Sample records for generation atomic absorption

  1. Absorption properties of identical atoms

    E-Print Network [OSTI]

    Pedro Sancho

    2013-07-31T23:59:59.000Z

    Emission rates and other optical properties of multiparticle systems in collective and entangled states differ from those in product ones. We show the existence of similar effects in the absorption probabilities for (anti)symmetrized states of two identical atoms. The effects strongly depend on the overlapping between the atoms and differ for bosons and fermions. We propose a viable experimental verification of these ideas.

  2. atomization atomic absorption: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    cells to modern observations of dust clouds in stellar nebulas and Bose-Einstein condensates. Here we show the first absorption imaging of a single atom isolated in vacuum. The...

  3. Transient x-ray absorption spectroscopy of hydrated halogen atom

    E-Print Network [OSTI]

    Elles, Christopher G.; Shkrob, Ilya A.; Crowell, Robert A.; Arms, Dohn A.; Landahl, Eric C.

    2008-02-11T23:59:59.000Z

    Time-resolved x-ray absorption spectroscopy has been used to observe the transient species generated by one-photon detachment of an electron from aqueous bromide. The K-edge spectrum of the short-lived Br(0) atom exhibits a resonant 1s-4p transition...

  4. Single photon absorption by a single atom: from heralded absorption to polarization state mapping

    E-Print Network [OSTI]

    Nicolas Piro; Jürgen Eschner

    2015-02-19T23:59:59.000Z

    Together with photon emission, the absorption of a single photon by a single atom is a fundamental process in matter-light interaction that manifests its quantum mechanical nature. As an experimentally controlled process, it is a key tool for the realization of quantum technologies. In particular, in an atom/photon based quantum network scenario, in which localized atomic particles are used as quantum information processing nodes while photons are used as carriers of quantum information between distant nodes, controlling both emission and absorption of single photons by single atoms is required for quantum coherent state mapping between the two entities. Most experimental efforts to date have focused on establishing the control of single photon emission by single trapped atoms, and the implementation of quantum networking protocols using this interaction. In this chapter, we describe experimental efforts to control the process of single photon absorption by single trapped ions. We describe a series of experiments in which polarization entangled photon pairs, generated by a spontaneous parametric down-conversion source, are coupled to a single ion. First the source is operated to generate heralded single photons, and coincidences between the absorption event of one photon of the pair and the detection of the heralding partner photon are observed. We then show how polarization control in the process is established, leading to the manifestation of the photonic polarization entanglement in the absorption process. Finally, we introduce protocols in which this interaction scheme is harnessed to perform tasks in a quantum network, such as entanglement distribution among distant nodes of the network, and we demonstrate a specific protocol for heralded, high-fidelity photon-to-atom quantum state transfer.

  5. atomic absorption spectrophotometric: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    atomic absorption spectrophotometric First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Absorption...

  6. Atomic Absorption Spectrometry Perkin Elmer 500, Chemistry & Biochemistry

    E-Print Network [OSTI]

    Gruner, Daniel S.

    Atomic Absorption Spectrometry · Perkin Elmer 500, Chemistry & Biochemistry · Perkin Elmer 560 AA Harvester-Luminometer scintillation counter, CBMG Centrifuges · Beckman Coulter Optima XL-I Analytical

  7. atomic absorption spectroscopic: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    atomic absorption spectroscopic First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Absorption properties...

  8. atomic absorption spectrometry-determination: Topics by E-print...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    atomic absorption spectrometry-determination First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Absorption...

  9. atomic absorption faa: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    atomic absorption faa First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Absorption properties of...

  10. atomic absorption spectrom: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    atomic absorption spectrom First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Absorption properties of...

  11. atomic absorption analysis: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    atomic absorption analysis First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Dressed-atom multiphoton...

  12. Quantized Media with Absorptive Scatterers and Modified Atomic Emission Rates

    E-Print Network [OSTI]

    L. G. Suttorp; A. J. van Wonderen

    2011-02-14T23:59:59.000Z

    Modifications in the spontaneous emission rate of an excited atom that are caused by extinction effects in a nearby dielectric medium are analyzed in a quantummechanical model, in which the medium consists of spherical scatterers with absorptive properties. Use of the dyadic Green function of the electromagnetic field near a a dielectric sphere leads to an expression for the change in the emission rate as a series of multipole contributions for which analytical formulas are obtained. The results for the modified emission rate as a function of the distance between the excited atom and the dielectric medium show the influence of both absorption and scattering processes.

  13. atomic absorption spectrometry: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    atomic absorption spectrometry First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Determination of...

  14. atomic absorption spectrometric: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    atomic absorption spectrometric First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Standard test method...

  15. atomic absorption determination: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    atomic absorption determination First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Determination of...

  16. atomic absorption spectrophotometry: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    atomic absorption spectrophotometry First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Wilolud Online...

  17. atomic absorption spectroscopy: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    atomic absorption spectroscopy First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Transient x-ray...

  18. atomic absorption spectrometr: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    atomic absorption spectrometr First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Standard test method for...

  19. Absorption spectrum of Ca atoms attached to $^4$He nanodroplets

    E-Print Network [OSTI]

    Alberto Hernando; Manuel Barranco; Marek Kro?nicki; Ricardo Mayol; Martí Pi

    2007-11-12T23:59:59.000Z

    Within density functional theory, we have obtained the structure of $^4$He droplets doped with neutral calcium atoms. These results have been used, in conjunction with newly determined {\\it ab-initio} $^1\\Sigma$ and $^1\\Pi$ Ca-He pair potentials, to address the $4s4p$ $^1$P$_1 \\leftarrow 4s^2$ $^1$S$_0$ transition of the attached Ca atom, finding a fairly good agreement with absorption experimental data. We have studied the drop structure as a function of the position of the Ca atom with respect of the center of mass of the helium moiety. The interplay between the density oscillations arising from the helium intrinsic structure and the density oscillations produced by the impurity in its neighborhood plays a role in the determination of the equilibrium state, and hence in the solvation properties of alkaline earth atoms. In a case of study, the thermal motion of the impurity within the drop surface region has been analyzed in a semi-quantitative way. We have found that, although the atomic shift shows a sizeable dependence on the impurity location, the thermal effect is statistically small, contributing by about a 10% to the line broadening. The structure of vortices attached to the calcium atom has been also addressed, and its effect on the calcium absorption spectrum discussed. At variance with previous theoretical predictions, we conclude that spectroscopic experiments on Ca atoms attached to $^4$He drops will be likely unable to detect the presence of quantized vortices in helium nanodrops.

  20. Etalon-induced Baseline Drift And Correction In Atom Flux Sensors Based On Atomic Absorption Spectroscopy

    SciTech Connect (OSTI)

    Du, Yingge; Chambers, Scott A.

    2014-10-20T23:59:59.000Z

    Atom flux sensors based on atomic absorption (AA) spectroscopy are of significant interest in thin film growth as they can provide unobtrusive, element specific, real-time flux sensing and control. The ultimate sensitivity and performance of the sensors are strongly affected by the long-term and short term baseline drift. Here we demonstrate that an etalon effect resulting from temperature changes in optical viewport housings is a major source of signal instability which has not been previously considered or corrected by existing methods. We show that small temperature variations in the fused silica viewports can introduce intensity modulations of up to 1.5%, which in turn significantly deteriorate AA sensor performance. This undesirable effect can be at least partially eliminated by reducing the size of the beam and tilting the incident light beam off the viewport normal.

  1. atomic absorption method: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption method First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Absorption properties of identical...

  2. atomic absorption flame: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption flame First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Absorption properties of identical...

  3. atomic absorption methods: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption methods First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Absorption properties of identical...

  4. Graphite Furnance Atomic Absorption as a detector for High Performance Liquid Chromatography

    E-Print Network [OSTI]

    Howell, Huston Edward

    1980-01-01T23:59:59.000Z

    tubing on peak broadening 38 Pulsed mode and uv chromatograms of two organo- selenium compounds 40 12. Pulsed mode and uv chromatograms of the organo- selenium compounds . . . . . . . . . . . . . . 41 13. An example of the variation of peak sizes... (8), flame and flameless atomic absorption (5), molecular (9) and atomic fluorescence (10), and electrochemical methods (11). By far the most widely used detection method for HPLC is ultraviolet (uv) absorption spectroscopy. The uv absorbance...

  5. atomic absorption spectrometer: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption spectrometer First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Educational Multiwavelength...

  6. atomic absorption spectrophotometer: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption spectrophotometer First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Wilolud Online...

  7. Atomic structure of machined semiconducting chips: An x-ray absorption spectroscopy study

    SciTech Connect (OSTI)

    Paesler, M.; Sayers, D.

    1988-12-01T23:59:59.000Z

    X-ray absorption spectroscopy (XAS) has been used to examine the atomic structure of chips of germanium that were produced by single point diamond machining. It is demonstrated that although the local (nearest neighbor) atomic structure is experimentally quite similar to that of single crystal specimens information from more distant atoms indicates the presence of considerable stress. An outline of the technique is given and the strength of XAS in studying the machining process is demonstrated.

  8. atomic absorption lines: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption lines First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 A survey for redshifted molecular and...

  9. atomic absorption technique: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption technique First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Determination of antimony in soils...

  10. Kaon Absorption from Kaonic Atoms and Formation Spectra of Kaonic Nuclei

    E-Print Network [OSTI]

    Junko Yamagata; Satoru Hirenzaki

    2006-12-09T23:59:59.000Z

    We considered the kaon absorption from atomic states into nucleus. We found that the nuclear density probed by the atomic kaon significantly depends on the kaon orbit. Then, we reexamined the meanings of the observed strengths of one-body and two-body kaon absorption, and investigated the effects to the formation spectra of kaon bound states by in-flight ($K^-,p$) reactions. As a natural consequence, if the atomic kaon probes the smaller nuclear density, the ratio of the two-body absorption at nuclear center is larger than the observed value, and the depth of the imaginary potential is deeper even at smaller kaon energies as in kaonic nuclear states because of the large phase space for the two-body processes.

  11. Subwavelength atom localization via amplitude and phase control of the absorption spectrum

    E-Print Network [OSTI]

    Mostafa Sahrai; Habib Tajalli; Kishore T. Kapale; M. Suhail Zubairy

    2005-07-21T23:59:59.000Z

    We propose a scheme for subwavelength localization of an atom conditioned upon the absorption of a weak probe field at a particular frequency. Manipulating atom-field interaction on a certain transition by applying drive fields on nearby coupled transitions leads to interesting effects in the absorption spectrum of the weak probe field. We exploit this fact and employ a four-level system with three driving fields and a weak probe field, where one of the drive fields is a standing-wave field of a cavity. We show that the position of an atom along this standing wave is determined when probe field absorption is measured. We find that absorption of the weak probe field at a certain frequency leads to subwavelength localization of the atom in either of the two half-wavelength regions of the cavity field by appropriate choice of the system parameters. We term this result as sub-half-wavelength localization to contrast it with the usual atom localization result of four peaks spread over one wavelength of the standing wave. We observe two localization peaks in either of the two half-wavelength regions along the cavity axis.

  12. atomic power generation: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    a squeezed atom laser is to use Queensland, University of 420 A Silicon-Based Micro Gas Turbine Engine for Power Generation CERN Preprints Summary: This paper reports on our...

  13. Remote generation of entanglement for individual atoms via optical fibers

    E-Print Network [OSTI]

    Y. Q. Guo; H. Y. Zhong; Y. H. Zhang; H. S. Song

    2008-05-29T23:59:59.000Z

    The generation of atomic entanglement is discussed in a system that atoms are trapped in separate cavities which are connected via optical fibers. Two distant atoms can be projected to Bell-state by synchronized turning off the local laser fields and then performing a single quantum measurement by a distant controller. The distinct advantage of this scheme is that it works in a regime that $\\Delta\\approx\\kappa\\gg g$, which makes the scheme insensitive to cavity strong leakage. Moreover, the fidelity is not affected by atomic spontaneous emission.

  14. Observation of recoil-induced resonances and electromagnetically induced absorption of diffuse light by cold atoms

    SciTech Connect (OSTI)

    Zhang Wenzhuo [Key Laboratory of Quantum Optics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800 (China); Graduate University of the Chinese Academy of Sciences, Beijing 100039 (China); Cheng Huadong; Wang Yuzhu [Key Laboratory of Quantum Optics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800 (China); Liu Liang [Key Laboratory of Quantum Optics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800 (China); State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200062 (China)

    2009-05-15T23:59:59.000Z

    In this paper we report an experiment on the observation of the recoil-induced resonances (RIR) and electromagnetically induced absorption (EIA) of cold {sup 87}Rb atoms in diffuse light. The pump light of the RIR and the EIA comes from the diffuse light in an integrating sphere, which also serves the cooling light. We measured the RIR and the EIA signal varying with the detuning of the diffuse laser light, and also measured the number and the temperature of the cold atoms at the different detunings. The mechanism of RIR and EIA in the configuration with diffuse-light pumping and laser probing are discussed, and the difference between the nonlinear spectra of cold atoms in a diffuse-light cooling system and in a magneto-optical trap is studied.

  15. The determination of some anions using ion chromatography and ion chromatography-graphite furnace atomic absorption spectrometry 

    E-Print Network [OSTI]

    Hillman, Daniel C

    1981-01-01T23:59:59.000Z

    THE DETERMINATION OF SOME ANIONS USING ION CHROMATOGRAPHY AND ION CHROMATOGRAPHY-GRAPHITE FURNACE ATOMIC ABSORPTION SPECTROMETRY A Thesis by DANIEL C. J. HILLMAN Submitted to the Graduate College of Texas A&M University in partial fulfillment... of the requirement for the degree of MASTER OF SCIENCE August 1981 Major Subject: Chemistry THE DETERMINATION OF SOME ANIONS USING ION CHROMATOGRAPHY AND ION CHROMATOGRAPHY-GRAPHITE FURNACE ATOMIC ABSORPTION SPECTROMETRY A Thesis by DANIEL C. J. HILLMAN...

  16. Very-high-order harmonic generation from Ar atoms and Ar+ ions in superintense pulsed laser

    E-Print Network [OSTI]

    Chu, Shih-I

    Very-high-order harmonic generation from Ar atoms and Ar+ ions in superintense pulsed laser fields-high-order harmonic generation HHG from Ar atoms and Ar+ ions by means of the self-interaction-free time-order harmonic generation HHG is one of the most rapidly developing topics in the field of laser-atom molecule

  17. Development of mixed-waste analysis capability for graphite furnace atomic absorption spectrophotometry

    SciTech Connect (OSTI)

    Bass, D.A.; TenKate, L.B.; Wroblewski, A.

    1995-03-01T23:59:59.000Z

    Graphite furnace atomic absorption spectrophotometer (GFAAS) are typically configured with ventilation to capture potentially toxic and corrosive gases emitted from the vaporization of sample aliquots. When radioactive elements are present, additional concerns (such as meeting safety guidelines and ALARA principles) must be addressed. This report describes a modification to a GFAAS that provides additional containment of vaporized sample aliquots. The modification was found to increase containment by a factor of 80, given expected operating conditions. The use of the modification allows more mixed-waste samples to be analyzed, permits higher levels of radioactive samples to be analyzed, or exposes the analyst to less airborne radioactivity. The containment apparatus was attached to a Perkin-Elmer Zeeman 5000 spectrophotometer for analysis of mixed-waste samples; however, it could also be used on other systems and in other applications where greater containment of vaporized material is desired.

  18. A passive measurement of dissociated atom densities in atmospheric pressure air discharge plasmas using vacuum ultraviolet self-absorption spectroscopy

    SciTech Connect (OSTI)

    Laity, George [Center for Pulsed Power and Power Electronics, Department of Electrical and Computer Engineering and Department of Physics, Texas Tech University, Lubbock, Texas 79409 (United States); Applied Science and Technology Maturation Department, Sandia National Laboratories, Albuquerque, New Mexico 87123 (United States); Fierro, Andrew; Dickens, James; Neuber, Andreas [Center for Pulsed Power and Power Electronics, Department of Electrical and Computer Engineering and Department of Physics, Texas Tech University, Lubbock, Texas 79409 (United States); Frank, Klaus [Erlangen Centre for Astroparticle Physics, Department of Physics, Friedrich–Alexander University at Erlangen-Nürnberg, 91058 Erlangen (Germany)

    2014-03-28T23:59:59.000Z

    We demonstrate a method for determining the dissociation degree of atmospheric pressure air discharges by measuring the self-absorption characteristics of vacuum ultraviolet radiation from O and N atoms in the plasma. The atom densities are determined by modeling the amount of radiation trapping present in the discharge, without the use of typical optical absorption diagnostic techniques which require external sources of probing radiation into the experiment. For an 8.0?mm spark discharge between needle electrodes at atmospheric pressure, typical peak O atom densities of 8.5?×?10{sup 17}?cm{sup ?3} and peak N atom densities of 9.9?×?10{sup 17}?cm{sup ?3} are observed within the first ?1.0?mm of plasma near the anode tip by analyzing the OI and NI transitions in the 130.0–132.0?nm band of the vacuum ultraviolet spectrum.

  19. SciTech Connect: The determination of aluminum by atomic absorption...

    Office of Scientific and Technical Information (OSTI)

    Language: English Subject: CHEMISTRY; ABSORPTION; ALUMINUM; CEMENTS; CHLORIDES; COMBUSTION; PHOTOMETRY; QUANTITATIVE ANALYSIS; SILICON OXIDES; SOLUTIONS; SPECTROSCOPY; STEELS...

  20. Nonlinear absorption and harmonic generation of laser in a gas with anharmonic clusters

    SciTech Connect (OSTI)

    Kumar, Manoj; Tripathi, V. K. [Department of Physics, Indian Institute of Technology Delhi, New Delhi 110016 (India)

    2013-02-15T23:59:59.000Z

    The nonlinear absorption and harmonic generation of intense short pulse laser in a gas embedded with anharmonic clusters are investigated theoretically. When the laser induced excursion of cluster electrons becomes comparable to cluster radius, the restoration force on electrons no longer remains linearly proportional to the excursion. As a consequence, the plasmon resonance is broadened, leading to broadband laser absorption. It also leads to second and third harmonic generations, at much higher level than the one due to ponderomotive nonlinearity. The harmonic yield is resonantly enhanced at the plasmon resonance {omega}={omega}{sub pe}/{radical}(3), where {omega} is the frequency of the laser and {omega}{sub pe} is the plasma frequency of cluster electrons.

  1. Velocity distribution measurements in atomic beams generated using laser induced back-ablation

    E-Print Network [OSTI]

    Denning, A; Lee, S; Ammonson, M; Bergeson, S D

    2008-01-01T23:59:59.000Z

    We present measurements of the velocity distribution of calcium atoms in an atomic beam generated using a dual-stage laser back-ablation apparatus. Distributions are measured using a velocity selective Doppler time-of-flight technique. They are Boltzmann-like with rms velocities corresponding to temperatures above the melting point for calcium. Contrary to a recent report in the literature, this method does not generate a sub-thermal atomic beam.

  2. atomic beams generated: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    of macroscopic pair-correlated atomic beams by four-wave mixing in Bose-Einstein condensates Condensed Matter (arXiv) Summary: By colliding two Bose-Einstein condensates we...

  3. Theory of attosecond transient absorption spectroscopy of strong-field-generated ions

    SciTech Connect (OSTI)

    Santra, Robin [Center for Free-Electron Laser Science, DESY, Notkestrasse 85, D-22607 Hamburg (Germany); Department of Physics, University of Hamburg, Jungiusstrasse 9, D-20355 Hamburg (Germany); Kavli Institute for Theoretical Physics, University of California, Santa Barbara, California 93106 (United States); Yakovlev, Vladislav S. [Department fuer Physik, Ludwig-Maximilians-Universitaet, Am Coulombwall 1, D-85748 Garching (Germany); Max-Planck-Institut fuer Quantenoptik, Hans-Kopfermann-Strasse 1, D-85748 Garching (Germany); Pfeifer, Thomas [Max Planck Institute for Nuclear Physics, Saupfercheckweg 1, D-69117 Heidelberg (Germany); Loh, Zhi-Heng [Departments of Chemistry and Physics, University of California, Berkeley, California 94720 (United States); Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States)

    2011-03-15T23:59:59.000Z

    Strong-field ionization generally produces ions in a superposition of ionic eigenstates. This superposition is generally not fully coherent and must be described in terms of a density matrix. A recent experiment [E. Goulielmakis et al., Nature (London) 466, 739 (2010)] employed attosecond transient absorption spectroscopy to determine the density matrix of strong-field-generated Kr{sup +} ions. The experimentally observed degree of coherence of the strong-field-generated Kr{sup +} ions is well reproduced by a recently developed multichannel strong-field-ionization theory, but there is significant disagreement between experiment and theory with respect to the degree of alignment of the Kr{sup +} ions. In the present paper, the theory underlying attosecond transient absorption spectroscopy of strong-field-generated ions is developed. The theory is formulated in such a way that the nonperturbative nature of the strong-field-ionization process is systematically taken into account. The impact of attosecond pulse propagation effects on the interpretation of experimental data is investigated both analytically and numerically. It is shown that attosecond pulse propagation effects cannot explain why the experimentally determined degree of alignment of strong-field-generated Kr{sup +} ions is much smaller than predicted by existing theory.

  4. Generation of genuine $?$-type four-particle entangled state of superconducting artificial atoms with broken symmetry

    E-Print Network [OSTI]

    Chun-Ling Leng; Qi Guo; Xin Ji; Shou Zhang

    2014-12-11T23:59:59.000Z

    We propose a scheme for generating a genuine $\\chi$-type four-particle entangled state of superconducting artificial atoms with broken symmetry by using one-dimensional transmission line resonator as a data bus. The $\\Delta$-type three-level artificial atom we use in the scheme is different from natural atom and has cyclic transitions. After suitable interaction time and simple operations, the desired entangled state can be obtained. Since artificial atomic excited states and photonic states are adiabatically eliminated, our scheme is robust against the spontaneous emissions of artificial atoms and the decays of transmission line resonator.

  5. A first principle study for the adsorption and absorption of carbon atom and the CO dissociation on Ir(100) surface

    SciTech Connect (OSTI)

    Erikat, I. A., E-mail: ihsanas@yahoo.com [Department of Physics, Jerash University, Jerash-26150 (Jordan); Hamad, B. A. [Department of Physics, The University of Jordan, Amman-11942 (Jordan)] [Department of Physics, The University of Jordan, Amman-11942 (Jordan)

    2013-11-07T23:59:59.000Z

    We employ density functional theory to examine the adsorption and absorption of carbon atom as well as the dissociation of carbon monoxide on Ir(100) surface. We find that carbon atoms bind strongly with Ir(100) surface and prefer the high coordination hollow site for all coverages. In the case of 0.75?ML coverage of carbon, we obtain a bridging metal structure due to the balance between Ir–C and Ir–Ir interactions. In the subsurface region, the carbon atom prefers the octahedral site of Ir(100) surface. We find large diffusion barrier for carbon atom into Ir(100) surface (2.70 eV) due to the strong bonding between carbon atom and Ir(100) surface, whereas we find a very small segregation barrier (0.22 eV) from subsurface to the surface. The minimum energy path and energy barrier for the dissociation of CO on Ir(100) surface are obtained by using climbing image nudge elastic band. The energy barrier of CO dissociation on Ir(100) surface is found to be 3.01 eV, which is appreciably larger than the association energy (1.61 eV) of this molecule.

  6. Entanglement generation between distant atoms by Lyapunov control

    SciTech Connect (OSTI)

    Wang Xiaoting; Schirmer, S. G. [Department of Applied Maths and Theoretical Physics, University of Cambridge, Wilberforce Road, Cambridge CB3 0WA (United Kingdom)

    2009-10-15T23:59:59.000Z

    We show how to apply Lyapunov control design to the problem of entanglement creation between two atoms in distant cavities connected by optical fibers. The Lyapunov control design is optimal in the sense that the distance from the target state decreases monotonically and exponentially, and the concurrence increases accordingly. This method is far more robust than simple geometric schemes.

  7. New Homogeneous Standards by Atomic Layer Deposition for Synchrotron X-ray Fluorescence and Absorption Spectroscopies.

    SciTech Connect (OSTI)

    Butterworth, A.L.; Becker, N.; Gainsforth, Z.; Lanzirotti, A.; Newville, M.; Proslier, T.; Stodolna, J.; Sutton, S.; Tyliszczak, T.; Westphal, A.J.; Zasadzinski, J. (UCB)

    2012-03-13T23:59:59.000Z

    Quantification of synchrotron XRF analyses is typically done through comparisons with measurements on the NIST SRM 1832/1833 thin film standards. Unfortunately, these standards are inhomogeneous on small scales at the tens of percent level. We are synthesizing new homogeneous multilayer standards using the Atomic Layer Deposition technique and characterizing them using multiple analytical methods, including ellipsometry, Rutherford Back Scattering at Evans Analytical, Synchrotron X-ray Fluorescence (SXRF) at Advanced Photon Source (APS) Beamline 13-ID, Synchrotron X-ray Absorption Spectroscopy (XAS) at Advanced Light Source (ALS) Beamlines 11.0.2 and 5.3.2.1 and by electron microscopy techniques. Our motivation for developing much-needed cross-calibration of synchrotron techniques is borne from coordinated analyses of particles captured in the aerogel of the NASA Stardust Interstellar Dust Collector (SIDC). The Stardust Interstellar Dust Preliminary Examination (ISPE) team have characterized three sub-nanogram, {approx}1{micro}m-sized fragments considered as candidates to be the first contemporary interstellar dust ever collected, based on their chemistries and trajectories. The candidates were analyzed in small wedges of aerogel in which they were extracted from the larger collector, using high sensitivity, high spatial resolution >3 keV synchrotron x-ray fluorescence spectroscopy (SXRF) and <2 keV synchrotron x-ray transmission microscopy (STXM) during Stardust ISPE. The ISPE synchrotron techniques have complementary capabilities. Hard X-ray SXRF is sensitive to sub-fg mass of elements Z {ge} 20 (calcium) and has a spatial resolution as low as 90nm. X-ray Diffraction data were collected simultaneously with SXRF data. Soft X-ray STXM at ALS beamline 11.0.2 can detect fg-mass of most elements, including cosmochemically important oxygen, magnesium, aluminum and silicon, which are invisible to SXRF in this application. ALS beamline 11.0.2 has spatial resolution better than 25 nm. Limiting factors for Stardust STXM analyses were self-imposed limits of photon dose due to radiation damage concerns, and significant attenuation of <1500 eV X-rays by {approx}80{micro}m thick, {approx}25 mg/cm{sup 3} density silica aerogel capture medium. In practice, the ISPE team characterized the major, light elements using STXM (O, Mg, Al, Si) and the heavier minor and trace elements using SXRF. The two data sets overlapped only with minor Fe and Ni ({approx}1% mass abundance), providing few quantitative cross-checks. New improved standards for cross calibration are essential for consortium-based analyses of Stardust interstellar and cometary particles, IDPs. Indeed, they have far reaching application across the whole synchrotron-based analytical community. We have synthesized three ALD multilayers simultaneously on silicon nitride membranes and silicon and characterized them using RBS (on Si), XRF (on Si{sub 3}N{sub 4}) and STXM/XAS (holey Si{sub 3}N{sub 4}). The systems we have started to work with are Al-Zn-Fe and Y-Mg-Er. We have found these ALD multi-layers to be uniform at {micro}m- to nm scales, and have found excellent consistency between four analytical techniques so far. The ALD films can also be used as a standard for e-beam instruments, eg., TEM EELS or EDX. After some early issues with the consistency of coatings to the back-side of the membrane windows, we are confident to be able to show multi-analytical agreement to within 10%. As the precision improves, we can use the new standards to verify or improve the tabulated cross-sections.

