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Sample records for geothermometry isotopic analysis

  1. Isotope Geothermometry | Open Energy Information

    Open Energy Info (EERE)

    Exploration Group: Geochemical Techniques Exploration Sub Group: Geochemical Data Analysis Parent Exploration Technique: Geothermometry Information Provided by Technique...

  2. Category:Geothermometry | Open Energy Information

    Open Energy Info (EERE)

    Technique Subcategories This category has the following 2 subcategories, out of 2 total. G Gas Geothermometry 1 pages I Isotope Geothermometry 1 pages Pages in...

  3. Liquid Geothermometry | Open Energy Information

    Open Energy Info (EERE)

    Exploration Group: Geochemical Techniques Exploration Sub Group: Geochemical Data Analysis Parent Exploration Technique: Geothermometry Information Provided by Technique...

  4. Gas Geothermometry | Open Energy Information

    Open Energy Info (EERE)

    Exploration Group: Geochemical Techniques Exploration Sub Group: Geochemical Data Analysis Parent Exploration Technique: Geothermometry Information Provided by Technique...

  5. Geothermometry | Open Energy Information

    Open Energy Info (EERE)

    In The Past 20 Years- Geochemistry In Geothermal Exploration Resource Evaluation And Reservoir Management Geothermometry (Powell and Cumming, 2010) Any Spreadsheets for...

  6. Category:Gas Geothermometry | Open Energy Information

    Open Energy Info (EERE)

    Gas Geothermometry Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Geothermalpower.jpg Looking for the Gas Geothermometry page? For detailed information on Gas...

  7. Geothermometry At Yellowstone Region (Fournier, 1979) | Open...

    Open Energy Info (EERE)

    Geothermal Region Exploration Technique Geothermometry Activity Date Usefulness useful DOE-funding Unknown Notes Enthalpy-Chloride digram. Not exactly cation geothermometry...

  8. Geology, hydrothermal petrology, stable isotope geochemistry, and fluid inclusion geothermometry of LASL geothermal test well C/T-1 (Mesa 31-1), East Mesa, Imperial Valley, California, USA

    SciTech Connect (OSTI)

    Miller, K.R.; Elders, W.A.

    1980-08-01

    Borehole Mesa 31-1 (LASL C/T-1) is an 1899-m (6231-ft) deep well located in the northwestern part of the East Mesa Geothermal Field. Mesa 31-1 is the first Calibration/Test Well (C/T-1) in the Los Alamos Scientific Laboratory (LASL), Geothermal Log Interpretation Program. The purpose of this study is to provide a compilation of drillhole data, drill cuttings, well lithology, and formation petrology that will serve to support the use of well LASL C/T-1 as a calibration/test well for geothermal logging. In addition, reviews of fluid chemistry, stable isotope studies, isotopic and fluid inclusion geothermometry, and the temperature log data are presented. This study provides the basic data on the geology and hydrothermal alteration of the rocks in LASL C/T-1 as background for the interpretation of wireline logs.

  9. Integrated Chemical Geothermometry System for Geothermal Exploration |

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Department of Energy Chemical Geothermometry System for Geothermal Exploration Integrated Chemical Geothermometry System for Geothermal Exploration DOE Geothermal Peer Review 2010 - Presentation. Develop practical and reliable system to predict geothermal reservoir temperatures from integrated chemical analyses of spring and well fluids. tracers_spycher_integrated_chemical.pdf (272.32 KB) More Documents & Publications Integrated Chemical Geothermometry System for Geothermal Exploration

  10. Multicomponent Equilibrium Models for Testing Geothermometry Approaches

    SciTech Connect (OSTI)

    Cooper, D. Craig; Palmer, Carl D.; Smith, Robert W.; McLing, Travis L.

    2013-02-01

    Geothermometry is an important tool for estimating deep reservoir temperature from the geochemical composition of shallower and cooler waters. The underlying assumption of geothermometry is that the waters collected from shallow wells and seeps maintain a chemical signature that reflects equilibrium in the deeper reservoir. Many of the geothermometers used in practice are based on correlation between water temperatures and composition or using thermodynamic calculations based a subset (typically silica, cations or cation ratios) of the dissolved constituents. An alternative approach is to use complete water compositions and equilibrium geochemical modeling to calculate the degree of disequilibrium (saturation index) for large number of potential reservoir minerals as a function of temperature. We have constructed several “forward” geochemical models using The Geochemist’s Workbench to simulate the change in chemical composition of reservoir fluids as they migrate toward the surface. These models explicitly account for the formation (mass and composition) of a steam phase and equilibrium partitioning of volatile components (e.g., CO2, H2S, and H2) into the steam as a result of pressure decreases associated with upward fluid migration from depth. We use the synthetic data generated from these simulations to determine the advantages and limitations of various geothermometry and optimization approaches for estimating the likely conditions (e.g., temperature, pCO2) to which the water was exposed in the deep subsurface. We demonstrate the magnitude of errors that can result from boiling, loss of volatiles, and analytical error from sampling and instrumental analysis. The estimated reservoir temperatures for these scenarios are also compared to conventional geothermometers. These results can help improve estimation of geothermal resource temperature during exploration and early development.

  11. Geothermometry At Central Nevada Seismic Zone Region (Shevenell...

    Open Energy Info (EERE)

    Geothermometry At Central Nevada Seismic Zone Region (Shevenell & De Rocher, 2005) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Geothermometry...

  12. Geothermometry At Nw Basin & Range Region (Shevenell & De Rocher...

    Open Energy Info (EERE)

    Geothermometry At Nw Basin & Range Region (Shevenell & De Rocher, 2005) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Geothermometry At Nw...

  13. Geothermometry At Blackfoot Reservoir Area (Hutsinpiller & Parry...

    Open Energy Info (EERE)

    Activity Details Location Blackfoot Reservoir Area Exploration Technique Geothermometry Activity Date Usefulness useful DOE-funding Unknown References Amy Hutsinpiller, W. T....

  14. Improvements in geothermometry. Final technical report

    SciTech Connect (OSTI)

    Potter, J.; Dibble, W.; Parks, G.; Nur, A.

    1982-07-01

    The following are covered: the basis of the Na-K-Ca geothermometer, geothermometry via model calculations, non ideality and complexing, and experimental calibration.

  15. Geothermometry At Mt St Helens Area (Shevenell & Goff, 1995)...

    Open Energy Info (EERE)

    St Helens Area (Shevenell & Goff, 1995) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Geothermometry At Mt St Helens Area (Shevenell & Goff,...

  16. Geothermometry At Walker-Lane Transitional Zone Region (Shevenell...

    Open Energy Info (EERE)

    (Shevenell & De Rocher, 2005) Exploration Activity Details Location Walker-Lane Transition Zone Geothermal Region Exploration Technique Geothermometry Activity Date Usefulness...

  17. Geothermometry At Walker-Lane Transitional Zone Region (Laney...

    Open Energy Info (EERE)

    Zone Region (Laney, 2005) Exploration Activity Details Location Walker-Lane Transition Zone Geothermal Region Exploration Technique Geothermometry Activity Date Usefulness...

  18. Geothermometry At Blue Mountain Geothermal Area (Casteel, Et...

    Open Energy Info (EERE)

    Details Location Blue Mountain Geothermal Area Exploration Technique Geothermometry Activity Date 2010 - 2010 Usefulness useful DOE-funding Unknown Exploration Basis A water...

  19. Geothermometry At Upper Hot Creek Ranch Area (Benoit & Blackwell...

    Open Energy Info (EERE)

    Activity Details Location Upper Hot Creek Ranch Area Exploration Technique Geothermometry Activity Date Usefulness useful DOE-funding Unknown Notes Ten water samples were collected...

  20. Geothermometry At Clear Lake Area (Thompson, Et Al., 1992) |...

    Open Energy Info (EERE)

    Activity Details Location Clear Lake Area Exploration Technique Geothermometry Activity Date Usefulness useful DOE-funding Unknown Notes Based on the above discussion,...

  1. Geothermometry At Silver Peak Area (DOE GTP) | Open Energy Information

    Open Energy Info (EERE)

    Silver Peak Area (DOE GTP) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Geothermometry At Silver Peak Area (DOE GTP) Exploration Activity...

  2. Geothermometry At Alum Area (DOE GTP) | Open Energy Information

    Open Energy Info (EERE)

    Alum Area (DOE GTP) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Geothermometry At Alum Area (DOE GTP) Exploration Activity Details Location...

  3. Geothermometry At The Needles Area (DOE GTP) | Open Energy Information

    Open Energy Info (EERE)

    The Needles Area (DOE GTP) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Geothermometry At The Needles Area (DOE GTP) Exploration Activity...

  4. Geothermometry At New River Area (DOE GTP) | Open Energy Information

    Open Energy Info (EERE)

    New River Area (DOE GTP) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Geothermometry At New River Area (DOE GTP) Exploration Activity Details...

  5. Geothermometry At Fort Bliss Area (DOE GTP) | Open Energy Information

    Open Energy Info (EERE)

    Fort Bliss Area (DOE GTP) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Geothermometry At Fort Bliss Area (DOE GTP) Exploration Activity...

  6. Geothermometry At Lassen Volcanic National Park Area (Thompson...

    Open Energy Info (EERE)

    Thompson, 1985) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Geothermometry At Lassen Volcanic National Park Area (Thompson, 1985) Exploration...

  7. Geothermometry At Chena Geothermal Area (Kolker, 2008) | Open...

    Open Energy Info (EERE)

    1973 - 1974 Usefulness not indicated DOE-funding Unknown Exploration Basis Masters thesis Norma Biggar, Geophysical Institute University of Alaska Notes Geothermometry...

  8. Geothermometry At Fish Lake Valley Area (DOE GTP) | Open Energy...

    Open Energy Info (EERE)

    Fish Lake Valley Area (DOE GTP) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Geothermometry At Fish Lake Valley Area (DOE GTP) Exploration...

  9. Geothermometry At Akutan Fumaroles Area (Kolker, Et Al., 2010...

    Open Energy Info (EERE)

    Geothermometry Activity Date Usefulness useful DOE-funding Unknown Notes The chemistry of the hot springs strongly suggests the existence of a neutral chloride reservoir...

  10. Geothermometry At Desert Queen Area (Garchar & Arehart, 2008...

    Open Energy Info (EERE)

    Desert Queen Area (Garchar & Arehart, 2008) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Geothermometry At Desert Queen Area (Garchar &...

  11. Geothermometry At Nevada Test And Training Range Area (Sabin...

    Open Energy Info (EERE)

    Nevada Test And Training Range Area (Sabin, Et Al., 2004) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Geothermometry At Nevada Test And...

  12. Analysis of hydrogen isotope mixtures

    DOE Patents [OSTI]

    Villa-Aleman, Eliel

    1994-01-01

    An apparatus and method for determining the concentrations of hydrogen isotopes in a sample. Hydrogen in the sample is separated from other elements using a filter selectively permeable to hydrogen. Then the hydrogen is condensed onto a cold finger or cryopump. The cold finger is rotated as pulsed laser energy vaporizes a portion of the condensed hydrogen, forming a packet of molecular hydrogen. The desorbed hydrogen is ionized and admitted into a mass spectrometer for analysis.

  13. New Mexico conservative ion water chemistry data and chalcedony geothermometry

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Shari Kelley

    2015-10-21

    Compilation of boron, lithium, bromine, and silica data from wells and springs throughout New Mexico from a wide variety of sources. The chalcedony geothermometry calculation is included in this file.

  14. Microbial impacts on geothermometry temperature predictions

    SciTech Connect (OSTI)

    Yoshiko Fujita; David W. Reed; Kaitlyn R. Nowak; Vicki S. Thompson; Travis L. McLing; Robert W. Smith

    2013-02-01

    Conventional geothermometry approaches assume that the composition of a collected water sample originating in a deep geothermal reservoir still reflects chemical equilibration of the water with the deep reservoir rocks. However, for geothermal prospecting samples whose temperatures have dropped to <120°C, temperature predictions may be skewed by the activity of microorganisms; microbial metabolism can drastically and rapidly change the water’s chemistry. We hypothesize that knowledge of microbial impacts on exploration sample geochemistry can be used to constrain input into geothermometry models and thereby improve the reliability of reservoir temperature predictions. To evaluate this hypothesis we have chosen to focus on sulfur cycling, because of the significant changes in redox state and pH associated with sulfur chemistry. Redox and pH are critical factors in defining the mineral-fluid equilibria that form the basis of solute geothermometry approaches. Initially we are developing assays to detect the process of sulfate reduction, using knowledge of genes specific to sulfate reducing microorganisms. The assays rely on a common molecular biological technique known as quantitative polymerase chain reaction (qPCR), which allows estimation of the number of target organisms in a particular sample by enumerating genes specific to the organisms rather than actually retrieving and characterizing the organisms themselves. For quantitation of sulfate reducing genes using qPCR, we constructed a plasmid (a piece of DNA) containing portions of two genes (known as dsrA and dsrB) that are directly involved with sulfate reduction and unique to sulfate reducing microorganisms. Using the plasmid as well as DNA from other microorganisms known to be sulfate reducers or non-sulfate reducers, we developed qPCR protocols and showed the assay’s specificity to sulfate reducers and that a qPCR standard curve using the plasmid was linear over >5 orders of magnitude. As a first test

  15. Isotopic Analysis- Fluid At Fenton Hill HDR Geothermal Area ...

    Open Energy Info (EERE)

    Interactions in the Fenton Hill, New Mexico, Hot Dry Rock Geothermal Systems I. Fluid Mixing and Chemical Geothermometry Additional References Retrieved from "http:...

  16. Isotopic Analysis At Fenton Hill Hdr Geothermal Area (Goff, Et...

    Open Energy Info (EERE)

    Isotopic Analysis At Fenton Hill Hdr Geothermal Area (Goff, Et Al., 1981) Redirect page Jump to: navigation, search REDIRECT Isotopic Analysis- Fluid At Fenton Hill Hdr Geothermal...

  17. Mineral Selection for Multicomponent Equilibrium Geothermometry

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Plamer, C. D.; Ohly, S. R.; Smith, R. W.; Neupane, G.; McLing, T.; Mattson, E.

    2015-04-01

    Multicomponent geothermometry requires knowledge of the mineral phases in the reservoir with which the geothermal fluids may be equilibrated. These minerals phases are most often alteration products rather than primary minerals. We have reviewed the literature on geothermal systems representing most major geologic environments typically associated with geothermal activity and identified potential alteration products in various environments. We have included this information in RTEst, a code we have developed to estimate reservoir conditions (temperature, CO2 fugacity) from the geochemistry of near-surface geothermal waters. The information has been included in RTEst through the addition of filters that decrease the potential numbermore » of minerals from all possibilities based on the basis species to those that are more relevant to the particular conditions in which the user is interested. The three groups of filters include host rock type (tholeiitic, calc-alkaline, silicic, siliciclastic, carbonate), water type (acidic, neutral), and the temperature range over which the alteration minerals were formed (low, medium, high). The user-chosen mineral assemblage is checked to make sure that it does not violate the Gibbs phase rule. The user can select one of three mineral saturation weighting schemes that decrease the chance the optimization from being skewed by reaction stoichiometry or analytical uncertainty.« less

  18. Mineral Selection for Multicomponent Equilibrium Geothermometry

    SciTech Connect (OSTI)

    Plamer, C. D.; Ohly, S. R.; Smith, R. W.; Neupane, G.; McLing, T.; Mattson, E.

    2015-04-01

    Multicomponent geothermometry requires knowledge of the mineral phases in the reservoir with which the geothermal fluids may be equilibrated. These minerals phases are most often alteration products rather than primary minerals. We have reviewed the literature on geothermal systems representing most major geologic environments typically associated with geothermal activity and identified potential alteration products in various environments. We have included this information in RTEst, a code we have developed to estimate reservoir conditions (temperature, CO2 fugacity) from the geochemistry of near-surface geothermal waters. The information has been included in RTEst through the addition of filters that decrease the potential number of minerals from all possibilities based on the basis species to those that are more relevant to the particular conditions in which the user is interested. The three groups of filters include host rock type (tholeiitic, calc-alkaline, silicic, siliciclastic, carbonate), water type (acidic, neutral), and the temperature range over which the alteration minerals were formed (low, medium, high). The user-chosen mineral assemblage is checked to make sure that it does not violate the Gibbs phase rule. The user can select one of three mineral saturation weighting schemes that decrease the chance the optimization from being skewed by reaction stoichiometry or analytical uncertainty.

  19. Isotope Geothermometry At Lightning Dock Geothermal Area (Witcher...

    Open Energy Info (EERE)

    Usefulness useful DOE-funding Unknown Exploration Basis Part of the Geothermal Resource Evaluation and Definition (GRED) Program administered by DOE-AAO under Cooperative...

  20. Improved Geothermometry Through Multivariate Reaction Path Modeling and Evaluation of Geomicrobiological Influences on Geochemical Temperature Indicators

    Broader source: Energy.gov [DOE]

    Improved Geothermometry Through Multivariate Reaction Path Modeling and Evaluation of Geomicrobiological Influences on Geochemical Temperature Indicators presentation at the April 2013 peer review meeting held in Denver, Colorado.

  1. Isotopic Analysis- Rock At Coso Geothermal Area (1984) | Open...

    Open Energy Info (EERE)

    Home Exploration Activity: Isotopic Analysis- Rock At Coso Geothermal Area (1984) Exploration Activity Details Location Coso Geothermal Area Exploration Technique...

  2. Isotopic Analysis At Mt St Helens Area (Shevenell & Goff, 2000...

    Open Energy Info (EERE)

    Home Exploration Activity: Isotopic Analysis At Mt St Helens Area (Shevenell & Goff, 2000) Exploration Activity Details Location Mt St Helens Area Exploration Technique...

  3. Isotopic Analysis At Valles Caldera - Redondo Geothermal Area...

    Open Energy Info (EERE)

    Goff, Et Al., 1982) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Isotopic Analysis At Valles Caldera - Redondo Geothermal Area (Goff, Et Al.,...

  4. Isotopic Analysis- Rock At Valles Caldera - Sulphur Springs Geothermal...

    Open Energy Info (EERE)

    WoldeGabriel & Goff, 1992) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Isotopic Analysis- Rock At Valles Caldera - Sulphur Springs Geothermal...

  5. Isotopic Analysis At Yellowstone Region (Goff & Janik, 2002)...

    Open Energy Info (EERE)

    Goff & Janik, 2002) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Isotopic Analysis At Yellowstone Region (Goff & Janik, 2002) Exploration...

  6. Isotopic Analysis At Mt St Helens Area (Shevenell & Goff, 1995...

    Open Energy Info (EERE)

    Home Exploration Activity: Isotopic Analysis At Mt St Helens Area (Shevenell & Goff, 1995) Exploration Activity Details Location Mt St Helens Area Exploration Technique...

  7. Isotopic Analysis- Fluid At Valles Caldera - Sulphur Springs...

    Open Energy Info (EERE)

    Activity: Isotopic Analysis- Fluid At Valles Caldera - Sulphur Springs Geothermal Area (Goff, Et Al., 1982) Exploration Activity Details Location Valles Caldera - Sulphur Springs...

