National Library of Energy BETA

Sample records for inelastic x-ray scattering

  1. Structure and dynamics of cadmium telluride studied by x-ray and inelastic neutron scattering

    SciTech Connect (OSTI)

    Niedziela, J. L., E-mail: niedzielajl@ornl.gov [Instrument and Source Division, Neutron Sciences Directorate, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831 (United States); Stone, M. B., E-mail: stonemb@ornl.gov [Quantum Condensed Matter Division, Neutron Sciences Directorate, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831 (United States)

    2014-09-08

    We present a combined study of density functional theory, x-ray diffraction, and inelastic neutron scattering examining the temperature dependent structure and lattice dynamics of commercially available cadmium telluride. A subtle change in the structure is evinced near 80?K, which manifests also in the measured phonon density of states. There is no change to the long-range ordered structure. The implications of the change in relation to structural defects are discussed.

  2. Structure and dynamics of cadmium telluride studied by x-ray and inelastic neutron scattering

    SciTech Connect (OSTI)

    Niedziela, Jennifer L [ORNL; Stone, Matthew B [ORNL

    2014-01-01

    We present a combined study of density functional theory, x-ray diffraction, and inelastic neutron scattering examining the temperature dependent structure and lattice dynamics of commercially available cadmium telluride. A subtle change in the structure is evinced near 80~K, which manifests also in the measured phonon density of states. There is no change to the long-range ordered structure. The implications of the change in relation to structural defects are discussed.

  3. SPEC application for achieving inelastic X-ray scattering experiment in the SSRF

    E-Print Network [OSTI]

    Lan, Xuying; Liang, Dongxu; Yan, Shuai; Mao, Chengwen; Li, Aiguo; Wang, Jie

    2015-01-01

    In order to carry out inelastic X-ray scattering (IXS) experiment at BL15U1 beamline of Shanghai Synchrotron Radiation Facility (SSRF), the data acquisition and control system based on SPEC software has been developed. The IXS experimental method needs linkage control of monochromator, silicon drift detector (SDD) and ionization chamber on continuous segment-scan mode with variable step size, and gains the data of energy, spectrum and light intensity synchronously. A method is presented for achieving this function which was not realized only by using SSCAN of Experimental Physics and Industrial Control System (EPICS). This paper shows work details including control system description, SPEC configurations for EPICS devices, macro definitions and applications in the BL15U1. An IXS experiment was executed by using the SPEC control system, its results prove that the method is feasible to perform the experiment.

  4. The simultaneous measurement of energy and linear polarization of the scattered radiation in resonant inelastic soft x-ray scattering

    SciTech Connect (OSTI)

    Braicovich, L. Minola, M.; Dellea, G.; Ghiringhelli, G.; Le Tacon, M.; Moretti Sala, M.; Morawe, C.; Peffen, J.-Ch.; Yakhou, F.; Brookes, N. B.; Supruangnet, R.

    2014-11-15

    Resonant Inelastic X-ray Scattering (RIXS) in the soft x-ray range is an element-specific energy-loss spectroscopy used to probe the electronic and magnetic excitations in strongly correlated solids. In the recent years, RIXS has been progressing very quickly in terms of energy resolution and understanding of the experimental results, but the interpretation of spectra could further improve, sometimes decisively, from a full knowledge of the polarization of incident and scattered photons. Here we present the first implementation, in a high resolution soft-RIXS spectrometer used to analyze the scattered radiation, of a device allowing the measurement of the degree of linear polarization. The system, based on a graded W/B{sub 4}C multilayer mirror installed in proximity of the CCD detector, has been installed on the AXES spectrometer at the ESRF (European Synchrotron Radiation Facility); it has been fully characterized and it has been used for a demonstration experiment at the Cu L{sub 3} edge on a high-T{sub c} superconducting cuprate. The loss in efficiency suffered by the spectrometer equipped with this test facility was a factor 17.5. We propose also a more advanced version, suitable for a routine use on the next generation of RIXS spectrometers and with an overall efficiency up to 10%.

  5. Novel opportunities for sub-meV inelastic X-ray scattering at high-repetition rate self-seeded X-ray free-electron lasers

    E-Print Network [OSTI]

    Chubar, Oleg; Kocharyan, Vitali; Madsen, Anders; Saldin, Evgeni; Serkez, Svitozar; Shvyd'ko, Yuri; Sutter, John

    2015-01-01

    Inelastic X-ray scattering (IXS) is an important tool for studies of equilibrium dynamics in condensed matter. A new spectrometer recently proposed for ultra-high-resolution IXS (UHRIX) has achieved 0.6~meV and 0.25~nm$^{-1}$ spectral and momentum transfer resolutions, respectively. However, further improvements down to 0.1~meV and 0.02~nm$^{-1}$ are required to close the gap in energy-momentum space between high and low frequency probes. We show that this goal can be achieved by further optimizing the X-ray optics and by increasing the spectral flux of the incident X-ray pulses. UHRIX performs best at energies from 5 to 10 keV, where a combination of self-seeding and undulator tapering at the SASE-2 beamline of the European XFEL promises up to a hundred-fold increase in average spectral flux compared with nominal SASE pulses at saturation, or three orders of magnitude more than possible with storage-ring based radiation sources. Wave-optics propagation shows that about $7\\times 10^{12}$~ph/s in a $90$-$\\mu$e...

  6. Probing single magnon excitations in Sr?IrO? using O K-edge resonant inelastic x-ray scattering

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Liu, X.; Dean, M. P. M.; Liu, J.; Chiuzbaian, S. G.; Jaouen, N.; Nicolaou, A.; Yin, W. G.; Rayan Serrao, C.; Ramesh, R.; Ding, H.; et al

    2015-04-28

    Resonant inelastic X-ray scattering (RIXS) at the L-edge of transition metal elements is now commonly used to probe single magnon excitations. Here we show that single magnon excitations can also be measured with RIXS at the K-edge of the surrounding ligand atoms when the center heavy metal elements have strong spin-orbit coupling. This is demonstrated with oxygen K-edge RIXS experiments on the perovskite Sr?IrO?, where low energy peaks from single magnon excitations were observed. This new application of RIXS has excellent potential to be applied to a wide range of magnetic systems based on heavy elements, for which the L-edgemore »RIXS energy resolutions in the hard X-ray region is usually poor.« less

  7. Probing single magnon excitations in Sr?IrO? using O K-edge resonant inelastic x-ray scattering

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Liu, X. [Chinese Academy of Sciences (CAS), Beijing (China). Beijing National Lab. for Condensed Matter Physics (BNLCP-CAS); Brookhaven National Lab. (BNL), Upton, NY (United States); Collaborative Innovation Center of Quantum Matter, Beijing (China); Dean, M. P. M. [Brookhaven National Lab. (BNL), Upton, NY (United States); Liu, J. [Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Chiuzbaian, S. G. [Sorbonne Univ., Paris (France); Synchrotron SOLEIL, Saint-Aubin (France); Jaouen, N. [Synchrotron SOLEIL, Saint-Aubin (France); Nicolaou, A. [Synchrotron SOLEIL, Saint-Aubin (France); Yin, W. G. [Brookhaven National Lab. (BNL), Upton, NY (United States); Rayan Serrao, C. [Univ. of California, Berkeley, CA (United States); Ramesh, R. [Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Ding, H. [Chinese Academy of Sciences (CAS), Beijing (China). Beijing National Lab. for Condensed Matter Physics (BNLCP-CAS); Collaborative Innovation Center of Quantum Matter, Beijing (China); Hill, J. P. [Brookhaven National Lab. (BNL), Upton, NY (United States)

    2015-05-27

    Resonant inelastic X-ray scattering (RIXS) at the L-edge of transition metal elements is now commonly used to probe single magnon excitations. Here we show that single magnon excitations can also be measured with RIXS at the K-edge of the surrounding ligand atoms when the center heavy metal elements have strong spin-orbit coupling. This is demonstrated with oxygen K-edge RIXS experiments on the perovskite Sr?IrO?, where low energy peaks from single magnon excitations were observed. This new application of RIXS has excellent potential to be applied to a wide range of magnetic systems based on heavy elements, for which the L-edge RIXS energy resolutions in the hard X-ray region is usually poor.

  8. Ultra-high Resolution Optics for EUV and Soft X-ray Inelastic Scattering

    E-Print Network [OSTI]

    Voronov, Dmitry L.

    2010-01-01

    16. Yu. Shvyd’ko, X-Ray Optics, Berlin: Springer-Verlag,Ultra-high Resolution Optics for EUV and Soft X-rayspectral resolution soft x-ray optics. Conventionally in the

  9. An alternative scheme of angular-dispersion analyzers for high-resolution medium-energy inelastic X-ray scattering

    E-Print Network [OSTI]

    Huang, Xian-Rong

    2011-01-01

    The development of medium-energy inelastic X-ray scattering (IXS) optics with meV and sub-meV resolution has attracted considerable efforts in recent years. Meanwhile, there are also concerns or debates about the fundamental and feasibility of the involved schemes. Here the central optical component, the back-reflection angular-dispersion monochromator or analyzer, is analyzed. The results show that the multiple-beam diffraction effect together with transmission-induced absorption can noticeably reduce the diffraction efficiency, although it may not be a fatal threat. In order to improve the efficiency, a simple four-bounce analyzer is proposed that completely avoids these two adverse effects. The new scheme is illustrated to be a feasible alternative approach for developing meV- to sub-meV-resolution IXS spectroscopy.

  10. Background proportional enhancement of the extended fine structure in nonresonant inelastic x-ray scattering

    E-Print Network [OSTI]

    Seidler, Gerald T.

    Background proportional enhancement of the extended fine structure in nonresonant inelastic x is proportional to the strong q-dependent evolution in shape and magnitude of the atomic background. This en

  11. High-energy magnetic excitations in overdoped La 2 - x Sr x CuO 4 studied by neutron and resonant inelastic x-ray scattering

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Wakimoto, S.; Ishii, K.; Kimura, H.; Fujita, M.; Dellea, G.; Kummer, K.; Braicovich, L.; Ghiringhelli, G.; Debeer-Schmitt, L. M.; Granroth, G. E.

    2015-05-21

    We have performed neutron inelastic scattering and resonant inelastic x-ray scattering (RIXS) at the Cu-L? edge to study high-energy magnetic excitations at energy transfers of more than 100 meV for overdoped La2-xSrxCuO? with x=0.25 (Tc=15 K) and x=0.30 (nonsuperconducting) using identical single-crystal samples for the two techniques. From constant-energy slices of neutron-scattering cross sections, we have identified magnetic excitations up to ~250 meV for x=0.25. Although the width in the momentum direction is large, the peak positions along the (?,?) direction agree with the dispersion relation of the spin wave in the nondoped La?CuO? (LCO), which is consistent with themore »previous RIXS results of cuprate superconductors. Using RIXS at the Cu-L? edge, we have measured the dispersion relations of the so-called paramagnon mode along both (?,?) and (?,0) directions. Although in both directions the neutron and RIXS data connect with each other and the paramagnon along (?,0) agrees well with the LCO spin-wave dispersion, the paramagnon in the (?,?) direction probed by RIXS appears to be less dispersive and the excitation energy is lower than the spin wave of LCO near (?/2,?/2). Thus, our results indicate consistency between neutron inelastic scattering and RIXS, and elucidate the entire magnetic excitation in the (?,?) direction by the complementary use of two probes. The polarization dependence of the RIXS profiles indicates that appreciable charge excitations exist in the same energy range of magnetic excitations, reflecting the itinerant character of the overdoped sample. A possible anisotropy in the charge excitation intensity might explain the apparent differences in the paramagnon dispersion in the (?,?) direction as detected by the x-ray scattering.« less

  12. High-energy magnetic excitations in overdoped La 2 - x Sr x CuO 4 studied by neutron and resonant inelastic x-ray scattering

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Wakimoto, S.; Ishii, K.; Kimura, H.; Fujita, M.; Dellea, G.; Kummer, K.; Braicovich, L.; Ghiringhelli, G.; Debeer-Schmitt, L. M.; Granroth, G. E.

    2015-05-01

    We have performed neutron inelastic scattering and resonant inelastic x-ray scattering (RIXS) at the Cu-L? edge to study high-energy magnetic excitations at energy transfers of more than 100 meV for overdoped La2-xSrxCuO? with x=0.25 (Tc=15 K) and x=0.30 (nonsuperconducting) using identical single-crystal samples for the two techniques. From constant-energy slices of neutron-scattering cross sections, we have identified magnetic excitations up to ~250 meV for x=0.25. Although the width in the momentum direction is large, the peak positions along the (?,?) direction agree with the dispersion relation of the spin wave in the nondoped La?CuO? (LCO), which is consistent with the previous RIXS results of cuprate superconductors. Using RIXS at the Cu-L? edge, we have measured the dispersion relations of the so-called paramagnon mode along both (?,?) and (?,0) directions. Although in both directions the neutron and RIXS data connect with each other and the paramagnon along (?,0) agrees well with the LCO spin-wave dispersion, the paramagnon in the (?,?) direction probed by RIXS appears to be less dispersive and the excitation energy is lower than the spin wave of LCO near (?/2,?/2). Thus, our results indicate consistency between neutron inelastic scattering and RIXS, and elucidate the entire magnetic excitation in the (?,?) direction by the complementary use of two probes. The polarization dependence of the RIXS profiles indicates that appreciable charge excitations exist in the same energy range of magnetic excitations, reflecting the itinerant character of the overdoped sample. A possible anisotropy in the charge excitation intensity might explain the apparent differences in the paramagnon dispersion in the (?,?) direction as detected by the x-ray scattering.

  13. Experimental and Theoretical Comparison of the O K-Edge Nonresonant Inelastic X-ray Scattering and X-ray Absorption Spectra of NaReO[subscript 4

    SciTech Connect (OSTI)

    Bradley, Joseph A.; Yang, Ping; Batista, Enrique R.; Boland, Kevin S.; Burns, Carol J.; Clark, David L.; Conradson, Steven D.; Kozimor, Stosh A.; Martin, Richard L.; Seidler, Gerald T.; Scott, Brian L.; Shuh, David K.; Tyliszczak, Tolek; Wilkerson, Marianne P.; Wolfsberg, Laura E. (PNNL); (UWASH); (LBNL); (LANL)

    2010-12-07

    Accurate X-ray absorption spectra (XAS) of first row atoms, e.g., O, are notoriously difficult to obtain due to the extreme sensitivity of the measurement to surface contamination, self-absorption, and saturation affects. Herein, we describe a comprehensive approach for determining reliable O K-edge XAS data for ReO{sub 4}{sup 1-} and provide methodology for obtaining trustworthy and quantitative data on nonconducting molecular systems, even in the presence of surface contamination. This involves comparing spectra measured by nonresonant inelastic X-ray scattering (NRIXS), a bulk-sensitive technique that is not prone to X-ray self-absorption and provides exact peak intensities, with XAS spectra obtained by three different detection modes, namely total electron yield (TEY), fluorescence yield (FY), and scanning transmission X-ray microscopy (STXM). For ReO{sub 4}{sup 1-}, TEY measurements were heavily influenced by surface contamination, while the FY and STXM data agree well with the bulk NRIXS analysis. These spectra all showed two intense pre-edge features indicative of the covalent interaction between the Re 5d and O 2p orbitals. Density functional theory calculations were used to assign these two peaks as O 1s excitations to the e and t{sub 2} molecular orbitals that result from Re 5d and O 2p covalent mixing in T{sub d} symmetry. Electronic structure calculations were used to determine the amount of O 2p character (%) in these molecular orbitals. Time dependent-density functional theory (TD-DFT) was also used to calculate the energies and intensities of the pre-edge transitions. Overall, under these experimental conditions, this analysis suggests that NRIXS, STXM, and FY operate cooperatively, providing a sound basis for validation of bulk-like excitation spectra and, in combination with electronic structure calculations, suggest that NaReO{sub 4} may serve as a well-defined O K-edge energy and intensity standard for future O K-edge XAS studies.

  14. Experimental and Theoretical Comparison of the O K-Edge Non-Resonant Inelastic X-ray Scattering and X-ray Absorption Spectra of NaReO4

    SciTech Connect (OSTI)

    Bradley, Joseph A.; Yang, Ping; Batista, Enrique R.; Boland, Kevin S.; Burns, Carol J.; Clark, David L.; Conradson, Steven D.; Kozimor, Stosh A.; Martin, Richard L.; Seidler, Gerald T.; Scott, Brian L.; Shuh, David K.; Tyliszczak, T.; Wilkerson, Marianne P.; Wolfsberg, Laura E.

    2010-09-14

    Accurate X-ray absorption spectra (XAS) of first row atoms, e.g. O, are notoriously difficult to obtain due to the extreme sensitivity of the measurement to surface contamination, self-absorption, and saturation effects. Herein, we describe a comprehensive approach for determining reliable O K-edge XAS data for ReO41- and provide methodology for obtaining trustworthy and quantitative data on non-conducting molecular systems, even in the presence of surface contamination. This involves comparing spectra measured by non-resonant inelastic X-ray scattering (NRIXS), a bulk-sensitive technique that is not prone to X-ray self-absorption and provides exact peak intensities, with XAS spectra obtained by three different detection modes, namely total electron yield (TEY), fluorescence yield (FY), and scanning transmission X-ray microscopy (STXM). For ReO41-, TEY measurements were heavily influenced by surface contamination, while the FY and STXM data agree well with the bulk NRIXS analysis. These spectra all showed two intense pre-edge features indicative of the covalent interaction between the Re 5d and O 2p orbitals. Time dependent density functional theory calculations were used to assign these two peaks as O 1s excitations to the e and t2 molecular orbitals that result from Re 5d and O 2p covalent mixing in Td symmetry. Electronic structure calculations were used to determine the amount of O 2p character (%) in these molecular orbitals. Time-dependent density functional theory (TD-DFT) was also used to calculate the energies and intensities of the pre-edge transitions. Overall, under these experimental conditions, this analysis suggests that NRIXS, STXM, and FY operate cooperatively, providing a sound basis for validation of bulk-like excitation spectra and, in combination with electronic structure calculations, suggest that NaReO4 may serve as a well-defined O K-edge energy and intensity standard for future O K edge XAS studies.

  15. Pressure-induced valence change in YbAl3: a combined high pressure inelastic x-ray scattering and theoretical investigation

    SciTech Connect (OSTI)

    Bauer, E D; Kumar, R S; Svane, A; Vaitheeswaran, G; Nicol, M F; Kanchana, V; Hu, M; Cornelius, A L

    2008-01-01

    High resolution x-ray absorption (XAS) experiments in the partial fluorescence yield mode (PFY) and resonant inelastic x-ray emission (RXES) measurements under pressure were performed on the intermediate valence compound YbAl{sub 3} up to 38 GPa. The results of the Yb L{sub 3} PFY-XAS and RXES studies show a smooth valence increase in YbAl{sub 3} from 2.75 to 2.93 at ambient to 38 GPa. In-situ angle dispersive synchrotron high pressure x-ray diffraction experiments carried out using a diamond cell at room temperature to study the equation of state showed the ambient cubic phase stable up to 40 GPa. The results obtained from self-interaction corrected local spin density functional calculations to understand the pressure effect on the Yb valence and compressibility are in good agreement with the experimental results.

  16. Fluctuation X-Ray Scattering

    SciTech Connect (OSTI)

    Saldin, PI: D. K.; Co-I's: J. C. H. Spence and P. Fromme

    2013-01-25

    The work supported by the grant was aimed at developing novel methods of finding the structures of biomolecules using x-rays from novel sources such as the x-ray free electron laser and modern synchrotrons

  17. Small Angle X-Ray Scattering Detector

    DOE Patents [OSTI]

    Hessler, Jan P.

    2004-06-15

    A detector for time-resolved small-angle x-ray scattering includes a nearly constant diameter, evacuated linear tube having an end plate detector with a first fluorescent screen and concentric rings of first fiber optic bundles for low angle scattering detection and an annular detector having a second fluorescent screen and second fiber optic bundles concentrically disposed about the tube for higher angle scattering detection. With the scattering source, i.e., the specimen under investigation, located outside of the evacuated tube on the tube's longitudinal axis, scattered x-rays are detected by the fiber optic bundles, to each of which is coupled a respective photodetector, to provide a measurement resolution, i.e., dq/q, where q is the momentum transferred from an incident x-ray to an x-ray scattering specimen, of 2% over two (2) orders of magnitude in reciprocal space, i.e., qmax/qmin approx=lO0.

  18. Small Angle X-ray Scattering (SAXS) Laboratory Learning Experiences

    E-Print Network [OSTI]

    Meagher, Mary

    .A. & Svergun D.I. (1987). Structure Analysis by Small-Angle X-Ray and Neutron Scattering. NY: Plenum PressSmall Angle X-ray Scattering (SAXS) Laboratory Learning Experiences o - Use of small angle X-ray scattering instrumentation o - Programs that you will use SAXS (BRUKER AXS) PRIMUS (Konarev, Volkov, Koch

  19. Measurements of Ionic Structure in Shock Compressed Lithium Hydride from Ultrafast X-Ray Thomson Scattering

    SciTech Connect (OSTI)

    Kritcher, A. L. [L-399, Lawrence Livermore National Laboratory, P.O. Box 808, Livermore, California 94551 (United States); Department of Nuclear Engineering, University of California Berkeley, Berkeley, California 94709 (United States); Neumayer, P.; Doeppner, T.; Landen, O. L.; Glenzer, S. H. [L-399, Lawrence Livermore National Laboratory, P.O. Box 808, Livermore, California 94551 (United States); Brown, C. R. D. [Department of Physics, Imperial College, London SW7 2AZ (United Kingdom); AWE plc., Aldermaston, Reading, RG7 4PR (United Kingdom); Davis, P. [L-399, Lawrence Livermore National Laboratory, P.O. Box 808, Livermore, California 94551 (United States); Department of Physics, University of California Berkeley, Berkeley, California 94709 (United States); Falcone, R. W.; Lee, H. J. [Department of Physics, University of California Berkeley, Berkeley, California 94709 (United States); Gericke, D. O.; Vorberger, J.; Wuensch, K. [CFSA, Department of Physics, University of Warwick, Coventry CV4 7AL (United Kingdom); Gregori, G. [Department of Physics, Oxford University, Oxford OX1 3PU (United Kingdom); Holst, B.; Redmer, R. [Universitaet Rostock, Institut fuer Physik, D-18051 Rostock (Germany); Morse, E. C. [Department of Nuclear Engineering, University of California Berkeley, Berkeley, California 94709 (United States); Pelka, A.; Roth, M. [Institut fuer Kernphysik, Technische Universitaet Darmstadt, Darmstadt (Germany)

    2009-12-11

    We present the first ultrafast temporally, spectrally, and angularly resolved x-ray scattering measurements from shock-compressed matter. The experimental spectra yield the absolute elastic and inelastic scattering intensities from the measured density of free electrons. Laser-compressed lithium-hydride samples are well characterized by inelastic Compton and plasmon scattering of a K-alpha x-ray probe providing independent measurements of temperature and density. The data show excellent agreement with the total intensity and structure when using the two-species form factor and accounting for the screening of ion-ion interactions.

  20. SMB, Small Angle X-Ray Scattering

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power AdministrationRobust, High-Throughput Analysis of Protein1-0845*RV 14800Small Angle X-Ray Scattering Home »

  1. Neutron and X-ray Scattering Study of Magnetic Manganites

    E-Print Network [OSTI]

    Boothroyd, Andrew

    Neutron and X-ray Scattering Study of Magnetic Manganites Graeme Eoin Johnstone A Thesis submitted are performed using a variety of neutron scattering and x-ray scattering techniques. The electronic ground for analysing the results of the polarised neutron scattering experiment. There are a large number of people who

  2. Probing Spatial, Electronic Structures with X-ray Scattering...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Probing Spatial, Electronic Structures with X-ray Scattering, Spectroscopic Techniques Wednesday, September 5, 2012 - 10:45am SLAC, Bldg. 137, Room 226 Gang Chen Seminar:...

  3. National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    15th National School on Neutron and X-ray Scattering August 10 - 24, 2013 at Argonne National of the National School on Neutron and X-ray Scattering is to educate graduate students on the utilization of major Ridge National Laboratory's Neutron Scattering Science Division. Scientific Directors: Jonathan C. Lang

  4. Thirteenth National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    Thirteenth National School on Neutron and X-ray Scattering June 11 ­ June 25, 2011 at Argonne of the National School on Neutron and X-ray Scattering is to educate graduate students on the utilization of major National Laboratory's Neutron Scattering Science Division. Scientific Directors: Jonathan C. Lang, Suzanne

  5. Sixteenth National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    Pennycook, Steve

    Sixteenth National School on Neutron and X-ray Scattering June 14-28, 2014 at Argonne National of the National School on Neutron and X-ray Scattering is to educate graduate students on the utilization of major's Neutron Scattering Science Division. Scientific Directors: Suzanne G.E. te Velthuis, Esen Ercan Alp

  6. National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    Pennycook, Steve

    National School on Neutron and X-ray Scattering May 30 ­ June 13, 2009 at Argonne National of the National School on Neutron and X-ray Scattering is to educate graduate students on the utilization of major National Laboratory's Neutron Scattering Science Division. Scientific Directors: Jonathan C. Lang, Suzanne

  7. Fourteenth National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    Pennycook, Steve

    Fourteenth National School on Neutron and X-ray Scattering August 12 - 25, 2012 at Argonne National of the National School on Neutron and X-ray Scattering is to educate graduate students on the utilization of major Ridge National Laboratory's Neutron Scattering Science Division. Scientific Directors: Jonathan C. Lang

  8. Twelfth National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    Pennycook, Steve

    Twelfth National School on Neutron and X-ray Scattering June 12 ­ June 26, 2010 at Argonne National of the National School on Neutron and X-ray Scattering is to educate graduate students on the utilization of major National Laboratory's Neutron Scattering Science Division. Scientific Directors: Jonathan C. Lang, Suzanne

  9. Tenth National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    Pennycook, Steve

    Tenth National School on Neutron and X-ray Scattering September 24 - October 11, 2008 at Argonne of the National School on Neutron and X-ray Scattering is to educate graduate students on the utilization of major National Laboratory's Neutron Scattering Science Division. Scientific Directors: Jonathan C. Lang, Suzanne

  10. Synchrotron X-ray Scattering Studies of Rapidly Evolving Nanoscale Interfacial Systems /

    E-Print Network [OSTI]

    Dai, Yeling

    2013-01-01

    Stanley. X-ray and neutron scattering from rough surfaces.Stanley. X-ray and neutron scattering from rough surfaces.grazing incidence x-ray and neutron scattering from ordered

  11. Analysis of Order Formation in Block Copolymer Thin Films Using Resonant Soft X-Ray Scattering

    E-Print Network [OSTI]

    Virgili, Justin M.; Tao, Yuefei; Kortright, Jeffrey B.; Balsara, Nitash P.; Segalman, Rachel A.

    2006-01-01

    Methods of X-Ray and Neutron Scattering in Polymer Science.µ t for X-ray and neutron scattering experiments is unity;18 In classical scattering of light, X-rays or neutrons the

  12. X-ray scattering studies of structure and dynamics of surfaces and interfaces of polymeric liquids

    E-Print Network [OSTI]

    Jiang, Zhang

    2007-01-01

    Evanescent X-ray and Neutron Scattering. Springer-Verlag,Methods of X-ray and neutron scattering in polymer science.Stanley. X-ray and neutron scattering from rough surfaces.

  13. National School on Neutron and X-ray Scattering Oak Ridge National Laboratory June 12-26, 2010 Oak Ridge, Tennessee

    E-Print Network [OSTI]

    Pennycook, Steve

    National School on Neutron and X-ray Scattering Oak Ridge National Laboratory June 12-26, 2010 Oak:30 Lecture Inelastic Neutron Scattering B. D. Gaulin McMaster University Lecture Magnetic Scattering B. D Break Break Break Break 9:45 - 10:45 Lecture Continued Inelastic Neutron Scattering B. D. Gaulin Mc

  14. Resonant x-ray magnetic scattering in holmium

    SciTech Connect (OSTI)

    Gibbs, D.

    1991-01-01

    We review the results of resonant x-ray magnetic scattering experiments on the rare earth metal holmium. When the incident incident x-ray energy is tuned near the L{sub III} absorption edge, large resonant enhancements of the magnetic scattering and resonant integer harmonics are observed. These results are analyzed within the theory of x-ray resonance exchange scattering assuming electric dipole (2p {yields} 5d) and quadrupole (2p {yields} 4f) transitions among atomic orbitals. 30 refs., 5 figs.

  15. High performance x-ray anti-scatter grid

    DOE Patents [OSTI]

    Logan, C.M.

    1995-05-23

    Disclosed are an x-ray anti-scatter grid for x-ray imaging, particularly for screening mammography, and method for fabricating same, x-rays incident along a direct path pass through a grid composed of a plurality of parallel or crossed openings, microchannels, grooves, or slots etched in a substrate, such as silicon, having the walls of the microchannels or slots coated with a high opacity material, such as gold, while x-rays incident at angels with respect to the slots of the grid, arising from scatter, are blocked. The thickness of the substrate is dependent on the specific application of the grid, whereby a substrate of the grid for mammography would be thinner than one for chest radiology. Instead of coating the walls of the slots, such could be filed with an appropriate liquid, such as mercury. 4 Figs.

  16. Imaging X-ray Thomson Scattering Spectrometer Design and Demonstration

    SciTech Connect (OSTI)

    Gamboa, E.J.; Huntington, C.M.; Trantham, M.R.; Keiter, P.A; Drake, R.P.; Montgomery, David; Benage, John F.; Letzring, Samuel A.

    2012-05-04

    In many laboratory astrophysics experiments, intense laser irradiation creates novel material conditions with large, one-dimensional gradients in the temperature, density, and ionization state. X-ray Thomson scattering is a powerful technique for measuring these plasma parameters. However, the scattered signal has previously been measured with little or no spatial resolution, which limits the ability to diagnose inhomogeneous plasmas. We report on the development of a new imaging x-ray Thomson spectrometer (IXTS) for the Omega laser facility. The diffraction of x-rays from a toroidally-curved crystal creates high-resolution images that are spatially resolved along a one-dimensional profile while spectrally dispersing the radiation. This focusing geometry allows for high brightness while localizing noise sources and improving the linearity of the dispersion. Preliminary results are presented from a scattering experiment that used the IXTS to measure the temperature profile of a shocked carbon foam.

  17. Operational properties of fluctuation X-ray scattering data

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Malmerberg, Erik; Kerfeld, Cheryl A.; Zwart, Petrus H.

    2015-03-20

    X-ray scattering images collected on timescales shorter than rotation diffusion times using a (partially) coherent beam result in a significant increase in information content in the scattered data. These measurements, named fluctuation X-ray scattering (FXS), are typically performed on an X-ray free-electron laser (XFEL) and can provide fundamental insights into the structure of biological molecules, engineered nanoparticles or energy-related mesoscopic materials beyond what can be obtained with standard X-ray scattering techniques. In order to understand, use and validate experimental FXS data, the availability of basic data characteristics and operational properties is essential, but has been absent up to this point.more »In this communication, an intuitive view of the nature of FXS data and their properties is provided, the effect of FXS data on the derived structural models is highlighted, and generalizations of the Guinier and Porod laws that can ultimately be used to plan experiments and assess the quality of experimental data are presented.« less

  18. Crystal defect studies using x-ray diffuse scattering

    SciTech Connect (OSTI)

    Larson, B.C.

    1980-01-01

    Microscopic lattice defects such as point (single atom) defects, dislocation loops, and solute precipitates are characterized by local electronic density changes at the defect sites and by distortions of the lattice structure surrounding the defects. The effect of these interruptions of the crystal lattice on the scattering of x-rays is considered in this paper, and examples are presented of the use of the diffuse scattering to study the defects. X-ray studies of self-interstitials in electron irradiated aluminum and copper are discussed in terms of the identification of the interstitial configuration. Methods for detecting the onset of point defect aggregation into dislocation loops are considered and new techniques for the determination of separate size distributions for vacancy loops and interstitial loops are presented. Direct comparisons of dislocation loop measurements by x-rays with existing electron microscopy studies of dislocation loops indicate agreement for larger size loops, but x-ray measurements report higher concentrations in the smaller loop range. Methods for distinguishing between loops and three-dimensional precipitates are discussed and possibilities for detailed studies considered. A comparison of dislocation loop size distributions obtained from integral diffuse scattering measurements with those from TEM show a discrepancy in the smaller sizes similar to that described above.

  19. Small-Angle X-Ray Scattering From RNA, Proteins, And Protein...

    Office of Scientific and Technical Information (OSTI)

    Small-Angle X-Ray Scattering From RNA, Proteins, And Protein Complexes Citation Details In-Document Search Title: Small-Angle X-Ray Scattering From RNA, Proteins, And Protein...

  20. X-ray and neutron scattering from nano-mgantic clusters | The...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-ray and neutron scattering from nano-mgantic clusters The student will participate in hands on X-ray scattering experiments on bio-inspired inorganic materials (i.e., magnetic...

  1. In Situ X-Ray Scattering Helps Optimize Printed Solar Cells

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    In Situ X-Ray Scattering Helps Optimize Printed Solar Cells In Situ X-Ray Scattering Helps Optimize Printed Solar Cells Print Wednesday, 25 February 2015 00:00 Plastic solar cells...

  2. National School on Neutron and X-ray Scattering August 10-24, 2013

    E-Print Network [OSTI]

    Kemner, Ken

    National School on Neutron and X-ray Scattering August 10-24, 2013 Argonne National Laboratory National Laboratory 3:15 ­ 3:30 Break #12;National School on Neutron and X-ray Scattering August 10 Dinner Week 1 wrap-up Picnic #12;National School on Neutron and X-ray Scattering August 10-24, 2012 Oak

  3. Week 2 AGENDA: National School on Neutron and X-ray Scattering page 1 of 5 Oak Ridge National Laboratory [9/30/08

    E-Print Network [OSTI]

    Pennycook, Steve

    Week 2 AGENDA: National School on Neutron and X-ray Scattering page 1 of 5 Oak Ridge National Ridge National Laboratory Dean Myles, Director ORNL Neutron Scattering Science Division 1 GROUPS [A,B,C,D,E,F,G,H,I] Iran Thomas Auditorium Lecture Inelastic Neutron Scattering R. Osborn, ANL ALL

  4. National School on Neutron and X-ray Scattering June 14-28, 2014

    E-Print Network [OSTI]

    Kemner, Ken

    National School on Neutron and X-ray Scattering June 14-28, 2014 Argonne National Laboratory:00 Dinner Dinner Dinner Dinner Week 1 wrap-up Picnic #12;National School on Neutron and X-ray Scattering Restaurant 9:45 - 10:45 Lecture Interaction of X-rays and Neutrons with Matter Roger Pynn University

  5. IN SITU SURFACE X-RAY SCATTERING STUDIES OF ELECTROSORPTION

    SciTech Connect (OSTI)

    WANG,J.X.; ADZIC,R.R.; OCKO,B.M.

    1998-07-01

    A short review of the application of surface x-ray scattering techniques to the electrode/electrolyte interfaces is presented. Recent results on metal, halide, and metal-halide adlayers with three specific systems: Bi on Au(100) and Au(110); Br on Au(100) and Ag(100); and the coadsorption of Tl with Br or I on Au(111), are given as an illustration. Factors affecting ordering of pure metal and halide adlayers and the metal-halide surface compounds are discussed in some detail.

  6. Neutron and X-ray Scattering Studies of Strongly Correlated Electron Systems

    E-Print Network [OSTI]

    Boothroyd, Andrew

    Neutron and X-ray Scattering Studies of Strongly Correlated Electron Systems Russell A. Ewings 2008 #12;Abstract Neutron and X-ray Scattering Studies of Strongly Correlated Electron Systems Russell-ray scattering and neutron scattering experiments on several strongly correlated transition metal oxides

  7. Air-core grid for scattered x-ray rejection

    DOE Patents [OSTI]

    Logan, Clinton M. (Pleasanton, CA); Lane, Stephen M. (Oakland, CA)

    1995-01-01

    The invention is directed to a grid used in x-ray imaging applications to block scattered radiation while allowing the desired imaging radiation to pass through, and to process for making the grid. The grid is composed of glass containing lead oxide, and eliminates the spacer material used in prior known grids, and is therefore, an air-core grid. The glass is arranged in a pattern so that a large fraction of the area is open allowing the imaging radiation to pass through. A small pore size is used and the grid has a thickness chosen to provide high scatter rejection. For example, the grid may be produced with a 200 .mu.m pore size, 80% open area, and 4 mm thickness.

  8. Air-core grid for scattered x-ray rejection

    DOE Patents [OSTI]

    Logan, C.M.; Lane, S.M.

    1995-10-03

    The invention is directed to a grid used in x-ray imaging applications to block scattered radiation while allowing the desired imaging radiation to pass through, and to process for making the grid. The grid is composed of glass containing lead oxide, and eliminates the spacer material used in prior known grids, and is therefore, an air-core grid. The glass is arranged in a pattern so that a large fraction of the area is open allowing the imaging radiation to pass through. A small pore size is used and the grid has a thickness chosen to provide high scatter rejection. For example, the grid may be produced with a 200 {micro}m pore size, 80% open area, and 4 mm thickness. 2 figs.

  9. TH SSRL SCHOOL ON SYNCHROTRON X-RAY SCATTERING TECHNIQUES IN...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    TH SSRL SCHOOL ON SYNCHROTRON X-RAY SCATTERING TECHNIQUES IN MATERIALS AND ENVIRONMENTAL SCIENCES: THEORY AND APPLICATION TUESDAY 03 JUNE THURSDAY 05 JUNE 2014 Last update: 02...

  10. Micellar structure from comparison of X-ray and neutron small-angle scattering

    E-Print Network [OSTI]

    Boyer, Edmond

    249 Micellar structure from comparison of X-ray and neutron small-angle scattering T. Zemb and P according to the method developed by Hayter and Penfold. Both X-ray and neutron scattering signals, or by a combination of both. It has been shown recent- ly [1, 2] that it is possible in neutron scattering studies

  11. X-ray and Neutron Scattering Studies of Magnetic Domain Dynamics and Spin Structures /

    E-Print Network [OSTI]

    Chen, San-Wen

    2014-01-01

    Stanley. X-ray and neutron scattering from rough surfaces.1988. [3] R. Pynn. Neutron scattering by rough surfaces at39] V. F. Sears. Neutron scattering lengths and cross

  12. High efficiency of soft X-ray radiation reprocessing in supersoft X-ray sources due to multiple scattering

    E-Print Network [OSTI]

    V. Suleimanov; F. Meyer; E. Meyer-Hofmeister

    2003-02-19

    Detailed analysis of the lightcurve of CAL 87 clearly has shown that the high optical luminosity comes from the accretion disc rim and can only be explained by a severe thickening of the disc rim near the location where the accretion stream impinges. This area is irradiated by the X-rays where it faces the white dwarf. Only if the reprocessing rate of X-rays to optical light is high a luminosity as high as observed can be understood. But a recent detailed study of the soft X-ray radiation reprocessing in supersoft X-ray sources has shown that the efficiency is not high enough. We here propose a solution for this problem. As already discussed in the earlier lightcurve analysis the impact of the accretion stream at the outer disc rim produces a ``spray'', consisting of a large number of individual gas blobs imbedded in a surrounding corona. For the high mass flow rate this constitutes an optically thick vertically extended screen at the rim of the accretion disc. We analyse the optical properties of this irradiated spray and find that the multiple scattering between these gas blobs leads to an effective reprocessing of soft X-rays to optical light as required by the observations.

  13. White dwarfs as the maximal soft x-ray scatterers

    SciTech Connect (OSTI)

    Akbari-Moghanjoughi, M. [Department of Physics, Faculty of Sciences, Azarbaijan Shahid Madani University, 51745-406 Tabriz (Iran, Islamic Republic of) [Department of Physics, Faculty of Sciences, Azarbaijan Shahid Madani University, 51745-406 Tabriz (Iran, Islamic Republic of); International Centre for Advanced Studies in Physical Sciences and Institute for Theoretical Physics, Ruhr University Bochum, D-44780 Bochum (Germany)

    2013-09-15

    In this paper, we explore the effect of density on the structure formation and the electromagnetic wave (EMw) elastic scattering on quantum plasmas, using the generalized quantum hydrodynamic model valid for a wide range of the plasma density and relativistic degeneracy. It is found that the electron quantum diffraction effect caused by the Bohm potential has a fundamental effect on the ion correlations in a degenerate electron fluid and crystallization in quantum plasmas in the solid-density regime and beyond. The ion correlations and structure formation are shown to be fundamentally affected by the plasma density and the relativistic degeneracy parameters. Moreover, distinct behavior is shown to exist between the non-relativistic and relativistic matter density regimes, regarding the normalized EMw elastic scattering cross-sections. It is theoretically discovered that the maximal Thomson scattering coincides with the average density of a typical white dwarf corresponding to the soft X-ray wavelength regime. Current research can be very useful in plasma optical diagnostic methods for a wide range of electron number-density from warm dense matter and inertial confinement fusion to the astrophysical compact objects.

  14. X-ray crystal structure and small-angle X-ray scattering of sheep liver sorbitol dehydrogenase

    SciTech Connect (OSTI)

    Yennawar, Hemant [Pennsylvania State University, 8 Althouse Laboratory, University Park, PA 16802 (United States); Møller, Magda [Cornell High Energy Synchrotron Source, Ithaca, NY 14853 (United States); University of Copenhagen, DK-2100 Copenhagen (Denmark); Gillilan, Richard [Cornell High Energy Synchrotron Source, Ithaca, NY 14853 (United States); Yennawar, Neela, E-mail: nhy1@psu.edu [Pennsylvania State University, 8 Althouse Laboratory, University Park, PA 16802 (United States)

    2011-05-01

    The X-ray crystal structure and a small-angle X-ray scattering solution structure of sheep liver sorbitol dehydrogenase have been determined. The details of the interactions that enable the tetramer scaffold to be the functional biological unit have been analyzed. The X-ray crystal structure of sheep liver sorbitol dehydrogenase (slSDH) has been determined using the crystal structure of human sorbitol dehydrogenase (hSDH) as a molecular-replacement model. slSDH crystallized in space group I222 with one monomer in the asymmetric unit. A conserved tetramer that superposes well with that seen in hSDH (despite belonging to a different space group) and obeying the 222 crystal symmetry is seen in slSDH. An acetate molecule is bound in the active site, coordinating to the active-site zinc through a water molecule. Glycerol, a substrate of slSDH, also occupies the substrate-binding pocket together with the acetate designed by nature to fit large polyol substrates. The substrate-binding pocket is seen to be in close proximity to the tetramer interface, which explains the need for the structural integrity of the tetramer for enzyme activity. Small-angle X-ray scattering was also used to identify the quaternary structure of the tetramer of slSDH in solution.

  15. Resonant Soft X-Ray Scattering - Combining Structural with Spectroscop...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    spectroscopy has become an important tool in understanding the electronic structure of materials. Resonant absorption edges in the soft x-ray regime are especially interesting...

  16. Acquisition of an In-House X-ray Scattering Facility for Nanostructure Characterization and Student Training

    SciTech Connect (OSTI)

    Schuller, Ivan K [UC San Diego

    2013-08-02

    This equipment grant was specifically dedicated to the development of a "state of the art" x-ray scattering facility...

  17. X-ray scattered halo around IGR J17544–2619

    SciTech Connect (OSTI)

    Mao, Junjie; Ling, Zhixing; Zhang, Shuang-Nan, E-mail: zhangsn@ihep.ac.cn [National Astronomical Observatories, Chinese Academy of Sciences, Beijing 100012 (China)

    2014-04-10

    X-ray photons coming from an X-ray point source not only arrive at the detector directly, but also can be strongly forward-scattered by the interstellar dust along the line of sight (LOS), leading to a detectable diffuse halo around the X-ray point source. The geometry of small-angle X-ray scattering is straightforward, namely, the scattered photons travel longer paths and thus arrive later than the unscattered ones; thus, the delay time of X-ray scattered halo photons can reveal information of the distances of the interstellar dust and the point source. Here we present a study of the X-ray scattered halo around IGR J17544–2619, which is one of the so-called supergiant fast X-ray transients. IGR J17544–2619 underwent a striking outburst when observed with Chandra on 2004 July 3, providing a near ?-function light curve. We find that the X-ray scattered halo around IGR J17544–2619 is produced by two interstellar dust clouds along the LOS. The one that is closer to the observer gives the X-ray scattered halo at larger observational angles, whereas the farther one, which is in the vicinity of the point source, explains the halo with a smaller angular size. By comparing the observational angle of the scattered halo photons with that predicted by different dust grain models, we are able to determine the normalized dust distance. With the delay times of the scattered halo photons, we can determine the point source distance, given a dust grain model. Alternatively, we can discriminate between the dust grain models, if the point source distance is known independently.

  18. 16th National School on Neutron and X-ray Scattering

    SciTech Connect (OSTI)

    Chakoumakos, Bryan; Achilles, Cherie; Cybulskis, Viktor; Gilbert, Ian

    2014-07-02

    Students talk about their experience at the 16th National School on Neutron and X-ray Scattering, or NXS 2014. Jointly conducted by Oak Ridge and Argonne national laboratories, NXS immerses graduate students in national user facilities to learn in a hands-on environment how to use neutrons and X-rays in their research.

  19. 16th National School on Neutron and X-ray Scattering

    ScienceCinema (OSTI)

    Chakoumakos, Bryan; Achilles, Cherie; Cybulskis, Viktor; Gilbert, Ian

    2014-07-23

    Students talk about their experience at the 16th National School on Neutron and X-ray Scattering, or NXS 2014. Jointly conducted by Oak Ridge and Argonne national laboratories, NXS immerses graduate students in national user facilities to learn in a hands-on environment how to use neutrons and X-rays in their research.

  20. SXST 2014 - 7th SSRL School on Synchrotron X-Ray Scattering Techniques

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    x-ray scattering. The school will address topics that are not commonly included in text books or class lectures, and typically obtained only through on-the-experiment training....

  1. X-ray and neutron scattering studies of the complex compounds...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-ray and neutron scattering studies of the complex compounds Wednesday, September 25, 2013 - 1:00pm SLAC, Conference Room 137-322 Presented by Dr. Hoyoung Jang, Max Planck...

  2. Safety & Security Guidelines Annual U.S. National School on Neutron and X-ray Scattering

    E-Print Network [OSTI]

    Safety & Security Guidelines 15th Annual U.S. National School on Neutron and X-ray Scattering-574-4600. Neutron Sciences User Programs and Outreach Office Oak Ridge National Laboratory #12;

  3. X-ray small-angle scattering from sputtered CeO{sub 2}/C bilayers

    SciTech Connect (OSTI)

    Haviar, S.; Dubau, M.; Khalakhan, I.; Vorokhta, M.; Matolinova, I.; Matolin, V.; Vales, V.; Endres, J.; Holy, V.; Buljan, M.; Bernstorff, S.

    2013-01-14

    Surface and interface morphology of cerium oxide/carbon bilayers used as thin-film catalysts is studied by grazing-incidence small-angle x-ray scattering, scanning electron microscopy, and atomic-force microscopy, and the dependence of the structural parameters on the thicknesses of the constituting layers is investigated. The applicability of x-ray scattering and its advantages over standard analytical methods are discussed.

  4. Resonant Inelastic Scattering Spectra of Free Molecules with Vibrational Resolution

    SciTech Connect (OSTI)

    Hennies, Franz; Pietzsch, Annette; Berglund, Martin; Foehlisch, Alexander; Schmitt, Thorsten; Strocov, Vladimir; Karlsson, Hans O.; Andersson, Joakim; Rubensson, Jan-Erik

    2010-05-14

    Inelastic x-ray scattering spectra excited at the 1s{sup -1{pi}}* resonance of gas phase O{sub 2} have been recorded with an overall energy resolution that allows for well-resolved vibrational progressions. The nuclear wave packet dynamics in the intermediate state is reflected in vibrational excitations of the electronic ground state, and by fine-tuning the excitation energy the dissociation dynamics in the predissociative B{sup '} {sup 3{Pi}}{sub g} final state is controlled.

  5. X-RAY SCATTERING ECHOES AND GHOST HALOS FROM THE INTERGALACTIC MEDIUM: RELATION TO THE NATURE OF AGN VARIABILITY

    E-Print Network [OSTI]

    Corrales, Lia

    X-ray bright quasars might be used to trace dust in the circumgalactic and intergalactic medium through the phenomenon of X-ray scattering, which is observed around Galactic objects whose light passes through a sufficient ...

  6. Neutron inelastic scattering in natural Pb as a background in...

    Office of Scientific and Technical Information (OSTI)

    Neutron inelastic scattering in natural Pb as a background in neutrinoless double-beta decay experiments Citation Details In-Document Search Title: Neutron inelastic scattering in...

  7. Probing warm dense lithium by inelastic X-ray scattering

    E-Print Network [OSTI]

    Loss, Daniel

    of warm dense matter states has practical applications for controlled thermonuclear fusion, where, Rutherford Appleton Laboratory, Chilton, Didcot, OX11 0QX, UK 4 Centre for Fusion, Space and Astrophysics

  8. Multiplet resonance lifetimes in resonant inelastic x-ray scattering

    Office of Scientific and Technical Information (OSTI)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantity of NaturalDukeWakefieldSulfate Reducing(JournalspectroscopyReport)Fermentativea(Patent) | SciTech

  9. International Conference on Surface X-ray and Neutron Scattering (SXNS-11)

    SciTech Connect (OSTI)

    Michael J. Bedzyk

    2011-06-17

    The 11th International Surface X-ray and Neutron Scattering (SXNS) Conference was held on July 13-17, 2010, on the Northwestern University (NU) campus, in Evanston Illinois and hosted by the NU Materials Research Science and Engineering Center. This biennial conference brought together a community of 164 attendees from 16 countries. The field now makes use of a broad range of new experimental capabilities that have been made possible through the development of increasingly brilliant X-ray and neutron sources around the world, including third generation synchrotron sources, neutron reactor and spallation sources, as well as the recent development of X-ray lasers.

  10. X-ray scattering of assembled nano-particles | The Ames Laboratory

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power AdministrationRobust,Field-effectWorkingLos Alamos verifies largest single goldWindX-RayX-RayX-ray scattering

  11. INELASTIC LIGHT SCATTERING STUDIES OF BOROCARBIDE SUPERCONDUCTORS

    E-Print Network [OSTI]

    Yang, In-Sang

    INELASTIC LIGHT SCATTERING STUDIES OF BOROCARBIDE SUPERCONDUCTORS IN­SANG YANG Department In recent years of studies in ``unconventional'' superconductivity, researchers have concentrated on exotic behavior of the heavy fermion and cuprate su­ perconductors. However, even superconductors that are thought

  12. HIV-1 Tat membrane interactions probed using X-ray and neutron scattering, CD spectroscopy and MD simulations

    E-Print Network [OSTI]

    Nagle, John F.

    HIV-1 Tat membrane interactions probed using X-ray and neutron scattering, CD spectroscopy and MD translocation, were provided by wide-angle X-ray scattering (WAXS) and neutron scattering. CD spectroscopy for Neutron Research, 100 Bureau Drive, Stop 6102, Gaithersburg, MD 20899, United States d CHESS, Cornell

  13. Exact limiting relation between the structure factors in neutron and x-ray scattering

    E-Print Network [OSTI]

    V. B. Bobrov; S. A. Trigger; S. N. Skovorod'ko

    2010-07-11

    The ratio of the static matter structure factor measured in experiments on coherent X-ray scattering to the static structure factor measured in experiments on neutron scattering is considered. It is shown theoretically that this ratio in the long-wavelength limit is equal to the nucleus charge at arbitrary thermodynamic parameters of a pure substance (the system of nuclei and electrons, where interaction between particles is pure Coulomb) in a disordered equilibrium state. This result is the exact relation of the quantum statistical mechanics. The experimental verification of this relation can be done in the long wavelength X-ray and neutron experiments.

  14. Magnetism studies using resonant, coherent, x-ray scattering...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    where the scattering vector q that can only be reached in reflection. The method is Fourier transform holography, where the exit wave from a sample interferes with a reference...

  15. UNIVERSITY OF CALIFORNIA Inelastic Neutron Scattering Study of the

    E-Print Network [OSTI]

    Lawrence, Jon

    UNIVERSITY OF CALIFORNIA IRVINE Inelastic Neutron Scattering Study of the Intermediate Valence . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2.2 Inelastic Neutron Scattering . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2.2.a Neutron Scattering Instruments . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 2.2.b

  16. Kevin Yager on the Nanoscience of Studying Scattered X-Rays

    ScienceCinema (OSTI)

    Yager; Kevin

    2014-06-04

    Kevin Yager, a scientist at Brookhaven Lab's Center for Functional Nanomaterials, discusses his research on materials spanning just billionths of a meter. Yager specializes in making new materials through meticulously guided self-assembly and probing nanoscale structures with a technique called x-ray scattering.

  17. Resonance scattering in X-ray line profiles of Pup Clumping in Hot Star Winds

    E-Print Network [OSTI]

    Cohen, David

    Resonance scattering in X-ray line profiles of Pup Clumping in Hot Star Winds W.-R. Hamann, A the same wind parameters. We show that the differences in profile shape can be accounted for in a model its effect is difficult to distinguish from a low effective continuum optical depth in the wind. Thus

  18. X-ray Thomson scattering measurements of temperature and density from multi-shocked CH capsules

    SciTech Connect (OSTI)

    Fletcher, L. B. [Department of Physics, University of California, Berkeley, California 94720 (United States)] [Department of Physics, University of California, Berkeley, California 94720 (United States); Kritcher, A.; Pak, A.; Ma, T.; Döppner, T.; Divol, L.; Landen, O. L.; Glenzer, S. H. [Lawrence Livermore National Laboratory, 7000 East Av., Livermore, California 94550 (United States)] [Lawrence Livermore National Laboratory, 7000 East Av., Livermore, California 94550 (United States); Fortmann, C. [Lawrence Livermore National Laboratory, 7000 East Av., Livermore, California 94550 (United States) [Lawrence Livermore National Laboratory, 7000 East Av., Livermore, California 94550 (United States); University of California, Los Angeles, California 90095 (United States); Vorberger, J.; Gericke, D. O. [Department of Physics, Centre for Fusion, Space, and Astrophysics, University of Warwick, Coventry CV4 7AL (United Kingdom)] [Department of Physics, Centre for Fusion, Space, and Astrophysics, University of Warwick, Coventry CV4 7AL (United Kingdom); Chapman, D. A. [Department of Physics, Centre for Fusion, Space, and Astrophysics, University of Warwick, Coventry CV4 7AL (United Kingdom) [Department of Physics, Centre for Fusion, Space, and Astrophysics, University of Warwick, Coventry CV4 7AL (United Kingdom); Plasma Physics Department, AWE plc, Aldermaston (United Kingdom); Falcone, R. W. [Department of Physics, University of California, Berkeley, California 94720 (United States) [Department of Physics, University of California, Berkeley, California 94720 (United States); Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States)

    2013-05-15

    Proof-of-principle measurements of the electron densities, temperatures, and ionization states of spherically compressed multi-shocked CH (polystyrene) capsules have been achieved using spectrally resolved x-ray Thomson scattering. A total energy of 13.5 kJ incident on target is used to compress a 70 ?m thick CH shell above solid-mass density using three coalescing shocks. Separately, a laser-produced zinc He-? x-ray source at 9 keV delayed 200 ps-800 ps after maximum compression is used to probe the plasma in the non-collective scattering regime. The data show that x-ray Thomson scattering enables a complete description of the time-dependent hydrodynamic evolution of shock-compressed CH capsules, with a maximum measured density of ? > 6 g cm{sup ?3}. In addition, the results demonstrate that accurate measurements of x-ray scattering from bound-free transitions in the CH plasma demonstrate strong evidence that continuum lowering is the primary ionization mechanism of carbon L-shell electrons.

  19. Alamethicin in lipid bilayers: Combined use of X-ray scattering and MD simulations Jianjun Pan a

    E-Print Network [OSTI]

    Nagle, John F.

    Alamethicin in lipid bilayers: Combined use of X-ray scattering and MD simulations Jianjun Pan of Biological Sciences, Carnegie Mellon University, Pittsburgh, PA 15213, USA d Canadian Neutron Beam Centre:1PC with varying amounts of alamethicin (Alm). We combine the use of X-ray diffuse scattering

  20. Structure Matters: Combining X-Ray Scattering and Ultraviolet Photoelectron

    E-Print Network [OSTI]

    Schreiber, Frank

    such structural data and electronic information from UPS new insights in the fundamental principles of organic Institute for Applied Physics, University of Tu¨bingen, Auf der Morgenstelle 10, 2076 Tu¨bingen, Germany e within the framework of dynamical scattering theory with a recursive formalism described by Parratt [6

  1. Neutron inelastic scattering in natural Pb as a background in...

    Office of Scientific and Technical Information (OSTI)

    SCATTERING; ISOTOPES; LEAD; LEAD 206; LEAD 207; LEVELS; NEUTRONS; SCATTERING Inelastic neutron scattering on Pb isotopes can result in gamma rays near the signature endpoint...