  8. Aspects of Graviton Detection: Graviton Emission and Absorption by Atomic Hydrogen

    E-Print Network [OSTI]

    Stephen Boughn; Tony Rothman

    2006-09-27T23:59:59.000Z

    Graviton absorption cross sections and emission rates for hydrogen are calculated by both semi-classical and field theoretic methods. We point out several mistakes in the literature concerning spontaneous emission of gravitons and related phenomena, some of which are due to a subtle issue concerning gauge invariance of the linearized interaction Hamiltonian.

  9. Pressure atomizer having multiple orifices and turbulent generation feature

    DOE Patents [OSTI]

    VanBrocklin, Paul G. (Pittsford, NY); Geiger, Gail E. (Caledonia, NY); Moran, Donald James (Rochester, NY); Fournier, Stephane (Rochester, NY)

    2002-01-01T23:59:59.000Z

    A pressure atomizer includes a silicon plate having a top surface and a bottom surface. A portion of the top surface defines a turbulent chamber. The turbulent chamber is peripherally bounded by the top surface of the plate. The turbulent chamber is recessed a predetermined depth relative to the top surface. The silicon plate further defines at least one flow orifice. Each flow orifice extends from the bottom surface of the silicon plate to intersect with and open into the turbulent chamber. Each flow orifice is in fluid communication with the turbulent chamber.

  10. Generation of Werner states via collective decay of coherently driven atoms

    E-Print Network [OSTI]

    Girish S. Agarwal; Kishore T. Kapale

    2005-10-13T23:59:59.000Z

    We show deterministic generation of Werner states as a steady state of the collective decay dynamics of a pair of neutral atom coupled to a leaky cavity and strong coherent drive. We also show how the scheme can be extended to generate $2N$-particle analogue of the bipartite Werner states.

  11. atomic hydrogen generated: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    hydrogen generated First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Evidence of Catalytic Production of...

  12. Beyond the single-atom response in absorption lineshapes: Probing a dense, laser-dressed helium gas with attosecond pulse trains

    E-Print Network [OSTI]

    Liao, Chen-Ting; Camp, Seth; Schafer, Kenneth J; Gaarde, Mette B

    2015-01-01T23:59:59.000Z

    We investigate the absorption line shapes of laser-dressed atoms beyond the single-atom response, by using extreme ultraviolet (XUV) attosecond pulse trains to probe an optically thick helium target under the influence of a strong infrared (IR) field. We study the interplay between the IR-induced phase shift of the microscopic time-dependent dipole moment and the resonant-propagation-induced reshaping of the macroscopic XUV pulse. Our experimental and theoretical results show that as the optical depth increases, this interplay leads initially to a broadening of the IR-modified line shape, and subsequently to the appearance of new, narrow features in the absorption line.

  13. Generation, characterization and use of atom-resonant indistinguishable photon pairs

    E-Print Network [OSTI]

    Morgan W. Mitchell

    2015-02-26T23:59:59.000Z

    We describe the generation of atom-resonant indistinguishable photon pairs using nonlinear optical techniques, their spectral purification using atomic filters, characterization using multi-photon interference, and application to quantum-enhanced sensing with atoms. Using either type-I or type-II cavity-enhanced spontaneous parametric down-conversion, we generate pairs of photons in the resonant modes of optical cavities with linewidths comparable to the 6 MHz natural linewidth of the D$_1$ line of atomic rubidium. The cavities and pump lasers are tuned so that emission occurs in a mode or a pair of orthogonally-polarized modes that are resonant to the D$_1$ line, at 794.7 nm. The emission from these frequency-degenerate modes is separated from other cavity emission using ultra-narrow atomic frequency filters, either a Faraday anomalous dispersion optical filter (FADOF) with a 445MHz linewidth and 57 dB of out-of-band rejection or an induced dichroism filter with an 80 MHz linewidth and $\\ge$35dB out-of-band rejection. Using the type-I source, we demonstrate interference of photon pair amplitudes against a coherent state and a new method for full characterization of the temporal wave-function of narrow-band photon pairs. With the type-II source we demonstrate high-visibility super-resolving interference, a high-fidelity atom-tuned NooN state, and quantum enhanced sensing of atoms using indistinguishable photon pairs.

  14. Protecting and Dynamically Generating Entanglement in a Two-Atom Two-Field-Mode Model

    E-Print Network [OSTI]

    K. Sinha; N. Cummings; B. L. Hu

    2010-10-06T23:59:59.000Z

    We analyze the time evolution of quantum entanglement in a model consisting of two two-level atoms interacting with a two-mode electromagnetic field for a variety of initial states. We study two different coupling schemes motivated by the forms that can arise due to atomic separation. We observe a variety of qualitative features such as entanglement sudden death, dynamical generation, protection, and transfer between subsystems. Our quantitative analysis shows that these cases with different couplings and initial states differ significantly in these qualitative features. The multifarious behaviors in these two-mode cases suggest the importance of considering atomic separation carefully for any model where two atoms interact with a common field.

  15. Absolute atomic oxygen and nitrogen densities in radio-frequency driven atmospheric pressure cold plasmas: Synchrotron vacuum ultra-violet high-resolution Fourier-transform absorption measurements

    SciTech Connect (OSTI)

    Niemi, K.; O'Connell, D.; Gans, T. [York Plasma Institute, Department of Physics, University of York, York YO10 5DD (United Kingdom); Oliveira, N. de; Joyeux, D.; Nahon, L. [Synchrotron Soleil, l'Orme des Merisiers, St. Aubin BP 48, 91192 Gif sur Yvette Cedex (France); Booth, J. P. [Laboratoire de Physique des Plasmas-CNRS, Ecole Polytechnique, 91128 Palaiseau (France)

    2013-07-15T23:59:59.000Z

    Reactive atomic species play a key role in emerging cold atmospheric pressure plasma applications, in particular, in plasma medicine. Absolute densities of atomic oxygen and atomic nitrogen were measured in a radio-frequency driven non-equilibrium plasma operated at atmospheric pressure using vacuum ultra-violet (VUV) absorption spectroscopy. The experiment was conducted on the DESIRS synchrotron beamline using a unique VUV Fourier-transform spectrometer. Measurements were carried out in plasmas operated in helium with air-like N{sub 2}/O{sub 2} (4:1) admixtures. A maximum in the O-atom concentration of (9.1 {+-} 0.7) Multiplication-Sign 10{sup 20} m{sup -3} was found at admixtures of 0.35 vol. %, while the N-atom concentration exhibits a maximum of (5.7 {+-} 0.4) Multiplication-Sign 10{sup 19} m{sup -3} at 0.1 vol. %.

  16. Arc plasma generator of atomic driver for steady-state negative ion source

    SciTech Connect (OSTI)

    Ivanov, A. A.; Belchenko, Yu. I.; Davydenko, V. I. [Budker Institute of Nuclear Physics, Novosibirsk (Russian Federation) [Budker Institute of Nuclear Physics, Novosibirsk (Russian Federation); Novosibirsk State University, Novosibirsk (Russian Federation); Ivanov, I. A.; Kolmogorov, V. V.; Listopad, A. A., E-mail: a.a.listopad@inp.nsk.su; Mishagin, V. V.; Shulzhenko, G. I. [Budker Institute of Nuclear Physics, Novosibirsk (Russian Federation)] [Budker Institute of Nuclear Physics, Novosibirsk (Russian Federation); Putvinsky, S. V.; Smirnov, A. [Tri Alpha Energy Inc., Rancho Santa Margarita, California 92688 (United States)] [Tri Alpha Energy Inc., Rancho Santa Margarita, California 92688 (United States)

    2014-02-15T23:59:59.000Z

    The paper reviews the results of development of steady-state arc-discharge plasma generator with directly heated LaB{sub 6} cathode. This arc-discharge plasma generator produces a plasma jet which is to be converted into an atomic one after recombination on a metallic plate. The plate is electrically biased relative to the plasma in order to control the atom energies. Such an intensive jet of hydrogen atoms can be used in negative ion sources for effective production of negative ions on a cesiated surface of plasma grid. All elements of the plasma generator have an augmented water cooling to operate in long pulse mode or in steady state. The thermo-mechanical stresses and deformations of the most critical elements of the plasma generator were determined by simulations. Magnetic field inside the discharge chamber was optimized to reduce the local power loads. The first tests of the steady-state arc plasma generator prototype have performed in long-pulse mode.

  17. Two photon absorption and third harmonic generation micro- spectroscopy : hemoglobin and other compounds

    E-Print Network [OSTI]

    Clay, Gabriel Omar

    2006-01-01T23:59:59.000Z

    As the absorption of ultrafast pulses in the vessel lumen isfocussed, ultrafast, ~2 nano-joule laser pulses at selectedwith ultrafast ( ~100-200 fs in duration) laser pulses at

  18. Two-color ghost interference with photon pairs generated in hot atoms

    SciTech Connect (OSTI)

    Ding Dongsheng; Zhou Zhiyuan; Shi Baosen; Zou Xubo; Guo Guangcan [Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei 230026 (China)

    2012-09-15T23:59:59.000Z

    We report on an experimental observation of a two-photon ghost interference experiment. A distinguishing feature of our experiment is that the photons are generated via a non-degenerated spontaneous four-wave mixing process in a hot atomic ensemble; therefore the photon has narrow bandwidth. Besides, there is a large difference in frequency between two photons in a pair. Our works may be important to achieve more secure, large transmission capacity long-distance quantum communication.

  19. Low temperature hydrogen plasma-assisted atomic layer deposition of copper studied using in situ infrared reflection absorption spectroscopy

    SciTech Connect (OSTI)

    Chaukulkar, Rohan P.; Rai, Vikrant R.; Agarwal, Sumit, E-mail: sagarwal@mines.edu [Department of Chemical and Biological Engineering, Colorado School of Mines, Golden, Colorado 80401 (United States); Thissen, Nick F. W. [Department of Applied Physics, Eindhoven University of Technology, 5600 MB Eindhoven (Netherlands)

    2014-01-15T23:59:59.000Z

    Atomic layer deposition (ALD) is an ideal technique to deposit ultrathin, conformal, and continuous metal thin films. However, compared to the ALD of binary materials such as metal oxides and metal nitrides, the surface reaction mechanisms during metal ALD are not well understood. In this study, the authors have designed and implemented an in situ reflection-absorption infrared spectroscopy (IRAS) setup to study the surface reactions during the ALD of Cu on Al{sub 2}O{sub 3} using Cu hexafluoroacetylacetonate [Cu(hfac){sub 2}] and a remote H{sub 2} plasma. Our infrared data show that complete ligand-exchange reactions occur at a substrate temperature of 80?°C in the absence of surface hydroxyl groups. Based on infrared data and previous studies, the authors propose that Cu(hfac){sub 2} dissociatively chemisorbs on the Al{sub 2}O{sub 3} surface, where the Al-O-Al bridge acts as the surface reactive site, leading to surface O-Cu-hfac and O-Al-hfac species. Surface saturation during the Cu(hfac){sub 2} half-cycle occurs through blocking of the available chemisorption sites. In the next half-reaction cycle, H radicals from an H{sub 2} plasma completely remove these surface hfac ligands. Through this study, the authors have demonstrated the capability of in situ IRAS as a tool to study surface reactions during ALD of metals. While transmission and internal reflection infrared spectroscopy are limited to the first few ALD cycles, IRAS can be used to probe all stages of metal ALD starting from initial nucleation to the formation of a continuous film.

  20. atomic nano-generators actinium-225-labeled: Topics by E-print...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    with atomic and molecular matter waves is a rich branch of atomic physics and quantum optics. It started with atom diffraction from crystal surfaces and the separated oscillatory...

  1. High-order harmonic generation in atomic hydrogen at 248 nm: Dipole-moment versus acceleration spectrum

    E-Print Network [OSTI]

    Jiang, Tsin-Fu; Chu, Shih-I

    1992-12-01T23:59:59.000Z

    We present a study of the high-order harmonic-generation (HG) spectra of atomic hydrogen at 248 nm based on the Fourier transform of the expectation values of the induced dipole moment and acceleration. The calculations ...

  2. Experimental generation of tripartite telecom photons via an atomic ensemble and a nonlinear waveguide

    E-Print Network [OSTI]

    Dong-Sheng Ding; Wei Zhang; Shuai Shi; Zhi-Yuan Zhou; Yan Li; Bao-Sen Shi; Guang-Can Guo

    2015-01-12T23:59:59.000Z

    Non-classical multi-photon and number states attracts many people because of their wide applications in fundamental quantum mechanics tests, quantum metrology and quantum computation, therefore it is a longstanding aim to generate such states experimentally. Here, we prepare photon triplets by using the spontaneously Raman scattering process in a hot atomic ensemble cascaded by the spontaneous parametric down conversion process in a periodical poled nonlinear waveguide, the strong temporal correlations of these three photons are observed. Our experiment represents the first combination of the different order nonlinear processes and different physical systems, showing the feasibility of such composite system in this research direction. In addition, the all photons in the prepared genuine triplet are in telecom band make them be suitable for long-distance quantum communication in optical fibre.

  3. COMBUSTION DRIVEN ATOMIC FLUORINE GENERATORS FOR DF CHEMICAL LASERS Abstract -Conventional high pressure corabustors delivering atomic fluorine for DF chemical

    E-Print Network [OSTI]

    Paris-Sud XI, Université de

    compositions assuming frozen isentropic expansion and with or without heat losses in the combustor. The values production at good overall laser power. 1. INTRODUCTION Available references describing combustors for also reactants. Solid propellant com- high production of F atom by thermal equilibrium positions such as NF

  4. Catheter based mid-infrared reflectance and reflectance generated absorption spectroscopy

    DOE Patents [OSTI]

    Holman, Hoi-Ying N

    2013-10-29T23:59:59.000Z

    A method of characterizing conditions in a tissue, by (a) providing a catheter that has a light source that emits light in selected wavenumbers within the range of mid-IR spectrum; (b) directing the light from the catheter to an area of tissue at a location inside a blood vessel of a subject; (c) collecting light reflected from the location and generating a reflectance spectra; and (d) comparing the reflectance spectra to a reference spectra of normal tissue, whereby a location having an increased number of absorbance peaks at said selected wavenumbers indicates a tissue inside the blood vessel containing a physiological marker for atherosclerosis.

  5. Characteristics of cooperative spontaneous radiation with applications to atom microscopy and coherent XUV radiation generation

    E-Print Network [OSTI]

    Chang, Juntao

    2009-05-15T23:59:59.000Z

    quicker than single atom decay, with a decay rate proportional to N(?/R)2, where N is the atom numbers, R is the size of the atom cloud, and ? is the wavelength. We call it Markovian regime because the sytem does not persist memory effect. The other regime...

  6. FINGERPRINTING INORGANIC ARSENIC AND ORGANOARSENIC COMPOUNDS IN IN SITU OIL SHALE RETORT AND PROCESS VOTERS USING A LIQUID CHROMATOGRAPH COUPLED WITH AN ATOMIC ABSORPTION SPECTROMETER AS A DETECTOR

    SciTech Connect (OSTI)

    Fish, Richard H.; Brinckman, Frederick E.; Jewett, Kenneth L.

    1981-07-01T23:59:59.000Z

    Inorganic arsenic and organoarsenic compounds were speciated in seven oil shale retort and process waters, including samples from simulated, true and modified in situ processes, using a high performance liquid chromatograph automatically coupled to a graphite furnace atomic absorption detector. The molecular forms of arsenic at ppm levels (({micro}g/mL) in these waters are identified for the first time, and shown to include arsenate, methylarsonic acid and phenylarsonic acid. An arsenic-specific fingerprint chromatogram of each retort or process water studied has significant impliestions regarding those arsenical species found and those marginally detected, such as dimethylarsinic acid and the suspected carcinogen arsenite. The method demonstrated suggests future means for quantifying environmental impacts of bioactive organometal species involved in oil shale retorting technology.

  7. Generating Entanglement between Atomic Spins with Low-Noise Probing of an Optical Cavity

    E-Print Network [OSTI]

    Cox, Kevin C; Greve, Graham P; Thompson, James K

    2015-01-01T23:59:59.000Z

    Atomic projection noise limits the ultimate precision of all atomic sensors, including clocks, inertial sensors, magnetometers, etc. The independent quantum collapse of $N$ atoms into a definite state (for example spin up or down) leads to an uncertainty $\\Delta \\theta_{SQL}=1/\\sqrt{N}$ in the estimate of the quantum phase accumulated during a Ramsey sequence or its many generalizations. This phase uncertainty is referred to as the standard quantum limit. Creating quantum entanglement between the $N$ atoms can allow the atoms to partially cancel each other's quantum noise, leading to reduced noise in the phase estimate below the standard quantum limit. Recent experiments have demonstrated up to $10$~dB of phase noise reduction relative to the SQL by making collective spin measurements. This is achieved by trapping laser-cooled Rb atoms in an optical cavity and precisely measuring the shift of the cavity resonance frequency by an amount that depends on the number of atoms in spin up. Detecting the probe light ...

  8. Generating Entanglement between Atomic Spins with Low-Noise Probing of an Optical Cavity

    E-Print Network [OSTI]

    Kevin C. Cox; Joshua M. Weiner; Graham P. Greve; James K. Thompson

    2015-04-20T23:59:59.000Z

    Atomic projection noise limits the ultimate precision of all atomic sensors, including clocks, inertial sensors, magnetometers, etc. The independent quantum collapse of $N$ atoms into a definite state (for example spin up or down) leads to an uncertainty $\\Delta \\theta_{SQL}=1/\\sqrt{N}$ in the estimate of the quantum phase accumulated during a Ramsey sequence or its many generalizations. This phase uncertainty is referred to as the standard quantum limit. Creating quantum entanglement between the $N$ atoms can allow the atoms to partially cancel each other's quantum noise, leading to reduced noise in the phase estimate below the standard quantum limit. Recent experiments have demonstrated up to $10$~dB of phase noise reduction relative to the SQL by making collective spin measurements. This is achieved by trapping laser-cooled Rb atoms in an optical cavity and precisely measuring the shift of the cavity resonance frequency by an amount that depends on the number of atoms in spin up. Detecting the probe light with high total efficiency reduces excess classical and quantum back-action of the probe. Here we discuss recent progress and a technique for reducing the relative frequency noise between the probe light and the optical cavity, a key requirement for further advances.

  9. High Harmonic Generation and the Role of Atomic Orbital Wave Functions

    SciTech Connect (OSTI)

    Levesque, J. [National Research Council of Canada, 100 Sussex Drive, Ottawa, Ontario K1A 0R6 (Canada); INRS-Energie et Materiaux, 1650 boul. Lionel-Boulet, C.P. 1020, Varennes (Quebec) J3X 1S2 (Canada); Zeidler, D. [National Research Council of Canada, 100 Sussex Drive, Ottawa, Ontario K1A 0R6 (Canada); Carl Zeiss SMT AG, Rudolf-Eber-Str. 2, 73447 Oberkochen (Germany); Marangos, J. P. [The Blackett Laboratory, Imperial College London, Prince Consort Road, London SW7 2BW (United Kingdom); Corkum, P. B.; Villeneuve, D. M. [National Research Council of Canada, 100 Sussex Drive, Ottawa, Ontario K1A 0R6 (Canada)

    2007-05-04T23:59:59.000Z

    High harmonic spectra were recorded from different rare-gas atoms under identical experimental conditions. It is shown that although each atom's spectrum is different, the differences are due almost entirely to the orbital influence in the recombination step. The amplitude of the continuum electron wave packet versus kinetic energy is derived from these data and is shown to be largely independent of the atom, in agreement with models of tunnel ionization. We compare the measurements with calculations in both the length gauge and the velocity gauge and show that the two gauges imply a different de Broglie wavelength.

  10. Kinetics of generation, relaxation, and accumulation of electronic excitations under two-photon interband picosecond absorption in tungstate and molibdate crystals

    SciTech Connect (OSTI)

    Lukanin, V. I.; Karasik, A. Ya., E-mail: karasik@lst.gpi.ru [Russian Academy of Sciences, Prokhorov General Physics Institute (Russian Federation)

    2013-08-15T23:59:59.000Z

    Under two-photon 523.5 nm interband picosecond laser excitation, we measured the kinetics of induced absorption in PbWO{sub 4}, ZnWO{sub 4}, and PbMoO{sub 4} crystals with 532 to 633 nm continuous probe radiation. We obtained real-time information about the dynamics of the generation, relaxation, and accumulations of electronic excitations over a wide time range (from picoseconds to hundreds of seconds) and the 77-300 K temperature range. For the studied crystals, exponential temperature-independent growth of the induced absorption (IA) with 60 ns rise time reflects the dynamics of the generation of electronic excitation. The kinetics of the IA exponential growth with temperature-dependent 3.5-11 {mu}s time constants reflect the dynamics of energy migration between neighboring tungstate (molibdate) ions to traps for the studied crystals. The multiexponential relaxation absorption kinetics strongly depend on temperature, and the relaxation decay time of induced absorption increased from tens to hundreds of milliseconds to seconds under crystal cooling from 300 to 77 K. We found that the increase in the laser pump repetition rate (0-10 Hz) leads to the accumulation of electronic excitations. Control of the repetition rate and the number of excitations allowed us to change the relaxation time of the induced absorption by more than two orders of magnitude. Due to accumulation of excitations at 77 K, the absorption relaxation time can exceed 100 s for PbWO{sub 4} and PbMoO{sub 4} crystals. In the initially transparent crystals, two-photon interband absorption (2PA) leads to crystals opacity at the 523 and 633 nm wavelengths. (An inverse optical transmission of the crystals exceeds 50-55 at a 50-100 GW/cm{sup 2} pump intensity.) Measured at {approx}1 mW probe radiation of 532 and 633 nm wavelengths, the induced absorption values are comparable with those obtained under two-photon absorption at {approx}5 kW pump power. An optical 2PA shutter for the visible spectral range is proposed with a variable shutting time from hundreds of microseconds to tens of seconds.

  11. Seven-effect absorption refrigeration

    DOE Patents [OSTI]

    DeVault, Robert C. (Knoxville, TN); Biermann, Wendell J. (Fayetteville, NY)

    1989-01-01T23:59:59.000Z

    A seven-effect absorption refrigeration cycle is disclosed utilizing three absorption circuits. In addition, a heat exchanger is used for heating the generator of the low absorption circuit with heat rejected from the condenser and absorber of the medium absorption circuit. A heat exchanger is also provided for heating the generator of the medium absorption circuit with heat rejected from the condenser and absorber of the high absorption circuit. If desired, another heat exchanger can also be provided for heating the evaporator of the high absorption circuit with rejected heat from either the condenser or absorber of the low absorption circuit.

  12. Seven-effect absorption refrigeration

    DOE Patents [OSTI]

    DeVault, R.C.; Biermann, W.J.

    1989-05-09T23:59:59.000Z

    A seven-effect absorption refrigeration cycle is disclosed utilizing three absorption circuits. In addition, a heat exchanger is used for heating the generator of the low absorption circuit with heat rejected from the condenser and absorber of the medium absorption circuit. A heat exchanger is also provided for heating the generator of the medium absorption circuit with heat rejected from the condenser and absorber of the high absorption circuit. If desired, another heat exchanger can also be provided for heating the evaporator of the high absorption circuit with rejected heat from either the condenser or absorber of the low absorption circuit. 1 fig.

  13. Comparative investigation of third- and fifth-harmonic generation in atomic and molecular gases driven by midinfrared ultrafast laser pulses

    SciTech Connect (OSTI)

    Ni Jielei; Yao Jinping; Zeng Bin; Chu Wei; Li Guihua; Zhang Haisu; Jing Chenrui [State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, P.O. Box 800-211, Shanghai 201800 (China); Graduate School of the Chinese Academy of Sciences, Beijing 100039 (China); Chin, S. L. [Department of Physics, Engineering Physics and Optics, and Center for Optics, Photonics and Laser (COPL), Laval University, Laval, Quebec, G1K 7P4 (Canada); Cheng, Y.; Xu, Z. [State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, P.O. Box 800-211, Shanghai 201800 (China)

    2011-12-15T23:59:59.000Z

    We report on the comparative experimental investigation on third- and fifth-harmonic generation (THG and FHG) in atomic and molecular gases driven by midinfrared ultrafast laser pulses at a wavelength of {approx}1500 nm. We observe that the conversion efficiencies of both the THG and FHG processes saturate at similar peak intensities close to {approx}1.5 x 10{sup 14} W/cm{sup 2} for argon, nitrogen, and air, whose ionization potentials are close to each other. Near the saturation intensity, the ratio of yields of the FHG and THG reaches {approx}10{sup -1} for all the gases. Our results show that high-order Kerr effect seems to exist; however, contribution from the fourth-order Kerr refractive index coefficient alone is insufficient to balance the Kerr self-focusing without the assistance of plasma generation.

  14. Atomic resolution mapping of the excited-state electronic structure of Cu2O with time-resolved x-ray absorption spectroscopy

    SciTech Connect (OSTI)

    Hillyard, P. W.; Kuchibhatla, S. V. N. T.; Glover, T. E.; Hertlein, M. P.; Huse, Nils; Nachimuthu, P.; Saraf, L. V.; Thevuthasan, S.; Gaffney, K. J.

    2010-05-02T23:59:59.000Z

    We have used time-resolved soft x-ray spectroscopy to investigate the electronic structure of optically excited cuprous oxide at the O K-edge and the Cu L3-edge. The 400 nm optical excitation shifts the Cu and O absorptions to lower energy, but does not change the integrated x-ray absorption significantly for either edge. The constant integrated x-ray absorption cross-section indicates that the conduction-band and valence-band edges have very similar Cu 3d and O 2p orbital contributions. The 2.1 eV optical band gap of Cu2O significantly exceeds the one eV shift in the Cu L3- and O K-edges absorption edges induced by optical excitation, demonstrating the importance of core-hole excitonic effects and valence electron screening in the x-ray absorption process.

