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1

Atomic vapor laser isotope separation of lead-210 isotope  

DOE Patents (OSTI)

An isotopically selective laser process and apparatus for removal of Pb-210 from natural lead that involves a one-photon near-resonant, two-photon resonant excitation of one or more Rydberg levels, followed by field ionization and then electrostatic extraction. The wavelength to the near-resonant intermediate state is counter propagated with respect to the second wavelength required to populate the final Rydberg state. This scheme takes advantage of the large first excited state cross section, and only modest laser fluences are required. The non-resonant process helps to avoid two problems: first, stimulated Raman Gain due to the nearby F=3/2 hyperfine component of Pb-207 and, second, direct absorption of the first transition process light by Pb-207.

Scheibner, Karl F. (Tracy, CA); Haynam, Christopher A. (Pleasanton, CA); Johnson, Michael A. (Pleasanton, CA); Worden, Earl F. (Diablo, CA)

1999-01-01T23:59:59.000Z

2

Atomic vapor laser isotope separation of lead-210 isotope  

DOE Patents (OSTI)

An isotopically selective laser process and apparatus for removal of Pb-210 from natural lead that involves a one-photon near-resonant, two-photon resonant excitation of one or more Rydberg levels, followed by field ionization and then electrostatic extraction. The wavelength to the near-resonant intermediate state is counter propagated with respect to the second wavelength required to populate the final Rydberg state. This scheme takes advantage of the large first excited state cross section, and only modest laser fluences are required. The non-resonant process helps to avoid two problems: first, stimulated Raman Gain due to the nearby F=3/2 hyperfine component of Pb-207 and, second, direct absorption of the first transition process light by Pb-207. 5 figs.

Scheibner, K.F.; Haynam, C.A.; Johnson, M.A.; Worden, E.F.

1999-08-31T23:59:59.000Z

3

Innovative lasers for uranium isotope separation. [Progress report  

SciTech Connect

Copper vapor lasers have important applications to uranium atomic vapor laser isotope separation (AVLIS). The authors have spent the first two years of their project investigating two innovative methods of exciting/pumping copper vapor lasers which have the potential to improve the efficiency and scaling of large laser systems used in uranium isotope separation. Experimental research has focused on the laser discharge kinetics of (1) microwave, and (2) electron beam excitation/pumping of large-volume copper vapor lasers. During the first year, the experiments have been designed and constructed and initial data has been taken. During the second year these experiments have been diagnosed. Highlights of some of the second year results as well as plans for the future include the following: Microwave resonant cavity produced copper vapor plasmas at 2.45 GHz, have been investigated. A CW (0--500 W) signal heats and vaporizes the copper chloride to provide the atomic copper vapor. A pulsed (5 kW, 0.5--5kHz) signal is added to the incoming CW signal via a hybrid mixer to excite the copper states to the laser levels. An enhancement of the visible radiation has been observed during the pulsed pardon of the signal. Electrical probe measurements have been implemented on the system to verify the results of the electromagnetic model formulated last year. Laser gain measurements have been initiated with the use of a commercial copper vapor laser. Measurements of the spatial profile of the emission are also currently being made. The authors plan to increase the amount of pulsed microwave power to the system by implementing a high power magnetron. A laser cavity will be designed and added to this system.

Brake, M.L.; Gilgenbach, R.M.

1991-06-01T23:59:59.000Z

4

Nuclear Proliferation Using Laser Isotope Separation -- Verification Options  

SciTech Connect

Two levels of nonproliferation verification exist. Signatories of the basic agreements under the Nuclear Non-proliferation Treaty (NPT) agree to open their nuclear sites to inspection by the IAEA. A more detailed and intrusive level was developed following the determination that Iraq had begun a nuclear weapons development program that was not detected by the original level of verification methods. This level, referred to as 93+2 and detailed in model protocol INFCIRC/540, allows the IAEA to do environmental monitoring of non-declared facilities that are suspected of containing proliferation activity, and possibly further inspections, as well as allowing more detailed inspections of declared sites. 56 countries have signed a Strengthened Safeguards Systems Additional Protocol as of 16 July 2001. These additional inspections can be done on the instigation of the IAEA itself, or after requests by other parties to the NPT, based on information that they have collected. Since information able to cause suspicion of proliferation could arrive at any country, it is important that countries have procedures in place that will assist them in making decisions related to these inspections. Furthermore, IAEA inspection resources are limited, and therefore care needs to be taken to make best use of these resources. Most of the nonproliferation verification inspections may be concentrated on establishing that diversion of nuclear materials is not occurring, but some fraction will be related to determining if undeclared sites have nuclear materials production taking place within them. Of these, most suspicions will likely be related to the major existing technologies for uranium enrichment and reprocessing for plutonium extraction, as it would seem most likely that nations attempting proliferation would use tested means of producing nuclear materials. However, as technology continues to advance and new methods of enrichment and reprocessing are developed, inspection-related procedures will need to be adapted to keep up with them. In order to make 93+2 inspections more useful, a systematic way of finding clues to nuclear proliferation would be useful. Also, to cope with the possible use of newer technology for proliferation, the list of clues might need to be expanded. This paper discusses the development and recognition of such clues. It concentrates on laser isotope separation (LIS) as a new proliferation technology, and uses Uranium Atomic Vapor Laser Isotope Separation (U-AVLIS) as an example of LIS that is well known.

Erickson, S A

2001-10-15T23:59:59.000Z

5

Laser separation of nitrogen isotopes by the IR+UV dissociation of ammonia molecules  

SciTech Connect

The separation of nitrogen isotopes is studied upon successive single-photon IR excitation and UV dissociation of ammonia molecules. The excitation selectivity was provided by tuning a CO{sub 2} laser to resonance with {sup 14}NH{sub 3} molecules [the 9R(30) laser line] or with {sup 15}NH{sub 3} molecules [the 9R(10) laser line]. Isotopic mixtures containing 4.8% and 0.37% (natural content) of the {sup 15}NH isotope were investigated. The dependences of the selectivity and the dissociation yield for each isotopic component on the buffer gas pressure (N{sub 2}, O{sub 2}, Ar) and the ammonia pressure were obtained. In the limit of low NH{sub 3} pressures (0.5-2 Torr), the dissociation selectivity {alpha}(15/14) for {sup 15}N was 17. The selectivity mechanism of the IR+UV dissociation is discussed and the outlook is considered for the development of the nitrogen isotope separation process based on this approach. (laser isotope separation)

Apatin, V M; Klimin, S A; Laptev, V B; Lokhman, V N; Ogurok, D D; Pigul'skii, S V; Ryabov, E A [Institute of Spectroscopy, Russian Academy of Sciences, Troitsk, Moscow region (Russian Federation)

2008-08-31T23:59:59.000Z

6

Atomic vapor laser isotope separation at Lawrence Livermore National Laboratory: a status report  

SciTech Connect

The field of laser induced chemistry began in earnest early in the 1970's with the initiation of major efforts in laser isotope separation (LIS) of uranium. Though many specialized, small-scale photochemical and diagnostic applications have been identified and evaluated experimentally, and continue to show promise, currently the only high payoff, large-scale applications remain LIS of special elements. Aspects of the physical scaling, technology status and economic basis of uranium LIS are examined with special emphasis on the effort at LLNL.

Davis, J.I.

1980-01-01T23:59:59.000Z

7

Application of atomic vapor laser isotope separation to the enrichment of mercury  

SciTech Connect

Workers at GTE/Sylvania have shown that the efficiency of fluorescent lighting may be markedly improved using mercury that has been enriched in the /sup 196/Hg isotope. A 5% improvement in the efficiency of fluorescent lighting in the United States could provide a savings of approx. 1 billion dollars in the corresponding reduction of electrical power consumption. We will discuss the results of recent work done at our laboratory to develop a process for enriching mercury. The discussion will center around the results of spectroscopic measurements of excited state lifetimes, photoionization cross sections and isotope shifts. In addition, we will discuss the mercury separator and supporting laser mesurements of the flow properties of mercury vapor. We will describe the laser system which will provide the photoionization and finally discuss the economic details of producing enriched mercury at a cost that would be attractive to the lighting industry.

Crane, J.K.; Erbert, G.V.; Paisner, J.A.; Chen, H.L.; Chiba, Z.; Beeler, R.G.; Combs, R.; Mostek, S.D.

1986-09-01T23:59:59.000Z

8

I CALCULATIONS ON ISOTOPE SEPARATION BY LASER INDUCED PHOTODISSOCIATION OF POLYATOMIC MOLECULES  

NLE Websites -- All DOE Office Websites (Extended Search)

; ; . I CALCULATIONS ON ISOTOPE SEPARATION BY LASER INDUCED PHOTODISSOCIATION OF POLYATOMIC MOLECULES F i n a l Report Willis E . Lamb, JY. U n i v e r s i t y of Arizona Tucson, Arizona 85721 NOTICE report was prepared 86 an account of work sponsored by the United Stater Government. Neither the United S t a m nor the United States Department of Encrwi, nor any of their employees, nor any of thelr contractors, Subcontractors, o r their employer, maker any warranty, exprels or Implied. or apumn my k@ liability or responsibility for the aceuraey. eompletencu or uvfulneu of any informtion, apparatus. product Process disclosed. or rtpreYnu that its ur would not infringe privately o m d righu. November 1978 Prepared f o r TIE UNITED STATES DEPARTMENT OF ENERGY Under Contract No. EN-77-S-02--000

9

Advanced isotope separation  

SciTech Connect

The Study Group briefly reviewed the technical status of the three Advanced Isotope Separation (AIS) processes. It also reviewed the evaluation work that has been carried out by DOE's Process Evaluation Board (PEB) and the Union Carbide Corporation-Nuclear Division (UCCND). The Study Group briefly reviewed a recent draft assessment made for DOE staff of the nonproliferation implications of the AIS technologies. The staff also very briefly summarized the status of GCEP and Advanced Centrifuge development. The Study Group concluded that: (1) there has not been sufficient progress to provide a firm scientific, technical or economic basis on which to select one of the three competing AIS processes for full-scale engineering development at this time; and (2) however, should budgetary restraints or other factors force such a selection, we believe that the evaluation process that is being carried out by the PEB provides the best basis available for making a decision. The Study Group recommended that: (1) any decisions on AIS processes should include a comparison with gas centrifuge processes, and should not be made independently from the plutonium isotope program; (2) in evaluating the various enrichment processes, all applicable costs (including R and D and sales overhead) and an appropriate discounting approach should be included in order to make comparisons on a private industry basis; (3) if the three AIS programs continue with limited resources, the work should be reoriented to focus only on the most pressing technical problems; and (4) if a decision is made to develop the Atomic Vapor Laser Isotope Separation process, the solid collector option should be pursued in parallel to alleviate the potential program impact of liquid collector thermal control problems.

Not Available

1982-05-04T23:59:59.000Z

10

Isotope separation apparatus  

DOE Patents (OSTI)

Isotope separation apparatus consisting of a plurality of cells disposed adjacent to each other in an evacuated container. A common magnetic field is established extending through all of the cells. A source of energetic electrons at one end of the container generates electrons which pass through the cells along the magnetic field lines. Each cell includes an array of collector plates arranged in parallel or in tandem within a common magnetic field. Sets of collector plates are disposed adjacent to each other in each cell. Means are provided for differentially energizing ions of a desired isotope by applying energy at the cyclotron resonant frequency of the desired isotope. As a result, the energized desired ions are preferentially collected by the collector plates.

Arnush, Donald (Rancho Palos Verdes, CA); MacKenzie, Kenneth R. (Pacific Palisades, CA); Wuerker, Ralph F. (Palos Verdes Estates, CA)

1980-01-01T23:59:59.000Z

11

Device and method for separating oxygen isotopes  

DOE Patents (OSTI)

A device and method for separating oxygen isotopes with an ArF laser which produces coherent radiation at approximately 193 nm. The output of the ArF laser is filtered in natural air and applied to an irradiation cell where it preferentially photodissociates molecules of oxygen gas containing .sup.17 O or .sup.18 O oxygen nuclides. A scavenger such as O.sub.2, CO or ethylene is used to collect the preferentially dissociated oxygen atoms and recycled to produce isotopically enriched molecular oxygen gas. Other embodiments utilize an ArF laser which is narrowly tuned with a prism or diffraction grating to preferentially photodissociate desired isotopes. Similarly, desired mixtures of isotopic gas can be used as a filter to photodissociate enriched preselected isotopes of oxygen.

Rockwood, Stephen D. (Los Alamos, NM); Sander, Robert K. (Los Alamos, NM)

1984-01-01T23:59:59.000Z

12

A Mass Spectrometry Study of Isotope Separation in the Laser Plume  

E-Print Network (OSTI)

1.4.2 Atomic Absorption5.3.2 Atomic Absorption Spectrometry . . . . . . . . . . .ablation and diode laser-atomic absorption spectrometry”,

Suen, Timothy Wu

2012-01-01T23:59:59.000Z

13

Atomic Spectroscopy and Separated Isotopes  

Science Journals Connector (OSTI)

The advantages in the use of separated isotopes in atomic spectroscopy for the determination of nuclear momentsI ? Q and for studies of the isotope-shift phenomena are discussed. Illustrations of spectra are given for mercury uranium and samarium. In addition a summary is given of twenty-two so-called problem nuclei i.e. those naturally occurring isotopes for which the nuclear moments are completely uncertain. Concluding remarks are made on such problems as the evaluation of the absolute magnitude of isotope shifts the role of “forbidden transitions” in isotope spectra and the potential future value of spectro-isotopic assay techniques.

J. R. McNally Jr.

1952-01-01T23:59:59.000Z

14

Application of atomic vapor laser isotope separation to the enrichment of mercury  

SciTech Connect

Workers at GTE/Sylvania have shown that the efficiency of fluorescent lighting may be markedly improved using mercury that has been enriched in the /sup 196/Hg isotope. A 5% improvement in the efficiency of fluorescent lighting in the United States could provide a savings of $450 million dollars in the corresponding reduction of electrical power consumption. We discuss the results of recent work done at our laboratory to develop a process for enriching mercury. The discussion centers around the results of spectroscopic measurements of excited-state lifetimes, photoionization cross sections, and isotope shifts.

Crane, J.; Erbert, G.; Paisner, J.; Chen, H.; Chiba, Z.; Beeler, R.; Combs, R.; Mostek, S.

1986-09-01T23:59:59.000Z

15

Hybrid isotope separation scheme  

DOE Patents (OSTI)

A method is described for yielding selectively a desired enrichment in a specific isotope including the steps of inputting into a spinning chamber a gas from which a scavenger, radiating the gas with a wave length or frequency characteristic of the absorption of a particular isotope of the atomic or molecular gas, thereby inducing a photochemical reaction between the scavenger, and collecting the specific isotope-containing chemical by using a recombination surface or by a scooping apparatus. 2 figures.

Maya, J.

1991-06-18T23:59:59.000Z

16

Hybrid isotope separation scheme  

DOE Patents (OSTI)

A method of yielding selectively a desired enrichment in a specific isotope including the steps of inputting into a spinning chamber a gas from which a scavenger, radiating the gas with a wave length or frequency characteristic of the absorption of a particular isotope of the atomic or molecular gas, thereby inducing a photochemical reaction between the scavenger, and collecting the specific isotope-containing chemical by using a recombination surface or by a scooping apparatus.

Maya, Jakob (Brookline, MA)

1991-01-01T23:59:59.000Z

17

Hydrogen isotope separation  

DOE Patents (OSTI)

A system of four cryogenic fractional distillation columns interlinked with two equilibrators for separating a DT and hydrogen feed stream into four product streams, consisting of a stream of high purity D.sub.2, DT, T.sub.2, and a tritium-free stream of HD for waste disposal.

Bartlit, John R. (Los Alamos, NM); Denton, William H. (Abingdon, GB3); Sherman, Robert H. (Los Alamos, NM)

1982-01-01T23:59:59.000Z

18

Apparatus and process for separating hydrogen isotopes  

DOE Patents (OSTI)

The apparatus and process for separating hydrogen isotopes is provided using dual columns, each column having an opposite hydrogen isotopic effect such that when a hydrogen isotope mixture feedstock is cycled between the two respective columns, two different hydrogen isotopes are separated from the feedstock.

Heung, Leung K; Sessions, Henry T; Xiao, Xin

2013-06-25T23:59:59.000Z

19

Electrochemical Isotope Effect and Lithium Isotope Separation  

Science Journals Connector (OSTI)

In a series of papers Kavner et al. (2005, 2008)(2, 3) derive an equation predicting isotopic fractionation due to an electrochemical isotope effect (?EIE), defined by the ratio of electron transfer rates (k?/k) for isotopically substituted species (prime for heavy isotopologues): where v, ?G, kB, T, m, ?eq, QP/QR, z, e, and ? denote collision frequency, activation free energy, Boltzmann’s constant, temperature, mass in motion, equilibrium fractionation factor, partition function ratio of abundant isotopologues of product (P) and reactant (R), number of electrons, charge of electron, and Marcus reorganization energy, respectively. ... fractional isotope evolution of Zn isotopes during an electroplating process which stepwise removes most of the Zn from the aq. ...

Jay R. Black; Grant Umeda; Bruce Dunn; William F. McDonough; Abby Kavner

2009-07-06T23:59:59.000Z

20

Electromagnetic Isotope Separation Lab (EMIS) | ORNL  

NLE Websites -- All DOE Office Websites (Extended Search)

Electromagnetic Isotope Separation Lab Electromagnetic Isotope Separation Lab May 30, 2013 ORNL established the Stable Isotope Enrichment Laboratory (SIEL) as part of a project funded by the DOE Office of Science, Nuclear Physics Program to develop a modernized electromagnetic isotope separator (EMIS), optimized for separation of a wide range of stable isotopes. The SIEL is located in the Building 6010 Shield Test Station, space formerly allocated to the Oak Ridge Electron Linear Accelerator, on the main campus of ORNL. ORNL staff have designed and built a nominal 10 mA ion current EMIS (sum of all isotopes at the collector) in the SIEL. This EMIS is currently being tested to determine basic performance metrics such as throughput and enrichment factor per pass. This EMIS unit and space will be used to

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


21

Laser Isotope Enrichment for Medical and Industrial Applications  

SciTech Connect

Laser Isotope Enrichment for Medical and Industrial Applications by Jeff Eerkens (University of Missouri), Jay Kunze (Idaho State University), and Leonard Bond (Idaho National Laboratory) The principal isotope enrichment business in the world is the enrichment of uranium for commercial power reactor fuels. However, there are a number of other needs for separated isotopes. Some examples are: 1) Pure isotopic targets for irradiation to produce medical radioisotopes. 2) Pure isotopes for semiconductors. 3) Low neutron capture isotopes for various uses in nuclear reactors. 4) Isotopes for industrial tracer/identification applications. Examples of interest to medicine are targets to produce radio-isotopes such as S-33, Mo-98, Mo-100, W-186, Sn-112; while for MRI diagnostics, the non-radioactive Xe-129 isotope is wanted. For super-semiconductor applications some desired industrial isotopes are Si-28, Ga-69, Ge-74, Se-80, Te-128, etc. An example of a low cross section isotope for use in reactors is Zn-68 as a corrosion inhibitor material in nuclear reactor primary systems. Neutron activation of Ar isotopes is of interest in industrial tracer and diagnostic applications (e.g. oil-logging). . In the past few years there has been a sufficient supply of isotopes in common demand, because of huge Russian stockpiles produced with old electromagnetic and centrifuge separators previously used for uranium enrichment. Production of specialized isotopes in the USA has been largely accomplished using old ”calutrons” (electromagnetic separators) at Oak Ridge National Laboratory. These methods of separating isotopes are rather energy inefficient. Use of lasers for isotope separation has been considered for many decades. None of the proposed methods have attained sufficient proof of principal status to be economically attractive to pursue commercially. Some of the authors have succeeded in separating sulfur isotopes using a rather new and different method, known as condensation repression. In this scheme a gas, of the selected isotopes for enrichment, is irradiated with a laser at a particular wavelength that would excite only one of the isotopes. The entire gas is subject to low temperatures sufficient to cause condensation on a cold surface. Those molecules in the gas that the laser excited are not as likely to condense as are the unexcited molecules. Hence the gas drawn out of the system will be enriched in the isotope that was excited by the laser. We have evaluated the relative energy required in this process if applied on a commercial scale. We estimate the energy required for laser isotope enrichment is about 20% of that required in centrifuge separations, and 2% of that required by use of "calutrons".

Leonard Bond

2006-07-01T23:59:59.000Z

22

Process for producing enriched uranium having a {sup 235}U content of at least 4 wt. % via combination of a gaseous diffusion process and an atomic vapor laser isotope separation process to eliminate uranium hexafluoride tails storage  

DOE Patents (OSTI)

An uranium enrichment process capable of producing an enriched uranium, having a {sup 235}U content greater than about 4 wt. %, is disclosed which will consume less energy and produce metallic uranium tails having a lower {sup 235}U content than the tails normally produced in a gaseous diffusion separation process and, therefore, eliminate UF{sub 6} tails storage and sharply reduce fluorine use. The uranium enrichment process comprises feeding metallic uranium into an atomic vapor laser isotope separation process to produce an enriched metallic uranium isotopic mixture having a {sup 235} U content of at least about 2 wt. % and a metallic uranium residue containing from about 0.1 wt. % to about 0.2 wt. % {sup 235} U; fluorinating this enriched metallic uranium isotopic mixture to form UF{sub 6}; processing the resultant isotopic mixture of UF{sub 6} in a gaseous diffusion process to produce a final enriched uranium product having a {sup 235}U content of at least 4 wt. %, and up to 93.5 wt. % or higher, of the total uranium content of the product, and a low {sup 235}U content UF{sub 6} having a {sup 235}U content of about 0.71 wt. % of the total uranium content of the low {sup 235}U content UF{sub 6}; and converting this low {sup 235}U content UF{sub 6} to metallic uranium for recycle to the atomic vapor laser isotope separation process. 4 figs.

Horton, J.A.; Hayden, H.W. Jr.

1995-05-30T23:59:59.000Z

23

Process for producing enriched uranium having a .sup.235 U content of at least 4 wt. % via combination of a gaseous diffusion process and an atomic vapor laser isotope separation process to eliminate uranium hexafluoride tails storage  

DOE Patents (OSTI)

An uranium enrichment process capable of producing an enriched uranium, having a .sup.235 U content greater than about 4 wt. %, is disclosed which will consume less energy and produce metallic uranium tails having a lower .sup.235 U content than the tails normally produced in a gaseous diffusion separation process and, therefore, eliminate UF.sub.6 tails storage and sharply reduce fluorine use. The uranium enrichment process comprises feeding metallic uranium into an atomic vapor laser isotope separation process to produce an enriched metallic uranium isotopic mixture having a .sup.235 U content of at least about 2 wt. % and a metallic uranium residue containing from about 0.1 wt. % to about 0.2 wt. % .sup.235 U; fluorinating this enriched metallic uranium isotopic mixture to form UF.sub.6 ; processing the resultant isotopic mixture of UF.sub.6 in a gaseous diffusion process to produce a final enriched uranium product having a .sup.235 U content of at least 4 wt. %, and up to 93.5 wt. % or higher, of the total uranium content of the product, and a low .sup.235 U content UF.sub.6 having a .sup.235 U content of about 0.71 wt. % of the total uranium content of the low .sup.235 U content UF.sub.6 ; and converting this low .sup.235 U content UF.sub.6 to metallic uranium for recycle to the atomic vapor laser isotope separation process.

Horton, James A. (Livermore, CA); Hayden, Jr., Howard W. (Oakridge, TN)

1995-01-01T23:59:59.000Z

24

Gaseous isotope separation using solar wind phenomena  

Science Journals Connector (OSTI)

...isotope separation using solar wind phenomena Chia-Gee...essentially the same as that of the solar wind propagation, in which...the author was measuring solar wind parameters under Dr. H. S. Bridge at Massachusetts Institute of Technology in...

Chia-Gee Wang

1980-01-01T23:59:59.000Z

25

EIS-0136: Special Isotope Separation Project Idaho National Engineering Laboratory, Idaho Falls, Idaho  

Energy.gov (U.S. Department of Energy (DOE))

The U.S. Department of Energy developed this EIS to provide environmental input to the decision to construct the Special Isotope Separation Project which would allow for the processing of existing fuel-grade plutonium into weapons-grade plutonium using the Atomic Laser Isotope Separation process.

26

Apparatus for separating and recovering hydrogen isotopes  

DOE Patents (OSTI)

An apparatus for recovering hydrogen and separating its isotopes. The apparatus includes a housing bearing at least a fluid inlet and a fluid outlet. A baffle is disposed within the housing, attached thereto by a bracket. A hollow conduit is coiled about the baffle, in spaced relation to the baffle and the housing. The coiled conduit is at least partially filled with a hydride. The hydride can be heated to a high temperature and cooled to a low temperature quickly by circulating a heat transfer fluid in the housing. The spacing between the baffle and the housing maximizes the heat exchange rate between the fluid in the housing and the hydride in the conduit. The apparatus can be used to recover hydrogen isotopes (protium, deuterium and tritium) from gaseous mixtures, or to separate hydrogen isotopes from each other.

Heung, Leung K. (Aiken, SC)

1994-01-01T23:59:59.000Z

27

Sulfur-isotope separation by distillation  

SciTech Connect

Sulfur-isotope separation by low-temperature distillation of hydrogen sulfide was studied in an 8-m, 25-mm diameter distillation column. Column temperature was controlled by a propane-propylene heat pipe. Column packing HETP was measured using nitric oxide in the column. The column was operated at pressures from 45 to 125 kPa. The relative volatility of S-32 vs. S-34 varied from 1.0008 to 1.0014.

Mills, T.R.

1982-01-01T23:59:59.000Z

28

Isotopically pumped isotopic CF4 laser  

Science Journals Connector (OSTI)

Single-mode optical pumping of CF4 to generate 16-µm frequencies has been extended to include the isotopic species 12CF4,...

Eckhardt, Roger; Telle, John; Haynes, Larry

1982-01-01T23:59:59.000Z

29

Hydrogen Isotope Separation From Noble Gasses in Plasma Exhausts...  

NLE Websites -- All DOE Office Websites (Extended Search)

Hydrogen Isotope Separation From Noble Gasses in Plasma Exhausts and Other Gas Streams --- Inventors Thomas A. Kozub, William R. Blanchard and Charles A. Gentile The objective of...

30

Novel hybrid isotope separation scheme and apparatus  

DOE Patents (OSTI)

A method is described for yielding selectively a desired enrichment in a specific isotope including the steps of inputting into a spinning chamber a gas from which the specific isotope is to be isolated, radiating the gas with frequencies characteristic of the absorption of a particular isotope of the atomic or molecular gas, thereby inducing a photoionization reaction of the desired isotope, and collecting the specific isotope ion by suitable ion collection means. 3 figures.

Maya, J.

1991-06-18T23:59:59.000Z

31

Novel hybrid isotope separation scheme and apparatus  

DOE Patents (OSTI)

A method of yielding selectively a desired enrichment in a specific isotope including the steps of inputting into a spinning chamber a gas from which the specific isotope is to be isolated, radiating the gas with frequencies characteristic of the absorption of a particular isotope of the atomic or molecular gas, thereby inducing a photoionization reaction of the desired isotope, and collecting the specific isotope ion by suitable ion collection means.

Maya, Jakob (Brookline, MA)

1991-01-01T23:59:59.000Z

32

Mantle Helium And Carbon Isotopes In Separation Creek Geothermal Springs,  

Open Energy Info (EERE)

Mantle Helium And Carbon Isotopes In Separation Creek Geothermal Springs, Mantle Helium And Carbon Isotopes In Separation Creek Geothermal Springs, Three Sisters Area, Central Oregon- Evidence For Renewed Volcanic Activity Or A Long Term Steady State System(Question) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Conference Paper: Mantle Helium And Carbon Isotopes In Separation Creek Geothermal Springs, Three Sisters Area, Central Oregon- Evidence For Renewed Volcanic Activity Or A Long Term Steady State System(Question) Details Activities (1) Areas (1) Regions (0) Abstract: Here we present the helium and carbon isotope results from the initial study of a fluid chemistry-monitoring program started in the summer of 2001 near the South Sister volcano in central Oregon. The Separation Creek area which is several miles due west of the volcano is the locus of

33

Laser Spectroscopy of Short Lived Rare Earth Isotopes  

Science Journals Connector (OSTI)

The ISAC facility at TRIUMF is able to produce intense beams of mass?separated radioactive isotopes of the alkali and the rare earth elements with unprecedented intensities. This will allow our laser spectroscopy collaboration to extend the studies of exotic nuclei for these elements further away from the valley of stability into regions so far inaccessible at other facilities thus allowing a more stringent test of the descriptive and predictive power of global nuclear models. Our effort which involves groups and researchers from the U.S. (TAMU) Japan (JAERI) and Canada (TRIUMF McGill and Calgary Universities) is based on collinear laser spectroscopy in a fast beam. In this method atoms or ions are excited by laser light in collinear geometry. In this way measurements of the optical isotope shift yield the nuclear charge radii and measurements of the hyperfine structure the nuclear moments. The excitation can be done by cw?lasers or alternatively by pulsed lasers without a loss in sensitivity if bunched radioactive ion beams are available. In its basic version the resonances of the spectral lines are observed optically at right angles. However the sensitivity will be increased through modifications using particle or nuclear radiation detection. The progress and the plans of our collaboration will be described.

H. A. Schuessler; F. Buchinger; H. Iimura

2003-01-01T23:59:59.000Z

34

METHOD TO TEST ISOTOPIC SEPARATION EFFICIENCY OF PALLADIUM PACKED COLUMNS  

SciTech Connect

The isotopic effect of palladium has been applied in different ways to separate hydrogen isotopes for many years. At Savannah River Site palladium deposited on kieselguhr (Pd/k) is used in a thermal cycling absorption process (TCAP) to purify tritium for over ten years. The need to design columns for different throughputs and the desire to advance the performance of TCAP created the need to evaluate different column designs and packing materials for their separation efficiency. In this work, columns with variations in length, diameter and metal foam use, were tested using an isotope displacement method. A simple computer model was also developed to calculate the number of theoretical separation stages using the test results. The effects of column diameter, metal foam and gas flow rate were identified.

Heung, L; Gregory Staack, G; James Klein, J; William Jacobs, W

2007-06-27T23:59:59.000Z

35

Gaseous isotope separation using solar wind phenomena  

Science Journals Connector (OSTI)

...the use of light carrier gas, a necessity that greatly...the separative process. Gases with low molecular weight...manner similar to that of a turbine, can be placed just outside...the calculation of light gases, we have not included...the author was measuring solar wind parameters under...

Chia-Gee Wang

1980-01-01T23:59:59.000Z

36

Autoresonant ion cyclotron isotope separation and J. Robiche  

E-Print Network (OSTI)

ion cyclotron resonance (ICR) heating1­10 are preferred but they do suffer of a very low throughout of methods related to Calutron and ICR heating: we used a cyclotron resonance, but in a purely static fieldAutoresonant ion cyclotron isotope separation J.-M. Raxa and J. Robiche Laboratoire de Physique et

37

Advancement of isotope separation for the production of reference standards  

SciTech Connect

Idaho National Laboratory (INL) operates a mass separator that is currently producing high purity isotopes for use as internal standards for high precision isotope dilution mass spectrometry (IDMS). In 2008, INL began the revival of the vintage 1970’s era instrument. Advancements thus far include the successful upgrading and development of system components such as the vacuum system, power supplies, ion-producing components, and beam detection equipment. Progress has been made in the separation and collection of isotopic species including those of Ar, Kr, Xe, Sr, and Ba. Particular focuses on ion source improvements and developments have proven successful with demonstrated output beam currents of over 10 micro-amps 138Ba and 350nA 134Ba from a natural abundance source charge (approximately 2.4 percent 134Ba). In order to increase production and collection of relatively high quantities (mg levels) of pure isotopes, several advancements have been made in ion source designs, source material introduction, and beam detection and collection. These advancements and future developments will be presented.

Jared Horkley; Christopher McGrath; Andrew Edwards; Gaven Knighton; Kevin Carney; Jacob Davies; James Sommers; Jeffrey Giglio

2012-03-01T23:59:59.000Z

38

Isotope separation with the RICH detector of the AMS Experiment  

E-Print Network (OSTI)

The Alpha Magnetic Spectrometer (AMS), to be installed on the International Space Station (ISS) in 2008, is a cosmic ray detector with several subsystems, one of which is a proximity focusing Ring Imaging Cherenkov (RICH) detector. This detector will be equipped with a dual radiator (aerogel+NaF), a lateral conical mirror and a detection plane made of 680 photomultipliers and light guides, enabling precise measurements of particle electric charge and velocity. Combining velocity measurements with data on particle rigidity from the AMS Tracker it is possible to obtain a measurement for particle mass, allowing the separation of isotopes. A Monte Carlo simulation of the RICH detector, based on realistic properties measured at ion beam tests, was performed to evaluate isotope separation capabilities. Results for three elements -- H (Z=1), He (Z=2) and Be (Z=4) -- are presented.

Luísa Arruda; Fernando Barão; João Borges; Fernando Carmo; Patrícia Gonçalves; Rui Pereira; Mário Pimenta

2007-10-03T23:59:59.000Z

39

Implications of Plutonium isotopic separation on closed fuel cycles and repository design  

SciTech Connect

Advances in laser enrichment may enable relatively low-cost plutonium isotopic separation. This would have large impacts on LWR closed fuel cycles and waste management. If Pu-240 is removed before recycling plutonium as mixed oxide (MOX) fuel, it would dramatically reduce the buildup of higher plutonium isotopes, Americium, and Curium. Pu-240 is a fertile material and thus can be replaced by U-238. Eliminating the higher plutonium isotopes in MOX fuel increases the Doppler feedback, simplifies reactor control, and allows infinite recycle of MOX plutonium in LWRs. Eliminating fertile Pu-240 and Pu-242 reduces the plutonium content in MOX fuel and simplifies fabrication. Reducing production of Pu-241 reduces production of Am-241 - the primary heat generator in spent nuclear fuels after several decades. Reducing heat generating Am-241 would reduce repository cost and waste toxicity. Avoiding Am- 241 avoids its decay product Np-237, a nuclide that partly controls long-term oxidizing repository performance. Most of these benefits also apply to LWR plutonium recycled into fast reactors. There are benefits for plutonium isotopic separation in fast reactor fuel cycles (particularly removal of Pu-242) but the benefits are less. (author)

Forsberg, C. [Massachusetts Institute of Technology, 77 Massachusetts Ave. Cambridge, MA 20129 (United States)

2013-07-01T23:59:59.000Z

40

Methods for separating medical isotopes using ionic liquids  

SciTech Connect

A method for extracting a radioisotope from an aqueous solution, the method comprising: a) intimately mixing a non-chelating ionic liquid with the aqueous solution to transfer at least a portion of said radioisotope to said non-chelating ionic liquid; and b) separating the non-chelating ionic liquid from the aqueous solution. In preferred embodiments, the method achieves an extraction efficiency of at least 80%, or a separation factor of at least 1.times.10.sup.4 when more than one radioisotope is included in the aqueous solution. In particular embodiments, the method is applied to the separation of medical isotopes pairs, such as Th from Ac (Th-229/Ac-225, Ac-227/Th-227), or Ra from Ac (Ac-225 and Ra-225, Ac-227 and Ra-223), or Ra from Th (Th-227 and Ra-223, Th-229 and Ra-225).

Luo, Huimin; Boll, Rose Ann; Bell, Jason Richard; Dai, Sheng

2014-10-21T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


41

Laser Ablation Molecular Isotopic Spectrometry: Parameter influence on boron isotope measurements  

Science Journals Connector (OSTI)

Laser Ablation Molecular Isotopic Spectrometry (LAMIS) was recently reported for optical isotopic analysis of condensed samples in ambient air and at ambient pressure. LAMIS utilizes molecular emissions which exhibit larger isotopic spectral shits than in atomic transitions. For boron monoxide 10BO and 11BO, the isotopic shifts extend from 114 cm?1 (0.74 nm) to 145–238 cm?1 (5–8 nm) at the B 2?+ (v = 0) ? X 2?+ (v = 2) and A 2?i (v = 0) ? X 2?+ (v = 3) transitions, respectively. These molecular isotopic shifts are over two orders of magnitude larger than the maximum isotopic shift of approximately 0.6 cm?1 in atomic boron. This paper describes how boron isotope abundance can be quantitatively determined using LAMIS and how atomic, ionic, and molecular optical emission develops in a plasma emanating from laser ablation of solid samples with various boron isotopic composition. We demonstrate that requirements for spectral resolution of the measurement system can be significantly relaxed when the isotopic abundance ratio is determined using chemometric analysis of spectra. Sensitivity can be improved by using a second slightly delayed laser pulse arriving into an expanding plume created by the first ablation pulse.

Xianglei Mao; Alexander A. Bol'shakov; Dale L. Perry; Osman Sorkhabi; Richard E. Russo

2011-01-01T23:59:59.000Z

42

Isotopic Analysis At Separation Creek Area (Van Soest, Et Al., 2002) | Open  

Open Energy Info (EERE)

Isotopic Analysis At Separation Creek Area (Van Soest, Et Al., 2002) Isotopic Analysis At Separation Creek Area (Van Soest, Et Al., 2002) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Isotopic Analysis- Fluid At Separation Creek Area (Van Soest, Et Al., 2002) Exploration Activity Details Location Separation Creek Area Exploration Technique Isotopic Analysis- Fluid Activity Date Usefulness useful DOE-funding Unknown References M. C. van Soest, B. M. Kennedy, W. C. Evans, R. H. Mariner (2002) Mantle Helium And Carbon Isotopes In Separation Creek Geothermal Springs, Three Sisters Area, Central Oregon- Evidence For Renewed Volcanic Activity Or A Long Term Steady State System(Question) Retrieved from "http://en.openei.org/w/index.php?title=Isotopic_Analysis_At_Separation_Creek_Area_(Van_Soest,_Et_Al.,_2002)&oldid=687475"

43

Liquid-phase thermal diffusion isotope separation apparatus and method having tapered column  

DOE Patents (OSTI)

A thermal diffusion counterflow method and apparatus for separating isotopes in solution in which the solution is confined in a long, narrow, vertical slit which tapers from bottom to top. The variation in the width of the slit permits maintenance of a stable concentration distribution with relatively long columns, thus permitting isotopic separation superior to that obtained in the prior art.

Rutherford, W.M.

1985-12-04T23:59:59.000Z

44

The laser ion source trap for highest isobaric selectivity in online exotic isotope production  

SciTech Connect

The improvement in the performance of a conventional laser ion source in the laser ion source and trap (LIST) project is presented, which envisages installation of a repeller electrode and a linear Paul trap/ion guide structure. This approach promises highest isobaric purity and optimum temporal and spatial control of the radioactive ion beam produced at an online isotope separator facility. The functionality of the LIST was explored at the offline test separators of University of Mainz (UMz) and ISOLDE/CERN, using the UMz solid state laser system. Ionization efficiency and selectivity as well as time structure and transversal emittance of the produced ion beam was determined. Next step after complete characterization is the construction and installation of the radiation-hard final trap structure and its first online application.

Schwellnus, F.; Gottwald, T.; Mattolat, C.; Wendt, K. [Institut fuer Physik, Johannes Gutenberg-Universitaet, D-55099 Mainz (Germany); Blaum, K. [Max-Planck-Institut fuer Kernphysik, Saupfercheckweg 1, D-69117 Heidelberg (Germany); Catherall, R.; Crepieux, B.; Fedosseev, V.; Marsh, B.; Rothe, S.; Stora, T. [CERN, CH-1211 Geneva 23 (Switzerland); Kluge, H.-J. [GSI, Planckstrasse 1, D-64291 Darmstadt (Germany)

2010-02-15T23:59:59.000Z

45

Quantifying Uranium Isotope Ratios Using Resonance Ionization Mass Spectrometry: The Influence of Laser Parameters on Relative Ionization Probability  

SciTech Connect

Resonance Ionization Mass Spectrometry (RIMS) has been developed as a method to measure relative uranium isotope abundances. In this approach, RIMS is used as an element-selective ionization process to provide a distinction between uranium atoms and potential isobars without the aid of chemical purification and separation. We explore the laser parameters critical to the ionization process and their effects on the measured isotope ratio. Specifically, the use of broad bandwidth lasers with automated feedback control of wavelength was applied to the measurement of {sup 235}U/{sup 238}U ratios to decrease laser-induced isotopic fractionation. By broadening the bandwidth of the first laser in a 3-color, 3-photon ionization process from a bandwidth of 1.8 GHz to about 10 GHz, the variation in sequential relative isotope abundance measurements decreased from >10% to less than 0.5%. This procedure was demonstrated for the direct interrogation of uranium oxide targets with essentially no sample preparation. A rate equation model for predicting the relative ionization probability has been developed to study the effect of variation in laser parameters on the measured isotope ratio. This work demonstrates that RIMS can be used for the robust measurement of uranium isotope ratios.

Isselhardt, B H

2011-09-06T23:59:59.000Z

46

Nuclear Charge Radii of Neutron-Deficient Lead Isotopes Beyond N=104 Midshell Investigated by In-Source Laser Spectroscopy  

Science Journals Connector (OSTI)

The shape of exotic even-mass Pb182–190 isotopes was probed by measurement of optical isotope shifts providing mean square charge radii (??r2?). The experiment was carried out at the isolde (cern) on-line mass separator, using in-source laser spectroscopy. Small deviations from the spherical droplet model are observed, but when compared to model calculations, those are explained by high sensitivity of ??r2? to beyond mean-field correlations and small admixtures of intruder configurations in the ground state. The data support the predominantly spherical shape of the ground state of the proton-magic Z=82 lead isotopes near neutron midshell (N=104).

H. De Witte et al.

2007-03-16T23:59:59.000Z

47

Mantle Helium And Carbon Isotopes In Separation Creek Geothermal...  

Open Energy Info (EERE)

we present the helium and carbon isotope results from the initial study of a fluid chemistry-monitoring program started in the summer of 2001 near the South Sister volcano in...

48

Laser isotope purification of lead for use in semiconductor chip interconnects  

SciTech Connect

Lead, used throughout the electronics industries, typically contains small amounts of radioactive {sup 210}Pb (a daughter product of the planet`s ubiquitous {sup 210}U) whose {sup 210}Po daughter emits and {alpha}-particle that is known to cause soft errors in electronic circuits. The {sup 210}Pb is not easily separable by chemical means. This paper describes the generic Atomic Vapor Laser Isotope Separation (AVLIS) process developed at the Lawrence Livermore National Laboratory (LLNL) over the last 20 years, with particular emphasis on recent efforts to develop the process physics and component technologies required to remove the offending {sup 210}Pb using lasers. We have constructed a developmental facility that includes a process laser development area and a test bed for the vaporizer and ion and product collectors. We will be testing much of the equipment and demonstrating pilot-scale AVLIS on a surrogate material later this year. Detection of the very low alpha emission even from commercially available low-alpha lead is challenging. LLNL`s detection capabilities will be described. The goal of the development of lead purification technology is to demonstrate the capability in FY97, and to begin filling orders of up to several MT/y of isotopically purified material in FY98.

Scheibner, K.; Haynam, C.; Worden, E.; Esser, B.

1996-02-01T23:59:59.000Z

49

Experimental studies of electron impact depopulation of excited states of atoms: applications to laser development for fusion and isotope separation. Final report, 1 January 1977-30 June 1979  

SciTech Connect

Motivated by the need for measurements of metastable depopulation mechanisms of Ar and Kr in the KrF rare-gas monohalide excimer laser, an ultra-high vacuum triple crossed-beams apparatus has been designed, fabricated, and assembled for the purpose of studying electron scattering from excited states of Ar and Kr atoms. A beam of metastable rare gas atoms, produced by near-resonant charge transfer of rare gas ions with alkali neutral atoms, is crossed by an electron beam and a far-red laser beam along mutually orthogonal axes. A hemispherical electron monochromator-spectrometer pair is used to measure the cross section for electron scattering from the 2p/sub 9/ excited state of the rare gas atom. Testing of parts of the assembled apparatus has been completed.

Lubell, M.S.

1980-06-01T23:59:59.000Z

50

Construction and Commissioning of a Collinear Laser Spectroscopy Setup at TRIGA Mainz and Laser Spectroscopy of Magnesium Isotopes at ISOLDE (CERN)  

E-Print Network (OSTI)

Construction and Commissioning of a Collinear Laser Spectroscopy Setup at TRIGA Mainz and Laser Spectroscopy of Magnesium Isotopes at ISOLDE (CERN)

Kraemer, Joerg

51

Laser trapping of short-lived radioactive isotopes  

Science Journals Connector (OSTI)

We describe an experiment which demonstrates the feasibility of trapping significant quantities of short-lived radioactive atoms with laser light. A thermal beam of 22.5 sec half-life Na21 atoms was produced on-line at the LBL 88’’ Cyclotron. After decelerating the beam using a Zeeman-tuned slowing technique we stored about 4×103 Na21 atoms in a magneto-optical trap. The number of trapped atoms is large enough to be used in experimental studies of the beta decay of Na21. The basic method can be adapted for other rare isotopes.

Z-T. Lu; C. Bowers; S. J. Freedman; B. K. Fujikawa; J. L. Mortara; S-Q. Shang; K. P. Coulter; L. Young

1994-06-13T23:59:59.000Z

52

Separation Processes, Second Edition  

E-Print Network (OSTI)

by; Uranium isotopes separation) Iteration methods (seemethod for activity coefficients, 43, 481 Uranium isotopes separation,

King, C. Judson

1980-01-01T23:59:59.000Z

53

Influence of liquid structure on diffusive isotope separation in molten silicates and aqueous solutions  

SciTech Connect

Molecular diffusion in natural volcanic liquids discriminates between isotopes of major ions (e.g., Fe, Mg, Ca, and Li). Although isotope separation by diffusion is expected on theoretical grounds, the dependence on mass is highly variable for different elements and in different media. Silicate liquid diffusion experiments using simple liquid compositions were carried out to further probe the compositional dependence of diffusive isotopic discrimination and its relationship to liquid structure. Two diffusion couples consisting of the mineral constituents anorthite (CaAl{sub 2}Si{sub 2}O{sub 8}; denoted AN), albite (NaAlSi{sub 3}O{sub 8}; denoted AB), and diopside (CaMgSi{sub 2}O{sub 6}; denoted DI) were held at 1450°C for 2 h and then quenched to ambient pressure and temperature. Major-element as well as Ca and Mg isotope profiles were measured on the recovered quenched glasses. In both experiments, Ca diffuses rapidly with respect to Si. In the AB–AN experiment, D{sub Ca}/D{sub Si} ~ 20 and the efficiency of isotope separation for Ca is much greater than in natural liquid experiments where D{sub Ca}/D{sub Si} ~ 1. In the AB–DI experiment, D{sub Ca}/D{sub Si} ~ 6 and the efficiency of isotope separation is between that of the natural liquid experiments and the AB–AN experiment. In the AB–DI experiment, D{sub Mg}/D{sub Si} ~ 1 and the efficiency of isotope separation for Mg is smaller than it is for Ca yet similar to that observed for Mg in natural liquids. The results from the experiments reported here, in combination with results from natural volcanic liquids, show clearly that the efficiency of diffusive separation of Ca isotopes is systematically related to the solvent-normalized diffusivity—the ratio of the diffusivity of the cation (D{sub Ca}) to the diffusivity of silicon (D{sub Si}). The results on Ca isotopes are consistent with available data on Fe, Li, and Mg isotopes in silicate liquids, when considered in terms of the parameter D{sub cation}/D{sub Si}. Cations diffusing in aqueous solutions display a similar relationship between isotopic separation efficiency and D{sub cation} =D{sub H 2 O} , although the efficiencies are smaller than in silicate liquids. Our empirical relationship provides a tool for predicting the magnitude of diffusive isotopic effects in many geologic environments and a basis for a more comprehensive theory of isotope separation in liquid solutions. We present a conceptual model for the relationship between diffusivity and liquid structure that is consistent with available data.