  2. Analysis of microroughness evolution in X-ray astronomical multilayer mirrors by surface topography with the MPES program and by X-ray scattering

    E-Print Network [OSTI]

    Canestrari, R; Pareschi, G

    2015-01-01

    Future hard X-ray telescopes (e.g. SIMBOL-X and Constellation-X) will make use of hard X-ray optics with multilayer coatings, with angular resolutions comparable to the achieved ones in the soft X-rays. One of the crucial points in X-ray optics, indeed, is multilayer interfacial microroughness that causes effective area reduction and X-Ray Scattering (XRS). The latter, in particular, is responsible for image quality degradation. Interfacial smoothness deterioration in multilayer deposition processes is commonly observed as a result of substrate profile replication and intrinsic random deposition noise. For this reason, roughness growth should be carefully investigated by surface topographic analysis, X-ray reflectivity and XRS measurements. It is convenient to express the roughness evolution in terms of interface Power Spectral Densities (PSD), that are directly related to XRS and, in turn, in affecting the optic HEW (Half Energy Width). In order to interpret roughness amplification and to help us to predict ...

  3. Predicting X-ray diffuse scattering from translation–libration–screw structural ensembles

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Van Benschoten, Andrew H.; Afonine, Pavel V.; Terwilliger, Thomas C.; Wall, Michael E.; Jackson, Colin J.; Sauter, Nicholas K.; Adams, Paul D.; Urzhumtsev, Alexandre; Fraser, James S.

    2015-07-28

    Identifying the intramolecular motions of proteins and nucleic acids is a major challenge in macromolecular X-ray crystallography. Because Bragg diffraction describes the average positional distribution of crystalline atoms with imperfect precision, the resulting electron density can be compatible with multiple models of motion. Diffuse X-ray scattering can reduce this degeneracy by reporting on correlated atomic displacements. Although recent technological advances are increasing the potential to accurately measure diffuse scattering, computational modeling and validation tools are still needed to quantify the agreement between experimental data and different parameterizations of crystalline disorder. A new tool, phenix.diffuse, addresses this need by employing Guinier'smore »equation to calculate diffuse scattering from Protein Data Bank (PDB)-formatted structural ensembles. As an example case, phenix.diffuse is applied to translation–libration–screw (TLS) refinement, which models rigid-body displacement for segments of the macromolecule. To enable the calculation of diffuse scattering from TLS-refined structures, phenix.tls_as_xyz builds multi-model PDB files that sample the underlying T, L and S tensors. In the glycerophosphodiesterase GpdQ, alternative TLS-group partitioning and different motional correlations between groups yield markedly dissimilar diffuse scattering maps with distinct implications for molecular mechanism and allostery. These methods demonstrate how, in principle, X-ray diffuse scattering could extend macromolecular structural refinement, validation and analysis.« less

  4. BIOISIS: Biological Macromolecules by Small Angle X-ray Scattering (SAXS)

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Tainer, John [Scripps Research Institute; Hura, Greg [LBNL; Rambo, Robert P. [LBNL

    BIOISIS is an open access database dedicated to the study of biological macromolecules by small angle X-ray scattering (SAXS). BIOISIS aims to become the complete source for the deposition, distribution and maintenance of small angle X-ray scattering data and technologies. The database is designed around the concept of an ôexperimentö and relates a specific experiment to a set of genes, organisms, computational models and experimental data. As of May 2012, BIOSIS contains 7,118 genes covering four different organisms. Forty-two modeled structures are available. Clicking on a structures reveals scattering curves, experimental conditions, and experimental values. The data are collected at Beamline 12.3.1 of the Advanced Light Source (ALS).[Copied with editing from http://www.bioisis.net/about

  5. SU-E-I-01: A Fast, Analytical Pencil Beam Based Method for First Order X-Ray Scatter Estimation of Kilovoltage Cone Beam X-Rays

    SciTech Connect (OSTI)

    Liu, J; Bourland, J [Wake Forest University, Winston-salem, NC (United States)

    2014-06-01

    Purpose: To analytically estimate first-order x-ray scatter for kV cone beam x-ray imaging with high computational efficiency. Methods: In calculating first-order scatter using the Klein-Nishina formula, we found that by integrating the point-to-point scatter along an interaction line, a “pencil-beam” scatter kernel (BSK) can be approximated to a quartic expression when the imaging field is small. This BSK model for monoenergetic, 100keV x-rays has been verified on homogeneous cube and cylinder water phantoms by comparing with the exact implementation of KN formula. For heterogeneous medium, the water-equivalent length of a BSK was acquired with an improved Siddon's ray-tracing algorithm, which was also used in calculating pre- and post- scattering attenuation. To include the electron binding effect for scattering of low-kV photons, the mean corresponding scattering angle is determined from the effective point of scattered photons of a BSK. The behavior of polyenergetic x-rays was also investigated for 120kV x-rays incident to a sandwiched infinite heterogeneous slab phantom, with the electron binding effect incorporated. Exact computation and Monte Carlo simulations were performed for comparisons, using the EGSnrc code package. Results: By reducing the 3D volumetric target (o(n{sup 3})) to 2D pencil-beams (o(n{sup 2})), the computation expense can be generally lowered by n times, which our experience verifies. The scatter distribution on a flat detector shows high agreement between the analytic BSK model and exact calculations. The pixel-to-pixel differences are within (-2%, 2%) for the homogeneous cube and cylinder phantoms and within (0, 6%) for the heterogeneous slab phantom. However, the Monte Carlo simulation shows increased deviation of the BSK model toward detector periphery. Conclusion: The proposed BSK model, accommodating polyenergetic x-rays and electron binding effect at low kV, shows great potential in efficiently estimating the first-order scatter from small imaging fields. We are investigating more thoroughly to improve performance and explore applications.

  6. Large-scale Nanostructure Simulations from X-ray Scattering Data On Graphics Processor Clusters

    SciTech Connect (OSTI)

    Sarje, Abhinav; Pien, Jack; Li, Xiaoye; Chan, Elaine; Chourou, Slim; Hexemer, Alexander; Scholz, Arthur; Kramer, Edward

    2012-01-15

    X-ray scattering is a valuable tool for measuring the structural properties of materialsused in the design and fabrication of energy-relevant nanodevices (e.g., photovoltaic, energy storage, battery, fuel, and carbon capture andsequestration devices) that are key to the reduction of carbon emissions. Although today's ultra-fast X-ray scattering detectors can provide tremendousinformation on the structural properties of materials, a primary challenge remains in the analyses of the resulting data. We are developing novelhigh-performance computing algorithms, codes, and software tools for the analyses of X-ray scattering data. In this paper we describe two such HPCalgorithm advances. Firstly, we have implemented a flexible and highly efficient Grazing Incidence Small Angle Scattering (GISAXS) simulation code based on theDistorted Wave Born Approximation (DWBA) theory with C++/CUDA/MPI on a cluster of GPUs. Our code can compute the scattered light intensity from any givensample in all directions of space; thus allowing full construction of the GISAXS pattern. Preliminary tests on a single GPU show speedups over 125x compared tothe sequential code, and almost linear speedup when executing across a GPU cluster with 42 nodes, resulting in an additional 40x speedup compared to usingone GPU node. Secondly, for the structural fitting problems in inverse modeling, we have implemented a Reverse Monte Carlo simulation algorithm with C++/CUDAusing one GPU. Since there are large numbers of parameters for fitting in the in X-ray scattering simulation model, the earlier single CPU code required weeks ofruntime. Deploying the AccelerEyes Jacket/Matlab wrapper to use GPU gave around 100x speedup over the pure CPU code. Our further C++/CUDA optimization deliveredan additional 9x speedup.

  7. Wide angle x-ray scattering of proteins : effect of beam exposure on protein integrity.

    SciTech Connect (OSTI)

    Fischetti, R. F.; Rodi, D. J.; Mirza, A.; Makowski, L.; Illinois Inst. of Tech.

    2003-01-01

    Wide-angle X-ray scattering patterns from proteins in solution contain information relevant to the determination of protein fold. At relevant scattering angles, however, these data are weak, and the degree to which they might be used to categorize the fold of a protein is unknown. Preliminary work has been performed at the BioCAT insertion-device beamline at the Advanced Photon Source which demonstrates that one can collect X-ray scattering data from proteins in solution to spacings of at least 2.2 {angstrom} (q = 2.8 {angstrom}-1). These data are sensitive to protein conformational states, and are in good agreement with the scattering predicted by the program CRYSOL using the known three-dimensional atomic coordinates of the protein. An important issue in the exploitation of this technique as a tool for structural genomics is the extent to which the high intensity of X-rays available at third-generation synchrotron sources chemically or structurally damage proteins. Various data-collection protocols have been investigated demonstrating conditions under which structural degradation of even sensitive proteins can be minimized, making this technique a viable tool for protein fold categorization, the study of protein folding, unfolding, protein-ligand interactions and domain movement.

  8. Deep Inelastic Scattering -- Theory and Phenomenology

    E-Print Network [OSTI]

    B. R. Webber

    1996-07-26

    Recent developments in theory and phenomenology relevant to deep inelastic lepton scattering are reviewed, concentrating on the following topics: Predicted behaviour of non-singlet and polarized structure functions at small $x$; Theoretical studies of saturation and unitarity effects at small $x$ in quarkonium scattering; Renormalons and higher twist contributions; Next-to-leading-order calculations of jet cross sections; Forward jet production as a probe of small-$x$ dynamics.

  9. Scattering Theory When an x-ray beam (or neutron or light) passes through a material with

    E-Print Network [OSTI]

    Beaucage, Gregory

    Scattering Theory When an x-ray beam (or neutron or light) passes through a material radiation is scattered in directions that differ from that of the incident beam. Scattering arises since x of scattered radiation resulting from this process bears a direct relationship to the structure (the pattern

  10. Compact x-ray source based on burst-mode inverse Compton scattering at 100 kHz

    E-Print Network [OSTI]

    Bessuille, J.

    A design for a compact x-ray light source (CXLS) with flux and brilliance orders of magnitude beyond existing laboratory scale sources is presented. The source is based on inverse Compton scattering of a high brightness ...

  11. X-ray Dust Scattering at Small Angles: The Complete Halo around GX13+1

    E-Print Network [OSTI]

    Randall K. Smith

    2008-05-04

    The exquisite angular resolution available with Chandra should allow precision measurements of faint diffuse emission surrounding bright sources, such as the X-ray scattering halos created by interstellar dust. However, the ACIS CCDs suffer from pileup when observing bright sources, and this creates difficulties when trying to extract the scattered halo near the source. The initial study of the X-ray halo around GX13+1 using only the ACIS-I detector done by Smith, Edgar & Shafer (2002) suffered from a lack of sensitivity within 50'' of the source, limiting what conclusions could be drawn. To address this problem, observations of GX13+1 were obtained with the Chandra HRC-I and simultaneously with the RXTE PCA. Combined with the existing ACIS-I data, this allowed measurements of the X-ray halo between 2-1000''. After considering a range of dust models, each assumed to be smoothly distributed with or without a dense cloud along the line of sight, the results show that there is no evidence in this data for a dense cloud near the source, as suggested by Xiang et al. (2005). Finally, although no model leads to formally acceptable results, the Weingartner & Draine (2001) and nearly all of the composite grain models from Zubko, Dwek & Arendt (2004) give poor fits.

  12. Inclusive Deep-Inelastic Scattering at HERA

    E-Print Network [OSTI]

    Zhiqing Zhang; for the H1; ZEUS Collaborations

    2014-12-19

    This contribution covers three recent results on deep-inelastic scattering at HERA: (i) new measurements of the proton longitudinal structure function $F_L$ from H1 and ZEUS experiments, (ii) a dedicated NC cross section measurement from ZEUS in the region of high Bjorken $x$, and (iii) preliminary combination results of all HERA inclusive data published up to now by H1 and ZEUS, taking into account the experimental correlations between measurements.

  13. Theoretical treatments of the bound-free contribution and experimental best practice in X-ray Thomson scattering from warm dense matter

    SciTech Connect (OSTI)

    Mattern, Brian A.; Seidler, Gerald T. [Department of Physics, University of Washington, Seattle, Washington 98195-1560 (United States)

    2013-02-15

    By comparison with high-resolution synchrotron x-ray experimental results, we assess several theoretical treatments for the bound-free (core-electron) contribution to x-ray Thomson scattering (i.e., also known as nonresonant inelastic x-ray scattering). We identify an often overlooked source of systematic error in the plane-wave form factor approximation (PWFFA) used in the inference of temperature, ionization state, and free electron density in some laser-driven compression studies of warm dense matter. This error is due to a direct violation of energy conservation in the PWFFA. We propose an improved practice for the bound-free term that will be particularly relevant for XRTS experiments performed with somewhat improved energy resolution at the National Ignition Facility or the Linac Coherent Light Source. Our results raise important questions about the accuracy of state variable determination in XRTS studies, given that the limited information content in low-resolution XRTS spectra does not strongly constrain the models of electronic structure being used to fit the spectra.

  14. Eur. J. Biochem. 85, 529-534 (1978) X-Ray and Neutron Small-Angle Scattering Studies

    E-Print Network [OSTI]

    1978-01-01

    Eur. J. Biochem. 85, 529-534 (1978) X-Ray and Neutron Small-Angle Scattering Studies of the Complex-ray and neutron scattering techniques. In this work, we concentrated mainly on radius of gyration analyses and a neutron scattering experiment is performed in 21-Iz0 solvent. This decrease simply reflects the fact

  15. Z .Reviews in Molecular Biotechnology 74 2000 207 231 X-ray and neutron surface scattering for studying

    E-Print Network [OSTI]

    Wong, Joyce

    Z .Reviews in Molecular Biotechnology 74 2000 207 231 X-ray and neutron surface scattering,U , Tonya L. Kuhlb , Joyce Y. Wongc , Gregory S. Smitha,1 a Manuel Lujan Jr. Neutron Scattering Center is defined as the Zratio of the number of particles neutrons or .photons elastically and specularly scattered

  16. The accurate assessment of small-angle X-ray scattering data

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Grant, Thomas D.; Luft, Joseph R.; Carter, Lester G.; Matsui, Tsutomu; Weiss, Thomas M.; Martel, Anne; Snell, Edward H.

    2015-01-23

    Small-angle X-ray scattering (SAXS) has grown in popularity in recent times with the advent of bright synchrotron X-ray sources, powerful computational resources and algorithms enabling the calculation of increasingly complex models. However, the lack of standardized data-quality metrics presents difficulties for the growing user community in accurately assessing the quality of experimental SAXS data. Here, a series of metrics to quantitatively describe SAXS data in an objective manner using statistical evaluations are defined. These metrics are applied to identify the effects of radiation damage, concentration dependence and interparticle interactions on SAXS data from a set of 27 previously described targetsmore »for which high-resolution structures have been determined via X-ray crystallography or nuclear magnetic resonance (NMR) spectroscopy. Studies show that these metrics are sufficient to characterize SAXS data quality on a small sample set with statistical rigor and sensitivity similar to or better than manual analysis. The development of data-quality analysis strategies such as these initial efforts is needed to enable the accurate and unbiased assessment of SAXS data quality.« less

  17. The accurate assessment of small-angle X-ray scattering data

    SciTech Connect (OSTI)

    Grant, Thomas D. [Hauptman–Woodward Medical Research Institute, 700 Ellicott Street, Buffalo, NY 14203 (United States); Luft, Joseph R. [Hauptman–Woodward Medical Research Institute, 700 Ellicott Street, Buffalo, NY 14203 (United States); SUNY Buffalo, 700 Ellicott Street, Buffalo, NY 14203 (United States); Carter, Lester G.; Matsui, Tsutomu; Weiss, Thomas M.; Martel, Anne [Stanford Synchrotron Radiation Lightsource, 2575 Sand Hill Road, MS69, Menlo Park, CA 94025 (United States); Snell, Edward H., E-mail: esnell@hwi.buffalo.edu [Hauptman–Woodward Medical Research Institute, 700 Ellicott Street, Buffalo, NY 14203 (United States); SUNY Buffalo, 700 Ellicott Street, Buffalo, NY 14203 (United States)

    2015-01-01

    A set of quantitative techniques is suggested for assessing SAXS data quality. These are applied in the form of a script, SAXStats, to a test set of 27 proteins, showing that these techniques are more sensitive than manual assessment of data quality. Small-angle X-ray scattering (SAXS) has grown in popularity in recent times with the advent of bright synchrotron X-ray sources, powerful computational resources and algorithms enabling the calculation of increasingly complex models. However, the lack of standardized data-quality metrics presents difficulties for the growing user community in accurately assessing the quality of experimental SAXS data. Here, a series of metrics to quantitatively describe SAXS data in an objective manner using statistical evaluations are defined. These metrics are applied to identify the effects of radiation damage, concentration dependence and interparticle interactions on SAXS data from a set of 27 previously described targets for which high-resolution structures have been determined via X-ray crystallography or nuclear magnetic resonance (NMR) spectroscopy. The studies show that these metrics are sufficient to characterize SAXS data quality on a small sample set with statistical rigor and sensitivity similar to or better than manual analysis. The development of data-quality analysis strategies such as these initial efforts is needed to enable the accurate and unbiased assessment of SAXS data quality.

  18. Protein folding and protein metallocluster studies using synchrotron small angler X-ray scattering

    SciTech Connect (OSTI)

    Eliezer, D.

    1994-06-01

    Proteins, biological macromolecules composed of amino-acid building blocks, possess unique three dimensional shapes or conformations which are intimately related to their biological function. All of the information necessary to determine this conformation is stored in a protein`s amino acid sequence. The problem of understanding the process by which nature maps protein amino-acid sequences to three-dimensional conformations is known as the protein folding problem, and is one of the central unsolved problems in biophysics today. The possible applications of a solution are broad, ranging from the elucidation of thousands of protein structures to the rational modification and design of protein-based drugs. The scattering of X-rays by matter has long been useful as a tool for the characterization of physical properties of materials, including biological samples. The high photon flux available at synchrotron X-ray sources allows for the measurement of scattering cross-sections of dilute and/or disordered samples. Such measurements do not yield the detailed geometrical information available from crystalline samples, but do allow for lower resolution studies of dynamical processes not observable in the crystalline state. The main focus of the work described here has been the study of the protein folding process using time-resolved small-angle x-ray scattering measurements. The original intention was to observe the decrease in overall size which must accompany the folding of a protein from an extended conformation to its compact native state. Although this process proved too fast for the current time-resolution of the technique, upper bounds were set on the probable compaction times of several small proteins. In addition, an interesting and unexpected process was detected, in which the folding protein passes through an intermediate state which shows a tendency to associate. This state is proposed to be a kinetic molten globule folding intermediate.

  19. Imaging method based on attenuation, refraction and ultra-small-angle-scattering of x-rays

    DOE Patents [OSTI]

    Wernick, Miles N.; Chapman, Leroy Dean; Oltulu, Oral; Zhong, Zhong

    2005-09-20

    A method for detecting an image of an object by measuring the intensity at a plurality of positions of a transmitted beam of x-ray radiation emitted from the object as a function of angle within the transmitted beam. The intensity measurements of the transmitted beam are obtained by a crystal analyzer positioned at a plurality of angular positions. The plurality of intensity measurements are used to determine the angular intensity spectrum of the transmitted beam. One or more parameters, such as an attenuation property, a refraction property and a scatter property, can be obtained from the angular intensity spectrum and used to display an image of the object.

  20. Time Resolved Collapse of a Folding Protein Observed with Small Angle X-Ray Scattering

    SciTech Connect (OSTI)

    Pollack, L.; Tate, M. W.; Finnefrock, A. C.; Kalidas, C.; Trotter, S.; Darnton, N. C.; Lurio, L.; Austin, R. H.; Batt, C. A.; Gruner, S. M. (and others)

    2001-05-21

    High-intensity, ''pink'' beam from an undulator was used in conjunction with microfabricated rapid-fluid mixing devices to monitor the early events in protein folding with time resolved small angle x-ray scattering. This Letter describes recent work on the protein bovine {beta} -lactoglobulin where collapse from an expanded to a compact set of states was directly observed on the millisecond time scale. The role of chain collapse, one of the initial stages of protein folding, is not currently understood. The characterization of transient, compact states is vital in assessing the validity of theories and models of the folding process.

  1. Characterization of porous materials using combined small-angle X-ray and neutron scattering techniques

    SciTech Connect (OSTI)

    Hu, Naiping; Borkar, Neha; Kohls, Doug; Schaefer, Dale W. (UCIN)

    2014-09-24

    A combination of ultra small angle X-ray scattering (USAXS) and ultra small angle neutron scattering (USANS) is used to characterize porous materials. The analysis methods yield quantitative information, including the mean skeletal chord length, mean pore chord length, skeletal density, and composition. A mixed cellulose ester (MCE) membrane with a manufacturer-labeled pore size of 0.1 {mu}m was used as a model to elucidate the specifics of the method. Four approaches describing four specific scenarios (different known parameters and form of the scattering data) are compared. Pore chords determined using all four approaches are in good agreement with the scanning electron microscopy estimates but are larger than the manufacturer's nominal pore size. Our approach also gives the average chord of the skeletal solid (struts) of the membrane, which is also consistent for all four approaches. Combined data from USAXS and USANS gives the skeletal density and the strut composition.

  2. Spectral softening in the X-RAY afterglow of GRB 130925A as predicted by the dust scattering model

    SciTech Connect (OSTI)

    Zhao, Yi-Nan; Shao, Lang, E-mail: lshao@hebtu.edu.cn [Department of Space Science and Astronomy, Hebei Normal University, Shijiazhuang 050024 (China)

    2014-07-01

    Gamma-ray bursts (GRBs) usually occur in a dense star-forming region with a massive circumburst medium. The small-angle scattering of intense prompt X-ray emission off the surrounding dust grains will have observable consequences and sometimes can dominate the X-ray afterglow. In most of the previous studies, only the Rayleigh-Gans (RG) approximation is employed for describing the scattering process, which works accurately for the typical size of grains (with radius of a ? 0.1 ?m) in the diffuse interstellar medium. When the size of the grains may significantly increase, as in a more dense region where GRBs would occur, the RG approximation may not be valid enough for modeling detailed observational data. In order to study the temporal and spectral properties of the scattered X-ray emission more accurately with potentially larger dust grains, we provide a practical approach using the series expansions of anomalous diffraction (AD) approximation based on the complicated Mie theory. We apply our calculations to understand the puzzling X-ray afterglow of recently observed GRB 130925A that showed a significant spectral softening. We find that the X-ray scattering scenarios with either AD or RG approximation adopted could well reproduce both the temporal and spectral profile simultaneously. Given the plateau present in the early X-ray light curve, a typical distribution of smaller grains as in the interstellar medium would be suggested for GRB 130925A.

  3. A New Polyethylene Scattering Law Determined Using Inelastic Neutron Scattering

    SciTech Connect (OSTI)

    Lavelle, Christopher M [ORNL; Liu, C [Oak Ridge National Laboratory (ORNL); Stone, Matthew B [ORNL

    2013-01-01

    Monte Carlo neutron transport codes such as MCNP rely on accurate data for nuclear physics cross-sections to produce accurate results. At low energy, this takes the form of scattering laws based on the dynamic structure factor, S (Q, E). High density polyethylene (HDPE) is frequently employed as a neutron moderator at both high and low temperatures, however the only cross-sections available are for T =300 K, and the evaluation has not been updated in quite some time. In this paper we describe inelastic neutron scattering measurements on HDPE at 5 and 300 K which are used to improve the scattering law for HDPE. We describe the experimental methods, review some of the past HDPE scattering laws, and compare computations using these models to the measured S (Q, E). The total cross-section is compared to available data, and the treatment of the carbon secondary scatterer as a free gas is assessed. We also discuss the use of the measurement itself as a scattering law via the 1 phonon approximation. We show that a scattering law computed using a more detailed model for the Generalized Density of States (GDOS) compares more favorably to this experiment, suggesting that inelastic neutron scattering can play an important role in both the development and validation of new scattering laws for Monte Carlo work.

  4. Inelastic electron-vortex-beam scattering

    E-Print Network [OSTI]

    Ruben Van Boxem; Bart Partoens; Jo Verbeeck

    2015-03-16

    Recent theoretical and experimental developments in the field of electron vortex beam physics have raised questions on what exactly this novelty in the field of electron microscopy (and other fields, such as particle physics) really provides. An important part in the answer to those questions lies in scattering theory. The present investigation explores various aspects of inelastic quantum scattering theory for cylindrically symmetric beams with orbital angular momentum. The model system of Coulomb scattering on a hydrogen atom provides the setting to address various open questions: How is momentum transferred? Do vortex beams selectively excite atoms, and how can one employ vortex beams to detect magnetic transitions? The analytical approach presented here provides answers to these questions. OAM transfer is possible, but not through selective excitation; rather, by pre- and post-selection one can filter out the relevant contributions to a specific signal.

  5. Test of factorization in diffractive deep inelastic scattering...

    Office of Scientific and Technical Information (OSTI)

    Test of factorization in diffractive deep inelastic scattering and photoproduction at HERA Citation Details In-Document Search Title: Test of factorization in diffractive deep...

  6. Supplementary data for HIV-1 Tat membrane interaction probed using X-ray and neutron scattering, CD, and MD simulations

    E-Print Network [OSTI]

    Nagle, John F.

    1 Supplementary data for HIV-1 Tat membrane interaction probed using X-ray and neutron scattering- spacing are linearly related. Figure S3. Neutron scattering from stacks of DOPC:DOPE (3:1)/Tat, x=0 of Physics, Rensselaer Polytechnic Institute, 110 Eighth Street, Troy, NY 12180, 3 NIST Center for Neutron

  7. Flat panel X-ray detector with reduced internal scattering for improved attenuation accuracy and dynamic range

    DOE Patents [OSTI]

    Smith, Peter D. (Santa Fe, NM); Claytor, Thomas N. (White Rock, NM); Berry, Phillip C. (Albuquerque, NM); Hills, Charles R. (Los Alamos, NM)

    2010-10-12

    An x-ray detector is disclosed that has had all unnecessary material removed from the x-ray beam path, and all of the remaining material in the beam path made as light and as low in atomic number as possible. The resulting detector is essentially transparent to x-rays and, thus, has greatly reduced internal scatter. The result of this is that x-ray attenuation data measured for the object under examination are much more accurate and have an increased dynamic range. The benefits of this improvement are that beam hardening corrections can be made accurately, that computed tomography reconstructions can be used for quantitative determination of material properties including density and atomic number, and that lower exposures may be possible as a result of the increased dynamic range.

  8. National School on Neutron and X-ray Scattering Building 223 Auditorium, Room B002 September 24 -October 11, 2008 Argonne National Laboratory

    E-Print Network [OSTI]

    Pennycook, Steve

    National School on Neutron and X-ray Scattering Building 223 Auditorium, Room B002 September 24 (HFIR) Neutron Scattering Science Division Oak Ridge Laboratory 10:15 - 10:30 Break 9:30 - 9:45 Break 10 School on Neutron and X-ray Scattering Building 8600, Main Lobby September 24 - October 11, 2008 Oak

  9. Bent crystal analyzer without grooves for inelastic scattering -- first experimental results

    SciTech Connect (OSTI)

    Kushnir, V.I.; Macrander, A.T.

    1996-11-01

    A new design of a bent crystal analyzer for high energy resolution inelastic X-ray scattering has been recently proposed. It has been theoretically predicted that an analyzer with reflecting planes at a certain angle with respect to a crystal surface, bent with two different radii of curvature, will have the same energy resolution as a perfect crystal. The first experimental measurement obtained at the Advanced Photon Source of a bandwidth of such an analyzer is presented. The overall energy resolution of the analyzer and monochromator observed with a narrow beam is equal to 16.4 meV (FWHM) at 13.84 KeV.

  10. Versatile wide angle diffraction setup for simultaneous wide and small angle x-ray scattering measurements with synchrotron radiation

    SciTech Connect (OSTI)

    Rueda, D.R.; Garcia-Gutierrez, M.C.; Nogales, A.; Capitan, M.J.; Ezquerra, T.A.; Labrador, A.; Fraga, E.; Beltran, D.; Juanhuix, J.; Herranz, J.F.; Bordas, J. [Instituto de Estructura de la Materia, CSIC, Serrano 119, 28006 Madrid (Spain); LLS, BM16-ESRF, 6 rue Jules Horowitz, BP220, 38043 Grenoble (France)

    2006-03-15

    Here we present a novel, simple, and versatile experimental setup aimed to perform wide angle x-ray scattering (WAXS) measurements alone or in simultaneous combination with small angle x-ray scattering measurements. The design of the WAXS goniometer allows one to obtain high resolution diffraction patterns in a broad angular range. The setup can incorporate a hot stage in order to evaluate temperature resolved experiments. The performance of the equipment has been verified in the BM16 beam line of the European Synchrotron Radiation Facility with different well known samples such as alumina, isotropic film of high density polyethylene (HDPE), and oriented HPDE fiber.

  11. Compton scattering for spectroscopic detection of ultra-fast, high flux, broad energy range X-rays

    SciTech Connect (OSTI)

    Cipiccia, S.; Wiggins, S. M.; Brunetti, E.; Vieux, G.; Yang, X.; Welsh, G. H.; Anania, M.; Islam, M. R.; Ersfeld, B.; Jaroszynski, D. A. [Scottish Universities Physics Alliance, Department of Physics, University of Strathclyde, John Anderson Building, 107 Rottenrow, Glasgow G4 0NG (United Kingdom)] [Scottish Universities Physics Alliance, Department of Physics, University of Strathclyde, John Anderson Building, 107 Rottenrow, Glasgow G4 0NG (United Kingdom); Maneuski, D.; Montgomery, R.; Smith, G.; Hoek, M.; Hamilton, D. J.; Shea, V. O. [Scottish Universities Physics Alliance, School of Physics and Astronomy, University of Glasgow, Glasgow G12 8QQ (United Kingdom)] [Scottish Universities Physics Alliance, School of Physics and Astronomy, University of Glasgow, Glasgow G12 8QQ (United Kingdom); Issac, R. C. [Scottish Universities Physics Alliance, Department of Physics, University of Strathclyde, John Anderson Building, 107 Rottenrow, Glasgow G4 0NG (United Kingdom) [Scottish Universities Physics Alliance, Department of Physics, University of Strathclyde, John Anderson Building, 107 Rottenrow, Glasgow G4 0NG (United Kingdom); Research Department of Physics, Mar Athanasius College, Kothamangalam 686666, Kerala (India); Lemos, N. R. C.; Dias, J. M. [GoLP/Instituto de Plasmas eFusão Nuclear, Instituto Superior Técnico, Universidade de Lisboa, Avenida Rovisco Pais, 1049-001 Lisbon (Portugal)] [GoLP/Instituto de Plasmas eFusão Nuclear, Instituto Superior Técnico, Universidade de Lisboa, Avenida Rovisco Pais, 1049-001 Lisbon (Portugal); Symes, D. R. [Central Laser Facility, Science and Technology Facilities Council, Rutherford Appleton Laboratory, Harwell Science and Innovation Campus, OX11 0QX Didcot (United Kingdom)] [Central Laser Facility, Science and Technology Facilities Council, Rutherford Appleton Laboratory, Harwell Science and Innovation Campus, OX11 0QX Didcot (United Kingdom); and others

    2013-11-15

    Compton side-scattering has been used to simultaneously downshift the energy of keV to MeV energy range photons while attenuating their flux to enable single-shot, spectrally resolved, measurements of high flux X-ray sources to be undertaken. To demonstrate the technique a 1 mm thick pixelated cadmium telluride detector has been used to measure spectra of Compton side-scattered radiation from a Cobalt-60 laboratory source and a high flux, high peak brilliance X-ray source of betatron radiation from a laser-plasma wakefield accelerator.

  12. Robust, high-throughput solution structural analyses by small angle X-ray scattering (SAXS)

    SciTech Connect (OSTI)

    Hura, Greg L.; Menon, Angeli L.; Hammel, Michal; Rambo, Robert P.; Poole II, Farris L.; Tsutakawa, Susan E.; Jenney Jr, Francis E.; Classen, Scott; Frankel, Kenneth A.; Hopkins, Robert C.; Yang, Sungjae; Scott, Joseph W.; Dillard, Bret D.; Adams, Michael W. W.; Tainer, John A.

    2009-07-20

    We present an efficient pipeline enabling high-throughput analysis of protein structure in solution with small angle X-ray scattering (SAXS). Our SAXS pipeline combines automated sample handling of microliter volumes, temperature and anaerobic control, rapid data collection and data analysis, and couples structural analysis with automated archiving. We subjected 50 representative proteins, mostly from Pyrococcus furiosus, to this pipeline and found that 30 were multimeric structures in solution. SAXS analysis allowed us to distinguish aggregated and unfolded proteins, define global structural parameters and oligomeric states for most samples, identify shapes and similar structures for 25 unknown structures, and determine envelopes for 41 proteins. We believe that high-throughput SAXS is an enabling technology that may change the way that structural genomics research is done.

  13. Changes in the Atomic Structure through Glass Transition Observed by X-Ray Scattering

    SciTech Connect (OSTI)

    Egami, Takeshi [ORNL

    2012-01-01

    The glass transition involves a minor change in the internal energy, and yet the physical and mechanical properties of a glass change dramatically. In order to determine the evolution of the atomic structure through the glass transition, we employed in-situ synchrotron X-ray scattering measurements as a function of temperature on a model material: Zr-Cu-Al metallic glass. We found that the thermal expansion at the atomic level is smaller than the macroscopic thermal expansion, and significantly increases above the glass transition temperature. The observed changes in the pair-distribution function (PDF) are explained in terms of the fluctuations in the local atomic volume and their change through the glass transition.

  14. Ultrasmall-angle X-ray scattering analysis of photonic crystal structure

    SciTech Connect (OSTI)

    Abramova, V. V.; Sinitskii, A. S.; Grigor'eva, N. A.; Grigor'ev, S. V.; Belov, D. V.; Petukhov, A. V.; Mistonov, A. A.; Vasil'eva, A. V.; Tret'yakov, Yu. D.

    2009-07-15

    The results of an ultrasmall-angle X-ray scattering study of iron(III) oxide inverse opal thin films are presented. The photonic crystals examined are shown to have fcc structure with amount of stacking faults varying among the samples. The method used in this study makes it possible to easily distinguish between samples with predominantly twinned fcc structure and nearly perfect fcc stacking. The difference observed between samples fabricated under identical conditions is attributed to random layer stacking in the self-assembled colloidal crystals used as templates for fabricating the inverse opals. The present method provides a versatile tool for analyzing photonic crystal structure in studies of inverse opals made of various materials, colloidal crystals, and three-dimensional photonic crystals of other types.

  15. Spatial frequency spectrum of the x-ray scatter distribution in CBCT projections

    SciTech Connect (OSTI)

    Bootsma, G. J.; Verhaegen, F.; Department of Oncology, Medical Physics Unit, McGill University, Montreal, Quebec H3G 1A4 ; Jaffray, D. A.; Radiation Medicine Program, Princess Margaret Hospital, Toronto, Ontario M5G 2M9; Ontario Cancer Institute, Princess Margaret Hospital, Toronto, Ontario M5G 2M9; Department of Radiation Oncology, University of Toronto, Toronto, Ontario M5G 2M9

    2013-11-15

    Purpose: X-ray scatter is a source of significant image quality loss in cone-beam computed tomography (CBCT). The use of Monte Carlo (MC) simulations separating primary and scattered photons has allowed the structure and nature of the scatter distribution in CBCT to become better elucidated. This work seeks to quantify the structure and determine a suitable basis function for the scatter distribution by examining its spectral components using Fourier analysis.Methods: The scatter distribution projection data were simulated using a CBCT MC model based on the EGSnrc code. CBCT projection data, with separated primary and scatter signal, were generated for a 30.6 cm diameter water cylinder [single angle projection with varying axis-to-detector distance (ADD) and bowtie filters] and two anthropomorphic phantoms (head and pelvis, 360 projections sampled every 1°, with and without a compensator). The Fourier transform of the resulting scatter distributions was computed and analyzed both qualitatively and quantitatively. A novel metric called the scatter frequency width (SFW) is introduced to determine the scatter distribution's frequency content. The frequency content results are used to determine a set basis functions, consisting of low-frequency sine and cosine functions, to fit and denoise the scatter distribution generated from MC simulations using a reduced number of photons and projections. The signal recovery is implemented using Fourier filtering (low-pass Butterworth filter) and interpolation. Estimates of the scatter distribution are used to correct and reconstruct simulated projections.Results: The spatial and angular frequencies are contained within a maximum frequency of 0.1 cm{sup ?1} and 7/(2?) rad{sup ?1} for the imaging scenarios examined, with these values varying depending on the object and imaging setup (e.g., ADD and compensator). These data indicate spatial and angular sampling every 5 cm and ?/7 rad (?25°) can be used to properly capture the scatter distribution, with reduced sampling possible depending on the imaging scenario. Using a low-pass Butterworth filter, tuned with the SFW values, to denoise the scatter projection data generated from MC simulations using 10{sup 6} photons resulted in an error reduction of greater than 85% for the estimating scatter in single and multiple projections. Analysis showed that the use of a compensator helped reduce the error in estimating the scatter distribution from limited photon simulations by more than 37% when compared to the case without a compensator for the head and pelvis phantoms. Reconstructions of simulated head phantom projections corrected by the filtered and interpolated scatter estimates showed improvements in overall image quality.Conclusions: The spatial frequency content of the scatter distribution in CBCT is found to be contained within the low frequency domain. The frequency content is modulated both by object and imaging parameters (ADD and compensator). The low-frequency nature of the scatter distribution allows for a limited set of sine and cosine basis functions to be used to accurately represent the scatter signal in the presence of noise and reduced data sampling decreasing MC based scatter estimation time. Compensator induced modulation of the scatter distribution reduces the frequency content and improves the fitting results.

  16. Caustic structures in the spectrum of x-ray Compton scattering off electrons driven by a short intense laser pulse

    E-Print Network [OSTI]

    Seipt, D; Fritzsche, S; Kampfer, B

    2015-01-01

    We study the Compton scattering of x-rays off electrons that are driven by a relativistically intense short optical laser pulse. The frequency spectrum of the laser-assisted Compton radiation shows a broad plateau in the vicinity of the laser-free Compton line due to a nonlinear mixing between x-ray and laser photons. Special emphasis is placed on how the shape of the short assisting laser pulse affects the spectrum of the scattered x-rays. In particular, we observe sharp peak structures in the plateau region, whose number and locations are highly sensitive to the laser pulse shape. These structures are interpreted as spectral caustics by using a semiclassical analysis of the laser-assisted QED matrix element.

  17. The 3D-architecture of individual free silver nanoparticles captured by X-ray scattering

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Barke, Ingo; Hartmann, Hannes; Rupp, Daniela; Flückiger, Leonie; Sauppe, Mario; Adolph, Marcus; Schorb, Sebastian; Bostedt, Christoph; Treusch, Rolf; Peltz, Christian; et al

    2015-02-04

    The diversity of nanoparticle shapes generated by condensation from gaseous matter reflects the fundamental competition between thermodynamic equilibration and the persistence of metastable configurations during growth. In the kinetically limited regime, intermediate geometries that are favoured only in early formation stages can be imprinted in the finally observed ensemble of differently structured specimens. Here we demonstrate that single-shot wide-angle scattering of femtosecond soft X-ray free-electron laser pulses allows three-dimensional characterization of the resulting metastable nanoparticle structures. For individual free ?silver particles, which can be considered frozen in space for the duration of photon exposure, both shape and orientation are uncoveredmore »from measured scattering images. We identify regular shapes, including species with fivefold symmetry and surprisingly large aspect ratio up to particle radii of the order of 100 nm. Our approach includes scattering effects beyond Born’s approximation and is remarkably efficient—opening up new routes in ultrafast nanophysics and free-electron laser science« less

  18. A semianalytic model to extract differential linear scattering coefficients of breast tissue from energy dispersive x-ray diffraction measurements

    SciTech Connect (OSTI)

    LeClair, Robert J.; Boileau, Michel M.; Wang Yinkun [Department of Physics and Astronomy, Laurentian University, 935 Ramsey Lake Road, Sudbury, Ontario, P3E 2C6 (Canada) and Biomolecular Sciences Program, Laurentian University, 935 Ramsey Lake Road, Sudbury, Ontario, P3E 2C6 (Canada); Department of Physics and Astronomy, Laurentian University, 935 Ramsey Lake Road, Sudbury, Ontario, P3E 2C6 (Canada); Department of Physics and Astronomy, Laurentian University, 935 Ramsey Lake Road, Sudbury, Ontario, P3E 2C6 (Canada)

    2006-04-15

    The goal of this work is to develop a technique to measure the x-ray diffraction signals of breast biopsy specimens. A biomedical x-ray diffraction technology capable of measuring such signals may prove to be of diagnostic use to the medical field. Energy dispersive x-ray diffraction measurements coupled with a semianalytical model were used to extract the differential linear scattering coefficients [{mu}{sub s}(x)] of breast tissues on absolute scales. The coefficients describe the probabilities of scatter events occurring per unit length of tissue per unit solid angle of detection. They are a function of the momentum transfer argument, x=sin({theta}/2)/{lambda}, where {theta}=scatter angle and {lambda}=incident wavelength. The technique was validated by using a 3 mm diameter 50 kV polychromatic x-ray beam incident on a 5 mm diameter 5 mm thick sample of water. Water was used because good x-ray diffraction data are available in the literature. The scatter profiles from 6 deg. to 15 deg. in increments of 1 deg. were measured with a 3 mmx3 mmx2 mm thick cadmium zinc telluride detector. A 2 mm diameter Pb aperture was placed on top of the detector. The target to detector distance was 29 cm and the duration of each measurement was 10 min. Ensemble averages of the results compare well with the gold standard data of A. H. Narten [''X-ray diffraction data on liquid water in the temperature range 4 deg. C-200 deg. C, ORNL Report No. 4578 (1970)]. An average 7.68% difference for which most of the discrepancies can be attributed to the background noise at low angles was obtained. The preliminary measurements of breast tissue are also encouraging.

  19. X-ray resonant magnetic scattering and x-ray magnetic circular dichroism branching ratios, L[subscript 3] / L[subscript 2], for heavy rare earths

    SciTech Connect (OSTI)

    Lee, Yongbin; Kim, Jong-Woo; Goldman, Alan I.; Harmon, Bruce N. (Iowa State)

    2010-07-19

    In this study we have used first principles electronic structure methods to investigate the detailed contributions to the L{sub 3}/L{sub 2} branching ratio in the heavy rare earth elements. The calculations use the full potential, relativistic, linear augmented plane wave method with the LSDA+U approach for consideration of the local 4f electronic orbitals. With no spin orbit coupling (SOC) in the conducting bands, and with the same radial function for the 2p{sub 3/2} and 2p{sub 1/2} core states, the branching ratio (BR) is exactly 1:-1 for the x-ray magnetic circular dichroism spectra of the ferromagnetic heavy rare earth metals. However, with full SOC the BR ranges from 1.5 to 6.0 in going from Gd to Er. The energy and spin dependence of the 5d radial functions are important. The results point to problems with modified atomic models which have been proposed to explain the BR. Recent x-ray resonant magentic scattering experiments on (Gd,Tb,Dy,Ho,Er,Tm)Ni{sub 2}Ge{sub 2} are discussed.

  20. Molecular structures of fluid phase phosphatidylglycerol bilayers as determined by small angle neutron and X-ray scattering

    E-Print Network [OSTI]

    Nagle, John F.

    neutron and X-ray scattering Jianjun Pan a, , Frederick A. Heberle a , Stephanie Tristram-Nagle b Matter Division, Neutron Sciences Directorate, Oak Ridge National Laboratory, Oak Ridge, TN 378316100 Institute for Neutron Sciences, Oak Ridge National Laboratory, Oak Ridge, TN 378316453, USA e Canadian

  1. Neutron and X-ray Scattering Techniques have proved so successful in condensed matter studies that a wide variety of sample environments have been developed in consquence. Many

    E-Print Network [OSTI]

    Boyer, Edmond

    Foreword Neutron and X-ray Scattering Techniques have proved so successful in condensed matter whose function is to develop and optimise the techniques appropriate to neutron scattering. Since other neutron and X-ray research centres have similar technical support groups, it was felt timely to unité

  2. Relaxation transition in glass-forming polybutadiene as revealed by nuclear resonance X-ray scattering

    SciTech Connect (OSTI)

    Kanaya, Toshiji; Inoue, Rintaro [Institute for Chemical Research, Kyoto University, Uji, Kyoto-fu 611-0011 (Japan)] [Institute for Chemical Research, Kyoto University, Uji, Kyoto-fu 611-0011 (Japan); Saito, Makina [Elettra-Sincrotrone Trieste, S. S. 14 Km 163.5, I-34149 Trieste (Italy)] [Elettra-Sincrotrone Trieste, S. S. 14 Km 163.5, I-34149 Trieste (Italy); Seto, Makoto [Research Reactor Institute, Kyoto University, Kumatori, Osaka-fu 590-0494 (Japan)] [Research Reactor Institute, Kyoto University, Kumatori, Osaka-fu 590-0494 (Japan); Yoda, Yoshitaka [Japan Synchrotron Radiation Research Institute, Sayo, Hyogo-ken 679-5198 (Japan)] [Japan Synchrotron Radiation Research Institute, Sayo, Hyogo-ken 679-5198 (Japan)

    2014-04-14

    We investigated the arrest mechanism of molecular motions in a glass forming polybutadiene near the glass transition using a new nuclear resonance synchrotron X-ray scattering technique to cover a wide time range (10{sup ?9} to 10{sup ?5} s) and a scattering vector Q range (9.6–40 nm{sup ?1}), which have never been accessed by other methods. Owing to the wide time and Q ranges it was found for the first time that a transition of the ?-process to the slow ?-process (or the Johari-Goldstein process) was observed in a Q range higher than the first peak in the structure factor S(Q) at the critical temperature T{sub c} in the mode coupling theory. The results suggest the important roles of hopping motions below T{sub c}, which was predicted by the recent extended mode coupling theory and the cooperative motions due to the strong correlation at the first peak in S(Q) in the arrest mechanism.

  3. Inelastic neutron scattering in valence fluctuation compounds

    SciTech Connect (OSTI)

    Jon M Lawrence

    2011-02-15

    The valence fluctuation compounds are rare earth intermetallics where hybridization of the nearly-localized 4f electrons with the conduction electrons leads to incorporation of the 4f's into the itinerant states. This hybridization slows down the conduction electrons and hence gives them a heavy effective mass, justifying application of the term 'heavy Fermion' (HF) to these materials. During the project period, we grew large single crystals of several such compounds and measured their properties using both standard thermodynamic probes and state-of-the-art inelastic neutron scattering. We obtained three main results. For the intermediate valence compounds CePd{sub 3} and YbAl{sub 3}, we showed that the scattering of neutrons by the fluctuations of the 4f magnetic moment does not have the momentum dependence expected for the itinerant heavy mass state; rather, the scattering is more typical of a localized spin fluctuation. We believe that incoherent scattering localizes the excitation. For the heavy Fermion compound Ce(Ni{sub 0.935}Pd{sub 0.065}){sub 2}Ge{sub 2}, which sits at a T = 0 critical point for transformation into an antiferromagnetic (AF) phase, we showed that the scattering from the AF fluctuations does not exhibit any of the divergences that are expected at a phase transition. We speculate that alloy disorder profoundly suppresses the growth of the fluctuating AF regions, leading to short range clusters rather than regions of infinite size. Finally, we explored the applicability of key concepts used to describe the behavior of rare earth heavy Fermions to uranium based HF compounds where the 5f electrons are itinerant as opposed to localized. We found that scaling laws relating the spin fluctuation energy measured in neutron scattering to the low temperature specific heat and susceptibility are valid for the uranium compounds, once corrections are made for AF fluctuations; however, the degeneracy of the high temperature moment is smaller than expected for rare-earth-like Hund's rule behavior, essentially because the orbital moment is suppressed for itinerant 5f electrons. We also found that the standard local-moment-based theory of the temperature dependence of the specific heat, susceptibility and neutron scattering fails badly for URu{sub 2}Zn{sub 20} and UCo{sub 2}Zn{sub 20}, even though the theory is phenomenally successful for the closely related rare earth compound YbFe{sub 2}Zn{sub 20}. Both these results highlight the distinction between the itineracy of the 5f's and the localization of the 4f's. It is our hope that these results are sufficiently significant as to stimulate deeper investigation of these compounds.

  4. Back-scattering channel-cut high-resolution monochromator for inelastic x-ray scattering

    SciTech Connect (OSTI)

    Kushnir, V.I.; Abbamonte, P.M.; Macrander, A.T.; Schwoerer-Boehning, M.

    1997-08-01

    We report on a design and on some experimental results for the performance of a new high energy resolution monochromator. It is a large channel-cut Si crystal with a 197 mm separation between the two faces designed to operate in a near-backscattering regime. The device was tested as a second monochromator on Sector 3 of the Synchrotron Radiation Instrumentation Collaborative Access Team (SRI-CAT) at the Advanced Photon Source using the Si(777) reflection at a photon energy of 13.84 keV. The same monochromator can be used for other energies with reflections of the type (hhh). Special care has been taken to equalize the temperature of the two faces by employing a Peltier heat pump. A Si(111) double-crystal pre-monochromator designed to withstand the high heat load of the undulator radiation was used upstream on the beamline. The measured throughput efficiency of the Si(777) channel-cut monochromator was less ideal by a factor of 1.9. Dynamical diffraction theory was used to calculate the throughput of an ideally perfect crystal.

  5. Boron phosphide under pressure: In situ study by Raman scattering and X-ray diffraction

    SciTech Connect (OSTI)

    Solozhenko, Vladimir L.; Kurakevych, Oleksandr O.; Le Godec, Yann; Kurnosov, Aleksandr V.; Oganov, Artem R.

    2014-07-21

    Cubic boron phosphide, BP, has been studied in situ by X-ray diffraction and Raman scattering up to 55?GPa at 300?K in a diamond anvil cell. The bulk modulus of B{sub 0}?=?174(2) GPa has been established, which is in excellent agreement with our ab initio calculations. The data on Raman shift as a function of pressure, combined with equation-of-state (EOS) data, allowed us to estimate the Grüneisen parameters of the TO and LO modes of zinc-blende structure, ?{sub G}{sup TO?}=?1.26 and ?{sub G}{sup LO?}=?1.13, just like in the case of other A{sup III}B{sup V} diamond-like phases, for which ?{sub G}{sup TO?}>??{sub G}{sup LO?}??1. We also established that the pressure dependence of the effective electro-optical constant ? is responsible for a strong change in relative intensities of the TO and LO modes from I{sub TO}/I{sub LO}???0.25 at 0.1?MPa to I{sub TO}/I{sub LO}???2.5 at 45?GPa, for which we also find excellent agreement between experiment and theory.

  6. Growth dynamics of pentacene thin films: Real-time synchrotron x-ray scattering study

    SciTech Connect (OSTI)

    Mayer, Alex C.; Ruiz, Ricardo; Malliaras, George G. [Materials Science and Engineering, Cornell University, Ithaca, New York 14853 (United States); Zhou, Hua; Headrick, Randall L. [Department of Physics, University of Vermont, Burlington, Vermont 05405 (United States); Kazimirov, Alexander [Cornell High Energy Synchrotron Source, Ithaca, New York 14853 (United States)

    2006-05-15

    Real-time synchrotron x-ray scattering in the anti-Bragg configuration was used to monitor the dynamics of pentacene film growth on inert substrates. A distributed-growth model, according to which pentacene molecules adsorbed on the nth layer can either nucleate and contribute to the growth of the (n+1)th layer or transfer downward and contribute to the growth of the nth layer, gave a good description of the data. For molecules adsorbed on the first and second layers, the probability of downward transfer was found to be dependent on the substrate, and independent of temperature within the range from 25 to 60 deg. C. For films grown on SiO{sub 2}, an Ehrlich-Schwoebel barrier of the order of 70 meV dominated downward transfer of pentacene molecules in layers away from the substrate. For films grown on an alkylated self-assembled monolayer, significant desorption of pentacene molecules from the substrate at elevated temperatures forced the growth mode toward the three-dimensional limit.

  7. Grazing-incidence small-angle X-ray scattering: application to the study of quantum dot lattices

    SciTech Connect (OSTI)

    Buljan, Maja Radi?, Nikola; Bernstorff, Sigrid; Draži?, Goran; Bogdanovi?-Radovi?, Iva; Holý, Václav

    2012-01-01

    The modelling of grazing-incidence small-angle X-ray scattering (GISAXS) from three-dimensional quantum dot lattices is described. The ordering of quantum dots in three-dimensional quantum dot lattices is investigated by grazing-incidence small-angle X-ray scattering (GISAXS). Theoretical models describing GISAXS intensity distributions for three general classes of lattices of quantum dots are proposed. The classes differ in the type of disorder of the positions of the quantum dots. The models enable full structure determination, including lattice type, lattice parameters, the type and degree of disorder in the quantum dot positions and the distributions of the quantum dot sizes. Applications of the developed models are demonstrated using experimentally measured data from several types of quantum dot lattices formed by a self-assembly process.

  8. Ion distributions at charged aqueous surfaces: Synchrotron X-ray scattering studies

    SciTech Connect (OSTI)

    Bu, Wei

    2009-08-15

    Surface sensitive synchrotron X-ray scattering studies were performed to obtain the distribution of monovalent ions next to a highly charged interface at room temperature. To control surface charge density, lipids, dihexadecyl hydrogen-phosphate (DHDP) and dimysteroyl phosphatidic acid (DMPA), were spread as monolayer materials at the air/water interface, containing CsI at various concentrations. Five decades in bulk concentrations (CsI) are investigated, demonstrating that the interfacial distribution is strongly dependent on bulk concentration. We show that this is due to the strong binding constant of hydronium H3O+ to the phosphate group, leading to proton-transfer back to the phosphate group and to a reduced surface charge. Using anomalous reflectivity off and at the L3 Cs+ resonance, we provide spatial counterion (Cs+) distributions next to the negatively charged interfaces. The experimental ion distributions are in excellent agreement with a renormalized surface charge Poisson-Boltzmann theory for monovalent ions without fitting parameters or additional assumptions. Energy Scans at four fixed momentum transfers under specular reflectivity conditions near the Cs+ L3 resonance were conducted on 10-3 M CsI with DHDP monolayer materials on the surface. The energy scans exhibit a periodic dependence on photon momentum transfer. The ion distributions obtained from the analysis are in excellent agreement with those obtained from anomalous reflectivity measurements, providing further confirmation to the validity of the renormalized surface charge Poisson-Boltzmann theory for monovalent ions. Moreover, the dispersion corrections f0 and f00 for Cs+ around L3 resonance, revealing the local environment of a Cs+ ion in the solution at the interface, were extracted simultaneously with output of ion distributions.

  9. Simulating x-ray Thomson scattering signals from high-density, millimetre-scale plasmas at the National Ignition Facility

    SciTech Connect (OSTI)

    Chapman, D. A., E-mail: david.chapman@awe.co.uk [Plasma Physics Group, Radiation Physics Department, AWE plc, Reading RG7 4PR (United Kingdom); Centre for Fusion, Space and Astrophysics, University of Warwick, Coventry CV4 7AL (United Kingdom); Kraus, D.; Falcone, R. W. [Department of Physics, University of California, Berkeley, California 94720 (United States); Kritcher, A. L.; Bachmann, B.; Collins, G. W.; Gaffney, J. A.; Hawreliak, J. A.; Landen, O. L.; Le Pape, S.; Ma, T.; Nilsen, J.; Pak, A.; Swift, D. C.; Döppner, T. [Lawrence Livermore National Laboratory, Livermore, California 94550 (United States); Gericke, D. O. [Centre for Fusion, Space and Astrophysics, University of Warwick, Coventry CV4 7AL (United Kingdom); Glenzer, S. H. [SLAC National Accelerator Laboratory, Menlo Park, California 94309 (United States); Guymer, T. M. [Plasma Physics Group, Radiation Physics Department, AWE plc, Reading RG7 4PR (United Kingdom); Neumayer, P. [Gesellschaft für Schwerionenforschung, 64291 Darmstadt (Germany); Redmer, R. [Institut für Physik, Universität Rostock, 18051 Rostock (Germany); and others

    2014-08-15

    We have developed a model for analysing x-ray Thomson scattering data from high-density, millimetre-scale inhomogeneous plasmas created during ultra-high pressure implosions at the National Ignition Facility in a spherically convergent geometry. The density weighting of the scattered signal and attenuation of the incident and scattered x-rays throughout the target are included using radial profiles of the density, opacity, ionization state, and temperature provided by radiation-hydrodynamics simulations. These simulations show that the scattered signal is strongly weighted toward the bulk of the shocked plasma and the Fermi degenerate material near the ablation front. We show that the scattered signal provides a good representation of the temperature of this highly nonuniform bulk plasma and can be determined to an accuracy of ca. 15% using typical data analysis techniques with simple 0D calculations. On the other hand, the mean ionization of the carbon in the bulk is underestimated. We suggest that this discrepancy is due to the convolution of scattering profiles from different regions of the target. Subsequently, we discuss modifications to the current platform to minimise the impact of inhomogeneities, as well as opacity, and also to enable probing of conditions more strongly weighted toward the compressed core.