  15. Generation of Free Oxygen Atoms O(3P) in Solution by Photolysis of 4-Benzoylpyridine N-Oxide

    SciTech Connect (OSTI)

    Carraher, Jack M. [Ames Laboratory; Bakac, Andreja [Ames Laboratory

    2014-08-04T23:59:59.000Z

    Laser flash photolysis of 4-benzoylpyridine N-oxide (BPyO) at 308 nm in aqueous solutions generates a triplet excited state 3BPyO* that absorbs strongly in the visible, ?max 490 and 380 nm. 3BPyO* decays with the rate law kdecay/s?1 = (3.3 ± 0.9) × 104 + (1.5 ± 0.2) × 109 [BPyO] to generate a mixture of isomeric hydroxylated benzoylpyridines, BPy(OH), in addition to small amounts of oxygen atoms, O(3P). Molecular oxygen quenches 3BPyO*, kQ = 1.4 × 109 M?1 s?1, but the yields of O(3P) increase in O2-saturated solutions to 36%. Other triplet quenchers have a similar effect, which rules out the observed 3BPyO* as a source of O(3P). It is concluded that O(3P) is produced from either 1BPyO* or a short-lived, unobserved, higher energy triplet generated directly from 1BPyO*. 3BPyO* is reduced by Fe2+ and by ABTS2? to the radical anion BPyO?? which exhibits a maximum at 510 nm, ? = 2200 M?1 cm?1. The anion engages in back electron transfer with ABTS?? with k = 1.7 × 109 M?1 s?1. The same species can be generated by reducing ground state BPyO with ?C(CH3)2OH. The photochemistry of BPyO in acetonitrile is similar to that in aqueous solutions.

  16. New generation polyphase resonant converter-modulators for the Korean atomic energy research institute

    SciTech Connect (OSTI)

    Reass, William A [Los Alamos National Laboratory; Baca, David M [Los Alamos National Laboratory; Gribble, Robert F [Los Alamos National Laboratory

    2009-01-01T23:59:59.000Z

    This paper will present operational data and performance parameters of the newest generation polyphase resonant high voltage converter modulator (HVCM) as developed and delivered to the KAERI 100 MeV ''PEFP'' accelerator [1]. The KAERI design realizes improvements from the SNS and SLAC designs [2]. To improve the IGBT switching performance at 20 kHz for the KAERI system, the HVCM utilizes the typical zero-voltage-switching (ZVS) at turn on and as well as artificial zero-current-switching (ZCS) at turn-off. The new technique of artificial ZCS technique should result in a 6 fold reduction of IGBT switching losses (3). This improves the HCVM conversion efficiency to better than 95% at full average power, which is 500 kW for the KAERI two klystron 105 kV, 50 A application. The artificial ZCS is accomplished by placing a resonant RLC circuit across the input busswork to the resonant boost transformer. This secondary resonant circuit provides a damped ''kick-back'' to assist in IGBT commutation. As the transformer input busswork is extremely low inductance (< 10 nH), the single RLC network acts like it is across each of the four IGBT collector-emitter terminals of the H-bridge switching network. We will review these topological improvements and the overall system as delivered to the KAERI accelerator and provide details of the operational results.

  17. Non-local Quantum Electrodynamics; 2, Possibility of correlated 2n-photon absorption in gases leading to VERY High frequency spontaneous emission and Very high order Harmonic Generation

    E-Print Network [OSTI]

    Dastidar, K R; Dastidar, Krishna Rai

    2002-01-01T23:59:59.000Z

    In a recent work [Mod. Phys. Lett A13, p-1265 (1998)] we expounded a non-local Quantum Electrodynamics (QED) which predicted a linear two-photon absorption by an atom placed in a laser field of appropriate intensity and frequency. In this paper we extend our earlier work to show that the theory allows for linear 2n-photon absorption by gaseous matter where, under suitable conditions, n may literally run upto thousands. The consequences of this extension of the theory are outlined and predictions are made which may be verified in laboratories.

  18. Potassium emission absorption system. Topical report 12

    SciTech Connect (OSTI)

    Bauman, L.E.

    1995-04-01T23:59:59.000Z

    The Potassium Emission Absorption System is one of the advanced optical diagnostics developed at Mississippi State University to provide support for the demonstration of prototype-scale coal-fired combustion magnetohydrodynamic (MHD) electrical power generation. Intended for application in the upstream of an MHD flow, the system directly measures gas temperature and neutral potassium atom number density through spectroscopic emission absorption techniques. From these measurements the electron density can be inferred from a statistical equilibrium calculation and the electron conductivity in the MHD channel found by use of an electron mobility model. The instrument has been utilized for field test measurements on MHD facilities for almost a decade and has been proven to provide useful measurements as designed for MHD nozzle, channel, and diffuser test sections. The theory of the measurements, a system description, its capabilities, and field test measurement results are reported here. During the development and application of the instrument several technical issues arose which when addressed advanced the state of the art in emission absorption measurement. Studies of these issues are also reported here and include: two-wavelength measurements for particle-laden flows, potassium D-line far wing absorption coefficient, bias in emission absorption measurements arising from dirty windows and misalignments, non-coincident multiwavelength emission absorption sampling errors, and lineshape fitting for boundary layer flow profile information. Although developed for NLHD application, the instrument could be applied to any high temperature flow with a resonance line in the 300 to 800 nm range, for instance other types of flames, rocket plumes or low temperature plasmas.

  19. JOURNAL DE PHYSIQUE ColZoque C9, suppZe'ment au nO1l, Tome 41, novembre 1980, page C9-449 A POTENTIAL ATOMIC IODINE LASER PUMPED BY ELECTRICALLY GENERATED 'A OXYGEN

    E-Print Network [OSTI]

    Paris-Sud XI, Université de

    -449 A POTENTIAL ATOMIC IODINE LASER PUMPED BY ELECTRICALLY GENERATED 'A OXYGEN G. Fournier, J. Bonnet and D ation. This paper shows that an electron generator of 1~ oxygen [21 . A condition beam controlled discharge could be an for lasing is a concentration ratio ['A] / efficient oxygen generator to lase with C3z

  20. Very-high-order harmonic generation from Ar atoms and Ar+ ions in superintense pulsed laser fields: An ab initio self-interaction-free time-dependent density-functional approach

    E-Print Network [OSTI]

    Carrera, Juan J.; Chu, Shih-I; Tong, Xiao-Min

    2005-06-21T23:59:59.000Z

    We present an ab initio nonpertubative investigation of the mechanisms responsible for the production of very-high-order harmonic generation (HHG) from Ar atoms and Ar+ ions by means of the self-interaction-free time-dependent density...

  1. absorption leaves: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    2007. ESTIMATION OF VANADIUM IN SELECTED LEAVES FROM AKURE, NIGERIA BY ATOMIC ABSORPTION SPECTROPHOTOMETRY. CiteSeer Summary: Estimation of the levels of vanadium in...

  2. Improved graphite furnace atomizer

    DOE Patents [OSTI]

    Siemer, D.D.

    1983-05-18T23:59:59.000Z

    A graphite furnace atomizer for use in graphite furnace atomic absorption spectroscopy is described wherein the heating elements are affixed near the optical path and away from the point of sample deposition, so that when the sample is volatilized the spectroscopic temperature at the optical path is at least that of the volatilization temperature, whereby analyteconcomitant complex formation is advantageously reduced. The atomizer may be elongated along its axis to increase the distance between the optical path and the sample deposition point. Also, the atomizer may be elongated along the axis of the optical path, whereby its analytical sensitivity is greatly increased.

  3. Dynamics of oxygen Rydberg atom generation following O 1s inner-shell excitation of H{sub 2}O

    SciTech Connect (OSTI)

    Gejo, T., E-mail: gejo@sci.u-hyogo.ac.jp; Ikegami, T.; Honma, K. [University of Hyogo, Koto 3-2-1, Kamigori-cho, Ako-gun, Hyogo 678-1297 (Japan); Takahashi, O. [Hiroshima University, 2-2 Kagamiyama 1-chome, Higashihiroshima 739-8512 (Japan); Shigemasa, E. [UVSOR Facility, Institute for Molecular Science, 38 Nishigo-Naka, Myodaiji, Okazaki 444-8585 (Japan); Hikosaka, Y. [Department of Environmental Science, Niigata University, 8050, Ikarashi 2-no-cho, Nishi-ku, Niigata 950-2181 (Japan); Tamenori, Y. [JASRI, Koto 1-1-1, Sayo-cho, Hyogo 679-5198 (Japan)

    2014-06-07T23:59:59.000Z

    The emission of low-energy electrons from H{sub 2}O has been investigated at photon excitation energies in the vicinity of the O 1s ionization threshold. Neutral oxygen Rydberg atoms (O*) were found to form, and the correlation between the initial inner-shell excited state of H{sub 2}O and the Rydberg state of O* was determined. The initially excited electron in a Rydberg orbital is shown to remain associated with O* even after the cleavage of two O-H bonds. We also show that the energy discrepancy between two Rydberg states of H{sub 2}O and O* can be explained by the influence of the post-collision interaction, which becomes stronger as the excitation energy approaches the 1s ionization threshold.

  4. Multiphoton ionization and high-order harmonic generation of He, Ne, and Ar atoms in intense pulsed laser fields: Self-interaction-free time-dependent density-functional theoretical approach

    E-Print Network [OSTI]

    Chu, Shih-I; Tong, Xiao-Min

    2001-06-12T23:59:59.000Z

    We present a detailed study of the multiphoton ionization and high-order harmonic generation (HHG) processes of rare-gas atoms (He, Ne, and Ar) in intense pulsed laser fields by means of a self-interaction-free time-dependent density...

  5. Elastic modulus mapping of atomically thin film based Lithium Ion Battery electrodes Lithium Ion Batteries (LIB) are one of the most promising class of next generation energy storage devices,

    E-Print Network [OSTI]

    Batteries (LIB) are one of the most promising class of next generation energy storage devices, which canElastic modulus mapping of atomically thin film based Lithium Ion Battery electrodes Lithium Ion the charging/discharging which otherwise lead to in efficient battery operation. The cyclically charging

  6. Comparative analysis of the high-order harmonic generation in the laser ablation plasmas prepared on the surfaces of complex and atomic targets

    SciTech Connect (OSTI)

    Ganeev, R. A. [Scientific Association Akadempribor, Academy of Sciences of Uzbekistan, Akademgorodok, Tashkent 100125 (Uzbekistan); Institute for Solid State Physics, University of Tokyo, 5-1-5 Kashiwanoha, Kashiwa, Chiba 277-8581 (Japan); Milosevic, D. B. [Faculty of Science, University of Sarajevo, Zmaja od Bosne 35, 71000 Sarajevo (Bosnia and Herzegowina); Max-Born-Institut, Max-Born-Strasse 2a, 12489 Berlin (Germany)

    2008-07-15T23:59:59.000Z

    We analyzed high-order harmonic generation from the plasma plumes prepared on the surfaces of complex targets. The studies of In-Ag targets showed that the characteristics of the high-order harmonics from the double-target plume were the same as those from the single-target plasmas. For the chromium-tellurium plasma, the enhancements of the 29th and 27th harmonics were obtained, thus indicating the appearance of the enhancement properties from both components of the double-target plasma. These comparative studies also showed higher enhancement of a single harmonic in the case of atomic plasma (Sb) with regard to the molecular one (InSb). The additional component can only decrease the enhancement factor of the medium, due to the change of the oscillator strength and spectral distribution of the transitions involved in the resonance enhancement of the specific harmonic order. The theoretical calculations have shown the enhancement of specific harmonics for the Sb, Te, and Cr plasmas in the double-target configurations.

  7. Calibration of a single atom detector for atomic micro chips

    E-Print Network [OSTI]

    A. Stibor; S. Kraft; T. Campey; D. Komma; A. Günther; J. Fortágh; C. J. Vale; H. Rubinsztein-Dunlop; C. Zimmermann

    2007-02-13T23:59:59.000Z

    We experimentally investigate a scheme for detecting single atoms magnetically trapped on an atom chip. The detector is based on the photoionization of atoms and the subsequent detection of the generated ions. We describe the characterization of the ion detector with emphasis on its calibration via the correlation of ions with simultaneously generated electrons. A detection efficiency of 47.8% (+-2.6%) is measured, which is useful for single atom detection, and close to the limit allowing atom counting with sub-Poissonian uncertainty.

  8. Detection of transient fluorine atoms

    SciTech Connect (OSTI)

    Loge, G.W.; Nereson, N.; Fry, H.A.

    1986-01-01T23:59:59.000Z

    A KrF eximer laser with a fluence of 50 mJ/cm/sup 2/ was used to photolyze either uranium hexafluoride or molecular fluorine, yielding a transient number density of fluorine atoms. The rise and decay of the atomic fluorine density was observed by transient absorption of a 25-..mu..m Pb-salt diode laser. To prevent the diode laser wavelength from drifting out of resonance with the atomic fluorine line, part of the beam was split off and sent through a microwave discharge fluorine atom cell. This allowed a wavelength modulation-feedback technique to be used to lock the diode laser wavelength onto the atomic line. The remaining diode laser beam was made collinear with the eximer laser beam using a LiF window with a 45/sup 0/ angle of incidence to reflect the infrared beam while transmitting most of the uv beam. Using this setup along with a transient digitizer to average between 100 and 200 transient absorption profiles, fluorine atom number densities on the order of 10/sup 14/ cm/sup -3/ in a 1.7 m pathlength were detected. The signals observed were about a factor of two less than expected from known photolysis and atomic fluorine absorption cross-sections. 2 refs., 4 figs.

  9. Optical control of nuclear resonant absorption: theory and experiment 

    E-Print Network [OSTI]

    Kolesov, Roman L.

    2004-09-30T23:59:59.000Z

    Modification of nuclear resonant absorption by means of laser radiation is analyzed both theoretically and experimentally. Theoretical analysis is done on the basis of four-level model of atom. This model includes both electronic and nuclear...

  10. Optical control of nuclear resonant absorption: theory and experiment

    E-Print Network [OSTI]

    Kolesov, Roman L.

    2004-09-30T23:59:59.000Z

    Modification of nuclear resonant absorption by means of laser radiation is analyzed both theoretically and experimentally. Theoretical analysis is done on the basis of four-level model of atom. This model includes both electronic and nuclear...

  11. absorption des wasserstoffs: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    . . . . . . . . 41 3.2.2 Kristallines Eis im Volumen Wolf, Martin 5 ABSORPTION PHOTOLECTRIQUE DES RAYONS 03B3 DANS LA COUCHE L DES ATOMES Par Mme NADINE MARTY....

  12. Oral Drug Absorption

    E-Print Network [OSTI]

    Yamashita, Shinji

    2006-10-26T23:59:59.000Z

    properties ? membrane permeability ? metabolic stability ? enzyme inhibition or induction ? protein binding ? transporter affinity ?. Chemical Optimization DDS technology 4 Strategy of Drug Delivery Absorption Distribution Metabolism Excretion Improve of drug... absorption absorption enhancement controlled releasecontrolled release new administration route Drug targeting to the tissue to the cell to the organelle Dr. Shinji Yamashita (Setsunan University) Issue: Oral Drug Absorption Dr. Valentino J. Stella...

  13. Atomic magnetometer

    DOE Patents [OSTI]

    Schwindt, Peter (Albuquerque, NM); Johnson, Cort N. (Albuquerque, NM)

    2012-07-03T23:59:59.000Z

    An atomic magnetometer is disclosed which uses a pump light beam at a D1 or D2 transition of an alkali metal vapor to magnetically polarize the vapor in a heated cell, and a probe light beam at a different D2 or D1 transition to sense the magnetic field via a polarization rotation of the probe light beam. The pump and probe light beams are both directed along substantially the same optical path through an optical waveplate and through the heated cell to an optical filter which blocks the pump light beam while transmitting the probe light beam to one or more photodetectors which generate electrical signals to sense the magnetic field. The optical waveplate functions as a quarter waveplate to circularly polarize the pump light beam, and as a half waveplate to maintain the probe light beam linearly polarized.

  14. Polymer microcantilevers fabricated via multiphoton absorption polymerization

    E-Print Network [OSTI]

    Teich, Malvin C.

    Polymer microcantilevers fabricated via multiphoton absorption polymerization Z. Bayindir, Y. Sun polymer cantilevers. Atomic force microscopy has been used to characterize the mechanical properties orders of magnitude smaller than would be predicted from the properties of the bulk polymer.6 If correct

  15. Lyman-alpha Absorption from Heliosheath Neutrals

    E-Print Network [OSTI]

    Brian E. Wood; Vladislav V. Izmodenov; Jeffrey L. Linsky; Yury G. Malama

    2006-11-30T23:59:59.000Z

    We assess what information HST observations of stellar Ly-alpha lines can provide on the heliosheath, the region of the heliosphere between the termination shock and heliopause. To search for evidence of heliosheath absorption, we conduct a systematic inspection of stellar Ly-alpha lines reconstructed after correcting for ISM absorption (and heliospheric/astrospheric absorption, if present). Most of the stellar lines are well centered on the stellar radial velocity, as expected, but the three lines of sight with the most downwind orientations relative to the ISM flow (Chi1 Ori, HD 28205, and HD 28568) have significantly blueshifted Ly-alpha lines. Since it is in downwind directions where heliosheath absorption should be strongest, the blueshifts are almost certainly caused by previously undetected heliosheath absorption. We make an initial comparison between the heliosheath absorption and the predictions of a pair of heliospheric models. A model with a complex multi-component treatment of plasma within the heliosphere predicts less absorption than a model with a simple single-fluid treatment, which leads to better agreement with the data. Finally, we find that nonplanetary energetic neutral atom (ENA) fluxes measured by the ASPERA-3 instrument on board Mars Express, which have been interpreted as being from the heliosheath, are probably too high to be consistent with the relative lack of heliosheath absorption seen by HST. This would argue for a local interplanetary source for these ENAs instead of a heliosheath source.

  16. Chemical factors influencing selenium atomization

    E-Print Network [OSTI]

    Buren, Mary Sue

    1980-01-01T23:59:59.000Z

    Atomization. (August 1980) Mary Sue Buren, B, S. , Angelo State University Chairman of Advisory Comm1ttee: Dr. Thomas M. Vickrey Selenium in an acid1c matrix was analyzed using graphite furnace atom1c absorption with Zeeman-effect background correct1on.... Nickel(II} and lanthanum( III) were introduced as matrix modifiers to determine their effect on interferences 1n selenium atom1zation. In add1tion to matr1x mod1ficat1on, surface coating the graphite furnace with z1rconium and tantalum salts was also...

  17. Chemical factors influencing selenium atomization 

    E-Print Network [OSTI]

    Buren, Mary Sue

    1980-01-01T23:59:59.000Z

    Atomization. (August 1980) Mary Sue Buren, B, S. , Angelo State University Chairman of Advisory Comm1ttee: Dr. Thomas M. Vickrey Selenium in an acid1c matrix was analyzed using graphite furnace atom1c absorption with Zeeman-effect background correct1on.... Nickel(II} and lanthanum( III) were introduced as matrix modifiers to determine their effect on interferences 1n selenium atom1zation. In add1tion to matr1x mod1ficat1on, surface coating the graphite furnace with z1rconium and tantalum salts was also...

  18. Analysis of interference in attosecond transient absorption in adiabatic condition

    E-Print Network [OSTI]

    Dong, Wenpu; Wang, Xiaowei; Zhao, Zengxiu

    2015-01-01T23:59:59.000Z

    We simulate the transient absorption of attosecond pulses of infrared laser-dressed atoms by considering a three-level system with the adiabatic approximation. We study the delay-dependent interference features in the transient absorption spectra of helium atoms from the perspective of the coherent interaction processes between the attosecond pulse and the quasi-harmonics, and find that many features of the interference fringes in the absorption spectra of the attosecond pulse can be attributed to the coherence phase difference. And the modulation signals of laser-induced sidebands of the dark state is found related to the dark state with population modulated by the dressing field.

  19. Characterization of the molecular structure and mechanical properties of polymer surfaces and protein/polymer interfaces by sum frequency generation vibrational spectroscopy and atomic force microscopy

    SciTech Connect (OSTI)

    Koffas, Telly Stelianos

    2004-05-15T23:59:59.000Z

    Sum frequency generation (SFG) vibrational spectroscopy, atomic force microscopy (AFM), and other complementary surface-sensitive techniques have been used to study the surface molecular structure and surface mechanical behavior of biologically-relevant polymer systems. SFG and AFM have emerged as powerful analytical tools to deduce structure/property relationships, in situ, for polymers at air, liquid and solid interfaces. The experiments described in this dissertation have been performed to understand how polymer surface properties are linked to polymer bulk composition, substrate hydrophobicity, changes in the ambient environment (e.g., humidity and temperature), or the adsorption of macromolecules. The correlation of spectroscopic and mechanical data by SFG and AFM can become a powerful methodology to study and engineer materials with tailored surface properties. The overarching theme of this research is the interrogation of systems of increasing structural complexity, which allows us to extend conclusions made on simpler model systems. We begin by systematically describing the surface molecular composition and mechanical properties of polymers, copolymers, and blends having simple linear architectures. Subsequent chapters focus on networked hydrogel materials used as soft contact lenses and the adsorption of protein and surfactant at the polymer/liquid interface. The power of SFG is immediately demonstrated in experiments which identify the chemical parameters that influence the molecular composition and ordering of a polymer chain's side groups at the polymer/air and polymer/liquid interfaces. In general, side groups with increasingly greater hydrophobic character will be more surface active in air. Larger side groups impose steric restrictions, thus they will tend to be more randomly ordered than smaller hydrophobic groups. If exposed to a hydrophilic environment, such as water, the polymer chain will attempt to orient more of its hydrophilic groups to the surface in order to minimize the total surface energy. With an understanding of the structural and environmental parameters which govern polymer surface structure, SFG is then used to explore the effects of surface hydrophobicity and solvent polarity on the orientation and ordering of amphiphilic neutral polymers adsorbed at the solid/liquid interface. SFG spectra show that poly(propylene glycol) (PPG) and poly(ethylene glycol) (PEG) adsorb with their hydrophobic moieties preferentially oriented toward hydrophobic polystyrene surfaces. These same moieties, however, disorder when adsorbed onto a hydrophilic silica/water interface. Water is identified as a critical factor for mediating the orientation and ordering of hydrophobic moieties in polymers adsorbed at hydrophobic interfaces. The role of bulk water content and water vapor, as they influence hydrogel surface structure and mechanics, continues to be explored in the next series of experiments. A method was developed to probe the surface viscoelastic properties of hydroxylethyl methacrylate (HEMA) based contact lens materials by analyzing AFM force-distance curves. AFM analysis indicates that the interfacial region is dehydrated, relative to the bulk. Experiments performed on poly(HEMA+MA) (MA = methacrylic acid), a more hydrophilic copolymer with greater bulk water content, show even greater water depletion at the surface. SFG spectra, as well as surface energy arguments, suggest that the more hydrophilic polymer component (such as MA) is not favored at the air interface; this may explain anomalies in water retention at the hydrogel surface. Adsorption of lysozyme onto poly(HEMA+MA) was found to further reduce near-surface viscous behavior, suggesting lower surface water content. Lastly, protein adsorption is studied using a model polymer system of polystyrene covalently bound with a monolayer of bovine serum albumin. SFG results indicate that some amino acid residues in proteins adopt preferred orientations. SFG spectra also show that the phenyl rings of the bare polystyrene substrate in contact with air or

  20. Dilution cycle control for an absorption refrigeration system

    DOE Patents [OSTI]

    Reimann, Robert C. (Lafayette, NY)

    1984-01-01T23:59:59.000Z

    A dilution cycle control system for an absorption refrigeration system is disclosed. The control system includes a time delay relay for sensing shutdown of the absorption refrigeration system and for generating a control signal only after expiration of a preselected time period measured from the sensed shutdown of the absorption refrigeration system, during which the absorption refrigeration system is not restarted. A dilution cycle for the absorption refrigeration system is initiated in response to generation of a control signal by the time delay relay. This control system is particularly suitable for use with an absorption refrigeration system which is frequently cycled on and off since the time delay provided by the control system prevents needless dilution of the absorption refrigeration system when the system is turned off for only a short period of time and then is turned back on.

  1. A narrow window of Rabi frequency for competition between electromagnetically induced transparency and Raman absorption

    SciTech Connect (OSTI)

    Chang, Ray-Yuan; Fang, Wei-Chia; Lee, Ming-Tsung; He, Zong-Syun; Ke, Bai-Cian [Department of Physics, National Cheng-Kung University, Tainan 70101, Taiwan (China); Lee, Yi-Chi [Institute of Electro-Optical Science and Engineering, National Cheng-Kung University, Tainan 70101, Taiwan (China); Tsai, Chin-Chun [Department of Physics, National Cheng-Kung University, Tainan 70101, Taiwan (China); Institute of Electro-Optical Science and Engineering, National Cheng-Kung University, Tainan 70101, Taiwan (China)

    2010-01-15T23:59:59.000Z

    This investigation clarifies the transition phenomenon between the electromagnetically induced transparency (EIT) and Raman absorption in a ladder-type system of Doppler-broadened cesium vapor. A competition window of this transition was found to be as narrow as 2 MHz defined by the probe Rabi frequency. For a weak probe, the spectrum of EIT associated with quantum interference suggests that the effect of the Doppler velocity on the spectrum is negligible. When the Rabi frequency of the probe becomes comparable with the effective decay rate, an electromagnetically induced absorption (EIA) dip emerges at the center of the power broadened EIT peak. While the Rabi frequency of the probe exceeds the effective decay rate, decoherence that is generated by the intensified probe field occurs and Raman absorption dominates the interaction process, yielding a pure absorption spectrum; the Doppler velocity plays an important role in the interaction. A theory that is based on density matrix simulation, with or without the Doppler effect, can qualitatively fit the experimental data. In this work, the coherence of atom-photon interactions is created or destroyed using the probe Rabi frequency as a decoherence source.

  2. Delay in Atomic Photoionization

    SciTech Connect (OSTI)

    Kheifets, A. S. [Research School of Physical Sciences, Australian National University, Canberra ACT 0200 (Australia); Kavli Institute for Theoretical Physics, University of California, Santa Barbara, California 93106-4030 (United States); Ivanov, I. A. [Research School of Physical Sciences, Australian National University, Canberra ACT 0200 (Australia)

    2010-12-03T23:59:59.000Z

    We analyze the time delay between emission of photoelectrons from the outer valence ns and np subshells in noble gas atoms following absorption of an attosecond extreme ultraviolet pulse. Various processes such as elastic scattering of the photoelectron on the parent ion and many-electron correlation affect the apparent 'time zero' when the photoelectron leaves the atom. This qualitatively explains the time delay between photoemission from the 2s and 2p subshells of Ne as determined experimentally by attosecond streaking [Science 328, 1658 (2010)]. However, with our extensive numerical modeling, we were only able to account for less than half of the measured time delay of 21{+-}5 as. We argue that the extreme ultraviolet pulse alone cannot produce such a large time delay and it is the streaking IR field that is most likely responsible for this effect.