  8. Isotopic Analysis- Fluid At Valles Caldera - Sulphur Springs...

    Open Energy Info (EERE)

    Activity: Isotopic Analysis- Fluid At Valles Caldera - Sulphur Springs Geothermal Area (Goff, Et Al., 1985) Exploration Activity Details Location Valles Caldera - Sulphur Springs...

  9. Isotopic Analysis At Jemez Springs Area (Goff & Janik, 2002)...

    Open Energy Info (EERE)

    Goff & Janik, 2002) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Isotopic Analysis At Jemez Springs Area (Goff & Janik, 2002) Exploration...

  10. Isotopic Analysis- Fluid At Long Valley Caldera Geothermal Area...

    Open Energy Info (EERE)

    Long Valley Caldera Geothermal Area (Taylor & Gerlach, 1983) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Isotopic Analysis- Fluid At Long...

  11. Isotopic Analysis-Fluid At Raft River Geothermal Area (1982)...

    Open Energy Info (EERE)

    GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Isotopic Analysis-Fluid At Raft River Geothermal Area (1982) Exploration Activity Details Location Raft River...

  12. Isotopic Analysis-Fluid At Raft River Geothermal Area (1977)...

    Open Energy Info (EERE)

    GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Isotopic Analysis-Fluid At Raft River Geothermal Area (1977) Exploration Activity Details Location Raft River...

  13. Isotopic Analysis At Walker-Lane Transitional Zone Region (Laney...

    Open Energy Info (EERE)

    Zone Region (Laney, 2005) Exploration Activity Details Location Walker-Lane Transition Zone Geothermal Region Exploration Technique Isotopic Analysis- Fluid Activity Date...

  14. Isotopic Analysis At Yellowstone Region (Sturchio, Et Al., 1990...

    Open Energy Info (EERE)

    Yellowstone Caldera Geothermal Region Exploration Technique Isotopic Analysis- Fluid Activity Date Usefulness could be useful with more improvements DOE-funding Unknown Notes...

  15. Isotopic Analysis- Fluid At Coso Geothermal Area (1982) | Open...

    Open Energy Info (EERE)

    Details Location Coso Geothermal Area Exploration Technique Isotopic Analysis- Fluid Activity Date 1982 Usefulness not indicated DOE-funding Unknown Exploration Basis...

  16. Isotopic Analysis At Long Valley Caldera Geothermal Area (Smith...

    Open Energy Info (EERE)

    Smith & Suemnicht, 1991) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Isotopic Analysis At Long Valley Caldera Geothermal Area (Smith &...

  17. Isotopic Analysis At Northern Basin & Range Region (Cole, 1983...

    Open Energy Info (EERE)

    Cole, 1983) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Isotopic Analysis At Northern Basin & Range Region (Cole, 1983) Exploration Activity...

  18. Isotopic Analysis- Fluid At Salt Wells Area (Shevenell & Garside...

    Open Energy Info (EERE)

    At Salt Wells Area (Shevenell & Garside, 2003) Exploration Activity Details Location Salt Wells Geothermal Area Exploration Technique Isotopic Analysis- Fluid Activity Date 2002 -...

  19. Isotopic Analysis- Fluid At Rose Valley Geothermal Area (1990...

    Open Energy Info (EERE)

    Rose Valley Geothermal Area (1990) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Isotopic Analysis- Fluid At Rose Valley Geothermal Area (1990)...

  20. Isotopic Analysis At Valles Caldera - Redondo Geothermal Area...

    Open Energy Info (EERE)

    Exploration Activity: Isotopic Analysis At Valles Caldera - Redondo Geothermal Area (Phillips, 2004) Exploration Activity Details Location Valles Caldera - Redondo Geothermal Area...

  1. Isotopic Analysis- Rock At Valles Caldera - Sulphur Springs Geothermal...

    Open Energy Info (EERE)

    Phillips, 2004) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Isotopic Analysis- Rock At Valles Caldera - Sulphur Springs Geothermal Area...

  2. Isotopic Analysis- Gas At Chena Geothermal Area (Kolker, Et Al...

    Open Energy Info (EERE)

    Date 2007 - 2007 Usefulness useful DOE-funding Unknown Exploration Basis Lawrence Berkeley National Laboratory sampling and analysis of He isotopes from Chena Hot Springs....

  3. Isotopic Analysis At Lassen Volcanic National Park Area (Janik...

    Open Energy Info (EERE)

    Park Area (Janik & Mclaren, 2010) Exploration Activity Details Location Lassen Volcanic National Park Area Exploration Technique Isotopic Analysis- Fluid Activity Date Usefulness...

  4. Isotopic Analysis At San Juan Volcanic Field Area (Larson & Jr...

    Open Energy Info (EERE)

    San Juan Volcanic Field Area (Larson & Jr, 1986) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Isotopic Analysis At San Juan Volcanic Field...

  5. Isotopic Analysis At Nw Basin & Range Region (Laney, 2005) |...

    Open Energy Info (EERE)

    Location Northwest Basin and Range Geothermal Region Exploration Technique Isotopic Analysis- Fluid Activity Date Usefulness not indicated DOE-funding Unknown Notes...

  6. Isotopic Analysis At Central Nevada Seismic Zone Region (Laney...

    Open Energy Info (EERE)

    Location Central Nevada Seismic Zone Geothermal Region Exploration Technique Isotopic Analysis- Fluid Activity Date Usefulness not indicated DOE-funding Unknown Notes...

  7. Isotopic Analysis- Fluid At Coso Geothermal Area (1990) | Open...

    Open Energy Info (EERE)

    Exploration Activity Details Location Coso Geothermal Area Exploration Technique Isotopic Analysis- Fluid Activity Date 1990 Usefulness not indicated DOE-funding Unknown...

  8. Isotopic Analysis At Clear Lake Area (Thompson, Et Al., 1992...

    Open Energy Info (EERE)

    Exploration Activity Details Location Clear Lake Area Exploration Technique Isotopic Analysis- Fluid Activity Date Usefulness useful DOE-funding Unknown Notes Deuterium and...

  9. Isotopic Analysis- Fluid At Indian Valley Hot Springs Geothermal...

    Open Energy Info (EERE)

    Details Location Indian Valley Hot Springs Geothermal Area Exploration Technique Isotopic Analysis- Fluid Activity Date 1990 Usefulness not indicated DOE-funding Unknown...

  10. Isotopic Analysis- Rock At Valles Caldera - Sulphur Springs Area...

    Open Energy Info (EERE)

    Details Location Valles Caldera - Sulphur Springs Area Exploration Technique Isotopic Analysis- Rock Activity Date Usefulness not indicated DOE-funding Unknown References...

  11. Isotopic Analysis At Northern Basin & Range Region (Laney, 2005...

    Open Energy Info (EERE)

    Location Northern Basin and Range Geothermal Region Exploration Technique Isotopic Analysis- Fluid Activity Date Usefulness not indicated DOE-funding Unknown Notes...

  12. Isotopic Analysis- Fluid At Sierra Valley Geothermal Area (1990...

    Open Energy Info (EERE)

    Activity Details Location Sierra Valley Geothermal Area Exploration Technique Isotopic Analysis- Fluid Activity Date 1990 Usefulness not indicated DOE-funding Unknown...

  13. Isotopic Analysis At Buffalo Valley Hot Springs Area (Laney,...

    Open Energy Info (EERE)

    Activity Details Location Buffalo Valley Hot Springs Area Exploration Technique Isotopic Analysis- Fluid Activity Date Usefulness not indicated DOE-funding Unknown Notes...

  14. Isotopic Analysis- Fluid At Roosevelt Hot Springs Geothermal...

    Open Energy Info (EERE)

    Unknown Exploration Basis Faulder 1991 Conceptual Geological Model compilation and literature review of the Roosevelt Hot Springs Geothermal Area. Notes Stable isotope analysis...

  15. Isotopic Analysis At Long Valley Caldera Geothermal Area (Evans...

    Open Energy Info (EERE)

    search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Isotopic Analysis At Long Valley Caldera Geothermal Area (Evans, Et Al., 2002) Exploration Activity Details...

  16. Plutonium Isotopic Gamma-Ray Analysis

    Energy Science and Technology Software Center (OSTI)

    1992-01-08

    The MGA8 (Multiple Group Analysis) program determines the relative abundances of plutonium and other actinide isotopes in different materials. The program analyzes spectra taken of such samples using a 4096-channel germanium (Ge) gamma-ray spectrometer. The code can be run in a one or two detector mode. The first spectrum, which is required and must be taken at a gain of 0.075 Kev/channel with a high resolution planar detector, contains the 0-300 Kev energy region. Themore »second spectrum, which is optional, must be taken at a gain of 0.25 Kev/channel; it becomes important when analyzing high burnup samples (concentration of Pu241 greater than one percent). Isotopic analysis precisions of one percent or better can be obtained, and no calibrations are required. The system also measures the abundances of U235, U238, Np237, and Am241. A special calibration option is available to perform a one-time peak-shape characterization when first using a new detector system.« less

  17. Plutonium Isotopic Gamma-Ray Analysis

    Energy Science and Technology Software Center (OSTI)

    1992-01-08

    The MGA8 (Multiple Group Analysis) program determines the relative abundances of plutonium and other actinide isotopes in different materials. The program analyzes spectra taken of such samples using a 4096-channel germanium (Ge) gamma-ray spectrometer. The code can be run in a one or two detector mode. The first spectrum, which is required and must be taken at a gain of 0.075 Kev/channel with a high resolution planar detector, contains the 0-300 Kev energy region. Themore » second spectrum, which is optional, must be taken at a gain of 0.25 Kev/channel; it becomes important when analyzing high burnup samples (concentration of Pu241 greater than one percent). Isotopic analysis precisions of one percent or better can be obtained, and no calibrations are required. The system also measures the abundances of U235, U238, Np237, and Am241. A special calibration option is available to perform a one-time peak-shape characterization when first using a new detector system.« less

  18. Category:Geochemical Data Analysis | Open Energy Information

    Open Energy Info (EERE)

    category, out of 4 total. G Geochemical Data Analysis Geothermometry T Thermal Ion Dispersion Thermochronometry Retrieved from "http:en.openei.orgwindex.php?titleCategory:Ge...

  19. TRIFID (TRansuranic Isotopic Fraction Interrogation Device): A second generation plutonium isotopic analysis system

    SciTech Connect (OSTI)

    Fleissner, J G; Coressel, T W; Freier, D A; Macklin, L L

    1989-01-01

    The TRIFID (Transuranic Isotopic Fraction Interrogation Device) system is a second generation plutonium isotopic analysis system which incorporates many new and unique features in the area of isotopic data acquisition and isotopic analysis instrument consisting of a Canberra Series 95-MCA interfaced to a Compaq 386 computer. The entire TRIFID software package, including MCA communications and isotopic analysis routines, was developed using the C programming language. Extensive use has been made of user friendly screens and menus for ease of operation and training and to facilitate use by technical level operators. Automated TRIFID features provide for MCA/ADC setup and acquisition, spectral storage, isotopic analysis, and report generation. One unique feature of the TRIFID system design allows it to be pre-programed for an entire day's counting. The isotopic analysis module (EPICS) contains an expert system formalism which is used to detect and assay for spectral interferences, and to automatically adjust peak fitting constraints based on spectral intensity variations. A TRIFID system has been in operation in a production laboratory at the Rocky Flats Plant since September 1988. Marked decreases in training and hands-on operation time have been achieved in comparison to the older, preceding isotopic systems. 2 refs., 3 figs.

  20. Improved Geothermometry Through Multivariate Reaction Path Modeling and Evaluation of Geomicrobiological Influences on Geochemical Temperature Indicators

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Improved Geothermometry Through Multivariate Reaction Path Modeling and Evaluation of Geomicrobiological Influences on Geochemical Temperature Indicators Project Officer: Eric Hass Total Project Funding: $999,000 April 24, 2013 Craig Cooper Larry Hull Idaho National Laboratory This presentation does not contain any proprietary confidential, or otherwise restricted information. 2 | US DOE Geothermal Program eere.energy.gov Relevance/Impact of Research Geothermometry enables estimation of

  1. Isotopes

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Office of Science » Nuclear Physics » Isotopes Isotopes Isotopes produced at Los Alamos National Laboratory are saving lives, advancing cutting-edge research and keeping the U.S. safe. Get Expertise Eva Birnbaum (505) 665-7167 Email Wolfgang Runde (505) 667-3350 Email Isotope Production and Applications isotopes Isotopes produced at IPF are critical for medical diagnosis and disease treatment. These positron emission tomography images were made possible using isotopes produced at LANL.

  2. System and method for high precision isotope ratio destructive analysis

    DOE Patents [OSTI]

    Bushaw, Bruce A; Anheier, Norman C; Phillips, Jon R

    2013-07-02

    A system and process are disclosed that provide high accuracy and high precision destructive analysis measurements for isotope ratio determination of relative isotope abundance distributions in liquids, solids, and particulate samples. The invention utilizes a collinear probe beam to interrogate a laser ablated plume. This invention provides enhanced single-shot detection sensitivity approaching the femtogram range, and isotope ratios that can be determined at approximately 1% or better precision and accuracy (relative standard deviation).

  3. Isotopes

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Eva Birnbaum (505) 665-7167 Email Wolfgang Runde (505) 667-3350 Email Isotope Production and Applications isotopes Isotopes produced at IPF are critical for medical diagnosis and ...

  4. Use of Stable Isotopes in Forensic Analysis of Microorganisms

    SciTech Connect (OSTI)

    Kreuzer-Martin, Helen W.; Hegg, Eric L.

    2012-01-18

    The use of isotopic signatures for forensic analysis of biological materials is well-established, and the same general principles that apply to interpretation of stable isotope content of C, N, O, and H apply to the analysis of microorganisms. Heterotrophic microorganisms derive their isotopic content from their growth substrates, which are largely plant and animal products, and the water in their culture medium. Thus the isotope signatures of microbes are tied to their growth environment. The C, N, O, and H isotope ratios of spores have been demonstrated to constitute highly discriminating signatures for sample matching. They can rule out specific samples of media and/or water as possible production media, and can predict isotope ratio ranges of the culture media and water used to produce a given sample. These applications have been developed and tested through analyses of approximately 250 samples of Bacillus subtilis spores and over 500 samples of culture media, providing a strong statistical basis for data interpretation. A Bayesian statistical framework for integrating stable isotope data with other types of signatures derived from microorganisms has been able to characterize the culture medium used to produce spores of various Bacillus species, leveraging isotopic differences in different medium types and demonstrating the power of data integration for forensic investigations.

  5. Isotopic abundance in atom trap trace analysis

    DOE Patents [OSTI]

    Lu, Zheng-Tian; Hu, Shiu-Ming; Jiang, Wei; Mueller, Peter

    2014-03-18

    A method and system for detecting ratios and amounts of isotopes of noble gases. The method and system is constructed to be able to measure noble gas isotopes in water and ice, which helps reveal the geological age of the samples and understand their movements. The method and system uses a combination of a cooled discharge source, a beam collimator, a beam slower and magneto-optic trap with a laser to apply resonance frequency energy to the noble gas to be quenched and detected.

  6. Method for isotopic analysis of chlorinated organic compounds

    DOE Patents [OSTI]

    Holt, Ben D.; Sturchio, Neil C.

    1999-01-01

    The present invention provides a method for preparing a VOC sample for carbon and chlorine isotope ratio analysis by mass spectrometer. A VOC sample is placed in a combustion tube and reacted with CuO to form CO.sub.2 and CuCl. The CO.sub.2 is then extracted and analyzed for the carbon isotope ratio. The CuCl is separated from the excess CuO and reacted with CH.sub.3 I to form CH.sub.3 Cl, extracted and analyzed for chlorine isotope ratio.

  7. Method for isotopic analysis of chlorinated organic compounds

    DOE Patents [OSTI]

    Holt, B.D.; Sturchio, N.C.

    1999-08-24

    The present invention provides a method for preparing a VOC sample for carbon and chlorine isotope ratio analysis by mass spectrometer. A VOC sample is placed in a combustion tube and reacted with CuO to form CO{sub 2} and CuCl. The CO{sub 2} is then extracted and analyzed for the carbon isotope ratio. The CuCl is separated from the excess CuO and reacted with CH{sub 3}I to form CH{sub 3}Cl, extracted and analyzed for chlorine isotope ratio. 9 figs.

  8. RESOLUTION OF URANIUM ISOTOPES WITH KINETIC PHOSPHORESCENCE ANALYSIS

    SciTech Connect (OSTI)

    Miley, Sarah M.; Hylden, Anne T.; Friese, Judah I.

    2013-04-01

    This study was conducted to test the ability of the Chemchek™ Kinetic Phosphorescence Analyzer Model KPA-11 with an auto-sampler to resolve the difference in phosphorescent decay rates of several different uranium isotopes, and therefore identify the uranium isotope ratios present in a sample. Kinetic phosphorescence analysis (KPA) is a technique that provides rapid, accurate, and precise determination of uranium concentration in aqueous solutions. Utilizing a pulsed-laser source to excite an aqueous solution of uranium, this technique measures the phosphorescent emission intensity over time to determine the phosphorescence decay profile. The phosphorescence intensity at the onset of decay is proportional to the uranium concentration in the sample. Calibration with uranium standards results in the accurate determination of actual concentration of the sample. Different isotopes of uranium, however, have unique properties which should result in different phosphorescence decay rates seen via KPA. Results show that a KPA is capable of resolving uranium isotopes.

  9. Geothermometry At Long Valley Caldera Geothermal Area (Mariner...

    Open Energy Info (EERE)

    California R.O. Fournier, Michael L. Sorey, Robert H. Mariner, Alfred H. Truesdell (1979) Chemical and Isotopic Prediction of Aquifer Temperatures in the Geothermal System at Long...

  10. Geothermometry At Coso Geothermal Area (1980) | Open Energy Informatio...

    Open Energy Info (EERE)

    DOE-funding Unknown Exploration Basis Fluid temperature of feed water Notes Cation and sulfate isotope geothermometers indicate that the reservoir feeding water to the Coso Hot...

  11. Isotopic Analysis (Lewicki & Oldenburg) | Open Energy Information

    Open Energy Info (EERE)

    Analysis- Fluid Activity Date Usefulness useful DOE-funding Unknown References Jennifer L. Lewicki, Curtis M. Oldenburg (Unknown) Near-Surface Co2 Monitoring And Analysis To...

