; Rubayo-Soneira, J.

    2012-08-07

    A high-dimensional quantum wave packet approach based on Gaussian wave packets in Cartesian coordinates is presented. In this method, the high-dimensional wave packet is expressed as a product of time-dependent complex Gaussian functions, which describe the motion of individual atoms. It is applied to the ultrafast geometrical rearrangement dynamics of NO doped cryogenic Ne matrices after femtosecond laser pulse excitation. The static deformation of the solid due to the impurity as well as the dynamical response after femtosecond excitation are analyzed and compared to reduced dimensionality studies. The advantages and limitations of this method are analyzed in the perspective of future applications to other quantum solids.

  9. Transfer mechanism in /sup 16/O+/sup 24/Mg and /sup 20/Ne+/sup 24/Mg elastic scattering

    SciTech Connect (OSTI)

    NING Ping-Zhi; GAO Cheng-Qun; HE Guo-Zhu

    1985-10-01

    The mechanism of transferring a cluster of nucleons between two colliding nuclei is considered to explain the backward angle oscillatory rise in the differential cross section of the elastic scattering between certain nuclei, such as /sup 16/O+/sup 24/Mg or /sup 20/Ne+/sup 24/Mg. The nuclear molecular orbit approximation theory is applied. For one-step transfer, if the parameter involved is assumed to be adjustable, the numerical calculations can be made to fit the experimental results naturally.

  10. 35 COFibE, Series A. U. S. ATOXIC ENERGY CCMMISSION r'C Cj NE# YORK OPERATIONS OFFICE

    Office of Legacy Management (LM)

    COFibE, Series A. - U. S. ATOXIC ENERGY CCMMISSION r'C Cj NE# YORK OPERATIONS OFFICE HEkLTH AND SAFETY DIVISION (Merril Eicsnbud, Dirsator) MONTHLY REPORT OF FIELD ACTIVITIES (This report%v,rs%~~~nth period) Indusorial Ii~iene Branoh m a . . 0 . . c . . . o W. B. Harris, Chief Radiation Branch . y y e 0e . e . e . . . . e . . . Hanson Blatz, Chief Fi:e and Accident Branch D e a o o . . . ..s . . B. J. Kehoe, Chief Medical Advioer, Dr. J. A. Quiglsy Siometrician, Dr. A. E. Brandt TABLF OF

  11. REPLY TO ATTN OF: NE-24 L SUBJECT: Authorization to Conduct Remedial Action at Vicinity Properties In Lodi,

    Office of Legacy Management (LM)

    HBS. - 2- United States Government '--Department of Energy | memorandum 4 ' It) |1~~~~~ e~~~~0i78 DATE: OCT 9 1984 REPLY TO ATTN OF: NE-24 L SUBJECT: Authorization to Conduct Remedial Action at Vicinity Properties In Lodi, New Jersey TO: J. LaGrone, Manager Oak Ridge Operations Office Based on the designation survey conducted by ORNL (Attachments 1-6), the following properties are being authorized for remedial action. It should be noted that the attached survey data are for designation purposes

  12. REP&V TO ATTNOF: NE-23 SUBJECT: Commercial Facilities Used by National Lead Company of Ohio in Support

    Office of Legacy Management (LM)

    x:Y" . .' 3023 I\ \ 'a' '. Unita? -&&s Coverament , ,Q,.l. ),&, ,(>.. Department of Energy riGmorandum / d6a 2/. $3 DATE: JL(L 2 8 ;;$5 co. /3 .-J/ co,/3 REP&V TO ATTNOF: NE-23 SUBJECT: Commercial Facilities Used by National Lead Company of Ohio in Support of FMPC Operations TO: Robert E. Lynch Procuremnent and Contracts Division, AD-42 Oak Ridge Operations Office The Division of Facility and Site Decommissioning Projects (DFSD) is responsible for managing the

  13. DOE-NE Light Water Reactor Sustainability Program and EPRI Long Term Operation Program … Joint Research & Development Plan

    Office of Environmental Management (EM)

    2-24562 Revision 4 DOE-NE Light Water Reactor Sustainability Program and EPRI Long Term Operations Program - Joint Research and Development Plan April 2015 U.S. Department of Energy Office of Nuclear Energy DISCLAIMER This information was prepared as an account of work sponsored by an agency of the U.S. Government. Neither the U.S. Government nor any agency thereof, nor any of their employees, makes any warranty, expressed or implied, or assumes any legal liability or responsibility for the

  14. Electric contributions to magnetic force microscopy response from graphene and MoS{sub 2} nanosheets

    SciTech Connect (OSTI)

    Li, Lu Hua Chen, Ying

    2014-12-07

    Magnetic force microscopy (MFM) signals have recently been detected from whole pieces of mechanically exfoliated graphene and molybdenum disulfide (MoS{sub 2}) nanosheets, and magnetism of the two nanomaterials was claimed based on these observations. However, non-magnetic interactions or artefacts are commonly associated with MFM signals, which make the interpretation of MFM signals not straightforward. A systematic investigation has been done to examine possible sources of the MFM signals from graphene and MoS{sub 2} nanosheets and whether the MFM signals can be correlated with magnetism. It is found that the MFM signals have significant non-magnetic contributions due to capacitive and electrostatic interactions between the nanosheets and conductive cantilever tip, as demonstrated by electric force microscopy and scanning Kevin probe microscopy analyses. In addition, the MFM signals of graphene and MoS{sub 2} nanosheets are not responsive to reversed magnetic field of the magnetic cantilever tip. Therefore, the observed MFM response is mainly from electric artefacts and not compelling enough to correlate with magnetism of graphene and MoS{sub 2} nanosheets.

  15. Ferromagnetic superexchange in insulating Cr2MoO6 by controlling orbital hybridization

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Zhu, M.; Do, D.; Dela Cruz, Clarina R.; Dun, Zhiling; Cheng, J. -G.; Goto, H.; Uwatoko, Yoshiya; Zou, T.; Zhou, Haidon D.; Mahanti, Subhendra D.; et al

    2015-09-11

    We report the magnetic and electronic structures of the newly synthesized inverse-trirutile compound Cr2MoO6. Despite the same crystal symmetry and similar bond-lengths and bond-angles to Cr2TeO6, Cr2MoO6 possesses a magnetic structure of the Cr2MoO6 type, different from that seen in Cr2TeO6. Ab-initio electronic structure calculations show that the sign and strength of the Cr-O-Cr exchange coupling is strongly influenced by the hybridization between Mo 4d and O 2p orbitals. This result further substantiates our recently proposed mechanism for tuning the exchange interaction between two magnetic atoms by modifying the electronic states of the non-magnetic atoms in the exchange path throughmore »orbital hybridization. This approach is fundamentally different from the conventional methods of controlling the exchange interaction by either carrier injection or through structural distortions.« less

  16. MoS{sub 2} functionalization for ultra-thin atomic layer deposited dielectrics

    SciTech Connect (OSTI)

    Azcatl, Angelica; McDonnell, Stephen; Santosh, K.C.; Peng, Xin; Dong, Hong; Qin, Xiaoye; Addou, Rafik; Lu, Ning; Kim, Moon J.; Cho, Kyeongjae; Wallace, Robert M.; Mordi, Greg I.; Kim, Jiyoung

    2014-03-17

    The effect of room temperature ultraviolet-ozone (UV-O{sub 3}) exposure of MoS{sub 2} on the uniformity of subsequent atomic layer deposition of Al{sub 2}O{sub 3} is investigated. It is found that a UV-O{sub 3} pre-treatment removes adsorbed carbon contamination from the MoS{sub 2} surface and also functionalizes the MoS{sub 2} surface through the formation of a weak sulfur-oxygen bond without any evidence of molybdenum-sulfur bond disruption. This is supported by first principles density functional theory calculations which show that oxygen bonded to a surface sulfur atom while the sulfur is simultaneously back-bonded to three molybdenum atoms is a thermodynamically favorable configuration. The adsorbed oxygen increases the reactivity of MoS{sub 2} surface and provides nucleation sites for atomic layer deposition of Al{sub 2}O{sub 3}. The enhanced nucleation is found to be dependent on the thin film deposition temperature.

  17. Magnetic Force Microscopy Study of Zr2Co11 -Based Nanocrystalline Materials: Effect of Mo Addition

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Yue, Lanping; Jin, Yunlong; Zhang, Wenyong; Sellmyer, David J.

    2015-01-01

    Tmore » he addition of Molybdenum was used to modify the nanostructure and enhance coercivity of rare-earth-free Zr2Co11-based nanocrystalline permanent magnets. he effect of Mo addition on magnetic domain structures of melt spun nanocrystalline Zr16Co84-xMox(x=0, 0.5, 1, 1.5, and 2.0) ribbons has been investigated. It was found that magnetic properties and local domain structures are strongly influenced by Mo doping. he coercivity of the samples increases with the increase in Mo content (x≤1.5). he maximum energy product(BH)maxincreases with increasingxfrom 0.5 MGOe forx=0to a maximum value of 4.2 MGOe forx=1.5. he smallest domain size with a relatively short magnetic correlation length of 128 nm and largest root-mean-square phase shiftΦrmsvalue of 0.66° are observed for thex=1.5. he optimal Mo addition promotes magnetic domain structure refinement and thus leads to a significant increase in coercivity and energy product in this sample.« less

  18. Equation of state of bcc-Mo by static volume compression to 410 GPa

    SciTech Connect (OSTI)

    Akahama, Yuichi; Hirao, Naohisa; Ohishi, Yasuo; Singh, Anil K.

    2014-12-14

    Unit cell volumes of Mo and Pt have been measured simultaneously to ≈400 GPa by x-ray powder diffraction using a diamond anvil cell and synchrotron radiation source. The body-centered cubic (bcc) phase of Mo was found to be stable up to 410 GPa. The equation of state (EOS) of bcc-Mo was determined on the basis of Pt pressure scale. A fit of Vinet EOS to the volume compression data gave K{sub 0} = 262.3(4.6) GPa, K{sub 0}′ = 4.55(16) with one atmosphere atomic volume V{sub 0} = 31.155(24) A{sup 3}. The EOS was in good agreement with the previous ultrasonic data within pressure difference of 2.5%–3.3% in the multimegabar range, though the EOS of Mo proposed from a shock compression experiment gave lower pressure by 7.2%–11.3% than the present EOS. The agreement would suggest that the Pt pressure scale provides an accurate pressure value in an ultra-high pressure range.

  19. Effect of mechanical strain on electronic properties of bulk MoS{sub 2}

    SciTech Connect (OSTI)

    Kumar, Sandeep Kumar, Jagdish Sastri, O. S. K. S.

    2015-05-15

    Ab-initio density functional theory based calculations of electronic properties of bulk and monolayer Molybdenum di-Sulfide (MoS{sub 2}) have been performed using all electron Full Potential Linearised Augmentad Plane Wave (FPLAPW) method using Elk code. We have used Generalised Gradient Approximation (GGA) for exchange and correlation functionals and performed calculaitons of Lattice parameters, Density Of States (DOS) and Band Structure (BS). Band structure calculations revealed that bulk MoS{sub 2} has indirect band gap of 0.97 eV and mono-layer MoS{sub 2} has direct band gap which has increased to 1.71 eV. These are in better agreement with experimental values as compared with the other calculations using pseudo-potential code. The effect of mechanical strain on the electronic properties of bulk MoS{sub 2} has also been studied. For the different values of compressive strain (varying from 2% to 8% in steps of 2%) along the c-axis, the corresponding DOS and BS are obtained. We observed that the band gap decreases by about 15% for every 2% increase in strain along the c-axis.

  20. On the combined gradient-stochastic plasticity model: Application to Mo-micropillar compression

    SciTech Connect (OSTI)

    Konstantinidis, A. A.; Zhang, X.; Aifantis, E. C.