Watkins, J.M.; DePaolo, D.J.; Ryerson, F.J.; Peterson, B.

2011-03-01T23:59:59.000Z

54

Investigation related to hydrogen isotopes separation by cryogenic distillation  

SciTech Connect

Research conducted in the last fifty years has shown that one of the most efficient techniques of removing tritium from the heavy water used as moderator and coolant in CANDU reactors (as that operated at Cernavoda (Romania)) is hydrogen cryogenic distillation. Designing and implementing the concept of cryogenic distillation columns require experiments to be conducted as well as computer simulations. Particularly, computer simulations are of great importance when designing and evaluating the performances of a column or a series of columns. Experimental data collected from laboratory work will be used as input for computer simulations run at larger scale (for The Pilot Plant for Tritium and Deuterium Separation) in order to increase the confidence in the simulated results. Studies carried out were focused on the following: - Quantitative analyses of important parameters such as the number of theoretical plates, inlet area, reflux flow, flow-rates extraction, working pressure, etc. - Columns connected in series in such a way to fulfil the separation requirements. Experiments were carried out on a laboratory-scale installation to investigate the performance of contact elements with continuous packing. The packing was manufactured in our institute. (authors)

Bornea, A.; Zamfirache, M.; Stefanescu, I.; Preda, A.; Balteanu, O.; Stefan, I. [INC-DTCI-ICSI Rm. Valcea, str.Uzinei, Nr.4, 240050 (Romania)

2008-07-15T23:59:59.000Z

55

Startup and Operation of a Metal Hydride Based Isotope Separation Process  

SciTech Connect

Production scale separation of tritium from other hydrogen isotopes at the Savannah River Site (SRS) in Aiken, SC, has been accomplished by several methods. These methods include thermal diffusion (1957--1986), fractional absorption (1964--1968), and cryogenic distillation (1967-present). Most recently, the Thermal Cycling Absorption Process (TCAP), a metal hydride based hydrogen isotope separation system, began production in the Replacement Tritium Facility (RTF) on April 9, 1994. TCAP has been in development at the Savannah River Technology Center since 1980. The production startup of this semi-continuous gas chromatographic separation process is a significant accomplishment for the Savannah River Site and was achieved after years of design, development, and testing.

Scogin, J.H.; Poore, A.S.

1995-02-27T23:59:59.000Z

56

Multiple isotope magneto-optical trap from a single diode laser  

Science Journals Connector (OSTI)

We present a dual isotope magneto-optical trap produced using a single diode laser. We generate all the optical frequencies needed for trapping both species using a fiber intensity...

Valenzuela, Victor Manuel; Hamzeloui, Saeed; Gutiérrez, Monica; Gomez, Eduardo

2013-01-01T23:59:59.000Z

57

Development of a compact quantum cascade laser spectrometer for field measurements of CO2 isotopes  

Science Journals Connector (OSTI)

We report the development of a field-deployable, pulsed quantum cascade laser spectrometer. The instrument is designed to measure...13C/12C isotopic ratio in the CO2 released from volcanic vents. Specific 12CO2 a...

D. Weidmann; G. Wysocki; C. Oppenheimer; F.K. Tittel

2005-02-01T23:59:59.000Z

58

Lithium Isotope Separation & Enrichment Technologies (4577), 2/9/2012  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

Lithium Isotope Separation & Enrichment Technologies (4577) Lithium Isotope Separation & Enrichment Technologies (4577) Program or Field Office: Y-12 Site Office Location(s) (City/County/State): Oak Ridge, Anderson County, Tennessee Proposed Action Description: Submit by E-mail This is entirely a paper study. The scope of this Cooperative Research and Development (CRADA) is to: 1) systematically review existing potential lithium enrichment processes, 2) evaluate the individual process, 3) determine the economic feasibility, 4) rank the processes as a function of economic feasibility, technical probability, Health, Safety and Environmental impacts, 5) identify best candidate technology for proof of principle evaluation, 6) develop outside funding proposals, and 7) pursue funding to perform proof of principle/prototyping of candidate

59

Carbon isotope separation by absorptive distillation. [Data between 77. 4 and 114. 3 K; Henry's law behavior  

SciTech Connect

The feasibility of separating carbon isotopes by absorptive distillation has been studied for CO absorption by cryogenic solvents. Phase equilibrium, isotopic separation, and mass transfer data were taken between 77.4 and 114.3 K for the following solvents: propane, propylene, 1:1 propane-propylene, 1-butene, isobutane and nitrogen. Carbon monoxide solubility followed Henry's Law, with a maximum experimental solubility of 6.5 mole per cent. Isotopic separation between CO in the gas and liquid phases using hydrocarbon solvents was several times that for pure CO vapor-liquid equilibrium. The maximum observed isotopic separation factor was 1.029 at 77.4 K with the propane-propylene solvent mixture. Mass transfer measurements yielded calculated HTU's of 2 to 5 cm for a possible separation system. An attempt has been made to correlate isotopic separation data using Hildebrand's theory of solutions. The differential absorption of isotopic CO species is expressed as a difference in solubility of the isotopic CO molecules. Data for propane, propylene, and 1-butene show approximately the same behavior at varying temperatures.

Mills, T.R.

1980-04-01T23:59:59.000Z

60

Determination of the separation coefficients of the isotopes of boron in the equilibrium evaporation of BCl3  

Science Journals Connector (OSTI)

The separation coefficients of the isotopes of boron are determined for equilibrium evaporation of boron chloride in the temperature interval 12.7 to 85 °C. The methods are described, and the equation relating...

N. N. Sevryugova; O. V. Uvarov; N. M. Zhavoronkov

1956-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


61

Isotopic Ratio Measurements of Atmospheric Carbon Dioxide Using a 4.3 ?m Pulsed Quantum Cascade Laser  

Science Journals Connector (OSTI)

We report CO2 isotopic ratios (13C, 18O) measured in air using a pulsed quantum cascade laser at 2310 cm-1. Performance is...

Nelson, David; McManus, John B; Zahniser, Mark S; Tuzson, Bela; Emmenegger, Lukas

62

Separation Of Uranium And Plutonium Isotopes For Measurement By Multi Collector Inductively Coupled Plasma Mass Spectroscopy  

SciTech Connect

Uranium (U) and plutonium (Pu) isotopes in coral soils, contaminated by nuclear weapons testing in the northern Marshall Islands, were isolated by ion-exchange chromatography and analyzed by mass spectrometry. The soil samples were spiked with {sup 233}U and {sup 242}Pu tracers, dissolved in minerals acids, and U and Pu isotopes isolated and purified on commercially available ion-exchange columns. The ion-exchange technique employed a TEVA{reg_sign} column coupled to a UTEVA{reg_sign} column. U and Pu isotope fractions were then further isolated using separate elution schemes, and the purified fractions containing U and Pu isotopes analyzed sequentially using multi-collector inductively coupled plasma mass spectrometer (MCICP-MS). High precision measurements of {sup 234}U/{sup 235}U, {sup 238}U/{sup 235}U, {sup 236}U/{sup 235}U, and {sup 240}Pu/{sup 239}Pu in soil samples were attained using the described methodology and instrumentation, and provide a basis for conducting more detailed assessments of the behavior and transfer of uranium and plutonium in the environment.

Martinelli, R E; Hamilton, T F; Williams, R W; Kehl, S R

2009-03-29T23:59:59.000Z

63

Periodic index separate confinement heterostructure multiple quantum well laser' n by organometailic vapor  

E-Print Network (OSTI)

similar conditions. The PINSCH laser uses cladding layers comprised of periodic semiconductor multilayers applied to 980 nm InGaAs/AlGaAs quantum well lasers.6 The cladding layers consist of alternating layersPeriodic index separate confinement heterostructure multiple quantum well laser' n

Florida, University of

64

A Transient Model of Induced Natural Circulation Thermal Cycling for Hydrogen Isotope Separation  

SciTech Connect

The property of selective temperature dependence of adsorption and desorption of hydrogen isotopes by palladium is used for isotope separation. A proposal to use natural circulation of nitrogen to alternately heat and cool a packed bed of palladium coated beads is under active investigation, and a device consisting of two interlocking natural convection loops is being designed. A transient numerical model of the device has been developed to aid the design process. It is a one-dimensional finite-difference model, using the Boussinesq approximation. The thermal inertia of the pipe walls and other heat structures as well as the heater control logic is included in the model. Two system configurations were modeled and results are compared.

SHADDAY, MARTIN

2005-07-12T23:59:59.000Z

65

Elemental and isotopic analysis of inorganic salts by laser desorption ionization mass spectrometry  

SciTech Connect

Laser desorption ionization mass spectrometry is applied for the analysis of elements as well as their isotopic composition in different inorganic salts. At very low laser energies the inorganic ions are desorbed and ionized from the thin layer of the sample surface. The naturally occurring isotopes of alkali and silver ions are resolved using time of flight mass spectrometer. Further increase in laser energy shows the appearance of Al, Cr, and Fe ions in the mass spectra. This indicates the penetration laser beam beyond the sample surface leading to the ablation of sample target at higher energies. The simultaneous appearance of atomic ions from the sample target at relatively higher laser energies hampers the unambiguous identification of amino acid residues from the biomolecular ions in MALDI-MS.

Jayasekharan, T.; Sahoo, N. K. [Applied Spectroscopy Division, Bhabha Atomic Research Centre, Mumbai 400 085 (India)

2013-02-05T23:59:59.000Z

66

Laser vaporization/ionization interface for coupling microscale separation techniques with mass spectrometry  

DOE Patents (OSTI)

The present invention provides a laser-induced vaporization and ionization interface for directly coupling microscale separation processes to a mass spectrometer. Vaporization and ionization of the separated analytes are facilitated by the addition of a light-absorbing component to the separation buffer or solvent. 8 figs.

Yeung, E.S.; Chang, Y.C.

1999-06-29T23:59:59.000Z

67

Laser annealing of neutron irradiated boron-10 isotope doped diamond  

Science Journals Connector (OSTI)

10B isotope doped p-type diamond epilayer grown by chemical vapor deposition on (110) oriented type IIa diamond single crystal substrate was subjected to neutron transmutation at a fluence of 2.4...

K. Jagannadham; M. J. Lance; J. E. Butler

2011-04-01T23:59:59.000Z

68

Isotopic Analysis of Uranium in NIST SRM Glass by Femtosecond Laser Ablation  

SciTech Connect

We employed femtosecond Laser Ablation Multicollector Inductively Coupled Mass Spectrometry for the 11 determination of uranium isotope ratios in a series of standard reference material glasses (NIST 610, 612, 614, and 12 616). This uranium concentration in this series of SRM glasses is a combination of isotopically natural uranium in 13 the materials used to make the glass matrix and isotopically depleted uranium added to increase the uranium 14 elemental concentration across the series. Results for NIST 610 are in excellent agreement with literature values. 15 However, other than atom percent 235U, little information is available for the remaining glasses. We present atom 16 percent and isotope ratios for 234U, 235U, 236U, and 238U for all four glasses. Our results show deviations from the 17 certificate values for the atom percent 235U, indicating the need for further examination of the uranium isotopes in 18 NIST 610-616. Our results are fully consistent with a two isotopic component mixing between the depleted 19 uranium spike and natural uranium in the bulk glass.

Duffin, Andrew M.; Hart, Garret L.; Hanlen, Richard C.; Eiden, Gregory C.

2013-05-19T23:59:59.000Z

69

Validation of Electrochemically Modulated Separations Performed On-Line with MC-ICP-MS for Uranium and Plutonium Isotopic Analyses  

SciTech Connect

The most time consuming process in uranium or plutonium isotopic analyses is performing the requisite chromatographic separation of the actinides. Filament preparation for thermal ionization (TIMS) adds further delays, but is generally accepted due to the unmatched performance in trace isotopic analyses. Advances in Multi-Collector Inductively Coupled Plasma Mass Spectrometry (MC-ICP-MS) are beginning to rival the performance of TIMS. Methods, such as Electrochemically Modulated Separations (EMS) can efficiently pre-concentrate U or Pu quite selectively from small solution volumes in a matrix of 0.5 M nitric acid. When performed in-line with ICP-MS, the rapid analyte release from the electrode is fast, and large transient analyte signal enhancements of >100 fold can be achieved as compared to more conventional continuous nebulization of the original starting solution. This makes the approach ideal for very low level isotope ratio measurements. In this paper, some aspects of EMS performance are described. These include low level Pu isotope ratio behavior versus concentration by MC-ICP-MS and uranium rejection characteristics that are also important for reliable low level Pu isotope ratio determinations.

Liezers, Martin; Olsen, Khris B.; Mitroshkov, Alexandre V.; Duckworth, Douglas C.

2010-08-11T23:59:59.000Z

70

Isotope shifts of natural Sr+ measured by laser fluorescence in a sympathetically cooled Coulomb crystal  

E-Print Network (OSTI)

We measured by laser spectroscopy the isotope shifts between naturally-occurring even-isotopes of strontium ions for both the $5s\\,\\,^2S_{1/2}\\to 5p\\,\\,^2P_{1/2}$ (violet) and the $4d\\,\\,^2D_{3/2}\\to 5p\\,\\,^2P_{1/2}$ (infrared) dipole-allowed optical transitions. Fluorescence spectra were taken by simultaneous measurements on a two-component Coulomb crystal in a linear Paul trap containing $10^3$--$10^4$ laser-cooled Sr$^+$ ions. The isotope shifts are extracted from the experimental spectra by fitting the data with the analytical solution of the optical Bloch equations describing a three-level atom in interaction with two laser beams. This technique allowed us to increase the precision with respect to previously reported data obtained by optogalvanic spectroscopy or fast atomic-beam techniques. The results for the $5s\\,\\,^2S_{1/2}\\to 5p\\,\\,^2P_{1/2}$ transition are $\

Brice Dubost; Romain Dubessy; Benjamin Szymanski; Samuel Guibal; Jean-Pierre Likforman; Luca Guidoni

2014-02-14T23:59:59.000Z

71

Quantum and classical separability of spin-orbit laser modes  

E-Print Network (OSTI)

In this work we investigate the quantum noise properties of polarization vortices in connection with an intensity based Clauser-Horne-Shimony-Holt inequality for their spin-orbit separability. We evaluate the inequality for different input quantum states and the corresponding intensity fluctuations. The roles played by coherence and photon number squeezing provide a suitable framework for characterizing pure state spin-orbit entanglement. Structural inseparability of the spin-orbit mode requires coherence, an issue concerning either classical or quantum descriptions. In both cases, it can be witnessed by violation of this intensity based CHSH inequality. However, in the quantum domain, entanglement requires both coherence and reduced photon number fluctuations.

L. J. Pereira; A. Z. Khoury; K. Dechoum

2014-09-02T23:59:59.000Z

72

Oxygen isotope ratio measurements in CO2 by means of a continuous-wave quantum cascade laser at 4.3 ?m  

Science Journals Connector (OSTI)

A mid-infrared laser spectrometer was developed for simultaneous high-precision 18O/16O and 17O/16O isotope ratio measurements in carbon...

Castrillo, Antonio; Casa, Giovanni; Gianfrani, Livio

2007-01-01T23:59:59.000Z

73

Laser Based Techniques for Ultra Trace Isotope Production, Spectroscopy and Detection  

SciTech Connect

A variety of research activities in the field of fundamental and applied nuclear physics has evolved in the last years using resonantly tuned radiation from powerful lasers. The technique of resonance ionization spectroscopy has delivered outstanding results and found broad acceptance in the last years as a particularly efficient and highly selective method for rare and exotic radioisotope studies. It is used for production, spectroscopy and detection of these species and provides complete isobaric, high isotopic and even some isomeric selection, which altogether is needed for on-line investigation of short lived species far off stability as well as for ultra trace determination. Good overall efficiency pushes the experimental limits of detection in elemental trace analysis down to below 106 atoms per sample, and additionally isotopic selectivity as high as 3 ? 1012 has been demonstrated. The widespread potential of resonance ionization techniques is discussed, focusing on the experimental arrangements for applications in selective on-line isotope production, spectroscopy of rare radioisotopes and ultra trace determination of radiotoxic isotopes like 238Pu to 244Pu, 135,137Cs, 89,90Sr or 41Ca in environmental, technical and biomedical samples.

Wendt, K.; Blaum, K; Geppert, C; Muller, P; Nortershauser, W.; Schmitt, Annette; Schumann, P; Trautmann, Norbert; Bushaw, Bruce A.

2006-06-26T23:59:59.000Z

74

Continuous production of tritium in an isotope-production reactor with a separate circulation system  

DOE Patents (OSTI)

A method is described for producing tritium in a fast breeder reactor cooled with liquid metal. Lithium is allowed to flow through the reactor in separate loops in order to facilitate the production and removal of tritium.

Cawley, W.E.; Omberg, R.P.

1982-08-19T23:59:59.000Z

75

Basic features of boron isotope separation by SILARC method in the two-step iterative static model  

Science Journals Connector (OSTI)

Boron isotopes have a broad spectrum of applications in industry. Naturally occurring boron consists of two stable isotopes—19.9 % of boron-10 and 81.1 % of boron-11. A useful property of pure boron-10 isotopes a...

K. A. Lyakhov; H. J. Lee

2013-05-01T23:59:59.000Z

76

Recent developments of the ion sources at Tri University Meson Factory/Isotope Separator and ACcelerator Facility  

SciTech Connect

This paper describes the recent progresses concerning the on-line ion source at the Tri University Meson Factory/Isotope Separator and ACcelerator (TRIUMF/ISAC) Radioactive Ion-Beam Facility; description of the new design of the surface-ion-source for improved stability of the beam intensity, description of the transport path to the east target station at ISAC, description of the new brazing techniques that solved recurrent problems with water leaks on the target/ion source assembly in the vacuum system, finally, recent developments concerning the Forced Electron Beam Induced Arc Discharge (FEBIAD) ion source are reported. In particular, a study on the effect of the plasma chamber volume on the ionization efficiency was completed.

Bricault, P. G.; Ames, F.; Dombsky, M.; Labrecque, F.; Lassen, J.; Mjos, A.; Minor, G. [TRIUMF, 4004 Wesbrook Mall, Vancouver, British Columbia V6T 2A3 (Canada); Tigelhoefer, A. [TRIUMF, 4004 Wesbrook Mall, Vancouver, British Columbia V6T 2A3 (Canada); Department Of Physics, University of Manitoba, Winnipeg, Manitoba R3T 2N2 (Canada)

2012-02-15T23:59:59.000Z

77

Isotopic imaging via nuclear resonance fluorescence with laser-based Thomson radiation  

DOE Patents (OSTI)

The present invention utilizes novel laser-based, high-brightness, high-spatial-resolution, pencil-beam sources of spectrally pure hard x-ray and gamma-ray radiation to induce resonant scattering in specific nuclei, i.e., nuclear resonance fluorescence. By monitoring such fluorescence as a function of beam position, it is possible to image in either two dimensions or three dimensions, the position and concentration of individual isotopes in a specific material configuration. Such methods of the present invention material identification, spatial resolution of material location and ability to locate and identify materials shielded by other materials, such as, for example, behind a lead wall. The foundation of the present invention is the generation of quasimonochromatic high-energy x-ray (100's of keV) and gamma-ray (greater than about 1 MeV) radiation via the collision of intense laser pulses from relativistic electrons. Such a process as utilized herein, i.e., Thomson scattering or inverse-Compton scattering, produces beams having diameters from about 1 micron to about 100 microns of high-energy photons with a bandwidth of .DELTA.E/E of approximately 10E.sup.-3.

Barty, Christopher P. J. (Hayward, CA); Hartemann, Frederic V. (San Ramon, CA); McNabb, Dennis P. (Alameda, CA); Pruet, Jason A. (Brentwood, CA)

2009-07-21T23:59:59.000Z

78

J. Phys. B AL Mol. Opt Phys. 26 (1993) 1569-1578. Printed in the UK Pure and mixed state calculationsof the laser-induced  

E-Print Network (OSTI)

, altemative methods for separating the elements of uranium are being studied, notably the use of lasers of the isotopes of uranium has major commercial importance in the nuclear fuel industry. As is well known to induce preferential ionization of 23sU(see Greenland 1991 for a review). Laser isotope separation relies

Ford, Ian

79

Fe isotope fractionation during phase separation in the NaCl–H2O system: An experimental study with implications for seafloor hydrothermal vents  

Science Journals Connector (OSTI)

Abstract Phase separation has been proposed as a possible mechanism contributing to the Fe isotope composition of hydrothermal fluids at mid-ocean ridges. The uncertainty results largely from the emphasis on field data that can involve competing processes that obscure cause and effect of any one process. To better understand the potential significance of phase separation in the NaCl–Fe–H2O system on Fe isotope fractionation, temperature and pressure of a Fe-bearing NaCl fluid in a titanium flow reactor were carefully adjusted to produce vapor ± liquid ± halite, while the Fe isotope composition between coexisting phases was monitored. Two different P–T regions were emphasized: (1) 424–420?°C, 35.2–31.5 MPa; and (2) 464–466?°C, 29.8–24.7 MPa. Both regions were chosen to simulate the range of physical conditions that are experienced by hydrothermal fluids at mid-ocean ridges (MORs). Decompression induced phase separation in both P–T regions results in the vapor phase becoming enriched in the heavier isotopes of Fe, as the Fe/Cl ratio decreases. The coexisting NaCl-rich liquid phase remains essentially constant with respect to Fe/Cl ratio and Fe isotope composition. Coinciding with the lowest vapor chlorinity in the vapor–liquid stability field, the Fe/Cl ratio of the vapor abruptly increases, while the Fe isotope fractionation between the vapor and liquid ( 10 3 ln ? ? V / L 56 / 54 ) reached a maximum value of + 0.145 ± 0.048 ‰ . Subsequently, Fe isotope fractionation decreased upon transition into the vapor–halite stability field (P–T region 2). We infer that the observed Fe isotope fractionation between vapor ± liquid ± halite is caused by differences in Fe speciation among coexisting chloride-bearing phases. The experimental study confirms for the first time that measurable Fe isotope variability can result from phase separation in high temperature hydrothermal systems. The species-dependent Fe isotope fractionation reported here is small relative to predicted mineral–mineral and mineral–fluid fractionations, especially if redox effects are involved as might occur during vent fluid–seawater mixing reactions and/or magmatic activity associated with seafloor eruptive episodes.

Drew D. Syverson; Nicholas J. Pester; Paul R. Craddock; William E. Seyfried Jr.

2014-01-01T23:59:59.000Z

80

A Mass Spectrometry Study of Isotope Separation in the Laser Plume  

E-Print Network (OSTI)

transition from the plasma in atmosphere to the high vacuumin atmosphere given the appropriate plasma conditions and

Suen, Timothy Wu

2012-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


81

A Mass Spectrometry Study of Isotope Separation in the Laser Plume  

E-Print Network (OSTI)

and Background 1.1 Nuclear Safeguards and Nuclearby TIMS for nuclear safeguards”, Analytica Chimica Acta 688,Atomic Energy Agency, IAEA Safeguards Glossary, 2002. [11

Suen, Timothy Wu

2012-01-01T23:59:59.000Z

82

A Mass Spectrometry Study of Isotope Separation in the Laser Plume  

E-Print Network (OSTI)

quantities of natural or depleted uranium [8]. Plutonium, on235 U abundance in depleted uranium. The sample was ablatedsuch as 235 U in depleted uranium [64] or short-lived

Suen, Timothy Wu

2012-01-01T23:59:59.000Z

83

Cr-doped scandium borate laser  

DOE Patents (OSTI)

A broadly wavelength-tunable laser is provided which comprises as the laser medium a single crystal of MBO.sub.3 :Cr.sup.3+, where M is selected from the group of Sc, In and Lu. The laser may be operated over a broad temperature range from cryogenic temperatures to elevated temperatures. Emission is in a spectral range from red to infrared, and the laser is useful in the fields of defense, communications, isotope separation, photochemistry, etc.

Chai, Bruce H. (Bridgewater, NJ); Lai, Shui T. (Florham Park, NJ); Long, Margaret N. (Landing, NJ)

1989-01-01T23:59:59.000Z

84

Detection of slow atoms confined in a Cesium vapor cell by spatially separated pump and probe laser beams  

E-Print Network (OSTI)

Detection of slow atoms confined in a Cesium vapor cell by spatially separated pump and probe laser distribution of atoms in a thermal gas is usually described through a Maxwell-Boltzman distribution of energy, and assumes isotropy. As a consequence, the probability for an atom to leave the surface under an azimuth

Boyer, Edmond

85

Research Directed at Developing a Classical Theory to Describe Isotope Separation of Polyatomic Molecules Illuminated by Intense Infrared Radiation. Final Report for period May 7, 1979 to September 30, 1979; Extension December 31, 1997  

DOE R&D Accomplishments (OSTI)

This final report describes research on the theory of isotope separation produced by the illumination of polyatomic molecules by intense infrared laser radiation. This process is investigated by treating the molecule, sulfur hexafluoride, as a system of seven classical particles that obey the Newtonian equations of motion. A minicomputer is used to integrate these differential equations. The particles are acted on by interatomic forces, and by the time-dependent electric field of the laser. We have a very satisfactory expression for the interaction of the laser and the molecule which is compatible with infrared absorption and spectroscopic data. The interatomic potential is capable of improvement, and progress on this problem is still being made. We have made several computer runs of the dynamical behavior of the molecule using a reasonably good model for the interatomic force law. For the laser parameters chosen, we find that typically the molecule passes quickly through the resonance region into the quasi-continuum and even well into the real continuum before dissociation actually occurs. When viewed on a display terminal, the motions are exceedingly complex. As an aid to the visualization of the process, we have made a number of 16 mm movies depicting a three-dimensional representation of the motion of the seven particles. These show even more clearly the enormous complexity of the motions, and make clear the desirability of finding ways of characterizing the motion in simple ways without giving all of the numerical detail. One of the ways to do this is to introduce statistical parameters such as a temperature associated with the distribution of kinetic energies of the single particle. We have made such an analysis of our data runs, and have found favorable indications that such methods will prove useful in keeping track of the dynamical histories.

Lamb, W. E. Jr.

1981-12-00T23:59:59.000Z

86

Laser beam control and diagnostic systems for the copper-pumped dye laser system at Lawrence Livermore National Laboratory  

SciTech Connect

The laser system described in the previous paper is used for experiments in which success requires tight tolerances on beam position, direction, and wavefront. Indeed, the optimum performance of the laser itself depends on careful delivery of copper laser light to the dye amplifiers, precise propagation of dye laser beams through restricted amplifier apertures, and accurate monitoring of laser power at key locations. This paper describes the alignment systems, wavefront correction systems, and laser diagnostics systems which ensure that the control requirements of both the laser and associated experiments are met. Because laser isotope separation processes utilize more than one wavelength, these systems monitor and control multiple wavelengths simultaneously.

Bliss, E.S.; Peterson, R.L.; Salmon, J.T.; Thomas, R.A.

1992-11-01T23:59:59.000Z

87

unstable isotope  

Science Journals Connector (OSTI)

unstable isotope, radioisotope ? unstabiles Isotop n, nichtstabiles Isotop, radioaktives Isotop, Radioisotop

2014-08-01T23:59:59.000Z

88

Purification, Recovery, and Laser-Driven Fluorination of Silicon from Dissolved and Particulate Silica for the Measurement of Natural Stable Isotope Abundances  

Science Journals Connector (OSTI)

Purification, Recovery, and Laser-Driven Fluorination of Silicon from Dissolved and Particulate Silica for the Measurement of Natural Stable Isotope Abundances ... At least three simple techniques exist for this:? fusion of SiO2 with Na2CO3 to form water-soluble sodium silicate, dissolution in HF, or dissolution in NaOH. ...

Christina L. De La Rocha; Mark A. Brzezinski; Michael J. DeNiro

1996-11-01T23:59:59.000Z

89

Separation of microparticles suspended in a minichannel using laser radiation pressure  

Science Journals Connector (OSTI)

Optical separation, which is a contactless and accurate technique, has been mostly used to manipulate single particles. This work mainly aims to present an effective technique for...

Zabetian, Mohammad; Saidi, Mohammad Said; Shafii, Mohammad Behshad; Saidi, Mohammad Hassan

2013-01-01T23:59:59.000Z

90

Solid-state Marx based two-switch voltage modulator for the On-Line Isotope Mass Separator accelerator at the European Organization for Nuclear Research  

SciTech Connect

A new circuit topology is proposed to replace the actual pulse transformer and thyratron based resonant modulator that supplies the 60 kV target potential for the ion acceleration of the On-Line Isotope Mass Separator accelerator, the stability of which is critical for the mass resolution downstream separator, at the European Organization for Nuclear Research. The improved modulator uses two solid-state switches working together, each one based on the Marx generator concept, operating as series and parallel switches, reducing the stress on the series stacked semiconductors, and also as auxiliary pulse generator in order to fulfill the target requirements. Preliminary results of a 10 kV prototype, using 1200 V insulated gate bipolar transistors and capacitors in the solid-state Marx circuits, ten stages each, with an electrical equivalent circuit of the target, are presented, demonstrating both the improved voltage stability and pulse flexibility potential wanted for this new modulator.

Redondo, L. M.; Canacsinh, H.; Ferrao, N.; Mendes, C. [Instituto Superior de Engenharia de Lisboa (ISEL), R. Conselheiro Emidio Navarro 1, Lisbon 1959-007 (Portugal); Nuclear Physics Center-Lisbon University (CFNUL), Av. Prof. Gama Pinto 2, Lisbon 1649-003 (Portugal); Silva, J. Fernando [Instituto Superior Tecnico (IST), Universidade Tecnica de Lisboa, Av. Rovisco Pais 1, Lisbon 1049-001 (Portugal); Center for Innovation in Electrical and Energy Engineering-TU Lisbon, Av. Rovisco Pais 1, Lisbon 1049-001 (Portugal); Soares, R. [Nuclear Physics Center--Lisbon University (CFNUL), Av. Prof. Gama Pinto 2, Lisbon 1649-003 (Portugal); ABT Group, TE Department, Site de Prevessin, FR-01631 CERN (Switzerland); Schipper, J.; Fowler, A. [ABT Group, TE Department, Site de Prevessin, FR-01631 CERN (Switzerland)

2010-07-15T23:59:59.000Z

91

Isotope analysis of water by means of near infrared dual-wavelength diode laser spectroscopy  

Science Journals Connector (OSTI)

A novel diode laser spectrometer was developed using dualwavelength multiplexing, ensuring ideal conditions for high-precision and simultaneous measurements of the 2H/1H, 17O/16O, and...

Gianfrani, L; Gagliardi, G; van Burgel, M; Kerstel, Erik

2003-01-01T23:59:59.000Z

92

Laser Ablation Inductively Coupled Plasma Mass Spectrometry Measurement of Isotope Ratios in Depleted Uranium Contaminated Soils  

Science Journals Connector (OSTI)

Laser ablation of pressed soil pellets was examined as a means of direct sample introduction to enable inductively coupled plasma mass spectrometry (ICP-MS) screening of soils for...

Seltzer, Michael D

2003-01-01T23:59:59.000Z

93

Laser spectroscopy of francium isotopes at the borders of the region of reflection asymmetry  

E-Print Network (OSTI)

The magnetic dipole moments and changes in mean-square charge radii of the neutron-rich $^{218m,219,229,231}\\text{Fr}$ isotopes were measured with the newly-installed Collinear Resonance Ionization Spectroscopy (CRIS) beam line at ISOLDE, CERN, probing the $7s~^{2}S_{1/2}$ to $8p~^{2}P_{3/2}$ atomic transition. The $\\delta\\langle r^{2}\\rangle^{A,221}$ values for $^{218m,219}\\text{Fr}$ and $^{229,231}\\text{Fr}$ follow the observed increasing slope of the charge radii beyond $N~=~126$. The charge radii odd-even staggering in this neutron-rich region is discussed, showing that $^{220}\\text{Fr}$ has a weakly inverted odd-even staggering while $^{228}\\text{Fr}$ has normal staggering. This suggests that both isotopes reside at the borders of a region of inverted staggering, which has been associated with reflection-asymmetric shapes. The $g(^{219}\\text{Fr}) = +0.69(1)$ value supports a $\\pi 1h_{9/2}$ shell model configuration for the ground state. The $g(^{229,231}\\text{Fr})$ values support the tentative $I^{\\pi}(^{229,231}\\text{Fr}) = (1/2^{+})$ spin, and point to a $\\pi s_{1/2}^{-1}$ intruder ground state configuration.

I. Budin?evi?; J. Billowes; M. L. Bissell; T. E. Cocolios; R. P. de Groote; S. De Schepper; V. N. Fedosseev; K. T. Flanagan; S. Franchoo; R. F. Garcia Ruiz; H. Heylen; K. M. Lynch; B. A. Marsh; G. Neyens; T. J. Procter; R. E. Rossel; S. Rothe; I. Strashnov; H. H. Stroke; K. D. A. Wendt

2014-07-02T23:59:59.000Z

94

Isotope Shift Measurements of Stable and Short-Lived Lithium Isotopes for Nuclear Charge Radii Determination  

E-Print Network (OSTI)

Changes in the mean-square nuclear charge radii along the lithium isotopic chain were determined using a combination of precise isotope shift measurements and theoretical atomic structure calculations. Nuclear charge radii of light elements are of high interest due to the appearance of the nuclear halo phenomenon in this region of the nuclear chart. During the past years we have developed a new laser spectroscopic approach to determine the charge radii of lithium isotopes which combines high sensitivity, speed, and accuracy to measure the extremely small field shift of an 8 ms lifetime isotope with production rates on the order of only 10,000 atoms/s. The method was applied to all bound isotopes of lithium including the two-neutron halo isotope Li-11 at the on-line isotope separators at GSI, Darmstadt, Germany and at TRIUMF, Vancouver, Canada. We describe the laser spectroscopic method in detail, present updated and improved values from theory and experiment, and discuss the results.

W. Nörtershäuser; R. Sánchez; G. Ewald; A. Dax; J. Behr; P. Bricault; B. A. Bushaw; J. Dilling; M. Dombsky; G. W. F. Drake; S. Götte; H. -J. Kluge; Th. Kühl; J. Lassen; C. D. P. Levy; K. Pachucki; M. Pearson; M. Puchalski; A. Wojtaszek; Z. -C. Yan; C. Zimmermann

2010-09-02T23:59:59.000Z

95

Development of an on-line isotope dilution laser ablation inductively coupled plasma mass spectrometry (LA–ICP-MS) method for determination of boron in silicon wafers  

Science Journals Connector (OSTI)

A method has been developed based on an on-line isotope dilution technique couple with laser ablation/inductively coupled plasma mass spectrometry (LA–ICP-MS), for the determination of boron in p-type silicon wafers. The laser-ablated sample aerosol was mixed on-line with an enriched boron aerosol supplied continuously using a conventional nebulization system. Upon mixing the two aerosol streams, the isotope ratio of boron changed rapidly and was then recorded by the ICP-MS system for subsequent quantification based on the isotope dilution principle. As an on-line solid analysis method, this system accurately quantifies boron concentrations in silicon wafers without the need for an internal or external solid reference standard material. Using this on-line isotope dilution technique, the limit of detection for boron in silicon wafers is 2.8 × 1015 atoms cm?3. The analytical results obtained using this on-line methodology agree well with those obtained using wet chemical digestion methods for the analysis of p-type silicon wafers containing boron concentrations ranging from 1.0 × 1016 to 9.6 × 1018 atoms cm?3.

Chao-Kai Yang; Po-Hsiang Chi; Yong-Chine Lin; Yuh-Chang Sun; Mo-Hsiung Yang

2010-01-01T23:59:59.000Z

96

JOURNAL DE PHYSIQUE CoZZoque C9, suppZ6ment au nOZ1, Tome 41, novembre 1980, page C9-167 THEORETICAL ANALYSIS OF 16-Pm C02 GASDYNAMIC LASER  

E-Print Network (OSTI)

uranium isotope separation6-8. The high ef - ficiency, powerful performance and well-de- veloped laser (GDL) has been evaluated theoretically by means of a modified ~nderson'stime-dependent method

Paris-Sud XI, Université de

97

Isotope Effect of Mercury Diffusion in Air  

Science Journals Connector (OSTI)

Isotope fractionation describes the separation of a reservoir with one isotope composition into “fractions” with different isotope compositions due to small isotopic differences in equilibrium partitioning, rates of mass transfer, or rates of transformation. ... (29) ?202Hg is the value most frequently used to examine mass dependent fractionation of mercury isotopes as 202Hg is the heaviest mercury isotope without significant isobaric interferences. ...

Paul G. Koster van Groos; Bradley K. Esser; Ross W. Williams; James R. Hunt

2013-12-23T23:59:59.000Z

98

Isotope Development & Production | Nuclear Science | ORNL  

NLE Websites -- All DOE Office Websites (Extended Search)

of the "Calutrons" (electromagnetic enrichment devices) were converted by ORNL to the separation and enrichment of stable isotopes and some actinide isotopes. Until 1998 when...

99

Broadly tunable chromium-doped beryllium aluminate lasers and operation thereof  

SciTech Connect

A high power, broadly wavelength-tunable laser is provided which comprises as the laser medium particular single crystals of chromium-doped beryllium aluminate (BeAl/sub 2/O/sub 4/:Cr/sup 3 +/) having the chrysoberyl structure, means for exciting the laser medium and tuning means. The laser may be operated over a broad temperature range from cryogenic temperatures to elevated temperatures. Elevated temperatures are preferred, however, since they result in higher laser gain. Emission is in a spectral range from red to infrared, and the laser is useful in the fields of defense, communications, isotope separation, photochemistry, etc.

Jenssen, H.P.; Morris, R.C.; Peterson, O.G.; Walling, J.C.

1981-06-09T23:59:59.000Z

100

Cascade Performance for Large Separation Factors  

Science Journals Connector (OSTI)

Technical Paper / Argonne National Laboratory Specialists’ Workshop on Basic Research Needs for Nuclear Waste Management / Isotopes Separation

George Emanuel*

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


101

E-Print Network 3.0 - applied isotope techniques Sample Search...  

NLE Websites -- All DOE Office Websites (Extended Search)

Sciences and Ecology ; Biology and Medicine 100 Electrochemical Isotope Effect and Lithium Isotope Separation Jay R. Black, Summary: that the magnitude of isotopic...

102

Isotope-specific detection of low-density materials with laser-based monoenergetic gamma-rays  

Science Journals Connector (OSTI)

What we believe to be the first demonstration of isotope-specific detection of a low-Z and low density object shielded by a high-Z and high-density material using monoenergetic gamma...

Albert, F; Anderson, S G; Anderson, G A; Betts, S M; Gibson, D J; Hagmann, C A; Hall, J; Johnson, M S; Messerly, M J; Semenov, V A; Shverdin, M Y; Tremaine, A M; Hartemann, F V; Siders, C W; McNabb, D P; Barty, C P J

2010-01-01T23:59:59.000Z

103

Determination of ultratrace boron concentrations in uranium oxide by isotope dilution-thermal ionization mass spectrometry using a simplified separation procedure  

Science Journals Connector (OSTI)

Exhaustive reviews on analytical methodologies and mass spectrometric instrumentation for the determination of boron in different matrices such as biological tissues,...1, 4, 5]. It is an established fact that Isotope

Radhika M. Rao; Ankush R. Parab; K. Sasi Bhushan; Suresh K. Aggarwal

2010-06-01T23:59:59.000Z

104

Doppler-free spectroscopy of the 1S0-3P0 optical clock transition in laser-cooled fermionic isotopes of neutral mercury  

E-Print Network (OSTI)

We have performed for the first time direct laser spectroscopy of the 1S0-3P0 optical clock transition at 265.6 nm in fermionic isotopes of neutral mercury laser-cooled in a magneto-optical trap. Spectroscopy is performed by measuring the depletion of the magneto-optical trap induced by the excitation of the long-lived 3P0 state by a probe at 265.6 nm. Measurements resolve the Doppler-free recoil doublet allowing for a determination of the transition frequency to an uncer- tainty well below the Doppler-broadened linewidth. We have performed absolute measurement of the frequency with respect to an ultra-stable reference monitored by LNE-SYRTE fountain pri- mary frequency standards using a femtosecond laser frequency comb. The measured frequency is 1128575290808 +/- 5.6 kHz in 199Hg and 1128569561140 +/- 5.3 kHz in 201Hg, more than 4 orders of magnitude better than previous indirect determinations. Owing to a low sensitivity to blackbody radiation, mercury is a promising candidate for reaching the ultimate performance of optical lattice clocks.

M. Petersen; R. Chicireanu; S. T. Dawkins; D. V. Magalhães; C. Mandache; Y. Lecoq; A. Clairon; S. Bize

2008-07-22T23:59:59.000Z

105

Magnetic Isotope Effect in the Photolysis of Organotin Compounds  

Science Journals Connector (OSTI)

Fractionation of isotopes in chemical and biochemical reactions is induced by two isotope effects; their origin and physical nature are shown in Figure 1. ... The classical isotope effect (CIE) sorts isotopic nuclei on their masses; the magnetic isotope effect (MIE) demonstrates nuclear spin selectivity of reactions and separates isotopic nuclei according to their magnetic moments.1 ...

Anatoly L. Buchachenko; Vladimir L. Ivanov; Vitaly A. Roznyatovsky; Yuri A. Ustynyuk

2006-03-02T23:59:59.000Z

106

Continuous-wave laser annealing of Si-rich oxide: A microscopic picture of macroscopic Si-SiO{sub 2} phase separation  

SciTech Connect

We report on the first observation of the macroscopic (long-range) Si-SiO{sub 2} phase separation in Si-rich oxide SiO{sub x}(x<2) obtained by continuous-wave laser annealing of free-standing SiO{sub x} films. The effect is analyzed by a unique combination of microscopic methods (Raman, transmission, photoluminescence, and infrared spectroscopy, transmission electron microscopy, electron energy loss spectroscopy, and x-ray photoelectron spectroscopy). Three regions can be distinguished on a SiO{sub x} free-standing film after 488 nm laser annealing at intensities above {approx}10{sup 4} W cm{sup -2}: central spot, ring around the central spot, and pristine film outside the irradiated area. In the pristine SiO{sub x} material, small Si nanocrystals (Si-nc) (diameters of a few nanometer) are surrounded by SiO{sub 2} with an addition of residual suboxides, the Si-nc being produced by annealing at 1100 deg. C in a furnace. The central spot of the laser-annealed area (up to {approx}30 {mu}m wide in these experiments) is practically free of Si excess and mainly consists of amorphous SiO{sub 2}. The ring around the central spot contains large spherical Si-nc (diameters up to {approx}100 nm) embedded in amorphous SiO{sub 2} without the presence of suboxides. Laser-induced temperatures in the structurally modified regions presumably exceed the Si melting temperature. The macroscopic Si-SiO{sub 2} phase separation is connected with extensive diffusion in temperature gradient leading to the Si concentration gradient. The present work demonstrates the advantages of high spatial resolution for analysis in materials research.

Khriachtchev, Leonid; Nikitin, Timur; Raesaenen, Markku; Domanskaya, Alexandra [Laboratory of Physical Chemistry, University of Helsinki, P.O. Box 55, FIN-00014 (Finland); Boninelli, Simona; Iacona, Fabio [MATIS IMM CNR, Via Santa Sofia 64, I-95123 Catania (Italy); Engdahl, Anders [MAX-lab, Lund University, P.O. Box 118, 22100 Lund (Sweden); Juhanoja, Jyrki [Top Analytica, Ruukinkatu 4, FIN-20540 Turku (Finland); Novikov, Sergei [Electron Physics Laboratory, Aalto University, P.O. Box 3000, FIN-02015 HUT (Finland)

2010-12-15T23:59:59.000Z

107

Safety approaches for high power modular laser operation  

SciTech Connect

Approximately 20 years ago, a program was initiated at the Lawrence Livermore National Laboratory (LLNL) to study the feasibility of using lasers to separate isotopes of uranium and other materials. Of particular interest has been the development of a uranium enrichment method for the production of commercial nuclear power reactor fuel to replace current more expensive methods. The Uranium Atomic Vapor Laser Isotope Separation (U-AVLIS) Program has progressed to the point where a plant-scale facility to demonstrate commercial feasibility has been built and is being tested. The U-AVLIS Program uses copper vapor lasers which pump frequency selective dye lasers to photoionize uranium vapor produced by an electron beam. The selectively ionized isotopes are electrostatically collected. The copper lasers are arranged in oscillator/amplifier chains. The current configuration consists of 12 chains, each with a nominal output of 800 W for a system output in excess of 9 kW. The system requirements are for continuous operation (24 h a day, 7 days a week) and high availability. To meet these requirements, the lasers are designed in a modular form allowing for rapid change-out of the lasers requiring maintenance. Since beginning operation in early 1985, the copper lasers have accumulated over 2 million unit hours at a >90% availability. The dye laser system provides approximately 2.5 kW average power in the visible wavelength range. This large-scale laser system has many safety considerations, including high-power laser beams, high voltage, and large quantities ({approximately}3000 gal) of ethanol dye solutions. The Laboratory`s safety policy requires that safety controls be designed into any process, equipment, or apparatus in the form of engineering controls. Administrative controls further reduce the risk to an acceptable level. Selected examples of engineering and administrative controls currently being used in the U-AVLIS Program are described.

Handren, R.T.

1993-03-01T23:59:59.000Z

108

On-Line Mid-IR (Quantum Cascade Laser and FTIR Spectrometric) Detection in Capillary Based Separation Systems  

Science Journals Connector (OSTI)

We introduce infrared spectrometry as a novel online molecule specific detection technique in capillary based separation systems. We report on the use of broad band FTIR detection for full spectral information on...

B. Lendl; M. Kölhed; P. Hinsmann; M. Haberkorn…

2002-01-01T23:59:59.000Z

109

Research with fast radioactive isotope beams at RIKEN  

Science Journals Connector (OSTI)

......moments of neutron-rich boron isotopes were measured by the...many neutron-rich isotopes. To exploit fully the...most straightforward determination of the charge distribution...called KISS (KEK isotope separation system......