  12. Geochemistry Sampling for Traditional and Multicomponent Equilibrium Geothermometry in Southeast Idaho

    SciTech Connect (OSTI)

    Cannon, Cody; Wood, Thomas; Neupane, Ghanashyam; McLing, Travis; Mattson, Earl; Dobson, Patrick; Conrad, Mark

    2014-10-01

    The Eastern Snake River Plain (ESRP) is an area of high regional heat flux due the movement of the North American Plate over the Yellowstone Hotspot beginning ca.16 Ma. Temperature gradients between 45-60 °C/km (up to double the global average) have been calculated from deep wells that penetrate the upper aquifer system (Blackwell 1989). Despite the high geothermal potential, thermal signatures from hot springs and wells are effectively masked by the rapid flow of cold groundwater through the highly permeable basalts of the Eastern Snake River Plain aquifer (ESRPA) (up to 500+ m thick). This preliminary study is part of an effort to more accurately predict temperatures of the ESRP deep thermal reservoir while accounting for the effects of the prolific cold water aquifer system above. This study combines the use of traditional geothermometry, mixing models, and a multicomponent equilibrium geothermometry (MEG) tool to investigate the geothermal potential of the ESRP. In March, 2014, a collaborative team including members of the University of Idaho, the Idaho National Laboratory, and the Lawrence Berkeley National Laboratory collected 14 thermal water samples from and adjacent to the Eastern Snake River Plain. The preliminary results of chemical analyses and geothermometry applied to these samples are presented herein.

  13. Hanford Isotope Project strategic business analysis Cesium-137 (Cs-137)

    SciTech Connect (OSTI)

    1995-10-01

    The purpose of this business analysis is to address the beneficial reuse of Cesium 137 (Cs-137) in order to utilize a valuable national asset and possibly save millions of tax dollars. Food irradiation is the front runner application along with other uses. This business analysis supports the objectives of the Department of Energy National Isotope Strategy distributed in August 1994 which describes the DOE plans for the production and distribution of isotope products and services. As part of the Department`s mission as stated in that document. ``The Department of Energy will also continue to produce and distribute other radioisotopes and enriched stable isotopes for medical diagnostics and therapeutics, industrial, agricultural, and other useful applications on a businesslike basis. This is consistent with the goals and objectives of the National Performance Review. The Department will endeavor to look at opportunities for private sector to co-fund or invest in new ventures. Also, the Department will seek to divest from ventures that can more profitably or reliably be operated by the private sector.``

  14. Isotopic Analysis At Seven Mile Hole Area (Larson, Et Al., 2009...

    Open Energy Info (EERE)

    Seven Mile Hole Area (Larson, Et Al., 2009) Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Exploration Activity: Isotopic Analysis At Seven Mile Hole Area (Larson, Et...

  15. Geothermometry At Teels Marsh Area (Coolbaugh, Et Al., 2006)...

    Open Energy Info (EERE)

    useful DOE-funding Unknown Notes Follow up (to ASTER satellite imaging) analysis of spring and well waters yielded geothermometer reservoir estimates up to 192C References...

  16. Geothermometry At Rhodes Marsh Area (Coolbaugh, Et Al., 2006...

    Open Energy Info (EERE)

    useful DOE-funding Unknown Notes Follow up (to ASTER satellite imaging) analysis of spring and well waters yielded geothermometer reservoir estimates up to 162C References...

  17. Geothermometry At Coso Geothermal Area (1978) | Open Energy Informatio...

    Open Energy Info (EERE)

    analysis to determine fluid origin. The surface expression of fumarole and acid sulfate pools and shallow steam wells gives a false indication of an extensive vapor...

  18. Isotopic Analysis- Fluid At Valles Caldera - Redondo Area (Rao...

    Open Energy Info (EERE)

    analyzed for their hydrogen and oxygen isotope contents as a part of previous studies (Goff & Grigsby, 1982; Vuataz & Goff, 1986). The present study focuses on the interpretation...

  19. Isotopic Analysis At Jemez Springs Area (Rao, Et Al., 1996) ...

    Open Energy Info (EERE)

    analyzed for their hydrogen and oxygen isotope contents as a part of previous studies (Goff & Grigsby, 1982; Vuataz & Goff, 1986). The present study focuses on the interpretation...

  20. Isotopic Analysis- Fluid At Valles Caldera - Sulphur Springs...

    Open Energy Info (EERE)

    analyzed for their hydrogen and oxygen isotope contents as a part of previous studies (Goff & Grigsby, 1982; Vuataz & Goff, 1986). The present study focuses on the interpretation...

  1. Isotopic Analysis- Fluid At Fenton Hill HDR Geothermal Area ...

    Open Energy Info (EERE)

    analyzed for their hydrogen and oxygen isotope contents as a part of previous studies (Goff & Grigsby, 1982; Vuataz & Goff, 1986). The present study focuses on the interpretation...

  2. Atomic weight and isotopic abundance data analysis 1993

    SciTech Connect (OSTI)

    Holden, N.E.

    1993-08-01

    Literature on isotopic abundance measurements and their variation in nature have been reviewed for impact on standard atomic weight values and associated uncertainties for recent measurements.

  3. Isotopic Analysis- Gas At Long Valley Caldera Geothermal Area...

    Open Energy Info (EERE)

    Through 30 September Activity T. Winnett, Cathy J. Janik (1986) Isotopic Composition of Carbon in Fluids from the Long Valley Geothermal System, California, In- Proceedings of...

  4. Isotopic Analysis At Newberry Caldera Area (Goles & Lambert,...

    Open Energy Info (EERE)

    Rock Activity Date Usefulness not indicated DOE-funding Unknown References Gordon G. Goles, Richard St J. Lambert (1990) A Strontium Isotopic Study Of Newberry Volcano,...

  5. Isotopic Analysis-Fluid At Long Valley Caldera Geothermal Area...

    Open Energy Info (EERE)

    Estimate deep reservoir temperature Notes The oxygen isotope compositions of dissolved sulfate and water from hot springs and shallow drillholes have been tested. Methods are...

  6. Isotopic Analysis-Fluid At Yellowstone Caldera Geothermal Region...

    Open Energy Info (EERE)

    Estimate deep reservoir temperature Notes The oxygen isotope compositions of dissolved sulfate and water from hot springs and shallow drillholes have been tested. Methods are...

  7. Hanford isotope project strategic business analysis yttrium-90 (Y-90)

    SciTech Connect (OSTI)

    1995-10-01

    The purpose of this analysis is to address the short-term direction for the Hanford yttrium-90 (Y-90) project. Hanford is the sole DOE producer of Y-90, and is the largest repository for its source in this country. The production of Y-90 is part of the DOE Isotope Production and Distribution (IP and D) mission. The Y-90 is ``milked`` from strontium-90 (Sr-90), a byproduct of the previous Hanford missions. The use of Sr-90 to produce Y-90 could help reduce the amount of waste material processed and the related costs incurred by the clean-up mission, while providing medical and economic benefits. The cost of producing Y-90 is being subsidized by DOE-IP and D due to its use for research, and resultant low production level. It is possible that the sales of Y-90 could produce full cost recovery within two to three years, at two curies per week. Preliminary projections place the demand at between 20,000 and 50,000 curies per year within the next ten years, assuming FDA approval of one or more of the current therapies now in clinical trials. This level of production would incentivize private firms to commercialize the operation, and allow the government to recover some of its sunk costs. There are a number of potential barriers to the success of the Y-90 project, outside the control of the Hanford Site. The key issues include: efficacy, Food and Drug Administration (FDA) approval and medical community acceptance. There are at least three other sources for Y-90 available to the US users, but they appear to have limited resources to produce the isotope. Several companies have communicated interest in entering into agreements with Hanford for the processing and distribution of Y-90, including some of the major pharmaceutical firms in this country.

  8. Direct analysis of air filter samples for alpha emitting isotopes

    SciTech Connect (OSTI)

    Mohagheghi, A.H.; Ghanbari, F.; Ebara, S.B.; Enghauser, M.E. [Sandia National Labs., Albuquerque, NM (United States); Bakhtiar, S.N. [Westinghouse WIPP, Carlsbad, NM (United States)

    1997-04-01

    The traditional method for determination of alpha emitting isotopes on air filters has been to process the samples by radiochemical methods. However, this method is too slow for cases of incidents involving radioactive materials where the determination of personnel received dose is urgent. A method is developed to directly analyze the air filters taken from personal and area air monitors. The site knowledge is used in combination with alpha spectral information to identify isotopes. A mathematical function is developed to estimate the activity for each isotope. The strengths and weaknesses of the method are discussed.

  9. Isotopic Analysis At Valles Caldera - Redondo Geothermal Area...

    Open Energy Info (EERE)

    of 36Cl- as a tracer isotope in geothermal systems. References F.M. Phillips, Fraser E. Goff, Francois D. Vuataz, H.W. Bentley, H.E. Gove (1984) 36Cl as a tracer in geothermal...

  10. Isotopic Analysis- Fluid At Dixie Valley Geothermal Area (Kennedy...

    Open Energy Info (EERE)

    suggest that helium isotopes are the best and possibly the only indication of deep permeability where high temperature fluids are masked beneath a cold reservoir. Notes 3He4He...

  11. Isotopic Analysis At Separation Creek Area (Van Soest, Et Al...

    Open Energy Info (EERE)

    Usefulness useful DOE-funding Unknown References M. C. van Soest, B. M. Kennedy, W. C. Evans, R. H. Mariner (2002) Mantle Helium And Carbon Isotopes In Separation Creek...

  12. GUM Analysis for TIMS and SIMS Isotopic Ratios in Graphite

    SciTech Connect (OSTI)

    Heasler, Patrick G.; Gerlach, David C.; Cliff, John B.; Petersen, Steven L.

    2007-04-01

    This report describes GUM calculations for TIMS and SIMS isotopic ratio measurements of reactor graphite samples. These isotopic ratios are used to estimate reactor burn-up, and currently consist of various ratios of U, Pu, and Boron impurities in the graphite samples. The GUM calculation is a propagation of error methodology that assigns uncertainties (in the form of standard error and confidence bound) to the final estimates.

  13. Neutron Activation Analysis and Product Isotope Inventory Code System.

    Energy Science and Technology Software Center (OSTI)

    1990-10-31

    Version 00 NAC was designed to predict the neutron-induced gamma-ray radioactivity for a wide variety of composite materials. The NAC output includes the input data, a list of all reactions for each constituent element, and the end-of-irradiation disintegration rates for each reaction. NAC also compiles a product isotope inventory containing the isotope name, the disintegration rate, the gamma-ray source strength, and the absorbed dose rate at 1 meter from an unshielded point source. The inducedmore » activity is calculated as a function of irradiation and decay times; the effect of cyclic irradiation can also be calculated.« less

  14. Femtosecond Laser Ablation Multicollector ICPMS Analysis of Uranium Isotopes in NIST Glass

    SciTech Connect (OSTI)

    Duffin, Andrew M.; Springer, Kellen WE; Ward, Jesse D.; Jarman, Kenneth D.; Robinson, John W.; Endres, Mackenzie C.; Hart, Garret L.; Gonzalez, Jhanis J.; Oropeza, Dayana; Russo, Richard; Willingham, David G.; Naes, Benjamin E.; Fahey, Albert J.; Eiden, Gregory C.

    2015-02-06

    We have utilized femtosecond laser ablation coupled to multi-collector inductively couple plasma mass spectrometry to measure the uranium isotopic content of NIST 61x (x=0,2,4,6) glasses. The uranium content of these glasses is a linear two-component mixing between isotopically natural uranium and the isotopically depleted spike used in preparing the glasses. Laser ablation results match extremely well, generally within a few ppm, with solution analysis following sample dissolution and chemical separation. In addition to isotopic data, sample utilization efficiency measurements indicate that over 1% of ablated uranium atoms reach a mass spectrometer detector, making this technique extremely efficient. Laser sampling also allows for spatial analysis and our data indicate that rare uranium concentration inhomogeneities exist in NIST 616 glass.

  15. Chemistry Data for Geothermometry Mapping of Deep Hydrothermal Reservoirs in Southeastern Idaho

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Earl Mattson

    2016-01-18

    This dataset includes chemistry of geothermal water samples of the Eastern Snake River Plain and surrounding area. The samples included in this dataset were collected during the springs and summers of 2014 and 2015. All chemical analysis of the samples were conducted in the Analytical Laboratory at the Center of Advanced Energy Studies in Idaho Falls, Idaho. This data set supersedes #425 submission and is the final submission for AOP 3.1.2.1 for INL. Isotopic data collected by Mark Conrad will be submitted in a separate file.

  16. Analysis of gas centrifuge cascade for separation of multicomponent isotopes and optimal feed position

    SciTech Connect (OSTI)

    Chuntong Ying; Hongjiang Wu; Mingsheng Zhou; Yuguang Nie; Guangjun Liu

    1997-10-01

    Analysis of the concentration distribution in a gas centrifuge cascade for separation of multicomponent isotope mixtures is different from that in a cascade for separation of two-component mixtures. This paper presents the governing equations for a multicomponent isotope separation cascade. Numerically predicted separation factors for the gas centrifuge cascade agree well with the experimental data. A theoretical optimal feed position is derived for a short square cascade for a two-component mixture in a close-separation case. The optimal feed position for a gas centrifuge cascade for separation of multicomponent mixture is discussed.

  17. Development of high through-put Sr isotope analysis for monitoring reservoir integrity for CO{sub 2} storage.

    SciTech Connect (OSTI)

    Wall, Andy; Jain, Jinesh; Stewart, Brian; Capo, Rosemary; Hakala, Alexandra J.; Hammack, Richard; Guthrie, George

    2012-01-01

    Recent innovations in multi-collector ICP-mass spectrometry (MC-ICP-MS) have allowed for rapid and precise measurements of isotope ratios in geological samples. Naturally occurring Sr isotopes has the potential for use in Monitoring, Verification, and Accounting (MVA) associated with geologic CO2 storage. Sr isotopes can be useful for: Sensitive tracking of brine migration; Determining seal rock leakage; Studying fluid/rock reactions. We have optimized separation chemistry procedures that will allow operators to prepare samples for Sr isotope analysis off site using rapid, low cost methods.

  18. Improved Geothermometry Through Multivariate Reaction-path Modeling and Evaluation of Geomicrobiological Influences on Geochemical Temperature Indicators: Final Report

    SciTech Connect (OSTI)

    Mattson, Earl; Smith, Robert; Fujita, Yoshiko; McLing, Travis; Neupane, Ghanashyam; Palmer, Carl; Reed, David; Thompson, Vicki

    2015-03-01

    The project was aimed at demonstrating that the geothermometric predictions can be improved through the application of multi-element reaction path modeling that accounts for lithologic and tectonic settings, while also accounting for biological influences on geochemical temperature indicators. The limited utilization of chemical signatures by individual traditional geothermometer in the development of reservoir temperature estimates may have been constraining their reliability for evaluation of potential geothermal resources. This project, however, was intended to build a geothermometry tool which can integrate multi-component reaction path modeling with process-optimization capability that can be applied to dilute, low-temperature water samples to consistently predict reservoir temperature within ±30 °C. The project was also intended to evaluate the extent to which microbiological processes can modulate the geochemical signals in some thermal waters and influence the geothermometric predictions.

  19. Elemental and isotopic analysis of inorganic salts by laser desorption ionization mass spectrometry

    SciTech Connect (OSTI)

    Jayasekharan, T.; Sahoo, N. K.

    2013-02-05

    Laser desorption ionization mass spectrometry is applied for the analysis of elements as well as their isotopic composition in different inorganic salts. At very low laser energies the inorganic ions are desorbed and ionized from the thin layer of the sample surface. The naturally occurring isotopes of alkali and silver ions are resolved using time of flight mass spectrometer. Further increase in laser energy shows the appearance of Al, Cr, and Fe ions in the mass spectra. This indicates the penetration laser beam beyond the sample surface leading to the ablation of sample target at higher energies. The simultaneous appearance of atomic ions from the sample target at relatively higher laser energies hampers the unambiguous identification of amino acid residues from the biomolecular ions in MALDI-MS.

  20. ANALYSIS OF RICIN TOXIN PREPARATIONS FOR CARBOHYDRATE AND FATTY ACID ABUNDANCE AND ISOTOPE RATIO INFORMATION

    SciTech Connect (OSTI)

    Wunschel, David S.; Kreuzer-Martin, Helen W.; Antolick, Kathryn C.; Colburn, Heather A.; Moran, James J.; Melville, Angela M.

    2009-12-01

    This report describes method development and preliminary evaluation for analyzing castor samples for signatures of purifying ricin. Ricin purification from the source castor seeds is essentially a problem of protein purification using common biochemical methods. Indications of protein purification will likely manifest themselves as removal of the non-protein fractions of the seed. Two major, non-protein, types of biochemical constituents in the seed are the castor oil and various carbohydrates. The oil comprises roughly half the seed weight while the carbohydrate component comprises roughly half of the remaining mash left after oil and hull removal. Different castor oil and carbohydrate components can serve as indicators of specific toxin processing steps. Ricinoleic acid is a relatively unique fatty acid in nature and is the most abundant component of castor oil. The loss of ricinoleic acid indicates a step to remove oil from the seeds. The relative amounts of carbohydrates and carbohydrate-like compounds, including arabinose, xylose, myo-inositol fucose, rhamnose, glucosamine and mannose detected in the sample can also indicate specific processing steps. For instance, the differential loss of arabinose relative to mannose and N-acetyl glucosamine indicates enrichment for the protein fraction of the seed using protein precipitation. The methods developed in this project center on fatty acid and carbohydrate extraction from castor samples followed by derivatization to permit analysis by gas chromatography-mass spectrometry (GC-MS). Method descriptions herein include: the source and preparation of castor materials used for method evaluation, the equipment and description of procedure required for chemical derivatization, and the instrument parameters used in the analysis. Two types of derivatization methods describe analysis of carbohydrates and one procedure for analysis of fatty acids. Two types of GC-MS analysis is included in the method development, one

  1. Using phylogenetic probes for quantification of stable isotope labeling and microbial community analysis

    DOE Patents [OSTI]

    Brodie, Eoin L; DeSantis, Todd Z; Karaoz, Ulas; Andersen, Gary L

    2014-12-09

    Herein is described methods for a high-sensitivity means to measure the incorporation of stable isotope labeled substrates into RNA following stable isotope probing experiments (SIP). RNA is hybridized to a set of probes such as phylogenetic microarrays and isotope incorporation is quantified such as by secondary ion mass spectrometer imaging (NanoSIMS).

  2. {sup 39}Ar Detection at the 10{sup -16} Isotopic Abundance Level with Atom Trap Trace Analysis

    SciTech Connect (OSTI)

    Jiang, W.; Williams, W.; Bailey, K.; O'Connor, T. P.; Mueller, P.; Davis, A. M.; Hu, S.-M.; Sun, Y. R.; Lu, Z.-T.; Purtschert, R.; Sturchio, N. C.

    2011-03-11

    Atom trap trace analysis, a laser-based atom counting method, has been applied to analyze atmospheric {sup 39}Ar (half-life=269 yr), a cosmogenic isotope with an isotopic abundance of 8x10{sup -16}. In addition to the superior selectivity demonstrated in this work, the counting rate and efficiency of atom trap trace analysis have been improved by 2 orders of magnitude over prior results. The significant applications of this new analytical capability lie in radioisotope dating of ice and water samples and in the development of dark matter detectors.