    2015-02-17

    A formulation for addressing heterogeneous material deformation is proposed. It is based on the use of a stochasticity-enhanced gradient plasticity model implemented through a cellular automaton. The specific application is on Mo-micropillar compression, for which the irregularities of the strain bursts observed have been experimentally measured and theoretically interpreted through Tsallis' q-statistics.

  1. EIS-0475: Disposition of the Bannister Federal Complex, Kansas City, MO

    Broader source: Energy.gov [DOE]

    NNSA/DOE announces its intent to prepare an EIS for the disposition of the Bannister Federal Complex, Kansas City, MO. NNSA previously decided in a separate NEPA review (EA-1592) to relocate its operations from the Bannister Federal Complex to a newly constructed industrial campus eight miles from the current location.

  2. The carburization of transition metal molybdates (MxMoO?, M= Cu, Ni or Co) and the generation of highly active metal/carbide catalysts for CO? hydrogenation

    SciTech Connect (OSTI)

    Rodriguez, Jose A.; Xu, Wenqian; Ramirez, Pedro J.; Stachiola, Dario; Brito, Joaquin L.

    2015-05-06

    A new approach has been tested for the preparation of metal/Mo?C catalysts using mixed-metal oxide molybdates as precursors. Synchrotron-based in situ time-resolved X-ray diffraction was used to study the reduction and carburization processes of Cu?(MoO?)?(OH)?, a-NiMoO? and CoMoO?nH?O by thermal treatment under mixtures of hydrogen and methane. In all cases, the final product was ?-Mo?C and a metal phase (Cu, Ni, or Co), but the transition sequence varied with the different metals, and it could be related to the reduction potential of the Cu?, Ni? and Co? cations inside each molybdate. The synthesized Cu/Mo?C, Ni/Mo?C and Co/Mo?C catalysts were highly active for the hydrogenation of CO?. The metal/Mo?C systems exhibited large variations in the selectivity towards methanol, methane and CnH?n?? (n > 2) hydrocarbons depending on the nature of the supported metal and its ability to cleave C-O bonds. Cu/Mo?C displayed a high selectivity for CO and methanol production. Ni/Mo?C and Co/Mo?C were the most active catalysts for the activation and full decomposition of CO?, showing high selectivity for the production of methane (Ni case) and CnH?n?? (n > 2) hydrocarbons (Co case).

  3. Modeling of Interaction Layer Growth Between U-Mo Particles and an Al Matrix

    SciTech Connect (OSTI)

    Yeon Soo Kim; G. L. Hofman; Ho Jin Ryu; Jong Man Park; A. B. Robinson; D. M. Wachs

    2013-12-01

    Interaction layer growth between U-Mo alloy fuel particles and Al in a dispersion fuel is a concern due to the volume expansion and other unfavorable irradiation behavior of the interaction product. To reduce interaction layer (IL) growth, a small amount of Si is added to the Al. As a result, IL growth is affected by the Si content in the Al matrix. In order to predict IL growth during fabrication and irradiation, empirical models were developed. For IL growth prediction during fabrication and any follow-on heating process before irradiation, out-of-pile heating test data were used to develop kinetic correlations. Two out-of-pile correlations, one for the pure Al matrix and the other for the Al matrix with Si addition, respectively, were developed, which are Arrhenius equations that include temperature and time. For IL growth predictions during irradiation, the out-of-pile correlations were modified to include a fission-rate term to consider fission enhanced diffusion, and multiplication factors to incorporate the Si addition effect and the effect of the Mo content. The in-pile correlation is applicable for a pure Al matrix and an Al matrix with the Si content up to 8 wt%, for fuel temperatures up to 200 degrees C, and for Mo content in the range of 6 10wt%. In order to cover these ranges, in-pile data were included in modeling from various tests, such as the US RERTR-4, -5, -6, -7 and -9 tests and Koreas KOMO-4 test, that were designed to systematically examine the effects of the fission rate, temperature, Si content in Al matrix, and Mo content in U-Mo particles. A model converting the IL thickness to the IL volume fraction in the meat was also developed.

  4. Novel Processing of mo-si-b Intermetallics for improved efficiency of power systems

    SciTech Connect (OSTI)

    M.J. Kramer; O. Degirmen; A.J. Thom; M. Akinc

    2004-09-30

    Multiphase composite alloys based on the Mo-Si-B system are candidate materials for ultra-high temperature applications. In non load-bearing applications such as thermal barrier coatings or heat exchangers in fossil fuel burners, these materials may be ideally suited. Alloys based on the Mo{sub 5}Si{sub 3}B{sub x} phase (Tl phase) possess excellent oxidation resistance to at least 1600 C in synthetic air atmospheres. However, the ability of Tl-based alloys to resist aggressive combustion environments has not yet been determined. The present work seeks to investigate the resistance of these Mo-Si-B alloys to simulated combustion atmospheres. Material was pre-alloyed by combustion synthesis, and samples for testing were prepared by classic powder metallurgical processing techniques. Precursor material synthesized by self-heating-synthesis was sintered to densities exceeding 98% in an argon atmosphere at 1800 C. The approximate phase assemblage of the material was 57% Tl, 29% MoB, 14% MoSi{sub 2} (wt%). The alloy was oxidized from 1000-1100 C in flowing air containing water vapor at 18 Torr. At 1000 C the material achieved a steady state mass loss, and at 1100 C the material undergoes a steady state mass gain. The oxidation rate of these alloys in this temperature regime was accelerated by the presence of water vapor compared to oxidation in dry air. The results of microstructural analysis of the tested alloys will be discussed. Techniques and preliminary results for fabricating near-net-shaped parts will also be presented.

  5. MoS{sub 2}@ZnO nano-heterojunctions with enhanced photocatalysis and field emission properties

    SciTech Connect (OSTI)

    Tan, Ying-Hua; Yu, Ke Li, Jin-Zhu; Fu, Hao; Zhu, Zi-Qiang

    2014-08-14

    The molybdenum disulfide (MoS{sub 2})@ZnO nano-heterojunctions were successfully fabricated through a facile three-step synthetic process: prefabrication of the ZnO nanoparticles, the synthesis of MoS{sub 2} nanoflowers, and the fabrication of MoS{sub 2}@ZnO heterojunctions, in which ZnO nanoparticles were uniformly self-assembled on the MoS{sub 2} nanoflowers by utilizing polyethyleneimine as a binding agent. The photocatalytic activities of the composite samples were evaluated by monitoring the photodegradation of methylene blue (MB). Compared with pure MoS{sub 2} nanoflowers, the composites show higher adsorption capability in dark and better photocatalytic efficiency due to the increased specific surface area and improved electron-hole pair separation. After irradiation for 100?min, the remaining MB in solution is about 7.3%. Moreover, the MoS{sub 2}@ZnO heterojunctions possess enhanced field emission properties with lower turn-on field of 3.08?V ?m{sup ?1}and lower threshold field of 6.9?V ?m{sup ?1} relative to pure MoS{sub 2} with turn-on field of 3.65?V ?m{sup ?1} and threshold field of 9.03?V ?m{sup ?1}.

  6. Study of structure of the TiO{sub 2}MoO{sub 3} bilayer films by Raman spectroscopy

    SciTech Connect (OSTI)

    Santos, Elias de Barros; Sigoli, Fernando Aparecido; Mazali, Italo Odone

    2014-12-15

    Highlights: TiO{sub 2}MoO{sub 3} bilayer thin films were easily prepared by dip-coating technique. Ti and Mo metallo-organic compounds were used as source of its respective oxide. TiO{sub 2} in anatase phase and orthorhombic phase of ?-MoO{sub 3} were identified. The bilayer structure was investigated by Raman spectroscopy. - Abstract: In this work, TiO{sub 2}MoO{sub 3} films were easily prepared by dip-coating technique and metallo-organic decomposition process (MOD). Raman analyses indicate the formation of TiO{sub 2} in anatase phase and orthorhombic phase of ?-MoO{sub 3}. It was observed that the Raman bands intensities attributed to TiO{sub 2} and MoO{sub 3} oxides were dependent on the number of decompositiondeposition cycles (DDC). The different number of DDC generates films with different thicknesses and the Raman signal was sensitive to this variation. Raman analyses provided qualitative information about the bilayer structure of the bi-component TiO{sub 2}MoO{sub 3} films, which was confirmed by scanning electron microscopy. In this direction, the dip-coating technique and MOD process can be an efficient strategy to facile preparation of many samples to be used in applications.

  7. Forward fitting of experimental data from a NE213 neutron detector installed with the magnetic proton recoil upgraded spectrometer at JET

    SciTech Connect (OSTI)

    Binda, F. Ericsson, G.; Eriksson, J.; Hellesen, C.; Conroy, S.; Sundn, E. Andersson; Collaboration: JET-EFDA Team

    2014-11-15

    In this paper, we present the results obtained from the data analysis of neutron spectra measured with a NE213 liquid scintillator at JET. We calculated the neutron response matrix of the instrument combining MCNPX simulations, a generic proton light output function measured with another detector and the fit of data from ohmic pulses. For the analysis, we selected a set of pulses with neutral beam injection heating (NBI) only and we applied a forward fitting procedure of modeled spectral components to extract the fraction of thermal neutron emission. The results showed the same trend of the ones obtained with the dedicated spectrometer TOFOR, even though the values from the NE213 analysis were systematically higher. This discrepancy is probably due to the different lines of sight of the two spectrometers (tangential for the NE213, vertical for TOFOR). The uncertainties on the thermal fraction estimates were from 4 to 7 times higher than the ones from the TOFOR analysis.

  8. Theoretical study on strain induced variations in electronic properties of 2H-MoS{sub 2} bilayer sheets

    SciTech Connect (OSTI)

    Dong, Liang; Dongare, Avinash M.; Namburu, Raju R.; O'Regan, Terrance P.; Dubey, Madan

    2014-02-03

    The strain dependence of the electronic properties of bilayer sheets of 2H-MoS{sub 2} is studied using ab initio simulations based on density functional theory. An indirect band gap for bilayer MoS{sub 2} is observed for all variations of strain along the basal plane. Several transitions for the indirect band gap are observed for various strains for the bilayer structure. The variation of the band gap and the carrier effective masses for the holes and the electrons for the bilayer MoS{sub 2} structure under conditions of uniaxial strain, biaxial strain, as well as uniaxial stress is investigated.

  9. Regulatory Safety Issues in the Structural Design Criteria of ASME Section III Subsection NH and for Very High Temperatures for VHTR & GEN IV

    SciTech Connect (OSTI)

    William J. O’Donnell; Donald S. Griffin

    2007-05-07

    The objective of this task is to identify issues relevant to ASME Section III, Subsection NH [1], and related Code Cases that must be resolved for licensing purposes for VHTGRs (Very High Temperature Gas Reactor concepts such as those of PBMR, Areva, and GA); and to identify the material models, design criteria, and analysis methods that need to be added to the ASME Code to cover the unresolved safety issues. Subsection NH was originally developed to provide structural design criteria and limits for elevated-temperature design of Liquid Metal Fast Breeder Reactor (LMFBR) systems and some gas-cooled systems. The U.S. Nuclear Regulatory Commission (NRC) and its Advisory Committee for Reactor Safeguards (ACRS) reviewed the design limits and procedures in the process of reviewing the Clinch River Breeder Reactor (CRBR) for a construction permit in the late 1970s and early 1980s, and identified issues that needed resolution. In the years since then, the NRC and various contractors have evaluated the applicability of the ASME Code and Code Cases to high-temperature reactor designs such as the VHTGRs, and identified issues that need to be resolved to provide a regulatory basis for licensing. This Report describes: (1) NRC and ACRS safety concerns raised during the licensing process of CRBR , (2) how some of these issues are addressed by the current Subsection NH of the ASME Code; and (3) the material models, design criteria, and analysis methods that need to be added to the ASME Code and Code Cases to cover unresolved regulatory issues for very high temperature service.