Tohru Motobayashi; Hiroyoshi Sakurai

2012-01-01T23:59:59.000Z

110

Isotopic Enrichment of Tritiated Water by a Bipolar Electrolysis Process  

Science Journals Connector (OSTI)

Isotope Separation / Proceedings of the Sixth International Conference on Tritium Science and Technology Tsukuba, Japan November 12-16, 2001

S. Heinze; D. Ducret; J.-P. Verdin; T. Pelletier

111

E-Print Network 3.0 - atomic lines isotope Sample Search Results  

NLE Websites -- All DOE Office Websites (Extended Search)

lines isotope Search Powered by Explorit Topic List Advanced Search Sample search results for: atomic lines isotope Page: << < 1 2 3 4 5 > >> 1 Isotope selectivity in laser cooling...

112

Isotope Analysis  

Science Journals Connector (OSTI)

Naturally occurring oxygen includes three stable isotopes,16O,17O, and18O, with the relative abundances of 99.763%, 0.0375%, and 0.1995%, respectively. Isotopic analysis does not consider the absolute abundances ...

Tandong Yao; Wusheng Yu; Huabiao Zhao…

2014-08-01T23:59:59.000Z

113

Definition: Isotopic Analysis | Open Energy Information  

Open Energy Info (EERE)

Analysis Analysis Jump to: navigation, search Dictionary.png Isotopic Analysis Isotopes are atoms of the same element that have different numbers of neutrons. An isotopic analysis looks at a particular isotopic element(s) in a given system, while the conditions which increase/decrease the number of neutrons are well understood and measurable.[1] View on Wikipedia Wikipedia Definition Isotope analysis is the identification of isotopic signature, the distribution of certain stable isotopes and chemical elements within chemical compounds. This can be applied to a food web to make it possible to draw direct inferences regarding diet, trophic level, and subsistence. Isotope ratios are measured using mass spectrometry, which separates the different isotopes of an element on the basis of their mass-to-charge

114

Mobility determination of lead isotopes in glass for retrospective radon measurements  

Science Journals Connector (OSTI)

......al. Retention of Pb isotopes in glass surfaces for...Vierinen K. The ion guide isotope separator online...Whitlow H. J. Boron diffusion in bulk cobalt...srim.org . Mobility determination of lead isotopes in glass for retrospective......

Mikko Laitinen; Iiro Riihimäki; Jörgen Ekman; A. R. Ananda Sagari; Lennart B. Karlsson; Somjai Sangyuenyongpipat; Sergey Gorelick; Heikki Kettunen; Heikki Penttilä; Ragnar Hellborg; Timo Sajavaara; Johan Helgesson; Harry J. Whitlow

2008-08-01T23:59:59.000Z

115

Difference in HETP and HTU for Isotopic Mixtures of Protium-Tritium and Protium Deuterium in Isotopic Exchange Between Water and Hydrogen on Hydrophobic Catalyst  

Science Journals Connector (OSTI)

Isotope Separation / Proceedings of the Sixth International Conference on Tritium Science and Technology Tsukuba, Japan November 12-16, 2001

A. Perevezentsev; B.M. Andreev; E.P. Magomedbekov; Yu.S. Pak; M.B. Rozenkevich; Yu.A. Sakharovskii

116

Modifying molecule-surface scattering by ultrashort laser pulses  

SciTech Connect

In recent years it has become possible to align molecules in free space using ultrashort laser pulses. Here we explore two schemes for controlling molecule-surface scattering processes and which are based on laser-induced molecular alignment. In the first scheme, a single ultrashort nonresonant laser pulse is applied to a molecular beam hitting the surface. This pulse modifies the angular distribution of the incident molecules and causes the scattered molecules to rotate with a preferred sense of rotation (clockwise or counterclockwise). In the second scheme, two properly delayed laser pulses are applied to a molecular beam composed of two chemically close molecular species (isotopes, or nuclear-spin isomers). As the result of the double-pulse excitation, these species are selectively scattered to different angles after the collision with the surface. These effects may provide new means for the analysis and separation of molecular mixtures.

Khodorkovsky, Yuri; Averbukh, Ilya Sh. [Department of Chemical Physics, Weizmann Institute of Science, Rehovot 76100 (Israel); Manson, J. R. [Department of Physics and Astronomy, Clemson University, Clemson, South Carolina 29634 (United States)

2011-11-15T23:59:59.000Z

117

Short wavelength laser  

DOE Patents (OSTI)

A short wavelength laser is provided that is driven by conventional-laser pulses. A multiplicity of panels, mounted on substrates, are supported in two separated and alternately staggered facing and parallel arrays disposed along an approximately linear path. When the panels are illuminated by the conventional-laser pulses, single pass EUV or soft x-ray laser pulses are produced.

Hagelstein, P.L.

1984-06-25T23:59:59.000Z

118

Carbon Isotopes  

NLE Websites -- All DOE Office Websites (Extended Search)

Atmospheric Trace Gases » Carbon Isotopes Atmospheric Trace Gases » Carbon Isotopes Carbon Isotopes Gateway Pages to Isotopes Data Modern Records of Carbon and Oxygen Isotopes in Atmospheric Carbon Dioxide and Carbon-13 in Methane 800,000 Deuterium Record and Shorter Records of Various Isotopic Species from Ice Cores Carbon-13 13C in CO Measurements from Niwot Ridge, Colorado and Montana de Oro, California (Tyler) 13C in CO2 NOAA/CMDL Flask Network (White and Vaughn) CSIRO GASLAB Flask Network (Allison, Francey, and Krummel) CSIRO in situ measurements at Cape Grim, Tasmania (Francey and Allison) Scripps Institution of Oceanography (Keeling et al.) 13C in CH4 NOAA/CMDL Flask Network (Miller and White) Northern & Southern Hemisphere Sites (Quay and Stutsman) Northern & Southern Hemisphere Sites (Stevens)

119

Electromagnetic Separation of Isotopes at Oak Ridge  

Science Journals Connector (OSTI)

...the local AEC operations office conferred...the silver was safe, being massively...pub-licity until the operation was complete. Fortunately...remain to haunt both operations and development...placed a calcium boiler below the beam adjacent...ratio-information fundamental to the concept of...

L. O. Love

1973-10-26T23:59:59.000Z

120

Separation Of Stable Isotopes By Electromagnetic Means  

Science Journals Connector (OSTI)

... A good illustration is the example of boron. As noted above, boron enriched in boron-10 is widely used as a neutron detector, having five times the sensitivity as a ...

W. D. ALLEN

1951-09-15T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


121

Gaseous isotope separation using solar wind phenomena  

Science Journals Connector (OSTI)

...industrial process with a solar dimension, but machines...of a centrifugal pump-like housing to...phe- nomena in the solar wind as a guide to...of a centrifugal pump evacuating the chamber...ratio of specific heats for diatomic molecules...velocity flow must be assisted by the use of light...

Chia-Gee Wang

1980-01-01T23:59:59.000Z

122

Y-12 begins to separate lithium isotopes  

NLE Websites -- All DOE Office Websites (Extended Search)

explosion patterned after Fat Man. The Soviets were now on equal footing with a thermonuclear weapon capability. Y-12 was charged with increasing production and adapting to...

123

Evaluation of Hydrogen Isotope Oxidation Process in an Atmospheric Pressure Plasma  

Science Journals Connector (OSTI)

Detritiation and Isotope Separation / Proceedings of the Ninth International Conference on Tritium Science and Technology (Part 2)

K. Akahane; N. Ezumi; Y. Uesugi; Y. Tanaka; M. Tanaka; K. Nishimura

124

Accelerated alpha-decay of 232U isotope achieved by exposure of its aqueous solution with gold nanoparticles to laser radiation  

E-Print Network (OSTI)

Experimental results are presented on laser-induced accelerated alpha-decay of Uranium-232 nuclei under laser exposure of Au nanoparticles in aqueous solutions of its salt. It is demonstrated that the decrease of alpha-activity strongly depends on the peak intensity of the laser radiation in the liquid and is highest at several terawatt per square centimeter. The decrease of alpha-activity of the exposed solutions is accompanied by the deviation of gamma-activities of daughter nuclides of Uranium-232 from their equilibrium values. Possible mechanisms of the laser influence on the alpha-activity are discussed on the basis of the amplification of the electric field of laser wave on metallic nanoparticles.

A. V. Simakin; G. A. Shafeev

2011-12-29T23:59:59.000Z

125

A test stand for off-line laser ion source development at TRIUMF  

SciTech Connect

A test stand for ion source development and laser resonance ionization spectroscopy was built and commissioned at TRIUMF. The test stand is needed to develop efficient ion sources that can function reliably in the hostile, high temperature, high radiation environment of TRIUMF's isotope separator on-line (ISOL) production target ion source. In addition, it enables laser resonance ionization spectroscopy to develop laser excitation schemes suitable for the solid-state laser systems used with TRIUMF's resonant ionization laser ion source . Also, it allows for possible improvement of current ion sources and validation of new designs. The test stand employs a copy of the ion optics used on-line, so that results can be transferred directly to radioactive ion beam production. Due to space restrictions and the need for rapid mass scans, a quadrupole mass spectrometer is used as a mass separator. One of the first experiments conducted on the laser ion source test stand (LIS STAND) was resonant ionization spectroscopy of gallium to improve on the ionization scheme previously used on-line, so that low yield isotopes (e.g., {sup 62}Ga) become available for experiments. Different Rydberg series in gallium were observed and autoionizing states were searched for. The overall LIS STAND system performance, characteristics, and the first resonant ionization spectroscopy are described.

Lavoie, J. P. [TRIUMF, 4004 Wesbrook Mall, Vancouver, British Columbia V6T 2A3 (Canada); Universite Laval, Quebec City, Quebec G1K 7P4 (Canada); Li, R.; Bricault, P.; Lassen, J. [TRIUMF, 4004 Wesbrook Mall, Vancouver, British Columbia V6T 2A3 (Canada); Chachkova, O. [TRIUMF, 4004 Wesbrook Mall, Vancouver, British Columbia V6T 2A3 (Canada); University of Victoria, Victoria, British Columbia V8N 1M5 (Canada); Teigelhoefer, A. [TRIUMF, 4004 Wesbrook Mall, Vancouver, British Columbia V6T 2A3 (Canada); University of Manitoba, Winnipeg, Manitoba R3T 2N2 (Canada)

2013-01-15T23:59:59.000Z

126

Determination of boron isotope compositions of geological materials by laser ablation MC-ICP-MS using newly designed high sensitivity skimmer and sample cones  

Science Journals Connector (OSTI)

Abstract The effects of addition of nitrogen gas with use of three different combinations of sample and skimmer cones on the performance of LA-MC-ICP-MS for in situ B isotope ratio measurements were investigated in detail. Compared to the standard arrangement (H skimmer cone + standard sample cone), sensitivities of B isotopes were improved by a factor of 2.4 and 3.8 with use of X skimmer cone + standard sampler cone and the X skimmer cone + Jet sample cone, respectively. The best within-run precision (2 s) of 11B/10B was approximately 50 ppm for B4 reference material (B content = 31,400 ?g/g) with use of X skimmer cone + Jet sample cone. It was found that different cone combinations had significant effects on the instrument mass bias, but had little effect on the precisions of B isotope ratios. Addition of nitrogen (2–4 ml/min) in the central channel gas did not improve the sensitivity of B. However, significant wider ion axial distribution profile and more stable mass-bias for B isotope ratios were evident. Under selected optimum conditions, good agreements between the measured ?11B values and the reference values were obtained for the international reference minerals (B4, Dravite, Elbaite, IMMRB1 and Schorl), the NIST SRM 610–612 synthetic soda-lime glasses and the MPI-DING glasses (GOR-128-G, GOR-132-G, and StHs6/80). It was found that for low-B containing (11 ppm and 31 ppm) materials, the precisions (2 s) of 11B/10B can be improved by a factor of 2–10 by using the newly designed X-skimmer cone and Jet sample cone, compared to that of using the standard cones. The international reference mineral Danburite (?11B of ? 14.92 ± 6.77 2SD, n = 32) showed a significant non-uniformity of B isotope ratio distribution. Our first boron isotopic results from standards GSD-1G (?11B: 11.92 ± 1.03, n = 30), GSE-1G (?11B: 1.63 ± 0.32, n = 30), GP-4 (?11B: ? 5.85 ± 1.01, n = 40) and DD-1 (?11B: ? 13.21 ± 0.56, n = 35) showed these materials were fairly homogeneous in boron isotope ratios, making them as good candidates as reference materials. The proposed LA-MC-ICPMS method is suitable for the direct determination of B isotope ratio in a variety of geological materials.

Lin Lin; Zhaochu Hu; Lu Yang; Wen Zhang; Yongsheng Liu; Shan Gao; Shenghong Hu

2014-01-01T23:59:59.000Z

127

Ultracapacitor separator  

DOE Patents (OSTI)

An ultracapacitor includes two solid, nonporous current collectors, two porous electrodes separating the collectors, a porous separator between the electrodes and an electrolyte occupying the pores in the electrodes and separator. The electrolyte is a polar aprotic organic solvent and a salt. The porous separator comprises a wet laid cellulosic material.

Wei, Chang (Niskayuna, NY); Jerabek, Elihu Calvin (Glenmont, NY); LeBlanc, Jr., Oliver Harris (Schenectady, NY)

2001-03-06T23:59:59.000Z

128

AVLIS enrichment of medical isotopes  

SciTech Connect

Under the Sponsorship of the United states Enrichment Corporation (USEC), we are currently investigating the large scale separation of several isotopes of medical interest using atomic vapor isotope separation (AVLIS). This work includes analysis and experiments in the enrichment of thallium 203 as a precursor to the production of thallium 201 used in cardiac imaging following heart attacks, on the stripping of strontium 84 from natural strontium as precursor to the production of strontium 89, and on the stripping of lead 210 from lead used in integrated circuits to reduce the number of alpha particle induced logic errors.

Haynam, C.A.; Scheibner, K.F.; Stern, R.C.; Worden, E.F. [Lawrence Livermore National Laboratory, CA (United States)

1996-12-31T23:59:59.000Z

129

Neptunium separations  

SciTech Connect

Two procedures for the separation of Np are presented; the first involves separation of /sup 239/Np from irradiated /sup 238/U, and the second involves separation of /sup 237/Np from a solution representing that from a dissolved fuel element.

Wild, J.F.

1983-05-09T23:59:59.000Z

130

from Isotope Production Facility  

NLE Websites -- All DOE Office Websites (Extended Search)

Cancer-fighting treatment gets boost from Isotope Production Facility April 13, 2012 Isotope Production Facility produces cancer-fighting actinium 2:32 Isotope cancer treatment...

131

The Ways to Increase Light Water Detritiation Efficiency by Chemical Isotope Exchange Between Hydrogen and Water in Membrane Contact Devices  

Science Journals Connector (OSTI)

Detritiation and Isotope Separation / Proceedings of the Ninth International Conference on Tritium Science and Technology (Part 2)

M. B. Rozenkevich; I. L. Rastunova

132

Isotope studies in photosynthesis  

Science Journals Connector (OSTI)

Isotope studies in photosynthesis ... Examines the use of isotopic oxygen, hydrogen, carbon, and phosphorus in the study of photosynthesis. ...

J. A. Bassham; A. A. Benson; Melvin Calvin

1953-01-01T23:59:59.000Z

133

Short wavelength laser  

DOE Patents (OSTI)

A short wavelength laser (28) is provided that is driven by conventional-laser pulses (30, 31). A multiplicity of panels (32), mounted on substrates (34), are supported in two separated and alternately staggered facing and parallel arrays disposed along an approximately linear path (42). When the panels (32) are illuminated by the conventional-laser pulses (30, 31), single pass EUV or soft x-ray laser pulses (44, 46) are produced.

Hagelstein, Peter L. (Livermore, CA)

1986-01-01T23:59:59.000Z

134

Deep-Sea Research I 53 (2006) 684688 Experimental evaluation of the isotopic exchange equilibrium  

E-Print Network (OSTI)

on the ion-exchange separation of boron isotopes. Bulletin of Chemical Society of Japan 50, 158­163]. Since strengths. r 2006 Elsevier Ltd. All rights reserved. Keywords: Boron isotopes; Boron isotopic exchange. Introduction The boron isotopic composition of marine carbonates constitutes a promising tracer of the paleo

Kaufman, Alan Jay

135

UW Cosmogenic Isotopes Al-Be 1 EXTRACTION OF Al & Be FROM QUARTZ FOR ISOTOPIC ANALYSIS  

E-Print Network (OSTI)

UW Cosmogenic Isotopes Al-Be 1 EXTRACTION OF Al & Be FROM QUARTZ FOR ISOTOPIC ANALYSIS Summary This method is used to separate Al and Be for AMS analysis from pure quartz samples. After adding Be carrier, quartz is dissolved in HF. The solution is sub-sampled for determination of total Al content, then dried

Stone, John

136

Low-energy Coulomb excitation of neutron-rich zinc isotopes  

SciTech Connect

At the radioactive ion beam facility REX-ISOLDE, neutron-rich zinc isotopes were investigated using low-energy Coulomb excitation. These experiments have resulted in B(E2,2{sub 1}{sup +}{yields}0{sub 1}{sup +}) values in {sup 74-80}Zn, B(E2,4{sub 1}{sup +}{yields}2{sub 1}{sup +}) values in {sup 74,76}Zn and the determination of the energy of the first excited 2{sub 1}{sup +} states in {sup 78,80}Zn. The zinc isotopes were produced by high-energy proton- (A=74,76,80) and neutron- (A=78) induced fission of {sup 238}U, combined with selective laser ionization and mass separation. The isobaric beam was postaccelerated by the REX linear accelerator and Coulomb excitation was induced on a thin secondary target, which was surrounded by the MINIBALL germanium detector array. In this work, it is shown how the selective laser ionization can be used to deal with the considerable isobaric beam contamination and how a reliable normalization of the experiment can be achieved. The results for zinc isotopes and the N=50 isotones are compared to collective model predictions and state-of-the-art large-scale shell-model calculations, including a recent empirical residual interaction constructed to describe the present experimental data up to 2004 in this region of the nuclear chart.

Walle, J. van de [Instituut voor Kern-en Stralingsfysica, K. U. Leuven, Leuven (Belgium); ISOLDE, CERN, Geneva (Switzerland); Aksouh, F. [Instituut voor Kern-en Stralingsfysica, K. U. Leuven, Leuven (Belgium); CEA Saclay, DAPNIA/SPhN, Gif-sur-Yvette (France); Behrens, T.; Gernhauser, R.; Kroell, T.; Kruecken, R. [Physik Department E12, Technische Universitaet Muenchen, Garching (Germany); Bildstein, V. [Physik Department E12, Technische Universitaet Muenchen, Garching (Germany); Max-Planck-Institut fuer Kernphysik, Heidelberg (Germany); Blazhev, A.; Eberth, J.; Jolie, J.; Reiter, P.; Warr, N.; Weisshaar, D. [Institut fuer Kernphysik, Universitaet Koeln, Koeln (Germany); Cederkaell, J.; Delahaye, P.; Fedosseev, V. N.; Franchoo, S.; Marsh, B. A.; Sieber, T.; Voulot, D. [ISOLDE, CERN, Geneva (Switzerland)] (and others)

2009-01-15T23:59:59.000Z

137

Laser-triggered ion acceleration and table top isotope production Central Research Institute of Electric Power Industry, 2-11-1, Iwado-kita, Komae-shi,  

E-Print Network (OSTI)

to accelerate protons and ions for experiments in nuclear physics and for applications in nuclear medicine It was shown that these accelerated protons can induce nuclear transformations.6 In this letter we report acceleration was attributed to the electrostatic field of charge separation due to ``vacuum heating,'' 9

Umstadter, Donald

138

Laser Roadshow  

NLE Websites -- All DOE Office Websites (Extended Search)

outreach Laser Roadshow The NIF Laser Roadshow includes a number of interactive laser demonstrations (Laser Light Fountain, Laser DJ, and NIF "3D ride") that have traveled across...

139

Laser cooling with ultrafast pulse trains  

E-Print Network (OSTI)

We propose a new laser cooling method for atomic species whose level structure makes traditional laser cooling difficult. For instance, laser cooling of hydrogen requires vacuum-ultraviolet laser light, while multielectron atoms need laser light at many widely separated frequencies. These restrictions can be eased by laser cooling on two-photon transitions with ultrafast pulse trains. Laser cooling of hydrogen, antihydrogen, and carbon appears feasible, and extension of the technique to molecules may be possible.

David Kielpinski

2003-06-14T23:59:59.000Z

140

Synthesis of a triblock polymer system for separation of actinides for nuclear waste remediation.  

E-Print Network (OSTI)

??Nuclear power waste contains radioactive isotopes with long half lives and the problem lies in the fact that the lanthanides and actinides must be separated… (more)

Hamilton, Doris Finley

2011-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


141

lead-isotope dating  

Science Journals Connector (OSTI)

lead-isotope dating, lead-lead dating, lead-isotope age measurement, lead-lead age measurement ? Blei-Isotopen(-Alters)bestimmung, f, Blei-Isotopen-Datierung

2014-08-01T23:59:59.000Z

142

isotopic ratio | EMSL  

NLE Websites -- All DOE Office Websites (Extended Search)

isotopic ratio isotopic ratio Leads No leads are available at this time. Magnesium behavior and structural defects in Mg+ ion implanted silicon carbide. Abstract: As a candidate...

143

Separation system  

DOE Patents (OSTI)

A separation system for dewatering radioactive waste materials includes a disposal container, drive structure for receiving the container, and means for releasably attaching the container to the drive structure. Separation structure disposed in the container adjacent the inner surface of the side wall structure retains solids while allowing passage of liquids. Inlet port structure in the container top wall is normally closed by first valve structure that is centrifugally actuated to open the inlet port and discharge port structure at the container periphery receives liquid that passes through the separation structure and is normally closed by second valve structure that is centrifugally actuated to open the discharge ports. The container also includes coupling structure for releasable engagement with the centrifugal drive structure. Centrifugal force produced when the container is driven in rotation by the drive structure opens the valve structures, and radioactive waste material introduced into the container through the open inlet port is dewatered, and the waste is compacted. The ports are automatically closed by the valves when the container drum is not subjected to centrifugal force such that containment effectiveness is enhanced and exposure of personnel to radioactive materials is minimized.

Rubin, Leslie S. (Newton, MA)

1986-01-01T23:59:59.000Z

144

E-Print Network 3.0 - atom nuclei isotopes Sample Search Results  

NLE Websites -- All DOE Office Websites (Extended Search)

decay... the name Borromean nuclei. The heaviest neutron rich carbon ... Source: TRIUMF Isotope Separation and ACceleration (ISAC) facility, beta-NMR Group Collection: Physics 27...

145

High-precision CO2 isotopologue spectrometer with a difference-frequency-generation laser source  

E-Print Network (OSTI)

High-precision CO2 isotopologue spectrometer with a difference-frequency-generation laser source A precision laser spectrometer for the detection of CO2 isotopes is reported. The spectrometer measures the fundamental absorption signatures of 13 C and 12 C isotopes in CO2 at 4.32 m using a tunable mid-IR laser

146

Resonance Ionization Laser Ion Sources  

E-Print Network (OSTI)

The application of the technique of laser resonance ionization to the production of singly charged ions at radioactive ion beam facilities is discussed. The ability to combine high efficiency and element selectivity makes a resonance ionization laser ion source (RILIS) an important component of many radioactive ion beam facilities. At CERN, for example, the RILIS is the most commonly used ion source of the ISOLDE facility, with a yearly operating time of up to 3000 hours. For some isotopes the RILIS can also be used as a fast and sensitive laser spectroscopy tool, provided that the spectral resolution is sufficiently high to reveal the influence of nuclear structure on the atomic spectra. This enables the study of nuclear properties of isotopes with production rates even lower than one ion per second and, in some cases, enables isomer selective ionization. The solutions available for the implementation of resonance laser ionization at radioactive ion beam facilities are summarized. Aspects such as the laser r...

Marsh, B

2013-01-01T23:59:59.000Z

147

Laser Ignition  

NLE Websites -- All DOE Office Websites (Extended Search)

Laser Ignition Laser Ignition A first excitation laser or other excitation light source is used in tandem with an ignitor laser to provide a compact, durable, engine deployable...

148

Separation processes using expulsion from dilute supercritical solutions  

DOE Patents (OSTI)

A process is described for separating isotopes as well as other mixtures by utilizing the behavior of dilute repulsive or weakly attractive elements of the mixtures as the critical point of the solvent is approached.

Cochran, H.D. Jr.

1993-04-20T23:59:59.000Z

149

Isotope Science and Production  

E-Print Network (OSTI)

of Energy National Isotope Program http://www.nuclear.energy.gov/isotopes/nelsotopes2a.html Isotopes for Environmental Science Isotopes produced at Los Alamos National Laboratory are used as environmental tracers change and its effects. Los Alamos National Laboratory can produce Si-32 needed for oceanographic tracing

150

Stable isotope studies  

SciTech Connect

The research has been in four general areas: (1) correlation of isotope effects with molecular forces and molecular structures, (2) correlation of zero-point energy and its isotope effects with molecular structure and molecular forces, (3) vapor pressure isotope effects, and (4) fractionation of stable isotopes. 73 refs, 38 figs, 29 tabs.

Ishida, T.

1992-01-01T23:59:59.000Z

151

Isotopic abundance in atom trap trace analysis  

DOE Patents (OSTI)

A method and system for detecting ratios and amounts of isotopes of noble gases. The method and system is constructed to be able to measure noble gas isotopes in water and ice, which helps reveal the geological age of the samples and understand their movements. The method and system uses a combination of a cooled discharge source, a beam collimator, a beam slower and magneto-optic trap with a laser to apply resonance frequency energy to the noble gas to be quenched and detected.

Lu, Zheng-Tian; Hu, Shiu-Ming; Jiang, Wei; Mueller, Peter

2014-03-18T23:59:59.000Z

152

Isotope-selective excitation of 41Ca isotope in Doppler-free two-photon continuous-wave excitation: a case study  

Science Journals Connector (OSTI)

Seven schemes are studied theoretically for Doppler-free two-photon excitation of rare 41Ca isotope using single-mode continuous-wave lasers. The ionization efficiencies...

Kumar, P V Kiran; Sankari, M; Acharyulu, G V S G; Suryanarayana, M V

2006-01-01T23:59:59.000Z

153

Direct mass measurements of neutron-rich zirconium isotopes up to Zr104  

Science Journals Connector (OSTI)

Atomic masses of radioactive zirconium isotopes from Zr96 to Zr104 have been measured with a relative accuracy of ?5×10?7 using a Penning trap coupled to the ion guide isotope separator on-line system. The obtained two-neutron separation energies show strong local correlation in relation to the shape change and shape coexistence between N=58 and 60.

S. Rinta-Antila; S. Kopecky; V. S. Kolhinen; J. Hakala; J. Huikari; A. Jokinen; A. Nieminen; J. Äystö; J. Szerypo

2004-07-14T23:59:59.000Z

154

NATURE | NEWS Laser fusion nears crucial milestone  

E-Print Network (OSTI)

Eric Hand NATURE | NEWS Laser fusion nears crucial milestone National Ignition Facility approaches the National Ignition Facility (NIF) finally lives up to its name. The facility, which boasts the world's largest laser, is designed to trigger fusion by imploding a target pellet of hydrogen isotopes, thereby

155

Isotope Geothermometry | Open Energy Information  

Open Energy Info (EERE)

Isotope Geothermometry Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Technique: Isotope Geothermometry Details Activities (0) Areas (0) Regions (0)...

156

THE ISOTOPES OF AMERICIUM  

E-Print Network (OSTI)

spectrographic analysis of the americium samples. It is a48 J'---_I" THE ISOTOPES OF AMERICIUM K. Street, Jr. , A.Elements THE ISOTOPES OF AMERICIUM K. Street, Jr. , A.

Street, K.; Ghiroso, A.; Seaborg, G.T.

2008-01-01T23:59:59.000Z

157

Perchlorate Isotope Forensics  

Science Journals Connector (OSTI)

In this study, comprehensive stable isotope analyses (37Cl/35Cl and 18O/17O/16O) of perchlorate from known synthetic and natural sources reveal systematic differences in isotopic characteristics that are related to the formation mechanisms. ... ?37Cl and ?18O are measures of mass-dependent fractionation of Cl and O isotopes by normal physical, chemical, or biological processes. ...

John Karl Böhlke; Neil C. Sturchio; Baohua Gu; Juske Horita; Gilbert M. Brown; W. Andrew Jackson; Jacimaria Batista; Paul B. Hatzinger

2005-11-04T23:59:59.000Z

158

Isotope Effect in Adhesion  

Science Journals Connector (OSTI)

Isotope Effect in Adhesion ... We report the first observation of an isotope effect in adhesion. ... The results are presented in Figure 3. Clearly, the isotope effect is very significant, substantiating the proposed H-bonding interactions between the PDMS and Si?OH(D) surfaces. ...

Gun Young Choi; Abraham Ulman; Yitzhak Shnidman; Walter Zurawsky; Cathy Fleischer

2000-05-25T23:59:59.000Z

159

Dual Magnetic Separator for TRI$?$P  

E-Print Network (OSTI)

The TRI$\\mu$P facility, under construction at KVI, requires the production and separation of short-lived and rare isotopes. Direct reactions, fragmentation and fusion-evaporation reactions in normal and inverse kinematics are foreseen to produce nuclides of interest with a variety of heavy-ion beams from the superconducting cyclotron AGOR. For this purpose, we have designed, constructed and commissioned a versatile magnetic separator that allows efficient injection into an ion catcher, i.e., gas-filled stopper/cooler or thermal ionizer, from which a low energy radioactive beam will be extracted. The separator performance was tested with the production and clean separation of $^{21}$Na ions, where a beam purity of 99.5% could be achieved. For fusion-evaporation products, some of the features of its operation as a gas-filled recoil separator were tested.

G. P. A. Berg; O. C. Dermois; U. Dammalapati; P. Dendooven M. N. Harakeh; K. Jungmann; C. J. G. Onderwater; A. Rogachevskiy; M. Sohani; E. Traykov; L. Willmann; H. W. Wilschut

2005-09-09T23:59:59.000Z

160

Laser and gas centrifuge enrichment  

SciTech Connect

Principles of uranium isotope enrichment using various laser and gas centrifuge techniques are briefly discussed. Examples on production of high enriched uranium are given. Concerns regarding the possibility of using low end technologies to produce weapons grade uranium are explained. Based on current assessments commercial enrichment services are able to cover the global needs of enriched uranium in the foreseeable future.

Heinonen, Olli [Senior Fellow, Belfer Center for Science and International Affairs, Harvard Kennedy School, Cambridge, Massachusetts (United States)

2014-05-09T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
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161

ARM - Measurement - Isotope ratio  

NLE Websites -- All DOE Office Websites (Extended Search)

govMeasurementsIsotope ratio govMeasurementsIsotope ratio ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Isotope ratio Ratio of stable isotope concentrations. Categories Atmospheric Carbon, Atmospheric State Instruments The above measurement is considered scientifically relevant for the following instruments. Refer to the datastream (netcdf) file headers of each instrument for a list of all available measurements, including those recorded for diagnostic or quality assurance purposes. ARM Instruments FLASK : Flask Samplers for Carbon Cycle Gases and Isotopes Field Campaign Instruments FLASK : Flask Samplers for Carbon Cycle Gases and Isotopes Datastreams FLASK : Flask Samplers for Carbon Cycle Gases and Isotopes

162

Laser Cladding  

Science Journals Connector (OSTI)

Laser cladding is a surface modification process in which a laser beam is used to melt an addition ... process must be clearly differentiated from that of laser surface alloying ( Laser Surface Al...

Prof. Dr. José L. Ocaña; Prof. Janez Grum

2013-01-01T23:59:59.000Z

163

Isotope Program Transportation | Department of Energy  

Office of Environmental Management (EM)

Isotope Program Transportation Isotope Program Transportation Isotope Program Transportation More Documents & Publications Nuclear Fuel Storage and Transportation Planning Project...

164

Mass-Independent Isotope Effects  

Science Journals Connector (OSTI)

Scientific interests: ESR and NMR spectroscopies, molecular magnets, mechanisms of chemical and biochemical reactions, spin physics and chemistry, isotopes and isotope effects in chemistry and biochemistry. ... Another mass-independent isotope effect was detected in 1983 as a deviation of isotopic distribution in reaction products from that which would be expected from the mass-dependent isotope effect. ... Later, Nomura et al.(92) have found isotopic 233U anomaly in the U4+–U6+ exchange reaction; they noted that the isotope effect was correlated with isotope shifts in the atomic spectra of uranium isotopes. ...

Anatoly L. Buchachenko

2013-01-09T23:59:59.000Z

165

Isotope hydrology of catchment basins: lithogenic and cosmogenic isotopic systems  

SciTech Connect

A variety of physical processes affect solute concentrations within catchment waters. The isotopic compositions of the solutes can indicate which processes have determined the observed concentrations. These processes together constitute the physical history of the water. Many solutes in natural waters are derived from the interaction between the water and the rock and/or soil within the system - these are termed `lithogenic` solutes. The isotopic compositions of these solutes provide information regarding rock-water interactions. Many other solutes have their isotopic compositions determined both within and outside of the catchment - i.e., in addition to being derived from catchment rock and soil, they are solutes that are also transported into the catchment. Important members of this group include solutes that have isotopic compositions produced by atomic particle interactions with other nuclides. The source of the atomic particles can be cosmic radiation (producing `cosmogenic` nuclides in the atmosphere and land surface), anthropogenic nuclear reactions (producing `thermonuclear` nuclides), or radioactive and fission decay of naturally-occurring elements, principally {sup 238}U (producing `in-situ` lithogenic nuclides in the deep subsurface). Current language usage often combines all of the atomic particle-produced nuclides under the heading `cosmogenic nuclides`, and for simplicity we will often follow that usage here, although always indicating which variety is being discussed. This paper addresses the processes that affect the lithogenic and cosmogenic solute concentrations in catchment waters, and how the isotopic compositions of the solutes can be used in integrative ways to identify these processes, thereby revealing the physical history of the water within a catchment system. The concept of a `system` is important in catchment hydrology. A catchment is the smallest landscape unit that can both participate in all of the aspects of the hydrologic cycle and also be treated as a mostly closed system for mass balance considerations. It is the near closure of the system that permits well- constrained chemical mass balance calculations to be made. These calculations generally focus of lithogenic solutes, and therefore in our discussions of lithogenic nuclides in the paper, the concept of chemical mass balance in a nearly dosed system will play an important role. Examination of the isotopic compositions of solutes provides a better understanding of the variety of processes controlling mass balance. It is with this approach that we examined the variety of processes occurring within the catchment system, such as weathering and soil production, generation of stormflow and streamflow (hydrograph separation), movement of soil pore water, groundwater flow, and the overall processes involved with basinal water balance. In this paper, the term `nuclide` will be used when referring to a nuclear species that contains a particular number of protons and neutrons. The term is not specific to any element. The term `isotope` will be used to distinguish nuclear species of a given element (atoms with the same number of protons). That is to say, there are many nuclides in nature - for example, {sup 36}Cl, {sup 87}Sr, {sup 238}U; the element has four naturally-occurring isotopes - {sup 87}Sr, and {sup 88}Sr. This paper will first discuss the general principles that underlie the study of lithogenic and cosmogenic nuclides in hydrology, and provide references to some of the more important studies applying these principles and nuclides. We then turn in the second section to a discussion of their specific applications in catchment- scale systems. The final section of this paper discusses new directions in the application of lithogenic and cosmogenic nuclides to catchment hydrology, with some thoughts concerning possible applications that still remain unexplored.

Nimz, G. J., LLNL

1998-06-01T23:59:59.000Z

166

Stable isotope enrichment  

SciTech Connect

Brian Egle is working to increase the nation's capacity to produce stable isotopes for use including medicine, industry and national security.

Egle, Brian

2014-07-14T23:59:59.000Z

167

EMSL - isotopic ratio  

NLE Websites -- All DOE Office Websites (Extended Search)

isotopic-ratio en Magnesium behavior and structural defects in Mg+ ion implanted silicon carbide. http:www.emsl.pnl.govemslwebpublicationsmagnesium-behavior-and-structural-def...

168

Noise suppressing capillary separation system  

DOE Patents (OSTI)

A noise-suppressing capillary separation system for detecting the real-time presence or concentration of an analyte in a sample is provided. The system contains a capillary separation means through which the analyte is moved, a coherent light source that generates a beam which is split into a reference beam and a sample beam that irradiate the capillary, and a detector for detecting the reference beam and the sample beam light that transmits through the capillary. The laser beam is of a wavelength effective to be absorbed by a chromophore in the capillary. The system includes a noise suppressing system to improve performance and accuracy without signal averaging or multiple scans. 13 figs.

Yeung, E.S.; Xue, Y.

1996-07-30T23:59:59.000Z

169

Gravitational Separation of Gases and Isotopes in Polar Ice Caps  

Science Journals Connector (OSTI)

...reported that 02 trapped in 2000-year-old ice from Camp Century, Green-land, has an 180/160 enrichment given by...values for 02 in 6,100-and 20,000-year-old Camp Century ice (1), and noting that mean seawater was enriched...

H. Craig; Y. Horibe; T. Sowers

1988-12-23T23:59:59.000Z

170

ISOTOPE SEPARATION BY IONIC EXPANSION IN A MAGNETIC FIELD  

Science Journals Connector (OSTI)

...To calculate the electric fields and potentials...than enough to bring the discharge out to the insulated...plate can have but one electric potential, and it must...ions and electrons is an electric arc of short length, 1...

Joseph Slepian

1955-01-01T23:59:59.000Z

171

Y-12 plant prepares to separate lithium isotopes  

NLE Websites -- All DOE Office Websites (Extended Search)

patterned after "Fat Man," because the Soviets were now on equal footing with a thermonuclear weapon capability -- and Y-12 was charged with increasing production and adapting...

172

Isotopes in Environmental and Health Studies Vol. 41, No. 4, December 2005, 293302  

E-Print Network (OSTI)

deployable quantum cascade laser-based sensor is described, along with line selection strategy for 13/12CO2 sensors; IR spectrometry; Natural isotope ratios; Volcanoes 1. Introduction Tunable laser absorption for the detection of low gas concentra- tion levels by improving the signal-to-noise ratio of the spectrometer

173

Celebrating The Isotope  

Science Journals Connector (OSTI)

Celebrating The Isotope ... The notion of isotopes and the rest of Soddy’s lifetime body of work on radioactivity, the group displacement laws, the social responsibility of scientists, and the environment have had a profound effect on science and society. ...

GEORGE B. KAUFFMAN

2013-12-02T23:59:59.000Z

174

Isotope - based Quantum Information  

E-Print Network (OSTI)

This paper is brief review of three aspects of the isotope - based quantum information: computation, teleportation and cryptography. Our results demonstrate not only that entanglement exists in elementary excitation of isotope - mixed solids but also it can be used for quantum information processing.

Vladimir G. Plekhanov

2009-09-04T23:59:59.000Z

175

Unattended Monitoring of HEU Production in Gaseous Centrifuge Enrichment Plants using Automated Aerosol Collection and Laser-based Enrichment Assay  

SciTech Connect

Nuclear power is enjoying rapid growth as government energy policies and public demand shift toward low carbon energy production. Pivotal to the global nuclear power renaissance is the development and deployment of robust safeguards instrumentation that allows the limited resources of the IAEA to keep pace with the expansion of the nuclear fuel cycle. Undeclared production of highly enriched uranium (HEU) remains a primary proliferation concern for modern gaseous centrifuge enrichment plants (GCEPs), due to their massive separative work unit (SWU) processing power and comparably short cascade equilibrium timescale. The Pacific Northwest National Laboratory is developing an unattended safeguards instrument, combining continuous aerosol particulate collection with uranium isotope assay, to provide timely detection of HEU production within a GCEP. This approach is based on laser vaporization of aerosol particulates, followed by laser spectroscopy to characterize the uranium enrichment level. Our prior investigation demonstrated single-shot detection sensitivity approaching the femtogram range and relative isotope ratio uncertainty better than 10% using gadolinium as a surrogate for uranium. In this paper we present measurement results on standard samples containing traces of depleted, natural, and low enriched uranium, as well as measurements on aerodynamic size uranium particles mixed in background materials (e.g., dust, minerals, soils). Improvements and optimizations in the detection electronics, signal timing, calibration, and laser alignment have lead to significant improvements in detection sensitivity and enrichment accuracy, contributing to an overall reduction in the false alarm probability. The sample substrate media was also found to play a significant role in facilitating laser-induced vaporization and the production of energetic plasma conditions, resulting in ablation optimization and further improvements in the isotope abundance sensitivity.

Anheier, Norman C.; Bushaw, Bruce A.

2010-08-11T23:59:59.000Z

176

Laser system using regenerative amplifier  

DOE Patents (OSTI)

High energy laser system using a regenerative amplifier, which relaxes all constraints on laser components other than the intrinsic damage level of matter, so as to enable use of available laser system components. This can be accomplished by use of segmented components, spatial filters, at least one amplifier using solid state or gaseous media, and separated reflector members providing a long round trip time through the regenerative cavity, thereby allowing slower switching and adequate time to clear the spatial filters, etc. The laser system simplifies component requirements and reduces component cost while providing high energy output.

Emmett, John L. [Pleasanton, CA

1980-03-04T23:59:59.000Z

177

Laser Ignition  

NLE Websites -- All DOE Office Websites (Extended Search)

Laser Ignition Laser Ignition Laser Ignition A first excitation laser or other excitation light source is used in tandem with an ignitor laser to provide a compact, durable, engine deployable fuel ignition laser system. Available for thumbnail of Feynman Center (505) 665-9090 Email Laser Ignition A first excitation laser or other excitation light source is used in tandem with an ignitor laser to provide a compact, durable, engine deployable fuel ignition laser system. Reliable fuel ignition is provided over a wide range of fuel conditions by using a single remote excitation light source for one or more small lasers located proximate to one or more fuel combustion zones. In two embodiments the beam from the excitation light source is split with a portion of it going to the ignitor laser and a second portion

178

A World without Sample Preparation: Developing Rapid Uranium Isotope Measurement Capabilities by Resonance Ionization Mass Spectrometry (RIMS)  

SciTech Connect

We are developing highly sensitive, highly discriminating laser-based techniques for rapid determination of isotopic compositions. Rapid command of such information is critical to assessment of the origin and history of nuclear materials, particularly in post-detonation scenarios.

Knight, K B; Hutcheon, I D; Isselhardt, B H; Savina, M R; Prussin, S G

2009-06-08T23:59:59.000Z

179

Raman spectroscopic and mass spectrometric investigations of the hydrogen isotopes and isotopically labelled methane  

SciTech Connect

Suitable analytical methods must be tested and developed for monitoring the individual process steps within the fuel cycle of a fusion reactor and for tritium accountability. The utility of laser-Raman spectroscopy accompanied by mass spectrometry with an Omegatron was investigated using the analysis of all hydrogen isotopes and isotopically labeled methanes as an example. The Omegatron is useful for analyzing all hydrogen isotopes mixed with the stable helium isotopes. The application of this mass spectrometer were demonstrated by analyzing mixtures of deuterated methanes. In addition, it was employed to study the radiochemical Witzbach exchange reaction between tritium and methanes. A laser-Raman spectrometer was designed for analysis of tritium-containing gases and was built from individual components. A tritium-compatible, metal-sealed Raman cuvette having windows with good optical properties and additional means for measuring the stray light was first used successfully in this work. The Raman spectra of the hydrogen isotopes were acquired in the pure rotation mode and in the rotation-vibration mode and were used for on. The deuterated methanes were measured by Raman spectroscopy, the wavenumbers determined were assigned to the corresponding vibrations, and the wavenumbers for the rotational fine-structure were summarized in tables. The fundamental Vibrations of the deuterated methanes produced Witzbach reactions were detected and assigned. The fundamental vibrations of the molecules were obtained with Raman spectroscopy for the first time in this work. The @-Raman spectrometer assembled is well suited for the analysis of tritium- containing gases and is practical in combination with mass spectrometry using an Omegatron, for studying gases used in fusion.

Jewett, J.R., Fluor Daniel Hanford

1997-02-24T23:59:59.000Z

180

Effects of nitrate and water on the oxygen isotopic analysis of barium sulfate precipitated from  

E-Print Network (OSTI)

on an anion-exchange resin such as IRA-4005 before being precipitated as BaSO4. Isotopic analyses of O (d18 O by (1) ion chromatographic separation of SO4 2S from NO3 S , (2) increasing the salinity- ing H2O and NO3 S . These procedures are demonstrated for SO4 2S isotopic reference materials

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


181

Understanding denitrification with stable isotope measurements of N2: proof of concept study  

E-Print Network (OSTI)

The biologically mediated removal of nitrogen from estuarine and shallow coastal waters was investigated using a new method for the determination of N? isotope ratios. This method employs the use of a chromatographic separation technique to purify...

Downer, Roswell Curtis

2012-06-07T23:59:59.000Z

182

lead-isotope age  

Science Journals Connector (OSTI)

lead-isotope age, lead-lead age [An age in years calculated from the ratio of lead-207 to lead-206, a by-product of the uranium-thorium-lead age method] ? Blei-Isotopen-Alter n

2014-08-01T23:59:59.000Z

183

ISOTOPES IN WATER  

Science Journals Connector (OSTI)

The study of isotopic prosies ha two different though related basic aims: an understanding of the way in which the water cycle in linked to alterations in climate, and how the carbon cycle has responded to the...

W. GEORGE DARLING; ADRIAN H. BATH…

2006-01-01T23:59:59.000Z

184

Oak Ridge Isotope Products and Services - Current and Expected Supply and Demand  

SciTech Connect

Oak Ridge National Laboratory (ORNL) has been a major center of isotope production research, development, and distribution for over 50 years. Currently, the major isotope production activities include (1) the production of transuranium element radioisotopes, including 252 Cf; (2) the production of medical and industrial radioisotopes; (3) maintenance and expansion of the capabilities for production of enriched stable isotopes; and, (4) preparation of a wide range of custom-order chemical and physical forms of isotope products, particularly in accelerator physics research. The recent supply of and demand for isotope products and services in these areas, research and development (R&D), and the capabilities for future supply are described in more detail below. The keys to continuing the supply of these important products and services are the maintenance, improvement, and potential expansion of specialized facilities, including (1) the High Flux Isotope Reactor (HFIR), (2) the Radiochemical Engineering Development Center (REDC) and Radiochemical Development Laboratory (RDL) hot cell facilities, (3) the electromagnetic calutron mass separators and the plasma separation process equipment for isotope enrichment, and (4) the Isotope Research Materials Laboratory (IRML) equipment for preparation of specialized chemical and physical forms of isotope products. The status and plans for these ORNL isotope production facilities are also described below.