  10. Your access to the Oak Ridge National Laboratory (ORNL) is approved beginning Sunday, June 20, 2010, for the second week of the Neutron X-ray Scattering School.

    E-Print Network [OSTI]

    Pennycook, Steve

    , for the second week of the Neutron X-ray Scattering School. Please be certain to bring photo identification access to the Target Facility.) · General User Access Training for Neutron Scattering Users, Neutron Scattering Science User Office Oak Ridge National Laboratory ORNL Neutron Scattering School June

  11. Phase-based x-ray scattering—A possible method to detect cancer cells in a very early stage

    SciTech Connect (OSTI)

    Feye-Treimer, U. Treimer, W.

    2014-05-15

    Purpose: This theoretical work contains a detailed investigation of the potential and sensitivity of phase-based x-ray scattering for cancer detection in biopsies if cancer is in a very early stage of development. Methods: Cancer cells in their early stage of development differ from healthy ones mainly due to their faster growing cell nuclei and the enlargement of their densities. This growth is accompanied by an altered nucleus–plasma relation for the benefit of the cell nuclei, that changes the physical properties especially the index of refraction of the cell and the one of the cell nuclei. Interaction of radiation with matter is known to be highly sensitive to small changes of the index of refraction of matter; therefore a detection of such changes of volume and density of cell nuclei by means of high angular resolved phase-based scattering of x rays might provide a technique to distinguish malignant cells from healthy ones ifthe cell–cell nucleus system is considered as a coherent phase shifting object. Then one can observe from a thin biopsy which represents a monolayer of cells (no multiple scattering) that phase-based x-ray scattering curves from healthy cells differ from those of cancer cells in their early stage of development. Results: Detailed calculations of x-ray scattering patterns from healthy and cancer cell nuclei yield graphs and numbers with which one can distinguish healthy cells from cancer ones, taking into account that both kinds of cells occur in a tissue within a range of size and density. One important result is the role and the influence of the (lateral) coherence width of the radiation on the scattering curves and the sensitivity of phase-based scattering for cancer detection. A major result is that a larger coherence width yields a larger sensitivity for cancer detection. Further import results are calculated limits for critical sizes and densities of cell nuclei in order to attribute the investigated tissue to be healthy or diseased. Conclusions: With this proposed method it should be in principle possible to detect cancer cells in apparently healthy tissues in biopsies and/or in samples of the far border region of abscised or excised tissues. Thus this method could support established methods in diagnostics of cancer-suspicious samples.

  12. Anomalous small angle x-ray scattering studies of amorphous metal-germanium alloys

    SciTech Connect (OSTI)

    Rice, M.

    1993-12-01

    This dissertation addresses the issue of composition modulation in sputtered amorphous metal-germanium thin films with the aim of understanding the intermediate range structure of these films as a function of composition. The investigative tool used in this work is anomalous small-angle X-ray scattering (ASAXS). The primary focus of this investigation is the amorphous iron-germanium (a-Fe{sub x}Ge{sub 100-x}) system with particular emphasis on the semiconductor-rich regime. Brief excursions are made into the amorphous tungsten-germanium (a-W{sub x}Ge{sub 100-x}) and the amorphous molybdenum-germanium (a-Mo{sub x}Ge{sub 100-x}) systems. All three systems exhibit an amorphous structure over a broad composition range extending from pure amorphous germanium to approximately 70 atomic percent metal when prepared as sputtered films. Across this composition range the structures change from the open, covalently bonded, tetrahedral network of pure a-Ge to densely packed metals. The structural changes are accompanied by a semiconductor-metal transition in all three systems as well as a ferromagnetic transition in the a-Fe{sub x}Ge{sub 100-x} system and a superconducting transition in the a-Mo{sub x}Ge{sub 100-x} system. A long standing question, particularly in the a-Fe{sub x}Ge{sub 100-x} and the a-Mo{sub x}Ge{sub 100-x} systems, has been whether the structural changes (and therefore the accompanying electrical and magnetic transitions) are accomplished by homogeneous alloy formation or phase separation. The application of ASAXS to this problem proves unambiguously that fine scale composition modulations, as distinct from the simple density fluctuations that arise from cracks and voids, are present in the a-Fe{sub x}Ge{sub 100-x}, a-W{sub x}Ge{sub 100-x}, and a-Mo{sub x}Ge{sub 100-x} systems in the semiconductor-metal transition region. Furthermore, ASAXS shows that germanium is distributed uniformly throughout each sample in the x<25 regime of all three systems.

  13. Tunable X-ray source

    DOE Patents [OSTI]

    Boyce, James R. (Williamsburg, VA)

    2011-02-08

    A method for the production of X-ray bunches tunable in both time and energy level by generating multiple photon, X-ray, beams through the use of Thomson scattering. The method of the present invention simultaneously produces two X-ray pulses that are tunable in energy and/or time.

  14. Nano-crystal growth in cordierite glass ceramics studied with X-ray scattering

    E-Print Network [OSTI]

    Bras, Wim

    2010-01-01

    By Small-Angle Neutron-Scattering, Electron-Paramagneticphases.. Small angle neutron scattering (SANS) experimentsand Small Angle Neutron Scattering (SANS) on some of the

  15. Focus characterization at an X-ray free-electron laser by coherent scattering and speckle analysis

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Sikorski, Marcin; Song, Sanghoon; Schropp, Andreas; Deutsches Elektronen-Synchrotron, Hamburg; Seiboth, Frank; Feng, Yiping; Alonso-Mori, Roberto; Chollet, Matthieu; Lemke, Henrik T.; Sokaras, Dimosthenis; et al

    2015-04-14

    X-ray focus optimization and characterization based on coherent scattering and quantitative speckle size measurements was demonstrated at the Linac Coherent Light Source. Its performance as a single-pulse free-electron laser beam diagnostic was tested for two typical focusing configurations. The results derived from the speckle size/shape analysis show the effectiveness of this technique in finding the focus' location, size and shape. In addition, its single-pulse compatibility enables users to capture pulse-to-pulse fluctuations in focus properties compared with other techniques that require scanning and averaging.

  16. The Investigation of Decomposition of Supersaturated Si Solid Solution by X-Ray Diffuse Scattering

    SciTech Connect (OSTI)

    Shcherbachev, Kirill; Privezentsev, Vladimir

    2010-04-06

    The results of investigation of microstructure of Zn doped n-type Si by X-ray Diffuse Scattering (XRDS) are presented. Experimental samples were made by a high-temperature Zn diffusion annealing with subsequent quenching and tempering. Reciprocal space maps of XRDS were obtained. They resulted in that crystal lattice of the samples contains spherical MDs of vacancy type and plane shape MDs of interstitial type. The MDs average radius and their type depend on Zn doping level and thermal treatment after Zn diffusion.

  17. Bent crystal spectrometer for both frequency and wavenumber resolved x-ray scattering at a seeded free-electron laser

    SciTech Connect (OSTI)

    Zastrau, Ulf; Fletcher, Luke B.; Galtier, Eric Ch.; Gamboa, Eliseo; Glenzer, Siegfried H.; Heimann, Philipp; Nagler, Bob; Schropp, Andreas; Lee, Hae Ja; Förster, Eckhart; Marschner, Heike; Wehrhan, Ortrud

    2014-09-15

    We present a cylindrically curved GaAs x-ray spectrometer with energy resolution ?E/E = 1.1 ×?10{sup ?4} and wave-number resolution of ?k/k = 3 ×?10{sup ?3}, allowing plasmon scattering at the resolution limits of the Linac Coherent Light Source (LCLS) x-ray free-electron laser. It spans scattering wavenumbers of 3.6 to 5.2/Å in 100 separate bins, with only 0.34% wavenumber blurring. The dispersion of 0.418 eV/13.5??m agrees with predictions within 1.3%. The reflection homogeneity over the entire wavenumber range was measured and used to normalize the amplitude of scattering spectra. The proposed spectrometer is superior to a mosaic highly annealed pyrolytic graphite spectrometer when the energy resolution needs to be comparable to the LCLS seeded bandwidth of 1 eV and a significant range of wavenumbers must be covered in one exposure.

  18. Bent crystal spectrometer for both frequency and wavenumber resolved x-ray scattering at a seeded free-electron laser

    E-Print Network [OSTI]

    Zastrau, Ulf; Foerster, Eckhart; Galtier, Eric Ch; Gamboa, Eliseo; Glenzer, Siegfried H; Heimann, Philipp; Marschner, Heike; Nagler, Bob; Schropp, Andreas; Wehrhan, Ortrud; Lee, Hae Ja

    2014-01-01

    We present a cylindrically curved GaAs x-ray spectrometer with energy resolution $\\Delta E/E = 1.1\\cdot 10^{-4}$ and wave-number resolution of $\\Delta k/k = 3\\cdot 10^{-3}$, allowing plasmon scattering at the resolution limits of the Linac Coherent Light Source (LCLS) x-ray free-electron laser. It spans scattering wavenumbers of 3.6 to $5.2/$\\AA\\ in 100 separate bins, with only 0.34\\% wavenumber blurring. The dispersion of 0.418~eV/$13.5\\,\\mu$m agrees with predictions within 1.3\\%. The reflection homogeneity over the entire wavenumber range was measured and used to normalize the amplitude of scattering spectra. The proposed spectrometer is superior to a mosaic HAPG spectrometer when the energy resolution needs to be comparable to the LCLS seeded bandwidth of 1~eV and a significant range of wavenumbers must be covered in one exposure.

  19. Center for X-Ray Optics, 1992

    SciTech Connect (OSTI)

    Not Available

    1993-08-01

    This report discusses the following topics: Center for X-Ray Optics; Soft X-Ray Imaging wit Zone Plate Lenses; Biological X-Ray microscopy; Extreme Ultraviolet Lithography for Nanoelectronic Pattern Transfer; Multilayer Reflective Optics; EUV/Soft X-ray Reflectometer; Photoemission Microscopy with Reflective Optics; Spectroscopy with Soft X-Rays; Hard X-Ray Microprobe; Coronary Angiography; and Atomic Scattering Factors.

  20. SU-E-I-76: Matching Primary and Scattered X-Ray Spectra for Use in Calculating the Diagnostic Radiation Index of Protection

    SciTech Connect (OSTI)

    Pasciak, A [University of Tennessee Medical Center, Knoxville, TN (United States); Jones, A [MD Anderson Cancer Center, Houston, TX (United States); Wagner, L [UT Medical School, Houston, TX (United States)

    2014-06-01

    Purpose: Lightweight lead-free or lead-composite protective garments exploit k-edge interactions to attenuate scattered X-rays. Manufacturers specify the protective value of garments in terms of lead equivalence at a single kVp. This is inadequate, as the protection provided by such garments varies with radiation quality in different use conditions. We present a method for matching scattered X-ray spectra to primary X-ray spectra. The resulting primary spectra can be used to measure penetration through protective garments, and such measurements can be weighted and summed to determine a Diagnostic Radiation Index for Protection (DRIP). Methods: Scattered X-ray spectra from fluoroscopic procedures were modeled using Monte Carlo techniques in MCNP-X 2.7. Data on imaging geometry, operator position, patient size, and primary beam spectra were gathered from clinical fluoroscopy procedures. These data were used to generate scattered X-ray spectra resulting from procedural conditions. Technical factors, including kV and added filtration, that yielded primary X-ray spectra that optimally matched the generated scattered X-ray spectra were identified through numerical optimization using a sequential quadratic programming (SQP) algorithm. Results: The primary spectra generated with shape functions matched the relative flux in each bin of the scattered spectra within 5%, and half and quarter-value layers matched within 0.1%. The DRIP for protective garments can be determined by measuring the penetration through protective garments using the matched primary spectra, then calculating a weighted average according to the expected clinical use of the garment. The matched primary spectra are specified in terms of first and second half-value layers in aluminum and acrylic. Conclusion: Lead equivalence is inadequate for completely specifying the protective value of garments. Measuring penetration through a garment using full scatter conditions is very difficult. The primary spectra determined in this work allow for practical primary penetration measurements to be made with equipment readily available to clinical medical physicists.

  1. Liquid Argon Cryogenic Detector Calibration by Inelastic Scattering of Neutrons

    E-Print Network [OSTI]

    Sergey Polosatkin; Evgeny Grishnyaev; Alexander Dolgov

    2014-07-10

    A method for calibration of cryogenic liquid argon detector response to recoils with certain energy -8.2 keV - is proposed. The method utilizes a process of inelastic scattering of monoenergetic neutrons produced by fusion DD neutron generator. Features of kinematics of inelastic scattering cause sufficient (forty times) increase in count rate of useful events relative to traditional scheme exploited elastic scattering with the same recoil energy and compatible energy resolution. The benefits of the proposed scheme of calibration most well implemented with the use of tagged neutron generator as a neutron source that allows to eliminate background originated from casual coincidence of signals on cryogenic detector and additional detector of scattered neutrons.

  2. Production of Charged Hadrons in Muon Deep Inelastic Scattering

    E-Print Network [OSTI]

    Mohammed Sultan Al-Buriahi; Mohammed Tarek Hussein; Mohammed Tawfik Ghoneim

    2015-08-06

    The production of charged hadrons, in muon Deep inelastic scattering (DIS), at light and heavy target is presented. The particles produced by the interaction with Xenon (Xe) is compared with that produced by the interaction with Deuteron (D), to obtain information on cascading process, forward-backward productions, and the rapidity distribution in different bins of the invariant mass of the interacting system W.

  3. Leading proton production in deep inelastic scattering at HERA

    E-Print Network [OSTI]

    Leading proton production in deep inelastic 1 scattering at HERA 2 ZEUS Collaboration 3 Draft, with a #28;nal-state proton carrying a large fraction of the incoming proton energy, x L > 0 photon virtualities Q 2 > 3 GeV 2 and mass of the photon-proton sys- tem 45

  4. The Physics of Deep-Inelastic Scattering at HERA

    E-Print Network [OSTI]

    Cristinel Diaconu

    2007-11-12

    In this paper an introduction to the physics of deep-inelastic scattering is given together with an account of some of the most recent results on the proton structure obtained in electron-- and positron--proton collisions at the HERA collider.

  5. Role of the nuclear vector potential in deep inelastic scattering

    E-Print Network [OSTI]

    W. Detmold; G. A. Miller; J. R. Smith

    2005-09-15

    We study the influence of the strong nuclear vector potential, treated using the mean-field approximation, in deep inelastic scattering. A consistent treatment of the electromagnetic current operator, combined with the use of the operator product expansion is presented and discussed.

  6. INELASTIC NEUTRON SCATTERING SELECTION RULES OF 03B1 HgI2 M. SIESKIND

    E-Print Network [OSTI]

    Boyer, Edmond

    899 INELASTIC NEUTRON SCATTERING SELECTION RULES OF 03B1 HgI2 M. SIESKIND Laboratoire de The inelastic neutron scattering selection rules of 03B1 HgI2 in the directions 0394, 03A3 and 039B are derived Abstracts 63.20D Introduction. - Inelastic neutron scattering is a powerful technique for the determination

  7. Nuclear resonant X-ray spectroscopy of (Mg,Fe)SiO3 orthoenstatites JENNIFER M. JACKSON1,*, EMILY A. HAMECHER1

    E-Print Network [OSTI]

    Jackson, Jennifer M.

    Nuclear resonant X-ray spectroscopy of (Mg,Fe)SiO3 orthoenstatites JENNIFER M. JACKSON1,*, EMILY A, 9700 S. Cass Ave., Argonne, IL 60439, USA Abstract: We present nuclear resonant inelastic X-ray scattering (NRIXS) and synchrotron Mo¨ssbauer spectroscopy (SMS) measurements, both nuclear resonant X

  8. Polarization periodicity in the B1 columnar phase determined by resonant x-ray scattering

    SciTech Connect (OSTI)

    Folcia, C.L.; Pindak, R.; Ortega, J.; Etxebarria, J.; Pan, L.; Wang, S.; Huang, C.C.; Ponsinet, V.; Barois, P. and Gimeno, N.

    2011-07-14

    We report structural results that evidence the polarization distribution of the blocks in the columnar phase of an achiral bent-core liquid crystal. The study was performed using resonant x-ray diffraction at the sulfur K edge on oriented samples aligned on substrates. The extra periodicity is revealed through the violation of the systematic extinction rule of the structural symmetry group along the experimentally accessible diffraction direction. Further data obtained from the polarization analysis of a resonant reflection give information concerning the transition mechanism between B{sub 1} and B{sub 2} phases.

  9. Polarization Periodicity in the B(1) Columnar Phase Determined by Resonant X-ray Scattering

    SciTech Connect (OSTI)

    C Folcia; J Ortega; J Etxebarria; L Pan; S Wang; C Huang; V Ponsinet; P Barois; R Pindak; N Gimeno

    2011-12-31

    We report structural results that evidence the polarization distribution of the blocks in the columnar phase of an achiral bent-core liquid crystal. The study was performed using resonant x-ray diffraction at the sulfur K edge on oriented samples aligned on substrates. The extra periodicity is revealed through the violation of the systematic extinction rule of the structural symmetry group along the experimentally accessible diffraction direction. Further data obtained from the polarization analysis of a resonant reflection give information concerning the transition mechanism between B{sub 1} and B{sub 2} phases.

  10. Resonant Soft X-Ray Scattering of Tri-Block Copolymers

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power Administration wouldMassR&D100Nationalquestionnaires 0serial codes on loginResonant Soft X-Ray

  11. X-ray Diffuse Scattering Measurements of Nucleation Dynamics at Femtosecond

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power AdministrationRobust,Field-effectWorkingLos Alamos verifies largest single goldWindX-Ray ImagingIn

  12. In Situ X-Ray Scattering Helps Optimize Printed Solar Cells

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power Administration would likeUniverseIMPACT EVALUATION PLAN FOR THE SITE-218 58ImprovingIn MemoriamInIn Situ X-Ray

  13. In Situ X-Ray Scattering Helps Optimize Printed Solar Cells

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantity ofkandz-cm11 Outreach Home Room NewsInformation CurrentHenry Bellamy,Impact AssessmentsImprovingIn Case ofIn Situ X-Ray

  14. In Situ X-Ray Scattering Helps Optimize Printed Solar Cells

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantity ofkandz-cm11 Outreach Home Room NewsInformation CurrentHenry Bellamy,Impact AssessmentsImprovingIn Case ofIn Situ X-RayIn Situ

  15. In Situ X-Ray Scattering Helps Optimize Printed Solar Cells

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantity ofkandz-cm11 Outreach Home Room NewsInformation CurrentHenry Bellamy,Impact AssessmentsImprovingIn Case ofIn Situ X-RayIn

  16. Turbulent pitch-angle scattering and diffusive transport of hard X-ray-producing electrons in flaring coronal loops

    SciTech Connect (OSTI)

    Kontar, Eduard P.; Bian, Nicolas H.; Emslie, A. Gordon; Vilmer, Nicole E-mail: emslieg@wku.edu

    2014-01-10

    Recent observations from RHESSI have revealed that the number of non-thermal electrons in the coronal part of a flaring loop can exceed the number of electrons required to explain the hard X-ray-emitting footpoints of the same flaring loop. Such sources cannot, therefore, be interpreted on the basis of the standard collisional transport model, in which electrons stream along the loop while losing their energy through collisions with the ambient plasma; additional physical processes, to either trap or scatter the energetic electrons, are required. Motivated by this and other observations that suggest that high-energy electrons are confined to the coronal region of the source, we consider turbulent pitch-angle scattering of fast electrons off low-frequency magnetic fluctuations as a confinement mechanism, modeled as a spatial diffusion parallel to the mean magnetic field. In general, turbulent scattering leads to a reduction of the collisional stopping distance of non-thermal electrons along the loop, and hence to an enhancement of the coronal hard X-ray source relative to the footpoints. The variation of source size L with electron energy E becomes weaker than the quadratic behavior pertinent to collisional transport, with the slope of L(E) depending directly on the mean free path ? associated with the non-collisional scattering mechanism. Comparing the predictions of the model with observations, we find that ? ? (10{sup 8}-10{sup 9}) cm for ?30 keV, less than the length of a typical flaring loop and smaller than, or comparable to, the size of the electron acceleration region.

  17. Resonant Inelastic X-ray Scattering of Rare-Earth and Copper Systems

    E-Print Network [OSTI]

    Kvashnina, Kristina

    2007-01-01

    container. In most nuclear waste management programs, thisthe Swedish Nuclear Fuel and Waste Management Co. (SKB), bythe Swedish Nuclear Fuel and Waste Management Co. (SKB), by

  18. Studies of Actinides Reduction on Iron Surfaces by Means of Resonant Inelastic X-ray Scattering

    E-Print Network [OSTI]

    2008-01-01

    that U(VI) (as soluble uranyl ion) was reduced to U(IV) ingroundwater solution of uranyl nitride for 17 days. The

  19. Resonant Inelastic X-ray Scattering of Rare-Earth and Copper Systems

    E-Print Network [OSTI]

    Kvashnina, Kristina

    2007-01-01

    bombardment for twelve rare-earths metals [1] . Accord- ingal. [3] have showed that rare-earth metals such as La has aof most of the rare- earths metals, oxides, and chlorides.

  20. Resonant Inelastic X-ray Scattering of Rare-Earth and Copper Systems

    E-Print Network [OSTI]

    Kvashnina, Kristina

    2007-01-01

    Y.Y. , Br. Corros. J. , 29 (1994) p.315. 34 Pourbaix M. ,Libredes Bruxelles (1945), Pourbaix M. , 1966. Atlas of37, 1903 (1995) [26] M. Pourbaix, PhD Thesis, Unversite

  1. Inelastic X-ray and Nuclear Resonant Scattering | Advanced Photon Source

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power Administration would likeUniverseIMPACT EVALUATION PLAN FOR THE SITE-218inperHygieneXSD-IXN XSD-IXN Home Staff

  2. Linear Dichroism in Resonant Inelastic X-Ray Scattering to Molecular

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power Administration would likeUniverseIMPACTThousand CubicResourcelogo and-E C H2015Tray and|ProjectsSpin-Orbit

  3. A general framework and review of scatter correction methods in x-ray cone-beam computerized tomography. Part 1: Scatter compensation approaches

    SciTech Connect (OSTI)

    Ruehrnschopf, Ernst-Peter; Klingenbeck, Klaus

    2011-07-15

    Since scattered radiation in cone-beam volume CT implies severe degradation of CT images by quantification errors, artifacts, and noise increase, scatter suppression is one of the main issues related to image quality in CBCT imaging. The aim of this review is to structurize the variety of scatter suppression methods, to analyze the common structure, and to develop a general framework for scatter correction procedures. In general, scatter suppression combines hardware techniques of scatter rejection and software methods of scatter correction. The authors emphasize that scatter correction procedures consist of the main components scatter estimation (by measurement or mathematical modeling) and scatter compensation (deterministic or statistical methods). The framework comprises most scatter correction approaches and its validity also goes beyond transmission CT. Before the advent of cone-beam CT, a lot of papers on scatter correction approaches in x-ray radiography, mammography, emission tomography, and in Megavolt CT had been published. The opportunity to avail from research in those other fields of medical imaging has not yet been sufficiently exploited. Therefore additional references are included when ever it seems pertinent. Scatter estimation and scatter compensation are typically intertwined in iterative procedures. It makes sense to recognize iterative approaches in the light of the concept of self-consistency. The importance of incorporating scatter compensation approaches into a statistical framework for noise minimization has to be underscored. Signal and noise propagation analysis is presented. A main result is the preservation of differential-signal-to-noise-ratio (dSNR) in CT projection data by ideal scatter correction. The objective of scatter compensation methods is the restoration of quantitative accuracy and a balance between low-contrast restoration and noise reduction. In a synopsis section, the different deterministic and statistical methods are discussed with respect to their properties and applications. The current paper is focused on scatter compensation algorithms. The multitude of scatter estimation models will be dealt with in a separate paper.

  4. Soft-x-ray spectroscopy study of nanoscale materials

    SciTech Connect (OSTI)

    Guo, J.-H.

    2005-07-30

    The ability to control the particle size and morphology of nanoparticles is of crucial importance nowadays both from a fundamental and industrial point of view considering the tremendous amount of high-tech applications. Controlling the crystallographic structure and the arrangement of atoms along the surface of nanostructured material will determine most of its physical properties. In general, electronic structure ultimately determines the properties of matter. Soft X-ray spectroscopy has some basic features that are important to consider. X-ray is originating from an electronic transition between a localized core state and a valence state. As a core state is involved, elemental selectivity is obtained because the core levels of different elements are well separated in energy, meaning that the involvement of the inner level makes this probe localized to one specific atomic site around which the electronic structure is reflected as a partial density-of-states contribution. The participation of valence electrons gives the method chemical state sensitivity and further, the dipole nature of the transitions gives particular symmetry information. The new generation synchrotron radiation sources producing intensive tunable monochromatized soft X-ray beams have opened up new possibilities for soft X-ray spectroscopy. The introduction of selectively excited soft X-ray emission has opened a new field of study by disclosing many new possibilities of soft X-ray resonant inelastic scattering. In this paper, some recent findings regarding soft X-ray absorption and emission studies of various nanostructured systems are presented.

  5. [Inelastic electron scattering from surfaces]. [Progress report

    SciTech Connect (OSTI)

    Not Available

    1993-10-01

    This program uses ab-initio and multiple scattering to study surface dynamical processes; high-resolution electron-energy loss spectroscopy is used in particular. Off-specular excitation cross sections are much larger if electron energies are in the LEED range (50--300 eV). The analyses have been extended to surfaces of ordered alloys. Phonon eigenvectors and eigenfrequencies were used as inputs to electron-energy-loss multiple scattering cross section calculations. Work on low-energy electron and positron holography is mentioned.

  6. Femtosecond X-ray Pulses at 0.4 A Generated by 900 Thomson Scattering: A Tool

    E-Print Network [OSTI]

    Geddes, Cameron Guy Robinson

    a significant limitation for generat- ing x-ray pulses of a duration that is rele- vant for fundamental studies

  7. Conformational dynamics of a crystalline protein from microsecond-scale molecular dynamics simulations and diffuse X-ray scattering

    SciTech Connect (OSTI)

    Wall, Michael E. [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Van Benschoten, Andrew H. [Univ. of California, San Francisco, CA (United States); Sauter, Nicholas K. [Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Adams, Paul D. [Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Univ. of California, Berkeley, CA (United States); Fraser, James S. [Univ. of California, San Francisco, CA (United States); Terwilliger, Thomas C. [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

    2014-12-01

    X-ray diffraction from protein crystals includes both sharply peaked Bragg reflections and diffuse intensity between the peaks. The information in Bragg scattering is limited to what is available in the mean electron density. The diffuse scattering arises from correlations in the electron density variations and therefore contains information about collective motions in proteins. Previous studies using molecular-dynamics (MD) simulations to model diffuse scattering have been hindered by insufficient sampling of the conformational ensemble. To overcome this issue, we have performed a 1.1-?s MD simulation of crystalline staphylococcal nuclease, providing 100-fold more sampling than previous studies. This simulation enables reproducible calculations of the diffuse intensity and predicts functionally important motions, including transitions among at least eight metastable states with different active-site geometries. The total diffuse intensity calculated using the MD model is highly correlated with the experimental data. In particular, there is excellent agreement for the isotropic component of the diffuse intensity, and substantial but weaker agreement for the anisotropic component. The decomposition of the MD model into protein and solvent components indicates that protein–solvent interactions contribute substantially to the overall diffuse intensity. We conclude that diffuse scattering can be used to validate predictions from MD simulations and can provide information to improve MD models of protein motions.

  8. Conformational dynamics of a crystalline protein from microsecond-scale molecular dynamics simulations and diffuse X-ray scattering

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Wall, Michael E.; Van Benschoten, Andrew H.; Sauter, Nicholas K.; Adams, Paul D.; Fraser, James S.; Terwilliger, Thomas C.

    2014-12-01

    X-ray diffraction from protein crystals includes both sharply peaked Bragg reflections and diffuse intensity between the peaks. The information in Bragg scattering is limited to what is available in the mean electron density. The diffuse scattering arises from correlations in the electron density variations and therefore contains information about collective motions in proteins. Previous studies using molecular-dynamics (MD) simulations to model diffuse scattering have been hindered by insufficient sampling of the conformational ensemble. To overcome this issue, we have performed a 1.1-?s MD simulation of crystalline staphylococcal nuclease, providing 100-fold more sampling than previous studies. This simulation enables reproducible calculationsmore »of the diffuse intensity and predicts functionally important motions, including transitions among at least eight metastable states with different active-site geometries. The total diffuse intensity calculated using the MD model is highly correlated with the experimental data. In particular, there is excellent agreement for the isotropic component of the diffuse intensity, and substantial but weaker agreement for the anisotropic component. The decomposition of the MD model into protein and solvent components indicates that protein–solvent interactions contribute substantially to the overall diffuse intensity. In conclusion, diffuse scattering can be used to validate predictions from MD simulations and can provide information to improve MD models of protein motions.« less

  9. X-ray magnetic circular dichroism and small angle neutron scattering studies of thiol capped gold nanoparticles.

    SciTech Connect (OSTI)

    de la Venta, J.; Bouzas, V.; Pucci, A.; Laguna-Marco, M. A.; Haskel, D.; te Velthuis, S. G. E; Hoffmann, A.; Lal, J.; Bleuel, M.; Ruggeri, G.; de Julian Fernandez, C.; Garcia, M. A.; Univ.Complutense de Madrid; Inst. de Magnetismo Aplicado; Univ. of Pisa; Lab. di Magnetismo Molecolare

    2009-01-01

    X-ray magnetic circular dichroism (XMCD) and Small Angle Neutron Scattering (SANS) measurements were performed on thiol capped Au nanoparticles (NPs) embedded into polyethylene. An XMCD signal of 0.8 {center_dot} 10{sup -4} was found at the Au L{sub 3} edge of thiol capped Au NPs embedded in a polyethylene matrix for which Superconducting Quantum Interference Device (SQUID) magnetometry yielded a saturation magnetization, M{sub s}, of 0.06 emu/g{sub Au}. SANS measurements showed that the 3.2 nm average-diameter nanoparticles are 28% polydispersed, but no detectable SANS magnetic signal was found with the resolution and sensitivity accessible with the neutron experiment. A comparison with previous experiments carried out on Au NPs and multilayers, yield to different values between XMCD signals and magnetization measured by SQUID magnetometer. We discuss the origin of those differences.

  10. X-ray magnetic circular dichroism and small angle neutron scattering study of thiol capped gold nanoparticles.

    SciTech Connect (OSTI)

    de la Venta, J.; Bouzas, V.; Pucci, A.; Laguna-Marco, M. A.; Haskel, D.; Pinel, E. F.; te Velthuis, S. G. E.; Hoffmann, A.; Lal, J.; Bleuel, M.; Ruggeri, G.; de Julian, C.; Garcia, M. A.; Univ. Complutense de Madrid; Inst. de Magnetismo Aplicado UCM; Univ. Pisa; Univ. di Padova

    2009-11-01

    X-ray magnetic circular dichroism (XMCD) and Small Angle Neutron Scattering (SANS) measurements were performed on thiol capped Au nanoparticles (NPs) embedded into polyethylene. An XMCD signal of 0.8 {center_dot} 10{sup -4} was found at the Au L{sub 3} edge of thiol capped Au NPs embedded in a polyethylene matrix for which Superconducting Quantum Interference Device (SQUID) magnetometry yielded a saturation magnetization, M{sub s}, of 0.06 emu/g{sub Au}. SANS measurements showed that the 3.2 nm average-diameter nanoparticles are 28% polydispersed, but no detectable SANS magnetic signal was found with the resolution and sensitivity accessible with the neutron experiment. A comparison with previous experiments carried out on Au NPs and multilayers, yield to different values between XMCD signals and magnetization measured by SQUID magnetometer. We discuss the origin of those differences.

  11. Small-angle x-ray scattering measurements of the microstructure of liquid helium mixtures adsorbed in aerogel

    SciTech Connect (OSTI)

    Lurio, L. B.; Mulders, N.; Paetkau, M.; Chan, M. H. W.; Mochrie, S. G. J. [Department of Physics, Northern Illinois University, DeKalb, Illinois 60115 (United States); Department of Physics, University of Delaware, Newark, Delaware 19716 (United States); Department of Physics and Astronomy, Okanagan College, British Columbia V1Y4X8 (Canada); Department of Physics, Pennsylvania State University, University Park, Pennsylvania 16802 (United States); Department of Physics, Yale University, New Haven, Connecticut 06511 (United States)

    2007-07-15

    Small-angle x-ray scattering (SAXS) was used to measure the microstructure of isotopic mixtures of {sup 3}He and {sup 4}He adsorbed into silica aerogels as a function of temperature and {sup 3}He concentration. The SAXS measurements could be well described by the formation of a nearly pure film of {sup 4}He which separates from the bulk mixture onto the aerogel strands and which thickens with decreasing temperature. Previous observations of a superfluid {sup 3}He-rich phase are consistent with superfluidity existing within this film phase. Observed differences between different density aerogels are explained in terms of the depletion of {sup 4}He from the bulk mixture due to film formation.

  12. Electronic and magnetic properties of manganite thin films with different compositions and its correlation with transport properties: An X-ray resonant magnetic scattering study

    SciTech Connect (OSTI)

    Singh, Surendra; Freeland, J. W.; Fitzsimmons, M. R.; Jeen, H.; Biswas, A.

    2014-12-14

    Here, we present x-ray resonant magnetic dichroism and x-ray resonant magnetic scattering measurements of the temperature dependence of magnetism in Pr-doped La-Ca-Mn-O films grown on (110) NdGaO{sub 3} substrates. We observed thermal hysteresis of the ferromagnetism in one film that also showed large thermal hysteresis of ?18?K in transport measurements. While in a second film of a different nominal chemistry, which showed very small thermal hysteresis ?3?K in transport measurements, no thermal hysteresis of the ferromagnetism was observed. These macroscopic properties are correlated with evolution of surface magnetization across metal insulator transition for these films as observed by soft x-ray resonant magnetic scattering measurements.

  13. Full multiple scattering analysis of XANES at the Cd L3 and O K edges in CdO films combined with a soft-x-ray emission investigation

    SciTech Connect (OSTI)

    Demchenko, I. N.; Denlinger, J. D.; Chernyshova, M.; Yu, K. M.; Speaks, D. T.; Olalde-Velasco, P.; Hemmers, O.; Walukiewicz, W.; Derkachova, A.; Lawniczak-Jablonska, K.

    2010-07-05

    X-ray absorption near edge structure (XANES) at the cadmium L3 and oxygen K edges for CdO thin films grown by pulsed laser deposition method, is interpreted within the real-space multiple scattering formalism, FEFF code. The features in the experimental spectra are well reproduced by calculations for a cluster of about six and ten coordination shells around the absorber for L3 edge of Cd and K edge of O, respectively. The calculated projected electronic density of states is found to be in good agreement with unoccupied electronic states in experimental data and allows to conclude that the orbital character of the lowest energy of the conductive band is Cd-5s-O-2p. The charge transfer has been quantified and not purely ionic bonding has been found. Combined XANES and resonant inelastic x-ray scattering measurements allow us to determine the direct and indirect band gap of investigated CdO films to be {approx}2.4-eV and {approx}0.9-eV, respectively.

  14. Inelastic pion scattering by /sup 13/C at low energies

    SciTech Connect (OSTI)

    Mitchell, J.H.

    1987-03-01

    Angular distributions for inelastically scattered pions were obtained for several states in /sup 13/C at an incident energy of 65 MeV. The data include results from both ..pi../sup +/ and ..pi../sup -/ measurements. In addition, ..pi../sup -/ measurements were made at T/sub ..pi../ = 50 MeV at one angle to give a two point fixed-q excitation function. The data are compared to theory and the data of others. As might be expected, medium corrections are shown to be considerably more important at low energies than at resonance. This is true for inelastic transitions of multipolarity 0,2 and 3. Parameters derived from an analysis of elastic pion scattering and SCX data also provide an adequate description of the inelastic transitions. The charge asymmetry in the cross sections for the 9/2/sup +/ state that was seen at resonance persists at these energies. This result is consistent with an impulse approximation treatment of the spin-flip amplitude. This is true even though the incoming energy of the pions is far below the range where the validity of an impulse treatment is expected. 65 refs., 45 figs.

  15. A short working distance multiple crystal x-ray spectrometer

    SciTech Connect (OSTI)

    Dickinson, B.; Seidler, G. T.; Webb, Z. W.; Bradley, J. A.; Nagle, K. P. [Department of Physics, University of Washington, Seattle, Washington 98195 (United States); Heald, S. M. [Advanced Photon Source, Argonne National Laboratories, Argonne, Illinois 60439 (United States); Gordon, R. A. [Department of Physics, Simon Fraser University, Burnaby, British Columbia V5A 1S6 (Canada); Chou, I. M. [U.S. Geological Survey, Reston, Virginia 20192 (United States)

    2008-12-15

    For x-ray spot sizes of a few tens of microns or smaller, a millimeter-sized flat analyzer crystal placed {approx}1 cm from the sample will exhibit high energy resolution while subtending a collection solid angle comparable to that of a typical spherically bent crystal analyzer (SBCA) at much larger working distances. Based on this observation and a nonfocusing geometry for the analyzer optic, we have constructed and tested a short working distance (SWD) multicrystal x-ray spectrometer. This prototype instrument has a maximum effective collection solid angle of 0.14 sr, comparable to that of 17 SBCA at 1 m working distance. We find good agreement with prior work for measurements of the Mn K{beta} x-ray emission and resonant inelastic x-ray scattering for MnO, and also for measurements of the x-ray absorption near-edge structure for Dy metal using L{alpha}{sub 2} partial-fluorescence yield detection. We discuss future applications at third- and fourth-generation light sources. For concentrated samples, the extremely large collection angle of SWD spectrometers will permit collection of high-resolution x-ray emission spectra with a single pulse of the Linac Coherent Light Source. The range of applications of SWD spectrometers and traditional multi-SBCA instruments has some overlap, but also is significantly complementary.

  16. Inelastic magnetic neutron scattering in CePd{sub 3}.

    SciTech Connect (OSTI)

    Lawrence, J. M.; Fanelli, V. R.; Goremychkin, E. A.; Osborn, R.; Bauer, E. D.; McClellan, K. J.; Christianson, A. D.; Univ. of California at Irvine; LANL; ORNL

    2008-01-01

    We have performed time-of-flight neutron scattering measurements on a single crystal of the intermediate valence compound CePd{sub 3}. At 10 K, a Kondo-esque inelastic magnetic scattering peak occurs near {Delta}E = 60 meV with maximum intensity for momentum transfer Q near the (1/2, 1/2, 0) zone boundary. Spectral weight is transferred to lower energy as Q varies until at zone center the intensity at 60 meV is considerably weaker. These results are in qualitative accord with predictions of the Anderson lattice. The Q-dependence may resolve an older controversy concerning the low-temperature scattering. We discuss the relationship of these results to our recent results in YbAl{sub 3}.

  17. Power Corrections to Event Shapes in Deep Inelastic Scattering

    E-Print Network [OSTI]

    M. Dasgupta; B. R. Webber

    1997-04-11

    We investigate the power-suppressed corrections to the mean values of various quantities that characterise the shapes of final states in deep inelastic lepton scattering. Our method is based on an analysis of one-loop Feynman graphs containing a massive gluon, which is equivalent to the evaluation of leading infrared renormalon contributions. As in $\\ee$ annihilation, we find that the leading corrections are proportional to $1/Q$. We give quantitative estimates based on the hypothesis of a universal low-energy effective coupling.

  18. Protein Folding Dynamics Detected By Time-Resolved Synchrotron X-ray Small-Angle Scattering Technique

    SciTech Connect (OSTI)

    Fujisawa, Tetsuro; Takahashi, Satoshi [RIKEN Harima Institute, SPring-8 Center, Laboratory for Biometal Science, Hyogo 679-5148 (Japan); Institute for Protein Research, Osaka University Suita Osaka 565-0871/CREST, JST (Japan)

    2007-03-30

    The polypeptide collapse is an essential dynamics in protein folding. To understand the mechanism of the collapse, in situ observation of folding by various probes is necessary. The changes in secondary and tertiary structures in the folding process of globular proteins, whose chain lengths are less than 300 polypeptides, were observed by circular dichrosim and intrinsic fluorescence spectroscopies, respectively. On the other hand, those in protein compactness could be only detected by using time-resolved synchrotron x-ray small-angle scattering technique. The observed dynamics for several proteins with different topologies suggested a common folding mechanism termed 'collapse and search' dynamics, in which the polypeptide collapse precedes the formation of the native contact formation. In 'collapse and search' dynamics, the most outstanding feature lied in the compactness of the initial intermediates. The collapsed intermediates demonstrated the scaling relationship between radius of gyration (Rg) and chain length with a scaling exponent of 0.35 {+-} 0.11, which is close to the value (1/3) predicted by mechano-statistical theory for the collapsed globules of polymers in poor solvent. Thus, it was suggested that the initial collapse is caused by the coil-globule transition of polymers. Since the collapse is essential to the folding of larger proteins, further investigations on the collapse likely lead to an important insight into the protein folding phenomena.

  19. Parallel Computational Modelling of Inelastic Neutron Scattering in Multi-node and Multi-core Architectures 

    E-Print Network [OSTI]

    Garba, M.T.; Gonzales-Velez, H.; Roach, D.L.

    2010-11-26

    This paper examines the initial parallel implementation of SCATTER, a computationally intensive inelastic neutron scattering routine with polycrystalline averaging capability, for the General Utility Lattice Program (GULP). Of particular importance...

  20. Thermal Effects on NeutrinoNucleus Inelastic Scattering in Stellar Environments

    E-Print Network [OSTI]

    Ponomarev, Vladimir

    NUCLEI Theory Thermal Effects on Neutrino­Nucleus Inelastic Scattering in Stellar Environments A. A, 2010 Abstract--Thermal effects for inelastic neutrino­nucleus scattering off even­even nuclei temperatures during the supernova core collapse. The thermal population of the excited states significantly

  1. Interrogation of Surface, Skin, and Core Orientation in Thermotropic Liquid-Crystalline Copolyester Moldings by Near-Edge X-ray Absorption Fine Structure and Wide-Angle X-ray Scattering

    SciTech Connect (OSTI)

    Rendon,S.; Bubeck, R.; Thomas, L.; Burghardt, W.; Hexemer, A.; Fischer, D.

    2007-01-01

    Injection molding thermotropic liquid-crystalline polymers (TLCPs) usually results in the fabrication of molded articles that possess complex states of orientation that vary greatly as a function of thickness. 'Skin-core' morphologies are often observed in TLCP moldings. Given that both 'core' and 'skin' orientation states may often differ both in magnitude and direction, deconvolution of these complex orientation states requires a method to separately characterize molecular orientation in the surface region. A combination of two-dimensional wide-angle X-ray scattering (WAXS) in transmission and near-edge X-ray absorption fine structure (NEXAFS) spectroscopy is used to probe the molecular orientation in injection molded plaques fabricated from a 4,4'-dihydroxy-{alpha}-methylstilbene (DH{alpha}MS)-based thermotropic liquid crystalline copolyester. Partial electron yield (PEY) mode NEXAFS is a noninvasive ex situ characterization tool with exquisite surface sensitivity that samples to a depth of 2 nm. The effects of plaque geometry and injection molding processing conditions on surface orientation in the regions on- and off- axis to the centerline of injection molded plaques are presented and discussed. Quantitative comparisons are made between orientation parameters obtained by NEXAFS and those from 2D WAXS in transmission, which are dominated by the microstructure in the skin and core regions. Some qualitative comparisons are also made with 2D WAXS results from the literature.

  2. An investigation of the spin structure of the proton in deep inelastic scattering of polarised muons on polarised protons

    E-Print Network [OSTI]

    Ashman, John Gavin; Baum, G; Beaufays, J; Bee, C P; Benchouk, C; Bird, I G; Brown, S C; Caputo, M C; Cheung, H W K; Chima, J S; Cibarowski, J; Clifft, R W; Coignet, G; Combley, F; Court, G R; D'Agostini, Giulio; Drees, J; Düren, M; Dyce, N; Edwards, A W; Edwards, M; Ernst, T; Ferrero, M I; Francis, D; Gabathuler, Erwin; Gamet, R; Gibson, V; Gillies, James D; Grafström, P; Hamacher, K; Von Harrach, D; Hayman, P J; Holt, J R; Hughes, V W; Jacholkowska, A; Jones, T; Kabuss, E M; Korzen, B; Krüner, U; Kullander, Sven; Landgraf, U; Lanske, D; Lattenstrom, F; Lindqvist, T; Loken, J G; Matthews, N; Mizuno, Y; Mönig, K; Montanet, François; Nagy, E; Nassalski, J P; Niinikoski, T O; Norton, P R; Oakham, F G; Oppenheim, R F; Osborne, A M; Papavassiliou, V; Pavel, N; Peroni, C; Peschel, H; Piegaia, R; Pietrzyk, B; Pietrzyk, U; Povh, B; Renton, P B; Rieubland, Jean Michel; Rijllart, A; Rith, K; Rondio, Ewa; Ropelewski, Leszek; Salmon, D P; Sandacz, A; Schröder, T B; Schüler, K P; Schultze, K; Shibata, T A; Sloan, Terence; Staiano, A; Stier, H E; Stock, J T; Taylor, G N; Thompson, J C; Walcher, T; Tóth, J; Urbàn, L; Wallucks, W; Wheeler, S; Williams, D A; Williams, W S C; Wimpenny, S J; Windmolders, R; Womersley, W J; Ziemons, K

    1989-01-01

    An investigation of the spin structure of the proton in deep inelastic scattering of polarised muons on polarised protons

  3. Mass fractal characteristics of silica sonogels as determined by small-angle x-ray scattering and nitrogen adsorption

    SciTech Connect (OSTI)

    Donatti, D.A.; Vollet, D.R.; Ibanez Ruiz, A.; Mesquita, A.; Silva, T.F.P. [Unesp-Universidade Estadual Paulista, IGCE, Departamento de Fisica, P.O. Box 178 CEP, 13500-970 Rio Claro, Sao Paulo (Brazil)

    2005-01-01

    A sample series of silica sonogels was prepared using different water-tetraethoxysilane molar ratio (r{sub w}) in the gelation step of the process in order to obtain aerogels with different bulk densities after the supercritical drying. The samples were analyzed by means of small-angle x-ray-scattering (SAXS) and nitrogen-adsorption techniques. Wet sonogels exhibit mass fractal structure with fractal dimension D increasing from {approx}2.1 to {approx}2.4 and mass-fractal correlation length {xi} diminishing from {approx}13 nm to {approx}2 nm, as r{sub w} is changed in the nominal range from 66 to 6. The process of obtaining aerogels from sonogels and heat treatment at 500 deg. C, in general, increases the mass-fractal dimension D, diminishes the characteristic length {xi} of the fractal structure, and shortens the fractal range at the micropore side for the formation of a secondary structured particle, apparently evolved from the original wet structure at a high resolution level. The overall mass-fractal dimension D of aerogels was evaluated as {approx}2.4 and {approx}2.5, as determined from SAXS and from pore-size distribution by nitrogen adsorption, respectively. The fine structure of the 'secondary particle' developed in the obtaining of aerogels could be described as a surface-mass fractal, with the correlated surface and mass-fractal dimensions decreasing from {approx}2.4 to {approx}2.0 and from {approx}2.7 to {approx}2.5, respectively, as the aerogel bulk density increases from 0.25 (r{sub w}=66) up to 0.91 g/cm{sup 3} (r{sub w}=6)

  4. Mass fractal characteristics of wet sonogels as determined by small-angle x-ray scattering and differential scanning calorimetry

    SciTech Connect (OSTI)

    Vollet, D. R.; Donatti, D. A.; Ibanez Ruiz, A.; Gatto, F. R. [Departamento de Fisica, Unesp-Univerisdade Estadual Paulista, IGCE, P.O. Box 178 CEP 13500-970 Rio Claro, SP (Brazil)

    2006-07-01

    Low density silica sonogels were prepared from acid sonohydrolysis of tetraethoxysilane. Wet gels were studied by small-angle x-ray scattering (SAXS) and differential scanning calorimetry (DSC). The DSC tests were carried out under a heating rate of 2 deg. C/min from -120 deg. C up to 30 deg. C. Aerogels were obtained by CO{sub 2} supercritical extraction and characterized by nitrogen adsorption and SAXS. The DSC thermogram displays two distinct endothermic peaks. The first, a broad peak extending from about -80 deg. C up to practically 0 deg. C, was associated to the melting of ice nanocrystals with a crystal size distribution with 'pore' diameter ranging from 1 or 2 nm up to about 60 nm, as estimated from Thomson's equation. The second, a sharp peak with onset temperature close to 0 deg. C, was attributed to the melting of macroscopic crystals. The DSC incremental 'nanopore' volume distribution is in reasonable agreement with the incremental pore volume distribution of the aerogel as determined from nitrogen adsorption. No macroporosity was detected by nitrogen adsorption, probably because the adsorption method applies stress on the sample during measurement, leading to a underestimation of pore volume, or because often positive curvature of the solid surface is in aerogels, making the nitrogen condensation more difficult. According to the SAXS results, the solid network of the wet gels behaves as a mass fractal structure with mass fractal dimension D=2.20{+-}0.01 in a characteristic length scale below {xi}=7.9{+-}0.1 nm. The mass fractal characteristics of the wet gels have also been probed from DSC data by means of an earlier applied modeling for generation of a mass fractal from the incremental ''pore'' volume distribution curves. The results are shown to be in interesting agreement with the results from SAXS.

  5. Inner-Shell Excitation Spectroscopy of Fused-Ring Aromatic Molecules by Electron Energy Loss and X-ray Raman Techniques

    E-Print Network [OSTI]

    Hitchcock, Adam P.

    recorded under scattering conditions where electric dipole transitions dominate (2.5 keV residual energy.08). These spectra are interpreted with the aid of ab initio calculations on selected species. They are compared,2-benzanthracene, recorded with inelastic X-ray Raman scattering in the dipole limit (qr

  6. Low-frequency Vibrational Anomalies in -Lactoglobulin: Contribution of Different Hydrogen Classes Revealed by Inelastic Neutron Scattering

    E-Print Network [OSTI]

    Tuscia, Università Degli Studi Della

    Revealed by Inelastic Neutron Scattering A. Orecchini, A. Paciaroni, A. R. Bizzarri, and S. Cannistraro -lactoglobulin has been investigated by inelastic neutron scattering, on both dry and D2O-hydrated samples. Both typically accessible energy and momentum transfers, inelastic thermal neutron scattering is probably

  7. Deep Inelastic Scattering from Holographic Spin-One Hadrons

    E-Print Network [OSTI]

    Ezequiel Koile; Sebastian Macaluso; Martin Schvellinger

    2011-12-30

    We study deep inelastic scattering structure functions from hadrons using different holographic dual models which describe the strongly coupled regime of gauge theories in the large $N$ limit. Particularly, we consider scalar and vector mesons obtained from holographic descriptions with fundamental degrees of freedom, corresponding to ${\\cal {N}}=2$ supersymmetric and non-supersymmetric Yang-Mills theories. We explicitly obtain analytic expressions for the full set of eight structure functions, i.e., $F_1$, $F_2$, $g_1$, $g_2$, $b_1$, $b_2$, $b_3$, $b_4$, arising from the standard decomposition of the hadronic tensor of spin-one hadrons. We obtain the relations $2 F_1 = F_2$ and $2 b_1 = b_2$. In addition, we find $b_1 \\sim {\\cal {O}}(F_1)$ as suggested by Hoodbhoy, Jaffe and Manohar for vector mesons. Also, we find new relations among some of these structure functions.

  8. Saturation in diffractive deep inelastic eA scattering

    E-Print Network [OSTI]

    M. S. Kugeratski; V. P. Goncalves; F. S. Navarra

    2006-02-24

    In this paper we investigate the saturation physics in diffractive deep inelastic electron-ion scattering. We estimate the energy and nuclear dependence of the ratio $\\sigma^{diff}/\\sigma^{tot}$ and predict the $x_{\\pom}$ and $\\beta$ behavior of the nuclear diffractive structure function $F_{2,A}^{D(3)}(Q^2, \\beta, x_{IP})$. Moreover, we analyze the ratio $R^{diff}_{A1,A2}(Q^2, \\beta, x_{IP}) = F_{2,A1} ^{D(3)}/F_{2,A2} ^{D(3)}$, which probes the nuclear dependence of the structure of the Pomeron. We show that saturation physics predicts that approximately 37 % of the events observed at eRHIC should be diffractive.

  9. Nuclear spin response studies in inelastic polarized proton scattering

    SciTech Connect (OSTI)

    Jones, K.W.

    1988-01-01

    Spin-flip probabilities S/sub nn/ have been measured for inelastic proton scattering at incident proton energies around 300 MeV from a number of nuclei. At low excitation energies S/sub nn/ is below the free value. For excitation energies above about 30 MeV for momentum transfers between about 0.35 fm/sup /minus/1/ and 0.65 fm/sup / minus/1/ S/sub nn/ exceeds free values significantly. These results suggest that the relative ..delta..S = 1(..delta..S = 0 + ..delta..S = 1) nuclear spin response approaches about 90% in the region of the enhancement. Comparison of the data with slab response calculations are presented. Decomposition of the measured cross sections into sigma(..delta..S = 0) and sigma(..delta..S = 1) permit extraction of nonspin-flip and spin-flip dipole and quadrupole strengths. 29 refs., 11 figs.

  10. Structural and magnetic properties of transition metal substituted BaFe{sub 2}As{sub 2} compounds studied by x-ray and neutron scattering

    SciTech Connect (OSTI)

    Kim, Min Gyu [Ames Laboratory

    2012-08-28

    The purpose of my dissertation is to understand the structural and magnetic properties of the newly discovered FeAs-based superconductors and the interconnection between superconductivity, antiferromagnetism, and structure. X-ray and neutron scattering techniques are powerful tools to directly observe the structure and magnetism in this system. I used both xray and neutron scattering techniques on di#11;erent transition substituted BaFe2As2 compounds in order to investigate the substitution dependence of structural and magnetic transitions and try to understand the connections between them.

  11. The structure of the nucleon Elastic and deep inelastic scattering from nucleons, 19561973

    E-Print Network [OSTI]

    Murayama, Hitoshi

    , scattering of electrons by protons and neutrons is open to direct interpretation. For the scattering8 The structure of the nucleon Elastic and deep inelastic scattering from nucleons, 1956­1973 Hadronic scattering experiments produced extensive and rich data revealing reso- nances and regularities

  12. Scattering Density Profile Model of POPG Bilayers as Determined by Molecular Dynamics Simulations and Small-Angle Neutron and X-ray Scattering Experiments

    SciTech Connect (OSTI)

    Kucerka, Norbert [Canadian Neutron Beam Centre and Comelius University (Slovakia); Holland, B [University of Guelph; Gray, C.G [University of Guelph; Tomberli, B [Brandon University; Katsaras, John [ORNL

    2012-01-01

    We combine molecular dynamics (MD) simulations and experiment, both small-angle neutron (SANS) and small-angle X-ray scattering (SAXS), to determine the precise structure of bilayers composed of 1-palmitoyl-2-oleoyl-sn-glycero-3-phosphatidylglycerol (POPG), a lipid commonly encountered in bacterial membranes. Experiment and simulation are used to develop a one-dimensional scattering density profile (SDP) model suitable for the analysis of experimental data. The joint refinement of such data (i.e., SANS and SAXS) results in the area per lipid that is then used in the fixed-area simulations. In the final step, the direct comparison of simulated-to-experimental data gives rise to the detailed structure of POPG bilayers. From these studies we conclude that POPG s molecular area is 66.0 +/- 1.3 ^2, its overall bilayer thickness is 36.7 +/- 0.7 , and its hydrocarbon region thickness is 27.9 ( 0.6 , assuming a simulated value of 1203 ^3 for the total lipid volume.

  13. Combining THz laser excitation with resonant soft X-ray scattering at the Linac Coherent Light Source

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Turner, Joshua J.; Dakovski, Georgi L.; Hoffmann, Matthias C.; Hwang, Harold Y.; Zarem, Alex; Schlotter, William F.; Moeller, Stefan; Minitti, Michael P.; Staub, Urs; Johnson, Steven; et al

    2015-04-11

    This paper describes the development of new instrumentation at the Linac Coherent Light Source for conducting THz excitation experiments in an ultra high vacuum environment probed by soft X-ray diffraction. This consists of a cantilevered, fully motorized mirror system which can provide 600 kV cm?¹ electric field strengths across the sample and an X-ray detector that can span the full Ewald sphere with in-vacuum motion. The scientific applications motivated by this development, the details of the instrument, and spectra demonstrating the field strengths achieved using this newly developed system are discussed.