  10. Exploiting parameter space in MOFs: a 20-fold enhancement of phosphate-ester hydrolysis with UiO-66-NH 2

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Katz, Michael J.; Moon, Su-Young; Mondloch, Joseph E.; Beyzavi, M. Hassan; Stephenson, Casey J.; Hupp, Joseph T.; Farha, Omar K.

    2015-02-24

    The hydrolysis of nerve agents is of primary concern due to the severe toxicity of these agents. Using a MOF-based catalyst (UiO-66), we have previously demonstrated that the hydrolysis can occur with relatively fast half-lives of 50 minutes. However, these rates are still prohibitively slow to be efficiently utilized for some practical applications (e.g., decontamination wipes used to clean exposed clothing/skin/vehicles). We thus turned our attention to derivatives of UiO-66 in order to probe the importance of functional groups on the hydrolysis rate. Three UiO-66 derivatives were explored; UiO-66-NO2 and UiO-66-(OH)2 showed little to no change in hydrolysis rate. However,more » UiO-66-NH2 showed a 20 fold increase in hydrolysis rate over the parent UiO-66 MOF. Half-lives of 1 minute were observed with this MOF. In order to probe the role of the amino moiety, we turned our attention to UiO-67, UiO-67-NMe2 and UiO-67-NH2. In these MOFs, the amino moiety is in close proximity to the zirconium node. We observed that UiO-67-NH2 is a faster catalyst than UiO-67 and UiO-67-NMe2. We conclude that the role of the amino moiety is to act as a proton-transfer agent during the catalytic cycle and not to hydrogen bond or to form a phosphorane intermediate.« less

  11. AMoRE: Collaboration for searches for the neutrinoless double-beta decay of the isotope of {sup 100}Mo with the aid of {sup 40}Ca{sup 100}MoO{sub 4} as a cryogenic scintillation detector

    SciTech Connect (OSTI)

    Khanbekov, N. D., E-mail: xanbekov@gmail.com [Institute of Theoretical and Experimental Physics (Russian Federation)

    2013-09-15

    The AMoRE (Advanced Mo based Rare process Experiment) Collaboration is planning to employ {sup 40}Ca{sup 100}MoO{sub 4} single crystals as a cryogenic Scintillation detector for studying the neutrinoless double-beta decay of the isotope {sup 100}Mo. A simultaneous readout of phonon and scintillation signals is performed in order to suppress the intrinsic background. The planned sensitivity of the experiment that would employ 100 kg of {sup 40}Ca{sup 100}MoO{sub 4} over five years of data accumulation would be T{sub 1/2}{sup 0{nu}} = 3 Multiplication-Sign 10{sup 26} yr, which corresponds to values of the effective Majorana neutrino mass in the range of Left-Pointing-Angle-Bracket m{sub {nu}} Right-Pointing-Angle-Bracket {approx} 0.02-0.06 eV.

  12. Synthesis and Evaluation of Cu/SAPO-34 Catalysts for NH3-SCR 2: Solid-state Ion Exchange and One-pot Synthesis

    SciTech Connect (OSTI)

    Gao, Feng; Walter, Eric D.; Washton, Nancy M.; Szanyi, Janos; Peden, Charles HF

    2015-01-01

    Cu-SAPO-34 catalysts are synthesized using two methods: solid-state ion exchange (SSIE) and one-pot synthesis. SSIE is conducted by calcining SAPO-34/CuO mixtures at elevated temperatures. For the one-pot synthesis method, Cu-containing chemicals (CuO and CuSO4) are added during gel preparation. A high-temperature calcination step is also needed for this method. Catalysts are characterized with surface area/pore volume measurements, temperature programmed reduction (TPR), electron paramagnetic resonance (EPR) and nuclear magnetic resonance (NMR) spectroscopies, and scanning electron microscopy (SEM). Catalytic properties are examined using standard ammonia selective catalytic reduction (NH3-SCR) and ammonia oxidation reactions. In Cu-SAPO-34 samples formed using SSIE, Cu presents both as isolated Cu2+ ions and unreacted CuO. The former is highly active and selective in NH3-SCR, while the latter catalyzes a side reaction; notably, the non-selective oxidation of NH3 above 350 C. Using the one-pot method followed by a high-temperature aging treatment, it is possible to form Cu SAPO-34 samples with predominately isolated Cu2+ ions at low Cu loadings. However at much higher Cu loadings, isolated Cu2+ ions that bind weakly with the CHA framework and CuO clusters also form. These Cu moieties are very active in catalyzing non-selective NH3 oxidation above 350 C. Low-temperature reaction kinetics indicate that Cu-SAPO-34 samples formed using SSIE have core-shell structures where Cu is enriched in the shell layers; while Cu is more evenly distributed within the one-pot samples. Reaction kinetics also suggest that at low temperatures, the local environment next to Cu2+ ion centers plays little role on the overall catalytic properties. The authors gratefully acknowledge the US Department of Energy (DOE), Energy Efficiency and Renewable Energy, Vehicle Technologies Office for the support of this work. The research described in this paper was performed at the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOEs Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is operated for the US DOE by Battelle under contract number DE-AC05-76RL01830. The authors also thank Shari Li (PNNL) for surface area/pore volume measurements, and Bruce W. Arey (PNNL) for SEM measurements. Discussions with Drs. A. Yezerets, K. Kamasamudram, J.H. Li, N. Currier and J.Y. Luo from Cummins, Inc. and H.Y. Chen and H. Hess from Johnson-Matthey are greatly appreciated.

  13. Effects of gaseous NH{sub 3} and SO{sub 2} on the concentration profiles of PCDD/F in flyash under post-combustion zone conditions

    SciTech Connect (OSTI)

    Hajizadeh, Yaghoub; Onwudili, Jude A.; Williams, Paul T.

    2012-07-15

    Highlights: Black-Right-Pointing-Pointer Influence of NH{sub 3} and SO{sub 2} on 2378-PCDD/F in flyash and flue gases was investigated. Black-Right-Pointing-Pointer NH{sub 3} decreased the concentration of PCDD and PCDF by 34-75% in the flyash. Black-Right-Pointing-Pointer NH{sub 3} decreased the concentration of PCDD and PCDF by 21-40% from the flue gases. Black-Right-Pointing-Pointer SO{sub 2} led to 99% PCDD and 93% PCDF reductions in the flyash. Black-Right-Pointing-Pointer SO{sub 2} led to 89% PCDD and 76% PCDF reductions in the flue gases. - Abstract: The influence of gaseous ammonia and sulphur dioxide on the formation of 2378-substituted PCDD/F on a reference flyash from a municipal waste incinerator has been investigated using a laboratory scale fixed-bed reactor. The reference flyash samples (BCR-490) was reacted under a simulated flue gas stream at temperatures of 225 and 375 Degree-Sign C for 96 h. The experiments were carried out in two series: first with simulated flue gas alone, and then with injection of NH{sub 3} or SO{sub 2} gas into the flue gas just before the reactor inlet. It was found that the injection of gaseous ammonia into the flue gas could decrease the concentration of both PCDD and PCDF by 34-75% from the solid phase and by 21-40% from the gas phase. Converting the results to I-TEQ values, it could reduce the total I-TEQ values of PCDD and PCDF in the sum of the flyash and exhaust flue gas by 42-75% and 24-57% respectively. The application of SO{sub 2} led to 99% and 93% reductions in the PCDD and PCDF average congener concentrations, respectively in the solid phase. In the gas phase, the total reductions were 89% and 76% for PCDD and PCDF, respectively. Moreover, addition of SO{sub 2} reduced the total I-TEQ value of PCDD and PCDF in the flyash and exhaust flue gas together by 60-86% and 72-82% respectively. Sulphur dioxide was more effective than ammonia in suppressing PCDD/F formation in flyash under the conditions investigated.

  14. Microstructure evolution in solution treated Ti15Mo alloy processed by high pressure torsion

    SciTech Connect (OSTI)

    Jane?ek, Milo; ?ek, Jakub; Strsk, Josef; Vclavov, Kristna; Hruka, Petr; Polyakova, Veronika; Gatina, Svetlana; Semenova, Irina

    2014-12-15

    Microstructure evolution and mechanical properties of ultra-fine grained Ti15Mo alloy processed by high pressure torsion were investigated. High pressure torsion straining resulted in strong grain refinement as-observed by transmission electron microscopy. Microhardness and light microscopy showed two distinct regions (i) a central region with radial material flow and low microhardness (340 HV) and (ii) a peripheral region with rotational material flow and high microhardness (430 HV). Positron annihilation spectroscopy showed that the only detectable defects in the material are dislocations, whose density increases with the radial distance and the number of high pressure torsion revolutions. The local chemical environment around defects does not differ significantly from the average composition. - Highlights: Beta-Ti alloy Ti15Mo was processed by high pressure torsion (HPT). Lateral inhomogeneity of the microstructure and microhardness was found. Dislocations are the only lattice defects detectable by positron annihilation. Molybdenum is not preferentially segregated along dislocation cores.

  15. LANL Experience Rolling Zr-Clad LEU-10Mo Foils for AFIP-7

    SciTech Connect (OSTI)

    Hammon, Duncan L.; Clarke, Kester D.; Alexander, David J.; Kennedy, Patrick K.; Edwards, Randall L.; Duffield, Andrew N.; Dombrowski, David E.

    2015-05-29

    The cleaning, canning, rolling and final trimming of Low Enriched Uranium-10 wt. pct. Molybdenum (LEU-10Mo) foils for ATR (Advanced Test Reactor) fuel plates to be used in the AFIP-7 (ATR Full Size Plate In Center Flux Trap Position) experiments are summarized. Six Zr-clad foils were produced from two LEU-10Mo castings supplied to Los Alamos National Laboratory (LANL) by Y-12 National Security Complex. Details of cleaning and canning procedures are provided. Hot- and cold-rolling results are presented, including rolling schedules, images of foils in-process, metallography and local compositions of regions of interest, and details of final foil dimensions and process yield. This report was compiled from the slides for the presentation of the same name given by Duncan Hammon on May 12, 2011 at the AFIP-7 Lessons Learned meeting in Salt Lake City, UT, with Los Alamos National Laboratory document number LA-UR 11-02898.

  16. Determination of the direct double- β -decay Q value of Zr 96 and atomic masses of Zr 90 <mo>-> 92 <mo>,> 94 <mo>,> 96 and Mo 92 <mo>,> 94 <mo>-> 98 <mo>,> 100

    SciTech Connect (OSTI)

    Gulyuz, K.; Ariche, J.; Bollen, G.; Bustabad, S.; Eibach, M.; Izzo, C.; Novario, S. J.; Redshaw, M.; Ringle, R.; Sandler, R.; Schwarz, S.; Valverde, A. A.

    2015-05-06

    Experimental searches for neutrinoless double-β decay offer one of the best opportunities to look for physics beyond the standard model. Detecting this decay would confirm the Majorana nature of the neutrino, and a measurement of its half-life can be used to determine the absolute neutrino mass scale. Important to both tasks is an accurate knowledge of the Q value of the double-β decay. The LEBIT Penning trap mass spectrometer was used for the first direct experimental determination of the ⁹⁶Zr double-β decay Q value: Qββ=3355.85(15) keV. This value is nearly 7 keV larger than the 2012 Atomic Mass Evaluation [M. Wang et al., Chin. Phys. C 36, 1603 (2012)] value and one order of magnitude more precise. The 3-σ shift is primarily due to a more accurate measurement of the ⁹⁶Zr atomic mass: m(⁹⁶Zr)=95.90827735(17) u. Using the new Q value, the 2νββ-decay matrix element, |M|, is calculated. Improved determinations of the atomic masses of all other zirconium (90-92,94,96Zr) and molybdenum (92,94-98,100Mo) isotopes using both ¹²C₈ and ⁸⁷Rb as references are also reported.