Aaron, W.S.; Alexander, C.W.; Cline, R.L.; Collins, E.D.; Klein, J.A.; Knauer, J.B., Jr.; Mirzadeh, S.

1999-08-29T23:59:59.000Z

185

Nuclear isotope thermometry  

Science Journals Connector (OSTI)

We discuss different aspects which might influence temperatures deduced from experimental isotopic yields in the multifragmentation process. It is shown that fluctuations due to the finite size of the system and distortions due to the decay of hot primary fragments conspire to blur the temperature determination in multifragmentation reactions. These facts suggest that caloric curves obtained through isotope thermometers, which were taken as evidence for a first-order phase transition in nuclear matter, should be investigated very carefully.

S. R. Souza, W. P. Tan, R. Donangelo, C. K. Gelbke, W. G. Lynch, and M. B. Tsang

2000-11-10T23:59:59.000Z

186

Actinide separations conference  

SciTech Connect

This report contains the abstracts for 55 presentations given at the fourteenth annual Actinide Separations Conference. (JDL)

Not Available

1990-01-01T23:59:59.000Z

187

On the Origin of the Lightest Molybdenum Isotopes  

SciTech Connect

We discuss implications of recent precision measurements for the {sup 93}Rh proton separation energy for the production of the lightest molybdenum isotopes in proton-rich type II supernova ejecta. It has recently been shown that a novel neutrino-induced process makes these ejecta a promising site for the production of the light molybdenum isotopes and other 'p-nuclei' with atomic mass near 100. The origin of these isotopes has long been uncertain. A distinguishing feature of nucleosynthesis in neutrino-irradiated outflows is that the relative production of {sup 92}Mo and {sup 94}Mo is set by a competition governed by the proton separation energy of {sup 93}Rh. We use detailed nuclear network calculations and the recent experimental results for this proton separation energy to place constraints on the outflow characteristics that produce the lightest molybdenum isotopes in their solar proportions. It is found that for the conditions calculated in recent two-dimensional supernova simulations, and also for a large range of outflow characteristics around these conditions, the solar ratio of {sup 92}Mo to {sup 94}Mo cannot be achieved. This suggests that either proton-rich winds from type II supernova do not exclusively produce both isotopes, or that these winds are qualitatively different than calculated in today's supernova models.

Fisker, J L; Hoffman, R D; Pruet, J

2007-10-24T23:59:59.000Z

188

Selection of Isotopes and Elements for Fuel Cycle Analysis  

SciTech Connect

Fuel cycle system analysis simulations examine how the selection among fuel cycle options for reactors, fuel, separation, and waste management impact uranium ore utilization, waste masses and volumes, radiotoxicity, heat to geologic repositories, isotope-dependent proliferation resistance measures, and so forth. Previously, such simulations have tended to track only a few actinide and fission product isotopes, those that have been identified as important to a few criteria from the standpoint of recycled material or waste, taken as a whole. After accounting for such isotopes, the residual mass is often characterized as “fission product other” or “actinide other”. However, detailed assessment of separation and waste management options now require identification of key isotopes and residual mass for Group 1A/2A elements (Rb, Cs, Sr, Ba), inert gases (Kr, Xe), halogens (Br, I), lanthanides, transition metals, transuranic (TRU), uranium, actinide decay products. The paper explains the rationale for a list of 81 isotopes and chemical elements to better support separation and waste management assessment in dynamic system analysis models such as Verifiable Fuel Cycle Simulation (VISION)

Steven J. Piet

2009-04-01T23:59:59.000Z

189

Molecular carbon isotopic evidence for the origin of geothermal hydrocarbons  

Science Journals Connector (OSTI)

... in the flask's headspace. This procedure produced negligible amounts of contaminating hydrocarbons. The geothermal hydrocarbons were separated and combusted, and the carbon dioxide product purified and measured using ... of the pyrolysis and spark discharge experiments, b, Isotopic abundance of hydrocarbons from four geothermal localities as follows: D, Cerro Prieto, well M-5, sampled January 1979; ...

David J. Des Marais; Jason H. Donchin; Nancy L. Nehring; Alfred H. Truesdell

1981-08-27T23:59:59.000Z

190

Exploring Neutron-Rich Oxygen Isotopes with MoNA  

E-Print Network (OSTI)

The Modular Neutron Array (MoNA) was used in conjunction with a large-gap dipole magnet (Sweeper) to measure neutron-unbound states in oxygen isotopes close to the neutron dripline. While no excited states were observed in 24O, a resonance at 45(2) keV above the neutron separation energy was observed in 23O.

N. Frank; T. Baumann; D. Bazin; J. Brown; P. A. DeYoung; J. E. Finck; A. Gade; J. Hinnefeld; R. Howes; J. -L. Lecouey; B. Luther; W. A. Peters; H. Scheit; A. Schiller; M. Thoennessen

2007-08-20T23:59:59.000Z

191

Laser ignition  

DOE Patents (OSTI)

In the apparatus of the invention, a first excitation laser or other excitation light source is used in tandem with an ignitor laser to provide a compact, durable, engine deployable fuel ignition laser system. The beam from the excitation light source is split with a portion of it going to the ignitor laser and a second portion of it being recombined with the first portion after a delay before injection into the ignitor laser. Reliable fuel ignition is provided over a wide range of fuel conditions by using a single remote excitation light source for one or more small lasers located proximate to one or more fuel combustion zones.

Early, James W. (Los Alamos, NM); Lester, Charles S. (San Juan Pueblo, NM)

2002-01-01T23:59:59.000Z

192

Radioactive Kr Isotopes  

Science Journals Connector (OSTI)

A radioactive isotope of 1.1-hour half-life has been produced in krypton by alpha-particle bombardment of Se74, enriched electromagnetically from 0.9 percent to 14.1 percent. Assignment of the isotope is made to Kr77. Aluminum absorption measurements indicate a positron end point of 1.7 Mev. In addition to annihilation radiation, gamma-rays and K-capture have been observed. The ratio of K-capture to positron emission from the Se74(?,n) reaction is computed as 2.6. The krypton 1.42-day isotope has been produced by an ?,n reaction on electromagnetically enriched Se76. The isotope is located as Kr79 and its half-life confirmed. A positron end point of 1.0 Mev is determined by aluminum absorption measurements. In addition to annihilation radiation, gamma-rays and K-capture have been observed. The ratio of K-capture to positron emission from the Se76(?,n) reaction is computed to be 50. The cross-section ratio for formation of Kr77 compared to Kr79 by alpha-particle bombardment of selenium is computed as 1.4. The 4.6-hour Kr85 isotope has been produced by a Se(?,n) reaction.

L. L. Woodward; D. A. Mccown; M. L. Pool

1948-10-01T23:59:59.000Z

193

Page 1Laser Safety Training Laser Institute of America Laser Safety Laser Institute of America  

E-Print Network (OSTI)

Page 1Laser Safety Training © Laser Institute of America 1 Laser Safety © Laser Institute of America Laser Safety: Hazards, Bioeffects, and Control Measures Laser Institute of America Gus Anibarro Education Manager 2Laser Safety © Laser Institute of America Laser Safety Overview Laser Safety Accidents

Farritor, Shane

194

Laser Telecommunication timeLaser beam  

E-Print Network (OSTI)

Laser Telecommunication Experiment Laser time Laser beam intensity timeLaser beam Laser battery Laser connected to a circuit without a modulator. Bottom graph illustrates what happen when a modulating signal is superimposed to the DC voltage driving the laser Laser beam intensity DC Input voltage DC

La Rosa, Andres H.

195

Membrane Separations Research  

E-Print Network (OSTI)

MEMBRANE SEPARATIONS RESEARCH James R. Fair Chemical Engineering Department The University of Texas at Austin Austin, TX 78712 ABSTRACT The use of membranes for separating gaseous and liquid mixtures has grown dramatically in the past 15... years. Applications have been dominated by light gas separations and water purification. During this pioneering period, equipment containing the membrane suIfaces has been developed to a point where failures are minimal and the membranes themselves...

Fair, J. R.

196

GENERATION OF RADIOXENON ISOTOPES  

SciTech Connect

With the continued population of the International Monitoring System (IMS) network and the certification of radioxenon laboratory systems it has become necessary to calibrate and test these systems using as many of the radioxenon isotopes as possible. Several very promising techniques have been explored recently that allow for convenient production of Xe-133, Xe-131m, the short-lived isotope Xe-135, and even the difficult to obtain Xe-133m. IMS national and international laboratories have traditionally obtained Xe-133 from medical isotope suppliers. The activity of these medical dose samples is extremely high (~ 740 MBq) and requires very careful fume hood work to dilute down to appropriate levels (~ 10 Bq). By waiting for 10 or more half-lives it is possible to reduce the handling regimen considerably, while also obtaining a strong Xe-131m signature due to its longer half-life (11.9 days). The short-lived isotope Xe-135 (9.14 hrs) and the longer lived parent nuclide Xe-133m (2.2 day half-life) are never present in these samples. To obtain these isotopes another source or technique is required. This paper will discuss the two techniques developed and implemented at Pacific Northwest National Lab (PNNL) and show the results obtained from each technique. The first is an in-house method that allows for on demand production of two of these isotopes, Xe-133 and Xe-135, using HEU and a modest flux neutron source. The second method uses a research reactor at the Pullman campus of Washington State University to produce Xe-133, Xe-133m and Xe-135.

McIntyre, Justin I.; Pratt, Sharon L.; Bowyer, Ted W.; Cooper, Matthew W.; Hayes, James C.; Heimbigner, Tom R.; Hubbard, Charles W.; Miley, Harry S.; Ripplinger, Mike D.

2008-09-23T23:59:59.000Z

197

Laser microphone  

DOE Patents (OSTI)

A microphone for detecting sound pressure waves includes a laser resonator having a laser gain material aligned coaxially between a pair of first and second mirrors for producing a laser beam. A reference cell is disposed between the laser material and one of the mirrors for transmitting a reference portion of the laser beam between the mirrors. A sensing cell is disposed between the laser material and one of the mirrors, and is laterally displaced from the reference cell for transmitting a signal portion of the laser beam, with the sensing cell being open for receiving the sound waves. A photodetector is disposed in optical communication with the first mirror for receiving the laser beam, and produces an acoustic signal therefrom for the sound waves.

Veligdan, James T. (Manorville, NY)

2000-11-14T23:59:59.000Z

198

High-Resolution Triple Resonance Autoionization of Uranium Isotopes  

SciTech Connect

The near-threshold autoionization (AI) spectrum of uranium has been investigated by triple-resonance excitation with single-mode continuous lasers. Spectra were recorded over the first {approx}30 cm-1 above the first ionization limit at a resolution of 3x10-4 cm 1 using intermediate states with different J values (6, 7, 8) to assign AI level total angular momentum JAI = 5 to 9. Resonances with widths ranging from 8 MHz to 30 GHz were observed; the strongest ones have JAI = 9 and widths of {approx} 60 MHz. Hyperfine structures for 235U and isotope shifts for 234,235U have been measured in the two intermediate levels and in the final AI level for the most favorable excitation path. These measurements were performed using aqueous samples containing sub-milligram quantities of uranium at natural isotopic abundances, indicating the potential of this approach for trace isotope ratio determinations.

Schumann, Philipp G.; Wendt, K; Bushaw, Bruce A.

2005-11-01T23:59:59.000Z

199

Separation technologies: Marketing factors  

SciTech Connect

The chemical and petroleum industries consume approximately 5.8 quads per year of energy. Within these industries, 43% of the energy is used by separation processes to recover and purify products. With 40,000 distillation columns in operation, distillation is used to make 95% of all separations in these two industries. Although separations are identified which are amenable to advanced separation technologies (that make distillation more energy-efficient), they are not implemented because of commercial barriers. The focus of this work was on barriers which can by overcome by implementing advanced separation-related technologies. Barriers were screened and prioritized, and Return On Investment (ROI) was calculated for each project designed to overcome a high priority barrier. Economic analyses were based on specific separations such as ethylene-ethane, propylene-propane, ethyl benzene-styrene, and ethanol-water. These separations were selected because they consume significant amounts of energy for separation. Thus, conclusions are based on a limited number of case studies; an approach necessary to complete this project within a reasonable time frame. Recommended projects are discussed and summarized.

Humphrey, J.L.; Seibert, A.F.; Goodpastor, C.V.

1991-12-01T23:59:59.000Z

200

Substituted polyacetylene separation membrane  

DOE Patents (OSTI)

A separation membrane is described which is useful for gas separation, particularly separation of C{sub 2+} hydrocarbons from natural gas. The invention encompasses the membrane itself, methods of making it and processes for using it. The membrane comprises a polymer having repeating units of a hydrocarbon-based, disubstituted polyacetylene, having the general formula shown in the accompanying diagram, wherein R{sub 1} is chosen from the group consisting of C{sub 1}-C{sub 4} alkyl and phenyl, and wherein R{sub 2} is chosen from the group consisting of hydrogen and phenyl. In the most preferred embodiment, the membrane comprises poly(4-methyl-2-pentyne) [PMP]. The membrane exhibits good chemical resistance and has super-glassy properties with regard to separating certain large, condensable permeant species from smaller, less-condensable permeant species. The membranes may also be useful in other fluid separations. 4 figs.

Pinnau, I.; Morisato, Atsushi

1998-01-13T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


201

Substituted polyacetylene separation membrane  

DOE Patents (OSTI)

A separation membrane useful for gas separation, particularly separation of C.sub.2+ hydrocarbons from natural gas. The invention encompasses the membrane itself, methods of making it and processes for using it. The membrane comprises a polymer having repeating units of a hydrocarbon-based, disubstituted polyacetylene, having the general formula: ##STR1## wherein R.sub.1 is chosen from the group consisting of C.sub.1 -C.sub.4 alkyl and phenyl, and wherein R.sub.2 is chosen from the group consisting of hydrogen and phenyl. In the most preferred embodiment, the membrane comprises poly(4-methyl-2-pentyne) ›PMP!. The membrane exhibits good chemical resistance and has super-glassy properties with regard to separating certain large, condensable permeant species from smaller, less-condensable permeant species. The membranes may also be useful in other fluid separations.

Pinnau, Ingo (Palo Alto, CA); Morisato, Atsushi (Tokyo, JP)

1998-01-13T23:59:59.000Z

202

Separators for flywheel rotors  

DOE Patents (OSTI)

A separator forms a connection between the rotors of a concentric rotor assembly. This separator allows for the relatively free expansion of outer rotors away from inner rotors while providing a connection between the rotors that is strong enough to prevent disassembly. The rotor assembly includes at least two rotors referred to as inner and outer flywheel rings or rotors. This combination of inner flywheel ring, separator, and outer flywheel ring may be nested to include an arbitrary number of concentric rings. The separator may be a segmented or continuous ring that abuts the ends of the inner rotor and the inner bore of the outer rotor. It is supported against centrifugal loads by the outer rotor and is affixed to the outer rotor. The separator is allowed to slide with respect to the inner rotor. It is made of a material that has a modulus of elasticity that is lower than that of the rotors. 10 figs.

Bender, D.A.; Kuklo, T.C.

1998-07-07T23:59:59.000Z

203

Separators for flywheel rotors  

DOE Patents (OSTI)

A separator forms a connection between the rotors of a concentric rotor assembly. This separator allows for the relatively free expansion of outer rotors away from inner rotors while providing a connection between the rotors that is strong enough to prevent disassembly. The rotor assembly includes at least two rotors referred to as inner and outer flywheel rings or rotors. This combination of inner flywheel ring, separator, and outer flywheel ring may be nested to include an arbitrary number of concentric rings. The separator may be a segmented or continuous ring that abuts the ends of the inner rotor and the inner bore of the outer rotor. It is supported against centrifugal loads by the outer rotor and is affixed to the outer rotor. The separator is allowed to slide with respect to the inner rotor. It is made of a material that has a modulus of elasticity that is lower than that of the rotors.

Bender, Donald A. (Dublin, CA); Kuklo, Thomas C. (Oakdale, CA)

1998-01-01T23:59:59.000Z

204

Laser ignition  

DOE Patents (OSTI)

In the apparatus of the invention, a first excitation laser or other excitation light source is used in tandem with an ignitor laser to provide a compact, durable, engine deployable fuel ignition laser system. Reliable fuel ignition is provided over a wide range of fuel conditions by using a single remote excitation light source for one or more small lasers located proximate to one or more fuel combustion zones. In a third embodiment, alternating short and long pulses of light from the excitation light source are directed into the ignitor laser. Each of the embodiments of the invention can be multiplexed so as to provide laser light energy sequentially to more than one ignitor laser.

Early, James W. (Los Alamos, NM); Lester, Charles S. (San Juan Pueblo, NM)

2003-01-01T23:59:59.000Z

205

Selective Dissociation of Sulfur Hexafluoride by Intense CO2 Laser Radiation in Pulsed Gas Dynamic Flow  

Science Journals Connector (OSTI)

Isotopically selective IR multiphoton dissociation (MPD) of SF6 in a pulsed gas dynamic flow was studied. The dependence of the yield of the product SF4 on the frequency of CO2 laser radiation exciting SF6 molecu...

G. N. Makarov; A. N. Petin

2000-11-01T23:59:59.000Z

206

Ca isotopic anomaly in the atmospheres of Ap stars  

E-Print Network (OSTI)

We present results of the Ca stratification analysis in the atmospheres of 21 magnetic chemically peculiar (Ap) stars. This analysis was based on the spectral observations carried out with the UVES spectrograph attached to the 8-m VLT telescope. Ca was found to be strongly stratified in all stars with different effective temperatures and magnetic field strengths. This element is overabundant by 1-1.5 dex below logtau_5000~-1 and strongly depleted above logtau_5000=-1.5. Based on the overall Ca abundance distributions, we modelled a profile of the IR-triplet Ca II 8498 line. It shows a significant contribution of the heavy isotopes 46Ca and 48Ca, which represent less than 1% of the solar Ca isotopic mixture. In Ap stars with the relatively small surface magnetic fields (Ca isotope is concentrated close to the photosphere, while the heavy isotopes are pushed towards the outer layers. Isotopic separation disappears in the atmospheres of stars with magnetic fields above 6-7 kG. The observed overall Ca stratification and isotopic anomalies may be explained by a combined action of the radiatively-driven diffusion and the light-induced drift.

T. Ryabchikova; O. Kochukhov; S. Bagnulo

2007-03-13T23:59:59.000Z

207

Unattended Environmental Sampling and Laser-based Enrichment Assay for Detection of Undeclared HEU Production in Enrichment Plants  

SciTech Connect

Nuclear power is enjoying rapid growth as government energy policies and public demand shift toward carbon neutral energy production. Accompanying the growth in nuclear power is the requirement for increased nuclear fuel production, including a significant expansion in uranium enrichment capacity. Essential to the success of the nuclear energy renaissance is the development and implementation of sustainable, proliferation-resistant nuclear power generation. Unauthorized production of highly enriched uranium (HEU) remains the primary proliferation concern for modern gaseous centrifuge enrichment plants (GCEPs). While to date there has been no indication of declared, safeguarded GCEPs producing HEU, the massive separative work unit (SWU) processing power of modern GCEPs presents a significant latent risk of nuclear breakout and suggests the need for more timely detection of potential facility misuse. The Pacific Northwest National Laboratory is developing an unattended safeguards instrument, combining continuous aerosol particulate collection with uranium isotope assay, to provide timely HEU detection within a GCEP. This approach is based on laser vaporization of aerosol particulates, followed by laser spectroscopy to characterize the uranium enrichment level. We demonstrate enrichment assay, with relative isotope abundance uncertainty <5%, on individual micron-sized particles that are trace components within a mixture ‘background’ particles

Anheier, Norman C.; Bushaw, Bruce A.

2010-04-15T23:59:59.000Z

208

Computational Nuclear Forensics Analysis of Weapons-grade Plutonium Separated from Fuel Irradiated in a Thermal Reactor  

E-Print Network (OSTI)

have been irradiated to the desired burnup in the Oak Ridge National Laboratory- High Flux Isotope Reactor (ORNL-HFIR), and then separated using the PUREX process to experimentally determine the intrinsic signature of the fuel. The experimental data...

Coles, Taylor Marie

2014-04-27T23:59:59.000Z

209

Continuous flow system for controlling phases separation near ? transition  

SciTech Connect

As demands on 3He are increasing and conventional 3He production through tritium decay is decreasing, alternative 3He production methods are becoming economically viable. One such possibility is to use entropy filters for extraction of the 3He isotope from natural gas. According to the phase diagram of the 3He, its solidification is impossible by only lowering of the temperature. Hence during the cooling process at stable pressure we can reach ?-point and pass to the special phase - He II. The total density of HeII is a sum of the two phases: normal the superfluid ones. It is possible to separate these two phases with an entropy filter - the barrier for the classically-behaving normal phase. This barrier can also be used to separate the two main isotopes of He: 4He and 3He, because at temperatures close to the 4He-?-point the 3He isotope is part of the normal phase. The paper presents continuous flow schemes of different separation methods of 3He from helium commodity coming from natural gas cryogenic processing. An overall thermodynamic efficiency of the 3He/4He separation process is presented. A simplified model of continuous flow HeI -HeII recuperative heat exchanger is given. Ceramic and carbon porous plugs have been tested in entropy filter applications.

Chorowski, M.; Poli?ski, J. [Wroc?aw University of Technology, Wybrze?e Wyspia?skiego 27,50-560 Wroc?aw (Poland); Kempi?ski, W.; Trybu?a, Z.; ?o?, Sz. [Institute of Molecular Physics, Polish Academy of Sciences, ul. Smoluchowskiego 17,60-179 Pozna? (Poland); Cho?ast, K.; Kociemba, A. [Polish Oil and Gas Company, Odolanow, ul. Krotoszynska 148, 63-430 Odolanow (Poland)

2014-01-29T23:59:59.000Z

210

Synthesis and investigation of neutron-rich transuranium isotopes  

SciTech Connect

Spontaneous fission activities produced in the reactions of /sup 13/C, /sup 15/N, /sup 16/O, and /sup 18/O ions with /sup 248/Cm and /sup 249/Bk targets are reported; excitation functions and half-lives of element 104 isotopes are given. Reactions that led to the formation of /sup 259/Fm are discussed in detail. The principal features of the SuperHILAC on-line isotope separator and some of the anticipated applications are described. 14 figures, 2 tables. (RWR)

Nitschke, J.M.

1980-09-01T23:59:59.000Z

211

Vacuum barrier for excimer lasers  

DOE Patents (OSTI)

A barrier for separating the vacuum area of a diode from the pressurized gas area of an excimer laser. The barrier is a composite material comprising layers of a metal such as copper, along with layers of polyimide, and a matrix of graphite fiber yarns impregnated with epoxy. The barrier is stronger than conventional foil barriers, and allows greater electron throughput. 3 figs.

Shurter, R.P.

1992-09-15T23:59:59.000Z

212

USABC Battery Separator Development  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

Separator Development P.I. - Ron Smith Presenter - Kristoffer Stokes, Ph.D. Celgard, LLC Project ID ES007 May 10, 2011 This presentation does not contain any proprietary,...

213

successfully demonstrated the separation  

NLE Websites -- All DOE Office Websites (Extended Search)

successfully demonstrated the separation and capture of 90 percent successfully demonstrated the separation and capture of 90 percent of the c arbon dioxide (CO 2 ) from a pulve rized coal plant. In t he ARRA-funded project, Membrane Technology and Research Inc. (MTR) and its partners tested the Polaris(tm) membrane system, which uses a CO 2 -selective polymeric membrane material and module to capture CO 2 from a plant's flue gas. Since the Polaris(tm) membranes

214

Hydrogen separation process  

DOE Patents (OSTI)

A method for separating a hydrogen-rich product stream from a feed stream comprising hydrogen and at least one carbon-containing gas, comprising feeding the feed stream, at an inlet pressure greater than atmospheric pressure and a temperature greater than 200.degree. C., to a hydrogen separation membrane system comprising a membrane that is selectively permeable to hydrogen, and producing a hydrogen-rich permeate product stream on the permeate side of the membrane and a carbon dioxide-rich product raffinate stream on the raffinate side of the membrane. A method for separating a hydrogen-rich product stream from a feed stream comprising hydrogen and at least one carbon-containing gas, comprising feeding the feed stream, at an inlet pressure greater than atmospheric pressure and a temperature greater than 200.degree. C., to an integrated water gas shift/hydrogen separation membrane system wherein the hydrogen separation membrane system comprises a membrane that is selectively permeable to hydrogen, and producing a hydrogen-rich permeate product stream on the permeate side of the membrane and a carbon dioxide-rich product raffinate stream on the raffinate side of the membrane. A method for pretreating a membrane, comprising: heating the membrane to a desired operating temperature and desired feed pressure in a flow of inert gas for a sufficient time to cause the membrane to mechanically deform; decreasing the feed pressure to approximately ambient pressure; and optionally, flowing an oxidizing agent across the membrane before, during, or after deformation of the membrane. A method of supporting a hydrogen separation membrane system comprising selecting a hydrogen separation membrane system comprising one or more catalyst outer layers deposited on a hydrogen transport membrane layer and sealing the hydrogen separation membrane system to a porous support.

Mundschau, Michael (Longmont, CO); Xie, Xiaobing (Foster City, CA); Evenson, IV, Carl (Lafayette, CO); Grimmer, Paul (Longmont, CO); Wright, Harold (Longmont, CO)

2011-05-24T23:59:59.000Z

215

Laser ignition  

DOE Patents (OSTI)

In the apparatus of the invention, a first excitation laser or other excitation light source is used in tandem with an ignitor laser to provide a compact, durable, engine deployable fuel ignition laser system. Reliable fuel ignition is provided over a wide range of fuel conditions by using a single remote excitation light source for one or more small lasers located proximate to one or more fuel combustion zones. In the embodiment of the invention claimed herein, the beam from the excitation light source is split with a portion of it going to the ignitor laser and a second portion of it being combined with either the first portion after a delay before injection into the ignitor laser.

Early, James W. (Los Alamos, NM); Lester, Charles S. (San Juan Pueblo, NM)

2002-01-01T23:59:59.000Z

216

Laser ignition  

DOE Patents (OSTI)

In the apparatus of the invention, a first excitation laser or other excitation light source capable of producing alternating beams of light having different wavelengths is used in tandem with one or more ignitor lasers to provide a compact, durable, engine deployable fuel ignition laser system. Reliable fuel ignition is provided over a wide range of fuel conditions by using the single remote excitation light source for pumping one or more small lasers located proximate to one or more fuel combustion zones with alternating wavelengths of light.

Early, James W. (Los Alamos, NM); Lester, Charles S. (San Juan Pueblo, NM)

2002-01-01T23:59:59.000Z

217

Stark-tuned, far-infrared laser for high-frequency plasma diagnostics  

Science Journals Connector (OSTI)

A Stark-tuned optically pumped far-infrared CH3OH laser operating at 119 ?m has been built. The laser is designed to operate at high power while exhibiting a well-separated...

Mansfield, D K; Krug, Peter A; Vocaturo, M; Guttadora, L; Rockmore, M; Micai, K

1992-01-01T23:59:59.000Z

218

Organic Separation Test Results  

SciTech Connect

Separable organics have been defined as “those organic compounds of very limited solubility in the bulk waste and that can form a separate liquid phase or layer” (Smalley and Nguyen 2013), and result from three main solvent extraction processes: U Plant Uranium Recovery Process, B Plant Waste Fractionation Process, and Plutonium Uranium Extraction (PUREX) Process. The primary organic solvents associated with tank solids are TBP, D2EHPA, and NPH. There is concern that, while this organic material is bound to the sludge particles as it is stored in the tanks, waste feed delivery activities, specifically transfer pump and mixer pump operations, could cause the organics to form a separated layer in the tank farms feed tank. Therefore, Washington River Protection Solutions (WRPS) is experimentally evaluating the potential of organic solvents separating from the tank solids (sludge) during waste feed delivery activities, specifically the waste mixing and transfer processes. Given the Hanford Tank Waste Treatment and Immobilization Plant (WTP) waste acceptance criteria per the Waste Feed Acceptance Criteria document (24590-WTP-RPT-MGT-11-014) that there is to be “no visible layer” of separable organics in the waste feed, this would result in the batch being unacceptable to transfer to WTP. This study is of particular importance to WRPS because of these WTP requirements.

Russell, Renee L.; Rinehart, Donald E.; Peterson, Reid A.

2014-09-22T23:59:59.000Z

219

United States Department of Energy Office of Nuclear Energy, Isotope Production and Distribution Program financial statements, September 30, 1996 and 1995  

SciTech Connect

The charter of the Department of Energy (DOE) Isotope Production and Distribution Program (Isotope Program) covers the production and sale of radioactive and stable isotopes, associated byproducts, surplus materials such as lithium, and related isotope services. Service provided include, but are not limited to, irradiation services, target preparation and processing, source encapsulation and other special preparations, analyses, chemical separations, and leasing of stable isotopes for research purposes. Isotope Program products and services are sold worldwide for use in a wide variety of research, development, biomedical, and industrial applications. This report presents the results of the independent certified public accountants` audit of the Isotope Production and Distribution Program`s (Isotope) financial statements as of September 30, 1996.

NONE

1997-04-01T23:59:59.000Z

220

Comparisons between stable isotope tr  

Science Journals Connector (OSTI)

Nitrogen spiraling in streams: Comparisons between stable isotope tracer and nutrient addition experiments. Abstract—A common method to quantify stream.

2007-05-31T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


221

Separators for electrochemical cells  

DOE Patents (OSTI)

Provided are separators for use in an electrochemical cell comprising (a) an inorganic oxide and (b) an organic polymer, wherein the inorganic oxide comprises organic substituents. Preferably, the inorganic oxide comprises an hydrated aluminum oxide of the formula Al.sub.2O.sub.3.xH.sub.2O, wherein x is less than 1.0, and wherein the hydrated aluminum oxide comprises organic substituents, preferably comprising a reaction product of a multifunctional monomer and/or organic carbonate with an aluminum oxide, such as pseudo-boehmite and an aluminum oxide. Also provided are electrochemical cells comprising such separators.

Carlson, Steven Allen; Anakor, Ifenna Kingsley

2014-11-11T23:59:59.000Z

222

Identification of Heavy and Superheavy Nuclides Using Chemical Separator Systems  

SciTech Connect

With the recent synthesis of superheavy nuclides produced in the reactions {sup 48}Ca+{sup 238}U and {sup 48}Ca+{sup 242,244}Pu, much longer-lived nuclei than the previously known neutron-deficient isotopes of the heaviest elements have been identified. Half-lives of several hours and up to several years have been predicted for the longest-lived isotopes of these elements. Thus, the sensitivity of radiochemical separation techniques may present a viable alternative to physical separator systems for the discovery of some of the predicted longer-lived heavy and superheavy nuclides. The advantages of chemical separator systems in comparison to kinematic separators lie in the possibility of using thick targets, high beam intensities spread over larger target areas and in providing access to nuclides emitted under large angles and low velocities. Thus, chemical separator systems are ideally suited to study also transfer and (HI, axn) reaction products. In the following, a study of (HI, axn) reactions will be presented and prospects to chemically identify heavy and superheavy elements discussed.

Turler, Andreas

1999-12-31T23:59:59.000Z

223

Evolution of isotopic composition of reprocessed uranium during the multiple recycling in light water reactors with natural uranium feed  

SciTech Connect

A complex approach based on the consistent modeling of neutron-physics processes and processes of cascade separation of isotopes is applied for analyzing physical problems of the multiple usage of reprocessed uranium in the fuel cycle of light water reactors. A number of scenarios of multiple recycling of reprocessed uranium in light water reactors are considered. In the process, an excess absorption of neutrons by the {sup 236}U isotope is compensated by re-enrichment in the {sup 235}U isotope. Specific consumptions of natural uranium for re-enrichment of the reprocessed uranium depending on the content of the {sup 232}U isotope are obtained.

Smirnov, A. Yu., E-mail: a.y.smirnoff@rambler.ru; Sulaberidze, G. A. [National Research Nuclear University MEPhI (Russian Federation); Alekseev, P. N.; Dudnikov, A. A.; Nevinitsa, V. A., E-mail: neva@dhtp.kiae.ru; Proselkov, V. N.; Chibinyaev, A. V. [Russian Research Centre Kurchatov Institute (Russian Federation)

2012-12-15T23:59:59.000Z

224

Development of high through-put Sr isotope analysis for monitoring reservoir integrity for CO{sub 2} storage.  

SciTech Connect

Recent innovations in multi-collector ICP-mass spectrometry (MC-ICP-MS) have allowed for rapid and precise measurements of isotope ratios in geological samples. Naturally occurring Sr isotopes has the potential for use in Monitoring, Verification, and Accounting (MVA) associated with geologic CO2 storage. Sr isotopes can be useful for: Sensitive tracking of brine migration; Determining seal rock leakage; Studying fluid/rock reactions. We have optimized separation chemistry procedures that will allow operators to prepare samples for Sr isotope analysis off site using rapid, low cost methods.

Wall, Andy; Jain, Jinesh; Stewart, Brian; Capo, Rosemary; Hakala, Alexandra J.; Hammack, Richard; Guthrie, George

2012-01-01T23:59:59.000Z

225

Laser device  

DOE Patents (OSTI)

A laser device includes a virtual source configured to aim laser energy that originates from a true source. The virtual source has a vertical rotational axis during vertical motion of the virtual source and the vertical axis passes through an exit point from which the laser energy emanates independent of virtual source position. The emanating laser energy is collinear with an orientation line. The laser device includes a virtual source manipulation mechanism that positions the virtual source. The manipulation mechanism has a center of lateral pivot approximately coincident with a lateral index and a center of vertical pivot approximately coincident with a vertical index. The vertical index and lateral index intersect at an index origin. The virtual source and manipulation mechanism auto align the orientation line through the index origin during virtual source motion.

Scott, Jill R. (Idaho Falls, ID); Tremblay, Paul L. (Idaho Falls, ID)

2008-08-19T23:59:59.000Z

226

Geometry of the CaOCH3 radical from isotope effects A1 transition  

E-Print Network (OSTI)

in a laser abla- tion source by reacting methanol with calcium vapour produced by ablating a calcium rod lengths to values obtained from OCH3 [3] and methanol [4], respectively, and had then determined the CaO12 CD3, CaO13 CH3, and CaO13 CD3 by using different varieties of isotopically substituted methanol

Le Roy, Robert J.

227

RADIOCHEMICAL STUDIES OF NEUTRON DEFICIENT ACTINIDE ISOTOPES  

E-Print Network (OSTI)

Isotope Targets and Foils, AERE-R 5097, Paper 10 (1965). V.Isotope Targets and Foils, AERE-R 5097 Paper 12 (1965). K.M.Isotope Targets and Foils, AERE-R-5097 Paper 11 (1965). M.

Williams, Kimberly Eve

2011-01-01T23:59:59.000Z

228

Advanced Nuclear Final Solicitation Fact Sheet_Dec-2014  

Office of Environmental Management (EM)

tails to a higher isotopic content of U235 including by (1) gas centrifuge or (2) laser isotope separation and; c) Nuclear Fuel Fabrication Projects that fabricate nuclear...

229

First decay study of the very neutron-rich isotope 93Br  

Science Journals Connector (OSTI)

The decay of the mass-separated, very neutron-rich isotope 93Br has been studied by ? spectroscopy. A level scheme of its daughter 93Kr has been constructed. Level energies, ?-ray branching ratios, and multipolarities suggest spins and parities which are in accord with a smooth systematics of the N=57 isotones for Z<~40, suggesting the N=56 subshell closure still to be effective in Kr isotopes. So far, there is no indication of a progressive onset of deformation in neutron-rich Kr isotopes.

G. Lhersonneau; A. Wöhr; B. Pfeiffer; K.-L. Kratz; the ISOLDE Collaboration

2001-02-20T23:59:59.000Z

230

Isotope and Nuclear Chemistry Division annual report FY 1986, October 1985-September 1986  

SciTech Connect

This report describes progress in the major research and development programs carried out in FY 1986 by the Isotope and Nuclear Chemistry Division. The report includes articles on radiochemical diagnostics and weapons tests; weapons radiochemical diagnostics research and development; other unclassified weapons research; stable and radioactive isotope production and separation; chemical biology and nuclear medicine; element and isotope transport and fixation; actinide and transition metal chemistry; structural chemistry, spectroscopy, and applications; nuclear structure and reactions; irradiation facilities; advanced concepts and technology; and atmospheric chemistry.

Heiken, J.H. (ed.)

1987-06-01T23:59:59.000Z

231

?-decay properties of the new neutron deficient isotope 212Pa  

Science Journals Connector (OSTI)

The new neutron deficient isotope 212Pa has been produced in the 182W(35Cl,5n) reaction at a beam energy of 182.5 MeV. Evaporation residues have been separated with the JAERI recoil mass separator and identified on the basis of time- and position-correlated ?-decay chains. The ? decay from the ground state of 212Pa has been observed with an ?-particle energy of 8.270(30) MeV and a half-life of 5.1-1.9+6.1 ms.

S. Mitsuoka; H. Ikezoe; T. Ikuta; Y. Nagame; K. Tsukada; I. Nishinaka; Y. Oura; Y. L. Zhao

1997-03-01T23:59:59.000Z

232

Isotopic Analysis- Fluid | Open Energy Information  

Open Energy Info (EERE)

Isotopic Analysis- Fluid Isotopic Analysis- Fluid Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Technique: Isotopic Analysis- Fluid Details Activities (61) Areas (32) Regions (6) NEPA(0) Exploration Technique Information Exploration Group: Lab Analysis Techniques Exploration Sub Group: Fluid Lab Analysis Parent Exploration Technique: Fluid Lab Analysis Information Provided by Technique Lithology: Water rock interaction Stratigraphic/Structural: Hydrological: Origin of hydrothermal fluids; Mixing of hydrothermal fluids Thermal: Isotopic ratios can be used to characterize and locate subsurface thermal anomalies. Dictionary.png Isotopic Analysis- Fluid: Isotopes are atoms of the same element that have different numbers of neutrons. An isotopic analysis looks at a particular isotopic element(s) in

233

Means and method of detection in chemical separation procedures  

DOE Patents (OSTI)

A means and method for indirect detection of constituent components of a mixture separated in a chemical separation process. Fluorescing ions are distributed across the area in which separation of the mixture will occur to provide a generally uniform background fluorescence intensity. For example, the mixture is comprised of one or more charged analytes which displace fluorescing ions where its constituent components separate to. Fluorescing ions of the same charge as the charged analyte components cause a displacement. The displacement results in the location of the separated components having a reduced fluorescence intensity to the remainder of the background. Detection of the lower fluorescence intensity areas can be visually, by photographic means and methods, or by automated laser scanning.

Yeung, Edward S. (Ames, IA); Koutny, Lance B. (Ames, IA); Hogan, Barry L. (Ames, IA); Cheung, Chan K. (Ames, IA); Ma, Yinfa (Ames, IA)

1993-03-09T23:59:59.000Z

234

Laser goniometer  

DOE Patents (OSTI)

The laser goniometer is an apparatus which permits an operator to sight along a geologic feature and orient a collimated lamer beam to match the attitude of the feature directly. The horizontal orientation (strike) and the angle from horizontal (dip), are detected by rotary incremental encoders attached to the laser goniometer which provide a digital readout of the azimuth and tilt of the collimated laser beam. A microprocessor then translates the square wave signal encoder outputs into an ASCII signal for use by data recording equipment.

Fairer, George M. (Boulder, CO); Boernge, James M. (Lakewood, CO); Harris, David W. (Lakewood, CO); Campbell, DeWayne A. (Littleton, CO); Tuttle, Gene E. (Littleton, CO); McKeown, Mark H. (Golden, CO); Beason, Steven C. (Lakewood, CO)

1993-01-01T23:59:59.000Z

235

Advanced Separation Consortium  

SciTech Connect

The Center for Advanced Separation Technologies (CAST) was formed in 2001 under the sponsorship of the US Department of Energy to conduct fundamental research in advanced separation and to develop technologies that can be used to produce coal and minerals in an efficient and environmentally acceptable manner. The CAST consortium consists of seven universities - Virginia Tech, West Virginia University, University of Kentucky, Montana Tech, University of Utah, University of Nevada-Reno, and New Mexico Tech. The consortium brings together a broad range of expertise to solve problems facing the US coal industry and the mining sector in general. At present, a total of 60 research projects are under way. The article outlines some of these, on topics including innovative dewatering technologies, removal of mercury and other impurities, and modelling of the flotation process. 1 photo.

NONE

2006-01-01T23:59:59.000Z

236

Innovative Separations Technologies  

SciTech Connect

Reprocessing used nuclear fuel (UNF) is a multi-faceted problem involving chemistry, material properties, and engineering. Technology options are available to meet a variety of processing goals. A decision about which reprocessing method is best depends significantly on the process attributes considered to be a priority. New methods of reprocessing that could provide advantages over the aqueous Plutonium Uranium Reduction Extraction (PUREX) and Uranium Extraction + (UREX+) processes, electrochemical, and other approaches are under investigation in the Fuel Cycle Research and Development (FCR&D) Separations Campaign. In an attempt to develop a revolutionary approach to UNF recycle that may have more favorable characteristics than existing technologies, five innovative separations projects have been initiated. These include: (1) Nitrogen Trifluoride for UNF Processing; (2) Reactive Fluoride Gas (SF6) for UNF Processing; (3) Dry Head-end Nitration Processing; (4) Chlorination Processing of UNF; and (5) Enhanced Oxidation/Chlorination Processing of UNF. This report provides a description of the proposed processes, explores how they fit into the Modified Open Cycle (MOC) and Full Recycle (FR) fuel cycles, and identifies performance differences when compared to 'reference' advanced aqueous and fluoride volatility separations cases. To be able to highlight the key changes to the reference case, general background on advanced aqueous solvent extraction, advanced oxidative processes (e.g., volumetric oxidation, or 'voloxidation,' which is high temperature reaction of oxide UNF with oxygen, or modified using other oxidizing and reducing gases), and fluorination and chlorination processes is provided.

J. Tripp; N. Soelberg; R. Wigeland

2011-05-01T23:59:59.000Z

237

Pulsed Laser Deposition | EMSL  

NLE Websites -- All DOE Office Websites (Extended Search)

Pulsed Laser Deposition Pulsed Laser Deposition EMSL's pulsed laser deposition (PLD) system is designed for epitaxial growth of oxide, ceramic, or synthetic mineral thin films and...

238

Laser barometer  

SciTech Connect

This paper describes an invention of a pressure measuring instrument which uses laser radiation to sense the pressure in an enclosed environment by means of measuring the change in refractive index of a gas - which is pressure dependent.

Abercrombie, K.R.; Shiels, D.; Rash, T.

1998-04-01T23:59:59.000Z

239

LASER ACCELERATORS  

E-Print Network (OSTI)

UNIVERSITY OF CALIFORNIA Accelerator & Fusion Researchat the 1983 Particle Accelerator Conference, Santa Fe, NM,March 21-23, 1983 LASER ACCELERATORS A.M. Sessler TWO-WEEK

Sessler, A.M.

2008-01-01T23:59:59.000Z

240

Laser ignition  

Science Journals Connector (OSTI)

Due to their thermodynamic benefits, second-generation spark-ignition engines with gasoline direct injection systems have ... combination of a spray-guided combustion process with laser-induced ignition allows th...

Bernhard Geringer; Dominikus Klawatsch; Josef Graf; Hans Peter Lenz…

2004-03-01T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


241

ISOTOPE FRACTIONATION Isotopes are atoms whose nuclei contain the same number of protons but a different number of neutrons. The  

E-Print Network (OSTI)

the most abundant isotope appears in the denominator: b R = b E / a E (stable boron isotopes = , [ ] [ ] [ ] [ ]OOCOOC2 OOCOOC2 O 16181616 16181818 CO 18 2 + + = . The isotopic composition, , of a sample, determined____________________________ ISOTOPE FRACTIONATION ____________________________ Isotopes are atoms

Zeebe, Richard E.

242

Laser Program annual report, 1985  

SciTech Connect

This volume presents the unclassified activities and accomplishments of the Inertial Confinement Fusion and Advanced Laser Development elements of the Laser Program at the Lawrence Livermore National Laboratory for the calendar year 1985. This report has been organized into major sections that correspond to our principal technical activities. Section 1 provides an overview. Section 2 comprises work in target theory, design, and code development. Target development and fabrication and the related topics in materials science are contained in Section 3. Section 4 presents work in experiments and diagnostics and includes developments in data acquisition and management capabilities. In Section 5 laser system (Nova) operation and maintenance are discussed. Activities related to supporting laser and optical technologies are described in Section 6. Basic laser research and development is reported in Section 7. Section 8 contains the results of studies in ICF applications where the work reported deals principally with the production of electric power with ICF. Finally, Section 9 is a comprehensive discussion of work to date on solid state lasers for average power applications. Individual sections, two through nine, have been cataloged separately.

Rufer, M.L.; Murphy, P.W. (eds.)

1986-11-01T23:59:59.000Z

243

NETL: Gasification Systems - Gas Separation  

NLE Websites -- All DOE Office Websites (Extended Search)

Separation Separation Ion-Transport Membrane Oxygen Separation Modules Ion-Transport Membrane Oxygen Separation Modules Gas separation unit operations represent major cost elements in gasification plants. The gas separation technology being supported in the DOE program promises significant reduction in cost of electricity, improved thermal efficiency, and superior environmental performance. Gasification-based energy conversion systems rely on two gas separation processes: (1) separation of oxygen from air for feed to oxygen-blown gasifiers; and (2) post-gasification separation of hydrogen from carbon dioxide following (or along with) the shifting of gas composition when carbon dioxide capture is required or hydrogen is the desired product. Research efforts include development of advanced gas separation

244

Laser EYE SURGERY LASIK and Excimer Lasers  

E-Print Network (OSTI)

Laser EYE SURGERY LASIK and Excimer Lasers Michael Hutchins #12;The PROBLEM opia - near sightedness - Laser Assisted in SItu Keratomileusis atomileusis is the procedure of opening the eye and ring the cornea. SIK uses an excimer laser to perform the alterations an er a knife or a femtosecond laser

Fygenson, Deborah Kuchnir

245

Penning trap mass measurements on nobelium isotopes  

SciTech Connect

The Penning trap mass spectrometer SHIPTRAP at GSI Darmstadt allows accurate mass measurements of radionuclides, produced in fusion-evaporation reactions and separated by the velocity filter SHIP from the primary beam. Recently, the masses of the three nobelium isotopes {sup 252-254}No were determined. These are the first direct mass measurements of transuranium elements, which provide new anchor points in this region. The heavy nuclides were produced in cold-fusion reactions by irradiating a PbS target with a {sup 48}Ca beam, resulting in production rates of the nuclei of interest of about one atom per second. In combination with data from decay spectroscopy our results are used to perform a new atomic-mass evaluation in this region.

