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1

Evaluating Global Aerosol Models and Aerosol and Water Vapor Properties Near Clouds  

SciTech Connect (OSTI)

The 'Evaluating Global Aerosol Models and Aerosol and Water Vapor Properties Near Clouds' project focused extensively on the analysis and utilization of water vapor and aerosol profiles derived from the ARM Raman lidar at the Southern Great Plains ARM site. A wide range of different tasks were performed during this project, all of which improved quality of the data products derived from the lidar or advanced the understanding of atmospheric processes over the site. These activities included: upgrading the Raman lidar to improve its sensitivity; participating in field experiments to validate the lidar aerosol and water vapor retrievals; using the lidar aerosol profiles to evaluate the accuracy of the vertical distribution of aerosols in global aerosol model simulations; examining the correlation between relative humidity and aerosol extinction, and how these change, due to horizontal distance away from cumulus clouds; inferring boundary layer turbulence structure in convective boundary layers from the high-time-resolution lidar water vapor measurements; retrieving cumulus entrainment rates in boundary layer cumulus clouds; and participating in a field experiment that provided data to help validate both the entrainment rate retrievals and the turbulent profiles derived from lidar observations.

Turner, David, D.; Ferrare, Richard, A.

2011-07-06T23:59:59.000Z

2

Global observations of desert dust and biomass burning aerosols  

E-Print Network [OSTI]

Global observations of desert dust and biomass burning aerosols Martin de Graaf KNMI #12; Outline · Absorbing Aerosol Index - Theory · Absorbing Aerosol Index - Reality · Biomass burning.6 Biomass burning over Angola, 09 Sep. 2004 Absorbing Aerosol Index PMD image #12;biomass burning ocean

Graaf, Martin de

3

Global distribution and climate forcing of marine organic aerosol: 1. Model improvements and evaluation  

SciTech Connect (OSTI)

Marine organic aerosol emissions have been implemented and evaluated within the National Center of Atmospheric Research (NCAR)'s Community Atmosphere Model (CAM5) with the Pacific Northwest National Laboratory's 7-mode Modal Aerosol Module (MAM-7). Emissions of marine primary organic aerosols (POA), phytoplanktonproduced isoprene- and monoterpenes-derived secondary organic aerosols (SOA) and methane sulfonate (MS{sup -}) are shown to affect surface concentrations of organic aerosols in remote marine regions. Global emissions of submicron marine POA is estimated to be 7.9 and 9.4 Tg yr{sup -1}, for the Gantt et al. (2011) and Vignati et al. (2010) emission parameterizations, respectively. Marine sources of SOA and particulate MS{sup -} (containing both sulfur and carbon atoms) contribute an additional 0.2 and 5.1 Tg yr{sup -1}, respectively. Widespread areas over productive waters of the Northern Atlantic, Northern Pacific, and the Southern Ocean show marine-source submicron organic aerosol surface concentrations of 100 ngm{sup -3}, with values up to 400 ngm{sup -3} over biologically productive areas. Comparison of long-term surface observations of water insoluble organic matter (WIOM) with POA concentrations from the two emission parameterizations shows that despite revealed discrepancies (often more than a factor of 2), both Gantt et al. (2011) and Vignati et al. (2010) formulations are able to capture the magnitude of marine organic aerosol concentrations, with the Gantt et al. (2011) parameterization attaining better seasonality. Model simulations show that the mixing state of the marine POA can impact the surface number concentration of cloud condensation nuclei (CCN). The largest increases (up to 20 %) in CCN (at a supersaturation (S) of 0.2 %) number concentration are obtained over biologically productive ocean waters when marine organic aerosol is assumed to be externally mixed with sea-salt. Assuming marine organics are internally-mixed with sea-salt provides diverse results with increases and decreases in the concentration of CCN over different parts of the ocean. The sign of the CCN change due to the addition of marine organics to seasalt aerosol is determined by the relative significance of the increase in mean modal diameter due to addition of mass, and the decrease in particle hygroscopicity due to compositional changes in marine aerosol. Based on emerging evidence for increased CCN concentration over biologically active surface ocean areas/periods, our study suggests that treatment of sea spray in global climate models (GCMs) as an internal mixture of marine organic aerosols and sea-salt will likely lead to an underestimation in CCN number concentration.

Meskhidze, N.; Xu, J.; Gantt, Brett; Zhang, Yang; Nenes, Athanasios; Ghan, Steven J.; Liu, Xiaohong; Easter, Richard C.; Zaveri, Rahul A.

2011-11-23T23:59:59.000Z

4

Production Mechanism, Number Concentration, Size Distribution, Chemical Composition, and Optical Properties of Sea Spray Aerosols Workshop, Summer 2012  

SciTech Connect (OSTI)

The objective of this workshop was to address the most urgent open science questions for improved quantification of sea spray aerosol-radiation-climate interactions. Sea spray emission and its influence on global climate remains one of the most uncertain components of the aerosol-radiation-climate problem, but has received less attention than other aerosol processes (e.g. production of terrestrial secondary organic aerosols). Thus, the special emphasis was placed on the production flux of sea spray aerosol particles, their number concentration and chemical composition and properties.

Meskhidze, Nicholas [NCSU] [NCSU

2013-10-21T23:59:59.000Z

5

ARM - PI Product - Niamey Aerosol Optical Depths  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

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6

Sensitivity of Remote Aerosol Distributions to Representation of Cloud-Aerosol Interactions in a Global Climate Model  

SciTech Connect (OSTI)

Many global aerosol and climate models, including the widely used Community Atmosphere Model version 5 (CAM5), have large biases in predicting aerosols in remote regions such as upper troposphere and high latitudes. In this study, we conduct CAM5 sensitivity simulations to understand the role of key processes associated with aerosol transformation and wet removal affecting the vertical and horizontal long-range transport of aerosols to the remote regions. Improvements are made to processes that are currently not well represented in CAM5, which are guided by surface and aircraft measurements together with results from a multi-scale aerosol-climate model (PNNL-MMF) that explicitly represents convection and aerosol-cloud interactions at cloud-resolving scales. We pay particular attention to black carbon (BC) due to its importance in the Earth system and the availability of measurements. We introduce into CAM5 a new unified scheme for convective transport and aerosol wet removal with explicit aerosol activation above convective cloud base. This new implementation reduces the excessive BC aloft to better simulate observed BC profiles that show decreasing mixing ratios in the mid- to upper-troposphere. After implementing this new unified convective scheme, we examine wet removal of submicron aerosols that occurs primarily through cloud processes. The wet removal depends strongly on the sub-grid scale liquid cloud fraction and the rate of conversion of liquid water to precipitation. These processes lead to very strong wet removal of BC and other aerosols over mid- to high latitudes during winter months. With our improvements, the Arctic BC burden has a10-fold (5-fold) increase in the winter (summer) months, resulting in a much better simulation of the BC seasonal cycle as well. Arctic sulphate and other aerosol species also increase but to a lesser extent. An explicit treatment of BC aging with slower aging assumptions produces an additional 30-fold (5-fold) increase in the Arctic winter (summer) BC burden. This BC aging treatment, however, has minimal effect on other under-predicted species. Interestingly, our modifications to CAM5 that aim at improving prediction of high-latitude and upper tropospheric aerosols also produce much better AOD and AAOD over various other regions globally when compared to multi-year AERONET retrievals. The improved aerosol distributions have impacts on other aspects of CAM5, improving the simulation of global mean liquid water path and cloud forcing.

Wang, Hailong; Easter, Richard C.; Rasch, Philip J.; Wang, Minghuai; Liu, Xiaohong; Ghan, Steven J.; Qian, Yun; Yoon, Jin-Ho; Ma, Po-Lun; Vinoj, V.

2013-06-05T23:59:59.000Z

7

Observations of Secondary Organic Aerosol Production and Soot Aging under Atmospheric Conditions Using a Novel Environmental Aerosol Chamber  

E-Print Network [OSTI]

of the processes leading to SOA production under ambient gaseous and particulate concentrations as well as the impact these aerosol types have on climate is poorly understood. Although the majority of atmospheric aerosols scatter radiation either directly...

Glen, Crystal

2012-02-14T23:59:59.000Z

8

Assessing the Effects of Anthropogenic Aerosols on Pacific Storm Track Using a Multiscale Global Climate Model  

SciTech Connect (OSTI)

Atmospheric aerosols impact weather and global general circulation by modifying cloud and precipitation processes, but the magnitude of cloud adjustment by aerosols remains poorly quantified and represents the largest uncertainty in estimated forcing of climate change. Here we assess the impacts of anthropogenic aerosols on the Pacific storm track using a multi-scale global aerosol-climate model (GCM). Simulations of two aerosol scenarios corresponding to the present day and pre-industrial conditions reveal long-range transport of anthropogenic aerosols across the north Pacific and large resulting changes in the aerosol optical depth, cloud droplet number concentration, and cloud and ice water paths. Shortwave and longwave cloud radiative forcing at the top of atmosphere are changed by - 2.5 and + 1.3 W m-2, respectively, by emission changes from pre-industrial to present day, and an increased cloud-top height indicates invigorated mid-latitude cyclones. The overall increased precipitation and poleward heat transport reflect intensification of the Pacific storm track by anthropogenic aerosols. Hence, this work provides for the first time a global perspective of the impacts of Asian pollution outflows from GCMs. Furthermore, our results suggest that the multi-scale modeling framework is essential in producing the aerosol invigoration effect of deep convective clouds on the global scale.

Wang, Yuan; Wang, Minghuai; Zhang, Renyi; Ghan, Steven J.; Lin, Yun; Hu, Jiaxi; Pan, Bowen; Levy, Misti; Jiang, Jonathan; Molina, Mario J.

2014-05-13T23:59:59.000Z

9

Global observations and spectral characteristics of desert dust and biomass burning aerosols  

E-Print Network [OSTI]

quantity, but a radiation difference in the UV. Its main advantages are its insensitivity to scattering in climate physics today is the effect of aerosols on the global energy budget. The amount and sign of the effect of aerosols on the incoming solar radiation are unknown and produce a large uncertainty

Graaf, Martin de

10

Understanding global secondary organic aerosol amount and size-resolved condensational behavior  

E-Print Network [OSTI]

Understanding global secondary organic aerosol amount and size-resolved condensational behavior and Adams, 2009b) ·Condensation, coagulation, nucleation ·40 size bins (1 nm ­ 10 µm) ·Nucleation rates the aerosol mass distribution. However, recent closure studies with field measurements show that a significant

11

Intercomparison and evaluation of global aerosol microphysical properties among AeroCom models of a range of complexity  

E-Print Network [OSTI]

Many of the next generation of global climate models will include aerosol schemes which explicitly simulate the microphysical processes that determine the particle size distribution. These models enable aerosol optical ...

Ridley, David Andrew

12

Evaluating Global Aerosol Models and Aerosol and Water Vapor Properties Near Clouds  

SciTech Connect (OSTI)

Project goals: (1) Use the routine surface and airborne measurements at the ARM SGP site, and the routine surface measurements at the NSA site, to continue our evaluations of model aerosol simulations; (2) Determine the degree to which the Raman lidar measurements of water vapor and aerosol scattering and extinction can be used to remotely characterize the aerosol humidification factor; (3) Use the high temporal resolution CARL data to examine how aerosol properties vary near clouds; and (4) Use the high temporal resolution CARL and Atmospheric Emitted Radiance Interferometer (AERI) data to quantify entrainment in optically thin continental cumulus clouds.

Richard A. Ferrare; David D. Turner

2011-09-01T23:59:59.000Z

13

FY 2011 Second Quarter: Demonstration of New Aerosol Measurement Verification Testbed for Present-Day Global Aerosol Simulations  

SciTech Connect (OSTI)

The regional-scale Weather Research and Forecasting (WRF) model is being used by a DOE Earth System Modeling (ESM) project titled Improving the Characterization of Clouds, Aerosols and the Cryosphere in Climate Models to evaluate the performance of atmospheric process modules that treat aerosols and aerosol radiative forcing in the Arctic. We are using a regional-scale modeling framework for three reasons: (1) It is easier to produce a useful comparison to observations with a high resolution model; (2) We can compare the behavior of the CAM parameterization suite with some of the more complex and computationally expensive parameterizations used in WRF; (3) we can explore the behavior of this parameterization suite at high resolution. Climate models like the Community Atmosphere Model version 5 (CAM5) being used within the Community Earth System Model (CESM) will not likely be run at mesoscale spatial resolutions (1020 km) until 510 years from now. The performance of the current suite of physics modules in CAM5 at such resolutions is not known, and current computing resources do not permit high-resolution global simulations to be performed routinely. We are taking advantage of two tools recently developed under PNNL Laboratory Directed Research and Development (LDRD) projects for this activity. The first is the Aerosol Modeling Testbed (Fast et al., 2011b), a new computational framework designed to streamline the process of testing and evaluating aerosol process modules over a range of spatial and temporal scales. The second is the CAM5 suite of physics parameterizations that have been ported into WRF so that their performance and scale dependency can be quantified at mesoscale spatial resolutions (Gustafson et al., 2010; with more publications in preparation).

Koch, D

2011-03-20T23:59:59.000Z

14

ARM - Evaluation Product - Organic Aerosol Component VAP  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

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15

ARM - PI Product - Direct Aerosol Forcing Uncertainty  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

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16

Aerosol products from GOME-2 on Metop-A: development and status report  

E-Print Network [OSTI]

of UV-absorbing aerosols. It is mostly sensitive to desert dust aerosols (DDA) and biomass burning, caused by instrument degradation, had to be removed from the GOME-2 AAI. Figure B. GOME-2 AAI versus degradation Instrument degradation is an annoying phenomenon affecting the AAI. Figure F presents the global

Graaf, Martin de

17

Predicted change in global secondary organic aerosol concentrations in response to future climate, emissions, and land use change  

E-Print Network [OSTI]

The sensitivity of secondary organic aerosol (SOA) concentration to changes in climate and emissions is investigated using a coupled global atmosphere-land model driven by the year 2100 IPCC A1B scenario predictions. The ...

Heald, C. L.; Henze, D. K.; Horowitz, L. W.; Feddema, Johannes J.; Lamarque, J. F.; Guenther, A.; Hess, P. G.; Vitt, F.; Seinfeld, J. H.; Goldstein, A. H.; Fung, I.

2008-03-01T23:59:59.000Z

18

Iron Speciation and Mixing in Single Aerosol Particles from the...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

iron from atmospheric aerosol is an essential nutrient that can control oceanic productivity, thereby impacting the global carbon budget and climate. Particles collected on...

19

Evaluating Clouds, Aerosols, and their Interactions in Three Global Climate Models using COSP and Satellite Observations  

SciTech Connect (OSTI)

Accurately representing aerosol-cloud interactions in global climate models is challenging. As parameterizations evolve, it is important to evaluate their performance with appropriate use of observations. In this work we compare aerosols, clouds, and their interactions in three climate models (AM3, CAM5, ModelE) to MODIS satellite observations. Modeled cloud properties were diagnosed using the CFMIP Observations Simulator Package (COSP). Cloud droplet number concentrations (N) were derived using the same algorithm for both satellite-simulated model values and observations. We find that aerosol optical depth tau simulated by models is similar to observations. For N, AM3 and CAM5 capture the observed spatial pattern of higher values in near-coast versus remote ocean regions, though modeled values in general are higher than observed. In contrast, ModelE simulates lower N in most near-coast versus remote regions. Aerosol- cloud interactions were computed as the sensitivity of N to tau for marine liquid clouds off the coasts of South Africa and Eastern Asia where aerosol pollution varies in time. AM3 and CAM5 are in most cases more sensitive than observations, while the sensitivity for ModelE is statistically insignificant. This widely used sensitivity could be subject to misinterpretation due to the confounding influence of meteorology on both aerosols and clouds. A simple framework for assessing the N tau sensitivity at constant meteorology illustrates that observed sensitivity can change from positive to statistically insignificant when including the confounding influence of relative humidity. Satellite simulated values of N were compared to standard model output and found to be higher with a bias of 83 cm-3.

Ban-Weiss, George; Jin, Ling; Bauer, S.; Bennartz, Ralph; Liu, Xiaohong; Zhang, Kai; Ming, Yi; Guo, Huan; Jiang, Jonathan

2014-09-23T23:59:59.000Z

20

Work distribution in global product development organizations  

E-Print Network [OSTI]

The evolution of the internet, digital design tools, and more importantly, increasing access to global markets and workforce, has increased the interest of firms in offshoring their engineering and product development ...

Tripathy, Anshuman

2010-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


21

Aerosol flow reactor production of superconducting ceramic powder  

SciTech Connect (OSTI)

Potential applications and basic studies of superconducting ceramics require the reproducible production of chemically homogeneous, ultrapure powders with controlled particle size distributions. Previous work has mainly examined the use of liquid and solid phase methods for superconducting powder production. In this work, it is shown that carbon-free, submicron powders based on the Y-Ba-Cu-O, La-Sr-Cu-O, Bi-Ca-Sr-Cu-O and Tl-Ca-Ba-Cu-O systems can be produced in a gaseous flow system by reacting aerosol particles containing the nitrate salts of the appropriate metals in flowing oxygen at temperatures of 900 - 1100C. It is also demonstrated that composite Cu/YBa/sub 2/Cu/sub 3/O/sub 7/ wires can be fabricated by thermophoretic deposition of the particles onto the inner surface of a Cu tube hby sintering/annealing.

Kodas, T. (New Mexico Univ., Albuquerque, NM (USA). Dept. of Nuclear Engineering); Engler, E.; Lee, V.; Parkin, L.S. (Research Div., Almaden Research Center, San Jose, CA (US))

1988-01-01T23:59:59.000Z

22

Direct Insertion of MODIS Radiances in a Global Aerosol Transport Model CLARK WEAVER,* ARLINDO DA SILVA, MIAN CHIN,# PAUL GINOUX,@ OLEG DUBOVIK,&,@@  

E-Print Network [OSTI]

is directly inserted into the Goddard Chemistry and Aerosol Radiation Transport model (GOCART), which aerosol radiative forcing in the thermody- namic equation of GCMs, 3) to account for the reduc- tionDirect Insertion of MODIS Radiances in a Global Aerosol Transport Model CLARK WEAVER,* ARLINDO DA

Chin, Mian

23

Global Distribution and Climate Forcing of Marine Organic Aerosol - Part 2: Effects on Cloud Properties and Radiative Forcing  

SciTech Connect (OSTI)

A series of simulations with the Community Atmosphere Model version 5 (CAM5) with a 7-mode Modal Aerosol Model were conducted to assess the changes in cloud microphysical properties and radiative forcing resulting from marine organic aerosols. Model simulations show that the anthropogenic aerosol indirect forcing (AIF) predicted by CAM5 is decreased in absolute magnitude by up to 0.09 Wm{sup -2} (7 %) when marine organic aerosols are included. Changes in the AIF from marine organic aerosols are associated with small global increases in low-level incloud droplet number concentration and liquid water path of 1.3 cm{sup -3} (1.5 %) and 0.22 gm{sup -2} (0.5 %), respectively. Areas especially sensitive to changes in cloud properties due to marine organic aerosol include the Southern Ocean, North Pacific Ocean, and North Atlantic Ocean, all of which are characterized by high marine organic emission rates. As climate models are particularly sensitive to the background aerosol concentration, this small but non-negligible change in the AIF due to marine organic aerosols provides a notable link for ocean-ecosystem marine low-level cloud interactions and may be a candidate for consideration in future earth system models.

Gantt, Brett; Xu, Jun; Meskhidze, N.; Zhang, Yang; Nenes, Athanasios; Ghan, Steven J.; Liu, Xiaohong; Easter, Richard C.; Zaveri, Rahul A.

2012-07-25T23:59:59.000Z

24

Global fish production and climate change  

SciTech Connect (OSTI)

Current global fisheries production of {approx}160 million tons is rising as a result of increases in aquaculture production. A number of climate-related threats to both capture fisheries and aquaculture are identified, but there is low confidence in predictions of future fisheries production because of uncertainty over future global aquatic net primary production and the transfer of this production through the food chain to human consumption. Recent changes in the distribution and productivity of a number of fish species can be ascribed with high confidence to regional climate variability, such as the El Nino-Southern Oscillation. Future production may increase in some high-latitude regions because of warming and decreased ice cover, but the dynamics in low-latitude regions are giverned by different processes, and production may decline as a result of reduced vertical mixing of the water column and, hence, reduced recycling of nutrients. There are strong interactions between the effects of fishing and the effects of climate because fishing reduces the age, size, and geographic diversity of populations and the biodiversity of marine ecosystems, making both more sensitive to additional stresses such as climate change. Inland fisheries are additionally threatened by changes in precipiation and water management. The frequency and intensity of extreme climate events is likely to have a major impact on future fisheries production in both inland and marine systems. Reducing fishing mortality in the majority of fisheries, which are currently fully exploited or overexploited, is the pricipal feasible means of reducing the impacts of climate change.

Brander, K.M. [International Council for the Exploration of the Sea, Copenhagen (Denmark)

2007-12-11T23:59:59.000Z

25

Aerosol Optical Depth Value-Added Product Report  

SciTech Connect (OSTI)

This document describes the process applied to retrieve aerosol optical depth (AOD) from multifilter rotating shadowband radiometers (MFRSR) and normal incidence multifilter radiometers (NIMFR) operated at the ARM Climate Research Facilitys ground-based facilities.

Koontz, A; Hodges, G; Barnard, J; Flynn, C; Michalsky, J

2013-03-17T23:59:59.000Z

26

Intercomparison and Evaluation of Global Aerosol Microphysical Properties among AeroCom Models of a Range of Complexity  

SciTech Connect (OSTI)

Many of the next generation of global climate models will include aerosol schemes which explicitly simulate the microphysical processes that determine the particle size distribution. These models enable aerosol optical properties and cloud condensation nuclei (CCN) concentrations to be determined by fundamental aerosol processes, which should lead to a more physically based simulation of aerosol direct and indirect radiative forcings. This study examines the global variation in particle size distribution simulated by twelve global aerosol microphysics models to quantify model diversity and to identify any common biases against observations. Evaluation against size distribution measurements from a new European network of aerosol supersites shows that the mean model agrees quite well with the observations at many sites on the annual mean, but there are some seasonal biases common to many sites. In particular, at many of these European sites, the accumulation mode number concentration is biased low during winter and Aitken mode concentrations tend to be overestimated in winter and underestimated in summer. At high northern latitudes, the models strongly underpredict Aitken and accumulation particle concentrations compared to the measurements, consistent with previous studies that have highlighted the poor performance of global aerosol models in the Arctic. In the marine boundary layer, the models capture the observed meridional variation in the size distribution, which is dominated by the Aitken mode at high latitudes, with an increasing concentration of accumulation particles with decreasing latitude. Considering vertical profiles, the models reproduce the observed peak in total particle concentrations in the upper troposphere due to new particle formation, although modelled peak concentrations tend to be biased high over Europe. Overall, the results suggest that most global aerosol microphysics models simulate the global variation of the particle size distribution with a good degree of skill, but some models are in poor agreement with the observations. Further work is required to better constrain size-resolved primary and secondary particle number sources, and an improved understanding of nucleation and growth (e.g. the role of nitrate and secondary organics) will improve the fidelity of simulated particle size distributions.

Mann, G. W.; Carslaw, K. S.; Reddington, C. L.; Pringle, K. J.; Schulz, M.; Asmi, A.; Spracklen, D. V.; Ridley, D. A.; Woodhouse, M. T.; Lee, L. A.; Zhang, Kai; Ghan, Steven J.; Easter, Richard C.; Liu, Xiaohong; Stier, P.; Lee, Y. H.; Adams, P. J.; Tost, H.; Lelieveld, J.; Bauer, S.; Tsigaridis, Kostas; van Noije, T.; Strunk, A.; Vignati, E.; Bellouin, N.; Dalvi, M.; Johnson, C. E.; Bergman, T.; Kokkola, H.; Von Salzen, Knut; Yu, Fangqun; Luo, Gan; Petzold, A.; Heintzenberg, J.; Clarke, A. D.; Ogren, J. A.; Gras, J.; Baltensperger, Urs; Kaminski, U.; Jennings, S. G.; O'Dowd, C. D.; Harrison, R. M.; Beddows, D. C.; Kulmala, M.; Viisanen, Y.; Ulevicius, V.; Mihalopoulos, Nikos; Zdimal, V.; Fiebig, M.; Hansson, H. C.; Swietlicki, E.; Henzing, J. S.

2014-05-13T23:59:59.000Z

27

The AeroCom Evaluation and Intercomparison of Organic Aerosol in Global Models  

DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

This paper evaluates the current status of global modeling of the organic aerosol (OA) occurrence in the troposphere and analyzes the differences calculated between models as well as between models and observations. Thirty-one global chemistry/transport and general circulation models have participated in this intercomparison, in the framework of AeroCom phase II. The simulation of OA varies greatly between models in terms of the magnitude of primary emissions, secondary OA (SOA) formation, the number of OA species used (2 to 62), the complexity of OA parameterizations (gas-particle partitioning, chemical aging, multiphase chemistry, aerosol microphysics), and the OA physical, chemical and optical properties. The diversity of the global OA simulation results has increased since earlier AeroCom experiments, mainly due to the increasing complexity of the SOA parameterization in models, and the implementation of new, highly uncertain, OA sources. Diversity of over an order of magnitude exists in the modeled vertical distribution of OA that deserves a dedicated future study. Furthermore, although the OA/OC ratio depends on OA sources and atmospheric processing and is important for model evaluation against OA and OC observations, it is resolved only by few global models. The median global primary OA source strength is 56 Tg a 1 (range 34 - 144 Tg a-1) and the median secondary OA source strength (natural and anthropogenic) is 19 Tg a-1 (range 13-121 Tg a-1). Among the models that take into account the semi-volatile SOA nature, the median source is calculated to be 51 Tg a-1 (range 16-121 Tg a-1), much larger than the median value of the models that calculate SOA in a more simplistic way (19 Tg a-1; range 13-20 Tg a-1, with one model at 37 Tg a-1). The median atmospheric burden of OA is 1.4 Tg (24 models in the range of 0.6-2.0 Tg and 4 between 2.4-3.8 Tg) with a median OA lifetime of 5.4 days (range 3.8-9.6 days). In models that reported both OA and sulfate burdens, the median value of the OA/sulfate burden ratio of is calculated to be 0.77; 13 models calculate a ratio lower than 1, and 9 models higher than 1. For 26 models that reported OA deposition fluxes, the median wet removal is 70 Tg a-1 (range 28-209 Tg a-1), which is on average 85% of the total OA deposition.

Tsigaridis, Kostas; Daskalakis, N.; Kanakidou, M.; Adams, P. J.; Artaxo, Paulo; Bahadur, R.; Balkanski, Y.; Bauer, S.; Bellouin, N.; Benedetti, Angela; Bergman, T.; Berntsen, T.; Beukes, J. P.; Bian, Huisheng; Carslaw, K. S.; Chin, M.; Curci, Gabriele; Diehl, Thomas; Easter, Richard C.; Ghan, Steven J.; Gong, S.; Hodzic, Alma; Hoyle, Christopher R.; Iversen, T.; Jathar, S.; Jimenez, J. L.; Kaiser, J. W.; Kirkevag, A.; Koch, Dorothy; Kokkola, H.; Lee, Y. H.; Lin, G.; Liu, Xiaohong; Luo, Gan; Ma, Xiaoyan; Mann, G. W.; Mihalopoulos, Nikos; Morcrette, J. -J.; Muller, J. F.; Myhre, G.; Myriokefalitakis, S.; Ng, Nga L.; O'Donell, D.; Penner, J. E.; Pozzoli, L.; Pringle, K. J.; Russell, Lynn; Schulz, M.; Sciare, J.; Seland, O.; Shindell, Drew; Sillman, S.; Skeie, R. B.; Spracklen, D. V.; Stavrakou, T.; Steenrod, Stephen D.; Takemura, T.; Tiitta, P.; Tilmes, S.; Tost, H.; van Noije, T.; van Zyl, P. G.; von Salzen, Knut; Yu, Fangqun; Wang, Zaizi; Wang, Zhilli; Zaveri, Rahul A.; Zhang, Hua; Zhang, Kai; Zhang, Qi; Zhang, Xiaoye

2014-10-15T23:59:59.000Z

28

Fission-product aerosol sampling system for LWR experiments in the TREAT reactor  

SciTech Connect (OSTI)

This work summarizes the design and collection characteristics of a fission-product aerosol sampling system that was developed for a series of light water reactor (LWR) source-term experiments under consideration for performance in 1984 at Argonne National Laboratory's TREAT reactor. These tests would be performed using a bundle of four preirradiated, Zircaloy-clad LWR fuel pins. In these tests, fuel pin integrity would be breached under various simulated accident conditions. The aerosol sampling system was designed to efficiently extract and collect these aerosols such that time-averaged aerosol size distributions, number concentrations and mass loadings could be determined accurately for each experiment, using a combination of real-time and time-interval measurements and post-test analytical techniques. The entire system also was designed to be disassembled remotely because of potentially high levels of radioactivity.

Dunn, P.F.

1983-01-01T23:59:59.000Z

29

AERONET: The Aerosol Robotic Network  

DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

AERONET collaboration provides globally distributed observations of spectral aerosol optical Depth (AOD), inversion products, and precipitable water in diverse aerosol regimes. Aerosol optical depth data are computed for three data quality levels: Level 1.0 (unscreened), Level 1.5 (cloud-screened), and Level 2.0 (cloud screened and quality-assured). Inversions, precipitable water, and other AOD-dependent products are derived from these levels and may implement additional quality checks.[Copied from http://aeronet.gsfc.nasa.gov/new_web/system_descriptions.html

30

Effect of Terrestrial and Marine Organic Aerosol on Regional and Global Climate: Model Development, Application, and Verification with Satellite Data  

SciTech Connect (OSTI)

In this DOE project the improvements to parameterization of marine primary organic matter (POM) emissions, hygroscopic properties of marine POM, marine isoprene derived secondary organic aerosol (SOA) emissions, surfactant effects, new cloud droplet activation parameterization have been implemented into Community Atmosphere Model (CAM 5.0), with a seven mode aerosol module from the Pacific Northwest National Laboratory (PNNL)???¢????????s Modal Aerosol Model (MAM7). The effects of marine aerosols derived from sea spray and ocean emitted biogenic volatile organic compounds (BVOCs) on microphysical properties of clouds were explored by conducting 10 year CAM5.0-MAM7 model simulations at a grid resolution 1.9???????°????????2.5???????° with 30 vertical layers. Model-predicted relationship between ocean physical and biological systems and the abundance of CCN in remote marine atmosphere was compared to data from the A-Train satellites (MODIS, CALIPSO, AMSR-E). Model simulations show that on average, primary and secondary organic aerosol emissions from the ocean can yield up to 20% increase in Cloud Condensation Nuclei (CCN) at 0.2% Supersaturation, and up to 5% increases in droplet number concentration of global maritime shallow clouds. Marine organics were treated as internally or externally mixed with sea salt. Changes associated with cloud properties reduced (absolute value) the model-predicted short wave cloud forcing from -1.35 Wm-2 to -0.25 Wm-2. By using different emission scenarios, and droplet activation parameterizations, this study suggests that addition of marine primary aerosols and biologically generated reactive gases makes an important difference in radiative forcing assessments. All baseline and sensitivity simulations for 2001 and 2050 using global-through-urban WRF/Chem (GU-WRF) were completed. The main objective of these simulations was to evaluate the capability of GU-WRF for an accurate representation of the global atmosphere by exploring the most accurate configuration of physics options in GWRF for global scale modeling in 2001 at a horizontal grid resolution of 1???????° x 1???????°. GU-WRF model output was evaluated using observational datasets from a variety of sources including surface based observations (NCDC and BSRN), model reanalysis (NCEP/ NCAR Reanalysis and CMAP), and remotely-sensed data (TRMM) to evaluate the ability of GU-WRF to simulate atmospheric variables at the surface as well as aloft. Explicit treatment of nanoparticles produced from new particle formation in GU-WRF/Chem-MADRID was achieved by expanding particle size sections from 8 to 12 to cover particles with the size range of 1.16 nm to 11.6 ???????µm. Simulations with two different nucleation parameterizations were conducted for August 2002 over a global domain at a 4???????º by 5???????º horizontal resolution. The results are evaluated against field measurement data from the 2002 Aerosol Nucleation and Real Time Characterization Experiment (ANARChE) in Atlanta, Georgia, as well as satellite and reanalysis data. We have also explored the relationship between ???¢????????clean marine???¢??????? aerosol optical properties and ocean surface wind speed using remotely sensed data from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) on board the CALIPSO satellite and the Advanced Microwave Scanning Radiometer (AMSR-E) on board the AQUA satellite. Detailed data analyses

Meskhidze, Nicholas; Zhang, Yang; Kamykowski, Daniel

2012-03-28T23:59:59.000Z

31

Development of an atmospheric aerosol model for studies of global budgets and effects of airborne particulate material  

SciTech Connect (OSTI)

A microphysics-removal Atmospheric Aerosol Model (AAM) is developed for use in General Circulation Models (GCM) to study global budgets and effects of particulate material. In this model the particle population is assumed to be composed of a set of log-normal modes whose time evolution due to microphysical processes is described via prognostic equations for an appropriate number of moments of the particle size distribution. This newly devised technique, by making use of a small number of prognostic equations for the aerosol variables and utilizing optimized numerical procedures, renders the model computationally efficient, hence particularly suitable for use in complex 3D GCMs. Detailed parameterizations of particle coagulation, sedimentation, dry deposition, and wet removal are incorporated into the AAM.

Giorgi, F.

1986-01-01T23:59:59.000Z

32

Global Biofuel Production and Food Security: Implications for Asia Pacific  

E-Print Network [OSTI]

Global Biofuel Production and Food Security: Implications for Asia Pacific 56th AARES Annual Conference Fremantle, Western Australia 7-10 February 2012 William T. Coyle #12;Global Biofuel Production and Food Security: Making the Connection --Past analysis and the evidence about biofuels and spiking

33

Global Forest Products Trade by Ed Pepke, EFI  

E-Print Network [OSTI]

change policies: escalation of wood energy production, consumption and trade 3. Globalization of forest Lacey Act Amendment f. EU renewable (wood) energy policies Forests, Markets, Policy & PracticeGlobal Forest Products Trade by Ed Pepke, EFI Forests, Markets, Policy & Practice Shanghai, China

34

Development of an atmospheric aerosol model for studies of global budgets and effects of airborne particulate material  

SciTech Connect (OSTI)

A microphysics-removal atmospheric aerosol model (AAM) is developed for use in general circulation models (GCMs) to study global budgets and effects of particulate material. In this model the particle population is composed of a set of log-normal modes whose time evolution due to microphysical processes is described via prognostic equations for an appropriate number of moments of the particle-size distribution. Detailed parameterizations of particle coagulation, sedimentation, dry deposition, and wet removal are developed and implemented into the AAM. The AAM is incorporated into a GCM and is applied to two types of studies: (1) characteristics of the particle wet and dry removal processes, and (2) climatic impact of massive particulate injections following a global nuclear war, with emphasis on the sensitivity of the simulated effects to the inclusion of particle microphysics. Results are discussed.

Giorgi, F.

1986-01-01T23:59:59.000Z

35

ARM - PI Product - Aerosol Retrievals from ARM SGP MFRSR Data  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr May JunDatastreamsmmcrcalgovInstrumentsruc Documentation RUC : XDCResearchWarmingMethane BackgroundFacilityOtherCF duringProductsASRC

36

Assessing the effects of anthropogenic aerosols on Pacific storm track using a multiscale global  

E-Print Network [OSTI]

, the aerosols have an indirect effect by serving as cloud condensation nuclei, and their interaction latent heating (6), leading to an enhanced pre- cipitation efficiency (7­12), invigorated convection Satellite Cloud Climatology Project and high-resolution infrared sounder. In addition, a trend of increasing

37

Sensitivity of Tropospheric Chemical Composition to Halogen-Radical Chemistry Using a Fully Coupled Size-Resolved Multiphase Chemistry-Global Climate System: Halogen Distributions, Aerosol Composition, and Sensitivity of Climate-Relevant Gases  

SciTech Connect (OSTI)

Observations and model studies suggest a significant but highly non-linear role for halogens, primarily Cl and Br, in multiphase atmospheric processes relevant to tropospheric chemistry and composition, aerosol evolution, radiative transfer, weather, and climate. The sensitivity of global atmospheric chemistry to the production of marine aerosol and the associated activation and cycling of inorganic Cl and Br was tested using a size-resolved multiphase coupled chemistry/global climate model (National Center for Atmospheric Researchs Community Atmosphere Model (CAM); v3.6.33). Simulation results showed strong meridional and vertical gradients in Cl and Br species. The simulation reproduced most available observations with reasonable confidence permitting the formulation of potential mechanisms for several previously unexplained halogen phenomena including the enrichment of Br- in submicron aerosol, and the presence of a BrO maximum in the polar free troposphere. However, simulated total volatile Br mixing ratios were generally high in the troposphere. Br in the stratosphere was lower than observed due to the lack of long-lived organobromine species in the simulation. Comparing simulations using chemical mechanisms with and without reactive Cl and Br species demonstrated a significant temporal and spatial sensitivity of primary atmospheric oxidants (O3, HOx, NOx), CH4, and non-methane hydrocarbons (NMHCs) to halogen cycling. Simulated O3 and NOx were globally lower (65% and 35%, respectively, less in the planetary boundary layer based on median values) in simulations that included halogens. Globally, little impact was seen in SO2 and non-sea-salt SO42- processing due to halogens. Significant regional differences were evident: The lifetime of nss-SO42- was extended downwind of large sources of SO2. The burden and lifetime of DMS (and its oxidation products) were lower by a factor of 5 in simulations that included halogens, versus those without, leading to a 20% reduction in nss-SO42- in the southern hemisphere planetary boundary layer based on median values.

Long, M.; Keene, W. C.; Easter, Richard C.; Sander, Rolf; Liu, Xiaohong; Kerkweg, A.; Erickson, D.

2014-04-07T23:59:59.000Z

38

Global Patterns of Ecological Productivity and Tropical Forest Biomass  

E-Print Network [OSTI]

those measurements in addition to climate data to construct a suite of empirical models of NPP productivity (NPP) on a global scale and biomass accumulation across thee tropics. Scientists have been model of terrestrial net primary productivity (NPP), and its simplicity and relative accuracy has led

Wisconsin at Madison, University of

39

A Global Volcano Product for Thermal Emission and Effusion Rate  

E-Print Network [OSTI]

for solar reflectance component #12;Hyperion Thermal Product: Basic ­Extract hot pixelsA Global Volcano Product for Thermal Emission and Effusion Rate: Hyperion of these have non-zero thermal signatures Geographical Distribution of Volcano Sensorweb Targets #12

Schaffer, Steven

40

Globally distributed product development : role of complexity in the what, where and how  

E-Print Network [OSTI]

This dissertation presents findings on four elements of the relationship between Global Product Development or Globally distributed Product Development (GPD) and product complexity. I examine this relationship in the context ...

Makumbe, Pedzisayi O

2008-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


41

Secondary organic aerosol from ozone-initiated reactions with terpene-rich household products  

SciTech Connect (OSTI)

We analyzed secondary organic aerosol (SOA) data from a series of small-chamber experiments in which terpene-rich vapors from household products were combined with ozone under conditions analogous to product use indoors. Reagents were introduced into a continuously ventilated 198 L chamber at steady rates. Consistently, at the time of ozone introduction, nucleation occurred exhibiting behavior similar to atmospheric events. The initial nucleation burst and growth was followed by a period in which approximately stable particle levels were established reflecting a balance between new particle formation, condensational growth, and removal by ventilation. Airborne particles were measured with a scanning mobility particle sizer (SMPS, 10 to 400 nm) in every experiment and with an optical particle counter (OPC, 0.1 to 2.0 ?m) in a subset. Parameters for a three-mode lognormal fit to the size distribution at steady state were determined for each experiment. Increasing the supply ozone level increased the steady-state mass concentration and yield of SOA from each product tested. Decreasing the air-exchange rate increased the yield. The steady-state fine-particle mass concentration (PM1.1) ranged from 10 to> 300 mu g m-3 and yields ranged from 5percent to 37percent. Steady-state nucleation rates and SOA mass formation rates were on the order of 10 cm-3 s-1 and 10 mu g m-3 min-1, respectively.

Coleman, Beverly; Coleman, Beverly K.; Lunden, Melissa M.; Destaillats, Hugo; Nazaroff, William W.

2008-01-01T23:59:59.000Z

42

Primary productivity demands of global fishing fleets Reg Watson1,2  

E-Print Network [OSTI]

Primary productivity demands of global fishing fleets Reg Watson1,2 , Dirk Zeller1 & Daniel Pauly1 production driven by solar energy. Primary production required (PPR) esti- mates how much primary production. Pauly. 2013. Primary productivity demands of global fisheries. Fish and Fisheries. #12;Introduction

Pauly, Daniel

43

aerosol ratio program: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

contribute a major portion of atmospheric aerosol mass loading 5. The estimated global annual Liou, K. N. 2 Studying Clouds and Aerosols with Lidar Depolarization Ratio and...

44

5, 79658026, 2005 Simulating aerosol  

E-Print Network [OSTI]

composition, number concentration, and size distribution of the global submicrometer aerosol. The present, coagulation, condensation, nucleation of sulfuric acid vapor, aerosol chemistry, cloud processing, and sizeACPD 5, 7965­8026, 2005 Simulating aerosol microphysics with ECHAM/MADE A. Lauer et al. Title Page

Paris-Sud XI, Université de

45

Globally Distributed Engineering Teams in Computational Fluid Dynamics and in Product Development  

E-Print Network [OSTI]

, experimental research on idea generation methods used in globally distributed teams during the conceptual design phase of the product development process is presented. An experimental study simulating the global distribution of a three person Computational...

Schmidt, Susanne R.

2010-10-12T23:59:59.000Z

46

Potential Direct and Indirect Effects of Global Cellulosic Biofuel Production on Greenhouse  

E-Print Network [OSTI]

Potential Direct and Indirect Effects of Global Cellulosic Biofuel Production on Greenhouse Gas on recycled paper #12;1 Potential Direct and Indirect Effects of Global Cellulosic Biofuel Production. Melillo*, John M. Reilly§ , and Sergey Paltsev§ Abstract The production of cellulosic biofuels may have

47

DO AEROSOLS CHANGE CLOUD COVER AND AFFECT CLIMATE?  

E-Print Network [OSTI]

BALANCE Global and annual average energy fluxes in watts per square meter Schwartz, 1996, modified from;AEROSOL INFLUENCES ON CLIMATE AND CLIMATE CHANGE #12;DMS #12;AEROSOL IN MEXICO CITY BASIN #12;AEROSOL IN MEXICO CITY BASIN Light scattering by aerosols decreases absorption of solar radiation. #12;AEROSOLS

Schwartz, Stephen E.

48

Supply Chain Networks with Global Outsourcing and Quick-Response Production Under Demand and Cost Uncertainty  

E-Print Network [OSTI]

Supply Chain Networks with Global Outsourcing and Quick-Response Production Under Demand and Cost framework for supply chain networks with global outsourcing and quick-response production under demand University of Massachusetts Amherst, Massachusetts 01003 May 2011; revised September 2011 Annals

Nagurney, Anna

49

Supply Chain Networks with Global Outsourcing and Quick-Response Production Under Demand and Cost Uncertainty  

E-Print Network [OSTI]

Supply Chain Networks with Global Outsourcing and Quick-Response Production Under Demand and Cost University of Massachusetts Amherst, Massachusetts 01003 May 2011 Abstract This paper develops a modeling and computational framework for supply chain networks with global outsourcing and quick-response production under

Nagurney, Anna

50

aerosols | EMSL  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

aerosols aerosols Leads No leads are available at this time. Magnesium behavior and structural defects in Mg+ ion implanted silicon carbide. Abstract: As a candidate material for...

51

Secondary organic aerosol from ozone-initiated reactions with terpene-rich household products  

E-Print Network [OSTI]

C.J. , 2004. Cleaning products and air fresheners: exposurepollutants from cleaning product and air freshener use in2006b. Cleaning products and air fresheners: emissions and

Coleman, Beverly K.

2008-01-01T23:59:59.000Z

52

Advanced skills required for engineering leaders in global product development  

E-Print Network [OSTI]

Observations from first hand experience on the Boeing 787 Program during development of perhaps the most important and exciting new commercial airplane in recent history has identified opportunities to enhance the global ...

Ayubi, Harry H

2011-01-01T23:59:59.000Z

53

Knowledge production at the global frontier : the case of China  

E-Print Network [OSTI]

China is increasingly seen as a participant in the global knowledge economy, with recent studies have highlighted the rising number of scientists and engineers educated in Chinese institutions of higher education, and the ...

Fensterheim, Devin Robert

2009-01-01T23:59:59.000Z

54

aerosols iii morphologic: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Sciences Websites Summary: of aerosols. Keywords: metal waste recycling; aerosols; fire hazard; explosion hazard. 1. OVERVIEW ProductsRisks generated by the treatment of...