  3. Coherent Atom Optics with fast metastable rare gas atoms

    SciTech Connect (OSTI)

    Grucker, J.; Baudon, J.; Karam, J.-C.; Perales, F.; Vassilev, G.; Ducloy, M. [Laboratoire de Physique des Lasers, Universite Paris 13, Avenue J.B. Clement, 93430-Villetaneuse (France); Bocvarski, V. [Institute of Physics, Pregrevica 118, 11080 - Belgrade-Zemun (Serbia and Montenegro)

    2006-12-01T23:59:59.000Z

    Coherent atom optics experiments making use of an ultra-narrow beam of fast metastable atoms generated by metastability exchange are reported. The transverse coherence of the beam (coherence radius of 1.7 {mu}m for He*, 1.2 {mu}m for Ne*, 0.87 {mu}m for Ar*) is demonstrated via the atomic diffraction by a non-magnetic 2{mu}m-period reflection grating. The combination of the non-scalar van der Waals (vdW) interaction with the Zeeman interaction generated by a static magnetic field gives rise to ''vdW-Zeeman'' transitions among Zeeman sub-levels. Exo-energetic transitions of this type are observed with Ne*(3P2) atoms traversing a copper micro-slit grating. They can be used as a tunable beam splitter in an inelastic Fresnel bi-prism atom interferometer.

  4. Quantum-fluid-dynamics approach for strong-field processes: Application to the study of multiphoton ionization and high-order harmonic generation of He and Ne atoms

    E-Print Network [OSTI]

    Chu, Shih-I

    of the hydrodynamical density and wave function in space and time. The procedure is applied to the study of multiphoton for Ne, good agreement is achieved. Four different exchange-correlation energy functionals are used systems. Among these novel high-intensity phenomena, multiple high-order har- monic generation HHG

  5. Generation and diagnostics of atmospheric pressure CO{sub 2} plasma by laser driven plasma wind tunnel

    SciTech Connect (OSTI)

    Matsui, Makoto; Yamagiwa, Yoshiki [Department of Mechanical Engineering, Shizuoka University, 3-5-4 Johoku, Naka, Hamamatsu, 432-8561 Shizuoka (Japan); Tanaka, Kensaku; Arakawa, Yoshihiro [Department of Aeronautics and Astronautics, University of Tokyo, 7-3-1 Hongo, Bunkyo, 113-0033 Tokyo (Japan); Nomura, Satoshi; Komurasaki, Kimiya [Department of Advanced Energy, University of Tokyo, 5-1-5 Kashiwanoha, Kashiwa, 277-8583 Chiba (Japan)

    2012-08-01T23:59:59.000Z

    Atmospheric pressure CO{sub 2} plasma was generated by a laser driven plasma wind tunnel. At an ambient pressure of 0.38 MPa, a stable plasma was maintained by a laser power of 1000 W for more than 20 min. The translational temperature was measured using laser absorption spectroscopy with the atomic oxygen line at 777.19 nm. The measured absorption profiles were analyzed by a Voigt function considering Doppler, Stark, and pressure-broadening effects. Under the assumption of thermochemical equilibrium, all broadening effects were consistent with each other. The measured temperature ranged from 8500 K to 8900 K.

  6. Coupled dual loop absorption heat pump

    DOE Patents [OSTI]

    Sarkisian, Paul H. (Watertown, MA); Reimann, Robert C. (Lafayette, NY); Biermann, Wendell J. (Fayetteville, NY)

    1985-01-01T23:59:59.000Z

    A coupled dual loop absorption system which utilizes two separate complete loops. Each individual loop operates at three temperatures and two pressures. This low temperature loop absorber and condenser are thermally coupled to the high temperature loop evaporator, and the high temperature loop condenser and absorber are thermally coupled to the low temperature generator.

  7. Absorption machine with desorber-resorber

    DOE Patents [OSTI]

    Biermann, Wendell J. (Fayetteville, NY)

    1985-01-01T23:59:59.000Z

    An absorption refrigeration system utilizing a low temperature desorber and intermediate temperature resorber. The system operates at three temperatures and three pressures to increase the efficiency of the system and is capable of utilizing a lower generator temperature than previously used.

  8. Carbon Dioxide Capture by Chemical Absorption: A Solvent Comparison Study

    E-Print Network [OSTI]

    1 Carbon Dioxide Capture by Chemical Absorption: A Solvent Comparison Study by Anusha Kothandaraman Students #12;2 #12;3 Carbon Dioxide Capture by Chemical Absorption: A Solvent Comparison Study by Anusha with electricity generation accounting for 40% of the total1 . Carbon capture and sequestration (CCS) is one

  9. Triple effect absorption chiller utilizing two refrigeration circuits

    DOE Patents [OSTI]

    DeVault, Robert C. (Knoxville, TN)

    1988-01-01T23:59:59.000Z

    A triple effect absorption method and apparatus having a high coefficient of performance. Two single effect absorption circuits are combined with heat exchange occurring between a condenser and absorber of a high temperature circuit, and a generator of a low temperature circuit. The evaporators of both the high and low temperature circuits provide cooling to an external heat load.

  10. Absorption heat pump system

    DOE Patents [OSTI]

    Grossman, Gershon (Oak Ridge, TN)

    1984-01-01T23:59:59.000Z

    The efficiency of an absorption heat pump system is improved by conducting liquid from a second stage evaporator thereof to an auxiliary heat exchanger positioned downstream of a primary heat exchanger in the desorber of the system.

  11. Absorption heat pump system

    DOE Patents [OSTI]

    Grossman, G.

    1982-06-16T23:59:59.000Z

    The efficiency of an absorption heat pump system is improved by conducting liquid from a second stage evaporator thereof to an auxiliary heat exchanger positioned downstream of a primary heat exchanger in the desorber of the system.

  12. Solar selective absorption coatings

    DOE Patents [OSTI]

    Mahoney, Alan R. (Albuquerque, NM); Reed, Scott T. (Albuquerque, NM); Ashley, Carol S. (Albuquerque, NM); Martinez, F. Edward (Horseheads, NY)

    2004-08-31T23:59:59.000Z

    A new class of solar selective absorption coatings are disclosed. These coatings comprise a structured metallic overlayer such that the overlayer has a sub-micron structure designed to efficiently absorb solar radiation, while retaining low thermal emissivity for infrared thermal radiation. A sol-gel layer protects the structured metallic overlayer from mechanical, thermal, and environmental degradation. Processes for producing such solar selective absorption coatings are also disclosed.

  13. Solar selective absorption coatings

    DOE Patents [OSTI]

    Mahoney, Alan R. (Albuquerque, NM); Reed, Scott T. (Albuquerque, NM); Ashley, Carol S. (Albuquerque, NM); Martinez, F. Edward (Horseheads, NY)

    2003-10-14T23:59:59.000Z

    A new class of solar selective absorption coatings are disclosed. These coatings comprise a structured metallic overlayer such that the overlayer has a sub-micron structure designed to efficiently absorb solar radiation, while retaining low thermal emissivity for infrared thermal radiation. A sol-gel layer protects the structured metallic overlayer from mechanical, thermal, and environmental degradation. Processes for producing such solar selective absorption coatings are also disclosed.

  14. Optical absorption measurement system

    DOE Patents [OSTI]

    Draggoo, Vaughn G. (Livermore, CA); Morton, Richard G. (San Diego, CA); Sawicki, Richard H. (Pleasanton, CA); Bissinger, Horst D. (Livermore, CA)

    1989-01-01T23:59:59.000Z

    The system of the present invention contemplates a non-intrusive method for measuring the temperature rise of optical elements under high laser power optical loading to determine the absorption coefficient. The method comprises irradiating the optical element with a high average power laser beam, viewing the optical element with an infrared camera to determine the temperature across the optical element and calculating the absorption of the optical element from the temperature.

  15. Atom Interferometry

    ScienceCinema (OSTI)

    Mark Kasevich

    2010-01-08T23:59:59.000Z

    Atom de Broglie wave interferometry has emerged as a tool capable of addressing a diverse set of questions in gravitational and condensed matter physics, and as an enabling technology for advanced sensors in geodesy and navigation. This talk will review basic principles, then discuss recent applications and future directions. Scientific applications to be discussed include measurement of G (Newton?s constant), tests of the Equivalence Principle and post-Newtonian gravity, and study of the Kosterlitz-Thouless phase transition in layered superfluids. Technology applications include development of precision gryoscopes and gravity gradiometers. The talk will conclude with speculative remarks looking to the future: Can atom interference methods be sued to detect gravity waves? Can non-classical (entangled/squeezed state) atom sources lead to meaningful sensor performance improvements?

  16. Advanced regenerative absorption refrigeration cycles

    DOE Patents [OSTI]

    Dao, Kim (14 Nace Ave., Piedmont, CA 94611)

    1990-01-01T23:59:59.000Z

    Multi-effect regenerative absorption cycles which provide a high coefficient of performance (COP) at relatively high input temperatures. An absorber-coupled double-effect regenerative cycle (ADR cycle) (10) is provided having a single-effect absorption cycle (SEA cycle) (11) as a topping subcycle and a single-effect regenerative absorption cycle (1R cycle) (12) as a bottoming subcycle. The SEA cycle (11) includes a boiler (13), a condenser (21), an expansion device (28), an evaporator (31), and an absorber (40), all operatively connected together. The 1R cycle (12) includes a multistage boiler (48), a multi-stage resorber (51), a multisection regenerator (49) and also uses the condenser (21), expansion device (28) and evaporator (31) of the SEA topping subcycle (11), all operatively connected together. External heat is applied to the SEA boiler (13) for operation up to about 500 degrees F., with most of the high pressure vapor going to the condenser (21) and evaporator (31) being generated by the regenerator (49). The substantially adiabatic and isothermal functioning of the SER subcycle (12) provides a high COP. For higher input temperatures of up to 700 degrees F., another SEA cycle (111) is used as a topping subcycle, with the absorber (140) of the topping subcycle being heat coupled to the boiler (13) of an ADR cycle (10). The 1R cycle (12) itself is an improvement in that all resorber stages (50b-f) have a portion of their output pumped to boiling conduits (71a-f) through the regenerator (49), which conduits are connected to and at the same pressure as the highest pressure stage (48a) of the 1R multistage boiler (48).

  17. Absorption heat pump system

    DOE Patents [OSTI]

    Grossman, Gershon (Oak Ridge, TN); Perez-Blanco, Horacio (Knoxville, TN)

    1984-01-01T23:59:59.000Z

    An improvement in an absorption heat pump cycle is obtained by adding adiabatic absorption and desorption steps to the absorber and desorber of the system. The adiabatic processes make it possible to obtain the highest temperature in the absorber before any heat is removed from it and the lowest temperature in the desorber before heat is added to it, allowing for efficient utilization of the thermodynamic availability of the heat supply stream. The improved system can operate with a larger difference between high and low working fluid concentrations, less circulation losses, and more efficient heat exchange than a conventional system.

  18. Absorption free superluminal light propagation in a three level pump-probe system

    E-Print Network [OSTI]

    M. Mahmoudi; S. Worya Rabiei; L. Ebrahimi Zohravi; M. Sahrai

    2007-11-21T23:59:59.000Z

    We investigate the dispersion and the absorption properties of a weak probe field in a three-level pump-probe atomic system. It is shown that the slope of dispersion changes from positive to negative just with the intensity of the coherent or indirect incoherent pumping fields. It is demonstrated that the absorption free superluminal light propagation is appeared in this system.

  19. Structure in multilayer films of zinc sulfide and copper sulfide via atomic layer deposition

    SciTech Connect (OSTI)

    Short, Andrew; Jewell, Leila; Bielecki, Anthony; Keiber, Trevor; Bridges, Frank; Carter, Sue; Alers, Glenn, E-mail: galers@ucsc.edu [Department of Physics, University of California at Santa Cruz, 1156 High Street, Santa Cruz, California 95064 (United States)

    2014-01-15T23:59:59.000Z

    Multilayer film stacks of ZnS and Cu{sub x}S (x???2) were made via atomic layer deposition. The precursors were bis(2,2,6,6-tetramethyl-3,5-heptanedionato)zinc, bis(2,2,6,6-tetramethyl-3,5-heptanedionato)copper, and H{sub 2}S generated in situ for sulfur. Samples were deposited at 200?°C, in layers ranging from approximately 2 to 20 nm thick, based on binary growth rates. The properties of the film stacks were studied with atomic force microscopy, ultraviolet–visible spectroscopy, and extended x-ray absorption fine structure. The results demonstrate that the structure of films with the thinnest layers is dominated by Cu{sub x}S, whereas in the thicker films, the structure is determined by whichever material is first deposited. This can be attributed to the crystal structure mismatch of ZnS and Cu{sub x}S.

  20. Analysis of Enhanced Two-Photon Absorption in Tapered Optical Fibers

    E-Print Network [OSTI]

    Hao You; S. M. Hendrickson; J. D. Franson

    2008-09-30T23:59:59.000Z

    We analyze the rate of two-photon absorption in tapered optical fibers with diameters less than the wavelength of the incident light. The rate of two-photon absorption is shown to be enhanced due to the small mode volume of the tapered fiber and the relatively large overlap of the evanescent field with an atomic vapor that surrounds the tapered region. The two-photon absorption rate is optimized as a function of the diameter of the tapered region.

  1. Intrinsic AGN Absorption Lines

    E-Print Network [OSTI]

    Fred Hamann

    2000-06-12T23:59:59.000Z

    Strong absorption lines are common in rest-frame UV spectra of AGNs due to a variety of resonant transitions, for example the HI Lyman series lines (most notably Ly-alpha 1216) and high-ionization doublets like CIV 1549,1551. The lines are called ``intrinsic'' if the absorbing gas is physically related to the AGN, e.g. if the absorber resides broadly within the radius of the AGN's surrounding ``host'' galaxy. Intrinsic absorption lines are thus valuable probes of the kinematics, physical conditions and elemental abundances in the gas near AGNs. Studies of intrinsic absorbers have historically emphasized the broad absorption lines (BALs) in quasars. Today we recognize a wider variety of intrinsic lines in a wider range of objects. For example, we now know that Seyfert 1 galaxies (the less luminous cousins of quasars) have intrinsic absorption. We also realize that intrinsic lines can form in a range of AGN environments --- from the dynamic inner regions like the BALs, to the more quiescent outer host galaxies >10 kpc away. This article provides a brief introduction to current observational and theoretical work on intrinsic AGN absorbers.

  2. AAS, see Atomic absorption spectrometry Acanthes lanceolata, 138

    E-Print Network [OSTI]

    Pitt, Robert E.

    ­112 selection of optimal assessment parameters, 113­118 specific study objectives and goals, 110 case case studies, 205­213 parallel creeks experimental design, 139­168 example outline of comprehensive studies of previous receiving water evaluations, 123­213 current, ongoing, stormwater projects, 181

  3. atomic-absorption spectrometry determinacion: Topics by E-print...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    (arXiv) Summary: A Monte Carlo code, known as AASI, is developed for simulating energy spectra in alpha spectrometry. The code documented here is a comprehensive package...

  4. Elementary reaction rate measurements at high temperatures by tunable-laser flash-absorption

    SciTech Connect (OSTI)

    Hessler, J.P. [Argonne National Laboratory, IL (United States)

    1993-12-01T23:59:59.000Z

    The major objective of this program is to measure thermal rate coefficients and branching ratios of elementary reactions. To perform these measurements, the authors constructed an ultrahigh-purity shock tube to generate temperatures between 1000 and 5500 K. The tunable-laser flash-absorption technique is used to measure the rate of change of the concentration of species which absorb below 50,000 cm{sup {minus}1} e.g.: OH, CH, and CH{sub 3}. This technique is being extended into the vacuum-ultraviolet spectral region where one can measure atomic species e.g.: H, D, C, O, and N; and diatomic species e.g.: O{sub 2}, CO, and OH.

  5. Measuring Atomic Properties with an Atom Interferometer

    E-Print Network [OSTI]

    Roberts, Tony David

    2006-06-28T23:59:59.000Z

    Two experiments are presented which measure atomic properties using an atom interferometer. The interferometer splits the sodium de Broglie wave into two paths,

  6. Suppression of thermal carrier escape and efficient photo-carrier generation by two-step photon absorption in InAs quantum dot intermediate-band solar cells using a dot-in-well structure

    SciTech Connect (OSTI)

    Asahi, S.; Teranishi, H.; Kasamatsu, N.; Kada, T.; Kaizu, T.; Kita, T. [Department of Electrical and Electronic Engineering, Graduate School of Engineering, Kobe University, 1-1 Rokkodai, Nada, Kobe 657-8501 (Japan)

    2014-08-14T23:59:59.000Z

    We investigated the effects of an increase in the barrier height on the enhancement of the efficiency of two-step photo-excitation in InAs quantum dot (QD) solar cells with a dot-in-well structure. Thermal carrier escape of electrons pumped in QD states was drastically reduced by sandwiching InAs/GaAs QDs with a high potential barrier of Al{sub 0.3}Ga{sub 0.7}As. The thermal activation energy increased with the introduction of the barrier. The high potential barrier caused suppression of thermal carrier escape and helped realize a high electron density in the QD states. We observed efficient two-step photon absorption as a result of the high occupancy of the QD states at room temperature.

  7. The Quantum Absorption Refrigerator

    E-Print Network [OSTI]

    Amikam Levy; Ronnie Kosloff

    2011-11-09T23:59:59.000Z

    A quantum absorption refrigerator driven by noise is studied with the purpose of determining the limitations of cooling to absolute zero. The model consists of a working medium coupled simultaneously to hot, cold and noise baths. Explicit expressions for the cooling power are obtained for Gaussian and Poisson white noise. The quantum model is consistent with the first and second laws of thermodynamics. The third law is quantified, the cooling power J_c vanishes as J_c proportional to T_c^{alpha}, when T_c approach 0, where alpha =d+1 for dissipation by emission and absorption of quanta described by a linear coupling to a thermal bosonic field, where d is the dimension of the bath.

  8. Laser-excited atomic fluorescence spectrometry in a graphite furnace with an

    E-Print Network [OSTI]

    Michel, Robert G.

    must provide high peak energy above sequentially with the analysis time determined primarilyLaser-excited atomic fluorescence spectrometry in a graphite furnace with an optical parametric for electrothermal atomic excited atomic ¯ uorescence spectrometry (LEAFS ) in a absorption spectrometry (ETAAS

  9. Atomic physics: An almost lightless laser

    E-Print Network [OSTI]

    Vuletic, Vladan

    Lasers are often described in terms of a light field circulating in an optical resonator system. Now a laser has been demonstrated in which the field resides primarily in the atomic medium that is used to generate the light.

  10. Absorption features of high redshift galactic winds

    E-Print Network [OSTI]

    A. P. M. Fangano; A. Ferrara; P. Richter

    2007-06-11T23:59:59.000Z

    The environment of high-redshift galaxies is characterized by both wind-driven outflowing gas and gravitationally infalling streams. To investigate such galaxy-IGM interplay we have generated synthetic optical absorption line spectra piercing the volume surrounding a starbursting analog of a Lyman Break Galaxy selected in a $z \\approx 3$ output from a SPH simulation, including a detailed treatment of mechanical feedback from winds. Distributions for several observable species (HI, CIII, CIV, SiII, SiIII, SiIV, OVI, OVII, and OVIII) have been derived by post-processing the simulation outputs. The hot wind material is characterized by the presence of high-ionization species such as OVI, OVII, and OVIII (the latter two observable only in X-ray bands); the colder ($Tgas clumps. However, both line profile and Pixel Optical Depth analysis of the synthetic spectra show that the intergalactic filament in which the wind-blowing galaxy is embedded produces absorption signatures that closely mimic those of the wind environment. We conclude that may be difficult to clearly identify wind-blowing galaxies and their complex gaseous environment at high redshift in optical QSO absorption-line spectra based solely on the observed ion absorption patterns.

  11. Phonon mediated electromagnetically induced absorption in cavity optomechanics

    E-Print Network [OSTI]

    Qu, Kenan

    2013-01-01T23:59:59.000Z

    We predict the existence of the electromagnetically induced absorption (EIA) in the double cavity configurations of the optomechanical systems (OMS). We discuss the origin of the EIA in OMS which exhibit the existence of an absorption peak within the transparency window. We provide analytical results for the width and the height of the EIA peak. The combination of the EIT and EIA is especially useful for photon switching applications. The EIA that we discuss is different from the one originally discovered by Lezama et al in atomic systems and can be understood in terms of the dynamics of three coupled oscillators (rather than two) under different conditions on the relaxation parameters.

  12. Molecular shock response of explosives: electronic absorption spectroscopy

    SciTech Connect (OSTI)

    Mcgrne, Shawn D [Los Alamos National Laboratory; Moore, David S [Los Alamos National Laboratory; Whitley, Von H [Los Alamos National Laboratory; Bolme, Cindy A [Los Alamos National Laboratory; Eakins, Daniel E [Los Alamos National Laboratory

    2009-01-01T23:59:59.000Z

    Electronic absorption spectroscopy in the range 400-800 nm was coupled to ultrafast laser generated shocks to begin addressing the question of the extent to which electronic excitations are involved in shock induced reactions. Data are presented on shocked polymethylmethacrylate (PMMA) thin films and single crystal pentaerythritol tetranitrate (PETN). Shocked PMMA exhibited thin film interference effects from the shock front. Shocked PETN exhibited interference from the shock front as well as broadband increased absorption. Relation to shock initiation hypotheses and the need for time dependent absorption data (future experiments) is briefly discussed.

  13. Engineering atom-atom thermal entanglement via two-photon process

    E-Print Network [OSTI]

    Y. Q. Guo; L. Zhou; H. S. Song

    2005-09-21T23:59:59.000Z

    We study the system that two atoms simultaneously interact with a single-mode thermal field via different couplings and different spontaneous emission rates when two-photon process is involved. It is found that we indeed can employ the different couplings to produce the atom-atom thermal entanglement in two-photon process. The different atomic spontaneous emission rates are also utilizable in generating thermal entanglement. We also investigate the effect of the cavity leakage. To the initial atomic state $|ee> ,$a slight leakage can relieve the restriction of interaction time and we can obtain a large and steady entanglement.

  14. Antiproton Absorption in Nuclei

    E-Print Network [OSTI]

    Yu. T. Kiselev; E. Ya. Paryev

    2006-01-24T23:59:59.000Z

    We present the analysis of experimental data on forward antiproton production on nuclei. The calculations are done in the framework of a folding model which takes properly into account both incoherent direct proton-nucleon and cascade pion-nucleon antiproton production processes as well as internal nucleon momentum distribution. The effective antiproton-nucleon cross section in nuclear matter and the imaginary part of the antiproton nuclear optical potential are estimated to be 25-45 mb and -(38-56) MeV at normal nuclear matter density, respectively. The results of the performed analysis evidence for the decreasing of antiproton absorption in the nuclear medium.

  15. OPTICAL DIFFERENCE FREQUENCY GENERATION OF FAR INFRARED RADIATION

    E-Print Network [OSTI]

    Morris, J.R.

    2010-01-01T23:59:59.000Z

    Absorption on Far-Infrared Generation IV. V. Comparison withIII CHAPTER IV. PHASE MATCHED FAR-INFRARED GENERATION BY THE1970). CHAPTER IV. PHASE MATCHED FAR-INFRARED GENERATION BY

  16. Method of trivalent chromium concentration determination by atomic spectrometry

    DOE Patents [OSTI]

    Reheulishvili, Aleksandre N. (Tbilisi, 0183, GE); Tsibakhashvili, Neli Ya. (Tbilisi, 0101, GE)

    2006-12-12T23:59:59.000Z

    A method is disclosed for determining the concentration of trivalent chromium Cr(III) in a sample. The addition of perchloric acid has been found to increase the atomic chromium spectrometric signal due to Cr(III), while leaving the signal due to hexavalent chromium Cr(VI) unchanged. This enables determination of the Cr(III) concentration without pre-concentration or pre-separation from chromium of other valences. The Cr(III) concentration may be measured using atomic absorption spectrometry, atomic emission spectrometry or atomic fluorescence spectrometry.

  17. Method of performing MRI with an atomic magnetometer

    DOE Patents [OSTI]

    Savukov, Igor Mykhaylovich; Matlashov, Andrei Nikolaevich; Espy, Michelle A; Volegov, Petr Lvovich; Kraus, Jr., Robert Henry; Zotev, Vadim Sergeyevich

    2013-08-27T23:59:59.000Z

    A method and apparatus are provided for performing an in-situ magnetic resonance imaging of an object. The method includes the steps of providing an atomic magnetometer, coupling a magnetic field generated by magnetically resonating samples of the object through a flux transformer to the atomic magnetometer and measuring a magnetic resonance of the atomic magnetometer.

  18. Method of performing MRI with an atomic magnetometer

    DOE Patents [OSTI]

    Savukov, Igor Mykhaylovich; Matlashov, Andrei Nikolaevich; Espy, Michelle A.; Volegov, Petr Lvovich; Kraus, Jr., Robert Henry; Zotev, Vadim Sergeyevich

    2012-11-06T23:59:59.000Z

    A method and apparatus are provided for performing an in-situ magnetic resonance imaging of an object. The method includes the steps of providing an atomic magnetometer, coupling a magnetic field generated by magnetically resonating samples of the object through a flux transformer to the atomic magnetometer and measuring a magnetic resonance of the atomic magnetometer.

  19. PHOTOIONIZATION MODELING OF OXYGEN K ABSORPTION IN THE INTERSTELLAR MEDIUM: THE CHANDRA GRATING SPECTRA OF XTE J1817-330

    SciTech Connect (OSTI)

    Gatuzz, E.; Mendoza, C. [Centro de Fisica, Instituto Venezolano de Investigaciones Cientificas (IVIC), P.O. Box 20632, Caracas 1020A (Venezuela, Bolivarian Republic of); Garcia, J.; Lohfink, A. [Department of Astronomy and Maryland Astronomy Center for Theory and Computation, University of Maryland, College Park, MD 20742 (United States); Kallman, T. R.; Witthoeft, M. [NASA Goddard Space Flight Center, Greenbelt, MD 20771 (United States); Bautista, M. A. [Department of Physics, Western Michigan University, Kalamazoo, MI 49008 (United States); Palmeri, P.; Quinet, P., E-mail: egatuzz@ivic.gob.ve, E-mail: claudio@ivic.gob.ve, E-mail: javier@astro.umd.edu, E-mail: alohfink@astro.umd.edu, E-mail: timothy.r.kallman@nasa.gov, E-mail: michael.c.witthoeft@nasa.gov, E-mail: manuel.bautista@wmich.edu, E-mail: palmeri@umons.ac.be, E-mail: quinet@umons.ac.be [Astrophysique et Spectroscopie, Universite de Mons-UMONS, B-7000 Mons (Belgium)

    2013-05-01T23:59:59.000Z

    We present detailed analyses of oxygen K absorption in the interstellar medium (ISM) using four high-resolution Chandra spectra toward the X-ray low-mass binary XTE J1817-330. The 11-25 A broadband is described with a simple absorption model that takes into account the pile-up effect and results in an estimate of the hydrogen column density. The oxygen K-edge region (21-25 A) is fitted with the physical warmabs model, which is based on a photoionization model grid generated with the XSTAR code with the most up-to-date atomic database. This approach allows a benchmark of the atomic data which involves wavelength shifts of both the K lines and photoionization cross sections in order to fit the observed spectra accurately. As a result we obtain a column density of N{sub H} = 1.38 {+-} 0.01 Multiplication-Sign 10{sup 21} cm{sup -2}; an ionization parameter of log {xi} = -2.70 {+-} 0.023; an oxygen abundance of A{sub O}= 0.689{sup +0.015}{sub -0.010}; and ionization fractions of O I/O = 0.911, O II/O = 0.077, and O III/O = 0.012 that are in good agreement with results from previous studies. Since the oxygen abundance in warmabs is given relative to the solar standard of Grevesse and Sauval, a rescaling with the revision by Asplund et al. yields A{sub O}=0.952{sup +0.020}{sub -0.013}, a value close to solar that reinforces the new standard. We identify several atomic absorption lines-K{alpha}, K{beta}, and K{gamma} in O I and O II and K{alpha} in O III, O VI, and O VII-the last two probably residing in the neighborhood of the source rather than in the ISM. This is the first firm detection of oxygen K resonances with principal quantum numbers n > 2 associated with ISM cold absorption.