Dworschak, M.; Block, M.; Ackermann, D.; Herfurth, F.; Hessberger, F. P.; Hofmann, S.; Vorobyev, G. K. [GSI Helmholtzzentrum fuer Schwerionenforschung, D-64291 Darmstadt (Germany); Audi, G. [CSNSM-IN2P3-CNRS, F-91405 Orsay-Campus (France); Blaum, K. [Max-Planck-Institut fuer Kernphysik, D-69117 Heidelberg (Germany); Ruprecht-Karls-Universitaet, D-69120 Heidelberg (Germany); Droese, C.; Marx, G.; Schweikhard, L. [Ernst-Moritz-Arndt-Universitaet, Institut fuer Physik, D-17487 Greifswald (Germany); Eliseev, S.; Ketter, J. [Max-Planck-Institut fuer Kernphysik, D-69117 Heidelberg (Germany); Fleckenstein, T. [Justus-Liebig-Universitaet Giessen, D-35390 Giessen (Germany); Haettner, E.; Plass, W. R.; Scheidenberger, C. [GSI Helmholtzzentrum fuer Schwerionenforschung, D-64291 Darmstadt (Germany); Justus-Liebig-Universitaet Giessen, D-35390 Giessen (Germany); Ketelaer, J. [Johannes Gutenberg-Universitaet, Institut fuer Physik, D-55099 Mainz (Germany); Kluge, H.-J. [GSI Helmholtzzentrum fuer Schwerionenforschung, D-64291 Darmstadt (Germany); Ruprecht-Karls-Universitaet, D-69120 Heidelberg (Germany)

2010-06-15T23:59:59.000Z

246

Coherence delay augmented laser beam homogenizer  

DOE Patents (OSTI)

The geometrical restrictions on a laser beam homogenizer are relaxed by ug a coherence delay line to separate a coherent input beam into several components each having a path length difference equal to a multiple of the coherence length with respect to the other components. The components recombine incoherently at the output of the homogenizer, and the resultant beam has a more uniform spatial intensity suitable for microlithography and laser pantogography. Also disclosed is a variable aperture homogenizer, and a liquid filled homogenizer.

Rasmussen, P.; Bernhardt, A.

1993-06-29T23:59:59.000Z

247

Coherence delay augmented laser beam homogenizer  

DOE Patents (OSTI)

The geometrical restrictions on a laser beam homogenizer are relaxed by ug a coherence delay line to separate a coherent input beam into several components each having a path length difference equal to a multiple of the coherence length with respect to the other components. The components recombine incoherently at the output of the homogenizer, and the resultant beam has a more uniform spatial intensity suitable for microlithography and laser pantogography. Also disclosed is a variable aperture homogenizer, and a liquid filled homogenizer.

Rasmussen, Paul (Livermore, CA); Bernhardt, Anthony (Berkeley, CA)

1993-01-01T23:59:59.000Z

248

Laser Safety Introduction  

E-Print Network (OSTI)

Laser Safety #12;Introduction · A Laser is a device that controls the way energized atoms release photons. · LASER is an acronym for "Light Amplification by Stimulated Emission of Radiation" · The light emitted by a laser is non

McQuade, D. Tyler

249

Along the Laser Beampath  

NLE Websites -- All DOE Office Websites (Extended Search)

8 20 | Next | Last Back to Index NIF Laser Bay Each NIF laser bay is 122 meters (400 feet) long and contains 96 beamlines. This side view of Laser Bay 2 shows the four-high laser...

250

Isotopic Analysis- Rock | Open Energy Information  

Open Energy Info (EERE)

Isotopic Analysis- Rock Isotopic Analysis- Rock Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Technique: Isotopic Analysis- Rock Details Activities (13) Areas (11) Regions (0) NEPA(0) Exploration Technique Information Exploration Group: Lab Analysis Techniques Exploration Sub Group: Rock Lab Analysis Parent Exploration Technique: Rock Lab Analysis Information Provided by Technique Lithology: Water rock interaction Stratigraphic/Structural: Hydrological: Thermal: Dictionary.png Isotopic Analysis- Rock: Isotopes are atoms of the same element that have different numbers of neutrons. An isotopic analysis looks at a particular isotopic element(s) in a given system, while the conditions which increase/decrease the number of neutrons are well understood and measurable.

251

Enhanced membrane gas separations  

SciTech Connect

An improved membrane gas separation process is described comprising: (a) passing a feed gas stream to the non-permeate side of a membrane system adapted for the passage of purge gas on the permeate side thereof, and for the passage of the feed gas stream in a counter current flow pattern relative to the flow of purge gas on the permeate side thereof, said membrane system being capable of selectively permeating a fast permeating component from said feed gas, at a feed gas pressure at or above atmospheric pressure; (b) passing purge gas to the permeate side of the membrane system in counter current flow to the flow of said feed gas stream in order to facilitate carrying away of said fast permeating component from the surface of the membrane and maintaining the driving force for removal of the fast permeating component through the membrane from the feed gas stream, said permeate side of the membrane being maintained at a subatmospheric pressure within the range of from about 0.1 to about 5 psia by vacuum pump means; (c) recovering a product gas stream from the non-permeate side of the membrane; and (d) discharging purge gas and the fast permeating component that has permeated the membrane from the permeate side of the membrane, whereby the vacuum conditions maintained on the permeate side of the membrane by said vacuum pump means enhance the efficiency of the gas separation operation, thereby reducing the overall energy requirements thereof.

Prasad, R.

1993-07-13T23:59:59.000Z

252

Explosively separable casing  

DOE Patents (OSTI)

An explosively separable casing including a cylindrical afterbody and a circular cover for one end of the afterbody is disclosed. The afterbody has a cylindrical tongue extending longitudinally from one end which is matingly received in a corresponding groove in the cover. The groove is sized to provide a pocket between the end of the tongue and the remainder of the groove so that an explosive can be located therein. A seal is also provided between the tongue and the groove for sealing the pocket from the atmosphere. A frangible holding device is utilized to hold the cover to the afterbody. When the explosive is ignited, the increase in pressure in the pocket causes the cover to be accelerated away from the afterbody. Preferably, the inner wall of the afterbody is in the same plane as the inner wall of the tongue to provide a maximum space for storage in the afterbody and the side wall of the cover is thicker than the side wall of the afterbody so as to provide a sufficiently strong surrounding portion for the pocket in which the explosion takes place. The detonator for the explosive is also located on the cover and is carried away with the cover during separation. The seal is preferably located at the longitudinal end of the tongue and has a chevron cross section.

Jacobson, Albin K. (Albuquerque, NM); Rychnovsky, Raymond E. (Livermore, CA); Visbeck, Cornelius N. (Livermore, CA)

1985-01-01T23:59:59.000Z

253

Time scales of large volume silicic magma systems: Sr isotopic systematics of phenocrysts and glass from the Bishop Tuff, Long Valley, California  

Science Journals Connector (OSTI)

The initial Sr isotopic compositions of glass and mineral separates from the 0.74 Ma Bishop Tuff ashflow in eastern California were determined to investigate the time scales of magmatic processes in a large si...

John N. Christensen; Donald J. DePaolo

1993-01-01T23:59:59.000Z

254

I. Nuclear Production Reaction and Chemical Isolation Procedure for 240Am II. New Superheavy Element Isotopes: 242Pu(48Ca,5n)285-114  

E-Print Network (OSTI)

for the separation of americium(III) and curium(III) fromFission cross sections of americium isotopes. Atomic Energy,fission cross sections for americium. Nucl. Sci. Eng. , 154(

Ellison, Paul Andrew

2011-01-01T23:59:59.000Z

255

Laser ablation in analytical chemistry - A review  

SciTech Connect

Laser ablation is becoming a dominant technology for direct solid sampling in analytical chemistry. Laser ablation refers to the process in which an intense burst of energy delivered by a short laser pulse is used to sample (remove a portion of) a material. The advantages of laser ablation chemical analysis include direct characterization of solids, no chemical procedures for dissolution, reduced risk of contamination or sample loss, analysis of very small samples not separable for solution analysis, and determination of spatial distributions of elemental composition. This review describes recent research to understand and utilize laser ablation for direct solid sampling, with emphasis on sample introduction to an inductively coupled plasma (ICP). Current research related to contemporary experimental systems, calibration and optimization, and fractionation is discussed, with a summary of applications in several areas.

Russo, Richard E.; Mao, Xianglei; Liu, Haichen; Gonzalez, Jhanis; Mao, Samuel S.

2001-10-10T23:59:59.000Z

256

Laser Cosmology  

E-Print Network (OSTI)

Recent years have seen tremendous progress in our understanding of the cosmos, which in turn points to even deeper questions to be further addressed. Concurrently the laser technology has undergone dramatic revolutions, providing exciting opportunity for science applications. History has shown that the symbiosis between direct observations and laboratory investigation is instrumental in the progress of astrophysics. We believe that this remains true in cosmology. Current frontier phenomena related to particle astrophysics and cosmology typically involve one or more of the following conditions: (1) extremely high energy events; (2) very high density, high temperature processes; (3) super strong field environments. Laboratory experiments using high intensity lasers can calibrate astrophysical observations, investigate underlying dynamics of astrophysical phenomena, and probe fundamental physics in extreme limits. In this article we give an overview of the exciting prospect of laser cosmology. In particular, we showcase its unique capability of investigating frontier cosmology issues such as cosmic accelerator and quantum gravity.

Pisin Chen

2014-02-24T23:59:59.000Z

257

Chromatographic Separations of Enantiomers and Underivatized Oligosaccharides  

SciTech Connect

My graduate research has focused on separation science and bioanalytical analysis, which emphasized in method development. It includes three major areas: enantiomeric separations using high performance liquid chromatography (HPLC), Super/subcritical fluid chromatography (SFC), and capillary electrophoresis (CE); drug-protein binding behavior studies using CE; and carbohydrate analysis using liquid chromatograph-electrospray ionization mass spectrometry (LC-ESI-MS). Enantiomeric separations continue to be extremely important in the pharmaceutical industry. An in-depth evaluation of the enantiomeric separation capabilities of macrocyclic glycopeptides CSPs with SFC mobile phases was investigated using a set of over 100 chiral compounds. It was found that the macrocyclic based CSPs were able to separate enantiomers of various compounds with different polarities and functionalities. Seventy percent of all separations were achieved in less than 4 min due to the high flow rate (4.0 ml/min) that can be used in SFC. Drug-protein binding is an important process in determining the activity and fate of a drug once it enters the body. Two drug/protein systems have been studied using frontal analysis CE method. More sensitive fluorescence detection was introduced in this assay, which overcame the problem of low sensitivity that is common when using UV detection for drug-protein studies. In addition, the first usage of an argon ion laser with 257 nm beam coupled with CCD camera as a frontal analysis detection method enabled the simultaneous observation of drug fluorescence as well as the protein fluorescence. LC-ESI-MS was used for the separation and characterization of underivatized oligosaccharide mixtures. With the limits of detection as low as 50 picograms, all individual components of oligosaccharide mixtures (up to 11 glucose-units long) were baseline resolved on a Cyclobond I 2000 column and detected using ESI-MS. This system is characterized by high chromatographic resolution, high column stability, and high sensitivity. In addition, this method showed potential usefulness for the sensitive and quick analysis of hydrolysis products of polysaccharides, and for trace level analysis of individual oligosaccharides or oligosaccharide isomers from biological systems.

Ying Liu

2004-12-19T23:59:59.000Z

258

Electrified Separation Processes in Industry  

E-Print Network (OSTI)

For any separation procedure in the chemical industry, a certain amount of reversible work in the form of free energy is required, as dictated by the second law of thermodynamics. Classical techniques for effecting liquid-phase separations...

Appleby, A. J.

1983-01-01T23:59:59.000Z

259

Actinide Separation Science and Technology  

Science Journals Connector (OSTI)

Both the science and technology of the actinides as we know them today owe much to separation science. Conversely, the field of metal ion separations, solvent extraction, and ion exchange in particular, would ...

Kenneth L. Nash; Charles Madic…

2011-01-01T23:59:59.000Z

260

Actinide Separation Science and Technology  

Science Journals Connector (OSTI)

Both the science and technology of the actinides as we know them today owe much to separation science. Conversely, the field of metal ion separations, solvent extraction, and ion exchange in particular, would ...

Kenneth L. Nash; Charles Madic…

2006-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


261

Separation Nanotechnology of Diethylenetriaminepentaacetic Acid...  

NLE Websites -- All DOE Office Websites (Extended Search)

Nanotechnology of Diethylenetriaminepentaacetic Acid Bonded Magnetic Nanoparticles for Spent Nuclear Fuel. Separation Nanotechnology of Diethylenetriaminepentaacetic Acid Bonded...

262

Isotope-specific detection of low density materials with mono-energetic (gamma)-rays  

SciTech Connect

The first demonstration of isotope-specific detection of a low-Z, low density object, shielded by a high-Z and high density material using mono-energetic gamma-rays is reported. Isotope-specific detection of LiH shielded by Pb and Al is accomplished using the nuclear resonance fluorescence line of {sup 7}Li at 0.478 MeV. Resonant photons are produced via laser-based Compton scattering. The detection techniques are general and the confidence level obtained is shown to be superior to that yielded by conventional x-ray/{gamma}-ray techniques in these situations.

Albert, F; Anderson, S G; Gibson, D J; Hagmann, C A; Johnson, M S; Messerly, M J; Semenov, V A; Shverdin, M Y; Tremaine, A M; Hartemann, F V; Siders, C W; McNabb, D P; Barty, C J

2009-03-16T23:59:59.000Z

263

Automated data extraction from in situ protein stable isotope...  

NLE Websites -- All DOE Office Websites (Extended Search)

data extraction from in situ protein stable isotope probing studies. Automated data extraction from in situ protein stable isotope probing studies. Abstract: Protein stable isotope...

264

Copper isotope fractionation in acid mine drainage. | EMSL  

NLE Websites -- All DOE Office Websites (Extended Search)

Copper isotope fractionation in acid mine drainage. Copper isotope fractionation in acid mine drainage. Abstract: We surveyed the Cu isotopic composition of primary minerals and...

265

Isotope production facility produces cancer-fighting actinium  

NLE Websites -- All DOE Office Websites (Extended Search)

Cancer therapy gets a boost from new isotope Isotope production facility produces cancer-fighting actinium A new medical isotope project shows promise for rapidly producing major...

266

Leading chiral three-nucleon forces along isotope chains in the calcium region  

E-Print Network (OSTI)

Three-nucleon forces (3NFs), and in particular terms of the Fujita-Miyazawa type, strongly influence the structure of neutron-rich exotic isotopes. Ab-initio calculations have shown that chiral two- and three-nucleon interactions correctly reproduce binding energy systematics and neutron driplines of oxygen and nearby isotopes. Exploiting the novel self-consistent Gorkov-Green's function approach, we present the first investigation of Ar, K, Ca, Sc and Ti isotopic chains. Leading chiral 3N interactions are mandatory to reproduce the trend of binding energies throughout these chains and to obtain a good description of two-neutron separation energies. At the same time, nuclei in this mass region are systematically overbound by about 40 MeV and the $N=20$ magic gap is significantly overestimated. We conclude that ab-initio many-body calculations of mid-mass isotopic chains challenge modern theories of elementary nuclear interactions.

V. Somà; A. Cipollone; C. Barbieri; P. Navrátil; T. Duguet

2013-12-07T23:59:59.000Z

267

Definition: Isotopic Analysis- Fluid | Open Energy Information  

Open Energy Info (EERE)

Definition Definition Edit with form History Facebook icon Twitter icon » Definition: Isotopic Analysis- Fluid Jump to: navigation, search Dictionary.png Isotopic Analysis- Fluid Isotopes are atoms of the same element that have different numbers of neutrons. An isotopic analysis looks at a particular isotopic element(s) in a given system, while the conditions which increase/decrease the number of neutrons are well understood and measurable. Fluid isotopes are used to characterize a fluids origin, age, and/or interaction with rocks or other fluids based on unique isotopic ratios or concentrations.[1] View on Wikipedia Wikipedia Definition Isotope geochemistry is an aspect of geology based upon study of the relative and absolute concentrations of the elements and their isotopes in

268

Modeling of temporal behavior of isotopic exchange between gaseous hydrogen and palladium hydride power  

SciTech Connect

A parametric rate-equation model is described which depicts the time dependent behavior of the isotopic exchange process occurring between the solid and gas phases in gaseous hydrogen (deuterium) flows through packed-powder palladium deuteride (hydride) beds. The exchange mechanism is assumed to be rate-limited by processes taking place on the surface of the powder. The fundamental kinetic parameter of the model is the isotopic exchange probability, p, which is the probability that an isotopic exchange event occurs during a collision of a gas phase atom with the surface. Isotope effects between the gas and solid phases are explicitly included in terms of the isotope separation factor, ..cap alpha... Results of the model are compared with recent experimental measurements of isotope exchange in the ..beta..-phase hydrogen/palladium system and, using a literature value of ..cap alpha.. = 2.4, a good description of the experimental data is obtained for p approx. 10/sup -7/. In view of the importance of the isotope effects in the hydrogen/palladium system and the range of ..cap alpha.. values reported for the ..beta..-phase in the literature, the sensitivity of the model results to a variation in the value of ..cap alpha.. is examined.

Melius, C F; Foltz, G W

1987-01-01T23:59:59.000Z

269

Proton Radioactivity Measurements at HRIBF: Ho, Lu, and Tm Isotopes  

SciTech Connect

Two new isotopes, {sup 145}Tm and {sup 140}Ho and three isomers in previously known isotopes, {sup 141m}Ho, {sup 150m}Lu and {sup 151m}Lu have been discovered and studied via their decay by proton emission. These proton emitters were produced at the Holifield Radioactive Ion Beam Facility (HRIBF) by heavy-ion fusion-evaporation reactions, separated in A/Q with a recoil mass spectrometer (RMS), and detected in a double-sided silicon strip detector (DSSD). The decay energy and half-life was measured for each new emitter. An analysis in terms of a spherical shell model is applied to the Tm and Lu nuclei, but Ho is considerably deformed and requires a collective model interpretation.

Akovali, Y.; Batchelder, J.C.; Bingham, C.R.; Davinson, T.; Ginter, T.N.; Gross, C.J.; Grzywacz, R.; Hamilton, J.H.; Janas, Z.; Karny, M.; Kim, S.H.; MacDonald, B.D.; Mas, J.F.; McConnell, J.W.; Piechaczek, A.; Ressler, J.J.; Rykaczewski, K.; Slinger, R.C.; Szerypo, J.; Toth, K.S.; Weintraub, W.; Woods, P.J.; Yu, C.-H.; Zganjar, E.F.

1998-11-13T23:59:59.000Z

270

Project EARTH-14-SHELLDP1: Developing Metal Isotope Tracers for Understanding Sediment Depositional Environments  

E-Print Network (OSTI)

Project EARTH-14-SHELLDP1: Developing Metal Isotope Tracers for Understanding Sediment Depositional and the mechanisms behind temporal and spatial variations in organic matter quantity and quality. The project work will involve becoming proficient in clean room procedures, chemical separation techniques

Henderson, Gideon

271

Gas separation process  

SciTech Connect

The method for production of high purity hydrogen and high purity carbon monoxide from a mixed gas stream comprising these components together with carbon dioxide and a zero to a minor amount of one or more other gaseous contaminants is described comprising the steps of: (a) passing the mixed gas stream into and through a first bed of solid adsorbent capable of selectively adsorbing carbon dioxide and water while discharging from the bed a dry CO/sub 2/-freed effluent; (b) introducing the dry CO/sub 2/-freed effluent into a cryogenic environment for cooling the same therein under conditions effective for condensation of at least the major part of the carbon monoxide present in the dry CO/sub 2/-freed effluent; (c) withdrawing from the cryogenic environment carbon monoxide of high purity; (d) separately withdrawing from the cryogenic environment an uncondensed first gas stream product comprised of crude hydrogen and subjecting the first gas stream product to selective adsorption of non-hydrogen components therefrom in a second bed of solid absorbent, while recovering from the second bed the non-sorbed fraction as a product stream of essentially pure hydrogen; (e) purging the second solid adsorbent bed to desorb non-hydrogen components sorbed therein in step (d), and withdrawing from the bed a gas stream comprising the desorbed non-hydrogen components.

Nicholas, D.M.; Hopkins, J.A.; Roden, T.M.; Bushinsky, J.P.

1988-03-22T23:59:59.000Z

272

Membrane gas separation. (Latest citations from the NTIS data base). Published Search  

SciTech Connect

The bibliography contains citations concerning the research and development of gas separation and purification techniques involving the use of plastic and metal membranes. Among the topics included are isotope separation, osmotic techniques, reverse osmosis, and preparation of membranes for specific separation processes. The permeability of polymer membranes is discussed in terms of physical properties as well as molecular structure. The selectivity of polymeric films for a variety of gases is also included. (Contains a minimum of 168 citations and includes a subject term index and title list.)

Not Available

1992-08-01T23:59:59.000Z

273

Membrane gas separation. (Latest citations from the NTIS bibliographic database). Published Search  

SciTech Connect

The bibliography contains citations concerning the research and development of gas separation and purification techniques involving the use of plastic and metal membranes. Citations review isotope separation, osmotic techniques, reverse osmosis, and preparation of membranes for specific separation processes. The permeability of polymer membranes is discussed in terms of physical properties as well as molecular structure. The selectivity of polymeric films for a variety of gases is also included. (Contains a minimum of 205 citations and includes a subject term index and title list.)

Not Available

1994-01-01T23:59:59.000Z

274

Membrane gas separation. (Latest citations from the NTIS bibliographic database). Published Search  

SciTech Connect

The bibliography contains citations concerning the research and development of gas separation and purification techniques involving the use of plastic and metal membranes. Citations review isotope separation, osmotic techniques, reverse osmosis, and preparation of membranes for specific separation processes. The permeability of polymer membranes is discussed in terms of physical properties as well as molecular structure. The selectivity of polymeric films for a variety of gases is also included. (Contains a minimum of 198 citations and includes a subject term index and title list.)

Not Available

1993-08-01T23:59:59.000Z

275

Separation process using microchannel technology  

DOE Patents (OSTI)

The disclosed invention relates to a process and apparatus for separating a first fluid from a fluid mixture comprising the first fluid. The process comprises: (A) flowing the fluid mixture into a microchannel separator in contact with a sorption medium, the fluid mixture being maintained in the microchannel separator until at least part of the first fluid is sorbed by the sorption medium, removing non-sorbed parts of the fluid mixture from the microchannel separator; and (B) desorbing first fluid from the sorption medium and removing desorbed first fluid from the microchannel separator. The process and apparatus are suitable for separating nitrogen or methane from a fluid mixture comprising nitrogen and methane. The process and apparatus may be used for rejecting nitrogen in the upgrading of sub-quality methane.

Tonkovich, Anna Lee (Dublin, OH); Perry, Steven T. (Galloway, OH); Arora, Ravi (Dublin, OH); Qiu, Dongming (Bothell, WA); Lamont, Michael Jay (Hilliard, OH); Burwell, Deanna (Cleveland Heights, OH); Dritz, Terence Andrew (Worthington, OH); McDaniel, Jeffrey S. (Columbus, OH); Rogers, Jr.; William A. (Marysville, OH); Silva, Laura J. (Dublin, OH); Weidert, Daniel J. (Lewis Center, OH); Simmons, Wayne W. (Dublin, OH); Chadwell, G. Bradley (Reynoldsburg, OH)

2009-03-24T23:59:59.000Z

276

Laser assisted nuclear decay spectroscopy: A new method for studying neutron-deficient francium  

E-Print Network (OSTI)

Radioactive decay studies of rare isotopes produced at radioactive ion beam facilities have often been hindered by the presence of isobaric and isomeric contamination. The Collinear Resonance Ionization Spectroscopy (CRIS) experiment at ISOLDE, CERN uses laser radiation to stepwise excite and ionize an atomic beam in a particular isomeric state. Deflection of this selectively ionized beam of exotic nuclei, from the remaining neutral contaminants, allows ultra-sensitive detection of rare isotopes and nuclear structure measurements in background-free conditions.\

Lynch, Kara Marie

2015-01-01T23:59:59.000Z

277

Identification of isotopically primitive interplanetary dust particles: A NanoSIMS isotopic imaging study  

E-Print Network (OSTI)

Identification of isotopically primitive interplanetary dust particles: A NanoSIMS isotopic imaging contain larger regions with more modest enrichments in 15 N, leading to average bulk N isotopic of those IDPs that have anomalous bulk N isotopic compositions. These particles typically also contain

278

Spinelolivine magnesium isotope thermometry in the mantle and implications for the Mg isotopic composition of Earth  

E-Print Network (OSTI)

Spinel­olivine magnesium isotope thermometry in the mantle and implications for the Mg isotopic: magnesium isotopes mantle geochemistry meteorites MC-ICPMS The magnesium isotopic composition of Earth., 2004; Poitrasson et al., 2005; Georg et al., 2007; Poitrasson, 2007; Weyer et al., 2007). Magnesium

Manning, Craig

279

Online Catalog of Isotope Products from DOE's National Isotope Development Center  

DOE Data Explorer (OSTI)

The National Isotope Development Center (NIDC) interfaces with the User Community and manages the coordination of isotope production across the facilities and business operations involved in the production, sale, and distribution of isotopes. A virtual center, the NIDC is funded by the Isotope Development and Production for Research and Applications (IDPRA) subprogram of the Office of Nuclear Physics in the U.S. Department of Energy Office of Science. The Isotope subprogram supports the production, and the development of production techniques of radioactive and stable isotopes that are in short supply for research and applications. Isotopes are high-priority commodities of strategic importance for the Nation and are essential for energy, medical, and national security applications and for basic research; a goal of the program is to make critical isotopes more readily available to meet domestic U.S. needs. This subprogram is steward of the Isotope Production Facility (IPF) at Los Alamos National Laboratory (LANL), the Brookhaven Linear Isotope Producer (BLIP) facility at BNL, and hot cell facilities for processing isotopes at ORNL, BNL and LANL. The subprogram also coordinates and supports isotope production at a suite of university, national laboratory, and commercial accelerator and reactor facilities throughout the Nation to promote a reliable supply of domestic isotopes. The National Isotope Development Center (NIDC) at ORNL coordinates isotope production across the many facilities and manages the business operations of the sale and distribution of isotopes.

280

Membrane Separations of Liquid Mixtures  

E-Print Network (OSTI)

MEMBRANE SEPARATIONS OF LIQUID MIXTURES Douglas R. Lloyd Separations Research Program Department of Chemical Engineering The University of Texas at Austin Austin, Texas In recent years considerable attention has been given to the need... for reduced energy costs in the chemical processing industry. A major portion of the energy consumed in this industry is associated with the separation and recovery of chemicals. Membrane processes offer energy-efficient, cost effective methods...

Lloyd, D. R.

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


281

The graphene phonon dispersion with C{sup 12} and C{sup 13} isotopes  

SciTech Connect

Using very uniform large scale chemical vapor deposition grown graphene transferred onto silicon, we were able to identify 15 distinct Raman lines associated with graphene monolayers. This was possible thanks to a combination of different carbon isotopes and different Raman laser energies and extensive averaging without increasing the laser power. This allowed us to obtain a detailed experimental phonon dispersion relation for many points in the Brillouin zone. We further identified a D+D' peak corresponding to a double phonon process involving both an inter- and intra-valley phonon. In order to both eliminate substrate effects and to probe large areas, we undertook to study Raman scattering for large scale chemical vapor deposition (CVD) grown graphene using two different isotopes (C12 and C13) so that we can effectively exclude and subtract the substrate contributions, since a heavier mass downshifts only the vibrational properties, while keeping all other properties the same.

Whiteway, Eric; Bernard, Simon; Yu, Victor; Hilke, Michael [Department of Physics, McGill University, Montréal H3A 2T8 (Canada); Austing, D. Guy [National Research Council of Canada, Ottawa, Ontario K1A 0R6 (Canada)

2013-12-04T23:59:59.000Z

282

Calibration of laser ablation inductively coupled plasma mass spectrometry using dried solution aerosols for the quantitative analysis of solid samples  

SciTech Connect

Inductively coupled plasma mass spectrometry (ICP-MS) has become the method of choice for elemental and isotopic analysis. Several factors contribute to its success. Modern instruments are capable of routine analysis at part per trillion levels with relative detection limits in part per quadrillion levels. Sensitivities in these instruments can be as high as 200 million counts per second per part per million with linear dynamic ranges up to eight orders of magnitude. With standards for only a few elements, rapid semiquantitative analysis of over 70 elements in an individual sample can be performed. Less than 20 years after its inception ICP-MS has shown to be applicable to several areas of science. These include geochemistry, the nuclear industry, environmental chemistry, clinical chemistry, the semiconductor industry, and forensic chemistry. In this introduction, the general attributes of ICP-MS will be discussed in terms of instrumentation and sample introduction. The advantages and disadvantages of current systems are presented. A detailed description of one method of sample introduction, laser ablation, is given. The paper also gives conclusions and suggestions for future work. Chapter 2, Quantitative analysis of solids by laser ablation inductively coupled plasma mass spectrometry using dried solution aerosols for calibration, has been removed for separate processing.

Leach, J.

1999-02-12T23:59:59.000Z

283

Respiration, photosynthesis, and oxygen isotope fractionation in ...  

Science Journals Connector (OSTI)

Jan 25, 1971 ... Respiration, photosynthesis, and oxygen isotope fractionation in oceanic surface water1. Peter M. Kroopnick. Department of Oceanography,.

2000-01-04T23:59:59.000Z

284

Magnesium Isotope Effects in Enzymatic Phosphorylation  

Science Journals Connector (OSTI)

So far as magnesium isotope effect in phosphorylation is an unexpected and unusual phenomenon, it is worthy to shortly describe materials and technologies used in isotopic biochemical experiments. ... Isotope-containing MgCl2 samples were obtained using treatment of magnesium oxides 24MgO, 25MgO, 26MgO, and *MgO with analytically pure HCl (*Mg means magnesium with natural abundance of the three isotopes; see Table 1). ...

Anatoly L. Buchachenko; Dmitry A. Kouznetsov; Natalia N. Breslavskaya; Marina A. Orlova

2008-02-05T23:59:59.000Z

285

Atomic-scale characterization of germanium isotopic multilayers by atom probe tomography  

SciTech Connect

We report comparison of the interfacial sharpness characterization of germanium (Ge) isotopic multilayers between laser-assisted atom probe tomography (APT) and secondary ion mass spectrometry (SIMS). An alternating stack of 8-nm-thick naturally available Ge layers and 8-nm-thick isotopically enriched {sup 70}Ge layers was prepared on a Ge(100) substrate by molecular beam epitaxy. The APT mass spectra consist of clearly resolved peaks of five stable Ge isotopes ({sup 70}Ge, {sup 72}Ge, {sup 73}Ge, {sup 74}Ge, and {sup 76}Ge). The degree of intermixing at the interfaces between adjacent layers was determined by APT to be around 0.8 {+-} 0.1 nm which was much sharper than that obtained by SIMS.

Shimizu, Y.; Takamizawa, H.; Toyama, T.; Inoue, K.; Nagai, Y. [Oarai Center, Institute for Materials Research, Tohoku University, 2145-2 Narita, Oarai, Ibaraki 311-1313 (Japan); Kawamura, Y.; Uematsu, M.; Itoh, K. M. [School of Fundamental Science and Technology, Keio University, 3-14-1 Hiyoshi, Kohoku-ku, Yokohama 223-8522 (Japan); Haller, E. E. [University of California at Berkeley and Lawrence Berkeley National Laboratory, 1 Cyclotron Road, Berkeley, California 94720 (United States)

2013-01-14T23:59:59.000Z

286

Separation of Transmutation - and Fission-Produced Radioisotopes from Irradiated Beryllium  

SciTech Connect

The primary objective of this study was to test the effectiveness of a two-step solvent extraction-precipitation process for separating transmutation and fission products from irradiated beryllium. Beryllium metal was dissolved in nitric and fluoroboric acids. Isotopes of 241Am, 239Pu, 85Sr, 60Co, and 137Cs were then added to make a surrogate beryllium waste solution. A series of batch contacts was performed with the spiked simulant using chlorinated cobalt dicarbollide and polyethylene glycol diluted with sulfone to extract the isotopes of Cs and Sr. Another series of batch contacts was performed using a combination of octyl (phenyl)-N,Ndiisobutylcarbamoylmethylphosphine oxide in tributyl phosphate diluted with dodecane for extracting the isotopes of Pu and Am. The 60Co was separated by first forming a cobalt complex and then selectively precipitating the beryllium as a hydroxide. The results indicate that greater than 99.9% removal can be achieved for each radionuclide. Transuranic isotope contamination levels are reduced to less than 100 nCi/g, and sources of high beta-gamma radiation (60Co, 137Cs, and 90Sr) are reduced to levels that will allow the beryllium to be contact handled. The separation process may be applicable to a recycle or waste disposition scenario.

Troy J. Tranter; RIchard D. Tillotson; Nick R. Mann; Glen R. Longhurst

2011-11-01T23:59:59.000Z

287

Photo-oxidation of Water by Molecular Oxygen: Isotope Exchange and Isotope Effects  

Science Journals Connector (OSTI)

In order to detect the reaction, we used water highly enriched with isotopes 17O and 18O, controlling the isotope composition of molecular oxygen before and after reaction. ... stability of heavy-isotope clumps'; slower kinetics of reactions requiring the breakage of bonds between heavy isotopes; the mass dependence of diffusive and thermo-gravitational fractionations; mixing between components that differ from one another in bulk isotopic compn.; biochem. ... Study of oxygen three-isotope behavior during thermal decompn. of naturally occurring carbonates of calcium and magnesium in vacuo revealed that, surprisingly, anomalous isotopic compns. ...

Anatoly L. Buchachenko; Elena O. Dubinina

2011-03-30T23:59:59.000Z

288

Fusion reactions initiated by laser-accelerated particle beams in a laser-produced plasma  

E-Print Network (OSTI)

The advent of high-intensity pulsed laser technology enables the generation of extreme states of matter under conditions that are far from thermal equilibrium. This in turn could enable different approaches to generating energy from nuclear fusion. Relaxing the equilibrium requirement could widen the range of isotopes used in fusion fuels permitting cleaner and less hazardous reactions that do not produce high energy neutrons. Here we propose and implement a means to drive fusion reactions between protons and boron-11 nuclei, by colliding a laser-accelerated proton beam with a laser-generated boron plasma. We report proton-boron reaction rates that are orders of magnitude higher than those reported previously. Beyond fusion, our approach demonstrates a new means for exploring low-energy nuclear reactions such as those that occur in astrophysical plasmas and related environments.

Labaune, C; Depierreux, S; Goyon, C; Loisel, G; Yahia, V; Rafelski, J

2013-01-01T23:59:59.000Z

289

Jupiter Laser Facility  

NLE Websites -- All DOE Office Websites (Extended Search)

Jupiter Laser Facility The commissioning of the Titan Petawatt-Class laser to LLNL's Jupiter Laser Facility (JLF) has provided a unique platform for the use of petawatt (PW)-class...

290

Hypersonic gasdynamic laser system  

SciTech Connect

This patent describes a visible, or near to mid infra-red, hypersonic gas dynamic laser system. It comprises: a hypersonic vehicle for carrying the hypersonic gas dynamic laser system, and also providing high energy ram air for thermodynamic excitation and supply of the laser gas; a laser cavity defined within the hypersonic vehicle and having a laser cavity inlet for the laser cavity formed by an opening in the hypersonic vehicle, such that ram air directed through the laser cavity opening supports gas dynamic lasing operations at wavelengths less than 10.6{mu} meters in the laser cavity; and an optical train for collecting the laser radiation from the laser cavity and directing it as a substantially collimated laser beam to an output aperture defined by an opening in the hypersonic vehicle to allow the laser beam to be directed against a target.

Foreman, K.M.; Maciulaitis, A.

1990-05-22T23:59:59.000Z

291

Terahertz quantum cascade lasers  

Science Journals Connector (OSTI)

...Michael Pepper Terahertz quantum cascade lasers Jerome Faist 1 Lassaad Ajili...developments in terahertz quantum cascade lasers are reviewed. Structures...magnetic confinement| Terahertz quantum cascade lasers. | Recent developments in...

2004-01-01T23:59:59.000Z

292

Three phase downhole separator process  

DOE Patents (OSTI)

Three Phase Downhole Separator Process (TPDSP) is a process which results in the separation of all three phases, (1) oil, (2) gas, and (3) water, at the downhole location in the well bore, water disposal injection downhole, and oil and gas production uphole.

Cognata, Louis John (Baytown, TX)

2008-06-24T23:59:59.000Z

293

Laser Desorption Analysis | EMSL  

NLE Websites -- All DOE Office Websites (Extended Search)

Laser Desorption Analysis Laser Desorption Analysis EMSL offers a suite of instrumentation dedicated to understanding photoreactivity in the condensed phase, on surfaces, and at...

294

Laser Desorption Analysis | EMSL  

NLE Websites -- All DOE Office Websites (Extended Search)

neutral particle detection using a second multiphoton ionization or REMPI laser system; and UHV surface diagnostic equipment (AES, LEED, XPS). User Portal Name: Laser...

295

Laser Safety Management Policy Statement ............................................................................................................1  

E-Print Network (OSTI)

Laser Safety Management Policy Statement...........................................................2 Laser Users.............................................................................................................2 Unit Laser Safety Officer (ULSO

Davidson, Fordyce A.

296

Isotope Evidence for Ozone Formation on Surfaces  

Science Journals Connector (OSTI)

Remarkably, the gas-phase recombination or association reaction of ozone has an unusually large (?10%) isotope effect and shows almost equal enrichments of the ozone molecules containing two different oxygen isotopes. ... For a better understanding of the pressure and temperature dependence of ozone isotopic composition in oxygen discharges, we developed a relatively simple isotope kinetic model that accounts for the processes of (i) heterogeneous ozone formation at the reactor walls, (ii) isotope exchange of oxygen atoms with O2 molecules, and (iii) ozone formation in the gas phase. ...

Christof Janssen; Béla Tuzson

2010-05-06T23:59:59.000Z

297

Magnesium-Isotope Fractionation During Plant Growth  

Science Journals Connector (OSTI)

With three stable isotopes naturally abundant (24Mg, 78.992%; 25Mg, 10.003%; 26Mg, 11.005%), magnesium stable isotope fractionation may provide insights into these cycles. ... Measurements of the magnesium isotopic composition of chlorophylls, seeds, shoots, roots, leaves, exudates, and the limiting nutrient solution over time show that the plant appears to establish an isotopic equilibrium with the nutrient available to it and that the plant (in particular, the seeds and exudates) becomes enriched in the heavy isotopes of magnesium in a mass-dependent relationship as the plant reaches maturity. ...

Jay R. Black; Emanuel Epstein; William D. Rains; Qing-zhu Yin; William H. Casey

2008-10-01T23:59:59.000Z

298

Slow Neutron Scattering by the Titanium Isotopes  

Science Journals Connector (OSTI)

Neutron diffraction studies are reported on isotopically enriched samples of TiO2 from which are evaluated the coherent scattering amplitudes of the titanium isotopes. Scattering amplitudes of +0.48, +0.33, -0.58, +0.08, and +0.55×10-12 cm were established for the titanium isotopes of mass 46, 47, 48, 49, and 50, respectively. The major isotope Ti48 is thus responsible for the anomalous scattering amplitude, -0.34×10-12 cm, characteristic of the normal element. Pronounced nuclear scattering resonance effects on the observed neutron scattering are suggested to occur for most of the isotopes.

C. G. Shull; M. K. Wilkinson; M. H. Mueller

1960-05-01T23:59:59.000Z

299

Isotope Effects in Isotope-Exchange Reactions:? Evidence for a Large 12C/13C Kinetic Isotope Effect in the Gas Phase  

Science Journals Connector (OSTI)

Isotope effects are key to understanding reaction mechanisms because isotopic substitution affects reaction rates and equilibrium constants. ... These values are considered in relation to the vapor pressures of isotopic compds., the geologic abundance of C and O isotopes, the relative abundance of O isotopes in air and H2O, and variations in the at. ...

Giulia de Petris; Anna Troiani

2008-03-05T23:59:59.000Z

300

Laser Stabilization  

SciTech Connect

This book chapter covers the basics of the field of stabilizing lasers to optical frequency references such as optical cavities and molecular transitions via the application of servo control systems. These discussions are given with reference to the real-life frequency metrology experienced in Hall-Labs (now Ye-Labs), JILA, University of Colorado. The subjects covered include: the basics of control system stability, a discussion of both the theoretical and experimental limitations, an outline of optical cavity susceptibility to environmental noise, and a brief introduction to the use and limitations of molecular transitions as frequency references.

Hall, John L.; Taubman, Matthew S.; Ye, Jun

2010-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


301

Omega Laser Facility - Laboratory for Laser Energetics  

NLE Websites -- All DOE Office Websites (Extended Search)

- Laboratory for Laser Energetics Laboratory for Laser Energetics Logo Search Home Around the Lab Past Issues Past Quick Shots About Office of the Director Map to LLE LLE Tours LLE...

302

OMEGA Laser - Laboratory for Laser Energetics  

NLE Websites -- All DOE Office Websites (Extended Search)

- Laboratory for Laser Energetics Laboratory for Laser Energetics Logo Search Home Around the Lab Past Issues Past Quick Shots About Office of the Director Map to LLE LLE Tours LLE...

303

OMEGA Laser Drivers - Laboratory for Laser Energetics  

NLE Websites -- All DOE Office Websites (Extended Search)

Drivers - Laboratory for Laser Energetics Laboratory for Laser Energetics Logo Search Home Around the Lab Past Issues Past Quick Shots About Office of the Director Map to LLE LLE...

304

High-accuracy mass measurements of neutron-rich Kr isotopes  

Science Journals Connector (OSTI)

The atomic masses of the neutron-rich krypton isotopes Kr84,86-95 have been determined with the tandem Penning trap mass spectrometer ISOLTRAP with uncertainties ranging from 20 to 220 ppb. The masses of the short-lived isotopes Kr94 and Kr95 were measured for the first time. The masses of the radioactive nuclides Kr89 and Kr91 disagree by 4 and 6 standard deviations, respectively, from the present Atomic-Mass Evaluation database. The resulting modification of the mass surface with respect to the two-neutron separation energies as well as implications for mass models and stellar nucleosynthesis are discussed.

P. Delahaye; G. Audi; K. Blaum; F. Carrel; S. George; F. Herfurth; A. Herlert; A. Kellerbauer; H.-J. Kluge; D. Lunney; L. Schweikhard; C. Yazidjian

2006-09-28T23:59:59.000Z

305

The table of isotopes-8th edition and beyond  

SciTech Connect

A new edition of the Table of Isotopes has been published this year by John Wiley and Sons, Inc. This edition is the eighth in a series started by Glenn T. Seaborg in 1940. The two-volume, 3168-page, cloth-bound edition is twice the size of the previous edition published in 1978. It contains nuclear structure and decay data, based mainly on the Evaluated Nuclear Structure Data File (ENSDF), for >3100 isotopes and isomers. Approximately 24000 references are cited, and the appendices have been updated and extended. The book is packaged with an interactive CD-ROM that contains the Table of Isotopes in Adobe Acrobat Portable Document Format for convenient viewing on personal computer (PC) and UNIX workstations. The CD-ROM version contains a chart of the nuclides graphical index and separate indices organized for radioisotope users and nuclear structure physicists. More than 100000 hypertext links are provided to move the user quickly through related information free from the limitations of page size. Complete references with keyword abstracts are provided. The CD-ROM also contains the Table of Super-deformed Nuclear Bands and Fission Isomers; Tables of Atoms, Atomic Nuclei, and Subatomic Particles by Ivan P. Selinov; the ENSDF and nuclear structure reference (NSR) databases; the ENSDF manual by Jagdish K. Tuli; and Abode Acrobat Reader software.

Firestone, R.B. [Lawrence Berkeley Laboratory, CA (United States)

1996-12-31T23:59:59.000Z

306

Apparatus, system, and method for laser-induced breakdown spectroscopy  

DOE Patents (OSTI)

In laser-induced breakdown spectroscopy (LIBS), an apparatus includes a pulsed laser configured to generate a pulsed laser signal toward a sample, a constructive interference object and an optical element, each located in a path of light from the sample. The constructive interference object is configured to generate constructive interference patterns of the light. The optical element is configured to disperse the light. A LIBS system includes a first and a second optical element, and a data acquisition module. The data acquisition module is configured to determine an isotope measurement based, at least in part, on light received by an image sensor from the first and second optical elements. A method for performing LIBS includes generating a pulsed laser on a sample to generate light from a plasma, generating constructive interference patterns of the light, and dispersing the light into a plurality of wavelengths.

Effenberger, Jr., Andrew J; Scott, Jill R; McJunkin, Timothy R

2014-11-18T23:59:59.000Z

307

Definition: Isotopic Analysis- Rock | Open Energy Information  

Open Energy Info (EERE)

Isotopic Analysis- Rock Isotopic Analysis- Rock Jump to: navigation, search Dictionary.png Isotopic Analysis- Rock Isotopes are atoms of the same element that have different numbers of neutrons. An isotopic analysis looks at a particular isotopic element(s) in a given system, while the conditions which increase/decrease the number of neutrons are well understood and measurable.[1] View on Wikipedia Wikipedia Definition References ↑ http://wwwrcamnl.wr.usgs.gov/isoig/isopubs/itchch2.html Ret LikeLike UnlikeLike You like this.Sign Up to see what your friends like. rieved from "http://en.openei.org/w/index.php?title=Definition:Isotopic_Analysis-_Rock&oldid=687702" Category: Definitions What links here Related changes Special pages Printable version Permanent link Browse properties

308

Isotopes Tell Origin and Operation of the Sun  

E-Print Network (OSTI)

The Iron Sun formed on the collapsed core of a supernova and now acts as a magnetic plasma diffuser, as did the precursor star, separating ions by mass. This process covers the solar surface with lightweight elements and with lighter isotopes of each element. Running difference images expose rigid, iron-rich structures below the fluid photosphere made of lightweight elements. The energy source for the Sun and ordinary stars seems to be neutron-emission and neutron-decay, with partial fusion of the decay product, rather than simple fusion of hydrogen into helium or heavier elements. Neutron-emission from the solar core and neutron-decay generate about sixty five percent of solar luminosity and H-fusion generates about thirty-five percent. The upward flow of H ions maintains mass-separation in the Sun. Only about one percent of this neutron decay product survives its upward journey to depart as solar-wind hydrogen.

O. Manuel; Sumeet A. Kamat; Michael Mozina

2005-09-28T23:59:59.000Z

309

The laser satellites communications and laser noises  

Science Journals Connector (OSTI)

The gain of advanced optical communication systems is reduced by the noise of optical source. Coherent optical communication systems are in particular very sensitive to the noise transmitter and local laser. Optical space communications is on the verge ... Keywords: laser, laser communication, noise limits, optical communication, range loss, satellite communications, satellite systems, signal transfer loss, space channel

Marketa Mazalkova

2008-08-01T23:59:59.000Z

310

Robust Polymer Composite Membranes for Hydrogen Separation |...  

Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

Robust Polymer Composite Membranes for Hydrogen Separation Robust Polymer Composite Membranes for Hydrogen Separation polymercompositemembranes.pdf More Documents & Publications...

311

Efficient separations & processing crosscutting program  

SciTech Connect

The Efficient Separations and Processing Crosscutting Program (ESP) was created in 1991 to identify, develop, and perfect chemical and physical separations technologies and chemical processes which treat wastes and address environmental problems throughout the DOE complex. The ESP funds several multiyear tasks that address high-priority waste remediation problems involving high-level, low-level, transuranic, hazardous, and mixed (radioactive and hazardous) wastes. The ESP supports applied research and development (R & D) leading to the demonstration or use of these separations technologies by other organizations within the Department of Energy (DOE), Office of Environmental Management.

NONE

1996-08-01T23:59:59.000Z

312

Methane/nitrogen separation process  

DOE Patents (OSTI)

A membrane separation process is described for treating a gas stream containing methane and nitrogen, for example, natural gas. The separation process works by preferentially permeating methane and rejecting nitrogen. The authors have found that the process is able to meet natural gas pipeline specifications for nitrogen, with acceptably small methane loss, so long as the membrane can exhibit a methane/nitrogen selectivity of about 4, 5 or more. This selectivity can be achieved with some rubbery and super-glassy membranes at low temperatures. The process can also be used for separating ethylene from nitrogen. 11 figs.

Baker, R.W.; Lokhandwala, K.A.; Pinnau, I.; Segelke, S.

1997-09-23T23:59:59.000Z

313

Methane/nitrogen separation process  

DOE Patents (OSTI)

A membrane separation process for treating a gas stream containing methane and nitrogen, for example, natural gas. The separation process works by preferentially permeating methane and rejecting nitrogen. We have found that the process is able to meet natural gas pipeline specifications for nitrogen, with acceptably small methane loss, so long as the membrane can exhibit a methane/nitrogen selectivity of about 4, 5 or more. This selectivity can be achieved with some rubbery and super-glassy membranes at low temperatures. The process can also be used for separating ethylene from nitrogen.

Baker, Richard W. (Palo Alto, CA); Lokhandwala, Kaaeid A. (Menlo Park, CA); Pinnau, Ingo (Palo Alto, CA); Segelke, Scott (Mountain View, CA)

1997-01-01T23:59:59.000Z

314

Kinetic Isotope Effects in Cycloreversion of Rhenium (V) Diolates  

Science Journals Connector (OSTI)

The isotope effects were all calculated from these ratios according to the equation25 (F = extent of reaction; R = isotopic ratio vs reference at extent of reaction F; R0 = initial isotopic ratio vs reference). ... The magnitudes of small kinetic isotope effects (KIEs) are amplified in the isotopic compn. of starting materials recovered from reactions taken to high conversions. ... The magnitudes of small kinetic isotope effects (KIEs) are amplified in the isotopic compn. of starting materials recovered from reactions taken to high conversions. ...

Kevin P. Gable; Fedor A. Zhuravlev

2002-03-21T23:59:59.000Z

315

High efficiency resonance ionization mass spectrometric analysis by external laser cavity enhancement techniques  

SciTech Connect

The demand to measure high dynamic range isotope ratios on small samples with resonance ionization mass spectrometry (RIMS) continues to increase. This paper discusses high ionization efficiency methods which can be applied to continuous wave (cw) RIMS to potentially achieve several tens of percent ionization efficiencies for certain elements. The primary technique under development to achieve this is an external laser cavity which can generate very high circulating laser powers. 12 refs., 3 figs.

Johnson, S.G.; Rios, E.L.; Miller, C.M.; Fearey, B.L.

1991-01-01T23:59:59.000Z

316

ablation laser spectrometer  

E-Print Network (OSTI)

ablation laser mass spectrometer molecular beam REMPI laser NREL has designed and developed a combined laser ablation/ pulsed sample introduction/mass spectrometry platform that integrates pyrolysis and/or laser ablation with resonance- enhanced multiphoton ionization (REMPI) time-of-flight mass

317

Narrow gap laser welding  

DOE Patents (OSTI)

A laser welding process including: (a) using optical ray tracing to make a model of a laser beam and the geometry of a joint to be welded; (b) adjusting variables in the model to choose variables for use in making a laser weld; and (c) laser welding the joint to be welded using the chosen variables. 34 figs.

Milewski, J.O.; Sklar, E.

1998-06-02T23:59:59.000Z

318

Narrow gap laser welding  

DOE Patents (OSTI)

A laser welding process including: (a) using optical ray tracing to make a model of a laser beam and the geometry of a joint to be welded; (b) adjusting variables in the model to choose variables for use in making a laser weld; and (c) laser welding the joint to be welded using the chosen variables.

Milewski, John O. (Santa Fe, NM); Sklar, Edward (Santa Fe, NM)

1998-01-01T23:59:59.000Z

319

Pump and centrifugal separator apparatus  

SciTech Connect

The invention relates to agitating means for preventing the accumulation of particulate matter at the contaminate outlet orifices in a pump and centrifugal separator apparatus. The pump separator apparatus includes a rotatable casing forming a chamber for centrifugally separating the oil, water and contaminant matter in an oil well production fluid. The clean oil is collected by a stationary pitot tube in the chamber, the clean water is drawn off at an outlet port near the outer periphery of the chamber, and the dirty water and contaminants are discharged through outlet orifices formed in the outer wall of the casing. The agitating means includes rotating jet ports for directing streams of pressurized fluid tangentially along the inner surface of the casing to agitate accumulations of separated solid contaminant matter thereby preventing the clogging of the outlet orifices.

Erickson, J.W.

1981-08-11T23:59:59.000Z

320

Continuous magnetic separator and process  

DOE Patents (OSTI)

A continuous magnetic separator and process for separating a slurry comprising magnetic particles into a clarified stream and a thickened stream. The separator has a container with a slurry inlet, an overflow outlet for the discharge of the clarified slurry stream, and an underflow outlet for the discharge of a thickened slurry stream. Magnetic particles in the slurry are attracted to, and slide down, magnetic rods within the container. The slurry is thus separated into magnetic concentrate and clarified slurry. Flow control means can be used to control the ratio of the rate of magnetic concentrate to the rate of clarified slurry. Feed control means can be used to control the rate of slurry feed to the slurry inlet.

Oder, Robin R. (Export, PA); Jamison, Russell E. (Lower Burrell, PA)

2008-04-22T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


321

Fluorine separation and generation device  

DOE Patents (OSTI)

A process and apparatus for the electrolytic separation of fluorine from a mixture of gases is disclosed. Also described is the process and apparatus for the generation of fluorine from fluorine/fluoride containing solids, liquids or gases.

The Regents of the University of California (Oakland, CA)

2008-12-23T23:59:59.000Z

322

Fusion reactions with germanium isotopes  

Science Journals Connector (OSTI)

Measurements of the fusion of 16O and 27Al with a series of germanium isotopes are analyzed within a coupled-channels approach. It is found that couplings based interactions that are linear in the deformation amplitudes are insufficient in reproducing the data. In order to obtain reasonable fits, it is necessary also to include couplings based on quadratic interactions. The analysis suggests that the nuclear radius of 72Ge is significantly smaller than predicted from a smooth interpolation between other germanium isotopes. The large prolate deformation of 74Ge, which has been proposed as the preferred solution to measurements of the quadrupole moment of the 2+ state, is not supported by the analysis; the near spherical solution is more likely.

H. Esbensen

2003-09-04T23:59:59.000Z

323

Technology Alert List From the U.S. Department of State  

E-Print Network (OSTI)

, including gaseous diffusion, centrifuge, aerodynamic, chemical, Electromagnetic Isotopic Separation (EMIS), Laser Isotope Separation (LIS) · Spent fuel reprocessing, plutonium, mixed oxide nuclear research countermeasures and systems · New or novel explosives and formulations · Automated explosive detection methods

Guenther, Frank

324

Laser Glazing of Railroad Rails [Laser Applications Laboratory] - Nuclear  

NLE Websites -- All DOE Office Websites (Extended Search)

Laser Glazing of Railroad Laser Glazing of Railroad Rails Capabilities Engineering Experimentation Reactor Safety Experimentation Aerosol Experiments System Components Laser Applications Overview Laser Oil & Gas Well Drilling Laser Heat Treatment Laser Welding of Metals On-line Monitoring Laser Beam Delivery Laser Glazing of Railroad Rails High Power Laser Beam Delivery Decontamination and Decommissioning Refractory Alloy Welding Robots Applications Other Facilities Other Capabilities Work with Argonne Contact us For Employees Site Map Help Join us on Facebook Follow us on Twitter NE on Flickr Laser Applications Laboratory Laser Glazing of Railroad Rails Project description: Laser glazing of rails. Category: Project with industrial partner (American Association of Railroads) Bookmark and Share

325

Laser Welding of Metals [Laser Applications Laboratory] - Nuclear  

NLE Websites -- All DOE Office Websites (Extended Search)

Laser Welding of Metals Laser Welding of Metals Capabilities Engineering Experimentation Reactor Safety Experimentation Aerosol Experiments System Components Laser Applications Overview Laser Oil & Gas Well Drilling Laser Heat Treatment Laser Welding of Metals On-line Monitoring Laser Beam Delivery Laser Glazing of Railroad Rails High Power Laser Beam Delivery Decontamination and Decommissioning Refractory Alloy Welding Robots Applications Other Facilities Other Capabilities Work with Argonne Contact us For Employees Site Map Help Join us on Facebook Follow us on Twitter NE on Flickr Laser Applications Laboratory Laser Welding of Metals Project description: High-speed laser welding of metals. Category: Project with industrial partner (Delphi Energy and Engine Management Systems) Bookmark and Share

326

Separations in the STATS report  

SciTech Connect

The Separations Technology and Transmutation Systems (STATS) Committee formed a Subcommittee on Separations. This subcommittee was charged with evaluating the separations proposed for the several reactor and accelerator transmutation systems. It was also asked to review the processing options for the safe management of high-level waste generated by the defense programs, in particular, the special problems involved in dealing with the waste at the U.S. Department of Energy (DOE) facility in Hanford, Washington. Based on the evaluations from the Subcommittee on Separations, the STATS Committee concluded that for the reactor transmutation programs, aqueous separations involving a combination of PUREX and TRUEX solvent extraction processes could be used. However, additional research and development (R&D) would be required before full plant-scale use of the TRUEX technology could be employed. Alternate separations technology for the reactor transmutation program involves pyroprocessing. This process would require a significant amount of R&D before its full-scale application can be evaluated.

Choppin, G.R. [Florida State Univ., Tallahassee, FL (United States)

1996-12-31T23:59:59.000Z

327

Magnesium Isotopes in Halo Stars  

E-Print Network (OSTI)

We have determined Mg isotope ratios in halo field dwarfs and giants in the globular cluster M71 based on high S/N high spectral resolution (R = 10$^5$) Keck HIRES spectra. Unlike previous claims of an important contribution from intermediate-mass AGB stars to the Galactic halo, we find that our $^{26}$Mg/$^{24}$Mg ratios can be explained by massive stars.

Jorge Melendez; Judith G. Cohen

2007-08-29T23:59:59.000Z

328

Laser-induced nonresonant nuclear excitation in muonic atoms  

E-Print Network (OSTI)

Coherent nuclear excitation in strongly laser-driven muonic atoms is calculated. The nuclear transition is caused by the time-dependent Coulomb field of the oscillating charge density of the bound muon. A closed-form analytical expression for electric multipole transitions is derived and applied to various isotopes; the excitation probabilities are in general very small. We compare the process with other nuclear excitation mechanisms through coupling with atomic shells and discuss the prospects to observe it in experiment.

A. Shahbaz; C. Müller; T. J. Buervenich; C. H. Keitel

2008-12-13T23:59:59.000Z

329

Nuclear Energy Protocol for Research Isotopes Owen Lowe  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

Protocol for Protocol for Research Isotopes Owen Lowe Office of Isotopes for Medicine and Science Office of Nuclear Energy, Science and Technology April 16, 2002 Isotopes for Life Isotopes for Life Isotopes for Life Office of Nuclear Energy, Science and Technology Lowe/April16_02 NEPRI to NERAC.ppt (2) Nuclear Energy Protocol For Research Isotopes Nuclear Energy Protocol For Research Isotopes Why NEPRI? 6 NEPRI implements DOE funding priorities for fiscal year 2003 6 NEPRI will * Bring order to DOE's responses to requests for research isotopes * Introduce a high-quality peer review to the selection of research isotopes * Enable DOE to concentrate on operating its unique isotope production facilities Isotopes for Life Isotopes for Life Isotopes for Life Office of Nuclear Energy, Science and Technology

330

Gamow-Teller response in deformed even and odd neutron-rich Zr and Mo isotopes  

E-Print Network (OSTI)

Beta-decay properties of neutron-rich Zr and Mo isotopes are investigated within a microscopic theoretical approach based on the proton-neutron quasiparticle random-phase approximation. The underlying mean field is described self-consistently from deformed Skyrme Hartree-Fock calculations with pairing correlations. Residual separable particle-hole and particle-particle forces are also included in the formalism. The structural evolution in these isotopic chains including both even and odd isotopes is analyzed in terms of the equilibrium deformed shapes. Gamow-Teller strength distributions, beta-decay half-lives, and beta-delayed neutron-emission probabilities are studied, stressing their relevance to describe the path of the nucleosynthesis rapid neutron capture process.

P. Sarriguren; A. Algora; J. Pereira

2014-03-05T23:59:59.000Z

331

PALM - Laser Capture Microdissection | EMSL  

NLE Websites -- All DOE Office Websites (Extended Search)

PALM - Laser Capture Microdissection PALM - Laser Capture Microdissection This Laser Capture Microdissection system is equipped with 100 x objective lens for enriching distinct...

332

Learn More about Fusion & Lasers  

NLE Websites -- All DOE Office Websites (Extended Search)

& Lasers How Lasers Work Learn how lasers were developed and how they work. Outreach NIF & Photon Science researchers take learning opportunities on the road. Glossary Don't...

333

Strategic Isotope Production | ornl.gov  

NLE Websites -- All DOE Office Websites (Extended Search)

Strategic Isotope Strategic Isotope Production SHARE Strategic Isotope Production Typical capsules used in the transport of 252Cf source material inside heavily shielded shipping casks. ORNL's unique facilities at the High Flux Isotope Reactor (HFIR), Radiochemical Engineering Development Center (REDC), Irradiated Fuels Examination Laboratory (IFEL), and Irradiated Materials Examination Testing facility (IMET) are routinely used in the production, purification, packaging, and shipping of a number of isotopes of national importance, including: 75Se, 63Ni, 238Pu, 252Cf, and others. The intense neutron flux of the HFIR (2.0 x 1015 neutrons/cm²·s) permits the rapid formation of such isotopes. These highly irradiated materials are then processed and packaged for shipping using the facilities at the REDC, IFEL, and IMET.

334

Two photon absorption laser induced fluorescence measurements of neutral density in a helicon plasma  

SciTech Connect

We have developed a new diagnostic based on two-photon absorption laser induced fluorescence (TALIF). We use a high intensity (5?MW/cm{sup 2}), narrow bandwidth (0.1?cm{sup ?1}) laser to probe the ground state of neutral hydrogen, deuterium and krypton with spatial resolution better than 0.2?cm, a time resolution of 10?ns, and a measurement cadence of 20?Hz. Here, we describe proof-of-principle measurements in a helicon plasma source that demonstrate the TALIF diagnostic is capable of measuring neutral densities spanning four orders of magnitude; comparable to the edge neutral gradients predicted in the DIII-D tokamak pedestal. The measurements are performed in hydrogen and deuterium plasmas and absolute calibration is accomplished through TALIF measurements in neutral krypton. The optical configuration employed is confocal, i.e., both light injection and collection are accomplished with a single lens through a single optical port in the vacuum vessel. The wavelength resolution of the diagnostic is sufficient to separate hydrogen and deuterium spectra and we present measurements from mixed hydrogen and deuterium plasmas that demonstrate isotopic abundance measurements are feasible. Time resolved measurements also allow us to explore the evolution of the neutral hydrogen density and temperature and effects of wall recycling. We find that the atomic neutral density grows rapidly at the initiation of the discharge, reaching the steady-state value within 1?ms. Additionally, we find that neutral hydrogen atoms are born with 0.08?eV temperatures, not 2?eV as is typically assumed.

Galante, M. E.; Magee, R. M.; Scime, E. E. [Department of Physics, West Virginia University, Morgantown, West Virginia 26506 (United States)] [Department of Physics, West Virginia University, Morgantown, West Virginia 26506 (United States)

2014-05-15T23:59:59.000Z

335

Enforcement Letter, International Isotopes Idaho Inc - August...  

Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

Isotopes Idaho, Inc. related to the Relocation of an Irradiated Pellet at the Test Reactor Area Hot Cell Facility at the Idaho National Engineering and Environmental...

336

EIS-0249: Medical Isotopes Production Project  

Energy.gov (U.S. Department of Energy (DOE))

This EIS evaluates the potential environmental impacts of a proposal to establish a production capability for molybdenum-99 (Mo-99) and related medical isotopes.

337

Category:Isotope Geothermometry | Open Energy Information  

Open Energy Info (EERE)

Login | Sign Up Search Category Edit History Facebook icon Twitter icon Category:Isotope Geothermometry Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home...

338

Integration of Nontraditional Isotopic Systems Into Reaction...  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

minerals in geothermal systems (feldspars, epidote, and calcite) often control fracture permeability changes. Measurements of Ca and Sr isotopic fractionation at high...

339

Science with Beams of Radioactive Isotopes  

NLE Websites -- All DOE Office Websites (Extended Search)

2015 The International Chemical Congress of Pacific Basin Societies Science with Beams of Radioactive Isotopes ( 340) Honolulu, Hawaii, USA December 15-20, 2015 Science...

340

Integration of Nontraditional Isotopic Systems Into Reaction...  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

of EGS For Exploration, Evaluation of Water-Rock Interaction, and Impacts of Water Chemistry on Reservoir Sustainability Integration of Nontraditional Isotopic Systems Into...

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


341

Technology verification phase. Dynamic isotope power system. Final report  

SciTech Connect

The Phase I requirements of the Kilowatt Isotope Power System (KIPS) program were to make a detailed Flight System Conceptual Design (FSCD) for an isotope fueled organic Rankine cycle power system and to build and test a Ground Demonstration System (GDS) which simulated as closely as possible the operational characteristics of the FSCD. The activities and results of Phase II, the Technology Verification Phase, of the program are reported. The objectives of this phase were to increase system efficiency to 18.1% by component development, to demonstrate system reliability by a 5000 h endurance test and to update the flight system design. During Phase II, system performance was improved from 15.1% to 16.6%, an endurance test of 2000 h was performed while the flight design analysis was limited to a study of the General Purpose Heat Source, a study of the regenerator manufacturing technique and analysis of the hardness of the system to a laser threat. It was concluded from these tests that the GDS is basically prototypic of a flight design; all components necessary for satisfactory operation were demonstrated successfully at the system level; over 11,000 total h of operation without any component failure attested to the inherent reliability of this type of system; and some further development is required, specifically in the area of performance. (LCL)

Halsey, D.G.

1982-03-10T23:59:59.000Z

342

BNL | CO2 Laser  

NLE Websites -- All DOE Office Websites (Extended Search)

CO2 Laser CO2 Laser The ATF is one of the only two facilities worldwide operating picosecond, terawatt-class CO2 lasers. Our laser system consists of a picoseconds pulse-injector based on fast optical switching from the output of a conventional CO2 laser oscillator, and a chain of high-pressure laser amplifiers. It starts with a wavelength converter wherein a near-IR picosecond solid-state laser with l»1 μm produces a mid-IR 10-μm pulse. This process employs two methods; semiconductor optical switching, and the Kerr effect. First, we combine the outputs from a multi-nanosecond CO2 laser oscillator with a picosecond Nd:YAG laser on a germanium Brewster-plate to produce an ~200 ps, 10μm pulse by semiconductor optical switching. Co-propagating this pulse with a Nd:YAG's 2nd harmonic in a

343

Microcellular foams via phase separation  

SciTech Connect

A study of wide variety of processes for making plastic foams shows that phase separation processes for polymers from solutions offers the most viable methods for obtaining rigid plastic foams which met the physical requirements for fusion target designs. Four general phase separation methods have been shown to give polymer foams with densities less than 0.1 g/cm/sup 3/ and cell sizes of 30..mu..m or less. These methods involve the utilization of non-solvent, chemical or thermal cooling processes to achieve a controlled phase separation wherein either two distinct phases are obtained where the polymer phase is a continuous phase or two bicontinuous phases are obtained where both the polymer and solvent are interpenetrating, continuous, labyrinthine phases. Subsequent removal of the solvent gives the final foam structure.

Young, A.T.

1985-01-01T23:59:59.000Z

344

Design of a New Recoil Separator for Measurements of Radiative Capture Reactions in Astrophysics  

SciTech Connect

The rates of proton- and alpha-capture reactions on unstable proton-rich nuclei are needed to understand the energy generation and element synthesis occurring in novae, X-ray bursts, and other explosions. Direct measurements of the cross sections of some of these reactions are now possible with radioactive beams and a recoil separator. A new device for such measurements, the Separator for CApture Reactions [SECAR], is being designed for use at the Facility for Rare Isotope Beams (FRIB). The specifications and preliminary conceptual design will be discussed along with plans for the first set of measurements.

Berg, Georg P. A.; Couder, Manoel; Wiescher, Michael [Dept. of Physics, Univ. of Notre Dame, Notre Dame, Indiana, 46556-5670 (United States); Joint Institute for Nuclear Astrophysics (JINA) (United States); Blackmon, Jeff C. [Dept. of Physics and Astronomy, Louisiana State Univ., Baton Rouge, Louisiana, 70803-4001 (United States); Greife, U. [Dept. of Physics, Colorado School of Mines, Golden, CO 80401 (United States); Montes, F.; Schatz, Hendrik [National Superconducting Cyclotron Laboratory, Michigan State Univ., East Lansing, Michigan, 48824 (United States); Joint Institute for Nuclear Astrophysics (JINA) (United States); Rehm, K. Ernst [Physics Division, Argonne National Lab, Argonne, Illinois, 60439 (United States); Joint Institute for Nuclear Astrophysics (JINA) (United States); Smith, Michael S. [Physics Division, Oak Ridge National Lab, Oak Ridge, Tennessee, 37831-6354 (United States); Zeller, Al [National Superconducting Cyclotron Laboratory, Michigan State Univ., East Lansing, Michigan, 48824 (United States)

2010-08-12T23:59:59.000Z

345

Sensitive detection of methane and nitrous oxide isotopomers using a continuous wave quantum cascade laser  

Science Journals Connector (OSTI)

A continuous wave quantum cascade laser (QCL), operating near 8.1 ?m...4) and nitrous oxide (N2O) stable isotopes. Several rotational transitions of 14N2 16O, 15N14N16O, 14N2 18O,

G. Gagliardi; F. Tamassia; P. De Natale…

2002-06-01T23:59:59.000Z

346

?-decay studies of the francium isotopes 198Fr and 199Fr  

Science Journals Connector (OSTI)

Very neutron deficient francium isotopes have been produced in fusion evaporation reactions using 60Ni ions on 141Pr targets. The gas-filled recoil separator RITU was employed to collect the fusion products and to separate them from the scattered beam. The activities were implanted into a position sensitive silicon detector after passing through a gas-counter system. The isotopes were identified using spatial and time correlations between the implants and the decays. Two ?-particle activities, with E?=7613(15) keV and T1/2 = (15?5+12) ms and E?=7684(15) keV and T1/2 = (16?5+13) ms were identified in the new isotope 198Fr. In addition, the half-life and ?-particle energy of 199Fr were measured with improved precision. The measured decay properties deduced for 199Fr and 198Fr suggest that there is an onset of ground-state deformation at N=112 in the Fr isotopes.

J. Uusitalo; J. Sarén; S. Juutinen; M. Leino; S. Eeckhaudt; T. Grahn; P. T. Greenlees; U. Jakobsson; P. Jones; R. Julin; S. Ketelhut; A.-P. Leppänen; M. Nyman; J. Pakarinen; P. Rahkila; C. Scholey; A. Semchenkov; J. Sorri; A. Steer; M. Venhart

2013-06-10T23:59:59.000Z

347

Actinide Lanthanide Separation Process – ALSEP  

SciTech Connect

Separation of the minor actinides (Am, Cm) from the lanthanides at an industrial scale remains a significant technical challenge for closing the nuclear fuel cycle. To increase the safety of used nuclear fuel (UNF) reprocessing, as well as reduce associated costs, a novel solvent extraction process has been developed. The process allows for partitioning minor actinides, lanthanides and fission products following uranium/plutonium/neptunium removal; minimizing the number of separation steps, flowsheets, chemical consumption, and waste. This new process, Actinide Lanthanide SEParation (ALSEP), uses an organic solvent consisting of a neutral diglycolamide extractant, either N,N,N',N'-tetra(2 ethylhexyl)diglycolamide (T2EHDGA) or N,N,N',N'-tetraoctyldiglycolamide (TODGA), and an acidic extractant 2-ethylhexylphosphonic acid mono-2-ethylhexyl ester (HEH[EHP]), dissolved in an aliphatic diluent (e.g. n-dodecane). The An/Ln co-extraction is conducted from moderate-to-strong nitric acid, while the selective stripping of the minor actinides from the lanthanides is carried out using a polyaminocarboxylic acid/citrate buffered solution at pH anywhere between 3 and 4.5. The extraction and separation of the actinides from the fission products is very effective in a wide range of HNO3 concentrations and the minimum separation factors for lanthanide/Am exceed 30 for Nd/Am, reaching > 60 for Eu/Am under some conditions. The experimental results presented here demonstrate the great potential for a combined system, consisting of a neutral extractant such as T2EHDGA or TODGA, and an acidic extractant such as HEH[EHP], for separating the minor actinides from the lanthanides.

Gelis, Artem V.; Lumetta, Gregg J.

2014-01-29T23:59:59.000Z

348

3D Relativistic Hartree-Bogoliubov model with a separable pairing interaction  

E-Print Network (OSTI)

A recently introduced separable pairing force for relativistic Hartree-Bogoliubov (RHB) calculations, adjusted in nuclear matter to the pairing gap of the Gogny force, is employed in the 3D RHB model for triaxial shapes. The pairing force is separable in momentum space but, when transformed to coordinate space in calculations of finite nuclei, it is no longer separable because of translational invariance. The corresponding pairing matrix elements are represented as a sum of a finite number of separable terms in the basis of a 3D harmonic oscillator. The 3D RHB model is applied to the calculation of binding energy surfaces and pairing energy maps for a sequence of even-A Sm isotopes.

T. Niksic; D. Vretenar; Y. Tian; Z. Y. Ma; P. Ring

2009-12-07T23:59:59.000Z

349

Isotope-Selective Detection and Imaging of Organic Nanolayers  

Science Journals Connector (OSTI)

Isotope-Selective Detection and Imaging of Organic Nanolayers ... We show isotopic selectivity of MRFM for three nuclei, 1H, 31P, and 13C, in organic materials. ... data to further distinguish and characterize the 2 isotopes. ...

H. J. Mamin; T. H. Oosterkamp; M. Poggio; C. L. Degen; C. T. Rettner; D. Rugar

2009-07-09T23:59:59.000Z

350

Electromagnetic separation of isotopes at Oak Ridge ? L.O. Love...  

NLE Websites -- All DOE Office Websites (Extended Search)

the natural mercury vapor and concentrate the mercury-202 striking the silver pocket. Dry ice was chosen as the cooling material, but a suitable transfer medium was needed. Love...

351

Electromagnetic separation of isotopes at Oak Ridge ? L.O. Love...  

NLE Websites -- All DOE Office Websites (Extended Search)

to ship it back. This routine went on until 1968. "By that time the Laboratory"s Thermonuclear division had emerged as the sole conceivable future user of the coils (for plasma...

352

Automated product recovery in a Hg-196 photochemical isotope separation process  

DOE Patents (OSTI)

A method of removing deposited product from a photochemical reactor used in the enrichment of [sup 196]Hg has been developed and shown to be effective for rapid re-cycling of the reactor system. Unlike previous methods relatively low temperatures are used in a gas and vapor phase process of removal. Importantly, the recovery process is understood in a quantitative manner so that scaling design to larger capacity systems can be easily carried out. 2 figs.

Grossman, M.W.; Speer, R.

1992-07-21T23:59:59.000Z

353

BNL | CFN Laser System Qualifications  

NLE Websites -- All DOE Office Websites (Extended Search)

Laser System Qualification There are multiple laser systems at the CFN. Users who will be working with the following class 3B or 4 laser systems are required to complete the Laser...

354

RAPID FUSION METHOD FOR DETERMINATION OF PLUTONIUM ISOTOPES IN LARGE RICE SAMPLES  

SciTech Connect

A new rapid fusion method for the determination of plutonium in large rice samples has been developed at the Savannah River National Laboratory (Aiken, SC, USA) that can be used to determine very low levels of plutonium isotopes in rice. The recent accident at Fukushima Nuclear Power Plant in March, 2011 reinforces the need to have rapid, reliable radiochemical analyses for radionuclides in environmental and food samples. Public concern regarding foods, particularly foods such as rice in Japan, highlights the need for analytical techniques that will allow very large sample aliquots of rice to be used for analysis so that very low levels of plutonium isotopes may be detected. The new method to determine plutonium isotopes in large rice samples utilizes a furnace ashing step, a rapid sodium hydroxide fusion method, a lanthanum fluoride matrix removal step, and a column separation process with TEVA Resin? cartridges. The method can be applied to rice sample aliquots as large as 5 kg. Plutonium isotopes can be determined using alpha spectrometry or inductively-coupled plasma mass spectrometry (ICP-MS). The method showed high chemical recoveries and effective removal of interferences. The rapid fusion technique is a rugged sample digestion method that ensures that any refractory plutonium particles are effectively digested. The MDA for a 5 kg rice sample using alpha spectrometry is 7E-5 mBq g{sup -1}. The method can easily be adapted for use by ICP-MS to allow detection of plutonium isotopic ratios.

Maxwell, S.

2013-03-01T23:59:59.000Z

355

? decay of the very neutron-deficient isotopes 197–199Fr  

Science Journals Connector (OSTI)

Decay properties of the very neutron-deficient isotopes 197–199Fr were studied at the velocity filter Separator for Heavy Ion reaction Products (SHIP) at GSI in Darmstadt. The isotopes were produced in the 2n–4n evaporation channels of the fusion-evaporation reaction 60Ni+141Pr ? 201Fr*. Improved ?-decay properties of 199Fr were determined and the possible existence of two ?-decaying states in this nucleus is discussed. For the isotope 198Fr a broad ?-decay energy distribution was detected in the range of (7470–7930) keV and two ?-decaying states were observed with half-lives of 1.1(7) and 15(3) ms. The new isotope 197Fr was identified based on the observation of one ?-decay chain yielding E?=7728(15) keV and T1/2=0.6?0.3+3.0 ms. The systematics of reduced ?-decay widths are presented for neutron-deficient francium, radon, and astatine isotopes.

Z. Kalaninová; A. N. Andreyev; S. Antalic; F. P. Heßberger; D. Ackermann; B. Andel; M. C. Drummond; S. Hofmann; M. Huyse; B. Kindler; J. F. W. Lane; V. Liberati; B. Lommel; R. D. Page; E. Rapisarda; K. Sandhu; Š. Šáro; A. Thornthwaite; P. Van Duppen

2013-04-29T23:59:59.000Z

356

A multifrequency interband two-cascade laser  

SciTech Connect

Multifrequency lasing in a new class of injection heterolasers, i.e., in an interband two-cascade laser with a tunneling p-n junction separating two active regions of quantum wells located in the same waveguide is obtained and studied. The developed laser structure with pulsed pumping provided the simultaneous emission of two first-order modes with the wavelengths of 1.063 and 0.98 {mu}m and two third-order modes with the wavelengths of 0.951 and 0.894 {mu}m. Due to nonlinear mixing of the modes within the laser cavity, the generation of the second harmonics and sum frequencies was observed.

Biryukov, A. A.; Zvonkov, B. N.; Nekorkin, S. M.; Demina, P. B.; Semenov, N. N. [Research Physicotechnical Institute at the Nizhni Novgorod State University (Russian Federation); Aleshkin, V. Ya.; Gavrilenko, V. I.; Dubinov, A. A., E-mail: sanya@ipm.sci-nnov.ru; Marem'yanin, K. V.; Morozov, S. V. [Russian Academy of Sciences, Institute for Physics of Microstructures (Russian Federation); Belyanin, A. A.; Kocharovsky, V. V. [Texas A and M University, Department of Physics (United States); Kocharovsky, Vl. V. [Russian Academy of Sciences, Institute of Applied Physics (Russian Federation)

2007-10-15T23:59:59.000Z

357

Energy Conservation Possibilities Using Gas Separating Membranes  

E-Print Network (OSTI)

The separation of gases using semi permeable membranes is a viable unit operation. A novel composite membrane combined with hollow fiber spinning technology enable Monsanto Co. to offer PRISM (TM); Separators to the industrial market. The separator...

Knieriem, H.; Henis, J. M. S.

1980-01-01T23:59:59.000Z

358

Solvent Isotope-Induced Equilibrium Perturbation for Isocitrate Lyase  

Science Journals Connector (OSTI)

Solvent Isotope-Induced Equilibrium Perturbation for Isocitrate Lyase ... Solvent isotopic composition can influence both the rates of enzyme-catalyzed reactions (solvent kinetic isotope effects) and, in the case of solvent-derived deuterium incorporation into nonexchangeable C–H bonds in products, solvent equilibrium isotope effects. ... In this study, we report the solvent isotope-induced transient change in the concentration and isotopic composition of the reactants. ...

Christine E. Quartararo; Timin Hadi; Sean M. Cahill; John S. Blanchard

2013-11-21T23:59:59.000Z

359

BUILDING A CHEMICAL LASER WEAPON  

Science Journals Connector (OSTI)

BUILDING A CHEMICAL LASER WEAPON ... Under fire, Airborne Laser program director confronts challenges of revolutionary weapons system ...

WILLIAM G. SCHULZ

2004-12-20T23:59:59.000Z

360

Stable isotope variations in Late Pennsylvanian brachiopods from cyclic sedimentary deposits: paleoenvironmental and diagenetic implications  

E-Print Network (OSTI)

. VeNication of Shell Chemistry Preservation Cathodo4minescence Energy Dispersive Spectrometry Comparable Studies Diagenetic Impkations Nature of Diagenetic System . CHAPTER V. ISOTOPIC ANALYSIS General Considerations . Sampling and Analysis... that paleotemperatures and relative salinities can be estimated quantitatively by analysis of skeletal carbonate compositions (Urey and others, 1951; Dodd and Stanton, 1975). Fossils, because of the relative ease of manual separation and the reasonable control...

Adlis, David Scott

2012-06-07T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


361

Separations innovative concepts: Project summary  

SciTech Connect

This project summary includes the results of 10 innovations that were funded under the US Department's Innovative Concept Programs. The concepts address innovations that can substantially reduce the energy used in industrial separations. Each paper describes the proposed concept, and discusses the concept's potential energy savings, market applications, technical feasibility, prior work and state of the art, and future development needs.

Lee, V.E. (ed.)

1988-05-01T23:59:59.000Z

362

33rd Actinide Separations Conference  

SciTech Connect

Welcome to the 33rd Actinide Separations Conference hosted this year by the Lawrence Livermore National Laboratory. This annual conference is centered on the idea of networking and communication with scientists from throughout the United States, Britain, France and Japan who have expertise in nuclear material processing. This conference forum provides an excellent opportunity for bringing together experts in the fields of chemistry, nuclear and chemical engineering, and actinide processing to present and discuss experiences, research results, testing and application of actinide separation processes. The exchange of information that will take place between you, and other subject matter experts from around the nation and across the international boundaries, is a critical tool to assist in solving both national and international problems associated with the processing of nuclear materials used for both defense and energy purposes, as well as for the safe disposition of excess nuclear material. Granlibakken is a dedicated conference facility and training campus that is set up to provide the venue that supports communication between scientists and engineers attending the 33rd Actinide Separations Conference. We believe that you will find that Granlibakken and the Lake Tahoe views provide an atmosphere that is stimulating for fruitful discussions between participants from both government and private industry. We thank the Lawrence Livermore National Laboratory and the United States Department of Energy for their support of this conference. We especially thank you, the participants and subject matter experts, for your involvement in the 33rd Actinide Separations Conference.

McDonald, L M; Wilk, P A

2009-05-04T23:59:59.000Z

363

Gas Separations using Ceramic Membranes  

SciTech Connect

This project has been oriented toward the development of a commercially viable ceramic membrane for high temperature gas separations. A technically and commercially viable high temperature gas separation membrane and process has been developed under this project. The lab and field tests have demonstrated the operational stability, both performance and material, of the gas separation thin film, deposited upon the ceramic membrane developed. This performance reliability is built upon the ceramic membrane developed under this project as a substrate for elevated temperature operation. A comprehensive product development approach has been taken to produce an economically viable ceramic substrate, gas selective thin film and the module required to house the innovative membranes for the elevated temperature operation. Field tests have been performed to demonstrate the technical and commercial viability for (i) energy and water recovery from boiler flue gases, and (ii) hydrogen recovery from refinery waste streams using the membrane/module product developed under this project. Active commercializations effort teaming with key industrial OEMs and end users is currently underway for these applications. In addition, the gas separation membrane developed under this project has demonstrated its economical viability for the CO2 removal from subquality natural gas and landfill gas, although performance stability at the elevated temperature remains to be confirmed in the field.

Paul KT Liu

2005-01-13T23:59:59.000Z

364

CRAD, Engineering - Oak Ridge National Laboratory High Flux Isotope...  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

Oak Ridge National Laboratory High Flux Isotope Reactor CRAD, Engineering - Oak Ridge National Laboratory High Flux Isotope Reactor February 2007 A section of Appendix C to DOE G...

365

CRAD, Maintenance - Oak Ridge National Laboratory High Flux Isotope...  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

Maintenance - Oak Ridge National Laboratory High Flux Isotope Reactor CRAD, Maintenance - Oak Ridge National Laboratory High Flux Isotope Reactor February 2007 A section of...

366

CRAD, Engineering - Oak Ridge National Laboratory High Flux Isotope...  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

Engineering - Oak Ridge National Laboratory High Flux Isotope Reactor Contractor ORR CRAD, Engineering - Oak Ridge National Laboratory High Flux Isotope Reactor Contractor ORR...

367

CRAD, Maintenance - Oak Ridge National Laboratory High Flux Isotope...  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

Maintenance - Oak Ridge National Laboratory High Flux Isotope Reactor Contractor ORR CRAD, Maintenance - Oak Ridge National Laboratory High Flux Isotope Reactor Contractor ORR...

368

CRAD, Management- Oak Ridge National Laboratory High Flux Isotope...  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

Management- Oak Ridge National Laboratory High Flux Isotope Reactor CRAD, Management- Oak Ridge National Laboratory High Flux Isotope Reactor February 2007 A section of Appendix C...

369

Stable Isotope, Site-Specific Mass Tagging For Protein Identification  

NLE Websites -- All DOE Office Websites (Extended Search)

Stable Isotope, Site-Specific Mass Tagging For Protein Identification Stable Isotope, Site-Specific Mass Tagging For Protein Identification Proteolytic peptide mass mapping as...

370

Enriched Stable Isotope Materials and Chemistry | ornl.gov  

NLE Websites -- All DOE Office Websites (Extended Search)

Enriched Stable Isotope Materials and Chemistry SHARE Enriched Stable Isotope Materials and Chemistry Reductiondistillation of calcium-48 metal valued at over 900,000. An...

371

Isotopic Analysis- Gas At Chena Geothermal Area (Kolker, Et Al...  

Open Energy Info (EERE)

Laboratory sampling and analysis of He isotopes from Chena Hot Springs. Notes Helium isotope measurements indicate there is no magmatic or mantle input at the Chena Geothermal...

372

Development of a Micropyrolyzer for Enhanced Isotope Ratio Measurement...  

NLE Websites -- All DOE Office Websites (Extended Search)

Micropyrolyzer for Enhanced Isotope Ratio Measurement. Development of a Micropyrolyzer for Enhanced Isotope Ratio Measurement. Abstract: This paper presents design, fabrication and...

373

Along the Laser Beampath  

NLE Websites -- All DOE Office Websites (Extended Search)

has been installed in the preamplifier modules (PAMs) at the front end of the NIF laser system. The spatial shapers can obscure the laser light at programmed locations within...

374

Laser particle sorter  

DOE Patents (OSTI)

Method and apparatus are provided for sorting particles, such as biological particles. A first laser is used to define an optical path having an intensity gradient which is effective to propel the particles along the path but which is sufficiently weak that the particles are not trapped in an axial direction. A probe laser beam is provided for interrogating the particles to identify predetermined phenotypical characteristics of the particles. A second laser beam is provided to intersect the driving first laser beam, wherein the second laser beam is activated by an output signal indicative of a predetermined characteristic. The second laser beam is switchable between a first intensity and a second intensity, where the first intensity is effective to displace selected particles from the driving laser beam and the second intensity is effective to propel selected particles along the deflection laser beam. The selected particles may then be propelled by the deflection beam to a location effective for further analysis. 2 figs.

Martin, J.C.; Buican, T.N.

1987-11-30T23:59:59.000Z

375

Laser preheat enhanced ignition  

DOE Patents (OSTI)

A method for enhancing fuel ignition performance by preheating the fuel with laser light at a wavelength that is absorbable by the fuel prior to ignition with a second laser is provided.

Early, James W. (Los Alamos, NM)

1999-01-01T23:59:59.000Z

376

Laser preheat enhanced ignition  

DOE Patents (OSTI)

A method for enhancing fuel ignition performance by preheating the fuel with laser light at a wavelength that is absorbable by the fuel prior to ignition with a second laser is provided. 11 figs.

Early, J.W.

1999-03-02T23:59:59.000Z

377

Laser-assisted electrochemistry  

SciTech Connect

The effect of laser irradiation on electrodeposition processes has been investigated. These studies demonstrated that the addition of laser irradiation to an electroplating process can dramatically enhance plating rates and current efficiencies, as well as improve the morphology of the resultant electrodeposit. During the course of these investigations, the mechanism for the laser enhancement of electrodeposition processes was determined. Experimental evidence was obtained to show that laser irradiation of the substrate results in increased metal ion concentrations at the surface of the electrode due to a laser-induced Soret effect. The laser-induced Soret effect has important implications for laser-assisted electrochemical processing. The increase in the surface concentration of ions allows efficient electrodeposition from dilute solutions. As such, laser- assisted electrodeposition may develop into an environmentally conscious manufacturing process by reducing waste and limiting worker exposure to toxic chemicals.

Glenn, D.F.

1995-05-01T23:59:59.000Z

378

The Quest for the Heaviest Uranium Isotope  

E-Print Network (OSTI)

We study Uranium isotopes and surrounding elements at very large neutron number excess. Relativistic mean field and Skyrme-type approaches with different parametrizations are used in the study. Most models show clear indications for isotopes that are stable with respect to neutron emission far beyond N=184 up to the range of around N=258.

S. Schramm; D. Gridnev; D. V. Tarasov; V. N. Tarasov; W. Greiner

2011-07-06T23:59:59.000Z

379

Advanced Mass Spectrometers for Hydrogen Isotope Analyses  

SciTech Connect

This report is a summary of the results of a joint Savannah River Laboratory (SRL) - Savannah River Plant (SRP) ''Hydrogen Isotope Mass Spectrometer Evaluation Program''. The program was undertaken to evaluate two prototype hydrogen isotope mass spectrometers and obtain sufficient data to permit SRP personnel to specify the mass spectrometers to replace obsolete instruments.

Chastagner, P.

2001-08-01T23:59:59.000Z

380

Separable Optical Potentials for (d,p) Reactions  

E-Print Network (OSTI)

An important ingredient for applications of nuclear physics to e.g. astrophysics or nuclear energy are the cross sections for reactions of neutrons with rare isotopes. Since direct measurements are often not possible, indirect methods like (d,p) reactions must be used instead. Those (d,p) reactions may be viewed as effective three-body reactions and described with Faddeev techniques. An additional challenge posed by (d,p) reactions involving heavier nuclei is the treatment of the Coulomb force. To avoid numerical complications in dealing with the screening of the Coulomb force, recently a new approach using the Coulomb distorted basis in momentum space was suggested. In order to implement this suggestion, one needs not only to derive a separable representation of neutron- and proton-nucleus optical potentials, but also compute the Coulomb distorted form factors in this basis.

Ch. Elster; L. Hlophe; V. Eremenko; F. M. Nunes; G. Arbanas; J. E. Escher; I. J. Thompson

2014-10-05T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


381

Separable Optical Potentials for (d,p) Reactions  

E-Print Network (OSTI)

An important ingredient for applications of nuclear physics to e.g. astrophysics or nuclear energy are the cross sections for reactions of neutrons with rare isotopes. Since direct measurements are often not possible, indirect methods like (d,p) reactions must be used instead. Those (d,p) reactions may be viewed as effective three-body reactions and described with Faddeev techniques. An additional challenge posed by (d,p) reactions involving heavier nuclei is the treatment of the Coulomb force. To avoid numerical complications in dealing with the screening of the Coulomb force, recently a new approach using the Coulomb distorted basis in momentum space was suggested. In order to implement this suggestion, one needs not only to derive a separable representation of neutron- and proton-nucleus optical potentials, but also compute the Coulomb distorted form factors in this basis.

Elster, Ch; Eremenko, V; Nunes, F M; Arbanas, G; Escher, J E; Thompson, I J

2014-01-01T23:59:59.000Z

382

Isotopes  

NLE Websites -- All DOE Office Websites (Extended Search)

are saving lives, advancing cutting-edge research and keeping the U.S. safe. Strontium-82 produced at Los Alamos is used in hospitals nation- and world-wide for critical...