  3. I ISOTOPES

    Office of Legacy Management (LM)

    fl6-6 ' , WTELEEYNE I ISOTOPES i - ' 50<77 /,' y. 6 IWL-5025-473 SUBSURFACE URASIUM OJ: THE GROUNDS OF NL BEARINGS, ALBAh'Y Heyitt Iv. Jeter Douglas M. Eagleson Fred J. Frullo TELEDYNE ISOTOPES 50 VAK BUREN A\!EMJE WESTKOOD, NEK JERSEY 07675 7 Dcccmhcr 1953 Prepnrcd for NL f%carings/NL Tndustrics, Inc. 1130 CCVltrill AXr~lMIC Allmy, New York 12205 TABLE OF CONTEhTS 1.0 INTRODUCTION 2.0 METHODS 2.1 Soil Sampling 2.2 Sample Preparation 2.3 Analysis of Samples 3.0 RESULTS 4.0 SUMMARY REFERENCES

  4. Isotopic Analysis of Spent Nuclear Fuel with an Ultra-High Rate HPGe Spectrometer

    SciTech Connect (OSTI)

    Fast, James E.; Glasgow, Brian D.; Rodriguez, Douglas C.; VanDevender, Brent A.; Wood, Lynn S.

    2014-06-06

    A longstanding challenge is the assay of spent nuclear fuel (SNF). Determining the isotopic content of SNF requires gamma-ray spectroscopy. PNNL has developed new digital filtering and analysis techniques to produce an ultra high-rate gamma-ray spectrometer from a standard coaxial high-purity germanium (HPGe) crystal. This ~40% efficient detector has been operated for SNF measurements at a throughput of about 400k gamma-ray counts per second (kcps) at an input rate of 1.3 Mcps. Optimized filtering algorithms preserve the spectroscopic capability of the system even at these high rates. This talk will present the results of a SNF measurement with aged SNF pellets at PNNL’s Radiochemical Processing Laboratory, first results with a FPGA front end processor capable of processing the data in real time, and the development path toward a multi-element system to assay fuel assemblies.

  5. FRAM isotopic analysis of uranium in thick-walled containers using high energy gamma rays and planar HPGe detectors.

    SciTech Connect (OSTI)

    Sampson, Thomas E.; Hypes, P. A.; Vo, Duc T.

    2002-01-01

    We describe the use of the Los Alamos FRAM isotopic analysis software to make the first reported measurements on thick-walled UF{sub 6} cylinders using small planar HPGe detectors of the type in common use at the IAEA. Heretofore, planar detector isotopic analysis measurements on uranium have used the 100-keV region and can be defeated by 10 mm of steel absorber. The analysis of planar detector measurements through 13-16 mm of steel shows that FRAM can successfully carry out these measurements and analysis in the 120-1024 keV energy range, a range previously thought to be the sole province of more efficient coaxial detectors. This paper describes the measurement conditions and results and also compares the results to other FRAM measurements with coaxial HPGe detectors. The technique of gamma-ray isotopic analysis of arbitrary samples is desirable for measuring the isotopic composition of uranium in UF{sub 6} cylinders because it does not require calibration with standards or knowledge of the cylinder wall thickness. The International Atomic Energy Agency (IAEA) uses the MGAU (Multi Group Analysis Uranium) uranium isotopic analysis software with planar high purity germanium (HPGe) detectors to measure the isotopic composition of uranium. Measurements on UF{sub 6} cylinders with 13-16-mm thick steel walls are usually unsuccessful because of the strong absorption of the 89-100 keV gamma rays and x-rays that MGAU requires for the measurement. This paper describes the use of the Los Alamos FRAM isotopic analysis software to make these measurements on UF{sub 6} cylinders. Uranium measurements with FRAM typically cover the energy range from 120-1001 keV and can easily be made through the walls of UF{sub 6} cylinders. While these measurements are usually performed with efficient coaxial HPGe detectors, this paper reports the first successful measurements using small planar HPGe detectors of the type in common use at the IAEA.

  6. Atomic line emission analyzer for hydrogen isotopes (Patent)...

    Office of Scientific and Technical Information (OSTI)

    Atomic line emission analyzer for hydrogen isotopes Title: Atomic line emission analyzer for hydrogen isotopes Apparatus for isotopic analysis of hydrogen comprises a low pressure ...

  7. A system analysis computer model for the High Flux Isotope Reactor (HFIRSYS Version 1)

    SciTech Connect (OSTI)

    Sozer, M.C.

    1992-04-01

    A system transient analysis computer model (HFIRSYS) has been developed for analysis of small break loss of coolant accidents (LOCA) and operational transients. The computer model is based on the Advanced Continuous Simulation Language (ACSL) that produces the FORTRAN code automatically and that provides integration routines such as the Gear`s stiff algorithm as well as enabling users with numerous practical tools for generating Eigen values, and providing debug outputs and graphics capabilities, etc. The HFIRSYS computer code is structured in the form of the Modular Modeling System (MMS) code. Component modules from MMS and in-house developed modules were both used to configure HFIRSYS. A description of the High Flux Isotope Reactor, theoretical bases for the modeled components of the system, and the verification and validation efforts are reported. The computer model performs satisfactorily including cases in which effects of structural elasticity on the system pressure is significant; however, its capabilities are limited to single phase flow. Because of the modular structure, the new component models from the Modular Modeling System can easily be added to HFIRSYS for analyzing their effects on system`s behavior. The computer model is a versatile tool for studying various system transients. The intent of this report is not to be a users manual, but to provide theoretical bases and basic information about the computer model and the reactor.

  8. Isotope Enrichment Detection by Laser Ablation - Laser Absorption Spectrometry: Automated Environmental Sampling and Laser-Based Analysis for HEU Detection

    SciTech Connect (OSTI)

    Anheier, Norman C.; Bushaw, Bruce A.

    2010-01-01

    The global expansion of nuclear power, and consequently the uranium enrichment industry, requires the development of new safeguards technology to mitigate proliferation risks. Current enrichment monitoring instruments exist that provide only yes/no detection of highly enriched uranium (HEU) production. More accurate accountancy measurements are typically restricted to gamma-ray and weight measurements taken in cylinder storage yards. Analysis of environmental and cylinder content samples have much higher effectiveness, but this approach requires onsite sampling, shipping, and time-consuming laboratory analysis and reporting. Given that large modern gaseous centrifuge enrichment plants (GCEPs) can quickly produce a significant quantity (SQ ) of HEU, these limitations in verification suggest the need for more timely detection of potential facility misuse. The Pacific Northwest National Laboratory (PNNL) is developing an unattended safeguards instrument concept, combining continuous aerosol particulate collection with uranium isotope assay, to provide timely analysis of enrichment levels within low enriched uranium facilities. This approach is based on laser vaporization of aerosol particulate samples, followed by wavelength tuned laser diode spectroscopy to characterize the uranium isotopic ratio through subtle differences in atomic absorption wavelengths. Environmental sampling (ES) media from an integrated aerosol collector is introduced into a small, reduced pressure chamber, where a focused pulsed laser vaporizes material from a 10 to 20-m diameter spot of the surface of the sampling media. The plume of ejected material begins as high-temperature plasma that yields ions and atoms, as well as molecules and molecular ions. We concentrate on the plume of atomic vapor that remains after the plasma has expanded and then cooled by the surrounding cover gas. Tunable diode lasers are directed through this plume and each isotope is detected by monitoring absorbance

  9. Capillary absorption spectrometer and process for isotopic analysis of small samples

    DOE Patents [OSTI]

    Alexander, M. Lizabeth; Kelly, James F.; Sams, Robert L.; Moran, James J.; Newburn, Matthew K.; Blake, Thomas A.

    2016-03-29

    A capillary absorption spectrometer and process are described that provide highly sensitive and accurate stable absorption measurements of analytes in a sample gas that may include isotopologues of carbon and oxygen obtained from gas and biological samples. It further provides isotopic images of microbial communities that allow tracking of nutrients at the single cell level. It further targets naturally occurring variations in carbon and oxygen isotopes that avoids need for expensive isotopically labeled mixtures which allows study of samples taken from the field without modification. The method also permits sampling in vivo permitting real-time ambient studies of microbial communities.

  10. The Multi-Isotope Process Monitor: Multivariate Analysis of Gamma Spectra

    SciTech Connect (OSTI)

    Orton, Christopher R.; Rutherford, Crystal E.; Fraga, Carlos G.; Schwantes, Jon M.

    2011-10-30

    The International Atomic Energy Agency (IAEA) has established international safeguards standards for fissionable material at spent fuel reprocessing plants to ensure that significant quantities of nuclear material are not diverted from these facilities. Currently, methods to verify material control and accountancy (MC&A) at these facilities require time-consuming and resource-intensive destructive assay (DA). The time delay between sampling and subsequent DA provides a potential opportunity to divert the material out of the appropriate chemical stream. Leveraging new on-line nondestructive assay (NDA) techniques in conjunction with the traditional and highly precise DA methods may provide a more timely, cost-effective and resource efficient means for MC&A verification at such facilities. Pacific Northwest National Laboratory (PNNL) is developing on-line NDA process monitoring technologies, including the Multi-Isotope Process (MIP) Monitor. The MIP Monitor uses gamma spectroscopy and pattern recognition software to identify off-normal conditions in process streams. Recent efforts have been made to explore the basic limits of using multivariate analysis techniques on gamma-ray spectra. This paper will provide an overview of the methods and report our on-going efforts to develop and demonstrate the technology.

  11. GUM Analysis for SIMS Isotopic Ratios in BEP0 Graphite Qualification Samples, Round 2

    SciTech Connect (OSTI)

    Gerlach, David C.; Heasler, Patrick G.; Reid, Bruce D.

    2009-01-01

    This report describes GUM calculations for TIMS and SIMS isotopic ratio measurements of reactor graphite samples. These isotopic ratios are used to estimate reactor burn-up, and currently consist of various ratios of U, Pu, and Boron impurities in the graphite samples. The GUM calculation is a propagation of error methodology that assigns uncertainties (in the form of standard error and confidence bound) to the final estimates.

  12. Isotopic Analysis of Uranium in NIST SRM Glass by Femtosecond Laser Ablation

    SciTech Connect (OSTI)

    Duffin, Andrew M.; Hart, Garret L.; Hanlen, Richard C.; Eiden, Gregory C.

    2013-05-19

    We employed femtosecond Laser Ablation Multicollector Inductively Coupled Mass Spectrometry for the 11 determination of uranium isotope ratios in a series of standard reference material glasses (NIST 610, 612, 614, and 12 616). This uranium concentration in this series of SRM glasses is a combination of isotopically natural uranium in 13 the materials used to make the glass matrix and isotopically depleted uranium added to increase the uranium 14 elemental concentration across the series. Results for NIST 610 are in excellent agreement with literature values. 15 However, other than atom percent 235U, little information is available for the remaining glasses. We present atom 16 percent and isotope ratios for 234U, 235U, 236U, and 238U for all four glasses. Our results show deviations from the 17 certificate values for the atom percent 235U, indicating the need for further examination of the uranium isotopes in 18 NIST 610-616. Our results are fully consistent with a two isotopic component mixing between the depleted 19 uranium spike and natural uranium in the bulk glass.

  13. Isotope Science

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Science and Production 35 years of experience in isotope production, processing, and applications. Llllll Committed to the safe and reliable production of radioisotopes, products, and services. Contact: Kevin John LANL Isotope Program Manager kjohn@lanl.gov 505-667-3602 Sponsored by the Department of Energy National Isotope Program http://www.nuclear.energy.gov/isotopes/nelsotopes2a.html Isotopes for Environmental Science Isotopes produced at Los Alamos National Laboratory are used as

  14. Isotopes Products

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Other isotopes that have recently shipped from LANL's isotope program include cadmium-109 (X-ray fluorescence sources), arsenic-72 (medical research), and sodium-22 (PET sources).

  15. Analysis of burnup and isotopic compositions of BWR 9 x 9 UO{sub 2} fuel assemblies

    SciTech Connect (OSTI)

    Suzuki, M.; Yamamoto, T.; Ando, Y.; Nakajima, T.

    2012-07-01

    In order to extend isotopic composition data focusing on fission product nuclides, measurements are progressing using facilities of JAEA for five samples taken from high burnup BWR 9 x 9 UO{sub 2} fuel assemblies. Neutronics analysis with an infinite assembly model was applied to the preliminary measurement data using a continuous-energy Monte Carlo burnup calculation code MVP-BURN with nuclear libraries based on JENDL-3.3 and JENDL-4.0. The burnups of the samples were determined to be 28.0, 39.3, 56.6, 68.1, and 64.0 GWd/t by the Nd-148 method. They were compared with those calculated using node-average irradiation histories of power and in-channel void fractions which were taken from the plant data. The comparison results showed that the deviations of the calculated burnups from the measurements were -4 to 3%. It was confirmed that adopting the nuclear data library based on JENDL-4.0 reduced the deviations of the calculated isotopic compositions from the measurements for {sup 238}Pu, {sup 144}Nd, {sup 145}Nd, {sup 146}Nd, {sup 148}Nd, {sup 134}Cs, {sup 154}Eu, {sup 152}Sm, {sup 154}Gd, and {sup 157}Gd. On the other hand, the effect of the revision in the nuclear. data library on the neutronics analysis was not significant for major U and Pu isotopes. (authors)

  16. Time-series analysis of ion and isotope geochemistry of selected springs of the Nevada Test Site, Nye County, Nevada

    SciTech Connect (OSTI)

    Lyles, B.F.; Edkins, J.; Jacobson, R.L.; Hess, J.W.

    1990-11-01

    The temporal variations of ion and isotope geochemistry were observed at six selected springs on the Nevada Test Site, Nye County, Nevada and included: Cane, Whiterock, Captain Jack, Topopah, Tippipah, and Oak Springs. The sites were monitored from 1980 to 1982 and the following parameters were measured: temperature, pH, electrical conductance, discharge, cations (Ca{sup 2+}, Mg{sup 2+}. Na{sup +}, K{sup +}), anions Cl{sup {minus}}, SO{sub 4}{sup 2{minus}}. HCO{sub 3}{sup {minus}}, silica, stable isotopes ({delta}{sup 18}O, {delta}D, {delta}{sup 13}C), and radioactive isotopes ({sup 3}H, {sup 14}C). A more detailed study was continued from 1982 to 1988 at Cane and Whiterock Springs. Field microloggers were installed at these sites in 1985 to measure the high frequency response of temperature, electrical conductance, and discharge to local precipitation. Stage fluctuations near the discharge point dissolve minerals/salts as groundwater inundates the mineralized zone immediately above the equilibrium water table. This phenomena was most noticeable at Whiterock Spring and lagged the discharge response by several hours. Stable isotope analysis of precipitation and groundwater suggests a 1.5 to 2 month travel time for meteoric water to migrate from the recharge area to the discharge point. Groundwater age determinations suggest a mean age of approximately 30 years at Whiterock Spring and possibly older at Cane Spring. However, the short travel time and geochemical integrity of recharge pulses suggest that the waters are poorly mixed along the flow paths. 25 refs., 25 figs., 24 tabs.

  17. PRINCIPAL ISOTOPE SELECTION REPORT

    SciTech Connect (OSTI)

    K. D. Wright

    1998-08-28

    Utilizing nuclear fuel to produce power in commercial reactors results in the production of hundreds of fission product and transuranic isotopes in the spent nuclear fuel (SNF). When the SNF is disposed of in a repository, the criticality analyses could consider all of the isotopes, some principal isotopes affecting criticality, or none of the isotopes, other than the initial loading. The selected set of principal isotopes will be the ones used in criticality analyses of the SNF to evaluate the reactivity of the fuel/waste package composition and configuration. This technical document discusses the process used to select the principal isotopes and the possible affect that these isotopes could have on criticality in the SNF. The objective of this technical document is to discuss the process used to select the principal isotopes for disposal criticality evaluations with commercial SNF. The principal isotopes will be used as supporting information in the ''Disposal Criticality Analysis Methodology Topical Report'' which will be presented to the United States Nuclear Regulatory Commission (NRC) when approved by the United States Department of Energy (DOE) Office of Civilian Radioactive Waste Management (OCRWM).

  18. Isotopic hydrogen analysis via conventional and surface-enhanced fiber optic Raman spectroscopy

    SciTech Connect (OSTI)

    LASCOLA, ROBERT

    2004-09-23

    This report describes laboratory development and process plant applications of Raman spectroscopy for detection of hydrogen isotopes in the Tritium Facilities at the Savannah River Site (SRS), a U.S. Department of Energy complex. Raman spectroscopy provides a lower-cost, in situ alternative to mass spectrometry techniques currently employed at SRS. Using conventional Raman and fiber optics, we have measured, in the production facility glove boxes, process mixtures of protium and deuterium at various compositions and total pressures ranging from 1000-4000 torr, with detection limits ranging from 1-2 percent for as low as 3-second integration times. We are currently investigating fabrication techniques for SERS surfaces in order to measure trace (0.01-0.1 percent) amounts of one isotope in the presence of the other. These efforts have concentrated on surfaces containing palladium, which promotes hydrogen dissociation and forms metal hydride bonds, essentially providing a chemical enhancement mechanism.

  19. A Capillary Absorption Spectrometer for Stable Carbon Isotope Ratio (13C/12C) Analysis in Very Small Samples

    SciTech Connect (OSTI)

    Kelly, James F.; Sams, Robert L.; Blake, Thomas A.; Newburn, Matthew K.; Moran, James J.; Alexander, M. L.; Kreuzer, Helen W.

    2012-02-06

    A capillary absorption spectrometer (CAS) suitable for IR laser isotope analysis of small CO{sub 2} samples is presented. The system employs a continuous-wave (cw) quantum cascade laser to study nearly adjacent rovibrational transitions of different isotopologues of CO{sub 2} near 2307 cm{sup -1} (4.34 {mu}m). This initial CAS system can achieve relative isotopic precision of about 10 ppm {sup 13}C, or {approx}1{per_thousand} (per mil in delta notation relative to Vienna Pee Dee Belemnite) with 20-100 picomoles of entrained sample within the hollow waveguide for CO{sub 2} concentrations {approx}400 to 750 ppm. Isotopic analyses of such gas fills in a 1-mm ID hollow waveguide of 0.8 m overall physical path length can be carried out down to {approx}2 Torr. Overall {sup 13}C/{sup 12}C ratios can be calibrated to {approx}2{per_thousand} accuracy with diluted CO{sub 2} standards. A novel, low-cost method to reduce cw-fringing noise resulting from multipath distortions in the hollow waveguide is presented, which allows weak absorbance features to be studied at the few ppm level (peak-to-rms) after 1,000 scans are co-added in {approx}10 sec. The CAS is meant to work directly with converted CO{sub 2} samples from a Laser Ablation-Catalytic-Combustion (LA CC) micro-sampler to provide {sup 13}C/{sup 12}C ratios of small biological isolates with spatial resolutions {approx}50 {mu}m.