  20. 7, 71717233, 2007 Aerosol absorption

    E-Print Network [OSTI]

    Paris-Sud XI, Université de

    black carbon refractive indices, new cloud radiative properties considering the effect of aerosol absorption and radiative forcing. The effect of the usage of more accurate effective medium approximations radiative properties re- sults in a small global annual-mean all-sky absorption of 0.05 W m-2 and a positive

  1. Neutron absorption detector

    DOE Patents [OSTI]

    Bell, Zane William (Oak Ridge, TN); Boatner, Lynn Allen (Oak Ridge, TN)

    2011-05-31T23:59:59.000Z

    A method of detecting an activator, the method including impinging a receptor material that is not predominately water and lacks a photoluminescent material with an activator and generating Cherenkov effect light due to the activator impinging the receptor material. The method further including identifying a characteristic of the activator based on the light.

  2. Optical absorption of silicon nanowires

    SciTech Connect (OSTI)

    Xu, T. [Key Laboratory of Advanced Display and System Application, Shanghai University, 149 Yanchang Road, Shanghai 200072 (China); Institut d'Electronique et de Microelectronique et de Nanotechnologies, IEMN (CNRS, UMR 8520), Groupe de Physique, Cite scientifique, avenue Poincare, 59652 Villeneuve d'Ascq (France); Lambert, Y.; Krzeminski, C.; Grandidier, B.; Stievenard, D.; Leveque, G.; Akjouj, A.; Pennec, Y.; Djafari-Rouhani, B. [Institut d'Electronique et de Microelectronique et de Nanotechnologies, IEMN (CNRS, UMR 8520), Groupe de Physique, Cite scientifique, avenue Poincare, 59652 Villeneuve d'Ascq (France)

    2012-08-01T23:59:59.000Z

    We report on simulations and measurements of the optical absorption of silicon nanowires (NWs) versus their diameter. We first address the simulation of the optical absorption based on two different theoretical methods: the first one, based on the Green function formalism, is useful to calculate the scattering and absorption properties of a single or a finite set of NWs. The second one, based on the finite difference time domain (FDTD) method, is well-adapted to deal with a periodic set of NWs. In both cases, an increase of the onset energy for the absorption is found with increasing diameter. Such effect is experimentally illustrated, when photoconductivity measurements are performed on single tapered Si nanowires connected between a set of several electrodes. An increase of the nanowire diameter reveals a spectral shift of the photocurrent intensity peak towards lower photon energies that allow to tune the absorption onset from the ultraviolet radiations to the visible light spectrum.

  3. atom-atom collisions: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Atomic Safronova, Marianna 3 Atom-atom correlations in colliding Bose-Einstein condensates Quantum Physics (arXiv) Summary: We analyze atom-atom correlations in the s-wave...

  4. Influence of nature of central metal atom in tetrapyrrole pigments on triplet state deactivation processes

    SciTech Connect (OSTI)

    Kapinus, E.I.; Staryi, V.P.; Dilung, I.I.

    1985-07-01T23:59:59.000Z

    A pulse photolysis method has been used to study the absorption spectra and kinetics of deactivation of triplet molecules of tetra-4-tert-butylphthalocyanine, meso-tetraphenylporphine, and their metal derivatives in degassed liquid toluene solutions. The position of the triplet-triplet absorption maximum is only very slightly dependent on the nature of the central atom. The lifetime tau of the triplet molecules of the phthalocyanines, in contrast to the porphyrins, decreases with increasing atomic number of the central atom. The lifetime tau of triplet molecules of the phthalocyanines, in contrast to the porphines, becomes shorter as the atomic number of the central atom increases. The inner heavy atom influence the magnitude of tau for the diphthalocyanines less than for the monophthalocyanines; this is related to the smaller degree of overlapping of the electron shells of the metal atom and the ligand in the case of the diphthalocyanines.

  5. Eta absorption by mesons

    E-Print Network [OSTI]

    W. Liu; C. M. Ko; L. W. Chen

    2005-12-12T23:59:59.000Z

    Using the $[SU(3)_{\\mathrm{L}} \\times SU(3)_{\\mathrm{R}}]_{\\mathrm{global}% }\\times [SU(3)_V]_{\\mathrm{local}}$ chiral Lagrangian with hidden local symmetry, we evaluate the cross sections for the absorption of eta meson ($% \\eta$) by pion ($\\pi$), rho ($\\rho$), omega ($\\omega$), kaon ($K$), and kaon star ($K^*$) in the tree-level approximation. With empirical masses and coupling constants as well as reasonable values for the cutoff parameter in the form factors at interaction vertices, we find that most cross sections are less than 1 mb, except the reactions $\\rho\\eta\\to K\\bar K^*(\\bar KK^*)$, $\\omega\\eta\\to K\\bar K^*(\\bar KK^*)$, $K^*\\eta\\to\\rho K$, and $K^*\\eta\\to\\omega K$, which are a few mb, and the reactions $\\pi\\eta\\to K\\bar K$ and $K\\eta\\to\\pi K$, which are more than 10 mb. Including these reactions in a kinetic model based on a schematic hydrodynamic description of relativistic heavy ion collisions, we find that the abundance of eta mesons likely reaches chemical equilibrium with other hadrons in nuclear collisions at the Relativistic Heavy Ion Collider.

  6. Absorption-free superluminal light propagation in a V-type system

    E-Print Network [OSTI]

    Khaled Saaidi; Bahareh Ruzbahani; S. Worya Rabiei; Mohammad Mahmoudi

    2010-05-19T23:59:59.000Z

    Dispersion and absorption properties of a weak probe field in a three-level V-type atomic system is studied. By application of indirect incoherent pump fields the effect of populating upper levels on optical properties of the atomic medium in presence of a strong coherent pump field is investigated. It is shown that the slope of dispersion changes from positive to negative just by changing the intensity of the coherent or indirect incoherent pump fields. It is demonstrated that the absorption-free subluminal and superluminal light propagation appears in this system.

  7. Heat exchanger bypass system for an absorption refrigeration system

    DOE Patents [OSTI]

    Reimann, Robert C. (Lafayette, NY)

    1984-01-01T23:59:59.000Z

    A heat exchanger bypass system for an absorption refrigeration system is disclosed. The bypass system operates to pass strong solution from the generator around the heat exchanger to the absorber of the absorption refrigeration system when strong solution builds up in the generator above a selected level indicative of solidification of strong solution in the heat exchanger or other such blockage. The bypass system includes a bypass line with a gooseneck located in the generator for controlling flow of strong solution into the bypass line and for preventing refrigerant vapor in the generator from entering the bypass line during normal operation of the refrigeration system. Also, the bypass line includes a trap section filled with liquid for providing a barrier to maintain the normal pressure difference between the generator and the absorber even when the gooseneck of the bypass line is exposed to refrigerant vapor in the generator. Strong solution, which may accumulate in the trap section of the bypass line, is diluted, to prevent solidification, by supplying weak solution to the trap section from a purge system for the absorption refrigeration system.

  8. Quantitative Z-Contrast Imaging of Supported Metal Complexes and Clusters - A Gateway to Understanding Catalysis on the Atomic Scale

    SciTech Connect (OSTI)

    Browning, Nigel D.; Aydin, C.; Lu, Jing; Kulkarni, Apoorva; Okamoto, Norihiko L.; Ortalan, V.; Reed, Bryan W.; Uzun, Alper; Gates, Bruce C.

    2013-09-01T23:59:59.000Z

    Z-contrast imaging in an aberration-corrected scanning transmission electron microscope can be used to observe and quantify the sizes, shapes, and compositions of the metal frames in supported mono-, bi-, and multimetallic metal clusters and can even detect the metal atoms in single-metal-atom complexes, as well as providing direct structural information characterizing the metal-support interface. Herein, we assess the major experimental challenges associated with obtaining atomic resolution Z-contrast images of the materials that are highly beam-sensitive, that is, the clusters readily migrate and sinter on support surfaces, and the support itself can drastically change in structure if the experiment is not properly controlled. Calibrated and quantified Z-contrast images are used in conjunction with exsitu analytical measurements and larger-scale characterization methods such as extended X-ray absorption fine structure spectroscopy to generate an atomic-scale understanding of supported catalysts and their function. Examples of the application of these methods include the characterization of a wide range of sizes and compositions of supported clusters, primarily those incorporating Ir, Os, and Au, on highly crystalline supports (zeolites and MgO).

  9. Ultrafast extended x-ray absorption fine structure ,,EXAFS...--theoretical considerations

    E-Print Network [OSTI]

    Cao, Jianshu

    13­20 to generate ultrafast x-ray pulses, however, the prospect of ultrafast EXAFS seems encouragingUltrafast extended x-ray absorption fine structure ,,EXAFS...--theoretical considerations Frank L by the recent experimental demonstration of ultrafast x-ray absorption spectroscopy, we present a framework

  10. H{alpha} ABSORPTION IN TRANSITING EXOPLANET ATMOSPHERES

    SciTech Connect (OSTI)

    Christie, Duncan; Arras, Phil; Li Zhiyun, E-mail: dac5zm@virginia.edu, E-mail: pla7y@virginia.edu, E-mail: zl4h@virginia.edu [Department of Astronomy, University of Virginia, P.O. Box 400325, Charlottesville, VA 22904-4325 (United States)

    2013-08-01T23:59:59.000Z

    Absorption of stellar H{alpha} by the upper atmosphere of the planet HD 189733b has recently been detected by Jensen et al. Motivated by this observation, we have developed a model for atomic hydrogen in the n = 2 state and compared the resulting H{alpha} line profile to the observations. The model atmosphere is in hydrostatic balance, as well as thermal and photoionization equilibrium. Collisional and radiative transitions are included in the determination of the n = 2 state level population. We find that H{alpha} absorption is dominated by an optical depth {tau} {approx} 1 shell, composed of hydrogen in the metastable 2s state that is located below the hydrogen ionization layer. The number density of the 2s state within the shell is found to vary slowly with radius, while that of the 1s state falls rapidly. Thus while the Ly{alpha} absorption, for a certain wavelength, occurs inside a relatively well defined impact parameter, the contribution to H{alpha} absorption is roughly uniform over the entire atomic hydrogen layer. The model can approximately reproduce the observed Ly{alpha} and H{alpha} integrated transit depths for HD 189733b by using an ionization rate enhanced over that expected for the star by an order of magnitude. For HD 209458b, we are unable to explain the asymmetric H{alpha} line profile observed by Jensen et al., as the model produces a symmetric line profile with transit depth comparable to that of HD 189733b. In an appendix, we study the effect of the stellar Ly{alpha} absorption on the net cooling rate.

  11. absorptivity: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    confondre Absorption Adsorption Mathematics Websites Summary: Ne pas confondre Absorption Adsorption et Quand des molcules sont amenes en contact avec un'attachent...

  12. Development of an Ionic-Liquid Absorption Heat Pump

    SciTech Connect (OSTI)

    Holcomb, Don

    2011-03-29T23:59:59.000Z

    Solar Fueled Products (SFP) is developing an innovative ionic-liquid absorption heat pump (ILAHP). The development of an ILAHP is extremely significant, as it could result in annual savings of more than 190 billion kW h of electrical energy and $19 billion. This absorption cooler uses about 75 percent less electricity than conventional cooling and heating units. The ILAHP also has significant environmental sustainability benefits, due to reduced CO2 emissions. Phase I established the feasibility and showed the economic viability of an ILAHP with these key accomplishments: • Used the breakthrough capabilities provided by ionic liquids which overcome the key difficulties of the common absorption coolers. • Showed that the theoretical thermodynamic performance of an ILAHP is similar to existing absorption-cooling systems. • Established that the half-effect absorption cycle reduces the peak generator temperature, improving collector efficiency and reducing collector area. • Component testing demonstrated that the most critical components, absorber and generator, operate well with conventional heat exchangers. • Showed the economic viability of an ILAHP. The significant energy savings, sustainability benefits, and economic viability are compelling reasons to continue the ILAHP development.

  13. Absorption Mode FT-ICR Mass Spectrometry Imaging

    SciTech Connect (OSTI)

    Smith, Donald F.; Kilgour, David P.; Konijnenburg, Marco; O'Connor, Peter B.; Heeren, Ronald M.

    2013-12-03T23:59:59.000Z

    Fourier transform ion cyclotron resonance mass spectrometry offers the highest mass resolving power for molecular imaging experiments. This high mass resolving power ensures that closely spaced peaks at the same nominal mass are resolved for proper image generation. Typically higher magnetic fields are used to increase mass resolving power. However, a gain in mass resolving power can also be realized by phase correction of the data for absorption mode display. In addition to mass resolving power, absorption mode offers higher mass accuracy and signal-to-noise ratio over the conventional magnitude mode. Here we present the first use of absorption mode for Fourier transform ion cyclotron resonance mass spectrometry imaging. The Autophaser algorithm is used to phase correct each spectrum (pixel) in the image and then these parameters are used by the Chameleon work-flow based data processing software to generate absorption mode ?Datacubes? for image and spectral viewing. Absorption mode reveals new mass and spatial features that are not resolved in magnitude mode and results in improved selected ion image contrast.

  14. Generation of graph-state streams

    E-Print Network [OSTI]

    Daniel Ballester; Jaeyoon Cho; M. S. Kim

    2010-12-08T23:59:59.000Z

    We propose a protocol to generate a stream of mobile qubits in a graph state through a single stationary parent qubit and discuss two types of its physical implementation, namely, the generation of photonic graph states through an atom-like qubit and those of flying atoms through a cavity-mode photonic qubit. The generated graph states fall into an important class that can hugely reduce the resource requirement of fault-tolerant linear optics quantum computation, which was previously known to be far from realistic. In regard to the flying atoms, we also propose a heralded generation scheme, which allows for high-fidelity graph states even under the photon loss.

  15. Active Reflection Absorption for a Three Dimensional Multidirectional Wave Generator

    E-Print Network [OSTI]

    Cruz Castro, Oscar

    2010-10-12T23:59:59.000Z

    frequency response control through tuned filtering of the system response. Here the problems mentioned above, related to control stability and time delay, were handled properly by the manufacturer (Bosch-Rexroth, 2004) by tuning up the 1D filters...

  16. Bistability and pulsations in cw semiconductor lasers with a controlled amount of saturable absorption

    SciTech Connect (OSTI)

    Harder, C.; Lau, K.Y.; Yariv, A.

    1981-09-01T23:59:59.000Z

    Experimental results of a buried heterostructure cw laser with a controllable amount of saturable absorption introduced by a segmented contact are presented. With no absorption the laser is stable and has a linear output characteristic. Increasing of the saturable absorption by changing the pump current through the control segment causes the light output of the device to pulsate and to show bistable and hysteretical behavior. The introduction of a controllable amount of saturable absorption suggest the usefulness of this device in generating extremely short pulses, for example, by passive mode locking and as a bistable optical device.

  17. Atomizing nozzle and process

    DOE Patents [OSTI]

    Anderson, I.E.; Figliola, R.S.; Molnar, H.M.

    1993-07-20T23:59:59.000Z

    High pressure atomizing nozzle includes a high pressure gas manifold having a divergent expansion chamber between a gas inlet and arcuate manifold segment to minimize standing shock wave patterns in the manifold and thereby improve filling of the manifold with high pressure gas for improved melt atomization. The atomizing nozzle is especially useful in atomizing rare earth-transition metal alloys to form fine powder particles wherein a majority of the powder particles exhibit particle sizes having near-optimum magnetic properties.

  18. High-frequency absorption and gain in superlattices: Semiquasistatic approach

    E-Print Network [OSTI]

    A. V. Shorokhov; K. N. Alekseev

    2006-02-08T23:59:59.000Z

    We consider a generation and an amplification of THz radiation in semiconductor superlattices under the action of microwave pump field. Electrons belonging to a single miniband of the superlattice interact quasistatically with the pump field and dynamically with a signal THz field. Within this semiquasistic approach we derive elegant difference formulas describing absorption (gain) of the weak THz signal. We present an instructive geometric interpretation of the absorption formulas which allows a search of optimum conditions for the gain employing only a simple qualitative analysis. Our theoretical findings contribute to the development of sources and detectors of THz radiation that are using nonlinear electric properties of semiconductor superlattices.

  19. Study atom-vacuum interaction by the weak measurement technique

    E-Print Network [OSTI]

    M. Zhang; S. Y. Zhu

    2014-10-27T23:59:59.000Z

    Quantum weak measurement attracts much interests recently [Rev. Mod. Phys. 86, 307 (2014)], as it could amplify some weak signals and provide a technique to observe the nonclassical phenomenons. Here, we apply this technique to study the interaction between the free atoms and the vacuum in a cavity. Due to the gradient field in the vacuum cavity, the external orbital motions and the internal electronic states of the atoms can be weakly coupled via the atom-field electric-dipole interaction. We show an interesting phenomenon that, within the properly post-selected internal states, the weak atom-vacuum interaction could generate a large change to the external motions of atoms.

  20. Driven Ratchets for Cold Atoms

    E-Print Network [OSTI]

    Renzoni, F

    2011-01-01T23:59:59.000Z

    Brownian motors, or ratchets, are devices which "rectify" Brownian motion, i.e. they can generate a current of particles out of unbiased fluctuations. The ratchet effect is a very general phenomenon which applies to a wide range of physical systems, and indeed ratchets have been realized with a variety of solid state devices, with optical trap setups as well as with synthetic molecules and granular gases. The present article reviews recent experimental realizations of ac driven ratchets with cold atoms in driven optical lattices. This is quite an unusual system for a Brownian motor as there is no a real thermal bath, and both the periodic potential for the atoms and the fluctuations are determined by laser fields. Such a system allowed us to realize experimentally rocking and gating ratchets, and to precisely investigate the relationship between symmetry and transport in these ratchets, both for the case of periodic and quasiperiodic driving.

  1. Driven Ratchets for Cold Atoms

    E-Print Network [OSTI]

    F. Renzoni

    2011-12-05T23:59:59.000Z

    Brownian motors, or ratchets, are devices which "rectify" Brownian motion, i.e. they can generate a current of particles out of unbiased fluctuations. The ratchet effect is a very general phenomenon which applies to a wide range of physical systems, and indeed ratchets have been realized with a variety of solid state devices, with optical trap setups as well as with synthetic molecules and granular gases. The present article reviews recent experimental realizations of ac driven ratchets with cold atoms in driven optical lattices. This is quite an unusual system for a Brownian motor as there is no a real thermal bath, and both the periodic potential for the atoms and the fluctuations are determined by laser fields. Such a system allowed us to realize experimentally rocking and gating ratchets, and to precisely investigate the relationship between symmetry and transport in these ratchets, both for the case of periodic and quasiperiodic driving.

  2. Atomic oxygen flux determined by mixed-phase Ag/Ag2O deposition...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    oxygen flux determined by mixed-phase AgAg2O deposition. Atomic oxygen flux determined by mixed-phase AgAg2O deposition. Abstract: The flux of atomic oxygen generated in a...

  3. Transient absorption spectroscopy of laser shocked explosives

    SciTech Connect (OSTI)

    Mcgrane, Shawn D [Los Alamos National Laboratory; Dang, Nhan C [Los Alamos National Laboratory; Whitley, Von H [Los Alamos National Laboratory; Bolome, Cindy A [Los Alamos National Laboratory; Moore, D S [Los Alamos National Laboratory

    2010-01-01T23:59:59.000Z

    Transient absorption spectra from 390-890 nm of laser shocked RDX, PETN, sapphire, and polyvinylnitrate (PVN) at sub-nanosecond time scales are reported. RDX shows a nearly linear increase in absorption with time after shock at {approx}23 GPa. PETN is similar, but with smaller total absorption. A broad visible absorption in sapphire begins nearly immediately upon shock loading but does not build over time. PVN exhibits thin film interference in the absorption spectra along with increased absorption with time. The absorptions in RDX and PETN are suggested to originate in chemical reactions happening on picosecond time scales at these shock stresses, although further diagnostics are required to prove this interpretation.

  4. Atomic swelling upon compression

    E-Print Network [OSTI]

    V. K. Dolmatov; J. L. King

    2012-08-18T23:59:59.000Z

    The hydrogen atom under the pressure of a spherical penetrable confinement potential of a decreasing radius $r_{0}$ is explored, as a case study. A novel counter-intuitive effect of atomic swelling rather than shrinking with decreasing $r_{0}$ is unraveled, when $r_{0}$ reaches, and remains smaller than, a certain critical value. Upon swelling, the size of the atom is shown to increase by an order of magnitude, or more, compared to the size of the free atom. Examples of changes of photoabsorption properties of confined hydrogen atom upon its swelling are uncovered and demonstrated.

  5. Backscatter absorption gas imaging systems and light sources therefore

    DOE Patents [OSTI]

    Kulp, Thomas Jan (Livermore, CA); Kliner, Dahv A. V. (San Ramon, CA); Sommers, Ricky (Oakley, CA); Goers, Uta-Barbara (Campbell, NY); Armstrong, Karla M. (Livermore, CA)

    2006-12-19T23:59:59.000Z

    The location of gases that are not visible to the unaided human eye can be determined using tuned light sources that spectroscopically probe the gases and cameras that can provide images corresponding to the absorption of the gases. The present invention is a light source for a backscatter absorption gas imaging (BAGI) system, and a light source incorporating the light source, that can be used to remotely detect and produce images of "invisible" gases. The inventive light source has a light producing element, an optical amplifier, and an optical parametric oscillator to generate wavelength tunable light in the IR. By using a multi-mode light source and an amplifier that operates using 915 nm pump sources, the power consumption of the light source is reduced to a level that can be operated by batteries for long periods of time. In addition, the light source is tunable over the absorption bands of many hydrocarbons, making it useful for detecting hazardous gases.

  6. Absorption-heat-pump system

    DOE Patents [OSTI]

    Grossman, G.; Perez-Blanco, H.

    1983-06-16T23:59:59.000Z

    An improvement in an absorption heat pump cycle is obtained by adding adiabatic absorption and desorption steps to the absorber and desorber of the system. The adiabatic processes make it possible to obtain the highest temperature in the absorber before any heat is removed from it and the lowest temperature in the desorber before heat is added to it, allowing for efficient utilization of the thermodynamic availability of the heat supply stream. The improved system can operate with a larger difference between high and low working fluid concentrations, less circulation losses, and more efficient heat exchange than a conventional system.

  7. Quasistellar Objects: Intervening Absorption Lines

    E-Print Network [OSTI]

    Jane C. Charlton; Christopher W. Churchill

    2000-05-31T23:59:59.000Z

    We briefly review, at a level appropriate for graduate students and non-specialists, the field of quasar absorption lines (QALs). Emphasis is on the intervening absorbers. We present the anatomy of a quasar spectrum due to various classes of intervening absorption systems, and a brief historical review of each absorber class (Lyman-alpha forest and Lyman limit systems, and metal-line and damped Lyman-alpha absorbers). We also provide several heuristic examples on how the physical properties of both the intergalactic medium and the gaseous environments associated with earlier epoch galaxies can be inferred from QALs. The evolution of these environments from z=4 are discussed.

  8. Saturable absorption and 'slow light'

    E-Print Network [OSTI]

    Adrian C Selden

    2006-03-25T23:59:59.000Z

    Quantitative evaluation of some recent 'slow light' experiments based on coherent population oscillations (CPO) shows that they can be more simply interpreted as saturable absorption phenomena. Therefore they do not provide an unambiguous demonstration of 'slow light'. Indeed a limiting condition on the spectral bandwidth is not generally satisfied, such that the requirements for burning a narrow spectral hole in the homogeneously broadened absorption line are not met. Some definitive tests of 'slow light' phenomena are suggested, derived from analysis of phase shift and pulse delay for a saturable absorber

  9. Absorption spectroscopy of a laboratory photoionized plasma experiment at Z

    SciTech Connect (OSTI)

    Hall, I. M.; Durmaz, T.; Mancini, R. C. [Physics Department, University of Nevada, Reno, Nevada 89557 (United States)] [Physics Department, University of Nevada, Reno, Nevada 89557 (United States); Bailey, J. E.; Rochau, G. A. [Sandia National Laboratories, Albuquerque, New Mexico 87185 (United States)] [Sandia National Laboratories, Albuquerque, New Mexico 87185 (United States); Golovkin, I. E.; MacFarlane, J. J. [Prism Computational Sciences, Madison, Wisconsin 53711 (United States)] [Prism Computational Sciences, Madison, Wisconsin 53711 (United States)

    2014-03-15T23:59:59.000Z

    The Z facility at the Sandia National Laboratories is the most energetic terrestrial source of X-rays and provides an opportunity to produce photoionized plasmas in a relatively well characterised radiation environment. We use detailed atomic-kinetic and spectral simulations to analyze the absorption spectra of a photoionized neon plasma driven by the x-ray flux from a z-pinch. The broadband x-ray flux both photoionizes and backlights the plasma. In particular, we focus on extracting the charge state distribution of the plasma and the characteristics of the radiation field driving the plasma in order to estimate the ionisation parameter.