383

ISOTOPES  

E-Print Network (OSTI)

Research, Division of Nuclear Sciences of the Basic Energy Sciences ProgramResearch, Division of Nuclear Sciences of the Basic Energy Sciences Program

Lederer, C. Michael

2013-01-01T23:59:59.000Z

384

ISOTOPES  

E-Print Network (OSTI)

5-7. 1975, British Nuclear Engineering Society (1975). 87.London, March British Nuclear Engineering Society (1975).T.H. Pigford, Nuclear Chemical Engineering (1St edition),

Lederer, C. Michael

2013-01-01T23:59:59.000Z

385

ISOTOPES  

E-Print Network (OSTI)

uranium, heavy-water-moderated CANDU reactor, as contrastedis important, and in the CANDU power reactor, which uses

Lederer, C. Michael

2013-01-01T23:59:59.000Z

386

Laser Heat Treatment [Laser Applications Laboratory] - Nuclear Engineering  

NLE Websites -- All DOE Office Websites (Extended Search)

Heat Treatment Heat Treatment Capabilities Engineering Experimentation Reactor Safety Experimentation Aerosol Experiments System Components Laser Applications Overview Laser Oil & Gas Well Drilling Laser Heat Treatment Laser Welding of Metals On-line Monitoring Laser Beam Delivery Laser Glazing of Railroad Rails High Power Laser Beam Delivery Decontamination and Decommissioning Refractory Alloy Welding Robots Applications Other Facilities Other Capabilities Work with Argonne Contact us For Employees Site Map Help Join us on Facebook Follow us on Twitter NE on Flickr Laser Applications Laboratory Laser Heat Treatment Project description: Optimization of laser beam heat treatment. Category: Project with industrial partner (Caterpillar and USCAR) Bookmark and Share Heat treatment optics

387

It's Elemental - Isotopes of the Element Francium  

NLE Websites -- All DOE Office Websites (Extended Search)

Radon Radon Previous Element (Radon) The Periodic Table of Elements Next Element (Radium) Radium Isotopes of the Element Francium [Click for Main Data] Most of the isotope data on this site has been obtained from the National Nuclear Data Center. Please visit their site for more information. Naturally Occurring Isotopes Francium has no naturally occurring isotopes. Known Isotopes Mass Number Half-life Decay Mode Branching Percentage 199 12 milliseconds Alpha Decay > 0.00% Electron Capture No Data Available 200 49 milliseconds Alpha Decay 100.00% 201 62 milliseconds Alpha Decay 100.00% 201m 19 milliseconds Alpha Decay 100.00% 202 0.30 seconds Alpha Decay 100.00% 202m 0.29 seconds Alpha Decay 100.00% 203 0.55 seconds Alpha Decay <= 100.00% 204 1.8 seconds Alpha Decay 92.00%

388

It's Elemental - Isotopes of the Element Radon  

NLE Websites -- All DOE Office Websites (Extended Search)

Astatine Astatine Previous Element (Astatine) The Periodic Table of Elements Next Element (Francium) Francium Isotopes of the Element Radon [Click for Main Data] Most of the isotope data on this site has been obtained from the National Nuclear Data Center. Please visit their site for more information. Naturally Occurring Isotopes Radon has no naturally occurring isotopes. Known Isotopes Mass Number Half-life Decay Mode Branching Percentage 193 1.15 milliseconds Alpha Decay 100.00% 194 0.78 milliseconds Alpha Decay 100.00% 195 6 milliseconds Alpha Decay 100.00% 195m 5 milliseconds Alpha Decay 100.00% 196 4.4 milliseconds Alpha Decay 99.90% Electron Capture ~ 0.10% 197 53 milliseconds Alpha Decay 100.00% 197m 25 milliseconds Alpha Decay 100.00% 198 65 milliseconds Alpha Decay No Data Available

389

Selected Isotopes for Optimized Fuel Assembly Tags  

SciTech Connect

In support of our ongoing signatures project we present information on 3 isotopes selected for possible application in optimized tags that could be applied to fuel assemblies to provide an objective measure of burnup. 1. Important factors for an optimized tag are compatibility with the reactor environment (corrosion resistance), low radioactive activation, at least 2 stable isotopes, moderate neutron absorption cross-section, which gives significant changes in isotope ratios over typical fuel assembly irradiation levels, and ease of measurement in the SIMS machine 2. From the candidate isotopes presented in the 3rd FY 08 Quarterly Report, the most promising appear to be Titanium, Hafnium, and Platinum. The other candidate isotopes (Iron, Tungsten, exhibited inadequate corrosion resistance and/or had neutron capture cross-sections either too high or too low for the burnup range of interest.

Gerlach, David C.; Mitchell, Mark R.; Reid, Bruce D.; Gesh, Christopher J.; Hurley, David E.

2008-10-01T23:59:59.000Z

390

Research and development of hydrogen separation technology with inorganic membranes  

SciTech Connect

Inorganic membrane technology has long been expected to provide new economical methods for industrial and waste management processes. At this time, the only commercially valuable inorganic membranes are the ultra filters derived from the French process that was used to produce the barrier for the French Gaseous Diffusion Plants. But these membranes are very expensive and have limited areas of application. Over the past fifteen years, scientists now in the Inorganic Membrane Technology Laboratory (IMTL) in Oak Ridge, Tennessee have developed theories and processes for inorganic membranes that can be used to design and produce inorganic membranes for a very broad range of applications. A part of the fabrication process is an adaptive spinoff from the still classified process used to manufacture barriers for the U.S. Gaseous Diffusion Process. Although that part of the process is classified, it is a very flexible and adaptable process and it can be used with a broad range of materials. With the theories and design capabilities developed in the last fifteen years, this new adaptive manufacturing technology can be used to manufacture commercial inorganic membranes that are not useful for the separation of uranium isotopes and they have little or no relation to the barriers that were used to separate uranium isotopes. The development and deployment of such inorganic membranes can be very beneficial to U.S. industry. Inorganic membranes can be specifically designed and manufactured for a large number of different applications. Such membranes can greatly improve the efficiency of a broad range of industrial processes and provide new technology for waste management. These inorganic membranes have the potential for major energy savings and conservation of energy. They can provide the means for significant improvements in the competitiveness of US Industry and improve the economy and health and welfare of the nation.

Fain, D.E.

1999-07-01T23:59:59.000Z

391

Laser-driven fusion  

Science Journals Connector (OSTI)

The use of intense laser light to bring about thermonuclear reactions in a plasma is of considerable current interest. We present detailed analytical and computational studies which show the feasibility of laser-driven fusion. The required laser technology and the presently anticipated practical difficulties are discussed in outline.

Keith A. Brueckner and Siebe Jorna

1974-04-01T23:59:59.000Z

392

Laser bottom hole assembly  

DOE Patents (OSTI)

There is provided for laser bottom hole assembly for providing a high power laser beam having greater than 5 kW of power for a laser mechanical drilling process to advance a borehole. This assembly utilizes a reverse Moineau motor type power section and provides a self-regulating system that addresses fluid flows relating to motive force, cooling and removal of cuttings.

Underwood, Lance D; Norton, Ryan J; McKay, Ryan P; Mesnard, David R; Fraze, Jason D; Zediker, Mark S; Faircloth, Brian O

2014-01-14T23:59:59.000Z

393

THE GENESIS SOLAR WIND CONCENTRATOR TARGET: MASS FRACTIONATION CHARACTERISED BY NE ISOTOPES  

SciTech Connect

The concentrator on Genesis provides samples of increased fluences of solar wind ions for precise determination of the oxygen isotopic composition of the solar wind. The concentration process caused mass fractionation as function of the radial target position. They measured the fractionation using Ne released by UV laser ablation along two arms of the gold cross from the concentrator target to compare measured Ne with modeled Ne. The latter is based on simulations using actual conditions of the solar wind during Genesis operation. Measured Ne abundances and isotopic composition of both arms agree within uncertainties indicating a radial symmetric concentration process. Ne data reveal a maximum concentration factor of {approx} 30% at the target center and a target-wide fractionation of Ne isotopes of 3.8%/amu with monotonously decreasing {sup 20}Ne/{sup 22}Ne ratios towards the center. The experimentally determined data, in particular the isotopic fractionation, differ from the modeled data. They discuss potential reasons and propose future attempts to overcome these disagreements.

WIENS, ROGER C. [Los Alamos National Laboratory; OLINGER, C. [Los Alamos National Laboratory; HEBER, V.S. [Los Alamos National Laboratory; REISENFELD, D.B. [Los Alamos National Laboratory; BURNETT, D.S. [Los Alamos National Laboratory; ALLTON, J.H. [Los Alamos National Laboratory; BAUR, H. [Los Alamos National Laboratory; WIECHERT, U. [Los Alamos National Laboratory; WIELER, R. [Los Alamos National Laboratory

2007-01-02T23:59:59.000Z

394

Extraction and Determination of Boron Isotopic Composition in Tourmalines  

Science Journals Connector (OSTI)

Tourmaline is an abundant boron-rich alumosilicate mineral with complex chemistry and rich in Fe, Mg, Al, Si elements. In this study, tourmaline samples were decomposed by alkali fusion method, and then the boron was separated and purified using three different procedures. It was found that both Fe3+ and Al3+ ions, rich in tourmaline samples seriously, which affected the accurate determination of boron concentration by Azomethine-H spectrophotometric method and also caused a loss of boron by specific adsorption when large amount of amorphous hydroxide precipitate formed in ion-exchange columns. The addition of small amount of EDTA can eliminate the influence, but brings serious isobaric interference on boron isotopic analysis by TIMS. Finally, a three-column ion-exchange procedure was established including the first mixed resin column, the peristaltic pump coupled boron specific resin column, and the second mixed resin column, which ensures the full recovery of boron (> 99%) from tourmaline samples with complex matrices. The PTIMS-Cs2BO2+-static double-collection method was established by selecting H3-H4 Faraday cups and optimizing parameters in Zoom Optics (Focus Quad: 15; Dispersion Quad: ?85) in a Triton TI mass spectrometer. The determined average 11B/10B value of NIST SRM 951 standard boron solution was 4.05044±0.00012 (2?, n = 8, 1 ?g B), which was superior to the dynamic collection method in internal/external precision. A ?11B value of ?0.3% for NIST SRM 951 through the same pretreatment procedure was obtained, indicating that there was no isotopic fractionation occurred during the extraction procedure. The comparison of boron isotopic compositions in natural samples by TIMS and MC-ICP-MS after the chemistry procedure indicated that ?11B values determined by the static PTIMS-Cs2BO2+ method were in good agreement with that by MC-ICP-MS.

Xiong YAN; Shao-Yong JIANG; Hai-Zhen WEI; Yan YAN; He-Pin WU; Wei PU

2012-01-01T23:59:59.000Z

395

Convex polytopes and quantum separability  

SciTech Connect

We advance a perspective of the entanglement issue that appeals to the Schlienz-Mahler measure [Phys. Rev. A 52, 4396 (1995)]. Related to it, we propose a criterium based on the consideration of convex subsets of quantum states. This criterium generalizes a property of product states to convex subsets (of the set of quantum states) that is able to uncover an interesting geometrical property of the separability property.

Holik, F.; Plastino, A. [Departamento de Matematica - Ciclo Basico Comun, Universidad de Buenos Aires - Pabellon III, Ciudad Universitaria, Buenos Aires, Argentina and CONICET (Argentina); National University La Plata and CONICET IFLP-CCT, C.C. 727 - 1900 La Plata (Argentina)

2011-12-15T23:59:59.000Z

396

Method to blend separator powders  

DOE Patents (OSTI)

A method for making a blended powder mixture, whereby two or more powders are mixed in a container with a liquid selected from nitrogen or short-chain alcohols, where at least one of the powders has an angle of repose greater than approximately 50 degrees. The method is useful in preparing blended powders of Li halides and MgO for use in the preparation of thermal battery separators.

Guidotti, Ronald A. (Albuquerque, NM); Andazola, Arthur H. (Albuquerque, NM); Reinhardt, Frederick W. (Albuquerque, NM)

2007-12-04T23:59:59.000Z

397

Guayule resin separation and purification  

E-Print Network (OSTI)

fraction and reducing the presence of these terpenes to practically non-detectable levels in the polar fraction. A single component, as identified by gas chromatograph (GC) was also effectively extracted from the Texas A&M resins. Saponification..., using an FID Solvent fractionation of the Firestone resin between methanol and hexane was also apparently effective in separating the low molecular weight rubber. Figure 16 and Figure 17 show the gas chromatographs of the bottom phase (fraction "a...

Bajwa, Mohinder P.S.

1992-01-01T23:59:59.000Z

398

Separation of Tritium from Wastewater  

SciTech Connect

A proprietary tritium loading bed developed by Molecular Separations, Inc (MSI) has been shown to selectively load tritiated water as waters of hydration at near ambient temperatures. Tests conducted with a 126 {micro}C{sub 1} tritium/liter water standard mixture showed reductions to 25 {micro}C{sub 1}/L utilizing two, 2-meter long columns in series. Demonstration tests with Hanford Site wastewater samples indicate an approximate tritium concentration reduction from 0.3 {micro}C{sub 1}/L to 0.07 {micro}C{sub 1}/L for a series of two, 2-meter long stationary column beds Further reduction to less than 0.02 {micro}C{sub 1}/L, the current drinking water maximum contaminant level (MCL), is projected with additional bed media in series. Tritium can be removed from the loaded beds with a modest temperature increase and the beds can be reused Results of initial tests are presented and a moving bed process for treating large quantities of wastewaters is proposed. The moving bed separation process appears promising to treat existing large quantities of wastewater at various US Department of Energy (DOE) sites. The enriched tritium stream can be grouted for waste disposition. The separations system has also been shown to reduce tritium concentrations in nuclear reactor cooling water to levels that allow reuse. Energy requirements to reconstitute the loading beds and waste disposal costs for this process appear modest.

JEPPSON, D.W.

2000-01-25T23:59:59.000Z

399

Anisotropic membranes for gas separation  

DOE Patents (OSTI)

A gas separation membrane has a dense separating layer about 10,000 Angstroms or less thick and a porous support layer 10 to 400 microns thick that is an integral unit with gradually and continuously decreasing pore size from the base of the support layer to the surface of the thin separating layer and is made from a casting solution comprising ethyl cellulose and ethyl cellulose-based blends, typically greater than 47.5 ethoxyl content ethyl cellulose blended with compatible second polymers, such as nitrocellulose. The polymer content of the casting solution is from about 10% to about 35% by weight of the total solution with up to about 50% of this polymer weight a compatible second polymer to the ethyl cellulose in a volatile solvent such as isopropanol, methylacetate, methanol, ethanol, and acetone. Typical nonsolvents for the casting solutions include water and formamide. The casting solution is cast in air from about zero to 10 seconds to allow the volatile solvent to evaporate and then quenched in a coagulation bath, typically water, at a temperature of 7--25 C and then air dried at ambient temperature, typically 10--30 C. 2 figs.

Gollan, A.Z.

1987-07-21T23:59:59.000Z

400

Anisotropic membranes for gas separation  

DOE Patents (OSTI)

A gas separation membrane has a dense separating layer about 10,000 Angstroms or less thick and a porous support layer 10 to 400 microns thick that is an integral unit with gradually and continuously decreasing pore size from the base of the support layer to the surface of the thin separating layer and is made from a casting solution comprising ethyl cellulose and ethyl cellulose-based blends, typically greater than 47.5 ethoxyl content ethyl cellulose blended with compatible second polymers, such as nitrocellulose. The polymer content of the casting solution is from about 10% to about 35% by weight of the total solution with up to about 50% of this polymer weight a compatible second polymer to the ethyl cellulose in a volatile solvent such as isopropanol, methylacetate, methanol, ethanol, and acetone. Typical nonsolvents for the casting solutions include water and formamide. The casting solution is cast in air from about zero to 10 seconds to allow the volatile solvent to evaporate and then quenched in a coagulation bath, typically water, at a temperature of 7.degree.-25.degree. C. and then air dried at ambient temperature, typically 10.degree.-30.degree. C.

Gollan, Arye Z. (Newton, MA)

1987-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


401

Martian laser surpasses 100,000 zaps  

NLE Websites -- All DOE Office Websites (Extended Search)

Martian laser surpasses 100,000 zaps Martian laser surpasses 100,000 zaps Martian laser surpasses 100,000 zaps ChemCam zaps rocks with a high-powered laser to determine their composition and carries a camera that can survey the Martian landscape. December 5, 2013 This figure is a ChemCam Remote Micro Imager (RMI) image of the target "Ithaca". The image is a mosaic of three separate images taken on Sol 439, with the scale as shown. The image shows the scars from the ten LIBS points labeled from point 1 to point 10. One of the 30 shots at point no. 1 was the 100,000th firing of the ChemCam laser! The distance to the target from the ChemCam telescope at the top of the mast was 4.04 m. The vertical line of ten points taken by ChemCam on Ithaca, starts in a pitted lower coarser grained unit and crosses into a finer grained, smoother, upper unit. The chemical composition appears to be very similar between units. (Image credit: NASA/JPL-Caltech/LANL/CNES/IRAP)

402

X-ray laser  

DOE Patents (OSTI)

An X-ray laser (10) that lases between the K edges of carbon and oxygen, i.e. between 44 and 23 Angstroms, is provided. The laser comprises a silicon (12) and dysprosium (14) foil combination (16) that is driven by two beams (18, 20) of intense line focused (22, 24) optical laser radiation. Ground state nickel-like dysprosium ions (34) are resonantly photo-pumped to their upper X-ray laser state by line emission from hydrogen-like silicon ions (32). The novel X-ray laser should prove especially useful for the microscopy of biological specimens.

Nilsen, Joseph (Livermore, CA)

1991-01-01T23:59:59.000Z

403

Ground-state properties of neutron-rich Mg isotopes  

E-Print Network (OSTI)

We analyze recently-measured total reaction cross sections for 24-38Mg isotopes incident on 12C targets at 240 MeV/nucleon by using the folding model and antisymmetrized molecular dynamics(AMD). The folding model well reproduces the measured reaction cross sections, when the projectile densities are evaluated by the deformed Woods-Saxon (def-WS) model with AMD deformation. Matter radii of 24-38Mg are then deduced from the measured reaction cross sections by ?ne-tuning the parameters of the def-WS model. The deduced matter radii are largely enhanced by nuclear deformation. Fully-microscopic AMD calculations with no free parameter well reproduce the deduced matter radii for 24-36Mg, but still considerably underestimate them for 37,38Mg. The large matter radii suggest that 37,38Mg are candidates for deformed halo nucleus. AMD also reproduces other existing measured ground-state properties (spin-parity, total binding energy, and one-neutron separation energy) of Mg isotopes. Neutron-number (N) dependence of deformation parameter is predicted by AMD. Large deformation is seen from 31Mg with N = 19 to a drip-line nucleus 40Mg with N = 28, indicating that both the N = 20 and 28 magicities disappear. N dependence of neutron skin thickness is also predicted by AMD.

Shin Watanabe; Kosho Minomo; Mitsuhiro Shimada; Shingo Tagami; Masaaki Kimura; Maya Takechi; Mitsunori Fukuda; Daiki Nishimura; Takeshi Suzuki; Takuma Matsumoto; Yoshifumi R. Shimizu; Masanobu Yahiro

2014-04-09T23:59:59.000Z

404

Description of C isotopes within RMF+BCS approach  

SciTech Connect

In the present investigations we have employed relativistic mean-field plus BCS (RMF + BCS) approach to carry out a systematic study for the ground state properties of even-even C Isotopes. One of the prime reason of this study has been to look into the role of low lying states in neutron rich reason near neutron drip line. It is found that irrespective of whether any resonant state exists or not, the occupancy of weakly bound neutron single particle states having low orbital angular momentum, (l = 0 or 1), with a well spread wave function due to the absence or very small strength of centrifugal barrier, helps to cause the occurrence of nuclei with widely extended neutron density. Such nuclei are found to have characteristically very small two-neutron separation energy and large neutron rms radius akin to that observed in weakly bound systems.

Saxena, G. [Department of Physics, Govt. Women Engineering College, Ajmer-305002 (India); Singh, D.; Kaushik, M. [Department of Physics, University of Rajasthan, Jaipur - 302004 (India)

2013-06-03T23:59:59.000Z

405

Ultrafast Laser Facility | Photosynthetic Antenna Research Center  

NLE Websites -- All DOE Office Websites (Extended Search)

Ultrafast Laser Facility Ultrafast Laser Facility Click for an Overview of the Ultrafast Laser Facility The PARC Ultrafast Laser Facility, under the direction of Associate Director...

406

Determination of the theoretical feasibility for the transmutation of europium isotopes from high flux isotope reactor control cylinders  

SciTech Connect

The High Flux Isotope Reactor (HFIR) at the Oak Ridge National Laboratory (ORNL) is a 100 MWth light-water research reactor designed and built in the 1960s primarily for the production of transuranic isotopes. The HFIR is equipped with two concentric cylindrical blade assemblies, known as control cylinders, that are used to control reactor power. These control cylinders, which become highly radioactive from neutron exposure, are periodically replaced as part of the normal operation of the reactor. The highly radioactive region of the control cylinders is composed of europium oxide in an aluminum matrix. The spent HFIR control cylinders have historically been emplaced in the ORNL Waste Area Grouping (WAG) 6. The control cylinders pose a potential radiological hazard due to the long lived radiotoxic europium isotopes {sup 152}Eu, {sup 154}Eu, and {sup 155}Eu. In a 1991 health evaluation of WAG 6 (ERD 1991) it was shown that these cylinders were a major component of the total radioactivity in WAG 6 and posed a potential exposure hazard to the public in some of the postulated assessment scenarios. These health evaluations, though preliminary and conservative in nature, illustrate the incentive to investigate methods for permanent destruction of the europium radionuclides. When the cost of removing the control cylinders from WAG 6, performing chemical separations and irradiating the material in HFIR are factored in, the option of leaving the control cylinders in place for decay must be considered. Other options, such as construction of an engineered barrier around the disposal silos to reduce the chance of migration, should also be analyzed.

Elam, K.R.; Reich, W.J.

1995-09-01T23:59:59.000Z

407

BNL | ATF Laser Safety  

NLE Websites -- All DOE Office Websites (Extended Search)

ATF Laser Safety ATF Laser Safety To be present in a secured laser area at ATF, a person must either have the required laser training, or be continuously escorted by someone who has such training: The training consists of an eye exam, BNL general laser safety lecture, and formal ATF laser familiarization. Untrained personnel should not be instructed to enter interlocked areas or be escorted into an area and left unattended. If someone without training must enter a secured area, they must be continuously escorted, and are considered spectators, which means they may not perform any work in the area. At ATF, there are 3 classes of personnel authorized to enter secured areas: Experimental operators may secure areas, perform approved experiments with beams from facility lasers (YAG + CO2) or FEL beams, and

408

Isotopic composition of Silurian seawater  

SciTech Connect

Direct isotopic analyses of 21 samples of the Silurian hydrosphere preserved as fluid inclusions in Silurian halite deposits in the Michigan Basin Salina Group yield delta/sup 18/O, deltaD ranging from 0.2 to +5.9 and -26 to -73, respectively. delta/sup 18/O has the same range as observed for modern halite facies evaporite waters and is a few per thousand higher than 100 analyses of fluid inclusions in Permian halite. deltaD is about 20 to 30 per thousand lower than modern and Permian examples. The trajectory of evaporating seawater on a deltaD-delta/sup 18/O diagram initially has a positive slope of 3-6, but hooks strongly downward to negative values, the shape of the hook depending upon humidity. Halite begins to precipitate at delta values similar to those observed for the most /sup 18/O rich fluid inclusions. Subsequent evaporation yields progressively more negative delta values as observed for the fluid inclusions. The fluid inclusion data can be readily explained in terms of evaporating seawater and are consistent with the degree of evaporation deduced from measured bromide profiles. These data are strongly inconsistent with arguments that Silurian seawater was 5.5 per thousand depleted in /sup 18/O. delta/sup 18/O for evaporite waters is systematically related to that of seawater, and does not show a -5.5 per thousand shift in the Silurian, even allowing for variables which affect the isotope evaporation trajectory. The lower deltaD may indicate a component of gypsum dehydration waters or may suggest a D-depleted Silurian hydrosphere.

Knauth, L.P.; Kealy, S.; Larimer, S.

1985-01-01T23:59:59.000Z

409

Laser system using ultra-short laser pulses  

DOE Patents (OSTI)

A laser system using ultrashort laser pulses is provided. In another aspect of the present invention, the system includes a laser, pulse shaper and detection device. A further aspect of the present invention employs a femtosecond laser and binary pulse shaping (BPS). Still another aspect of the present invention uses a laser beam pulse, a pulse shaper and a SHG crystal.

Dantus, Marcos (Okemos, MI); Lozovoy, Vadim V. (Okemos, MI); Comstock, Matthew (Milford, MI)

2009-10-27T23:59:59.000Z

410

Quantum statistical effect on ionizing collisions of ultracold metastable Kr isotopes  

Science Journals Connector (OSTI)

Ultracold ionizing collisions of laser-cooled Kr isotopes in the 1s5[4p55s:3P2] metastable state are investigated. When the collision energy is reduced below the p-wave centrifugal barrier of 80 ?K, the ratio of the ionizing collision rate between polarized and unpolarized Kr83 atoms is found to decrease. This is a direct evidence of the quantum interference of two identical Fermi particles. The experimental results are compared with the calculation based on the simplified inelastic collision theory.

Hidetoshi Katori; Hideyuki Kunugita; Tetsuya Ido

1995-12-01T23:59:59.000Z

411

LASER SAFETY POLICY Policy Statement  

E-Print Network (OSTI)

LASER SAFETY POLICY Policy Statement Each department that acquires or operates lasers for use in laboratories or research is responsible for reporting laser acquisition to the Office of Laboratory Safety, selecting a departmental deputy laser safety officer, mandating training for its laser operators

Vertes, Akos

412

OMEGA Extended Performance Laser System  

E-Print Network (OSTI)

at UR-LLE is close to that required for ignition to occur. #12;The OMEGA Extended Performance (EP) laserOMEGA Extended Performance Laser System R. L. McCrory University of Rochester Laboratory for Laser­18 February 2008 #12;OMEGA Extended Performance Laser System R.L. McCrory Laboratory for Laser Energetics

413

Separations and safeguards model integration.  

SciTech Connect

Research and development of advanced reprocessing plant designs can greatly benefit from the development of a reprocessing plant model capable of transient solvent extraction chemistry. This type of model can be used to optimize the operations of a plant as well as the designs for safeguards, security, and safety. Previous work has integrated a transient solvent extraction simulation module, based on the Solvent Extraction Process Having Interaction Solutes (SEPHIS) code developed at Oak Ridge National Laboratory, with the Separations and Safeguards Performance Model (SSPM) developed at Sandia National Laboratory, as a first step toward creating a more versatile design and evaluation tool. The goal of this work was to strengthen the integration by linking more variables between the two codes. The results from this integrated model show expected operational performance through plant transients. Additionally, ORIGEN source term files were integrated into the SSPM to provide concentrations, radioactivity, neutron emission rate, and thermal power data for various spent fuels. This data was used to generate measurement blocks that can determine the radioactivity, neutron emission rate, or thermal power of any stream or vessel in the plant model. This work examined how the code could be expanded to integrate other separation steps and benchmark the results to other data. Recommendations for future work will be presented.

Cipiti, Benjamin B.; Zinaman, Owen

2010-09-01T23:59:59.000Z

414

It's Elemental - Isotopes of the Element Magnesium  

NLE Websites -- All DOE Office Websites (Extended Search)

Sodium Sodium Previous Element (Sodium) The Periodic Table of Elements Next Element (Aluminum) Aluminum Isotopes of the Element Magnesium [Click for Main Data] Most of the isotope data on this site has been obtained from the National Nuclear Data Center. Please visit their site for more information. Naturally Occurring Isotopes Mass Number Natural Abundance Half-life 24 78.99% STABLE 25 10.00% STABLE 26 11.01% STABLE Known Isotopes Mass Number Half-life Decay Mode Branching Percentage 19 4.0 picoseconds Double Proton Emission 100.00% 20 90.8 milliseconds Electron Capture 100.00% Electron Capture with delayed Proton Emission ~ 27.00% 21 122 milliseconds Electron Capture 100.00% Electron Capture with delayed Proton Emission 32.60% Electron Capture with delayed Alpha Decay < 0.50%

415

It's Elemental - Isotopes of the Element Chlorine  

NLE Websites -- All DOE Office Websites (Extended Search)

Sulfur Sulfur Previous Element (Sulfur) The Periodic Table of Elements Next Element (Argon) Argon Isotopes of the Element Chlorine [Click for Main Data] Most of the isotope data on this site has been obtained from the National Nuclear Data Center. Please visit their site for more information. Naturally Occurring Isotopes Mass Number Natural Abundance Half-life 35 75.76% STABLE 37 24.24% STABLE Known Isotopes Mass Number Half-life Decay Mode Branching Percentage 28 No Data Available Proton Emission (suspected) No Data Available 29 < 20 nanoseconds Proton Emission No Data Available 30 < 30 nanoseconds Proton Emission No Data Available 31 150 milliseconds Electron Capture 100.00% Electron Capture with delayed Proton Emission 0.70% 32 298 milliseconds Electron Capture 100.00%

416

It's Elemental - Isotopes of the Element Potassium  

NLE Websites -- All DOE Office Websites (Extended Search)

Argon Argon Previous Element (Argon) The Periodic Table of Elements Next Element (Calcium) Calcium Isotopes of the Element Potassium [Click for Main Data] Most of the isotope data on this site has been obtained from the National Nuclear Data Center. Please visit their site for more information. Naturally Occurring Isotopes Mass Number Natural Abundance Half-life 39 93.2581% STABLE 40 0.0117% 1.248×10+9 years 41 6.7302% STABLE Known Isotopes Mass Number Half-life Decay Mode Branching Percentage 32 No Data Available Proton Emission (suspected) No Data Available 33 < 25 nanoseconds Proton Emission No Data Available 34 < 25 nanoseconds Proton Emission No Data Available 35 178 milliseconds Electron Capture 100.00% Electron Capture with delayed Proton Emission 0.37% 36 342 milliseconds Electron Capture 100.00%

417

It's Elemental - Isotopes of the Element Phosphorus  

NLE Websites -- All DOE Office Websites (Extended Search)

Silicon Silicon Previous Element (Silicon) The Periodic Table of Elements Next Element (Sulfur) Sulfur Isotopes of the Element Phosphorus [Click for Main Data] Most of the isotope data on this site has been obtained from the National Nuclear Data Center. Please visit their site for more information. Naturally Occurring Isotopes Mass Number Natural Abundance Half-life 31 100% STABLE Known Isotopes Mass Number Half-life Decay Mode Branching Percentage 24 No Data Available Electron Capture (suspected) No Data Available Proton Emission (suspected) No Data Available 25 < 30 nanoseconds Proton Emission 100.00% 26 43.7 milliseconds Electron Capture 100.00% Electron Capture with delayed Proton Emission No Data Available 27 260 milliseconds Electron Capture 100.00% Electron Capture with

418

It's Elemental - Isotopes of the Element Oxygen  

NLE Websites -- All DOE Office Websites (Extended Search)

Nitrogen Nitrogen Previous Element (Nitrogen) The Periodic Table of Elements Next Element (Fluorine) Fluorine Isotopes of the Element Oxygen [Click for Main Data] Most of the isotope data on this site has been obtained from the National Nuclear Data Center. Please visit their site for more information. Naturally Occurring Isotopes Mass Number Natural Abundance Half-life 16 99.757% STABLE 17 0.038% STABLE 18 0.205% STABLE Known Isotopes Mass Number Half-life Decay Mode Branching Percentage 12 1.139×10-21 seconds Proton Emission No Data Available 13 8.58 milliseconds Electron Capture 100.00% Electron Capture with delayed Proton Emission 100.00% 14 70.620 seconds Electron Capture 100.00% 15 122.24 seconds Electron Capture 100.00% 16 STABLE - - 17 STABLE - - 18 STABLE - - 19 26.88 seconds Beta-minus Decay 100.00%

419

It's Elemental - Isotopes of the Element Gallium  

NLE Websites -- All DOE Office Websites (Extended Search)

Zinc Zinc Previous Element (Zinc) The Periodic Table of Elements Next Element (Germanium) Germanium Isotopes of the Element Gallium [Click for Main Data] Most of the isotope data on this site has been obtained from the National Nuclear Data Center. Please visit their site for more information. Naturally Occurring Isotopes Mass Number Natural Abundance Half-life 69 60.108% STABLE 71 39.892% STABLE Known Isotopes Mass Number Half-life Decay Mode Branching Percentage 56 No Data Available Proton Emission (suspected) No Data Available 57 No Data Available Proton Emission (suspected) No Data Available 58 No Data Available Proton Emission (suspected) No Data Available 59 No Data Available Proton Emission (suspected) No Data Available 60 70 milliseconds Electron Capture 98.40%

420

It's Elemental - Isotopes of the Element Sodium  

NLE Websites -- All DOE Office Websites (Extended Search)

Neon Neon Previous Element (Neon) The Periodic Table of Elements Next Element (Magnesium) Magnesium Isotopes of the Element Sodium [Click for Main Data] Most of the isotope data on this site has been obtained from the National Nuclear Data Center. Please visit their site for more information. Naturally Occurring Isotopes Mass Number Natural Abundance Half-life 23 100% STABLE Known Isotopes Mass Number Half-life Decay Mode Branching Percentage 18 1.3×10-21 seconds Proton Emission 100.00% 19 < 40 nanoseconds Proton Emission No Data Available 20 447.9 milliseconds Electron Capture with delayed Alpha Decay 20.05% Electron Capture 100.00% 21 22.49 seconds Electron Capture 100.00% 22 2.6027 years Electron Capture 100.00% 23 STABLE - - 24 14.997 hours Beta-minus Decay 100.00%

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


421

It's Elemental - Isotopes of the Element Neon  

NLE Websites -- All DOE Office Websites (Extended Search)

Fluorine Fluorine Previous Element (Fluorine) The Periodic Table of Elements Next Element (Sodium) Sodium Isotopes of the Element Neon [Click for Main Data] Most of the isotope data on this site has been obtained from the National Nuclear Data Center. Please visit their site for more information. Naturally Occurring Isotopes Mass Number Natural Abundance Half-life 20 90.48% STABLE 21 0.27% STABLE 22 9.25% STABLE Known Isotopes Mass Number Half-life Decay Mode Branching Percentage 16 9×10-21 seconds Double Proton Emission 100.00% 17 109.2 milliseconds Electron Capture with delayed Alpha Decay No Data Available Electron Capture 100.00% Electron Capture with delayed Proton Emission 100.00% 18 1.6670 seconds Electron Capture 100.00% 19 17.22 seconds Electron Capture 100.00% 20 STABLE - -

422

It's Elemental - Isotopes of the Element Copper  

NLE Websites -- All DOE Office Websites (Extended Search)

Nickel Nickel Previous Element (Nickel) The Periodic Table of Elements Next Element (Zinc) Zinc Isotopes of the Element Copper [Click for Main Data] Most of the isotope data on this site has been obtained from the National Nuclear Data Center. Please visit their site for more information. Naturally Occurring Isotopes Mass Number Natural Abundance Half-life 63 69.15% STABLE 65 30.85% STABLE Known Isotopes Mass Number Half-life Decay Mode Branching Percentage 52 No Data Available Proton Emission No Data Available 53 < 300 nanoseconds Electron Capture No Data Available Proton Emission No Data Available 54 < 75 nanoseconds Proton Emission No Data Available 55 27 milliseconds Electron Capture 100.00% Electron Capture with delayed Proton Emission 15.0% 56 93 milliseconds Electron Capture 100.00%

423

It's Elemental - Isotopes of the Element Boron  

NLE Websites -- All DOE Office Websites (Extended Search)

Beryllium Beryllium Previous Element (Beryllium) The Periodic Table of Elements Next Element (Carbon) Carbon Isotopes of the Element Boron [Click for Main Data] Most of the isotope data on this site has been obtained from the National Nuclear Data Center. Please visit their site for more information. Naturally Occurring Isotopes Mass Number Natural Abundance Half-life 10 19.9% STABLE 11 80.1% STABLE Known Isotopes Mass Number Half-life Decay Mode Branching Percentage 6 No Data Available Double Proton Emission (suspected) No Data Available 7 3.255×10-22 seconds Proton Emission No Data Available Alpha Decay No Data Available 8 770 milliseconds Electron Capture 100.00% Electron Capture with delayed Alpha Decay 100.00% 9 8.439×10-19 seconds Proton Emission 100.00% Double Alpha Decay 100.00%

424

It's Elemental - Isotopes of the Element Tungsten  

NLE Websites -- All DOE Office Websites (Extended Search)

Tantalum Tantalum Previous Element (Tantalum) The Periodic Table of Elements Next Element (Rhenium) Rhenium Isotopes of the Element Tungsten [Click for Main Data] Most of the isotope data on this site has been obtained from the National Nuclear Data Center. Please visit their site for more information. Naturally Occurring Isotopes Mass Number Natural Abundance Half-life 180 0.12% >= 6.6×10+17 years 182 26.50% STABLE 183 14.31% > 1.3×10+19 years 184 30.64% STABLE 186 28.43% > 2.3×10+19 years Known Isotopes Mass Number Half-life Decay Mode Branching Percentage 157 275 milliseconds Electron Capture No Data Available 158 1.25 milliseconds Alpha Decay 100.00% 158m 0.143 milliseconds Isomeric Transition No Data Available Alpha Decay No Data Available 159 7.3 milliseconds Alpha Decay ~ 99.90%

425

It's Elemental - Isotopes of the Element Carbon  

NLE Websites -- All DOE Office Websites (Extended Search)

Boron Boron Previous Element (Boron) The Periodic Table of Elements Next Element (Nitrogen) Nitrogen Isotopes of the Element Carbon [Click for Main Data] Most of the isotope data on this site has been obtained from the National Nuclear Data Center. Please visit their site for more information. Naturally Occurring Isotopes Mass Number Natural Abundance Half-life 12 98.93% STABLE 13 1.07% STABLE Known Isotopes Mass Number Half-life Decay Mode Branching Percentage 8 1.981×10-21 seconds Proton Emission 100.00% Alpha Decay No Data Available 9 126.5 milliseconds Electron Capture 100.00% Electron Capture with delayed Proton Emission 61.60% Electron Capture with delayed Alpha Decay 38.40% 10 19.308 seconds Electron Capture 100.00% 11 20.334 minutes Electron Capture 100.00% 12 STABLE - -

426

It's Elemental - Isotopes of the Element Rhenium  

NLE Websites -- All DOE Office Websites (Extended Search)

Tungsten Tungsten Previous Element (Tungsten) The Periodic Table of Elements Next Element (Osmium) Osmium Isotopes of the Element Rhenium [Click for Main Data] Most of the isotope data on this site has been obtained from the National Nuclear Data Center. Please visit their site for more information. Naturally Occurring Isotopes Mass Number Natural Abundance Half-life 185 37.40% STABLE 187 62.60% 4.33×10+10 years Known Isotopes Mass Number Half-life Decay Mode Branching Percentage 159 No Data Available No Data Available No Data Available 160 0.82 milliseconds Proton Emission 91.00% Alpha Decay 9.00% 161 0.44 milliseconds Proton Emission 100.00% Alpha Decay <= 1.40% 161m 14.7 milliseconds Alpha Decay 93.00% Proton Emission 7.00% 162 107 milliseconds Alpha Decay 94.00% Electron Capture 6.00%

427

Isotope ratio determination in boron analysis  

Science Journals Connector (OSTI)

Traditionally, boron (B) isotope ratios have been determined using thermal ionization...+, Cs+, or O-...for analyte ionization. TIMS can be used in negative or positive ion modes with high sensitivity and precisi...

Ram N. Sah; Patrick H. Brown

1998-12-01T23:59:59.000Z

428

Magnetic moments of long isotopic chains  

E-Print Network (OSTI)

Dipole magnetic moments of several long isotopic chains are analyzed within the self-consistent Finite Fermi System theory based on the Generalized Energy Density Functional method with exact account for the pairing and quasi-particle continuum. New data for nuclei far from the beta-stability valley are included in the analysis. For a number of semi-magic isotopes of the tin and lead chains a good description of the data is obtained, with accuracy of 0.1 - 0.2 mu_N. A chain of non-magic isotopes of copper is also analyzed in detail. It is found that the systematic analysis of magnetic moments of this long chain yields rich information on the evolution of the nuclear structure of the Cu isotopes. In particular, it may give a signal of deformation for the ground state of some nuclei in the chain.

I. N. Borzov; E. E. Saperstein; S. V. Tolokonnikov; G. Neyens; N. Severijns

2008-04-28T23:59:59.000Z

429

ICE CORE RECORDS | Greenland Stable Isotopes  

Science Journals Connector (OSTI)

Abstract Greenland ice cores contain a wealth of information on past climatic conditions throughout the Northern Hemisphere. A historical perspective on the climatic interpretation of stable isotopes in water and ice is presented in the introduction, while the remainder of the article is devoted to the current interpretation of stable isotope data from Greenland ice cores. The progress in our understanding of stable isotope signals, on timescales from seasons to glacial cycles, is discussed and evaluated through numerous examples from Greenland ice cores. Stable isotope profiles from the Camp Century, Dye-3, GISP2, GRIP, NGRIP, and Renland deep ice cores are emphasized, as they all provide climatic information dating back into the Eemian period.

B.M. Vinther; S.J. Johnsen

2013-01-01T23:59:59.000Z

430

Nuclear Astrophysics in Rare Isotope Facilities  

E-Print Network (OSTI)

Nuclear reactions in stars are difficult to measure directly in the laboratory at the small astrophysical energies. In recent years indirect methods with rare isotopes have been developed and applied to extract low-energy astrophysical cross sections.

C. A. Bertulani

2009-11-02T23:59:59.000Z

431

NONRADIOGENIC ISOTOPES IN GEOLOGY: A REVIEW  

Science Journals Connector (OSTI)

...has revised Brown's figures. Seaborg and Pearlman (1948) and more recently...51, p. 263-300. and Jenks, Glenn (1944) Isotopic composition of...Science,vol. 79, p. 565. Seaborg, Glenn T., and Pearlman, I. (1948...

432

Storage of Hydrogen Isotopes in Uranium Alloys  

Science Journals Connector (OSTI)

Tritium Properties and Interactions with Material / Proceedings of the Third Topical Meeting on Tritium Technology in Fission, Fusion and Isotopic Applications (Toronto, Ontario, Canada, May 1-6, 1988)

T. Yamamoto; Supardjo; T. Terai; F. Ono; S. Tanaka; M. Yamawaki

433

Norman Ramsey and the Separated Oscillatory Fields Method  

Office of Scientific and Technical Information (OSTI)

Norman Ramsey and the Norman Ramsey and the Separated Oscillatory Fields Method Resources with Additional Information Norman F. Ramsey Photo Credit: Courtesy of Fermilab Norman F. Ramsey was born in Washington, D.C. and 'was educated in the United States and England; he earned five degrees in physics including the Ph.D. (Columbia 1940) and the D.Sc. (Cambridge, 1964). Ramsey's scientific research focused on the properties of molecules, atoms, nuclei and elementary particles and includes key contributions to the knowledge of magnetic moments, the structural shape of nuclear particles, the nature of nuclear forces, the thermodynamics of energized populations of atoms and molecules (e.g. those in masers and lasers) and spectroscopy. Ramsey not only contributed basic advances in the theoretical understanding of the physics involved in his research, he also made pioneering advances in the methods of investigation; in particular, he contributed many refinements of the molecular beam method for the study of atomic and molecular properties, he invented the separated oscillatory field method of exciting resonances and, with the collaboration of his students, he was the principal inventor of the atomic hydrogen maser. The separated oscillatory field method provides extremely high resolution in atomic and molecular spectroscopy and it is the practical basis for the most precise atomic clocks; likewise the atomic hydrogen maser made even higher levels of spectroscopic resolution possible and it also functions as the basis for atomic clocks having the highest levels of stability for periods extending to several hours.'1

434

Laser-Induced Damage in DKDP Crystals under Simultaneous Exposure to Laser Harmonics  

SciTech Connect

While KDP and DKDP crystals remain the only viable solution for frequency conversion in large aperture laser systems in the foreseeable future, our understanding of damage behavior in the presence of multiple colors is very limited. Such conditions exist during normal operation where, for third harmonic generation, 1{omega}, 2{omega} and 3{omega} components are present with different energy ratios as they propagate inside the crystal. The objective of this work is to shed light into the damage behavior of frequency conversion crystals during operational conditions as well as probe the fundamental mechanisms of damage initiation. We have performed a series of experiments to quantify the damage performance of pristine (unconditioned) DKDP material under simultaneous exposure to 2{omega} and 3{omega} laser pulses from a 3-ns Nd:YAG laser system as a function of the laser influences at each frequency. Results show that simultaneous dual wavelength exposure leads to a much larger damage density as compared to the total damage resulting from separate exposure at each wavelength. Furthermore, under such excitation conditions, the damage performance is directly related to and can be predicted from the damage behavior of the crystal at each wavelength separately while the mechanism and type of defects responsible for damage initiation are shown to be the same at both 2{omega} and 3{omega} excitation.

Negres, R A; DeMange, P; Radousky, H B; Demos, S G

2005-10-28T23:59:59.000Z

435

Laser Safety Inspection Criteria  

SciTech Connect

A responsibility of the Laser Safety Officer (LSO) is to perform laser safety audits. The American National Standard Z136.1 Safe use of Lasers references this requirement in several sections: (1) Section 1.3.2 LSO Specific Responsibilities states under Hazard Evaluation, ''The LSO shall be responsible for hazards evaluation of laser work areas''; (2) Section 1.3.2.8, Safety Features Audits, ''The LSO shall ensure that the safety features of the laser installation facilities and laser equipment are audited periodically to assure proper operation''; and (3) Appendix D, under Survey and Inspections, it states, ''the LSO will survey by inspection, as considered necessary, all areas where laser equipment is used''. Therefore, for facilities using Class 3B and or Class 4 lasers, audits for laser safety compliance are expected to be conducted. The composition, frequency and rigueur of that inspection/audit rests in the hands of the LSO. A common practice for institutions is to develop laser audit checklists or survey forms. In many institutions, a sole Laser Safety Officer (LSO) or a number of Deputy LSO's perform these audits. For that matter, there are institutions that request users to perform a self-assessment audit. Many items on the common audit list and the associated findings are subjective because they are based on the experience and interest of the LSO or auditor in particular items on the checklist. Beam block usage is an example; to one set of eyes a particular arrangement might be completely adequate, while to another the installation may be inadequate. In order to provide more consistency, the National Ignition Facility Directorate at Lawrence Livermore National Laboratory (NIF-LLNL) has established criteria for a number of items found on the typical laser safety audit form. These criteria are distributed to laser users, and they serve two broad purposes: first, it gives the user an expectation of what will be reviewed by an auditor, and second, it is an opportunity to explain audit items to the laser user and thus the reasons for some of these items. Some examples are given from the audit criteria handout. As an explanatory key to the reader, an Operational Safety Procedure (OSP) as a formally reviewed safety procedure required for all Class 3B and Class 4 laser installations. An ''OSP Binder'' contains all safety documentation related to a given laser operation and serves as a central repository for documents, such as the OSP, interlock logs, lessons learned, contact information etc. ''Unattended Operation'' refers to approved procedures for unattended operation of the laser installation and may include operation beyond normal working hours. ''L-train'' is the LLNL training tracking system.

Barat, K

2005-02-11T23:59:59.000Z

436

Mechanistic studies using kinetic isotope effects  

E-Print Network (OSTI)

MECHANISTIC STUDIES USING KINETIC ISOTOPE EFFECTS A Thesis by BRIAN E. SCHULMFIER Submitted to the Office of Graduate Studies of Texas ARM University in partial fulfillment of the requtrements for the degree of MASTER OF SCIENCE December... 1999 Major Subject: Chemistry MECHANISTIC STUDIES USING KINETIC ISOTOPE EFFECTS A Thesis by BRIAN E. SCHULMEIER Submitted to Texas A&M University in partial fulfillment of the requirements for the degree of MASTER OF SCIENCE Approved...