  20. Evaluation of Groundwater Movement in the Frenchman Flat CAU Using Geochemical and Isotopic Analysis

    SciTech Connect (OSTI)

    R. Hershey; J. Thomas; T. Rose; J. Paces; I. Farnham; C. Benedict, Jr.

    2005-03-01

    The principal pathway for radionuclide migration from underground tests in Frenchman Flat, on the Nevada Test Site, to the accessible environment is groundwater flow. Two potential pathways for radionuclide transport via groundwater have been identified from hydrologic data: (1) radionuclide transport downward from the alluvial and volcanic aquifers into the underlying carbonate aquifer; and (2) radionuclide transport laterally to the carbonate aquifer surrounding Frenchman Flat. This report presents an evaluation of geochemical and environmental isotopic data to test these potential pathways and to identify other groundwater flowpaths in, and out of, Frenchman Flat.

  1. High Flux Isotope Reactor Core Analysis-Challenges and Recent Enhancements in Modeling and Simulation

    SciTech Connect (OSTI)

    Ilas, Germina

    2016-01-01

    A concerted effort over the past few years has focused on enhancing the core depletion models for the High Flux Isotope Reactor (HFIR) as part of a comprehensive study for designing a HFIR core that would use low-enriched uranium (LEU) fuel. A HFIR core depletion model that is based on current state-of-the-art methods and nuclear data was needed for use as a reference for the design of an LEU fuel for HFIR and to improve the basis for analyses that support HFIR s current operation with high-enriched uranium (HEU) fuel. This paper summarizes the recent improvements in modeling and simulation for HFIR core analyses, with a focus on core depletion models.

  2. Isotope separation

    DOE Patents [OSTI]

    Bartlett, Rodney J.; Morrey, John R.

    1978-01-01

    A method and apparatus is described for separating gas molecules containing one isotope of an element from gas molecules containing other isotopes of the same element in which all of the molecules of the gas are at the same electronic state in their ground state. Gas molecules in a gas stream containing one of the isotopes are selectively excited to a different electronic state while leaving the other gas molecules in their original ground state. Gas molecules containing one of the isotopes are then deflected from the other gas molecules in the stream and thus physically separated.

  3. Analysis of Experimental Data for High Burnup PWR Spent Fuel Isotopic Validation - Vandellos II Reactor

    SciTech Connect (OSTI)

    Ilas, Germina; Gauld, Ian C

    2011-01-01

    This report is one of the several recent NUREG/CR reports documenting benchmark-quality radiochemical assay data and the use of the data to validate computer code predictions of isotopic composition for spent nuclear fuel, to establish the uncertainty and bias associated with code predictions. The experimental data analyzed in the current report were acquired from a high-burnup fuel program coordinated by Spanish organizations. The measurements included extensive actinide and fission product data of importance to spent fuel safety applications, including burnup credit, decay heat, and radiation source terms. Six unique spent fuel samples from three uranium oxide fuel rods were analyzed. The fuel rods had a 4.5 wt % {sup 235}U initial enrichment and were irradiated in the Vandellos II pressurized water reactor operated in Spain. The burnups of the fuel samples range from 42 to 78 GWd/MTU. The measurements were used to validate the two-dimensional depletion sequence TRITON in the SCALE computer code system.

  4. Isotope geochemistry

    SciTech Connect (OSTI)

    Cole, D.R.; Curtis, D.B.; DePaolo, D.J.; Gerlach, T.M.; Laul, J.C.; Shaw, H.; Smith, B.M.; Sturchio, N.C.

    1990-09-01

    This document represents the consensus of members of the ad hoc Committee on Isotope Geochemistry in the US Department of Energy; the committee is composed of researchers in isotope geochemistry from seven of the national laboratories. Information included in this document was presented at workshops at Lawrence Berkeley Laboratory (April 1989) and at Los Alamos National Laboratory (August 1989).

  5. GADRAS isotope ID users manual for analysis of gamma-ray measurements and API for Linux and Android .

    SciTech Connect (OSTI)

    Mitchell, Dean J; Harding, Lee T.

    2014-05-01

    Isotope identification algorithms that are contained in the Gamma Detector Response and Analysis Software (GADRAS) can be used for real-time stationary measurement and search applications on platforms operating under Linux or Android operating sys-tems. Since the background radiation can vary considerably due to variations in natu-rally-occurring radioactive materials (NORM), spectral algorithms can be substantial-ly more sensitive to threat materials than search algorithms based strictly on count rate. Specific isotopes or interest can be designated for the search algorithm, which permits suppression of alarms for non-threatening sources, such as such as medical radionuclides. The same isotope identification algorithms that are used for search ap-plications can also be used to process static measurements. The isotope identification algorithms follow the same protocols as those used by the Windows version of GADRAS, so files that are created under the Windows interface can be copied direct-ly to processors on fielded sensors. The analysis algorithms contain provisions for gain adjustment and energy lineariza-tion, which enables direct processing of spectra as they are recorded by multichannel analyzers. Gain compensation is performed by utilizing photopeaks in background spectra. Incorporation of this energy calibration tasks into the analysis algorithm also eliminates one of the more difficult challenges associated with development of radia-tion detection equipment.

  6. GUM Analysis for TIMS Isotopic Ratios in BEP0 Graphite Qualification Samples, Round 2

    SciTech Connect (OSTI)

    Gerlach, David C.; Heasler, Patrick G.; Reid, Bruce D.

    2009-01-01

    In May 2007, one set of three samples from NBL were addressed to Steve Petersen for TIMS analysis, and included BEP0 samples numbered 27008, 30986, and 50846. All cores were trimmed by tooling, and lightly cleaned by CO2 pellet blasting. Small discs were cut from the second set of samples for SIMS analysis, with the remainder of each used for TIMS preparation.

  7. Isotopes Products

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Isotopes Products Isotopes Products Isotopes produced at Los Alamos National Laboratory are saving lives, advancing cutting-edge research and keeping the U.S. safe. Products stress and rest Stress and rest Rb-82 PET images in a patient with dipyridamole stress-inducible lateral wall and apical ischemia. (http://www.fac.org.ar/scvc/llave/image/machac/machaci.htm#f2,3,4) Strontium-82 is supplied to our customers for use in Sr-82/Rb-82 generator technologies. The generators in turn are supplied to

  8. Geochemistry and Isotopes of Fluids from Sulphur Springs, Valles...

    Open Energy Info (EERE)

    >Non-condensible gases consist of roughly 99% CO2 with minor amounts of H2S, H2, and CH4. Empirical gas geothermometry suggests a deep reservoir temperature of 215 to 280C....

  9. International Workshop on Gamma Spectrometry Analysis Codes for U and Pu Isotopics: Workshop Results and Next Steps

    SciTech Connect (OSTI)

    McGinnis, Brent R; Solodov, Alexander A; Shipwash, Jacqueline L; Zhernosek, Alena V; McKinney, Teressa L; Pickett, Chris A; Peerani, Paolo

    2009-01-01

    In November 2008, the Institute of Nuclear Materials Management (INMM) and the European Safeguards Research and Development Association (ESARDA) co-hosted the International Workshop on Gamma Spectrometry Analysis Codes for U and Pu Isotopics at the Oak Ridge National Laboratory (ORNL). This workshop was conducted in response to needs expressed by the international safeguards community to understand better the capabilities and limitations of the codes; to ensure these codes are sustained; and to ensure updates or revisions are performed in a controlled manner. The workshop was attended by approximately 100 participants. The participants included code developers, code suppliers, safeguards specialists, domestic and international inspectors, process operators, regulators, and programme sponsors from various government agencies. The workshop provided a unique opportunity for code developers, commercial distributors and end users to interact in a hands-on laboratory environment to develop solutions for programmatic and technical issues associated with the various codes. The workshop also provided an international forum for discussing development of an internationally accepted standard test method. This paper discusses the organization of the workshop, its goals and objectives and feedback received from the participants. The paper also describes the significance of the working group's contribution to improving codes that are commonly used during inspections to verify that nuclear facilities are compliant with treaty obligations that ensure nuclear fuel cycle facilities are used for peaceful purposes.

  10. Measuring SNM Isotopic Distributions using FRAM

    SciTech Connect (OSTI)

    Geist, William H.

    2015-12-02

    The first group of slides provides background information on the isotopic composition of plutonium. It is shown that 240Pu is the critical isotope in neutron coincidence/multiplicity counting. Next, response function analysis to determine isotopic composition is discussed. The isotopic composition can be determined by measuring the net peak counts from each isotope and then taking the ratio of the counts for each isotope relative to the total counts for the element. Then FRAM (Fixed energy Response function Analysis with Multiple efficiencies) is explained. FRAM can control data acquisition, automatically analyze newly acquired data, analyze previously acquired data, provide information on the quality of the analysis, and facilitate analysis in unusual situations (non-standard energy calibrations, gamma rays from non-SNM isotopes, poor spectra (within limits)).

  11. Transportation of medical isotopes

    SciTech Connect (OSTI)

    Nielsen, D.L.

    1997-11-19

    A Draft Technical Information Document (HNF-1855) is being prepared to evaluate proposed interim tritium and medical isotope production at the Fast Flux Test Facility (FFTF). This assessment examines the potential health and safety impacts of transportation operations associated with the production of medical isotopes. Incident-free and accidental impacts are assessed using bounding source terms for the shipment of nonradiological target materials to the Hanford Site, the shipment of irradiated targets from the FFTF to the 325 Building, and the shipment of medical isotope products from the 325 Building to medical distributors. The health and safety consequences to workers and the public from the incident-free transportation of targets and isotope products would be within acceptable levels. For transportation accidents, risks to works and the public also would be within acceptable levels. This assessment is based on best information available at this time. As the medical isotope program matures, this analysis will be revised, if necessary, to support development of a final revision to the Technical Information Document.

  12. ISOTOPE SEPARATORS

    DOE Patents [OSTI]

    Bacon, C.G.

    1958-08-26

    An improvement is presented in the structure of an isotope separation apparatus and, in particular, is concerned with a magnetically operated shutter associated with a window which is provided for the purpose of enabling the operator to view the processes going on within the interior of the apparatus. The shutier is mounted to close under the force of gravity in the absence of any other force. By closing an electrical circuit to a coil mouated on the shutter the magnetic field of the isotope separating apparatus coacts with the magnetic field of the coil to force the shutter to the open position.

  13. Supplement Analysis for the Programmatic Environmental Impact Statement (PEIS) for Accomplishing Expanded Civilian Nuclear Energy Research and Development and Isotope Production Missions in the United States, (DOE/EIS-0310-SA-01) (08/05/04)

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    0-SA-01 Supplement Analysis for the Programmatic Environmental Impact Statement (PEIS) for Accomplishing Expanded Civilian Nuclear Energy Research and Development and Isotope Production Missions in the United States, Including the Role of the Fast Flux Test Facility Introduction and Background The Department of Energy (DOE), pursuant to the National Environmental Policy Act (NEPA), issued the Final PEIS for Accomplishing Expanded Civilian Nuclear Energy Research and Development and Isotope

  14. Method for separating isotopes

    DOE Patents [OSTI]

    Jepson, B.E.

    1975-10-21

    Isotopes are separated by contacting a feed solution containing the isotopes with a cyclic polyether wherein a complex of one isotope is formed with the cyclic polyether, the cyclic polyether complex is extracted from the feed solution, and the isotope is thereafter separated from the cyclic polyether.

  15. Stable isotope studies

    SciTech Connect (OSTI)

    Ishida, T.

    1992-01-01

    The research has been in four general areas: (1) correlation of isotope effects with molecular forces and molecular structures, (2) correlation of zero-point energy and its isotope effects with molecular structure and molecular forces, (3) vapor pressure isotope effects, and (4) fractionation of stable isotopes. 73 refs, 38 figs, 29 tabs.

  16. Isotope separation by photochromatography

    DOE Patents [OSTI]

    Suslick, K.S.

    1975-10-03

    A photochromatographic method for isotope separation is described. An isotopically mixed molecular species is adsorbed on an adsorptive surface, and the adsorbed molecules are irradiated with radiation of a predetermined wavelength which will selectively excite desired isotopic species. Sufficient energy is transferred to the excited molecules to desorb them from the surface and thus separate them from the undesired isotopic species. The method is particularly applicable to the separation of hydrogen isotopes. (BLM)

  17. Isotope separation by photochromatography

    DOE Patents [OSTI]

    Suslick, Kenneth S.

    1977-01-01

    An isotope separation method which comprises physically adsorbing an isotopically mixed molecular species on an adsorptive surface and irradiating the adsorbed molecules with radiation of a predetermined wavelength which will selectively excite a desired isotopic species. Sufficient energy is transferred to the excited molecules to desorb them from the surface and thereby separate them from the unexcited undesired isotopic species. The method is particularly applicable to the separation of hydrogen isotopes.

  18. AVLIS enrichment of medical isotopes

    SciTech Connect (OSTI)

    Haynam, C.A.; Scheibner, K.F.; Stern, R.C.; Worden, E.F.

    1996-12-31

    Under the Sponsorship of the United states Enrichment Corporation (USEC), we are currently investigating the large scale separation of several isotopes of medical interest using atomic vapor isotope separation (AVLIS). This work includes analysis and experiments in the enrichment of thallium 203 as a precursor to the production of thallium 201 used in cardiac imaging following heart attacks, on the stripping of strontium 84 from natural strontium as precursor to the production of strontium 89, and on the stripping of lead 210 from lead used in integrated circuits to reduce the number of alpha particle induced logic errors.

  19. Manus Water Isotope Investigation

    Office of Scientific and Technical Information (OSTI)

    ENERGY Office of Science DOESC-ARM-15-079 Manus Water Isotope Investigation Field ... DOESC-ARM-15-079 Manus Water Isotope Investigation Field Campaign Report JL Conroy, ...

  20. Manus Water Isotope Investigation

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    9 Manus Water Isotope Investigation Field Campaign Report JL Conroy D Noone KM Cobb March ... DOESC-ARM-15-079 Manus Water Isotope Investigation Field Campaign Report JL Conroy, ...

  1. Isotope analysis of diamond-surface passivation effect of high-temperature H{sub 2}O-grown atomic layer deposition-Al{sub 2}O{sub 3} films

    SciTech Connect (OSTI)

    Hiraiwa, Atsushi E-mail: qs4a-hriw@asahi-net.or.jp; Saito, Tatsuya; Matsumura, Daisuke; Kawarada, Hiroshi

    2015-06-07

    The Al{sub 2}O{sub 3} film formed using an atomic layer deposition (ALD) method with trimethylaluminum as Al precursor and H{sub 2}O as oxidant at a high temperature (450?C) effectively passivates the p-type surface conduction (SC) layer specific to a hydrogen-terminated diamond surface, leading to a successful operation of diamond SC field-effect transistors at 400?C. In order to investigate this excellent passivation effect, we carried out an isotope analysis using D{sub 2}O instead of H{sub 2}O in the ALD and found that the Al{sub 2}O{sub 3} film formed at a conventional temperature (100?C) incorporates 50 times more CH{sub 3} groups than the high-temperature film. This CH{sub 3} is supposed to dissociate from the film when heated afterwards at a higher temperature (550?C) and causes peeling patterns on the H-terminated surface. The high-temperature film is free from this problem and has the largest mass density and dielectric constant among those investigated in this study. The isotope analysis also unveiled a relatively active H-exchange reaction between the diamond H-termination and H{sub 2}O oxidant during the high-temperature ALD, the SC still being kept intact. This dynamic and yet steady H termination is realized by the suppressed oxidation due to the endothermic reaction with H{sub 2}O. Additionally, we not only observed the kinetic isotope effect in the form of reduced growth rate of D{sub 2}O-oxidant ALD but found that the mass density and dielectric constant of D{sub 2}O-grown Al{sub 2}O{sub 3} films are smaller than those of H{sub 2}O-grown films. This is a new type of isotope effect, which is not caused by the presence of isotopes in the films unlike the traditional isotope effects that originate from the presence of isotopes itself. Hence, the high-temperature ALD is very effective in forming Al{sub 2}O{sub 3} films as a passivation and/or gate-insulation layer of high-temperature-operation diamond SC devices, and the knowledge of the

  2. Pathways and transformations of dissolved methane and dissolved inorganic carbon in Arctic tundra watersheds: Evidence from analysis of stable isotopes

    SciTech Connect (OSTI)

    Throckmorton, Heather M.; Heikoop, Jeffrey M.; Newman, Brent D.; Altmann, Garrett L.; Conrad, Mark S.; Muss, Jordan D.; Perkins, George B.; Smith, Lydia J.; Torn, Margaret S.; Wullschleger, Stan D.; Wilson, Cathy J.

    2015-11-08

    Arctic soils contain a large pool of terrestrial C and are of interest due to their potential for releasing significant carbon dioxide (CO2) and methane (CH4) to the atmosphere. Due to substantial landscape heterogeneity, predicting ecosystem-scale CH4 and CO2 production is challenging. This study assessed dissolved inorganic carbon (DIC = Σ (total) dissolved CO2) and CH4 in watershed drainages in Barrow, Alaska as critical convergent zones of regional geochemistry, substrates, and nutrients. In July and September of 2013, surface waters and saturated subsurface pore waters were collected from 17 drainages. Based on simultaneous DIC and CH4 cycling, we synthesized isotopic and geochemical methods to develop a subsurface CH4 and DIC balance by estimating mechanisms of CH4 and DIC production and transport pathways and oxidation of subsurface CH4. We observed a shift from acetoclastic (July) toward hydrogenotropic (September) methanogenesis at sites located toward the end of major freshwater drainages, adjacent to salty estuarine waters, suggesting an interesting landscape-scale effect on CH4 production mechanism. The majority of subsurface CH4 was transported upward by plant-mediated transport and ebullition, predominantly bypassing the potential for CH4 oxidation. Thus, surprisingly, CH4 oxidation only consumed approximately 2.51± 0.82% (July) and 0.79 ± 0.79% (September) of CH4 produced at the frost table, contributing to <0.1% of DIC production. DIC was primarily produced from respiration, with iron and organic matter serving as likely e- acceptors. Furthermore, this work highlights the importance of spatial and temporal variability of CH4 production at the watershed scale and suggests broad scale investigations are required to build better regional or pan-Arctic representations of CH

  3. High Flux Isotope Reactor | Neutron Science at ORNL

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    HFIR is also used for medical, industrial, and research isotope production; research on severe neutron damage to materials; and neutron activation analysis to examine trace ...

  4. ISOTOPE CONVERSION DEVICE

    DOE Patents [OSTI]

    Wigner, E.P.; Young, G.J.; Ohlinger, L.A.

    1957-12-01

    This patent relates to nuclear reactors of tbe type utilizing a liquid fuel and designed to convert a non-thermally fissionable isotope to a thermally fissionable isotope by neutron absorption. A tank containing a reactive composition of a thermally fissionable isotope dispersed in a liquid moderator is disposed within an outer tank containing a slurry of a non-thermally fissionable isotope convertible to a thermally fissionable isotope by neutron absorption. A control rod is used to control the chain reaction in the reactive composition and means are provided for circulating and cooling the reactive composition and slurry in separate circuits.