  10. Dynamic Absorption Model for Off-Gas Separation

    SciTech Connect (OSTI)

    Veronica J. Rutledge

    2011-07-01T23:59:59.000Z

    Modeling and simulations will aid in the future design of U.S. advanced reprocessing plants for the recovery and recycle of actinides in used nuclear fuel. The specific fuel cycle separation process discussed in this report is the off-gas treatment system. The off-gas separation consists of a series of scrubbers and adsorption beds to capture constituents of interest. Dynamic models are being developed to simulate each unit operation involved so each unit operation can be used as a stand-alone model and in series with multiple others. Currently, a rate based, dynamic absorption model is being developed in gPROMS software. Inputs include liquid and gas stream constituents, column properties, liquid and gas phase reactions, number of stages, and inlet conditions. It simulates multiple component absorption with countercurrent flow and accounts for absorption by mass transfer and chemical reaction. The assumption of each stage being a discrete well-mixed entity was made. Therefore, the model is solved stagewise. The simulation outputs component concentrations in both phases as a function of time from which the rate of absorption is determined. Temperature of both phases is output as a function of time also. The model will be used able to be used as a standalone model in addition to in series with other off-gas separation unit operations. The current model is being generated based on NOx absorption; however, a future goal is to develop a CO2 specific model. The model will have the capability to be modified for additional absorption systems. The off-gas models, both adsorption and absorption, will be made available via the server or web for evaluation by customers.

  11. Four-level atom interferometer with trichromatic laser fields

    SciTech Connect (OSTI)

    Honda, Kazuhito; Kobayashi, Yoshiyuki; Morinaga, Atsuo [Faculty of Science and Technology, Tokyo University of Science, 2641 Yamazaki, Noda-shi, Chiba 278-8510 (Japan)

    2007-02-15T23:59:59.000Z

    A four-level atom interferometer comprised of three excited states and one ground state with trichromatic fields coupled between them is investigated using Zeeman sublevels of {sup 3}P{sub 1} and {sup 1}S{sub 0} states of a calcium atom. A theoretical description of the interaction of four-level atoms with trichromatic laser fields is presented and compared with the experimental results of the interference fringes which are generated by the three excited states.

  12. Ne pas confondre Absorption Adsorption

    E-Print Network [OSTI]

    Liège, Université de

    Ne pas confondre Absorption Adsorption et Quand des molécules sont amenées en contact avec un'attachent simplement à la surface du solide on parle d'adsorption. L'adsorption est donc le « collage » de molécules à la surface d'un solide. Quand le charbon nettoie Principes physiques de l'adsorption Cédric Gommes

  13. Ultrasonic absorption in liquid mixtures

    E-Print Network [OSTI]

    Davis, James Madison

    1954-01-01T23:59:59.000Z

    snd water and of methanol and water, Since Storey's work on ethanol and water at 0 C showed that for the three different frequencies at, which his investigation wms carried outx the ratio of ths absorption to the frequency squared increased...

  14. Interferometric tunability of the absorption

    E-Print Network [OSTI]

    Vittorio Giovannetti; Seth Lloyd; Lorenzo Maccone

    2006-03-27T23:59:59.000Z

    We propose an interferometric setup that permits to tune the quantity of radiation absorbed by an object illuminated by a fixed light source. The method can be used to selectively irradiate portions of an object based on their transmissivities or to accurately estimate the transmissivities from rough absorption measurements.

  15. Full Quantum Analysis of Two-Photon Absorption Using Two-Photon Wavefunction: Comparison with One-Photon Absorption

    E-Print Network [OSTI]

    Toshihiro Nakanishi; Hirokazu Kobayashi; Kazuhiko Sugiyama; Masao Kitano

    2009-06-01T23:59:59.000Z

    For dissipation-free photon-photon interaction at the single photon level, we analyze one-photon transition and two-photon transition induced by photon pairs in three-level atoms using two-photon wavefunctions. We show that the two-photon absorption can be substantially enhanced by adjusting the time correlation of photon pairs. We study two typical cases: Gaussian wavefunction and rectangular wavefunction. In the latter, we find that under special conditions one-photon transition is completely suppressed while the high probability of two-photon transition is maintained.

  16. Vacuum - induced stationary entanglement in radiatively coupled three - level atoms

    E-Print Network [OSTI]

    L. Derkacz; L. Jakobczyk

    2008-05-05T23:59:59.000Z

    We consider a pair of three - level atoms interacting with a common vacuum and analyze the process of entanglement production due to spontaneous emission. We show that in the case of closely separated atoms, collective damping can generate robust entanglement of the asymptotic states.

  17. Gauge invariant hydrogen atom Hamiltonian

    E-Print Network [OSTI]

    Wei-Min Sun; Xiang-Song Chen; Xiao-Fu Lu; Fan Wang

    2010-06-22T23:59:59.000Z

    For quantum mechanics of a charged particle in a classical external electromagnetic field, there is an apparent puzzle that the matrix element of the canonical momentum and Hamiltonian operators is gauge dependent. A resolution to this puzzle is recently provided by us in [2]. Based on the separation of the electromagnetic potential into pure gauge and gauge invariant parts, we have proposed a new set of momentum and Hamiltonian operators which satisfy both the requirement of gauge invariance and the relevant commutation relations. In this paper we report a check for the case of the hydrogen atom problem: Starting from the Hamiltonian of the coupled electron, proton and electromagnetic field, under the infinite proton mass approximation, we derive the gauge invariant hydrogen atom Hamiltonian and verify explicitly that this Hamiltonian is different from the Dirac Hamiltonian, which is the time translation generator of the system. The gauge invariant Hamiltonian is the energy operator, whose eigenvalue is the energy of the hydrogen atom. It is generally time-dependent. In this case, one can solve the energy eigenvalue equation at any specific instant of time. It is shown that the energy eigenvalues are gauge independent, and by suitably choosing the phase factor of the time-dependent eigenfunction, one can ensure that the time-dependent eigenfunction satisfies the Dirac equation.

  18. Atomic Collapse Observed

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Scientists Observe Atomic Collapse State Quantum Mechanics Prediction Confirmed in Graphene Using NERSC's Hopper April 26, 2013 | Tags: Hopper, Materials Science Contact: Linda...

  19. Modification of the Absorption Cross Section in the Optical Near-field

    E-Print Network [OSTI]

    Moritz Striebel; Jeff F. Young; Jörg Wrachtrup; Ilja Gerhardt

    2014-11-20T23:59:59.000Z

    The optical interaction of light and matter is modeled as an oscillating dipole in a plane wave. We analyze absorption, scattering and extinction for this system by the energy flow, which is depicted by streamlines of the Poynting vector. Depending on the dissipative damping of the oscillator, the streamlines end up in the dipole. Based on a graphical investigation of the streamlines, this represents the absorption cross section, and forms a far-field absorption aperture. In the near-field of the oscillator, a modification of the aperture is observed. This scheme can be adapted to a single dipolar emitter, interacting with a light field. In the case of the absorption by a single atom, where the oscillator has a circular dipole characteristics, we model the energy flow and derive the apertures.

  20. Absorption of Cu/sup + +/ by long-term cultures of Dunaliella salina, D. tertiolecta, and D. viridis

    SciTech Connect (OSTI)

    Lustigman, B.; Korky, J.; Zabady, A.; McCormick, J.M.

    1985-09-01T23:59:59.000Z

    By means of atomic absorption analysis, the authors measured the effect of salinity on the absorption of copper. They used long term cultures of Dunaliella in order to determine if alterations in plasmalemma permeability occur as a result of adaptation to different osmotic conditions. Since copper appears to affect the mechanisms involved in osmotic resistance with Dunaliella, they hoped to elucidate some of the characteristics of permeability.

  1. Energy Saving with Absorption Refrigeration Technologies

    E-Print Network [OSTI]

    Davis, R. C.

    1984-01-01T23:59:59.000Z

    Absorption refrigeration technology can be an economical and cost effective means of reducing energy cost and/or improving the efficiency and output of your process. We believe the potential benefits of absorption refrigeration technology have...

  2. Method and apparatus for atomic imaging

    DOE Patents [OSTI]

    Saldin, Dilano K. (Milwaukee, WI); de Andres Rodriquez, Pedro L. (Madrid, ES)

    1993-01-01T23:59:59.000Z

    A method and apparatus for three dimensional imaging of the atomic environment of disordered adsorbate atoms are disclosed. The method includes detecting and measuring the intensity of a diffuse low energy electron diffraction pattern formed by directing a beam of low energy electrons against the surface of a crystal. Data corresponding to reconstructed amplitudes of a wave form is generated by operating on the intensity data. The data corresponding to the reconstructed amplitudes is capable of being displayed as a three dimensional image of an adsorbate atom. The apparatus includes a source of a beam of low energy electrons and a detector for detecting the intensity distribution of a DLEED pattern formed at the detector when the beam of low energy electrons is directed onto the surface of a crystal. A device responsive to the intensity distribution generates a signal corresponding to the distribution which represents a reconstructed amplitude of a wave form and is capable of being converted into a three dimensional image of the atomic environment of an adsorbate atom on the crystal surface.

  3. DOUBLE SHELL TANK (DST) HYDROXIDE DEPLETION MODEL FOR CARBON DIOXIDE ABSORPTION

    SciTech Connect (OSTI)

    OGDEN DM; KIRCH NW

    2007-10-31T23:59:59.000Z

    This document generates a supernatant hydroxide ion depletion model based on mechanistic principles. The carbon dioxide absorption mechanistic model is developed in this report. The report also benchmarks the model against historical tank supernatant hydroxide data and vapor space carbon dioxide data. A comparison of the newly generated mechanistic model with previously applied empirical hydroxide depletion equations is also performed.

  4. Effects of thermal motion on electromagnetically induced absorption

    SciTech Connect (OSTI)

    Tilchin, E.; Wilson-Gordon, A. D.; Firstenberg, O. [Department of Chemistry, Bar-Ilan University, Ramat Gan IL-52900 (Israel); Department of Physics, Technion-Israel Institute of Technology, Haifa IL-32000 (Israel)

    2011-05-15T23:59:59.000Z

    We describe the effect of thermal motion and buffer-gas collisions on a four-level closed N system interacting with strong pump(s) and a weak probe. This is the simplest system that experiences electromagnetically induced absorption (EIA) due to transfer of coherence via spontaneous emission from the excited state to the ground state. We investigate the influence of Doppler broadening, velocity-changing collisions (VCC), and phase-changing collisions (PCC) with a buffer gas on the EIA spectrum of optically active atoms. In addition to exact expressions, we present an approximate solution for the probe absorption spectrum, which provides physical insight into the behavior of the EIA peak due to VCC, PCC, and the wave-vector difference between the pump and probe beams. VCC are shown to produce a wide pedestal at the base of the EIA peak, which is scarcely affected by the pump-probe angular deviation, whereas the sharp central EIA peak becomes weaker and broader due to the residual Doppler-Dicke effect. Using diffusionlike equations for the atomic coherences and populations, we construct a spatial-frequency filter for a spatially structured probe beam and show that Ramsey narrowing of the EIA peak is obtained for beams of finite width.

  5. Effects of thermal motion on electromagnetically induced absorption

    E-Print Network [OSTI]

    E. Tilchin; O. Firstenberg; A. D. Wilson-Gordon

    2011-07-04T23:59:59.000Z

    We describe the effect of thermal motion and buffer-gas collisions on a four-level closed N system interacting with strong pump(s) and a weak probe. This is the simplest system that experiences electromagnetically induced absorption (EIA) due to transfer of coherence via spontaneous emission from the excited to ground state. We investigate the influence of Doppler broadening, velocity-changing collisions (VCC), and phase-changing collisions (PCC) with a buffer gas on the EIA spectrum of optically active atoms. In addition to exact expressions, we present an approximate solution for the probe absorption spectrum, which provides physical insight into the behavior of the EIA peak due to VCC, PCC, and wave-vector difference between the pump and probe beams. VCC are shown to produce a wide pedestal at the base of the EIA peak, which is scarcely affected by the pump-probe angular deviation, whereas the sharp central EIA peak becomes weaker and broader due to the residual Doppler-Dicke effect. Using diffusion-like equations for the atomic coherences and populations, we construct a spatial-frequency filter for a spatially structured probe beam and show that Ramsey narrowing of the EIA peak is obtained for beams of finite width.

  6. Producing and Detecting Correlated atoms

    E-Print Network [OSTI]

    Christoph I. Westbrook; Martijn Schellekens; Aurélien Perrin; Valentina Krachmalnicoff; Jose Carlos Viana Gomes; Jean-Baptiste Trebbia; Jérôme Estève; Hong Chang; Isabelle Bouchoule; Denis Boiron; Alain Aspect; Tom Jeltes; John McNamara; Wim Hogervorst; Wim Vassen

    2006-09-04T23:59:59.000Z

    We discuss experiments to produce and detect atom correlations in a degenerate or nearly degenerate gas of neutral atoms. First we treat the atomic analog of the celebrated Hanbury Brown Twiss experiment, in which atom correlations result simply from interference effects without any atom interactions.We have performed this experiment for both bosons and fermions. Next we show how atom interactions produce correlated atoms using the atomic analog of spontaneous four-wavemixing. Finally, we briefly mention experiments on a one dimensional gas on an atom chip in which correlation effects due to both interference and interactions have been observed.

  7. Thermochemical Analysis of Hydrogen Absorption in Welding

    E-Print Network [OSTI]

    Eagar, Thomas W.

    '' .' j I ~l Thermochemical Analysis of Hydrogen Absorption in Welding A new model that addresses the shortcomings of Sievert's law for predicting hydrogen absorption is proposed ABSTRACT. A systematic review of diatomic hydrogen) to calcu· late the hydrogen absorption reaction temperature in the weld pool is invalid

  8. Absorption cross section in Lifshitz black hole

    E-Print Network [OSTI]

    Taeyoon Moon; Yun Soo Myung

    2012-10-05T23:59:59.000Z

    We derive the absorption cross section of a minimally coupled scalar in the Lifshitz black hole obtained from the new massive gravity. The absorption cross section reduces to the horizon area in the low energy and massless limit of s-wave mode propagation, indicating that the Lifshitz black hole also satisfies the universality of low energy absorption cross section for black holes.

  9. Inversion symmetry breaking of atomic bound states in strong and short laser fields

    E-Print Network [OSTI]

    Stooß, Veit; Ott, Christian; Blättermann, Alexander; Ding, Thomas; Pfeifer, Thomas

    2015-01-01T23:59:59.000Z

    In any atomic species, the spherically symmetric potential originating from the charged nucleus results in fundamental symmetry properties governing the structure of atomic states and transition rules between them. If atoms are exposed to external electric fields, these properties are modified giving rise to energy shifts such as the AC Stark-effect in varying fields and, contrary to this in a constant (DC) electric field for high enough field strengths, the breaking of the atomic symmetry which causes fundamental changes in the atom's properties. This has already been observed for atomic Rydberg states with high principal quantum numbers. Here, we report on the observation of symmetry breaking effects in Helium atoms for states with principal quantum number n=2 utilizing strong visible laser fields. These findings were enabled by temporally resolving the dynamics better than the sub-optical cycle of the applied laser field, utilizing the method of attosecond transient absorption spectroscopy (ATAS). We ident...

  10. Triple loop heat exchanger for an absorption refrigeration system

    DOE Patents [OSTI]

    Reimann, Robert C. (Lafayette, NY)

    1984-01-01T23:59:59.000Z

    A triple loop heat exchanger for an absorption refrigeration system is disclosed. The triple loop heat exchanger comprises portions of a strong solution line for conducting relatively hot, strong solution from a generator to a solution heat exchanger of the absorption refrigeration system, conduit means for conducting relatively cool, weak solution from the solution heat exchanger to the generator, and a bypass system for conducting strong solution from the generator around the strong solution line and around the solution heat exchanger to an absorber of the refrigeration system when strong solution builds up in the generator to an undesirable level. The strong solution line and the conduit means are in heat exchange relationship with each other in the triple loop heat exchanger so that, during normal operation of the refrigeration system, heat is exchanged between the relatively hot, strong solution flowing through the strong solution line and the relatively cool, weak solution flowing through the conduit means. Also, the strong solution line and the bypass system are in heat exchange relationship in the triple loop heat exchanger so that if the normal flow path of relatively hot, strong solution flowing from the generator to an absorber is blocked, then this relatively, hot strong solution which will then be flowing through the bypass system in the triple loop heat exchanger, is brought into heat exchange relationship with any strong solution which may have solidified in the strong solution line in the triple loop heat exchanger to thereby aid in desolidifying any such solidified strong solution.

  11. Performance of hybrid quad generation system consisting of solid oxide fuel cell system and

    E-Print Network [OSTI]

    Liso, Vincenzo

    Performance of hybrid quad generation system consisting of solid oxide fuel cell system. Keywords: Energy system modeling, Solid oxide fuel cell, Absorption heat pump. 1. Introduction 1

  12. Spectroscopy of barium atoms in liquid and solid helium matrices

    SciTech Connect (OSTI)

    Lebedev, V.; Moroshkin, P.; Weis, A. [Departement de Physique, Universite de Fribourg, Chemin du Musee 3, CH-1700 Fribourg (Switzerland)

    2011-08-15T23:59:59.000Z

    We present an exhaustive overview of optical absorption and laser-induced fluorescence lines of Ba atoms in liquid and solid helium matrices in visible and near-infrared spectral ranges. Due to the increased density of isolated atoms, we have found a large number of spectral lines that were not observed in condensed helium matrices before. We have also measured the lifetimes of metastable states. The lowest {sup 3}D{sub 1} metastable state has lifetime of 2.6 s and can be used as an intermediate state in two-step excitations of high-lying states. Various matrix-induced radiationless population transfer channels have been identified.

  13. Optically Detected Extended X-Ray Absorption Fine Structure Study of InGaN/GaN Single Quantum Wells

    SciTech Connect (OSTI)

    Rigopoulos, N.; Hamilton, B.; Davies, G. J.; Towlson, B. M. [School of Electrical and Electronic Engineering, University of Manchester, Manchester M60 1QD (United Kingdom); Poolton, N. R. J. [Synchrotron Radiation Department, Daresbury Laboratory, Daresbury, Warrington WA4 4AD (United Kingdom); Dawson, P.; Graham, D. M. [School of Physics and Astronomy, University of Manchester, Manchester M60 1QD (United Kingdom); Kappers, M. J.; Humphreys, C. J. [Dept. of Materials Science and Metallurgy, University of Cambridge, Pembroke Street, Cambridge CB2 3QZ (United Kingdom); Carlson, S. [MAX-lab, Lund University, P.O. Box 118, SE- 221 00 Lund (Sweden)

    2007-04-10T23:59:59.000Z

    We have investigated the local atomic environment of the Ga atoms in an InxGa1-xN single quantum well structure using Optically Detected Extended X-ray Absorption Fine Structure (OD-EXAFS). A comparison of the OD-EXAFS data with a theoretical model shows the technique to be site selective for this particular structure and reveals that the quantum well emission originates from regions with x=0.15.

  14. X-ray absorption spectroscopy elucidates the impact of structural disorder on electron mobility in amorphous zinc-tin-oxide thin films

    SciTech Connect (OSTI)

    Siah, Sin Cheng, E-mail: siahsincheng@gmail.com, E-mail: buonassisi@mit.edu; Lee, Yun Seog; Buonassisi, Tonio, E-mail: siahsincheng@gmail.com, E-mail: buonassisi@mit.edu [Massachusetts Institute of Technology, Cambridge, Massachusetts 02139 (United States); Lee, Sang Woon; Gordon, Roy G. [Department of Chemistry and Chemical Biology, Harvard University, Cambridge, Massachusetts 02138 (United States); Heo, Jaeyeong [Department of Materials Science and Engineering, Chonnam National University, Gwangju 500-757 (Korea, Republic of); Shibata, Tomohiro; Segre, Carlo U. [Physics Department and CSRRI, Illinois Institute of Technology, Chicago, Illinois 606016 (United States)

    2014-06-16T23:59:59.000Z

    We investigate the correlation between the atomic structures of amorphous zinc-tin-oxide (a-ZTO) thin films grown by atomic layer deposition (ALD) and their electronic transport properties. We perform synchrotron-based X-ray absorption spectroscopy at the K-edges of Zn and Sn with varying [Zn]/[Sn] compositions in a-ZTO thin films. In extended X-ray absorption fine structure (EXAFS) measurements, signal attenuation from higher-order shells confirms the amorphous structure of a-ZTO thin films. Both quantitative EXAFS modeling and X-ray absorption near edge spectroscopy (XANES) reveal that structural disorder around Zn atoms increases with increasing [Sn]. Field- and Hall-effect mobilities are observed to decrease with increasing structural disorder around Zn atoms, suggesting that the degradation in electron mobility may be correlated with structural changes.

  15. Nitric Oxide Production from Surface Recombination of Oxygen and Nitrogen Atoms

    E-Print Network [OSTI]

    Martín, Pino

    of hypersonic reentry vehicles. In the Earth's atmosphere, oxygen and nitrogen atoms are generated in the shock1 Nitric Oxide Production from Surface Recombination of Oxygen and Nitrogen Atoms Dusan A. Pejakovi from the recombination of oxygen and nitrogen atoms on quartz. The experiments employ two-photon laser

  16. Generator-absorber-heat exchange heat transfer apparatus and method and use thereof in a heat pump

    DOE Patents [OSTI]

    Phillips, Benjamin A. (Benton Harbor, MI); Zawacki, Thomas S. (St. Joseph, MI); Marsala, Joseph (Glen Ellyn, IL)

    1994-11-29T23:59:59.000Z

    Numerous embodiments and related methods for generator-absorber heat exchange (GAX) are disclosed, particularly for absorption heat pump systems. Such embodiments and related methods use the working solution of the absorption system for the heat transfer medium.

  17. Atomic and molecular supernovae

    SciTech Connect (OSTI)

    Liu, W.

    1997-12-01T23:59:59.000Z

    Atomic and molecular physics of supernovae is discussed with an emphasis on the importance of detailed treatments of the critical atomic and molecular processes with the best available atomic and molecular data. The observations of molecules in SN 1987A are interpreted through a combination of spectral and chemical modelings, leading to strong constraints on the mixing and nucleosynthesis of the supernova. The non-equilibrium chemistry is used to argue that carbon dust can form in the oxygen-rich clumps where the efficient molecular cooling makes the nucleation of dust grains possible. For Type Ia supernovae, the analyses of their nebular spectra lead to strong constraints on the supernova explosion models.

  18. Generation of energy

    DOE Patents [OSTI]

    Kalina, Alexander I. (12214 Clear Fork, Houston, TX 77077)

    1984-01-01T23:59:59.000Z

    A method of generating energy which comprises utilizing relatively lower temperature available heat to effect partial distillation of at least portion of a multicomponent working fluid stream at an intermediate pressure to generate working fluid fractions of differing compositions. The fractions are used to produce at least one main rich solution which is relatively enriched with respect to the lower boiling component, and to produce at least one lean solution which is relatively improverished with respect to the lower boiling component. The pressure of the main rich solution is increased whereafter it is evaporated to produce a charged gaseous main working fluid. The main working fluid is expanded to a low pressure level to release energy. The spent low pressure level working fluid is condensed in a main absorption stage by dissolving with cooling in the lean solution to regenerate an initial working fluid for reuse.

  19. Temperature activated absorption during laser-induced damage: The evolution of laser-supported solid-state absorption fronts

    SciTech Connect (OSTI)

    Carr, C W; Bude, J D; Shen, N; Demange, P

    2010-10-26T23:59:59.000Z

    Previously we have shown that the size of laser induced damage sites in both KDP and SiO{sub 2} is largely governed by the duration of the laser pulse which creates them. Here we present a model based on experiment and simulation that accounts for this behavior. Specifically, we show that solid-state laser-supported absorption fronts are generated during a damage event and that these fronts propagate at constant velocities for laser intensities up to 4 GW/cm{sup 2}. It is the constant absorption front velocity that leads to the dependence of laser damage site size on pulse duration. We show that these absorption fronts are driven principally by the temperature-activated deep sub band-gap optical absorptivity, free electron transport, and thermal diffusion in defect-free silica for temperatures up to 15,000K and pressures < 15GPa. In addition to the practical application of selecting an optimal laser for pre-initiation of large aperture optics, this work serves as a platform for understanding general laser-matter interactions in dielectrics under a variety of conditions.

  20. Metal atomization spray nozzle

    DOE Patents [OSTI]

    Huxford, T.J.

    1993-11-16T23:59:59.000Z

    A spray nozzle for a magnetohydrodynamic atomization apparatus has a feed passage for molten metal and a pair of spray electrodes mounted in the feed passage. The electrodes, diverging surfaces which define a nozzle throat and diverge at an acute angle from the throat. Current passes through molten metal when fed through the throat which creates the Lorentz force necessary to provide atomization of the molten metal. 6 figures.

  1. Atomizing nozzle and method

    DOE Patents [OSTI]

    Ting, Jason (Ames, IA); Anderson, Iver E. (Ames, IA); Terpstra, Robert L. (Ames, IA)

    2000-03-16T23:59:59.000Z

    A high pressure close-coupled gas atomizing nozzle includes multiple discrete gas jet discharge orifices having aerodynamically designed convergent-divergent geometry with an first converging section communicated to a gas supply manifold and to a diverging section by a constricted throat section to increase atomizing gas velocity. The gas jet orifices are oriented at gas jet apex angle selected relative to the melt supply tip apex angle to establish a melt aspiration condition at the melt supply tip.

  2. Optical atomic magnetometer

    DOE Patents [OSTI]

    Budker, Dmitry; Higbie, James; Corsini, Eric P

    2013-11-19T23:59:59.000Z

    An optical atomic magnetometers is provided operating on the principles of nonlinear magneto-optical rotation. An atomic vapor is optically pumped using linearly polarized modulated light. The vapor is then probed using a non-modulated linearly polarized light beam. The resulting modulation in polarization angle of the probe light is detected and used in a feedback loop to induce self-oscillation at the resonant frequency.

  3. DEVELOPMENT OF SOLAR DRIVEN ABSORPTION AIR CONDITIONERS AND HEAT PUMPS

    E-Print Network [OSTI]

    Dao, K.

    2013-01-01T23:59:59.000Z

    DRIVEN ABSORPTION AIR CONDITIONERS AND HEAT PUMPS K. Dao, M.ABSORPTION AIR CONDITIONERS AND HEAT PUMPS* K. DAO, M.

  4. Atomic mass compilation 2012

    SciTech Connect (OSTI)

    Pfeiffer, B., E-mail: bpfeiffe@uni-mainz.de [II. Physikalisches Institut, Justus-Liebig-Universität Gießen, Gießen (Germany); GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt (Germany); Venkataramaniah, K. [Sri Sathya Sai Institute of Higher Learning, Prasanthinilayam (India)] [Sri Sathya Sai Institute of Higher Learning, Prasanthinilayam (India); Czok, U. [II. Physikalisches Institut, Justus-Liebig-Universität Gießen, Gießen (Germany)] [II. Physikalisches Institut, Justus-Liebig-Universität Gießen, Gießen (Germany); Scheidenberger, C. [GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt (Germany) [GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt (Germany); II. Physikalisches Institut, Justus-Liebig-Universität Gießen, Gießen (Germany)

    2014-03-15T23:59:59.000Z

    Atomic mass reflects the total binding energy of all nucleons in an atomic nucleus. Compilations and evaluations of atomic masses and derived quantities, such as neutron or proton separation energies, are indispensable tools for research and applications. In the last decade, the field has evolved rapidly after the advent of new production and measuring techniques for stable and unstable nuclei resulting in substantial ameliorations concerning the body of data and their precision. Here, we present a compilation of atomic masses comprising the data from the evaluation of 2003 as well as the results of new measurements performed. The relevant literature in refereed journals and reports as far as available, was scanned for the period beginning 2003 up to and including April 2012. Overall, 5750 new data points have been collected. Recommended values for the relative atomic masses have been derived and a comparison with the 2003 Atomic Mass Evaluation has been performed. This work has been carried out in collaboration with and as a contribution to the European Nuclear Structure and Decay Data Network of Evaluations.