  14. In situ x-ray scattering study on the evolution of Ge island morphology and relaxation for low growth rate: Advanced transition to superdomes

    SciTech Connect (OSTI)

    Richard, M.-I. [Departement de Recherche Fondamentale sur la Matiere Condensee/SP2M/NRS, CEA Grenoble, 17 Avenue des Martyrs, F-38054 Grenoble Cedex 9 (France); ID01/ESRF, 6 rue Jules Horowitz, BP 220, F-38043 Grenoble Cedex (France); Schuelli, T. U.; Renaud, G. [Departement de Recherche Fondamentale sur la Matiere Condensee/SP2M/NRS, CEA Grenoble, 17 Avenue des Martyrs, F-38054 Grenoble Cedex 9 (France); Wintersberger, E.; Chen, G.; Bauer, G. [Institut fuer Halbleiter- und Festkrperphysik, Johannes Kepler Universitaet Linz, 4040 Linz (Austria); Holy, V. [Faculty of Mathematics and Physics, Charles University, Ke Karlovu 5, 121 16 Prague (Czech Republic)

    2009-07-15

    The kinetics of the growth of Ge superdomes and their facets on Si(001) surfaces are analyzed as a function of deposited Ge thickness for different growth temperatures and at a low growth rate by in situ grazing-incidence small-angle x-ray scattering in combination with in situ grazing-incidence x-ray diffraction. At a low growth rate, intermixing is found to be enhanced and superdomes are formed already at lower coverages than previously reported. In addition, we observe that at the dome-to-superdome transition, a large amount of material is transferred into dislocated islands, either by dome coalescence or by anomalous coarsening. Once dislocated islands are formed, island coalescence is a rare event and introduction of dislocations is preferred. The superdome growth is thus stabilized by the insertion of dislocations during growth.

  15. Resonant Soft X-Ray Contrast Variation Methods as Composition-Specific Probes of Thin Polymer Film Structure

    E-Print Network [OSTI]

    Welch, Cynthia F.

    2008-01-01

    traditional x-ray and neutron scattering techniques is oftentechniques used in neutron scattering, which requiretraditional x-ray and neutron scattering techniques. 16, 32

  16. A Survey of Students from the National School on Neutron and X-ray Scattering: Communication Habits and Preferences

    SciTech Connect (OSTI)

    Bryant, Rebecca [Bryant Research, LLC

    2010-12-01

    Oak Ridge National Laboratory (ORNL) offers the scientific community unique access to two types of world-class neutron sources at a single site - the Spallation Neutron Source (SNS) and the High Flux Isotope Reactor (HFIR). The 85-MW HFIR provides one of the highest steady-state neutron fluxes of any research reactor in the world. And the SNS is one of the world's most intense pulse neutron beams. Management of these resources is the responsibility of the Neutron Sciences Directorate (NScD). NScD started conducting the National School on Neutron and X-ray Scattering (NXS) in conjunction with the Advanced Photon Source (APS) at Argonne National Laboratory in 2007. This survey was conducted to determine the most effective ways to reach students with information about what SNS and HFIR offer the scientific community, including content and communication vehicles. The emphasis is on gaining insights into compelling messages and the most effective channels, e.g., Web sites and social media, for communicating with students about neutron science The survey was conducted in two phases using a classic qualitative investigation to confirm language and content followed by a survey designed to quantify issues, assumptions, and working hypotheses. Phase I consisted of a focus group in late June 2010 with students attending NXS. The primary intent of the group was to inform development of an online survey. Phase two consisted of an online survey that was developed and pre-tested in July 2010 and launched on August 9, 2010 and remained in the field until September 9, 2010. The survey achieved an overall response rate of 48% for a total of 157 completions. The objective of this study is to determine the most effective ways to reach students with information about what SNS and HFIR offer the scientific community, including content and communication vehicles. The emphasis is on gaining insights into compelling messages and the most effective channels, e.g., Web sites, social media, for communicating with students about neutron science.

  17. Measurement of parity-violating asymmetry in electron-deuteron inelastic scattering

    E-Print Network [OSTI]

    Wang, D.

    The parity-violating asymmetries between a longitudinally polarized electron beam and an unpolarized deuterium target have been measured recently. The measurement covered two kinematic points in the deep-inelastic scattering ...

  18. BioSAXS Sample Changer: a robotic sample changer for rapid and reliable high-throughput X-ray solution scattering experiments

    SciTech Connect (OSTI)

    Round, Adam, E-mail: around@embl.fr; Felisaz, Franck [European Molecular Biology Laboratory, Grenoble Outstation, 71 Avenue des Martyrs, CS 90181, 38042 Grenoble (France); Université Grenoble Alpes–EMBL–CNRS, 71 Avenue des Martyrs, CS 90181, 38042 Grenoble (France); Fodinger, Lukas; Gobbo, Alexandre [European Molecular Biology Laboratory, Grenoble Outstation, 71 Avenue des Martyrs, CS 90181, 38042 Grenoble (France); Huet, Julien [European Molecular Biology Laboratory, Grenoble Outstation, 71 Avenue des Martyrs, CS 90181, 38042 Grenoble (France); Université Grenoble Alpes–EMBL–CNRS, 71 Avenue des Martyrs, CS 90181, 38042 Grenoble (France); Villard, Cyril [European Molecular Biology Laboratory, Grenoble Outstation, 71 Avenue des Martyrs, CS 90181, 38042 Grenoble (France); Blanchet, Clement E., E-mail: around@embl.fr [EMBL c/o DESY, Notkestrasse 85, 22603 Hamburg (Germany); Pernot, Petra; McSweeney, Sean [ESRF, 6 Rue Jules Horowitz, 38000 Grenoble (France); Roessle, Manfred; Svergun, Dmitri I. [EMBL c/o DESY, Notkestrasse 85, 22603 Hamburg (Germany); Cipriani, Florent, E-mail: around@embl.fr [European Molecular Biology Laboratory, Grenoble Outstation, 71 Avenue des Martyrs, CS 90181, 38042 Grenoble (France); Université Grenoble Alpes–EMBL–CNRS, 71 Avenue des Martyrs, CS 90181, 38042 Grenoble (France)

    2015-01-01

    A robotic sample changer for solution X-ray scattering experiments optimized for speed and to use the minimum amount of material has been developed. This system is now in routine use at three high-brilliance European synchrotron sites, each capable of several hundred measurements per day. Small-angle X-ray scattering (SAXS) of macromolecules in solution is in increasing demand by an ever more diverse research community, both academic and industrial. To better serve user needs, and to allow automated and high-throughput operation, a sample changer (BioSAXS Sample Changer) that is able to perform unattended measurements of up to several hundred samples per day has been developed. The Sample Changer is able to handle and expose sample volumes of down to 5 µl with a measurement/cleaning cycle of under 1 min. The samples are stored in standard 96-well plates and the data are collected in a vacuum-mounted capillary with automated positioning of the solution in the X-ray beam. Fast and efficient capillary cleaning avoids cross-contamination and ensures reproducibility of the measurements. Independent temperature control for the well storage and for the measurement capillary allows the samples to be kept cool while still collecting data at physiological temperatures. The Sample Changer has been installed at three major third-generation synchrotrons: on the BM29 beamline at the European Synchrotron Radiation Facility (ESRF), the P12 beamline at the PETRA-III synchrotron (EMBL@PETRA-III) and the I22/B21 beamlines at Diamond Light Source, with the latter being the first commercial unit supplied by Bruker ASC.

  19. PHYSICAL REVIEW B 85, 205440 (2012) Inelastic neutron scattering investigations of the quantum molecular dynamics of a H2 molecule

    E-Print Network [OSTI]

    Turro, Nicholas J.

    2012-01-01

    PHYSICAL REVIEW B 85, 205440 (2012) Inelastic neutron scattering investigations of the quantum transfer arising from the neutron scattering event has also been investigated. The -dependence spectra investigations using infrared (IR),3,13­15 inelastic neutron scattering (INS),3,16,17 and nuclear magnetic

  20. Inelastic scattering of electrons by metastable hydrogen atoms in a laser field

    E-Print Network [OSTI]

    Buica, Gabriela

    2015-01-01

    The inelastic scattering of fast electrons by metastable hydrogen atoms in the presence of a linearly polarized laser field is theoretically studied in the domain of moderate field intensities. The interaction of the hydrogen atom with the laser field is described by first-order time-dependent perturbation theory, while the projectile electrons interacting with the laser field are described by the Gordon-Volkov wave functions. An analytic expression is obtained for the differential scattering cross section in the first-order Born approximation for laser-assisted inelastic e-H(2s) scattering for the 2s-nl excitation. Detailed analytical and numerical results are presented for inelastic scattering accompanied by one-photon absorption, and the angular dependence and resonance structure of the differential cross sections is discussed for the 2s -4l excitation of metastable hydrogen.

  1. Test of the consistency of various linearized semiclassical initial value time correlation functions in application to inelastic neutron scattering from liquid para-hydrogen

    E-Print Network [OSTI]

    Liu, Jian

    2008-01-01

    Theory of Thermal Neutron Scattering. (Dover Publications,S. W. Lovesey, Theory of Neutron Scattering from Condensedwith the inelastic neutron scattering experiment results.

  2. Ultrafast X-ray Sources

    SciTech Connect (OSTI)

    George Neil

    2010-04-19

    Since before the scattering of X-rays off of DNA led to the first understanding of the double helix structure, sources of X-rays have been an essential tool for scientists examining the structure and interactions of matter. The resolution of a microscope is proportional to the wavelength of light so x-rays can see much finer structures than visible light, down to single atoms. In addition, the energy of X-rays is resonant with the core atomic levels of atoms so with appropriate wavelengths the placement of specific atoms in a large molecule can be determined. Over 10,000 scientists use synchrotron sources, storage rings of high energy electrons, each year worldwide. As an example of such use, virtually every picture of a protein or drug molecule that one sees in the scientific press is a reconstruction based on X-ray scattering of synchrotron light from the crystallized form of that molecule. Unfortunately those pictures are static and proteins work through configuration (shape) changes in response to energy transfer. To understand how biological systems work requires following the energy flow to these molecules and tracking how shape changes drive their interaction with other molecules. We'd like to be able to freeze the action of these molecules at various steps along the way with an X-ray strobe light. How fast does it have to be? To actually get a picture of a molecule in a fixed configuration requires X-ray pulses as short as 30 femtoseconds (1/30 of a millionth of a millionth of a second). To capture the energy flow through changes in electronic levels requires a faster strobe, less than 1 femtosecond! And to acquire such information in smaller samples with higher accuracy demands brighter and brighter X-rays. Unfortunately modern synchrotrons (dubbed 3rd Generation Light Sources) cannot deliver such short bright pulses of X-rays. An entirely new approach is required, linear-accelerator (linac-)-based light sources termed 4th or Next Generation Light Sources (NGLSs). Although NGLSs will not displace synchrotrons from their role they do offer exciting new capabilities which can be understood from the physics of the light production in each device.

  3. Test of factorization in diffractive deep inelastic scattering and

    Office of Scientific and Technical Information (OSTI)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantity of NaturalDukeWakefieldSulfateSciTechtail. (Conference)Feedback SystemGimbaled X-RayChinaNanotube(Journal

  4. Ray tracing flux calculation for the small and wide angle x-ray scattering diffraction station at the SESAME synchrotron radiation facility

    SciTech Connect (OSTI)

    Salah, Wa'el; Sanchez del Rio, M.; Hoorani, H.

    2009-09-15

    The calculation for the optics of the synchrotron radiation small and wide angle x-ray scattering beamline, currently under construction at SESAME is described. This beamline is based on a cylindrically bent germanium (111) single crystal with an asymmetric cut of 10.5 deg., followed by a 1.2 m long rhodium coated plane mirror bent into a cylindrical form. The focusing properties of bent asymmetrically cut crystals have not yet been studied in depth. The present paper is devoted to study of a particular application of a bent asymmetrically cut crystal using ray tracing simulations with the SHADOW code. These simulations show that photon fluxes of order of 1.09x10{sup 11} photons/s will be available at the experimental focus at 8.79 keV. The focused beam dimensions will be 2.2 mm horizontal full width at half maximum (FWHM) by 0.12 mm vertical (FWHM).

  5. Changes in Delta-Plutonium Due to Aging as Observed by Continuous in-situ X-ray Scattering

    SciTech Connect (OSTI)

    Saw, Cheng K.; Wall, Mark A.; Chung, Brandon W. [MSTD-CMS, Lawrence Livermore National Laboratory, Livermore, California (United States)

    2007-07-01

    The aging in plutonium is predominantly caused by its internal self irradiation. The self-irradiation in Pu-239 is by the decay process of transmuting the Pu atom into uranium atom and emitting an {alpha}-particle. Most of the lattice damage comes from the uranium recoil resulting in Frenkel type defects consisting of vacancies and self-interstitial atoms, helium in growth and defect clusters and possibly even though it is not yet observed, the generation of voids. As part of the stockpile stewardship, it is important to understand the changes in the structure and microstructures and their correlations to the physical properties. Changes in the physical properties has direct relationship to the quality of the structure, in terms of formation of defects and defect clustering, accumulation of voids, grain boundaries, phase changes and etc. which can adversely affects the stability of the material. These changes are very difficult to monitor because of the high activity of the sample, high atomic number making x-ray and synchrotron probe into the bulk very difficult (neutron probe is not feasible) and the long life time which normally requires decades to measure. In this paper we describe the development of an in-situ in-house transmission X-ray diffraction (XRD) experimental technique used to monitor the structural changes in these materials. This technique calls for a very thin sample of less that 2 {mu}m and to accelerate the aging process due to self-irradiation, spiked alloy of 7.5 weight percent of Pu-238 is used. This is equivalent to roughly 17 times the normal rate of aging. Current results suggest that over a period of 2.8 equivalent years, an increase of 0.5% in unit cell parameter is observed. The increase appears to be an abrupt jump at about 1.1 equivalent years, brought about by the collapsing of the atoms from the interstitials to the lattice sites. Further data analysis is on the way. (authors)

  6. Crystal Structures and Small-angle X-ray Scattering Analysis of UDP-galactopyranose Mutase from the Pathogenic Fungus Aspergillus fumigatus

    SciTech Connect (OSTI)

    Dhatwalia, Richa; Singh, Harkewal; Oppenheimer, Michelle; Karr, Dale B.; Nix, Jay C.; Sobrado, Pablo; Tanner, John J. (Missouri); (LBNL); (VPI-SU)

    2012-05-14

    UDP-galactopyranose mutase (UGM) is a flavoenzyme that catalyzes the conversion of UDP-galactopyranose to UDP-galactofuranose, which is a central reaction in galactofuranose biosynthesis. Galactofuranose has never been found in humans but is an essential building block of the cell wall and extracellular matrix of many bacteria, fungi, and protozoa. The importance of UGM for the viability of many pathogens and its absence in humans make UGM a potential drug target. Here we report the first crystal structures and small-angle x-ray scattering data for UGM from the fungus Aspergillus fumigatus, the causative agent of aspergillosis. The structures reveal that Aspergillus UGM has several extra secondary and tertiary structural elements that are not found in bacterial UGMs yet are important for substrate recognition and oligomerization. Small-angle x-ray scattering data show that Aspergillus UGM forms a tetramer in solution, which is unprecedented for UGMs. The binding of UDP or the substrate induces profound conformational changes in the enzyme. Two loops on opposite sides of the active site move toward each other by over 10 {angstrom} to cover the substrate and create a closed active site. The degree of substrate-induced conformational change exceeds that of bacterial UGMs and is a direct consequence of the unique quaternary structure of Aspergillus UGM. Galactopyranose binds at the re face of the FAD isoalloxazine with the anomeric carbon atom poised for nucleophilic attack by the FAD N5 atom. The structural data provide new insight into substrate recognition and the catalytic mechanism and thus will aid inhibitor design.

  7. Conversion method of powder inelastic scattering data for one-dimensional systems

    SciTech Connect (OSTI)

    Tomiyasu, Dr. Keisuke; Fujita, Prof. Masaki; Kolesnikov, Alexander I; Bewley, Robert I.; Bull, Dr. Martyn J.; Bennington, Dr. Stephen M.

    2009-01-01

    Extracting dispersive magnetic excitations from inelastic neutron scattering data usually requires large single crystals. We present a simple yet powerful method for extracting such information from polycrystalline or powder data for one-dimensional systems. We demonstrate the effectiveness of this data treatment by extracting dispersion curves from powder inelastic neutron scattering data on the one-dimensional spin-half systems: CuGeO3 and Rb2Cu2Mo3O12. For many such materials it is not possible to grow sufficiently large crystals and this method offers a quick and efficient way to study their magnetic excitations.

  8. Photoluminescence due to inelastic exciton-exciton scattering in ZnMgO-alloy thin film

    SciTech Connect (OSTI)

    Chia, C. H.; Chen, J. N.; Hu, Y. M. [Department of Applied Physics, National University of Kaohsiung, Kaohsiung 81148, Taiwan (China)

    2011-09-26

    We studied the photoluminescence of ZnMgO thin film, grown by the radiofrequency sputtering method, as a function of excitation intensity and temperature. As the excitation intensity increases, a nonlinear emission band caused by the radiative recombination of the inelastic exciton-exciton scattering was detected at low temperature. We found that the inelastic exciton-exciton scattering process can only persist up to T {approx} 260 K. The nonlinear emission band observed at room temperature is due to the radiative recombination of the electron-hole plasma.

  9. A scaler-based data acquisition system for measuring parity violation asymmetry in deep inelastic scattering

    E-Print Network [OSTI]

    Pan, Kai, S.M. Massachusetts Institute of Technology

    2013-01-01

    An experiment that measured the parity violating (PV) asymmetry Ad in e- 2H deep inelastic scattering (DIS) at Q2 ~ 1.10 and 1.90 (GeV/c) 2 and XB ~ 0.3 was completed in experimental Hall A at the Thomas Jefferson National ...

  10. LETTER doi:10.1038/nature09866 Controlling inelastic light scattering quantum

    E-Print Network [OSTI]

    Wang, Feng

    with transition energies close to the laser photon energy. Here we achieve this goal by combining highly efficient transport, optical transmis- sion and inelastic light scattering are measured on the same graphene devices- mediate electronic states, which then generate crystal elementary excitations and radiate energy

  11. The AdS Graviton/Pomeron Description of Deep Inelastic Scattering at Small x

    E-Print Network [OSTI]

    Richard C. Brower; Marko Djuric; Ina Sarcevic; Chung-I Tan

    2011-06-28

    In the holographic or AdS/CFT dual to QCD, the Pomeron is identified with a Reggeized Graviton in $AdS_5$. We emphasize the importance of confinement, which in this context corresponds to a deformation of $AdS_5$ geometry in the IR. The holographic Pomeron provides a very good fit to the combined data from HERA for Deep Inelastic Scattering at small $x$, lending new confidence to this AdS dual approach to high energy diffractive scattering.

  12. Inelastic neutron scattering spectrum of H2@C60 and its temperature dependence decoded using rigorous quantum calculations and a new

    E-Print Network [OSTI]

    Turro, Nicholas J.

    Inelastic neutron scattering spectrum of H2@C60 and its temperature dependence decoded using://jcp.aip.org/about/rights_and_permissions #12;THE JOURNAL OF CHEMICAL PHYSICS 139, 064309 (2013) Inelastic neutron scattering spectrum of H2@C60 quantum cal- culations of the inelastic neutron scattering (INS) spectra of this prototypical endohedral

  13. Monitoring simultaneously the growth of nanoparticles and aggregates by in situ ultra-small-angle x-ray scattering

    E-Print Network [OSTI]

    Beaucage, Gregory

    information about primary particles and aggregates from a single scattering experiment. This technique reactor to study the growth dynamics of silica nano- particles. Information about primary Research Center, Cincinnati, Ohio 45221-0012 Jan Ilavsky UNICAT, Advanced Photon Source, Building 438D

  14. Small-Angle X-ray Scattering and Single-Molecule FRET Spectroscopy Produce Highly Divergent Views of the Low-Denaturant Unfolded State

    SciTech Connect (OSTI)

    Yoo, Tae Yeon; Meisburger, Steve P.; Hinshaw, James; Pollack, Lois; Haran, Gilad; Sosnick, Tobin R.; Plaxco, Kevin (Cornell); (WIS-I); (UCSB); (UC)

    2012-10-10

    The results of more than a dozen single-molecule Foerster resonance energy transfer (smFRET) experiments suggest that chemically unfolded polypeptides invariably collapse from an expanded random coil to more compact dimensions as the denaturant concentration is reduced. In sharp contrast, small-angle X-ray scattering (SAXS) studies suggest that, at least for single-domain proteins at non-zero denaturant concentrations, such compaction may be rare. Here, we explore this discrepancy by studying protein L, a protein previously studied by SAXS (at 5 C), which suggested fixed unfolded-state dimensions from 1.4 to 5 M guanidine hydrochloride (GuHCl), and by smFRET (at 25 C), which suggested that, in contrast, the chain contracts by 15-30% over this same denaturant range. Repeating the earlier SAXS study under the same conditions employed in the smFRET studies, we observe little, if any, evidence that the unfolded state of protein L contracts as the concentration of GuHCl is reduced. For example, scattering profiles (and thus the shape and dimensions) collected within {approx} 4 ms after dilution to as low as 0.67 M GuHCl are effectively indistinguishable from those observed at equilibrium at higher denaturant. Our results thus argue that the disagreement between SAXS and smFRET is statistically significant and that the experimental evidence in favor of obligate polypeptide collapse at low denaturant cannot be considered conclusive yet.

  15. Nuclear medium effects in $?(\\bar?)$-nucleus deep inelastic scattering

    E-Print Network [OSTI]

    H. Haider; I. Ruiz Simo; M. Sajjad Athar; M. J. Vicente Vacas

    2011-08-16

    We study the nuclear medium effects in the weak structure functions $F_2(x,Q^2)$ and $F_3(x,Q^2)$ in the deep inelastic neutrino/antineutrino reactions in nuclei. We use a theoretical model for the nuclear spectral functions which incorporates the conventional nuclear effects, such as Fermi motion, binding and nucleon correlations. We also consider the pion and rho meson cloud contributions calculated from a microscopic model for meson-nucleus self-energies. The calculations have been performed using relativistic nuclear spectral functions which include nucleon correlations. Our results are compared with the experimental data of NuTeV and CDHSW.

  16. X-Ray Data from the X-Ray Data Booklet Online

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Thompson, Albert C.; Attwood, David T.; Gullikson, Eric M.; Howells, Malcolm R.; Kortright, Jeffrey B.; Robinson, Arthur L.; Underwood, James H.; Kim, Kwang-Je; Kirz, Janos; Lindau, Ingolf; Pianetta, Piero; Winick, Herman; Williams, Gwyn P.; Scofield, James H.

    The original X-Ray Data Booklet, published in 1985, became a classic reference source. The online version has been significantly revised and updated to reflect today's science. Hundreds of pages of authoritative data provide the x-ray properties of elements, information on synchrotron radiation, scattering processes, optics and detectors, and other related calculations, formulas, and data tables.

  17. Transient x-ray diffraction and its application to materials science and x-ray optics

    SciTech Connect (OSTI)

    Hauer, A.A.; Kopp, R.; Cobble, J.; Kyrala, G.; Springer, R.

    1997-12-01

    Time resolved x-ray diffraction and scattering have been applied to the measurement of a wide variety of physical phenomena from chemical reactions to shock wave physics. Interest in this method has heightened in recent years with the advent of versatile, high power, pulsed x-ray sources utilizing laser plasmas, electron beams and other methods. In this article, we will describe some of the fundamentals involved in time resolved x-ray diffraction, review some of the history of its development, and describe some recent progress in the field. In this article we will emphasize the use of laser-plasmas as the x-ray source for transient diffraction.

  18. The Nature of the Surface Species Formed on Au/TiO2 during the Reaction of H2 and O2: An Inelastic Neutron Scattering Study

    E-Print Network [OSTI]

    Goodman, Wayne

    Neutron Scattering Study Chinta Sivadinarayana, Tushar V. Choudhary, Luke L. Daemen, Juergen Eckert of obvious interest for understanding this process. Vibrational spectroscopy by inelastic neutron scattering

  19. Inelastic neutron and low-frequency Raman scattering in a niobium-phosphate glass for Raman gain applications

    E-Print Network [OSTI]

    Schirmacher, Walter

    Inelastic neutron and low-frequency Raman scattering in a niobium-phosphate glass for Raman gain: Raman scattering; Neutron scattering; Raman gain; Boson peak We present measurements of the vibrational, extracted from specific-heat or neutron scattering measurements [7,8]. Only very recently two of the present

  20. Time-, frequency-, and wavevector-resolved x-ray diffraction from single molecules

    SciTech Connect (OSTI)

    Bennett, Kochise, E-mail: kcbennet@uci.edu; Biggs, Jason D.; Zhang, Yu; Dorfman, Konstantin E.; Mukamel, Shaul, E-mail: smukamel@uci.edu [University of California, Irvine, California 92697-2025 (United States)

    2014-05-28

    Using a quantum electrodynamic framework, we calculate the off-resonant scattering of a broadband X-ray pulse from a sample initially prepared in an arbitrary superposition of electronic states. The signal consists of single-particle (incoherent) and two-particle (coherent) contributions that carry different particle form factors that involve different material transitions. Single-molecule experiments involving incoherent scattering are more influenced by inelastic processes compared to bulk measurements. The conditions under which the technique directly measures charge densities (and can be considered as diffraction) as opposed to correlation functions of the charge-density are specified. The results are illustrated with time- and wavevector-resolved signals from a single amino acid molecule (cysteine) following an impulsive excitation by a stimulated X-ray Raman process resonant with the sulfur K-edge. Our theory and simulations can guide future experimental studies on the structures of nano-particles and proteins.

  1. Chest x-Rays

    Broader source: Energy.gov [DOE]

    The B-reading is a special reading of a standard chest x-ray film performed by a physician certified by the National Institute for Occupational Safety and Health (NIOSH). The reading looks for changes on the chest x-ray that may indicate exposure and disease caused by agents such as asbestos or silica.

  2. X-ray beamsplitter

    DOE Patents [OSTI]

    Ceglio, Natale M. (Livermore, CA); Stearns, Daniel S. (Mountain View, CA); Hawryluk, Andrew M. (Modesto, CA); Barbee, Jr., Troy W. (Palo Alto, CA)

    1989-01-01

    An x-ray beamsplitter which splits an x-ray beam into two coherent parts by reflecting and transmitting some fraction of an incident beam has applications for x-ray interferometry, x-ray holography, x-ray beam manipulation, and x-ray laser cavity output couplers. The beamsplitter is formed of a wavelength selective multilayer thin film supported by a very thin x-ray transparent membrane. The beamsplitter resonantly transmits and reflects x-rays through thin film interference effects. A thin film is formed of 5-50 pairs of alternate Mo/Si layers with a period of 20-250 A. The support membrane is 10-200 nm of silicon nitride or boron nitride. The multilayer/support membrane structure is formed across a window in a substrate by first forming the structure on a solid substrate and then forming a window in the substrate to leave a free-standing structure over the window.

  3. X-ray beamsplitter

    DOE Patents [OSTI]

    Ceglio, N.M.; Stearns, D.G.; Hawryluk, A.M.; Barbee, T.W. Jr.

    1987-08-07

    An x-ray beamsplitter which splits an x-ray beam into two coherent parts by reflecting and transmitting some fraction of an incident beam has applications for x-ray interferometry, x-ray holography, x-ray beam manipulation, and x-ray laser cavity output couplers. The beamsplitter is formed of a wavelength selective multilayer thin film supported by a very thin x-ray transparent membrane. The beamsplitter resonantly transmits and reflects x-rays through thin film interference effects. A thin film is formed of 5--50 pairs of alternate Mo/Si layers with a period of 20--250 A. The support membrane is 10--200 nm of silicon nitride or boron nitride. The multilayer/support membrane structure is formed across a window in a substrate by first forming the structure on a solid substrate and then forming a window in the substrate to leave a free-standing structure over the window. 6 figs.

  4. Deep inelastic scattering cross sections from the gauge/string duality

    E-Print Network [OSTI]

    Ezequiel Koile; Nicolas Kovensky; Martin Schvellinger

    2015-07-28

    Differential cross sections of deep inelastic scattering of charged leptons from hadrons are investigated by using the gauge/string duality. We consider vector mesons derived from different holographic dual models obtaining a general expression. We focus on the strongly coupled regime of dual gauge theories for different values of the Bjorken parameter. We find new predictions which are particularly interesting for differential scattering cross sections of polarized leptons scattered off polarized vector mesons. We also carry out a detailed comparison of the moments of the structure functions with lattice QCD results.

  5. X-Ray Interactions with Matter from the Center for X-Ray Optics (CXRO)

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Henke, B. L.; Gullikson, E. M.; Davis, J. C.

    The primary interactions of low-energy x-rays within condensed matter, viz. photoabsorption and coherent scattering, are described for photon energies outside the absorption threshold regions by using atomic scattering factors. The atomic scattering factors may be accurately determined from the atomic photoabsorption cross sections using modified Kramers-Kronig dispersion relations. From a synthesis of the currently available experimental data and recent theoretical calculations for photoabsorption, the angle-independent, forward-scattering components of the atomic scattering factors have been thus semiempirically determined and tabulated here for 92 elements and for the region 50-30,000 eV. Atomic scattering factors for all angles of coherent scattering and at the higher photon energies are obtained from these tabulated forward-scattering values by adding a simple angle-dependent form-factor correction. The incoherent scattering contributions that become significant for the light elements at the higher photon energies are similarly determined. The basic x-ray interaction relations that are used in applied x-ray physics are presented here in terms of the atomic scattering factors. The bulk optical constants are also related to the atomic scattering factors. These atomic and optical relations are applied to the detailed calculation of the reflectivity characteristics of a series of practical x-ray mirror, multilayer, and crystal monochromators. Comparisons of the results of this semiempirical,"atom-like", description of x-ray interactions for the low-energy region with those of experiment and ab initio theory are presented.

  6. Extracting magnetic cluster size and its distributions in advanced perpendicular recording media with shrinking grain size using small angle x-ray scattering

    SciTech Connect (OSTI)

    Mehta, Virat; Ikeda, Yoshihiro; Takano, Ken; Terris, Bruce D.; Hellwig, Olav; Wang, Tianhan; Wu, Benny; Graves, Catherine; Dürr, Hermann A.; Scherz, Andreas; Stöhr, Jo

    2015-05-18

    We analyze the magnetic cluster size (MCS) and magnetic cluster size distribution (MCSD) in a variety of perpendicular magnetic recording (PMR) media designs using resonant small angle x-ray scattering at the Co L{sub 3} absorption edge. The different PMR media flavors considered here vary in grain size between 7.5 and 9.5?nm as well as in lateral inter-granular exchange strength, which is controlled via the segregant amount. While for high inter-granular exchange, the MCS increases rapidly for grain sizes below 8.5?nm, we show that for increased amount of segregant with less exchange the MCS remains relatively small, even for grain sizes of 7.5 and 8?nm. However, the MCSD still increases sharply when shrinking grains from 8 to 7.5?nm. We show evidence that recording performance such as signal-to-noise-ratio on the spin stand correlates well with the product of magnetic cluster size and magnetic cluster size distribution.

  7. Characterization of nanostructured zirconia prepared by hydrolysis and reverse micelle synthesis by small-angle neutron and X-ray scattering

    SciTech Connect (OSTI)

    Thiyagarajan, P.; Li, X.; Littrell, K.; Seifert, S.; Csencsits, R.; Loong, C.

    1999-12-07

    Low temperature techniques such as hydrolysis and reverse micelle syntheses provide the opportunity to determine the relationship between the structural properties and preparation conditions of zirconia powders as well as to tailor their physicochemical properties. The authors have performed small-angle neutron and synchrotron X-ray scattering (SANS and SAXS) experiments to study the nucleation and organization of zirconia nanoparticles via different preparation routes. First, the formation of reverse micelles in individual and mixed solutions of (ZrOCl{sub 2}+D{sub 2}O)/AOT/C{sub 6}D{sub 5}CD{sub 3}, and (NH{sub 4}OH+H{sub 2}O)/AOT/C{sub 6}D{sub 5}CD{sub 3} systems at water/AOT molar ratio of 20 was characterized. Second, the aggregation of zirconia gels obtained from the reaction of the reverse micelle solutions after heat treatments was studied. Third, the nanostructure of zirconia powders prepared by the reverse micelle method is compared with the corresponding powders prepared by hydrolysis after different heat treatments.

  8. Nuclear Effects in Deep Inelastic Scattering of Charged-Current Neutrino off Nuclear

    E-Print Network [OSTI]

    Duan ChunGui; Li GuangLie; Shen PengNian

    2006-04-18

    Nuclear effect in the neutrino-nucleus charged-Current inelastic scattering process is studied by analyzing the CCFR and NuTeV data. Structure functions $F_2(x,Q^2)$ and $xF_3(x,Q^2)$ as well as differential cross sections are calculated by using CTEQ parton distribution functions and EKRS and HKN nuclear parton distribution functions, and compared with the CCFR and NuTeV data. It is found that the corrections of nuclear effect to the differential cross section for the charged-current anti-neutrino scattering on nucleus are negligible, the EMC effect exists in the neutrino structure function $F_2(x,Q^2)$ in the large $x$ region, the shadowing and anti-shadowing effect occurs in the distribution functions of valence quarks in the small and medium $x$ region,respectively. It is also found that shadowing effects on $F_2(x,Q^2)$ in the small $x$ region in the neutrino-nucleus and the charged-lepton-nucleus deep inelastic scattering processes are different. It is clear that the neutrino-nucleus deep inelastic scattering data should further be employed in restricting nuclear parton distributions.

  9. Intrinsic vs. extrinsic inelastic scattering contributions in kappa-(BEDT-TTF){sub 2}Cu[N(CN){sub 2}]Br - transport measurements under hydrostatic pressure.

    SciTech Connect (OSTI)

    Strack, C.; Akinci, C.; Paschenko, V.; Wolf, B.; Uhrig, E.; Assmus, W.; Schreuer, J.; Wiehl, L.; Schlueter, J.; Wosnitza, J.; Schweitzer, D.; Lang , M.; Materials Science Division; J.W. Goethe-Universitat Frankfurt; Inst.fur Festkorperphysik; Univ. Stuttgart

    2006-12-05

    Interlayer-resistivity measurements have been performed on a variety of single crystals of the quasi-two-dimensional organic superconductor {kappa}-(BEDT-TTF){sub 2}Cu[N(CN){sub 2}]Br. These crystals, which have been synthesized along two somewhat different routes, reveal strongly sample-dependent resistivity profiles: while the majority of samples shows a more or less pronounced {rho}(T) maximum around 90 K with a semiconducting behavior above, some crystals remain metallic at all temperatures T {le} 300 K. In the absence of significant differences in the crystals' structural parameters and chemical compositions, as proved by high-resolution X-ray and electron-probe-microanalysis, these results indicate that real structure phenomena, i.e. disorder and/or defects, may strongly affect the inelastic scattering. Comparative resistivity measurements under He-gas pressure on two crystals with strongly differing {rho}(T) profiles indicate that these additional, sample-dependent scattering contributions are characterized by an extraordinarily strong pressure response which is highly non-monotonous as a function of temperature. No correlations have been found between the strength of these scattering contributions and other characteristic properties such as the glass transition at T{sub g} = 77 K, the temperature T* {approx} 40 K, where the temperature dependence of the resistivity changes rather abruptly, or the superconducting transition temperature T{sub c}.

  10. The new method of interference contributions accounting for inelastic scattering diagrams

    E-Print Network [OSTI]

    Sharph, I V; Deliyergiyev, M A; Merkotan, K K; Chudak, N O; Ptashynskyy, D A; Sokhrannyi, G O; Tykhonov, A V; Volkotrub, Yu V; Shabatura, U V; Rusov, V D

    2015-01-01

    A new method of interference contributions accounting is proposed. This method makes it possible to solve the problem of accounting the particles identity in the final state of the scattering process. This problem requires the calculation of a huge number of multidimensional integrals that express the scattering cross-section through the square modulus of the scattering amplitude. Our method is based on the physical features of the scattering amplitude. We show that the set of all interference contributions may be divided into subsets with the similar contributions. Therefore one does not need to calculate each of them separately. Within this approach it is possible to describe inelastic scattering processes with large number of secondary particles. The method was also verified within the $\\phi^3$ model using the Laplace method for the calculation of multidimensional integrals in order to compute the inclusive rapidity cross-sections. A qualitative description of experimental data was obtained. An important r...

  11. GRS computation of deep inelastic electron scattering on 4He

    E-Print Network [OSTI]

    M. Viviani; A. Kievsky; A. Rinat

    2001-11-16

    We compute cross sections for inclusive scattering of high energy electrons on 4He, based on the two lowest orders of the Gersch-Rodriguez-Smith (GRS) series. The required one- and two-particle density matrices are obtained from non-relativistic 4He wave functions using realistic models for the nucleon-nucleon and three-nucleon interaction. Predictions for E=3.6 GeV agree well with the NE3 SLAC-Virginia data.

  12. Thermal effects on neutrino-nucleus inelastic scattering in stellar environments

    E-Print Network [OSTI]

    Alan A. Dzhioev; A. I. Vdovin; V. Yu. Ponomarev; J. Wambach

    2010-12-12

    Thermal effects for inelastic neutrino-nucleus scattering off even-even nuclei in the iron region are studied. Allowed and first-forbidden contributions to the cross sections are calculated within the quasiparticle random phase approximation, extended to finite temperatures within the Thermo-Field-Dynamics formalism. The GT$_0$ strength distribution at finite temperatures is calculated for the sample nucleus $^{54}$Fe. The neutral-current neutrino-nucleus inelastic cross section is calculated for relevant temperatures during the supernova core collapse. The thermal population of the excited states significantly enhances the cross section at low neutrino energies. In agreement with studies using a large scale shell-model approach the enhancement is mainly due to neutrino up-scattering at finite temperatures.

  13. Measurement of Leading Neutron Production in Deep-Inelastic Scattering at HERA

    E-Print Network [OSTI]

    H1 Collaboration

    2010-01-04

    The production of leading neutrons, where the neutron carries a large fraction x_L of the incoming proton's longitudinal momentum, is studied in deep-inelastic positron-proton scattering at HERA. The data were taken with the H1 detector in the years 2006 and 2007 and correspond to an integrated luminosity of 122 pb^{-1}. The semi-inclusive cross section is measured in the phase space defined by the photon virtuality 6 neutron transverse momentum p_T neutron structure function, F_2^{LN(3)}(Q^2,x,x_L), and the fraction of deep-inelastic scattering events containing a leading neutron are studied as a function of Q^2, x and x_L. Assuming that the pion exchange mechanism dominates leading neutron production, the data provide constraints on the shape of the pion structure function.

  14. X-ray laser

    DOE Patents [OSTI]

    Nilsen, Joseph (Livermore, CA)

    1991-01-01

    An X-ray laser (10) that lases between the K edges of carbon and oxygen, i.e. between 44 and 23 Angstroms, is provided. The laser comprises a silicon (12) and dysprosium (14) foil combination (16) that is driven by two beams (18, 20) of intense line focused (22, 24) optical laser radiation. Ground state nickel-like dysprosium ions (34) are resonantly photo-pumped to their upper X-ray laser state by line emission from hydrogen-like silicon ions (32). The novel X-ray laser should prove especially useful for the microscopy of biological specimens.

  15. Double spin asymmetry AL?T? in charged pion production from deep inelastic scattering on a transversely polarized ³He target

    E-Print Network [OSTI]

    Huang, Jin, Ph. D. Massachusetts Institute of Technology

    2012-01-01

    In this thesis I discuss the first measurement of the beam-target double-spin asymmetry ALT for charged pion electroproduction in deep inelastic electron scattering on a transversely polarized 3He target. These data were ...

  16. Two-loop enhancement factor for 1/Q corrections to event shapes in deep inelastic scattering

    E-Print Network [OSTI]

    Mrinal Dasgupta; Bryan R. Webber

    2000-10-22

    We compute the two-loop enhancement factors for our earlier one-loop calculations of leading (1/Q) power corrections to the mean values of some event shape variables in deep inelastic lepton scattering. The enhancement is found to be equal to the universal ``Milan factor'' for those shape variables considered, provided the one-loop calculation is performed in a particular way. As a result, the phenomenology of power corrections to DIS event shapes remains largely unaffected.

  17. Measurements of transverse momentum in semi-inclusive deep-inelastic scattering at CLAS

    SciTech Connect (OSTI)

    K.A. Griffioen

    2012-12-01

    With mounting experimental evidence that only a small fraction of the proton's spin comes from the spins of its quarks and gluons, the quest for orbital angular momentum has begun. The parton distributions relevant to this depend on transverse quark momenta. Recent CLAS semi-inclusive deep-inelastic scattering measurements probe these new transverse-momentum-dependent parton distributions using longitudinally polarized beams and targets and detecting {pi}{sup +},{pi}{sup -} and {pi}{sup 0} in the final state.

  18. In-Situ Monitoring of the Microstructure of TATB-based Explosive Formulations During Temperature Cycling using Ultra-small Angle X-ray Scattering

    SciTech Connect (OSTI)

    Willey, T M; Hoffman, D M; van Buuren, T; Lauderbach, L; Ilavsky, J; Gee, R H; Maiti, A; Overturf, G; Fried, L

    2008-02-06

    TATB (1,3,5 triamino-2,4,6-trinitrobenzene), an extremely insensitive explosive, is used both in plastic-bonded explosives (PBXs) and as an ultra-fine pressed powder (UFTATB). With both PBXs and UFTATB, an irreversible expansion occurs with temperature cycling known as ratchet growth. In TATB-based explosives using Kel-F 800 as binder (LX-17 and PBX-9502), additional voids, sizes hundreds of nanometers to a few microns account for much of the volume expansion caused by temperature cycling. These voids are in the predicted size regime for hot-spot formation during ignition and detonation, and thus an experimental measure of these voids is important feedback for hot-spot theory and for determining the relationship between void size distributions and detonation properties. Also, understanding the mechanism of ratchet growth allows future choice of explosive/binder mixtures to minimize these types of changes to explosives, further extending PBX shelf life. This paper presents the void size distributions of LX-17, UFTATB, and PBXs using commercially available Cytop M, Cytop A, and Hyflon AD60 binders during temperature cycling between -55 C and 70 C. These void size distributions are derived from ultra-small angle x-ray scattering (USAXS), a technique sensitive to structures from about 10 nm to about 2 mm. Structures with these sizes do not appreciably change in UFTATB, indicating voids or cracks larger than a few microns appear in UFTATB during temperature cycling. Compared to Kel-F 800 binders, Cytop M and Cytop A show relatively small increases in void volume from 0.9% to 1.3% and 0.6% to 1.1%, respectively, while Hyflon fails to prevent irreversible volume expansion (1.2% to 4.6%). Computational mesoscale models of ratchet growth and binder wetting and adhesion properties point to mechanisms of ratchet growth, and are discussed in combination with the experimental results.

  19. Chemical Bonding in Aqueous Ferrocyanide: Experimental and Theoretical X-ray Spectroscopic Study

    E-Print Network [OSTI]

    Engel, Nicholas; Suljoti, Edlira; Garcia-Diez, Raul; Lange, Kathrin M; Atak, Kaan; Golnak, Ronny; Kothe, Alexander; Dantz, Marcus; Kühn, Oliver; Aziz, Emad F

    2013-01-01

    Resonant inelastic X-ray scattering (RIXS) and X-ray absorption (XA) experiments at the iron L- and nitrogen K-edge are combined with high-level first principles restricted active space self-consistent field (RASSCF) calculations for a systematic investigation of the nature of the chemical bond in potassium ferrocyanide in aqueous solution. The atom- and site-specific RIXS excitations allow for direct observation of ligand-to-metal (Fe L-edge) and metal-to-ligand (N K-edge) charge transfer bands and thereby evidence for strong {\\sigma}-donation and {\\pi}-back-donation. The effects are identified by comparing experimental and simulated spectra related to both the unoccupied and occupied molecular orbitals in solution.

  20. [Inelastic electron scattering from surfaces]. [Annual] progress report

    SciTech Connect (OSTI)

    Not Available

    1993-10-01

    This program is aimed at the quantitative study of surface dynamical processes (vibrational, magnetic excitations) in crystalline slabs, ultrathin-layered materials, and chemisorbed systems on substrates, and of the geometric structure connected to these dynamical excitations. High-resolution electron-energy loss spectroscopy (HREELS) is a powerful probe. Off-specular excitation cross sections are much larger if electron energies are in the LEED range (50-300 eV). The analyses has been used to study surfaces of ordered alloys (NiAl). Ab-initio surface lattice dynamical results were combined with phonon-loss cross sections to achieve a more accurate microscopic description. First-principles phonon eigenvectors and eigenfrequencies were used as inputs to electron-energy-loss multiple scattering cross-section calculations. The combined microscopic approach was used to analyze EELS data of Cu(0001) and Ag(001) at two points. Positron diffraction is discussed as a structural and imaging tool. The relation between geometric structure of a film and its local magnetic properties will be studied in the future, along with other things.

  1. Photon Correlations Generated by Inelastic Scattering in a One-Dimensional Waveguide Coupled to Three-Level Systems

    E-Print Network [OSTI]

    Fang, Yao-Lung L

    2015-01-01

    We study photon correlations generated by scattering from three-level systems (3LS) in one dimension. The two systems studied are a 3LS in a semi-infinite waveguide (3LS plus a mirror) and two 3LS in an infinite waveguide (double 3LS). Our scattering approach naturally connects photon correlation effects with inelastically scattered photons; it corresponds to input-output theory in the weak-probe limit. At the resonance where electromagnetically induced transparency (EIT) occurs, we find that no photons are scattered inelastically and hence there are no induced correlations. Slightly away from EIT, the total inelastically scattered flux is large, being substantially enhanced due to the additional interference paths. This enhancement carries over to the two-photon correlation function, which exhibits non-classical behavior such as strong bunching with a very long time-scale. The long time scale originates from the slow-light effect associated with EIT.

  2. High-order multilayer coated blazed gratings for high resolution soft x-ray spectroscopy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Voronov, Dmitriy L.; Goray, Leonid I.; Warwick, Tony; Yashchuk, Valeriy V.; Padmore, Howard A.

    2015-02-17

    A grand challenge in soft x-ray spectroscopy is to drive the resolving power of monochromators and spectrometers from the 104 achieved routinely today to well above 105. This need is driven mainly by the requirements of a new technique that is set to have enormous impact in condensed matter physics, Resonant Inelastic X-ray Scattering (RIXS). Unlike x-ray absorption spectroscopy, RIXS is not limited by an energy resolution dictated by the core-hole lifetime in the excitation process. Using much higher resolving power than used for normal x-ray absorption spectroscopy enables access to the energy scale of soft excitations in matter. Thesemore »excitations such as magnons and phonons drive the collective phenomena seen in correlated electronic materials such as high temperature superconductors. RIXS opens a new path to study these excitations at a level of detail not formerly possible. However, as the process involves resonant excitation at an energy of around 1 keV, and the energy scale of the excitations one would like to see are at the meV level, to fully utilize the technique requires the development of monochromators and spectrometers with one to two orders of magnitude higher energy resolution than has been conventionally possible. Here we investigate the detailed diffraction characteristics of multilayer blazed gratings. These elements offer potentially revolutionary performance as the dispersive element in ultra-high resolution x-ray spectroscopy. In doing so, we have established a roadmap for the complete optimization of the grating design. Traditionally 1st order gratings are used in the soft x-ray region, but we show that as in the optical domain, one can work in very high spectral orders and thus dramatically improve resolution without significant loss in efficiency.« less

  3. Polarized Deep Inelastic Scattering Off the "Neutron" From Gauge/String Duality

    E-Print Network [OSTI]

    Jian-Hua Gao; Zong-Gang Mou

    2010-05-25

    We investigate deep inelastic scattering off the polarized "neutron" using gauge/string duality. The "neutron" corresponds to a supergravity mode of the neutral dilatino. Through introducing the Pauli interaction term into the action in $\\textrm{AdS}_{5}$ space, we calculate the polarized deep inelastic structure functions of the "neutron" in supergravity approximation at large t' Hooft coupling $\\lambda$ and finite $x$ with $\\lambda^{-1/2}\\ll xneutron" are power suppressed at the same order as the ones of the "proton." Especially, we find the Burkhardt-Cottingham-like sum rule, which is satisfied in the work by Gao and Xiao, is broken due to the Pauli interaction term. We also illustrate how such a Pauli interaction term can arise naturally from higher dimensional fermion-graviton coupling through the usual Kaluza-Klein reduction.

  4. Measurement of parity-violating asymmetry in electron-deuteron inelastic scattering

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Wang, D.; Pan, K.; Subedi, R.; Ahmed, Z.; Allada, K.; Aniol, K. A.; Armstrong, D. S.; Arrington, J.; Bellini, V.; Beminiwattha, R.; et al

    2015-04-01

    The parity-violating asymmetries between a longitudinally-polarized electron beam and an unpolarized deuterium target have been measured recently. The measurement covered two kinematic points in the deep inelastic scattering region and five in the nucleon resonance region. We provide here details of the experimental setup, data analysis, and results on all asymmetry measurements including parity-violating electron asymmetries and those of inclusive pion production and beam-normal asymmetries. The parity-violating deep-inelastic asymmetries were used to extract the electron-quark weak effective couplings, and the resonance asymmetries provided the first evidence for quark-hadron duality in electroweak observables. These electron asymmetries and their interpretation were publishedmore »earlier, but are presented here in more detail.« less

  5. Measurement of Parity-Violating Asymmetry in Electron-Deuteron Inelastic Scattering

    E-Print Network [OSTI]

    D. Wang; K. Pan; R. Subedi; Z. Ahmed; K. Allada; K. A. Aniol; D. S. Armstrong; J. Arrington; V. Bellini; R. Beminiwattha; J. Benesch; F. Benmokhtar; W. Bertozzi; A. Camsonne; M. Canan; G. D. Cates; J. -P. Chen; E. Chudakov; E. Cisbani; M. M. Dalton; C. W. de Jager; R. De Leo; W. Deconinck; X. Deng; A. Deur; C. Dutta; L. El Fassi; J. Erler; D. Flay; G. B. Franklin; M. Friend; S. Frullani; F. Garibaldi; S. Gilad; A. Giusa; A. Glamazdin; S. Golge; K. Grimm; K. Hafidi; J. -O. Hansen; D. W. Higinbotham; R. Holmes; T. Holmstrom; R. J. Holt; J. Huang; C. E. Hyde; C. M. Jen; D. Jones; Hoyoung Kang; P. M. King; S. Kowalski; K. S. Kumar; J. H. Lee; J. J. LeRose; N. Liyanage; E. Long; D. McNulty; D. J. Margaziotis; F. Meddi; D. G. Meekins; L. Mercado; Z. -E. Meziani; R. Michaels; M. Mihovilovic; N. Muangma; K. E. Mesick; S. Nanda; A. Narayan; V. Nelyubin; A. Nuruzzaman; Y. Oh; D. Parno; K. D. Paschke; S. K. Phillips; X. Qian; Y. Qiang; B. Quinn; A. Rakhman; P. E. Reimer; K. Rider; S. Riordan; J. Roche; J. Rubin; G. Russo; K. Saenboonruang; A. Saha; B. Sawatzky; A. Shahinyan; R. Silwal; S. Širca; P. A. Souder; R. Suleiman; V. Sulkosky; C. M. Sutera; W. A. Tobias; G. M. Urciuoli; B. Waidyawansa; B. Wojtsekhowski; L. Ye; B. Zhao; X. Zheng

    2014-11-12

    The parity-violating asymmetries between a longitudinally-polarized electron beam and an unpolarized deuterium target have been measured recently. The measurement covered two kinematic points in the deep inelastic scattering region and five in the nucleon resonance region. We provide here details of the experimental setup, data analysis, and results on all asymmetry measurements including parity-violating electron asymmetries and those of inclusive pion production and beam-normal asymmetries. The parity-violating deep-inelastic asymmetries were used to extract the electron-quark weak effective couplings, and the resonance asymmetries provided the first evidence for quark-hadron duality in electroweak observables. These electron asymmetries and their interpretation were published earlier, but are presented here in more detail.

  6. Large volume high-pressure cell for inelastic neutron scattering W. Wang, D. A. Sokolov, A. D. Huxley, and K. V. Kamenev

    E-Print Network [OSTI]

    Hall, Christopher

    Large volume high-pressure cell for inelastic neutron scattering W. Wang, D. A. Sokolov, A. D for inelastic neutron scattering measurements of quantum fluids and solids Rev. Sci. Instrum. 84, 015101 (2013) TOF-SEMSANS--Time-of-flight spin-echo modulated small-angle neutron scattering J. Appl. Phys. 112

  7. Compton backscattered collmated X-ray source

    DOE Patents [OSTI]

    Ruth, Ronald D. (Woodside, CA); Huang, Zhirong (Stanford, CA)

    2000-01-01

    A high-intensity, inexpensive and collimated x-ray source for applications such as x-ray lithography is disclosed. An intense pulse from a high power laser, stored in a high-finesse resonator, repetitively collides nearly head-on with and Compton backscatters off a bunched electron beam, having relatively low energy and circulating in a compact storage ring. Both the laser and the electron beams are tightly focused and matched at the interaction region inside the optical resonator. The laser-electron interaction not only gives rise to x-rays at the desired wavelength, but also cools and stabilizes the electrons against intrabeam scattering and Coulomb repulsion with each other in the storage ring. This cooling provides a compact, intense bunch of electrons suitable for many applications. In particular, a sufficient amount of x-rays can be generated by this device to make it an excellent and flexible Compton backscattered x-ray (CBX) source for high throughput x-ray lithography and many other applications.

  8. Compton backscattered collimated x-ray source

    DOE Patents [OSTI]

    Ruth, R.D.; Huang, Z.

    1998-10-20

    A high-intensity, inexpensive and collimated x-ray source is disclosed for applications such as x-ray lithography is disclosed. An intense pulse from a high power laser, stored in a high-finesse resonator, repetitively collides nearly head-on with and Compton backscatters off a bunched electron beam, having relatively low energy and circulating in a compact storage ring. Both the laser and the electron beams are tightly focused and matched at the interaction region inside the optical resonator. The laser-electron interaction not only gives rise to x-rays at the desired wavelength, but also cools and stabilizes the electrons against intrabeam scattering and Coulomb repulsion with each other in the storage ring. This cooling provides a compact, intense bunch of electrons suitable for many applications. In particular, a sufficient amount of x-rays can be generated by this device to make it an excellent and flexible Compton backscattered x-ray (CBX) source for high throughput x-ray lithography and many other applications. 4 figs.

  9. Compton backscattered collimated x-ray source

    DOE Patents [OSTI]

    Ruth, Ronald D. (Woodside, CA); Huang, Zhirong (Stanford, CA)

    1998-01-01

    A high-intensity, inexpensive and collimated x-ray source for applications such as x-ray lithography is disclosed. An intense pulse from a high power laser, stored in a high-finesse resonator, repetitively collides nearly head-on with and Compton backscatters off a bunched electron beam, having relatively low energy and circulating in a compact storage ring. Both the laser and the electron beams are tightly focused and matched at the interaction region inside the optical resonator. The laser-electron interaction not only gives rise to x-rays at the desired wavelength, but also cools and stabilizes the electrons against intrabeam scattering and Coulomb repulsion with each other in the storage ring. This cooling provides a compact, intense bunch of electrons suitable for many applications. In particular, a sufficient amount of x-rays can be generated by this device to make it an excellent and flexible Compton backscattered x-ray (CBX) source for high throughput x-ray lithography and many other applications.

  10. X-ray microtomography

    SciTech Connect (OSTI)

    Landis, Eric N.; Keane, Denis T.

    2010-12-15

    In this tutorial, we describe X-ray microtomography as a technique to nondestructively characterize material microstructure in three dimensions at a micron level spatial resolution. While commercially available laboratory scale instrumentation is available, we focus our attention on synchrotron-based systems, where we can exploit a high flux, monochromatic X-ray beam to produce high fidelity three-dimensional images. A brief description of the physics and the mathematical analysis behind the technique is followed by example applications to specific materials characterization problems, with a particular focus on the utilization of three-dimensional image processing that can be used to extract a wide range of useful information.

  11. Final-state interactions in semi-inclusive deep inelastic scattering off the Deuteron

    SciTech Connect (OSTI)

    Wim Cosyn, Misak Sargsian

    2011-07-01

    Semi-inclusive deep inelastic scattering off the Deuteron with production of a slow nucleon in recoil kinematics is studied in the virtual nucleon approximation, in which the final state interaction (FSI) is calculated within general eikonal approximation. The cross section is derived in a factorized approach, with a factor describing the virtual photon interaction with the off-shell nucleon and a distorted spectral function accounting for the final-state interactions. One of the main goals of the study is to understand how much the general features of the diffractive high energy soft rescattering accounts for the observed features of FSI in deep inelastic scattering (DIS). Comparison with the Jefferson Lab data shows good agreement in the covered range of kinematics. Most importantly, our calculation correctly reproduces the rise of the FSI in the forward direction of the slow nucleon production angle. By fitting our calculation to the data we extracted the W and Q{sup 2} dependences of the total cross section and slope factor of the interaction of DIS products, X, off the spectator nucleon. This analysis shows the XN scattering cross section rising with W and decreasing with an increase of Q{sup 2}. Finally, our analysis points at a largely suppressed off-shell part of the rescattering amplitude.