  5. Generation of Radixenon Isotopes

    SciTech Connect (OSTI)

    McIntyre, Justin I.; Bowyer, Ted W.; Hayes, James C.; Heimbigner, Tom R.; Morris, Scott J.; Panisko, Mark E.; Pitts, W. K.; Pratt, Sharon L.; Reeder, Paul L.; Thomas, Charles W.

    2003-06-30

    Pacific Northwest National Laboratory has developed an automated system for separating Xe from air and can detect the following radioxenon isotopes, 131mXe, 133mXe, 133Xe, and 135Xe. This report details the techniques used to generate the various radioxenon isotopes that are used for the calibration of the detector as well as other isotopes that have the potential to interfere with the fission produced radioxenon isotopes. Fission production is covered first using highly enriched uranium followed by a description and results from an experiment to produce radioxenon isotopes from neutron activation of ambient xenon.

  6. Conceptual Geologic Model and Native State Model of the Roosevelt...

    Open Energy Info (EERE)

    (Faulder, 1991) Geothermometry At Roosevelt Hot Springs Geothermal Area (Faulder, 1991) Ground Gravity Survey At Roosevelt Hot Springs Geothermal Area (Faulder, 1991) Isotopic...

  7. Compound and Elemental Analysis At Blackfoot Reservoir Area ...

    Open Energy Info (EERE)

    References Amy Hutsinpiller, W. T. Parry (1985) Geochemistry And Geothermometry Of Spring Water From The Blackfoot Reservoir Region, Southeastern Idaho Additional References...

  8. Compound and Elemental Analysis At Fenton Hill HDR Geothermal...

    Open Energy Info (EERE)

    Interactions in the Fenton Hill, New Mexico, Hot Dry Rock Geothermal Systems I. Fluid Mixing and Chemical Geothermometry Additional References Retrieved from "http:...

  9. HYDROGEN ISOTOPE TARGETS

    DOE Patents [OSTI]

    Ashley, R.W.

    1958-08-12

    The design of targets for use in the investigation of nuclear reactions of hydrogen isotopes by bombardment with accelerated particles is described. The target con struction eomprises a backing disc of a metal selected from the group consisting of molybdenunn and tungsten, a eoating of condensed titaniunn on the dise, and a hydrogen isotope selected from the group consisting of deuterium and tritium absorbed in the coatiag. The proeess for preparing these hydrogen isotope targets is described.

  10. Uranium Isotopic Assay Instrument

    SciTech Connect (OSTI)

    Anheier, Norman C.; Wojcik, Michael D.; Bushaw, Bruce A.

    2006-12-01

    The isotopic assay instrument under development at Pacific Northwest National Laboratory (PNNL) is capable of rapid prescreening to detect small and rare particles containing high concentrations of uranium in a heterogeneous sample. The isotopic measurement concept is based on laser vaporization of solid samples followed with sensitive isotope specific detection using either uranium atomic fluorescence emission or uranium atomic absorbance. Both isotopes are measured concurrently, following a single ablation laser pulse, using two external-cavity violet diode lasers. The simultaneous measurement of both isotopes enables the correlation of the fluorescence and absorbance signals on a shot-to-shot basis. This measurement approach demonstrated negligible channel crosstalk between isotopes. Rapid sample scanning provides high spatial resolution isotopic fluorescence and absorbance sample imagery of heterogeneous samples. Laser ablation combined with measurements of laser-induced fluorescence (LALIF) and through-plume laser absorbance (LAPLA) was applied to measure gadolinium isotope ratios in solid samples. Gadolinium has excitation wavelengths very close to the transitions of interest in uranium. Gadolinium has seven stable isotopes, and the natural 152Gd:160Gd ratio of 0.009 is in the range of what will be encountered for 235U:238U isotopic ratios. LAPLA measurements were demonstrated clearly using 152Gd (0.2% isotopic abundance) with a good signal-to-noise ratio. The ability to measure gadolinium abundances at this level indicates that measurements of 235U/238U isotopic ratios for natural (0.72%), depleted (0.25%), and low enriched uranium samples will be feasible.

  11. ARM - Measurement - Isotope ratio

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govMeasurementsIsotope ratio ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Isotope ratio Ratio of stable isotope concentrations. Categories Atmospheric State, Atmospheric Carbon Instruments The above measurement is considered scientifically relevant for the following instruments. Refer to the datastream (netcdf) file headers of each instrument for a list of all available measurements, including those

  12. Hybrid isotope separation scheme

    DOE Patents [OSTI]

    Maya, J.

    1991-06-18

    A method is described for yielding selectively a desired enrichment in a specific isotope including the steps of inputting into a spinning chamber a gas from which a scavenger, radiating the gas with a wave length or frequency characteristic of the absorption of a particular isotope of the atomic or molecular gas, thereby inducing a photochemical reaction between the scavenger, and collecting the specific isotope-containing chemical by using a recombination surface or by a scooping apparatus. 2 figures.

  13. Hybrid isotope separation scheme

    DOE Patents [OSTI]

    Maya, Jakob

    1991-01-01

    A method of yielding selectively a desired enrichment in a specific isotope including the steps of inputting into a spinning chamber a gas from which a scavenger, radiating the gas with a wave length or frequency characteristic of the absorption of a particular isotope of the atomic or molecular gas, thereby inducing a photochemical reaction between the scavenger, and collecting the specific isotope-containing chemical by using a recombination surface or by a scooping apparatus.

  14. Stable isotope enrichment

    ScienceCinema (OSTI)

    Egle, Brian

    2014-07-15

    Brian Egle is working to increase the nation's capacity to produce stable isotopes for use including medicine, industry and national security.

  15. Stable isotope enrichment

    SciTech Connect (OSTI)

    Egle, Brian

    2014-07-14

    Brian Egle is working to increase the nation's capacity to produce stable isotopes for use including medicine, industry and national security.

  16. Analysis of carbon-oxygen reactions by use of a square-input response technique and {sup 18}O isotope

    SciTech Connect (OSTI)

    Miura, Kouichi; Nakagawa, Hiroyuki

    1996-12-31

    Carbon gasification reaction has been investigated for decades including the pioneering works of Walker and his co-workers, but its mechanism has not been completely elucidated. The concept of the active surface area (ASA) was proposed by them, and its importance has been recognized. However, since ASA was measured by O{sub 2} chemisorption at below 300{degrees}C where carbon loss through gasification is negligible, it does not reflect the actual gasification situation. To overcome this weak point, measurements of ASA in a batch reactor and the so-called transient kinetic (TK) method were proposed. Ahmed and Back successfully measured the chemisorbed oxygen during the gasification using a batch reactor, and proposed a new mechanistic sequence for carbon-oxygen reaction which stresses the importance of the reaction between the gaseous oxygen and the chemisorbed oxygen. Radovic et al. proposed the concept of the reactive surface area (RSA), and reported excellent proportionality between the CO{sub 2} gasification rate and the RSA estimated by the TK and the TPD methods. Kapteijn et al. showed that the TK method with labeled molecules is more powerful to examine the mechanism. They found the presence of two types of surface oxygen complexes which desorb at different rates. A Square-input response (SIR) method is applied to the carbon-oxygen reaction. This method allows the observation of transient changes on two step changes. This method has been successfully applied to the analysis of a coal char gasification.

  17. Price Quotes and Isotope Ordering

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ordering Price Quotes and Isotope Ordering Isotopes produced at Los Alamos National Laboratory are saving lives, advancing cutting-edge research and keeping the U.S. safe. Isotope...

  18. Photochemical isotope separation

    DOE Patents [OSTI]

    Robinson, C.P.; Jensen, R.J.; Cotter, T.P.; Greiner, N.R.; Boyer, K.

    1987-04-28

    A process is described for separating isotopes by selective excitation of isotopic species of a volatile compound by tuned laser light. A highly cooled gas of the volatile compound is produced in which the isotopic shift is sharpened and defined. Before substantial condensation occurs, the cooled gas is irradiated with laser light precisely tuned to a desired wavelength to selectively excite a particular isotopic species in the cooled gas. The laser light may impart sufficient energy to the excited species to cause it to undergo photochemical reaction or even to photoionize. Alternatively, a two-photon irradiation may be applied to the cooled gas to induce photochemical reaction or photoionization. The process is particularly applicable to the separation of isotopes of uranium and plutonium. 8 figs.

  19. Laser isotope separation

    DOE Patents [OSTI]

    Robinson, C. Paul; Jensen, Reed J.; Cotter, Theodore P.; Boyer, Keith; Greiner, Norman R.

    1988-01-01

    A process and apparatus for separating isotopes by selective excitation of isotopic species of a volatile compound by tuned laser light. A highly cooled gas of the volatile compound is produced in which the isotopic shift is sharpened and defined. Before substantial condensation occurs, the cooled gas is irradiated with laser light precisely tuned to a desired wavelength to selectively excite a particular isotopic species in the cooled gas. The laser light may impart sufficient energy to the excited species to cause it to undergo photolysis, photochemical reaction or even to photoionize. Alternatively, a two-photon irradiation may be applied to the cooled gas to induce photolysis, photochemical reaction or photoionization. The process is particularly applicable to the separation of isotopes of uranium.

  20. Photochemical isotope separation

    DOE Patents [OSTI]

    Robinson, C. Paul; Jensen, Reed J.; Cotter, Theodore P.; Greiner, Norman R.; Boyer, Keith

    1987-01-01

    A process for separating isotopes by selective excitation of isotopic species of a volatile compound by tuned laser light. A highly cooled gas of the volatile compound is produced in which the isotopic shift is sharpened and defined. Before substantial condensation occurs, the cooled gas is irradiated with laser light precisely tuned to a desired wavelength to selectively excite a particular isotopic species in the cooled gas. The laser light may impart sufficient energy to the excited species to cause it to undergo photochemical reaction or even to photoionize. Alternatively, a two-photon irradiation may be applied to the cooled gas to induce photochemical reaction or photoionization. The process is particularly applicable to the separation of isotopes of uranium and plutonium.

  1. Laser isotope separation

    DOE Patents [OSTI]

    Robinson, C.P.; Reed, J.J.; Cotter, T.P.; Boyer, K.; Greiner, N.R.

    1975-11-26

    A process and apparatus for separating isotopes by selective excitation of isotopic species of a volatile compound by tuned laser light is described. A highly cooled gas of the volatile compound is produced in which the isotopic shift is sharpened and defined. Before substantial condensation occurs, the cooled gas is irradiated with laser light precisely tuned to a desired wavelength to selectively excite a particular isotopic species in the cooled gas. The laser light may impart sufficient energy to the excited species to cause it to undergo photolysis, photochemical reaction or even to photoionize. Alternatively, a two-photon irradiation may be applied to the cooled gas to induce photolysis, photochemical reaction or photoionization. The process is particularly applicable to the separation of isotopes of uranium.

  2. Determination of the origin of elevated uranium at a Former Air Force Landfill using non-parametric statistics analysis and uranium isotope ratio analysis

    SciTech Connect (OSTI)

    Weismann, J.; Young, C.; Masciulli, S.; Caputo, D.

    2007-07-01

    factors so that gross alpha action levels can be applied to future long-term landfill monitoring to track radiological conditions at lower cost. Ratios of isotopic uranium results were calculated to test whether the elevated uranium displayed signatures indicative of military use. Results of all ratio testing strongly supports the conclusion that the uranium found in groundwater, surface water, and sediment at OU 2 is naturally-occurring and has not undergone anthropogenic enrichment or processing. U-234:U-238 ratios also show that a disequilibrium state, i.e., ratio greater than 1, exists throughout OU 2 which is indicative of long-term aqueous transport in aged aquifers. These results all support the conclusion that the elevated uranium observed at OU 2 is due to the high concentrations in the regional watershed. Based on the results of this monitoring program, we concluded that the elevated uranium concentrations measured in OU 2 groundwater, surface water, and sediment are due to the naturally-occurring uranium content of the regional watershed and are not the result of waste burials in the former landfill. Several lines of evidence indicate that natural uranium has been naturally concentrated beneath OU 2 in the geologic past and the higher of uranium concentrations in down-gradient wells is the result of geochemical processes and not the result of a uranium ore disposal. These results therefore provide the data necessary to support radiological closure of OU 2. (authors)

  3. Science on Tap - Isotopes

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Science on Tap - Isotopes Science on Tap - Isotopes WHEN: Jun 16, 2016 5:30 PM - 7:00 PM WHERE: UnQuarked Wine Room 145 Central Park Square, Los Alamos, New Mexico 87544 USA CONTACT: Linda Anderman (505) 665-9196 CATEGORY: Bradbury INTERNAL: Calendar Login Event Description Short presentation followed by lively interaction on the topic at hand. While isotopes are chemical elements (think periodic table), their varying numbers of neutrons mean they can be used in lots of different way. Join us

  4. Atomic vapor laser isotope separation

    SciTech Connect (OSTI)

    Stern, R.C.; Paisner, J.A.

    1986-08-15

    The atomic vapor laser isotope separation (AVLIS) process for the enrichment of uranium is evaluated. (AIP)

  5. Plasma isotope separation methods

    SciTech Connect (OSTI)

    Grossman, M.W. ); Shepp, T.A. )

    1991-12-01

    Isotope separation has many important industrial, medical, and research applications. Large-scale processes have typically utilized complex cascade systems; for example, the gas centrifuge. Alternatively, high single-stage enrichment processes (as in the case of the calutron) are very energy intensive. Plasma-based methods being developed for the past 15 to 20 years have attempted to overcome these two drawbacks. In this review, six major types of isotope separation methods which involve plasma phenomena are discussed. These methods are: plasma centrifuge, AVLIS (atomic vapor laser isotope separation), ion wave, ICR (ion-cyclotron resonance), calutron, and gas discharge. The emphasis of this paper is to describe the plasma phenomena in these major categories. An attempt was made to include enough references so that more detailed study or evaluation of a particular method could readily be pursued. A brief discussion of isotope separation using mass balance concepts is also carried out.

  6. Separation of sulfur isotopes

    DOE Patents [OSTI]

    DeWitt, Robert; Jepson, Bernhart E.; Schwind, Roger A.

    1976-06-22

    Sulfur isotopes are continuously separated and enriched using a closed loop reflux system wherein sulfur dioxide (SO.sub.2) is reacted with sodium hydroxide (NaOH) or the like to form sodium hydrogen sulfite (NaHSO.sub.3). Heavier sulfur isotopes are preferentially attracted to the NaHSO.sub.3, and subsequently reacted with sulfuric acid (H.sub.2 SO.sub.4) forming sodium hydrogen sulfate (NaHSO.sub.4) and SO.sub.2 gas which contains increased concentrations of the heavier sulfur isotopes. This heavy isotope enriched SO.sub.2 gas is subsequently separated and the NaHSO.sub.4 is reacted with NaOH to form sodium sulfate (Na.sub.2 SO.sub.4) which is subsequently decomposed in an electrodialysis unit to form the NaOH and H.sub.2 SO.sub.4 components which are used in the aforesaid reactions thereby effecting sulfur isotope separation and enrichment without objectionable loss of feed materials.

  7. Atomic line emission analyzer for hydrogen isotopes

    DOE Patents [OSTI]

    Kronberg, James W.

    1993-01-01

    Apparatus for isotopic analysis of hydrogen comprises a low pressure chamber into which a sample of hydrogen is introduced and then exposed to an electrical discharge to excite the electrons of the hydrogen atoms to higher energy states and thereby cause the emission of light on the return to lower energy states, a Fresnel prism made at least in part of a material anomalously dispersive to the wavelengths of interest for dispersing the emitted light, and a photodiode array for receiving the dispersed light. The light emitted by the sample is filtered to pass only the desired wavelengths, such as one of the lines of the Balmer series for hydrogen, the wavelengths of which differ slightly from one isotope to another. The output of the photodiode array is processed to determine the relative amounts of each isotope present in the sample. Additionally, the sample itself may be recovered using a metal hydride.

  8. Atomic line emission analyzer for hydrogen isotopes

    DOE Patents [OSTI]

    Kronberg, J.W.

    1991-05-08

    Apparatus for isotopic analysis of hydrogen comprises a low pressure chamber into which a sample of hydrogen is introduced and then exposed to an electrical discharge to excite the electrons of the hydrogen atoms to higher energy states and thereby cause the emission of light on the return to lower energy states, a Fresnel prism made at least in part of a material anomalously dispersive to the wavelengths of interest for dispersing the emitted light, and a photodiode array for receiving the dispersed light. The light emitted by the sample is filtered to pass only the desired wavelengths, such as one of the lines of the Balmer series for hydrogen, the wavelengths of which differ slightly from one isotope to another. The output of the photodiode array is processed to determine the relative amounts of each isotope present in the sample. Additionally, the sample itself may be recovered using, a metal hydride.

  9. Atomic line emission analyzer for hydrogen isotopes

    DOE Patents [OSTI]

    Kronberg, J.W.

    1993-03-30

    Apparatus for isotopic analysis of hydrogen comprises a low pressure chamber into which a sample of hydrogen is introduced and then exposed to an electrical discharge to excite the electrons of the hydrogen atoms to higher energy states and thereby cause the emission of light on the return to lower energy states, a Fresnel prism made at least in part of a material anomalously dispersive to the wavelengths of interest for dispersing the emitted light, and a photodiode array for receiving the dispersed light. The light emitted by the sample is filtered to pass only the desired wavelengths, such as one of the lines of the Balmer series for hydrogen, the wavelengths of which differ slightly from one isotope to another. The output of the photodiode array is processed to determine the relative amounts of each isotope present in the sample. Additionally, the sample itself may be recovered using a metal hydride.

  10. Isotope separation apparatus

    DOE Patents [OSTI]

    Arnush, Donald; MacKenzie, Kenneth R.; Wuerker, Ralph F.

    1980-01-01

    Isotope separation apparatus consisting of a plurality of cells disposed adjacent to each other in an evacuated container. A common magnetic field is established extending through all of the cells. A source of energetic electrons at one end of the container generates electrons which pass through the cells along the magnetic field lines. Each cell includes an array of collector plates arranged in parallel or in tandem within a common magnetic field. Sets of collector plates are disposed adjacent to each other in each cell. Means are provided for differentially energizing ions of a desired isotope by applying energy at the cyclotron resonant frequency of the desired isotope. As a result, the energized desired ions are preferentially collected by the collector plates.

  11. Improved Geothermometry Through Multivariate Reaction Path Modeling...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    at the April 2013 peer review meeting held in Denver, Colorado. geothermometrycooperpeer2013.pdf (922.86 KB) More Documents & Publications track 4: enhanced geothermal ...

  12. Geothermometry (Klein, 2007) | Open Energy Information

    Open Energy Info (EERE)

    In The Past 20 Years- Geochemistry In Geothermal Exploration Resource Evaluation And Reservoir Management Additional References Retrieved from "http:en.openei.orgw...

  13. Improvements in geothermometry. Final technical report. Rev

    SciTech Connect (OSTI)

    Potter, J.; Dibble, W.; Parks, G.; Nur, A.