55

aerosol particles emitted: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

aerosols scatter and absorb solar, estimates of the impact of aerosols on visibility, the solar radiation balance, and crop production is presented. 1. INTRODUCTION The attenuation...

56

Aerosol engineering: design and stability of aerosol reactors  

SciTech Connect (OSTI)

A theoretical study of the performance of aerosol reactors is presented. The goals of this study are (1) to identify the appropriate reactor types (batch, CSTR, and tubular) for production of aerosol with specific properties (for example, uniform size particles, high aerosol surface area, etc.) and (2) to investigate the effect of various process parameters on product aerosol characteristics and on the stability of operation of aerosol reactors. In all the reactors considered, the aerosol dynamics were detemined by chemical reaction, nucleation, and aerosol growth in the free molecule regime in the absence of coagulation at isothermal conditions. Formulation of the aerosol dynamics in terms of moments of the aerosol size distribution facilitated the numerical solution of the resulting systems of ordinary or partial differential equations. The stability characteristics of a continuous stirred tank aerosol reactor (CSTAR) were investigated since experimental data in the literature indicate that under certain conditions this reactor exhibits oscillatory behavior with respect to product aerosol concentration and size distribution.

Pratsinis, S.E.

1985-01-01T23:59:59.000Z

57

6, 93519388, 2006 Aerosol-cloud  

E-Print Network [OSTI]

ACPD 6, 9351­9388, 2006 Aerosol-cloud interaction inferred from MODIS and models G. Myhre et al Chemistry and Physics Discussions Aerosol-cloud interaction inferred from MODIS satellite data and global 6, 9351­9388, 2006 Aerosol-cloud interaction inferred from MODIS and models G. Myhre et al. Title

Paris-Sud XI, Université de

58

The importance of aerosol composition and mixing state on predicted CCN concentration and the variation of the importance with atmospheric processing of aerosol  

SciTech Connect (OSTI)

The influences of atmospheric aerosols on cloud properties (i.e., aerosol indirect effects) strongly depend on the aerosol CCN concentrations, which can be effectively predicted from detailed aerosol size distribution, mixing state, and chemical composition using Khler theory. However, atmospheric aerosols are complex and heterogeneous mixtures of a large number of species that cannot be individually simulated in global or regional models due to computational constraints. Furthermore, the thermodynamic properties or even the molecular identities of many organic species present in ambient aerosols are often not known to predict their cloud-activation behavior using Khler theory. As a result, simplified presentations of aerosol composition and mixing state are necessary for large-scale models. In this study, aerosol microphysics, CCN concentrations, and chemical composition measured at the T0 urban super-site in Mexico City during MILAGRO are analyzed. During the campaign in March 2006, aerosol size distribution and composition often showed strong diurnal variation as a result of both primary emissions and aging of aerosols through coagulation and local photochemical production of secondary aerosol species. The submicron aerosol composition was ~1/2 organic species. Closure analysis is first carried out by comparing CCN concentrations calculated from the measured aerosol size distribution, mixing state, and chemical composition using extended Khler theory to concurrent CCN measurements at five supersaturations ranging from 0.11% to 0.35%. The closure agreement and its diurnal variation are studied. CCN concentrations are also derived using various simplifications of the measured aerosol mixing state and chemical composition. The biases associated with these simplifications are compared for different supersaturations, and the variation of the biases is examined as a function of aerosol age. The results show that the simplification of internally mixed, size-independent particle composition leads to substantial overestimation of CCN concentration for freshly emitted aerosols in early morning, but can reasonably predict the CCN concentration after the aerosols underwent atmospheric processing for several hours. This analysis employing various simplifications provides insights into the essential information of particle chemical composition that needs to be represented in models to adequately predict CCN concentration and cloud microphysics.

Wang, J.; Cubison, M.; Aiken, A.; Jimenez, J.; Collins, D.; Gaffney, J.; Marley, N.

2010-03-15T23:59:59.000Z

59

Direct Aerosol Forcing Uncertainty  

DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

Understanding sources of uncertainty in aerosol direct radiative forcing (DRF), the difference in a given radiative flux component with and without aerosol, is essential to quantifying changes in Earth's radiation budget. We examine the uncertainty in DRF due to measurement uncertainty in the quantities on which it depends: aerosol optical depth, single scattering albedo, asymmetry parameter, solar geometry, and surface albedo. Direct radiative forcing at the top of the atmosphere and at the surface as well as sensitivities, the changes in DRF in response to unit changes in individual aerosol or surface properties, are calculated at three locations representing distinct aerosol types and radiative environments. The uncertainty in DRF associated with a given property is computed as the product of the sensitivity and typical measurement uncertainty in the respective aerosol or surface property. Sensitivity and uncertainty values permit estimation of total uncertainty in calculated DRF and identification of properties that most limit accuracy in estimating forcing. Total uncertainties in modeled local diurnally averaged forcing range from 0.2 to 1.3 W m-2 (42 to 20%) depending on location (from tropical to polar sites), solar zenith angle, surface reflectance, aerosol type, and aerosol optical depth. The largest contributor to total uncertainty in DRF is usually single scattering albedo; however decreasing measurement uncertainties for any property would increase accuracy in DRF. Comparison of two radiative transfer models suggests the contribution of modeling error is small compared to the total uncertainty although comparable to uncertainty arising from some individual properties.

Mccomiskey, Allison

60

GLOBAL OPTIMIZATION OF MULTIPHASE FLOW NETWORKS IN OIL AND GAS PRODUCTION SYSTEMS  

E-Print Network [OSTI]

1 GLOBAL OPTIMIZATION OF MULTIPHASE FLOW NETWORKS IN OIL AND GAS PRODUCTION SYSTEMS MSc. Hans in an oil production system is developed. Each well may be manipulated by injecting lift gas and adjusting in the maximum oil flow rate, water flow rate, liquid flow rate, and gas flow rate. The wells may also

Johansen, Tor Arne

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


61

Global Simulation of Bioenergy Crop Productivity: Analytical framework and Case Study for Switchgrass  

SciTech Connect (OSTI)

Contemporary global assessments of the deployment potential and sustainability aspects of biofuel crops lack quantitative details. This paper describes an analytical framework capable of meeting the challenges associated with global scale agro-ecosystem modeling. We designed a modeling platform for bioenergy crops, consisting of five major components: (i) standardized global natural resources and management data sets, (ii) global simulation unit and management scenarios, (iii) model calibration and validation, (iv) high-performance computing (HPC) modeling, and (v) simulation output processing and analysis. A case study with the HPC- Environmental Policy Integrated Climate model (HPC-EPIC) to simulate a perennial bioenergy crop, switchgrass (Panicum virgatum L.) and global biomass feedstock analysis on grassland demonstrates the application of this platform. The results illustrate biomass feedstock variability of switchgrass and provide insights on how the modeling platform can be expanded to better assess sustainable production criteria and other biomass crops. Feedstock potentials on global grasslands and within different countries are also shown. Future efforts involve developing databases of productivity, implementing global simulations for other bioenergy crops (e.g. miscanthus, energycane and agave), and assessing environmental impacts under various management regimes. We anticipated this platform will provide an exemplary tool and assessment data for international communities to conduct global analysis of biofuel biomass feedstocks and sustainability.

Nair, S. Surendran [University of Tennessee, Knoxville (UTK)] [University of Tennessee, Knoxville (UTK); Nichols, Jeff A. {Cyber Sciences} [ORNL; Post, Wilfred M [ORNL] [ORNL; Wang, Dali [ORNL] [ORNL; Wullschleger, Stan D [ORNL] [ORNL; Kline, Keith L [ORNL] [ORNL; Wei, Yaxing [ORNL] [ORNL; Singh, Nagendra [ORNL] [ORNL; Kang, Shujiang [ORNL] [ORNL

2014-01-01T23:59:59.000Z

62

Aerosol Cans? -Aerosol cans use a pressurized  

E-Print Network [OSTI]

? - The waste generated in the processing of images/photos contains silver. Silver is a toxic heavy metal the product. Propellants are often flammable and/or toxic. Therefore, never store aerosol cans near ignition of this pamphlet. -Carefully transfer the old paint thinner from the one gallon closable can to the 30 gallon metal

Jia, Songtao

63

QUESTIONS ABOUT GLOBAL WARMING  

E-Print Network [OSTI]

QUESTIONS ABOUT GLOBAL WARMING ¥IS IT REAL? ¥IS IT IMPORTANT? ¥WHAT IS IT DUE TO? ¥HOW MUCH MORE in the atmosphere, giving Earth its temperate climate. Global Atmosphere, Global Warming GLOBAL TEMPERATURE TREND?t a cure for global warming! Aerosols only last a short while in the atmosphere, they would have

64

EMSL - aerosols  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

aerosols en Magnesium behavior and structural defects in Mg+ ion implanted silicon carbide. http:www.emsl.pnl.govemslwebpublicationsmagnesium-behavior-and-structural-defects-m...

65

Climate change and the socioeconomics of global food production: A quantitative analysis  

E-Print Network [OSTI]

1 Climate change and the socioeconomics of global food production: A quantitative analysis of how, Andrew J. Dougill and Piers M. Forster August 2010 Centre for Climate Change Economics and Policy Working Paper No. 29 #12;2 The Centre for Climate Change Economics and Policy (CCCEP) was established

Rambaut, Andrew

66

Global Indirect Effects of U.S. Corn Ethanol Production: A Review of the Evidence  

E-Print Network [OSTI]

Global Indirect Effects of U.S. Corn Ethanol Production: A Review of the Evidence Energy security) requires 36 billion gallons of ethanol by 2022 to replace about 20 percent of U.S. gasoline consumption. Since 2001 ethanol produc- tion, mainly from corn, has increased dramatically at an annual average

Grissino-Mayer, Henri D.

67

Supporting Information for: A Global Comparison of National Biodiesel Production Potentials  

E-Print Network [OSTI]

Supporting Information for: A Global Comparison of National Biodiesel Production Potentials Matt Biodiesel Potential · Table S.2: Variables Used in Calculating Biodiesel Volumes and Prices · Figure S.3: U) · Table S.5: Well-Managed Vegetable Oil Yields · Table S.6: A Complete List of Absolute Biodiesel

Wisconsin at Madison, University of

68

The Economic Impact of Global Climate and Tropospheric Ozone on World Agricultural Production  

E-Print Network [OSTI]

by Xiaodu (Dulles) Wang Bachelor of Science with majors in Electrical Engineering, Economics and ComputerThe Economic Impact of Global Climate and Tropospheric Ozone on World Agricultural Production Engineering The Johns Hopkins University, June 2003 Submitted to the Engineering Systems Division

69

Constraining the influence of natural variability to improve estimates of global aerosol indirect effects in a nudged version of the Community Atmosphere Model 5  

E-Print Network [OSTI]

Zhao (2006), A simulated climatology of Asian dust aerosolN) PI (F) ? PI (F) ? X ? 2000 (PD Climatology) ? ? 2000 (PD Climatology) ? PD (F) X a All simulations used the same

Kooperman, Gabriel J; Pritchard, Michael S; Ghan, Steven J; Wang, Minghuai; Somerville, Richard C. J; Russell, Lynn M

2012-01-01T23:59:59.000Z

70

Global Simulation of Bioenergy Crop Productivity: Analytical Framework and Case Study for Switchgrass  

SciTech Connect (OSTI)

A global energy crop productivity model that provides geospatially explicit quantitative details on biomass potential and factors affecting sustainability would be useful, but does not exist now. This study describes a modeling platform capable of meeting many challenges associated with global-scale agro-ecosystem modeling. We designed an analytical framework for bioenergy crops consisting of six major components: (i) standardized natural resources datasets, (ii) global field-trial data and crop management practices, (iii) simulation units and management scenarios, (iv) model calibration and validation, (v) high-performance computing (HPC) simulation, and (vi) simulation output processing and analysis. The HPC-Environmental Policy Integrated Climate (HPC-EPIC) model simulated a perennial bioenergy crop, switchgrass (Panicum virgatum L.), estimating feedstock production potentials and effects across the globe. This modeling platform can assess soil C sequestration, net greenhouse gas (GHG) emissions, nonpoint source pollution (e.g., nutrient and pesticide loss), and energy exchange with the atmosphere. It can be expanded to include additional bioenergy crops (e.g., miscanthus, energy cane, and agave) and food crops under different management scenarios. The platform and switchgrass field-trial dataset are available to support global analysis of biomass feedstock production potential and corresponding metrics of sustainability.

Kang, Shujiang [ORNL; Kline, Keith L [ORNL; Nair, S. Surendran [University of Tennessee, Knoxville (UTK); Nichols, Dr Jeff A [ORNL; Post, Wilfred M [ORNL; Brandt, Craig C [ORNL; Wullschleger, Stan D [ORNL; Wei, Yaxing [ORNL; Singh, Nagendra [ORNL

2013-01-01T23:59:59.000Z

71

The effects of potential changes in United States beef production on global grazing systems and greenhouse gas emissions  

E-Print Network [OSTI]

and greenhouse gas emissions Jerome Dumortier1 , Dermot J Hayes2 , Miguel Carriquiry2 , Fengxia Dong3 , Xiaodong in the U.S. causes a net increase in GHG emissions on a global scale. We couple a global agricultural production in the United States. The effects on emissions from agricultural production (i.e., methane

Zhou, Yaoqi

72

aerosol characteristic researching: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

as they have significant impacts both on localregional air pollution and global climate. Recent for Aerosol and Cloud Chemistry, Aerodyne Research, Incorporated, Billerica,...

73

he Impact of Primary Marine Aerosol on Atmospheric Chemistry, Radiation and Climate: A CCSM Model Development Study  

SciTech Connect (OSTI)

This project examined the potential large-scale influence of marine aerosol cycling on atmospheric chemistry, physics and radiative transfer. Measurements indicate that the size-dependent generation of marine aerosols by wind waves at the ocean surface and the subsequent production and cycling of halogen-radicals are important but poorly constrained processes that influence climate regionally and globally. A reliable capacity to examine the role of marine aerosol in the global-scale atmospheric system requires that the important size-resolved chemical processes be treated explicitly. But the treatment of multiphase chemistry across the breadth of chemical scenarios encountered throughout the atmosphere is sensitive to the initial conditions and the precision of the solution method. This study examined this sensitivity, constrained it using high-resolution laboratory and field measurements, and deployed it in a coupled chemical-microphysical 3-D atmosphere model. First, laboratory measurements of fresh, unreacted marine aerosol were used to formulate a sea-state based marine aerosol source parameterization that captured the initial organic, inorganic, and physical conditions of the aerosol population. Second, a multiphase chemical mechanism, solved using the Max Planck Institute for Chemistry??s MECCA (Module Efficiently Calculating the Chemistry of the Atmosphere) system, was benchmarked across a broad set of observed chemical and physical conditions in the marine atmosphere. Using these results, the mechanism was systematically reduced to maximize computational speed. Finally, the mechanism was coupled to the 3-mode modal aerosol version of the NCAR Community Atmosphere Model (CAM v3.6.33). Decadal-scale simulations with CAM v.3.6.33, were run both with and without reactive-halogen chemistry and with and without explicit treatment of particulate organic carbon in the marine aerosol source function. Simulated results were interpreted (1) to evaluate influences of marine aerosol production on the microphysical properties of aerosol populations and clouds over the ocean and the corresponding direct and indirect effects on radiative transfer; (2) atmospheric burdens of reactive halogen species and their impacts on O3, NOx, OH, DMS, and particulate non-sea-salt SO42-; and (3) the global production and influences of marine-derived particulate organic carbon. The model reproduced major characteristics of the marine aerosol system and demonstrated the potential sensitivity of global, decadal-scale climate metrics to multiphase marine-derived components of Earth??s troposphere. Due to the combined computational burden of the coupled system, the currently available computational resources were the limiting factor preventing the adequate statistical analysis of the overall impact that multiphase chemistry might have on climate-scale radiative transfer and climate.

Keene, William C. [University of Virginia] [University of Virginia; Long, Michael S. [University of Virginia] [University of Virginia

2013-05-20T23:59:59.000Z

74

Global  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr MayAtmospheric Optical Depth7-1D: Vegetation ProposedUsingFun with Big Sky LearningGet Assistance GetGiant ProteaseGlass andT.2 -Global

75

Organic and Inorganic Aerosol Below-Cloud Scavenging by  

E-Print Network [OSTI]

concentrations, with an average gravimetric PM1.0 of 8.2 ( 1.6 µg m-3 and an average Fourier transform infrared-rinsing behavior was unaffected by source type. The aerosol OM was hydrophilic throughout the sampling period the description of aerosol lifetimes in global models. Introduction Wet and dry deposition of aerosol particles

Russell, Lynn

76

6, 48974927, 2006 A global emission  

E-Print Network [OSTI]

aerosol causes atmospheric warming through the direct aerosol effect, i.e. the trans- mission of absorbedACPD 6, 4897­4927, 2006 A global emission inventory of carbon aerosol for 1860­1997 C. Junker and C a Creative Commons License. Atmospheric Chemistry and Physics Discussions A global emission inventory

Paris-Sud XI, Université de

77

Heterogeneous Chemistry: Understanding Aerosol/Oxidant Interactions  

SciTech Connect (OSTI)

Global radiative forcing of nitrate and ammonium aerosols has mostly been estimated from aerosol concentrations calculated at thermodynamic equilibrium or using approximate treatments for their uptake by aerosols. In this study, a more accurate hybrid dynamical approach (DYN) was used to simulate the uptake of nitrate and ammonium by aerosols and the interaction with tropospheric reactive nitrogen chemistry in a three-dimensional global aerosol and chemistry model, IMPACT, which also treats sulfate, sea salt and mineral dust aerosol. 43% of the global annual average nitrate aerosol burden, 0.16 TgN, and 92% of the global annual average ammonium aerosol burden, 0.29 TgN, exist in the fine mode (D<1.25 {micro}m) that scatters most efficiently. Results from an equilibrium calculation differ significantly from those of DYN since the fraction of fine-mode nitrate to total nitrate (gas plus aerosol) is 9.8%, compared to 13% in DYN. Our results suggest that the estimates of aerosol forcing from equilibrium concentrations will be underestimated. We also show that two common approaches used to treat nitrate and ammonium in aerosol in global models, including the first-order gas-to-particle approximation based on uptake coefficients (UPTAKE) and a hybrid method that combines the former with an equilibrium model (HYB), significantly overpredict the nitrate uptake by aerosols especially that by coarse particles, resulting in total nitrate aerosol burdens higher than that in DYN by +106% and +47%, respectively. Thus, nitrate aerosol in the coarse mode calculated by HYB is 0.18 Tg N, a factor of 2 more than that in DYN (0.086 Tg N). Excessive formation of the coarse-mode nitrate in HYB leads to near surface nitrate concentrations in the fine mode lower than that in DYN by up to 50% over continents. In addition, near-surface HNO{sub 3} and NO{sub x} concentrations are underpredicted by HYB by up to 90% and 5%, respectively. UPTAKE overpredicts the NO{sub x} burden by 56% and near-surface NO{sub x} concentrations by a factor of 2-5. These results suggest the importance of using the more accurate hybrid dynamical method in the estimates of both aerosol forcing and tropospheric ozone chemistry.

Joyce E. Penner

2005-03-14T23:59:59.000Z

78

Atmospheric Aerosol Systems | EMSL  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Science Themes Atmospheric Aerosol Systems Overview Atmospheric Aerosol Systems Biosystem Dynamics & Design Energy Materials & Processes Terrestrial & Subsurface Ecosystems...

79

Present and potential future contributions of sulfate, black and organic carbon aerosols from China to global air quality, premature mortality and  

E-Print Network [OSTI]

analysis indicates that increased effort to reduce greenhouse gases is essential to address climate change mortality and climate change has not been well quantified. Through both direct radiative effects, they have not considered the effect of aerosols on radiative forcing (RF) and climate change. Although

Mauzerall, Denise

80

Sources and production of organic aerosol in Mexico City: insights from the combination of a chemical transport model (PMCAMx-2008) and measurements  

E-Print Network [OSTI]

Urban areas are large sources of organic aerosols and their precursors. Nevertheless, the contributions of primary (POA) and secondary organic aerosol (SOA) to the observed particulate matter levels have been difficult to ...

Tsimpidi, A. P.

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


81

Stratospheric Aerosol Geoengineering ALAN ROBOCK  

E-Print Network [OSTI]

Stratospheric Aerosol Geoengineering ALAN ROBOCK ABSTRACT In response to global warming, one suggested geoengineering response involves creating a cloud of particles in the stratosphere to reflect some, the volcano analog also warns against geoengineering because of responses such as ozone depletion, regional

Robock, Alan

82

Laboratory Studies of Processing of Carbonaceous Aerosols by Atmospheric Oxidants/Hygroscopicity and CCN Activity of Secondary & Processed Primary Organic Aerosols  

SciTech Connect (OSTI)

The atmosphere is composed of a complex mixture of gases and suspended microscopic aerosol particles. The ability of these particles to take up water (hygroscopicity) and to act as nuclei for cloud droplet formation significantly impacts aerosol light scattering and absorption, and cloud formation, thereby influencing air quality, visibility, and climate in important ways. A substantial, yet poorly characterized component of the atmospheric aerosol is organic matter. Its major sources are direct emissions from combustion processes, which are referred to as primary organic aerosol (POA), or in situ processes in which volatile organic compounds (VOCs) are oxidized in the atmosphere to low volatility reaction products that subsequent condense to form particles that are referred to as secondary organic aerosol (SOA). POA and VOCs are emitted to the atmosphere from both anthropogenic and natural (biogenic) sources. The overall goal of this experimental research project was to conduct laboratory studies under simulated atmospheric conditions to investigate the effects of the chemical composition of organic aerosol particles on their hygroscopicity and cloud condensation nucleation (CCN) activity, in order to develop quantitative relationships that could be used to more accurately incorporate aerosol-cloud interactions into regional and global atmospheric models. More specifically, the project aimed to determine the products, mechanisms, and rates of chemical reactions involved in the processing of organic aerosol particles by atmospheric oxidants and to investigate the relationships between the chemical composition of organic particles (as represented by molecule sizes and the specific functional groups that are present) and the hygroscopicity and CCN activity of oxidized POA and SOA formed from the oxidation of the major classes of anthropogenic and biogenic VOCs that are emitted to the atmosphere, as well as model hydrocarbons. The general approach for this project was to carry out reactions of representative anthropogenic and biogenic VOCs and organic particles with ozone (O3), and hydroxyl (OH), nitrate (NO3), and chlorine (Cl) radicals, which are the major atmospheric oxidants, under simulated atmospheric conditions in large-volume environmental chambers. A combination of on-line and off-line analytical techniques were used to monitor the chemical and physical properties of the particles including their hygroscopicity and CCN activity. The results of the studies were used to (1) improve scientific understanding of the relationships between the chemical composition of organic particles and their hygroscopicity and CCN activity, (2) develop an improved molecular level theoretical framework for describing these relationships, and (3) establish a large database that is being used to develop parameterizations relating organic aerosol chemical properties and SOA sources to particle hygroscopicity and CCN activity for use in regional and global atmospheric air quality and climate models.

Ziemann, P.J.; Arey, J.; Atkinson, R.; Kreidenweis, S.M.; Petters, M.D.

2012-06-13T23:59:59.000Z

83

Characterization of aerosols produced by surgical procedures  

SciTech Connect (OSTI)

In many surgeries, especially orthopedic procedures, power tools such as saws and drills are used. These tools may produce aerosolized blood and other biological material from bone and soft tissues. Surgical lasers and electrocautery tools can also produce aerosols when tissues are vaporized and condensed. Studies have been reported in the literature concerning production of aerosols during surgery, and some of these aerosols may contain infectious material. Garden et al. (1988) reported the presence of papilloma virus DNA in the fumes produced from laser surgery, but the infectivity of the aerosol was not assessed. Moon and Nininger (1989) measured the size distribution and production rate of emissions from laser surgery and found that particles were generally less than 0.5 {mu}m diameter. More recently there has been concern expressed over the production of aerosolized blood during surgical procedures that require power tools. In an in vitro study, the production of an aerosol containing the human immunodeficiency virus (HIV) was reported when power tools were used to cut tissues with blood infected with HIV. Another study measured the size distribution of blood aerosols produced by surgical power tools and found blood-containing particles in a number of size ranges. Health care workers are anxious and concerned about whether surgically produced aerosols are inspirable and can contain viable pathogens such as HIV. Other pathogens such as hepatitis B virus (HBV) are also of concern. The Occupational Safety and Health funded a project at the National Institute for Inhalation Toxicology Research Institute to assess the extent of aerosolization of blood and other tissues during surgical procedures. This document reports details of the experimental and sampling approach, methods, analyses, and results on potential production of blood-associated aerosols from surgical procedures in the laboratory and in the hospital surgical suite.

Yeh, H.C.; Muggenburg, B.A.; Lundgren, D.L.; Guilmette, R.A.; Snipes, M.B.; Jones, R.K. [Inhalation Toxicology Research Institute, Albuquerque, NM (United States); Turner, R.S. [Lovelace Health Systems, Albuquerque, NM (United States)

1994-07-01T23:59:59.000Z

84

Recent studies suggest that human activities accelerate the production of reactive nitrogen on a global scale. Increased  

E-Print Network [OSTI]

agricultural sources in the U.S. and Europe. In addition, several best management practices are explored on a global scale. Increased nitrogen emissions may lead to environmental impacts including photochemical air production in many developed countries. These agricultural production practices are increasingly subject

Niyogi, Dev

85

The importance of aerosol mixing state and size-resolved composition on CCN concentration and the variation of the importance with atmospheric aging of aerosols  

SciTech Connect (OSTI)

Aerosol microphysics, chemical composition, and CCN concentrations were measured at the T0 urban supersite in Mexico City during Megacity Initiative: Local and Global Research Observations (MILAGRO) in March 2006. The aerosol size distribution and composition often showed strong diurnal variation associated with traffic emissions and aging of aerosols through coagulation and local photochemical production of secondary aerosol species. CCN concentrations (N{sub CCN}) are derived using Kohler theory from the measured aerosol size distribution and various simplified aerosol mixing state and chemical composition, and are compared to concurrent measurements at five supersaturations ranging from 0.11% to 0.35%. The influence of assumed mixing state on calculated N{sub CCN} is examined using both aerosols observed during MILAGRO and representative aerosol types. The results indicate that while ambient aerosols often consist of particles with a wide range of compositions at a given size, N{sub CCN} may be derived within {approx}20% assuming an internal mixture (i.e., particles at a given size are mixtures of all participating species, and have the identical composition) if great majority of particles has an overall {kappa} (hygroscopicity parameter) value greater than 0.1. For a non-hygroscopic particle with a diameter of 100 nm, a 3 nm coating of sulfate or nitrate is sufficient to increase its {kappa} from 0 to 0.1. The measurements during MILAGRO suggest that the mixing of non-hygroscopic primary organic aerosol (POA) and black carbon (BC) particles with photochemically produced hygroscopic species and thereby the increase of their {kappa} to 0.1 take place in a few hours during daytime. This rapid process suggests that during daytime, a few tens of kilometers away for POA and BC sources, N{sub CCN} may be derived with sufficient accuracy by assuming an internal mixture, and using bulk chemical composition. The rapid mixing also indicates that, at least for very active photochemical environments such as Mexico City, a substantially shorter timescale during daytime for the conversion of hydrophobic POA and BC to hydrophilic particles than the 1-2 days used in some global models. The conversion time scale is substantially longer during night. Most POA and BC particles emitted during evening hours likely remain non-hygroscopic until efficiently internally mixed with secondary species in the next morning. The results also suggest that the assumed mixing state strongly impacts calculated N{sub CCN} only when POA and BC represent a large fraction of the total aerosol volume. One of the implications is that while physically unrealistic, external mixtures, which are used in many global models, may also sufficiently predict N{sub CCN} for aged aerosol, as the contribution of non-hygroscopic POA and BC to overall aerosol volume is often substantially reduced due to the condensation of secondary species.

Wang, J.; Cubison, M. J.; Aiken, A. C.; Jimenez, J. L.; Collins, D. R.

2010-05-01T23:59:59.000Z

86

Aerosol Characterization Data from the Asian Pacific Regional Aerosol Characterization Project (ACE-Asia)  

DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

The Aerosol Characterization Experiments (ACE) were designed to increase understanding of how atmospheric aerosol particles affect the Earth's climate system. These experiments integrated in-situ measurements, satellite observations, and models to reduce the uncertainty in calculations of the climate forcing due to aerosol particles and improve the ability of models to predict the influences of aerosols on the Earth's radiation balance. ACE-Asia was the fourth in a series of experiments organized by the International Global Atmospheric Chemistry (IGAC) Program (A Core Project of the International Geosphere Biosphere Program). The Intensive Field Phase for ACE-Asia took place during the spring of 2001 (mid-March through early May) off the coast of China, Japan and Korea. ACE-Asia pursued three specific objectives: 1) Determine the physical, chemical, and radiative properties of the major aerosol types in the Eastern Asia and Northwest Pacific region and investigate the relationships among these properties. 2) Quantify the physical and chemical processes controlling the evolution of the major aerosol types and in particular their physical, chemical, and radiative properties. 3) Develop procedures to extrapolate aerosol properties and processes from local to regional and global scales, and assess the regional direct and indirect radiative forcing by aerosols in the Eastern Asia and Northwest Pacific region [Edited and shortened version of summary at http://data.eol.ucar.edu/codiac/projs?ACE-ASIA]. The Ace-Asia collection contains 174 datasets.

87

Creating ladders out of chains : China's technological development in a world of global production  

E-Print Network [OSTI]

With the advent of economic globalization, the terms of debate over the political and social conditions necessary to foster development in the Global South have shifted. Examining technological development, one important ...

Fuller, Douglas Brian

2005-01-01T23:59:59.000Z

88

Do biomass burning aerosols intensify drought in equatorial Asia during El Nio?  

E-Print Network [OSTI]

fication of drought-induced biomass burning in Indonesiavariability in global biomass burning emissions from 1997 toChemistry and Physics Do biomass burning aerosols intensify

Tosca, M. G; Randerson, J. T; Zender, C. S; Flanner, M. G; Rasch, P. J

2010-01-01T23:59:59.000Z

89

E-Print Network 3.0 - aerosol features biomass Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

features biomass Search Powered by Explorit Topic List Advanced Search Sample search results for: aerosol features biomass Page: << < 1 2 3 4 5 > >> 1 Global observations and...

90

E-Print Network 3.0 - aerosol situation monitoring Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

with the highly nonuniform distribution... . Schwartz Workshop on Use of Satellite Data, Global Models, and Analysis to Advance Understanding of Aerosol... transport models...

91

Sulfate Aerosol Geoengineering: The Question of Justice Toby Svoboda1,*  

E-Print Network [OSTI]

Sulfate Aerosol Geoengineering: The Question of Justice Toby Svoboda1,* , Klaus Keller2 , Marlos of geoengineering as a means to address global climate change. This paper focuses on the question of whether a particular form of geoengineering, namely deploying sulfate aerosols in the stratosphere to counteract some

92

Spatial and Seasonal Trends in Biogenic Secondary Organic Aerosol  

E-Print Network [OSTI]

Spatial and Seasonal Trends in Biogenic Secondary Organic Aerosol Tracers and Water-Soluble Organic biogenic secondary organic aerosol (SOA) tracers via gas chromatography-mass spectrometry (GC natural and anthropogenic sources and is dominated by terrestrial plant foliage (7). The global

Zheng, Mei

93

Two Hundred Fifty Years of Aerosols and Climate: The End of the Age of Aerosols  

SciTech Connect (OSTI)

Carbonaceous and sulfur aerosols have a substantial global and regional influence on climate in addition to their impact on health and ecosystems. The magnitude of this influence has changed substantially over the past and is expected to continue to change into the future. An integrated picture of the changing climatic influence of black carbon, organic carbon and sulfate over the period 1850 through 2100, focusing on uncertainty, is presented using updated historical inventories and a coordinated set of emission projections. While aerosols have had a substantial impact on climate over the past century, by the end of the 21st century aerosols will likely be only a minor contributor to radiative forcing due to increases in greenhouse gas forcing and a global decrease in pollutant emissions. This outcome is even more certain under a successful implementation of a policy to limit greenhouse gas emissions as low-carbon energy technologies that do not emit appreciable aerosol or SO2 are deployed.

Smith, Steven J.; Bond, Tami C.

2014-01-20T23:59:59.000Z

94

Probing nuclear dynamics in jet production with a global event shape  

E-Print Network [OSTI]

We study single jet production in electron-nucleus collisions e^- + N_A -> J + X, using the 1-jettiness (\\tau_1) global event shape. It inclusively quantifies the pattern of radiation in the final state, gives enhanced sensitivity to soft radiation at wide angles from the nuclear beam and final-state jet, and facilitates the resummation of large Sudakov logarithms associated with the veto on additional jets. Through their effect on the observed pattern of radiation, 1-jettiness can be a useful probe of nuclear PDFs and power corrections from dynamical effects in the nuclear medium. This formalism allows for the standard jet shape analysis while simultaneously providing sensitivity to soft radiation at wide angles from the jet. We use a factorization framework for cross-sections differential in $\\tau_1$ and the transverse momentum (P_{J_T}) and rapidity (y) of the jet, in the region \\tau_1theoretical control over resummation, while providing enhanced sensitivity to nuclear medium effects. We give numerical results at leading twist, with resummation at the next-to-next-to-leading logarithmic (NNLL) level of accuracy, for a variety of nuclear targets. Such studies would be ideal for the EIC and the LHeC proposals for a future electron-ion collider, where a range of nuclear targets are planned.

Zhong-Bo Kang; Xiaohui Liu; Sonny Mantry; Jian-Wei Qiu

2014-07-25T23:59:59.000Z

95

A review of Secondary Organic Aerosol (SOA) formation from isoprene  

E-Print Network [OSTI]

Recent field and laboratory evidence indicates that the oxidation of isoprene, (2-methyl-1,3-butadiene, C[subscript 5]H[subscript 8]) forms secondary organic aerosol (SOA). Global biogenic emissions of isoprene (600 Tg ...

Kroll, Jesse

96

Climate impacts of carbonaceous and other non-sulfate aerosols: A proposed study  

SciTech Connect (OSTI)

In addition to sulfate aerosols, carbonaceous and other non-sulfate aerosols are potentially significant contributors to global climate change. We present evidence that strongly suggests that current assessments of the effects of aerosols on climate may be inadequate because major aerosol components, especially carbonaceous aerosols, are not included in these assessments. Although data on the properties and distributions of anthropogenic carbonaceous aerosols are insufficient to allow quantification of their climate impacts, the existing information suggests that climate forcing by this aerosol component may be significant and comparable to that by sulfate aerosols. We propose that a research program be undertaken to support a quantitative assessment of the role in climate forcing of non-sulfate, particularly carbonaceous, aerosols.

Andreae, M.O.; Crutzen, P.J. [Max Planck Institute for Chemistry, Mainz (Germany); Cofer, W.R. III; Hollande, J.M. [NASA Langley Research Center, Hampton, VA (United States). Atmospheric Sciences Division] [and others

1995-06-01T23:59:59.000Z

97

Attachment of radon progeny to cigarette-smoke aerosols  

SciTech Connect (OSTI)

The daughter products of radon gas are now recognized as a significant contributor to radiation exposure to the general public. It is also suspected that a synergistic effect exists with the combination cigarette smoking and radon exposure. We have conducted an experimental investigation to determine the physical nature of radon progeny interactions with cigarette smoke aerosols. The size distributions of the aerosols are characterized and attachment rates of radon progeny to cigarette-smoke aerosols are determined. Both the mainstream and sidestream portions of the smoke aerosol are investigated. Unattached radon progeny are very mobile and, in the presence of aerosols, readily attach to the particle surfaces. In this study, an aerosol chamber is used to contain the radon gas, progeny and aerosol mixture while allowing the attachment process to occur. The rate of attachment is dependent on the size distribution, or diffusion coefficient, of the radon progeny as well as the aerosol size distribution. The size distribution of the radon daughter products is monitored using a graded-screen diffusion battery. The diffusion battery also enables separation of the unattached radon progeny from those attached to the aerosol particles. Analysis of the radon decay products is accomplished using alpha spectrometry. The aerosols of interest are size fractionated with the aid of a differential mobility analyzer and cascade impactor. The measured attachment rates of progeny to the cigarette smoke are compared to those found in similar experiments using an ambient aerosol. The lowest attachment coefficients observed, {approximately}10{sup {minus}6} cm{sup 3}/s, occurred for the ambient aerosol. The sidestream and mainstream smoke aerosols exhibited higher attachment rates in that order. The results compared favorably with theories describing the coagulation process of aerosols.

Biermann, A.H.; Sawyer, S.R.

1995-05-01T23:59:59.000Z

98

The behavior of constant rate aerosol reactors  

SciTech Connect (OSTI)

An aerosol reactor is a gaseous system in which fine particles are formed by chemical reaction in either a batch or flow process. The particle sizes of interest range from less than 10 angstrom (molecular clusters) to 10 ..mu..m. Such reactors may be operated to study the aerosol formation process, as in a smog reactor, or to generate a product such as a pigment or a catalytic aerosol. Aerosol reactors can be characterized by three temporal or spatial zones or regions of operation for batch and flow reactors, respectively. In zone I, chemical reaction results in the formation of condensable molecular products which nucleate and form very high concentrations of small particles. The number density depends on the concentration of preexisting aerosol. Zone II is a transition region in which the aerosol number concentration levels off as a result of hetergeneous condensation by the stable aerosol. In zone III coagulation becomes sufficiently rapid to reduce the particle number concentration. There may be a zone IV in which agglomerates form.

Friedlander, S.K.

1982-01-01T23:59:59.000Z

99

Total aerosol effect: forcing or radiative flux perturbation?  

SciTech Connect (OSTI)

Uncertainties in aerosol forcings, especially those associated with clouds, contribute to a large extent to uncertainties in the total anthropogenic forcing. The interaction of aerosols with clouds and radiation introduces feedbacks which can affect the rate of rain formation. Traditionally these feedbacks were not included in estimates of total aerosol forcing. Here we argue that they should be included because these feedbacks act quickly compared with the time scale of global warming. We show that for different forcing agents (aerosols and greenhouse gases) the radiative forcings as traditionally defined agree rather well with estimates from a method, here referred to as radiative flux perturbations (RFP), that takes these fast feedbacks and interactions into account. Thus we propose replacing the direct and indirect aerosol forcing in the IPCC forcing chart with RFP estimates. This implies that it is better to evaluate the total anthropogenic aerosol effect as a whole.

Lohmann, Ulrike; Storelvmo, Trude; Jones, Andy; Rotstayn, Leon; Menon, Surabi; Quaas, Johannes; Ekman, Annica; Koch, Dorothy; Ruedy, Reto

2009-09-25T23:59:59.000Z

100

Emerging Issues in Nanoparticle Aerosol Science and Technology Workshop report sponsored by: NSF, Southern California Particle Center and UCLA  

E-Print Network [OSTI]

has responsibility for nuclear reactor safety which includes emissions of radioactive particles pollution sources, (2) industrial production of nanoparticle reinforcing fillers such as carbon black nanoparticle products by aerosol processes, (4) atmospheric dynamics of fractal-like nanoparticle aerosols (e

Jimenez, Jose-Luis

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


101

Electrically Driven Technologies for Radioactive Aerosol Abatement  

SciTech Connect (OSTI)

The purpose of this research project was to develop an improved understanding of how electriexecy driven processes, including electrocoalescence, acoustic agglomeration, and electric filtration, may be employed to efficiently treat problems caused by the formation of aerosols during DOE waste treatment operations. The production of aerosols during treatment and retrieval operations in radioactive waste tanks and during thermal treatment operations such as calcination presents a significant problem of cost, worker exposure, potential for release, and increased waste volume.

David W. DePaoli; Ofodike A. Ezekoye; Costas Tsouris; Valmor F. de Almeida

2003-01-28T23:59:59.000Z

102

Institutions, public policy and the product life cycle : the globalization of biomanufacturing and implications for Massachusetts  

E-Print Network [OSTI]

Globalization has brought about a major shift in our understanding of how companies organize themselves and how they compete. The fragmentation of firms in their scope and structure, the vertical disintegration of firms ...

Reynolds, Elisabeth B

2010-01-01T23:59:59.000Z

103

Improved solid aerosol generator  

DOE Patents [OSTI]

An improved solid aerosol generator used to produce a gas borne stream of dry, solid particles of predetermined size and concentration. The improved solid aerosol generator nebulizes a feed solution of known concentration with a flow of preheated gas and dries the resultant wet heated aerosol in a grounded, conical heating chamber, achieving high recovery and flow rates. 2 figs.

Prescott, D.S.; Schober, R.K.; Beller, J.

1988-07-19T23:59:59.000Z

104

How well do we know northern land cover? Comparison of four global vegetation and wetland products  

E-Print Network [OSTI]

Advanced Very High Resolution Radiometer data (GLCC.AVHRR), (2) the Global Land Cover Classification.AVHRR database underestimates evergreen needleleaf forest in favor of mixed forest; and (3) at high latitudes impacts of climate change on land- atmosphere exchanges of energy, water, carbon and green- house gases [e

Smith, Laurence C.

105

Conference for Biomass and Energy, Copenhagen, 1996 published by Elsevier BIOMASS ENERGY PRODUCTION: THE GLOBAL POTENTIAL  

E-Print Network [OSTI]

.g. in conventional forestry equals today's global demand for primary energy, namely about 380 Exajoule net heating brought about by mainly two human activities: deforestation and fossil energy consumption (see Fig. 19th Conference for Biomass and Energy, Copenhagen, 1996 ­ published by Elsevier 1 BIOMASS ENERGY

Keeling, Stephen L.

106

Tales From the 'Global' Economy: Cross National Production Networks and the Re-organization of the European Economy  

E-Print Network [OSTI]

The Problem of Globalization," Economy and Society , 21,Globalization and the Future of the Nation State," Economy

Zysman, John; Doherty, Eileen; Schwartz, Andrew

1996-01-01T23:59:59.000Z

107

McDonnell Academy Global Energy and  

E-Print Network [OSTI]

in Solar Energy, Clean Coal Combustion, Distributed Energy Production, Integrated Assessment, Energy include those for clean coal utilization; aerosol science and engineering; energy and environmental issues

Subramanian, Venkat

108

Aerosol radiative forcing and the accuracy of satellite aerosol optical depth retrieval  

E-Print Network [OSTI]

) of the AVHRR (Advanced Very High Resolution Radiometer) is typically between 0.06 and 0.15, while the RMSE between t = 0.1 and t = 0.8. The Department of Energy research satellite instrument, the Multispectral aerosol radiative forcing are known, the predictions of future global warming may remain unacceptably high

109

Extraction of nucleon resonances from global analysis of meson production reactions at EBAC  

SciTech Connect (OSTI)

We report the current status of exploring the dynamical aspect of the excited nucleon states through the comprehensive coupled-channels analysis of meson production reactions at the Excited Baryon Analysis Center of Jefferson Lab.

Kamano, Hiroyuki [Excited Baryon Analysis Center, Thomas Jefferson National Accelerator Facility, Newport News, Virginia 23606 (United States)

2011-10-21T23:59:59.000Z

110

The economic impact of global climate and tropospheric oxone on world agricultural production  

E-Print Network [OSTI]

The objective of my thesis is to analyze the economic impact on agriculture production from changes in climate and tropospheric ozone, and related policy interventions. The analysis makes use of the Emissions Prediction ...

Wang, Xiaodu

2005-01-01T23:59:59.000Z

111

The Aerosol Modeling Testbed: A community tool to objectively evaluate aerosol process modules  

SciTech Connect (OSTI)

This study describes a new modeling paradigm that significantly advances how the third activity is conducted while also fully exploiting data and findings from the first two activities. The Aerosol Modeling Testbed (AMT) is a computational framework for the atmospheric sciences community that streamlines the process of testing and evaluating aerosol process modules over a wide range of spatial and temporal scales. The AMT consists of a fully-coupled meteorology-chemistry-aerosol model, and a suite of tools to evaluate the performance of aerosol process modules via comparison with a wide range of field measurements. The philosophy of the AMT is to systematically and objectively evaluate aerosol process modules over local to regional spatial scales that are compatible with most field campaigns measurement strategies. The performance of new treatments can then be quantified and compared to existing treatments before they are incorporated into regional and global climate models. Since the AMT is a community tool, it also provides a means of enhancing collaboration and coordination among aerosol modelers.

Fast, Jerome D.; Gustafson, William I.; Chapman, Elaine G.; Easter, Richard C.; Rishel, Jeremy P.; Zaveri, Rahul A.; Grell, Georg; Barth, Mary

2011-03-02T23:59:59.000Z

112

Global Aerosol Health Impacts: Quantifying Uncertainties  

E-Print Network [OSTI]

Atmospheric fine particulate matter <2.5 ?m (PM2.5) can cause cardiovasculatory and respiratory damages and mortalities. Assessing population exposure to and damages from PM2.5 is important for policy, but measurement ...

Selin, Noelle E.

113

atmospheric aerosol limb: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

coefficient is 0.5 and then 1.0 2. For the same conditions calculate the H Weber, Rodney 5 Secondary organic aerosol 1. Atmospheric chemical mechanism for production...