  12. A phenomenological analysis of azimuthal asymmetries in unpolarized semi-inclusive deep inelastic scattering

    E-Print Network [OSTI]

    V. Barone; M. Boglione; J. O. Gonzalez Hernandez; S. Melis

    2015-04-03

    We present a phenomenological analysis of the cos-phi and cos-2phi asymmetries in unpolarized semi-inclusive deep inelastic scattering, based on the recent multidimensional data released by the COMPASS and HERMES Collaborations. In the TMD framework, valid at relatively low transverse momenta, these asymmetries arise from intrinsic transverse momentum and transverse spin effects, and from their correlations. The role of the Cahn and Boer-Mulders effects in both azimuthal moments is explored up to order 1/Q. As the kinematics of the present experiments is dominated by the low-Q^2 region, higher-twist contributions turn out to be important, affecting the results of our fits.

  13. A phenomenological analysis of azimuthal asymmetries in unpolarized semi-inclusive deep inelastic scattering

    E-Print Network [OSTI]

    Barone, V; Hernandez, J O Gonzalez; Melis, S

    2015-01-01

    We present a phenomenological analysis of the cos-phi and cos-2phi asymmetries in unpolarized semi-inclusive deep inelastic scattering, based on the recent multidimensional data released by the COMPASS and HERMES Collaborations. In the TMD framework, valid at relatively low transverse momenta, these asymmetries arise from intrinsic transverse momentum and transverse spin effects, and from their correlations. The role of the Cahn and Boer-Mulders effects in both azimuthal moments is explored up to order 1/Q. As the kinematics of the present experiments is dominated by the low-Q^2 region, higher-twist contributions turn out to be important, affecting the results of our fits.

  14. Partonic Transverse Motion in Unpolarized Semi-Inclusive Deep Inelastic Scattering Processes

    SciTech Connect (OSTI)

    M. Boglione, S. Melis, A. Prokudin

    2011-08-01

    We analyse the role of partonic transverse motion in unpolarized Semi-Inclusive Deep Inelastic Scattering (SIDIS) processes. Imposing appropriate kinematical conditions, we find some constraints which fix an upper limit to the range of allowed k_perp values. We show that, applying these additional requirements on the partonic kinematics, we obtain different results with respect to the usual phenomenological approach based on the Gaussian smearing with analytical integration over an unlimited range of k_perp values. These variations are particularly interesting for some observables, like the < cos phi_h > azimuthal modulation of the unpolarized SIDIS cross section or the average transverse momentum of the final, detected hadron.

  15. Beauty Production in Deep Inelastic Scattering at HERA using Decays into Electrons

    E-Print Network [OSTI]

    R. Shehzadi

    2011-09-22

    The results from a recent analysis on beauty production in deep inelastic scattering at HERA using decays into electrons from the ZEUS collaboration are presented. The fractions of events containing b quarks were extracted from a likelihood fit using variables sensitive to electron identification as well as to semileptonic decays. Total and differential cross sections were measured and compared with next-to-leading-order QCD calculations. The beauty contribution to the proton structure function F_2 was extracted from the double-differential cross sections.

  16. PDF Nuclear Corrections for Charged Lepton and Neutrino Deep Inelastic Scattering Processes

    E-Print Network [OSTI]

    I. Schienbein; J. Y. Yu; K. Kovarik; C. Keppel; J. G. Morfin; F. Olness; J. F. Owens

    2010-02-11

    We perform a \\chi^2-analysis of Nuclear Parton Distribution Functions (NPDFs) using neutral current charged-lepton Deeply Inelastic Scattering (DIS) and Drell-Yan data for several nuclear targets. The nuclear A dependence of the NPDFs is extracted in a next-to-leading order fit. We compare the nuclear corrections factors F2(Fe)/F2(D) for this charged-lepton data with other results from the literature. In particular, we compare and contrast fits based upon the charged-lepton DIS data with those using neutrino-nucleon DIS data.

  17. Measurement of Dijet Production in Diffractive Deep-Inelastic Scattering at HERA

    E-Print Network [OSTI]

    Schmitt, Stefan

    2015-01-01

    The production of dijets is measured in diffractive deep-inelastic scattering at HERA. The data were recorded with the H1 detector at DESY in the years 2003-2007. Diffractive events are selected by requiring a gap in the rapidity distribution of the hadronic systen, where no particles are produced. Two jets are selected with transverse momenta in the hadronic-centre-of-mass system larger than 4 and 5.5GeV, respectively. Cross sections are measured single- and doubledifferentially in various kinematic quantities. The data are found to be in good agreement with NLO QCD calculations based on diffractive parton densities determined frominclusive diffractive cross section measurements.

  18. Nuclear shadowing in deep inelastic scattering on nuclei at low and medium Q^2

    E-Print Network [OSTI]

    Bugaev, Edgar V

    2015-01-01

    Nuclear shadowing corrections to the structure functions of deep inelastic scattering of intermediate-mass nuclei are calculated at very low values of Bjorken x and small values of Q^2 (Q^2<5 GeV^2). The two-component approach (generalized VMD plus hard pomeron) is used for a description of the underlying virtual photon - nucleon interaction. The hard component of the nucleon structure function is calculated in a framework of the colour dipole model with dipole cross section having Regge-type energy dependence. Numerical results for nuclear shadowing corrections are compared with available data of E665 and NMC collaborations.

  19. Final-state interactions in inclusive deep-inelastic scattering from the deuteron

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Cosyn, Wim; Melnitchouk, Wally; Sargsian, Misak M.

    2014-01-01

    We explore the role of final-state interactions (FSI) in inclusive deep-inelastic scattering from the deuteron. Relating the inclusive cross section to the deuteron forward virtual Compton scattering amplitude, a general formula for the FSI contribution is derived in the generalized eikonal approximation, utilizing the diffractive nature of the effective hadron-nucleon interaction. The calculation uses a factorized model with a basis of three resonances with mass W~ 0.6 andmore »Q2 2 increasing in magnitude for lower Q2, but vanishing in the high-Q2 limit due to phase space constraints. The off-shell rescattering contributes at x ~> 0.8 and is taken as an uncertainty on the on-shell result.« less

  20. 6 GeV Parity Violating Deep Inelastic Scattering at Jefferson Laboratory

    SciTech Connect (OSTI)

    Subedi, Ramesh R.; Deng Xiaoyan; Wang Diancheng; Zheng Xiaochao; Michaels, Robert; Pan Kai; Reimer, Paul E.

    2011-10-24

    The 6 GeV Parity Violating Deep Inelastic Scattering (PVDIS) experiment has measured a 10{sup -4} level asymmetry through polarized electron scattering off a liquid deuterium target with a beam energy of 6 GeV. This experiment has a goal of measuring a combination of the product of the weak neutral couplings of the electron and the quark with a factor of six improvement in precision over world data. Precise data for the couplings are essential to search for physics beyond the Standard Model. The experiment took place in Hall A at Thomas Jefferson National Accelerator Facility (Jefferson Laboratory) and data collection was completed in the end of 2009. A highly specialized counting data acquisition system with an inherent particle identification was developed and utilized. We have taken data at two Q{sup 2} points in order to possibly address the hadronic correction due to higher twist effects. An overview of the experiment will be presented.

  1. The new method of interference contributions accounting for inelastic scattering diagrams

    E-Print Network [OSTI]

    I. V. Sharph; O. S. Potiienko; M. A. Deliyergiyev; K. K. Merkotan; N. O. Chudak; D. A. Ptashynskyy; G. O. Sokhrannyi; A. V. Tykhonov; Yu. V. Volkotrub; U. V. Shabatura; V. D. Rusov

    2015-09-14

    A new method of interference contributions accounting is proposed. This method makes it possible to solve the problem of accounting the particles identity in the final state of the scattering process. This problem requires the calculation of a huge number of multidimensional integrals that express the scattering cross-section through the square modulus of the scattering amplitude. Our method is based on the physical features of the scattering amplitude. We show that the set of all interference contributions may be divided into subsets with the similar contributions. Therefore one does not need to calculate each of them separately. Within this approach it is possible to describe inelastic scattering processes with large number of secondary particles. The method was also verified within the $\\phi^3$ model using the Laplace method for the calculation of multidimensional integrals in order to compute the inclusive rapidity cross-sections. A qualitative description of experimental data was obtained. An important result of this work is the explanation of peaks behavior in the inclusive rapidity distributions and their possible interference origin.

  2. X-Ray Data Booklet X-RAY DATA BOOKLET

    E-Print Network [OSTI]

    X-Ray Data Booklet X-RAY DATA BOOKLET Center for X-ray Optics and Advanced Light Source Lawrence Electromagnetic Relations Radioactivity and Radiation Protection Useful Formulas CXRO Home | ALS Home | LBL Home in PDF format Data Booklet Authors CXRO Home | ALS Home | LBL Home Privacy and Security Notice Please

  3. Characterization of a Fe/Y{sub 2}O{sub 3} metal/oxide interface using neutron and x-ray scattering

    SciTech Connect (OSTI)

    Watkins, E. B.; Majewski, J. E-mail: jarek@lanl.gov; Kashinath, A.; Wang, P.; Baldwin, J. K.; Demkowicz, M. J. E-mail: jarek@lanl.gov

    2014-07-28

    The structure of metal/oxide interfaces is important to the radiation resistance of oxide dispersion-strengthened steels. We find evidence of gradual variations in stoichiometry and magnetization across a Fe/Y{sub 2}O{sub 3} metal/oxide heterophase interface using neutron and x-ray reflectometry. These findings suggest that the Fe/Y{sub 2}O{sub 3} interface is a transitional zone approximately ?64?Å-thick containing mixtures or compounds of Fe, Y, and O. Our results illustrate the complex chemical and magnetic nature of Fe/oxide interfaces and demonstrate the utility of combined neutron and x-ray techniques as tools for characterizing them.

  4. Inelastic neutron scattering study of hydrogen in d8-THF/D2O ice clathrate Kimberly T. Tait,a

    E-Print Network [OSTI]

    Downs, Robert T.

    materials is of considerable interest from the per- spective of hydrogen storage for a future hydrogen fuelInelastic neutron scattering study of hydrogen in d8-THF/D2O ice clathrate Kimberly T. Tait,a Frans October 2007 In situ neutron inelastic scattering experiments on hydrogen adsorbed into a fully deutrated

  5. Elastic and inelastic neutron scattering cross sections for fission reactor applications

    SciTech Connect (OSTI)

    Hicks, S. F.; Combs, B.; Downes, L.; Girgis, J.; Kersting, L. J.; Lueck, C. J.; McDonough, P. J.; Schniederjan, J.; Sidwell, L.; Sigillito, A. J. [Department of Physics, University of Dallas, Irving TX 75019 (United States); Chakraborty, A.; Crider, B. P.; Kumar, A.; McEllistrem, M. T.; Peters, E. E.; Prados-Estevz, F. M. [Department of Physics and Astronomy, University of Kentucky, Lexington, KY 40506 (United States); Vanhoy, J. R.; Watts, D. [Department of Physics, United States Naval Academy, Annapolis MD 21402 (United States); Yates, S. W. [Department of Physics and Astronomy, University of Kentucky, Lexington, KY 40506 (United States) and Department of Chemistry, University of Kentucky, Lexington, KY 40506 (United States)

    2013-04-19

    Nuclear data important for the design and development of the next generation of light-water reactors and future fast reactors include neutron elastic and inelastic scattering cross sections on important structural materials, such as Fe, and on coolant materials, such as Na. These reaction probabilities are needed since neutron reactions impact fuel performance during irradiations and the overall efficiency of reactors. While neutron scattering cross sections from these materials are available for certain incident neutron energies, the fast neutron region, particularly above 2 MeV, has large gaps for which no measurements exist, or the existing uncertainties are large. Measurements have been made at the University of Kentucky Accelerator Laboratory to measure neutron scattering cross sections on both Fe and Na in the region where these gaps occur and to reduce the uncertainties on scattering from the ground state and first excited state of these nuclei. Results from measurements on Fe at incident neutron energies between 2 and 4 MeV will be presented and comparisons will be made to model calculations available from data evaluators.

  6. X-ray lithography source

    DOE Patents [OSTI]

    Piestrup, Melvin A. (Woodside, CA); Boyers, David G. (Mountain View, CA); Pincus, Cary (Sunnyvale, CA)

    1991-01-01

    A high-intensity, inexpensive X-ray source for X-ray lithography for the production of integrated circuits. Foil stacks are bombarded with a high-energy electron beam of 25 to 250 MeV to produce a flux of soft X-rays of 500 eV to 3 keV. Methods of increasing the total X-ray power and making the cross section of the X-ray beam uniform are described. Methods of obtaining the desired X-ray-beam field size, optimum frequency spectrum and elminating the neutron flux are all described. A method of obtaining a plurality of station operation is also described which makes the process more efficient and economical. The satisfying of these issues makes transition radiation an exellent moderate-priced X-ray source for lithography.

  7. Pressure-Induced Structural Phase Transition in CeNi: X-ray and Neutron Scattering Studies and First-Principles Calculations

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Mirmelstein, A.; Podlesnyak, Andrey A.; dos Santos, Antonio M.; Ehlers, Georg; Kerbel, O.; Matvienko, V.; Sefat, A. S.; Saporov, B.; Halder, G. J.; Tobin, J. G.

    2015-08-03

    The pressure-induced structural phase transition in the intermediate-valence compound CeNi has been investigated by x-ray and neutron powder diffraction techniques. It is shown that the structure of the pressure-induced CeNi phase (phases) can be described in terms of the Pnma space group. Equations of state for CeNi on both sides of the phase transition are derived and an approximate P-T phase diagram is suggested for Pmore »the phase transition.« less

  8. Test of the consistency of various linearized semiclassical initial value time correlation functions in application to inelastic neutron scattering

    E-Print Network [OSTI]

    Miller, William H.

    -IVR is approximate. Some of the correlation functions involve only linear operators, and others involve nonlinearTest of the consistency of various linearized semiclassical initial value time correlation functions in application to inelastic neutron scattering from liquid para-hydrogen Jian Liua and William H

  9. Unpolarised TMD Distribution and Fragmentation Functions from recent HERMES and COMPASS Semi-inclusive Deep Inelastic Scattering Multiplicities

    SciTech Connect (OSTI)

    Prokudin, Alexey; Anselmino, Mauro; Boglione, Mariaelena; Melis, Stefano; Gonzalez, J. O.

    2014-10-01

    The unpolarised transverse momentum dependent distribution and fragmentation functions (TMDs) are extracted from HERMES and COMPASS experimental measurements of semi- inclusive deep inelastic scattering multiplicities for charged hadron production. A simple factorised functional form of the TMDs is adopted, with a Gaussian dependence on the intrinsic transverse momentum, which turns out to be quite adequate in shape.

  10. Measurement of “pretzelosity” asymmetry of charged pion production in semi-inclusive deep inelastic scattering on a polarized ³He target

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Zhang, Y.; Qian, X.; Allada, K.; Dutta, C.

    2014-11-01

    An experiment to measure single-spin asymmetries in semi-inclusive production of charged pions in deep-inelastic scattering on a transversely polarized ³He target was performed at Jefferson Lab in the kinematic region of 0.16 ± on He3 and on neutron pretzelosity asymmetries are consistent with zero within experimental uncertainties.

  11. X-Ray Diagnostics

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantity ofkandz-cm11 Outreach Home RoomPreservationBio-Inspired SolarAbout /Two0PhotosPresentationsWorld's largest singleX-Ray

  12. Inelastic neutron scattering of a quantum translator-rotator encapsulated in a closed fullerene cage: Isotope effects and translation-rotation coupling in H2@C60 and HD@C60

    E-Print Network [OSTI]

    Turro, Nicholas J.

    Inelastic neutron scattering of a quantum translator-rotator encapsulated in a closed fullerene, New York 10027, USA Received 1 July 2010; published 20 August 2010 We report an inelastic neutron-scattering inelastic neutron scattering INS ,6 and specific heat7 inves- tigations have recently been reported

  13. Deep-inelastic scattering and the operator product expansion in lattice QCD

    E-Print Network [OSTI]

    William Detmold; C. -J. David Lin

    2005-12-13

    We discuss the determination of deep-inelastic hadron structure in lattice QCD. By using a fictitious heavy quark, direct calculations of the Compton scattering tensor can be performed in Euclidean space that allow the extraction of the moments of structure functions. This overcomes issues of operator mixing and renormalisation that have so far prohibited lattice computations of higher moments. This approach is especially suitable for the study of the twist-two contributions to isovector quark distributions, which is practical with current computing resources. While we focus on the isovector unpolarised distribution, our method is equally applicable to other quark distributions and to generalised parton distributions. By looking at matrix elements such as $$ (where $V^\\mu$ and $A^\

  14. Power Corrections to Fragmentation Functions in Non-Singlet Deep Inelastic Scattering

    E-Print Network [OSTI]

    M. Dasgupta; G. E. Smye; B. R. Webber

    1998-03-18

    We investigate the power-suppressed corrections to the fragmentation functions of the current jet in non-singlet deep inelastic lepton-hadron scattering. The current jet is defined by selecting final-state particles in the current hemisphere in the Breit frame of reference. Our method is based on an analysis of one-loop Feynman graphs containing a massive gluon, which is equivalent to the evaluation of leading infrared renormalon contributions. We find that the leading corrections are proportional to $1/Q^2$, as in $e^+e^-$ annihilation, but their functional forms are different. We give quantitative estimates based on the hypothesis of universal low-energy behaviour of the strong coupling.

  15. Longitudinal polarization of hyperon and anti-hyperon in semi-inclusive deep-inelastic scattering

    E-Print Network [OSTI]

    Shan-shan Zhou; Ye Chen; Zuo-tang Liang; Qing-hua Xu

    2009-02-11

    We make a detailed study of the longitudinal polarization of hyperons and anti-hyperons in semi-inclusive deep-inelastic lepton-nucleon scattering. We present the numerical results for spin transfer in quark fragmentation processes, analyze the possible origins for a difference between the polarization for hyperon and that for the corresponding anti-hyperon. We present the results obtained in the case that there is no asymmetry between sea and anti-sea distribution in nucleon as well as those obtained when such an asymmetry is taken into account. We compare the results with the available data such as those from COMPASS and make predictions for future experiments including those at even higher energies such as at eRHIC.

  16. Longitudinal polarization of hyperon and anti-hyperon in semi-inclusive deep-inelastic scattering

    E-Print Network [OSTI]

    Zhou, Shan-shan; Liang, Zuo-tang; Xu, Qing-hua

    2009-01-01

    We make a detailed study of the longitudinal polarization of hyperons and anti-hyperons in semi-inclusive deep-inelastic lepton-nucleon scattering. We present the numerical results for spin transfer in quark fragmentation processes, analyze the possible origins for a difference between the polarization for hyperon and that for the corresponding anti-hyperon. We present the results obtained in the case that there is no asymmetry between sea and anti-sea distribution in nucleon as well as those obtained when such an asymmetry is taken into account. We compare the results with the available data such as those from COMPASS and make predictions for future experiments including those at even higher energies such as at eRHIC.

  17. Resummation for Polarized Semi-Inclusive Deep-Inelastic Scattering at Small Transverse Momentum

    E-Print Network [OSTI]

    Koike, Y; Vogelsang, W; Koike, Yuji; Nagashima, Junji; Vogelsang, Werner

    2006-01-01

    We study the transverse-momentum distribution of hadrons produced in semi-inclusive deep-inelastic scattering (SIDIS). We consider cross sections for various combinations of polarizations of the initial lepton and nucleon or the produced hadron, for which we perform the resummation of large double-logarithmic perturbative corrections arising at small transverse momentum. We present phenomenological results for the processes $lp\\to l\\pi X$ with longitudinally polarized leptons and protons. We discuss the impact of the perturbative resummation and of estimated non-perturbative contributions on the corresponding cross sections and their spin asymmetry. Our results should be relevant for ongoing studies in the COMPASS experiment at CERN, and for future experiments at the proposed eRHIC collider at BNL.

  18. Resummation for Polarized Semi-Inclusive Deep-Inelastic Scattering at Small Transverse Momentum

    E-Print Network [OSTI]

    Yuji Koike; Junji Nagashima; Werner Vogelsang

    2006-05-17

    We study the transverse-momentum distribution of hadrons produced in semi-inclusive deep-inelastic scattering (SIDIS). We consider cross sections for various combinations of polarizations of the initial lepton and nucleon or the produced hadron, for which we perform the resummation of large double-logarithmic perturbative corrections arising at small transverse momentum. We present phenomenological results for the processes $lp\\to l\\pi X$ with longitudinally polarized leptons and protons. We discuss the impact of the perturbative resummation and of estimated non-perturbative contributions on the corresponding cross sections and their spin asymmetry. Our results should be relevant for ongoing studies in the COMPASS experiment at CERN, and for future experiments at the proposed eRHIC collider at BNL.

  19. Leading neutron energy and pT distributions in deep inelastic scattering and photoproduction at HERA

    E-Print Network [OSTI]

    ZEUS Collaboration; S. Chekanov

    2007-03-09

    The production of energetic neutrons in $ep$ collisions has been studied with the ZEUS detector at HERA. The neutron energy and $p_T^2$ distributions were measured with a forward neutron calorimeter and tracker in a $40 \\pb^{-1}$ sample of inclusive deep inelastic scattering (DIS) data and a $6 \\pb^{-1}$ sample of photoproduction data. The neutron yield in photoproduction is suppressed relative to DIS for the lower neutron energies and the neutrons have a steeper $p_T^2$ distribution, consistent with the expectation from absorption models. The distributions are compared to HERA measurements of leading protons. The neutron energy and transverse-momentum distributions in DIS are compared to Monte Carlo simulations and to the predictions of particle exchange models. Models of pion exchange incorporating absorption and additional secondary meson exchanges give a good description of the data.

  20. Hard x-ray emission spectroscopy: a powerful tool for the characterization of magnetic semiconductors

    E-Print Network [OSTI]

    Rovezzi, Mauro

    2014-01-01

    This review aims to introduce the x-ray emission spectroscopy (XES) and resonant inelastic x-ray scattering (RIXS) techniques to the materials scientist working with magnetic semiconductors (e.g. semiconductors doped with 3d transition metals) for applications in the field of spin-electronics. We focus our attention on the hard part of the x-ray spectrum (above 3 keV) in order to demonstrate a powerful element- and orbital-selective characterization tool in the study of bulk electronic structure. XES and RIXS are photon-in/photon-out second order optical processes described by the Kramers-Heisenberg formula. Nowadays, the availability of third generation synchrotron radiation sources permits to apply such techniques also to dilute materials, opening the way for a detailed atomic characterization of impurity-driven materials. We present the K{\\ss} XES as a tool to study the occupied valence states (directly, via valence-to-core transitions) and to probe the local spin angular momentum (indirectly, via intra-at...

  1. Crystal structure of fluorite-related Ln{sub 3}SbO{sub 7} (Ln=La–Dy) ceramics studied by synchrotron X-ray diffraction and Raman scattering

    SciTech Connect (OSTI)

    Siqueira, K.P.F.; Borges, R.M.; Granado, E.; Malard, L.M.; Paula, A.M. de; Moreira, R.L.; Bittar, E.M.; Dias, A.

    2013-07-15

    Ln{sub 3}SbO{sub 7} (Ln=La, Pr, Nd, Sm, Eu, Gd, Tb and Dy) ceramics were synthesized by solid-state reaction in optimized conditions of temperature and time to yield single-phase ceramics. The crystal structures of the obtained ceramics were investigated by synchrotron X-ray diffraction, second harmonic generation (SHG) and Raman scattering. All samples exhibited fluorite-type orthorhombic structures with different oxygen arrangements as a function of the ionic radius of the lanthanide metal. For ceramics with the largest ionic radii (La–Nd), the ceramics crystallized into the Cmcm space group, while the ceramics with intermediate and smallest ionic radii (Sm–Dy) exhibited a different crystal structure belonging to the same space group, described under the Ccmm setting. The results from SHG and Raman scattering confirmed these settings and ruled out any possibility for the non-centrosymmetric C222{sub 1} space group describing the structure of the small ionic radii ceramics, solving a recent controversy in the literature. Besides, the Raman modes for all samples are reported for the first time, showing characteristic features for each group of samples. - Graphical abstract: Raman spectrum for La{sub 3}SbO{sub 7} ceramics showing their 22 phonon modes adjusted through Lorentzian lines. According to synchrotron X-ray diffraction and Raman scattering, this material belongs to the space group Cmcm. - Highlights: • Ln{sub 3}SbO{sub 7} ceramics belonging to the space groups Cmcm and Ccmm are synthesized. • SXRD, SHG and Raman scattering confirmed the orthorhombic structures. • Ccmm instead of C222{sub 1} is the correct one based on SHG and Raman data.

  2. X-ray spectrometry

    SciTech Connect (OSTI)

    Markowicz, A.A.; Van Grieken, R.E.

    1986-04-01

    In the period under review, i.e, through 1984 and 1985, some 600 articles on XRS (X-ray spectrometry) were published; most of these have been scanned and the most fundamental ones are discussed. All references will refer to English-language articles, unless states otherwise. Also general books have appeared on quantitative EPXMA (electron-probe X-ray microanalysis) and analytical electron microscopy (AEM) as well as an extensive review on the application of XRS to trace analysis of environmental samples. In the period under review no radically new developments have been seen in XRS. However, significant improvements have been made. Gain in intensities has been achieved by more efficient excitation, higher reflectivity of dispersing media, and better geometry. Better understanding of the physical process of photon- and electron-specimen interactions led to complex but more accurate equations for correction of various interelement effects. Extensive use of micro- and minicomputers now enables fully automatic operation, including qualitative analysis. However, sample preparation and presentation still put a limit to further progress. Although some authors find XRS in the phase of stabilization or even stagnation, further gradual developments are expected, particularly toward more dedicated equipment, advanced automation, and image analysis systems. Ways are outlined in which XRS has been improved in the 2 last years by excitation, detection, instrumental, methodological, and theoretical advances. 340 references.

  3. A seven-crystal Johann-type hard x-ray spectrometer at the Stanford Synchrotron Radiation Lightsource

    SciTech Connect (OSTI)

    Sokaras, D.; Weng, T.-C.; Nordlund, D.; Velikov, P.; Wenger, D.; Garachtchenko, A.; George, M.; Borzenets, V.; Johnson, B.; Rabedeau, T.; Alonso-Mori, R.; Bergmann, U.

    2013-05-15

    We present a multicrystal Johann-type hard x-ray spectrometer ({approx}5-18 keV) recently developed, installed, and operated at the Stanford Synchrotron Radiation Lightsource. The instrument is set at the wiggler beamline 6-2 equipped with two liquid nitrogen cooled monochromators - Si(111) and Si(311) - as well as collimating and focusing optics. The spectrometer consists of seven spherically bent crystal analyzers placed on intersecting vertical Rowland circles of 1 m of diameter. The spectrometer is scanned vertically capturing an extended backscattering Bragg angular range (88 Degree-Sign -74 Degree-Sign ) while maintaining all crystals on the Rowland circle trace. The instrument operates in atmospheric pressure by means of a helium bag and when all the seven crystals are used (100 mm of projected diameter each), has a solid angle of about 0.45% of 4{pi} sr. The typical resolving power is in the order of (E/{Delta}E){approx}10 000. The spectrometer's high detection efficiency combined with the beamline 6-2 characteristics permits routine studies of x-ray emission, high energy resolution fluorescence detected x-ray absorption and resonant inelastic x-ray scattering of very diluted samples as well as implementation of demanding in situ environments.

  4. Folding model analysis of 240 MeV (6)Li elastic scattering on (116)Sn and inelastic scattering to low-lying states of (116)Sn 

    E-Print Network [OSTI]

    Chen, X.; Lui, Y. -W; Clark, H. L.; Tokimoto, Y.; Youngblood, David H.

    2007-01-01

    with and without density dependence. DWBA calculations with the fitted parameters were used to calculate cross sections for inelastic scattering to low-lying 2(+)and 3(-) states. B(E2) and B(E3) values were extracted and compared with electromagnetic values...

  5. Miniature x-ray source

    DOE Patents [OSTI]

    Trebes, James E. (Livermore, CA); Stone, Gary F. (Livermore, CA); Bell, Perry M. (Tracy, CA); Robinson, Ronald B. (Modesto, CA); Chornenky, Victor I. (Minnetonka, MN)

    2002-01-01

    A miniature x-ray source capable of producing broad spectrum x-ray emission over a wide range of x-ray energies. The miniature x-ray source comprises a compact vacuum tube assembly containing a cathode, an anode, a high voltage feedthru for delivering high voltage to the anode, a getter for maintaining high vacuum, a connection for an initial vacuum pump down and crimp-off, and a high voltage connection for attaching a compact high voltage cable to the high voltage feedthru. At least a portion of the vacuum tube wall is highly x-ray transparent and made, for example, from boron nitride. The compact size and potential for remote operation allows the x-ray source, for example, to be placed adjacent to a material sample undergoing analysis or in proximity to the region to be treated for medical applications.

  6. X-ray and neutron scattering studies of the Rb?MnF? and Cu?â??õxMgx̳GeO? in an external magnetic field

    E-Print Network [OSTI]

    Christianson, Rebecca J. (Rebecca Jean), 1973-

    2001-01-01

    This thesis presents results of two scattering studies of low dimensional magnetic materials. The first is a neutron scattering study of Rb2MnF4, a nearly ideal two-dimensional square lattice Heisenberg antiferromagnet ...

  7. A Preliminary Report on X-Ray Photoabsorption Coefficients and Atomic Scattering Factors for 92 Elements in the 10-10,000 eV Region

    E-Print Network [OSTI]

    Henke, B.L.; Davis, J.C.; Gullikson, E.M.; Perera, R.C.C.

    1988-01-01

    Ref. Atomic Scattering Factors, f 1 +if 2 71 - Lutetium (Lu ) Lutetium ( Lu ) - 71 Atomic Weight = 174.97 (barns/

  8. Connectivity of the Hexagonal, Cubic, and Isotropic Phases of the C$_{12}$EO$_6$/H$_2$O Lyotropic Mixture Investigated by Tracer Diffusion and X-ray Scattering

    E-Print Network [OSTI]

    Doru Constantin; Patrick Oswald; Marianne Impéror-Clerc; Patrick Davidson; Paul Sotta

    2015-04-09

    The connectivity of the hydrophobic medium in the nonionic binary system C$_{12}$EO$_6$/H$_2$O is studied by monitoring the diffusion constants of tracer molecules at the transition between the hexagonal mesophase and the fluid isotropic phase. The increase in the transverse diffusion coefficient on approaching the isotropic phase reveals the proliferation of bridgelike defects connecting the surfactant cylinders. This suggests that the isotropic phase has a highly connected structure. Indeed, we find similar diffusion coefficients in the isotropic and cubic bicontinuous phases. The temperature dependence of the lattice parameter in the hexagonal phase confirms the change in connectivity close to the hexagonal-isotropic transition. Finally, an X-ray investigation of the isotropic phase shows that its structure is locally similar to that of the hexagonal phase.

  9. Diffractive deep inelastic scattering in an AdS/CFT inspired model: A phenomenological study

    E-Print Network [OSTI]

    M. A. Betemps; V. P. Goncalves; J. T. de Santana Amaral

    2010-04-29

    The analytical treatment of the nonperturbative QCD dynamics is one of main open questions of the strong interactions. Currently, it is only possible to get some qualitative information about this regime considering other QCD-like theories, as for example the N=4 super Yang-Mills (SYM), where one can perform calculations in the nonperturbative limit of large 't Hooft coupling using the Anti-de Sitter space/Conformal field theory (AdS/CFT). Recently, the high energy scattering amplitude was calculated in the AdS/CFT approach, applied to deep inelastic scattering (DIS) and confronted with the $F_2$ HERA data. In this work we extend the nonperturbative AdS/CFT inspired model for diffractive processes and compare its predictions with a perturbative approach based on the Balitsky - Kovchegov (BK) equation. We demonstrate that the AdS/CFT inspired model is not able to describe the current $F_2^{D(3)}$ HERA data and predicts a similar behavior to that from BK equation in the range $10^{-7} \\lesssim x_{IP} \\lesssim 10^{-4}$. At smaller values of $x_{IP}$ the diffractive structure function is predicted to be energy independent.

  10. Ray tracing flux calculation for the small and wide angle x-ray...

    Office of Scientific and Technical Information (OSTI)

    station at the SESAME synchrotron radiation facility The calculation for the optics of the synchrotron radiation small and wide angle x-ray scattering beamline, currently...

  11. Neutron and X-ray experiments at high temperature P. Aldebert (*)

    E-Print Network [OSTI]

    Boyer, Edmond

    neutron scattering have appeared as power- ful tools to get information, mainly structural temperature scattering devices compared to X-rays. At the present time thermal neutron high flux reactors be investigated by neutron scattering.

  12. Changes in delta-Plutonium due to self-irradiation aging observed by Continuous in-situ X-ray Scattering

    SciTech Connect (OSTI)

    Saw, C K; Chung, B W; Wall, M A

    2007-01-05

    The aging in plutonium is predominantly caused by its internal self-irradiation. The self-irradiation in Pu-239 is by the decay process of transmuting the Pu atom into uranium atom and emitting an {alpha}-particle. Most of the lattice damage comes from the uranium recoil resulting in Frenkel-type defects consisting of vacancies and self-interstitial atoms, helium in-growth and defect clusters and possibly even though it is not yet observed, the generation of voids. As part of the stockpile stewardship, it is important to understand the changes in the structure and microstructures and their correlations to the physical properties. Changes in the physical properties have a direct relationship to the quality of the structure, in terms of formation of defects and defect clustering, accumulation of voids, grain boundaries, phase changes and etc. which can adversely affect the stability of the material. These changes are very difficult to monitor because of the high activity of the sample, high atomic number making x-ray and synchrotron probe into the bulk very difficult (neutron probe is not feasible) and the long life time which normally requires decades to measure. In this paper we describe the development of an in-situ in-house transmission x-ray diffraction (XRD) experimental technique used to monitor the structural changes in these materials. This technique calls for a very thin sample of less that 2 mm and to accelerate the aging process due to self-irradiation, spiked alloy of 7.5 weight percent of Pu-238 is used. This is equivalent to roughly 17 times the normal rate of aging. Current results suggest that over a period of 2.8 equivalent years, an increase of 0.5% in unit cell parameter is observed. The increase appears to be an abrupt jump at about 1.1 equivalent years, brought about by the collapsing of the atoms from the interstitials to the lattice sites. Further data analysis is on the way.

  13. Pressure induced valence change of Eu in EuFe2As2 at low temperature and high pressures probed by resonant inelastic x-ray scattering

    E-Print Network [OSTI]

    Svane, Axel Torstein

    and Astronomy, Aarhus University, DK-8000 Aarhus C, Denmark 4 Advanced Centre of Research in High Energy Pradesh, India 6 HPCAT, Geophysical Laboratory, Carnegie Institution of Washington, Advanced Photon Source:Fe:As:Sn in the ratio 1:2:2:19. The Sn was removed by centrifugal method. The grown crystals were characterized

  14. Studies of structure and dynamics of biological macro-molecular assemblies by low angle neutron diffraction and inelastic X-ray scattering

    E-Print Network [OSTI]

    Liu, Yun, 1973-

    2005-01-01

    This thesis is organized into two parts which focus on the studies of the dynamic structure factor and static inter-particle structure factor respectively. In the first part, we have measured and analyzed the dynamic ...

  15. X-ray shearing interferometer

    DOE Patents [OSTI]

    Koch, Jeffrey A. (Livermore, CA)

    2003-07-08

    An x-ray interferometer for analyzing high density plasmas and optically opaque materials includes a point-like x-ray source for providing a broadband x-ray source. The x-rays are directed through a target material and then are reflected by a high-quality ellipsoidally-bent imaging crystal to a diffraction grating disposed at 1.times. magnification. A spherically-bent imaging crystal is employed when the x-rays that are incident on the crystal surface are normal to that surface. The diffraction grating produces multiple beams which interfere with one another to produce an interference pattern which contains information about the target. A detector is disposed at the position of the image of the target produced by the interfering beams.

  16. Structural characterization of Green River oil-shale at high-pressure using pair distribution function analysis and small angle x-ray scattering.

    SciTech Connect (OSTI)

    Locke, D. R.; Chupas, P. J.; Chapman, K. W.; Pugmire, R. J.; Winans, R. E.; Univ. of Utah

    2008-01-01

    The compression behavior of a silicate-rich oil shale from the Green River formation in the pressure range 0.0-2.4 GPa was studied using in situ high pressure X-ray pair distribution function (PDF) measurements for the sample contained within a Paris-Edinburgh cell. The real-space local structural information in the PDF, G(r), was used to evaluate the compressibility of the oil shale. Specifically, the pressure-induced reduction in the medium- to long-range atom distances (6-20 {angstrom}) yielded an average sample compressibility corresponding to a bulk modulus of ca. 61-67 GPa. A structural model consisting of a three phase mixture of the principal crystalline oil shale components (quartz, albite and Illite) provided a good fit to the ambient pressure PDF data (R 30.7%). Indeed the features in the PDF beyond 6 {angstrom}, were similarly well fit by a single phase model of the highest symmetry, highly crystalline quartz component.

  17. Johann Spectrometer for High Resolution X-ray Spectroscopy

    SciTech Connect (OSTI)

    Machek, Pavel; Froeba, Michael; Welter, Edmund; Caliebe, Wolfgang; Brueggmann, Ulf; Draeger, Guenter

    2007-01-19

    A newly designed vacuum Johann spectrometer with a large focusing analyzer crystal for inelastic x-ray scattering and high resolution fluorescence spectroscopy has been installed at the DORIS III storage ring. Spherically bent crystals with a maximum diameter of 125 mm, and cylindrically bent crystals are employed as dispersive optical elements. Standard radius of curvature of the crystals is 1000 mm, however, the design of the mechanical components also facilitates measurements with smaller and larger bending radii. Up to four crystals are mounted on a revolving crystal changer which enables crystal changes without breaking the vacuum. The spectrometer works at fixed Bragg angle. It is preferably designed for the measurements in non-scanning mode with a broad beam spot, and offers a large flexibility to set the sample to the optimum position inside the Rowland circle. A deep depletion CCD camera is employed as a position sensitive detector to collect the energy-analyzed photons on the circumference of the Rowland circle. The vacuum in the spectrometer tank is typically 10-6 mbar. The sample chamber is separated from the tank either by 25 {mu}m thick Kapton windows, which allows samples to be measured under ambient conditions, or by two gate valves. The spectrometer is currently installed at wiggler beamline W1 whose working range is 4-10.5 keV with typical flux at the sample of 5x1010photons/s/mm2. The capabilities of the spectrometer are illustrated by resonant inelastic experiments on 3d transition metals and rare earth compounds, and by chemical shift measurements on chromium compounds.

  18. Elastic and inelastic scattering of 240-MeV (6)Li ions from (40)Ca and (48)Ca and tests of a systematic optical potential 

    E-Print Network [OSTI]

    Chen, Krishichayan X.; Lui, Y. -W; Button, J.; Youngblood, David H.

    2010-01-01

    Elastic and inelastic scattering of 240-MeV (6)Li particles from (40)Ca and (48)Ca were measured with the multipole-dipole-multipole spectrometer from 4 degrees <= theta(c.m.) <= 40 degrees. Optical potential parameters ...

  19. Single spin asymmetries in charged kaon production from semi-inclusive deep inelastic scattering on a transversely polarized [superscript 3]He target

    E-Print Network [OSTI]

    Zhao, Y. X.

    We report the first measurement of target single spin asymmetries of charged kaons produced in semi-inclusive deep inelastic scattering of electrons off a transversely polarized [superscript 3]He target. Both the Collins ...

  20. Measurement of “pretzelosity” asymmetry of charged pion production in semi-inclusive deep inelastic scattering on a polarized ³He target

    SciTech Connect (OSTI)

    Zhang, Y.; Qian, X.; Allada, K.; Dutta, C.

    2014-11-01

    An experiment to measure single-spin asymmetries in semi-inclusive production of charged pions in deep-inelastic scattering on a transversely polarized ³He target was performed at Jefferson Lab in the kinematic region of 0.16 < x < 0.35 and 1.4 < Q² < 2.7 GeV². Our results show that both ?± on He3 and on neutron pretzelosity asymmetries are consistent with zero within experimental uncertainties.

  1. Discrimination of gamma rays due to inelastic neutron scattering in AGATA

    E-Print Network [OSTI]

    A. Ataç; A. Ka?ka?; S. Akkoyun; M. ?enyi?it; T. Hüyük; S. O. Kara; J. Nyberg

    2009-06-10

    Possibilities of discriminating neutrons and gamma rays in the AGATA gamma-ray tracking spectrometer have been investigated with the aim of reducing the background due to inelastic scattering of neutrons in the high-purity germanium crystals. This background may become a serious problem especially in experiments with neutron-rich radioactive ion beams. Simulations using the Geant4 toolkit and a tracking program based on the forward tracking algorithm were carried out by emitting neutrons and gamma rays from the center of AGATA. Three different methods were developed and tested in order to find 'fingerprints' of the neutron interaction points in the detectors. In a simulation with simultaneous emission of six neutrons with energies in the range 1-5 MeV and ten gamma rays with energies between 150 and 1450 keV, the peak-to-background ratio at a gamma-ray energy of 1.0 MeV was improved by a factor of 2.4 after neutron rejection with a reduction of the photopeak efficiency at 1.0 MeV of only a factor of 1.25.

  2. Structure of water in mesoporous organosilica by calorimetry and inelastic neutron scattering

    SciTech Connect (OSTI)

    Levy, Esthy [Institute of Nanotechnology Bar-Ilan University, Ramat-Gan, Israel; Kolesnikov, Alexander I [ORNL; Li, Jichen [University of Manchester, UK; Mastai, Yitzhak [Institute of Nanotechnology Bar-Ilan University, Ramat-Gan, Israel

    2009-01-01

    In this paper, we describe the preparation of mesoporous organosilica samples with hydrophilic or hydrophobic organic functionality inside the silica channel. We synthesized mesoporous organosilica of identical pore sizes based on two different organic surface functionality namely hydrophobic (based on octyltriethoxysilane OTES) and hydrophilic (3-aminopropyltriethoxysilane ATES) and MCM-41 was used as a reference system. The structure of water/ice in those porous silica samples have been investigated over a range temperatures by differential scanning calorimetry (DSC) and inelastic neutron scattering (INS). INS study revealed that water confined in hydrophobic mesoporous organosilica shows vibrational behavior strongly different than bulk water. It consists of two states: water with strong and weak hydrogen bonds (with ratio 1:2.65, respectively), compared to ice-Ih. The corresponding O-O distances in these water states are 2.67 and 2.87 ?, which strongly differ compared to ice-Ih (2.76 ?). INS spectra for water in hydrophilic mesoporous organosilica ATES show behavior similar to bulk water, but with greater degree of disorder.

  3. CT14QED PDFs from Isolated Photon Production in Deep Inelastic Scattering

    E-Print Network [OSTI]

    Schmidt, Carl; Stump, Daniel; Yuan, C -P

    2015-01-01

    We describe the implementation of Quantum Electrodynamic (QED) evolution at Leading Order (LO) along with Quantum Chromodynamic (QCD) evolution at Next-to-Leading Order (NLO) in the CTEQ-TEA Global analysis package. The photon Parton Distribution Function (PDF) is described by a two-parameter ansatz, coming from radiation off the valence quarks, and based on the CT14 NLO PDFs. Setting the two parameters equal, allows us to completely specify the photon PDF in terms of the momentum fraction carried by the photon, $p_0^\\gamma$, at the initial scale $Q_0=1.295$ GeV. We obtain constraints on the photon PDF by comparing with ZEUS data~\\cite{Chekanov:2009dq} on the production of isolated photons in deep inelastic scattering, $ep\\rightarrow e\\gamma+X$. For this comparison we present a new perturbative calculation of the process that consistently combines the photon-initiated contribution with the quark-initiated contribution. Comparison with the data allows us to put a constraint at the 90% confidence level of $p_0^...

  4. CT14QED PDFs from Isolated Photon Production in Deep Inelastic Scattering

    E-Print Network [OSTI]

    Carl Schmidt; Jon Pumplin; Daniel Stump; C. -P. Yuan

    2015-09-09

    We describe the implementation of Quantum Electrodynamic (QED) evolution at Leading Order (LO) along with Quantum Chromodynamic (QCD) evolution at Next-to-Leading Order (NLO) in the CTEQ-TEA Global analysis package. The photon Parton Distribution Function (PDF) is described by a two-parameter ansatz, coming from radiation off the valence quarks, and based on the CT14 NLO PDFs. Setting the two parameters equal, allows us to completely specify the photon PDF in terms of the momentum fraction carried by the photon, $p_0^\\gamma$, at the initial scale $Q_0=1.295$ GeV. We obtain constraints on the photon PDF by comparing with ZEUS data~\\cite{Chekanov:2009dq} on the production of isolated photons in deep inelastic scattering, $ep\\rightarrow e\\gamma+X$. For this comparison we present a new perturbative calculation of the process that consistently combines the photon-initiated contribution with the quark-initiated contribution. Comparison with the data allows us to put a constraint at the 90% confidence level of $p_0^\\gamma\\lesssim0.14\\%$ for the photon PDF at the initial scale of $Q_0=1.295$ GeV in the one-parameter radiative ansatz. The resulting CT14QED PDFs will be made available to the public.

  5. Method and apparatus for molecular imaging using X-rays at resonance wavelengths

    DOE Patents [OSTI]

    Chapline, Jr., George F. (Alamo, CA)

    1985-01-01

    Holographic X-ray images are produced representing the molecular structure of a microscopic object, such as a living cell, by directing a beam of coherent X-rays upon the object to produce scattering of the X-rays by the object, producing interference on a recording medium between the scattered X-rays from the object and unscattered coherent X-rays and thereby producing holograms on the recording surface, and establishing the wavelength of the coherent X-rays to correspond with a molecular resonance of a constituent of such object and thereby greatly improving the contrast, sensitivity and resolution of the holograms as representations of molecular structures involving such constituent. For example, the coherent X-rays may be adjusted to the molecular resonant absorption line of nitrogen at about 401.3 eV to produce holographic images featuring molecular structures involving nitrogen.

  6. Coulomb-Excitation of the Giant-Dipole Resonance in Light-Ion Inelastic-Scattering from Pb-208 

    E-Print Network [OSTI]

    Izumoto, T.; Lui, YW; Youngblood, David H.; Udagawa, T.; Tamura, T.

    1981-01-01

    VOLUME 24, NUMBER 5 NOVEMBER 1981 Coulomb excitation of the giant dipole resonance in light-ion inelastic scattering from Pb T. Izumoto, Y. -%. Lui, and D. H. Youngblood Cyclotron Institute, Texas A&M University, College Station, Texas 77843 T... the contribution from Coulomb excitation of 24 2179 , 1981 The American Physical Society 2180 IZUMOTO, LUI, YOUNGSLOOD, UDAGAW'A, AND TAMUWk 24 the GDR in the region of the GMR in Pb in (a,a') scattering with incident energies between 96 and 218 MeV. There is a...

  7. X-ray fluorescence mapping

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power AdministrationRobust,Field-effectWorkingLos Alamos verifies largest single goldWindX-RayX-Ray ScienceX-Ray

  8. VOLUME 86, NUMBER 21 P H Y S I C A L R E V I E W L E T T E R S 21 MAY 2001 Time Resolved Collapse of a Folding Protein Observed with Small Angle X-Ray Scattering

    E-Print Network [OSTI]

    Gruner, Sol M.

    of a Folding Protein Observed with Small Angle X-Ray Scattering L. Pollack,1, * M. W. Tate,1 A. C. Finnefrock,1 in conjunction with microfabricated rapid-fluid mixing devices to monitor the early events in protein folding scale. The role of chain collapse, one of the initial stages of protein folding, is not currently

  9. Miniature x-ray source

    DOE Patents [OSTI]

    Trebes, James E. (Livermore, CA); Bell, Perry M. (Tracy, CA); Robinson, Ronald B. (Modesto, CA)

    2000-01-01

    A miniature x-ray source utilizing a hot filament cathode. The source has a millimeter scale size and is capable of producing broad spectrum x-ray emission over a wide range of x-ray energies. The miniature source consists of a compact vacuum tube assembly containing the hot filament cathode, an anode, a high voltage feedthru for delivering high voltage to the cathode, a getter for maintaining high vacuum, a connector for initial vacuum pump down and crimp-off, and a high voltage connection for attaching a compact high voltage cable to the high voltage feedthru. At least a portion of the vacuum tube wall is fabricated from highly x-ray transparent materials, such as sapphire, diamond, or boron nitride.

  10. Structure of low-density nanoporous dielectrics revealed by low-vacuum electron microscopy and small-angle x-ray scattering

    SciTech Connect (OSTI)

    Kucheyev, S O; Toth, M; Baumann, T F; Hamza, A V; Ilavsky, J; Knowles, W R; Thiel, B L; Tileli, V; van Buuren, T; Wang, Y M; Willey, T M

    2006-06-05

    We use low-vacuum scanning electron microscopy to image directly the ligament and pore size and shape distributions of representative aerogels over a wide range of length scales ({approx} 10{sup 0}-10{sup 5} nm). The images are used for unambiguous, real-space interpretation of small-angle scattering data for these complex nanoporous systems.

  11. SMB, X-ray Absorption Spectroscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power AdministrationRobust, High-Throughput Analysis of Protein1-0845*RV 14800Small Angle X-Ray Scattering Home

  12. SMB, X-ray Emission Spectroscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power AdministrationRobust, High-Throughput Analysis of Protein1-0845*RV 14800Small Angle X-Ray Scattering

  13. Inelastic Neutron-Scattering Measurements of a Three-Dimensional Spin Resonance in the FeAs-Based BaFe1:9Ni0:1As2 Superconductor

    E-Print Network [OSTI]

    Hu, Jiangping

    Inelastic Neutron-Scattering Measurements of a Three-Dimensional Spin Resonance in the Fe, Purdue University, West Lafayette, Indiana 47907, USA 5 Neutron Scattering Science Division, Oak Ridge 2009) We use inelastic neutron scattering to study magnetic excitations of the Fe

  14. Large-angle elastic and inelastic scattering of Pi(+) and Pi(-) from (28)Si and (40)Ca. Master's thesis

    SciTech Connect (OSTI)

    Snell, M.P.

    1989-05-01

    Differential cross sections were measured for Pi(+) and Pi(-) elastic scattering of Calcium 40 and Silicon 28 at incident pion energies ranging from 100 to 260 MeV at a scattering angle of 175 degs. Differential cross sections were also measured for Pi(+) and Pi(-) inelastic scattering to the 2(+), 1.78 MeV, 4(+), 4.62 MeV, and 3(-) 6.88 MeV states of 28Si at incident pion energies of 130, 180, and 226 MeV and scattering angles between 115 and 175{degrees} in 6{degrees} increments. The data are compared to previously obtained forward angle data through 120{degrees} and agree quite well. The data show a generally flat angular dependence for angles greater than 100{degrees}. Several theoretical codes are reviewed for their ability to predict large angle scattering. Coordinate-space and momentum-space models generally thought to be sufficient for predicting forward angle scattering have proved to be inappropriate for use at large angles. A new phenomenological delta-hole model, currently under modification, shows a greatly enhanced ability to predict scattering at back angles.

  15. Status report on the analysis of inelastic neutron scattering from carbon, iron, yttrium and lead at 96 MeV

    E-Print Network [OSTI]

    C. Gustavsson; C. Hellesen; S. Pomp; A. Öhrn; J. Blomgren; U. Tippawan

    2013-03-27

    This work is part of an effort to provide more experimental data for the (n,n'x) reaction. The experiments were carried out at The Svedberg Laboratory in Uppsala, Sweden, at the quasi-mono-energetic neutron beam of 96 MeV, before the facility was upgraded in 2004. Using an extended data analysis of data primarily intended for measuring elastic neutron scattering only, it was found to be possible to extract information on the inelastic scattering from several nuclei. In the preliminary data analysis, an iterative forward-folding technique was applied, in which a physically reasonable trial spectrum was folded with the response function of the detector system and the output was compared to the experimental data. As a result, double-differential cross sections and angular distributions of inelastic neutron scattering from 12-C, 56-Fe, 89-Y and 208-Pb could be obtained. In this paper, a status update on the efforts to improve the description of the detector response function is given.

  16. Single transverse-spin asymmetry for $D$-meson production in semi-inclusive deep inelastic scattering

    E-Print Network [OSTI]

    Kang, Zhong-Bo

    2008-01-01

    We study the single-transverse spin asymmetry for open charm production in the semi-inclusive lepton-hadron deep inelastic scattering. We calculate the asymmetry in terms of the QCD collinear factorization approach for $D$ mesons at high enough $P_{h\\perp}$, and find that the asymmetry is proportional to the twist-three tri-gluon correlation function in the proton. With a simple model for the tri-gluon correlation function, we estimate the asymmetry for both COMPASS and eRHIC kinematics, and discuss the possibilities of extracting the tri-gluon correlation function in these experiments.

  17. Single transverse-spin asymmetry for $D$-meson production in semi-inclusive deep inelastic scattering

    E-Print Network [OSTI]

    Zhong-Bo Kang; Jian-Wei Qiu

    2008-06-12

    We study the single-transverse spin asymmetry for open charm production in the semi-inclusive lepton-hadron deep inelastic scattering. We calculate the asymmetry in terms of the QCD collinear factorization approach for $D$ mesons at high enough $P_{h\\perp}$, and find that the asymmetry is proportional to the twist-three tri-gluon correlation function in the proton. With a simple model for the tri-gluon correlation function, we estimate the asymmetry for both COMPASS and eRHIC kinematics, and discuss the possibilities of extracting the tri-gluon correlation function in these experiments.

  18. Measurement of cross sections for inelastic cold-neutron scattering in metals and polymers by the method of (n, {gamma}) analysis

    SciTech Connect (OSTI)

    Arzumanov, S. S.; Bondarenko, L. N.; Geltenbort, P.; Morozov, V. I.; Panin, Yu. N.; Chernyavsky, S. M.

    2008-11-15

    The results obtained by measuring the cross sections for the inelastic scattering of very cold neutrons for a number of metals and polymers by the method of a neutron-irradiation analysis are presented. The method is based on simultaneously measuring events of inelastic scattering and neutron capture in the sample under investigation via recording gamma radiation with a semiconductor germanium detector. Neutron capture by a nucleus of the sample is accompanied by the prompt radiation of gamma rays having a known spectrum. Upon inelastic scattering, a neutron acquires thermal energy. Upon leaving the sample, this neutron is absorbed in a special converter that contains the isotope {sup 10}B. The capture of the neutron by a {sup 10}B nucleus is followed by the emission of a 477-keV gamma ray. The probabilities of capture and inelastic scattering are proportional to the respective neutron-interaction cross sections, and the ratio of the recorded detector counts corresponding to events of the two types does not depend on the spectrum of the incident flux of very cold neutrons or on the trajectory of neutron motion in the sample. The sought inelastic-scattering cross section at a fixed sample temperature is calculated by using this ratio and the known cross section for neutron capture by the sample isotope having a known gamma-radiation spectrum.

  19. Combined Use of Residual Dipolar Couplings and Solution X-ray Scattering To Rapidly Probe Rigid-Body Conformational Transitions in a Non-phosphorylatable Active-Site Mutant of the 128 kDa Enzyme I Dimer

    SciTech Connect (OSTI)

    Takayama, Yuki; Schwieters, Charles D.; Grishaev, Alexander; Ghirlando, Rodolfo; Clore, G. Marius (NIH)

    2012-10-23

    The first component of the bacterial phosphotransferase system, enzyme I (EI), is a multidomain 128 kDa dimer that undergoes large rigid-body conformational transitions during the course of its catalytic cycle. Here we investigate the solution structure of a non-phosphorylatable active-site mutant in which the active-site histidine is substituted by glutamine. We show that perturbations in the relative orientations and positions of the domains and subdomains can be rapidly and reliably determined by conjoined rigid-body/torsion angle/Cartesian simulated annealing calculations driven by orientational restraints from residual dipolar couplings and shape and translation information afforded by small- and wide-angle X-ray scattering. Although histidine and glutamine are isosteric, the conformational space available to a Gln side chain is larger than that for the imidazole ring of His. An additional hydrogen bond between the side chain of Gln189 located on the EIN{sup {alpha}/{beta}} subdomain and an aspartate (Asp129) on the EIN{sup {alpha}} subdomain results in a small ({approx}9{sup o}) reorientation of the EIN{sup {alpha}} and EIN{sup {alpha}/{beta}} subdomains that is in turn propagated to a larger reorientation ({approx}26{sup o}) of the EIN domain relative to the EIC dimerization domain, illustrating the positional sensitivity of the EIN domain and its constituent subdomains to small structural perturbations.

  20. Structural dynamics and ssDNA binding activity of the three N-terminal domains of the large subunit of Replication Protein A from small angle X-ray scattering

    SciTech Connect (OSTI)

    Pretto, Dalyir I.; Tsutakawa, Susan; Brosey, Chris A.; Castillo, Amalchi; Chagot, Marie-Eve; Smith, Jarrod A.; Tainer, John A.; Chazin, Walter J.