    1982-08-01

    Alkali and alkaline earth geothermometers are useful for estimating geothermal reservoir temperatures, though a general theoretical basis has yet to be established and experimental calibration needs improvement. Equilibrium cation exchange between feldspars provided the original basis for the Na-K and Na-K-Ca geothermometers (Fournier and Truesdell, 1973), but theoretical, field and experimental evidence prove that neither equilibrium nor feldspars are necessary. Here, evidence is summarized in support of these observations, concluding that these geothermometers can be expected to have a surprisingly wide range of applicability, but that the reasons behind such broad applicability are not yet understood. Early experimental work proved that water-rock interactions are slow at low temperatures, so experimental calibration at temperatures below 150/sup 0/ is impractical. Theoretical methods and field data were used instead for all work at low temperatures. Experimental methods were emphasized for temperatures above 150/sup 0/C, and the simplest possible solid and solution compositions were used to permit investigation of one process or question at a time. Unexpected results in experimental work prevented complete integration of the various portions of the investigation.

  14. Colorado thermal spring water geothermometry (public dataset...

    Open Energy Info (EERE)

    chemical geothermometers for Colorado thermal springs. Data citations include Barrett, J. K. and Pearl, R. H. (1976), George, R. D., Curtis, H. A., Lester, O. C., Crook, J. K.,...

  15. Integrated Chemical Geothermometry System for Geothermal Exploration

    Broader source: Energy.gov [DOE]

    DOE Geothermal Peer Review 2010 - Presentation. Develop practical and reliable system to predict geothermal reservoir temperatures from integrated chemical analyses of spring and well fluids.

  16. DEEP WATER ISOTOPIC CURRENT ANALYZER

    DOE Patents [OSTI]

    Johnston, W.H.

    1964-04-21

    A deepwater isotopic current analyzer, which employs radioactive isotopes for measurement of ocean currents at various levels beneath the sea, is described. The apparatus, which can determine the direction and velocity of liquid currents, comprises a shaft having a plurality of radiation detectors extending equidistant radially therefrom, means for releasing radioactive isotopes from the shaft, and means for determining the time required for the isotope to reach a particular detector. (AEC)

  17. Method for separating boron isotopes

    DOE Patents [OSTI]

    Rockwood, Stephen D.

    1978-01-01

    A method of separating boron isotopes .sup.10 B and .sup.11 B by laser-induced selective excitation and photodissociation of BCl.sub.3 molecules containing a particular boron isotope. The photodissociation products react with an appropriate chemical scavenger and the reaction products may readily be separated from undissociated BCl.sub.3, thus effecting the desired separation of the boron isotopes.

  18. Isotope Production and Distribution Program`s Fiscal Year 1997 financial statement audit

    SciTech Connect (OSTI)

    1998-03-27

    The Department of Energy Isotope Production and Distribution Program mission is to serve the national need for a reliable supply of isotope products and services for medicine, industry and research. The program produces and sells hundreds of stable and radioactive isotopes that are widely utilized by domestic and international customers. Isotopes are produced only where there is no U.S. private sector capability or other production capacity is insufficient to meet U.S. needs. The Department encourages private sector investment in new isotope production ventures and will sell or lease its existing facilities and inventories for commercial purposes. The Isotope Program reports to the Director of the Office of Nuclear Energy, Science and Technology. The Isotope Program operates under a revolving fund established by the Fiscal Year (FY) 1990 Energy and Water Appropriations Act and maintains financial viability by earning revenues from the sale of isotopes and services and through annual appropriations. The FY 1995 Energy and Water Appropriations Act modified predecessor acts to allow prices charged for Isotope Program products and services to be based on production costs, market value, the needs of the research community, and other factors. Although the Isotope Program functions as a business, prices set for small-volume, high-cost isotopes that are needed for research purposes may not achieve full-cost recovery. As a result, isotopes produced by the Isotope Program for research and development are priced to provide a reasonable return to the U.S. Government without discouraging their use. Commercial isotopes are sold on a cost-recovery basis. Because of its pricing structure, when selecting isotopes for production, the Isotope Program must constantly balance current isotope demand, market conditions, and societal benefits with its determination to operate at the lowest possible cost to U.S. taxpayers. Thus, this report provides a financial analysis of this situation.

  19. Health and safety consequences of medical isotope processing at the Hanford Site 325 building

    SciTech Connect (OSTI)

    Nielsen, D. L.

    1997-11-19

    Potential activities associated with medical isotope processing at the Hanford Site 325 Building laboratory and hot cell facilities are evaluated to assess the health and safety consequences if these activities are to be implemented as part of a combined tritium and medical isotope production mission for the Fast Flux Text Facility (FFTF). The types of activities included in this analysis are unloading irradiated isotope production assemblies at the 325 Building, recovery and dissolution of the target materials, separation of the product isotopes as required, and preparation of the isotopes for shipment to commercial distributors who supply isotopes to the medical conunuriity. Possible consequences to members of the public and to workers from both radiological and non-radiological hazards are considered in this evaluation. Section 2 of this docinnent describes the assumptions and methods used for the health and safety consequences analysis, section 3 presents the results of the analysis, and section 4 summarizes the results and conclusions from the analysis.

  20. ISOTOPE SEPARATING APPARATUS CONTROL

    DOE Patents [OSTI]

    Barnes, S.W.

    1959-08-25

    An improved isotope separating apparatus of the electromagnetic type, commonly referred to as a calutron, is described. Improvements in detecting and maintaining optimum position and focus of the ion beam are given. The calutron collector is provided with an additional electrode insulated from and positioned between the collecting pockets. The ion beams are properly positioned and focused until the deionizing current which flows from ground to this additional electrode ts a minimum.

  1. Isotopic Generation and Confirmation of the PWR Application Model 

    SciTech Connect (OSTI)

    L.B. Wimmer

    2003-11-10

    The objective of this calculation is to establish an isotopic database to represent commercial spent nuclear fuel (CSNF) from pressurized water reactors (PWRs) in criticality analyses performed for the proposed Monitored Geologic Repository at Yucca Mountain, Nevada. Confirmation of the conservatism with respect to criticality in the isotopic concentration values represented by this isotopic database is performed as described in Section 3.5.3.1.2 of the ''Disposal Criticality Analysis Methodology Topical Report'' (YMP 2000). The isotopic database consists of the set of 14 actinides and 15 fission products presented in Section 3.5.2.1.1 of YMP 2000 for use in CSNF burnup credit. This set of 29 isotopes is referred to as the principal isotopes. The oxygen isotope from the UO{sub 2} fuel is also included in the database. The isotopic database covers enrichments of {sup 235}U ranging from 1.5 to 5.5 weight percent (wt%) and burnups ranging from approximately zero to 75 GWd per metric ton of uranium (mtU). The choice of fuel assembly and operating history values used in generating the isotopic database are provided is Section 5. Tables of isotopic concentrations for the 29 principal isotopes (plus oxygen) as a function of enrichment and burnup are provided in Section 6.1. Results of the confirmation of the conservatism with respect to criticality in the isotopic concentration values are provided in Section 6.2.

  2. Laser isotope separation of erbium and other isotopes

    DOE Patents [OSTI]

    Haynam, Christopher A.; Worden, Earl F.

    1995-01-01

    Laser isotope separation is accomplished using at least two photoionization pathways of an isotope simultaneously, where each pathway comprises two or more transition steps. This separation method has been applied to the selective photoionization of erbium isotopes, particularly for the enrichment of .sup.167 Er. The hyperfine structure of .sup.167 Er was used to find two three-step photoionization pathways having a common upper energy level.

  3. Laser isotope separation of erbium and other isotopes

    DOE Patents [OSTI]

    Haynam, C.A.; Worden, E.F.

    1995-08-22

    Laser isotope separation is accomplished using at least two photoionization pathways of an isotope simultaneously, where each pathway comprises two or more transition steps. This separation method has been applied to the selective photoionization of erbium isotopes, particularly for the enrichment of {sup 167}Er. The hyperfine structure of {sup 167}Er was used to find two three-step photoionization pathways having a common upper energy level. 3 figs.

  4. Isotope shifts in francium isotopes Fr 206 - 213 and Fr 221

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Collister, R.; Gwinner, G.; Tandecki, M.; Behr, J. A.; Pearson, M. R.; Zhang, J.; Orozco, L. A.; Aubin, S.; Gomez, E.; FrPNC Collaboration

    2014-11-07

    We present the isotope shifts of the 7s1/2 to 7p1/2 transition for francium isotopes ²⁰⁶⁻²¹³Fr with reference to ²²¹Fr collected from two experimental periods. The shifts are measured on a sample of atoms prepared within a magneto-optical trap by a fast sweep of radio-frequency sidebands applied to a carrier laser. King plot analysis, which includes literature values for 7s1/2 to 7p3/2 isotope shifts, provides a field shift constant ratio of 1.0520(10) and a difference between the specific mass shift constants of 170(100) GHz amu between the D₁ and D₂ transitions, of sufficient precision to differentiate between ab initio calculations.

  5. EIS-0310-SA-01: Supplement Analysis | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    and Development and Isotope Production Missions in the United States Supplement Analysis ... Energy Research and Development and Isotope Production Missions in the United States. ...

  6. Heavy neodymium isotopes in the interacting boson (IBA-2) model

    SciTech Connect (OSTI)

    Giannatiempo, A.

    2011-08-15

    The N>82 even neodymium isotopes were studied in the framework of the IBA-2 model. The analysis was performed by using a very schematic Hamiltonian, particularly suited to investigate the U(5) {yields} SU(3) transition. The evolution of the excitation energy patterns and of the spectroscopic properties along the isotopic chain can be correctly reproduced when the role played by states of mixed symmetry character is also taken into account.

  7. Stable isotope research pool inventory

    SciTech Connect (OSTI)

    Not Available

    1988-02-01

    This report contains a listing of electromagnetically separated stable isotopes which are available at the Oak Ridge National Laboratory for distribution for nondestructive research use on a loan basis. This inventory includes all samples of stable isotopes in the Research Materials Collection and does not designate whether a sample is out on loan or is in reprocessing. For some of the high-abundance, naturally occurring isotopes, larger amounts can be made available; for example, Ca-40 and Fe-56.

  8. Stable isotope research pool inventory

    SciTech Connect (OSTI)

    Not Available

    1982-01-01

    This report contains a listing of electromagnetically separated stable isotopes which are available for distribution within the United States for nondestructive research use from the Oak Ridge National Laboratory on a loan basis. This inventory includes all samples of stable isotopes in the Material Research Collection and does not designate whether a sample is out on loan or in reprocessing. For some of the high abundance naturally occurring isotopes, larger amounts can be made available; for example, Ca-40 and Fe-56.

  9. Stable isotope research pool inventory

    SciTech Connect (OSTI)

    Not Available

    1984-03-01

    This report contains a listing of electromagnetically separated stable isotopes which are available at the Oak Ridge National Laboratory for distribution for nondestructive research use on a loan basis. This inventory includes all samples of stable isotopes in the Research Materials Collection and does not designate whether a sample is out on loan or is in reprocessing. For some of the high abundance naturally occurring isotopes, larger amounts can be made available; for example, Ca-40 and Fe-56.

  10. Isotopically labeled compositions and method

    DOE Patents [OSTI]

    Schmidt, Jurgen G.; Kimball, David B.; Alvarez, Marc A.; Williams, Robert F.; Martinez, Rudolfo A.

    2011-07-12

    Compounds having stable isotopes .sup.13C and/or .sup.2H were synthesized from precursor compositions having solid phase supports or affinity tags.

  11. Advanced isotope separation

    SciTech Connect (OSTI)

    Not Available

    1982-05-04

    The Study Group briefly reviewed the technical status of the three Advanced Isotope Separation (AIS) processes. It also reviewed the evaluation work that has been carried out by DOE's Process Evaluation Board (PEB) and the Union Carbide Corporation-Nuclear Division (UCCND). The Study Group briefly reviewed a recent draft assessment made for DOE staff of the nonproliferation implications of the AIS technologies. The staff also very briefly summarized the status of GCEP and Advanced Centrifuge development. The Study Group concluded that: (1) there has not been sufficient progress to provide a firm scientific, technical or economic basis on which to select one of the three competing AIS processes for full-scale engineering development at this time; and (2) however, should budgetary restraints or other factors force such a selection, we believe that the evaluation process that is being carried out by the PEB provides the best basis available for making a decision. The Study Group recommended that: (1) any decisions on AIS processes should include a comparison with gas centrifuge processes, and should not be made independently from the plutonium isotope program; (2) in evaluating the various enrichment processes, all applicable costs (including R and D and sales overhead) and an appropriate discounting approach should be included in order to make comparisons on a private industry basis; (3) if the three AIS programs continue with limited resources, the work should be reoriented to focus only on the most pressing technical problems; and (4) if a decision is made to develop the Atomic Vapor Laser Isotope Separation process, the solid collector option should be pursued in parallel to alleviate the potential program impact of liquid collector thermal control problems.

  12. Chromatographic hydrogen isotope separation

    DOE Patents [OSTI]

    Aldridge, Frederick T.

    1981-01-01

    Intermetallic compounds with the CaCu.sub.5 type of crystal structure, particularly LaNiCo.sub.4 and CaNi.sub.5, exhibit high separation factors and fast equilibrium times and therefore are useful for packing a chromatographic hydrogen isotope separation colum. The addition of an inert metal to dilute the hydride improves performance of the column. A large scale mutli-stage chromatographic separation process run as a secondary process off a hydrogen feedstream from an industrial plant which uses large volumes of hydrogen can produce large quantities of heavy water at an effective cost for use in heavy water reactors.

  13. ISOTOPE FRACTIONATION PROCESS

    DOE Patents [OSTI]

    Clewett, G.H.; Lee, DeW.A.

    1958-05-20

    A new method is described for isotopic enrichment of uranium. It has been found that when an aqueous acidic solution of ionic tetravalent uraniunn is contacted with chelate complexed tetravalent uranium, the U/sup 238/ preferentially concentrates in the complexed phase while U/sup 235/ concentrates in the ionic phase. The effect is enhanced when the chelate compound is water insoluble and is dissolved in a water-immiscible organic solvent. Cupferron is one of a number of sultable complexing agents, and chloroform is a suitable organic solvent.

  14. Chromatographic hydrogen isotope separation

    DOE Patents [OSTI]

    Aldridge, F.T.

    Intermetallic compounds with the CaCu/sub 5/ type of crystal structure, particularly LaNiCo/sub 4/ and CaNi/sub 5/, exhibit high separation factors and fast equilibrium times and therefore are useful for packing a chromatographic hydrogen isotope separation column. The addition of an inert metal to dilute the hydride improves performance of the column. A large scale multi-stage chromatographic separation process run as a secondary process off a hydrogen feedstream from an industrial plant which uses large volumes of hydrogen cn produce large quantities of heavy water at an effective cost for use in heavy water reactors.

  15. Isotope Program Transportation | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Isotope Program Transportation Isotope Program Transportation Isotope Program Transportation (894.11 KB) More Documents & Publications Nuclear Fuel Storage and Transportation Planning Project Overview Section 180(c) Ad Hoc Working Group DOE Office of Nuclear Energy

  16. Uranium accountancy in Atomic Vapor Laser Isotope Separation

    SciTech Connect (OSTI)

    Carver, R.D.

    1986-01-01

    The AVLIS program pioneers the large scale industrial application of lasers to produce low cost enriched uranium fuel for light water reactors. In the process developed at Lawrence Livermore National Laboratory, normal uranium is vaporized by an electron beam, and a precisely tuned laser beam selectively photo-ionizes the uranium-235 isotopes. These ions are moved in an electromagnetic field to be condensed on the product collector. All other uranium isotopes remain uncharged and pass through the collector section to condense as tails. Tracking the three types of uranium through the process presents special problems in accountancy. After demonstration runs, the uranium on the collector was analyzed for isotopic content by Battelle Pacific Northwest Laboratory. Their results were checked at LLNL by analysis of parallel samples. The differences in isotopic composition as reported by the two laboratories were not significant.

  17. Phonon coherence in isotopic silicon superlattices

    SciTech Connect (OSTI)

    Frieling, R.; Radek, M.; Eon, S.; Bracht, H.; Wolf, D. E.

    2014-09-29

    Recent experimental and theoretical investigations have confirmed that a reduction in thermal conductivity of silicon is achieved by isotopic silicon superlattices. In the present study, non-equilibrium molecular dynamics simulations are performed to identify the isotope doping and isotope layer ordering with minimum thermal conductivity. Furthermore, the impact of isotopic intermixing at the superlattice interfaces on phonon transport is investigated. Our results reveal that the coherence of phonons in isotopic Si superlattices is prevented if interfacial mixing of isotopes is considered.

  18. Method of separating boron isotopes

    DOE Patents [OSTI]

    Jensen, Reed J.; Thorne, James M.; Cluff, Coran L.; Hayes, John K.

    1984-01-01

    A method of boron isotope enrichment involving the isotope preferential photolysis of (2-chloroethenyl)dichloroborane as the feed material. The photolysis can readily be achieved with CO.sub.2 laser radiation and using fluences significantly below those required to dissociate BCl.sub.3.

  19. Method of separating boron isotopes

    DOE Patents [OSTI]

    Jensen, R.J.; Thorne, J.M.; Cluff, C.L.

    1981-01-23

    A method of boron isotope enrichment involving the isotope preferential photolysis of (2-chloroethenyl)-dichloroborane as the feed material. The photolysis can readily by achieved with CO/sub 2/ laser radiation and using fluences significantly below those required to dissociate BCl/sub 3/.

  20. Stable isotope research pool inventory

    SciTech Connect (OSTI)

    Not Available

    1980-12-01

    This report contains a listing of electromagnetically separated stable isotopes which are available for distribution within the United States for non-destructive research use from the Oak Ridge National Laboratory on a loan basis. This inventory includes all samples of stable isotopes in the Materials Research Collection and does not designate whether a sample is out on loan or in reprocessing.

  1. Isotopic Trends in Production of Superheavies

    SciTech Connect (OSTI)

    Antonenko, N.V.; Adamian, G.G.; Zubov, A.S.; Scheid, W.

    2005-11-21

    The isotopic trends are discussed for cold and hot fusion reactions leading to superheavies. The possibilities of production of new isotopes in incomplete fusion reactions are treated.

  2. Heavy Isotopes Lead Materials Management Organization (LMMO)...

    Office of Scientific and Technical Information (OSTI)

    Heavy Isotopes Lead Materials Management Organization (LMMO) Update Citation Details In-Document Search Title: Heavy Isotopes Lead Materials Management Organization (LMMO) Update ...

  3. Isotope separation by laser means

    DOE Patents [OSTI]

    Robinson, C. Paul; Jensen, Reed J.; Cotter, Theodore P.; Greiner, Norman R.; Boyer, Keith

    1982-06-15

    A process for separating isotopes by selective excitation of isotopic species of a volatile compound by tuned laser light. A highly cooled gas of the volatile compound is produced in which the isotopic shift is sharpened and defined. Before substantial condensation occurs, the cooled gas is irradiated with laser light precisely tuned to a desired wavelength to selectively excite a particular isotopic species in the cooled gas. The laser light may impart sufficient energy to the excited species to cause it to undergo photochemical reaction or even to photoionize. Alternatively, a two-photon irradiation may be applied to the cooled gas to induce photochemical reaction or photoionization. The process is particularly applicable to the separation of isotopes of uranium and plutonium.