114

atmospheric aerosols recorded: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

coefficient is 0.5 and then 1.0 2. For the same conditions calculate the H Weber, Rodney 4 Secondary organic aerosol 1. Atmospheric chemical mechanism for production...

115

atmospheric aerosols relation: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

coefficient is 0.5 and then 1.0 2. For the same conditions calculate the H Weber, Rodney 4 Secondary organic aerosol 1. Atmospheric chemical mechanism for production...

116

ARM: 1-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm  

DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

1-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

Sivaraman, Chitra; Flynn, Connor

117

ARM: 10-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm  

DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

10-minute Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

Newsom, Rob; Goldsmith, John

118

Global Livestock Production and Health Atlas (GLiPHA) | Open Energy  

Open Energy Info (EERE)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Home Page on Google Bookmark EERE: Alternative Fuels Data Center Home5b9fcbce19 No revision hasInformation Earth's Heat Jump to: navigation,GigaCreteInformation Livestock Production and

119

Modal aerosol dynamics modeling  

SciTech Connect (OSTI)

The report presents the governing equations for representing aerosol dynamics, based on several different representations of the aerosol size distribution. Analytical and numerical solution techniques for these governing equations are also reviewed. Described in detail is a computationally efficient numerical technique for simulating aerosol behavior in systems undergoing simultaneous heat transfer, fluid flow, and mass transfer in and between the gas and condensed phases. The technique belongs to a general class of models known as modal aerosol dynamics (MAD) models. These models solve for the temporal and spatial evolution of the particle size distribution function. Computational efficiency is achieved by representing the complete aerosol population as a sum of additive overlapping populations (modes), and solving for the time rate of change of integral moments of each mode. Applications of MAD models for simulating aerosol dynamics in continuous stirred tank aerosol reactors and flow aerosol reactors are provided. For the application to flow aerosol reactors, the discussion is developed in terms of considerations for merging a MAD model with the SIMPLER routine described by Patankar (1980). Considerations for incorporating a MAD model into the U.S. Environmental Protection Agency's Regional Particulate Model are also described. Numerical and analytical techniques for evaluating the size-space integrals of the modal dynamics equations (MDEs) are described. For multimodal logonormal distributions, an analytical expression for the coagulation integrals of the MDEs, applicable for all size regimes, is derived, and is within 20% of accurate numerical evaluation of the same moment coagulation integrals. A computationally efficient integration technique, based on Gauss-Hermite numerical integration, is also derived.

Whitby, E.R.; McMurry, P.H.; Shankar, U.; Binkowski, F.S.

1991-02-01T23:59:59.000Z

120

The Two-Column Aerosol Project (TCAP) Science Plan  

SciTech Connect (OSTI)

The Two-Column Aerosol Project (TCAP) field campaign will provide a detailed set of observations with which to (1) perform radiative and cloud condensation nuclei (CCN) closure studies, (2) evaluate a new retrieval algorithm for aerosol optical depth (AOD) in the presence of clouds using passive remote sensing, (3) extend a previously developed technique to investigate aerosol indirect effects, and (4) evaluate the performance of a detailed regional-scale model and a more parameterized global-scale model in simulating particle activation and AOD associated with the aging of anthropogenic aerosols. To meet these science objectives, the Atmospheric Radiation Measurement (ARM) Climate Research Facility will deploy the ARM Mobile Facility (AMF) and the Mobile Aerosol Observing System (MAOS) on Cape Cod, Massachusetts, for a 12-month period starting in the summer of 2012 in order to quantify aerosol properties, radiation, and cloud characteristics at a location subject to both clear and cloudy conditions, and clean and polluted conditions. These observations will be supplemented by two aircraft intensive observation periods (IOPs), one in the summer and a second in the winter. Each IOP will deploy one, and possibly two, aircraft depending on available resources. The first aircraft will be equipped with a suite of in situ instrumentation to provide measurements of aerosol optical properties, particle composition and direct-beam irradiance. The second aircraft will fly directly over the first and use a multi-wavelength high spectral resolution lidar (HSRL) and scanning polarimeter to provide continuous optical and cloud properties in the column below.

Berkowitz, CM; Berg, LK; Cziczo, DJ; Flynn, CJ; Kassianov, EI; Fast, JD; Rasch, PJ; Shilling, JE; Zaveri, RA; Zelenyuk, A; Ferrare, RA; Hostetler, CA; Cairns, B; Russell, PB; Ervens, B

2011-07-27T23:59:59.000Z

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


121

Aerosol Sampler Operations Manual  

E-Print Network [OSTI]

-1123 Laboratory FAX (916) 752-4107 Standard Operating Procedures Technical Information Document TI 201A #12;TI 201.................................................................................................................................................. 3 1.0 Weekly Maintenance ProceduresIMPROVE Aerosol Sampler Operations Manual February 10, 1997 Air Quality Group Crocker Nuclear

Fischer, Emily V.

122

E-Print Network 3.0 - aerosol infection model Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

under Contract No. DE-AC02-98CH10886. Summary: . Schwartz Workshop on Use of Satellite Data, Global Models, and Analysis to Advance Understanding of Aerosol... transport models...

123

Determination of particulate lead using aerosol mass spectrometry: MILAGRO/MCMA-2006 observations  

E-Print Network [OSTI]

We report the first measurements of particulate lead (Pb) from Aerodyne Aerosol Mass Spectrometers, which were deployed in and around Mexico City during the Megacity Initiative: Local and Global Research Observations ...

Salcedo, D.

124

Formation of ozone and growth of aerosols in young smoke plumes from biomass burning  

E-Print Network [OSTI]

The combustion of biomass is a major source of atmospheric trace gases and aerosols. Regional and global-scale models of atmospheric chemistry and climate take estimates for these emissions and arbitrarily "mix" them into ...

Alvarado, Matthew James

2008-01-01T23:59:59.000Z

125

FY 2011 Third Quarter Report Estimate of Historical Aerosol Direct and Indirect Effects  

SciTech Connect (OSTI)

The global and annual mean aerosol direct and indirect effects estimated from Community Earth System Model (CESM) simulations are -0.06 W m-2 and -1.39 W m-2, respectively.

Koch, D

2011-06-22T23:59:59.000Z

126

Home Page > Business > Industrial > Global Trade Of Wood Chips Down 26% In 2009 As Pulpmills Reduce Production Worldwide, Reports Wood Resources International  

E-Print Network [OSTI]

from South Africa have declined 40%. With pulp production slowly increasing this fall and energy are Australia, South Africa, Vietnam and Uruguay. Australia, the world's largest exporter, has reduced shipmentsHome Page > Business > Industrial > Global Trade Of Wood Chips Down 26% In 2009 As Pulpmills Reduce

127

Cloud/Aerosol Parameterizations: Application and Improvement of General Circulation Models  

SciTech Connect (OSTI)

One of the biggest uncertainties associated with climate models and climate forcing is the treatment of aerosols and their effects on clouds. The effect of aerosols on clouds can be divided into two components: The first indirect effect is the forcing associated with increases in droplet concentrations; the second indirect effect is the forcing associated with changes in liquid water path, cloud morphology, and cloud lifetime. Both are highly uncertain. This project applied a cloud-resolving model to understand the response of clouds under a variety of conditions to changes in aerosols. These responses are categorized according to the large-scale meteorological conditions that lead to the response. Meteorological conditions were sampled from various fields, which, together with a global aerosol model determination of the change in aerosols from present day to pre-industrial conditions, was used to determine a first order estimate of the response of global cloud fields to changes in aerosols. The response of the clouds in the NCAR CAM3 GCM coupled to our global aerosol model were tested by examining whether the response is similar to that of the cloud resolving model and methods for improving the representation of clouds and cloud/aerosol interactions were examined.

Penner, Joyce

2012-06-30T23:59:59.000Z

128

A Physically Based Framework for Modelling the Organic Fractionation of Sea Spray Aerosol from Bubble Film Langmuir Equilibria  

SciTech Connect (OSTI)

The presence of a large fraction of organic matter in primary sea spray aerosol (SSA) can strongly affect its cloud condensation nuclei activity and interactions with marine clouds. Global climate models require new parameterizations of the SSA composition in order to improve the representation of these processes. Existing proposals for such a parameterization use remotely-sensed chlorophyll-a concentrations as a proxy for the biogenic contribution to the aerosol. However, both observations and theoretical considerations suggest that existing relationships with chlorophyll-a, derived from observations at only a few locations, may not be representative for all ocean regions. We introduce a novel framework for parameterizing the fractionation of marine organic matter into SSA based on a competitive Langmuir adsorption equilibrium at bubble surfaces. Marine organic matter is partitioned into classes with differing molecular weights, surface excesses, and Langmuir adsorption parameters. The classes include a lipid-like mixture associated with labile dissolved organic carbon (DOC), a polysaccharide-like mixture associated primarily with semi-labile DOC, a protein-like mixture with concentrations intermediate between lipids and polysaccharides, a processed mixture associated with recalcitrant surface DOC, and a deep abyssal humic-like mixture. Box model calculations have been performed for several cases of organic adsorption to illustrate the underlying concepts. We then apply the framework to output from a global marine biogeochemistry model, by partitioning total dissolved organic carbon into several classes of macromolecule. Each class is represented by model compounds with physical and chemical properties based on existing laboratory data. This allows us to globally map the predicted organic mass fraction of the nascent submicron sea spray aerosol. Predicted relationships between chlorophyll-\\textit{a} and organic fraction are similar to existing empirical parameterizations, but can vary between biologically productive and non-productive regions, and seasonally within a given region. Major uncertainties include the bubble film thickness at bursting and the variability of organic surfactant activity in the ocean, which is poorly constrained. In addition, marine colloids and cooperative adsorption of polysaccharides may make important contributions to the aerosol, but are not included here. This organic fractionation framework is an initial step towards a closer linking of ocean biogeochemistry and aerosol chemical composition in Earth system models. Future work should focus on improving constraints on model parameters through new laboratory experiments or through empirical fitting to observed relationships in the real ocean and atmosphere, as well as on atmospheric implications of the variable composition of organic matter in sea spray.

Burrows, Susannah M.; Ogunro, O.; Frossard, Amanda; Russell, Lynn M.; Rasch, Philip J.; Elliott, S.

2014-12-19T23:59:59.000Z

129

Laboratory Experiments and Instrument Development for the Study of Atmospheric Aerosols  

SciTech Connect (OSTI)

Soot particles are generated by incomplete combustion of fossil and biomass fuels. Through direct effects clear air aerosols containing black carbon (BC) such as soot aerosols, absorb incoming light heating the atmosphere, while most other aerosols scatter light and produce cooling. Even though BC represents only 1-2% of the total annual emissions of particulate mass to the atmosphere, it has been estimated that the direct radiative effect of BC is the second-most important contributor to global warming after absorption by CO2. Ongoing studies continue to underscore the climate forcing importance of black carbon. However, estimates of the radiative effects of black carbon on climate remain highly uncertain due to the complexity of particles containing black carbon. Quantitative measurement of BC is challenging because BC often occurs in highly non-spherical soot particles of complex morphology. Freshly emitted soot particles are typically fractal hydrophobic aggregates. The aggregates consist of black carbon spherules with diameters typically in the range of about 15-40 nm, and they are usually coated by adsorbed polyaromatic hydrocarbons (PAHs) produced during combustion. Diesel-generated soot particles are often emitted with an organic coating composed primarily of lubricating oil and unburned fuel, as well as well as PAH compounds. Sulfuric acid has also been detected in diesel and aircraft-emitted soot particles. In the course of aging, these particle coatings may be substantially altered by chemical reactions and/or the deposition of other materials. Such processes transform the optical and CCN properties of the soot aerosols in ways that are not yet well understood. Our work over the past seven years consisted of laboratory research, instrument development and characterization, and field studies with the central focus of improving our understanding of the black carbon aerosol climate impacts. During the sixth year as well as during this seventh year (no-cost extension period) of our grant, we extended our studies to perform experiments on the controlled production and characterization of secondary organic aerosol.

Davidovits, Paul

2011-12-10T23:59:59.000Z

130

Constraining cloud lifetime effects of aerosols using A-Train satellite observations  

SciTech Connect (OSTI)

Aerosol indirect effects have remained the largest uncertainty in estimates of the radiative forcing of past and future climate change. Observational constraints on cloud lifetime effects are particularly challenging since it is difficult to separate aerosol effects from meteorological influences. Here we use three global climate models, including a multi-scale aerosol-climate model PNNL-MMF, to show that the dependence of the probability of precipitation on aerosol loading, termed the precipitation frequency susceptibility (S{sub pop}), is a good measure of the liquid water path response to aerosol perturbation ({lambda}), as both Spop and {lambda} strongly depend on the magnitude of autoconversion, a model representation of precipitation formation via collisions among cloud droplets. This provides a method to use satellite observations to constrain cloud lifetime effects in global climate models. S{sub pop} in marine clouds estimated from CloudSat, MODIS and AMSR-E observations is substantially lower than that from global climate models and suggests a liquid water path increase of less than 5% from doubled cloud condensation nuclei concentrations. This implies a substantially smaller impact on shortwave cloud radiative forcing (SWCF) over ocean due to aerosol indirect effects than simulated by current global climate models (a reduction by one-third for one of the conventional aerosol-climate models). Further work is needed to quantify the uncertainties in satellite-derived estimates of S{sub pop} and to examine S{sub pop} in high-resolution models.

Wang, Minghuai; Ghan, Steven J.; Liu, Xiaohong; Ecuyer, Tristan L.; Zhang, Kai; Morrison, H.; Ovchinnikov, Mikhail; Easter, Richard C.; Marchand, Roger; Chand, Duli; Qian, Yun; Penner, Joyce E.

2012-08-15T23:59:59.000Z

131

DOE research on atmospheric aerosols  

SciTech Connect (OSTI)

Atmospheric aerosols are the subject of a significant component of research within DOE`s environmental research activities, mainly under two programs within the Department`s Environmental Sciences Division, the Atmospheric Radiation Measurement (ARM) Program and the Atmospheric Chemistry Program (ACP). Research activities conducted under these programs include laboratory experiments, field measurements, and theoretical and modeling studies. The objectives and scope of these programs are briefly summarized. The ARM Program is the Department`s major research activity focusing on atmospheric processes pertinent to understanding global climate and developing the capability of predicting global climate change in response to energy related activities. The ARM approach consists mainly of testing and improving models using long-term measurements of atmospheric radiation and controlling variables at highly instrumented sites in north central Oklahoma, in the Tropical Western Pacific, and on the North Slope of Alaska. Atmospheric chemistry research within DOE addresses primarily the issue of atmospheric response to emissions from energy-generation sources. As such this program deals with the broad topic known commonly as the atmospheric source-receptor sequence. This sequence consists of all aspects of energy-related pollutants from the time they are emitted from their sources to the time they are redeposited at the Earth`s surface.

Schwartz, S.E.

1995-11-01T23:59:59.000Z

132

Characterizing the formation of secondary organic aerosols  

SciTech Connect (OSTI)

Organic aerosol is an important fraction of the fine particulate matter present in the atmosphere. This organic aerosol comes from a variety of sources; primary organic aerosol emitted directly from combustion process, and secondary aerosol formed in the atmosphere from condensable vapors. This secondary organic aerosol (SOA) can result from both anthropogenic and biogenic sources. In rural areas of the United States, organic aerosols can be a significant part of the aerosol load in the atmosphere. However, the extent to which gas-phase biogenic emissions contribute to this organic load is poorly understood. Such an understanding is crucial to properly apportion the effect of anthropogenic emissions in these rural areas that are sometimes dominated by biogenic sources. To help gain insight on the effect of biogenic emissions on particle concentrations in rural areas, we have been conducting a field measurement program at the University of California Blodgett Forest Research Facility. The field location includes has been used to acquire an extensive suite of measurements resulting in a rich data set, containing a combination of aerosol, organic, and nitrogenous species concentration and meteorological data with a long time record. The field location was established in 1997 by Allen Goldstein, a professor in the Department of Environmental Science, Policy and Management at the University of California at Berkeley to study interactions between the biosphere and the atmosphere. The Goldstein group focuses on measurements of concentrations and whole ecosystem biosphere-atmosphere fluxes for volatile organic compounds (VOC's), oxygenated volatile organic compounds (OVOC's), ozone, carbon dioxide, water vapor, and energy. Another important collaborator at the Blodgett field location is Ronald Cohen, a professor in the Chemistry Department at the University of California at Berkeley. At the Blodgett field location, his group his group performs measurements of the concentrations of important gas phase nitrogen compounds. Experiments have been ongoing at the Blodgett field site since the fall of 2000, and have included portions of the summer and fall of 2001, 2002, and 2003. Analysis of both the gas and particle phase data from the year 2000 show that the particle loading at the site correlates with both biogenic precursors emitted in the forest and anthropogenic precursors advected to the site from Sacramento and the Central Valley of California. Thus the particles at the site are affected by biogenic processing of anthropogenic emissions. Size distribution measurements show that the aerosol at the site has a geometric median diameter of approximately 100 nm. On many days, in the early afternoon, growth of nuclei mode particles (<20 nm) is also observed. These growth events tend to occur on days with lower average temperatures, but are observed throughout the summer. Analysis of the size resolved data for these growth events, combined with typical measured terpene emissions, show that the particle mass measured in these nuclei mode particles could come from oxidation products of biogenic emissions, and can serve as a significant route for SOA partitioning into the particle phase. During periods of each year, the effect of emissions for forest fires can be detected at the Blodgett field location. During the summer of 2002 emissions from the Biscuit fire, a large fire located in Southwest Oregon, was detected in the aerosol data. The results show that increases in particle scattering can be directly related to increased black carbon concentration and an appearance of a larger mode in the aerosol size distribution. These results show that emissions from fires can have significant impact on visibility over large distances. The results also reinforce the view that forest fires can be a significant source of black carbon in the atmosphere, which has important climate and visibility. Continuing work with the 2002 data set, particularly the combination of the aerosol and gas phase data, will continue to provide important information o

Lunden, Melissa; Black, Douglas; Brown, Nancy

2004-02-01T23:59:59.000Z

133

Highly stable aerosol generator  

DOE Patents [OSTI]

An improved compressed air nebulizer has been developed such that a uniform aerosol particle size and concentration may be produced over long time periods. This result is achieved by applying a vacuum pressure to the makeup assembly and by use of a vent tube between the atmosphere and the makeup solution. By applying appropriate vacuum pressures to the makeup solution container and by proper positioning of the vent tube, a constant level of aspirating solution may be maintained within the aspirating assembly with aspirating solution continuously replaced from the makeup solution supply. This device may also be adapted to have a plurality of aerosol generators and only one central makeup assembly. 2 figs.

DeFord, H.S.; Clark, M.L.

1981-11-03T23:59:59.000Z

134

Aerosol Data Sources and Their Roles within PARAGON  

SciTech Connect (OSTI)

We briefly but systematically review major sources of aerosol data, emphasizing suites of measurements that seem most likely to contribute to assessments of global aerosol climate forcing. The strengths and limitations of existing satellite, surface, and aircraft remote-sensing systems are described, along with those of direct sampling networks and ship-based stations. It is evident that an enormous number of aerosol-related observations have been made, on a wide range of spatial and temporal sampling scales, and that many of the key gaps in this collection of data could be filled by technologies that either exist or are expected in the near future. Emphasis must be given to combining remote sensing, in situ, active and passive observations, and integrating them with aerosol chemical transport models, in order to create a more complete environmental picture having sufficient detail to address current climate-forcing questions. The Progressive Aerosol Retrieval and Assimilation Global Observing Network (PARAGON) initiative would provide an organizational framework to meet this goal.

Kahn, Ralph A.; Ogren, J. A.; Ackerman, Thomas P.; Bosenberg, Jens; Charlson, Robert J.; Diner, David J.; Holben, B. N.; Menzies, Robert T.; Miller, Mark A.; Seinfeld, John H.

2004-10-01T23:59:59.000Z

135

Secondary Aerosol: Precursors and Formation Mechanisms. Technical Report on Grant  

SciTech Connect (OSTI)

This project focused on studying trace gases that participate in chemical reactions that form atmospheric aerosols. Ammonium sulfate is a major constituent of these tiny particles, and one important pathway to sulfate formation is oxidation of dissolved sulfur dioxide by hydrogen peroxide in cloud, fog and rainwater. Sulfate aerosols influence the number and size of cloud droplets, and since these factors determine cloud radiative properties, sulfate aerosols also influence climate. Peroxide measurements, in conjunction with those of other gaseous species, can used to distinguish the contribution of in-cloud reaction to new sulfate aerosol formation from gas-phase nucleation reactions. This will lead to more reliable global climate models. We constructed and tested a new 4-channel fluorescence detector for airborne detection of peroxides. We integrated the instrument on the G-1 in January, 2006 and took a test flight in anticipation of the MAX-Mex field program, where we planned to fly under pressurized conditions for the first time. We participated in the 2006 Megacity Initiative: Local and Global Research Observations (MILAGRO) - Megacity Aerosol EXperiment ?? Mexico City (MAX-Mex) field measurement campaign. Peroxide instrumentation was deployed on the DOE G-1 research aircraft based in Veracruz, and at the surface site at Tecamac University.

Weinstein-Lloyd, Judith B

2009-05-04T23:59:59.000Z

136

Electrostatics and radioactive aerosol behavior  

SciTech Connect (OSTI)

Radioactive aerosols differ from their nonradioactive counterparts by their ability to charge themselves by emitting charged particles during the radioactive decay process. Evidence that electrostatics, including this charging process, can affect the transport of the aerosols was summarized previously. Charge distributions and the mean charge for a monodisperse radioactive aerosol have been considered in detail. The principal results of theory to calculate charge distributions on a aerosol with a size distribution, changes to Brownian coagulation rates for an aerosol in a reactor containment, and possible changes to aerosol deposition resulting from the charging will be presented. The main purpose of the work has been to improve calculations of aerosol behavior in reactor containments, but behavior in less ionizing environments will be affected more strongly, and some problems remain to be solved in performing reliable calculations.

Clement, C.F.

1994-12-31T23:59:59.000Z

137

aerosols and climate : uncertainties  

E-Print Network [OSTI]

contributes to creating a level playing field. (BC emissions tradeble like CO2 emissions?) OUTLINE #12;size. policy measures, is even more uncertain (emissions & their chemical fingerprint are uncertain (not just aerosol emissions, not just climate impacts) OUTLINE #12;- Standardization doesn't reduce

138

Results from simulated upper-plenum aerosol transport tests  

SciTech Connect (OSTI)

A series of eight aerosol transport experiments, designated as Aerosol Transport Tests (ATT) A101 through A108, has recently been completed at the Oak Ridge National Laboratory (ORNL). These tests provide a data base for validation of aerosol transport modeling used in the TRAP-MELT2 computer code (Jordan and Kuhlman, 1985), which was developed at Battelle Columbus Laboratories to calculate aerosol/fission-product transport in the reactor coolant system in postulated light-water reactor (LWR) core-melt accidents. Results from tests A103 and A104 have been summarized in a previous paper (Wright and Pattison, 1985a); the present paper discusses results from tests A105 through A108.

Wright, A.L.; Pattison, W.L.

1986-01-01T23:59:59.000Z

139

SAGE II long-term measurements of stratospheric and upper tropospheric aerosols  

SciTech Connect (OSTI)

The Stratospheric Aerosol and Gas Experiment (SAGE) II solar occultation instrument has been making measurements on stratospheric aerosols and gases continually since October 1984. Observations from the SAGE II instrument provide a valuable long-term data set for study of the aerosol in the stratosphere and aerosol and cloud in the upper troposphere. The period of observation covers the decay phase of material injected by the El Chichon volcanic eruption in 1982, the years 1988--1990 when stratospheric aerosol levels approached background levels, and the period after the eruption of Mount Pinatubo in 1991. The Mount Pinatubo eruption caused the largest perturbation in stratospheric aerosol loading in this century, with effects on stratospheric dynamics and chemistry. The SAGE II data sequence shows the global dispersion of aerosols following the Mount Pinatubo eruption, as well as the changes occurring in stratospheric aerosol mass and surface area. The downward transfer of stratospheric aerosols into the upper troposphere following the earlier eruption of El Chichon is clearly visible. Estimates have been made of the amount of volcanic material lying in the upper troposphere and the way in which this varies with latitude and season.

Wang, P.H.; Kent, G.S. [Science and Technology Corp., Hampton, VA (United States); McCormick, M.P.; Thomason, L.W. [NASA Langley Research Center, Hampton, VA (United States). Atmospheric Sciences Div.

1995-12-31T23:59:59.000Z

140

Stumbling Toward Capitalism: The State, Global Production Networks, and the Unexpected Emergence of China's Independent Auto Industry  

E-Print Network [OSTI]

To increase the security of Chinese oil tankers throughChinas Oil Diplomacy: Is it a Global Security Threat? ?s energy security concerns over rapidly growing oil demand

Chang, Crystal Whai-ku

2011-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


141

Global Statistics  

E-Print Network [OSTI]

1996). Globalization in Question: International Economy andGlobalization; Justice; Poverty; Underground Economy; United

Crow, Ben D

2006-01-01T23:59:59.000Z

142

Influence of anthropogenic aerosol on cloud optical depth and albedo shown by satellite measurements  

E-Print Network [OSTI]

- flux of sulfate aerosol from industrial regions of Europe or North America to remote areas of the North- atmosphere system over the industrial period and a cooling influence on climate. Estimates of the global), the negative sign indicating a cooling influence. Such a global mean forcing would more than offset the warming

143

Effective Henry's Law Partitioning and the Salting Constant of Glyoxal in Aerosols Containing Sulfate  

E-Print Network [OSTI]

-resolved measurements of gas-phase and particle-phase concentrations in sulfate- containing aerosols. Two complementary utilizing filter sampling of chamber aerosols followed by HPLC-MS/MS analysis and (2) positive matrix and irreversible condensed-phase reactions of these compounds yield products of lower volatility; e.g. acetal

144

GOME-2 ABSORBING AEROSOL INDEX: STATISTICAL ANALYSIS, COMPARISON TO GOME-1 AND IMPACT OF INSTRUMENT  

E-Print Network [OSTI]

DEGRADATION Lieuwe G. Tilstra, Olaf N.E. Tuinder, and Piet Stammes Royal Netherlands Meteorological Institute the presence of UV-absorbing aerosols. These aerosols are mainly injected into the atmosphere by desert dust that the GOME-2 AAI product is suffering more and more from the effects of instrument degradation. In particular

Tilstra, Gijsbert

145

ARM: 10-minute TEMPORARY Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm  

DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

10-minute TEMPORARY Raman Lidar: aerosol extinction profiles and aerosol optical thickness, from first Ferrare algorithm

Sivaraman, Chitra; Flynn, Connor

146

Experimental study of nuclear workplace aerosol samplers  

E-Print Network [OSTI]

LITERATURE REVIEW Aerosol Losses in an Inlet . Aerosol Losses in a Transport System Aerosol Losses in CAMs Critical Flow Venturi 8 13 15 16 EXPERIMENT PROCEDURE 18 CAM Evaluation Consideration FAS Evaluation Consideration Test Protocol Mixing... Chamber Setup High Speed Aerosol Wind Tunnel Setup Low Speed Aerosol Wind Tunnel Setup Critical Flow Venturi 18 19 21 22 24 25 27 RESULTS AND DISCUSSION Page 28 Aerosol Penetration through Transport Systems and CAM Areal Uniformity Deposits...

Parulian, Antony

2012-06-07T23:59:59.000Z

147

Distinguishing Aerosol Impacts on Climate Over the Past Century  

SciTech Connect (OSTI)

Aerosol direct (DE), indirect (IE), and black carbon-snow albedo (BAE) effects on climate between 1890 and 1995 are compared using equilibrium aerosol-climate simulations in the Goddard Institute for Space Studies General Circulation Model coupled to a mixed layer ocean. Pairs of control(1890)-perturbation(1995) with successive aerosol effects allow isolation of each effect. The experiments are conducted both with and without concurrent changes in greenhouse gases (GHG's). A new scheme allowing dependence of snow albedo on black carbon snow concentration is introduced. The fixed GHG experiments global surface air temperature (SAT) changed -0.2, -1.0 and +0.2 C from the DE, IE, and BAE. Ice and snow cover increased 1.0% from the IE and decreased 0.3% from the BAE. These changes were a factor of 4 larger in the Arctic. Global cloud cover increased by 0.5% from the IE. Net aerosol cooling effects are about half as large as the GHG warming, and their combined climate effects are smaller than the sum of their individual effects. Increasing GHG's did not affect the IE impact on cloud cover, however they decreased aerosol effects on SAT by 20% and on snow/ice cover by 50%; they also obscure the BAE on snow/ice cover. Arctic snow, ice, cloud, and shortwave forcing changes occur mostly during summer-fall, but SAT, sea level pressure, and long-wave forcing changes occur during winter. An explanation is that aerosols impact the cryosphere during the warm-season but the associated SAT effect is delayed until winter.

Koch, Dorothy; Menon, Surabi; Del Genio, Anthony; Ruedy, Reto; Alienov, Igor; Schmidt, Gavin A.

2008-08-22T23:59:59.000Z

148

The oceanic cycle and global atmospheric budget of carbonyl sulfide  

SciTech Connect (OSTI)

A significant portion of stratospheric air chemistry is influenced by the existence of carbonyl sulfide (COS). This ubiquitous sulfur gas represents a major source of sulfur to the stratosphere where it is converted to sulfuric acid aerosol particles. Stratospheric aerosols are climatically important because they scatter incoming solar radiation back to space and are able to increase the catalytic destruction of ozone through gas phase reactions on particle surfaces. COS is primarily formed at the surface of the earth, in both marine and terrestrial environments, and is strongly linked to natural biological processes. However, many gaps in the understanding of the global COS cycle still exist, which has led to a global atmospheric budget that is out of balance by a factor of two or more, and a lack of understanding of how human activity has affected the cycling of this gas. The goal of this study was to focus on COS in the marine environment by investigating production/destruction mechanisms and recalculating the ocean-atmosphere flux.

Weiss, P.S.

1994-12-31T23:59:59.000Z

149

Electrospray neutralization process and apparatus for generation of nano-aerosol and nano-structured materials  

DOE Patents [OSTI]

The claimed invention describes methods and apparatuses for manufacturing nano-aerosols and nano-structured materials based on the neutralization of charged electrosprayed products with oppositely charged electrosprayed products. Electrosprayed products include molecular ions, nano-clusters and nano-fibers. Nano-aerosols can be generated when neutralization occurs in the gas phase. Neutralization of electrospan nano-fibers with molecular ions and charged nano-clusters may result in the formation of fibrous aerosols or free nano-mats. Nano-mats can also be produced on a suitable substrate, forming efficient nano-filters.

Bailey, Charles L. (Cross Junction, VA); Morozov, Victor (Manassas, VA); Vsevolodov, Nikolai N. (Kensington, MD)

2010-08-17T23:59:59.000Z

150

Molecular Characterization of Biomass Burning Aerosols Using...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Biomass Burning Aerosols Using High Resolution Mass Spectrometry. Molecular Characterization of Biomass Burning Aerosols Using High Resolution Mass Spectrometry. Abstract: Chemical...

151

Nonequilibrium Atmospheric Secondary Organic Aerosol Formation...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Aerosol Formation and Growth. Abstract: Airborne particles play a critical role in air quality, human health effects, visibility and climate. Secondary organic aerosols (SOA)...

152

The impact of biogenic carbon emissions on aerosol absorption inMexico City  

SciTech Connect (OSTI)

In order to determine the wavelength dependence of atmospheric aerosol absorption in the Mexico City area, the absorption angstrom exponents (AAEs) were calculated from aerosol absorption measurements at seven wavelengths obtained with a seven-channel aethalometer during two field campaigns, the Mexico City Metropolitan Area study in April 2003 (MCMA 2003) and the Megacity Initiative: Local and Global Research Observations in March 2006 (MILAGRO). The AAEs varied from 0.76 to 1.56 in 2003 and from 0.54 to 1.52 in 2006. The AAE values determined in the afternoon were consistently higher than the corresponding morning values, suggesting the photochemical formation of absorbing secondary organic aerosols (SOA) in the afternoon. The AAE values were compared to stable and radiocarbon isotopic measurements of aerosol samples collected at the same time to determine the sources of the aerosol carbon. The fraction of modern carbon (fM) in the aerosol samples, as determined from {sup 14}C analysis, showed that 70% of the carbonaceous aerosols in Mexico City were from modern sources, indicating a significant impact from biomass burning during both field campaigns. The {sup 13}C/{sup 12}C ratios of the aerosol samples illustrate the significant impact of Yucatan forest fires (C-3 plants) in 2003 and local grass fires (C-4 plants) at site T1 in 2006. A direct comparison of the fM values, stable carbon isotope ratios, and calculated aerosol AAEs suggested that the wavelength dependence of the aerosol absorption was controlled by the biogenically derived aerosol components.

Marley, N; Gaffney, J; Tackett, M J; Sturchio, N; Hearty, L; Martinez, N; Hardy, K D; Machany-Rivera, A; Guilderson, T P; MacMillan, A; Steelman, K

2009-02-24T23:59:59.000Z

153

Global Statistics  

E-Print Network [OSTI]

of Globalization: Statistics Weiss, L. (1997). "of Globalization: Statistics Milanovic, B. (1999). Truethe focus of global statistics, particularly in relation to

Crow, Ben D

2006-01-01T23:59:59.000Z

154

Speciation of Fe in ambient aerosol and cloudwater  

SciTech Connect (OSTI)

Atmospheric iron (Fe) is thought to play an important role in cloudwater chemistry (e.g., S(IV) oxidation, oxidant production, etc.), and is also an important source of Fe to certain regions of the worlds oceans where Fe is believed to be a rate-limiting nutrient for primary productivity. This thesis focuses on understanding the chemistry, speciation and abundance of Fe in cloudwater and aerosol in the troposphere, through observations of Fe speciation in the cloudwater and aerosol samples collected over the continental United States and the Arabian Sea. Different chemical species of atmospheric Fe were measured in aerosol and cloudwater samples to help assess the role of Fe in cloudwater chemistry.

Siefert, L. [California Institute of Technology, Pasadena, CA (United States)

1996-08-15T23:59:59.000Z

155

6, 75197562, 2006 Simulating aerosol  

E-Print Network [OSTI]

, particle number concentration and aerosol size-distribution. The model takes into account sulfate (SO4. This model system enables explicit simulations of the particle number concentration and size-distribution of aerosol dynamical processes (nucleation, condensation, coagulation) is evaluated by comparison

Paris-Sud XI, Université de

156

TROPOSPHERIC AEROSOL PROGRAM, PROGRAM PLAN, MARCH 2001  

SciTech Connect (OSTI)

The goal of Tropospheric Aerosol Program (TAP) will be to develop the fundamental scientific understanding required to construct tools for simulating the life cycle of tropospheric aerosols--the processes controlling their mass loading, composition, and microphysical properties, all as a function of time, location, and altitude. The TAP approach to achieving this goal will be by conducting closely linked field, modeling, laboratory, and theoretical studies focused on the processes controlling formation, growth, transport, and deposition of tropospheric aerosols. This understanding will be represented in models suitable for describing these processes on a variety of geographical scales; evaluation of these models will be a key component of TAP field activities. In carrying out these tasks TAP will work closely with other programs in DOE and in other Federal and state agencies, and with the private sector. A forum to directly work with our counterparts in industry to ensure that the results of this research are translated into products that are useful to that community will be provided by NARSTO (formerly the North American Research Strategy on Tropospheric Ozone), a public/private partnership, whose membership spans government, the utilities, industry, and university researchers in Mexico, the US, and Canada.

SCHWARTZ,S.E.; LUNN,P.

2001-03-01T23:59:59.000Z

157

atmospheric aerosol source-receptor: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

coefficient is 0.5 and then 1.0 2. For the same conditions calculate the H Weber, Rodney 6 Secondary organic aerosol 1. Atmospheric chemical mechanism for production...

158

Overview of the 2010 Carbonaceous Aerosols and Radiative Effects Study (CARES)  

E-Print Network [OSTI]

Substantial uncertainties still exist in the scientific understanding of the possible interactions between urban and natural (biogenic) emissions in the production and transformation of atmospheric aerosol and the resulting ...

Cziczo, Daniel James

159

The Nearby Supernova Factory Ozone + Aerosol + Rayleigh  

E-Print Network [OSTI]

Rayleigh + Aerosol Extinction monitor filter Auxiliary Camera CCD Spectrograph picko ff mirror Umbra

160

Past and Future Effects of Ozone on Net Primary Production and Carbon Sequestration Using a Global Biogeochemical Model  

E-Print Network [OSTI]

Exposure of plants to ozone inhibits photosynthesis and therefore reduces vegetation production and carbon sequestration. Simulations with the Terrestrial Ecosystem Model (TEM) for the historical period (1860-1995) show ...

Felzer, Benjamin Seth.

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


161

High-resolution mass spectrometric analysis of secondary organic aerosol produced by ozonation of limonenew  

E-Print Network [OSTI]

and measured reaction products in the monomer product range. Introduction Atmospheric aerosols impact local air of both monomeric (m/z o 300) and oligomeric (m/z 4 300) condensed products of oxidation. A combination by previous studies. The isomerization reactions yield numerous products with a progressively increasing

Nizkorodov, Sergey

162

aerosol particles collected: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Saller 2002-05-07 6 Nanomaterials from Aerosols Aerosols are suspensions of liquid or solid particles in a gas. Aerosol particles Materials Science Websites Summary: being clouds...

163

Mexico City Aerosol Analysis during MILAGRO using High Resolution...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

2: Mexico City Aerosol Analysis during MILAGRO using High Resolution Aerosol Mass Spectrometry at the Urban Supersite (T0). Part 2: Abstract: Submicron aerosol was analyzed during...

164

Mexico City Aerosol Analysis during MILAGRO using High Resolution...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

1: Mexico City Aerosol Analysis during MILAGRO using High Resolution Aerosol Mass Spectrometry at the Urban Supersite (T0). Part 1: Abstract: Submicron aerosol was analyzed during...

165

Parameterizations of Cloud Microphysics and Indirect Aerosol Effects  

SciTech Connect (OSTI)

1. OVERVIEW Aerosols and especially their effect on clouds are one of the key components of the climate system and the hydrological cycle [Ramanathan et al., 2001]. Yet, the aerosol effect on clouds remains largely unknown and the processes involved not well understood. A recent report published by the National Academy of Science states "The greatest uncertainty about the aerosol climate forcing - indeed, the largest of all the uncertainties about global climate forcing - is probably the indirect effect of aerosols on clouds [NRC, 2001]." The aerosol effect on clouds is often categorized into the traditional "first indirect (i.e., Twomey)" effect on the cloud droplet sizes for a constant liquid water path [Twomey, 1977] and the "semi-direct" effect on cloud coverage [e.g., Ackerman et al., 2000]. Enhanced aerosol concentrations can also suppress warm rain processes by producing a narrow droplet spectrum that inhibits collision and coalescence processes [e.g., Squires and Twomey, 1961; Warner and Twomey, 1967; Warner, 1968; Rosenfeld, 1999]. The aerosol effect on precipitation processes, also known as the second type of aerosol indirect effect [Albrecht, 1989], is even more complex, especially for mixed-phase convective clouds. Table 1 summarizes the key observational studies identifying the microphysical properties, cloud characteristics, thermodynamics and dynamics associated with cloud systems from high-aerosol continental environments. For example, atmospheric aerosol concentrations can influence cloud droplet size distributions, warm-rain process, cold-rain process, cloud-top height, the depth of the mixed phase region, and occurrence of lightning. In addition, high aerosol concentrations in urban environments could affect precipitation variability by providing an enhanced source of cloud condensation nuclei (CCN). Hypotheses have been developed to explain the effect of urban regions on convection and precipitation [van den Heever and Cotton, 2007 and Shepherd, 2005]. Recently, a detailed spectral-bin microphysical scheme was implemented into the Goddard Cumulus Ensemble (GCE) model. Atmospheric aerosols are also described using number density size-distribution functions. A spectral-bin microphysical model is very expensive from a computational point of view and has only been implemented into the 2D version of the GCE at the present time. The model is tested by studying the evolution of deep tropical clouds in the west Pacific warm pool region and summertime convection over a mid-latitude continent with different concentrations of CCN: a low "clean" concentration and a high "dirty" concentration. The impact of atmospheric aerosol concentration on cloud and precipitation will be investigated. 2. MODEL DESCRIPTION AND CASE STUDIES 2.1 GCE MODEL The model used in this study is the 2D version of the GCE model. Modeled flow is anelastic. Second- or higher-order advection schemes can produce negative values in the solution. Thus, a Multi-dimensional Positive Definite Advection Transport Algorithm (MPDATA) has been implemented into the model. All scalar variables (potential temperature, water vapor, turbulent coefficient and all five hydrometeor classes) use forward time differencing and the MPDATA for advection. Dynamic variables, u, v and w, use a second-order accurate advection scheme and a leapfrog time integration (kinetic energy semi-conserving method). Short-wave (solar) and long-wave radiation as well as a subgrid-scale TKE turbulence scheme are also included in the model. Details of the model can be found in Tao and Simpson (1993) and Tao et al. (2003). 2.2 Microphysics (Bin Model) The formulation of the explicit spectral-bin microphysical processes is based on solving stochastic kinetic equations for the size distribution functions of water droplets (cloud droplets and raindrops), and six types of ice particles: pristine ice crystals (columnar and plate-like), snow (dendrites and aggregates), graupel and frozen drops/hail. Each type is described by a special size distribution function containing 33 categories (bin

Tao, Wei-Kuo [NASA/GSFC] [NASA/GSFC

2014-05-19T23:59:59.000Z

166

The China-in-Global Energy Model  

E-Print Network [OSTI]

The China-in-Global Energy Model (C-GEM) is a global Computable General Equilibrium (CGE) model that captures the interaction of production, consumption and trade among multiple global regions and sectors including five ...

Qi, T.

167

Global Development Our Responsibility  

E-Print Network [OSTI]

of expertise cover urgent global issues such as food production, energy supply, climate change, biodiversity e ort to address urgent global issues particularly a ecting developing countries e.g. climate change of Communication, 2012 · Project Leader: Karin Nilsson · Graphic Design: Viktor Wrange & Michael Kvick Cover Photo

168

Production of polystyrene particles via aerosolization  

E-Print Network [OSTI]

that of the blowing agent out of the cells. Conversely, the higher diffusion rates of hydrogen and carbon dioxide leaving cells, compared to the diffusion rate of infiltrating air, may result in shrinkage or partial breakdown of cell walls. Furthermore... in structure. Also, cell shrinkage can take place if the cells are not strong enough to resist the external hydrostatic pressure. Moreover, the exchange of blowing agent for air inside the cells may have a considerable effect on cell structure. For example...

Norasetthekul, Somchintana

1995-01-01T23:59:59.000Z

169

Aerosol reactor production of uniform submicron powders  

DOE Patents [OSTI]

A method of producing submicron nonagglomerated particles in a single stage reactor includes introducing a reactant or mixture of reactants at one end while varying the temperature along the reactor to initiate reactions at a low rate. As homogeneously small numbers of seed particles generated in the initial section of the reactor progress through the reactor, the reaction is gradually accelerated through programmed increases in temperature along the length of the reactor to promote particle growth by chemical vapor deposition while minimizing agglomerate formation by maintaining a sufficiently low number concentration of particles in the reactor such that coagulation is inhibited within the residence time of particles in the reactor. The maximum temperature and minimum residence time is defined by a combination of temperature and residence time that is necessary to bring the reaction to completion. In one embodiment, electronic grade silane and high purity nitrogen are introduced into the reactor and temperatures of approximately 770.degree. K. to 1550.degree. K. are employed. In another embodiment silane and ammonia are employed at temperatures from 750.degree. K. to 1800.degree. K.

Flagan, Richard C. (Pasadena, CA); Wu, Jin J. (Pasadena, CA)

1991-02-19T23:59:59.000Z

170

ARM - Evaluation Product - Aerosol Modeling Testbed  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr May JunDatastreamsmmcrcal Documentation

171

8, 68456901, 2008 Aerosol optical  

E-Print Network [OSTI]

of solar radiation by atmospheric aerosols is a key el- ement of the Earth's radiative energy balance, Germany 2 Helmholtz Center Munich, German Research Center for Environmental Health, Institute

Paris-Sud XI, Université de

172

AEROSOL, CLOUDS, AND CLIMATE CHANGE  

SciTech Connect (OSTI)

Earth's climate is thought to be quite sensitive to changes in radiative fluxes that are quite small in absolute magnitude, a few watts per square meter, and in relation to these fluxes in the natural climate. Atmospheric aerosol particles exert influence on climate directly, by scattering and absorbing radiation, and indirectly by modifying the microphysical properties of clouds and in turn their radiative effects and hydrology. The forcing of climate change by these indirect effects is thought to be quite substantial relative to forcing by incremental concentrations of greenhouse gases, but highly uncertain. Quantification of aerosol indirect forcing by satellite- or ground-based remote sensing has proved quite difficult in view of inherent large variation in the pertinent observables such as cloud optical depth, which is controlled mainly by liquid water path and only secondarily by aerosols. Limited work has shown instances of large magnitude of aerosol indirect forcing, with local instantaneous forcing upwards of 50 W m{sup 66}-2. Ultimately it will be necessary to represent aerosol indirect effects in climate models to accurately identify the anthropogenic forcing at present and over secular time and to assess the influence of this forcing in the context of other forcings of climate change. While the elements of aerosol processes that must be represented in models describing the evolution and properties of aerosol particles that serve as cloud condensation particles are known, many important components of these processes remain to be understood and to be represented in models, and the models evaluated against observation, before such model-based representations can confidently be used to represent aerosol indirect effects in climate models.