  17. Co-Rolled U10Mo/Zirconium-Barrier-Layer Monolithic Fuel Foil Fabrication Process

    SciTech Connect (OSTI)

    G. A. Moore; M. C. Marshall

    2010-01-01

    Integral to the current UMo fuel foil processing scheme being developed at Idaho National Laboratory (INL) is the incorporation of a zirconium barrier layer for the purpose of controlling UMo-Al interdiffusion at the fuel-meat/cladding interface. A hot co-rolling process is employed to establish a ~25-m-thick zirconium barrier layer on each face of the ~0.3-mm-thick U10Mo fuel foil.

  18. NNSA Works to Establish a Reliable Supply of Mo-99 Produced Without Highly

    National Nuclear Security Administration (NNSA)

    Enriched Uranium | National Nuclear Security Administration Works to Establish a Reliable Supply of Mo-99 Produced Without Highly Enriched Uranium | National Nuclear Security Administration Facebook Twitter Youtube Flickr RSS People Mission Managing the Stockpile Preventing Proliferation Powering the Nuclear Navy Emergency Response Recapitalizing Our Infrastructure Countering Nuclear Terrorism About Our Programs Our History Who We Are Our Leadership Our Locations Budget Our Operations

  19. Tribological properties of self-lubricating NiAl/Mo-based composites containing AgVO{sub 3} nanowires

    SciTech Connect (OSTI)

    Liu, Eryong; Gao, Yimin; Bai, Yaping; Yi, Gewen; Wang, Wenzhen; Zeng, Zhixiang; Jia, Junhong

    2014-11-15

    Silver vanadate (AgVO{sub 3}) nanowires were synthesized by hydrothermal method and self-lubricating NiAl/Mo-AgVO{sub 3} composites were fabricated by powder metallurgy technique. The composition and microstructure of NiAl/Mo-based composites were characterized and the tribological properties were investigated from room temperature to 900 C. The results showed that NiAl/Mo-based composites were consisted of nanocrystalline B2 ordered NiAl matrix, Al{sub 2}O{sub 3}, Mo{sub 2}C, metallic Ag and vanadium oxide phase. The appearance of metallic Ag and vanadium oxide phase can be attributed to the decomposition of AgVO{sub 3} during sintering. Wear testing results confirmed that NiAl/Mo-based composites have excellent tribological properties over a wide temperature range. For example, the friction coefficient and wear rate of NiAl/Mo-based composites containing AgVO{sub 3} were significantly lower than the composites containing only metallic Mo or AgVO{sub 3} lubricant when the temperature is above 300 C, which can be attributed to the synergistic lubricating action of metallic Mo and AgVO{sub 3} lubricants. Furthermore, Raman results indicated that the composition on the worn surface of NiAl-based composites was self-adjusted after wear testing at different temperatures. For example, Ag{sub 3}VO{sub 4} and Fe{sub 3}O{sub 4} lubricants were responsible for the improvement of tribological properties at 500 C, AgVO{sub 3}, Ag{sub 3}VO{sub 4} and molybdate for 700 C, and AgVO{sub 3} and molybdate for 900 C of NiAl-based composites with the addition of metallic Mo and AgVO{sub 3}. - Highlights: NiAl/Mo-AgVO{sub 3} nanocomposites were prepared by mechanical alloying and sintering. AgVO{sub 3} decomposed to metallic Ag and vanadium oxide during the sintering process. NiAl/Mo-AgVO{sub 3} exhibited superior tribological properties at a board temperature range. Phase composition on the worn surface was varied with temperatures. Self-adjusted action was responsible for the improvement of tribological properties.

  20. Study on Shielding Requirements for Radioactive Waste Transportation in a Mo-99 Production Plant - 13382

    SciTech Connect (OSTI)

    Melo Rego, Maria Eugenia de; Kazumi Sakata, Solange; Vicente, Roberto; Hiromoto, Goro [Nuclear and Energy Research Institute, IPEN-CNEN/SP (Brazil)] [Nuclear and Energy Research Institute, IPEN-CNEN/SP (Brazil)

    2013-07-01

    Brazil is currently planning to produce {sup 99}Mo from fission of low enriched uranium (LEU) targets. The planned end of irradiation activity of {sup 99}Mo is about 185 TBq (5 kCi) per week to meet the present domestic demand of {sup 99m}Tc generators. The radioactive wastes from the production plant will be transferred to a waste treatment facility at the same site. The total activity of the actinides, fission and activation products present in the wastes can be predicted based on the yields of fission and activation data for the irradiation conditions, such as composition and mass of uranium targets, irradiation time, neutron flux, production schedule, etc., which were in principle already established by the project management. The transportation of the wastes from the production plant to the treatment facility will be done by means of special shielded packages. An assessment of the shielding required for the packages has been done and the results are presented here, aiming at contributing to the design of the waste management facility for the {sup 99}Mo production plant. (authors)

  1. Exciton-dominated dielectric function of atomically thin MoS2 films

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Yu, Yiling; Yu, Yifei; Cai, Yongqing; Li, Wei; Gurarslan, Alper; Peelaers, Hartwin; Aspnes, David E.; Van de Walle, Chris G.; Nguyen, Nhan V.; Zhang, Yong -Wei; et al

    2015-11-24

    We systematically measure the dielectric function of atomically thin MoS2 films with different layer numbers and demonstrate that excitonic effects play a dominant role in the dielectric function when the films are less than 5–7 layers thick. The dielectric function shows an anomalous dependence on the layer number. It decreases with the layer number increasing when the films are less than 5–7 layers thick but turns to increase with the layer number for thicker films. We show that this is because the excitonic effect is very strong in the thin MoS2 films and its contribution to the dielectric function maymore » dominate over the contribution of the band structure. We also extract the value of layer-dependent exciton binding energy and Bohr radius in the films by fitting the experimental results with an intuitive model. The dominance of excitonic effects is in stark contrast with what reported at conventional materials whose dielectric functions are usually dictated by band structures. Lastly, the knowledge of the dielectric function may enable capabilities to engineer the light-matter interactions of atomically thin MoS2 films for the development of novel photonic devices, such as metamaterials, waveguides, light absorbers, and light emitters.« less

  2. Electrical properties of a-C:Mo films produced by dual-cathode filtered cathodic arc plasma deposition

    SciTech Connect (OSTI)

    Sansongsiri, Sakon; Anders, Andre; Yodsombat, Banchob

    2008-01-20

    Molybdenum-containing amorphous carbon (a-C:Mo) thin films were prepared using a dual-cathode filtered cathodic arc plasma source with a molybdenum and a carbon (graphite) cathode. The Mo content in the films was controlled by varying the deposition pulse ratio of Mo and C. Film sheet resistance was measured in situ at process temperature, which was close to room temperature, as well as ex situ as a function of temperature (300-515 K) in ambient air. Film resistivity and electrical activation energy were derived for different Mo and C ratios and substrate bias. Film thickness was in the range 8-28 nm. Film resistivity varied from 3.55x10-4 Omega m to 2.27x10-6 Omega m when the Mo/C pulse ratio was increased from 0.05 to 0.4, with no substrate bias applied. With carbon-selective bias, the film resistivity was in the range of 4.59x10-2 and 4.05 Omega m at a Mo/C pulse ratio of 0.05. The electrical activation energy decreased from 3.80x10-2 to 3.36x10-4 eV when the Mo/C pulse ratio was increased in the absence of bias, and from 0.19 to 0.14 eV for carbon-selective bias conditions. The resistivity of the film shifts systematically with the amounts of Mo and upon application of substrate bias voltage. The intensity ratio of the Raman D-peak and G-peak (ID/IG) correlated with the pre-exponential factor (sigma 0) which included charge carrier density and density of states.

  3. Superconducting and structural properties of {delta}-MoC{sub 0.681} cubic molybdenum carbide phase

    SciTech Connect (OSTI)

    Sathish, C.I. [Graduate School of Chemical Sciences and Engineering, Hokkaido University, Sapporo, Hokkaido 060-0810 (Japan) [Graduate School of Chemical Sciences and Engineering, Hokkaido University, Sapporo, Hokkaido 060-0810 (Japan); Superconducting Properties Unit, National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044 (Japan); Guo, Yanfeng, E-mail: GUO.Yanfeng@nims.go.jp [Superconducting Properties Unit, National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044 (Japan)] [Superconducting Properties Unit, National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044 (Japan); Wang, Xia [Graduate School of Chemical Sciences and Engineering, Hokkaido University, Sapporo, Hokkaido 060-0810 (Japan) [Graduate School of Chemical Sciences and Engineering, Hokkaido University, Sapporo, Hokkaido 060-0810 (Japan); Superconducting Properties Unit, National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044 (Japan); Tsujimoto, Yoshihiro [International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044 (Japan)] [International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044 (Japan); Li, Jun [Graduate School of Chemical Sciences and Engineering, Hokkaido University, Sapporo, Hokkaido 060-0810 (Japan) [Graduate School of Chemical Sciences and Engineering, Hokkaido University, Sapporo, Hokkaido 060-0810 (Japan); Superconducting Properties Unit, National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044 (Japan); Zhang, Shoubao [International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044 (Japan)] [International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044 (Japan); Matsushita, Yoshitaka [Synchrotron X-ray Station at SPring-8, National Institute for Materials Science, 1-1-1 Kouto, Sayo-cho, Hyogo 679-5148 (Japan)] [Synchrotron X-ray Station at SPring-8, National Institute for Materials Science, 1-1-1 Kouto, Sayo-cho, Hyogo 679-5148 (Japan); Shi, Youguo; Tian, Huanfang; Yang, Huaixin; Li, Jianqi [Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190 (China)] [Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190 (China); Yamaura, Kazunari, E-mail: YAMAURA.Kazunari@nims.go.jp [Graduate School of Chemical Sciences and Engineering, Hokkaido University, Sapporo, Hokkaido 060-0810 (Japan) [Graduate School of Chemical Sciences and Engineering, Hokkaido University, Sapporo, Hokkaido 060-0810 (Japan); Superconducting Properties Unit, National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044 (Japan)

    2012-12-15

    The superconducting and lattice properties of {delta}-MoC{sub 0.681} were studied by electromagnetic measurements, synchrotron X-ray diffraction, neutron diffraction, and electron diffraction. The superconducting properties (T{sub c}=12 K) of {delta}-MoC{sub 0.681} were well characterized by a weak coupling model. The carbon vacancies present in the host cubic structure were found to be robust, although the material was synthesized from stoichiometric carbon and Mo powder under a high-pressure of 6 GPa. A thermodynamically-stable structure with ordered vacancies did not account for the robust features of {delta}-MoC{sub 0.681} since the vacancies are unlikely to be ordered in long range in the host structure. A model based on inherent phonon instability theoretically predicted for a stoichiometric MoC phase might be responsible for the robust features of {delta}-MoC{sub 0.681}. - Graphical Abstract: The cubic molybdenum carbide shows an excellent superconductivity with robust carbon vacancies. Inherent phonon instability theoretically predicted for a stoichiometric MoC phase might be responsible for the vacancies rather than a thermodynamically-stable structure with vacancies ordering. Highlights: Black-Right-Pointing-Pointer The 12 K superconductivity is well characterized by a weakly coupling model. Black-Right-Pointing-Pointer Carbon vacancies are robust and disordered in the cubic host structure. Black-Right-Pointing-Pointer Inherent phonon instability might be responsible for the robust carbon vacancies in {delta}-MoC{sub 0.681}.