  5. Resonances and excitation pathways in four-level N-scheme atomic systems

    SciTech Connect (OSTI)

    Abi-Salloum, T. Y.; Henry, B. [Physics and Astronomy Department, Widener University, Chester, Pennsylvania 19013 (United States); Davis, J. P.; Narducci, F. A. [Naval Air Systems Command, EO Sensors Division, Bldg 2187, Suite 3190 Patuxent River, Maryland 20670 (United States)

    2010-07-15T23:59:59.000Z

    In this work, we theoretically study the absorption and dispersion coefficients of a probe field in four-level N-scheme atomic systems driven by two additional fields. We separate the steady-state solution of the appropriate density matrix element into the sum of three resonances. The effect of each resonance on the overall absorption and dispersion experienced by the probe is studied as a function of the strengths of the two other fields. In the limit of low saturation, we reveal the physics of these resonances and associate them with atomic excitation pathways, which we explicitly explain in the bare-states picture.

  6. Role of transient processes in resonance line spectroscopy of caesium atoms in cells with antirelaxation coating

    SciTech Connect (OSTI)

    Sevost'yanov, D I; Yakovlev, V P; Kozlov, A N; Vasil'ev, V V; Zibrov, S A; Velichansky, Vladimir L

    2013-07-31T23:59:59.000Z

    We study the peculiarities of the absorption spectra in D{sub 1,2}-lines of Cs, caused by optical pumping in cells with antirelaxation coating. In these cells the internal state of the atom, which arose under optical pumping by a monochromatic laser field, is preserved with a high probability in a collision with the wall. As a result, the optical pumping action extends to the entire volume of the cell and to all the velocities of the atoms. This leads to the speed-dependent scanning distortions of the absorption line profile. The detected features should be considered when using laserpumped quantum magnetometers with antirelaxation-coated cells. (laser spectroscopy)

  7. Request for Support for the Conference on Super Intense Laser Atom Physics

    SciTech Connect (OSTI)

    Todd Ditmire

    2004-10-21T23:59:59.000Z

    The Conference on Super Intense Laser Atom Physics (SILAP) was held in November 2003 in Dallas, Texas. The venue for the meeting was South Fork Ranch in the outskirts of Dallas. The topics of the meeting included high harmonic generation and attosecond pulse generation, strong field interactions with molecules and clusters, particle acceleration, and relativistic laser atom interactions.

  8. Saturated absorption at nanowatt power levels using metastable xenon in a high-finesse optical cavity

    E-Print Network [OSTI]

    G. T. Hickman; T. B. Pittman; J. D. Franson

    2014-09-19T23:59:59.000Z

    Strong saturated absorption at nanowatt power levels has been demonstrated using metastable xenon in a high-finesse optical cavity. The use of metastable xenon allows a high quality factor of Q=2*10^8 to be achieved at relatively high atomic densities without any contamination or damage to the optical surfaces, which is often a problem when using high-density rubidium or other alkali atoms. This technique provides a relatively straightforward way to produce nonlinearities at the single-photon level with possible applications in quantum communications and computing.

  9. X-ray absorption in GaGdN: A study of local structure

    SciTech Connect (OSTI)

    Martinez-Criado, G.; Sans, J. A.; Susini, J. [Experiments Division, European Synchrotron Radiation Facility, 38043-Grenoble (France); Sancho-Juan, O.; Cantarero, A. [Institut de Ciencia dels Materials, Universitat de Valencia, P.O. Box 22085, 46071-Valencia (Spain); Garro, N. [Institut de Ciencia dels Materials, Universitat de Valencia, P.O. Box 22085, 46071-Valencia (Spain); Fundacio General de la Universitat de Valencia, P.O. Box 22085, 46071-Valencia (Spain); Roever, M.; Mai, D.-D.; Bedoya-Pinto, A.; Malindretos, J.; Rizzi, A. [IV. Physikalisches Institut and Virtual Institute of Spin Electronics (VISel), Georg-August Universitaet Goettingen, D-37077 Goettingen (Germany)

    2008-07-14T23:59:59.000Z

    In this study, we report on the incorporation of dilute Gd amounts into GaN films grown by molecular beam epitaxy. A combination of x-ray fluorescence with x-ray absorption spectroscopic techniques enabled us to examine not only the distribution of rare earth atoms in the GaN matrix but also the short-range structural order. Our results show Gd atoms in a trivalent state with tetrahedral coordination, thus substituting Ga in the wurtzite GaN structure.

  10. Sensing mode atomic force microscope

    DOE Patents [OSTI]

    Hough, Paul V. C. (Port Jefferson, NY); Wang, Chengpu (Upton, NY)

    2003-01-01T23:59:59.000Z

    An atomic force microscope utilizes a pulse release system and improved method of operation to minimize contact forces between a probe tip affixed to a flexible cantilever and a specimen being measured. The pulse release system includes a magnetic particle affixed proximate the probe tip and an electromagnetic coil. When energized, the electromagnetic coil generates a magnetic field which applies a driving force on the magnetic particle sufficient to overcome adhesive forces exhibited between the probe tip and specimen. The atomic force microscope includes two independently displaceable piezo elements operable along a Z-axis. A controller drives the first Z-axis piezo element to provide a controlled approach between the probe tip and specimen up to a point of contact between the probe tip and specimen. The controller then drives the first Z-axis piezo element to withdraw the cantilever from the specimen. The controller also activates the pulse release system which drives the probe tip away from the specimen during withdrawal. Following withdrawal, the controller adjusts the height of the second Z-axis piezo element to maintain a substantially constant approach distance between successive samples.

  11. Graphene plasmonics for light trapping and absorption engineering

    E-Print Network [OSTI]

    Zhang, Jianfa; Liu, Wei; Yuan, Xiaodong; Qin, Shiqiao

    2015-01-01T23:59:59.000Z

    Plasmonics can be used to improve absorption in optoelectronic devices and has been intensively studied for solar cells and photodetectors. Graphene has recently emerged as a powerful plasmonic material. It shows significantly less losses compared to traditional plasmonic materials such as gold and silver and its plasmons can be tuned by changing the Fermi energy with chemical or electrical doping. Here we propose the usage of graphene plasmonics for light trapping in optoelectronic devices and show that the excitation of localized plasmons in doped, nanostructured graphene can enhance optical absorption in its surrounding media including both bulky and two-dimensional materials by tens of times, which may lead to a new generation of highly efficient, spectrally selective photodetectors in mid-infrared and THz ranges. The proposed concept could even revolutionize the field of plasmonic solar cells if graphene plasmons in the visible and near-infrared are realized.

  12. Universal bosonic tetramers of dimer-atom-atom structure

    E-Print Network [OSTI]

    A. Deltuva

    2012-03-28T23:59:59.000Z

    Unstable four-boson states having an approximate dimer-atom-atom structure are studied using momentum-space integral equations for the four-particle transition operators. For a given Efimov trimer the universal properties of the lowest associated tetramer are determined. The impact of this tetramer on the atom-trimer and dimer-dimer collisions is analyzed. The reliability of the three-body dimer-atom-atom model is studied.

  13. Universal bosonic tetramers of dimer-atom-atom structure

    E-Print Network [OSTI]

    Deltuva, A

    2012-01-01T23:59:59.000Z

    Unstable four-boson states having an approximate dimer-atom-atom structure are studied using momentum-space integral equations for the four-particle transition operators. For a given Efimov trimer the universal properties of the lowest associated tetramer are determined. The impact of this tetramer on the atom-trimer and dimer-dimer collisions is analyzed. The reliability of the three-body dimer-atom-atom model is studied.

  14. Silicate absorption in heavily obscured galaxy nuclei

    E-Print Network [OSTI]

    P. F. Roche; C. Packham; D. K. Aitken; R. E. Mason

    2006-10-19T23:59:59.000Z

    Spectroscopy at 8-13 microns with T-ReCS on Gemini-S is presented for 3 galaxies with substantial silicate absorption features, NGC 3094, NGC 7172 and NGC 5506. In the galaxies with the deepest absorption bands, the silicate profile towards the nuclei is well represented by the emissivity function derived from the circumstellar emission from the red supergiant, mu Cephei which is also representative of the mid-infrared absorption in the diffuse interstellar medium in the Galaxy. There is spectral structure near 11.2 microns in NGC 3094 which may be due to a component of crystalline silicates. In NGC 5506, the depth of the silicate absorption increases from north to south across the nucleus, suggestive of a dusty structure on scales of 10s of parsecs. We discuss the profile of the silicate absorption band towards galaxy nuclei and the relationship between the 9.7 micron silicate and 3.4 micron hydrocarbon absorption bands.

  15. Dicke-Type Energy Level Crossings in Cavity-Induced Atom Cooling: Another Superradiant Cooling

    E-Print Network [OSTI]

    Masao Hirokawa

    2008-12-19T23:59:59.000Z

    This paper is devoted to energy-spectral analysis for the system of a two-level atom coupled with photons in a cavity. It is shown that the Dicke-type energy level crossings take place when the atom-cavity interaction of the system undergoes changes between the weak coupling regime and the strong one. Using the phenomenon of the crossings we develop the idea of cavity-induced atom cooling proposed by the group of Ritsch, and we lay mathematical foundations of a possible mechanism for another superradiant cooling in addition to that proposed by Domokos and Ritsch. The process of our superradiant cooling can function well by cavity decay and by control of the position of the atom, at least in (mathematical) theory, even if there is neither atomic absorption nor atomic emission of photons.

  16. Cr Atom Alignment in Cr-Delta-Doped GaN

    SciTech Connect (OSTI)

    Kimura, S.; Emura, S.; Zhou, Y. K.; Choi, S. W.; Yamauchi, Y.; Hasegawa, S.; Asahi, H. [Institute of Scientific and Industrial Research, Osaka University, 8-1, Mihogaoka, Osaka, 567-0047 (Japan); Ofuchi, H. [SPring-8 / Japan Synchrotron Radiation Research Institute (JASRI), Sayo, Hyogo 679-5198 (Japan); Nakata, Y. [College of Science and Engineering, Iwaki Meisei University, Iwaki, Fukushima 970-8551 (Japan)

    2007-02-02T23:59:59.000Z

    Structural properties and Cr atom alignments in Cr-delta doped GaN grown by molecular beam epitaxy are studied with transmission electron microscopy and X-ray absorption fine structure (XAFS) measurements. It is found that the environment around Cr atoms in delta-doped samples is dramatically changed under various growth conditions. The XAFS analysis of these synthesized layers suggests that new Cr-related complexes are grown.

  17. X-ray absorption fine structure spectroscopic study of uranium nitrides

    SciTech Connect (OSTI)

    Poineau, Frederic [University of Nevada, Las Vegas; Yeamans, Charles B. [University of California, Berkeley; Cerefice, Gary S. [University of Nevada, Las Vegas; Sattelberger, Alfred P [Argonne National Laboratory (ANL); Czerwinski, Ken R. [University of Nevada, Las Vegas

    2012-01-01T23:59:59.000Z

    Uranium mononitride (UN), sesquinitride (U2N3) and dinitride (UN2) were characterized by extended X-Ray absorption fine structure spectroscopy. Analysis on UN indicate the presence of three uranium shells at distances of 3.46(3), 4.89(5) and 6.01(6) A and a nitrogen shell at a distance of 2.46(2) A . For U2N3, two absorbing uranium atoms at different crystallographic positions are present in the structure. One of the uranium atoms is surrounded by nitrogen atoms at 2.28(2) A and by uranium atoms at 3.66(4) and 3.95(4) A . The second type of uranium atom is surrounded by nitrogen atoms at 2.33(2) and 2.64(3) A and by uranium atoms at 3.66(4), 3.95(4) and 5.31(5) A . Results on UN2 indicate two uranium shells at 3.71(4) and 5.32(5) A and two nitrogen shells at 2.28(2).

  18. Combining Feedback Absorption Spectroscopy, Amplified Resonance...

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Compounds in Automotive Emissions Discusses a novel combination of multi-component scanning direct absorption spectroscopy, resonant cavity and low-pressure sampling to...

  19. Direct and quantitative absorptive spectroscopy of nanowires

    E-Print Network [OSTI]

    Tong, Jonathan Kien-Kwok

    2012-01-01T23:59:59.000Z

    Photonic nanostructures exhibit unique optical properties that are attractive in many different applications. However, measuring the optical properties of individual nanostructures, in particular the absorptive properties, ...

  20. Advanced Low Temperature Absorption Chiller Module Integrated...

    Broader source: Energy.gov (indexed) [DOE]

    Advanced Low Temperature Absorption Chiller Module Integrated with a CHP System at a Distributed Data Center - Presentation by Exergy Partners Corp., June 2011 Advanced Low...

  1. Nuclear-Motion Effects in Attosecond Transient Absorption Spectroscopy of Molecules

    E-Print Network [OSTI]

    Bækhøj, Jens E; Madsen, Lars Bojer

    2015-01-01T23:59:59.000Z

    We investigate the characteristic effects of nuclear motion on attosecond transient absorption spectra in molecules by calculating the spectrum for different model systems. Two models of the hydrogen molecular ion are considered: one where the internuclear separation is fixed, and one where the nuclei are free to vibrate. The spectra for the fixed nuclei model are similar to atomic spectra reported elsewhere, while the spectra obtained in the model including nuclear motion are very different and dominated by extremely broad absorption features. These broad absorption features are analyzed and their relation to molecular dissociation investigated. The study of the hydrogen molecular ion validates an approach based on the Born-Oppenheimer approximation and a finite electronic basis. This latter approach is then used to study the three-dimensional hydrogen molecule including nuclear vibration. The spectrum obtained from H$_2$ is compared to the result of a fixed-nuclei calculation. In the attosecond transient ab...

  2. Enhanced Two-Photon Absorption Using Entangled States and Small Mode Volumes

    E-Print Network [OSTI]

    Hao You; S. M. Hendrickson; J. D. Franson

    2009-07-13T23:59:59.000Z

    We calculate the rate of two-photon absorption for frequency entangled photons in a tapered optical fiber whose diameter is comparable to the wavelength of the light. The confinement of the electric field in the transverse direction increases the intensity associated with a single photon, while the two-photon absorption rate is further enhanced by the fact that the sum of the frequencies of the two photons is on resonance with the upper atomic state, even though each photon has a relatively broad linewidth. As a result, the photons are effectively confined in all three dimensions and the two-photon absorption rate for frequency-entangled photons in a tapered fiber was found to be comparable to that for unentangled photons in a microcavity with a small mode volume.

  3. Change in atomic coordination in a heavily deformed metallic glass

    SciTech Connect (OSTI)

    Liu, Y. [Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials, Ministry of Education, Shandong University, Jinan 250061 (China); Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Hahn-Meitner Platz 1, D-14109 Berlin (Germany); Schumacher, G. [Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Hahn-Meitner Platz 1, D-14109 Berlin (Germany); Riesemeier, H. [Bundesanstalt für Materialforschung und-prüfung, Unter den Eichen 87, D-12205 Berlin (Germany); Banhart, J. [Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Hahn-Meitner Platz 1, D-14109 Berlin (Germany); Technische Universität Berlin, Materials Science and Technology, Hardenbergstr. 36, 10623 Berlin (Germany)

    2014-05-28T23:59:59.000Z

    The local structure around Ni and La atoms in Al{sub 85}Ni{sub 10}La{sub 5} amorphous powder after ball milling was investigated by X-ray absorption spectroscopy. A continuous decrease in coordination number of Ni and La as a function of milling time was observed, while the nearest neighbour distance and the mean square atomic displacement did not change, pointing at the creation of free volume around the Ni and La atoms. These structural changes resemble those of a liquid upon temperature increase. The results are described by a shear band model in which the coordination numbers of Ni and La are different within and outside a shear band.

  4. X-ray absorption spectroscopic studies of the active sites of nickel- and copper-containing metalloproteins

    SciTech Connect (OSTI)

    Tan, G.O.

    1993-06-01T23:59:59.000Z

    X-ray absorption spectroscopy (XAS) is a useful tool for obtaining structural and chemical information about the active sites of metalloproteins and metalloenzymes. Information may be obtained from both the edge region and the extended X-ray absorption fine structure (EXAFS) or post-edge region of the K-edge X-ray absorption spectrum of a metal center in a compound. The edge contains information about the valence electronic structure of the atom that absorbs the X-rays. It is possible in some systems to infer the redox state of the metal atom in question, as well as the geometry and nature of ligands connected to it, from the features in the edge in a straightforward manner. The EXAFS modulations, being produced by the backscattering of the ejected photoelectron from the atoms surrounding the metal atom, provide, when analyzed, information about the number and type of neighbouring atoms, and the distances at which they occur. In this thesis, analysis of both the edge and EXAFS regions has been used to gain information about the active sites of various metalloproteins. The metalloproteins studied were plastocyanin (Pc), laccase and nickel carbon monoxide dehydrogenase (Ni CODH). Studies of Cu(I)-imidazole compounds, related to the protein hemocyanin, are also reported here.

  5. Atomic Force Microscope

    SciTech Connect (OSTI)

    Day, R.D.; Russell, P.E.

    1988-12-01T23:59:59.000Z

    The Atomic Force Microscope (AFM) is a recently developed instrument that has achieved atomic resolution imaging of both conducting and non- conducting surfaces. Because the AFM is in the early stages of development, and because of the difficulty of building the instrument, it is currently in use in fewer than ten laboratories worldwide. It promises to be a valuable tool for obtaining information about engineering surfaces and aiding the .study of precision fabrication processes. This paper gives an overview of AFM technology and presents plans to build an instrument designed to look at engineering surfaces.

  6. Iowa Powder Atomization Technologies

    ScienceCinema (OSTI)

    None

    2013-03-01T23:59:59.000Z

    The same atomization effect seen in a fuel injector is being applied to titanium metal resulting in fine titanium powders that are less than half the width of a human hair. Titanium melts above 3,000°F and is highly corrosive therefore requiring specialized containers. The liquid titanium is poured through an Ames Laboratory - USDOE patented tube which is intended to increase the energy efficiency of the atomization process, which has the ability to dramatically decrease the cost of fine titanium powders. This novel process could open markets for green manufacturing of titanium components from jet engines to biomedical implants.

  7. Iowa Powder Atomization Technologies

    SciTech Connect (OSTI)

    None

    2012-01-01T23:59:59.000Z

    The same atomization effect seen in a fuel injector is being applied to titanium metal resulting in fine titanium powders that are less than half the width of a human hair. Titanium melts above 3,000°F and is highly corrosive therefore requiring specialized containers. The liquid titanium is poured through an Ames Laboratory - USDOE patented tube which is intended to increase the energy efficiency of the atomization process, which has the ability to dramatically decrease the cost of fine titanium powders. This novel process could open markets for green manufacturing of titanium components from jet engines to biomedical implants.

  8. Tunable electromagnetically induced transparency and absorption with dressed superconducting qubits

    SciTech Connect (OSTI)

    Ian, Hou [Advanced Science Institute, RIKEN, Wako-shi, Saitama 351-0198 (Japan); Liu, Yu-xi [Advanced Science Institute, RIKEN, Wako-shi, Saitama 351-0198 (Japan); Institute of Microelectronics, Tsinghua University, Beijing 100084 (China); Tsinghua National Laboratory for Information Science and Technology (TNList), Tsinghua University, Beijing 100084 (China); Nori, Franco [Advanced Science Institute, RIKEN, Wako-shi, Saitama 351-0198 (Japan); Physics Department, The University of Michigan, Ann Arbor, Michagan 48109 (United States)

    2010-06-15T23:59:59.000Z

    Electromagnetically induced transparency and absorption (EIT and EIA) are usually demonstrated using three-level atomic systems. In contrast to the usual case, we theoretically study the EIT and EIA in an equivalent three-level system: a superconducting two-level system (qubit) dressed by a single-mode cavity field. In this equivalent system, we find that both the EIT and the EIA can be tuned by controlling the level-spacing of the superconducting qubit and hence controlling the dressed system. This tunability is due to the dressed relaxation and dephasing rates which vary parametrically with the level-spacing of the original qubit and thus affect the transition properties of the dressed qubit and the susceptibility. These dressed relaxation and dephasing rates characterize the reaction of the dressed qubit to an incident probe field. Using recent experimental data on superconducting qubits (charge, phase, and flux qubits) to demonstrate our approach, we show the possibility of experimentally realizing this proposal.

  9. Absorption-emission optrode and methods of use thereof

    DOE Patents [OSTI]

    Hirschfeld, Tomas B. (Livermore, CA)

    1990-01-01T23:59:59.000Z

    A method and apparatus for monitoring the physical and chemical properties of a sample fluid by measuring an optical signal generated by a fluorescent substance and modulated by an absorber substance. The emission band of the fluorescent substance overlaps the absorption band of the absorber substance, and the degree of overlap is dependent on the physical and chemical properties of the sample fluid. The fluorescent substance and absorber substance are immobilized on a substrate so that an effective number of molecules thereof are sufficiently close for resonant energy transfer to occur, thereby providing highly efficient modulation of the fluorescent emissions of the fluorescent substance by the absorber substance.

  10. Absorption-emission optrode and methods of use thereof

    DOE Patents [OSTI]

    Hirschfeld, T.B.

    1990-05-29T23:59:59.000Z

    A method and apparatus are described for monitoring the physical and chemical properties of a sample fluid by measuring an optical signal generated by a fluorescent substance and modulated by an absorber substance. The emission band of the fluorescent substance overlaps the absorption band of the absorber substance, and the degree of overlap is dependent on the physical and chemical properties of the sample fluid. The fluorescent substance and absorber substance are immobilized on a substrate so that an effective number of molecules thereof are sufficiently close for resonant energy transfer to occur, thereby providing highly efficient modulation of the fluorescent emissions of the fluorescent substance by the absorber substance. 4 figs.

  11. United States Department of Energy large commercial absorption chiller development program

    SciTech Connect (OSTI)

    Garland, P.W.; DeVault, R.C.; Zaltash, A.

    1998-11-01T23:59:59.000Z

    The US Department of Energy (DOE) is working with partners from the gas cooling industry to improve energy efficiency and US competitiveness by using advanced absorption technologies that eliminate the use of chlorofluorocarbons (CFCs) and hydrochlorofluorocarbons (HCFCs), refrigerants that contribute to ozone depletion and global warming. Absorption cooling uses natural gas as the heat source, which produces much lower NO{sub x} emissions than oil- or coal-generated electricity. Gas-fired chillers also have the advantage of helping reduce peak electrical usage during summer months. To assist industry in developing advanced absorption cooling technologies, DOE sponsors the Large Commercial Chiller Development Program. The goal of the program is to improve chiller cooling efficiency by 30--50% compared with the best currently available absorption systems.

  12. Cost reductions in absorption chillers. Final report, June 1984-May 1985

    SciTech Connect (OSTI)

    Leigh, R.W.

    1986-05-01T23:59:59.000Z

    Absorption chillers have great difficulty competing with the electric-driven compression alternative, due in part to modest operating efficiencies and largely to high first costs. This project is an assessment of the possibility of lowering the costs of absorption chillers dramatically by the use of low material intensity in the design of a new generation of these machines. Breakeven costs for absorption chillers, their heat exchangers and heat exchanger materials were established which will allow commercial success. Polymeric and metallic materials appropriate to particular components and which meet the cost goals were identified. A subset of these materials were tested and ordered by success in tolerating conditions and materials found in absorption chiller applications. Conceptual designs which indicate the practicality of the low material intensity approach were developed. The work reported here indicates that there is a high probability that this apporach will be successful.

  13. INCREASED LEAD ABSORPTION AND LEAD POISONING

    E-Print Network [OSTI]

    INCREASED LEAD ABSORPTION AND LEAD POISONING IN YOUNG CHILDREN A STATDIE:"IT BY THE CEJde slnt:t! the Surgeon GenerJi's Statement. "~edicJI Aspects of Childhood Lead POisoning," was issued:ld absorption Jnd lead poisoning. Such JCtivities for children will continue to be necessary until sources

  14. Broadband solar absorption enhancement via periodic

    E-Print Network [OSTI]

    Province, 230009, P. R. China. Solution processed colloidal quantum dot (CQD) solar cells have greatBroadband solar absorption enhancement via periodic nanostructuring of electrodes Michael M. Adachi demonstrate a bottom- illuminated periodic nanostructured CQD solar cell that enhances broadband absorption

  15. absorption: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Planning of Axiom Absorptions CiteSeer...

  16. Elements & Compounds Atoms (Elements)

    E-Print Network [OSTI]

    Frey, Terry

    #12;Elements & Compounds #12;Atoms (Elements) Molecules (Compounds) Cells Elements & Compounds #12 #12;First shell Second shell Third shell Hydrogen 1H Lithium 3Li Sodium 11Na Beryllium 4Be Magnesium energy Higher energy (a) A ball bouncing down a flight of stairs provides an analogy for energy levels

  17. Novel absorption detection techniques for capillary electrophoresis

    SciTech Connect (OSTI)

    Xue, Y.

    1994-07-27T23:59:59.000Z

    Capillary electrophoresis (CE) has emerged as one of the most versatile separation methods. However, efficient separation is not sufficient unless coupled to adequate detection. The narrow inner diameter (I.D.) of the capillary column raises a big challenge to detection methods. For UV-vis absorption detection, the concentration sensitivity is only at the {mu}M level. Most commercial CE instruments are equipped with incoherent UV-vis lamps. Low-brightness, instability and inefficient coupling of the light source with the capillary limit the further improvement of UV-vis absorption detection in CE. The goals of this research have been to show the utility of laser-based absorption detection. The approaches involve: on-column double-beam laser absorption detection and its application to the detection of small ions and proteins, and absorption detection with the bubble-shaped flow cell.

  18. Hydrogen Absorption in Pd-based Nanostructures - Final Report

    SciTech Connect (OSTI)

    David Lederman

    2012-10-22T23:59:59.000Z

    Pd is known to absorb hydrogen. Molecules are normally chemisorbed at the surface in a process where the molecule breaks into two hydrogen atoms, and the protons are then absorbed into the bulk. This process consists of electron filling holes in the Pd 4d band near the Fermi energy, which due to the high density of states at the Fermi energy, is an energetically favorable process. Our aim with this project was to determine possible changes in magnetic properties with Pd nm-length-scale thick layers intercalated by magnetic materials. Before the start of this work, the literature indicated that there were several possible scenarios by which this could happen: i) the Pd will be magnetized due to a proximity effect with nearby magnetic layers, resulting in changes in the magnetization due to H2 absorption; ii) some H will be absorbed into the magnetic layers, causing a change in the magnetic exchange interactions; or iii) absorption of H2 will cause an expansion of the lattice, resulting in a magnetoelastic effect which changes the magnetic properties.