SCHWARTZ, S.E.

2005-09-01T23:59:59.000Z

173

Phosphorus associations in aerosols: What can they tell us about P bioavailability? L.D. Anderson a,  

E-Print Network [OSTI]

. Aerosols include both natural components such as mineral dust and anthropogenic components such as bio-burning and diesel fuel by-products. Aerosols from industrialized and urban areas such as Western and Eastern Europe particulates and diesel fuel standards (SRM 1648 and SRM 1650) have high levels of total P (250 mol g-1

Paytan, Adina

174

Estimates of global, regional, and national annual CO{sub 2} emissions from fossil-fuel burning, hydraulic cement production, and gas flaring: 1950--1992  

SciTech Connect (OSTI)

This document describes the compilation, content, and format of the most comprehensive C0{sub 2}-emissions database currently available. The database includes global, regional, and national annual estimates of C0{sub 2} emissions resulting from fossil-fuel burning, cement manufacturing, and gas flaring in oil fields for 1950--92 as well as the energy production, consumption, and trade data used for these estimates. The methods of Marland and Rotty (1983) are used to calculate these emission estimates. For the first time, the methods and data used to calculate CO, emissions from gas flaring are presented. This C0{sub 2}-emissions database is useful for carbon-cycle research, provides estimates of the rate at which fossil-fuel combustion has released C0{sub 2} to the atmosphere, and offers baseline estimates for those countries compiling 1990 C0{sub 2}-emissions inventories.

Boden, T.A.; Marland, G. [Oak Ridge National Lab., TN (United States); Andres, R.J. [University of Alaska, Fairbanks, AK (United States). Inst. of Northern Engineering

1995-12-01T23:59:59.000Z

175

Large historical changes of fossil-fuel black carbon aerosols  

SciTech Connect (OSTI)

Anthropogenic emissions of fine black carbon (BC) particles, the principal light-absorbing atmospheric aerosol, have varied during the past century in response to changes of fossil-fuel utilization, technology developments, and emission controls. We estimate historical trends of fossil-fuel BC emissions in six regions that represent about two-thirds of present day emissions and extrapolate these to global emissions from 1875 onward. Qualitative features in these trends show rapid increase in the latter part of the 1800s, the leveling off in the first half of the 1900s, and the re-acceleration in the past 50 years as China and India developed. We find that historical changes of fuel utilization have caused large temporal change in aerosol absorption, and thus substantial change of aerosol single scatter albedo in some regions, which suggests that BC may have contributed to global temperature changes in the past century. This implies that the BC history needs to be represented realistically in climate change assessments.

Novakov, T.; Ramanathan, V.; Hansen, J.E.; Kirchstetter, T.W.; Sato, M.; Sinton, J.E.; Sathaye, J.A.

2002-09-26T23:59:59.000Z

176

Investigation of warm-cloud microphysics using a multi-component cloud model: Interactive effects of the aerosol spectrum. Master's thesis  

SciTech Connect (OSTI)

Clouds, especially low, warm, boundary-layer clouds, play an important role in regulating the earth's climate due to their significant contribution to the global albedo. The radiative effects of individual clouds are controlled largely by cloud microstructure, which is itself sensitive to the concentration and spectral distribution of the atmospheric aerosol. Increases in aerosol particle concentrations from anthropogenic activity could result in increased cloud albedo and global cloudiness, increasing the amount of reflected solar radiation. However, the effects of increased aerosol particle concentrations could be offset by the presence of giant or ultragiant aerosol particles. A one-dimensional, multi-component microphysical cloud model has been used to demonstrate the effects of aerosol particle spectral variations on the microstructure of warm clouds. Simulations performed with this model demonstrate that the introduction of increased concentrations of giant aerosol particles has a destabilizing effect on the cloud microstructure. Also, it is shown that warm-cloud microphysical processes modify the aerosol particle spectrum, favoring the generation of the largest sized particles via the collision-coalescence process. These simulations provide further evidence that the effect of aerosol particles on cloud microstructure must be addressed when considering global climate forecasts.

Zahn, S.G.

1993-12-01T23:59:59.000Z

177

A New Aerosol Flow System for Photochemical and Thermal Studies of Tropospheric Aerosols  

SciTech Connect (OSTI)

For studying the formation and photochemical/thermal reactions of aerosols relevant to the troposphere, a unique, high-volume, slow-flow, stainless steel aerosol flow system equipped with 5 UV lamps has been constructed and characterized experimentally. The total flow system length 6 is 8.5 m and includes a 1.2 m section used for mixing, a 6.1 m reaction section and a 1.2 m 7 transition cone at the end. The 45.7 cm diameter results in a smaller surface to volume ratio than is found in many other flow systems and thus reduces the potential contribution from wall reactions. The latter are also reduced by frequent cleaning of the flow tube walls which is made feasible by the ease of disassembly. The flow tube is equipped with ultraviolet lamps for photolysis. This flow system allows continuous sampling under stable conditions, thus increasing the amount of sample available for analysis and permitting a wide variety of analytical techniques to be applied simultaneously. The residence time is of the order of an hour, and sampling ports located along the length of the flow tube allow for time-resolved measurements of aerosol and gas-phase products. The system was characterized using both an inert gas (CO2) and particles (atomized NaNO3). Instruments interfaced directly to this flow system include a NOx analyzer, an ozone analyzer, relative humidity and temperature probes, a scanning mobility particle sizer spectrometer, an aerodynamic particle sizer spectrometer, a gas chromatograph-mass spectrometer, an integrating nephelometer, and a Fourier transform infrared spectrophotometer equipped with a long path (64 m) cell. Particles collected with impactors and filters at the various sampling ports can be analyzed subsequently by a variety of techniques. Formation of secondary organic aerosol from ?-pinene reactions (NOx photooxidation and ozonolysis) are used to demonstrate the capabilities of this new system.

Ezell, Michael J.; Johnson, Stanley N.; Yu, Yong; Perraud, Veronique; Bruns, Emily; Alexander, M. L.; Zelenyuk, Alla; Dabdub, Donald; Finlayson-Pitts, Barbara J.

2010-05-01T23:59:59.000Z

178

Direct and semi-direct aerosol effects of Southern African1 biomass burning aerosol2  

E-Print Network [OSTI]

1 Direct and semi-direct aerosol effects of Southern African1 biomass burning aerosol2 Naoko effects of biomass burning aerosols from Southern African fires9 during July-October are investigated region the overall TOA radiative effect from the23 biomass burning aerosols is almost zero due

Wood, Robert

179

A model simulation of Pinatubo volcanic aerosols in the stratosphere  

SciTech Connect (OSTI)

A one-dimensional, time-dependent model is used to study the chemical, microphysical, and radiative properties of volcanic aerosols produced by the Mount Pinatubo eruption on June 15, 1991. The authors` model treats gas-phase sulfur photochemistry, gas-to-particle conversion of sulfur, and the microphysics of sulfate aerosols and ash particles under stratospheric conditions. The dilution and diffusion of the volcanic eruption clouds are also accounted for in these conditions. Heteromolecular homogeneous and heterogeneous binary H{sub 2}SO{sub 4}/H{sub 2}O nucleation, acid and water condensational growth, coagulation, and gravitational sedimentation are treated in detail in the model. Simulations suggested that after several weeks, the volcanic cloud was composed mainly of sulfuric acid/water droplets produced in situ from the SO{sub 2} emissions. The large amounts of SO{sub 2} (around 20 Mt) injected into the stratosphere by the Pinatubo eruption initiated homogeneous nucleation which generated a high concentration of small H{sub 2}SO{sub 4}/H{sub 2}O droplets. These newly formed particles grew rapidly by condensation and coagulation in the first few months and then reached their stabilized sizes with effective radii in a range between 0.3 and 0.5 {mu}m approximately one-half year after the eruption. The predicted volcanic cloud parameters reasonably agree with measurements in term of the vertical distribution and lifetime of the volcanic aerosols, their basic microphysical structures (e.g., size distribution, concentration, mass ratio, and surface area) and radiative properties. The persistent volcanic aerosols can produce significant anomalies in the radiation field, which have important climatic consequences. The large enhancement in aerosol surface area can result in measurable global stratospheric ozone depletion. 57 refs., 15 figs., 1 tab.

Zhao, J. [Univ. of Hawaii, Honolulu, HI (United States)] [Univ. of Hawaii, Honolulu, HI (United States); Turco, R.P. [Univ. of California, Los Angeles, CA (United States)] [Univ. of California, Los Angeles, CA (United States); Toon, O.B. [NASA Ames Research Center, Moffett Field, CA (United States)] [NASA Ames Research Center, Moffett Field, CA (United States)

1995-04-20T23:59:59.000Z

180

Composition and Reactions of Atmospheric Aerosol Particles  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Source type and mechanism information for the four aerosol samples gathered from the Caribbean, the Sea of Japan, and New Jersey. One way to gauge an aerosol's ability to stay...

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


181

Aerosol indirect effects -- general circulation model intercomparison and evaluation with satellite data  

SciTech Connect (OSTI)

Aerosol indirect effects continue to constitute one of the most important uncertainties for anthropogenic climate perturbations. Within the international AEROCOM initiative, the representation of aerosol-cloud-radiation interactions in ten different general circulation models (GCMs) is evaluated using three satellite datasets. The focus is on stratiform liquid water clouds since most GCMs do not include ice nucleation effects, and none of the model explicitly parameterizes aerosol effects on convective clouds. We compute statistical relationships between aerosol optical depth (Ta) and various cloud and radiation quantities in a manner that is consistent between the models and the satellite data. It is found that the model-simulated influence of aerosols on cloud droplet number concentration (Nd) compares relatively well to the satellite data at least over the ocean. The relationship between Ta and liquid water path is simulated much too strongly by the models. It is shown that this is partly related to the representation of the second aerosol indirect effect in terms of autoconversion. A positive relationship between total cloud fraction (fcld) and Ta as found in the satellite data is simulated by the majority of the models, albeit less strongly than that in the satellite data in most of them. In a discussion of the hypotheses proposed in the literature to explain the satellite-derived strong fcld - Ta relationship, our results indicate that none can be identified as unique explanation. Relationships similar to the ones found in satellite data between Ta and cloud top temperature or outgoing long-wave radiation (OLR) are simulated by only a few GCMs. The GCMs that simulate a negative OLR - Ta relationship show a strong positive correlation between Ta and fcld The short-wave total aerosol radiative forcing as simulated by the GCMs is strongly influenced by the simulated anthropogenic fraction of Ta, and parameterisation assumptions such as a lower bound on Nd. Nevertheless, the strengths of the statistical relationships are good predictors for the aerosol forcings in the models. An estimate of the total short-wave aerosol forcing inferred from the combination of these predictors for the modelled forcings with the satellite-derived statistical relationships yields a global annual mean value of -1.5+-0.5 Wm-2. An alternative estimate obtained by scaling the simulated clear- and cloudy-sky forcings with estimates of anthropogenic Ta and satellite-retrieved Nd - Ta regression slopes, respectively, yields a global annual mean clear-sky (aerosol direct effect) estimate of -0.4+-0.2 Wm-2 and a cloudy-sky (aerosol indirect effect) estimate of -0.7+-0.5 Wm-2, with a total estimate of -1.2+-0.4 Wm-2.

Quaas, Johannes; Ming, Yi; Menon, Surabi; Takemura, Toshihiko; Wang, Minghuai; Penner, Joyce E.; Gettelman, Andrew; Lohmann, Ulrike; Bellouin, Nicolas; Boucher, Olivier; Sayer, Andrew M.; Thomas, Gareth E.; McComiskey, Allison; Feingold, Graham; Hoose, Corinna; Kristjansson, Jon Egill; Liu, Xiaohong; Balkanski, Yves; Donner, Leo J.; Ginoux, Paul A.; Stier, Philip; Feichter, Johann; Sednev, Igor; Bauer, Susanne E.; Koch, Dorothy; Grainger, Roy G.; Kirkevag, Alf; Iversen, Trond; Seland, Oyvind; Easter, Richard; Ghan, Steven J.; Rasch, Philip J.; Morrison, Hugh; Lamarque, Jean-Francois; Iacono, Michael J.; Kinne, Stefan; Schulz, Michael

2009-04-10T23:59:59.000Z

182

CHARACTERIZING THE INFLUENCE OF ANTHROPOGENIC EMISSIONS AND TRANSPORT VARIABILITY ON SULFATE AEROSOL CONCENTRATIONS AT MAUNA  

E-Print Network [OSTI]

CONCENTRATIONS AT MAUNA LOA OBSERVATORY Sulfate aerosol in the atmosphere has substantial impacts on human health confirmed that anthropogenic pollutants from Asian sources can be transported long distances with important implications for future air quality and global climate change. Located in the remote Pacific Ocean (19.54°N

Pierce, Jeffrey

183

Direct radiative forcing due to aerosols in Asia during Soon-Ung Parka,, Jaein I. Jeongb  

E-Print Network [OSTI]

Direct radiative forcing due to aerosols in Asia during March 2002 Soon-Ung Parka,, Jaein I. Jeongb Model (CRM) of Community Climate Model 3 and the output of the fifth generation of meso-scale model (MM5 in the global climate system by changing atmospheric radiation balance (Tegen and Fung, 1994; Andreae, 1996; Li

Park, Rokjin

184

Potential Land Use Implications of a Global Biofuels Industry  

E-Print Network [OSTI]

In this paper we investigate the potential production and implications of a global biofuels industry. We

Gurgel, Angelo C.

185

Global climate feedbacks  

SciTech Connect (OSTI)

The important physical, chemical, and biological events that affect global climate change occur on a mesoscale -- requiring high spatial resolution for their analysis. The Department of Energy has formulated two major initiatives under the US Global Change Program: ARM (Atmospheric Radiation Measurements), and CHAMMP (Computer Hardware Advanced Mathematics and Model Physics). ARM is designed to use ground and air-craft based observations to document profiles of atmospheric composition, clouds, and radiative fluxes. With research and models of important physical processes, ARM will delineate the relationships between trace gases, aerosol and cloud structure, and radiative transfer in the atmosphere, and will improve the parameterization of global circulation models. The present GCMs do not model important feedbacks, including those from clouds, oceans, and land processes. The purpose of this workshop is to identify such potential feedbacks, to evaluate the uncertainties in the feedback processes (and, if possible, to parameterize the feedback processes so that they can be treated in a GCM), and to recommend research programs that will reduce the uncertainties in important feedback processes. Individual reports are processed separately for the data bases.

Manowitz, B.

1990-10-01T23:59:59.000Z

186

Hyperspectral Aerosol Optical Depths from TCAP Flights  

SciTech Connect (OSTI)

4STAR (Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research), the worlds first hyperspectral airborne tracking sunphotometer, acquired aerosol optical depths (AOD) at 1 Hz during all July 2012 flights of the Two Column Aerosol Project (TCAP). Root-mean square differences from AERONET ground-based observations were 0.01 at wavelengths between 500-1020 nm, 0.02 at 380 and 1640 nm and 0.03 at 440 nm in four clear-sky fly-over events, and similar in ground side-by-side comparisons. Changes in the above-aircraft AOD across 3-km-deep spirals were typically consistent with integrals of coincident in situ (on DOE Gulfstream 1 with 4STAR) and lidar (on NASA B200) extinction measurements within 0.01, 0.03, 0.01, 0.02, 0.02, 0.02 at 355, 450, 532, 550, 700, 1064 nm, respectively, despite atmospheric variations and combined measurement uncertainties. Finer vertical differentials of the 4STAR measurements matched the in situ ambient extinction profile within 14% for one homogeneous column. For the AOD observed between 350-1660 nm, excluding strong water vapor and oxygen absorption bands, estimated uncertainties were ~0.01 and dominated by (then) unpredictable throughput changes, up to +/-0.8%, of the fiber optic rotary joint. The favorable intercomparisons herald 4STARs spatially-resolved high-frequency hyperspectral products as a reliable tool for climate studies and satellite validation.

Shinozuka, Yohei; Johnson, Roy R.; Flynn, Connor J.; Russell, P. B.; Schmid, Beat; Redemann, Jens; Dunagan, Stephen; Kluzek, Celine D.; Hubbe, John M.; Segal-Rosenheimer, Michal; Livingston, J. M.; Eck, T.; Wagener, Richard; Gregory, L.; Chand, Duli; Berg, Larry K.; Rogers, Ray; Ferrare, R. A.; Hair, John; Hostetler, Chris A.; Burton, S. P.

2013-11-13T23:59:59.000Z

187

Production  

Broader source: Energy.gov [DOE]

Algae production R&D focuses on exploring resource use and availability, algal biomass development and improvements, characterizing algal biomass components, and the ecology and engineering of...

188

Spatial characteristics of the difference between MISR and MODIS aerosol optical depth retrievals over mainland Southeast Asia  

E-Print Network [OSTI]

autoregressive (SAR) model Spatial clustering Data assimilation Mainland Southeast Asia The difference between satellite, aerosol products generated using data from these two sensors often exhibit noticeable differences Resolution Imaging Spectroradiometer (MODIS) aboard the NASA Earth Observation System's Terra satellite

Shi, Tao

189

Spent fuel sabotage aerosol test program :FY 2005-06 testing and aerosol data summary.  

SciTech Connect (OSTI)

This multinational, multi-phase spent fuel sabotage test program is quantifying the aerosol particles produced when the products of a high energy density device (HEDD) interact with and explosively particulate test rodlets that contain pellets of either surrogate materials or actual spent fuel. This program has been underway for several years. This program provides source-term data that are relevant to some sabotage scenarios in relation to spent fuel transport and storage casks, and associated risk assessments. This document focuses on an updated description of the test program and test components for all work and plans made, or revised, primarily during FY 2005 and about the first two-thirds of FY 2006. It also serves as a program status report as of the end of May 2006. We provide details on the significant findings on aerosol results and observations from the recently completed Phase 2 surrogate material tests using cerium oxide ceramic pellets in test rodlets plus non-radioactive fission product dopants. Results include: respirable fractions produced; amounts, nuclide content, and produced particle size distributions and morphology; status on determination of the spent fuel ratio, SFR (the ratio of respirable particles from real spent fuel/respirables from surrogate spent fuel, measured under closely matched test conditions, in a contained test chamber); and, measurements of enhanced volatile fission product species sorption onto respirable particles. We discuss progress and results for the first three, recently performed Phase 3 tests using depleted uranium oxide, DUO{sub 2}, test rodlets. We will also review the status of preparations and the final Phase 4 tests in this program, using short rodlets containing actual spent fuel from U.S. PWR reactors, with both high- and lower-burnup fuel. These data plus testing results and design are tailored to support and guide, follow-on computer modeling of aerosol dispersal hazards and radiological consequence assessments. This spent fuel sabotage--aerosol test program, performed primarily at Sandia National Laboratories, with support provided by both the U.S. Department of Energy and the Nuclear Regulatory Commission, had significant inputs from, and is strongly supported and coordinated by both the U.S. and international program participants in Germany, France, and the U.K., as part of the international Working Group for Sabotage Concerns of Transport and Storage Casks, WGSTSC.

Gregson, Michael Warren; Brockmann, John E.; Nolte, O. (Fraunhofer institut fur toxikologie und experimentelle Medizin, Germany); Loiseau, O. (Institut de radioprotection et de Surete Nucleaire, France); Koch, W. (Fraunhofer institut fur toxikologie und experimentelle Medizin, Germany); Molecke, Martin Alan; Autrusson, Bruno (Institut de radioprotection et de Surete Nucleaire, France); Pretzsch, Gunter Guido (Gesellschaft fur anlagen- und Reaktorsicherheit, Germany); Billone, M. C. (Argonne National Laboratory, USA); Lucero, Daniel A.; Burtseva, T. (Argonne National Laboratory, USA); Brucher, W (Gesellschaft fur anlagen- und Reaktorsicherheit, Germany); Steyskal, Michele D.

2006-10-01T23:59:59.000Z

190

PARAGON - An Integrated Approach for Characterizing Aerosol Climate Impacts and Environmental Interactions  

SciTech Connect (OSTI)

Aerosols exert myriad influences on the Earth?s environment and climate and on human health. The complexity of aerosol-related processes requires that information gathered to improve our understanding of climate change must originate from multiple sources, and that effective strategies for data integration need to be established. Currently, the aerosol community lacks the necessary tools and infrastructure to reap maximum scientific benefit from a vast array of observed and modeled data. Spatial and temporal sampling differences among a diverse set of sensors, nonuniform data qualities, aerosol mesoscale variabilities, and difficulties in separating cloud effects are some of the challenges that need to be addressed. A sustained, long-term program also requires maintaining consistently well-understood accuracies as measurement approaches evolve and improve. Achieving a comprehensive understanding of how aerosol physical, chemical, and radiative processes impact the Earth system can only be achieved through a multidisciplinary, interagency, and international initiative capable of dealing with these issues. A systematic approach, capitalizing on modern measurement and modeling techniques, geospatial statistics methodologies, and high-performance information technologies can provide the necessary machinery to support this objective. We outline a framework for integrating and interpreting observations and models and establishing an accurate, consistent and cohesive long-term record, following a strategy whereby information and tools of progressively greater sophistication are incorporated as problems of increasing complexity are tackled. This concept is named the Progressive Aerosol Retrieval and Assimilation Global Observing Network (PARAGON). To encompass the breadth of effort required, we present a set of recommendations dealing with data interoperability, integration, synergy, summarization and mining, model evaluation, calibration and validation, augmentation of surface and in situ measurements, advances in passive and active remote sensing, and design of satellite missions. Without an initiative of this nature, the scientific and policy communities will continue to struggle with understanding the quantitative impact of complex aerosol processes on regional and global climate change and air quality.

Diner, David J.; Ackerman, Thomas P.; Anderson, Theodore L.; Bosenberg, Jens; Braverman, Amy J.; Charlson, Robert J.; Collins, William D.; Davies, Roger; Holben, B. N.; Hostetler, Chris A.; Kahn, Ralph A.; Martonchik, John V.; Menzies, Robert T.; Miller, Mark A.; Ogren, J. A.; Penner, Joyce E.; Rasch, P; Schwartz, Stephen E.; Seinfeld, John H.; Stephens, Graeme L.; Torres, Omar; Travis, Larry D.; Wielicki, Bruce A.; Yu, Bin

2004-10-01T23:59:59.000Z

191

Review of models applicable to accident aerosols  

SciTech Connect (OSTI)

Estimations of potential airborne-particle releases are essential in safety assessments of nuclear-fuel facilities. This report is a review of aerosol behavior models that have potential applications for predicting aerosol characteristics in compartments containing accident-generated aerosol sources. Such characterization of the accident-generated aerosols is a necessary step toward estimating their eventual release in any accident scenario. Existing aerosol models can predict the size distribution, concentration, and composition of aerosols as they are acted on by ventilation, diffusion, gravity, coagulation, and other phenomena. Models developed in the fields of fluid mechanics, indoor air pollution, and nuclear-reactor accidents are reviewed with this nuclear fuel facility application in mind. The various capabilities of modeling aerosol behavior are tabulated and discussed, and recommendations are made for applying the models to problems of differing complexity.

Glissmeyer, J.A.

1983-07-01T23:59:59.000Z

192

Aerosol-cloud Interactions from Urban, Regional, to Global Scales  

E-Print Network [OSTI]

&M University help me tackle several technical problems. Special thanks go to Jiwen Fan from Pacific Northwest National Laboratory, who offered me substantial helps during my visit to PNNL. I also benefits a lot from the collaboration with Minghuai Wang from... PNNL to analyze the results from the super-parameterized climate model. I also want to extend my gratitude to the National Aeronautics and Space Administration fellowship program, which provided me a three-year funding support. vii TABLE...

Wang, Yuan

2013-07-30T23:59:59.000Z

193

Production  

Broader source: Energy.gov [DOE]

Algae production R&D focuses on exploring resource use and availability, algal biomass development and improvements, characterizing algal biomass components, and the ecology and engineering of cultivation systems.

194

Linearity of Climate Response to Increases in Black Carbon Aerosols  

SciTech Connect (OSTI)

The impact of absorbing aerosols on global climate are not completely understood. Here, we present results of idealized experiments conducted with the Community Atmosphere Model (CAM4) coupled to a slab ocean model (CAM4-SOM) to simulate the climate response to increases in tropospheric black carbon aerosols (BC) by direct and semi-direct effects. CAM4-SOM was forced with 0, 1x, 2x, 5x and 10x an estimate of the present day concentration of BC while maintaining their estimated present day global spatial and vertical distribution. The top of the atmosphere (TOA) radiative forcing of BC in these experiments is positive (warming) and increases linearly as the BC burden increases. The total semi-direct effect for the 1x experiment is positive but becomes increasingly negative for higher BC concentrations. The global average surface temperature response is found to be a linear function of the TOA radiative forcing. The climate sensitivity to BC from these experiments is estimated to be 0.42 K $\\textnormal W^{-1} m^{2}$ when the semi-direct effects are accounted for and 0.22 K $\\textnormal W^{-1} m^{2}$ with only the direct effects considered. Global average precipitation decreases linearly as BC increases, with a precipitation sensitivity to atmospheric absorption of 0.4 $\\%$ $\\textnormal W^{-1} \\textnormal m^{2}$ . The hemispheric asymmetry of BC also causes an increase in southward cross-equatorial heat transport and a resulting northward shift of the inter-tropical convergence zone in the simulations at a rate of 4$^{\\circ}$N $\\textnormal PW^{-1}$. Global average mid- and high-level clouds decrease, whereas the low-level clouds increase linearly with BC. The increase in marine stratocumulus cloud fraction over the south tropical Atlantic is caused by increased BC-induced diabatic heating of the free troposphere.

Mahajan, Salil [ORNL; Evans, Katherine J [ORNL; Hack, James J [ORNL; Truesdale, John [National Center for Atmospheric Research (NCAR)

2013-01-01T23:59:59.000Z

195

Going Global: Tight Oil Production  

Annual Energy Outlook 2013 [U.S. Energy Information Administration (EIA)]

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr May Jun Jul(Summary) " ,"ClickPipelines AboutDecember 2005 (Thousand9,0, 1997Environment >7,99 DiagramLearnOutlook Mary

196

Remote sensing of terrestrial tropospheric aerosols from aircraft and satellites  

E-Print Network [OSTI]

Remote sensing of terrestrial tropospheric aerosols from aircraft and satellites M I Mishchenko1 instruments suitable for aerosol remote sensing and give examples of aerosol retrievals obtained forcing directly by absorbing and reflecting sunlight, thereby cooling or heating the atmosphere

197

Assessing historical global sulfur emission patterns for the period 1850--1990  

SciTech Connect (OSTI)

Anthropogenic sulfur dioxide emissions from energy-producing and metal production activities have become an important factor in better understanding the relationship between humans and the environment. Concerns about (1) acid rain effects on the environment and (2) anthropogenic aerosols affecting possible global change have prompted interest in the transformation and fate of sulfur in the environment. One step in assessing the importance of sulfur emissions is the development of a reliable regional emission inventory of sulfur as a function of time. The objective of this research effort was to create a homogeneous database for historical sulfur emission estimates for the world. The time from 1850--1990 was selected to include the period of industrialization form the time the main production of fuels and minerals began until the most recent year for which complete production data exist. This research effort attempts to correct some of the deficiencies associated with previous global sulfur emission estimates by (1) identifying those production activities that resulted in sulfur emissions by country and (2) calculating historical emission trends by country across years. An important component of this study was the comparison of the sulfur emission results with those of previous studies.

Lefohn, A.S. [A.S.L. and Associates, Helena, MT (United States); Husar, J.D.; Husar, R.B. [Washington Univ., St. Louis, MO (United States). Center for Air Pollution Impact and Trend Analysis; Brimblecombe, P. [Univ. of East Anglia, Norwich (United Kingdom)

1996-07-19T23:59:59.000Z

198

Optimization of aerosol penetration through transport lines  

E-Print Network [OSTI]

will be minimum and -' he penetration of aerosols through the transport system will be maximal. It is the purpose of the study reported herein to experimentally investigate the optimization of aerosol penetration through transport systems and to obtain a... numbers less than 869, bounded the use of this model to Reynolds numbers less than or equal to 1100. 19 IV. SUNNARY OF WORK AND EXPERINENTAL NETHODOLOGY The purpose of the study reported herein was to further analyze the optimization of aerosol...

Wong Luque, Fermin Samuel

1992-01-01T23:59:59.000Z

199

Direct and semidirect aerosol effects of southern African biomass burning aerosol  

E-Print Network [OSTI]

Direct and semidirect aerosol effects of southern African biomass burning aerosol Naoko Sakaeda,1 2011; published 21 June 2011. [1] Direct and semidirect radiative effects of biomass burning aerosols static stability. Over the entire region the overall TOA radiative effect from the biomass burning

Wood, Robert

200

EMSL - Atmospheric Aerosol Systems  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr May JunDatastreamsmmcrcalgovInstrumentsruc DocumentationP-Series to UserProduct:DirectivesSAND2015-21271 7 6 EIA-176Page 1What's New

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


201

Researchers Model Impact of Aerosols Over California  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Impact of Aerosols Over California Research may clarify the effectiveness of regional pollution controls May 28, 2013 | Tags: Climate Research, Hopper Contact: Linda Vu,...

202

Separating Cloud Forming Nuclei from Interstitial Aerosol  

SciTech Connect (OSTI)

It has become important to characterize the physicochemical properties of aerosol that have initiated the warm and ice clouds. The data is urgently needed to better represent the aerosol-cloud interaction mechanisms in the climate models. The laboratory and in-situ techniques to separate precisely the aerosol particles that act as cloud condensation nuclei (CCN) and ice nuclei (IN), termed as cloud nuclei (CN) henceforth, have become imperative in studying aerosol effects on clouds and the environment. This review summarizes these techniques, design considerations, associated artifacts and challenges, and briefly discusses the need for improved designs to expand the CN measurement database.

Kulkarni, Gourihar R.

2012-09-12T23:59:59.000Z

203

Indirect and Semi-Direct Aerosol Campaign  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

October? 2. To what extent do the different properties of the Arctic aerosol during April produce differences in clouds? * Do the more polluted conditions during April in the...

204

Unintended consequences of atmospheric injection of sulphate aerosols.  

SciTech Connect (OSTI)

Most climate scientists believe that climate geoengineering is best considered as a potential complement to the mitigation of CO{sub 2} emissions, rather than as an alternative to it. Strong mitigation could achieve the equivalent of up to -4Wm{sup -2} radiative forcing on the century timescale, relative to a worst case scenario for rising CO{sub 2}. However, to tackle the remaining 3Wm{sup -2}, which are likely even in a best case scenario of strongly mitigated CO{sub 2} releases, a number of geoengineering options show promise. Injecting stratospheric aerosols is one of the least expensive and, potentially, most effective approaches and for that reason an examination of the possible unintended consequences of the implementation of atmospheric injections of sulphate aerosols was made. Chief among these are: reductions in rainfall, slowing of atmospheric ozone rebound, and differential changes in weather patterns. At the same time, there will be an increase in plant productivity. Lastly, because atmospheric sulphate injection would not mitigate ocean acidification, another side effect of fossil fuel burning, it would provide only a partial solution. Future research should aim at ameliorating the possible negative unintended consequences of atmospheric injections of sulphate injection. This might include modeling the optimum rate and particle type and size of aerosol injection, as well as the latitudinal, longitudinal and altitude of injection sites, to balance radiative forcing to decrease negative regional impacts. Similarly, future research might include modeling the optimum rate of decrease and location of injection sites to be closed to reduce or slow rapid warming upon aerosol injection cessation. A fruitful area for future research might be system modeling to enhance the possible positive increases in agricultural productivity. All such modeling must be supported by data collection and laboratory and field testing to enable iterative modeling to increase the accuracy and precision of the models, while reducing epistemic uncertainties.

Brady, Patrick Vane; Kobos, Peter Holmes; Goldstein, Barry

2010-10-01T23:59:59.000Z

205

Comparative Analysis of Urban Atmospheric Aerosol by Particle...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Analysis of Urban Atmospheric Aerosol by Particle-Induced X-ray Emission (PIXE), Proton Elastic Scattering Analysis Comparative Analysis of Urban Atmospheric Aerosol by...

206

Reduction in biomass burning aerosol light absorption upon humidificat...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

in biomass burning aerosol light absorption upon humidification: Roles of inorganically-induced hygroscopicity, Reduction in biomass burning aerosol light absorption upon...

207

aerosol optical thickness: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

of solar radiation by atmospheric aerosols is a key el- ement of the Earth's radiative energy balance and climate. The optical properties of aerosol particles are, however,...

208

aerosol black carbon: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

of solar radiation by atmospheric aerosols is a key el- ement of the Earth's radiative energy balance and climate. The optical properties of aerosol particles are, however,...

209

The Indirect and Semi-Direct Aerosol Campaign  

ScienceCinema (OSTI)

Research projects like the Indirect and Semi-Direct Aerosol Campaign, or ISDAC, increase our knowledge of atmospheric aerosol particles and cloud physics.

Ghan, Steve

2014-06-12T23:59:59.000Z

210

ambient ultrafine aerosols: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

soluble in water: 2. Isolation of acid, neutral, and basic fractions by modified size Weber, Rodney 4 Ambient aerosol sampling using the Aerodyne Aerosol Mass Spectrometer...

211

The Indirect and Semi-Direct Aerosol Campaign  

SciTech Connect (OSTI)

Research projects like the Indirect and Semi-Direct Aerosol Campaign, or ISDAC, increase our knowledge of atmospheric aerosol particles and cloud physics.

Ghan, Steve

2014-03-24T23:59:59.000Z

212

Synergy between Secondary Organic Aerosols and Long Range Transport...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

between Secondary Organic Aerosols and Long Range Transport of Polycyclic Aromatic Hydrocarbons. Synergy between Secondary Organic Aerosols and Long Range Transport of Polycyclic...

213

acid aerosol exposure: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Nenes, Athanasios 8 Neutralization of soil aerosol and its impact on the distribution of acid rain over east Asia Geosciences Websites Summary: Neutralization of soil aerosol and...

214

Aerosol Composition and Source Apportionment in the Mexico City...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Aerosol Composition and Source Apportionment in the Mexico City Metropolitan Area with PIXEPESASTIM and Multivariate Analysis. Aerosol Composition and Source Apportionment in the...

215

Molecular Chemistry of Organic Aerosols Through the Application...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Chemistry of Organic Aerosols Through the Application of High Resolution Mass Spectrometry. Molecular Chemistry of Organic Aerosols Through the Application of High Resolution Mass...

216

aerosol samples collected: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

elements analysis of aerosol samples from some CiteSeer Summary: Aerosols deposits on filters from ten Romanian towns with different kinds and levels of industrial development...

217

Optical, physical, and chemical properties of springtime aerosol...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Optical, physical, and chemical properties of springtime aerosol over Barrow Alaska in 2008. Optical, physical, and chemical properties of springtime aerosol over Barrow Alaska in...

218

aerosolized pentamidine effect: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

ON CCN CONCENTRATION AND AEROSOL FIRST INDIRECT RADIATIVE composition, aerosol size distribution is the more dominant parameter on CCN activation Feingold, GRL 2003;...

219

aerosols radioactifs artificiels: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

ON CCN CONCENTRATION AND AEROSOL FIRST INDIRECT RADIATIVE composition, aerosol size distribution is the more dominant parameter on CCN activation Feingold, GRL 2003;...

220

aerosol particle analysis: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Summary: data analysis algorithm is presented. Our earlier algorithm assumed a monomodal aerosol size distribution, while the new algorithm allows us to partition the aerosol...

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


221

aerosol research study: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

in atmospheric thermal structure, burning, bio-sources changes? 12;Aerosol microphysics: size distribution, mixing state, morphology, shape 9 Aerosol Science and Technology,...

222

Building America Webinar: Sealing of Home Enclosures with Aerosol...  

Energy Savers [EERE]

Sealing of Home Enclosures with Aerosol Particles Building America Webinar: Sealing of Home Enclosures with Aerosol Particles This webinar was presented by research team Building...

223

The dependence of ice microphysics on aerosol concentration in...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

The dependence of ice microphysics on aerosol concentration in arctic mixed-phase stratus clouds during ISDAC and M-PACE. The dependence of ice microphysics on aerosol...

224

Iron Speciation and Mixing in Single Aerosol Particles from the Asian Continental Outflow  

SciTech Connect (OSTI)

Bioavailable iron from atmospheric aerosol is an essential nutrient that can control oceanic productivity, thereby impacting the global carbon budget and climate. Particles collected on Okinawa Island during an atmospheric pollution transport event from China were analyzed using complementary single particle techniques to determine the iron source and speciation. Comparing the spatial distribution of iron within ambient particles and standard Asian mineral dust, it was determined that field-collected atmospheric Fe-containing particles have numerous sources, including anthropogenic sources such as coal combustion. Fe-containing particles were found to be internally mixed with secondary species such as sulfate, soot, and organic carbon. The mass weighted average Fe(II) fraction (defined as Fe(II)/[Fe(II)+Fe(III)]) was determined to be 0.33 {+-} 0.08. Within the experimental uncertainty, this value lies close to the range of 0.26-0.30 determined for representative Asian mineral dust. Previous studies have indicated that the solubility of iron from combustion is much higher than that from mineral dust. Therefore, chemical and/or physical differences other than oxidation state may help explain the higher solubility of iron in atmospheric particles.

Moffet, Ryan C.; Furutani, Hiroshi; Rodel, Tobias; Henn, Tobias R.; Sprau, Peter; Laskin, Alexander; Uematsu, Mitsuo; Gilles, Marry K.

2012-04-04T23:59:59.000Z

225

Assessing regional scale predictions of aerosols, marine stratocumulus, and their interactions during VOCALS-REx using WRF-Chem  

SciTech Connect (OSTI)

This study assesses the ability of the recent chemistry version (v3.3) of the Weather Research and Forecasting (WRF-Chem) model to simulate boundary layer structure, aerosols, stratocumulus clouds, and energy fluxes over the Southeast Pacific Ocean. Measurements from the VAMOS Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-REx) and satellite retrievals (i.e., products from the MODerate resolution Imaging Spectroradiometer (MODIS), Clouds and Earth's Radiant Energy System (CERES), and GOES-10) are used for this assessment. The Morrison double-moment microphysics scheme is newly coupled with interactive aerosols in the model. The 31-day (15 October-16 November 2008) WRF-Chem simulation with aerosol-cloud interactions (AERO hereafter) is also compared to a simulation (MET hereafter) with fixed cloud droplet number concentrations in the microphysics scheme and simplified cloud and aerosol treatments in the radiation scheme. The well-simulated aerosol quantities (aerosol number, mass composition and optical properties), and the inclusion of full aerosol-cloud couplings lead to significant improvements in many features of the simulated stratocumulus clouds: cloud optical properties and microphysical properties such as cloud top effective radius, cloud water path, and cloud optical thickness. In addition to accounting for the aerosol direct and semi-direct effects, these improvements feed back to the simulation of boundary-layer characteristics and energy budgets. Particularly, inclusion of interactive aerosols in AERO strengthens the temperature and humidity gradients within the capping inversion layer and lowers the marine boundary layer (MBL) depth by 130 m from that of the MET simulation. These differences are associated with weaker entrainment and stronger mean subsidence at the top of the MBL in AERO. Mean top-of-atmosphere outgoing shortwave fluxes, surface latent heat, and surface downwelling longwave fluxes are in better agreement with observations in AERO, compared to the MET simulation. Nevertheless, biases in some of the simulated meteorological quantities (e.g., MBL temperature and humidity) and aerosol quantities (e.g., underestimations of accumulation mode aerosol number) might affect simulated stratocumulus and energy fluxes over the Southeastern Pacific, and require further investigation. The well-simulated timing and outflow patterns of polluted and clean episodes demonstrate the model's ability to capture daily/synoptic scale variations of aerosol and cloud properties, and suggest that the model is suitable for studying atmospheric processes associated with pollution outflow over the ocean. The overall performance of the regional model in simulating mesoscale clouds and boundary layer properties is encouraging and suggests that reproducing gradients of aerosol and cloud droplet concentrations and coupling cloud-aerosol-radiation processes are important when simulating marine stratocumulus over the Southeast Pacific.

Yang Q.; Lee Y.; GustafsonJr., W. I.; Fast, J. D.; Wang, H.; Easter, R. C.; Morrison, H.; Chapman, E. G.; Spak, S. N.; Mena-Carrasco, M. A.

2011-12-02T23:59:59.000Z

226

IX. IMPACT OF AEROSOLS FROM THE ERUPTION OF EL CHICHN ON BEAM RADIATION IN THE PACIFIC NORTHWEST  

E-Print Network [OSTI]

measured on clear days the effects of normal climatic differences are avoided. Solar radiation data taken of following this procedure for the clear day solar noon global radiation is shown in Fig. 21. The data shown27 IX. IMPACT OF AEROSOLS FROM THE ERUPTION OF EL CHICH?N ON BEAM RADIATION IN THE PACIFIC

Oregon, University of

227

EMSP Final Report: Electrically Driven Technologies for Radioactive Aerosol Abatement  

SciTech Connect (OSTI)

The purpose of this research project was to develop an improved understanding of how electrically driven processes, including electrocoalescence, acoustic agglomeration, and electric filtration, may be employed to efficiently treat problems caused by the formation of aerosols during DOE waste treatment operations. The production of aerosols during treatment and retrieval operations in radioactive waste tanks and during thermal treatment operations such as calcination presents a significant problem of cost, worker exposure, potential for release, and increased waste volume. There was anecdotal evidence in the literature that acoustic agglomeration and electrical coalescence could be used together to change the size distribution of aerosol particles in such a way as to promote easier filtration and less frequent maintenance of filtration systems. As such, those electrically driven technologies could potentially be used as remote technologies for improved treatment; however, existing theoretical models are not suitable for prediction and design. To investigate the physics of such systems, and also to prototype a system for such processes, a collaborative project was undertaken between Oak Ridge National Laboratory (ORNL) and the University of Texas at Austin (UT). ORNL was responsible for the larger-scale prototyping portion of the project, while UT was primarily responsible for the detailed physics in smaller scale unit reactors. It was found that both electrical coalescence and acoustic agglomeration do in fact increase the rate of aggregation of aerosols. Electrical coalescence requires significantly less input power than acoustic agglomeration, but it is much less effective in its ability to aggregate/coalesce aerosols. The larger-scale prototype showed qualitatively similar results as the unit reactor tests, but presented more difficulty in interpretation of the results because of the complex multi-physics coupling that necessarily occur in all larger-scale system tests. An additional finding from this work is that low-amplitude oscillation may provide an alternative, non-invasive, non-contact means of controlling settling and/or suspension of solids. Further investigation would be necessary to evaluate its utility for radioactive waste treatment applications. This project did not uncover a new technology for radioactive waste treatment. While it may be possible that an efficient electrically driven technology for aerosol treatment could be developed, it appears that other technologies, such as steel and ceramic HEPA filters, can suitably solve this problem. If further studies are to be undertaken, additional fundamental experimentation and modeling is necessary to fully capture the physics; in addition, larger-scale tests are needed to demonstrate the treatment of flowing gas streams through the coupling of acoustic agglomeration with electrocoalescence.

DePaoli, D.W.

2003-01-22T23:59:59.000Z

228

Spent fuel sabotage aerosol ratio program : FY 2004 test and data summary.  

SciTech Connect (OSTI)

This multinational, multi-phase spent fuel sabotage test program is quantifying the aerosol particles produced when the products of a high energy density device (HEDD) interact with and explosively particulate test rodlets that contain pellets of either surrogate materials or actual spent fuel. This program has been underway for several years. This program provides data that are relevant to some sabotage scenarios in relation to spent fuel transport and storage casks, and associated risk assessments. The program also provides significant technical and political benefits in international cooperation. We are quantifying the Spent Fuel Ratio (SFR), the ratio of the aerosol particles released from HEDD-impacted actual spent fuel to the aerosol particles produced from surrogate materials, measured under closely matched test conditions, in a contained test chamber. In addition, we are measuring the amounts, nuclide content, size distribution of the released aerosol materials, and enhanced sorption of volatile fission product nuclides onto specific aerosol particle size fractions. These data are the input for follow-on modeling studies to quantify respirable hazards, associated radiological risk assessments, vulnerability assessments, and potential cask physical protection design modifications. This document includes an updated description of the test program and test components for all work and plans made, or revised, during FY 2004. It also serves as a program status report as of the end of FY 2004. All available test results, observations, and aerosol analyses plus interpretations--primarily for surrogate material Phase 2 tests, series 2/5A through 2/9B, using cerium oxide sintered ceramic pellets are included. Advanced plans and progress are described for upcoming tests with unirradiated, depleted uranium oxide and actual spent fuel test rodlets. This spent fuel sabotage--aerosol test program is coordinated with the international Working Group for Sabotage Concerns of Transport and Storage Casks (WGSTSC) and supported by both the U.S. Department of Energy and the Nuclear Regulatory Commission.