  4. DOE-NE Light Water Reactor Sustainability Program and EPRI Long-Term Operations Program. Joint Research and Development Plan

    SciTech Connect (OSTI)

    Williams, Don

    2014-04-01

    Nuclear power has contributed almost 20% of the total amount of electricity generated in the United States over the past two decades. High capacity factors and low operating costs make nuclear power plants (NPPs) some of the most economical power generators available. Further, nuclear power remains the single largest contributor (nearly 70%) of non-greenhouse gas-emitting electric power generation in the United States. Even when major refurbishments are performed to extend operating life, these plants continue to represent cost-effective, low-carbon assets to the nation’s electrical generation capability. By the end of 2014, about one-third of the existing domestic fleet will have passed their 40th anniversary of power operations, and about one-half of the fleet will reach the same 40-year mark within this decade. Recognizing the challenges associated with pursuing extended service life of commercial nuclear power plants, the U.S. Department of Energy’s (DOE) Office of Nuclear Energy (NE) and the Electric Power Research Institute (EPRI) have established separate but complementary research and development programs (DOE-NE’s Light Water Reactor Sustainability [LWRS] Program and EPRI’s Long-Term Operations [LTO] Program) to address these challenges. To ensure that a proper linkage is maintained between the programs, DOE-NE and EPRI executed a memorandum of understanding in late 2010 to “establish guiding principles under which research activities (between LWRS and LTO) could be coordinated to the benefit of both parties.” This document represents the third annual revision to the initial version (March 2011) of the plan as called for in the memorandum of understanding.

  5. Using the X-FEL to photo-pump X-ray laser transitions in He-like Ne

    SciTech Connect (OSTI)

    Nilsen, J; Rohringer, N

    2011-08-30

    Nearly four decades ago H-like and He-like resonantly photo-pumped laser schemes were proposed for producing X-ray lasers. However, demonstrating these schemes in the laboratory has proved to be elusive because of the difficulty of finding a strong resonant pump line. With the advent of the X-ray free electron laser (X-FEL) at the SLAC Linac Coherent Light Source (LCLS) we now have a tunable X-ray laser source that can be used to replace the pump line in previously proposed laser schemes and allow researchers to study the physics and feasibility of resonantly photo-pumped laser schemes. In this paper we use the X-FEL at 1174 eV to photo-pump the singly excited 1s2p state of He-like Ne to the doubly excited 2p3p state and model gain on the 2p3p-2p2s transition at 175 eV and the 2p3p-1s3p transition at 1017 eV. One motivation for studying this scheme is to explore possible quenching of the gain due to strong non-linear coupling effects from the intense X-FEL beam We compare this scheme with photo-pumping the He-like Ne ground state to the 1s3p singly excited state followed by lasing on the 3p-2s and 3d-2p transitions at 158 and 151 eV. Experiments are being planned at LCLS to study these laser processes and coherent quantum effects.

  6. Low-frequency 1/f noise in MoS{sub 2} transistors: Relative contributions of the channel and contacts

    SciTech Connect (OSTI)

    Renteria, J.; Jiang, C.; Samnakay, R.; Rumyantsev, S. L.; Goli, P.; Balandin, A. A.; Shur, M. S.

    2014-04-14

    We report on the results of the low-frequency (1/f, where f is frequency) noise measurements in MoS{sub 2} field-effect transistors revealing the relative contributions of the MoS{sub 2} channel and Ti/Au contacts to the overall noise level. The investigation of the 1/f noise was performed for both as fabricated and aged transistors. It was established that the McWhorter model of the carrier number fluctuations describes well the 1/f noise in MoS{sub 2} transistors, in contrast to what is observed in graphene devices. The trap densities extracted from the 1/f noise data for MoS{sub 2} transistors, are 2??10{sup 19}?eV{sup ?1}cm{sup ?3} and 2.5??10{sup 20}?eV{sup ?1}cm{sup ?3} for the as fabricated and aged devices, respectively. It was found that the increase in the noise level of the aged MoS{sub 2} transistors is due to the channel rather than the contact degradation. The obtained results are important for the proposed electronic applications of MoS{sub 2} and other van der Waals materials.

  7. Preparation of Al{sub 2}O{sub 3}/Mo nanocomposite powder via chemical route and spray drying

    SciTech Connect (OSTI)

    Lo, M.; Cheng, F.; Wei, W.J.

    1996-08-01

    A route to prepare nanometer-sized Mo particulates in Al{sub 2}O{sub 3} was attempted by a combination of solution reactions in molecular scale and forcing precipitation by a spray-drying technique. MoO{sub 3} was first dissolved in ammonia water and then added in the slurry with high purity, submicrometer Al{sub 2}O{sub 3} powder. Mixed suspension was spray-dried, and then the dried granules were reduced by hydrogen gas and further hot-pressing to a bulky composite at various temperatures. Dissolution of Mo oxide, adsorption reactions on alumina surface, and surface potential of alumina particles in homogeneous ammonia suspension were studied. Characterization of the granules, including compactability, flowing properties, surface morphology, grain growth of Mo and Al{sub 2}O{sub 3}, and mixing homogeneity, were examined. Homogeneity of the spray-dried granules was determined by the calculation of mixing index and the observation of the microstructure of sintered body. The existence of intergranular, intragranular, and nanosized Mo particulates within Al{sub 2}O{sub 3} grains was observed by transmission electron microscopy (TEM). All the evidences revealed that homogeneous composites with nanometer-sized Mo had been successfully prepared by this attempt with the proposed chemical route and following spray-drying process. {copyright}{ital 1996 Materials Research Society.}

  8. Quantum wells on 3C-SiC/NH-SiC heterojunctions. Calculation of spontaneous polarization and electric field strength in experiments

    SciTech Connect (OSTI)

    Sbruev, I. S.; Sbruev, S. B.

    2010-10-15

    The results of experiments with quantum wells on 3C-SiC/4H-SiC and 3C-SiC/6H-SiC heterojunctions obtained by various methods are reconsidered. Spontaneous polarizations, field strengths, and energies of local levels in quantum wells on 3C-SiC/NH-SiC heterojunctions were calculated within a unified model. The values obtained are in agreement with the results of all considered experiments. Heterojunction types are determined. Approximations for valence band offsets on heterojunctions between silicon carbide polytypes and the expression for calculating local levels in quantum wells on the 3C-SiC/NH-SiC heterojunction are presented. The spontaneous polarizations and field strengths induced by spontaneous polarization on 3C-SiC/4H-SiC and 3C-SiC/6H-SiC heterojunctions were calculated as 0.71 and 0.47 C/m{sup 2} and 0.825 and 0.55 MV/cm, respectively.

  9. AFFECTS OF MECHANICAL MILLING AND METAL OXIDE ADDITIVES ON SORPTION KINETICS OF 1:1 LiNH2/MgH2 MIXTURE

    SciTech Connect (OSTI)

    Erdy, C.; Anton, D.; Gray, J.

    2010-12-08

    The destabilized complex hydride system composed of LiNH{sub 2}:MgH{sub 2} (1:1 molar ratio) is one of the leading candidates of hydrogen storage with a reversible hydrogen storage capacity of 8.1 wt%. A low sorption enthalpy of {approx}32 kJ/mole H{sub 2} was first predicted by Alapati et al. utilizing first principle density function theory (DFT) calculations and has been subsequently confirmed empirically by Lu et al. through differential thermal analysis (DTA). This enthalpy suggests that favorable sorption kinetics should be obtainable at temperatures in the range of 160 C to 200 C. Preliminary experiments reported in the literature indicate that sorption kinetics are substantially lower than expected in this temperature range despite favorable thermodynamics. Systematic isothermal and isobaric sorption experiments were performed using a Sievert's apparatus to form a baseline data set by which to compare kinetic results over the pressure and temperature range anticipated for use of this material as a hydrogen storage media. Various material preparation methods and compositional modifications were performed in attempts to increase the kinetics while lowering the sorption temperatures. This paper outlines the results of these systematic tests and describes a number of beneficial additions which influence kinetics as well as NH{sub 3} formation.

  10. Kinetic study of hydrogen evolution reaction on Ni{sub 30} Mo{sub 70}, Co{sub 30}Mo{sub 70}, Co{sub 30}Ni{sub 70} and Co{sub 10}Ni{sub 20}Mo{sub 70} alloy electrodes

    SciTech Connect (OSTI)

    Dominguez-Crespo, M.A.; Plata-Torres, M.; Torres-Huerta, A.M.; Arce-Estrada, E.M. . E-mail: earce@ipn.mx; Hallen-Lopez, J.M.

    2005-07-15

    The hydrogen evolution reaction on nanocrystalline Ni{sub 30}Mo{sub 70}, Co{sub 30}Mo{sub 70}, Co{sub 30}Ni{sub 70}, and Co{sub 10}Ni{sub 20}Mo{sub 70}, metallic powders prepared by mechanical alloying was investigated with linear polarization and ac impedance methods, in 30 wt.% KOH aqueous solution at room temperature. The formation process and structural properties of these nanocrystalline materials were characterized by X-ray diffraction and transmission electron microscopy. Alloyed powders showed the presence of two phases: an fcc solid solution and intermetallic compounds of Ni, Co and Mo. Based on polarization and ac impedance measurements, an improved electrocatalytic activity for hydrogen evolution reaction was observed in mechanically alloyed Co{sub 30}Ni{sub 70} powders, which is slightly higher than milled metallic Ni powders.

  11. Application of the explicitly correlated coupled-cluster models CCSD(F12*) and CC3(F12*) to the hyperpolarizability of the Ne atom

    SciTech Connect (OSTI)

    Hanauer, Matthias; Khn, Andreas

    2015-01-22

    This work demonstrates the performance of the recently proposed explicitly correlated coupled-cluster method CCSD(F12*) and a new method using explicitly correlated triple excitations, CC3(F12*), in the calculation of the static ESHG hyperpolarizability of the Ne atom.

  12. Characterization of few-layer 1T-MoSe{sub 2} and its superior performance in the visible-light induced hydrogen evolution reaction

    SciTech Connect (OSTI)

    Gupta, Uttam; Naidu, B. S.; Maitra, Urmimala; Rao, C. N. R.; Singh, Anjali; Shirodkar, Sharmila N.; Waghmare, Umesh V.

    2014-09-01

    Based on earlier results on the photocatalytic properties of MoS{sub 2}, the 1T form of MoSe{sub 2}, prepared by lithium intercalation and exfoliation of bulk MoSe{sub 2}, has been employed for the visible-light induced generation of hydrogen. 1T-MoSe{sub 2} is found to be superior to both 2H and 1T MoS{sub 2} as well as 2H-MoSe{sub 2} in producing hydrogen from water, the yield being in the 6075 mmol?h{sup ?1}?g{sup ?1} range with a turn over frequency of 1519 h{sup ?1}. First principles calculations reveal that 1T-MoSe{sub 2} has a lower work function than 2H-MoSe{sub 2} as well as 1T and 2H-MoS{sub 2}, making it easier to transfer an electron from 1T-MoSe{sub 2} for the production of H{sub 2}.