    2010-03-11

    Replication Protein A (RPA) is the primary eukaryotic ssDNA binding protein utilized in diverse DNA transactions in the cell. RPA is a heterotrimeric protein with seven globular domains connected by flexible linkers, which enable substantial inter-domain motion that is essential to its function. Small angle X-ray scattering (SAXS) experiments on two multi-domain constructs from the N-terminus of the large subunit (RPA70) were used to examine the structural dynamics of these domains and their response to the binding of ssDNA. The SAXS data combined with molecular dynamics simulations reveal substantial interdomain flexibility for both RPA70AB (the tandem high affinity ssDNA binding domains A and B connected by a 10-residue linker) and RPA70NAB (RPA70AB extended by a 70-residue linker to the RPA70N protein interaction domain). Binding of ssDNA to RPA70NAB reduces the interdomain flexibility between the A and B domains, but has no effect on RPA70N. These studies provide the first direct measurements of changes in orientation of these three RPA domains upon binding ssDNA. The results support a model in which RPA70N remains structurally independent of RPA70AB in the DNA bound state and therefore freely available to serve as a protein recruitment module.

  1. Evaluation of partial coherence correction in X-ray ptychography

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Burdet, Nicolas; Shi, Xiaowen; Parks, Daniel; Clark, Jesse N.; Huang, Xiaojing; Kevan, Stephen D.; Robinson, Ian K.

    2015-02-23

    Coherent X-ray Diffraction Imaging (CDI) and X-ray ptychography both heavily rely on the high degree of spatial coherence of the X-ray illumination for sufficient experimental data quality for reconstruction convergence. Nevertheless, the majority of the available synchrotron undulator sources have a limited degree of partial coherence, leading to reduced data quality and a lower speckle contrast in the coherent diffraction patterns. It is still an open question whether experimentalists should compromise the coherence properties of an X-ray source in exchange for a higher flux density at a sample, especially when some materials of scientific interest are relatively weak scatterers. Amore »previous study has suggested that in CDI, the best strategy for the study of strong phase objects is to maintain a high degree of coherence of the illuminating X-rays because of the broadening of solution space resulting from the strong phase structures. In this article, we demonstrate the first systematic analysis of the effectiveness of partial coherence correction in ptychography as a function of the coherence properties, degree of complexity of illumination (degree of phase diversity of the probe) and sample phase complexity. We have also performed analysis of how well ptychographic algorithms refine X-ray probe and complex coherence functions when those variables are unknown at the start of reconstructions, for noise-free simulated data, in the case of both real-valued and highly-complex objects.« less

  2. Compact x-ray source and panel

    DOE Patents [OSTI]

    Sampayon, Stephen E. (Manteca, CA)

    2008-02-12

    A compact, self-contained x-ray source, and a compact x-ray source panel having a plurality of such x-ray sources arranged in a preferably broad-area pixelized array. Each x-ray source includes an electron source for producing an electron beam, an x-ray conversion target, and a multilayer insulator separating the electron source and the x-ray conversion target from each other. The multi-layer insulator preferably has a cylindrical configuration with a plurality of alternating insulator and conductor layers surrounding an acceleration channel leading from the electron source to the x-ray conversion target. A power source is connected to each x-ray source of the array to produce an accelerating gradient between the electron source and x-ray conversion target in any one or more of the x-ray sources independent of other x-ray sources in the array, so as to accelerate an electron beam towards the x-ray conversion target. The multilayer insulator enables relatively short separation distances between the electron source and the x-ray conversion target so that a thin panel is possible for compactness. This is due to the ability of the plurality of alternating insulator and conductor layers of the multilayer insulators to resist surface flashover when sufficiently high acceleration energies necessary for x-ray generation are supplied by the power source to the x-ray sources.

  3. Solution Structure of the 128 kDa Enzyme I Dimer from Escherichia coli and Its 146 kDa Complex with HPr Using Residual Dipolar Couplings and Small- and Wide-Angle X-ray Scattering

    SciTech Connect (OSTI)

    Schwieters, Charles D.; Suh, Jeong-Yong; Grishaev, Alexander; Ghirlando, Rodolfo; Takayama, Yuki; Clore, G. Marius (NIH)

    2010-09-17

    The solution structures of free Enzyme I (EI, {approx}128 kDa, 575 x 2 residues), the first enzyme in the bacterial phosphotransferase system, and its complex with HPr ({approx}146 kDa) have been solved using novel methodology that makes use of prior structural knowledge (namely, the structures of the dimeric EIC domain and the isolated EIN domain both free and complexed to HPr), combined with residual dipolar coupling (RDC), small- (SAXS) and wide- (WAXS) angle X-ray scattering and small-angle neutron scattering (SANS) data. The calculational strategy employs conjoined rigid body/torsion/Cartesian simulated annealing, and incorporates improvements in calculating and refining against SAXS/WAXS data that take into account complex molecular shapes in the description of the solvent layer resulting in a better representation of the SAXS/WAXS data. The RDC data orient the symmetrically related EIN domains relative to the C{sub 2} symmetry axis of the EIC dimer, while translational, shape, and size information is provided by SAXS/WAXS. The resulting structures are independently validated by SANS. Comparison of the structures of the free EI and the EI-HPr complex with that of the crystal structure of a trapped phosphorylated EI intermediate reveals large ({approx}70-90{sup o}) hinge body rotations of the two subdomains comprising the EIN domain, as well as of the EIN domain relative to the dimeric EIC domain. These large-scale interdomain motions shed light on the structural transitions that accompany the catalytic cycle of EI.

  4. Focused X-ray source

    DOE Patents [OSTI]

    Piestrup, Melvin A. (Woodside, CA); Boyers, David G. (Mountain View, CA); Pincus, Cary I. (Sunnyvale, CA); Maccagno, Pierre (Stanford, CA)

    1990-01-01

    An intense, relatively inexpensive X-ray source (as compared to a synchrotron emitter) for technological, scientific, and spectroscopic purposes. A conical radiation pattern produced by a single foil or stack of foils is focused by optics to increase the intensity of the radiation at a distance from the conical radiator.

  5. Soft X-ray microflares

    E-Print Network [OSTI]

    Mirzoeva, I K

    2015-01-01

    Soft X-ray solar bursts are studied. Weak bursts with powers up to 10-8 W/m2 were detected. All the events were confirmed by GOES observations. Parameters of these microflares are determined. A physical mechanism for the low-intensity solar events is discussed.

  6. Focused X-ray source

    DOE Patents [OSTI]

    Piestrup, M.A.; Boyers, D.G.; Pincus, C.I.; Maccagno, P.

    1990-08-21

    Disclosed is an intense, relatively inexpensive X-ray source (as compared to a synchrotron emitter) for technological, scientific, and spectroscopic purposes. A conical radiation pattern produced by a single foil or stack of foils is focused by optics to increase the intensity of the radiation at a distance from the conical radiator. 8 figs.

  7. A scaler-based data acquisition system for measuring parity-violating asymmetry in deep inelastic scattering

    SciTech Connect (OSTI)

    Subedi, Ramesh R.; Wang, Diancheng; Pan, Kai; Deng, Xiaoyan; Michaels, Robert W.; Shahinyan, Albert; Wojtsekhowski, Bogdan B.; Zheng, Xiaochao

    2013-10-01

    An experiment that measured the parity violating asymmetries in deep inelastic scattering was completed at the Thomas Jefferson National Accelerator Facility in experimental Hall A. From these asymmetries, a combination of the quark weak axial charge could be extracted with a factor of five improvement in precision over world data. To achieve this, asymmetries at the 10^-4 level needed to be measured at event rates up to 500 kHz and the high pion background typical to deep inelastic scattering experiments needed to be rejected efficiently. A specialized data acquisition (DAQ) system with intrinsic particle identification (PID) was successfully developed and used: The pion contamination in the electron samples was controlled at the order of 2 × 10^-4 or below with an electron efficiency of higher than 91% throughout the production period of the experiment, the systematic uncertainty in the measured asymmetry due to DAQ deadtime was below 0.2%, and the statistical quality of the asymmetry measurement agreed with the Gaussian distribution to over five orders of magnitudes. The DAQ system is presented here with an emphasis on its design scheme, the achieved PID performance, deadtime effect and the capability of measuring small asymmetries.

  8. Measurement of the Parity-Violating Asymmetry in Deep Inelastic Scattering at JLab 6 GeV

    SciTech Connect (OSTI)

    Wang, Diancheng

    2013-12-01

    The parity-violating asymmetry in deep inelastic scattering (PVDIS) offers us a useful tool to study the weak neutral couplings and the hadronic structure of the nucleon, and provides high precision tests on the Standard Model. During the 6 GeV PVDIS experiment at the Thomas Jefferson National Accelerator Facility, the parity-violating asymmetries A{sub PV} of a polarized electron beam scattering off an unpolarized deuteron target in the deep inelastic scattering region were precisely measured at two Q{sup 2} values of 1.1 and 1.9 (GeV/c){sup 2}. The asymmetry at Q{sup 2}=1.9 (GeV/c){sup 2} can be used to extract the weak coupling combination 2C{sub 2u} - C{sub 2d}, assuming the higher twist effect is small. The extracted result from this measurement is in good agreement with the Standard Model prediction, and improves the precision by a factor of five over previous data. In addition, combining the asymmetries at both Q{sup 2} values provides us extra knowledge on the higher twist effects. The parity violation asymmetries in the resonance region were also measured during this experiment. These results are the first A{sub PV} data in the resonance region beyond the {Delta}#1;(1232). They provide evidence that the quark hadron duality works for A{sub PV} at the (10-15)% level, and set constraints on nucleon resonance models that are commonly used for background calculations to other parity-violating electron scattering measurements.

  9. X-ray characterization of solid small molecule organic materials

    SciTech Connect (OSTI)

    Billinge, Simon; Shankland, Kenneth; Shankland, Norman; Florence, Alastair

    2014-06-10

    The present invention provides, inter alia, methods of characterizing a small molecule organic material, e.g., a drug or a drug product. This method includes subjecting the solid small molecule organic material to x-ray total scattering analysis at a short wavelength, collecting data generated thereby, and mathematically transforming the data to provide a refined set of data.

  10. Pressure dependence of the exchange interaction in the dimeric single-molecule magnet [Mn{sub 4}O{sub 3}Cl{sub 4}(O{sub 2}CEt){sub 3}(py){sub 3}]{sub 2} from inelastic neutron scattering

    SciTech Connect (OSTI)

    Sieber, A.; Waldmann, O.; Ochsenbein, S. T.; Carver, G.; Guedel, H. U.; Foguet-Albiol, D.; Christou, G.; Mutka, H.; Fernandez-Alonso, F.; Mezouar, M.; Weber, H. P.

    2006-07-01

    The low-lying magnetic excitations in the dimers of single-molecule magnets [Mn{sub 4}O{sub 3}Cl{sub 4}(O{sub 2}CEt){sub 3}(py){sub 3}]{sub 2}, or (Mn{sub 4}){sub 2}, are studied by inelastic neutron scattering as a function of hydrostatic pressure. The anisotropy parameters D and B{sub 0}{sup 4}, which describe each Mn{sub 4} subunit, are essentially pressure independent, while the antiferromagnetic exchange coupling J between the two Mn{sub 4} subunits strongly depends on pressure, with an increase of 42% at 17 kbar. Additional pressure-dependent powder x-ray measurements allow a structural interpretation of the findings.

  11. Toward Control of Matter: Basic Energy Science Needs for a New Class of X-Ray Light Sources

    E-Print Network [OSTI]

    Arenholz, Elke

    2008-01-01

    technique such as neutron scattering. B. Key Types ofARPES and inelastic neutron scattering (INS), which measuresextensively via neutron scattering, the critical behavior of

  12. Time-resolved x-ray Raman spectroscopy of photoexcited polydiacetylene oligomer: A simulation study

    E-Print Network [OSTI]

    Mukamel, Shaul

    , Osaka Prefecture University, Sakai 599-8531, Japan Sergei Volkov Department of Chemistry, University of the x-ray Raman peaks on the scattering wave vector k and energy . The electronic excitation energies progress in generating ultrafast x-ray pulses and bringing them down to the attosecond regime has opened up

  13. Accuracy evaluation of a Compton X-ray spectrometer with bremsstrahlung X-rays generated by a 6 MeV electron bunch

    SciTech Connect (OSTI)

    Kojima, Sadaoki Arikawa, Yasunobu; Zhang, Zhe; Ikenouchi, Takahito; Morace, Alessio; Nagai, Takahiro; Abe, Yuki; Sakata, Shouhei; Inoue, Hiroaki; Utsugi, Masaru; Nakai, Mitsuo; Nishimura, Hiroaki; Shiraga, Hiroyuki; Fujioka, Shinsuke; Azechi, Hiroshi; Nishimura, Yasuhiko; Togawa, Hiromi; Ozaki, Tetsuo; Kato, Ryukou

    2014-11-15

    A Compton-scattering-based X-ray spectrometer is developed to obtain the energy distribution of fast electrons produced by intense laser and matter interactions. Bremsstrahlung X-rays generated by fast electrons in a material are used to measure fast electrons’ energy distribution in matter. In the Compton X-ray spectrometer, X-rays are converted into recoil electrons by Compton scattering in a converter made from fused silica glass, and a magnet-based electron energy analyzer is used to measure the energy distribution of the electrons that recoil in the direction of the incident X-rays. The spectrum of the incident X-rays is reconstructed from the energy distribution of the recoil electrons. The accuracy of this spectrometer is evaluated using a quasi-monoenergetic 6 MeV electron bunch that emanates from a linear accelerator. An electron bunch is injected into a 1.5 mm thick tungsten plate to produce bremsstrahlung X-rays. The spectrum of these bremsstrahlung X-rays is obtained in the range from 1 to 9 MeV. The energy of the electrons in the bunch is estimated using a Monte Carlo simulation of particle-matter interactions. The result shows that the spectrometer's energy accuracy is ±0.5 MeV for 6.0 MeV electrons.

  14. Serial femtosecond X-ray diffraction of enveloped virus microcrystals

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Lawrence, Robert M.; Conrad, Chelsie E.; Zatsepin, Nadia A.; Grant, Thomas D.; Liu, Haiguang; James, Daniel; Nelson, Garrett; Subramanian, Ganesh; Aquila, Andrew; Hunter, Mark S.; et al

    2015-08-20

    Serial femtosecond crystallography (SFX) using X-ray free-electron lasers has produced high-resolution, room temperature, time-resolved protein structures. We report preliminary SFX of Sindbis virus, an enveloped icosahedral RNA virus with ~700 Å diameter. Microcrystals delivered in viscous agarose medium diffracted to ~40 Å resolution. Small-angle diffuse X-ray scattering overlaid Bragg peaks and analysis suggests this results from molecular transforms of individual particles. Viral proteins undergo structural changes during entry and infection, which could, in principle, be studied with SFX. This is a pertinent step toward determining room temperature structures from virus microcrystals that may enable time-resolved studies of enveloped viruses.

  15. Distorted spin dependent spectral function of {sup 3}He and semi-inclusive deep inelastic scattering processes

    SciTech Connect (OSTI)

    Kaptari, Leonya P. [University of Perugia (Italy); INFN-Perugia (Italy); Thomas Jefferson National Accelerator Facility, Newport News, VA (United States); Joint Inst. for Nuclear Research, Dubna (Russia); Del Dotto, Alessio [University of Rome, Rome (Italy); INFN-Roma (Italy); Pace, Emanuele [University of Rome (Italy); INFN-Tor Vergata (Italy); Salme, Giovanni [INFN-Roma (Italy); Scopetta, Sergio [University of Perugia (Italy); INFN-Perugia (Italy)

    2014-03-01

    The spin dependent spectral function, relevant to describe polarized electron scattering off polarized {sup 3}He, is studied, within the Plane Wave Impulse Approximation and taking into account final state interaction effects (FSI). In particular, the case of semi-inclusive deep inelastic scattering (SiDIS) is considered, evaluating the FSI of the hadronizing quark with the nuclear remnants. It is shown that particular kinematical regions can be selected to minimize the latter effects, so that parton distributions in the neutron can be accessed. On the other side, in the regions where FSI dominates, the considered reactions can elucidate the mechanism of hadronization of quarks during the propagation in the nuclear medium. It is shown that the obtained spin dependent spectral function can be directly applied to investigate the SiDIS reaction e-vector + {sup 3}He-vector to h+X, where the hadron h originates from the current fragmentation. Experiments of this type are being performed at JLab to extract neutron transverse momentum dependent parton distributions. As a case study, a different SiDIS process, with detection of slow (A-1) systems in the final state, is considered in more details, in order to establish when nuclear structure effects and FSI can be distinguished from elementary reactions on quasi-free nucleons. It is argued that, by a proper choice of kinematics, the origin of nuclear effects in polarized DIS phenomena and the details of the interaction between the hadronizing quark and the nuclear medium can be investigated at a level which is not reachable in inclusive deep inelastic scattering.

  16. Producing X-rays at the APS

    ScienceCinema (OSTI)

    None

    2013-04-19

    An introduction and overview of the Advanced Photon Source at Argonne National Laboratory, the technology that produces the brightest X-ray beams in the Western Hemisphere, and the research carried out by scientists using those X-rays.

  17. Microgap x-ray detector

    DOE Patents [OSTI]

    Wuest, Craig R. (Danville, CA); Bionta, Richard M. (Livermore, CA); Ables, Elden (Livermore, CA)

    1994-01-01

    An x-ray detector which provides for the conversion of x-ray photons into photoelectrons and subsequent amplification of these photoelectrons through the generation of electron avalanches in a thin gas-filled region subject to a high electric potential. The detector comprises a cathode (photocathode) and an anode separated by the thin, gas-filled region. The cathode may comprise a substrate, such a beryllium, coated with a layer of high atomic number material, such as gold, while the anode can be a single conducting plane of material, such as gold, or a plane of resistive material, such as chromium/silicon monoxide, or multiple areas of conductive or resistive material, mounted on a substrate composed of glass, plastic or ceramic. The charge collected from each electron avalanche by the anode is passed through processing electronics to a point of use, such as an oscilloscope.

  18. Microgap x-ray detector

    DOE Patents [OSTI]

    Wuest, C.R.; Bionta, R.M.; Ables, E.

    1994-05-03

    An x-ray detector is disclosed which provides for the conversion of x-ray photons into photoelectrons and subsequent amplification of these photoelectrons through the generation of electron avalanches in a thin gas-filled region subject to a high electric potential. The detector comprises a cathode (photocathode) and an anode separated by the thin, gas-filled region. The cathode may comprise a substrate, such a beryllium, coated with a layer of high atomic number material, such as gold, while the anode can be a single conducting plane of material, such as gold, or a plane of resistive material, such as chromium/silicon monoxide, or multiple areas of conductive or resistive material, mounted on a substrate composed of glass, plastic or ceramic. The charge collected from each electron avalanche by the anode is passed through processing electronics to a point of use, such as an oscilloscope. 3 figures.

  19. Neutron and X-ray Scattering

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power Administration wouldMass map shinesSolar Photovoltaic(MillionNature andNeutrinos from

  20. Phase-sensitive X-ray imager

    DOE Patents [OSTI]

    Baker, Kevin Louis

    2013-01-08

    X-ray phase sensitive wave-front sensor techniques are detailed that are capable of measuring the entire two-dimensional x-ray electric field, both the amplitude and phase, with a single measurement. These Hartmann sensing and 2-D Shear interferometry wave-front sensors do not require a temporally coherent source and are therefore compatible with x-ray tubes and also with laser-produced or x-pinch x-ray sources.

  1. Lensless x-ray imaging in reflection geometry

    SciTech Connect (OSTI)

    Roy, S.; Parks, D.H.; Seu, K.A.; Turner, J.J.; Chao, W.; Anderson, E.H.; Cabrini, S.; Kevan, S.D.; Su, R.

    2011-02-03

    Lensless X-ray imaging techniques such as coherent diffraction imaging and ptychography, and Fourier transform holography can provide time-resolved, diffraction-limited images. Nearly all examples of these techniques have focused on transmission geometry, restricting the samples and reciprocal spaces that can be investigated. We report a lensless X-ray technique developed for imaging in Bragg and small-angle scattering geometries, which may also find application in transmission geometries. We demonstrate this by imaging a nanofabricated pseudorandom binary structure in small-angle reflection geometry. The technique can be used with extended objects, places no restriction on sample size, and requires no additional sample masking. The realization of X-ray lensless imaging in reflection geometry opens up the possibility of single-shot imaging of surfaces in thin films, buried interfaces in magnetic multilayers, organic photovoltaic and field-effect transistor devices, or Bragg planes in a single crystal.

  2. Inelastic scattering in a monolayer graphene sheet: A weak-localization study Dong-Keun Ki, Dongchan Jeong, Jae-Hyun Choi, and Hu-Jong Lee*

    E-Print Network [OSTI]

    Lee, Hu-Jong

    ,7 II. SAMPLE PREPARATION AND MEASUREMENTS A monolayer graphene sheet used in this study was meInelastic scattering in a monolayer graphene sheet: A weak-localization study Dong-Keun Ki in a graphene sheet, a single layer of graphite, exhibit distinct characteristics from those in other two

  3. Measurement of pretzelosity asymmetry of charged pion production in Semi-Inclusive Deep Inelastic Scattering on a polarized 3He target

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Zhang, Y; Qian, X; Allada, K; Dutta, C; Huang, J; Katich, J; Wang, Y; Aniol, K; Annand, J R.; Averett, T; et al

    2014-11-01

    An experiment to measure single-spin asymmetries in semi-inclusive production of charged pions in deep-inelastic scattering on a transversely polarized 3He target was performed at Jefferson Lab in the kinematic region of 0.16

  4. Measurement of “pretzelosity” asymmetry of charged pion production in semi-inclusive deep inelastic scattering on a polarized He3 target

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Zhang, Y.; Qian, X.; Allada, K.; Dutta, C.; Huang, J.; Katich, J.; Wang, Y.; Aniol, K.; Annand, J. R. M.; Averett, T.; et al

    2014-11-24

    An experiment to measure single-spin asymmetries in semi-inclusive production of charged pions in deep-inelastic scattering on a transversely polarized ³He target was performed at Jefferson Lab in the kinematic region of 0.16 ± on 3He and on neutron pretzelosity asymmetries are consistent with zero within experimental uncertainties.

  5. Single spin asymmetries in charged kaon production from semi-inclusive deep inelastic scattering on a transversely polarized 3He target

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Zhao, Y X; Wang, Y; Allada, K; Aniol, K; Annand, J R; Averett, T; Benmokhtar, F; Bertozzi, W; Bradshaw, P C; Bosted, P; et al

    2014-11-01

    We report the first measurement of target single spin asymmetries of charged kaons produced in semi-inclusive deep inelastic scattering of electrons off a transversely polarized 3He target. Both the Collins and Sivers moments, which are related to the nucleon transversity and Sivers distributions, respectively, are extracted over the kinematic range of 0.1

  6. Single spin asymmetries in charged kaon production from semi-inclusive deep inelastic scattering on a transversely polarized 3He target

    SciTech Connect (OSTI)

    Zhao, Y X; Wang, Y; Allada, K; Aniol, K; Annand, J R; Averett, T; Benmokhtar, F; Bertozzi, W; Bradshaw, P C; Bosted, P; Camsonne, A; Canan, M; Cates, G D; Chen, C; Chen, J -P; Chen, W; Chirapatpimol, K; Chudakov, E; Cisbani, E; Cornejo, J C; Cusanno, F; Dalton, M M; Deconinck, W; de Jager, C W; De Leo, R; Deng, X; Deur, A; Ding, H; Dolph, P A; Dutta, C; Dutta, D; El Fassi, L; Frullani, S; Gao, H; Garibaldi, F; Gaskell, D; Gilad, S; Gilman, R; Glamazdin, O; Golge, S; Guo, L; Hamilton, D; Hansen, O; Higinbotham, D W; Holmstrom, T; Huang, J; Huang, M; Ibrahim, H F; Iodice, M; Jiang, X; Jin, G; Jones, M K; Katich, J; Kelleher, A; Kim, W; Kolarkar, A; Korsch, W; LeRose, J J; Li, X; Li, Y; Lindgren, R; Liyanage, N; Long, E; Lu, H -J; Margaziotis, D J; Markowitz, P; Marrone, S; McNulty, D; Meziani, Z -E; Michaels, R; Moffit, B; Munoz Camacho, C; Nanda, S; Narayan, A; Nelyubin, V; Norum, B; Oh, Y; Osipenko, M; Parno, D; Peng, J -C; Phillips, S K; Posik, M; Puckett, A J; Qian, X; Qiang, Y; Rakhman, A; Ransome, R; Riordan, S; Saha, A; Sawatzky, B; Schulte, E; Shahinyan, A; Shabestari, M H; Sirca, S; Stepanyan, S; Subedi, R; Sulkosky, V; Tang, L -G; Tobias, A; Urciuoli, G M; Vilardi, I; Wang, K; Wojtsekhowski, B; Yan, X; Yao, H; Ye, Y; Ye, Z; Yuan, L; Zhan, X; Zhang, Y; Zhang, Y -W; Zhao, B; Zheng, X; Zhu, L; Zhu, X; Zong, X

    2014-11-01

    We report the first measurement of target single spin asymmetries of charged kaons produced in semi-inclusive deep inelastic scattering of electrons off a transversely polarized 3He target. Both the Collins and Sivers moments, which are related to the nucleon transversity and Sivers distributions, respectively, are extracted over the kinematic range of 0.1

  7. Measurement of charged current deep inelastic scattering cross sections with a longitudinally polarised electron beam at HERA

    E-Print Network [OSTI]

    ZEUS Collaboration

    2009-03-24

    Measurements of the cross sections for charged current deep inelastic scattering in e-p collisions with longitudinally polarised electron beams are presented. The measurements are based on a data sample with an integrated luminosity of 175 pb-1 collected with the ZEUS detector at HERA at a centre-of-mass energy of 318 GeV. The total cross section is given for positively and negatively polarised electron beams. The differential cross-sections dsigma/dQ2, dsigma/dx and dsigma/dy are presented for Q2>200 GeV2. The double-differential cross-section d2sigma/dxdQ2 is presented in the kinematic range 280

  8. Q-dependence of the inelastic neutron scattering cross section for molecular spin clusters with high molecular symmetry

    E-Print Network [OSTI]

    O. Waldmann

    2003-04-21

    For powder samples of polynuclear metal complexes the dependence of the inelastic neutron scattering intensity on the momentum transfer Q is known to be described by a combination of so called interference terms. They reflect the interplay between the geometrical structure of the compound and the spatial properties of the wave functions involved in the transition. In this work, it is shown that the Q-dependence is strongly interrelated with the molecular symmetry of molecular nanomagnets, and, if the molecular symmetry is high enough, is actually completely determined by it. A general formalism connecting spatial symmetry and interference terms is developed. The arguments are detailed for cyclic spin clusters, as experimentally realized by e.g. the octanuclear molecular wheel Cr8, and the star like tetranuclear cluster Fe4.

  9. The Microlocal Analysis of some X-ray transforms in Electron ...

    E-Print Network [OSTI]

    Todd Quinto Joint work with Raluca Felea (lines), Hans Rullgård (curvilinear model)

    2012-06-23

    The Model of Electron Tomography (ET) and the Goal. Intro f is the scattering potential of an object. ? is a line or curve over which electrons travel. The X-ray ...

  10. Pressure-Induced Structural Phase Transition in CeNi: X-ray and...

    Office of Scientific and Technical Information (OSTI)

    Pressure-Induced Structural Phase Transition in CeNi: X-ray and Neutron Scattering Studies and First-Principles Calculations Citation Details In-Document Search This content will...

  11. X-ray emission from O stars

    E-Print Network [OSTI]

    David H. Cohen

    2008-02-01

    Young O stars are strong, hard, and variable X-ray sources, properties which strongly affect their circumstellar and galactic environments. After ~1 Myr, these stars settle down to become steady sources of soft X-rays. I use high-resolution X-ray spectroscopy and MHD modeling to show that young O stars like theta-1 Ori C are well explained by the magnetically channeled wind shock scenario. After their magnetic fields dissipate, older O stars produce X-rays via shock heating in their unstable stellar winds. Here too I use X-ray spectroscopy and numerical modeling to confirm this scenario. In addition to elucidating the nature and cause of the O star X-ray emission, modeling of the high-resolution X-ray spectra of O supergiants provides strong evidence that mass-loss rates of these O stars have been overestimated.

  12. X-ray Imaging Workshop

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power AdministrationRobust,Field-effectWorkingLos Alamos verifies largest single goldWindX-Ray ImagingInImaging and

  13. Soft X-ray techniques to study mesoscale magnetism

    E-Print Network [OSTI]

    Kortright, Jeffrey B.

    2003-01-01

    X-Ray Techniques to Study Mesoscale Magnetism Jeffrey B.X-Ray Techniques to Study Mesoscale Magnetism Jeffrey B.

  14. Apparatus for generating x-ray holograms

    DOE Patents [OSTI]

    Rhodes, C.K.; Boyer, K.; Solem, J.C.; Haddad, W.S.

    1990-09-11

    Apparatus for x-ray microholography of living biological materials. A Fourier transform holographic configuration is described as being most suitable for the 3-dimensional recording of the physical characteristics of biological specimens. The use of a spherical scatterer as a reference and a charge-coupled device two-dimensional detector array placed in the forward direction relative to the incident x-radiation for viewing electromagnetic radiation simultaneously scattered from both the specimen and the reference scatterer permits the ready reconstruction of the details of the specimen from the fringe pattern detected by the charge-coupled device. For example, by using a nickel reference scatter at 4.5 nm, sufficient reference illumination is provided over a wide enough angle to allow similar resolution in both transverse and longitudinal directions. Both laser and synchrotron radiation sources are feasible for generating microholographs. Operation in the water window (2.4 to 4.5 nm) should provide maximum contrast for features of the specimen and spatial resolution on the order of the wavelength of x-radiation should be possible in all three dimensions, which is sufficient for the visualization of many biological features. It is anticipated that the present apparatus will find utility in other areas as well where microscopic physical details of a specimen are important. A computational procedure which enables the holographic data collected by the detector to be used to correct for misalignments introduced by inexact knowledge of the relative positions of the spherical reference scatterer and the sample under investigation has been developed. If the correction is performed prior to reconstruction, full compensation can be achieved and a faithfully reconstructed image produced. 7 figs.

  15. Apparatus for generating x-ray holograms

    DOE Patents [OSTI]

    Rhodes, Charles K. (Chicago, IL); Boyer, Keith (Los Alamos, NM); Solem, Johndale C. (Los Alamos, NM); Haddad, Waleed S. (Chicago, IL)

    1990-01-01

    Apparatus for x-ray microholography of living biological materials. A Fourier transform holographic configuration is described as being most suitable for the 3-dimensional recording of the physical characteristics of biological specimens. The use of a spherical scatterer as a reference and a charge-coupled device two-dimensional detector array placed in the forward direction relative to the incident x-radiation for viewing electromagnetic radiation simultaneously scattered from both the specimen and the reference scatterer permits the ready reconstruction of the details of the specimen from the fringe pattern detected by the charge-coupled device. For example, by using a nickel reference scatter at 4.5 nm, sufficient reference illumination is provided over a wide enough angle to allow similar resolution in both transverse and longitudinal directions. Both laser and synchrotron radiation sources are feasible for generating microholographs. Operation in the water window (2.4 to 4.5 nm) should provide maximum contrast for features of the specimen and spatial resolution on the order of the wavelength of x-radiation should be possible in all three dimensions, which is sufficient for the visualization of many biological features. It is anticipated that the present apparatus will find utility in other areas as well where microscopic physical details of a specimen are important. A computational procedure which enables the holographic data collected by the detector to be used to correct for misalignments introduced by inexact knowledge of the relative positions of the spherical reference scatterer and the sample under investigation has been developed. If the correction is performed prior to reconstruction, full compensation can be achieved and a faithfully reconstructed image produced.

  16. X-ray Observations of Mrk 231

    E-Print Network [OSTI]

    T. J. Turner

    1998-08-10

    This paper presents new X-ray observations of Mrk 231, an active galaxy of particular interest due to its large infrared luminosity and the presence of several blueshifted broad absorption line (BAL) systems, a phenomenon observed in a small fraction of QSOs. A ROSAT HRI image of Mrk 231 is presented, this shows an extended region of soft X-ray emission, covering several tens of kpc, consistent with the extent of the host galaxy. An ASCA observation of Mrk 231 is also presented. Hard X-rays are detected but the data show no significant variability in X-ray flux. The hard X-ray continuum is heavily attenuated and X-ray column estimates range from ~ 2 x 10^{22} - 10^{23} cm^{-2} depending on whether the material is assumed to be neutral or ionized, and on the model assumed for the extended X-ray component. These ASCA data provide only the second hard X-ray spectrum of a BAL AGN presented to date. The broad-band spectral-energy-distribution of the source is discussed. While Mrk 231 is X-ray weak compared to Seyfert 1 galaxies, it has an optical-to-X-ray spectrum typical of a QSO.

  17. Controlling X-rays With Light

    SciTech Connect (OSTI)

    Glover, Ernie; Hertlein, Marcus; Southworth, Steve; Allison, Tom; van Tilborg, Jeroen; Kanter, Elliot; Krassig, B.; Varma, H.; Rude, Bruce; Santra, Robin; Belkacem, Ali; Young, Linda

    2010-08-02

    Ultrafast x-ray science is an exciting frontier that promises the visualization of electronic, atomic and molecular dynamics on atomic time and length scales. A largelyunexplored area of ultrafast x-ray science is the use of light to control how x-rays interact with matter. In order to extend control concepts established for long wavelengthprobes to the x-ray regime, the optical control field must drive a coherent electronic response on a timescale comparable to femtosecond core-hole lifetimes. An intense field is required to achieve this rapid response. Here an intense optical control pulse isobserved to efficiently modulate photoelectric absorption for x-rays and to create an ultrafast transparency window. We demonstrate an application of x-ray transparencyrelevant to ultrafast x-ray sources: an all-photonic temporal cross-correlation measurement of a femtosecond x-ray pulse. The ability to control x-ray/matterinteractions with light will create new opportunities at current and next-generation x-ray light sources.

  18. Anharmonic lattice dynamics of Ag2O studied by inelastic neutron scattering and first-principles molecular dynamics simulations

    SciTech Connect (OSTI)

    Lan, Tian [California Institute of Technology, Pasadena] [California Institute of Technology, Pasadena; Li, Chen [ORNL] [ORNL; Niedziela, Jennifer L [ORNL] [ORNL; Smith, Hillary [California Institute of Technology, Pasadena] [California Institute of Technology, Pasadena; Abernathy, Douglas L [ORNL] [ORNL; Rossman, George [California Institute of Technology, Pasadena] [California Institute of Technology, Pasadena; Fultz, B. [California Institute of Technology, Pasadena] [California Institute of Technology, Pasadena

    2014-01-01

    Inelastic neutron scattering measurements on silver oxide (Ag2O) with the cuprite structure were performed at temperatures from 40 to 400 K, and Fourier transform far-infrared spectra were measured from 100 to 300 K. The measured phonon densities of states and the infrared spectra showed unusually large energy shifts with temperature, and large linewidth broadenings. First principles molecular dynamics (MD) calculations were performed at various temperatures, successfully accounting for the negative thermal expansion (NTE) and local dynamics. Using the Fourier-transformed velocity autocorrelation method, the MD calculations reproduced the large anharmonic effects of Ag2O, and were in excellent agreement with the neutron scattering data. The quasiharmonic approximation (QHA) was less successful in accounting for much of the phonon behavior. The QHA could account for some of the NTE below 250 K, although not at higher temperatures. Strong anharmonic effects were found for both phonons and for the NTE. The lifetime broadenings of Ag2O were explained by anharmonic perturbation theory, which showed rich interactions between the Ag-dominated modes and the O-dominated modes in both up- and down-conversion processes.

  19. STUDY MAGNETIC EXCITATIONS IN DOPED TRANSITION METAL OXIDES USING INELASTIC NEUTRON SCATTERING

    SciTech Connect (OSTI)

    Dai, Pengcheng

    2014-02-18

    Understanding the interplay between magnetism and superconductivity continues to be a “hot” topic in modern condensed matter physics. The discovery of high-temperature superconductivity in iron-based materials in 2008 provided an unique opportunity to compare and contrast these materials with traditional high-Tc copper oxide superconductors. Neutron scattering plays an important role in determining the dynamical spin properties in these materials. This proposal is a continuation of previous DOE supported proposal. This report summarizes the final progress we have made over from May 2005 till Aug. 2013. Overall, we continue to carry out extensive neutron scattering experiments on Fe-based materials, focusing on understanding their magnetic properties. In addition, we have established a materials laboratory at UT that has allowed us to grow these superconductors. Because neutron scattering typically demands a large amount of samples, by growing these materials in our own laboratory, we can now pursuit neutron scattering experiments over the entire electronic phase diagram, focusing on regions of interests. The material synthesis laboratory at UT was established entirely with the support of DOE funding. This not only allowed us to carry out neutron scattering experiments, but also permit us to provide samples to other US/International collaborators for studying these materials.

  20. X-ray transmissive debris shield

    DOE Patents [OSTI]

    Spielman, Rick B. (Albuquerque, NM)

    1994-01-01

    A composite window structure is described for transmitting x-ray radiation and for shielding radiation generated debris. In particular, separate layers of different x-ray transmissive materials are laminated together to form a high strength, x-ray transmissive debris shield which is particularly suited for use in high energy fluences. In one embodiment, the composite window comprises alternating layers of beryllium and a thermoset polymer.

  1. A criterion for the dynamical to kinematical transition of x-ray diffraction on a bent crystal

    SciTech Connect (OSTI)

    Kushnir, V.I.; Macrander, A.T.

    1993-09-01

    It is well known that the peak reflectivity of a bent crystal, generally speaking, is smaller than that of a plane crystal, and it goes to zero when the crystal curvature goes to infinity. The reason for this is the transition between dynamical and kinematical diffraction that takes place as the crystal curvature increases. The physical explanation is as follows: the deviation from exact Bragg position along the beam changes so fast that the thickness over which the beam is within a Darwin width becomes too small to reflect the beam. Bent crystals are widely used as focusing elements in X-ray optics, and estimation of whether or not a bent crystal is still perfect enough to provide good reflectivity is of great importance. Currently the Advanced Photon Source (APS) is considering a number of bent crystals as focusing elements for future APS beamlines, including a sagittaly focusing monochromator and bent backscattering analyzer for inelastic X-ray scattering experiments. A criterion is given in answer to the question: To what extent is it possible to bend a crystal without loss of X-ray peak reflectivity? An expression based on the work of Chukhovskii, Gabrielyan and Petrashen, is formulated that applies to anisotropic cubic crystal and that can be used not only for conventional asymmetric Bragg diffraction, but also for inclined crystal diffraction. The following special cases are treated as examples: isotropic crystal, standard symmetrical Bragg diffraction, extremely asymmetric diffraction, and backscattering with Bragg angles near 90{degree}. In addition, an asymptotic behavior for high energies is detailed.

  2. Laser plasma x-ray source for ultrafast time-resolved x-ray absorption spectroscopy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Miaja-Avila, L.; O'Neil, G. C.; Uhlig, J.; Cromer, C. L.; Dowell, M. L.; Jimenez, R.; Hoover, A. S.; Silverman, K. L.; Ullom, J. N.

    2015-03-02

    We describe a laser-driven x-ray plasma source designed for ultrafast x-ray absorption spectroscopy. The source is comprised of a 1 kHz, 20 W, femtosecond pulsed infrared laser and a water target. We present the x-ray spectra as a function of laser energy and pulse duration. Additionally, we investigate the plasma temperature and photon flux as we vary the laser energy. We obtain a 75 ?m FWHM x-ray spot size, containing ~106 photons/s, by focusing the produced x-rays with a polycapillary optic. Since the acquisition of x-ray absorption spectra requires the averaging of measurements from >107 laser pulses, we also presentmore »data on the source stability, including single pulse measurements of the x-ray yield and the x-ray spectral shape. In single pulse measurements, the x-ray flux has a measured standard deviation of 8%, where the laser pointing is the main cause of variability. Further, we show that the variability in x-ray spectral shape from single pulses is low, thus justifying the combining of x-rays obtained from different laser pulses into a single spectrum. Finally, we show a static x-ray absorption spectrum of a ferrioxalate solution as detected by a microcalorimeter array. Altogether, our results demonstrate that this water-jet based plasma source is a suitable candidate for laboratory-based time-resolved x-ray absorption spectroscopy experiments.« less

  3. X-ray microscopy. Beyond ensemble averages

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Ice, Gene E.; Budai, John D.

    2015-06-23

    This work exemplifies emerging tools to characterize local materials structure and dynamics, made possible by powerful X-ray synchrotron and transmission electron microscopy methods.

  4. X-ray laser microscope apparatus

    DOE Patents [OSTI]

    Suckewer, Szymon (Princeton, NJ); DiCicco, Darrell S. (Plainsboro, NJ); Hirschberg, Joseph G. (Coral Gables, FL); Meixler, Lewis D. (East Windsor, NJ); Sathre, Robert (Princeton, NJ); Skinner, Charles H. (Lawrenceville, NJ)

    1990-01-01

    A microscope consisting of an x-ray contact microscope and an optical microscope. The optical, phase contrast, microscope is used to align a target with respect to a source of soft x-rays. The source of soft x-rays preferably comprises an x-ray laser but could comprise a synchrotron or other pulse source of x-rays. Transparent resist material is used to support the target. The optical microscope is located on the opposite side of the transparent resist material from the target and is employed to align the target with respect to the anticipated soft x-ray laser beam. After alignment with the use of the optical microscope, the target is exposed to the soft x-ray laser beam. The x-ray sensitive transparent resist material whose chemical bonds are altered by the x-ray beam passing through the target mater GOVERNMENT LICENSE RIGHTS This invention was made with government support under Contract No. De-FG02-86ER13609 awarded by the Department of Energy. The Government has certain rights in this invention.

  5. Compound refractive X-ray lens

    DOE Patents [OSTI]

    Nygren, David R. (Berkeley, CA); Cahn, Robert (Walnut Creek, CA); Cederstrom, Bjorn (Traellborg, SE); Danielsson, Mats (Stocksund, SE); Vestlund, Jonas (Stockholm, SE)

    2000-01-01

    An apparatus and method for focusing X-rays. In one embodiment, his invention is a commercial-grade compound refractive X-ray lens. The commercial-grade compound refractive X-ray lens includes a volume of low-Z material. The volume of low-Z material has a first surface which is adapted to receive X-rays of commercially-applicable power emitted from a commercial-grade X-ray source. The volume of low-Z material also has a second surface from which emerge the X-rays of commercially-applicable power which were received at the first surface. Additionally, the commercial-grade compound refractive X-ray lens includes a plurality of openings which are disposed between the first surface and the second surface. The plurality of openings are oriented such that the X-rays of commercially-applicable power which are received at the first surface, pass through the volume of low-Z material and through the plurality openings. In so doing, the X-rays which emerge from the second surface are refracted to a focal point.

  6. X-Ray Nanoimaging: Instruments and Methods

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantity ofkandz-cm11 Outreach Home RoomPreservationBio-Inspired SolarAbout /Two0PhotosPresentationsWorld's largestX-RayX-RayX-RayX-Ray

  7. X-ray Spectral Properties of the BAT AGN Sample

    E-Print Network [OSTI]

    L. M. Winter; R. Mushotzky; C. S. Reynolds; J. Tueller

    2008-08-04

    The 9-month Swift Burst Alert Telescope (BAT) catalog provides the first unbiased (log N_H = 0.03) AGN. In this paper, we present the collected X-ray properties (0.3 - 12keV) for the 153 AGN detected. In addition, we examine the X-ray properties for a complete sample of non-beamed sources, above the Galactic plane. Of these, 45% are best fit by simple power law models while 55% require the more complex partial covering model. One of our goals was to determine the fraction of "hidden" AGN, which we define as sources with scattering fractions Marshall et al. 1980). From the log N-log S relationship, we show that we are complete to log S < -11 in the 2-10 keV band. Both the collected X-ray properties of our uniform sample and the log N-log S relationship will now provide valuable input to X-ray background models for z ~ 0. (abridged)

  8. Magnetic Transitions in Iron Porphyrin Halides by Inelastic Neutron Scattering and Ab-initio Studies of Zero-Field Splittings

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Stavretis, Shelby E.; Atanasov, Mihail; Podlesnyak, Andrey A.; Hunter, Seth C.; Neese, Frank; Xue, Zi-Ling

    2015-10-02

    Zero-field splitting (ZFS) parameters of nondeuterated metalloporphyrins [Fe(TPP)X] (X = F, Br, I; H2TPP = tetraphenylporphyrin) are determined by inelastic neutron scattering (INS). The ZFS values are D = 4.49(9) cm–1 for tetragonal polycrystalline [Fe(TPP)F], and D = 8.8(2) cm–1, E = 0.1(2) cm–1 and D = 13.4(6) cm–1, E = 0.3(6) cm–1 for monoclinic polycrystalline [Fe(TPP)Br] and [Fe(TPP)I], respectively. Along with our recent report of the ZFS value of D = 6.33(8) cm–1 for tetragonal polycrystalline [Fe(TPP)Cl], these data provide a rare, complete determination of ZFS parameters in a metalloporphyrin halide series. The electronic structure of [Fe(TPP)X] (X =more »F, Cl, Br, I) has been studied by multireference ab initio methods: the complete active space self-consistent field (CASSCF) and the N-electron valence perturbation theory (NEVPT2) with the aim of exploring the origin of the large and positive zero-field splitting D of the 6A1 ground state. D was calculated from wave functions of the electronic multiplets spanned by the d5 configuration of Fe(III) along with spin–orbit coupling accounted for by quasi degenerate perturbation theory. Results reproduce trends of D from inelastic neutron scattering data increasing in the order from F, Cl, Br, to I. A mapping of energy eigenvalues and eigenfunctions of the S = 3/2 excited states on ligand field theory was used to characterize the ?- and ?-antibonding effects decreasing from F to I. This is in agreement with similar results deduced from ab initio calculations on CrX63- complexes and also with the spectrochemical series showing a decrease of the ligand field in the same directions. A correlation is found between the increase of D and decrease of the ?- and ?-antibonding energies e?X (? = ?, ?) in the series from X = F to I. Analysis of this correlation using second-order perturbation theory expressions in terms of angular overlap parameters rationalizes the experimentally deduced trend. Furthermore, D parameters from CASSCF and NEVPT2 results have been calibrated against those from the INS data, yielding a predictive power of these approaches. Methods to improve the quantitative agreement between ab initio calculated and experimental D and spectroscopic transitions for high-spin Fe(III) complexes are proposed.« less

  9. X-ray spectroscopy of neutron star low-mass X-ray binaries

    E-Print Network [OSTI]

    Krauss, Miriam Ilana

    2007-01-01

    In this thesis, I present work spanning a variety of topics relating to neutron star lowmass X-ray binaries (LMXBs) and utilize spectral information from X-ray observations to further our understanding of these sources. ...

  10. HEW simulations and quantification of the microroughness requirements for X-ray telescopes by means of numerical and analytical methods

    E-Print Network [OSTI]

    Spiga, D; Pareschi, G

    2015-01-01

    Future X-ray telescopes like SIMBOL-X will operate in a wide band of the X-ray spectrum (from 0.1 to 80 keV); these telescopes will extend the optical performances of the existing soft X-ray telescopes to the hard X-ray band, and in particular they will be characterized by a angular resolution (conveniently expressed in terms of HEW, Half-Energy- Width) less than 20 arcsec. However, it is well known that the microroughness of the reflecting surfaces of the optics causes the scattering of X-rays. As a consequence, the imaging quality can be severely degraded. Moreover, the X-ray scattering can be the dominant problem in hard X-rays because its relevance is an increasing function of the photon energy. In this work we consistently apply a numerical method and an analytical one to evaluate the X-ray scattering impact on the HEW of an X-ray optic, as a function of the photon energy: both methods can also include the effects of figure errors in determining the final HEW. A comparison of the results obtained with th...

  11. Optical module HEW simulations for the X-ray telescopes SIMBOL-X, EDGE and XEUS

    E-Print Network [OSTI]

    Spiga, D

    2015-01-01

    One of the most important parameters defining the angular resolution of an X-ray optical module is its Half-Energy Width (HEW) as a function of the photon energy. Future X-ray telescopes with imaging capabilities (SIMBOL-X, Constellation-X, NeXT, EDGE, XEUS,...) should be characterized by a very good angular resolution in soft ( 10 keV) X-rays. As a consequence, an important point in the optics development for these telescopes is the simulation of the achievable HEW for a system of X-ray mirrors. This parameter depends on the single mirror profile and nesting accuracy, but also on the mirrors surface microroughness that causes X-ray Scattering (XRS). In particular, owing to its dependence on the photon energy, XRS can dominate the profile errors in hard X-rays: thus, its impact has to be accurately evaluated in every single case, in order to formulate surface finishing requirements for X-ray mirrors. In this work we provide with some simulations of the XRS term of the HEW for some future soft and hard X-ray t...

  12. Measurement of the Target-Normal Single-Spin Asymmetry in Deep-Inelastic Scattering from the Reaction $^{3}\\mathrm{He}^{\\uparrow}(e,e')X$

    E-Print Network [OSTI]

    J. Katich; X. Qian; Y. X. Zhao; K. Allada; K. Aniol; J. R. M. Annand; T. Averett; F. Benmokhtar; W. Bertozzi; P. C. Bradshaw; P. Bosted; A. Camsonne; M. Canan; G. D. Cates; C. Chen; J. -P. Chen; W. Chen; K. Chirapatpimol; E. Chudakov; E. Cisbani; J. C. Cornejo; F. Cusanno; M. M. Dalton; W. Deconinck; C. W. de Jager; R. De Leo; X. Deng; A. Deur; H. Ding; P. A. M. Dolph; C. Dutta; D. Dutta; L. El Fassi; S. Frullani; H. Gao; F. Garibaldi; D. Gaskell; S. Gilad; R. Gilman; O. Glamazdin; S. Golge; L. Guo; D. Hamilton; O. Hansen; D. W. Higinbotham; T. Holmstrom; J. Huang; M. Huang; H. F. Ibrahim; M. Iodice; X. Jiang; G. Jin; M. K. Jones; A. Kelleher; W. Kim; A. Kolarkar; W. Korsch; J. J. LeRose; X. Li; Y. Li; R. Lindgren; N. Liyanage; E. Long; H. -J. Lu; D. J. Margaziotis; P. Markowitz; S. Marrone; D. McNulty; Z. -E. Meziani; R. Michaels; B. Moffit; C. Mu?oz Camacho; S. Nanda; A. Narayan; V. Nelyubin; B. Norum; Y. Oh; M. Osipenko; D. Parno; J. C. Peng; S. K. Phillips; M. Posik; A. J. R. Puckett; Y. Qiang; A. Rakhman; R. D. Ransome; S. Riordan; A. Saha; B. Sawatzky; E. Schulte; A. Shahinyan; M. H. Shabestari; S. Širca; S. Stepanyan; R. Subedi; V. Sulkosky; L. -G. Tang; A. Tobias; G. M. Urciuoli; I. Vilardi; K. Wang; Y. Wang; B. Wojtsekhowski; X. Yan; H. Yao; Y. Ye; Z. Ye; L. Yuan; X. Zhan; Y. Zhang; Y. -W. Zhang; B. Zhao; X. Zheng; L. Zhu; X. Zhu; X. Zong

    2014-08-04

    We report the first measurement of the target-normal single-spin asymmetry in deep-inelastic scattering from the inclusive reaction $^3$He$^{\\uparrow}\\left(e,e' \\right)X$ on a polarized $^3$He gas target. Assuming time-reversal invariance, this asymmetry is strictly zero in the Born approximation but can be non-zero if two-photon-exchange contributions are included. The experiment, conducted at Jefferson Lab using a 5.89 GeV electron beam, covers a range of $1.7 2$ GeV, which is non-zero at the $2.89\\sigma$ level. Our measured asymmetry agrees both in sign and magnitude with a two-photon-exchange model prediction that uses input from the Sivers transverse momentum distribution obtained from semi-inclusive deep-inelastic scattering.

  13. Neutron Scattering Tutorials | Neutron Science | ORNL

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Neutron Scattering Tutorials SHARE Neutron Scattering Tutorials The following lectures were presented at the 2011 and 2010 National School on Neutron & X-Ray Scattering. This...

  14. Neutron inelastic scattering and reactions in natural Pb as a background in neutrinoless double-beta-decay experiments

    E-Print Network [OSTI]

    V. E. Guiseppe; M. Devlin; S. R. Elliott; N. Fotiades; A. Hime; D. -M. Mei; R. O. Nelson; D. V. Perepelitsa

    2009-09-24

    Inelastic neutron scattering and reactions on Pb isotopes can result in gamma rays near the signature endpoint energy in a number of double-beta decay isotopes. In particular, there are gamma-ray transitions in Pb-206,207,208 that might produce energy deposits at the 76-Ge Q value in Ge detectors used for double-beta decay searches. The levels that produce these gamma rays can be excited by (n,n'gamma) or (n,xngamma) reactions, but the cross sections are small and previously unmeasured. This work uses the pulsed neutron beam at the Los Alamos Neutron Science Center to directly measure reactions of interest to double-beta decay experiments. The cross section on natural Pb to produce the 2041-keV gamma ray from Pb-206 is measured to be 3.6 +/- 0.7 (stat.) +/- 0.3 (syst.) mb at ~9.6 MeV. The cross section on natural Pb to produce the 3062-keV gamma ray from Pb-207 and Pb-208 is measured to be 3.9 +/- 0.8 (stat.) +/- 0.4 (syst.) mb at the same energy. We report cross sections or place upper limits on the cross sections for exciting some other levels in Pb that have transition energies corresponding to Q value in other double-beta decay isotopes.

  15. Diffractive Dijet Production in Deep Inelastic Scattering and Photon-Hadron Collisions in the Color Glass Condensate

    E-Print Network [OSTI]

    Tolga Altinoluk; Néstor Armesto; Guillaume Beuf; Amir H. Rezaeian

    2015-11-23

    We study diffractive dijet production in deep inelastic scattering and real (and virtual) photon-hadron ($\\gamma^{(*)}$-h) collisions in the Color Glass Condensate formalism at leading order. We show that the diffractive dijet cross section is sensitive to the color-dipole orientation in the transverse plane, and is a good probe of possible correlations between the $q\\bar{q}$-dipole transverse separation vector $\\vec r$ and the dipole impact parameter $\\vec b$. We also investigate the diffractive dijet azimuthal angle correlations and $t$-distributions in $\\gamma^{(*)}$-h collisions and show that they are sensitive to gluon saturation effects in the small-$x$ region. In particular, we show that the $t$-distribution of diffractive dijet photo-production off a proton target exhibits a dip-type structure in the saturation region. This effect is similar to diffractive vector meson production. Besides, at variance with the inclusive case, the effect of saturation leads to stronger azimuthal correlations between the jets.

  16. Diffractive Dijet Production in Deep Inelastic Scattering and Photon-Hadron Collisions in the Color Glass Condensate

    E-Print Network [OSTI]

    Altinoluk, Tolga; Beuf, Guillaume; Rezaeian, Amir H

    2015-01-01

    We study diffractive dijet production in deep inelastic scattering and real (and virtual) photon-hadron ($\\gamma^{(*)}$-h) collisions in the Color Glass Condensate formalism at leading order. We show that the diffractive dijet cross section is sensitive to the color-dipole orientation in the transverse plane, and is a good probe of possible correlations between the $q\\bar{q}$-dipole transverse separation vector $\\vec r$ and the dipole impact parameter $\\vec b$. We also investigate the diffractive dijet azimuthal angle correlations and $t$-distributions in $\\gamma^{(*)}$-h collisions and show that they are sensitive to gluon saturation effects in the small-$x$ region. In particular, we show that the $t$-distribution of diffractive dijet photo-production off a proton target exhibits a dip-type structure in the saturation region. This effect is similar to diffractive vector meson production. Besides, at variance with the inclusive case, the effect of saturation leads to stronger azimuthal correlations between th...

  17. Phased Contrast X-Ray Imaging

    ScienceCinema (OSTI)

    Erin Miller

    2012-12-31

    The Pacific Northwest National Laboratory is developing a range of technologies to broaden the field of explosives detection. Phased contrast X-ray imaging, which uses silicon gratings to detect distortions in the X-ray wave front, may be applicable to mail or luggage scanning for explosives; it can also be used in detecting other contraband, small-parts inspection, or materials characterization.

  18. Proceedings of the 1984 workshop on high-energy excitations in condensed matter. Volume I

    SciTech Connect (OSTI)

    Silver, R.N. (comp.)