Brucher, Wenzel (Gesellschaft fur Anlagen- und Reaktorsicherheit, Germany); Koch, Wolfgang (Fraunhofer Institut fur Toxikologie und Experimentelle Medizin, Germany); Pretzsch, Gunter Guido (Gesellschaft fur Anlagen- und Reaktorsicherheit, Germany); Loiseau, Olivier (Institut de Radioprotection et de Surete Nucleaire, France); Mo, Tin (U.S. Nuclear Regulatory Commission, Washington, DC); Billone, Michael C. (Argonne National Laboratory, Argonne, IL); Autrusson, Bruno A. (Institut de Radioprotection et de Surete Nucleaire, France); Young, F. I. (U.S. Nuclear Regulatory Commission, Washington, DC); Coats, Richard Lee; Burtseva, Tatiana (Argonne National Laboratory, Argonne, IL); Luna, Robert Earl; Dickey, Roy R.; Sorenson, Ken Bryce; Nolte, Oliver (Fraunhofer Institut fur Toxikologie und Experimentelle Medizin, Germany); Thompson, Nancy Slater (U.S. Department of Energy, Washington, DC); Hibbs, Russell S. (U.S. Department of Energy, Washington, DC); Gregson, Michael Warren; Lange, Florentin (Gesellschaft fur Anlagen- und Reaktorsicherheit, Germany); Molecke, Martin Alan; Tsai, Han-Chung (Argonne National Laboratory, Argonne, IL)

2005-07-01T23:59:59.000Z

229

Improving Bulk Microphysics Parameterizations in Simulations of Aerosol Effects  

SciTech Connect (OSTI)

To improve the microphysical parameterizations for simulations of the aerosol indirect effect (AIE) in regional and global climate models, a double-moment bulk microphysical scheme presently implemented in the Weather Research and Forecasting (WRF) model is modified and the results are compared against atmospheric observations and simulations produced by a spectral bin microphysical scheme (SBM). Rather than using prescribed aerosols as in the original bulk scheme (Bulk-OR), a prognostic doublemoment aerosol representation is introduced to predict both the aerosol number concentration and mass mixing ratio (Bulk-2M). The impacts of the parameterizations of diffusional growth and autoconversion and the selection of the embryonic raindrop radius on the performance of the bulk microphysical scheme are also evaluated. Sensitivity modeling experiments are performed for two distinct cloud regimes, maritime warm stratocumulus clouds (SC) over southeast Pacific Ocean from the VOCALS project and continental deep convective clouds (DCC) in the southeast of China from the Department of Energy/ARM Mobile Facility (DOE/AMF) - China field campaign. The results from Bulk-2M exhibit a much better agreement in the cloud number concentration and effective droplet radius in both the SC and DCC cases with those from SBM and field measurements than those from Bulk-OR. In the SC case particularly, Bulk-2M reproduces the observed drizzle precipitation, which is largely inhibited in Bulk-OR. Bulk-2M predicts enhanced precipitation and invigorated convection with increased aerosol loading in the DCC case, consistent with the SBM simulation, while Bulk-OR predicts the opposite behaviors. Sensitivity experiments using four different types of autoconversion schemes reveal that the autoconversion parameterization is crucial in determining the raindrop number, mass concentration, and drizzle formation for warm 2 stratocumulus clouds. An embryonic raindrop size of 40 ?m is determined as a more realistic setting in the autoconversion parameterization. The saturation adjustment employed in calculating condensation/evaporation in the bulk scheme is identified as the main factor responsible for the large discrepancies in predicting cloud water in the SC case, suggesting that an explicit calculation of diffusion growth with predicted supersaturation is necessary for further improvements of the bulk microphysics scheme. Lastly, a larger rain evaporation rate below cloud is found in the bulk scheme in comparison to the SBM simulation, which could contribute to a lower surface precipitation in the bulk scheme.

Wang, Yuan; Fan, Jiwen; Zhang, Renyi; Leung, Lai-Yung R.; Franklin, Charmaine N.

2013-06-05T23:59:59.000Z

230

ENCAPSULATION EFFECTS ON CARBONACEOUS AEROSOL LIGHT ABSORPTION  

E-Print Network [OSTI]

ENCAPSULATION EFFECTS ON CARBONACEOUS AEROSOL LIGHT ABSORPTION Arthur Sedlacek, Brookhaven National of aerosol absorption on direct radiative forcing is still an active area of research, in part, because. This poster presents data on black carbon (BC) light absorption measured by Photothermal Interferometry

231

2, 12871315, 2002 Aerosol sources and  

E-Print Network [OSTI]

in climate variability and climate change studies (IPCC, 2001). Radiative forcing of natural and their contribution to the chemical composition of aerosols in the Eastern Mediterranean Sea during summertime J aerosol sources in the Eastern Mediterranean5 Basin could be investigated at this location since the site

Paris-Sud XI, Université de

232

6, 1217912197, 2006 Aerosol formation in  

E-Print Network [OSTI]

troposphere and lower stratosphere. The model implements a first order scheme for resolving the aerosol size distribution within its geometric size10 sections, which efficiently suppresses numerical diffusion. We operate removes freshly nucleated particles by coagulation. The observation of high ultrafine aerosol

Paris-Sud XI, Université de

233

6, 32653319, 2006 Study aerosol with  

E-Print Network [OSTI]

ACPD 6, 3265­3319, 2006 Study aerosol with two emission inventories and time factors A. de Meij et in Europe to two different emission inventories and temporal distribution of emissions A. de Meij 1 , M Study aerosol with two emission inventories and time factors A. de Meij et al. Title Page Abstract

Paris-Sud XI, Université de

234

Influence of sky radiance measurement errors on inversion-retrieved aerosol properties  

SciTech Connect (OSTI)

Remote sensing of the atmospheric aerosol is a well-established technique that is currently used for routine monitoring of this atmospheric component, both from ground-based and satellite. The AERONET program, initiated in the 90's, is the most extended network and the data provided are currently used by a wide community of users for aerosol characterization, satellite and model validation and synergetic use with other instrumentation (lidar, in-situ, etc.). Aerosol properties are derived within the network from measurements made by ground-based Sun-sky scanning radiometers. Sky radiances are acquired in two geometries: almucantar and principal plane. Discrepancies in the products obtained following both geometries have been observed and the main aim of this work is to determine if they could be justified by measurement errors. Three systematic errors have been analyzed in order to quantify the effects on the inversion-derived aerosol properties: calibration, pointing accuracy and finite field of view. Simulations have shown that typical uncertainty in the analyzed quantities (5% in calibration, 0.2 Degree-Sign in pointing and 1.2 Degree-Sign field of view) yields to errors in the retrieved parameters that vary depending on the aerosol type and geometry. While calibration and pointing errors have relevant impact on the products, the finite field of view does not produce notable differences.

Torres, B.; Toledano, C.; Cachorro, V. E.; Bennouna, Y. S.; Fuertes, D.; Gonzalez, R.; Frutos, A. M. de [Atmospheric Optics Group (GOA), University of Valladolid, Valladolid (Spain); Berjon, A. J. [Izana Atmospheric Research Center, Meteorological State Agency of Spain (AEMET), Sta. Cruz de Tenerife (Spain); Dubovik, O.; Goloub, P.; Podvin, T.; Blarel, L. [Laboratory of Atmospheric Optics, Universite Lille 1, Villeneuve d'Ascq (France)

2013-05-10T23:59:59.000Z

235

Plenia Locatel Group: Globalizing from Venezuela  

E-Print Network [OSTI]

In 2009 the founders and top executives of Plenia Locatel Group, a retail business in Venezuela specializing in health care products and services, were planning a global

Gibson, Cyrus

2009-05-01T23:59:59.000Z

236

AEROSOL PARTICLE COLLECTOR DESIGN STUDY  

SciTech Connect (OSTI)

A computational evaluation of a particle collector design was performed to evaluate the behavior of aerosol particles in a fast flowing gas stream. The objective of the work was to improve the collection efficiency of the device while maintaining a minimum specified air throughput, nominal collector size, and minimal power requirements. The impact of a range of parameters was considered subject to constraints on gas flow rate, overall collector dimensions, and power limitations. Potential improvements were identified, some of which have already been implemented. Other more complex changes were identified and are described here for further consideration. In addition, fruitful areas for further study are proposed.

Lee, S; Richard Dimenna, R

2007-09-27T23:59:59.000Z

237

ARM - Field Campaign - Aerosol IOP  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr May JunDatastreamsmmcrcalgovInstrumentsrucLasDelivered‰PNGExperience4AJ01)3, 2010SeptemberInfrared SpectralgovCampaignsAerosol IOP

238

Indirect radiative forcing by ion-mediated nucleation of aerosol  

SciTech Connect (OSTI)

A clear understanding of particle formation mechanisms is critical for assessing aerosol indirect radiative forcing and associated climate feedback processes. Recent studies reveal the importance of ion-mediated nucleation (IMN) in generating new particles and cloud condensation nuclei (CCN) in the atmosphere. Here we implement for the first time a physically based treatment of IMN into the Community Atmosphere Model version 5. Our simulations show that, compared to globally averaged results based on binary homogeneous nucleation (BHN), the presence of ionization (i.e., IMN) halves H2SO4 column burden, but increases the column integrated nucleation rate by around one order of magnitude, total particle number burden by a factor of ~ 3, CCN burden by ~ 10% (at 0.2% supersaturation) to 65% (at 1.0% supersaturation), and cloud droplet number burden by ~ 18%. Compared to BHN, IMN increases cloud liquid water path by 7.5%, decreases precipitation by 1.1%, and increases total cloud cover by 1.9%. This leads to an increase of total shortwave cloud radiative forcing by 3.67 W/m2 (more negative) and longwave cloud forcing by 1.78 W/m2 (more positive), resulting in a -1.9 W/m2 net change in cloud radiative forcing associated with IMN. The significant impacts of ionization on global aerosol formation, CCN abundance, and cloud radiative forcing may provide an important physical mechanism linking the global energy balance to various processes affecting atmospheric ionization, which should be properly represented in climate models.

Yu, Fangqun; Luo, Gan; Liu, Xiaohong; Easter, Richard C.; Ma, Xiaoyan; Ghan, Steven J.

2012-12-03T23:59:59.000Z

239

FY 2011 4th Quarter Metric: Estimate of Future Aerosol Direct and Indirect Effects  

SciTech Connect (OSTI)

The global and annual mean aerosol direct and indirect effects, relative to 1850 conditions, estimated from CESM simulations are 0.02 W m-2 and -0.39 W m-2, respectively, for emissions in year 2100 under the IPCC RCP8.5 scenario. The indirect effect is much smaller than that for 2000 emissions because of much smaller SO2 emissions in 2100; the direct effects are small due to compensation between warming by black carbon and cooling by sulfate.

Koch, D

2011-09-21T23:59:59.000Z

240

Atmospheric Radiation Measurement (ARM) Data from Cape Cod, Massachusetts for the Two-Column Aerosol Project (TCAP)  

DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

The Two-Column Aerosol Project (TCAP) was designed to provide a detailed set of observations with which to (1) perform radiative and cloud condensation nuclei (CCN) closure studies, (2) evaluate a new retrieval algorithm for aerosol optical depth (AOD) in the presence of clouds using passive remote sensing, (3) extend a previously developed technique to investigate aerosol indirect effects, and (4) evaluate the performance of a detailed regional-scale model and a more parameterized global-scale model in simulating particle activation and AOD associated with the aging of anthropogenic aerosols. To meet these science objectives, the ARM Mobile Facility and the Mobile Aerosol Observing System were deployed on Cape Cod, Massachusetts, for a 12-month period starting in the summer of 2012 in order to quantify aerosol properties, radiation, and cloud characteristics at a location subject to both clear and cloudy conditions, and clean and polluted conditions. These observations were supplemented by two aircraft intensive observation periods, one in the summer and a second in the winter.

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241

Aerosol, Cloud, and Climate: From Observation to Model (457th Brookhaven Lecture)  

SciTech Connect (OSTI)

In the last 100 years, the Earth has warmed by about 1F, glaciers and sea ice have been melting more quickly than previously, especially during the past decade, and the level of the sea has risen about 6-8 inches worldwide. Scientists have long been investigating this phenomenon of global warming, which is believed to be at least partly due to the increased carbon dioxide (CO2) concentration in the air from burning fossil fuels. Funded by DOE, teams of researchers from BNL and other national labs have been gathering data in the U.S. and internationally to build computer models of climate and weather to help in understanding general patterns, causes, and perhaps, solutions. Among many findings, researchers observed that atmospheric aerosols, minute particles in the atmosphere, can significantly affect global energy balance and climate. Directly, aerosols scatter and absorb sunlight. Indirectly, increased aerosol concentration can lead to smaller cloud droplets, changing clouds in ways that tend to cool global climate and potentially mask overall warming from man-made CO2.

Wang, Jian (Ph.D., Environmental Sciences Department) [Ph.D., Environmental Sciences Department

2010-05-12T23:59:59.000Z

242

Rapid Solar-thermal Dissociation of Natural Gas in an Aerosol Flow Reactor  

E-Print Network [OSTI]

/or hydrogen powered fuel cell vehicles could help to mitigate the energy supply and environmental problems black production. For solar-thermal processing, where carbon black is sold, fossil energy usageRapid Solar-thermal Dissociation of Natural Gas in an Aerosol Flow Reactor Jaimee Dahl a , Karen

243

Influence of transport and ocean ice extent on biogenic aerosol sulfur in the Arctic atmosphere  

E-Print Network [OSTI]

Influence of transport and ocean ice extent on biogenic aerosol sulfur in the Arctic atmosphere S, such as methanesulfonic acid (MSA). This study examines relationships between changes in total sea ice extent north of 70. These results suggest that a decrease in seasonal ice cover influencing other mechanisms of DMS production could

244

An Aerosol Condensation Model for Sulfur Trioxide  

SciTech Connect (OSTI)

This document describes a model for condensation of sulfuric acid aerosol given an initial concentration and/or source of gaseous sulfur trioxide (e.g. fuming from oleum). The model includes the thermochemical effects on aerosol condensation and air parcel buoyancy. Condensation is assumed to occur heterogeneously onto a preexisting background aerosol distribution. The model development is both a revisiting of research initially presented at the Fall 2001 American Geophysical Union Meeting [1] and a further extension to provide new capabilities for current atmospheric dispersion modeling efforts [2]. Sulfuric acid is one of the most widely used of all industrial chemicals. In 1992, world consumption of sulfuric acid was 145 million metric tons, with 42.4 Mt (mega-tons) consumed in the United States [10]. In 2001, of 37.5 Mt consumed in the U.S., 74% went into producing phosphate fertilizers [11]. Another significant use is in mining industries. Lawuyi and Fingas [7] estimate that, in 1996, 68% of use was for fertilizers and 5.8% was for mining. They note that H{sub 2}SO{sub 4} use has been and should continue to be very stable. In the United States, the elimination of MTBE (methyl tertiary-butyl ether) and the use of ethanol for gasoline production are further increasing the demand for petroleum alkylate. Alkylate producers have a choice of either a hydrofluoric acid or sulfuric acid process. Both processes are widely used today. Concerns, however, over the safety or potential regulation of hydrofluoric acid are likely to result in most of the growth being for the sulfuric acid process, further increasing demand [11]. The implication of sulfuric acid being a pervasive industrial chemical is that transport is also pervasive. Often, this is in the form of oleum tankers, having around 30% free sulfur trioxide. Although sulfuric acid itself is not a volatile substance, fuming sulfuric acid (referred to as oleum) is [7], the volatile product being sulfur trioxide. Sulfate aerosols and mist may form in the atmosphere on tank rupture. From chemical spill data from 1990-1996, Lawuyi02 and Fingas [7] prioritize sulfuric acid as sixth most serious. During this period, they note 155 spills totaling 13 Mt, out of a supply volume of 3700 Mt. Lawuyi and Fingas [7] summarize information on three major sulfuric acid spills. On 12 February 1984, 93 tons of sulfuric acid were spilled when 14 railroad cars derailed near MacTier, Parry Sound, Ontario. On 13 December 1978, 51 railroad cars derailed near Springhill, Nova Scotia. One car, containing 93% sulfuric acid, ruptured, spilling nearly its entire contents. In July 1993, 20 to 50 tons of fuming sulfuric acid spilled at the General Chemical Corp. plant in Richmond, California, a major industrial center near San Francisco. The release occurred when oleum was being loaded into a nonfuming acid railroad tank car that contained only a rupture disk as a safety device. The tank car was overheated and this rupture disk blew. The resulting cloud of sulfuric acid drifted northeast with prevailing winds over a number of populated areas. More than 3,000 people subsequently sought medical attention for burning eyes, coughing, headaches, and nausea. Almost all were treated and released on the day of the spill. By the day after the release, another 5,000 people had sought medical attention. The spill forced the closure of five freeways in the region as well as some Bay Area Rapid Transit System stations. Apart from corrosive toxicity, there is the additional hazard that the reactions of sulfur trioxide and sulfuric acid vapors with water are extremely exothermic [10, 11]. While the vapors are intrinsically denser than air, there is thus the likelihood of strong, warming-induced buoyancy from reactions with ambient water vapor, water-containing aerosol droplets, and wet environmental surface. Nordin [12] relates just such an occurrence following the Richmond, CA spill, with the plume observed to rise to 300 m. For all practical purposes, sulfur trioxide was the constituent released from the heated tank

Grant, K E

2008-02-07T23:59:59.000Z

245

Studying trends in biomass burning aerosol using the Absorbing Aerosol Index derived from GOME, SCIAMACHY, and GOME-2  

E-Print Network [OSTI]

Studying trends in biomass burning aerosol using the Absorbing Aerosol Index derived from GOME the resulting time series, we use tropospheric NO2 data as a reference in the regions dominated by biomass sensitive to desert dust aerosols (DDA) and biomass burning aerosols (BBA). See Figure 1. The AAI

Tilstra, Gijsbert

246

Indirect and Semi-Direct Aerosol Campaign: The Impact of Arctic...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Aerosol Campaign: The Impact of Arctic Aerosols on Clouds . Abstract: A comprehensive dataset of microphysical and radiative properties of aerosols and clouds in the arctic...

247

CARES: Carbonaceous Aerosol and Radiative Effects Study Science Plan  

SciTech Connect (OSTI)

Carbonaceous aerosol components, which include black carbon (BC), urban primary organic aerosols (POA), biomass burning aerosols, and secondary organic aerosols (SOA) from both urban and biogenic precursors, have been previously shown to play a major role in the direct and indirect radiative forcing of climate. The primary objective of the CARES 2010 intensive field study is to investigate the evolution of carbonaceous aerosols of different types and their effects on optical and cloud formation properties.

Zaveri, RA; Shaw, WJ; Cziczo, DJ

2010-05-27T23:59:59.000Z

248

Climatological simulations of ozone and atmospheric aerosols in the Greater Cairo region  

SciTech Connect (OSTI)

An integrated chemistry-climate model (RegCM4-CHEM) simulates present-day climate, ozone and tropospheric aerosols over Egypt with a focus on Greater Cairo (GC) region. The densley populated GC region is known for its severe air quality issues driven by high levels of anthropogenic pollution in conjuction with natural sources such as dust and agricultural burning events. We find that current global emission inventories underestimate key pollutants such as nitrogen oxides and anthropogenic aerosol species. In the GC region, average-ground-based NO2 observations of 40-60 ppb are substantially higher than modeled estimates (5-10 ppb), likely due to model grid resolution, improper boundary layer representation, and poor emissions inventories. Observed ozone concentrations range from 35 ppb (winter) to 80 ppb (summer). The model reproduces the seasonal cycle fairly well, but modeled summer ozone is understimated by approximately 15 ppb and exhibits little interannual variability. For aerosols, springtime dust events dominate the seasonal aerosol cycle. The chemistry-climate model captures the springtime peak aerosol optical depth (AOD) of 0.7-1 but is slightly greater than satellite-derived AOD. Observed AOD decreases in the summer and increases again in the fall due to agricultural burning events in the Nile Delta, yet the model underestimates this fall observed AOD peak, as standard emissions inventories underestimate this burning and the resulting aerosol emissions. Our comparison of modeled gas and particulate phase atmospheric chemistry in the GC region indicates that improved emissions inventories of mobile sources and other anthropogenic activities are needed to improve air quality simulations in this region.

Steiner, A. L.; Tawfik, A. B.; Shalaby, A.; Zakey, A. S.; Abdel Wahab, M. M.; Salah, Z.; Solmon, F.; Sillman, S.; Zaveri, Rahul A.

2014-04-16T23:59:59.000Z

249

The Emerging Chinese economy & its Global Impacts  

E-Print Network [OSTI]

The Emerging Chinese economy & its Global Impacts Department of Geography & IDS University of Sussex 5 February: The Emerging Chinese Economy & its Global Impacts + Decoding the Harmonious Socialist of Leicester 19 February: Global Production Network & the Chinese Economy Prof. John Humphrey, IDS 26 February

Sussex, University of

250

Global Optimization in Generalized Geometric Programming  

E-Print Network [OSTI]

exchangernetwork design 5], chemical reactor design 2, 6], optimal condenser design 7], oxygen production 8Global Optimization in Generalized Geometric Programming Costas D. Maranas1 and Christodoulos A Abstract A deterministic global optimization algorithm is proposed for locating the global minimum

Maranas, Costas

251

Global Proteomics Reveal An Atypical Strategy for Carbon/Nitrogen...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

crucial to global oxygen production and worldwide carbon and nitrogen cycles. These microalgae are robust organisms capable carbon neutral biofuel production. Synechocystis sp....

252

Characterizing Aerosol Distributions and Optical Properties Using the NASA Langley High Spectral Resolution Lidar  

SciTech Connect (OSTI)

The objective of this project was to provide vertically and horizontally resolved data on aerosol optical properties to assess and ultimately improve how models represent these aerosol properties and their impacts on atmospheric radiation. The approach was to deploy the NASA Langley Airborne High Spectral Resolution Lidar (HSRL) and other synergistic remote sensors on DOE Atmospheric Science Research (ASR) sponsored airborne field campaigns and synergistic field campaigns sponsored by other agencies to remotely measure aerosol backscattering, extinction, and optical thickness profiles. Synergistic sensors included a nadir-viewing digital camera for context imagery, and, later in the project, the NASA Goddard Institute for Space Studies (GISS) Research Scanning Polarimeter (RSP). The information from the remote sensing instruments was used to map the horizontal and vertical distribution of aerosol properties and type. The retrieved lidar parameters include profiles of aerosol extinction, backscatter, depolarization, and optical depth. Products produced in subsequent analyses included aerosol mixed layer height, aerosol type, and the partition of aerosol optical depth by type. The lidar products provided vertical context for in situ and remote sensing measurements from other airborne and ground-based platforms employed in the field campaigns and was used to assess the predictions of transport models. Also, the measurements provide a data base for future evaluation of techniques to combine active (lidar) and passive (polarimeter) measurements in advanced retrieval schemes to remotely characterize aerosol microphysical properties. The project was initiated as a 3-year project starting 1 January 2005. It was later awarded continuation funding for another 3 years (i.e., through 31 December 2010) followed by a 1-year no-cost extension (through 31 December 2011). This project supported logistical and flight costs of the NASA sensors on a dedicated aircraft, the subsequent analysis and archival of the data, and the presentation of results in conferences, workshops, and publications. DOE ASR field campaigns supported under this project included - MAX-Mex /MILAGRO (2006) - TexAQS 2006/GoMACCS (2006) - CHAPS (2007) - RACORO (2009) - CARE/CalNex (2010) In addition, data acquired on HSRL airborne field campaigns sponsored by other agencies were used extensively to fulfill the science objectives of this project and the data acquired have been made available to other DOE ASR investigators upon request.

Hostetler, Chris; Ferrare, Richard

2013-02-14T23:59:59.000Z

253

Capstone Depleted Uranium Aerosols: Generation and Characterization  

SciTech Connect (OSTI)

In a study designed to provide an improved scientific basis for assessing possible health effects from inhaling depleted uranium (DU) aerosols, a series of DU penetrators was fired at an Abrams tank and a Bradley fighting vehicle. A robust sampling system was designed to collect aerosols in this difficult environment and continuously monitor the sampler flow rates. Aerosols collected were analyzed for uranium concentration and particle size distribution as a function of time. They were also analyzed for uranium oxide phases, particle morphology, and dissolution in vitro. The resulting data provide input useful in human health risk assessments.

Parkhurst, MaryAnn; Szrom, Fran; Guilmette, Ray; Holmes, Tom; Cheng, Yung-Sung; Kenoyer, Judson L.; Collins, John W.; Sanderson, T. Ellory; Fliszar, Richard W.; Gold, Kenneth; Beckman, John C.; Long, Julie

2004-10-19T23:59:59.000Z

254

Old and new sinks in the global nitrogen cycle Bernhard Wehrli (wehrli@eawag.ch)  

E-Print Network [OSTI]

> 15% of global food production - hydroelectricity ~20% of total - rate of dam construction 360 to 170

Einat, Aharonov

255

Global Warming  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr MayAtmospheric Optical Depth7-1D: Vegetation ProposedUsingFun with Big Sky LearningGet Assistance GetGiantOn The VergeGlobal Threat1 Global

256

MIT Joint Program on the Science and Policy of Global Change  

E-Print Network [OSTI]

, and environmental effects. In turn, the greenhouse gas and atmospheric aerosol assumptions underlying climate-Range Weather Forecasts (ECMWF) Re- Analysis (ERA-40). In this budget analysis, the chemical net production term

257

7, 1709917116, 2007 Smoke aerosol,  

E-Print Network [OSTI]

area model REMOTE driven at its lateral boundaries by ERA40 reanalysis data. REMOTE was extended5 on global circulation (Nober et al., 2003) arising from changes in latent heat release due to diminished

Boyer, Edmond

258

Southern hemisphere tropospheric aerosol microphysics  

SciTech Connect (OSTI)

Aerosol particle size distribution data have been obtained in the southern hemisphere from approximately 4{degree}S to 44{degree}S and between ground level and 6 km, in the vicinity of eastern Australia. The relative shape of the free-tropospheric size distribution for particles with radii larger than approximately 0.04 {mu}m was found to be remarkably stable with time, altitude, and location for the autumn-winter periods considered. This was despite some large concentration changes which were found to be typical of the southeastern Australian coastal region. The majority of free-troposphere large particles were found to have sulfuric acid or lightly ammoniated sulfate morphology. Large particles in the boundary layer almost exclusively had a sea-salt morphology.

Gras, J.L. (Commonwealth Scientific and Industrial Research Organization, Aspendale (Australia))

1991-03-20T23:59:59.000Z

259

Radiative and climate impacts of absorbing aerosols  

E-Print Network [OSTI]

incident radiation are distinguished, and albedos for oceanOceans using multiple satellite datasets in conjunction with MACR (Monte Carlo Aerosol-Cloud-Radiation)ocean temperature is coupled with the rest of the climate system, the dimming of surface radiation

Zhu, Aihua

2010-01-01T23:59:59.000Z

260

Aerosol remote sensing in polar regions  

DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

Multi-year sets of ground-based sun-photometer measurements conducted at 12 Arctic sites and 9 Antarctic sites were examined to determine daily mean values of aerosol optical thickness ?(?) at visible and near-infrared wavelengths, from which best-fit values of ngstrm's exponent ? were calculated. Analysing these data, the monthly mean values of ?(0.50 ?m) and ? and the relative frequency histograms of the daily mean values of both parameters were determined for winterspring and summerautumn in the Arctic and for austral summer in Antarctica. The Arctic and Antarctic covariance plots of the seasonal median values of ? versus ?(0.50 ?m) showed: (i) a considerable increase in ?(0.50 ?m) for the Arctic aerosol from summer to winterspring, without marked changes in ?; and (ii) a marked increase in ?(0.50 ?m) passing from the Antarctic Plateau to coastal sites, whereas ? decreased considerably due to the larger fraction of sea-salt aerosol. Good agreement was found when comparing ground-based sun-photometer measurements of ?(?) and ? at Arctic and Antarctic coastal sites with Microtops measurements conducted during numerous AERONET/MAN cruises from 2006 to 2013 in three Arctic Ocean sectors and in coastal and off-shore regions of the Southern Atlantic, Pacific, and Indian Oceans, and the Antarctic Peninsula. Lidar measurements were also examined to characterise vertical profiles of the aerosol backscattering coefficient measured throughout the year at Ny-lesund. Satellite-based MODIS, MISR, and AATSR retrievals of ?(?) over large parts of the oceanic polar regions during spring and summer were in close agreement with ship-borne and coastal ground-based sun-photometer measurements. An overview of the chemical composition of mode particles is also presented, based on in-situ measurements at Arctic and Antarctic sites. Fourteen log-normal aerosol number size-distributions were defined to represent the average features of nuclei, accumulation and coarse mode particles for Arctic haze, summer background aerosol, Asian dust and boreal forest fire smoke, and for various background austral summer aerosol types at coastal and high-altitude Antarctic sites. The main columnar aerosol optical characteristics were determined for all 14 particle modes, based on in-situ measurements of the scattering and absorption coefficients. Diurnally averaged direct aerosol-induced radiative forcing and efficiency were calculated for a set of multimodal aerosol extinction models, using various Bidirectional Reflectance Distribution Function models over vegetation-covered, oceanic and snow-covered surfaces. These gave a reliable measure of the pronounced effects of aerosols on the radiation balance of the surfaceatmosphere system over polar regions.

Tomasi, C.; Wagener, R.; Kokhanovsky, A. A.; Lupi, A.; Ritter, C.; Smirnov, A.; O Neill, N. T.; Stone, R. S.; Holben, B. N.; Nyeki, S.; Wehrli, C.; Stohl, A.; Mazzola, M.; Lanconelli, C.; Vitale, V.; Stebel, K.; Aaltonen, V.; de Leeuw, G.; Rodriguez, E.; Herber, A. B.; Radionov, V. F.; Zielinski, T.; Petelski, T.; Sakerin, S. M.; Kabanov, D. M.; Xue, Y.; Mei, L.; Istomina, L.; Wagener, R.; McArthur, B.; Sobolewski, P. S.; Kivi, R.; Courcoux, Y.; Larouche, P.; Broccardo, S.; Piketh, S. J.

2015-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


261

Aerosol fabrication methods for monodisperse nanoparticles  

DOE Patents [OSTI]

Exemplary embodiments provide materials and methods for forming monodisperse particles. In one embodiment, the monodisperse particles can be formed by first spraying a nanoparticle-containing dispersion into aerosol droplets and then heating the aerosol droplets in the presence of a shell precursor to form core-shell particles. By removing either the shell layer or the nanoparticle core of the core-shell particles, monodisperse nanoparticles can be formed.

Jiang, Xingmao; Brinker, C Jeffrey

2014-10-21T23:59:59.000Z

262

Development of plutonium aerosol fractionation system  

E-Print Network [OSTI]

DEVELOPMENT OF A PLUTONIUM AEROSOL FRACTIONATION SYSTEM A Thesis by MALLA R. MEKALA Submitted to the Office of Graduate Studies of Texas A&M University in partial fulfillment of the requirements for the degree of MASTER OF SCIENCE August... 1993 Major Subject: Mechanical Engineering DEVELOPMENT OP A PLUTONIUM AEROSOL FRACTIONATION SYSTEM A Thesis by MALLA R. MEKALA Approved as to style and content by: A. R. McFarland (Chair of Committee) N. K. Anand (Mer toer) (', & C. B...

Mekala, Malla R.

1993-01-01T23:59:59.000Z

263

WRF-Chem Simulations of Aerosols and Anthropogenic Aerosol Radiative Forcing in East Asia  

SciTech Connect (OSTI)

This study aims to provide a first comprehensive evaluation of WRF-Chem for modeling aerosols and anthropogenic aerosol radiative forcing (RF) over East Asia. Several numerical experiments were conducted from November 2007 to December 2008. Comparison between model results and observations shows that the model can generally reproduce the observed spatial distributions of aerosol concentration, aerosol optical depth (AOD) and single scattering albedo (SSA) from measurements at different sites, including the relatively higher aerosol concentration and AOD over East China and the relatively lower AOD over Southeast Asia, Korean, and Japan. The model also depicts the seasonal variation and transport of pollutions over East Asia. Particulate matter of 10 um or less in the aerodynamic diameter (PM10), black carbon (BC), sulfate (SO42-), nitrate (NO3-) and ammonium (NH4+) concentrations are higher in spring than other seasons in Japan due to the pollutant transport from polluted area of East Asia. AOD is high over Southwest and Central China in winter, spring and autumn and over North China in summer while is low over South China in summer due to monsoon precipitation. SSA is lowest in winter and highest in summer. The model also captures the dust events at the Zhangye site in the semi-arid region of China. Anthropogenic aerosol RF is estimated to range from -5 to -20 W m-2 over land and -20 to -40 W m-2 over ocean at the top of atmosphere (TOA), 5 to 30 W m-2 in the atmosphere (ATM) and -15 to -40 W m-2 at the bottom (BOT). The warming effect of anthropogenic aerosol in ATM results from BC aerosol while the negative aerosol RF at TOA is caused by scattering aerosols such as SO4 2-, NO3 - and NH4+. Positive BC RF at TOA compensates 40~50% of the TOA cooling associated with anthropogenic aerosol.

Gao, Yi; Zhao, Chun; Liu, Xiaohong; Zhang, Meigen; Leung, Lai-Yung R.

2014-08-01T23:59:59.000Z

264

Study of Mechanisms of Aerosol Indirect Effects on Glaciated Clouds: Progress during the Project Final Technical Report  

SciTech Connect (OSTI)

This 3-year project has studied how aerosol pollution influences glaciated clouds. The tool applied has been an 'aerosol-cloud model'. It is a type of Cloud-System Resolving Model (CSRM) modified to include 2-moment bulk microphysics and 7 aerosol species, as described by Phillips et al. (2009, 2013). The study has been done by, first, improving the model and then performing sensitivity studies with validated simulations of a couple of observed cases from ARM. These are namely the Tropical Warm Pool International Cloud Experiment (TWP-ICE) over the tropical west Pacific and the Cloud and Land Surface Interaction Campaign (CLASIC) over Oklahoma. During the project, sensitivity tests with the model showed that in continental clouds, extra liquid aerosols (soluble aerosol material) from pollution inhibited warm rain processes for precipitation production. This promoted homogeneous freezing of cloud droplets and aerosols. Mass and number concentrations of cloud-ice particles were boosted. The mean sizes of cloud-ice particles were reduced by the pollution. Hence, the lifetime of glaciated clouds, especially ice-only clouds, was augmented due to inhibition of sedimentation and ice-ice aggregation. Latent heat released from extra homogeneous freezing invigorated convective updrafts, and raised their maximum cloud-tops, when aerosol pollution was included. In the particular cases simulated in the project, the aerosol indirect effect of glaciated clouds was twice than of (warm) water clouds. This was because glaciated clouds are higher in the troposphere than water clouds and have the first interaction with incoming solar radiation. Ice-only clouds caused solar cooling by becoming more extensive as a result of aerosol pollution. This 'lifetime indirect effect' of ice-only clouds was due to higher numbers of homogeneously nucleated ice crystals causing a reduction in their mean size, slowing the ice-crystal process of snow production and slowing sedimentation. In addition to the known indirect effects (glaciation, riming and thermodynamic), new indirect effects were discovered and quantified due to responses of sedimentation, aggregation and coalescence in glaciated clouds to changing aerosol conditions. In summary, the change in horizontal extent of the glaciated clouds ('lifetime indirect effects'), especially of ice-only clouds, was seen to be of higher importance in regulating aerosol indirect effects than changes in cloud properties ('cloud albedo indirect effects').

None

2013-10-18T23:59:59.000Z

265

Chemical Composition and Sources of Coastal Marine Aerosol Particles during the 2008 VOCALS-REx Campaign  

SciTech Connect (OSTI)

The chemical composition of aerosol particles (Dp 1.5 ?m) was measured over the southeast Pacific Ocean during the VAMOS (Variability of the American Monsoon Systems) Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-Rex) between 16 October and 15 November 2008 using the US Department of Energy (DOE) G-1 aircraft. The objective of these flights was to gain an understanding of the sources and evolution of these aerosols, and of how they interact with the marine stratus cloud layer that prevails in this region of the globe. Our measurements showed that the marine boundary layer (MBL) aerosol mass was dominated by non-sea-salt SO2?4, followed by Na+, Cl?, Org (total organics), NH+4 , and NO?3 , in decreasing order of importance; CH3SO?3 (MSA), Ca2+, and K+ rarely exceeded their limits of detection. Aerosols were strongly acidic with a NH+4 to SO2?4 equivalents ratio typically < 0.3. Sea-salt aerosol (SSA) particles, represented by NaCl, exhibited Cl? deficits caused by both HNO3 and H2SO4, but for the most part were externally mixed with particles, mainly SO2?4. SSA contributed only a small fraction of the total accumulation mode particle number concentration. It was inferred that all aerosol species (except SSA) were of predominantly continental origin because of their strong land-to-sea concentration gradient. Comparison of relative changes in median values suggests that (1) an oceanic source of NH3 is present between 72 W and 76 W, (2) additional organic aerosols from biomass burns or biogenic precursors were emitted from coastal regions south of 31 S, with possible cloud processing, and (3) free tropospheric (FT) contributions to MBL gas and aerosol concentrations were negligible. The very low levels of CH3SO?3 observed as well as the correlation between SO2?4 and NO?3 (which is thought primarily anthropogenic) suggest a limited contribution of DMS to SO2?4 aerosol production during VOCALS.

Lee, Y.- N.; Springston, S.; Jayne, John T.; Wang, Jian; Hubbe, John M.; Senum, Gunnar I.; Kleinman, Lawrence I.; Daum, Peter H.

2014-05-23T23:59:59.000Z

266

Global Assessment of Hydrogen Technologies Tasks 3 & 4 Report Economic, Energy, and Environmental Analysis of Hydrogen Production and Delivery Options in Select Alabama Markets: Preliminary Case Studies  

SciTech Connect (OSTI)

This report documents a set of case studies developed to estimate the cost of producing, storing, delivering, and dispensing hydrogen for light-duty vehicles for several scenarios involving metropolitan areas in Alabama. While the majority of the scenarios focused on centralized hydrogen production and pipeline delivery, alternative delivery modes were also examined. Although Alabama was used as the case study for this analysis, the results provide insights into the unique requirements for deploying hydrogen infrastructure in smaller urban and rural environments that lie outside the DOEs high priority hydrogen deployment regions. Hydrogen production costs were estimated for three technologies steam-methane reforming (SMR), coal gasification, and thermochemical water-splitting using advanced nuclear reactors. In all cases examined, SMR has the lowest production cost for the demands associated with metropolitan areas in Alabama. Although other production options may be less costly for larger hydrogen markets, these were not examined within the context of the case studies.

Fouad, Fouad H.; Peters, Robert W.; Sisiopiku, Virginia P.; Sullivan Andrew J.; Gillette, Jerry; Elgowainy, Amgad; Mintz, Marianne

2007-12-01T23:59:59.000Z

267

E-Print Network 3.0 - aerosol chemical vapor Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

chemical and microphysical properties influence aerosol optical properties and radiative effects... distribution of aerosol extensive and intensive properties will aid ......

268

Global Health Research | 2 Global Health Research  

E-Print Network [OSTI]

Global Health Research | 2 Global Health Research Supporting researchers in low- and middle-income countries to carry out health- related research within their own countries. Gl bal Health #12;3 | Global Health Research #12;Global Health Research | 4 We are a global charitable foundation dedicated

Rambaut, Andrew

269

AEROSOL CHEMICAL COMPOSITION CHARACTERIZATION AT THE ARM SOUTHERN GREAT PLAINS (SGP) SITE USING AN AEROSOL CHEMICAL  

E-Print Network [OSTI]

AEROSOL CHEMICAL COMPOSITION CHARACTERIZATION AT THE ARM SOUTHERN GREAT PLAINS (SGP) SITE USING AN AEROSOL CHEMICAL SPECIATION MONITOR Yin-Nan Lee1 , Fan Mei1 , Stephanie DeJong1 , Anne Jefferson2 1 Atmospheric Sciences Division, Brookhaven National Lab, Upton, NY 2 CIRES, University of Colorado, Boulder, CO

270

Spent fuel sabotage test program, characterization of aerosol dispersal : interim final report.  

SciTech Connect (OSTI)

This multinational, multi-phase spent fuel sabotage test program is quantifying the aerosol particles produced when the products of a high energy density device (HEDD) interact with and explosively particulate test rodlets that contain pellets of either surrogate materials or actual spent fuel. This program provides source-term data that are relevant to plausible sabotage scenarios in relation to spent fuel transport and storage casks and associated risk assessments. We present details and significant results obtained from this program from 2001 through 2007. Measured aerosol results include: respirable fractions produced; amounts, nuclide content, and produced particle size distributions and morphology; measurements of volatile fission product species enhanced sorption--enrichment factors onto respirable particles; and, status on determination of the spent fuel ratio, SFR, needed for scaling studies. Emphasis is provided on recent Phase 3 tests using depleted uranium oxide pellets plus non-radioactive fission product dopants in surrogate spent fuel test rodlets, plus the latest surrogate cerium oxide results and aerosol laboratory supporting calibration work. The DUO{sub 2}, CeO{sub 2}, plus fission product dopant aerosol particle results are compared with available historical data. We also provide a status review on continuing preparations for the final Phase 4 in this program, tests using individual short rodlets containing actual spent fuel from U.S. PWR reactors, with both high- and lower-burnup fuel. The source-term data, aerosol results, and program design have been tailored to support and guide follow-on computer modeling of aerosol dispersal hazards and radiological consequence assessments. This spent fuel sabotage, aerosol test program was performed primarily at Sandia National Laboratories, with support provided by both the U.S. Department of Energy and the Nuclear Regulatory Commission. This program has significant input from, and is cooperatively supported and coordinated by both the U.S. and international program participants in Germany, France, and others, as part of the International Working Group for Sabotage Concerns of Transport and Storage Casks (WGSTSC).

Gregson, Michael Warren; Brockmann, John E.; Loiseau, Olivier (Institut de Radioprotection et de Surete Nucleaire, France); Klennert, Lindsay A.; Nolte, Oliver (Fraunhofer Institut fur Toxikologie und Experimentelle Medizin, Germany); Molecke, Martin Alan; Autrusson, Bruno A. (Institut de Radioprotection et de Surete Nucleaire, France); Koch, Wolfgang (Fraunhofer Institut fur Toxikologie und Experimentelle Medizin, Germany); Pretzsch, Gunter Guido (Gesellschaft fur Anlagen- und Reaktorsicherheit, Germany); Brucher, Wenzel (Gesellschaft fur Anlagen- und Reaktorsicherheit, Germany); Steyskal, Michele D.

2008-03-01T23:59:59.000Z

271

Understanding Global Capitalism  

E-Print Network [OSTI]

sociology; globalization; political economy; development;economy fueled through 700 billion dollars injected into globalizationGlobalization Studies, also called CGS. I would economy and

Robinson, William I.

2008-01-01T23:59:59.000Z

272

Review: Global Climate Change  

E-Print Network [OSTI]

introduction to global climate change, the greenhouseReview: Global Climate Change: A Primer By Orrin H PilkeyPilkey, Keith C. Global Climate Change: a primer. Durham,

Smith, Jennifer

2013-01-01T23:59:59.000Z

273

Application of computational fluid dynamics to aerosol sampling and concentration  

E-Print Network [OSTI]

An understanding of gas-liquid two-phase interactions, aerosol particle deposition, and heat transfer is needed. Computational Fluid Dynamics (CFD) is becoming a powerful tool to predict aerosol behavior for related design work. In this study...

Hu, Shishan

2009-05-15T23:59:59.000Z

274

Aerosol beam-focus laser-induced plasma spectrometer device  

DOE Patents [OSTI]

An apparatus for detecting elements in an aerosol includes an aerosol beam focuser for concentrating aerosol into an aerosol beam; a laser for directing a laser beam into the aerosol beam to form a plasma; a detection device that detects a wavelength of a light emission caused by the formation of the plasma. The detection device can be a spectrometer having at least one grating and a gated intensified charge-coupled device. The apparatus may also include a processor that correlates the wavelength of the light emission caused by the formation of the plasma with an identity of an element that corresponds to the wavelength. Furthermore, the apparatus can also include an aerosol generator for forming an aerosol beam from bulk materials. A method for detecting elements in an aerosol is also disclosed.

Cheng, Meng-Dawn (Oak Ridge, TN)

2002-01-01T23:59:59.000Z

275

aerosol particle penetration: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

the subsequent aerosol penetration performance through these tubes were conducted for a aerosol particle size range of 5 nm to 20 nm and a flow rate range of 28 Lmin to 169.9...