  13. A practical grinding-assisted dry synthesis of nanocrystalline NiMoO{sub 4} polymorphs for oxidative dehydrogenation of propane

    SciTech Connect (OSTI)

    Chen Miao; Wu Jialing; Liu Yongmei; Cao Yong; Guo Li; He Heyong; Fan Kangnian

    2011-12-15

    A practical two-stage reactive grinding-assisted pathway waste-free and cost-effective for the synthesis of NiMoO{sub 4} has been successfully developed. It was demonstrated that proper design in synthetic strategy for grinding plays a crucial role in determining the ultimate polymorph of NiMoO{sub 4}. Specifically, direct grinding (DG) of MoO{sub 3} and NiO rendered {alpha}-NiMoO{sub 4} after annealing, whereas sequential grinding (SG) of the two independently pre-ground oxides followed by annealing generated {beta}-NiMoO{sub 4} solid solution. Characterizations in terms of Raman and X-ray diffraction suggest the creation of {beta}-NiMoO{sub 4} precursor in the latter alternative is the key aspect for the formation of {beta}-NiMoO{sub 4}. The DG-derived {alpha}-NiMoO{sub 4} tested by oxidative dehydrogenation of propane exhibited superior activity in contrast to its analog synthesized via conventional coprecipitation. It is suggested that the favorable chemical composition facilely obtained via grinding in contrast to that by coprecipitation was essential for achieving a more selective production of propylene. - Graphical Abstract: Grinding-assisted synthesis of NiMoO{sub 4} offers higher and more reproducible activities in contrast to coprecipitation for oxidative dehydrogenation of propane, and both {alpha}- and {beta}-NiMoO{sub 4} can be synthesized. Highlights: Black-Right-Pointing-Pointer NiMoO{sub 4} was prepared through grinding-assisted pathway. Black-Right-Pointing-Pointer Direct/sequential grinding rendered {alpha}-, {beta}-NiMoO{sub 4}, respectively. Black-Right-Pointing-Pointer Grinding-derived {alpha}-NiMoO{sub 4} showed high and reproducible activity for oxidative dehydrogenation of propane.

  14. METALLICITIES, DUST, AND MOLECULAR CONTENT OF A QSO-DAMPED Ly{alpha} SYSTEM REACHING log N(H I) = 22: AN ANALOG TO GRB-DLAs

    SciTech Connect (OSTI)

    Guimaraes, R.; Noterdaeme, P.; Petitjean, P.; Ledoux, C.; Srianand, R.; Rahmani, H.; Lopez, S.

    2012-06-15

    We present the elemental abundance and H{sub 2} content measurements of a damped Ly{alpha} (DLA) system with an extremely large H I column density, log N(H I) (cm{sup -2}) = 22.0 {+-} 0.10, at z{sub abs} = 3.287 toward the QSO SDSS J081634+144612. We measure column densities of H{sub 2}, C I, C I*, Zn II, Fe II, Cr II, Ni II, and Si II from a high signal-to-noise and high spectral resolution VLT-UVES spectrum. The overall metallicity of the system is [Zn/H] = -1.10 {+-} 0.10 relative to solar. Two molecular hydrogen absorption components are seen at z = 3.28667 and 3.28742 (a velocity separation of Almost-Equal-To 52 km s{sup -1}) in rotational levels up to J = 3. We derive a total H{sub 2} column density of log N(H{sub 2}) (cm{sup -2}) = 18.66 and a mean molecular fraction of f = 2N(H{sub 2})/[2N(H{sub 2}) + N(H I)] = 10{sup -3.04{+-}0.37}, typical of known H{sub 2}-bearing DLA systems. From the observed abundance ratios we conclude that dust is present in the interstellar medium of this galaxy, with an enhanced abundance in the H{sub 2}-bearing clouds. However, the total amount of dust along the line of sight is not large and does not produce any significant reddening of the background QSO. The physical conditions in the H{sub 2}-bearing clouds are constrained directly from the column densities of H{sub 2} in different rotational levels, C I and C I*. The kinetic temperature is found to be T Almost-Equal-To 75 K and the particle density lies in the range n{sub H} = 50-80 cm{sup -3}. The neutral hydrogen column density of this DLA is similar to the mean H I column density of DLAs observed at the redshift of {gamma}-ray bursts (GRBs). We explore the relationship between GRB-DLAs and the high column density end of QSO-DLAs finding that the properties (metallicity and depletion) of DLAs with log N(H I) > 21.5 in the two populations do not appear to be significantly different.

  15. Annual Energy Outlook 2015 - Appendix F

    Gasoline and Diesel Fuel Update (EIA)

    8 Regional maps Figure F7. Coal demand regions Figure F7. Coal Demand Regions CT,MA,ME,NH,RI,VT OH 1. NE 3. S1 4. S2 5. GF 6. OH 7. EN AL,MS MN,ND,SD IA,NE,MO,KS TX,LA,OK,AR MT,WY,ID CO,UT,NV AZ,NM 9. AM 11. C2 12. WS 13. MT 14. CU 15. ZN WV,MD,DC,DE 2. YP Region Content Region Code NY,PA,NJ VA,NC,SC GA,FL IN,IL,MI,WI Region Content Region Code 14. CU 13. MT 16. PC 15. ZN 12. WS 11. C2 9. AM 5. GF 8. KT 4. S2 7. EN 6. OH 2. YP 1. NE 3. S1 10. C1 KY,TN 8. KT 16. PC AK,HI,WA,OR,CA 10. C1

  16. Origin and elimination of photocurrent hysteresis by fullerene passivation in CH3NH3PbI3 planar heterojunction solar cells

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Shao, Yuchuan; Xiao, Zhengguo; Bi, Cheng; Yuan, Yongbo; Huang, Jinsong

    2014-12-15

    The large photocurrent hysteresis observed in many organometal trihalide perovskite solar cells has become a major hindrance impairing the ultimate performance and stability of these devices, while its origin was unknown. Here we demonstrate the trap states on the surface and grain boundaries of the perovskite materials to be the origin of photocurrent hysteresis and that the fullerene layers deposited on perovskites can effectively passivate these charge trap states and eliminate the notorious photocurrent hysteresis. Fullerenes deposited on the top of the perovskites reduce the trap density by two orders of magnitude and double the power conversion efficiency of CH3NH3PbI3more » solar cells. As a result, the elucidation of the origin of photocurrent hysteresis and its elimination by trap passivation in perovskite solar cells provides important directions for future enhancements to device efficiency.« less

  17. Simplification of femtosecond transient absorption microscopy data from CH3NH3PbI3 perovskite thin films into decay associated amplitude maps

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Doughty, Benjamin; Simpson, Mary Jane; Yang, Bin; Xiao, Kai; Ma, Ying -Zhong

    2016-02-16

    This work aims to simplify multi-dimensional femtosecond transient absorption microscopy (TAM) data into decay associated amplitude maps that describe the spatial distributions of dynamical processes occurring on various characteristic timescales. Application of this method to TAM data obtained from a model methyl-ammonium lead iodide (CH3NH3PbI3) perovskite thin film allows us to simplify the dataset consisting of a 68 time-resolved images into 4 decay associated amplitude maps. These maps provide a simple means to visualize the complex electronic excited-state dynamics in this system by separating distinct dynamical processes evolving on characteristic timescales into individual spatial images. This approach provides new insightmore » into subtle aspects of ultrafast relaxation dynamics associated with excitons and charge carriers in the perovskite thin film, which have recently been found to coexist at spatially distinct locations.« less

  18. Qualifying composition dependent p and n self-doping in CH{sub 3}NH{sub 3}PbI{sub 3}

    SciTech Connect (OSTI)

    Wang, Qi; Shao, Yuchuan; Huang, Jinsong; Xie, Haipeng; Lyu, Lu; Liu, Xiaoliang; Gao, Yongli

    2014-10-20

    We report the observation of self-doping in perovskite. CH{sub 3}NH{sub 3}PbI{sub 3} was found to be either n- or p-doped by changing the ratio of methylammonium halide (MAI) and lead iodine (PbI{sub 2}) which are the two precursors for perovskite formation. MAI-rich and PbI{sub 2}-rich perovskite films are p and n self-doped, respectively. Thermal annealing can convert the p-type perovskite to n-type by removing MAI. The carrier concentration varied as much as six orders of magnitude. A clear correlation between doping level and device performance was also observed.

  19. Interaction of vacuum ultraviolet light with a low-k organosilicate glass film in the presence of NH{sub 3}

    SciTech Connect (OSTI)

    Behera, Swayambhu; Lee, Joe; Graves, David; Gaddam, Sneha; Pokharel, Sundari; Wilks, Justin; Pasquale, Frank; Kelber, Jeffry A.

    2010-07-19

    In situ x-ray photoemission spectroscopy (XPS) and ex situ Fourier transform infrared spectroscopy (FTIR) were used to characterize effects on organosilicate films of 147 nm irradiation in the presence of 10{sup -4} Torr NH{sub 3}. XPS and FTIR data indicate Si-O and Si-C bond scission, with nitridation only at Si sites. Photoirradiation causes the surface layer to become enriched in sp{sup 2} carbon. FTIR spectra of silanol formation upon exposure to ambient indicate reactive sites in the bulk have lifetimes of up to six days. XPS data indicate lifetimes of approxminutes for surface states. Nitrogen uptake passivates with longer exposure times, indicating surface densification.

  20. Martensitic transformation behaviors of rapidly solidified TiNiMo powders

    SciTech Connect (OSTI)

    Kim, Yeon-wook

    2012-10-15

    For the fabrication of bulk near-net-shape shape memory alloys and porous metallic biomaterials, consolidation of TiNiMo alloy powders is more useful than that of elemental powders of Ti, Ni and Mo. Ti{sub 50}Ni{sub 49.9}Mo{sub 0.1} shape memory alloy powders were prepared by gas atomization, and transformation temperatures and microstructures of those powders were investigated as a function of powder size. XRD analysis showed that the B2RB19 martensitic transformation occurred in powders smaller than 150 ?m. According to DSC analysis of the as-atomized powders, the B2R transformation temperature (T{sub R}) of the 2550 ?m powders was 18.4 C. The T{sub R} decreased with increasing powder size, however, the difference in T{sub R} between 2550 ?m powders and 100150 ?m powders is only 1 C. Evaluation of powder microstructures was based on SEM examination of the surface and the polished and etched powder cross sections and the typical images of the rapidly solidified powders showed cellular morphology. Porous cylindrical foams of 10 mm diameter and 1.5 mm length were fabricated by spark plasma sintering (SPS) at 800 C and 5 MPa. Finally these porous TiNi alloy samples are heat-treated for 1 h at 850 C, and then quenched in ice water. The bulk samples have 23% porosity and 4.6 g/cm{sup 3} density and their T{sub R} is 17.8 C.

  1. In Situ Time-Resolved Characterization of Novel Cu-MoO2 Catalysts During the Water-Gas Shift Reaction

    SciTech Connect (OSTI)

    Wen ,W.; Liu, J.; White, M.; Marinkovic, N.; Hanson, J.; Rodriguez, J.

    2007-01-01

    A novel and active Cu-MoO{sub 2} catalyst was synthesized by partial reduction of a precursor CuMoO{sub 4} mixed-metal oxide with CO or H{sub 2} at 200-250 C. The phase transformations of Cu-MoO{sub 2} during H{sub 2} reduction and the water-gas shift reaction could be followed by In situ time resolved XRD techniques. During the reduction process the diffraction pattern of the CuMoO{sub 4} collapsed and the copper metal lines were observed on an amorphous material background that was assigned to molybdenum oxides. During the first pass of water-gas shift (WGS) reaction, diffraction lines for Cu{sub 6}Mo{sub 5}O{sub 18} and MoO{sub 2} appeared around 350 C and Cu{sub 6}Mo{sub 5}O{sub 18} was further transformed to Cu/MoO{sub 2} at higher temperature. During subsequent passes, significant WGS catalytic activity was observed with relatively stable plateaus in product formation around 350, 400 and 500 C. The interfacial interactions between Cu clusters and MoO{sub 2} increased the water-gas shift catalytic activities at 350 and 400 C.