Schulmeier, Brian E.

2012-06-07T23:59:59.000Z

437

Isotope/element fractionation during surface adsorption  

Science Journals Connector (OSTI)

The adsorption of ions onto mineral surfaces accompanies isotope/element fractionation in planets and asteroids. A model based on simple classical physics is presented to predict these fractionations. The agreement between the experimentally observed isotope/element ratios and their predicted values is found to be excellent. This fractionation can be demonstrated experimentally in advanced physics laboratories using macroscopic particles. The success of the model shows students that even a very complex naturally occurring process can be explained quantitatively with simple physics.

Gamini Seneviratne; Asiri Nanayakkara

2004-01-01T23:59:59.000Z

438

Manifestation and Origin of the Isotope Effect  

E-Print Network (OSTI)

This article reviews from one point of view the current status of the manifestations of isotope effect in a nuclear, atomic and molecular as well as solid state physics. Although these manifestations vary, they have one common feature - they all depend on mass. At present time the Standard Model can't explain the origin of the mass of elementary particles and their hierarchy. The last one don't permit to find the origin of the isotope effect.

V. G. Plekhanov

2009-07-12T23:59:59.000Z

439

The Oxygen core inside the Magnesium isotopes  

E-Print Network (OSTI)

We have studied the ground state bulk properties of magnesium isotopes using axially symmetric relativistic mean field formalism. The BCS pairing approach is employed to take care of the pairing correlation for the open shell nuclei. The contour plot of the nucleons distribution are analyzed at various parts of the nucleus, where clusters are located. The presence of an $^{16}$O core along bubble like $\\alpha$-particle(s) and few {\\it nucleons} are found in the Mg isotopes.

Bhuyan, M

2013-01-01T23:59:59.000Z

440

Laser-PlasmaWakefield Acceleration with Higher Order Laser Modes  

E-Print Network (OSTI)

Design considerations for a laser-plasma linear collider,"E.Esarey, and W.P.Leemans, "Free-electron laser driven bythe LBNL laser-plasma accelerator," in Proc. Adv. Acc. Con.

Geddes, C.G.R.

2011-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


441

Laser induced nuclear reactions  

SciTech Connect

Dramatic improvements in laser technology since 1984 have revolutionised high power laser technology. Application of chirped-pulse amplification techniques has resulted in laser intensities in excess of 10{sup 19} W/cm{sup 2}. In the mid to late eighties, C. K. Rhodes and K. Boyer discussed the possibility of shining laser light of this intensity onto solid surfaces and to cause nuclear transitions. In particular, irradiation of a uranium target could induce electro- and photofission in the focal region of the laser. In this paper it is shown that {mu}Ci of {sup 62}Cu can be generated via the ({gamma},n) reaction by a laser with an intensity of about 10{sup 19} Wcm{sup -2}.

Ledingham, Ken; McCanny, Tom; Graham, Paul; Fang Xiao; Singhal, Ravi; Magill, Joe; Creswell, Alan; Sanderson, David; Allott, Ric; Neely, David; Norreys, Peter; Santala, Marko; Zepf, Matthew; Watts, Ian; Clark, Eugene; Krushelnick, Karl; Tatarakis, Michael; Dangor, Bucker; Machecek, Antonin; Wark, Justin [Department of Physics and Astronomy, University of Glasgow, Glasgow G12 8QQ, Scotland (United Kingdom); European Commission, Institute for Transuranic Elements, Karlsruhe, Postfach 2340, D-76125 (Germany); Scottish Universities Research and Reactor Centre, East Kilbride, Glasgow G75 0QU (United Kingdom); Rutherford Appleton Laboratory, Chilton, Didcot (United Kingdom); Blackett Laboratory, Imperial College, London SW7 2BZ (United Kingdom); Clarendon Laboratory, Department of Physics, University of Oxford, OX1 3PU (United Kingdom)

1998-12-16T23:59:59.000Z

442

Production of exotic, short lived carbon isotopes in ISOL-type facilities  

E-Print Network (OSTI)

The beam intensities of short-lived carbon isotopes at Isotope Separation On-Line (ISOL) facilities have been limited in the past for technical reasons. The production of radioactive ion beams of carbon isotopes is currently of high interest for fundamental nuclear physics research. To produce radioactive ions a target station consisting of a target in a container connected to an ion source via a transfer line is commonly used. The target is heated to vaporize the product for transport. Carbon in elementary form is a very reactive element and react strongly with hot metal surfaces. Due to the strong chemisorption interaction, in the target and ion source unit, the atoms undergo significant retention on their way from the target to the ion source. Due to this the short lived isotopes decays and are lost leading to low ion yields. A first approach to tackle these limitations consists of incorporating the carbon atoms into less reactive molecules and to use materials for the target housing and the transfer line ...

Franberg, Hanna; Köster, Ulli; Ammann, Markus

2008-01-01T23:59:59.000Z

443

Production yields of noble-gas isotopes from ISOLDE UC$_{x}$/graphite targets  

E-Print Network (OSTI)

Yields of He, Ne, Ar, Kr and Xe isotopic chains were measured from UC$_{x}$/graphite and ThC$_{x}$/graphite targets at the PSB-ISOLDE facility at CERN using isobaric selectivity achieved by the combination of a plasma-discharge ion source with a water-cooled transfer line. %The measured half-lives allowed %to calculate the decay losses of neutron-rich isotopes in the %target and ion-source system, and thus to obtain information on the in-target %productions from the measured yields. The delay times measured for a UC$_x$/graphite target allow for an extrapolation to the expected yields of very neutron-rich noble gas isotopes, in particular for the ``NuPECC reference elements'' Ar and Kr, at the next-generation radioactive ion-beam facility EURISOL. \\end{abstract} \\begin{keyword} % keywords here, in the form: keyword \\sep keyword radioactive ion beams \\sep release \\sep ion yields \\sep ISOL (Isotope Separation On-Line) \\sep uranium and thorium carbide targets. % PACS codes here, in the form: \\PACS code \\sep code...

Bergmann, U C; Catherall, R; Cederkäll, J; Diget, C A; Fraile-Prieto, L M; Franchoo, S; Fynbo, H O U; Gausemel, H; Georg, U; Giles, T; Hagebø, E; Jeppesen, H B; Jonsson, O C; Köster, U; Lettry, Jacques; Nilsson, T; Peräjärvi, K; Ravn, H L; Riisager, K; Weissman, L; Äystö, J

2003-01-01T23:59:59.000Z

444

NEWGOOGIN2  

NLE Websites -- All DOE Office Websites (Extended Search)

a senior consultant to the Gaseous Diffu- sion Plants, was a senior investigator in the Gas Centrifuge Program, an advisor to the early Plasma Separation and Laser Isotope...

445

Polarization feedback laser stabilization  

DOE Patents (OSTI)

A system for locking two Nd:YAG laser oscillators includes an optical path for feeding the output of one laser into the other with different polarizations. Elliptical polarization is incorporated into the optical path so that the change in polarization that occurs when the frequencies coincide may be detected to provide a feedback signal to control one laser relative to the other. 4 figs.

Esherick, P.; Owyoung, A.

1987-09-28T23:59:59.000Z

446

RFNC-VNIIEF Capabilities to Production High Pure Isotopes for Scientific and Medical Applications  

SciTech Connect

In the technical paper there is presented the information on the basic equipment and more than thirty-year experience of RFNC-VNIIEF activities in the sphere of producing highly enriched isotopes of actinide elements--thorium, uranium, neptunium, plutonium, americium and curium--for scientific researches and practical applications. Electromagnetic separator and radiochemical methods provide obtaining of superpure isotope samples for nuclear-physical radiometric and mass-spectrometric equipment, and also as tracers when analyzing environmental contamination. There are presented the structure of the laboratory occupied with these isotopes electromagnetic separation as well as the nomenclature and characteristics of the specimens supplied. There are stated science and engineering elaborations of technologies aimed at producing alpha-ray radiating radionuclides--thorium-229, thorium-228, actinium-225, radium-224--for the purpose of anti-cancer therapy using bismuth-212 and bismuth-213 produced by the specially developed generators. There are presented the basic directions of cooperation with other Russian Institutes in developing this promising line of conversion.

Vesnovskii, S. P.

2002-02-26T23:59:59.000Z

447

Method and apparatus for producing durationally short ultraviolet or x-ray laser pulses  

DOE Patents (OSTI)

A method and apparatus is disclosed for producing ultraviolet or x- ray laser pulses of short duration. An ultraviolet or x-ray laser pulse of long duration is progressively refracted, across the surface of an opaque barrier, by a streaming plasma that is produced by illuminating a solid target with a pulse of conventional line focused high power laser radiation. The short pulse of ultraviolet or x-ray laser radiation, which may be amplified to high power, is separated out by passage through a slit aperture in the opaque barrier.

MacGowan, B.J.; Matthews, D.L.; Trebes, J.E.

1987-05-05T23:59:59.000Z

448

Method and apparatus for producing durationally short ultraviolet or X-ray laser pulses  

DOE Patents (OSTI)

A method and apparatus is disclosed for producing ultraviolet or X-ray laser pulses of short duration (32). An ultraviolet or X-ray laser pulse of long duration (12) is progressively refracted, across the surface of an opaque barrier (28), by a streaming plasma (22) that is produced by illuminating a solid target (16, 18) with a pulse of conventional line focused high power laser radiation (20). The short pulse of ultraviolet or X-ray laser radiation (32), which may be amplified to high power (40, 42), is separated out by passage through a slit aperture (30) in the opaque barrier (28).

MacGowan, Brian J. (Livermore, CA); Matthews, Dennis L. (El Granada, CA); Trebes, James E. (Livermore, CA)

1988-01-01T23:59:59.000Z

449

Terahertz Quantum Cascade Lasers  

Science Journals Connector (OSTI)

We provide an overview of terahertz quantum cascade lasers based on resonant-phonon depopulation and metal-metal waveguides, including two-phonon resonant-phonon depopulation...

Williams, Benjamin; Kumar, Sushil; Qin, Qi; Lee, Alan Wei Min; Hu, Qing; Reno, John L; Wasilewski, Z R; Liu, H C

450

OMEGA EP Laser Dedication Movie - Laboratory for Laser Energetics  

NLE Websites -- All DOE Office Websites (Extended Search)

Dedication Movie - Laboratory for Laser Energetics Laboratory for Laser Energetics Logo Search Home Around the Lab Past Issues Past Quick Shots About Office of the Director Map to...

451

Chirped Laser Dispersion Spectroscopy with Directly Modulated Quantum Cascade Laser  

Science Journals Connector (OSTI)

A feasibility study of chirped laser dispersion spectroscopy (CLaDS) with utilizing direct modulation of a quantum cascade laser instead of external modulators is presented....

Hangauer, Andreas; Spinner, Georg; Nikodem, Michal; Wysocki, Gerard

452

Documentation - Laboratory for Laser Energetics  

NLE Websites -- All DOE Office Websites (Extended Search)

Daily Securing Checklist (S-AB-P-482) EP Bay and OAA Securing Walkthrough (S-AB-P-582) Laser StartupShutdown LOTF Laser Startup (S-AB-P-038) LOTF Laser Shutdown (S-AB-P-039) IRAT...

453

Guidelines For Developing Low Energy Separation Processes  

E-Print Network (OSTI)

A large portion of the energy required by the process industry is consumed by separation processes. This paper discusses current engineering techniques that can be used in the development and optimization of low energy separation processes....

Bojnowski, J. H.; Hanks, D. L.

1981-01-01T23:59:59.000Z

454

Separation of magnetic field lines  

SciTech Connect

The field lines of magnetic fields that depend on three spatial coordinates are shown to have a fundamentally different behavior from those that depend on two coordinates. Unlike two-coordinate cases, a flux tube in a magnetic field that depends on all three spatial coordinates that has a circular cross section at one location along the tube characteristically has a highly distorted cross section at other locations. In an ideal evolution of a magnetic field, the current densities typically increase. Crudely stated, if the current densities increase by a factor {sigma}, the ratio of the long to the short distance across a cross section of a flux tube characteristically increases by e{sup 2{sigma}}, and the ratio of the longer distance to the initial radius increases as e{sup {sigma}}. Electron inertia prevents a plasma from isolating two magnetic field structures on a distance scale shorter than c/{omega}{sub pe}, which is about 10 cm in the solar corona, and reconnection must be triggered if {sigma} becomes sufficiently large. The radius of the sun, R{sub Circled-Dot-Operator }=7 Multiplication-Sign 10{sup 10}cm is about e{sup 23} times larger, so when {sigma} Greater-Than-Or-Equivalent-To 23, two lines separated by c/{omega}{sub pe} at one location can be separated by the full scale of any magnetic structures in the corona at another. The conditions for achieving a large exponentiation, {sigma}, are derived, and the importance of exponentiation is discussed.

Boozer, Allen H. [Department of Applied Physics and Applied Mathematics, Columbia University, New York, New York 10027 (United States)

2012-11-15T23:59:59.000Z

455

E-Print Network 3.0 - abundance isotopic Sample Search Results  

NLE Websites -- All DOE Office Websites (Extended Search)

Search Sample search results for: abundance isotopic Page: << < 1 2 3 4 5 > >> 1 ISOTOPE FRACTIONATION Isotopes are atoms whose nuclei contain the same number of protons but...

456

E-Print Network 3.0 - alpha-deuterium isotope effects Sample...  

NLE Websites -- All DOE Office Websites (Extended Search)

deuterium isotope effects Search Powered by Explorit Topic List Advanced Search Sample search results for: alpha-deuterium isotope effects Page: << < 1 2 3 4 5 > >> 1 ISOTOPE...

457

Strontium and carbon isotope stratigraphy of the Llandovery (Early Silurian): Implications for tectonics and weathering  

E-Print Network (OSTI)

Strontium and carbon isotope stratigraphy of the Llandovery (Early Silurian): Implications online 2 June 2010 Keywords: Silurian Strontium isotopes Carbon isotopes Weathering K-bentonites A high

Saltzman, Matthew R.

458

Isotope Program Facilities | U.S. DOE Office of Science (SC)  

Office of Science (SC) Website

include the High Flux Isotope Reactor at Oak Ridge National Laboratory and the Advanced Test Reactor at Idaho National Laboratory. The DOE Isotope Program also supports isotope...

459

Oxygen isotope fractionation in the vacuum ultraviolet photodissociation of carbon monoxide: Wavelength, pressure and temperature dependency.  

E-Print Network (OSTI)

Oxygen isotope fractionation in the vacuum ultravioletmeasurement of the associated oxygen isotopic composition ofwavelength dependency of the oxygen isotopic composition in

Chakraborty, Subrata

2013-01-01T23:59:59.000Z

460

Separable Representation of Phenomenological Optical Potentials of Woods-Saxon Type  

E-Print Network (OSTI)

Background: One important ingredient for many applications of nuclear physics to astrophysics, nuclear energy, and stockpile stewardship are cross sections for reactions of neutrons with rare isotopes. Since direct measurements are often not feasible, indirect methods, e.g. (d,p) reactions, should be used.} Those (d,p) reactions may be viewed as three-body reactions and described with Faddeev techniques. Purpose: Faddeev equations in momentum space have a long tradition of utilizing separable interactions in order to arrive at sets of coupled integral equations in one variable. While there exist several separable representations for the nucleon-nucleon interaction, the optical potential between a neutron (proton) and a nucleus is not readily available in separable form. The purpose of this paper is to introduce a separable representation for complex phenomenological optical potentials of Woods-Saxon type. Results: Starting from a global optical potential, a separable representation thereof is introduced based on the Ernst-Shakin-Thaler (EST) scheme. This scheme is generalized to non-hermitian potentials. Applications to n$+^{48}$Ca, n$+^{132}$Sn and n$+^{208}$Pb are investigated for energies from 0 to 50 MeV and the quality of the representation is examined. Conclusions: We find a good description of the on-shell t-matrix for all systems with rank up to 5. The required rank depends inversely on the angular momentum. The resulting separable interaction exhibits a different off-shell behavior compared to the original potential, reducing the high momentum contributions.

L. Hlophe; Ch. Elster; R. C. Johnson; N. J. Upadhyay; F. M. Nunes; G. Arbanas; V. Eremenko; J. E. Escher; I. J. Thompson

2013-10-30T23:59:59.000Z

Note: This page contains sample records for the topic "laser isotope separation" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


461

Composition analysis by scanning femtosecond laser ultraprobing (CASFLU).  

DOE Patents (OSTI)

The composition analysis by scanning femtosecond ultraprobing (CASFLU) technology scans a focused train of extremely short-duration, very intense laser pulses across a sample. The partially-ionized plasma ablated by each pulse is spectrometrically analyzed in real time, determining the ablated material's composition. The steering of the scanned beam thus is computer directed to either continue ablative material-removal at the same site or to successively remove nearby material for the same type of composition analysis. This invention has utility in high-speed chemical-elemental, molecular-fragment and isotopic analyses of the microstructure composition of complex objects, e.g., the oxygen isotopic compositions of large populations of single osteons in bone.

Ishikawa, Muriel Y. (Livermore, CA); Wood, Lowell L. (Simi Valley, CA); Campbell, E. Michael (Danveille, CA); Stuart, Brent C. (Livermore, CA); Perry, Michael D. (Livermore, CA)

2002-01-01T23:59:59.000Z

462

Device for hydrogen separation and method  

DOE Patents (OSTI)

A device for hydrogen separation has a porous support and hydrogen separation material on the support. The support is prepared by heat treatment of metal microparticles, preferably of iron-based or nickel-based alloys that also include aluminum and/or yttrium. The hydrogen separation material is then deposited on the support. Preferred hydrogen separation materials include metals such as palladium, alloys, platinum, refractory metals, and alloys.

Paglieri, Stephen N. (White Rock, NM); Anderson, Iver E. (Ames, IA); Terpstra, Robert L. (Ames, IA)

2009-11-03T23:59:59.000Z

463

GEOMETRIC SOURCE SEPARATION: MERGING CONVOLUTIVE SOURCE  

E-Print Network (OSTI)

adaptive beamforming algorithms by a cross-power criteria, we gain new geometric source separation with convo- lutive blind source separation. We concentrate on cross-power spectral min- imization which is su to ambiguities in the choice of separating lters. There are in theory multiple lters that invert the room

Parra, Lucas C.

464

Final Report, NEAC Subcommittee for Isotope Research & Production Planning  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

Final Report, NEAC Subcommittee for Isotope Research & Production Final Report, NEAC Subcommittee for Isotope Research & Production Planning Final Report, NEAC Subcommittee for Isotope Research & Production Planning Isotopes, including both radioactive and stable isotopes, make important contributions to research, medicine, and industry in the United States and throughout the world. For nearly fifty years, the Department of Energy (DOE) has actively promoted the use of isotopes by funding (a) production of isotopes at a number of national laboratories with unique nuclear reactors or particle accelerators, (b) nuclear medicine research at the laboratories and in academia, (c) research into industrial applications of isotopes, and (d) research into isotope production and processing methods. The radio- pharmaceutical and radiopharmacy industries have their origin in

465

TRIFID (TRansuranic Isotopic Fraction Interrogation Device): A second generation plutonium isotopic analysis system  

SciTech Connect

The TRIFID (Transuranic Isotopic Fraction Interrogation Device) system is a second generation plutonium isotopic analysis system which incorporates many new and unique features in the area of isotopic data acquisition and isotopic analysis instrument consisting of a Canberra Series 95-MCA interfaced to a Compaq 386 computer. The entire TRIFID software package, including MCA communications and isotopic analysis routines, was developed using the C programming language. Extensive use has been made of user friendly screens and menus for ease of operation and training and to facilitate use by technical level operators. Automated TRIFID features provide for MCA/ADC setup and acquisition, spectral storage, isotopic analysis, and report generation. One unique feature of the TRIFID system design allows it to be pre-programed for an entire day's counting. The isotopic analysis module (EPICS) contains an expert system formalism which is used to detect and assay for spectral interferences, and to automatically adjust peak fitting constraints based on spectral intensity variations. A TRIFID system has been in operation in a production laboratory at the Rocky Flats Plant since September 1988. Marked decreases in training and hands-on operation time have been achieved in comparison to the older, preceding isotopic systems. 2 refs., 3 figs.

Fleissner, J G; Coressel, T W; Freier, D A; Macklin, L L

1989-01-01T23:59:59.000Z

466

Ultrafast magneto-photocurrents in GaAs: Separation of surface and bulk contributions  

E-Print Network (OSTI)

We induce ultrafast magneto-photocurrents in a GaAs crystal employing interband excitation with femtosecond laser pulses at room temperature and non-invasively separate surface and bulk contributions to the overall current response. The separation between the different symmetry contributions is achieved by measuring the simultaneously emitted terahertz radiation for different sample orientations. Excitation intensity and photon energy dependences of the magneto-photocurrents for linearly and circularly polarized excitations reveal an involvement of different microscopic origins, one of which we believe is the inverse Spin-Hall effect. Our experiments are important for a better understanding of the complex momentum-space carrier dynamics in magnetic fields.

Schmidt, Christian B; Tarasenko, Sergey A; Bieler, Mark

2015-01-01T23:59:59.000Z

467

Single Particle Laser Ablation | EMSL  

NLE Websites -- All DOE Office Websites (Extended Search)

Single Particle Laser Ablation Single Particle Laser Ablation Leads No leads are available at this time. Effect of Solar Radiation on the Optical Properties and Molecular...

468

Plasmonic Quantum Cascade Laser Antenna  

Science Journals Connector (OSTI)

We demonstrate the plasmonic quantum cascade laser antenna, that can confine mid-infrared radiation beyond the diffraction limit, by integrating gold optical antennas on the laser...

Yu, Nanfang; Cubukcu, Ertugrul; Diehl, Laurent; Crozier, Kenneth; Capasso, Federico

469

From Gas Lasers and Tunable Raman Lasers to Quantum Cascade Lasers  

Science Journals Connector (OSTI)

I will describe my involvement in lasers from 1961 to the present, ecompassing high power carbon dioxide lasers, tunable spin-flip Raman lasers, and now high power CW room temperature...

Patel, Kumar

470

Energy exchange between a laser beam and charged particles using inverse transition radiation and method for its use  

DOE Patents (OSTI)

A method and apparatus for exchanging energy between relativistic charged particles and laser radiation using inverse diffraction radiation or inverse transition radiation. The beam of laser light is directed onto a particle beam by means of two optical elements which have apertures or foils through which the particle beam passes. The two apertures or foils are spaced by a predetermined distance of separation and the angle of interaction between the laser beam and the particle beam is set at a specific angle. The separation and angle are a function of the wavelength of the laser light and the relativistic energy of the particle beam. In a diffraction embodiment, the interaction between the laser and particle beams is determined by the diffraction effect due to the apertures in the optical elements. In a transition embodiment, the interaction between the laser and particle beams is determined by the transition effect due to pieces of foil placed in the particle beam path.

Kimura, Wayne D. (Bellevue, WA); Romea, Richard D. (Seattle, WA); Steinhauer, Loren C. (Bothell, WA)

1998-01-01T23:59:59.000Z

471

Optical pumping and g-factor of the 3P0 state of the first excited configuration of rare gases odd isotopes  

E-Print Network (OSTI)

in Paschen notation) atoms of odd isotopes of neon, krypton and xenon have been optically pumped in a beam.1 GENERALITIES. - For krypton and xenon atoms, it is probably impossible to perform a magnetic reso- nance, is derived from that of Stan- ley [6]. The vacuum tank is divided into two chambers which are separately

Boyer, Edmond

472

Isotope loss from exhaled moisture and correlation of multifrequency bioelectrical impedance to body fluid compartments measured by intravenous deuterium oxide and sodium bromide dilution in dogs  

E-Print Network (OSTI)

for this route of isotope loss was necessary. Sodium bromide concentrations at 90 minutes and 180 minutes were tested for statistical equivalency to determine if NaBr had equilibrated by 90 minutes. Finally, impedance measured with electrodes separated by 2...

Witten, Tiffani Tipton

2012-06-07T23:59:59.000Z

473

Membrane separation processes for clean production  

SciTech Connect

Clean production can be considered as a strategic element in manufacturing technology for present and future products in the chemical industry. Demand is focused on the development of cost-effective technologies, the optimization of processes including separation steps, alternative processes for the reduction of waste, optimization of the use of resources and improvements in production efficiency. In many cases an environmentally friendly alternative to conventional separation processes could be membrane separation. Membrane separation techniques are suitable for mixtures of liquids, gases and vapors. Some examples of successful applications in the areas of waste water treatment and vapor recovery are given. Demands, advantages and problems of separation with membranes are also discussed.

Paul, D.; Ohlrogge, K. [GKSS Research Center, Geesthacht (Germany)

1998-12-31T23:59:59.000Z

474

Liquid heat capacity lasers  

DOE Patents (OSTI)

The heat capacity laser concept is extended to systems in which the heat capacity lasing media is a liquid. The laser active liquid is circulated from a reservoir (where the bulk of the media and hence waste heat resides) through a channel so configured for both optical pumping of the media for gain and for light amplification from the resulting gain.

Comaskey, Brian J. (Walnut Creek, CA); Scheibner, Karl F. (Tracy, CA); Ault, Earl R. (Livermore, CA)

2007-05-01T23:59:59.000Z

475

Explosively pumped laser light  

DOE Patents (OSTI)

A single shot laser pumped by detonation of an explosive in a shell casing. The shock wave from detonation of the explosive causes a rare gas to luminesce. The high intensity light from the gas enters a lasing medium, which thereafter outputs a pulse of laser light to disable optical sensors and personnel.

Piltch, Martin S. (Los Alamos, NM); Michelotti, Roy A. (Los Alamos, NM)

1991-01-01T23:59:59.000Z

476

Isotope Effects on the Enzymatic and Nonenzymatic Reactions of Chorismate  

Science Journals Connector (OSTI)

The isotopic composition of the latter was determined by isotope ratio mass spectrometry, enabling determination of isotope effects at the mechanistically interesting key positions O7, C1, and C9. ... Heavy atom isotope effects on the nonenzymatic Claisen rearrangement to give prephenate, 18k1 and 13k1, were determined at 60 °C as described for the enzymatic reactions and calculated from the following relationship: where xk1 is the apparent isotope effect, expressed as a ratio of the rate constants for the light and heavy (x) isotopes. ...

S. Kirk Wright; Michael S. DeClue; Ajay Mandal; Lac Lee; Olaf Wiest; W. Wallace Cleland; Donald Hilvert

2005-08-27T23:59:59.000Z

477

Long-term changes in solar wind elemental and isotopic ratios: A compairosn of two lunar ilmenites of different antiquities  

SciTech Connect

An ilmenite separate from lunar regolith breccia 79035, a sample presumed to have been exposed to solar wind more than 2 Ga ago, was analyzed for noble gas and nitrogen elemental and isotopic abundances by stepwise oxidation and pyrolysis. The gases appear to be distributed between two distinct reservoirs in the ilmenite, defined by release patterns and isotopic considerations. One of the reservoirs, near grain surfaces, yields elemental ratios that for the most part are solar while the other, sited at greater depths within grains, has severely fractionated elemental abundances and generally heavier isotopic ratios as well. Xenon provides an exception to the solar abundance pattern in the near-surface reservoir, being enhanced by about a factor of 2 relative to the expected value. A comparison of the 79035 separate with a previously analyzed ilmenite from soil 71501, which received its solar wind exposure much more recently, indicates that the two-fold xenon enhancement occurs in the fractionated reservoir as well as the solar one, and that it may therefore be attributable to a change in the solar wind elemental abundances. Other differences between the two ilmenites occur in helium and neon isotopic ratios and in He/Ar elemental ratios. Since mineralogical influences on retentivities of the gases in the two samples should be the same, and possible contributions of non-solar wind components to one ilmenite in preference to the other can generally be eliminated or accounted for, all of these differences may reflect changes in the solar wind over time.

Becker, R.H.; Pepin, R.O. (Univ. of Minneapolis, MN (USA))

1989-05-01T23:59:59.000Z

478

Process for strontium-82 separation  

DOE Patents (OSTI)

A process for selective separation of strontium-82 and strontium-85 from proton irradiated molybdenum targets comprises dissolving the molybdenum target in a hydrogen peroxide solution to form a first solution containing ions selected from a group consisting of molybdenum, niobium, technetium, selenium, vanadium, arsenic, germanium, zirconium, rubidium, zinc, beryllium, cobalt, iron, manganese, chromium, strontium, and yttrium; passing the solution through a first cationic resin whereby ions selected from a group consisting of zinc, beryllium, cobalt, iron, manganese, chromium, strontium, yttrium a portion of zirconium and a portion of rubidium are selectively absorbed by the first resin; contacting the first resin with an acid solution to strip and remove the absorbed ions from the first cationic exchange resin to form a second solution; evaporating the second solution for a time sufficient to remove substantially all of the acid and water from the solution whereby a residue remains; dissolving the residue in a dilute acid to form a third solution; passing the third solution through a second cationic resin whereby the ions are absorbed by the second resin; contacting the second resin with a dilute sulfuric acid solution whereby the absorbed ions selected from the group consisting of rubidium, zinc, beryllium, cobalt, iron, manganese, chromium and zirconium are selectively removed from the second resin; and contacting the second resin with a dilute acid solution whereby the absorbed strontium ions are selectively removed. 1 fig.

Heaton, R.C.; Jamriska, D.J. Sr.; Taylor, W.A.

1992-12-01T23:59:59.000Z

479

Laser dividing apparatus  

DOE Patents (OSTI)

A laser beam dividing apparatus (10) having a first beam splitter (14) with an aperture (16) therein positioned in the path of a laser beam (12) such that a portion of the laser beam (12) passes through the aperture (16) onto a second beam splitter (20) and a portion of the laser beam (12) impinges upon the first beam splitter (14). Both the first beam splitter (14) and the second beam splitter (20) are, optionally, made from a dichroic material such that a green component (24) of the laser beam (12) is reflected therefrom and a yellow component (26) is refracted therethrough. The first beam splitter (14) and the second beam splitter (20) further each have a plurality of facets (22) such that the components (24, 26) are reflected and refracted in a number equaling the number of facets (22).

English, Jr., R. Edward (Tracy, CA); Johnson, Steve A. (Tracy, CA)

1995-01-01T23:59:59.000Z

480

Guest Editorial: Laser Damage  

SciTech Connect

Laser damage of optical materials, first reported in 1964, continues to limit the output energy and power of pulsed and continuous-wave laser systems. In spite of some 48 years of research in this area, interest from the international laser community to laser damage issues remains at a very high level and does not show any sign of decreasing. Moreover, it grows with the development of novel laser systems, for example, ultrafast and short-wavelength lasers that involve new damage effects and specific mechanisms not studied before. This interest is evident from the high level of attendance and presentations at the annual SPIE Laser Damage Symposium (aka, Boulder Damage Symposium) that has been held in Boulder, Colorado, since 1969. This special section of Optical Engineering is the first one devoted to the entire field of laser damage rather than to a specific part. It is prepared in response to growing interest from the international laser-damage community. Some papers in this special section were presented at the Laser Damage Symposium; others were submitted in response to the general call for papers for this special section. The 18 papers compiled into this special section represent many sides of the broad field of laser-damage research. They consider theoretical studies of the fundamental mechanisms of laser damage including laser-driven electron dynamics in solids (O. Brenk and B. Rethfeld; A. Nikiforov, A. Epifanov, and S. Garnov; T. Apostolova et al.), modeling of propagation effects for ultrashort high-intensity laser pulses (J. Gulley), an overview of mechanisms of inclusion-induced damage (M. Koldunov and A. Manenkov), the formation of specific periodic ripples on a metal surface by femtosecond laser pulses (M. Ahsan and M. Lee), and the laser-plasma effects on damage in glass (Y. Li et al). Material characterization is represented by the papers devoted to accurate and reliable measurements of absorption with special emphasis on thin films (C. Mühlig and S. Bublitz; B. Cho, E. Danielewicz, and J. Rudisill; W. Palm et al; and J. Lu et al.). Statistical treatment of measurements of the laser-damage threshold (J. Arenberg) and the relationship to damage mechanisms (F. Wagner et al.) represent the large subfield of laser-damage measurements. Various aspects of multilayer coating and thin-film characterization are considered in papers by B. Cho, J. Rudisill, and E. Danielewicz (spectral shift in multilayer mirrors) and R. Weber et al. (novel approach to damage studies based on third-harmonic generation microscopy). Of special interest for readers is the paper by C. Stolz that summarizes the results of four “thin-film damage competitions” organized as a part of the Laser Damage Symposium. Another paper is devoted to thermal annealing of damage precursors (N. Shen et al.). Finally, the influence of nano-size contamination on initiation of laser damage by ultrashort pulses is considered in paper of V. Komolov et al.

Vitaly Gruzdev, Michelle D. Shinn

2012-12-01T23:59:59.000Z

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481

The Theta Laser A Low Noise Chirped Pulse Laser  

E-Print Network (OSTI)

The Theta Laser A Low Noise Chirped Pulse Laser Dimitrios Mandridis dmandrid@creol.ucf.edu April 29, 2011 CREOL Affiliates Day 2011 #12;2 Objective: Frequency Swept (FM) Mode-locked Laser · Develop a frequency swept laser, · linear f-sweep, · uniform-intensity, · low noise, · with long-term stability

Van Stryland, Eric

482

Thorium isotopes in colloidal fraction of water from San Marcos Dam, Chihuahua, Mexico  

Science Journals Connector (OSTI)

The main interest of this stiidy is to assess the contents and distribution of Th-series isotopes in colloidal fraction of surface water from San Marcos dam because the suspended particulate matter serves as transport medium for several pollutants. The aim of this work was to assess the distribution of thorium isotopes ( 232 Th and 230 Th ) contained in suspended matter. Samples were taken from three surface points along the San Marcos dam: water input midpoint and near to dam wall. In this last point a depth sampling was also carried out. Here three depth points were taken at 0.4 8 and 15 meters. To evaluate the thorium behavior in surface water from every water sample the colloidal fraction was separated between 1 and 0.1 ?m. Thorium isotopes concentraron in samples were obtained by alpha spectrometry. Activity concentrations obtained of 232 Th and 230 Th in surface points ranged from 0.3 to 0.5 Bq ? L-1 whereas in depth points ranged from 0.4 to 3.2 Bq ? L-1 respectively. The results show that 230 Th is in higher concentration than 232 Th in colloidal fraction. This can be attributed to a preference of these colloids to adsorb uranium. Thus the activity ratio 230 Th / 232 Th in colloidal fraction showed values from 2.3 to 10.2. In surface points along the dam 230 Th activity concentration decreases while 232 Th concentration remains constant. On the other hand activity concentrations of both isotopes showed a pointed out enhancement with depth. The results have shown a possible lixiviation of uranium from geological substrate into the surface water and an important fractionation of thorium isotopes which suggest that thorium is non-homogeneously distributed along San Marcos dam.

2013-01-01T23:59:59.000Z

483

The setup of an extraction system coupled to a hydrogen isotopes distillation column  

SciTech Connect

Among the most difficult problems of cryogenic distillation one stands apart: the extraction of the heavy fraction. By an optimal design of the cycle scheme, this problem could be avoided. A 'worst case scenario' is usually occurring when the extracted fraction consists of one prevalent isotope such as hydrogen and small amounts of the other two hydrogen isotopes (deuterium and/or tritium). This situation is further complicated by two parameters of the distillation column: the extraction flow rate and the hold-up. The present work proposes the conceptual design of an extraction system associated to the cryogenic distillation column used in hydrogen separation processes. During this process, the heavy fraction (DT, T{sub 2}) is separated, its concentration being the highest at the bottom of the distillation column. From this place the extraction of the gaseous phase can now begin. Being filled with adsorbent, the extraction system is used to temporarily store the heavy fraction. Also the extraction system provides samples for the gas Chromatograph. The research work is focused on the existent pilot plant for tritium and deuterium separation from our institute to validate the experiments carried out until now. (authors)

Zamfirache, M.; Bornea, A.; Stefanescu, I.; Bidica, N.; Balteanu, O.; Bucur, C. [INC-DTCI, ICSIRm. Valcea, Uzinei Street 4, Rm. Valcea (Romania)

2008-07-15T23:59:59.000Z

484

Isotope Work at Oak Ridge  

Science Journals Connector (OSTI)

The special training division of the Oak Ridge Institute of Nuclear Studies has announced that three additional courses in the techniques of using radioisotopes in research have been scheduled during the winter and spring of 1951. They are to be held from January 8th to February 2nd from February 19th to March 16th and from April 16th to May 11th. Designed to acquaint research workers with the safe and efficient use of radioisotopes the courses include laboratory work lectures and special?topic seminars. Experiments cover such matters as the use and calibration of instruments purification and separation of radioactive materials from inert and other radioactive materials and pile activation technology. The seminars cover various biological and medical uses of radioisotopes and the design of radiochemical laboratories.

C. P. Keim; H. W. Savage; Boyd Weaver

1951-01-01T23:59:59.000Z

485

Testing of concrete by laser ablation  

DOE Patents (OSTI)

A method is disclosed for testing concrete in a structure in situ, by: directing a succession of pulses of laser radiation at a point on the structure so that each pulse effects removal of a quantity of concrete and transfers energy to the concrete; detecting a characteristic of energy which has been transferred to the concrete; determining, separately from the detecting step, the total quantity of concrete removed by the succession of pulses; and calculating a property of the concrete on the basis of the detected energy characteristic and the determined total quantity of concrete removed. 1 fig.

Flesher, D.J.; Becker, D.L.; Beem, W.L.; Berry, T.C.; Cannon, N.S.

1997-01-07T23:59:59.000Z

486

Testing of concrete by laser ablation  

DOE Patents (OSTI)

A method of testing concrete in a structure in situ, by: directing a succession of pulses of laser radiation at a point on the structure so that each pulse effects removal of a quantity of concrete and transfers energy to the concrete; detecting a characteristic of energy which has been transferred to the concrete; determining, separately from the detecting step, the total quantity of concrete removed by the succession of pulses; and calculating a property of the concrete on the basis of the detected energy characteristic and the determined total quantity of concrete removed.

Flesher, Dann J. (Benton City, WA); Becker, David L. (Kennewick, WA); Beem, William L. (Kennewick, WA); Berry, Tommy C. (Kennewick, WA); Cannon, N. Scott (Kennewick, WA)

1997-01-01T23:59:59.000Z

487

REPORT OF SURVEY OF OAK RIDGE ISOTOPE  

Energy.gov (U.S. Department of Energy (DOE)) Indexed Site

OAK RIDGE ISOTOPE OAK RIDGE ISOTOPE ENRICHMENT (CALUTRON) FACILITY BUILDING 9204-3 U.S. Department of Energy Office of Environmental Management & Office of Nuclear Energy Report of Survey of Oak Ridge Isotope Enrichment (Calutron) Facility Building 9204-3 FINAL May 8, 2000 Contents 1. Introduction 1.1 Purpose 1.2 Facility Description 1.3 Organization Representatives 1.4 Survey Participants 2. Summary, Conclusions & Recommendations 2.1 Transfer Considerations 2.2 Post-Transfer EM Path Forward & Management Risk 3. Survey Results 4. Stabilization and Other Actions Required for Transfer 5. Surveillance & Maintenance After Transfer 6. Other Transfer Details 7. Attachments and References Appendix A - Detailed Survey Notes

488

Isotopic substitution in a model polaronic system  

Science Journals Connector (OSTI)

The effect of isotopic substitution in the excitation spectrum of a model polaronic system is presented. To study this effect we use a three-site many-body Hamiltonian, with two phonon modes, which includes electronic correlations and electron-phonon interactions. Under isotopic substitution, the shift of the lowest excitation energy changes sign for intermediate electron-phonon coupling, coinciding with the onset of polaronic behavior. This manifests as a strong change of the dynamics of polaron tunneling, a behavior opposite to that found in purely phonon excitations. Additionally, a small change in the static polaronic distortion appears under isotopic substitution. This change in the local structure has opposite signs for low and intermediate electron-phonon coupling compared to that found in the strong-coupling limit.

J. Mustre de Leon; R. de Coss; A. R. Bishop; S. A. Trugman

1999-04-01T23:59:59.000Z

489

Atomic line emission analyzer for hydrogen isotopes  

DOE Patents (OSTI)

Apparatus for isotopic analysis of hydrogen comprises a low pressure chamber into which a sample of hydrogen is introduced and then exposed to an electrical discharge to excite the electrons of the hydrogen atoms to higher energy states and thereby cause the emission of light on the return to lower energy states, a Fresnel prism made at least in part of a material anomalously dispersive to the wavelengths of interest for dispersing the emitted light, and a photodiode array for receiving the dispersed light. The light emitted by the sample is filtered to pass only the desired wavelengths, such as one of the lines of the Balmer series for hydrogen, the wavelengths of which differ slightly from one isotope to another. The output of the photodiode array is processed to determine the relative amounts of each isotope present in the sample. Additionally, the sample itself may be recovered using a metal hydride.

Kronberg, James W. (108 Independent Blvd., Aiken, SC 29801)

1993-01-01T23:59:59.000Z

490

Atomic line emission analyzer for hydrogen isotopes  

DOE Patents (OSTI)

Apparatus for isotopic analysis of hydrogen comprises a low pressure chamber into which a sample of hydrogen is introduced and then exposed to an electrical discharge to excite the electrons of the hydrogen atoms to higher energy states and thereby cause the emission of light on the return to lower energy states, a Fresnel prism made at least in part of a material anomalously dispersive to the wavelengths of interest for dispersing the emitted light, and a photodiode array for receiving the dispersed light. The light emitted by the sample is filtered to pass only the desired wavelengths, such as one of the lines of the Balmer series for hydrogen, the wavelengths of which differ slightly from one isotope to another. The output of the photodiode array is processed to determine the relative amounts of each isotope present in the sample. Additionally, the sample itself may be recovered using, a metal hydride.

Kronberg, J.W.

1991-05-08T23:59:59.000Z

491

Atomic line emission analyzer for hydrogen isotopes  

DOE Patents (OSTI)

Apparatus for isotopic analysis of hydrogen comprises a low pressure chamber into which a sample of hydrogen is introduced and then exposed to an electrical discharge to excite the electrons of the hydrogen atoms to higher energy states and thereby cause the emission of light on the return to lower energy states, a Fresnel prism made at least in part of a material anomalously dispersive to the wavelengths of interest for dispersing the emitted light, and a photodiode array for receiving the dispersed light. The light emitted by the sample is filtered to pass only the desired wavelengths, such as one of the lines of the Balmer series for hydrogen, the wavelengths of which differ slightly from one isotope to another. The output of the photodiode array is processed to determine the relative amounts of each isotope present in the sample. Additionally, the sample itself may be recovered using a metal hydride.

Kronberg, J.W.

1993-03-30T23:59:59.000Z

492

Quantum electrodynamics in a laser and the electron laser collision  

E-Print Network (OSTI)

Quantum electrodynamics in a laser is formulated, in which the electron-laser interaction is exactly considered, while the interaction of an electron and a single photon is considered by perturbation. The formulation is applied to the electron-laser collisions. The effect of coherence between photons in the laser is therefore fully considered in these collisions. The possibility of $\\gamma-$ray laser generation by use of this kind of collision is discussed.

Qi-Ren Zhang

2014-08-08T23:59:59.000Z

493

Ultra-fast laser system  

DOE Patents (OSTI)

A laser system is provided which selectively excites Raman active vibrations in molecules. In another aspect of the present invention, the system includes a laser, pulse shaper and detection device. A further aspect of the present invention employs a femtosecond laser and binary pulse shaping (BPS). Still another aspect of the present invention uses a laser beam pulse, a pulse shaper and remote sensing.

Dantus, Marcos; Lozovoy, Vadim V

2014-01-21T23:59:59.000Z

494

1982 laser program annual report  

SciTech Connect

This annual report covers the following eight sections: (1) laser program review, (2) laser systems and operation, (3) target design, (4) target fabrication, (5) fusion experiments program, (6) Zeus laser project, (7) laser research and development, and (8) energy applications. (MOW)

Hendricks, C.D.; Grow, G.R. (eds.)

1983-08-01T23:59:59.000Z

495

Report of Survey of Oak Ridge Isotope Enrichment (Calutron) Facility...  

Office of Environmental Management (EM)

Report of Survey of Oak Ridge Isotope Enrichment (Calutron) Facility Building 9204-3 Report of Survey of Oak Ridge Isotope Enrichment (Calutron) Facility Building 9204-3 The...

496

Isotope effects in methanol synthesis and the reactivity of copper...  

NLE Websites -- All DOE Office Websites (Extended Search)

Isotope effects in methanol synthesis and the reactivity of copper formates on a CuSiO2 catalyst. Isotope effects in methanol synthesis and the reactivity of copper formates on a...

497

A Helium Isotope Perspective On The Dixie Valley, Nevada, Hydrothermal...  

Open Energy Info (EERE)

gas abundances and isotopic compositions. The helium isotopic compositions of fluids produced from the Dixie Valley geothermal field range from 0.70 to 0.76 Ra, are among the...

498

Hydrogen isotope fractionation during lipid biosynthesis by Haloarcula marismortui  

E-Print Network (OSTI)

Hydrogen isotope fractionation during lipid biosynthesis by Haloarcula marismortui Sitindra S studied the controls on the fractionation of hydrogen isotopes during lipid biosynthesis by Haloarcula marismortui, a halophilic archaea, in pure culture experiments by varying organic substrate, the hydrogen

499

CARBONATE STABLE ISOTOPES | Terrestrial Teeth and Bones  

Science Journals Connector (OSTI)

Teeth and bones of fossil vertebrates can preserve a record of Quaternary terrestrial environments in the form of isotopic compositions of carbon (13C/12C), nitrogen (15N/14N), and oxygen (18O/16O). These isotopic signatures in teeth and bones have yielded valuable information on the extent of savanna environments under tropical climates, on the ancient levels of aridity, on the spread of dense forests at the beginning of the Holocene, and on the paleodiet of hominids and their associated fauna.

H. Bocherens; D.G. Drucker

2007-01-01T23:59:59.000Z

500

CARBONATE STABLE ISOTOPES | Terrestrial Teeth and Bones  

Science Journals Connector (OSTI)

Abstract Teeth and bones of fossil vertebrates can preserve a record of Quaternary terrestrial environments in the form of the isotopic compositions of carbon (13C/12C), nitrogen (15N/14N), and oxygen (18O/16O). These isotopic signatures in teeth and bones have yielded valuable information on the extent of savanna environments under tropical climates, on the ancient levels of aridity, on the spread of dense forests at the beginning of the Holocene, and on the paleodiet of Hominids and their associated fauna.

H. Bocherens; D.G. Drucker

2013-01-01T23:59:59.000Z