276

Effects of operating conditions on a heat transfer fluid aerosol  

E-Print Network [OSTI]

of heat transfer fluid aerosols from process leaks. To simulate industrial leaks, aerosol formation from a plain orifice into ambient air is studied by measuring liquid drop sizes and size distributions at various distances from an orifice. Measurements...

Sukmarg, Passaporn

2000-01-01T23:59:59.000Z

277

Academy for Global Engagement  

E-Print Network [OSTI]

Academy for Global Engagement 2013-2014 Global Fellows #12;Meredith Gore and Wildlife #12;Global Research Interests · risk percepHon and public support and Agricultural Engineering #12;Global Research Interests · catalyHc conversion of biomass

278

global warming's six indias  

E-Print Network [OSTI]

global warming's six indias: An Audience Segmentation Analysis #12;Global Warming's Six Indias 1............................................................................................................................................20 2. Global Warming Beliefs and Attitudes................................................................................ 21 Knowledge about global warming varies widely by group

Haller, Gary L.

279

Project of Aerosol Optical Depth Change in South America  

E-Print Network [OSTI]

AerosolDepth Brazil Bolivia French Guiana Suriname Guyana Venezuela Colombia Ecuador Peru Chile Argentina Suriname Guyana Venezuela Colombia Ecuador Peru Chile Argentina Paraguay Uruguay #12;Statistics of Aerosol M ean D ec 01 to 06 Mean Month AerosolDepth Brazil Bolivia French Guiana Suriname Guyana Venezuela

Frank, Thomas D.

280

Sulfuric acid deposition from stratospheric geoengineering with sulfate aerosols  

E-Print Network [OSTI]

aerosols can potentially result in an increase in acid deposition. [4] Acid rain has been studiedSulfuric acid deposition from stratospheric geoengineering with sulfate aerosols Ben Kravitz,1 Alan limit of hydration of all sulfate aerosols into sulfuric acid. For annual injection of 5 Tg of SO2

Robock, Alan

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


281

Aerosol composition, chemistry, and source characterization during the 2008 VOCALS Experiment  

SciTech Connect (OSTI)

Chemical composition of fine aerosol particles over the northern Chilean coastal waters was determined onboard the U.S. DOE G-1 aircraft during the VOCALS (VAMOS Ocean-Cloud-Atmosphere-Land Study) field campaign between October 16 and November 15, 2008. SO42-, NO3-, NH4+, and total organics (Org) were determined using an Aerodyne Aerosol Mass Spectrometer, and SO42-, NO3-, NH4+, Na+, Cl-, CH3SO3-, Mg2+, Ca2+, and K+ were determined using a particle-into-liquid sampler-ion chromatography technique. The results show the marine boundary layer (MBL) aerosol mass was dominated by non- sea-salt SO42- followed by Na+, Cl-, Org, NO3-, and NH4+, in decreasing importance; CH3SO3-, Ca2+, and K+ rarely exceeded their respective limits of detection. The SO42- aerosols were strongly acidic as the equivalent NH4+ to SO42- ratio was only {approx}0.25 on average. NaCl particles, presumably of sea-salt origin, showed chloride deficits but retained Cl- typically more than half the equivalency of Na+, and are externally mixed with the acidic sulfate aerosols. Nitrate was observed only on sea-salt particles, consistent with adsorption of HNO3 on sea-salt aerosols, responsible for the Cl- deficit. Dust particles appeared to play a minor role, judging from the small volume differences between that derived from the observed mass concentrations and that calculated based on particle size distributions. Because SO42- concentrations were substantial ({approx}0.5 - {approx}3 {micro}g/m3) with a strong gradient (highest near the shore), and the ocean-emitted dimethylsulfide and its unique oxidation product, CH3SO3-, were very low (i.e., {le} 40 parts per trillion and <0.05 {micro}g/m3, respectively), the observed SO42- aerosols are believed to be primarily of terrestrial origin. Back trajectory calculations indicate sulfur emissions from smelters and power plants along coastal regions of Peru and Chile are the main sources of these SO4- aerosols. However, compared to observations, model calculations appeared to underestimate sulfate concentrations based on an existing emission inventory. The agreement between observations and model predictions of CO as well as total sulfur is reexamined in this work with a new emission inventory made available recently.

Lee, Y.; Springston, S.; Jayne, J.; Wang, J.; Senum, G.; Hubbe, J.; Alexander, L.; Brioude, J.; Spak, S.; Mena-Carrasco, M.; Kleinman, L.; Daum, P.

2010-03-15T23:59:59.000Z

282

Phase transformation and growth of hygroscopic aerosols  

SciTech Connect (OSTI)

Ambient aerosols play an important role in many atmospheric processes affecting air quality, visibility degradation, and climatic changes as well. Both natural and anthropogenic sources contribute to the formation of ambient aerosols, which are composed mostly of sulfates, nitrates, and chlorides in either pure or mixed forms. These inorganic salt aerosols are hygroscopic by nature and exhibit the properties of deliquescence and efflorescence in humid air. For pure inorganic salt particles with diameter larger than 0.1 micron, the phase transformation from a solid particle to a saline droplet occurs only when the relative humidity in the surrounding atmosphere reaches a certain critical level corresponding to the water activity of the saturated solution. The droplet size or mass in equilibrium with relative humidity can be calculated in a straightforward manner from thermodynamic considerations. For aqueous droplets 0.1 micron or smaller, the surface curvature effect on vapor pressure becomes important and the Kelvin equation must be used.

Tang, I.N.

1999-11-01T23:59:59.000Z

283

CADS:Cantera Aerosol Dynamics Simulator.  

SciTech Connect (OSTI)

This manual describes a library for aerosol kinetics and transport, called CADS (Cantera Aerosol Dynamics Simulator), which employs a section-based approach for describing the particle size distributions. CADS is based upon Cantera, a set of C++ libraries and applications that handles gas phase species transport and reactions. The method uses a discontinuous Galerkin formulation to represent the particle distributions within each section and to solve for changes to the aerosol particle distributions due to condensation, coagulation, and nucleation processes. CADS conserves particles, elements, and total enthalpy up to numerical round-off error, in all of its formulations. Both 0-D time dependent and 1-D steady state applications (an opposing-flow flame application) have been developed with CADS, with the initial emphasis on developing fundamental mechanisms for soot formation within fires. This report also describes the 0-D application, TDcads, which models a time-dependent perfectly stirred reactor.

Moffat, Harry K.

2007-07-01T23:59:59.000Z

284

The Global Energy Challenge  

ScienceCinema (OSTI)

The expected doubling of global energy demand by 2050 challenges our traditional patterns of energy production, distribution and use. The continued use of fossil fuels raises concerns about supply, security, environment and climate. New routes are needed for the efficient conversion of energy from chemical fuel, sunlight, and heat to electricity or hydrogen as an energy carrier and finally to end uses like transportation, lighting, and heating. Opportunities for efficient new energy conversion routes based on nanoscale materials will be presented, with emphasis on the sustainable energy technologies they enable.

George Crabtree

2010-01-08T23:59:59.000Z

285

VOL. 59, NO. 3 1 FEBRUARY 2002J O U R N A L O F T H E A T M O S P H E R I C S C I E N C E S Global Aerosol Climatology Project  

E-Print Network [OSTI]

High Resolution Radiometer (AVHRR) retrievals and on Total Ozone Mapping Spectrometer (TOMS) data and indirect forcing of climate, but the magnitude of this forcing remains highly uncertain because Sciences Program and the Global Energy and Water Cycle Experiment (GEWEX) established in 1998 a joint

286

Aerodynamic Focusing Of High-Density Aerosols  

SciTech Connect (OSTI)

High-density micron-sized particle aerosols might form the basis for a number of applications in which a material target with a particular shape might be quickly ionized to form a cylindrical or sheet shaped plasma. A simple experimental device was built in order to study the properties of high-density aerosol focusing for 1#22; m silica spheres. Preliminary results recover previous findings on aerodynamic focusing at low densities. At higher densities, it is demonstrated that the focusing properties change in a way which is consistent with a density dependent Stokes number.

Ruiz, D. E.; Fisch, Nathaniel

2014-02-24T23:59:59.000Z

287

Global energy demand to 2060  

SciTech Connect (OSTI)

The projection of global energy demand to the year 2060 is of particular interest because of its relevance to the current greenhouse concerns. The long-term growth of global energy demand in the time scale of climatic change has received relatively little attention in the public discussion of national policy alternatives. The sociological, political, and economic issues have rarely been mentioned in this context. This study emphasizes that the two major driving forces are global population growth and economic growth (gross national product per capita), as would be expected. The modest annual increases assumed in this study result in a year 2060 annual energy use of >4 times the total global current use (year 1986) if present trends continue, and >2 times with extreme efficiency improvements in energy use. Even assuming a zero per capita growth for energy and economics, the population increase by the year 2060 results in a 1.5 times increase in total annual energy use.

Starr, C. (Electric Power Research Institute, Palo Alto, CA (USA))

1989-01-01T23:59:59.000Z

288

Near real time vapor detection and enhancement using aerosol adsorption  

SciTech Connect (OSTI)

A vapor sample detection method where the vapor sample contains vapor and ambient air and surrounding natural background particles. The vapor sample detection method includes the steps of generating a supply of aerosol that have a particular effective median particle size, mixing the aerosol with the vapor sample forming aerosol and adsorbed vapor suspended in an air stream, impacting the suspended aerosol and adsorbed vapor upon a reflecting element, alternatively directing infrared light to the impacted aerosol and adsorbed vapor, detecting and analyzing the alternatively directed infrared light in essentially real time using a spectrometer and a microcomputer and identifying the vapor sample.

Novick, Vincent J.; Johnson, Stanley A.

1997-12-01T23:59:59.000Z

289

Technical Note: Estimating Aerosol Effects on Cloud Radiative Forcing  

SciTech Connect (OSTI)

Estimating anthropogenic aerosol effects on the planetary energy balance through the aerosol influence on clouds using the difference in cloud radiative forcing from simulations with and without anthropogenic emissions produces estimates that are positively biased. A more representative method is suggested using the difference in cloud radiative forcing calculated with aerosol radiative effects neglected. The method also yields an aerosol radiative forcing decomposition that includes a term quantifying the impact of changes in surface albedo. The method requires only two additional diagnostic calculations: the whole-sky and clear-sky top-of-atmosphere radiative flux with aerosol radiative effects neglected.

Ghan, Steven J.

2013-10-09T23:59:59.000Z

290

Near real time vapor detection and enhancement using aerosol adsorption  

DOE Patents [OSTI]

A vapor sample detection method is described where the vapor sample contains vapor and ambient air and surrounding natural background particles. The vapor sample detection method includes the steps of generating a supply of aerosol that have a particular effective median particle size, mixing the aerosol with the vapor sample forming aerosol and adsorbed vapor suspended in an air stream, impacting the suspended aerosol and adsorbed vapor upon a reflecting element, alternatively directing infrared light to the impacted aerosol and adsorbed vapor, detecting and analyzing the alternatively directed infrared light in essentially real time using a spectrometer and a microcomputer and identifying the vapor sample. 13 figs.

Novick, V.J.; Johnson, S.A.

1999-08-03T23:59:59.000Z

291

Near real time vapor detection and enhancement using aerosol adsorption  

DOE Patents [OSTI]

A vapor sample detection method where the vapor sample contains vapor and ambient air and surrounding natural background particles. The vapor sample detection method includes the steps of generating a supply of aerosol that have a particular effective median particle size, mixing the aerosol with the vapor sample forming aerosol and adsorbed vapor suspended in an air stream, impacting the suspended aerosol and adsorbed vapor upon a reflecting element, alternatively directing infrared light to the impacted aerosol and adsorbed vapor, detecting and analyzing the alternatively directed infrared light in essentially real time using a spectrometer and a microcomputer and identifying the vapor sample.

Novick, Vincent J. (Downers Grove, IL); Johnson, Stanley A. (Countryside, IL)

1999-01-01T23:59:59.000Z

292

Raman lidar profiling of water vapor and aerosols over the ARM SGP Site  

SciTech Connect (OSTI)

The authors have developed and implemented automated algorithms to retrieve profiles of water vapor mixing ratio, aerosol backscattering, and aerosol extinction from Southern Great Plains (SGP) Cloud and Radiation Testbed (CART) Raman Lidar data acquired during both daytime and nighttime operations. The Raman lidar sytem is unique in that it is turnkey, automated system designed for unattended, around-the-clock profiling of water vapor and aerosols. These Raman lidar profiles are important for determining the clear-sky radiative flux, as well as for validating the retrieval algorithms associated with satellite sensors. Accurate, high spatial and temporal resolution profiles of water vapor are also required for assimilation into mesoscale models to improve weather forecasts. The authors have also developed and implemented routines to simultaneously retrieve profiles of relative humidity. These routines utilize the water vapor mixing ratio profiles derived from the Raman lidar measurements together with temperature profiles derived from a physical retrieval algorithm that uses data from a collocated Atmospheric Emitted Radiance Interferometer (AERI) and the Geostationary Operational Environmental Satellite (GOES). These aerosol and water vapor profiles (Raman lidar) and temperature profiles (AERI+GOES) have been combined into a single product that takes advantage of both active and passive remote sensors to characterize the clear sky atmospheric state above the CART site.

Ferrare, R.A.

2000-01-09T23:59:59.000Z

293

RAMAN LIDAR PROFILING OF WATER VAPOR AND AEROSOLS OVER THE ARM SGP SITE.  

SciTech Connect (OSTI)

We have developed and implemented automated algorithms to retrieve profiles of water vapor mixing ratio, aerosol backscattering, and aerosol extinction from Southern Great Plains (SGP) Cloud and Radiation Testbed (CART) Raman Lidar data acquired during both daytime and nighttime operations. This Raman lidar system is unique in that it is turnkey, automated system designed for unattended, around-the-clock profiling of water vapor and aerosols (Goldsmith et al., 1998). These Raman lidar profiles are important for determining the clear-sky radiative flux, as well as for validating the retrieval algorithms associated with satellite sensors. Accurate, high spatial and temporal resolution profiles of water vapor are also required for assimilation into mesoscale models to improve weather forecasts. We have also developed and implemented routines to simultaneously retrieve profiles of relative humidity. These routines utilize the water vapor mixing ratio profiles derived from the Raman lidar measurements together with temperature profiles derived from a physical retrieval algorithm that uses data from a collocated Atmospheric Emitted Radiance Interferometer (AERI) and the Geostationary Operational Environmental Satellite (GOES) (Feltz et al., 1998; Turner et al., 1999). These aerosol and water vapor profiles (Raman lidar) and temperature profiles (AERI+GOES) have been combined into a single product that takes advantage of both active and passive remote sensors to characterize the clear sky atmospheric state above the CART site.

FERRARE,R.A.

2000-01-09T23:59:59.000Z

294

Preparation of ferric-sulfide-based catalysts using an aerosol technique  

SciTech Connect (OSTI)

Iron sulfides are used as catalysts for direct coal liquefaction. They are reasonably active, cheap, and environmentally benign. This permits their use as once-through, non-regenerated catalysts. Our work in this area is based on the products of disproportionation of ferric sulfide, produced in sufficiently small particle sizes. The small particle sizes have been produced by in-situ impregnation or by using an aerosol reactor. This talk will concentrate on the aerosol process. The resulting particles have been characterized and used as catalysts for coal liquefaction. The effects of precursor solution concentration and the pressure and temperature in the aerosol reactor on the performance of the catalysts have been noted. We have recently investigated the effect of adding small amounts of a second metal to the catalyst. Multi-metal catalysts prepared to date with the aerosol technique include Fe-Cu-S and Fe-Zn-S, each with 10% additive, and Fe-Cu-Zn-S, with 10% Cu and 5% Zn.

Stiller, A.H.; Dadyburjor, D.B.; Stinespring, C.D. [West Virginia Univ., Morgantown, WV (United States)] [and others

1995-12-01T23:59:59.000Z

295

MIT Joint Program on the Science and Policy of Global Change  

E-Print Network [OSTI]

and aerosols. They are also connected because the atmospheric lifecycles of common air pollutants such as CO, atmospheric chemistry, climate and ecosystems to illustrate some effects of air pollution policy aloneMIT Joint Program on the Science and Policy of Global Change Effects of Air Pollution Control

296

Effect of Humidity on the Composition of Isoprene Photooxidation Secondary Organic Aerosol  

SciTech Connect (OSTI)

The effect of relative humidity (RH) on the composition and concentrations of gas-phase products and secondary organic aerosol (SOA) generated from the photooxidation of isoprene under high-NOx conditions was investigated. The yields of most gas-phase products were the same regardless of initial water vapor concentration with exception of hydroxyacetone and glycolaldehyde, which were considerably affected by RH. A significant change was observed in the SOA composition, with many unique condensed-phase products formed under humid (90% RH) vs. dry (<2% RH) conditions, without any observable effect on the rate and extent of the SOA mass growth.

Nguyen, Tran B.; Roach, Patrick J.; Laskin, Julia; Laskin, Alexander; Nizkorodov, Serguei

2011-07-18T23:59:59.000Z

297

Aerosol Science and Technology, 41:202216, 2007 Copyright c American Association for Aerosol Research  

E-Print Network [OSTI]

processes, such as con- densation, coagulation, gas-to-particle conversion (Reid et al. 1998), and particle Aerosol size distribution is, along with particle refractive in- dex and shape, one of important

298

Organic aerosol components observed in Northern Hemispheric datasets from Aerosol Mass Spectrometry  

E-Print Network [OSTI]

In this study we compile and present results from the factor analysis of 43 Aerosol Mass Spectrometer (AMS) datasets (27 of the datasets are reanalyzed in this work). The components from all sites, when taken together, ...

Kroll, Jesse

299

Characterization of the bi-directional reflectance (BRDF) of sea-ice in response to deposited aerosol for the inter-  

E-Print Network [OSTI]

aerosol for the inter- calibration and validation of satellite remotes sensing products. Supervisors of large areas of the globe. Remote sensing observations performed in the visible and near infrared (e-ice will be measured in the UV-Vis part of the solar spectrum as a function of zenith and azimuthal angles. The BRDF

Royal Holloway, University of London

300

Sources of organic aerosol investigated using organic compounds as tracers measured during CalNex in Bakersfield  

E-Print Network [OSTI]

to be mainly through gas-to-particle condensation of gas-phase oxidation products during the day. Our results) and provide insights into secondary organic aerosol (SOA) formation, positive matrix factorization analysis in the afternoon. Although contributions to SOA from oxidation of biogenic gas-phase compounds were less

Cohen, Ronald C.

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


301

GLOBAL WOOD SUPPLY Sten Nilsson  

E-Print Network [OSTI]

GLOBAL WOOD SUPPLY Sten Nilsson Biomass and Resource Efficiency: the need for a supply led approach to forest productivity European Parliament, Brussels, 10 November 2011 #12;MEGATREND WOOD SUPPLY 2020 the trees on the right Source: JP Management Consulting (Asia-Pacific) Ltd., 2006 #12;BAMBOO FOREST Source

302

Inter-annual Tropospheric Aerosol Variability in Late Twentieth Century and its Impact on Tropical Atlantic and West African Climate by Direct and Semi-direct Effects  

SciTech Connect (OSTI)

A new high-resolution (0.9$^{\\circ}$x1.25$^{\\circ}$ in the horizontal) global tropospheric aerosol dataset with monthly resolution is generated using the finite-volume configuration of Community Atmosphere Model (CAM4) coupled to a bulk aerosol model and forced with recent estimates of surface emissions for the latter part of twentieth century. The surface emissions dataset is constructed from Coupled Model Inter-comparison Project (CMIP5) decadal-resolution surface emissions dataset to include REanalysis of TROpospheric chemical composition (RETRO) wildfire monthly emissions dataset. Experiments forced with the new tropospheric aerosol dataset and conducted using the spectral configuration of CAM4 with a T85 truncation (1.4$^{\\circ}$x1.4$^{\\circ}$) with prescribed twentieth century observed sea surface temperature, sea-ice and greenhouse gases reveal that variations in tropospheric aerosol levels can induce significant regional climate variability on the inter-annual timescales. Regression analyses over tropical Atlantic and Africa reveal that increasing dust aerosols can cool the North African landmass and shift convection southwards from West Africa into the Gulf of Guinea in the spring season in the simulations. Further, we find that increasing carbonaceous aerosols emanating from the southwestern African savannas can cool the region significantly and increase the marine stratocumulus cloud cover over the southeast tropical Atlantic ocean by aerosol-induced diabatic heating of the free troposphere above the low clouds. Experiments conducted with CAM4 coupled to a slab ocean model suggest that present day aerosols can shift the ITCZ southwards over the tropical Atlantic and can reduce the ocean mixed layer temperature beneath the increased marine stratocumulus clouds in the southeastern tropical Atlantic.

Evans, Katherine J [ORNL; Hack, James J [ORNL; Truesdale, John [National Center for Atmospheric Research (NCAR); Mahajan, Salil [ORNL; Lamarque, J-F [University Center for Atmospheric Research

2012-01-01T23:59:59.000Z

303

Calibration of the On-Line Aerosol Monitor (OLAM) with ammonium chloride and sodium chloride aerosols  

SciTech Connect (OSTI)

The On-Line Aerosol Monitor (OLAM) is a light attenuation device designed and built at the Idaho National Engineering Laboratory (INEL) by EG&G Idaho. Its purpose is to provide an on-line indication of aerosol concentration in the PHEBUS-FP tests. It does this by measuring the attenuation of a light beam across a tube through which an aerosol is flowing. The OLAM does not inherently give an absolute response and must be calibrated. A calibration has been performed at Sandia National Laboratories` (SNL) Sandia Aerosol Research Laboratory (SARL) and the results are described here. Ammonium chloride and sodium chloride calibration aerosols are used for the calibration and the data for the sodium chloride aerosol is well described by a model presented in this report. Detectable instrument response is seen over a range of 0.1 cm{sup 3} of particulate material per m{sup 3} of gas to 10 cm{sup 3} of particulate material per m{sup 3} of gas.

Brockmann, J.E.; Lucero, D.A.; Romero, T. [Sandia National Labs., Albuquerque, NM (United States); Pentecost, G. [Idaho National Engineering Lab., Idaho Falls, ID (United States)

1993-12-01T23:59:59.000Z

304

A new aerosol collector for quasi on-line analysis of particulate organic matter: the Aerosol Collection Module (ACM) and first applications with a GC/MS-FID  

E-Print Network [OSTI]

In many environments organic matter significantly contributes to the composition of atmospheric aerosol particles influencing its properties. Detailed chemical characterization of ambient aerosols is critical in order to ...

Hohaus, T.

305

The Contribution of Biomass to Emissions Mitigation under a Global Climate Policy  

E-Print Network [OSTI]

What will large-scale global bioenergy production look like? We investigate this question by developing a detailed representation of bioenergy in a global economy-wide model. We develop a scenario with a global carbon ...

Winchester, N.

306

Uncertainties and Frontiers in Aerosol Research  

E-Print Network [OSTI]

;Transport Power Industry Biomass burning Residential Human activity Perspective Aerosol Sources (rather than, Mixing, Chemistry, Climate) Climate Effects Resource: AeroCom, an international model intercomparison of fossil fuel (coal, oil, diesel, gasoline), domestic wood burning, forest fires #12;Natural sources

307

Aerosol Spray Synthesis of Porous Molybdenum Sulfide  

E-Print Network [OSTI]

, and colloidal silica, SiO2, was ultrasonically nebulized using a household humidifier; the resulting aerosol in materials science because of their ability to be scaled-up for industrial applications.[2] USP solution, as indicated by Eq. 2. Typically, micron-sized particles are obtained; however, by adding

Suslick, Kenneth S.

308

3, 59195976, 2003 The nitrate aerosol  

E-Print Network [OSTI]

ACPD 3, 5919­5976, 2003 The nitrate aerosol field over Europe M. Schaap et al. Title Page Abstract of Utrecht, Institute of Marine and Atmospheric Science, PO Box 80005, 3508 TA, Utrecht, The Netherlands 2, The Netherlands 3 Netherlands Energy Research Foundation (ECN), PO Box 1, 1755 LE Petten, The Netherlands 4 Joint

Paris-Sud XI, Université de

309

Source Apportionment of Carbonaceous Aerosols using  

E-Print Network [OSTI]

are different than the collection of particles from water Filtration has high efficiency for all sizes Size Condensation Nuclei (CCN) Human health Carbonaceous aerosol implicated as important for toxicity and adverse of particulate matter Again, agreement between these two approaches would give a high level of confidence

Einat, Aharonov

310

A Global Assessment of Manufacturing: Economic  

E-Print Network [OSTI]

A Global Assessment of Manufacturing: Economic Development, Energy Use, Carbon Emissions Keywords production, materials, closed loop, China, emerging economies Abstract We present in two parts an assessment of global manufacturing. In the first part, we review economic development, pollution, and carbon

Gutowski, Timothy

311

A Computational Approach to Understanding Aerosol Formation and Oxidant Chemistry in the Troposphere  

SciTech Connect (OSTI)

An understanding of the mechanisms and kinetics of aerosol formation and ozone production in the troposphere is currently a high priority because these phenomena are recognized as two major effects of energy-related air pollution. Atmospheric aerosols are of concern because of their effect on visibility, climate, and human health. Equally important, aerosols can change the chemistry of the atmosphere, in dramatic fashion, by providing new chemical pathways (in the condensed phase) unavailable in the gas phase. The oxidation of volatile organic compounds (VOCs) and inorganic compounds (e.g., sulfuric acid, ammonia, nitric acid, ions, and mineral) can produce precursor molecules that act as nucleation seeds. The U.S. Department of Energy (DOE) Atmospheric Chemistry Program (ACP) has identified the need to evaluate the causes of variations in tropospheric aerosol chemical composition and concentrations, including determining the sources of aerosol particles and the fraction of such that are of primary and secondary origin. In particular, the ACP has called for a deeper understanding into aerosol formation because nucleation creates substantial concentrations of fresh particles that, via growth and coagulation, influence the Earth's radiation budget. Tropospheric ozone is also of concern primarily because of its impact on human health. Ozone levels are controlled by NOx and by VOCs in the lower troposphere. The VOCs can be either from natural emissions from such sources as vegetation and phytoplankton or from anthropogenic sources such as automobiles and oil-fueled power production plants. The major oxidant for VOCs in the atmosphere is the OH radical. With the increase in VOC emissions, there is rising concern regarding the available abundance of HOx species needed to initiate oxidation. Over the last five years, there have been four field studies aimed at initial measurements of HOx species (OH and HO? radicals). These measurements revealed HOx levels that are two to four times higher than expected from the commonly assumed primary sources. Such elevated abundances of HOx imply a more photochemically active troposphere than previously thought. This implies that rates of ozone formation in the lower region of the atmosphere and the oxidation of SO? can be enhanced, thus promoting the formation of new aerosol properties. Central to unraveling this chemistry is the ability to assess the photochemical product distributions resulting from the photodissociation of by-products of VOC oxidation. We propose to use state-of-the-art theoretical techniques to develop a detailed understanding of the mechanisms of aerosol formation in multicomponent (mixed chemical) systems and the photochemistry of atmospheric organic species. The aerosol studies involve an approach that determines homogeneous gas-particle nucleation rates from knowledge of the molecular interactions that are used to define properties of molecular clusters. Over the past several years we developed Dynamical Nucleation Theory (DNT), a novel advance in the theoretical description of homogeneous gas-liquid nucleation, and applied it to gas-liquid nucleation of a single component system (e.g., water). The goal of the present research is to build upon these advances by extending the theory to multicomponent systems important in the atmosphere (such as clusters containing sulfuric acid, water, ions, ammonia, and organics). In addition, high-level ab initio electronic structure calculations will be used to unravel the chemical reactivity of the OH radical and water clusters.

Francisco, Joseph S.; Kathmann, Shawn M.; Schenter, Gregory K.; Dang, Liem X.; Xantheas, Sotiris S.; Garrett, Bruce C.; Du, Shiyu; Dixon, David A.; Bianco, Roberto; Wang, Shuzhi; Hynes, James T.; Morita, Akihiro; Peterson, Kirk A.

2006-04-18T23:59:59.000Z

312

Integrated decision support model for global sourcing  

E-Print Network [OSTI]

Over the last decade, the U.S. aircraft industry has experienced increasing levels of international integration as companies seek to access global talent and resources, cut production costs, spread financial risk, and ...

Mroczkowski, Victor A. (Victor Adam)

2008-01-01T23:59:59.000Z

313

Global Climate Change and National Security  

E-Print Network [OSTI]

5/16/2014 1 Global Climate Change and National Security RADM Jon White Oceanographer and Navigator months. · Oil, gas, and mineral resource exploitation expected to continue · Production/transportatio n

Howat, Ian M.

314

Direct and semidirect aerosol effects of Southern African biomass burning aerosol  

SciTech Connect (OSTI)

The direct and semi-direct radiative effects of biomass burning aerosols from Southern African fires during July-October are investigated using 20 year runs of the Community Atmospheric Model (CAM) coupled to a slab ocean model. The aerosol optical depth is constrained using observations in clear skies from MODIS and for aerosol layers above clouds from CALIPSO. Over the ocean, where the absorbing biomass burning aerosol layers are primarily located above cloud, negative top of atmosphere (TOA) semi-direct radiative effects associated with increased low cloud cover dominate over a weaker positive all-sky direct radiative effect (DRE). In contrast, over the land where the aerosols are often below or within cloud layers, reductions in cloud liquid water path (LWP) lead to a positive semi-direct radiative effect that dominates over a near-zero DRE. Over the ocean, the cloud response can be understood as a response to increased lower tropospheric stability (LTS) which is caused both by aerosol absorptive warming in overlying layers and surface cooling in response to direct aerosol forcing. The ocean cloud changes are robust to changes in the cloud parameterization (removal of the hard-wired dependence of clouds on LTS), suggesting that they are physically realistic. Over land where cloud cover changes are minimal, decreased LWP is consistent with weaker convection driven by increased static stability. Over the entire region the overall TOA radiative effect from the biomass burning aerosols is almost zero due to opposing effects over the land and ocean. However, the surface forcing is strongly negative requiring a reduction in precipitation. This is primarily realized through reductions in convective precipitation on both the southern and northern flanks of the convective precipitation region spanning the equatorial rainforest and the ITCZ in the southern Sahel. The changes are consistent with the low-level aerosol forced cooling pattern. The results highlight the importance of semi-direct radiative effects and precipitation responses for determining the climatic effects of aerosols in the African region.

Sakaeda, Naoko; Wood, Robert; Rasch, Philip J.

2011-06-21T23:59:59.000Z

315

Composition analyses of size-resolved aerosol samples taken from aircraft downwind of Kuwait, Spring 1991  

SciTech Connect (OSTI)

Analyses are reported for eight aerosol samples taken from the National Center for Atmospheric Research Electra typically 200 to 250 km downwind of Kuwait between May 19 and June 1, 1991. Aerosols were separated into fine (D{sub p} < 2.5 {mu}m) and coarse (2.5 < D{sub p} 10 {mu}m) particles for optical, gravimetric, X ray and nuclear analyses, yielding information on the morphology, mass, and composition of aerosols downwind of Kuwait. The mass of coarse aerosols ranged between 60 and 1971 {mu}g/m{sup 3} and, while dominated by soil derived aerosols, contained considerable content of sulfates and salt (NaCl) and soot in the form of fluffy agglomerates. The mass of fine aerosols varied between 70 and 785 {mu}g/m{sup 3}, of which about 70% was accounted for via compositional analyses performed in vacuum. While most components varied greatly from flight to flight, organic matter and fine soils each accounted for about 1/4 of the fine mass, while salt and sulfates contributed about 10% and 7%, respectively. The Cl/S ratios were remarkably constant, 2.4 {+-} 1.2 for coarse particles and 2.0 {+-} 0.2 for fine particles, with one flight deleted in each case. Vanadium, when observed, ranged from 9 to 27 ng/m{sup 3}, while nickel ranged from 5 to 25 ng/m{sup 3}. In fact, fine sulfates, vanadium, and nickel occurred in levels typical of Los Angeles, California, during summer 1986. The V/Ni ratio, 1.7 {+-} 0.4, was very similar to the ratios measured in fine particles from combusted Kuwaiti oil, 1.4 {+-} 0.9. Bromine, copper, zinc, and arsenic/lead were also observed at levels between 2 and 190 ng/m{sup 3}. The presence of massive amounts of fine, typically alkaline soils in the Kuwaiti smoke plumes significantly modified their behavior and probably mitigated their impacts, locally and globally. 16 refs., 1 fig., 3 tabs.

Cahill, T.A.; Wilkinson, K. [Univ. of California, Davis, CA (United States); Schnell, R. [National Center for Atmospheric Research, Boulder, CO (United States)

1992-09-20T23:59:59.000Z

316

15 Minutes about satellite aerosol products (from VIIRS)  

E-Print Network [OSTI]

.221 MISR N=903 r=0.107 #12;Conditions for success of Empirical AODtoPM conversion · Calibration case (AOD

Jacob, Daniel J.

317

Climate Engineering with Stratospheric Aerosols and Associated Engineering Parameters  

SciTech Connect (OSTI)

Climate engineering with stratospheric aerosols, an idea inspired by large volcaniceruptions, could cool the Earths surface and thus alleviate some of the predicted dangerous impacts of anthropogenic climate change. However, the effectiveness of climate engineering to achieve a particular climate goal, and any associated side effects, depend on certain aerosol parameters and how the aerosols are deployed in the stratosphere. Through the examples of sulfate and black carbon aerosols, this paper examines "engineering" parameters-aerosol composition, aerosol size, and spatial and temporal variations in deployment-for stratospheric climate engineering. The effects of climate engineering are sensitive to these parameters, suggesting that a particle could be found ordesigned to achieve specific desired climate outcomes. This prospect opens the possibility for discussion of societal goals for climate engineering.

Kravitz, Benjamin S.

2013-02-12T23:59:59.000Z

318

Retrieval of ozone and nitrogen dioxide concentrations from Stratospheric Aerosol and Gas Experiment III (SAGE III)  

E-Print Network [OSTI]

Retrieval of ozone and nitrogen dioxide concentrations from Stratospheric Aerosol and Gas extinction. We retrieve ozone and nitrogen dioxide number densities and aerosol extinction from transmission), Retrieval of ozone and nitrogen dioxide concentrations from Stratospheric Aerosol and Gas Experiment III

319

Correction to "Sulfuric acid deposition from stratospheric geoengineering with sulfate aerosols"  

E-Print Network [OSTI]

Correction to "Sulfuric acid deposition from stratospheric geoengineering with sulfate aerosols (2010), Correction to "Sulfuric acid deposition from stratospheric geoengineering with sulfate aerosols from stratospheric geoengineering with sulfate aerosols" (Journal of Geophysical Research, 114, D14109

Robock, Alan

320

Statistical analysis of aerosol species, trace gasses, and meteorology in Chicago  

E-Print Network [OSTI]

possible pollutant sources. Keywords Atmospheric aerosols . Canonical correlation analysis . Chicago air pollution studies involve collection and anal- ysis of atmospheric aerosols and concurrent meteorol- ogy) and principal component analysis (PCA) were applied to atmospheric aerosol and trace gas concentrations

O'Brien, Timothy E.

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


321

AEROSOL METROLOGY FOR MARCH 14 15, 2011  

E-Print Network [OSTI]

to leading the charge to reduce the dangerous pollution that causes global warming. #12;NIST GREENHOUSE GAS

322

Aerosol Retrievals from ARM SGP MFRSR Data  

DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

The Multi-Filter Rotating Shadowband Radiometer (MFRSR) makes precise simultaneous measurements of the solar direct normal and diffuse horizontal irradiances at six wavelengths (nominally 415, 500, 615, 673, 870, and 940 nm) at short intervals (20 sec for ARM instruments) throughout the day. Time series of spectral optical depth are derived from these measurements. Besides water vapor at 940 nm, the other gaseous absorbers within the MFRSR channels are NO2 (at 415, 500, and 615 nm) and ozone (at 500, 615, and 670 nm). Aerosols and Rayleigh scattering contribute atmospheric extinction in all MFRSR channels. Our recently updated MFRSR data analysis algorithm allows us to partition the spectral aerosol optical depth into fine and coarse modes and to retrieve the fine mode effective radius. In this approach we rely on climatological amounts of NO2 from SCIAMACHY satellite retrievals and use daily ozone columns from TOMS.

Alexandrov, Mikhail

323

Stackable differential mobility analyzer for aerosol measurement  

DOE Patents [OSTI]

A multi-stage differential mobility analyzer (MDMA) for aerosol measurements includes a first electrode or grid including at least one inlet or injection slit for receiving an aerosol including charged particles for analysis. A second electrode or grid is spaced apart from the first electrode. The second electrode has at least one sampling outlet disposed at a plurality different distances along its length. A volume between the first and the second electrode or grid between the inlet or injection slit and a distal one of the plurality of sampling outlets forms a classifying region, the first and second electrodes for charging to suitable potentials to create an electric field within the classifying region. At least one inlet or injection slit in the second electrode receives a sheath gas flow into an upstream end of the classifying region, wherein each sampling outlet functions as an independent DMA stage and classifies different size ranges of charged particles based on electric mobility simultaneously.

Cheng, Meng-Dawn (Oak Ridge, TN); Chen, Da-Ren (Creve Coeur, MO)

2007-05-08T23:59:59.000Z

324

Aerosol Working Group Contributions Accomplishments for 2006  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr MayAtmospheric Optical Depth (AOD)ProductssondeadjustsondeadjustAbout the BuildingInnovation 2011 Simulation StudiesAerosol

325

Review: engineering particles using the aerosol-through-plasma method  

SciTech Connect (OSTI)

For decades, plasma processing of materials on the nanoscale has been an underlying enabling technology for many 'planar' technologies, particularly virtually every aspect of modern electronics from integrated-circuit fabrication with nanoscale elements to the newest generation of photovoltaics. However, it is only recent developments that suggest that plasma processing can be used to make 'particulate' structures of value in fields, including catalysis, drug delivery, imaging, higher energy density batteries, and other forms of energy storage. In this paper, the development of the science and technology of one class of plasma production of particulates, namely, aerosol-through-plasma (A-T-P), is reviewed. Various plasma systems, particularly RF and microwave, have been used to create nanoparticles of metals and ceramics, as well as supported metal catalysts. Gradually, the complexity of the nanoparticles, and concomitantly their potential value, has increased. First, unique two-layer particles were generated. These were postprocessed to create unique three-layer nanoscale particles. Also, the technique has been successfully employed to make other high-value materials, including carbon nanotubes, unsupported graphene, and spherical boron nitride. Some interesting plasma science has also emerged from efforts to characterize and map aerosol-containing plasmas. For example, it is clear that even a very low concentration of particles dramatically changes plasma characteristics. Some have also argued that the local-thermodynamic-equilibrium approach is inappropriate to these systems. Instead, it has been suggested that charged- and neutral-species models must be independently developed and allowed to 'interact' only in generation terms.

Phillips, Jonathan [Los Alamos National Laboratory; Luhrs, Claudia C [UNM; Richard, Monique [TEMA

2009-01-01T23:59:59.000Z

326

ARM - Surface Aerosol Observing System  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr May JunDatastreamsmmcrcalgovInstrumentsruc Documentation RUC :ProductsSCM Forcing DataScienceSteering Committee RelatedFacilitiesSurface

327

aerosol challenge model: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

climate change is important because of its strong capability in causing extinction of solar radiation. A three-dimensional interactive aerosol-climate model has been used to...

328

aircraft exhaust aerosol: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Window Location on a King Air 200 Aircraft:aerosol.atmos.und.edu) Objective A Raytheon Beechcraft King Air 200 aircraft has been used to obtain Condensation Particle...

329

aerosol mass spectrometry: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

analysis of aerosol organic nitrates with electron ionization high-resolution mass spectrometry MIT - DSpace Summary: Four hydroxynitrates (R(OH)R'ONO2) representative of...

330

aerosol assisted chemical: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

soluble in water: 2. Isolation of acid, neutral, and basic fractions by modified size Weber, Rodney 5 Simulating Aerosols Using a Chemical Transport Model with Assimilation of...

331

ambient fine aerosols: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

soluble in water: 2. Isolation of acid, neutral, and basic fractions by modified size Weber, Rodney 4 Chemical characterization of the ambient organic aerosol soluble in water:...

332

aerosol chemical characteristion: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

soluble in water: 2. Isolation of acid, neutral, and basic fractions by modified size Weber, Rodney 5 Simulating Aerosols Using a Chemical Transport Model with Assimilation of...

333

aerosol characterization experiment: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

soluble in water: 2. Isolation of acid, neutral, and basic fractions by modified size Weber, Rodney 8 Desert dust aerosol age characterized by massage tracking of tracers...

334

aerosol generation characterization: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

soluble in water: 2. Isolation of acid, neutral, and basic fractions by modified size Weber, Rodney 5 Desert dust aerosol age characterized by massage tracking of tracers...

335

aerosol monitor development: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Paris May 2003John Matthews Monitoring the Aerosol Phase Function University of New Mexico 12;AstroParticles & Atmosphere, Paris May 2003John Matthews 12;AstroParticles &...

336

aerosol particle charger: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Introduction The Universal Serial Bus (USB) port Allen, Jont 9 New approaches for the chemical and physical characterization of aerosols using a single particle mass spectrometry...

337

aerosol mass spectrometer: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

2004. The concentration of a species Zhang, Qi 8 Development of a thermal desorption chemical ionization mobility mass spectrometer for the speciation of ultrafine aerosols. Open...

338

aerosol particles generated: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

the chemical and physical characterization of aerosols using a single particle mass spectrometry based technique University of California eScholarship Repository Summary: Real-...

339

aerosol monitors including: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

schemes which explicitly simulate the microphysical processes that determine the particle size distribution. These models enable aerosol optical ... Ridley, David Andrew 33...

340

aerosol retrieval validation: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

off the coast of Chile and Peru, where aerosol-cloud interactions are important to the energy balance (15), and limitations in current observing and modeling capabilities...

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


341

aerosol detection equipment: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Daniel, Rosenfeld 464 Mixtures of pollution, dust, sea salt, and volcanic aerosol during ACE-Asia: Radiative properties Energy Storage, Conversion and Utilization Websites...

342

Aerosol generation and entrainment model for cough simulations.  

E-Print Network [OSTI]

??The airborne transmission of diseases is of great concern to the public health community. The possible spread of infectious disease by aerosols is of particular (more)

Ersahin, Cem.

2007-01-01T23:59:59.000Z

343

atmospheric aerosols basic: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

of atmospheric aerosol. Aplin, KL 2012-01-01 13 1. Introduction The atmospheric greenhouse effect is the basic mechanism Environmental Sciences and Ecology Websites Summary: 1....

344

Aerosols, Clouds, and Climate Change Stephen E. Schwartz  

E-Print Network [OSTI]

in atmospheric carbon dioxide associated with fossil fuel combustion. Briefly the options are mitigation work has shown instances of large magnitude of aerosol indirect forcing, with local instantaneous

Schwartz, Stephen E.

345

Atmospheric pressure flow reactor / aerosol mass spectrometer studies of tropospheric aerosol nucleat and growth kinetics. Final report, June, 2001  

SciTech Connect (OSTI)

The objective of this program was to determine the mechanisms and rates of growth and transformation and growth processes that control secondary aerosol particles in both the clear and polluted troposphere. The experimental plan coupled an aerosol mass spectrometer (AMS) with a chemical ionization mass spectrometer to provide simultaneous measurement of condensed and particle phases. The first task investigated the kinetics of tropospheric particle growth and transformation by measuring vapor accretion to particles (uptake coefficients, including mass accommodation coefficients and heterogeneous reaction rate coefficients). Other work initiated investigation of aerosol nucleation processes by monitoring the appearance of submicron particles with the AMS as a function of precursor gas concentrations. Three projects were investigated during the program: (1) Ozonolysis of oleic acid aerosols as model of chemical reactivity of secondary organic aerosol; (2) Activation of soot particles by measurement deliquescence in the presence of sulfuric acid and water vapor; (3) Controlled nucleation and growth of sulfuric acid aerosols.

Worsnop, Douglas R.