  2. Microsoft Word - chapter FeNiCrMo_ver4.doc

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Low-Alloy Ferritic Steels: Tempered Fe-Ni-Cr-Mo Alloys (code 1212) Prepared by: B.P. Somerday, Sandia National Laboratories Editors C. San Marchi B.P. Somerday Sandia National Laboratories This report may be updated and revised periodically in response to the needs of the technical community; up-to-date versions can be requested from the editors at the address given below or downloaded at http://www.ca.sandia.gov/matlsTechRef/ . The success of this reference depends upon feedback from the

  3. Corrosion and degradation of a polyurethane/Co-Ni-Cr-Mo pacemaker lead

    SciTech Connect (OSTI)

    Sung, P.; Fraker, A.C.

    1987-12-01

    An investigation to study changes in the metal surfaces and the polyurethane insulation of heart pacemaker leads under controlled in vitro conditions was conducted. A polyurethane (Pellethane 2363-80A)/Co-Ni-Cr-Mo (MP35N) wire lead was exposed in Hanks' physiological saline solution for 14 months and then analyzed using scanning electron microscopy, x-ray energy dispersive analysis, and small angle x-ray scattering. Results showed that some leakage of solution into the lead had occurred and changes were present on both the metal and the polyurethane surfaces.

  4. New operation strategy for driving the selectivity of NOx reduction to N2, NH3 or N2O during lean/rich cycling of a lean NOx trap catalyst

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Mr?ek, David; Koci, Petr; Choi, Jae -Soon; Partridge, Jr., William P.

    2015-09-08

    Periodical regeneration of NOx storage catalyst (also known as lean NOx trap) by short rich pulses of CO, H2 and hydrocarbons is necessary for the reduction of nitrogen oxides adsorbed on the catalyst surface. Ideally, the stored NOx is converted into N2, but N2O and NH3 by-products can be formed as well, particularly at low-intermediate temperatures. The N2 and N2O products are formed concurrently in two peaks. The primary peaks appear immediately after the rich-phase inception, and tail off with the breakthrough of the reductant front accompanied by NH3 product. In addition, the secondary N2 and N2O peaks then appearmoreat the rich-to-lean transition as a result of reactions between surface-deposited reductants/intermediates (CO, HC, NH3, NCO) and residual stored NOx under increasingly lean conditions.less

  5. PETROPHYSICAL INVESTIGATION OF THE SECONDARY RECOVERY POTENTIAL IN THE CHERRY CANYON FORMATION NE LEA FIELD LEA COUNTY, NEW MEXICO

    SciTech Connect (OSTI)

    T. Scott Hickman

    2002-06-01

    Read and Stevens has proposed the evaluation of the waterflood potential from the Cherry Canyon formation in the NE Lea Field in lea County, New Mexico. Much of the development in this area is approaching primary recovery limitations; additional recovery of remaining oil reserves by waterflood needs to be evaluated. The Cherry Canyon formation is composed of fine grained sandstone, containing clay material which results in high water saturation, and also has the tendency to swell and reduce reservoir permeability--the ability of fluid to flow through the rock pores and fractures. There are also abundant organic materials that interfere with obtaining reliable well logs. These complications have limited oil in place calculations and identification of net pay zones, presenting a challenge to the planned waterflood. Core analysis of the Cherry Canyon should improve the understanding of existing well logs and possibly indicate secondary recovery measures, such as waterflood, to enhance field recovery. Lacking truly representative core to provide accurate analyses, Read and Stevens will obtain and preserve fresh core. The consulting firm of T. Scott Hickman and Associates will then collaborate on special core analyses and obtain additional well logs for a more detailed analysis of reservoir properties. The log interpretation will be compared to the core analysis results, and the entire collected data set will be used to assess the potential and economic viability of successfully waterflooding the identified oil zones. Successful results from the project will improve accuracy of log interpretation and establish a methodology for evaluating secondary recovery by waterflood.

  6. Spin and valley transport in monolayers of MoS{sub 2}

    SciTech Connect (OSTI)

    Sun, J. F.; Cheng, F.

    2014-04-07

    We investigate theoretically quantum transport and Goos-Hnchen (GH) effect of electrons in a p-n-p junction on monolayers of MoS{sub 2}. We find that the transmission properties of spin-up (spin-down) electrons in K valley are the same with spin-down (spin-up) electrons in K? valley due to the time-reversal symmetry. The GH shifts for the transmitted K and K? beams in the n-p interface are in the opposite direction, and GH shifts for the spin-up and spin-down electron beams at the same valley have different values in the same direction due to the different group velocities. Therefore, the spin-up and spin-down electrons can be separated after passing a sufficiently long channel created by a p-n-p junction. These features provide us a new way to generate a fully spin- and valley-polarized current in monolayers of MoS{sub 2}.

  7. On the bonding nature of electron states for the Fe-Mo double perovskite

    SciTech Connect (OSTI)

    Carvajal, E.; Cruz-Irisson, M.; Oviedo-Roa, R.; Navarro, O.

    2014-05-15

    The electronic transport as well as the effect of an external magnetic field has been investigated on manganese-based materials, spinels and perovskites. Potential applications of double perovskites go from magnetic sensors to electrodes in solid-oxide fuel cells; besides the practical interests, it is known that small changes in composition modify radically the physical properties of double perovskites. We have studied the Sr{sub 2}FeMoO{sub 6} double perovskite compound (SFMO) using first-principles density functional theory. The calculations were done within the generalized gradient approximation (GGA) scheme with the Perdew-Burke-Ernzerhof (PBE) functional. We have made a detailed analysis of each electronic state and the charge density maps around the Fermi level. For the electronic properties of SFMO it was used a primitive cell, for which we found the characteristic half-metallic behavior density of states composed by e{sub g} and t{sub 2g} electrons from Fe and Mo atoms. Those peaks were tagged as bonding or antibonding around the Fermi level at both, valence and conduction bands.

  8. Experimental study of the electric dipole strength in the even Mo nuclei and its deformation dependence

    SciTech Connect (OSTI)

    Erhard, M.; Junghans, A. R.; Nair, C.; Schwengner, R.; Beyer, R.; Klug, J.; Kosev, K.; Wagner, A.; Grosse, E.

    2010-03-15

    Two methods based on bremsstrahlung were applied to the stable even Mo isotopes for the experimental determination of the photon strength function covering the high excitation energy range above 4 MeV with its increasing level density. Photon scattering was used up to the neutron separation energies S{sub n} and data up to the maximum of the isovector giant resonance (GDR) were obtained by photoactivation. After a proper correction for multistep processes the observed quasicontinuous spectra of scattered photons show a remarkably good match to the photon strengths derived from nuclear photoeffect data obtained previously by neutron detection and corrected in absolute scale by using the new activation results. The combined data form an excellent basis to derive a shape dependence of the E1 strength in the even Mo isotopes with increasing deviation from the N=50 neutron shell (i.e., with the impact of quadrupole deformation and triaxiality). The wide energy coverage of the data allows for a stringent assessment of the dipole sum rule and a test of a novel parametrization developed previously which is based on it. This parametrization for the electric dipole strength function in nuclei with A>80 deviates significantly from prescriptions generally used previously. In astrophysical network calculations it may help to quantify the role the p-process plays in cosmic nucleosynthesis. It also has impact on the accurate analysis of neutron capture data of importance for future nuclear energy systems and waste transmutation.

  9. Electronic structure and conductivity of nanocomposite metal (Au,Ag,Cu,Mo)-containing amorphous carbon films

    SciTech Connect (OSTI)

    Endrino, Jose L.; Horwat, David; Gago, Raul; Andersson, Joakim; Liu, Y.S.; Guo, Jinghua; Anders, Andre

    2008-05-14

    In this work, we study the influence of the incorporation of different metals (Me = Au, Ag, Cu, Mo) on the electronic structure of amorphous carbon (a-C:Me) films. The films were produced at room temperature using a novel pulsed dual-cathode arc deposition technique. Compositional analysis was performed with secondary neutral mass spectroscopy whereas X-ray diffraction was used to identify the formation of metal nanoclusters in the carbon matrix. The metal content incorporated in the nanocomposite films induces a drastic increase in the conductivity, in parallel with a decrease in the band gap corrected from Urbach energy. The electronic structure as a function of the Me content has been monitored by x-ray absorption near edge structure (XANES) at the C K-edge. XANES showed that the C host matrix has a dominant graphitic character and that it is not affected significantly by the incorporation of metal impurities, except for the case of Mo, where the modifications in the lineshape spectra indicated the formation of a carbide phase. Subtle modifications of the spectral lineshape are discussed in terms of nanocomposite formation.

  10. Study of the K{sub stop}{sup -}A{yields}{Sigma}{sup {+-}}{pi}{sup {+-}}A' reaction at DA{Phi}NE

    SciTech Connect (OSTI)

    Agnello, M.; Benussi, L.; Bertani, M.; Fabbri, F. L.; Gianotti, P.; Lucherini, V.; Bhang, H. C.; Bonomi, G.; Moia, F.; Zenoni, A.; Botta, E.; Bressani, T.; Bufalino, S.; Busso, L.; Calvo, D.; De Mori, F.; Feliciello, A.; Filippi, A.; Marcello, S.; Wheadon, R.

    2010-12-28

    This work describes an experimental study of the K{sub stop}{sup -}A{yields}{pi}{sup {+-}}{Sigma}{sup {+-}}A' reaction performed with the FINUDA spectrometer at the DA{Phi}NE {phi}-factory. The reaction is studied via the detection of {pi}{sup +}{pi}{sup -}n events on {sup 6,7}Li, {sup 9}Be, {sup 13}C and {sup 16}O.

  11. Measurement of K+ production cross section by 8 GeV protons using high energy neutrino interactions in the SciBooNE detector

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Cheng, G.

    2011-07-28

    The SciBooNE Collaboration reports K+ production cross section and rate measurements using high energy daughter muon neutrino scattering data off the SciBar polystyrene (C8H8) target in the SciBooNE detector. The K+ mesons are produced by 8 GeV protons striking a beryllium target in Fermilab Booster Neutrino Beam line (BNB). Using observed neutrino and antineutrino events in SciBooNE, we measure d2σ/dpdΩ = (5.34 ±0.76) mb/(GeV/c x sr) for p + Be =K+ + X at mean K+ energy of 3.9 GeV and angle (with respect to the proton beam direction) of 3.7 degrees, corresponding to the selected K+ sample. Compared tomore » Monte Carlo predictions using previous higher energy K+ production measurements, this measurement, which uses the NUANCE neutrino interaction generator, is consistent with a normalization factor of 0.85 ± 0.12. This agreement is evidence that the extrapolation of the higher energy K+ measurements to an 8 GeV beam energy using Feynman scaling is valid. This measurement reduces the error on the K+ production cross section from 40% to 14%.« less

  12. Measurement of K+ production cross section by 8 GeV protons using high energy neutrino interactions in the SciBooNE detector

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Cheng, G.

    2011-07-28

    The SciBooNE Collaboration reports K+ production cross section and rate measurements using high energy daughter muon neutrino scattering data off the SciBar polystyrene (C8H8) target in the SciBooNE detector. The K+ mesons are produced by 8 GeV protons striking a beryllium target in Fermilab Booster Neutrino Beam line (BNB). Using observed neutrino and antineutrino events in SciBooNE, we measure d2σ/dpdΩ = (5.34 ±0.76) mb/(GeV/c x sr) for p + Be =K+ + X at mean K+ energy of 3.9 GeV and angle (with respect to the proton beam direction) of 3.7 degrees, corresponding to the selected K+ sample. Compared tomore »Monte Carlo predictions using previous higher energy K+ production measurements, this measurement, which uses the NUANCE neutrino interaction generator, is consistent with a normalization factor of 0.85 ± 0.12. This agreement is evidence that the extrapolation of the higher energy K+ measurements to an 8 GeV beam energy using Feynman scaling is valid. This measurement reduces the error on the K+ production cross section from 40% to 14%.« less

  13. Two-chord interferometry using 3.39 {mu}m He-Ne laser on a flux-coil-generated FRC

    SciTech Connect (OSTI)

    Gota, H.; Deng, B. H.; Gupta, D.; Kiyashko, V.; Knapp, K.; Mendoza, R.; Morehouse, M.; Bolte, N.; Roche, T.; Wessel, F.