    1984-12-01

    This volume covers neutron scattering inelastic instrumentation, x-ray scattering inelastic instrumentation, and magnetic excitations. (GHT)

  19. Anti-contamination device for cryogenic soft X-ray diffraction microscopy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Huang, Xiaojing; Miao, Huijie; Nelson, Johanna; Turner, Joshua; Steinbrener, Jan; Shapiro, David; Kirz, Janos; Jacobsen, Chris

    2011-05-01

    Cryogenic microscopy allows one to view frozen hydrated biological and soft matter specimens with good structural preservation and a high degree of stability against radiation damage. We describe a liquid nitrogen-cooled anti-contamination device for cryogenic X-ray diffraction microscopy. The anti-contaminator greatly reduces the buildup of ice layers on the specimen due to condensation of residual water vapor in the experimental vacuum chamber. We show by coherent X-ray diffraction measurements that this leads to fivefold reduction of background scattering, which is important for far-field X-ray diffraction microscopy of biological specimens.

  20. X-rays from Hot Subdwarfs

    E-Print Network [OSTI]

    Mereghetti, Sandro

    2015-01-01

    Thanks to the high sensitivity of the instruments on board the XMM-Newton and Chandra satellites, it has become possible to explore the properties of the X-ray emission from hot subdwarfs. The small but growing sample of hot subdwarfs detected in X-rays includes binary systems, in which the X-rays result from wind accretion onto a compact companion (white dwarf or neutron star), as well as isolated sdO stars in which X-rays are probably due to shock instabilities in the wind. X-ray observations of these low mass stars provide information which can be useful also for our understanding of the winds of more luminous and massive early-type stars and can lead to the discovery of particularly interesting binary systems.

  1. High Energy Vision: Processing X-rays

    E-Print Network [OSTI]

    DePasquale, Joseph; Edmonds, Peter

    2015-01-01

    Astronomy is by nature a visual science. The high quality imagery produced by the world's observatories can be a key to effectively engaging with the public and helping to inspire the next generation of scientists. Creating compelling astronomical imagery can, however, be particularly challenging in the non-optical wavelength regimes. In the case of X-ray astronomy, where the amount of light available to create an image is severely limited, it is necessary to employ sophisticated image processing algorithms to translate light beyond human vision into imagery that is aesthetically pleasing while still being scientifically accurate. This paper provides a brief overview of the history of X-ray astronomy leading to the deployment of NASA's Chandra X-ray Observatory, followed by an examination of the specific challenges posed by processing X-ray imagery. The authors then explore image processing techniques used to mitigate such processing challenges in order to create effective public imagery for X-ray astronomy. ...

  2. Elastic and inelastic scattering to low-lying states of {sup 58}Ni and {sup 90}Zr using 240-MeV {sup 6}Li

    SciTech Connect (OSTI)

    Krishichayan; Chen, X.; Lui, Y.-W.; Tokimoto, Y.; Button, J.; Youngblood, D. H. [Cyclotron Institute, Texas A and M University, College Station, Texas 77843 (United States)

    2010-01-15

    Elastic and inelastic scattering of 240-MeV {sup 6}Li particles from {sup 58}Ni and {sup 90}Zr were measured with the multipole-dipole-multipole spectrometer from 4 deg. <={theta}{sub c.m.}<=43 deg. The elastic scattering data were fitted with the double-folding model using the density-dependent M3Y NN effective interaction and with a phenomenological Woods-Saxon potential. B(E2) and B(E3) values obtained for low-lying 2{sup +} and 3{sup -} states with the double-folding calculations agreed with the adopted values.

  3. Fiber fed x-ray/gamma ray imaging apparatus

    DOE Patents [OSTI]

    Hailey, Charles J. (San Francisco, CA); Ziock, Klaus-Peter (Livermore, CA)

    1992-01-01

    X-ray/gamma ray imaging apparatus is disclosed for detecting the position, energy, and intensity of x-ray/gamma ray radiation comprising scintillation means disposed in the path of such radiation and capable of generating photons in response to such radiation; first photodetection means optically bonded to the scintillation means and capable of generating an electrical signal indicative of the intensity, and energy of the radiation detected by the scintillation means; second photodetection means capable of generating an electrical signal indicative of the position of the radiation in the radiation pattern; and means for optically coupling the scintillation means to the second photodetection means. The photodetection means are electrically connected to control and storage means which may also be used to screen out noise by rejecting a signal from one photodetection means not synchronized to a signal from the other photodetection means; and also to screen out signals from scattered radiation.

  4. Towards phasing using high X-ray intensity

    SciTech Connect (OSTI)

    Galli, Lorenzo; Son, Sang -Kil; Barends, Thomas R. M.; White, Thomas A.; Barty, Anton; Botha, Sabine; Boutet, Sébastien; Caleman, Carl; Doak, R. Bruce; Nanao, Max H.; Nass, Karol; Shoeman, Robert L.; Timneanu, Nicusor; Santra, Robin; Schlichting, Ilme; Chapman, Henry N.

    2015-09-30

    X-ray free-electron lasers (XFELs) show great promise for macromolecular structure determination from sub-micrometre-sized crystals, using the emerging method of serial femtosecond crystallography. The extreme brightness of the XFEL radiation can multiply ionize most, if not all, atoms in a protein, causing their scattering factors to change during the pulse, with a preferential `bleaching' of heavy atoms. This paper investigates the effects of electronic damage on experimental data collected from a Gd derivative of lysozyme microcrystals at different X-ray intensities, and the degree of ionization of Gd atoms is quantified from phased difference Fourier maps. In conclusion, a pattern sorting scheme is proposed to maximize the ionization contrast and the way in which the local electronic damage can be used for a new experimental phasing method is discussed.

  5. Towards phasing using high X-ray intensity

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Galli, Lorenzo; Son, Sang -Kil; Barends, Thomas R. M.; White, Thomas A.; Barty, Anton; Botha, Sabine; Boutet, Sébastien; Caleman, Carl; Doak, R. Bruce; Nanao, Max H.; et al

    2015-09-30

    X-ray free-electron lasers (XFELs) show great promise for macromolecular structure determination from sub-micrometre-sized crystals, using the emerging method of serial femtosecond crystallography. The extreme brightness of the XFEL radiation can multiply ionize most, if not all, atoms in a protein, causing their scattering factors to change during the pulse, with a preferential `bleaching' of heavy atoms. This paper investigates the effects of electronic damage on experimental data collected from a Gd derivative of lysozyme microcrystals at different X-ray intensities, and the degree of ionization of Gd atoms is quantified from phased difference Fourier maps. In conclusion, a pattern sorting schememore »is proposed to maximize the ionization contrast and the way in which the local electronic damage can be used for a new experimental phasing method is discussed.« less

  6. Pressure-induced amorphization of CuFeS2 studied by 57 Fe nuclear resonant inelastic scattering

    E-Print Network [OSTI]

    Alfè, Dario

    Hisao Kobayashi,* Junpei Umemura, Yutaka Kazekami, and Nobuhiko Sakai Graduate School of Material structural properties of CuFeS2 under high pressure were investigated by x-ray diffrac- tion and 57 Fe centered tetragonal lattice with space group I4¯2d, which is an antiferromagnetic semiconductor with high

  7. X-ray diffraction study of the structure of detonation nanodiamonds

    SciTech Connect (OSTI)

    Ozerin, A. N. Kurkin, T. S.; Ozerina, L. A.; Dolmatov, V. Yu.

    2008-01-15

    The spatial structure of aggregates formed by detonation nanodiamonds is investigated using the wide-angle and small-angle X-ray scattering techniques. The effective sizes of crystallites and the crystallite size distribution function are determined. The shape of scattering aggregates is restored from the small-angle X-ray scattering data. An analysis of the results obtained allowed the conclusion that the nanodiamond aggregates have an extended spatial structure composed of nine to ten clusters, each involving four to five crystallites with a crystal lattice of the diamond type.

  8. X-ray phase-contrast methods

    SciTech Connect (OSTI)

    Lider, V. V., E-mail: lider@ns.crys.ras.ru; Kovalchuk, M. V. [Russian Academy of Sciences, Shubnikov Institute of Crystallography (Russian Federation)] [Russian Academy of Sciences, Shubnikov Institute of Crystallography (Russian Federation)

    2013-11-15

    This review is devoted to a comparative description of the methods for forming X-ray phase-contrast images of weakly absorbing (phase) objects. These include the crystal interferometer method, the Talbot interferometer method, diffraction-enhanced X-ray imaging, and the in-line method. The potential of their practical application in various fields of science and technology is discussed. The publications on the development and optimization of X-ray phase-contrast methods and the experimental study of phase objects are analyzed.

  9. X-rays Illuminate Ancient Archimedes Text

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power AdministrationRobust,Field-effectWorkingLos Alamos verifies largest single goldWindX-RayX-RayX-ray

  10. NMR studies of chiral P,S-chelate platinum, rhodium, and iridium complexes and the X-ray structure of a palladium(II) allyl derivative

    SciTech Connect (OSTI)

    Albinati, A. [Univ. of Milan (Italy)] [Univ. of Milan (Italy); Eckert, J. [Los Alamos National Lab., NM (United States)] [Los Alamos National Lab., NM (United States); Pregosin, P.; Ruegger, H.; Salzmann, R.; Stoessel, C. [ETH-Zentrum, Zuerich (Switzerland)] [ETH-Zentrum, Zuerich (Switzerland)

    1997-02-18

    Several Rh(I), Ir(III), and Pt(II) complexes of the chiral P,S-bidentate ligand 2 have been prepared and characterized. Detailed two-dimensional NMR studies show that (i) the boat-type chelate ring and the stereogenic sulfur center can invert rapidly at ambient temperature and (ii) the sulfur donor may dissociate, essentially destroying the chiral pocket. The solid-state structure of [Pt({eta}{sup 3}-C{sub 3}H{sub 5})(2)]PF{sub 6} (3) has been determined and the sulfur substituent shown to have an axial orientation. The six-membered chelate ring takes up a boat-like conformation. As shown by an X-ray diffraction study for 3, and via incoherent inelastic neutron scattering (IINS) measurements for the Pd analog, 4, the OH group is remote from the metal atom. 42 refs., 11 figs., 6 tabs.

  11. Combination of Measurements of Inclusive Deep Inelastic $e^{\\pm}p$ Scattering Cross Sections and QCD Analysis of HERA Data

    E-Print Network [OSTI]

    H1; ZEUS Collaborations

    2015-06-19

    A combination is presented of all inclusive deep inelastic cross sections previously published by the H1 and ZEUS collaborations at HERA for neutral and charged current $e^{\\pm}p$ scattering for zero beam polarisation. The data were taken at proton beam energies of 920, 820, 575 and 460 GeV and an electron beam energy of 27.5 GeV. The data correspond to an integrated luminosity of about 1 fb$^{-1}$ and span six orders of magnitude in negative four-momentum-transfer squared, $Q^2$, and Bjorken $x$. The correlations of the systematic uncertainties were evaluated and taken into account for the combination. The combined cross sections were input to QCD analyses at leading order, next-to-leading order and at next-to-next-to-leading order, providing a new set of parton distribution functions, called HERAPDF2.0. In addition to the experimental uncertainties, model and parameterisation uncertainties were assessed for these parton distribution functions. Variants of HERAPDF2.0 with an alternative gluon parameterisation, HERAPDF2.0AG, and using fixed-flavour-number schemes, HERAPDF2.0FF, are presented. The analysis was extended by including HERA data on charm and jet production, resulting in the variant HERAPDF2.0Jets. The inclusion of jet-production cross sections made a simultaneous determination of these parton distributions and the strong coupling constant possible, resulting in $\\alpha_s(M_Z)=0.1183 \\pm 0.0009 {\\rm(exp)} \\pm 0.0005{\\rm (model/parameterisation)} \\pm 0.0012{\\rm (hadronisation)} ^{+0.0037}_{-0.0030}{\\rm (scale)}$. An extraction of $xF_3^{\\gamma Z}$ and results on electroweak unification and scaling violations are also presented.

  12. X-Ray Nanoimaging: Instruments and Methods

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Instruments and Methods X-Ray Nanoimaging: Instruments and Methods Print To be held as part of SPIE. http:spie.orgOP318 August 28-29, 2013; San Diego, California, USA...

  13. X-ray source for mammography

    DOE Patents [OSTI]

    Logan, Clinton M. (Pleasanton, CA)

    1994-01-01

    An x-ray source utilizing anode material which shifts the output spectrum to higher energy and thereby obtains higher penetrating ability for screening mammography application, than the currently utilized anode material. The currently used anode material (molybdenum) produces an energy x-ray spectrum of 17.5/19.6 keV, which using the anode material of this invention (e.g. silver, rhodium, and tungsten) the x-ray spectrum would be in the 20-35 keV region. Thus, the anode material of this invention provides for imaging of breasts with higher than average x-ray opacity without increase of the radiation dose, and thus reduces the risk of induced breast cancer due to the radiation dose administered for mammograms.

  14. X-ray source for mammography

    DOE Patents [OSTI]

    Logan, C.M.

    1994-12-20

    An x-ray source is described utilizing anode material which shifts the output spectrum to higher energy and thereby obtains higher penetrating ability for screening mammography application, than the currently utilized anode material. The currently used anode material (molybdenum) produces an energy x-ray spectrum of 17.5/19.6 keV, which using the anode material of this invention (e.g. silver, rhodium, and tungsten) the x-ray spectrum would be in the 20-35 keV region. Thus, the anode material of this invention provides for imaging of breasts with higher than average x-ray opacity without increase of the radiation dose, and thus reduces the risk of induced breast cancer due to the radiation dose administered for mammograms. 6 figures.

  15. Polarized inelastic neutron scattering of the partially ordered Tb2Sn2O7 K. C. Rule,1 G. Ehlers,2 J. R. Stewart,3 A. L. Cornelius,4 P. P. Deen,3 Y. Qiu,5,6 C. R. Wiebe,7,8 J. A. Janik,7 H. D. Zhou,7

    E-Print Network [OSTI]

    Weston, Ken

    Polarized inelastic neutron scattering of the partially ordered Tb2Sn2O7 K. C. Rule,1 G. Ehlers,2 J 17 August 2007; published 21 December 2007 We present inelastic neutron scattering results neutron scattering, susceptibility, and specific heat techniques have shown that below 0.87 K Tb2Sn2O7

  16. New opportunities for quasielastic and inelastic neutron scattering at steady-state sources using mechanical selection of the incident and final neutron energy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Mamantov, Eugene

    2015-06-12

    We propose a modification of the neutron wide-angle velocity selector (WAVES) device that enables inelastic (in particular, quasielastic) scattering measurements not relying on the neutron time-of-flight. The proposed device is highly suitable for a steady-state neutron source, somewhat similar to a triple-axis spectrometer, but with simultaneous selection of the incident and final neutron energy over a broad range of scattering momentum transfer. Both the incident and final neutron velocities are defined by the WAVES geometry and rotation frequency. The variable energy transfer is achieved through the natural variation of the velocity of the transmitted neutrons as a function of themore »scattering angle component out of the equatorial plane.« less

  17. X-ray laser driven gold targets

    SciTech Connect (OSTI)

    Petrova, Tz. B., E-mail: lina.petrova@nrl.navy.mil; Whitney, K. G.; Davis, J. [Plasma Physics Division, Naval Research Laboratory, 4555 Overlook Ave. SW, Washington, DC 20375 (United States)] [Plasma Physics Division, Naval Research Laboratory, 4555 Overlook Ave. SW, Washington, DC 20375 (United States)

    2014-03-15

    The femtosecond population dynamics of gold irradiated by a coherent high-intensity (>10{sup 17}?W/cm{sup 2}) x-ray laser pulse is investigated theoretically. There are two aspects to the assembled model. One is the construction of a detailed model of platinum-like gold inclusive of all inner-shell states that are created by photoionization of atomic gold and decay either by radiative or Auger processes. Second is the computation of the population dynamics that ensues when an x-ray pulse is absorbed in gold. The hole state generation depends on the intensity and wavelength of the driving x-ray pulse. The excited state populations reached during a few femtosecond timescales are high enough to generate population inversions, whose gain coefficients are calculated. These amplified lines in the emitted x-ray spectrum provide important diagnostics of the radiation dynamics and also suggest a nonlinear way to increase the frequency of the coherent output x-ray pulses relative to the frequency of the driver input x-ray pulse.

  18. Characteristic x-ray emission from undermines plasmas irradiated by ultra-intense lasers

    SciTech Connect (OSTI)

    Niemann, Christoph

    2012-05-05

    Between FY09 and FY11 we have conducted more than a dozen three-week experimental campaigns at high-power laser facilities around the world to investigate laser-channeling through x-ray and optical imaging and the conversion from laser-energy to xrays. We have performed simultaneous two-wavelength x-ray imaging (K-alpha and He-alpha) to distinguish the hot-plasma region (hot-spot) from the laser-produced electrons (K-alpha). In addition, we have initiated a new collaboration with SNL and have performed first shots on the 100 TW beamlet chamber to commission a fast x-ray streak camera to be used to investigate the temporal evolution of our K-alpha sources. We also collaborated on campaigns at the Rutherford Appleton Laboratory (UK) and the LANL Trident laser to employ laser produced x-ray sources for Thomson scattering off dense matter.

  19. High-resolution ab initio three-dimensional x-ray diffraction microscopy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Chapman, Henry N.; Barty, Anton; Marchesini, Stefano; Noy, Aleksandr; Hau-Riege, Stefan P.; Cui, Congwu; Howells, Malcolm R.; Rosen, Rachel; He, Haifeng; Spence, John C. H.; et al

    2006-01-01

    Coherent x-ray diffraction microscopy is a method of imaging nonperiodic isolated objects at resolutions limited, in principle, by only the wavelength and largest scattering angles recorded. We demonstrate x-ray diffraction imaging with high resolution in all three dimensions, as determined by a quantitative analysis of the reconstructed volume images. These images are retrieved from the three-dimensional diffraction data using no a priori knowledge about the shape or composition of the object, which has never before been demonstrated on a nonperiodic object. We also construct two-dimensional images of thick objects with greatly increased depth of focus (without loss of transverse spatialmore »resolution). These methods can be used to image biological and materials science samples at high resolution with x-ray undulator radiation and establishes the techniques to be used in atomic-resolution ultrafast imaging at x-ray free-electron laser sources.« less

  20. Beam-Target Double Spin Asymmetry ALT in Charged Pion Production from Deep Inelastic Scattering on a Transversely Polarized 3He Target at 1.422

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Meziani, Z -E; Michaels, R; Munoz Camacho, C; Nanda, S; Narayan, A; Nelyubin, V; Norum, B; Oh, Y; Osipenko, M; Parno, D; Peng, J C; Phillips, S K; Posik, M; Puckett, A.J. R; Qiang, Y; Rakhman, A; Ransome, R D; Riordan, S; Saha, A; Sawatzky, B; Schulte, E; Shahinyan, A; Shabestari, M H; Sirca, S; Stepanyan, S; Subedi, R; Sulkosky, V; Tang, L -G; Tobias, A; Urciuoli, G M; Vilardi, I; Wang, K; Wojtsekhowski, B; Yan, X; Yao, H; Ye, Y; Ye, Z; Yuan, L; Zhan, X; Zhang, Y -W; Zhao, B; Zheng, X; Zhu, L; Zhu, X

    2012-01-30

    We report the first measurement of the double-spin asymmetry ALT for charged pion electroproduction in semi-inclusive deep inelastic electron scattering on a transversely polarized 3He target. The kinematics focused on the valence quark region, 0.16 2 2. The corresponding neutron ALT asymmetries were extracted from the measured 3He asymmetries and proton/3He cross section ratios using the effective polarization approximation. These new data probe the transverse momentum dependent parton distribution function gq and therefore provide access to quark spin-orbit correlations. Our results indicate a positive azimuthal asymmetry for ?- production on 3He and the neutron, while our ?+ asymmetries are consistent with zero.

  1. Earth X-ray albedo for cosmic X-ray background radiation in the 1--1000 keV band

    E-Print Network [OSTI]

    E. Churazov; S. Sazonov; R. Sunyaev; M. Revnivtsev

    2008-02-11

    We present calculations of the reflection of the cosmic X-ray background (CXB) by the Earth's atmosphere in the 1--1000 keV energy range. The calculations include Compton scattering and X-ray fluorescent emission and are based on a realistic chemical composition of the atmosphere. Such calculations are relevant for CXB studies using the Earth as an obscuring screen (as was recently done by INTEGRAL). The Earth's reflectivity is further compared with that of the Sun and the Moon -- the two other objects in the Solar system subtending a large solid angle on the sky, as needed for CXB studies.

  2. Differential phase contrast X-ray imaging system and components

    DOE Patents [OSTI]

    Stutman, Daniel; Finkenthal, Michael

    2014-07-01

    A differential phase contrast X-ray imaging system includes an X-ray illumination system, a beam splitter arranged in an optical path of the X-ray illumination system, and a detection system arranged in an optical path to detect X-rays after passing through the beam splitter.

  3. Pyroelectric crystal-based X-ray diffractometer

    E-Print Network [OSTI]

    Fernandes, Louis Edward

    2007-01-01

    We investigate the use of an Amptek Cool-X X-ray Generator for an instructional tool in the physics of x-rays, as well as a source for x-rays for crystal diffraction experiments. The x-ray source is a solid-state two-phase ...

  4. Ultrafast X-Ray Coherent Control

    SciTech Connect (OSTI)

    Reis, David

    2009-05-01

    This main purpose of this grant was to develop the nascent #12;eld of ultrafast x-ray science using accelerator-based sources, and originally developed from an idea that a laser could modulate the di#11;racting properties of a x-ray di#11;racting crystal on a fast enough time scale to switch out in time a shorter slice from the already short x-ray pulses from a synchrotron. The research was carried out primarily at the Advanced Photon Source (APS) sector 7 at Argonne National Laboratory and the Sub-Picosecond Pulse Source (SPPS) at SLAC; in anticipation of the Linac Coherent Light Source (LCLS) x-ray free electron laser that became operational in 2009 at SLAC (all National User Facilities operated by BES). The research centered on the generation, control and measurement of atomic-scale dynamics in atomic, molecular optical and condensed matter systems with temporal and spatial resolution . It helped develop the ultrafast physics, techniques and scienti#12;c case for using the unprecedented characteristics of the LCLS. The project has been very successful with results have been disseminated widely and in top journals, have been well cited in the #12;eld, and have laid the foundation for many experiments being performed on the LCLS, the world's #12;rst hard x-ray free electron laser.

  5. Oscillations During Thermonuclear X-ray Bursts

    E-Print Network [OSTI]

    Tod E. Strohmayer

    2001-01-12

    High amplitude, nearly coherent X-ray brightness oscillations during thermonuclear X-ray bursts were discovered with the Rossi X-ray Timing Explorer (RXTE) in early 1996. Spectral and timing evidence strongly supports the conclusion that these oscillations are caused by rotational modulation of the burst emission and that they reveal the spin frequency of neutron stars in low mass X-ray binaries, a long sought goal of X-ray astronomy. Studies carried out over the past year have led to the discovery of burst oscillations in four new sources, bringing to ten the number with confirmed burst oscillations. I review the status of our knowledge of these oscillations and indicate how they can be used to probe the physics of neutron stars. For a few burst oscillation sources it has been proposed that the strongest and most ubiquitous frequency is actually the first overtone of the spin frequency and hence that two nearly antipodal hot spots are present on the neutron star. This inference has important implications for both the physics of thermonuclear burning as well as the mass - radius relation for neutron stars, so its confirmation is crucial. I discuss recent attempts to confirm this hypothesis for 4U 1636-53, the source for which a signal at the putative fundamental (290 Hz) has been claimed.

  6. X-ray lithography using holographic images

    DOE Patents [OSTI]

    Howells, M.S.; Jacobsen, C.

    1997-03-18

    Methods for forming X-ray images having 0.25 {micro}m minimum line widths on X-ray sensitive material are presented. A holographic image of a desired circuit pattern is projected onto a wafer or other image-receiving substrate to allow recording of the desired image in photoresist material. In one embodiment, the method uses on-axis transmission and provides a high flux X-ray source having modest monochromaticity and coherence requirements. A layer of light-sensitive photoresist material on a wafer with a selected surface is provided to receive the image(s). The hologram has variable optical thickness and variable associated optical phase angle and amplitude attenuation for transmission of the X-rays. A second embodiment uses off-axis holography. The wafer receives the holographic image by grazing incidence reflection from a hologram printed on a flat metal or other highly reflecting surface or substrate. In this second embodiment, an X-ray beam with a high degree of monochromaticity and spatial coherence is required. 15 figs.

  7. In Operando X-ray Diffraction and Transmission X-ray Microscopy of Lithium Sulfur Batteries

    E-Print Network [OSTI]

    Cui, Yi

    In Operando X-ray Diffraction and Transmission X-ray Microscopy of Lithium Sulfur Batteries Johanna Information ABSTRACT: Rechargeable lithium-sulfur (Li-S) batteries hold great potential for high not well understood. In this Article, these changes in Li-S batteries are studied in operando by X

  8. X-ray Point Source Populations Constituting the Galactic Ridge X-ray Emission

    E-Print Network [OSTI]

    Morihana, Kumiko; Yoshida, Tessei; Ebisawa, Ken

    2013-01-01

    Apparently diffuse X-ray emission has been known to exist along the central quarter of the Galactic Plane since the beginning of the X-ray astronomy, which is referred to as the Galactic Ridge X-ray emission (GRXE). Recent deep X-ray observations have shown that numerous X-ray point sources account for a large fraction of the GRXE in the hard band (2-8 keV). However, the nature of these sources is poorly understood. Using the deepest X-ray observations made in the Chandra Bulge Field (Revnivtsev et al., 2009,2011), we present the result of a coherent photometric and spectroscopic analysis of individual X-ray point sources for the purpose of constraining their nature and deriving their fractional contributions to the hard band continuum and Fe K\\alpha line emission of the GRXE. Based on the X-ray color-color diagram, we divided the point sources into three groups: A (hard), B (soft and broad spectrum), and C (soft and peaked spectrum). The group A sources are further decomposed spectrally into thermal and non-...

  9. Boron carbide coatings for neutron detection probed by x-rays, ions, and neutrons to determine thin film quality

    SciTech Connect (OSTI)

    Nowak, G. Störmer, M.; Horstmann, C.; Kampmann, R.; Höche, D.; Lorenz, U.; Müller, M.; Schreyer, A.; Becker, H.-W.; Haese-Seiller, M.; Moulin, J.-F.; Pomm, M.; Randau, C.; Hall-Wilton, R.

    2015-01-21

    Due to the present shortage of {sup 3}He and the associated tremendous increase of its price, the supply of large neutron detection systems with {sup 3}He becomes unaffordable. Alternative neutron detection concepts, therefore, have been invented based on solid {sup 10}B converters. These concepts require development in thin film deposition technique regarding high adhesion, thickness uniformity and chemical purity of the converter coating on large area substrates. We report on the sputter deposition of highly uniform large-area {sup 10}B{sub 4}C coatings of up to 2??m thickness with a thickness deviation below 4% using the Helmholtz-Zentrum Geesthacht large area sputtering system. The {sup 10}B{sub 4}C coatings are x-ray amorphous and highly adhesive to the substrate. Material analysis by means of X-ray-Photoelectron Spectroscopy, Secondary-Ion-Mass-Spectrometry, and Rutherford-Back-Scattering (RBS) revealed low impurities concentration in the coatings. The isotope composition determined by Secondary-Ion-Mass-Spectrometry, RBS, and inelastic nuclear reaction analysis of the converter coatings evidences almost identical {sup 10}B isotope contents in the sputter target and in the deposited coating. Neutron conversion and detection test measurements with variable irradiation geometry of the converter coating demonstrate an average relative quantum efficiency ranging from 65% to 90% for cold neutrons as compared to a black {sup 3}He-monitor. Thus, these converter coatings contribute to the development of {sup 3}He-free prototype detectors based on neutron grazing incidence. Transferring the developed coating process to an industrial scale sputtering system can make alternative {sup 3}He-free converter elements available for large area neutron detection systems.

  10. Elastic and inelastic scattering of 240-MeV {sup 6}Li ions from {sup 40}Ca and {sup 48}Ca and tests of a systematic optical potential

    SciTech Connect (OSTI)

    Krishichayan,; Chen, X.; Lui, Y.-W.; Button, J.; Youngblood, D. H. [Cyclotron Institute, Texas A and M University, College Station, Texas 77843 (United States)

    2010-04-15

    Elastic and inelastic scattering of 240-MeV {sup 6}Li particles from {sup 40}Ca and {sup 48}Ca were measured with the multipole-dipole-multipole spectrometer from 4 deg. <=theta{sub c.m.}<=40 deg. Optical potential parameters were obtained by fitting the elastic-scattering data with the double-folding model using the density-dependent M3Y NN effective interaction and B(E2) and B(E3) values obtained for low-lying 2{sup +} and 3{sup -} states agreed with the adopted values. The results are compared with those obtained using potentials derived from the systematics of potentials previously obtained for {sup 24}Mg, {sup 28}Si, {sup 58}Ni, and {sup 90}Zr. Cross sections for excitation of giant resonances were also calculated with the potentials obtained.

  11. X-ray Clusters at High Redshift

    E-Print Network [OSTI]

    I. M. Gioia

    1997-11-30

    As the largest gravitationally bound structures known, clusters provide clear constraints on the formation of structure and on the composition of the universe. Despite their extreme importance for cosmology the number of clusters at high redshift (z > 0.75) is rather small. There are only a few X-ray emitting examples reported and a handful of optically-selected ones. These clusters can provide stringent constrains on theories of large scale structure formation, if they are massive enough. I will review the status of these distant X-ray selected clusters. These objects are of special importance because their X-ray emission implies that they are massive, comparable to low redshift examples, and their existence is problematic for some theories of structure formation.

  12. A Lack of Radio Emission from Neutron Star Low Mass X-ray Binaries

    E-Print Network [OSTI]

    Michael P. Muno; Tomaso Belloni; Vivek Dhawan; Edward H. Morgan; Ronald A. Remillard; Michael P. Rupen

    2004-11-11

    We report strict upper limits to the radio luminosities of three neutron star low-mass X-ray binaries obtained with the Very Large Array while they were in hard X-ray states as observed with the Rossi X-ray Timing Explorer: 1E 1724-307, 4U 1812-12, and SLX 1735-269. We compare these upper limits to the radio luminosities of several black hole binaries in very similar hard states, and find that the neutron star systems are as faint as or fainter than all of the black hole candidates. The differences in luminosities can partly be attributed to the lower masses of the neutron star systems, which on theoretical and observational grounds are expected to decrease the radio luminosities as M^0.8. However, there still remains a factor of 30 scatter in the radio luminosities of black hole and neutron star X-ray binaries, particularly at X-ray luminosities of a few percent Eddington. We find no obvious differences in the X-ray timing and spectral properties that can be correlated with the radio luminosity. We discuss the implications of these results on current models for the relationship between accretion and jets.

  13. Measurement of the Target-Normal Single-Spin Asymmetry in Deep-Inelastic Scattering from the Reaction 3He{uparrow}(e,e')X

    SciTech Connect (OSTI)

    Katich, Joseph; Qian, Xin; Zhao, Yuxiang; Allada, Kalyan; Aniol, Konrad; Annand, John; Averett, Todd; Benmokhtar, Fatiha; Bertozzi, William; Bradshaw, Elliott; Bosted, Peter; Camsonne, Alexandre; Canan, Mustafa; Cates, Gordon; Chen, Chunhua; Chen, Jian-Ping; Chen, Wei; Chirapatpimol, Khem; Chudakov, Eugene; Cisbani, Evaristo; Cornejo, Juan; Cusanno, Francesco; Dalton, Mark; Deconinck, Wouter; De Jager, Cornelis; De Leo, Raffaele; Deng, Xiaoyan; Deur, Alexandre; Ding, Huaibo; Dolph, Peter; Dutta, Chiranjib; Dutta, Dipangkar; El Fassi, Lamiaa; Frullani, Salvatore; Gao, Haiyan; Garibaldi, Franco; Gaskell, David; Gilad, Gilad; Gilman, Ronald; Glamazdin, Oleksandr; Golge, Serkan; Guo, Lei; Hamilton, David; Hansen, Jens-Ole; Higinbotham, Douglas; Holmstrom, Timothy; Huang, Jijun; Huang, Min; Ibrahim Abdalla, Hassan; Iodice, Mauro; Jin, Ge; Jones, Mark; Kelleher, Aidan; Kim, Wooyoung; Kolarkar, Ameya; Korsch, Wolfgang; LeRose, John; Li, Xiaomei; Li, Y.; Lindgren, Richard; Liyanage, Nilanga; Long, Elena; Lu, Hai-jiang; Margaziotis, Demetrius; Markowitz, Pete; Marrone, Stefano; McNulty, Dustin; Meziani, Zein-Eddine; Michaels, Robert; Moffit, Bryan; Munoz Camacho, Carlos; Nanda, Sirish; Narayan, Amrendra; Nelyubin, Vladimir; Norum, Blaine; Oh, Yoomin; Osipenko, Mikhail; Parno, Diana; Peng, Jen-chieh; Phillips, Sarah; Posik, Matthew; Puckett, Andrew; Qiang, Yi; Rakhman, Abdurahim; Ransome, Ronald; Riordan, Seamus; Saha, Arunava; Sawatzky, Bradley; Schulte, Elaine; Shahinyan, Albert; Hashemi Shabestari, Mitra; Sirca, Simon; Stepanyan, Stepan; Subedi, Ramesh; Sulkosky, Vincent; Tang, Liguang; Tobias, William; Urciuoli, Guido; Vilardi, Ignazio; Wang, Kebin; Wang, Y.; Wojtsekhowski, Bogdan; Yan, X; Yao, Huan; Ye, Yunxiu; Ye, Z.; Yuan, Lulin; Zhan, Xiaohui; Zhang, Yi; Zhang, Y.-W.; Zhao, Bo; Zheng, Xiaochao; Zhu, Lingyan; Zhu, Xiaofeng; Zong, Xing

    2014-07-01

    We report the first measurement of the target single-spin asymmetry in deep-inelastic scattering from the inclusive reaction 3He{uparrow}(e,e')X on a 3He gas target polarized normal to the lepton plane. Assuming time-reversal invariance, this asymmetry is strictly zero in the Born approximation. The experiment, conducted at Jefferson Lab using a 5.89 GeV electron beam, covers a range of 1.72 GeV, which is non-zero at the 2.75sigma level. Theoretical calculations, which assume two-photon exchange with quasi-free quarks, predict a neutron asymmetry of O(10?4) when both photons couple to one quark, and O(10?2) for the photons coupling to different quarks. Our measured asymmetry agrees both in sign and magnitude with the prediction that uses input based on the Sivers transverse momentum distribution obtained from semi-inclusive deep-inelastic scattering.

  14. Structure Functions in Deep Inelastic Lepton Scattering: Data from DOE laboratory experiments as compiled in data reviews by the Durham High Energy Physics Database Group

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Gehrmann, T; Roberts, R. G.; Whalley, M. R.; Durham HEP Database Group

    Gehrmann, Roberts, and Whalley in their 1999 paper, A Compilation of Structure Functions in Deep Inelastic Scattering, published in volume 25 of Journal of Physics G (Nuclear and Particle Physics) note that these data will continue to be relevant to the next generation of hadron colliders. They present data on the unpolarized structure functions F2 and xF3, R D ._L=_T /, the virtual photon asymmetries A1 and A2 and the polarized structure functions g1 and g2, from deep inelastic lepton scattering off protons, deuterium and nuclei. Data are presented in both tabular and graphical format and include predictions based on the MRST98 and CTEQ4 parton distribution functionsö as well. The data gathered from the relevant collaborations at DOE's Fermilab, SLAC, and JLAB are available, and so are data from related collaborations based at CERN and DESY. The Durham High Energy Physics (HEP) Database Group makes these data, extracted from papers and data reviews, available in one place in an easy-to-access format. These data are also include in the Durham HEP Reaction Data Database which can be searched at http://hepdata.cedar.ac.uk/reaction

  15. Measurement of the structure function of the nearly free neutron using spectator tagging in inelastic $^2$H(e, e'p)X scattering with CLAS

    E-Print Network [OSTI]

    S. Tkachenko; N. Baillie; S. E. Kuhn; J. Zhang; J. Arrington; P. Bosted; S. Bültmann; M. E. Christy; D. Dutta; R. Ent; H. Fenker; K. A. Griffioen; M. Ispiryan; N. Kalantarians; C. E. Keppel; W. Melnitchouk; V. Tvaskis; K. P. Adhikari; M. Aghasyan; M. J. Amaryan; S. Anefalos Pereira; H. Avakian; J. Ball; N. A. Baltzell; M. Battaglieri; I. Bedlinskiy; A. S. Biselli; W. J. Briscoe; W. K. Brooks; V. D. Burkert; D. S. Carman; A. Celentano; S. Chandavar; G. Charles; P. L. Cole; M. Contalbrigo; O. Cortes; V. Crede; A. D'Angelo; N. Dashyan; R. De Vita; E. De Sanctis; A. Deur; C. Djalali; G. E. Dodge; D. Doughty; R. Dupre; H. Egiyan; A. El Alaoui; L. El Fassi; L. Elouadrhiri; P. Eugenio; G. Fedotov; J. A. Fleming; B. Garillon; N. Gevorgyan; Y. Ghandilyan; G. P. Gilfoyle; K. L. Giovanetti; F. X. Girod; J. T. Goetz; E. Golovatch; R. W. Gothe; M. Guidal; L. Guo; K. Hafidi; H. Hakobyan; C. Hanretty; N. Harrison; M. Hattawy; K. Hicks; D. Ho; M. Holtrop; C . E. Hyde; Y. Ilieva; D. G. Ireland; B. S. Ishkhanov; H. S. Jo; D. Keller; M. Khandaker; A. Kim; W. Kim; P. M. King; A. Klein; F. J. Klein; S. Koirala; V. Kubarovsky; S. V. Kuleshov; P. Lenisa; S. Lewis; K. Livingston; H. Lu; M. MacCormick; I. J. D. MacGregor; N. Markov; M. Mayer; B. McKinnon; T. Mineeva; M. Mirazita; V. Mokeev; R. A. Montgomery; H. Moutarde; C. Munoz Camacho; P. Nadel-Turonski; S. Niccolai; G. Niculescu; I. Niculescu; M. Osipenko; L. L. Pappalardo; R. Paremuzyan; K. Park; E. Pasyuk; J. J. Phillips; S. Pisano; O. Pogorelko; S. Pozdniakov; J. W. Price; S. Procureur; D. Protopopescu; A. J . R. Puckett; D. Rimal; M. Ripani; A. Rizzo; G. Rosner; P. Rossi; P. Roy; F. Sabatié; D. Schott; R. A. Schumacher; E. Seder; I. Senderovich; Y. G. Sharabian; A. Simonyan; G. D. Smith; D. I. Sober; D. Sokhan; S. Stepanyan; S. S. Stepanyan; S. Strauch; W. Tang; M. Ungaro; A. V. Vlassov; H. Voskanyan; E. Voutier; N. K. Walford; D. Watts; X. Wei; L. B. Weinstein; M. H. Wood; L. Zana; I. Zonta

    2014-10-03

    Much less is known about neutron structure than that of the proton due to the absence of free neutron targets. Neutron information is usually extracted from data on nuclear targets such as deuterium, requiring corrections for nuclear binding and nucleon off-shell effects. These corrections are model dependent and have significant uncertainties, especially for large values of the Bjorken scaling variable x. The Barely Off-shell Nucleon Structure (BONuS) experiment at Jefferson Lab measured the inelastic electron deuteron scattering cross section, tagging spectator protons in coincidence with the scattered electrons. This method reduces nuclear binding uncertainties significantly and has allowed for the first time a (nearly) model independent extraction of the neutron structure function. A novel compact radial time projection chamber was built to detect protons with momentum between 70 and 150 MeV/c. For the extraction of the free neutron structure function $F_{2n}$, spectator protons at backward angle and with momenta below 100 MeV/c were selected, ensuring that the scattering took place on a nearly free neutron. The scattered electrons were detected with Jefferson Lab's CLAS spectrometer. The extracted neutron structure function $F_{2n}$ and its ratio to the deuteron structure function $F_{2d}$ are presented in both the resonance and deep inelastic regions. The dependence of the cross section on the spectator proton momentum and angle is investigated, and tests of the spectator mechanism for different kinematics are performed. Our data set can be used to study neutron resonance excitations, test quark hadron duality in the neutron, develop more precise parametrizations of structure functions, as well as investigate binding effects (including possible mechanisms for the nuclear EMC effect) and provide a first glimpse of the asymptotic behavior of d/u as x goes to 1.

  16. Radiobiological studies using gamma and x rays.

    SciTech Connect (OSTI)

    Potter, Charles Augustus; Longley, Susan W.; Scott, Bobby R. [Lovelace Respiratory Research Institute, Albuquerque, NM; Lin, Yong [Lovelace Respiratory Research Institute, Albuquerque, NM; Wilder, Julie [Lovelace Respiratory Research Institute, Albuquerque, NM; Hutt, Julie A. [Lovelace Respiratory Research Institute, Albuquerque, NM; Padilla, Mabel T. [Lovelace Respiratory Research Institute, Albuquerque, NM; Gott, Katherine M. [Lovelace Respiratory Research Institute, Albuquerque, NM

    2013-02-01

    There are approximately 500 self-shielded research irradiators used in various facilities throughout the U.S. These facilities use radioactive sources containing either 137Cs or 60Co for a variety of biological investigations. A report from the National Academy of Sciences[1] described the issues with security of particular radiation sources and the desire for their replacement. The participants in this effort prepared two peer-reviewed publications to document the results of radiobiological studies performed using photons from 320-kV x rays and 137Cs on cell cultures and mice. The effectiveness of X rays was shown to vary with cell type.

  17. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantity ofkandz-cm11 Outreach Home Room NewsInformationJesse Bergkamp GraduateResidentialLensless Imaging of WholeX-Ray Imaging inX-Ray

  18. Catalog of supersoft X-ray sources

    E-Print Network [OSTI]

    J. Greiner

    2000-05-11

    This catalog comprises an up-to-date (December 1999) list of luminous (>10^36 erg/s), binary supersoft X-ray sources. This electronic version (including the accompannying Web-pages) supersedes the printed version of Greiner (1996).

  19. Multiple wavelength X-ray monochromators

    DOE Patents [OSTI]

    Steinmeyer, P.A.

    1992-11-17

    An improved apparatus and method is provided for separating input x-ray radiation containing first and second x-ray wavelengths into spatially separate first and second output radiation which contain the first and second x-ray wavelengths, respectively. The apparatus includes a crystalline diffractor which includes a first set of parallel crystal planes, where each of the planes is spaced a predetermined first distance from one another. The crystalline diffractor also includes a second set of parallel crystal planes inclined at an angle with respect to the first set of crystal planes where each of the planes of the second set of parallel crystal planes is spaced a predetermined second distance from one another. In one embodiment, the crystalline diffractor is comprised of a single crystal. In a second embodiment, the crystalline diffractor is comprised of a stack of two crystals. In a third embodiment, the crystalline diffractor includes a single crystal that is bent for focusing the separate first and second output x-ray radiation wavelengths into separate focal points. 3 figs.

  20. Multiple wavelength X-ray monochromators

    DOE Patents [OSTI]

    Steinmeyer, Peter A. (Arvada, CO)

    1992-11-17

    An improved apparatus and method is provided for separating input x-ray radiation containing first and second x-ray wavelengths into spatially separate first and second output radiation which contain the first and second x-ray wavelengths, respectively. The apparatus includes a crystalline diffractor which includes a first set of parallel crystal planes, where each of the planes is spaced a predetermined first distance from one another. The crystalline diffractor also includes a second set of parallel crystal planes inclined at an angle with respect to the first set of crystal planes where each of the planes of the second set of parallel crystal planes is spaced a predetermined second distance from one another. In one embodiment, the crystalline diffractor is comprised of a single crystal. In a second embodiment, the crystalline diffractor is comprised of a stack of two crystals. In a third embodiment, the crystalline diffractor includes a single crystal that is bent for focussing the separate first and second output x-ray radiation wavelengths into separate focal points.

  1. SLAC All Access: X-ray Microscope

    ScienceCinema (OSTI)

    Nelson, Johanna; Liu, Yijin

    2014-06-13

    SLAC physicists Johanna Nelson and Yijin Liu give a brief overview of the X-ray microscope at the Stanford Synchrotron Radiation Lightsource (SSRL) that is helping improve rechargeable-battery technology by letting researchers peek into the inner workings of batteries as they operate.

  2. Rise Time Measurement for Ultrafast X-Ray Pulses

    DOE Patents [OSTI]

    Celliers, Peter M.; Weber, Franz A.; Moon, Stephen J.

    2005-04-05

    A pump-probe scheme measures the rise time of ultrafast x-ray pulses. Conventional high speed x-ray diagnostics (x-ray streak cameras, PIN diodes, diamond PCD devices) do not provide sufficient time resolution to resolve rise times of x-ray pulses on the order of 50 fs or less as they are being produced by modern fast x-ray sources. Here, we are describing a pump-probe technique that can be employed to measure events where detector resolution is insufficient to resolve the event. The scheme utilizes a diamond plate as an x-ray transducer and a p-polarized probe beam.

  3. FROM X-RAY DIPS TO ECLIPSE: WITNESSING DISK REFORMATION IN THE RECURRENT NOVA U Sco

    SciTech Connect (OSTI)

    Ness, J.-U.; Talavera, A.; Gonzalez-Riestra, R. [XMM-Newton Science Operations Centre, ESA, P.O. Box 78, 28691 Villanueva de la Canada, Madrid (Spain); Schaefer, B. E. [Department of Physics and Astronomy, Louisiana State University, Baton Rouge, LA 70803 (United States); Dobrotka, A. [Department of Physics, Institute of Materials Science, Faculty of Materials Science and Technology, Slovak University of Technology, Jana Bottu 25, 91724 Trnava (Slovakia); Sadowski, A. [N. Copernicus Astronomical Center, Polish Academy of Sciences, Bartycka 18, 00-716 Warszawa (Poland); Drake, J. J.; Barnard, R. [Harvard-Smithsonian Center for Astrophysics, 60 Garden Street, Cambridge, MA 02138 (United States); Page, K. L. [Department of Physics and Astronomy, University of Leicester, Leicester LE1 7RH (United Kingdom); Hernanz, M. [Institut de Ciencies de l'Espai (CSIC-IEEC), Campus UAB, Facultat de Ciencies, C5 parell 2on, 08193 Bellaterra (Barcelona) (Spain); Sala, G. [Departament Fisica i Enginyeria Nuclear, EUETIB (UPC-IEEC), Comte d'Urgell 187, 08036 Barcelona (Spain); Starrfield, S., E-mail: juness@sciops.esa.int [School of Earth and Space Exploration, Arizona State University, Tempe, AZ 85287-1404 (United States)

    2012-01-20

    The tenth recorded outburst of the recurrent eclipsing nova U Sco was observed simultaneously in X-ray, UV, and optical by XMM-Newton on days 22.9 and 34.9 after the outburst. Two full passages of the companion in front of the nova ejecta were observed, as was the reformation of the accretion disk. On day 22.9, we observed smooth eclipses in UV and optical but deep dips in the X-ray light curve that disappeared by day 34.9, yielding clean eclipses in all bands. X-ray dips can be caused by clumpy absorbing material that intersects the line of sight while moving along highly elliptical trajectories. Cold material from the companion could explain the absence of dips in UV and optical light. The disappearance of X-ray dips before day 34.9 implies significant progress in the formation of the disk. The X-ray spectra contain photospheric continuum emission plus strong emission lines, but no clear absorption lines. Both continuum and emission lines in the X-ray spectra indicate a temperature increase from day 22.9 to day 34.9. We find clear evidence in the spectra and light curves for Thompson scattering of the photospheric emission from the white dwarf. Photospheric absorption lines can be smeared out during scattering in a plasma of fast electrons. We also find spectral signatures of resonant line scattering that lead to the observation of the strong emission lines. Their dominance could be a general phenomenon in high-inclination systems such as Cal 87.

  4. X-ray imaging crystal spectrometer for extended X-ray sources

    DOE Patents [OSTI]

    Bitter, Manfred L. (Princeton, NJ); Fraenkel, Ben (Jerusalem, IL); Gorman, James L. (Bordentown, NJ); Hill, Kenneth W. (Lawrenceville, NJ); Roquemore, A. Lane (Cranbury, NJ); Stodiek, Wolfgang (Princeton, NJ); von Goeler, Schweickhard E. (Princeton, NJ)

    2001-01-01

    Spherically or toroidally curved, double focusing crystals are used in a spectrometer for X-ray diagnostics of an extended X-ray source such as a hot plasma produced in a tokomak fusion experiment to provide spatially and temporally resolved data on plasma parameters using the imaging properties for Bragg angles near 45. For a Bragg angle of 45.degree., the spherical crystal focuses a bundle of near parallel X-rays (the cross section of which is determined by the cross section of the crystal) from the plasma to a point on a detector, with parallel rays inclined to the main plain of diffraction focused to different points on the detector. Thus, it is possible to radially image the plasma X-ray emission in different wavelengths simultaneously with a single crystal.

  5. X-ray Diffraction of Photonic Colloidal Single Crystals Willem L. Vos,*, Mischa Megens, Carlos M. van Kats,, and Peter Bosecke,|

    E-Print Network [OSTI]

    Vos, Willem L.

    X-ray Diffraction of Photonic Colloidal Single Crystals Willem L. Vos,*, Mischa Megens, Carlos M of Bragg peaks of photonic colloidal single crystals by synchrotron small angle X-ray scattering (SAXS). We find that charge-stabilized colloids form face-centered cubic crystals at all densities up to 60 vol

  6. X-RAY POINT-SOURCE POPULATIONS CONSTITUTING THE GALACTIC RIDGE X-RAY EMISSION

    SciTech Connect (OSTI)

    Morihana, Kumiko [Institute of Physical and Chemical Research (RIKEN), 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan)] [Institute of Physical and Chemical Research (RIKEN), 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Tsujimoto, Masahiro; Ebisawa, Ken [Japan Aerospace Exploration Agency, Institute of Space and Astronautical Science, 3-1-1 Yoshino-dai, Chuo-ku, Sagamihara, Kanagawa 252-5210 (Japan)] [Japan Aerospace Exploration Agency, Institute of Space and Astronautical Science, 3-1-1 Yoshino-dai, Chuo-ku, Sagamihara, Kanagawa 252-5210 (Japan); Yoshida, Tessei, E-mail: morihana@crab.riken.jp [National Astronomical Observatory of Japan, 2-21-1, Osawa, Mitaka, Tokyo 181-8588 (Japan)] [National Astronomical Observatory of Japan, 2-21-1, Osawa, Mitaka, Tokyo 181-8588 (Japan)

    2013-03-20

    Apparently diffuse X-ray emission has been known to exist along the central quarter of the Galactic Plane since the beginning of X-ray astronomy; this is referred to as the Galactic Ridge X-ray emission (GRXE). Recent deep X-ray observations have shown that numerous X-ray point sources account for a large fraction of the GRXE in the hard band (2-8 keV). However, the nature of these sources is poorly understood. Using the deepest X-ray observations made in the Chandra bulge field, we present the result of a coherent photometric and spectroscopic analysis of individual X-ray point sources for the purpose of constraining their nature and deriving their fractional contributions to the hard-band continuum and Fe K line emission of the GRXE. Based on the X-ray color-color diagram, we divided the point sources into three groups: A (hard), B (soft and broad spectrum), and C (soft and peaked spectrum). The group A sources are further decomposed spectrally into thermal and non-thermal sources with different fractions in different flux ranges. From their X-ray properties, we speculate that the group A non-thermal sources are mostly active galactic nuclei and the thermal sources are mostly white dwarf (WD) binaries such as magnetic and non-magnetic cataclysmic variables (CVs), pre-CVs, and symbiotic stars, whereas the group B and C sources are X-ray active stars in flares and quiescence, respectively. In the log N-log S curve of the 2-8 keV band, the group A non-thermal sources are dominant above Almost-Equal-To 10{sup -14} erg cm{sup -2} s{sup -1}, which is gradually taken over by Galactic sources in the fainter flux ranges. The Fe K{alpha} emission is mostly from the group A thermal (WD binaries) and the group B (X-ray active stars) sources.

  7. An x-ray setup to investigate the atomic order of confined liquids in slit geometry

    SciTech Connect (OSTI)

    Lippmann, M.; Ehnes, A.; Seeck, O. H.

    2014-01-15

    A setup has been designed to investigate thin films of confined liquids with the use of X-ray scattering methods. The confinement is realized between the flat culets of a pair of diamonds by positioning and orienting the lower diamond with nanometer and micro radian accuracy. We routinely achieve gaps between 5 and 50 nm at culet diameters of 200 ?m. With this setup and a micro focused X-ray beam we have investigated the in-plane and the out-off-plane atomic order of benzene with atomic resolution.

  8. The spectra of accretion discs in low-mass X-ray binaries

    E-Print Network [OSTI]

    R. R. Ross; A. C. Fabian

    1995-11-14

    We present self-consistent models for the radiative transfer in Shakura-Sunyaev accretion discs in bright low-mass X-ray binaries (LMXB). Our calculations include the full effects of incoherent Compton scattering and the vertical temperature structure within the disc, as well as the effects of Doppler blurring and gravitational redshift. We find that the observed X-ray spectra are well fit by exponentially cutoff power-law models. The difference between the observed total spectrum and our calculated disc spectrum should reveal the spectrum of the disc/neutron star boundary layer and other emitting regions considered to be present in LMXB.

  9. Logical operations with single x-ray photons via dynamically-controlled nuclear resonances

    E-Print Network [OSTI]

    Jonas Gunst; Christoph H. Keitel; Adriana Pálffy

    2015-06-01

    The implementation of logical operations on polarization-encoded x-rays via resonant light-nucleus interactions is theoretically investigated. We show that by means of resonant scattering off nuclei and fast rotations of the nuclear hyperfine magnetic field to control the polarization of the output photon, single-qubit logical gates can be simulated. A second control qubit may be employed to trigger the magnetic field rotation, thus allowing several implementation choices for a controlled NOT gate for x-ray photons.

  10. Maskelynite formation via solid-state transformation: Evidence of infrared and x-ray anisotropy

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Jaret, Steven J.; Ehm, Lars; Woerner, William R.; Phillips, Brian L.; Nekvasil, Hanna; Wright, Shawn P.; Glotch, Timothy D.

    2015-03-24

    We present optical microscopy, micro-Raman spectroscopy, nuclear magnetic resonance (NMR) spectroscopy, high-energy X-ray total scattering experiments, and micro-Fourier transform infrared (micro-FTIR) spectroscopy on shocked labradorite from the Lonar Crater, India. We show that maskelynite of shock class 2 is structurally more similar to fused glass than to crystalline plagioclase. However, there are slight but significant differences – preservation of original pre-impact igneous zoning, anisotropy at Infrared wavelengths, X-ray anisotropy, and preservation of some intermediate range order – which are all consistent with a solid-state transformation formation of maskelynite.

  11. ASCA Discovery of Diffuse 6.4 keV Emission Near the Sgr C Complex: A New X-ray Reflection Nebula

    E-Print Network [OSTI]

    H. Murakami; K. Koyama; M. Tsujimoto; Y. Maeda; M. Sakano

    2000-12-14

    We present an ASCA discovery of diffuse hard X-ray emission from the Sgr C complex with its peak in the vicinity of the molecular cloud core. The X-ray spectrum is characterized by a strong 6.4-keV line and large absorption. These properties suggest that Sgr C is a new X-ray reflection nebula which emits fluorescent and scattered X-rays via irradiation from an external X-ray source. We found no adequately bright source in the immediate Sgr C vicinity to fully account for the fluorescence. The irradiating source may be the Galactic nucleus Sgr A*, which was brighter in the past than it is now as is suggested from observations of the first X-ray reflection nebula Sgr B2.

  12. X-Ray Diffraction Microscopy of Magnetic Structures

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    X-Ray Diffraction Microscopy of Magnetic Structures Print science brief icon Scientists working at ALS Beamline 12.0.2.2 have demonstrated a new x-ray technique for producing...

  13. ALS X-Rays Shine a New Light on Catalysis

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    times science has used high-brilliance x-rays to look so closely at these reactions. Lead author Dr. David Mueller at the ALS using x-rays to characterize working fuel cells....

  14. Using Light to Control How X Rays Interact with Matter

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Using Light to Control How X Rays Interact with Matter Using Light to Control How X Rays Interact with Matter Print Wednesday, 27 January 2010 00:00 Schemes that use one light...

  15. A World's Top-10 X-ray Crystal Structure

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    A World's Top-10 X-ray Crystal Structure October 7, 2014 Bookmark and Share Philip Coppens An x-ray crystal structure solved by Philip Coppens has been chosen as one of the world's...

  16. Dawn of x-ray nonlinear optics | Stanford Synchrotron Radiation...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Dawn of x-ray nonlinear optics Wednesday, July 8, 2015 - 3:00pm SLAC, Redtail Hawk Conference Room 108A Speaker: David Reis, PULSE Program Description X-ray free electron lasers...

  17. Staff Research Physicist (X-Ray Spectroscopy) | Princeton Plasma...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    position to work on X-ray spectroscopy, atomic physics, X-ray instrumentation, and high energy density physics. Near-term research goals include participating in the design,...