2001-06-01T23:59:59.000Z

346

Global Health Seminar Series  

E-Print Network [OSTI]

Bay Area Global Health Seminar Series Moving beyond millennium targets in global health: The challenges of investing in health and universal health coverage Although targets can help to focus global health efforts, they can also detract attention from deeper underlying challenges in global health

Klein, Ophir

347

Global Warming Observations  

E-Print Network [OSTI]

Global Warming Observations: 1. Global temperature has been gradually rising in recent years #15 in range 8000 12000 nm { CFC's, methane and N 2 O important for global warming even though concentra- tions in concentration of \\greenhouse gases" like CO 2 What determines global temperature? Energy budget of earth: 1

Schofield, Jeremy

348

Final Report for ?¢????Cloud-Aerosol Physics in Super-Parameterized Atmospheric Regional Climate Simulations (CAP-SPARCS)?¢??? (DE-SC0002003) for 8/15/2009 through 8/14/2012  

SciTech Connect (OSTI)

Improving the representation of local and non-local aerosol interactions in state-of-the-science regional climate models is a priority for the coming decade (Zhang, 2008). With this aim in mind, we have combined two new technologies that have a useful synergy: (1) an aerosol-enabled regional climate model (Advanced Weather Research and Forecasting Model with Chemistry WRF-Chem), whose primary weakness is a lack of high quality boundary conditions and (2) an aerosol-enabled multiscale modeling framework (PNNL Multiscale Aerosol Climate Model (MACM)), which is global but captures aerosol-convection-cloud feedbacks, and thus an ideal source of boundary conditions. Combining these two approaches has resulted in an aerosol-enabled modeling framework that not only resolves high resolution details in a particular region, but crucially does so within a global context that is similarly faithful to multi-scale aerosol-climate interactions. We have applied and improved the representation of aerosol interactions by evaluating model performance over multiple domains, with (1) an extensive evaluation of mid-continent precipitation representation by multiscale modeling, (2) two focused comparisons to transport of aerosol plumes to the eastern United States for comparison with observations made as part of the International Consortium for Atmospheric Research on Transport and Transformation (ICARTT), with the first being idealized and the second being linked to an extensive wildfire plume, and (3) the extension of these ideas to the development of a new approach to evaluating aerosol indirect effects with limited-duration model runs by ?¢????nudging?¢??? to observations. This research supported the work of one postdoc (Zhan Zhao) for two years and contributed to the training and research of two graduate students. Four peer-reviewed publications have resulted from this work, and ground work for a follow-on project was completed.

Lynn M. Russell; Richard C.J. Somerville

2012-11-05T23:59:59.000Z

349

1CHILE'S FRONTIER FORESTS: CONSERVING A GLOBAL TREASURE FRONTIER FORESTS  

E-Print Network [OSTI]

1CHILE'S FRONTIER FORESTS: CONSERVING A GLOBAL TREASURE CHILE´S FRONTIER FORESTS: CONSERVING forests & people #12;2 CHILE'S FRONTIER FORESTS: CONSERVING A GLOBAL TREASURE REPORT PRODUCTION'S FRONTIER FORESTS: CONSERVING A GLOBAL TREASURE CONTENTSCONTENTS ACKNOWLEDGMENTS 5 FOREWORD 6 KEY FINDINGS 8

350

Emission and Chemistry of Organic Carbon in the Gas and Aerosol Phase at a Sub-Urban Site Near Mexico City in March 2006 During the MILAGRO Study  

SciTech Connect (OSTI)

Volatile organic compounds (VOCs) and carbonaceous aerosol were measured at a sub-urban site near Mexico City in March of 2006 during the MILAGRO study (Megacity Initiative: Local and Global Research Objectives). Diurnal variations of hydrocarbons, elemental carbon (EC) and hydrocarbon-like organic aerosol (HOA) were dominated by a high peak in the early morning when local emissions accumulated in a shallow boundary layer, and a minimum in the afternoon when the emissions were diluted in a significantly expanded boundary layer and, in case of the reactive gases, removed by OH. In comparison, diurnal variations of species with secondary sources such as the aldehydes, ketones, oxygenated organic aerosol (OOA) and water-soluble organic carbon (WSOC) stayed relatively high in the afternoon indicating strong photochemical formation. Emission ratios of many hydrocarbon species relative to CO were higher in Mexico City than in the U.S., but we found similar emission ratios for most oxygenated VOCs and organic aerosol. Secondary formation of acetone may be more efficient in Mexico City than in the U.S., due to higher emissions of alkane precursors from the use of liquefied petroleum gas. Secondary formation of organic aerosol was similar between Mexico City and the U.S. Combining the data for all measured gas and aerosol species, we describe the budget of total observed organic carbon (TOOC), and find that the enhancement ratio of TOOC relative to CO is conserved between the early morning and mid afternoon despite large compositional changes. Finally, the influence of biomass burning is investigated using the measurements of acetonitrile, which was found to correlate with levoglucosan in the particle phase. Diurnal variations of acetonitrile indicate a contribution from local burning sources. Scatter plots of acetonitrile versus CO suggest that the contribution of biomass burning to the enhancement of most gas and aerosol species was not dominant and perhaps not dissimilar from observations in the U.S.

de Gouw, Joost A.; Welsh-Bon, Daniel; Warneke, Carsten; Kuster, W. C.; Alexander, M. L.; Baker, Angela K.; Beyersdorf, Andreas J.; Blake, D. R.; Canagaratna, Manjula R.; Celada, A. T.; Huey, L. G.; Junkermann, W.; Onasch, Timothy B.; Salcido, A.; Sjostedt, S. J.; Sullivan, Amy; Tanner, David J.; Vargas-Ortiz, Leroy; Weber, R. J.; Worsnop, Douglas R.; Yu, Xiao-Ying; Zaveri, Rahul A.

2009-05-28T23:59:59.000Z

351

E-Print Network 3.0 - administrado como aerosol Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

del ozono estratosfrico, los aerosoles atmosfricos y... a los cambios en las emisiones que los GEI de larga duracin, como el CO2. Los aerosoles antropgenos... ms...

352

E-Print Network 3.0 - aerosol robotic network Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

), AERONET--A federated instrument network and data archive for aerosol characterization, Remote Sens... Period examining aerosol properties and radiative ... Source: Brookhaven...

353

E-Print Network 3.0 - aerosol condensation model Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Applied Science Collection: Environmental Sciences and Ecology 8 DETERMINING AEROSOL RADIATIVE FORCING AT ARM SITES Summary: OF AEROSOL DIRECT FORCING By linear model and by...

354

SciTech Connect: Results and code predictions for ABCOVE aerosol...  

Office of Scientific and Technical Information (OSTI)

Results and code predictions for ABCOVE aerosol code validation - Test AB5 Citation Details In-Document Search Title: Results and code predictions for ABCOVE aerosol code...

355

E-Print Network 3.0 - aerosolized polymerized type Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

spheric aerosol particles and isolated from fog... in atmospheric aerosol particles and rainwater in the 1980's (Si- moneit, 1980; Likens and ... Source: Ecole Polytechnique,...

356

E-Print Network 3.0 - aerosol radiative forcing Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

No. DE- Summary: : WHY MEASUREMENTS ALONE CANNOT QUANTIFY AEROSOL RADIATIVE FORCING OF CLIMATE CHANGE Stephen E. Schwartz... of radiative forcing of climate change by aerosols,...

357

E-Print Network 3.0 - aerosols nanometriques application Sample...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

is studying how aerosol particles affect everything from Summary: of aerosol particles on climate change, public health, and renewable energy applications. In particular, he......

358

E-Print Network 3.0 - aerosol main physical Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AND INTEGRAL AEROSOL PROPERTIES RETRIEVAL FROM RAMAN LIDAR DATA USING PRINCIPLE COMPONENT ANALYSIS Summary: retrievals of physical aerosol parameters from ground-based and...

359

Aerosol-Cloud-Precipitation Interactions in the Trade Wind Boundary Layer.  

E-Print Network [OSTI]

??This dissertation includes an overview of aerosol, cloud, and precipitation properties associated with shallow marine cumulus clouds observed during the Barbados Aerosol Cloud Experiment (BACEX, (more)

Jung, Eunsil

2012-01-01T23:59:59.000Z

360

E-Print Network 3.0 - aerosol light absorption Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AND Summary: population centers were used to calculate the aerosol forcing due to light scattering and absorption. Directly... , NY www.bnl.gov ABSTRACT Aerosols influence...

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


361

Large Aerosols Play Unexpected Role in Ganges Valley | U.S. DOE...  

Office of Science (SC) Website

The data have revealed that large aerosols in this region absorb a greater amount of light than expected. The Science Aerosol particles in the atmosphere may absorb solar...

362

E-Print Network 3.0 - aerosol atmospheric interactions Sample...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

for Climate Summary: order estimates of aerosol-climate interaction But... only Earth System Models can include all... of the interactions (in theory at least) 12;Aerosols <>...

363

E-Print Network 3.0 - atmospheric aerosol size Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

for about ten percent of all aerosols in the atmosphere. We... , can actually absorb solar energy and warm the atmosphere. Atmospheric aerosols are very important... by...

364

aerosol source-receptor relationships: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

ON CCN CONCENTRATION AND AEROSOL FIRST INDIRECT RADIATIVE composition, aerosol size distribution is the more dominant parameter on CCN activation Feingold, GRL 2003;...

365

E-Print Network 3.0 - aerosol particle size Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Summary: of aerosol over many orders-of-magnitude of particle size range, from subcritical clusters on the molecular... to modeling aerosol dynamics under conditions of new...

366

E-Print Network 3.0 - aerosol load study Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

conditions... reserved. Keywords: India; Aerosol loading; Aerosol forcing; MODIS; TOMS; Remote sensing 1. Introduction... heating effect on the earth surface and in turn...

367

E-Print Network 3.0 - analysis od aerosol Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Tivanski, Rebecca Hopkins, Yury Desyaterik... of Aerosols 12;Aerosol Transport From Mexico City During MILAGRO T0 T1 T2 Mexico ... Source: Brookhaven National Laboratory,...

368

Changing Global Petroleum Product Trade Flows  

Gasoline and Diesel Fuel Update (EIA)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr May Jun Jul(Summary) " ,"Click worksheet9,1,50022,3,,,,6,1,,781Title: Telephone:shortOil andMCKEESPORTfor the 2012 CBECS

369

Changing Global Petroleum Product Trade Flows  

Gasoline and Diesel Fuel Update (EIA)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr May Jun Jul(Summary) " ,"Click worksheet9,1,50022,3,,,,6,1,,781Title: Telephone:shortOil andMCKEESPORTfor the 2012 CBECS4 ©

370

Development and Characterization of a Thermodenuder for Aerosol Volatility Measurements  

SciTech Connect (OSTI)

This SBIR Phase I project addressed the critical need for improved characterization of carbonaceous aerosol species in the atmosphere. The proposed work focused on the development of a thermodenuder (TD) system capable of systematically measuring volatility profiles of primary and secondary organic aerosol species and providing insight into the effects of absorbing and nonabsorbing organic coatings on particle absorption properties. This work provided the fundamental framework for the generation of essential information needed for improved predictions of ambient aerosol loadings and radiative properties by atmospheric chemistry models. As part of this work, Aerodyne Research, Inc. (ARI) continued to develop and test, with the final objective of commercialization, an improved thermodenuder system that can be used in series with any aerosol instrument or suite of instruments (e.g., aerosol mass spectrometers-AMS, scanning mobility particle sizers-SMPS, photoacoustic absorption spectrometers-PAS, etc.) to obtain aerosol chemical, physical, and optical properties as a function of particle volatility. In particular, we provided the proof of concept for the direct coupling of our improved TD design with a full microphysical model to obtain volatility profiles for different organic aerosol components and to allow for meaningful comparisons between different TD-derived aerosol measurements. In a TD, particles are passed through a heated zone and a denuding (activated charcoal) zone to remove semi-volatile material. Changes in particle size, number concentration, optical absorption, and chemical composition are subsequently detected with aerosol instrumentation. The aerosol volatility profiles provided by the TD will strengthen organic aerosol emission inventories, provide further insight into secondary aerosol formation mechanisms, and provide an important measure of particle absorption (including brown carbon contributions and identification, and absorption enhancements due to coatings on soot particles). The successfully completed Phase I project included construction of a prototype design for the TD with detailed physical modeling, testing with laboratory and ambient aerosol particles, and the initiation of a detailed microphysical model of the aerosol particles passing through the TD to extract vapor pressure distributions. The objective of the microphysical model is to derive vapor pressure distributions (i.e. vapor pressure ranges, including single chemical compounds, mixtures of known compounds, and complex real-world aerosols, such as SOA, and soot particles with absorbing and nonabsorbing coatings) from TD measurements of changes in particle size, mass, and chemical composition for known TD temperatures and flow rates (i.e. residence times). The proposed Phase II project was designed to optimize several TD systems for different instrument applications and to combine the hardware and modeling into a robust package for commercial sales.

Dr. Timothy Onasch

2009-09-09T23:59:59.000Z

371

Evaluation of source-term data for plutonium aerosolization  

SciTech Connect (OSTI)

Relevant data are reviewed and evaluated in an effort to define the time dependence and maximum value of the source term for plutonium aerosolization during a fuel fire. The rate of plutonium oxidation at high temperatures is a major determinant of the time dependence. Analysis of temperature-time data for oxidation of plutonium shows that the rate is constant (0.2 g PUO{sub 2}/cm{sup 2} of metal surface per min) and independent of temperature above 500{degrees}C. Total mass and particle distributions are derived for oxide products formed by reactions of plutonium metal and hydride. The mass distributions for products of all metal-gas reactions are remarkably similar with approximately 0.07 mass% of the oxide particles having geometric diameters {le} 10 {mu}m. In comparison, 25 mass% of the oxide formed by the PuH{sub 2}+O{sub 2} reaction is in this range. Experimental values of mass fractions released during oxidation are evaluated and factors that alter the release fraction are discussed.

Haschke, J.M.

1992-07-01T23:59:59.000Z

372

Variability of Aerosol Optical Properties from Long-term  

E-Print Network [OSTI]

%) controlled measurements: sp ­ Aerosol total light scattering coefficient at 450, 550, and 700 nm wavelengths automated generation and review of quality control plots · Weekly editing of data by station scientist]. Indirect Forcing Direct Forcing Carbon Dioxide Forcing Total Forcing Importance of Aerosols #12;Direct

Delene, David J.

373

An overview of geoengineering of climate using stratospheric sulphate aerosols  

E-Print Network [OSTI]

REVIEW An overview of geoengineering of climate using stratospheric sulphate aerosols BY PHILIP J, MD 21218, USA We provide an overview of geoengineering by stratospheric sulphate aerosols. The state after geoengineering, with some regions experiencing significant changes in temperature or precipitation

Robock, Alan

374

aerosol ratio test: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

aerosol ratio test First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Effect of mineral dust aerosol...

375

Organic Aerosol Formation Downwind from the Deepwater Horizon Oil Spill  

E-Print Network [OSTI]

Organic Aerosol Formation Downwind from the Deepwater Horizon Oil Spill Nicole ONeill - ATOC 3500 and aerosol composition of air over the Deepwater Horizon oil spill in the Gulf of Mexico. · The lightest chemicals in the oil evaporated within hours, as scientists expected them to do. What they didn't expect

Toohey, Darin W.

376

CLOUD PHYSICS From aerosol-limited to invigoration  

E-Print Network [OSTI]

CLOUD PHYSICS From aerosol-limited to invigoration of warm convective clouds Ilan Koren,1 * Guy Dagan,1 Orit Altaratz1 Among all cloud-aerosol interactions, the invigoration effect is the most elusive. Most of the studies that do suggest this effect link it to deep convective clouds with a warm base

Napp, Nils

377

Deposition of Biological Aerosols on HVAC Heat Exchangers  

E-Print Network [OSTI]

LBNL-47669 Deposition of Biological Aerosols on HVAC Heat Exchangers Jeffrey Siegel and Iain Walker of Biological Aerosols on HVAC Heat Exchangers Jeffrey A. Siegel Iain S. Walker, Ph.D. ASHRAE Student Member that are found in commercial and residential HVAC systems of 1 - 6 m/s (200 - 1200 ft/min), particle diameters

378

Climatology of aerosol optical depth in northcentral Oklahoma: 19922008  

E-Print Network [OSTI]

of aerosol models; for identification of aerosols from spe- cific events (e.g., the Central American fires Radiation Measurement Program central facility near Lamont, Oklahoma, since the fall of 1992. Most dimming; that is, the decrease in solar radiation reaching Earth's surface. Additionally, the wavelength

379

Absorption cross-section 139 Accumulation mode, of aerosol 146  

E-Print Network [OSTI]

133, 151 residence times 153 size distributions 144 Air composition 2 molecular weight 4, 6 Albedo 122 dioxide Coagulation (aerosol) 146 Column model 32 Conditional unstability 56 Continuity equation 75261 INDEX A Absorption cross-section 139 Accumulation mode, of aerosol 146 Acetaldehyde (CH3CHO

Jacob, Daniel J.

380

Laboratory Measurements of Sea Salt Aerosol Refractive Index  

E-Print Network [OSTI]

. . . . . . . . . . . . . . . . . . . . . . 6 1.2.3 Complex Refractive Index . . . . . . . . . . . . . . . . . . . . 6 1.2.4 Size Distribution . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 13 1.3.5 Coagulation . . . . . . . . . . . . . . . . . . . . . . . . . . . . 14 1.4 Sea Salt AerosolsLaboratory Measurements of Sea Salt Aerosol Refractive Index Thesis submitted for the degree

Oxford, University of

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


381

Cloud Condensation Nuclei (CCN) Analysis of Biogenic Secondary Organic Aerosol  

E-Print Network [OSTI]

Cloud Condensation Nuclei (CCN) Analysis of Biogenic Secondary Organic Aerosol Rachel L. Atlas1' gas-phase emissions and the aerosols they form (figure 6), including a cloud condensation nuclei Cloud condensation nuclei (CCN) are particles which water vapor condenses onto to form cloud droplets

Collins, Gary S.

382

Method of dispersing particulate aerosol tracer  

DOE Patents [OSTI]

A particulate aerosol tracer which comprises a particulate carrier of sheet silicate composition having a particle size up to one micron, and a cationic dopant chemically absorbed in solid solution in the carrier. The carrier is preferably selected from the group consisting of natural mineral clays such as bentonite, and the dopant is selected from the group consisting of rare earth elements and transition elements. The tracers are dispersed by forming an aqueous salt solution with the dopant present as cations, dispersing the carriers in the solution, and then atomizing the solution under heat sufficient to superheat the solution droplets at a level sufficient to prevent reagglomeration of the carrier particles.

O'Holleran, Thomas P. (Belleville, MI)

1988-01-01T23:59:59.000Z

383

Study of Aerosol Indirect Effects in China  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr MayAtmosphericNuclear Security AdministrationcontrollerNanocrystalline Gallium Oxide Thin Films.AdministrationAerosol Indirect

384

Aerosol Remote Sealing System - Energy Innovation Portal  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr MayAtmospheric Optical Depth (AOD)ProductssondeadjustsondeadjustAbout the BuildingInnovation 2011 Simulation StudiesAerosol Remote Sealing

385

Light Absorption by Secondary Organic Aerosol from ?-Pinene: Effects of Oxidants, Seed Aerosol Acidity, and Relative Humidity  

SciTech Connect (OSTI)

It is well known that light absorption from dust and black carbon aerosols has a warming effect on climate while light scattering from sulfate, nitrate, and sea salt aerosols has a cooling effect. However, there are large uncertainties associated with light absorption and scattering by different types of organic aerosols, especially in the near-UV and UV spectral regions. In this paper, we present the results from a systematic laboratory study focused on measuring light absorption by secondary organic aerosols (SOA) generated from ozonolysis or NO3 oxidation of ?-pinene in the presence of neutral and acidic sulfate seed aerosols. Light absorption was monitored using photoacoustic spectrometers at four different wavelengths: 355, 405, 532 and 870 nm. Light absorption at 355 and 405 nm was observed by SOA generated from oxidation of ?-pinene in the presence of acidic sulfate seed aerosols, under dry conditions. No absorption was observed when the relative humidity was elevated to greater than 27%, or in the presence of neutral sulfate seed aerosols. The light-absorbing compounds are speculated to be aldol condensation oligomers with organosulfate and organic nitrate groups. The results of this study also indicate that organic nitrates from ?-pinene SOA formed in the presence of neutral sulfate seed aerosols do not appear to absorb near-UV and UV radiation.

Song, Chen; Gyawali, Madhu S.; Zaveri, Rahul A.; Shilling, John E.; Arnott, W. Patrick

2013-10-25T23:59:59.000Z

386

Globalization of biopharmaceutical manufacturing  

E-Print Network [OSTI]

The biomanufacturing industry is changing due to increasing globalization. However, it is changing differently from other high tech industries like software/ semiconductor/ automobiles. In this study we use global ...

Pande, Rachna

2011-01-01T23:59:59.000Z

387

Nonsingular static global string  

E-Print Network [OSTI]

A new solution for the spacetime outside the core of a U(1) static global string has been presented which is nonsingular. This is the first example of a nonsingular spacetime around a static global string.}}

A. A. Sen; N. Banerjee

2000-04-12T23:59:59.000Z

388

Review: Globalization of Water  

E-Print Network [OSTI]

Review: Globalization of Water: Sharing the PlanetsAshok K. Globalization of Water: Sharing the Planets140) liters of virtual water (p. 15). This is one of the

Tennant, Matthew Aaron

2009-01-01T23:59:59.000Z

389

Global Environmental Course Title  

E-Print Network [OSTI]

Department Global Environmental Studies Room Course Title Frontier of Sustainability Science Instructor Akihisa MORI, Global Environmental Studies Satoshi KONISHI, Institute of Advanced consisting from a variety of academic field, including philosophy, politics, economics, energy, architecture

Takada, Shoji

390

Cows Causing Global Warming  

E-Print Network [OSTI]

Broadcast Transcript: Remember when President Reagan blamed trees for air pollution? Well now the Japanese are blaming cows for global warming. Apparently, the methane emissions from burping cows account for 5% of all global greenhouse gases. Simple...

Hacker, Randi

2008-08-06T23:59:59.000Z

391

ARM: 10-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm  

DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

10-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

Newsom, Rob; Goldsmith, John

392

ARM: 2-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm  

DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

2-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

Sivaraman, Chitra; Flynn, Connor

393

ARM: 10-second Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm  

DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

10-second Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

Sivaraman, Chitra; Flynn, Connor

394

ARM: 1-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm  

DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

1-minute Raman Lidar: aerosol scattering ratio and backscattering coefficient profiles, from first Ferrare algorithm

Sivaraman, Chitra; Flynn, Connor

395

spectra from size-resolved particle samples col-lected from the Southeastern Aerosol Visibility  

E-Print Network [OSTI]

and acrolein aerosols. We believe that these transformations are due to acid-catalyzed heterogeneous reac

Bishop, James K.B.

396

Assessment of the Upper Particle Size Limit for Quantitative Analysis of Aerosols Using  

E-Print Network [OSTI]

the vaporization dynamics of individual aerosol particles, such as thermophoretic forces and vapor expulsion. Since

Hahn, David W.

397

Modeling the Direct and Indirect Effects of Atmospheric Aerosols on Tropical Cyclones  

E-Print Network [OSTI]

are conducted under the three aerosol scenarios: 1) the clean case with an aerosol number concentration of 200 cm-1, 2) the polluted case with a number concentration of 1000 cm-1, and 3) the aerosol radiative effects (AR) case with same aerosol concentration...

Lee, Keun-Hee

2012-02-14T23:59:59.000Z

398

AEROSOLS AND CLIMATE THE SCIENTIFIC BASIS  

E-Print Network [OSTI]

to address two major pollutants that have an impact on warming: black soot and tropospheric ozone. Both are proven health hazards. Reducing both would not only address climate change, but also dramatically improve people's health. " #12;#12;GLOBAL ENERGY BALANCE Global and annual average energy fluxes in watts per

Schwartz, Stephen E.

399

CARES Helps Explain Secondary Organic Aerosols  

SciTech Connect (OSTI)

What happens when urban man-made pollution mixes with what we think of as pristine forest air? To know more about what this interaction means for the climate, the Carbonaceous Aerosol and Radiative Effects Study, or CARES, field campaign was designed in 2010. The sampling strategy during CARES was coordinated with CalNex 2010, another major field campaign that was planned in California in 2010 by the California Air Resources Board (CARB), the National Oceanic and Atmospheric Administration (NOAA), and the California Energy Commission (CEC). "We found two things. When urban pollution mixes with forest pollutions we get more secondary organic aerosols," said Rahul Zaveri, FCSD scientist and project lead on CARES. "SOAs are thought to be formed primarily from forest emissions but only when they interact with urban emissions. The data is saying that there will be climate cooling over the central California valley because of these interactions." Knowledge gained from detailed analyses of data gathered during the CARES campaign, together with laboratory experiments, is being used to improve existing climate models.

Zaveri, Rahul

2014-03-28T23:59:59.000Z

400

CARES Helps Explain Secondary Organic Aerosols  

ScienceCinema (OSTI)

What happens when urban man-made pollution mixes with what we think of as pristine forest air? To know more about what this interaction means for the climate, the Carbonaceous Aerosol and Radiative Effects Study, or CARES, field campaign was designed in 2010. The sampling strategy during CARES was coordinated with CalNex 2010, another major field campaign that was planned in California in 2010 by the California Air Resources Board (CARB), the National Oceanic and Atmospheric Administration (NOAA), and the California Energy Commission (CEC). "We found two things. When urban pollution mixes with forest pollutions we get more secondary organic aerosols," said Rahul Zaveri, FCSD scientist and project lead on CARES. "SOAs are thought to be formed primarily from forest emissions but only when they interact with urban emissions. The data is saying that there will be climate cooling over the central California valley because of these interactions." Knowledge gained from detailed analyses of data gathered during the CARES campaign, together with laboratory experiments, is being used to improve existing climate models.

Zaveri, Rahul

2014-06-02T23:59:59.000Z

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


401

Particle size distribution of indoor aerosol sources  

SciTech Connect (OSTI)

As concern about Indoor Air Quality (IAQ) has grown in recent years, it has become necessary to determine the nature of particles produced by different indoor aerosol sources and the typical concentration that these sources tend to produce. These data are important in predicting the dose of particles to people exposed to these sources and it will also enable us to take effective mitigation procedures. Further, it will also help in designing appropriate air cleaners. A new state of the art technique, DMPS (Differential Mobility Particle Sizer) System is used to determine the particle size distributions of a number of sources. This system employs the electrical mobility characteristics of these particles and is very effective in the 0.01--1.0 {mu}m size range. A modified system that can measure particle sizes in the lower size range down to 3 nm was also used. Experimental results for various aerosol sources is presented in the ensuing chapters. 37 refs., 20 figs., 2 tabs.

Shah, K.B.

1990-10-24T23:59:59.000Z

402

Vapor scavenging by atmospheric aerosol particles  

SciTech Connect (OSTI)

Particle growth due to vapor scavenging was studied using both experimental and computational techniques. Vapor scavenging by particles is an important physical process in the atmosphere because it can result in changes to particle properties (e.g., size, shape, composition, and activity) and, thus, influence atmospheric phenomena in which particles play a role, such as cloud formation and long range transport. The influence of organic vapor on the evolution of a particle mass size distribution was investigated using a modified version of MAEROS (a multicomponent aerosol dynamics code). The modeling study attempted to identify the sources of organic aerosol observed by Novakov and Penner (1993) in a field study in Puerto Rico. Experimentally, vapor scavenging and particle growth were investigated using two techniques. The influence of the presence of organic vapor on the particle`s hydroscopicity was investigated using an electrodynamic balance. The charge on a particle was investigated theoretically and experimentally. A prototype apparatus--the refractive index thermal diffusion chamber (RITDC)--was developed to study multiple particles in the same environment at the same time.

Andrews, E.

1996-05-01T23:59:59.000Z

403

Asthmatic responses to airborne acid aerosols  

SciTech Connect (OSTI)

Controlled exposure studies suggest that asthmatics may be more sensitive to the respiratory effects of acidic aerosols than individuals without asthma. This study investigates whether acidic aerosols and other air pollutants are associated with respiratory symptoms in free-living asthmatics. Daily concentrations of hydrogen ion (H+), nitric acid, fine particulates, sulfates and nitrates were obtained during an intensive air monitoring effort in Denver, Colorado, in the winter of 1987-88. A panel of 207 asthmatics recorded respiratory symptoms, frequency of medication use, and related information in daily diaries. We used a multiple regression time-series model to analyze which air pollutants, if any, were associated with health outcomes reported by study participants. Airborne H+ was found to be significantly associated with several indicators of asthma status, including moderate or severe cough and shortness of breath. Cough was also associated with fine particulates, and shortness of breath with sulfates. Incorporating the participants' time spent outside and exercise intensity into the daily measure of exposure strengthened the association between these pollutants and asthmatic symptoms. Nitric acid and nitrates were not significantly associated with any respiratory symptom analyzed. In this population of asthmatics, several outdoor air pollutants, particularly airborne acidity, were associated with daily respiratory symptoms.

Ostro, B.D.; Lipsett, M.J.; Wiener, M.B.; Selner, J.C. (California Department of Health Services, Berkeley (USA))

1991-06-01T23:59:59.000Z

404

Biological Safety Cabinets n Product protection  

E-Print Network [OSTI]

2.7 #12;Biological Safety Cabinets Purpose n Product protection n Personal protection n Environmental protection 2.7 #12;Biological Safety Cabinets Types A. Class I n inward airflow protects worker n" work area n use for work with aerosol-transmissible micro- organisms n use also for tissue culture

Collins, Gary S.

405

DOE/SC-ARM-TR-142 ARM Aerosol Measurement Science Group Charter  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr May JunDatastreamsmmcrcalgovInstrumentsruc DocumentationP-Series to UserProduct: CrudeOffice ofINL is a U.S. Department of422 ARM Aerosol

406

DOE/SC-ARM/TR-133 Aerosol Optical Depth Value-Added  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr May JunDatastreamsmmcrcalgovInstrumentsruc DocumentationP-Series to UserProduct: CrudeOffice ofINL is a U.S. Department of4223 Aerosol

407

The Radiative Role of Free Tropospheric Aerosols and Marine Clouds over the Central North Atlantic  

SciTech Connect (OSTI)

The scientific scope of the project was to exploit the unique location of the Pico Mountain Observatory (PMO) located in the summit caldera of the Pico Volcano in Pico Island in the Azores, for atmospheric studies. The observatory, located at 2225m a.s.l., typically samples free tropospheric aerosols laying above the marine low-level clouds and long-range transported from North America. The broad purpose of this research was to provide the scientific community with a better understanding of fundamental physical processes governing the effects of aerosols on radiative forcing and climate; with the ultimate goal of improving our abilities to understand past climate and to predict future changes through numerical models. The project was 'exploratory' in nature, with the plan to demonstrate the feasibility of deploying for the first time, an extensive aerosol research package at PMO. One of the primary activities was to test the deployment of these instruments at the site, to collect data during the 2012 summer season, and to further develop the infrastructure and the knowledge for performing novel research at PMO in follow-up longer-term aerosol-cloud studies. In the future, PMO could provide an elevated research outpost to support the renewed DOE effort in the Azores that was intensified in 2013 with the opening of the new sea-level ARM-DOE Eastern North Atlantic permanent facility at Graciosa Island. During the project period, extensive new data sets were collected for the planned 2012 season. Thanks to other synergistic activities and opportunities, data collection was then successfully extended to 2013 and 2014. Highlights of the scientific findings during this project include: a) biomass burning contribute significantly to the aerosol loading in the North Atlantic free troposphere; however, long-range transported black carbon concentrations decreased substantially in the last decade. b) Single black carbon particles analyzed off-line at the electron microscope were often very compacted, suggesting cloud processing and exhibiting different optical properties from fresh emissions. In addition, black carbon was found to be sometimes mixed with mineral dust, affecting its optical properties and potential forcing. c) Some aerosols collected at PMO acted as ice nuclei, potentially contributing to cirrus cloud formation during their transport in the upper free troposphere. Identified good ice nuclei were often mineral dust particles. d) The free tropospheric aerosols studied at PMO have relevance to low level marine clouds due, for example, to synoptic subsidence entraining free tropospheric aerosols into the marine boundary layer. This has potentially large consequences on cloud condensation nuclei concentrations and compositions in the marine boundary layer; therefore, having an effect on the marine stratus clouds, with potentially important repercussions on the radiative forcing. The scientific products of this project currently include contributions to two papers published in the Nature Publishing group (Nature Communications and Scientific Reports), one paper under revision for Atmospheric Chemistry and Physics, one in review in Geophysical Research Letters and one recently submitted to Atmospheric Chemistry and Physics Discussion. In addition, four manuscripts are in advanced state of preparation. Finally, twenty-eight presentations were given at international conferences, workshops and seminars.

Mazzoleni, Claudio [Michigan Technological University; Kumar, Sumit [Michigan Technological University; Wright, Kendra [Michigan Technological University; Kramer, Louisa [Michigan Technological University; Mazzoleni, Lynn [Michigan Technological University; Owen, Robert [Michigan Technological University; Helmig, Detlev [University of Colorado at Boulder

2014-12-09T23:59:59.000Z

408

Predicting and mitigating the global warming potential of agro-ecosystems  

E-Print Network [OSTI]

Predicting and mitigating the global warming potential of agro-ecosystems S. Lehugera 1 , B and methane are the main biogenic greenhouse gases (GHG) con-2 tributing to the global warming potential (GWP to design productive16 agro-ecosystems with low global warming impact.17 Keywords18 Global warming potential

Paris-Sud XI, Université de

409

Aerodynamic size associations of natural radioactivity with ambient aerosols  

SciTech Connect (OSTI)

The aerodynamic size of /sup 214/Pb, /sup 212/Pb, /sup 210/Pb, /sup 7/Be, /sup 32/P, /sup 35/S (as SO/sub 4//sup 2 -/), and stable SO/sub 4//sup 2 -/ was measured using cascade impactors. The activity distribution of /sup 212/Pb and /sup 214/Pb, measured by alpha spectroscopy, was largely associated with aerosols smaller than 0.52 ..mu..m. Based on 46 measurements, the activity median aerodynamic diameter of /sup 212/Pb averaged 0.13 ..mu..m (sigma/sub g/ = 2.97), while /sup 214/Pb averaged 0.16 ..mu..m (sigma/sub g/ = 2.86). The larger median size of /sup 214/Pb was attributed to ..cap alpha..-recoil depletion of smaller aerosols following decay of aerosol-associated /sup 218/Po. Subsequent /sup 214/Pb condensation on all aerosols effectively enriches larger aerosols. /sup 212/Pb does not undergo this recoil-driven redistribution. Low-pressure impactor measurements indicated that the mass median aerodynamic diameter of SO/sub 4//sup 2 -/ was about three times larger than the activity median diameter /sup 212/Pb, reflecting differences in atmospheric residence times as well as the differences in surface area and volume distributions of the atmospheric aerosol. Cosmogenic radionuclides, especially /sup 7/Be, were associated with smaller aerosols than SO/sub 4//sup 2 -/ regardless of season, while /sup 210/Pb distributions in summer measurements were similar to sulfate but smaller in winter measurements. Even considering recoil following /sup 214/Po ..cap alpha..-decay, the avervage /sup 210/Pb labeled aerosol grows by about a factor of two during its atmospheric lifetime. The presence of 5 to 10% of the /sup 7/Be on aerosols greater than 1 ..mu..m was indicative of post-condensation growth, probably either in the upper atmosphere or after mixing into the boundary layer.

Bondietti, E.A.; Papastefanou, C.; Rangarajan, C.

1986-04-01T23:59:59.000Z

410

Criteria pollutant and acid aerosol characterization study, Catano, Puerto Rico  

SciTech Connect (OSTI)

The primary objective of the Catano Criteria Pollutant and Acid Aerosol Characterization Study (CPAACS) was to measure criteria pollutant concentrations and acid aerosol concentrations in and around the Ward of Catano, Puerto Rico, during the summer of 1994. Continuous air sampling for criteria pollutants was performed at three fixed stations and one moobile station that was deployed to four locations. Air samples for acid aerosol analyses and particulate matter measurements were collected at three sites. Semicontinuous sulfate analysis was performed at the primary site. Continuous measurements of wind speed, wind direction, temperature, and relative humidity were also made at each site. The study was conducted from June 1 through September 30, 1994.

Edgerton, E.S.; Harlos, D.P.; Sune, J.M.; Akland, G.G.; Vallero, D.A.

1995-07-01T23:59:59.000Z

411

Design Editorial Globalization and Internationalism  

E-Print Network [OSTI]

; especially, the development of an increasingly integrated global economy marked especially by free tradeJournal of Mechanical Design Editorial Globalization and Internationalism There has always been and Strabo, but to Friedman's empirical observations of globalization. According to Wikipedia, "globalization

Papalambros, Panos

412

Frontiers in Global Change Seminar Series  

E-Print Network [OSTI]

particles ("aerosols") exert a net cooling effect by directly scattering and absorption of solar radiation (or ice crystal) formation; polluted clouds tend to have more droplets than their pristine that aerosol impacts on clouds (known as "aerosol indirect climatic effects") have a net cooling effect

413

Mexico City Aerosol Analysis During Milagro Using High Resolution Aerosol Mass Spectrometry at the Urban Supersite (T0) - Part 1: Fine Particle Composition and Organic Source Apportionment.  

E-Print Network [OSTI]

Submicron aerosol was analyzed during the MILAGRO field campaign in March 2006 at the T0 urban supersite in Mexico City with a High-Resolution Aerosol Mass Spectrometer (AMS) and complementary instrumentation. Positive ...

Aiken, A. C.

414

Sensitivity of aerosol properties to new particle formation mechanism and to primary emissions in a continental-scale chemical  

E-Print Network [OSTI]

of aerosol particles and in turn their number concentration and size distribution. Aerosol particles can grow contribution from coagulation. The aerosol mass concentration, which is primarily in the accumulation mode of aerosol number concentration and size distri- bution is important for considerations of the aerosol

415

Testing for the Possible Influence of Unknown Climate Forcings upon Global Temperature Increases from 1950-2000  

SciTech Connect (OSTI)

Global-scale variations in the climate system over the last half of the twentieth century, including long-term increases in global-mean near-surface temperatures, are consistent with concurrent human-induced emissions of radiatively active gases and aerosols. However, such consistency does not preclude the possible influence of other forcing agents, including internal modes of climate variability or unaccounted for aerosol effects. To test whether other unknown forcing agents may have contributed to multidecadal increases in global-mean near-surface temperatures from 1950 to 2000, data pertaining to observed changes in global-scale sea surface temperatures and observed changes in radiatively active atmospheric constituents are incorporated into numerical global climate models. Results indicate that the radiative forcing needed to produce the observed long-term trends in sea surface temperaturesand global-mean near-surface temperaturesis provided predominantly by known changes in greenhouse gases and aerosols. Further, results indicate that less than 10% of the long-term historical increase in global-mean near-surface temperatures over the last half of the twentieth century could have been the result of internal climate variability. In addition, they indicate that less than 25%of the total radiative forcing needed to produce the observed long-term trend in global-mean near-surface temperatures could have been provided by changes in net radiative forcing from unknown sources (either positive or negative). These results, which are derived from simple energy balance requirements, emphasize the important role humans have played in modifying the global climate over the last half of the twentieth century.

Anderson, Bruce T.; Knight, Jeff R.; Ringer, Mark A.; Yoon, Jin-Ho; Cherchi, Annalisa

2012-10-15T23:59:59.000Z

416

Shale Gas Production: Potential versus Actual GHG Emissions  

E-Print Network [OSTI]

Shale Gas Production: Potential versus Actual GHG Emissions Francis O'Sullivan and Sergey Paltsev, and environmental effects. In turn, the greenhouse gas and atmospheric aerosol assumptions underlying climate://globalchange.mit.edu/ Printed on recycled paper #12;1 Shale Gas Production: Potential versus Actual GHG Emissions Francis O

417

INTERNATIONAL RELATIONS &INTERNATIONAL RELATIONS &INTERNATIONAL RELATIONS & THE GLOBAL ECONOMYTHE GLOBAL ECONOMYTHE GLOBAL ECONOMY  

E-Print Network [OSTI]

GLOBAL ECONOMYTHE GLOBAL ECONOMY This major offers students rigorous interdisciplinary training 331: The Global Economy 2030 -- Examination of key ideas from economics, demography and technology. Guest lecturers illuminate possible conditions of the global economy in 2030. IR 454: International

Krylov, Anna I.

418

27 February 2014 SENT TO LSU AGCENTER/LOUISIANA FOREST PRODUCTS DEVELOPMENT CENTER -FOREST SECTOR / FORESTY PRODUCTS INTEREST GROUP  

E-Print Network [OSTI]

27 February 2014 SENT TO LSU AGCENTER/LOUISIANA FOREST PRODUCTS DEVELOPMENT CENTER - FOREST SECTOR / FORESTY PRODUCTS INTEREST GROUP 1 Smell of forest pine can limit climate change- researchers Matt Mc of atmospheric aerosols on temperatures. Perfumed air These particles form clouds that block sunlight as well

419

Aerosol mass spectrometry systems and methods  

DOE Patents [OSTI]

A system according to one embodiment includes a particle accelerator that directs a succession of polydisperse aerosol particles along a predetermined particle path; multiple tracking lasers for generating beams of light across the particle path; an optical detector positioned adjacent the particle path for detecting impingement of the beams of light on individual particles; a desorption laser for generating a beam of desorbing light across the particle path about coaxial with a beam of light produced by one of the tracking lasers; and a controller, responsive to detection of a signal produced by the optical detector, that controls the desorption laser to generate the beam of desorbing light. Additional systems and methods are also disclosed.

Fergenson, David P.; Gard, Eric E.

2013-08-20T23:59:59.000Z

420

Soot particle aerosol dynamics at high pressure  

SciTech Connect (OSTI)

The authors have used detailed calculations to analyze the coagulation dynamics of a soot aerosol at high pressures (20 and 50 atm). They find that the soot size distribution is altered compared to lower-pressure conditions because the mean free path at high pressures is reduced to the point that the particles are similar in size to the mean free path. At lower pressures the form of the size distribution becomes constant (self-preserving) in time, allowing optical measurements to be easily interpreted. However, the authors find that at pressures above about 5 atm the shape of the size distribution continually changes. As a result, proper and accurate interpretation of optical data at high pressures is more difficult than at lower pressures.

Harris, S.J. (General Motors Research Labs., Warren, MI (USA). Physics Dept.); Kennedy, I.M. (California Univ., Davis, CA (USA). Dept. of Mechanical Engineering)

1989-12-01T23:59:59.000Z

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


421

Diesel Aerosol Sampling in the Atmosphere  

SciTech Connect (OSTI)

The University of Minnesota Center for Diesel Research along with a research team including Caterpillar, Cummins, Carnegie Mellon University, West Virginia University (WVU), Paul Scherrer Institute in Switzerland, and Tampere University in Finland have performed measurements of Diesel exhaust particle size distributions under real-world dilution conditions. A mobile aerosol emission laboratory (MEL) equipped to measure particle size distributions, number concentrations, surface area concentrations, particle bound PAHs, as well as CO 2 and NO x concentrations in real time was built and will be described. The MEL was used to follow two different Cummins powered tractors, one with an older engine (L10) and one with a state-of-the-art engine (ISM), on rural highways and measure particles in their exhaust plumes. This paper will describe the goals and objectives of the study and will describe representative particle size distributions observed in roadway experiments with the truck powered by the ISM engine.

David Kittelson; Jason Johnson; Winthrop Watts; Qiang Wei; Marcus Drayton; Dwane Paulsen; Nicolas Bukowiecki

2000-06-19T23:59:59.000Z

422

aerosol content monitoring: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Rings, Jrg 2008-01-01 6 The impact of aerosols on simulated ocean temperature and heat content in the 20th century Environmental Sciences and Ecology Websites Summary: The...

423

Effects of aerosols on deep convective cumulus clouds  

E-Print Network [OSTI]

This work investigates the effects of anthropogenic aerosols on deep convective clouds and the associated radiative forcing in the Houston area. The Goddard Cumulus Ensemble model (GCE) coupled with a spectral-bin microphysics is employed...

Fan, Jiwen

2009-05-15T23:59:59.000Z

424

Continuous air monitor for alpha-emitting aerosol particles  

SciTech Connect (OSTI)

A new alpha Continuous Air Monitor (CAM) sampler is being developed for use in detecting the presence of alpha-emitting aerosol particles. The effort involves design, fabrication and evaluation of systems for the collection of aerosol and for the processing of data to speciate and quantify the alpha emitters of interest. At the present time we have a prototype of the aerosol sampling system and we have performed wind tunnel tests to characterize the performance of the device for different particle sizes, wind speeds, flow rates and internal design parameters. The results presented herein deal with the aerosol sampling aspects of the new CAM sampler. Work on the data processing, display and alarm functions is being done in parallel with the particle sampling work and will be reported separately at a later date. 17 refs., 5 figs., 3 tabs.

McFarland, A.R.; Ortiz, C.A. (Texas A and M Univ., College Station, TX (USA). Dept. of Mechanical Engineering); Rodgers, J.C.; Nelson, D.C. (Los Alamos National Lab., NM (USA))

1990-01-01T23:59:59.000Z

425

Pressure-flow reducer for aerosol focusing devices  

DOE Patents [OSTI]

A pressure-flow reducer, and an aerosol focusing system incorporating such a pressure-flow reducer, for performing high-flow, atmosphere-pressure sampling while delivering a tightly focused particle beam in vacuum via an aerodynamic focusing lens stack. The pressure-flow reducer has an inlet nozzle for adjusting the sampling flow rate, a pressure-flow reduction region with a skimmer and pumping ports for reducing the pressure and flow to enable interfacing with low pressure, low flow aerosol focusing devices, and a relaxation chamber for slowing or stopping aerosol particles. In this manner, the pressure-flow reducer decouples pressure from flow, and enables aerosol sampling at atmospheric pressure and at rates greater than 1 liter per minute.