    2010-10-15

    A two-chord {lambda}{sub IR}{approx}3.39 {mu}m He-Ne laser interferometer system was developed for a flux-coil-generated field-reversed configuration to estimate the electron density and the total temperature of the field-reversed configuration (FRC) plasma. This two-chord heterodyne interferometer system consists of a single {approx}2 mW infrared He-Ne laser, a visible ({lambda}{sub vis}{approx}632.8 nm) He-Ne laser for the alignment, a 40 MHz acousto-optic modulator, photodetectors, and quadrature phase detectors. Initial measurement was performed and the measured average electron densities were 2-10x10{sup 19} m{sup -3} at two different radial positions in the midplane. A time shift in density was observed as the FRC expands radially. The time evolution of the line-averaged density agrees with the density estimated from the in situ internal magnetic probes, based on a rigid-rotor profile model.

  14. MoO3 as combined hole injection layer and tapered spacer in combinatorial multicolor microcavity organic light emitting diodes

    SciTech Connect (OSTI)

    Liu, R.; Xu, Chun; Biswas, Rana; Shinar, Joseph; Shinar, Ruth

    2011-09-01

    Multicolor microcavity ({mu}C) organic light-emitting diode (OLED) arrays were fabricated simply by controlling the hole injection and spacer MoO{sub 3} layer thickness. The normal emission was tunable from {approx}490 to 640 nm and can be further expanded. A compact, integrated spectrometer with two-dimensional combinatorial arrays of {mu}C OLEDs was realized. The MoO{sub 3} yields more efficient and stable devices, revealing a new breakdown mechanism. The pixel current density reaches {approx}4 A/cm{sup 2} and a maximal normal brightness {approx}140 000 Cd/m{sup 2}, which improves photoluminescence-based sensing and absorption measurements.

  15. Comparison of Two Preparation Methods on Catalytic Activity and Selectivity of Ru-Mo/HZSM5 for Methane Dehydroaromatization

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Petkovic, Lucia M.; Ginosar, Daniel M.

    2014-01-01

    Catalytic performance of Mo/HZSM5 and Ru-Mo/HZSM5 catalysts prepared by vaporization-deposition of molybdenum trioxide and impregnation with ammonium heptamolybdate was analyzed in terms of catalyst activity and selectivity, nitrogen physisorption analyses, temperature-programmed oxidation of carbonaceous residues, and temperature-programmed reduction. Vaporization-deposition rendered the catalyst more selective to ethylene and coke than the catalyst prepared by impregnation. This result was assigned to lower interaction of molybdenum carbide with the zeolite acidic sites.

  16. Enhancing the photocurrent and photoluminescence of single crystal monolayer MoS{sub 2} with resonant plasmonic nanoshells

    SciTech Connect (OSTI)

    Sobhani, Ali [Department of Electrical and Computer Engineering, Rice University, Houston, Texas 77005 (United States); Lauchner, Adam [Department of Physics and Astronomy, Rice University, Houston, Texas 77005 (United States); Najmaei, Sina; Lou, Jun [Department of Materials Science and NanoEngineering, Rice University, Houston, Texas 77005 (United States); Ayala-Orozco, Ciceron; Wen, Fangfang [Department of Chemistry, Rice University, Houston, Texas 77005 (United States); Halas, Naomi J., E-mail: halas@rice.edu [Department of Electrical and Computer Engineering, Rice University, Houston, Texas 77005 (United States); Department of Physics and Astronomy, Rice University, Houston, Texas 77005 (United States)

    2014-01-20

    Monolayer molybdenum disulfide (MoS{sub 2}) produced by controlled vapor-phase synthesis is a commercially promising new two-dimensional material for optoelectronics because of its direct bandgap and broad absorption in the visible and ultraviolet regimes. By tuning plasmonic core-shell nanoparticles to the direct bandgap of monolayer MoS{sub 2} and depositing them sparsely (<1% coverage) onto the material's surface, we observe a threefold increase in photocurrent and a doubling of photoluminescence signal for both excitonic transitions, amplifying but not altering the intrinsic spectral response.

  17. Improved Search for ν̄μ→ν̄e Oscillations in the MiniBooNE Experiment

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Aguilar-Arevalo, A. A.; Brown, B. C.; Bugel, L.; Cheng, G.; Church, E. D.; Conrad, J. M.; Dharmapalan, R.; Djurcic, Z.; Finley, D. A.; Ford, R.; et al

    2013-04-15

    The MiniBooNE experiment at Fermilab reports results from an analysis of ν¯e appearance data from 11.27×10²⁰ protons on target in the antineutrino mode, an increase of approximately a factor of 2 over the previously reported results. An event excess of 78.4±28.5 events (2.8σ) is observed in the energy range 200QEν<1250 MeV. If interpreted in a two-neutrino oscillation model, ν¯μ→ν¯e, the best oscillation fit to the excess has a probability of 66% while the background-only fit has a χ² probability of 0.5% relative to the best fit. The data are consistent with antineutrino oscillations in the 0.01<Δm²<1.0 eV² range and havemore » some overlap with the evidence for antineutrino oscillations from the Liquid Scintillator Neutrino Detector. All of the major backgrounds are constrained by in situ event measurements so nonoscillation explanations would need to invoke new anomalous background processes. The neutrino mode running also shows an excess at low energy of 162.0±47.8 events (3.4σ) but the energy distribution of the excess is marginally compatible with a simple two neutrino oscillation formalism. Expanded models with several sterile neutrinos can reduce the incompatibility by allowing for CP violating effects between neutrino and antineutrino oscillations.« less

  18. Preparation and structural study from neutron diffraction data of Pr{sub 5}Mo{sub 3}O{sub 16}

    SciTech Connect (OSTI)

    Martinez-Lope, M.J.; Alonso, J.A.; Sheptyakov, D.; Pomjakushin, V.

    2010-12-15

    The title compound has been prepared as polycrystalline powder by thermal treatments of mixtures of Pr{sub 6}O{sub 11} and MoO{sub 2} in air. In the literature, an oxide with a composition Pr{sub 2}MoO{sub 6} has been formerly described to present interesting catalytic properties, but its true stoichiometry and crystal structure are reported here for the first time. It is cubic, isostructural with CdTm{sub 4}Mo{sub 3}O{sub 16} (space group Pn-3n, Z=8), with a=11.0897(1) A. The structure contains MoO{sub 4} tetrahedral units, with Mo-O distances of 1.788(2) A, fully long-range ordered with PrO{sub 8} polyhedra; in fact it can be considered as a superstructure of fluorite (M{sub 8}O{sub 16}), containing 32 MO{sub 2} fluorite formulae per unit cell, with a lattice parameter related to that of cubic fluorite (a{sub f}=5.5 A) as a{approx}2a{sub f}. A bond valence study indicates that Mo exhibits a mixed oxidation state between 5+ and 6+ (perhaps accounting for the excellent catalytic properties). One kind of Pr atoms is trivalent whereas the second presents a mixed Pr{sup 3+}-Pr{sup 4+} oxidation state. The similarity of the XRD pattern with that published for Ce{sub 2}MoO{sub 6} suggests that this compound also belongs to the same structural type, with an actual stoichiometry Ce{sub 5}Mo{sub 3}O{sub 16}. -- Graphical Abstract: Formerly formulated as Pr{sub 2}MoO{sub 6}, the title compound is a cubic superstructure of fluorite (a=11.0897(1) A, space group Pn-3n) due to the long-range ordering of PrO{sub 8} scalenohedra and MoO{sub 4} tetrahedral units, showing noticeable shifts of the oxygen positions in order to provide a tetrahedral coordination for Mo ions. A mixed valence Mo{sup 5+}-Mo{sup 6+} is identified, which could account for the excellent catalytic properties of this material. Display Omitted

  19. Toward epitaxially grown two-dimensional crystal hetero-structures: Single and double MoS{sub 2}/graphene hetero-structures by chemical vapor depositions

    SciTech Connect (OSTI)

    Lin, Meng-Yu [Graduate Institute of Electronics Engineering, National Taiwan University, Taipei, Taiwan (China); Research Center for Applied Sciences, Academia Sinica, Nankang, Taipei, Taiwan (China); Chang, Chung-En [Department of Photonics, National Chiao-Tung University, Hsinchu, Taiwan (China); Wang, Cheng-Hung [Institute of Display, National Chiao-Tung University, Hsinchu, Taiwan (China); Su, Chen-Fung; Chen, Chi [Research Center for Applied Sciences, Academia Sinica, Nankang, Taipei, Taiwan (China); Lee, Si-Chen [Graduate Institute of Electronics Engineering, National Taiwan University, Taipei, Taiwan (China); Lin, Shih-Yen, E-mail: shihyen@gate.sinica.edu.tw [Graduate Institute of Electronics Engineering, National Taiwan University, Taipei, Taiwan (China); Research Center for Applied Sciences, Academia Sinica, Nankang, Taipei, Taiwan (China); Department of Photonics, National Chiao-Tung University, Hsinchu, Taiwan (China)

    2014-08-18

    Uniform large-size MoS{sub 2}/graphene hetero-structures fabricated directly on sapphire substrates are demonstrated with layer-number controllability by chemical vapor deposition (CVD). The cross-sectional high-resolution transmission electron microscopy (HRTEM) images provide the direct evidences of layer numbers of MoS{sub 2}/graphene hetero-structures. Photo-excited electron induced Fermi level shift of the graphene channel are observed on the single MoS{sub 2}/graphene hetero-structure transistors. Furthermore, double hetero-structures of graphene/MoS{sub 2}/graphene are achieved by CVD fabrication of graphene layers on top of the MoS{sub 2}, as confirmed by the cross-sectional HRTEM. These results have paved the possibility of epitaxially grown multi-hetero-structures for practical applications.

  20. A survey of Existing V&V, UQ and M&S Data and Knowledge Bases in Support of the Nuclear Energy - Knowledge base for Advanced Modeling and Simulation (NE-KAMS)

    SciTech Connect (OSTI)

    Hyung Lee; Rich Johnson, Ph.D.; Kimberlyn C. Moussesau

    2011-12-01

    The Nuclear Energy - Knowledge base for Advanced Modeling and Simulation (NE-KAMS) is being developed at the Idaho National Laboratory in conjunction with Bettis Laboratory, Sandia National Laboratories, Argonne National Laboratory, Oak Ridge National Laboratory, Utah State University and others. The objective of this consortium is to establish a comprehensive knowledge base to provide Verification and Validation (V&V) and Uncertainty Quantification (UQ) and other resources for advanced modeling and simulation (M&S) in nuclear reactor design and analysis. NE-KAMS will become a valuable resource for the nuclear industry, the national laboratories, the U.S. NRC and the public to help ensure the safe operation of existing and future nuclear reactors. A survey and evaluation of the state-of-the-art of existing V&V and M&S databases, including the Department of Energy and commercial databases, has been performed to ensure that the NE-KAMS effort will not be duplicating existing resources and capabilities and to assess the scope of the effort required to develop and implement NE-KAMS. The survey and evaluation have indeed highlighted the unique set of value-added functionality and services that NE-KAMS will provide to its users. Additionally, the survey has helped develop a better understanding of the architecture and functionality of these data and knowledge bases that can be used to leverage the development of NE-KAMS.