  4. Container for hydrogen isotopes

    DOE Patents [OSTI]

    Solomon, David E.

    1977-01-01

    A container for the storage, shipping and dispensing of hydrogen isotopes such as hydrogen, deuterium, tritium, or mixtures of the same which has compactness, which is safe against fracture or accident, and which is reusable. The container consists of an outer housing with suitable inlet and outlet openings and electrical feed elements, the housing containing an activated sorber material in the form, for example, of titanium sponge or an activated zirconium aluminate cartridge. The gas to be stored is introduced into the chamber under conditions of heat and vacuum and will be retained in the sorber material. Subsequently, it may be released by heating the unit to drive off the stored gas at desired rates.

  5. Laser separation of medical isotopes

    SciTech Connect (OSTI)

    Eerkens, J.W.; Puglishi, D.A.; Miller, W.H.

    1996-12-31

    There is an increasing demand for different separated isotopes as feed material for reactor and cyclotron-produced radioisotopes used by a fast-growing radiopharmaceutical industry. One new technology that may meet future demands for medical isotopes is molecular laser isotope separation (MLIS). This method was investigated for the enrichment of uranium in the 1970`s and 1980s by Los Alamos National Laboratory, Isotope Technologies, and others around the world. While South Africa and Japan have continued the development of MLIS for uranium and are testing pilot units, around 1985 the United States dropped the LANL MLIS program in favor of AVLIS (atomic vapor LIS), which uses electron-beam-heated uranium metal vapor. AVLIS appears difficult and expensive to apply to most isotopes of medical interest, however, whereas MLIS technology, which is based on cooled hexafluorides or other gaseous molecules, can be adapted more readily. The attraction of MLIS for radiopharmaceutical firms is that it allows them to operate their own dedicated separators for small-quantity productions of critical medical isotopes, rather than having to depend on large enrichment complexes run by governments, which are only optimal for large-quantity productions. At the University of Missouri, the authors are investigating LIS of molybdenum isotopes using MoF{sub 6}, which behaves in a way similar to UF{sub 6}, studied in the past.

  6. First AID (Atom counting for Isotopic Determination).

    SciTech Connect (OSTI)

    Roach, J. L.; Israel, K. M.; Steiner, R. E.; Duffy, C. J.; Roench, F. R.

    2002-01-01

    Los Alamos National Laboratory (LANL) has established an in vitro bioassay monitoring program in compliance with the requirements in the Code of Federal Regulations, 10 CFR 835, Occupational Radiation Protection. One aspect of this program involves monitoring plutonium levels in at-risk workers. High-risk workers are monitored using the ultra-sensitive Therrnal Ionization Mass Spectrometry (TIMS) technique to ensure compliance with DOE standards. TIMS is used to measure atom ratios of 239Pua nd 240Puw ith respect to a tracer isotope ('Pu). These ratios are then used to calculate the amount of 239Pu and 240Pup resent. This low-level atom counting technique allows the calculation of the concentration levels of 239Pu and 240Pu in urine for at risk workers. From these concentration levels, dose assessments can be made and worker exposure levels can be monitored. Detection limits for TIMS analysis are on the order of millions of atoms, which translates to activity levels of 150 aCi 239Pua nd 500 aCi for 240Pu. pCi for Our poster presentation will discuss the ultra-sensitive, low-level analytical technique used to measure plutonium isotopes and the data verification methods used for validating isotopic measurements.

  7. Stable isotope research pool inventory

    SciTech Connect (OSTI)

    Not Available

    1981-01-01

    This report contains a listing of electromagnetically separated stable isotopes which are available for distribution within the United States for non-destructive research use from the Oak Ridge National Laboratory on a loan basis. This inventory includes all samples of stable isotopes in the Materials Research Collection and does not designate whether a sample is out on loan or in reprocessing. For some of the high abundance naturally occurring isotopes, larger amounts can be made available; for example, Ca-40 and Fe-56.

  8. Stable isotope research pool inventory

    SciTech Connect (OSTI)

    Not Available

    1983-03-01

    This report contains a listing of electromagnetically separated stable isotopes which are available for distribution within the United States for non-destructive research use from the Oak Ridge National Laboratory on a loan basis. This inventory includes all samples of stable isotopes in the Materials Research Collection and does not designate whether a sample is out on loan or in reprocessing. For some of the high abundance naturally occurring isotopes, larger amounts can be made available; for example, Ca-40 and Fe-56.

  9. Compelling Research Opportunities using Isotopes

    SciTech Connect (OSTI)

    2009-04-23

    Isotopes are vital to the science and technology base of the US economy. Isotopes, both stable and radioactive, are essential tools in the growing science, technology, engineering, and health enterprises of the 21st century. The scientific discoveries and associated advances made as a result of the availability of isotopes today span widely from medicine to biology, physics, chemistry, and a broad range of applications in environmental and material sciences. Isotope issues have become crucial aspects of homeland security. Isotopes are utilized in new resource development, in energy from bio-fuels, petrochemical and nuclear fuels, in drug discovery, health care therapies and diagnostics, in nutrition, in agriculture, and in many other areas. The development and production of isotope products unavailable or difficult to get commercially have been most recently the responsibility of the Department of Energy's Nuclear Energy program. The President's FY09 Budget request proposed the transfer of the Isotope Production program to the Department of Energy's Office of Science in Nuclear Physics and to rename it the National Isotope Production and Application program (NIPA). The transfer has now taken place with the signing of the 2009 appropriations bill. In preparation for this, the Nuclear Science Advisory Committee (NSAC) was requested to establish a standing subcommittee, the NSAC Isotope Subcommittee (NSACI), to advise the DOE Office of Nuclear Physics. The request came in the form of two charges: one, on setting research priorities in the short term for the most compelling opportunities from the vast array of disciplines that develop and use isotopes and two, on making a long term strategic plan for the NIPA program. This is the final report to address charge 1. NSACI membership is comprised of experts from the diverse research communities, industry, production, and homeland security. NSACI discussed research opportunities divided into three areas: (1) medicine

  10. Apparatus and process for separating hydrogen isotopes

    DOE Patents [OSTI]

    Heung, Leung K; Sessions, Henry T; Xiao, Xin

    2013-06-25

    The apparatus and process for separating hydrogen isotopes is provided using dual columns, each column having an opposite hydrogen isotopic effect such that when a hydrogen isotope mixture feedstock is cycled between the two respective columns, two different hydrogen isotopes are separated from the feedstock.

  11. Method for laser induced isotope enrichment

    DOE Patents [OSTI]

    Pronko, Peter P.; Vanrompay, Paul A.; Zhang, Zhiyu

    2004-09-07

    Methods for separating isotopes or chemical species of an element and causing enrichment of a desired isotope or chemical species of an element utilizing laser ablation plasmas to modify or fabricate a material containing such isotopes or chemical species are provided. This invention may be used for a wide variety of materials which contain elements having different isotopes or chemical species.

  12. Raman scattering method and apparatus for measuring isotope ratios and isotopic abundances

    DOE Patents [OSTI]

    Harney, Robert C.; Bloom, Stewart D.

    1978-01-01

    Raman scattering is used to measure isotope ratios and/or isotopic abundances. A beam of quasi-monochromatic photons is directed onto the sample to be analyzed, and the resulting Raman-scattered photons are detected and counted for each isotopic species of interest. These photon counts are treated mathematically to yield the desired isotope ratios or isotopic abundances.

  13. Stable isotope research pool inventory

    SciTech Connect (OSTI)

    Not Available

    1985-02-01

    This report contains a listing of electromagnetically separated stable isotopes which are available at the Oak Ridge National Laboratory for distribution for non-destructive research use on a loan basis. This inventory includes all samples of stable isotopes in the Research Materials Collection and does not designate whether a sample is out on loan or is in reprocessing. For some of the high abundance naturally occurring isotopes, larger amounts can be made available; for example, /sup 40/Ca and /sup 56/Fe. All request for the loan of samples should be submitted with a summary of the purpose of the loan to: Isotope Distribution Office, Oak Ridge National Laboratory, P.O. Box X, Oak Ridge, Tennessee 37831. Requests from non-DOE contractors and from foreign institutions require DOE approval.

  14. Physics with isotopically controlled semiconductors

    SciTech Connect (OSTI)

    Haller, E. E.

    2010-07-15

    This paper is based on a tutorial presentation at the International Conference on Defects in Semiconductors (ICDS-25) held in Saint Petersburg, Russia in July 2009. The tutorial focused on a review of recent research involving isotopically controlled semiconductors. Studies with isotopically enriched semiconductor structures experienced a dramatic expansion at the end of the Cold War when significant quantities of enriched isotopes of elements forming semiconductors became available for worldwide collaborations. Isotopes of an element differ in nuclear mass, may have different nuclear spins and undergo different nuclear reactions. Among the latter, the capture of thermal neutrons which can lead to neutron transmutation doping, is the most prominent effect for semiconductors. Experimental and theoretical research exploiting the differences in all the properties has been conducted and will be illustrated with selected examples.

  15. Novel hybrid isotope separation scheme and apparatus

    DOE Patents [OSTI]

    Maya, Jakob

    1991-01-01

    A method of yielding selectively a desired enrichment in a specific isotope including the steps of inputting into a spinning chamber a gas from which the specific isotope is to be isolated, radiating the gas with frequencies characteristic of the absorption of a particular isotope of the atomic or molecular gas, thereby inducing a photoionization reaction of the desired isotope, and collecting the specific isotope ion by suitable ion collection means.

  16. Novel hybrid isotope separation scheme and apparatus

    DOE Patents [OSTI]

    Maya, J.

    1991-06-18

    A method is described for yielding selectively a desired enrichment in a specific isotope including the steps of inputting into a spinning chamber a gas from which the specific isotope is to be isolated, radiating the gas with frequencies characteristic of the absorption of a particular isotope of the atomic or molecular gas, thereby inducing a photoionization reaction of the desired isotope, and collecting the specific isotope ion by suitable ion collection means. 3 figures.

  17. Isotope separation apparatus and method

    DOE Patents [OSTI]

    Feldman, Barry J.

    1985-01-01

    The invention relates to an improved method and apparatus for laser isotope separation by photodeflection. A molecular beam comprising at least two isotopes to be separated intersects, preferably substantially perpendicular to one broad side of the molecular beam, with a laser beam traveling in a first direction. The laser beam is reflected back through the molecular beam, preferably in a second direction essentially opposite to the first direction. Because the molecules in the beam occupy various degenerate energy levels, if the laser beam comprises chirped pulses comprising selected wavelengths, the laser beam will very efficiently excite substantially all unexcited molecules and will cause stimulated emission of substantially all excited molecules of a selected one of the isotopes in the beam which such pulses encounter. Excitation caused by first direction chirped pulses moves molecules of the isotope excited thereby in the first direction. Stimulated emission of excited molecules of the isotope is brought about by returning chirped pulses traveling in the second direction. Stimulated emission moves emitting molecules in a direction opposite to the photon emitted. Because emitted photons travel in the second direction, emitting molecules move in the first direction. Substantial molecular movement of essentially all the molecules containing the one isotope is accomplished by a large number of chirped pulse-molecule interactions. A beam corer collects the molecules in the resulting enriched divergent portions of the beam.

  18. Communication: Localized molecular orbital analysis of the effect of electron correlation on the anomalous isotope effect in the NMR spin-spin coupling constant in methane

    SciTech Connect (OSTI)

    Zarycz, M. Natalia C. Provasi, Patricio F.; Sauer, Stephan P. A.

    2014-10-21

    We discuss the effect of electron correlation on the unexpected differential sensitivity (UDS) in the {sup 1}J(CH) coupling constant of CH{sub 4} using a decomposition into contributions from localized molecular orbitals and compare with the {sup 1}J(NH) coupling constant in NH{sub 3}. In particular, we discuss the well known fact that uncorrelated coupled Hartree-Fock (CHF) calculations are not able to reproduce the UDS in methane. For this purpose we have implemented for the first time a localized molecular orbital analysis for the second order polarization propagator approximation with coupled cluster singles and doubles amplitudesSOPPA(CCSD) in the DALTON program. Comparing the changes in the localized orbital contributions at the correlated SOPPA and SOPPA(CCSD) levels and at the uncorrelated CHF level, we find that the latter overestimates the effect of stretching the bond between the coupled atoms on the contribution to the coupling from the localized bonding orbital between these atoms. This disturbs the subtle balance between the molecular orbital contributions, which lead to the UDS in methane.

  19. Isotope separation by photochromatography (Patent) | SciTech...

    Office of Scientific and Technical Information (OSTI)

    Patent: Isotope separation by photochromatography Citation Details In-Document Search Title: Isotope separation by photochromatography An isotope separation method which comprises ...

  20. Department of Energy's Isotope Development and Production for...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    ... The Isotope Program prices isotopes sold for medical and industrial applications to recover full cost. Isotopes sold for research and development are priced to recover direct costs ...

  1. Isotope production facility produces cancer-fighting actinium

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Cancer therapy gets a boost from new isotope Isotope production facility produces cancer-fighting actinium A new medical isotope project shows promise for rapidly producing major ...

  2. Isotope separation apparatus and method

    DOE Patents [OSTI]

    Cotter, Theodore P.

    1982-12-28

    The invention relates to a method and apparatus for laser isotope separation by photodeflection. A molecular beam comprising at least two isotopes to be separated intersects, preferable substantially perpendicular to one broad side of the molecular beam, with a laser beam traveling in a first direction. The laser beam is reflected back through the molecular beam, preferably in a second direction essentially opposite to the first direction. The laser beam comprises .pi.-pulses of a selected wavelength which excite unexcited molecules, or cause stimulated emission of excited molecules of one of the isotopes. Excitation caused by first direction .pi.-pulses moves molecules of the isotope excited thereby in the first direction. Stimulated emission of excited molecules of the isotope is brought about by returning .pi.-pulses traveling in the second direction. Stimulated emission moves emitting molecules in a direction opposite to the photon emitted. Because emitted photons travel in the second direction, emitting molecules move in the first direction. Substantial molecular movement is accomplished by a large number of .pi.-pulse-molecule interactions. A beam corer collects the molecules in the resulting enriched divergent portions of the beam.

  3. Isotope specific arbitrary material sorter

    DOE Patents [OSTI]

    Barty, Christopher P.J.

    2015-12-08

    A laser-based mono-energetic gamma-ray source is used to provide a rapid and unique, isotope specific method for sorting materials. The objects to be sorted are passed on a conveyor in front of a MEGa-ray beam which has been tuned to the nuclear resonance fluorescence transition of the desired material. As the material containing the desired isotope traverses the beam, a reduction in the transmitted MEGa-ray beam occurs. Alternately, the laser-based mono-energetic gamma-ray source is used to provide non-destructive and non-intrusive, quantitative determination of the absolute amount of a specific isotope contained within pipe as part of a moving fluid or quasi-fluid material stream.

  4. Stable isotope research pool inventory

    SciTech Connect (OSTI)

    Not Available

    1986-08-01

    This report contains a listing of electromagnetically separated stable isotopes which are available at the Oak Ridge National Laboratory for distribution for nondestructive research use on a loan basis. This inventory includes all samples of stable isotopes in the Research Materials Collection and does not designate whether a sample is out on loan or is in reprocessing. For some of the high-abundance, naturally occurring isotopes, larger amounts can be made available; for example, Ca-40 and Fe-56. All requests for the loan of samples should be submitted with a summary of the purpose of the loan to: Iotope Distribution Office, Oak Ridge National Laboratory, P.O. Box X, Oak Ridge, Tennessee 37831. Requests from non-DOE contractors and from foreign institutions require DOE approval.

  5. Isotope geochronology of metamorphic processes

    SciTech Connect (OSTI)

    Ovchinnikov, L.N.; Voronovskiy, S.N.; Ovchinnikova, L.V.

    1986-05-01

    The long history of the earth and its crust is a history of uninterrupted and continuing transformation, making metamorphism the most common and most extensive geological process on this planet. Metamorphism has occurred in all epochs and is a factor in all endogenic processes: geodynamics, magmatism, and the action of intratelluric fluids. But it varies in scale, type, and mechanism, and is always combined with metasomatism - the chemical and mineral transformation of material. This paper discusses methodological principles of isotope dating, laws characterizing changes in indicator minerals, internal stability of isotopic systems, and interesting geological problems. 13 references.

  6. Isotopic Analysis (Not Available) | Open Energy Information

    Open Energy Info (EERE)

    and characterization. References (Unknown) Advisory Group On The Application Of Nuclear Techniques To Geothermal Studies-Meeting In Pisa 8-12 Sep 1975 Additional References...

  7. Isotopic Analysis (Klein, 2007) | Open Energy Information

    Open Energy Info (EERE)

    In The Past 20 Years- Geochemistry In Geothermal Exploration Resource Evaluation And Reservoir Management Additional References Retrieved from "http:en.openei.orgw...

  8. Isotopic Analysis- Rock | Open Energy Information

    Open Energy Info (EERE)

    and Acquisition Photo of the plasma sampler from an ICP-MS system used by the Atomic Energy and Alternative Energies Commission (CEA), France. Photo from the CEA Website, last...

  9. Isotopic Analysis- Fluid | Open Energy Information

    Open Energy Info (EERE)

    and Acquisition Photo of the plasma sampler from an ICP-MS system used by the Atomic Energy and Alternative Energies Commission (CEA), France. Photo from the CEA Website, last...

  10. Online Catalog of Isotope Products from DOE's National Isotope Development Center

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    The National Isotope Development Center (NIDC) interfaces with the User Community and manages the coordination of isotope production across the facilities and business operations involved in the production, sale, and distribution of isotopes. A virtual center, the NIDC is funded by the Isotope Development and Production for Research and Applications (IDPRA) subprogram of the Office of Nuclear Physics in the U.S. Department of Energy Office of Science. The Isotope subprogram supports the production, and the development of production techniques of radioactive and stable isotopes that are in short supply for research and applications. Isotopes are high-priority commodities of strategic importance for the Nation and are essential for energy, medical, and national security applications and for basic research; a goal of the program is to make critical isotopes more readily available to meet domestic U.S. needs. This subprogram is steward of the Isotope Production Facility (IPF) at Los Alamos National Laboratory (LANL), the Brookhaven Linear Isotope Producer (BLIP) facility at BNL, and hot cell facilities for processing isotopes at ORNL, BNL and LANL. The subprogram also coordinates and supports isotope production at a suite of university, national laboratory, and commercial accelerator and reactor facilities throughout the Nation to promote a reliable supply of domestic isotopes. The National Isotope Development Center (NIDC) at ORNL coordinates isotope production across the many facilities and manages the business operations of the sale and distribution of isotopes.