  18. Recent Measurements of the cos(n{phi}{sub h}) Azimuthal Modulations of the Unpolarized Deep Inelastic Scattering Cross-section at HERMES

    SciTech Connect (OSTI)

    Lamb, Rebecca; Giordano, Francesca [University of Illinois (United States)

    2009-12-17

    The cross section for hadron production in deep-inelastic lepton scattering contains azimuthal modulations which can be related to transverse momentum dependent (TMD) distribution and fragmentation functions. The former provide a picture of how the quarks are moving within nucleons. Specifically, the cos{phi}{sub h} and cos2{phi}{sub h} modulations of the unpolarized cross section relate quark spin and quark transverse momentum. These moments have been carefully measured at the HERMES experiment in a fully differential way, as a function of x, y, z, and P{sub hperpendicular} for positive and negative hadrons produced from hydrogen and deuterium targets. These measurements give new access to the flavor dependent TMDs via their charge and target dependence. These data must be compared to comprehensive models to determine which terms contribute significantly to the cos{phi}{sub h} and cos2{phi}{sub h} moments and allow access to the underlying structure functions.

  19. Measurement of pretzelosity asymmetry of charged pion production in Semi-Inclusive Deep Inelastic Scattering on a polarized $^3$He target

    E-Print Network [OSTI]

    Y. Zhang; X. Qian; K. Allada; C. Dutta; J. Huang; J. Katich; Y. Wang; K. Aniol; J. R. M. Annand; T. Averett; F. Benmokhtar; W. Bertozzi; P. C. Bradshaw; P. Bosted; A. Camsonne; M. Canan; G. D. Cates; C. Chen; J. -P. Chen; W. Chen; K. Chirapatpimol; E. Chudakov; E. Cisbani; J. C. Cornejo; F. Cusanno; M. M. Dalton; W. Deconinck; C. W. de Jager; R. De Leo; X. Deng; A. Deur; H. Ding; P. A. M. Dolph; D. Dutta; L. El Fassi; S. Frullani; H. Gao; F. Garibaldi; D. Gaskell; S. Gilad; R. Gilman; O. Glamazdin; S. Golge; L. Guo; D. Hamilton; O. Hansen; D. W. Higinbotham; T. Holmstrom; M. Huang; H. F. Ibrahim; M. Iodice; X. Jiang; G. Jin; M. K. Jones; A. Kelleher; W. Kim; A. Kolarkar; W. Korsch; J. J. LeRose; X. Li; Y. Li; R. Lindgren; N. Liyanage; E. Long; H. -J. Lu; D. J. Margaziotis; P. Markowitz; S. Marrone; D. McNulty; Z. -E. Meziani; R. Michaels; B. Moffit; C. Muñoz Camacho; S. Nanda; A. Narayan; V. Nelyubin; B. Norum; Y. Oh; M. Osipenko; D. Parno; J. C. Peng; S. K. Phillips; M. Posik; A. J. R. Puckett; Y. Qiang; A. Rakhman; R. D. Ransome; S. Riordan; A. Saha; B. Sawatzky; E. Schulte; A. Shahinyan; M. H. Shabestari; S. Sirca; S. Stepanyan; R. Subedi; V. Sulkosky; L. -G. Tang; W. A. Tobias; G. M. Urciuoli; I. Vilardi; K. Wang; B. Wojtsekhowski; X. Yan; H. Yao; Y. Ye; Z. Ye; L. Yuan; X. Zhan; Y. -W. Zhang; B. Zhao; X. Zheng; L. Zhu; X. Zhu; X. Zong

    2013-12-15

    An experiment to measure single-spin asymmetries in semi-inclusive production of charged pions in deep-inelastic scattering on a transversely polarized $^3$He target was performed at Jefferson Lab in the kinematic region of $0.16

  20. Single Spin Asymmetries in Charged Kaon Production from Semi-Inclusive Deep Inelastic Scattering on a Transversely Polarized $^3{\\rm{He}}$ Target

    E-Print Network [OSTI]

    Y. X. Zhao; Y. Wang; K. Allada; K. Aniol; J. R. M. Annand; T. Averett; F. Benmokhtar; W. Bertozzi; P. C. Bradshaw; P. Bosted; A. Camsonne; M. Canan; G. D. Cates; C. Chen; J. -P. Chen; W. Chen; K. Chirapatpimol; E. Chudakov; E. Cisbani; J. C. Cornejo; F. Cusanno; M. M. Dalton; W. Deconinck; C. W. de Jager; R. De Leo; X. Deng; A. Deur; H. Ding; P. A. M. Dolph; C. Dutta; D. Dutta; L. El Fassi; S. Frullani; H. Gao; F. Garibaldi; D. Gaskell; S. Gilad; R. Gilman; O. Glamazdin; S. Golge; L. Guo; D. Hamilton; O. Hansen; D. W. Higinbotham; T. Holmstrom; J. Huang; M. Huang; H. F Ibrahim; M. Iodice; X. Jiang; G. Jin; M. K. Jones; J. Katich; A. Kelleher; W. Kim; A. Kolarkar; W. Korsch; J. J. LeRose; X. Li; Y. Li; R. Lindgren; N. Liyanage; E. Long; H. -J. Lu; D. J. Margaziotis; P. Markowitz; S. Marrone; D. McNulty; Z. -E. Meziani; R. Michaels; B. Moffit; C. Muñoz Camacho; S. Nanda; A. Narayan; V. Nelyubin; B. Norum; Y. Oh; M. Osipenko; D. Parno; J. -C. Peng; S. K. Phillips; M. Posik; A. J. R. Puckett; X. Qian; Y. Qiang; A. Rakhman; R. Ransome; S. Riordan; A. Saha; B. Sawatzky; E. Schulte; A. Shahinyan; M. H. Shabestari; S. Širca; S. Stepanyan; R. Subedi; V. Sulkosky; L. -G. Tang; A. Tobias; G. M. Urciuoli; I. Vilardi; K. Wang; B. Wojtsekhowski; X. Yan; H. Yao; Y. Ye; Z. Ye; L. Yuan; X. Zhan; Y. Zhang; Y. -W. Zhang; B. Zhao; X. Zheng; L. Zhu; X. Zhu; X. Zong

    2014-04-29

    We report the first measurement of target single spin asymmetries of charged kaons produced in semi-inclusive deep inelastic scattering of electrons off a transversely polarized $^3{\\rm{He}}$ target. Both the Collins and Sivers moments, which are related to the nucleon transversity and Sivers distributions, respectively, are extracted over the kinematic range of 0.1$<$$x_{bj}$$<$0.4 for $K^{+}$ and $K^{-}$ production. While the Collins and Sivers moments for $K^{+}$ are consistent with zero within the experimental uncertainties, both moments for $K^{-}$ favor negative values. The Sivers moments are compared to the theoretical prediction from a phenomenological fit to the world data. While the $K^{+}$ Sivers moments are consistent with the prediction, the $K^{-}$ results differ from the prediction at the 2-sigma level.

  1. Level crossings and zero-field splitting in the {Cr8}-cubane spin-cluster studied using inelastic neutron scattering and magnetization

    SciTech Connect (OSTI)

    Vaknin, D.; Garlea, Vasile O; Demmel, F.; Mamontov, Eugene; Nojiri, H; Martin, Catalin; Chiorescu, Irinel; Qiu, Y.; Luban, M.; Kogerler, P.; Fielden, J.; Engelhardt, L; Rainey, C

    2010-01-01

    Inelastic neutron scattering (INS) in variable magnetic field and high-field magnetization measurements in the millikelvin temperature range were performed to gain insight into the low-energy magnetic excitation spectrum and the field-induced level crossings in the molecular spin cluster {Cr8}-cubane. These complementary techniques provide consistent estimates of the lowest level-crossing field. The overall features of the experimental data are explained using an isotropic Heisenberg model, based on three distinct exchange interactions linking the eight CrIII paramagnetic centers (spins s = 3/2), that is supplemented with a relatively large molecular magnetic anisotropy term for the lowest S = 1 multiplet. It is noted that the existence of the anisotropy is clearly evident from the magnetic field dependence of the excitations in the INS measurements, while the magnetization measurements are not sensitive to its effects.

  2. Single spin asymmetries in charged kaon production from semi-inclusive deep inelastic scattering on a transversely polarized He3 target

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Zhao, Y. X.; Wang, Y.; Allada, K.; Aniol, K.; Annand, J. R.M.; Averett, T.; Benmokhtar, F.; Bertozzi, W.; Bradshaw, P. C.; Bosted, P.; et al

    2014-11-03

    We report the first measurement of target single spin asymmetries of charged kaons produced in semi-inclusive deep inelastic scattering of electrons off a transversely polarized 3He target. Both the Collins and Sivers moments, which are related to the nucleon transversity and Sivers distributions, respectively, are extracted over the kinematic range of 0.1 bj+ and K– production. While the Collins and Sivers moments for K+ are consistent with zero within the experimental uncertainties, both moments for K– favor negative values. The Sivers moments are compared to the theoretical prediction from a phenomenological fit to the world data. Whilemore »the K+ Sivers moments are consistent with the prediction, the K– results differ from the prediction at the 2-sigma level.« less

  3. Beam-Target Double Spin Asymmetry ALT in Charged Pion Production from Deep Inelastic Scattering on a Transversely Polarized 3He Target at 1.422

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Meziani, Z -E; Michaels, R; Munoz Camacho, C; Nanda, S; Narayan, A; Nelyubin, V; Norum, B; Oh, Y; Osipenko, M; Parno, D; et al

    2012-01-30

    We report the first measurement of the double-spin asymmetry ALT for charged pion electroproduction in semi-inclusive deep inelastic electron scattering on a transversely polarized 3He target. The kinematics focused on the valence quark region, 0.16 2 2. The corresponding neutron ALT asymmetries were extracted from the measured 3He asymmetries and proton/3He cross section ratios using the effective polarization approximation. These new data probe the transverse momentum dependent parton distribution function gq and therefore provide access to quark spin-orbit correlations. Our results indicate a positive azimuthal asymmetry for ?- production onmore »3He and the neutron, while our ?+ asymmetries are consistent with zero.« less

  4. An X-ray, IR, and Submillimeter Flare of Sagittarius A*

    E-Print Network [OSTI]

    D. P. Marrone; F. K. Baganoff; M. R. Morris; J. M. Moran; A. M. Ghez; S. D. Hornstein; C. D. Dowell; D. J. Munoz; M. W. Bautz; G. R. Ricker; W. N. Brandt; G. P. Garmire; J. R. Lu; K. Matthews; J. -H. Zhao; R. Rao; G. C. Bower

    2008-07-14

    Energetic flares are observed in the Galactic supermassive black hole Sagittarius A* from radio to X-ray wavelengths. On a few occasions, simultaneous flares have been detected in IR and X-ray observations, but clear counterparts at longer wavelengths have not been seen. We present a flare observed over several hours on 2006 July 17 with the Chandra X-Ray Observatory, the Keck II telescope, the Caltech Submillimeter Observatory, and the Submillimeter Array. All telescopes observed strong flare events, but the submillimeter peak is found to occur nearly 100 minutes after the X-ray peak. Submillimeter polarization data show linear polarization in the excess flare emission, increasing from 9% to 17% as the flare passes through its peak, consistent with a transition from optically thick to thin synchrotron emission. The temporal and spectral behavior of the flare require that the energetic electrons responsible for the emission cool faster than expected from their radiative output. This is consistent with adiabatic cooling in an expanding emission region, with X-rays produced through self-Compton scattering, although not consistent with the simplest model of such expansion. We also present a submillimeter flare that followed a bright IR flare on 2005 July 31. Compared to 2006, this event had a larger peak IR flux and similar submillimeter flux, but it lacked measurable X-ray emission. It also showed a shorter delay between the IR and submillimeter peaks. Based on these events we propose a synchrotron and self-Compton model to relate the submillimeter lag and the variable IR/X-ray luminosity ratio.

  5. X-ray mammography with synchrotron radiation

    SciTech Connect (OSTI)

    Burattini, E. (CNR and INFN-Laboratori Nazionali di Frascati, Frascati, Rome (Italy)); Gambaccini, M.; Marziani, M.; Rimondi, O. (Dipartimento di Fisica dell'Universita and Sezione INFN di Ferrara, Ferrara (Italy)); Indovina, P.L. (Dipartimento di Scienze Fisiche dell'Universita and Sezione INFN di Napoli, Naples (Italy)); Pocek, M.; Simonetti, G. (Istituto di Radiologia, Ospedale Sant'Eugenio, Universita di Tor Vergata, Rome (Italy)); Benassi, M.; Tirelli, C. (Istituto Nazionale del Cancro, Regina Elena, Rome (Italy)); Passariello, R. (Cattedra di Radiologia, Universita dell'Aquila, L'Aquila (Italy))

    1992-01-01

    For the first time in the literature, radiographs of breast phantoms were obtained using several monochromatic synchrotron radiation x-ray beams of selected energy in the range from 14 to 26 keV. In addition, after optimization of the photon energy as a function of the phantom thickness, several mammographs were obtained on surgically removed human breast specimens containing cancer nodules. Comparison between radiographs using a conventional x-ray unit and those obtained of the same specimens utilizing synchrotron monochromatic beams clearly shows that higher contrast and better resolution can be achieved with synchrotron radiation. These results demonstrate the possibility of obtaining radiographs of excised human breast tissue containing a greater amount of radiological information using synchrotron radiation.

  6. X-ray radiography for container inspection

    DOE Patents [OSTI]

    Katz, Jonathan I. (Clayton, MO); Morris, Christopher L. (Los Alamos, NM)

    2011-06-07

    Arrangements of X-ray inspection systems are described for inspecting high-z materials in voluminous objects such as containers. Inspection methods may involve generating a radiographic image based on detected attenuation corresponding to a pulsed beams of radiation transmitted through a voluminous object. The pulsed beams of radiation are generated by a high-energy source and transmitted substantially downward along an incident angle, of approximately 1.degree. to 30.degree., to a vertical axis extending through the voluminous object. The generated radiographic image may be analyzed to detect on localized high attenuation representative of high-z materials and to discriminate high-z materials from lower and intermediate-z materials on the basis of the high density and greater attenuation of high-z material for higher energy (3-10 MeV) X-rays, and the compact nature of threatening masses of fissionable materials.

  7. Compact 'diode-based' multi-energy soft x-ray diagnostic for NSTX

    SciTech Connect (OSTI)

    Tritz, K.; Clayton, D. J.; Stutman, D.; Finkenthal, M. [Johns Hopkins University, Baltimore, Maryland 21218 (United States)

    2012-10-15

    A novel and compact, diode-based, multi-energy soft x-ray (ME-SXR) diagnostic has been developed for the National Spherical Tokamak Experiment. The new edge ME-SXR system tested on NSTX consists of a set of vertically stacked diode arrays, each viewing the plasma tangentially through independent pinholes and filters providing an overlapping view of the plasma midplane which allows simultaneous SXR measurements with coarse sub-sampling of the x-ray spectrum. Using computed x-ray spectral emission data, combinations of filters can provide fast (>10 kHz) measurements of changes in the electron temperature and density profiles providing a method to 'fill-in' the gaps of the multi-point Thomson scattering system.

  8. Spectrometer for Hard X-Ray Free Electron Laser Based on Diffraction Focusing

    E-Print Network [OSTI]

    Kohn, V G; Vartanyants, I A

    2012-01-01

    X-ray free electron lasers (XFELs) generate sequences of ultra-short, spatially coherent pulses of x-ray radiation. We propose the diffraction focusing spectrometer (DFS), which is able to measure the whole energy spectrum of the radiation of a single XFEL pulse with an energy resolution of $\\Delta E/E\\approx 2\\times 10^{-6}$. This is much better than for most modern x-ray spectrometers. Such resolution allows one to resolve the fine spectral structure of the XFEL pulse. The effect of diffraction focusing occurs in a single crystal plate due to dynamical scattering, and is similar to focusing in a Pendry lens made from the metamaterial with a negative refraction index. Such a spectrometer is easier to operate than those based on bent crystals. We show that the DFS can be used in a wide energy range from 5 keV to 20 keV.

  9. In Situ X-Ray Probing Reveals Fingerprints of Surface Platinum Oxide

    SciTech Connect (OSTI)

    Friebel, Daniel

    2011-08-24

    In situ x-ray absorption spectroscopy (XAS) at the Pt L{sub 3} edge is a useful probe for Pt-O interactions at polymer electrolyte membrane fuel cell (PEMFC) cathodes. We show that XAS using the high energy resolution fluorescence detection (HERFD) mode, applied to a well-defined monolayer Pt/Rh(111) sample where the bulk penetrating hard x-rays probe only surface Pt atoms, provides a unique sensitivity to structure and chemical bonding at the Pt-electrolyte interface. Ab initio multiple-scattering calculations using the FEFF8 code and complementary extended x-ray absorption fine structure (EXAFS) results indicate that the commonly observed large increase of the white-line at high electrochemical potentials on PEMFC cathodes originates from platinum oxide formation, whereas previously proposed chemisorbed oxygen-containing species merely give rise to subtle spectral changes.

  10. X-rays from Supernova Remnants

    E-Print Network [OSTI]

    B. Aschenbach

    2002-08-28

    A summary of X-ray observations of supernova remnants is presented including the explosion fragment A of the Vela SNR, Tycho, N132D, RX J0852-4622, the Crab Nebula and the 'bulls eye', and SN 1987A, high-lighting the progress made with Chandra and XMM-Newton and touching upon the questions which arise from these observations and which might inspire future research.

  11. The X-ray Telescope of CAST

    E-Print Network [OSTI]

    M. Kuster; H. Bräuninger; S. Cébrian; M. Davenport; C. Elefteriadis; J. Englhauser; H. Fischer; J. Franz; P. Friedrich; R. Hartmann; F. H. Heinsius; D. H. H. Hoffmann; G. Hoffmeister; J. N. Joux; D. Kang; K. Königsmann; R. Kotthaus; T. Papaevangelou; C. Lasseur; A. Lippitsch; G. Lutz; J. Morales; A. Rodríguez; L. Strüder; J. Vogel; K. Zioutas

    2007-05-10

    The Cern Axion Solar Telescope (CAST) is in operation and taking data since 2003. The main objective of the CAST experiment is to search for a hypothetical pseudoscalar boson, the axion, which might be produced in the core of the sun. The basic physics process CAST is based on is the time inverted Primakoff effect, by which an axion can be converted into a detectable photon in an external electromagnetic field. The resulting X-ray photons are expected to be thermally distributed between 1 and 7 keV. The most sensitive detector system of CAST is a pn-CCD detector combined with a Wolter I type X-ray mirror system. With the X-ray telescope of CAST a background reduction of more than 2 orders off magnitude is achieved, such that for the first time the axion photon coupling constant g_agg can be probed beyond the best astrophysical constraints g_agg < 1 x 10^-10 GeV^-1.

  12. Accretion Disk Boundary Layers Around Neutron Stars: X-ray Production in Low-Mass X-ray Binaries

    E-Print Network [OSTI]

    Robert Popham; Rashid Sunyaev

    2000-04-03

    We present solutions for the structure of the boundary layer where the accretion disk meets the neutron star, which is expected to be the dominant source of high-energy radiation in low-mass X-ray binaries which contain weakly magnetized accreting neutron stars. We find that the main portion of the boundary layer gas is hot (> ~10^8 K), low in density, radially and vertically extended, and optically thick to scattering but optically thin to absorption. It will produce large X-ray luminosity by Comptonization. Energy is transported inward by viscosity, concentrating the energy dissipation in the dense, optically thick zone close to the stellar surface. We explore the dependence of the boundary layer structure on the mass accretion rate, the rotation rate of the star, the alpha viscosity parameter and the viscosity prescription. Radiation pressure is the dominant source of pressure in the boundary layer; the flux is close to the Eddington limiting flux even for luminosities well below (~0.01 times) L(Edd). At luminosities near L(Edd), the boundary layer expands radially, and has a radial extent larger than one stellar radius. Based on the temperatures and optical depths which characterize the boundary layer, we expect that Comptonization will produce a power-law spectrum at low source luminosities. At high luminosities, a Planckian spectrum will be produced in the dense region where most of the energy is released, and modified by Comptonization as the radiation propagates outward.

  13. Portable Parallel Beam X-Ray Diffraction System | Department...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    than 50 pounds, and uses about 50 watts of power. The X-Beam uses polycapillary x-ray optics to collect x-rays over a large solid angle from a low-power x-ray source and to form...

  14. Femtosecond laser-electron x-ray source

    DOE Patents [OSTI]

    Hartemann, Frederic V.; Baldis, Hector A.; Barty, Chris P.; Gibson, David J.; Rupp, Bernhard

    2004-04-20

    A femtosecond laser-electron X-ray source. A high-brightness relativistic electron injector produces an electron beam pulse train. A system accelerates the electron beam pulse train. The femtosecond laser-electron X-ray source includes a high intra-cavity power, mode-locked laser and an x-ray optics system.

  15. First Simultaneous NIR/X-ray Detection of a Flare from SgrA*

    E-Print Network [OSTI]

    A. Eckart; F. K. Baganoff; M. Morris; M. W. Bautz; W. N. Brandt; G. P. Garmire; R. Genzel; T. Ott; G. R. Ricker; C. Straubmeier; T. Viehmann; R. Schödel

    2004-06-17

    We report on the first simultaneous near-infrared/X-ray detection of the Sgr A* counterpart which is associated with the massive black hole at the center of the Milky Way. The observations have been carried out using the NACO adaptive optics (AO) instrument at the European Southern Observatory's Very Large Telescope and the ACIS-I instrument aboard the Chandra X-ray Observatory. We also report on quasi-simultaneous observations at a wavelength of 3.4 mm using the Berkeley-Illinois-Maryland Association (BIMA) array. A flare was detected in the X-domain with an excess 2-8 keV luminosity of about 6$\\times10^{33}$ erg/s. A fading flare of Sgr A* with $>$2 times the interim-quiescent flux was also detected at the beginning of the NIR observations, that overlapped with the fading part of the X-ray flare. Compared to 8-9 hours before the NIR/X-ray flare we detected a marginally significant increase in the millimeter flux density of Sgr A* during measurements about 7-9 hours afterwards. We find that the flaring state can be conveniently explained with a synchrotron self-Compton model involving up-scattered sub-millimeter photons from a compact source component, possibly with modest bulk relativistic motion. The size of that component is assumed to be of the order of a few times the Schwarzschild radius. The overall spectral indices $\\alpha_{NIR/X-ray}$ ($S_{\

  16. ASCA Observations of the Sgr B2 Cloud: An X-Ray Reflection Nebula

    E-Print Network [OSTI]

    H. Murakami; K. Koyama; M. Sakano; M. Tsujimoto; Y. Maeda

    1999-08-20

    We present the ASCA results of imaging spectroscopy of the giant molecular cloud Sgr B2. The X-ray spectrum is found to be very peculiar; it exhibits a strong emission line at 6.4 keV, a low energy cutoff below about 4 keV and a pronounced edge-structure at 7.1 keV. The X-ray image is extended and its peak position is shifted from the core of the molecular cloud toward the Galactic center by about 1--2 arcminute. The X-ray spectrum and the morphology are well reproduced by a scenario that X-rays from an external source located in the Galactic center direction are scattered by the molecular cloud Sgr B2, and come into our line of sight. Thus Sgr B2 may be called an X-ray reflection nebula. Possible implications of the Galactic center activity related to this unique source are presented.

  17. Monitoring x-ray beam damage on lipid films by an integrated Brewster angle microscope/x-ray diffractometer

    E-Print Network [OSTI]

    Lee, Ka Yee C.

    Polyunsaturated lipids with conjugated tails are easily dam- aged by x-ray irradiation in the presence of oxygen samples and thin films has been detected since the beginning of x-ray studies. Dam- age to lipid samples

  18. High resolution monochromator for inelastic scattering studies of high energy phonons using undulator radiation at the advanced photon source

    SciTech Connect (OSTI)

    Macrander, A.T.; Schwoerer-Boehning, M.; Abbamonte, P.M.; Hu, M.

    1997-08-01

    A monochromator for use at 13.84 keV with a calculated bandpass of 5.2 meV was designed built, and tested. Tuning was performed by rotating the inner crystal of a pair of nested silicon channel-cut crystals. The inner crystal employs the (884) reflection, and the outer crystal employs a collimating asymmetric (422) reflection (dynamical asymmetry factor, b, equal to {minus}17.5). Tests were done with a double-crystal Si(111) pre-monochromator situated upstream of the high resolution monochromator and a Si(777) backscattering crystal situated downstream. For this optical arrangement an ideal value of 6.3 meV as calculated by x-ray dynamical diffraction theory applies for the FWHM of the convolution of the net monochromator reflectivity function with that of the Si(777) reflection. This calculated value is to be compared to the value of 7.1 meV measured by tuning the high resolution monochromator. Measured efficiencies were less than ideal by a factor of 3.2 to 4.9, where the larger flux reduction factors were found with higher positron storage ring currents.

  19. X-ray studies of concentrated aqueous solutions

    SciTech Connect (OSTI)

    Ludwig, K.F. Jr.; Warburton, W.K.; Fontaine, A.

    1987-07-01

    Concentrated aqueous solutions of three transition metal bromides (ZnBr/sub 2/, CuBr/sub 2/, and NiBr/sub 2/) and an alkali bromide (RbBr) have been studied with differential anomalous scattering (DAS) and extended x-ray absorption fine structure (EXAFS). The aq-ZnBr/sub 2/ solutions exhibit considerable inner-shell ion complexing with the formation of tetrahedral complexes about the Zn/sup 2 +/. In aq-CuBr/sub 2/, the Cu/sup 2 +/ has an octahedral coordination shell. Most of the anions are bound directly to the cations in both solutions. In contrast, there are only a few Ni--Br nearest neighbors in aq-NiBr/sub 2/. Instead, cations and anions share hydrating water molecules. Preliminary data show that any ion complexing in aq-RbBr must be weak. These results are in good agreement with published thermodynamic studies.

  20. Experimental investigation of beam heating in a soft X-ray scanning transmission X-ray microscope

    E-Print Network [OSTI]

    Hitchcock, Adam P.

    Experimental investigation of beam heating in a soft X-ray scanning transmission X-ray microscope and an accuracy of Æ1 C has been fabricated for scanning transmission X-ray microscopes (STXM). Here we describe at temperatures near their respective melting points as a means of checking for possible sample heating caused

  1. The X-ray Halo of G21.5-0.9

    E-Print Network [OSTI]

    R. Bandiera; F. Bocchino

    2003-05-21

    The emission of the plerion G21.5-0.9 appears more extended in X rays than in radio. This is an unexpected result because it would imply that short-lived X-ray electrons may reach distances even larger than radio electrons. Applying an empirical relationship between dust scattering optical depth and photoelectric column density, the measured column density leads to a large optical depth at 1 keV, of about 1. Therefore we investigate the hypothesis that the detected halo be an effect of dust scattering, re-analyzing an Cal/PV XMM-Newton observation of G21.5-0.9 and critically examining it in terms of a dust scattering model. We also present a spectral analysis of a prominent extended feature in the northern sector of the halo.

  2. Virtual Compton scattering and neutral pion electroproduction in the resonance region up to the deep inelastic region at backward angles

    E-Print Network [OSTI]

    Zhou, Z. -L.

    We have made the first measurements of the virtual Compton scattering (VCS) process via the H(e, e'p)? exclusive reaction in the nucleon resonance region, at backward angles. Results are presented for the W-dependence at ...

  3. Apparatus for monitoring X-ray beam alignment

    DOE Patents [OSTI]

    Steinmeyer, P.A.

    1991-10-08

    A self-contained, hand-held apparatus is provided for monitoring alignment of an X-ray beam in an instrument employing an X-ray source. The apparatus includes a transducer assembly containing a photoresistor for providing a range of electrical signals responsive to a range of X-ray beam intensities from the X-ray beam being aligned. A circuit, powered by a 7.5 VDC power supply and containing an audio frequency pulse generator whose frequency varies with the resistance of the photoresistor, is provided for generating a range of audible sounds. A portion of the audible range corresponds to low X-ray beam intensity. Another portion of the audible range corresponds to high X-ray beam intensity. The transducer assembly may include an a photoresistor, a thin layer of X-ray fluorescent material, and a filter layer transparent to X-rays but opaque to visible light. X-rays from the beam undergoing alignment penetrate the filter layer and excite the layer of fluorescent material. The light emitted from the fluorescent material alters the resistance of the photoresistor which is in the electrical circuit including the audio pulse generator and a speaker. In employing the apparatus, the X-ray beam is aligned to a complete alignment by adjusting the X-ray beam to produce an audible sound of the maximum frequency. 2 figures.

  4. HgMn Stars as apparent X-ray emitters

    E-Print Network [OSTI]

    Hubrig, S; Mathys, G

    1998-01-01

    In the ROSAT all-sky survey 11 HgMn stars were detected as soft X-ray emitters (Berghoefer, Schmitt & Cassinelli 1996). Prior to ROSAT, X-ray observations with the Einstein Observatory had suggested that stars in the spectral range B5-A7 are devoid of X-ray emission. Since there is no X-ray emitting mechanism available for these stars (also not for HgMn stars), the usual argument in the case of an X-ray detected star of this spectral type is the existence of an unseen low-mass companion which is responsible for the X-ray emission. The purpose of the present work is to use all available data for our sample of X-ray detected HgMn stars and conclude on the nature of possible companions.

  5. X-Ray Imaging Crystal Spectrometer for Extended X-Ray Sources

    SciTech Connect (OSTI)

    Bitter, Manfred L.; Fraekel, Benjamin; Gorman, James L.; Hill, Kenneth W.; Roquemore, Lane A.; Stodiek, Wolfgang; Goeler, Schweickhard von

    1999-05-01

    Spherically or toroidally curved, double focusing crystals are used in a spectrometer for X-ray diagnostics of an extended X-ray source such as a hot plasma produced in a tokamak fusion experiment to provide spatially and temporally resolved data on plasma parameters such as ion temperature, toroidal and poloidal rotation, electron temperature, impurity ion charge-state distributions, and impurity transport. The imaging properties of these spherically or toroidally curved crystals provide both spectrally and spatially resolved X-ray data from the plasma using only one small spherically or toroidally curved crystal, thus eliminating the requirement for a large array of crystal spectrometers and the need to cross-calibrate the various crystals.

  6. Single/Double-Spin Asymmetry Measurements of Semi-Inclusive Pion Electroproduction on a Transversely Polarized 3He Target through Deep Inelastic Scattering

    SciTech Connect (OSTI)

    Xin Qian

    2012-06-01

    Parton distribution functions, which represent the flavor and spin structure of the nucleon, provide invaluable information in illuminating quantum chromodynamics in the confinement region. Among various processes that measure such parton distribution functions, semi-inclusive deep inelastic scattering is regarded as one of the golden channels to access transverse momentum dependent parton distribution functions, which provide a 3-D view of the nucleon structure in momentum space. The Jefferson Lab experiment E06-010 focuses on measuring the target single and double spin asymmetries in the 3He(e, e'pi+,-)X reaction with a transversely polarized 3He target in Hall A with a 5.89 GeV electron beam. A leading pion and the scattered electron are detected in coincidence by the left High-Resolution Spectrometer at 16{sup o} and the BigBite spectrometer at 30{sup o} beam right, respectively. The kinematic coverage concentrates in the valence quark region, x {approx} 0.1-0.4, at Q2 {approx}1-3 Gev{sub 2}. The Collins and Sivers asymmetries of 3He and neutron are extracted. In this review, an overview of the experiment and the final results are presented. Furthermore, an upcoming 12-GeV program with a large acceptance solenoidal device and the future possibilities at an electron-ion collider are discussed.

  7. Isotropic Detectable X-ray Counterparts to Gravitational Waves from Neutron Star Binary Mergers

    E-Print Network [OSTI]

    Shota Kisaka; Kunihito Ioka; Takashi Nakamura

    2015-07-18

    Neutron star binary mergers are strong sources of gravitational waves (GWs). Promising electromagnetic counterparts are short gamma-ray bursts (GRBs) but the emission is highly collimated. We propose that the scattering of the long-lasting plateau emission in short GRBs by the merger ejecta produces nearly isotropic emission for $\\sim 10^4$ s with flux $10^{-13}-10^{-10}$ erg cm$^{-2}$ s$^{-1}$ at 100 Mpc in X-ray. This is detectable by Swift XRT and wide field X-ray detectors such as ISS-Lobster, Einstein Probe, eROSITA and WF-MAXI, which are desired by the infrared and optical follow-ups to localize and measure the distance to the host galaxy. The scattered X-rays obtain linear polarization, which correlates with the jet direction, X-ray luminosity and GW polarizations. The activity of plateau emission is also a natural energy source of a macronova (or kilonova) detected in short GRB 130603B without the $r$-process radioactivity.

  8. Isotropic Detectable X-ray Counterparts to Gravitational Waves from Neutron Star Binary Mergers

    E-Print Network [OSTI]

    Kisaka, Shota; Nakamura, Takashi

    2015-01-01

    Neutron star binary mergers are strong sources of gravitational waves (GWs). Promising electromagnetic counterparts are short gamma-ray bursts (GRBs) but the emission is highly collimated. We propose that the scattering of the long-lasting plateau emission in short GRBs by the merger ejecta produces nearly isotropic emission for $\\sim 10^4$ s with flux $10^{-10}-10^{-13}$ erg cm$^{-2}$ s$^{-1}$ in X-ray. This is detectable by wide field X-ray detectors such as ISS-Lobster, eROSITA and WF-MAXI, which are desired by the infrared and optical follow-ups to localize and measure the distance to the host galaxy. The scattered X-rays obtain linear polarization, which correlates with the jet direction, X-ray luminosity and GW polarizations. The activity of plateau emission is also a natural energy source of a macronova (or kilonova) detected in short GRB 130603B without the $r$-process radioactivity.

  9. Method and apparatus for enhanced sensitivity filmless medical x-ray imaging, including three-dimensional imaging

    DOE Patents [OSTI]

    Parker, Sherwood (Berkeley, CA)

    1995-01-01

    A filmless X-ray imaging system includes at least one X-ray source, upper and lower collimators, and a solid-state detector array, and can provide three-dimensional imaging capability. The X-ray source plane is distance z.sub.1 above upper collimator plane, distance z.sub.2 above the lower collimator plane, and distance z.sub.3 above the plane of the detector array. The object to be X-rayed is located between the upper and lower collimator planes. The upper and lower collimators and the detector array are moved horizontally with scanning velocities v.sub.1, v.sub.2, v.sub.3 proportional to z.sub.1, z.sub.2 and z.sub.3, respectively. The pattern and size of openings in the collimators, and between detector positions is proportional such that similar triangles are always defined relative to the location of the X-ray source. X-rays that pass through openings in the upper collimator will always pass through corresponding and similar openings in the lower collimator, and thence to a corresponding detector in the underlying detector array. Substantially 100% of the X-rays irradiating the object (and neither absorbed nor scattered) pass through the lower collimator openings and are detected, which promotes enhanced sensitivity. A computer system coordinates repositioning of the collimators and detector array, and X-ray source locations. The computer system can store detector array output, and can associate a known X-ray source location with detector array output data, to provide three-dimensional imaging. Detector output may be viewed instantly, stored digitally, and/or transmitted electronically for image viewing at a remote site.

  10. Method and apparatus for enhanced sensitivity filmless medical x-ray imaging, including three-dimensional imaging

    DOE Patents [OSTI]

    Parker, S.

    1995-10-24

    A filmless X-ray imaging system includes at least one X-ray source, upper and lower collimators, and a solid-state detector array, and can provide three-dimensional imaging capability. The X-ray source plane is distance z{sub 1} above upper collimator plane, distance z{sub 2} above the lower collimator plane, and distance z{sub 3} above the plane of the detector array. The object to be X-rayed is located between the upper and lower collimator planes. The upper and lower collimators and the detector array are moved horizontally with scanning velocities v{sub 1}, v{sub 2}, v{sub 3} proportional to z{sub 1}, z{sub 2} and z{sub 3}, respectively. The pattern and size of openings in the collimators, and between detector positions is proportional such that similar triangles are always defined relative to the location of the X-ray source. X-rays that pass through openings in the upper collimator will always pass through corresponding and similar openings in the lower collimator, and thence to a corresponding detector in the underlying detector array. Substantially 100% of the X-rays irradiating the object (and neither absorbed nor scattered) pass through the lower collimator openings and are detected, which promotes enhanced sensitivity. A computer system coordinates repositioning of the collimators and detector array, and X-ray source locations. The computer system can store detector array output, and can associate a known X-ray source location with detector array output data, to provide three-dimensional imaging. Detector output may be viewed instantly, stored digitally, and/or transmitted electronically for image viewing at a remote site. 5 figs.

  11. X-ray emission properties of galaxies in Abell 3128

    E-Print Network [OSTI]

    Russell J. Smith

    2003-07-15

    We use archival Chandra X-ray Observatory data to investigate X-ray emission from early-type galaxies in the rich z=0.06 cluster Abell 3128. By combining the X-ray count-rates from an input list of optically-selected galaxies, we obtain a statistical detection of X-ray flux, unbiased by X-ray selection limits. Using 87 galaxies with reliable Chandra data, X-ray emission is detected for galaxies down to M_B ~ -19.0, with only an upper limit determined for galaxies at M_B ~ -18.3. The ratio of X-ray to optical luminosities is consistent with recent determinations of the low-mass X-ray binary content of nearby elliptical galaxies. Taken individually, in contrast, we detect significant (3sigma) flux for only six galaxies. Of these, one is a foreground galaxy, while two are optically-faint galaxies with X-ray hardness ratios characteristic of active galactic nuclei. The remaining three detected galaxies are amongst the optically-brightest cluster members, and have softer X-ray spectra. Their X-ray flux is higher than that expected from X-ray binaries, by a factor 2-10; the excess suggests these galaxies have retained their hot gaseous haloes. The source with the highest L_X / L_B ratio is of unusual optical morphology with prominent sharp-edged shells. Notwithstanding these few exceptions, the cluster population overall exhibits X-ray properties consistent with their emission being dominated by X-ray binaries. We conclude that in rich cluster environments, interaction with the ambient intra-cluster medium acts to strip most galaxies of their hot halo gas.

  12. Metrology for the advancement of x-ray optics at the ALS

    E-Print Network [OSTI]

    Goldberg, Kenneth

    2014-01-01

    S. Yuan et al. , X-ray Optics and Instrumentation 2010,in X-ray and Neutron Optics, Springer, Berlin S. G. AlcockX-ray beam metrology and X-ray optic alignment by Hartmann

  13. X-ray Selected Clusters of Galaxies

    E-Print Network [OSTI]

    Isabella M. Gioia

    1996-01-21

    This paper given at the meeting on "Mapping, Measuring and Modelling the Universe" presents three topics: 1) the study of the clusters and groups of galaxies found serendipitously in the North Ecliptic Pole (NEP) region of the ROSAT all-sky survey; 2) the highest redshift clusters found in the EMSS (up to z=0.82) and the cosmological implications of their very existence; 3) the gravitational lensing in the EMSS X-ray selected clusters of galaxies observed by the Hubble Space Telescope.

  14. SMB, X-ray Fluorescence Imaging

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power AdministrationRobust, High-Throughput Analysis of Protein1-0845*RV 14800Small Angle X-Ray

  15. X-Ray Microscopy | Argonne National Laboratory

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power AdministrationRobust,Field-effectWorkingLos Alamos verifies largest single goldWindX-Ray ImagingIn the

  16. X-ray Microscopy and Imaging: FAQs

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power AdministrationRobust,Field-effectWorkingLos Alamos verifies largest single goldWindX-Ray

  17. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantity ofkandz-cm11 Outreach Home Room NewsInformationJesse Bergkamp GraduateResidentialLensless Imaging of WholeX-Ray Imaging in

  18. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantity ofkandz-cm11 Outreach Home Room NewsInformationJesse Bergkamp GraduateResidentialLensless Imaging of WholeX-Ray Imaging

  19. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power Administration would likeUniverseIMPACTThousand CubicResourcelogo and-E C H N I CLensless X-Ray Imaging in

  20. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power Administration would likeUniverseIMPACTThousand CubicResourcelogo and-E C H N I CLensless X-Ray Imaging

  1. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power Administration would likeUniverseIMPACTThousand CubicResourcelogo and-E C H N I CLensless X-Ray ImagingLensless

  2. Lensless X-Ray Imaging in Reflection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Homesum_a_epg0_fpd_mmcf_m.xls" ,"Available from WebQuantityBonneville Power Administration would likeUniverseIMPACTThousand CubicResourcelogo and-E C H N I CLensless X-Ray

  3. A New On-the-Fly Sampling Method for Incoherent Inelastic Thermal Neutron Scattering Data in MCNP6

    SciTech Connect (OSTI)

    Pavlou, Andrew Theodore; Brown, Forrest B.; Ji, Wei

    2014-09-02

    At thermal energies, the scattering of neutrons in a system is complicated by the comparable velocities of the neutron and target, resulting in competing upscattering and downscattering events. The neutron wavelength is also similar in size to the target's interatomic spacing making the scattering process a quantum mechanical problem. Because of the complicated nature of scattering at low energies, the thermal data files in ACE format used in continuous-energy Monte Carlo codes are quite large { on the order of megabytes for a single temperature and material. In this paper, a new storage and sampling method is introduced that is orders of magnitude less in size and is used to sample scattering parameters at any temperature on-the-fly. In addition to the reduction in storage, the need to pre-generate thermal scattering data tables at fine temperatures has been eliminated. This is advantageous for multiphysics simulations which may involve temperatures not known in advance. A new module was written for MCNP6 that bypasses the current S(?,?) table lookup in favor of the new format. The new on-the-fly sampling method was tested for graphite for two benchmark problems at ten temperatures: 1) an eigenvalue test with a fuel compact of uranium oxycarbide fuel homogenized into a graphite matrix, 2) a surface current test with a \\broomstick" problem with a monoenergetic point source. The largest eigenvalue difference was 152pcm for T= 1200K. For the temperatures and incident energies chosen for the broomstick problem, the secondary neutron spectrum showed good agreement with the traditional S(?,?) sampling method. These preliminary results show that sampling thermal scattering data on-the-fly is a viable option to eliminate both the storage burden of keeping thermal data at discrete temperatures and the need to know temperatures before simulation runtime.

  4. A laboratory-based hard x-ray monochromator for high-resolution x-ray emission spectroscopy and x-ray absorption near edge structure measurements

    SciTech Connect (OSTI)

    Seidler, G. T. Mortensen, D. R.; Remesnik, A. J.; Pacold, J. I.; Ball, N. A.; Barry, N.; Styczinski, M.; Hoidn, O. R.

    2014-11-15

    We report the development of a laboratory-based Rowland-circle monochromator that incorporates a low power x-ray (bremsstrahlung) tube source, a spherically bent crystal analyzer, and an energy-resolving solid-state detector. This relatively inexpensive, introductory level instrument achieves 1-eV energy resolution for photon energies of ?5 keV to ?10 keV while also demonstrating a net efficiency previously seen only in laboratory monochromators having much coarser energy resolution. Despite the use of only a compact, air-cooled 10 W x-ray tube, we find count rates for nonresonant x-ray emission spectroscopy comparable to those achieved at monochromatized spectroscopy beamlines at synchrotron light sources. For x-ray absorption near edge structure, the monochromatized flux is small (due to the use of a low-powered x-ray generator) but still useful for routine transmission-mode studies of concentrated samples. These results indicate that upgrading to a standard commercial high-power line-focused x-ray tube or rotating anode x-ray generator would result in monochromatized fluxes of order 10{sup 6}–10{sup 7} photons/s with no loss in energy resolution. This work establishes core technical capabilities for a rejuvenation of laboratory-based hard x-ray spectroscopies that could have special relevance for contemporary research on catalytic or electrical energy storage systems using transition-metal, lanthanide, or noble-metal active species.

  5. Results from the NSTX X-ray Crystal Spectrometer

    SciTech Connect (OSTI)

    M. Bitter; K. Hill; L. Roquemore; P. Beiersdorfer; D. Thorn; Ming Feng Gu

    2003-01-14

    A high-resolution X-ray crystal spectrometer has recently been installed at the National Spherical Torus Experiment to record the satellite spectra of helium-like argon, ArXVII, in the wavelength range from 3.94 to 4.00 {angstrom} for measurements of ion and electron temperatures, and measurements of the ionization equilibrium of argon, which is of interest for studies of ion transport. The instrument presently consists of a spherically bent quartz crystal and a conventional one-dimensional position-sensitive multi-wire proportional counter, but it will soon be upgraded to a new type of X-ray imaging crystal spectrometer by the installation of a large size (10 cm x 30 cm) two-dimensional position-sensitive detector that will allow us to obtain temporally and spatially resolved spectra from an 80 cm high cross-section of the plasma. In its present configuration, the spectrometer has been optimized for high throughput so that it is possible to record spectra with small statistical errors with a time resolution of 10 ms by adding only small, nonperturbing amounts of argon to the plasma. The spectrometer is most valuable for measurements of the ion temperature in the absence of a neutral beam in ohmically heated and radio-frequency heated discharges, when charge exchange recombination spectroscopy does not function. Electron temperature measurements from the satellite-to-resonance line ratios have been important for a quantitative comparison with (and verification of) the Thomson scattering data. The paper will describe the instrumental details of the present and future spectrometer configurations, and present recent experimental results.

  6. Twisted X-rays: incoming waveforms yielding discrete diffraction patterns for helical structures

    E-Print Network [OSTI]

    Friesecke, Gero; Jüstel, Dominik

    2015-01-01

    Conventional X-ray methods use incoming plane waves and result in discrete diffraction patterns when scattered at crystals. Here we find, by a systematic method, incoming waveforms which exhibit discrete diffraction patterns when scattered at helical structures. As examples we present simulated diffraction patterns of carbon nanotubes and tobacco mosaic virus. The new incoming waveforms, which we call twisted waves due to their geometric shape, are found theoretically as closed-form solutions to Maxwell's equations. The theory of the ensuing diffraction patterns is developed in detail. A twisted analogue of the Von Laue condition is seen to hold, with the peak locations encoding the symmetry and the helix parameters, and the peak intensities indicating the electronic structure in the unit cell. If suitable twisted X-ray sources can in the future be realized experimentally, it appears from our mathematical results that they will provide a powerful tool for directly determining the detailed atomic structure of ...

  7. Soft x-ray reduction camera for submicron lithography

    DOE Patents [OSTI]

    Hawryluk, Andrew M. (2708 Rembrandt Pl., Modesto, CA 95356); Seppala, Lynn G. (7911 Mines Rd., Livermore, CA 94550)

    1991-01-01

    Soft x-ray projection lithography can be performed using x-ray optical components and spherical imaging lenses (mirrors), which form an x-ray reduction camera. The x-ray reduction is capable of projecting a 5x demagnified image of a mask onto a resist coated wafer using 4.5 nm radiation. The diffraction limited resolution of this design is about 135 nm with a depth of field of about 2.8 microns and a field of view of 0.2 cm.sup.2. X-ray reflecting masks (patterned x-ray multilayer mirrors) which are fabricated on thick substrates and can be made relatively distortion free are used, with a laser produced plasma for the source. Higher resolution and/or larger areas are possible by varying the optic figures of the components and source characteristics.

  8. Fabrication process for a gradient index x-ray lens

    DOE Patents [OSTI]

    Bionta, Richard M. (Livermore, CA); Makowiecki, Daniel M. (Livermore, CA); Skulina, Kenneth M. (Livermore, CA)

    1995-01-01

    A process for fabricating high efficiency x-ray lenses that operate in the 0.5-4.0 keV region suitable for use in biological imaging, surface science, and x-ray lithography of integrated circuits. The gradient index x-ray optics fabrication process broadly involves co-sputtering multi-layers of film on a wire, followed by slicing and mounting on block, and then ion beam thinning to a thickness determined by periodic testing for efficiency. The process enables the fabrication of transmissive gradient index x-ray optics for the 0.5-4.0 keV energy range. This process allows the fabrication of optical elements for the next generation of imaging and x-ray lithography instruments m the soft x-ray region.

  9. Fabrication process for a gradient index x-ray lens

    DOE Patents [OSTI]

    Bionta, R.M.; Makowiecki, D.M.; Skulina, K.M.

    1995-01-17

    A process is disclosed for fabricating high efficiency x-ray lenses that operate in the 0.5-4.0 keV region suitable for use in biological imaging, surface science, and x-ray lithography of integrated circuits. The gradient index x-ray optics fabrication process broadly involves co-sputtering multi-layers of film on a wire, followed by slicing and mounting on block, and then ion beam thinning to a thickness determined by periodic testing for efficiency. The process enables the fabrication of transmissive gradient index x-ray optics for the 0.5-4.0 keV energy range. This process allows the fabrication of optical elements for the next generation of imaging and x-ray lithography instruments in the soft x-ray region. 13 figures.

  10. Density gradient free electron collisionally excited x-ray laser

    DOE Patents [OSTI]

    Campbell, E.M.; Rosen, M.D.

    1984-11-29

    An operational x-ray laser is provided that amplifies 3p-3s transition x-ray radiation along an approximately linear path. The x-ray laser is driven by a high power optical laser. The driving line focused optical laser beam illuminates a free-standing thin foil that may be associated with a substrate for improved structural integrity. This illumination produces a generally cylindrically shaped plasma having an essentially uniform electron density and temperature, that exists over a long period of time, and provides the x-ray laser gain medium. The x-ray laser may be driven by more than one optical laser beam. The x-ray laser has been successfully demonstrated to function in a series of experimental tests.

  11. Density gradient free electron collisionally excited X-ray laser

    DOE Patents [OSTI]

    Campbell, Edward M. (Pleasanton, CA); Rosen, Mordecai D. (Berkeley, CA)

    1989-01-01

    An operational X-ray laser (30) is provided that amplifies 3p-3s transition X-ray radiation along an approximately linear path. The X-ray laser (30) is driven by a high power optical laser. The driving line focused optical laser beam (32) illuminates a free-standing thin foil (34) that may be associated with a substrate (36) for improved structural integrity. This illumination produces a generally cylindrically shaped plasma having an essentially uniform electron density and temperature, that exists over a long period of time, and provides the X-ray laser gain medium. The X-ray laser (30) may be driven by more than one optical laser beam (32, 44). The X-ray laser (30) has been successfully demonstrated to function in a series of experimental tests.

  12. Dispersive x-ray synchrotron studies of Pt-C multilayers

    SciTech Connect (OSTI)

    Smither, R.K.; Rodricks, B.; Lamelas, F.; Medjahed, D.; Dos Passos, W.; Clarke, R.; Ziegler, E.; Fontaine, A.

    1989-02-01

    We demonstrate the simultaneous acquisition of high-resolution x-ray absorption spectra and scattering data, using a combination of energy-dispersive optics and a two-dimensional CCD detector. Results are presented on the optical constants of Pt and on the reflectivity of a platinum-carbon multilayer at the L/sub III/ absorption edge of Pt. 12 refs., 5 figs.

  13. ISOCAM Photometry of Narrow-Line X-ray Galaxies

    E-Print Network [OSTI]

    J. D. Law-Green; A. Zezas; M. J. Ward; C. Boisson

    1998-12-23

    Mid-infrared photometry of the hosts of Narrow-Line X-ray Galaxies at 6 microns and 12 microns has been attempted with ISOCAM. No conclusive detections have been made. This implies that these are quiescent objects with little or no active star-formation. Neither X-ray binaries nor starburst-driven superwinds are consistent explanations for the X-ray emission in these objects. We conclude that these NLXGs are predominantly AGN-powered.

  14. X-ray transmission movies of spontaneous dynamic events

    SciTech Connect (OSTI)

    Smilowitz, L.; Henson, B. F.; Holmes, M.; Novak, A.; Oschwald, D.; Dolgonos, P.; Qualls, B.

    2014-11-15

    We describe a new x-ray radiographic imaging system which allows for continuous x-ray transmission imaging of spontaneous dynamic events. We demonstrate this method on thermal explosions in three plastic bonded formulations of the energetic material octahydro-1,3,5,7-tetranitro-1,3,5,7-tetrazocine. We describe the x-ray imaging system and triggering developed to enable the continuous imaging of a thermal explosion.

  15. X-ray interferometry with spherically bent crystals (abstract)

    SciTech Connect (OSTI)

    Koch, Jeffrey A.

    2001-01-01

    Recent progress in manufacturing high-quality spherically bent crystals allows highly monochromatic x-ray beams to be produced, and allows efficient x-ray imaging with {mu}m-scale resolution. This article explores some of the constraints for x-ray interferometry utilizing spherically bent crystals and laser-produced plasma sources, and discusses several shearing interferometer concepts that might be experimentally investigated.

  16. Legacy of the X-Ray Laser Program

    SciTech Connect (OSTI)

    Nilsen, J.

    1993-08-06

    The X-Ray Laser Program has evolved from a design effort focusing on developing a Strategic Defense Initiative weapon that protects against Soviet ICBMs to a scientific project that is producing new technologies for industrial and medical research. While the great technical successes and failures of the X-ray laser itself cannot be discussed, this article presents the many significant achievements made as part of the X-ray laser effort that are now being used for other applications at LLNL.

  17. Ultra-short wavelength x-ray system

    DOE Patents [OSTI]

    Umstadter, Donald (Ann Arbor, MI); He, Fei (Ann Arbor, MI); Lau, Yue-Ying (Potomac, MD)

    2008-01-22

    A method and apparatus to generate a beam of coherent light including x-rays or XUV by colliding a high-intensity laser pulse with an electron beam that is accelerated by a synchronized laser pulse. Applications include x-ray and EUV lithography, protein structural analysis, plasma diagnostics, x-ray diffraction, crack analysis, non-destructive testing, surface science and ultrafast science.

  18. Boosting the Light: X-ray Physics in Confinement

    ScienceCinema (OSTI)

    Rhisberger, Ralf [HASYLAB/ DESY

    2010-01-08

    Remarkable effects are observed if light is confined to dimensions comparable to the wavelength of the light. The lifetime of atomic resonances excited by the radiation is strongly reduced in photonic traps, such as cavities or waveguides. Moreover, one observes an anomalous boost of the intensity scattered from the resonant atoms. These phenomena results from the strong enhancement of the photonic density of states in such geometries. Many of these effects are currently being explored in the regime of vsible light due to their relevance for optical information processing. It is thus appealing to study these phenomena also for much shorter wavelengths. This talk illuminates recent experiments where synchrotron x-rays were trapped in planar waveguides to resonantly excite atomos ([57]Fe nuclei_ embedded in them. In fact, one observes that the radiative decay of these excited atoms is strongly accelerated. The temporal acceleration of the decay goes along with a strong boost of the radiation coherently scattered from the confined atmos. This can be exploited to obtain a high signal-to-noise ratio from tiny quantities of material, leading to manifold applications in the investigation of nanostructured materials. One application is the use of ultrathin probe layers to image the internal structure of magnetic layer systems.

  19. X-RAY ECLIPSE DIAGNOSIS OF THE EVOLVING MASS LOSS IN THE RECURRENT NOVA U SCORPII 2010

    SciTech Connect (OSTI)

    Takei, D.; Drake, J. J. [Smithsonian Astrophysical Observatory, 60 Garden Street, Cambridge, MA 02138 (United States); Tsujimoto, M. [Japan Aerospace Exploration Agency, Institute of Space and Astronautical Science, 3-1-1 Yoshino-dai, Chuo-ku, Sagamihara, Kanagawa 252-5210 (Japan); Ness, J.-U. [European Space Agency, XMM-Newton Observatory SOC, SRE-OAX, Apartado 78, E-28691 Villanueva de la Canada, Madrid (Spain); Osborne, J. P. [Department of Physics and Astronomy, University of Leicester, Leicester LE1 7RH (United Kingdom); Starrfield, S. [School of Earth and Space Exploration, Arizona State University, Tempe, AZ 85287-1404 (United States); Kitamoto, S., E-mail: dtakei@head.cfa.harvard.edu [Department of Physics, Rikkyo University, 3-34-1 Nishi-Ikebukuro, Toshima, Tokyo 171-8501 (Japan)

    2013-05-20

    We report the Suzaku detection of the earliest X-ray eclipse seen in the recurrent nova U Scorpii 2010. A target-of-opportunity observation 15 days after the outburst found a 27% {+-} 5% dimming in the 0.2-1.0 keV energy band at the predicted center of an eclipse. In comparison with the X-ray eclipse depths seen at two later epochs by XMM-Newton, the source region shrank by about 10%-20% between days 15 and 35 after the outburst. The X-ray eclipses appear to be deeper than or similar to contemporaneous optical eclipses, suggesting the X-ray and optical source region extents are comparable on day 15. We raise the possibility of the energy dependency in the photon escape regions, and that this would be a result of the supersoft X-ray opacity being higher than the Thomson scattering opacity at the photosphere due to bound-free transitions in abundant metals that are not fully ionized. Assuming a spherically symmetric model, we constrain the mass-loss rate as a function of time. For a ratio of actual to Thomson opacity of 10-100 in supersoft X-rays, we find an ejecta mass of about 10{sup -7}-10{sup -6} M{sub Sun }.

  20. X-ray micromodulated luminescence tomography in dual-cone ...

    E-Print Network [OSTI]

    2014-07-01

    Jul 16, 2014 ... source, a polycapillary lens, and an electron multiplying charge coupled device ... sources generate x-rays by accelerating electrons into high-z.