Gard, Eric (San Francisco, CA); Riot, Vincent (Oakland, CA); Coffee, Keith (Diablo Grande, CA); Woods, Bruce (Livermore, CA); Tobias, Herbert (Kensington, CA); Birch, Jim (Albany, CA); Weisgraber, Todd (Brentwood, CA)

2008-04-22T23:59:59.000Z

426

MELCOR 1. 8. 1 assessment: LACE aerosol experiment LA4  

SciTech Connect (OSTI)

The MELCOR code has been used to simulate LACE aerosol experiment LA4. In this test, the behavior of single- and double-component, hygroscopic and nonhygroscopic, aerosols in a condensing environment was monitored. Results are compared to experimental data, and to CONTAIN calculations. Sensitivity studies have been done on time step effects and machine dependencies; thermal/hydraulic parameters such as condensation on heat structures and on pool surface, and radiation heat transfer; and aerosol parameters such as number of MAEROS components and sections assumed, the degree to which plated aerosols are washed off heat structures by condensate film draining, and the effect of non-default values for shape factors and diameter limits. 9 refs., 50 figs., 13 tabs.

Kmetyk, L.N.

1991-09-01T23:59:59.000Z

427

Distinguishing Aerosol Impacts on Climate Over the Past Century  

E-Print Network [OSTI]

Figure 8a). The IE cooling increases snow/ice by about 10% (Their cooling e?ect on surface temperatures promotes ice androw), cooling from the aerosol DE increases snow/ice cover

Koch, Dorothy

2009-01-01T23:59:59.000Z

428

aerosol source apportionment: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

was analyzed during the MILAGRO field campaign in March 2006 at the T0 urban supersite in Mexico City with a High-Resolution Aerosol Mass Spectrometer (AMS) and complementary...

429

aerosolized bacillus anthracis: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

and remotely sensed aerosol observations. William D. Collins; Phillip J. Rasch; Brian E. Eaton; Boris V. Khattatov; Jean-francois Lamarque; C. Zender 2001-01-01 118 THESE DE...

430

Aerosol-Cloud interactions : a new perspective in precipitation enhancement  

E-Print Network [OSTI]

Increased industrialization and human activity modified the atmospheric aerosol composition and size-distribution during the last several decades. This has affected the structure and evolution of clouds, and precipitation ...

Gunturu, Udaya Bhaskar

2010-01-01T23:59:59.000Z

431

MICS Asia Phase II - Sensitivity to the aerosol module  

E-Print Network [OSTI]

In the framework of the model inter-comparison study - Asia Phase II (MICS2), where eight models are compared over East Asia, this paper studies the influence of different parameterizations used in the aerosol module on the aerosol concentrations of sulfate and nitrate in PM10. An intracomparison of aerosol concentrations is done for March 2001 using different configurations of the aerosol module of one of the model used for the intercomparison. Single modifications of a reference setup for model configurations are performed and compared to a reference case. These modifications concern the size distribution, i.e. the number of sections, and physical processes, i.e. coagulation, condensation/evaporation, cloud chemistry, heterogeneous reactions and sea-salt emissions. Comparing monthly averaged concentrations at different stations, the importance of each parameterization is first assessed. It is found that sulfate concentrations are little sensitive to sea-salt emissions and to whether condensation is computed...

Sartelet, Karine; Sportisse, Bruno

2007-01-01T23:59:59.000Z

432

aerosol optical depths: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AERONET, AVHRR and 3 MODIS 4 A. Hauser, D. Oesch have been used to 9 retrieve the spatial distribution of aerosol optical depth for 10 central Europe. At eight AERONET sites,...

433

aerosol optical depth: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AERONET, AVHRR and 3 MODIS 4 A. Hauser, D. Oesch have been used to 9 retrieve the spatial distribution of aerosol optical depth for 10 central Europe. At eight AERONET sites,...

434

aerosol strong acidity: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

nucleation theories. Citation: Erupe, M. E., et al Lee, Shan-Hu 12 Neutralization of soil aerosol and its impact on the distribution of acid rain over east Asia Geosciences...

435

Thermophoresis and Its Thermal Parameters for Aerosol Collection  

E-Print Network [OSTI]

K/cm (a) Figure 3. (a). Thermophoretic collection ratio vs.Lin, J. , et al. , Thermophoretic deposition of particles inof a plate- to-plate thermophoretic precipitator, Aerosol

Huang, Z.

2008-01-01T23:59:59.000Z

436

aerosol particle deposition: Topics by E-print Network  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

aerosol particles as an alternative way to determine the electron mean free path of low energy electrons in solid and liquid materials. The mean free path is obtained from fits...

437

An investigation of aerosol physical properties in Houston, Texas  

E-Print Network [OSTI]

From June through October 2001, three Tandem Differential Mobility Analyzer (TDMA) systems were operated around Houston, Texas, to obtain a large, high-quality dataset in order to explore characteristics of aerosol size distributions...

Gasparini, Roberto

2002-01-01T23:59:59.000Z

438

Computational Fluid Dynamics Study of Aerosol Transport and Deposition Mechanisms  

E-Print Network [OSTI]

In this work, various aerosol particle transport and deposition mechanisms were studied through the computational fluid dynamics (CFD) modeling, including inertial impaction, gravitational effect, lift force, interception, and turbophoresis, within...

Tang, Yingjie

2012-07-16T23:59:59.000Z

439

Modeling kinetic partitioning of secondary organic aerosol and size distribution dynamics: representing effects of volatility, phase state, and particle-phase reaction  

SciTech Connect (OSTI)

Evidence is mounting that the majority of the climatically active aerosols are produced through the growth of smaller particles via secondary organic aerosol (SOA) formation from gas-to-particle conversion of anthropogenic and biogenic volatile organic compounds (VOCs). The timescale of SOA partitioning and the associated size distribution dynamics are expected to depend on the gas-phase oxidation of the precursor VOCs and their products, volatility of these organic solutes, composition and phase state of the pre-existing particles, and diffusivity and reactivity of the solute within the particle phase. This paper describes a new framework for modeling kinetic gas-particle partitioning of SOA, with an analytical treatment for the diffusion-reaction process within the particle phase. The formulation is amenable for eventual use in regional and global climate models, although it currently awaits implementation of the actual particle-phase reactions that are important for SOA formation. In the present work, the model is applied to investigate the competitive growth dynamics of the Aitken and accumulation mode particles while the Kelvin effect and coagulation are neglected for simplicity. The timescale of SOA partitioning and evolution of number and composition size distributions are evaluated for a range of solute volatilities (C*), particle-phase bulk diffusivities (Db), and particle-phase reactivity, as exemplified by a pseudo-first-order rate constant (kc). Results show that irreversible condensation of non-volatile organic vapors (equivalent to ) produces significant narrowing of the size distribution. At the other extreme, non-reactive partitioning of semi-volatile organic vapors is volume-controlled in which the final (equilibrium) size distribution simply shifts to the right on the diameter axis while its shape remains unchanged. However, appreciable narrowing of the size distribution may occur when the pre-existing particles are highly viscous semi-solids such that small particles reach quasi-equilibrium much faster than the large ones. In the case of reactive partitioning (finite ), the size distribution experiences permanent narrowing, which is especially pronounced for Db < 10-13 cm2 s-1 and kc > 0.01 s-1. As a result, both number and composition size distributions are needed to effectively constrain and evaluate the next generation of SOA models that treat phase state thermodynamics, particle-phase diffusion and particle-phase chemical reactions.

Zaveri, Rahul A.; Easter, Richard C.; Shilling, John E.; Seinfeld, J. H.

2014-05-27T23:59:59.000Z

440

Engineering the global ecosystem  

E-Print Network [OSTI]

of humans deliberately engineering agricultural landscapes.010-0302-8 EDITORIAL Engineering the global ecosystemtale about human explorers engineering the ecosystem of Mars

Stringfellow, William T.; Jain, Ravi

2010-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


441

Global Nuclear Security  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Global Nuclear Security Both DOE and the National Nuclear Security Administration are working to reduce the risk of nuclear proliferation and provide technologies to improve...

442

Subsidizing Global Solar Power.  

E-Print Network [OSTI]

?? With national cuts on solar PV subsidies and the current oversupply of panels, the global solar market is clearly threatened by a contraction. Yet, (more)

Arnesson, Daniel

2013-01-01T23:59:59.000Z

443

Balloon-borne photometric studies of the stratospheric aerosol layer after Mt. Pinatubo eruption  

SciTech Connect (OSTI)

Using Sun-tracking photometers on board balloons, the Pinatubo volcanic aerosol layer has been studied over Hyderabad (17.5 deg N) during October 1991 and April 1992. From the angular distribution of the scattered radiation intensity measurements the aerosol size parameters is derived. Over a decade of aerosol measurements at Hyderabad, aerosol extinction and number density obtained during October 1991 in the stratosphere are found to be the highest ever obtained with a distinct aerosol layer between 16 and 30 km. The derived aerosol size parameter shows layered structures. Analysis of the size parameter obtained during April 1992 indicates formation of aerosols at higher altitudes by coagulation with a subsequent reduction in the aerosol number density. The obtained results are found to agree well with that of an independent lidar measurement made over Ahmedabad (23 deg N) and with the stratospheric aerosol and gas experiment II (SAGE II) results.

Ramachandran, S.; Jayaraman, A.; Acharya, Y.B.; Subbaraya, B.H. [Physical Research Laboratory, Ahmedabad (India)

1994-08-01T23:59:59.000Z

444

Representing Cloud Processing of Aerosol in Numerical Models  

SciTech Connect (OSTI)

The satellite imagery in Figure 1 provides dramatic examples of how aerosol influences the cloud field. Aerosol from ship exhaust can serve as nucleation centers in otherwise cloud-free regions, forming ship tracks (top image), or can enhance the reflectance/albedo in already cloudy regions. This image is a demonstration of the first indirect effect, in which changes in aerosol modulate cloud droplet radius and concentration, which influences albedo. It is thought that, through the effects it has on precipitation (drizzle), aerosol can also affect the structure and persistence of planetary boundary layer (PBL) clouds. Regions of cellular convection, or open pockets of cloudiness (bottom image) are thought to be remnants of strongly drizzling PBL clouds. Pockets of Open Cloudiness (POCs) (Stevens et al. 2005) or Albrecht's ''rifts'' are low cloud fraction regions characterized by anomalously low aerosol concentrations, implying they result from precipitation. These features may in fact be a demonstration of the second indirect effect. To accurately represent these clouds in numerical models, we have to treat the coupled cloud-aerosol system. We present the following series of mesoscale and large eddy simulation (LES) experiments to evaluate the important aspects of treating the coupled cloud-aerosol problem. 1. Drizzling and nondrizzling simulations demonstrate the effect of drizzle on a mesoscale forecast off the California coast. 2. LES experiments with explicit (bin) microphysics gauge the relative importance of the shape of the aerosol spectrum on the 3D dynamics and cloud structure. 3. Idealized mesoscale model simulations evaluate the relative roles of various processes, sources, and sinks.

Mechem, D.B.; Kogan, Y.L.

2005-03-18T23:59:59.000Z

445

Simulation of aerosol dynamics: a comparative review of mathematical models  

SciTech Connect (OSTI)

Three modeling approaches used are based-continuous, discrete (sectional), and parameterized representations of the aerosol size distribution. Simulations of coagulation and condensation are performed with the three models for clear, hazy, and urban atmospheric conditions. Relative accuracies and computational costs are compared. Reference for the comparison is the continuous approach. The results of the study provide useful information for the selection of an aerosol model, depending on the accuracy requirements and computational constraints associated with a specific application.

Seigneur, C.; Hudischewskyj, A.B.; Seinfeld, J.H.; Whitby, K.T.; Whitby, E.R.

1986-01-01T23:59:59.000Z

446

Cloud Scavenging Effects on Aerosol Radiative and Cloud-nucleating Properties - Final Technical Report  

SciTech Connect (OSTI)

The optical properties of aerosol particles are the controlling factors in determining direct aerosol radiative forcing. These optical properties depend on the chemical composition and size distribution of the aerosol particles, which can change due to various processes during the particles lifetime in the atmosphere. Over the course of this project we have studied how cloud processing of atmospheric aerosol changes the aerosol optical properties. A counterflow virtual impactor was used to separate cloud drops from interstitial aerosol and parallel aerosol systems were used to measure the optical properties of the interstitial and cloud-scavenged aerosol. Specifically, aerosol light scattering, back-scattering and absorption were measured and used to derive radiatively significant parameters such as aerosol single scattering albedo and backscatter fraction for cloud-scavenged and interstitial aerosol. This data allows us to demonstrate that the radiative properties of cloud-processed aerosol can be quite different than pre-cloud aerosol. These differences can be used to improve the parameterization of aerosol forcing in climate models.

Ogren, John A.; Sheridan, Patrick S.; Andrews, Elisabeth

2009-03-05T23:59:59.000Z

447

Cloud-Driven Changes in Aerosol Optical Properties - Final Technical Report  

SciTech Connect (OSTI)

The optical properties of aerosol particles are the controlling factors in determining direct aerosol radiative forcing. These optical properties depend on the chemical composition and size distribution of the aerosol particles, which can change due to various processes during the particles lifetime in the atmosphere. Over the course of this project we have studied how cloud processing of atmospheric aerosol changes the aerosol optical properties. A counterflow virtual impactor was used to separate cloud drops from interstitial aerosol and parallel aerosol systems were used to measure the optical properties of the interstitial and cloud-scavenged aerosol. Specifically, aerosol light scattering, back-scattering and absorption were measured and used to derive radiatively significant parameters such as aerosol single scattering albedo and backscatter fraction for cloud-scavenged and interstitial aerosol. This data allows us to demonstrate that the radiative properties of cloud-processed aerosol can be quite different than pre-cloud aerosol. These differences can be used to improve the parameterization of aerosol forcing in climate models.

Ogren, John A.; Sheridan, Patrick S.; Andrews, Elisabeth

2007-09-30T23:59:59.000Z

448

Evaluation of the carbon content of aerosols from the burn- ing of biomass in the Brazilian Amazon using thermal, op- tical and thermal-optical analysis methods  

SciTech Connect (OSTI)

Aerosol samples were collected at a pasture site in the Amazon Basin as part of the project LBA-SMOCC-2002 (Large-Scale Biosphere-Atmosphere Experiment in Amazonia - Smoke Aerosols, Clouds, Rainfall and Climate: Aerosols from Biomass Burning Perturb Global and Regional Climate). Sampling was conducted during the late dry season, when the aerosol composition was dominated by biomass burning emissions, especially in the submicron fraction. A 13-stage Dekati low-pressure impactor (DLPI) was used to collect particles with nominal aerodynamic diameters (D{sub p}) ranging from 0.03 to 0.10 m. Gravimetric analyses of the DLPI substrates and filters were performed to obtain aerosol mass concentrations. The concentrations of total, apparent elemental, and organic carbon (TC, EC{sub a}, and OC) were determined using thermal and thermal-optical analysis (TOA) methods. A light transmission method (LTM) was used to determine the concentration of equivalent black carbon (BC{sub e}) or the absorbing fraction at 880 nm for the size-resolved samples. During the dry period, due to the pervasive presence of fires in the region upwind of the sampling site, concentrations of fine aerosols (D{sub p} < 2.5 {mu}m: average 59.8 {mu}g m{sup -3}) were higher than coarse aerosols (D{sub p} > 2.5 {mu}m: 4.1 {mu}g m{sup -3}). Carbonaceous matter, estimated as the sum of the particulate organic matter (i.e., OC x 1.8) plus BC{sub e}, comprised more than 90% to the total aerosol mass. Concentrations of EC{sub a} (estimated by thermal analysis with a correction for charring) and BCe (estimated by LTM) averaged 5.2 {+-} 1.3 and 3.1 {+-} 0.8 {mu}g m{sup -3}, respectively. The determination of EC was improved by extracting water-soluble organic material from the samples, which reduced the average light absorption {angstrom} exponent of particles in the size range of 0.1 to 1.0 {mu}m from > 2.0 to approximately 1.2. The size-resolved BC{sub e} measured by the LTM showed a clear maximum between 0.4 and 0.6 m in diameter. The concentrations of OC and BC{sub e} varied diurnally during the dry period, and this variation is related to diurnal changes in boundary layer thickness and in fire frequency.

Soto-Garcia, Lydia L.; Andreae, Meinrat O.; Andreae, Tracey W.; taxo, Paulo Ar-; Maenhaut, Willy; Kirchstetter, Thomas; Novakov, T.; Chow, Judith C.; Mayol-Bracero, Olga L.

2011-06-03T23:59:59.000Z

449

TOWARDS AN IMPROVED HIGH RESOLUTION GLOBAL LONG-TERM SOLAR RESOURCE DATABASE  

E-Print Network [OSTI]

TOWARDS AN IMPROVED HIGH RESOLUTION GLOBAL LONG- TERM SOLAR RESOURCE DATABASE Paul W. Stackhouse and test an improved production system that will enable the longest-term global solar resource database

Perez, Richard R.

450

The modeling of aerosol dynamics during degraded core events  

SciTech Connect (OSTI)

There is substantial interest in developing simple, yet accurate, models for the prediction of aerosol dynamics during degraded core events. The exact aerosol transport equation is given by {partial derivative}n(v,t)/{partial derivative}t = 1/2 {integral}{sub 0}{sup {infinity}} K(u,v {minus} u)n(u,t)n(v {minus} u,t)du {minus} {integral}{sub 0}{sup {infinity}} K(u,v)n(v,t)n(u,t)du {minus} n(v,t)c(v)/h + n{sub p}(v), where n(v,t) is the particle size density distribution function. The kernel, K(v,u), is related to the frequency of coagulation between aerosol particles of volume u and v, and the quantity c(v) is the deposition velocity. The quantity h is the effective height for deposition of aerosol; it is the volume of the aerosol cloud divided by the projected horizontal area A. Finally, the term n{sub p} (v) is the source rate of aerosol. Evaluation of the above equation is discussed.

Clausse, A.; Lahey, R.T. Jr.

1989-01-01T23:59:59.000Z

451

Investigations of cloud altering effects of atmospheric aerosols using a new mixed Eulerian-Lagrangian aerosol model  

E-Print Network [OSTI]

Industry, urban development, and other anthropogenic influences have substantially altered the composition and size-distribution of atmospheric aerosol particles over the last century. This, in turn, has altered cloud ...

Steele, Henry Donnan, 1974-

2004-01-01T23:59:59.000Z

452

UC Irvine's Earth System Science Department has opportunities for postdocs and grad. students interested in global-scale cryospheric modeling. Our projects  

E-Print Network [OSTI]

interested in global-scale cryospheric modeling. Our projects (http://www.ess.uci.edu/~zender#ans and http://www.ess among the groups of Professors Charlie Zender (Aerosols, Radiation, http://www.ess.uci.edu/~zender), Jay Famiglietti (Hydrology, http://www.ess.uci.edu/~famiglietti), and Jim Randerson (Fire, C, H2O, http://www.ess

Zender, Charles

453

Real-time characterization of particle-bound polycyclic aromatic hydrocarbons in ambient aerosols and from motor-vehicle exhaust  

E-Print Network [OSTI]

Response of the Photo-Electric Aerosol Sensor (PAS) to2008 Abstract. A photo-electric aerosol sensor, a diffusionthe measured photo-electric aerosol sensor signal (fA) was

Polidori, A.; Hu, S.; Biswas, S.; Delfino, R. J; Sioutas, C.

2008-01-01T23:59:59.000Z

454

Ganges Valley Aerosol Experiment: Science and Operations Plan  

SciTech Connect (OSTI)

The Ganges Valley region is one of the largest and most rapidly developing sections of the Indian subcontinent. The Ganges River, which provides the region with water needed for sustaining life, is fed primarily by snow and rainfall associated with Indian summer monsoons. Impacts of changes in precipitation patterns, temperature, and the flow of the snow-fed rivers can be immense. Recent satellite-based measurements have indicated that the upper Ganges Valley has some of the highest persistently observed aerosol optical depth values. The aerosol layer covers a vast region, extending across the Indo-Gangetic Plain to the Bay of Bengal during the winter and early spring of each year. The persistent winter fog in the region is already a cause of much concern, and several studies have been proposed to understand the economic, scientific, and societal dimensions of this problem. During the INDian Ocean EXperiment (INDOEX) field studies, aerosols from this region were shown to affect cloud formation and monsoon activity over the Indian Ocean. This is one of the few regions showing a trend toward increasing surface dimming and enhanced mid-tropospheric warming. Increasing air pollution over this region could modify the radiative balance through direct, indirect, and semi-indirect effects associated with aerosols. The consequences of aerosols and associated pollution for surface insolation over the Ganges Valley and monsoons, in particular, are not well understood. The proposed field study is designed for use of (1) the ARM Mobile Facility (AMF) to measure relevant radiative, cloud, convection, and aerosol optical characteristics over mainland India during an extended period of 912 months and (2) the G-1 aircraft and surface sites to measure relevant aerosol chemical, physical, and optical characteristics in the Ganges Valley during a period of 612 weeks. The aerosols in this region have complex sources, including burning of coal, biomass, and biofuels; automobile emissions; and dust. The extended AMF deployment will enable measurements under different regimes of the climate and aerosol abundancein the wet monsoon period with low aerosol loading; in the dry, hot summer with aerosols dispersed throughout the atmospheric column; and in the cool, dry winter with aerosols confined mostly to the boundary later and mid-troposphere. Each regime, in addition, has its own distinct radiative and atmospheric dynamic drivers. The aircraft operational phase will assist in characterizing the aerosols at times when they have been observed to be at the highest concentrations. A number of agencies in India will collaborate with the proposed field study and provide support in terms of planning, aircraft measurements, and surface sites. The high concentration of aerosols in the upper Ganges Valley, together with hypotheses involving several possible mechanisms with direct impacts on the hydrologic cycle of the region, gives us a unique opportunity to generate data sets that will be useful both in understanding the processes at work and in providing answers regarding the effects of aerosols on climate in a region where the perturbation is the highest.

Kotamarthi, VR

2010-06-21T23:59:59.000Z

455

GLOBAL LUMBER/SAWNWOOD COST BENCHMARKING REPORT  

E-Print Network [OSTI]

& Trends 3.2 Global Log Harvest Outlook 3.2.1 Log Price Outlook 3.3 Plantation Pine Log Harvest Outlook 3, FEATURING: Industry Overviews by Country Historical Timber Harvest and Lumber Production Historical Lumber/Log Exports (and By Destination) Manufacturing and Log Costs/Prices for Selected Countries SAWN WOOD

456

CHILLING CONSIDERATIONS GLOBAL WARMING  

E-Print Network [OSTI]

(millionsofsquarekilometers) 30 20 10 MELTING OF GREENLAND ICE CAP Satellite determination of maximum extent of glacial melt Complete melt of the Greenland ice sheet would raise the level of the global ocean 23 feet. ASAN Steffen IS INCREASING Global carbon dioxide concentration over the last thousand years Polar ice cores #12;Mann et al

Schwartz, Stephen E.

457

Global Change Sustainability  

E-Print Network [OSTI]

Global Change and Sustainability Center The GCSC is an inclusionary and interdisciplinary hub that promotes, coordinates, and conducts local to global environmental- and sustainability-related research to complex environmental and sustainability issues and challenges. 2012 Annual Report #12;1GCSC 2012 ANNUAL

Tipple, Brett

458

Global distribution of solid and aqueous sulfate aerosols: Effect of the hysteresis of particle phase transitions  

E-Print Network [OSTI]

of dimethylsulfide from the ocean biosphere. The timescale of phase transitions, as driven by changes in relative radiation back to space less effectively [Ramaswamy et al., 2001; Martin et al., 2004; Wang and Martin, 2007

459

Global impact of smoke aerosols from landscape fires on climate and the Hadley circulation  

E-Print Network [OSTI]

smoke clouds associated with peat and deforestation fires inforest, agricultural, and peat fires (1997 2009), Atmos.of carbon released from peat and forest fires in Indonesia

Tosca, M. G; Randerson, J. T; Zender, C. S

2013-01-01T23:59:59.000Z

460

GLOBAL BIOGEOCHEMICAL CYCLES, VOL. ???, XXXX, DOI:10.1029/, Estimating mineral aerosol iron and aluminum1  

E-Print Network [OSTI]

and aluminum1 solubility from particle size using diffusion-controlled2 and surface [Jickells et al., 2005].34 Aluminum, on the other hand, is not found to be an important nutrient chemistry compared to Fe, aluminum has been used as a39 tracer for quantifying the dust deposition

Zender, Charles

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


461

Urban-scale impacts on the global-scale composition and climate effects of anthropogenic aerosols  

E-Print Network [OSTI]

A reduced form meta model has been produced to simulate the effects of physical, chemical, and meteorological processing of highly reactive trace species in hypothetical urban areas, which is capable of efficiently simulating ...

Cohen, Jason Blake

2010-01-01T23:59:59.000Z

462

Posters Cloud Parameterizations in Global Climate Models: The Role of Aerosols  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr MayAtmosphericNuclear Security Administration the1 - September 2006PhotovoltaicSeptember 22, 2014SocietyJ. Dudhia51 Posters A594173

463

International conference on the role of the polar regions in global change: Proceedings. Volume 2  

SciTech Connect (OSTI)

The International Conference on the Role of the Polar Regions in Global Change took place on the campus of the University of Alaska Fairbanks on June 11--15, 1990. The goal of the conference was to define and summarize the state of knowledge on the role of the polar regions in global change, and to identify gaps in knowledge. To this purpose experts in a wide variety of relevant disciplines were invited to present papers and hold panel discussions. While there are numerous conferences on global change, this conference dealt specifically with the polar regions which occupy key positions in the global system. These two volumes of conference proceedings include papers on (1) detection and monitoring of change; (2) climate variability and climate forcing; (3) ocean, sea ice, and atmosphere interactions and processes; and (4) effects on biota and biological feedbacks; (5) ice sheet, glacier and permafrost responses and feedbacks, (6) paleoenvironmental studies; and, (7) aerosol and trace gases.

Weller, G.; Wilson, C.L.; Severin, B.A.B. [eds.

1991-12-01T23:59:59.000Z

464

International conference on the role of the polar regions in global change: Proceedings. Volume 1  

SciTech Connect (OSTI)

The International Conference on the Role of the Polar Regions in Global Change took place on the campus of the University of Alaska Fairbanks on June 11--15, 1990. The goal of the conference was to define and summarize the state of knowledge on the role of the polar regions in global change, and to identify gaps in knowledge. To this purpose experts in a wide variety of relevant disciplines were invited to present papers and hold panel discussions. While there are numerous conferences on global change, this conference dealt specifically with polar regions which occupy key positions in the global system. These two volumes of conference proceedings include papers on (1) detection and monitoring of change; (2) climate variability and climate forcing; (3) ocean, sea ice, and atmosphere interactions and processes; (4) effects on biota and biological feedbacks; (5) ice sheet, glacier and permafrost responses and feedbacks; (6) paleoenvironmental studies; and, (7) aerosols and trace gases.

Weller, G.; Wilson, C.L.; Severin, B.A.B. [eds.

1991-12-01T23:59:59.000Z

465

Simulating land use change in China from a global perspective  

E-Print Network [OSTI]

and consequent crop production with prescribed population, GDP and yield data. The model simulates a decline markets and turbulence in global energy markets can affect food prices and supply costs. Therefore% of the global population with less than 9% of the world's cultivated land (Chen 2007). Furthermore, heavy

Palmer, Paul

466

Scale-free Universal Spectrum for Atmospheric Aerosol Size Distribution for Davos, Mauna Loa and Izana  

E-Print Network [OSTI]

Atmospheric flows exhibit fractal fluctuations and inverse power law form for power spectra indicating an eddy continuum structure for the selfsimilar fluctuations. A general systems theory for fractal fluctuations developed by the author is based on the simple visualisation that large eddies form by space-time integration of enclosed turbulent eddies, a concept analogous to Kinetic Theory of Gases in Classical Statistical Physics. The ordered growth of atmospheric eddy continuum is in dynamical equilibrium and is associated with Maximum Entropy Production. The model predicts universal (scale-free) inverse power law form for fractal fluctuations expressed in terms of the golden mean. Atmospheric particulates are held in suspension in the fractal fluctuations of vertical wind velocity. The mass or radius (size) distribution for homogeneous suspended atmospheric particulates is expressed as a universal scale-independent function of the golden mean, the total number concentration and the mean volume radius. Model predicted spectrum is in agreement (within two standard deviations on either side of the mean) with total averaged radius size spectra for the AERONET (aerosol inversions) stations Davos and Mauna Loa for the year 2010 and Izana for the year 2009 daily averages. The general systems theory model for aerosol size distribution is scale free and is derived directly from atmospheric eddy dynamical concepts. At present empirical models such as the log normal distribution with arbitrary constants for the size distribution of atmospheric suspended particulates are used for quantitative estimation of earth-atmosphere radiation budget related to climate warming/cooling trends. The universal aerosol size spectrum will have applications in computations of radiation balance of earth-atmosphere system in climate models.

A. M. Selvam

2014-08-14T23:59:59.000Z

467

Photolytic processing of secondary organic aerosols dissolved in cloud droplets  

SciTech Connect (OSTI)

The effect of UV irradiation on the molecular composition of aqueous extracts of secondary organic aerosol (SOA) was investigated. SOA was prepared by the dark reaction of ozone and d-limonene at 0.05 - 1 ppm precursor concentrations and collected with a particle-into-liquid sampler (PILS). The PILS extracts were photolyzed by 300 - 400 nm radiation for up to 24 hours. Water-soluble SOA constituents were analyzed using high-resolution electrospray ionization mass spectrometry (HR-ESI-MS) at different stages of photolysis for all SOA precursor concentrations. Exposure to UV radiation increased the average O/C ratio and decreased the average double bond equivalent (DBE) of the dissolved SOA compounds. Oligomeric compounds were significantly reduced by photolysis relative to the monomeric compounds. Direct pH measurements showed that compounds containing carboxylic acids increased upon photolysis. Methanol reactivity analysis revealed significant photodissociation of molecules containing carbonyl groups and formation of carboxylic acids. Aldehydes, such as limononaldehyde, were almost completely removed. The removal of carbonylswas confirmed by the UV-Vis absorption spectroscopy of the SOA extracts where the absorbance in the carbonyl n??* band decreased significantly upon photolysis. The effective quantum yield (the number of carbonyls destroyed per photon absorbed) was estimated as ~ 0.03. The concentration of peroxides did not change significantly during photolysis as quantified with an iodometric test. Although organic peroxides were photolyzed, the likely end products of photolysis were smaller peroxides, including hydrogen peroxide, resulting in a no net change in the peroxide content.

Bateman, Adam P.; Nizkorodov, Serguei; Laskin, Julia; Laskin, Alexander

2011-05-26T23:59:59.000Z

468

Global warming, bad weather, insurance losses and the global economy  

SciTech Connect (OSTI)

Global warming causes extremely bad weather in the near term. The impact on the insurance industry is described. Why global warming in the near term causes very bad weather is explained. The continuing trend of very bad weather and the future impact on the insurance industry is explored. How very bad weather can affect the global financial market is explained. Taking a historical view of the development of the modern economy, the authors describe in the near term the impact of global warming on the global economy. The long term impact of global warming on the global economy and the human race is explored. Opportunities presented by global warming are described.

Low, N.C. [UOB Life Assurance Ltd., Singapore (Singapore); Shen, S. [Global Warming International Center, Woodridge, IL (United States)

1996-09-01T23:59:59.000Z

469

E-Print Network 3.0 - assessing aerosol retention Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

sources of aerosol OC and assessing its transformations before... ACPD 8, 6539-6569, 2008 ESI FT-ICR MS characterization of aerosol WSOC A. S. Wozniak et al. Title... .0 License....

470

Investigation of the aerosol-cloud interaction using the WRF framework  

E-Print Network [OSTI]

. Simulations with various aerosol profiles demonstrate that the response of precipitation to the increase of aerosol concentrations is non-monotonic. The maximal cloud cover, core updraft, and maximal vertical velocity exhibit similar responses as precipitation...

Li, Guohui

2009-05-15T23:59:59.000Z

471

Aerodynamic Focusing of High-Density Aerosols D.E. Ruiza,  

E-Print Network [OSTI]

Aerodynamic Focusing of High-Density Aerosols D.E. Ruiza, , L. Gundersona , M.J. Haya , E. Merinob-density aerosol focusing for 1µm silica spheres. Preliminary results recover previous findings on aerodynamic

472

Investigation of the optical and cloud forming properties of pollution, biomass burning, and mineral dust aerosols  

E-Print Network [OSTI]

properties of a biomass burning aerosol generated from fires on the Yucatan Peninsula. Measured aerosol size distributions and size-resolved hygroscopicity and volatility were used to infer critical supersaturation distributions of the distinct particle types...

Lee, Yong Seob

2006-08-16T23:59:59.000Z

473

Climate effects of seasonally varying Biomass Burning emitted Carbonaceous Aerosols (BBCA)  

E-Print Network [OSTI]

The climate impact of the seasonality of Biomass Burning emitted Carbonaceous Aerosols (BBCA) is studied using an aerosol-climate model coupled with a slab ocean model in a set of 60-year long simulations, driven by BBCA ...

Jeong, Gill-Ran

474

E-Print Network 3.0 - aerosolized red tide Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

characteristics of desert dust and biomass burning aerosols Summary: in the right panel of Fig. 6. The aerosol scenes spectra are drawn in green, the clear sky scenes in...

475

High Flash-point Fluid Flow System Aerosol Flammability Study and Combustion Mechanism Analysis  

E-Print Network [OSTI]

understanding of this combustion process. The potential application of the ignition delay will be beneficial to the mitigation timing and detector sensor setting of facilities to prevent aerosol cloud fires. Finally, the scientific method of aerosol...

Huang, Szu-Ying

2013-12-02T23:59:59.000Z

476

CHASER: An Innovative Satellite Mission Concept to Measure the Effects of Aerosols on Clouds and Climate  

E-Print Network [OSTI]

The formation of cloud droplets on aerosol particles, technically known as the activation of cloud condensation nuclei (CCN), is the fundamental process driving the interactions of aerosols with clouds and precipitation. ...

Rosenfeld, Daniel

477

Mechanisms of aerosol-forced AMOC variability in a state of the art climate model  

E-Print Network [OSTI]

with a new state-of-the-art Earth system model. Anthropogenic aerosols have previously been highlighted anthropogenic aerosols force a strengthening of the AMOC by up to 20% in our state-of-the-art Earth system model

478

Elucidating secondary organic aerosol from diesel and gasoline vehicles through detailed characterization of  

E-Print Network [OSTI]

Elucidating secondary organic aerosol from diesel and gasoline vehicles through detailed 19, 2012 (received for review July 22, 2012) Emissions from gasoline and diesel vehicles composition, mass distribu- tion, and organic aerosol formation potential of emissions from gasoline

Silver, Whendee

479

The effects of volcanic aerosols on mid-latitude ozone recovery  

E-Print Network [OSTI]

In this paper, comparisons between the derived Chemistry Climate Model Initiative aerosol data set to balloon sonde measurements of aerosols made in Laramie, Wyoming are made between 1979- 2012. Using the derived CCMI ...

Haskins, Jessica D

2014-01-01T23:59:59.000Z

480

E-Print Network 3.0 - aerosol pool scrubbing Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

sensing of non-aerosol absorption in cloud free atmosphere Yoram J. Kaufman,1 Summary: Remote sensing of non-aerosol absorption in cloud free atmosphere Yoram J. Kaufman,1 Oleg...

Note: This page contains sample records for the topic "global aerosol products" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


481

Aerosol effects on the photochemistry in Mexico City during MCMA-2006/MILAGRO campaign  

E-Print Network [OSTI]

In the present study, the impact of aerosols on the photochemistry in Mexico City is evaluated using the WRF-CHEM model for the period from 24 to 29 March during the MCMA-2006/MILAGRO campaign. An aerosol radiative module ...

Li, Guohui

482

Sources and Composition of Submicron Organic Mass in Marine Aerosol Particles  

DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

Recent studies have proposed a variety of interpretations of the sources and composition of atmospheric marine aerosol particles (aMAP) based on a range of physical and chemical measurements collected during open-ocean research cruises. To investigate the processes that affect marine organic particles, this study uses the characteristic functional group composition (from Fourier transform infrared (FTIR) spectroscopy) of aMAP from five ocean regions to show that: (i) The organic functional group composition of aMAP that can be identified as atmospheric primary marine (ocean-derived) aerosol (aPMA) is 6512% hydroxyl, 219% alkane, 66% amine, and 78% carboxylic acid functional groups. Contributions from photochemical reactions add carboxylic acid groups (15%-25%), shipping effluent in seawater and ship emissions add additional alkane groups (up to 70%), and coastal emissions mix in alkane and carboxylic acid groups from coastal pollution sources. (ii) The organic composition of aPMA is nearly identical to model generated primary marine aerosol particles (gPMA) from bubbled seawater (55% hydroxyl, 32% alkane, and 13% amine functional groups), indicating that its overall functional group composition is the direct consequence of the organic constituents of the seawater source. (iii) While the seawater organic functional group composition was nearly invariant across all three ocean regions studied, the gPMA alkane group fraction increased with chlorophyll-a concentrations (r = 0.79). gPMA from productive seawater had a larger fraction of alkane functional groups (35%) compared to gPMA from non-productive seawater (16%), likely due to the presence of surfactants in productive seawater that stabilize the bubble film and lead to preferential drainage of the more soluble (lower alkane group fraction) organic components. gPMA has a hydroxyl group absorption peak location characteristic of monosaccharides and disaccharides, where the seawater OM hydroxyl group peak location is closer to that of polysaccharides. This may result from the larger saccharides preferentially remaining in the seawater during gPMA and aPMA production

Frossard, Amanda; Russell, Lynn; Burrows, Susannah M.; Elliott, Scott; Bates, Timothy S.; Quinn, P. K.

2014-11-27T23:59:59.000Z

483

CARES: Carbonaceous Aerosol and Radiative Effects Study Operations Plan  

SciTech Connect (OSTI)

The CARES field campaign is motivated by the scientific issues described in the CARES Science Plan. The primary objectives of this field campaign are to investigate the evolution and aging of carbonaceous aerosols and their climate-affecting properties in the urban plume of Sacramento, California, a mid-size, mid-latitude city that is located upwind of a biogenic volatile organic compound (VOC) emission region. Our basic observational strategy is to make comprehensive gas, aerosol, and meteorological measurements upwind, within, and downwind of the urban area with the DOE G-1 aircraft and at strategically located ground sites so as to study the evolution of urban aerosols as they age and mix with biogenic SOA precursors. The NASA B-200 aircraft, equipped with the High Spectral Resolution Lidar (HSRL), digital camera, and the Research Scanning Polarimeter (RSP), will be flown in coordination with the G-1 to characterize the vertical and horizontal distribution of aerosols and aerosol optical properties, and to provide the vertical context for the G-1 and ground in situ measurements.

Zaveri, RA; Shaw, WJ; Cziczo, DJ

2010-07-12T23:59:59.000Z

484

E-Print Network 3.0 - arctic aerosol burden Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

and surface... generally exhibits low aerosol ... Source: National Oceanic and Atmospheric Administration, Pacific Marine Environmental Laboratory, Atmopsheric Chemistry and...

485

E-Print Network 3.0 - aerosol sellest rgivad Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

October 4, 2004 Abstract Atmospheric aerosol particles scatter and absorb shortwave (solar) radiation and Source: Brookhaven National Laboratory, Environmental Chemistry...

486

E-Print Network 3.0 - aerosol biokinetics concentrations Sample...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

October 4, 2004 Abstract Atmospheric aerosol particles scatter and absorb shortwave (solar) radiation and Source: Brookhaven National Laboratory, Environmental Chemistry...

487

E-Print Network 3.0 - aerosols Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

October 4, 2004 Abstract Atmospheric aerosol particles scatter and absorb shortwave (solar) radiation and Source: Brookhaven National Laboratory, Environmental Chemistry...

488

China's Global Oil Strategy  

E-Print Network [OSTI]

nations began to seek out oil reserves around the world. 3on the limited global oil reserves and spiking prices. Manyto the largest proven oil reserves, making up 61 percent of

Thomas, Bryan G

2009-01-01T23:59:59.000Z

489

KRFTWRK Global Human Electricity  

E-Print Network [OSTI]

Power Network 2.1.1 Virtual Power Plants The Global Powernetwork, based on "Virtual Power Plants", called "VPP". A "participant runs a virtual human power plant. Per every "

Prohaska, Rainer

2009-01-01T23:59:59.000Z

490

China's Global Oil Strategy  

E-Print Network [OSTI]

21, 2008. Ying, Wang. China, Venezuela firms to co-developoilfields. China Daily (27 August 2005) http://David and Bi Jianhai. Chinas Global Hunt for Energy.

Thomas, Bryan G

2009-01-01T23:59:59.000Z

491

Global Cool Cities Alliance  

Broader source: Energy.gov [DOE]

The Department of Energy (DOE) is currently supporting the Global Cool Cities Alliance (GCCA), a non-profit organization that works with cities, regions, and national governments to speed the...

492

Global warming elucidated  

SciTech Connect (OSTI)

The meaning of global warming and its relevance to everyday life is explained. Simple thermodynamics is used to predict an oscillatory nature of the change in climate due to global warming. Global warming causes extreme events and bad weather in the near term. In the long term it may cause the earth to transition to another equilibrium state through many oscillation in climatic patterns. The magnitudes of these oscillations could easily exceed the difference between the end points. The author further explains why many no longer fully understands the nature and magnitudes of common phenomena such as storms and wind speeds because of these oscillations, and the absorptive properties of clouds. The author links the increase in duration of the El Nino to global warming, and further predicts public health risks as the earth transitions to another equilibrium state in its young history.

Shen, S. [Global Warming International Center, Woodridge, IL (United States)

1995-03-01T23:59:59.000Z

493

Toxicity of atmospheric aerosols on marine phytoplankton  

E-Print Network [OSTI]

fertilization on carbon sequestration in the Southern Ocean.production, and carbon sequestration (47). In areas whereproductivity and carbon sequestration and thus influence

2009-01-01T23:59:59.000Z

494

BNL-65388-AB PROPERTIES OF AMMONIATED SULFATE AEROSOLS AT LOW TEMPERATURES  

E-Print Network [OSTI]

BNL-65388-AB PROPERTIES OF AMMONIATED SULFATE AEROSOLS AT LOW TEMPERATURES: WHY ARE THE MODELS SO of Energy under Contract No. DE-AC02-98CH10886. #12;PROPERTIES OF AMMONIATED SULFATE AEROSOLS AT LOW will present a study of the properties of ammoniated sulfate aerosols ((NH4)2SO4, NH4HSO4, and in- between

495

REPRESENTING AEROSOL DYNAMICS AND PROPERTIES IN CHEMICAL TRANSPORT MODELS BY THE METHOD OF MOMENTS  

E-Print Network [OSTI]

understanding of the key processes that govern the aerosol size distribution: · Gas-to-particle conversion--conversion, suspensions of solid or liquid particles, are an important multi- phase system. Aerosols scatter and absorb retrospectively and prospectively for different emissions scenarios. Important aerosol properties and processes

496

Sensitivity of stratospheric geoengineering with black carbon to aerosol size and altitude of injection  

E-Print Network [OSTI]

Sensitivity of stratospheric geoengineering with black carbon to aerosol size and altitude geoengineering with black carbon (BC) aerosols using a general circulation model with fixed sea surface involving sulfate aerosols, black carbon geoengineering likely carries too many risks to make it a viable

497

Cloud and Aerosol Properties, Precipitable Water, and Profiles of Temperature and Water Vapor from MODIS  

E-Print Network [OSTI]

Cloud and Aerosol Properties, Precipitable Water, and Profiles of Temperature and Water Vapor from such as cloud mask, atmos- pheric profiles, aerosol properties, total precipitable water, and cloud properties vapor amount, aerosol particles, and the subsequently formed clouds [9]. Barnes et al. [2] provide

Sheridan, Jennifer

498

Significant reduction of surface solar irradiance induced by aerosols in a suburban region in northeastern China  

E-Print Network [OSTI]

Significant reduction of surface solar irradiance induced by aerosols in a suburban region in northeastern China Xiangao Xia,1 Hongbin Chen,1 Zhanqing Li,1,2 Pucai Wang,1 and Jiankai Wang1 Received 25 May region in northeastern China. Aerosol properties derived from Sun photometer measurements and aerosol

Li, Zhanqing

499

Business Development - Predictive Maintenance Products  

E-Print Network [OSTI]

BUSINESS DEVELOPMENT - PREDICTIVE MAINTENANCE PRODUCTS Phillip Sceiczina, ifm efector, inc. In this time of global competitiveness, more companies are focusing on reducing manufacturing costs to increase profits. Energy costs can be a...

Sceiczina, P.

2005-01-01T23:59:59.000Z

500

Educational Product Educators Grades 58  

E-Print Network [OSTI]

Educational Product Educators Grades 5­8 WEATHER Investigating the Climate System WEATHER Global Theon, Former Program for your favorite music group!. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 3 Scientist for NASA TRMM Editorial Assistance, Dan Stillman, Science Communications Specialist

Waliser, Duane E.