  19. New results in atomic physics at the Advanced Light Source

    SciTech Connect (OSTI)

    Schlachter, A.S.

    1995-01-01T23:59:59.000Z

    The Advanced Light Source is the world's first low-energy third-generation synchrotron radiation source. It has been running reliably and exceeding design specifications since it began operation in October 1993. It is available to a wide community of researchers in many scientific fields, including atomic and molecular science and chemistry. Here, new results in atomic physics at the Advanced Light Source demonstrate the opportunities available in atomic and molecular physics at this synchrotron light source. The unprecedented brightness allows experiments with high flux, high spectral resolution, and nearly 100% linear polarization.

  20. The energy distribution of atoms in the field of thermal blackbody radiation

    E-Print Network [OSTI]

    F. V. Prigara

    2002-02-06T23:59:59.000Z

    Using the principle of detailed balance and the assumption on the absorption cross-section consistent with available astrophysical data, we obtain the energy distribution of atoms in the field of thermal blackbody radiation and show that this distribution diverges from the Boltzmann law.

  1. Atom-by-atom nucleation and growth of graphene nanopores

    E-Print Network [OSTI]

    Golovchenko, Jene A.

    Atom-by-atom nucleation and growth of graphene nanopores Christopher J. Russoa,b and J. A February 17, 2012 (received for review December 9, 2011) Graphene is an ideal thin membrane substrate structures in graphene with atomic preci- sion. It consists of inducing defect nucleation centers with ener

  2. Multimode Raman light-atom interface in warm atomic ensemble as multiple three-mode quantum operations

    E-Print Network [OSTI]

    Micha? Parniak; Daniel P?cak; Wojciech Wasilewski

    2015-06-08T23:59:59.000Z

    We analyze the properties of a Raman quantum light-atom interface in long atomic ensemble and its applications as a quantum memory or two-mode squeezed state generator. We include both Stokes and anti-Stokes scattering and the effects of Doppler broadening in buffer gas assuming frequent velocity-averaging collisions. We find the Green functions describing multimode transformation from input to output fields of photons and atomic excitations. Further considerations (following Sec. II D) are incorrect due to a mistake in finding a proper mode basis. Correct description is being worked out and should be published soon.

  3. Triple-effect absorption refrigeration system with double-condenser coupling

    DOE Patents [OSTI]

    DeVault, R.C.; Biermann, W.J.

    1993-04-27T23:59:59.000Z

    A triple effect absorption refrigeration system is provided with a double-condenser coupling and a parallel or series circuit for feeding the refrigerant-containing absorbent solution through the high, medium, and low temperature generators utilized in the triple-effect system. The high temperature condenser receiving vaporous refrigerant from the high temperature generator is double coupled to both the medium temperature generator and the low temperature generator to enhance the internal recovery of heat within the system and thereby increase the thermal efficiency thereof.

  4. Triple-effect absorption refrigeration system with double-condenser coupling

    DOE Patents [OSTI]

    DeVault, Robert C. (Knoxville, TN); Biermann, Wendell J. (Fayetteville, NY)

    1993-01-01T23:59:59.000Z

    A triple effect absorption refrigeration system is provided with a double-condenser coupling and a parallel or series circuit for feeding the refrigerant-containing absorbent solution through the high, medium, and low temperature generators utilized in the triple-effect system. The high temperature condenser receiving vaporous refrigerant from the high temperature generator is double coupled to both the medium temperature generator and the low temperature generator to enhance the internal recovery of heat within the system and thereby increase the thermal efficiency thereof.

  5. Atomic phenomena in dense plasmas

    SciTech Connect (OSTI)

    Weisheit, J.C.

    1981-03-01T23:59:59.000Z

    The following chapters are included: (1) the plasma environment, (2) perturbations of atomic structure, (3) perturbations of atomic collisions, (4) formation of spectral lines, and (5) dielectronic recombination. (MOW)

  6. Atom chip apparatus for experiments with ultracold rubidium and potassium gases

    SciTech Connect (OSTI)

    Ivory, M. K.; Ziltz, A. R.; Fancher, C. T.; Pyle, A. J.; Sensharma, A.; Chase, B.; Field, J. P.; Garcia, A.; Aubin, S., E-mail: saaubi@wm.edu [Department of Physics, College of William and Mary, Williamsburg, Virginia 23187 (United States); Jervis, D. [Department of Physics, University of Toronto, Toronto, Ontario M5S 1A7 (Canada)] [Department of Physics, University of Toronto, Toronto, Ontario M5S 1A7 (Canada)

    2014-04-15T23:59:59.000Z

    We present a dual chamber atom chip apparatus for generating ultracold {sup 87}Rb and {sup 39}K atomic gases. The apparatus produces quasi-pure Bose-Einstein condensates of 10{sup 4} {sup 87}Rb atoms in an atom chip trap that features a dimple and good optical access. We have also demonstrated production of ultracold {sup 39}K and subsequent loading into the chip trap. We describe the details of the dual chamber vacuum system, the cooling lasers, the magnetic trap, the multicoil magnetic transport system, the atom chip, and two optical dipole traps. Due in part to the use of light-induced atom desorption, the laser cooling chamber features a sufficiently good vacuum to also support optical dipole trap-based experiments. The apparatus is well suited for studies of atom-surface forces, quantum pumping and transport experiments, atom interferometry, novel chip-based traps, and studies of one-dimensional many-body systems.

  7. Tunable Electromagnetically Induced Transparency and Absorption with Dressed Superconducting Qubits

    E-Print Network [OSTI]

    Hou Ian; Yu-xi Liu; Franco Nori

    2010-07-06T23:59:59.000Z

    Electromagnetically induced transparency and absorption (EIT and EIA) are usually demonstrated by three-level atomic or atom-like systems. In contrast to the usual case, we theoretically study the EIT and EIA in an equivalent three-level system, which is constructed by dressing a superconducting two-level system (qubit) dressed by a single-mode cavity field. In this equivalent system, we find that both the EIT and the EIA can be tuned by controlling the level-spacing of the superconducting qubit and hence controlling the dressed system. This tunability is due to the dressed relaxation and dephasing rates which vary parametrically with the level-spacing of the original qubit and thus affect the transition properties of the dressed qubit and the susceptibility. These dressed relaxation and dephasing rates characterize the reaction of the dressed qubit to an incident probe field. We also use recent experimental data on superconducting qubits (charge, phase, and flux qubits) to demonstrate our approach and show the possibility of experimentally realizing this proposal.

  8. Structure and Mass Absorption of Hypothetical Terrestrial Black Holes

    E-Print Network [OSTI]

    A. P. VanDevender; J. Pace VanDevender

    2011-05-02T23:59:59.000Z

    The prospect of mini black holes, either primordial or in planned experiments at the Large Hadron Collider, interacting with the earth motivate us to examine how they may be detected and the scope of their impact on the earth. We propose that the more massive of these objects may gravitationally bind matter without significant absorption. Since the wave functions of gravitationally bound atoms orbiting a black hole are analogous to those of electrons around a nucleus, we call such an object the Gravitationally Equivalent of an Atom (GEA). Mini black holes are expected to lose mass through quantum evaporation, which has become well accepted on purely theoretical grounds. Since all attempts to directly observe x-rays from an evaporating black hole have failed, we examine the possibility of the inverse test: search for extant mini black holes by looking for emissions from matter bound in a GEA. If quantum evaporation does not occur, then miniature black holes left over from the early universe may be stable, contribute to dark matter, and in principle be detectable through emissions associated with the bound matter. We show that small black holes-with masses below \\sim10^12 kg-can bind matter without readily absorbing it into the black hole but the emissions are too weak to be detected from earth.

  9. atoms: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    with atomic and molecular matter waves is a rich branch of atomic physics and quantum optics. It started with atom diffraction from crystal surfaces and the separated oscillatory...

  10. The development and application of a diode-laser-based ultraviolet absorption sensor for nitric oxide

    E-Print Network [OSTI]

    Anderson, Thomas Nathan

    2004-09-30T23:59:59.000Z

    by the NO molecule to determine the concentration via optical absorption spectroscopy. UV radiation at 226.8 nm is generated by sum frequency mixing the outputs from a 395-nm external cavity diode laser (ECDL) and a 532-nm diode-pumped, intracavity frequency doubled...

  11. Solar control of radar wave absorption by the Martian ionosphere D. D. Morgan,1

    E-Print Network [OSTI]

    California at Berkeley, University of

    ionosphere, fails to detect the planetary surface. We have generated a statistical measure of the surface reflection visibility, which we plot as a time series and compare with both in situ particle data taken that are observed and that impede the use of the subsurface sounder. [4] Luckily, an analogous case of absorption

  12. Removal of hydrophobic Volatile Organic Compounds1 in an integrated process coupling Absorption and2

    E-Print Network [OSTI]

    Boyer, Edmond

    is an interesting method, owing to the low pressure drop generated and68 the low maintenance needed, contrarily to membrane processes that require high working pressures to69 treat low gas flow rates (Fig. 1). An emerging of the process, hydrophobic VOC27 absorption in a gas-liquid contactor, and biodegradation in the TPPB. VOC

  13. Influence of pp ions on pion absorption in H2 S. Jonsell,1

    E-Print Network [OSTI]

    energies before the moment of pion absorption by the proton, with significant impact on the interpretation pp state, giving, respectively, a discrete or a continuous distribution of kinetic energies questions of interest for the new generation of experiments determining the strong-force shift and width

  14. Thermoelectric Generators 1. Thermoelectric generator

    E-Print Network [OSTI]

    Lee, Ho Sung

    1 Thermoelectric Generators HoSung Lee 1. Thermoelectric generator 1.1 Basic Equations In 1821 effects are called the thermoelectric effects. The mechanisms of thermoelectricity were not understood. Cold Hot I - -- - - - - -- Figure 1 Electron concentration in a thermoelectric material. #12;2 A large

  15. automated hydride generation-cryotrapping-atomic: Topics by E...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Mohammad 3 Geoneutrino and Hydridic Earth model CERN Preprints Summary: Uranium, Thorium and Potassium-40 abundances in the Earth were calculated in the frame of Hydridic...

  16. A microfabricated atomic clock

    SciTech Connect (OSTI)

    Knappe, Svenja; Shah, Vishal; Schwindt, Peter D.D.; Hollberg, Leo; Kitching, John; Liew, Li-Anne; Moreland, John [Time and Frequency Division, National Institute of Standards and Technology, Boulder, Colorado 80305-3328 (United States); Electromagnetics Division, National Institute of Standards and Technology, Boulder, Colorado 80305-3328 (United States)

    2004-08-30T23:59:59.000Z

    Fabrication techniques usually applied to microelectromechanical systems (MEMS) are used to reduce the size and operating power of the core physics assembly of an atomic clock. With a volume of 9.5 mm{sup 3}, a fractional frequency instability of 2.5x10{sup -10} at 1 s of integration, and dissipating less than 75 mW of power, the device has the potential to bring atomically precise timing to hand-held, battery-operated devices. In addition, the design and fabrication process allows for wafer-level assembly of the structures, enabling low-cost mass-production of thousands of identical units with the same process sequence, and easy integration with other electronics.

  17. Total absorption by degenerate critical coupling

    SciTech Connect (OSTI)

    Piper, Jessica R., E-mail: jrylan@stanford.edu; Liu, Victor; Fan, Shanhui, E-mail: shanhui@stanford.edu [Ginzton Laboratory, Department of Electrical Engineering, Stanford University, Stanford, California 94305 (United States)

    2014-06-23T23:59:59.000Z

    We consider a mirror-symmetric resonator with two ports. We show that, when excited from a single port, complete absorption can be achieved through critical coupling to degenerate resonances with opposite symmetry. Moreover, any time two resonances with opposite symmetry are degenerate in frequency and absorption is always significantly enhanced. In contrast, when two resonances with the same symmetry are nearly degenerate, there is no absorption enhancement. We numerically demonstrate these effects using a graphene monolayer on top of a photonic crystal slab, illuminated from a single side in the near-infrared.

  18. DEVELOPMENT OF SOLAR DRIVEN ABSORPTION AIR CONDITIONERS AND HEAT PUMPS

    E-Print Network [OSTI]

    Dao, K.

    2013-01-01T23:59:59.000Z

    SOLAR DRIVEN ABSORPTION AIR CONDITIONERS AND HEAT PUMPS K.Driven Absorption Air-Conditioner", K. Dao, M. Simmons, R.SOLAR DRIVEN ABSORPTION AIR CONDITIONERS AND HEAT PUMPS* K.

  19. Self-consistent modeling of radio-frequency plasma generation in stellarators

    SciTech Connect (OSTI)

    Moiseenko, V. E., E-mail: moiseenk@ipp.kharkov.ua; Stadnik, Yu. S., E-mail: stadnikys@kipt.kharkov.ua [National Academy of Sciences of Ukraine, National Science Center Kharkov Institute of Physics and Technology (Ukraine); Lysoivan, A. I., E-mail: a.lyssoivan@fz-juelich.de [Royal Military Academy, EURATOM-Belgian State Association, Laboratory for Plasma Physics (Belgium); Korovin, V. B. [National Academy of Sciences of Ukraine, National Science Center Kharkov Institute of Physics and Technology (Ukraine)] [National Academy of Sciences of Ukraine, National Science Center Kharkov Institute of Physics and Technology (Ukraine)

    2013-11-15T23:59:59.000Z

    A self-consistent model of radio-frequency (RF) plasma generation in stellarators in the ion cyclotron frequency range is described. The model includes equations for the particle and energy balance and boundary conditions for Maxwell’s equations. The equation of charged particle balance takes into account the influx of particles due to ionization and their loss via diffusion and convection. The equation of electron energy balance takes into account the RF heating power source, as well as energy losses due to the excitation and electron-impact ionization of gas atoms, energy exchange via Coulomb collisions, and plasma heat conduction. The deposited RF power is calculated by solving the boundary problem for Maxwell’s equations. When describing the dissipation of the energy of the RF field, collisional absorption and Landau damping are taken into account. At each time step, Maxwell’s equations are solved for the current profiles of the plasma density and plasma temperature. The calculations are performed for a cylindrical plasma. The plasma is assumed to be axisymmetric and homogeneous along the plasma column. The system of balance equations is solved using the Crank-Nicholson scheme. Maxwell’s equations are solved in a one-dimensional approximation by using the Fourier transformation along the azimuthal and longitudinal coordinates. Results of simulations of RF plasma generation in the Uragan-2M stellarator by using a frame antenna operating at frequencies lower than the ion cyclotron frequency are presented. The calculations show that the slow wave generated by the antenna is efficiently absorbed at the periphery of the plasma column, due to which only a small fraction of the input power reaches the confinement region. As a result, the temperature on the axis of the plasma column remains low, whereas at the periphery it is substantially higher. This leads to strong absorption of the RF field at the periphery via the Landau mechanism.

  20. Hydrogen atom in Palatini theories of gravity

    E-Print Network [OSTI]

    Gonzalo J. Olmo

    2008-06-03T23:59:59.000Z

    We study the effects that the gravitational interaction of $f(R)$ theories of gravity in Palatini formalism has on the stationary states of the Hydrogen atom. We show that the role of gravity in this system is very important for lagrangians $f(R)$ with terms that grow at low curvatures, which have been proposed to explain the accelerated expansion rate of the universe. We find that new gravitationally induced terms in the atomic Hamiltonian generate a strong backreaction that is incompatible with the very existence of bound states. In fact, in the 1/R model, Hydrogen disintegrates in less than two hours. The universe that we observe is, therefore, incompatible with that kind of gravitational interaction. Lagrangians with high curvature corrections do not lead to such instabilities.

  1. Matter pulse carving: Manipulating quantum wave packets via time-dependent absorption

    E-Print Network [OSTI]

    Goussev, Arseni

    2015-01-01T23:59:59.000Z

    A pulse of matter waves may dramatically change its shape when traversing an absorbing barrier with time-dependent transparency. Here we show that this effect can be utilized for controlled manipulation of spatially-localized quantum states. In particular, in the context of atom-optics experiments, we explicitly demonstrate how the proposed approach can be used to generate spatially shifted, split, squeezed and cooled atomic wave packets. We expect our work to be useful in devising new interference experiments with atoms and molecules and, more generally, to enable new ways of coherent control of matter waves.

  2. Absorption Heat Pumping- Have You Tried It? 

    E-Print Network [OSTI]

    Davis, R. C.

    1985-01-01T23:59:59.000Z

    The concept of a thermal powered absorption heat pump is not a new or revolutionary idea. It has been successfully demonstrated in the lab and prototypes have been installed in the field. Units have been successfully applied in a number...

  3. Variable effect desorber-resorber absorption cycle

    DOE Patents [OSTI]

    Biermann, Wendell J. (Fayetteville, NY)

    1985-01-01T23:59:59.000Z

    An absorption refrigeration system has an intermediate temperature desorber-resorber pair. A valve between the desorber-resorber pair is modulated to control the capacity for load matching.

  4. Visible spectrometer utilizing organic thin film absorption

    E-Print Network [OSTI]

    Tiefenbruck, Laura C. (Laura Christine)

    2004-01-01T23:59:59.000Z

    In this thesis, I modeled and developed a spectrometer for the visible wavelength spectrum, based on absorption characteristics of organic thin films. The device uses fundamental principles of linear algebra to reconstruct ...

  5. Absorption chillers: Part of the solution

    SciTech Connect (OSTI)

    Occhionero, A.J. (American Gas Cooling Center, Arlington, VA (United States)); Hughes, P.J. (Oak Ridge National Lab., TN (United States)); Reid, E.A. (Columbia Gas Distribution Co., Columbus, OH (United States))

    1991-01-01T23:59:59.000Z

    Acid rain, ozone depletion, global warming, and implementation economics are considered as they relate to the advisability of expanding the application of absorption chillers. Introductory and background information are provided to put the discussion in the proper context. Then all four issues are discussed separately as they relate to absorption chillers. Acid rain and ozone depletion concerns, and implementation economics, are found to support the expanded use of absorption chillers. The global warming concern is found to be more of a gray area, but the areas of benefit correspond well with the conditions of greatest economic advantage. All things considered, absorption chillers are believed to be part of the environmental and economic solution. It is further believed that integrated resource planning (IRP) processes that consider electric and gas technologies on an equal footing would come to the same conclusion for many regions of the United States. 9 refs., 3 tabs.

  6. Absorption Heat Pumping- Have You Tried It?

    E-Print Network [OSTI]

    Davis, R. C.

    The concept of a thermal powered absorption heat pump is not a new or revolutionary idea. It has been successfully demonstrated in the lab and prototypes have been installed in the field. Units have been successfully applied in a number...

  7. Reduction in biomass burning aerosol light absorption upon humidificat...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    in biomass burning aerosol light absorption upon humidification: Roles of inorganically-induced hygroscopicity, Reduction in biomass burning aerosol light absorption upon...

  8. absorption heat: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    drive compressor heat pump; (3) absorption heat pump; (4) high temperature heat powered compressor heat pump; (5) reverse absorption heat... Erickson, D. C. 1983-01-01 26...

  9. acoustic power absorption: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The distribution of acoustic power over sunspots shows an enhanced absorption near the umbra--penumbra boundary. Earlier studies revealed that the region of enhanced absorption...

  10. The Future of Absorption Technology in America: A Critical Look...

    Broader source: Energy.gov (indexed) [DOE]

    The Future of Absorption Technology in America: A Critical Look at the Impact of Building, Cooling, Heating, and Power (BCHP) and Innovation, June 2000 The Future of Absorption...

  11. Influence of atomic polarization and horizontal illumination on the Stokes profiles of the He I 10830 multiplet

    E-Print Network [OSTI]

    J. Trujillo Bueno; A. Asensio Ramos

    2006-10-04T23:59:59.000Z

    The polarization observed in the spectral lines of the He I 10830 multiplet carries valuable information on the dynamical and magnetic properties of plasma structures in the solar chromosphere and corona, such as spicules, prominences, filaments, emerging magnetic flux regions, etc. Here we investigate the influence of atomic level polarization on the emergent Stokes profiles for a broad range of magnetic field strengths, in both 90 degree and forward scattering geometry. We show that, contrary to a widespread belief, the selective emission and absorption processes caused by the presence of atomic level polarization may have an important influence on the emergent linear polarization, even for magnetic field strengths as large as 1000 G. Consequently, the modeling of the Stokes Q and U profiles should not be done by taking only into account the contribution of the transverse Zeeman effect within the framework of the Paschen-Back effect theory, unless the magnetic field intensity of the observed plasma structure is sensibly larger than 1000 G. We point out also that in low-lying optically thick plasma structures, such as those of active region filaments, the (horizontal) radiation field generated by the structure itself may substantially reduce the positive contribution to the anisotropy factor caused by the (vertical) radiation field coming from the underlying solar photosphere, so that the amount of atomic level polarization may turn out to be negligible. Only under such circumstances may the emergent linear polarization of the He I 10830 multiplet in such regions of the solar atmosphere be dominated by the contribution caused by the transverse Zeeman effect.

  12. Absorption cross section of RN black hole

    E-Print Network [OSTI]

    Sini R.; V. C. Kuriakose

    2007-08-23T23:59:59.000Z

    The behavior of a charged scalar field in the RN black hole space time is studied using WKB approximation. In the present work it is assumed that matter waves can get reflected from the event horizon. Using this effect, the Hawking temperature and the absorption cross section for RN black hole placed in a charged scalar field are calculated. The absorption cross section $\\sigma _{abs}$ is found to be inversely proportional to square of the Hawking temperature of the black hole.

  13. Optics and interferometry with atoms and molecules

    E-Print Network [OSTI]

    Cronin, Alexander D.

    Interference with atomic and molecular matter waves is a rich branch of atomic physics and quantum optics. It started with atom diffraction from crystal surfaces and the separated oscillatory fields technique used in atomic ...

  14. Resonant absorption and not-so-resonant absorption in short, intense laser irradiated plasma

    SciTech Connect (OSTI)

    Ge, Z. Y.; Zhuo, H. B.; Ma, Y. Y.; Yang, X. H.; Yu, T. P.; Zou, D. B.; Yin, Y.; Shao, F. Q. [College of Science, National University of Defense Technology, Changsha 410073 (China)] [College of Science, National University of Defense Technology, Changsha 410073 (China); Yu, W.; Luan, S. X. [Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800 (China)] [Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800 (China); Zhou, C. T. [College of Science, National University of Defense Technology, Changsha 410073 (China) [College of Science, National University of Defense Technology, Changsha 410073 (China); Institute of Applied Physics and Computational Mathematics, Beijing 100088 (China); Peng, X. J. [Institute of Applied Physics and Computational Mathematics, Beijing 100088 (China)] [Institute of Applied Physics and Computational Mathematics, Beijing 100088 (China)

    2013-07-15T23:59:59.000Z

    An analytical model for laser-plasma interaction during the oblique incidence by an ultrashort ultraintense p-polarized laser on a solid-density plasma is proposed. Both the resonant absorption and not-so-resonant absorption are self-consistently included. Different from the previous theoretical works, the physics of resonant absorption is found to be valid in more general conditions as the steepening of the electron density profile is considered. Even for a relativistic intensity laser, resonant absorption can still exist under certain plasma scale length. For shorter plasma scale length or higher laser intensity, the not-so-resonant absorption tends to be dominant, since the electron density is steepened to a critical level by the ponderomotive force. The laser energy absorption rates for both mechanisms are discussed in detail, and the difference and transition between these two mechanisms are presented.

  15. Force-controlled absorption in a fully-nonlinear numerical wave tank

    SciTech Connect (OSTI)

    Spinneken, Johannes, E-mail: j.spinneken@imperial.ac.uk; Christou, Marios; Swan, Chris

    2014-09-01T23:59:59.000Z

    An active control methodology for the absorption of water waves in a numerical wave tank is introduced. This methodology is based upon a force-feedback technique which has previously been shown to be very effective in physical wave tanks. Unlike other methods, an a-priori knowledge of the wave conditions in the tank is not required; the absorption controller being designed to automatically respond to a wide range of wave conditions. In comparison to numerical sponge layers, effective wave absorption is achieved on the boundary, thereby minimising the spatial extent of the numerical wave tank. In contrast to the imposition of radiation conditions, the scheme is inherently capable of absorbing irregular waves. Most importantly, simultaneous generation and absorption can be achieved. This is an important advance when considering inclusion of reflective bodies within the numerical wave tank. In designing the absorption controller, an infinite impulse response filter is adopted, thereby eliminating the problem of non-causality in the controller optimisation. Two alternative controllers are considered, both implemented in a fully-nonlinear wave tank based on a multiple-flux boundary element scheme. To simplify the problem under consideration, the present analysis is limited to water waves propagating in a two-dimensional domain. The paper presents an extensive numerical validation which demonstrates the success of the method for a wide range of wave conditions including regular, focused and random waves. The numerical investigation also highlights some of the limitations of the method, particularly in simultaneously generating and absorbing large amplitude or highly-nonlinear waves. The findings of the present numerical study are directly applicable to related fields where optimum absorption is sought; these include physical wavemaking, wave power absorption and a wide range of numerical wave tank schemes.

  16. Testing of Crystallization Temperature of a New Working Fluid for Absorption Heat Pump Systems

    SciTech Connect (OSTI)

    Wang, Kai [ORNL] [ORNL; Kisari, Padmaja [ORNL] [ORNL; Abdelaziz, Omar [ORNL] [ORNL; Vineyard, Edward Allan [ORNL] [ORNL

    2010-01-01T23:59:59.000Z

    Lithium bromide/water (LiBr/water) absorption systems are potential candidates for absorption heat pump water heating applications since they have been widely commercialized for cooling applications. One drawback to LiBr/water absorption water heater systems is that they are unable to operate at typical water heating temperatures due to solution crystallization hazards. Binary or ternary mixtures, serving as working fluids, were reported (Ally, 1988; Herold et al., 1991; Iyoki and Uemura, 1981; Yasuhide Nemoto et al., 2010; Zogg et al., 2005) to help improve the absorption performance or avoid crystallization of absorption heat pump systems. A recent development (De Lucas et al., 2007) investigated the use of a ternary mixture of aqueous mixture of lithium bromide and sodium formate (CHO2Na). The new working fluid composition maintains a ratio of LiBr/CHO2Na of 2 by weight. This new working fluid is a potential competitor to aqueous LiBr solution in absorption system due to higher water vapor absorption rates and lower generation temperature needed (De Lucas et al., 2004). There exists data on equilibrium performance and other physical properties of this new working fluid. However, there is no available data on crystallization behavior. Crystallization temperature is crucial for the design of absorption heat pump water heater in order to avoid crystallization hazards during operation. We have therefore conducted a systematic study to explore the crystallization temperature of LiBr/CHO2Na water solution and compared it against aqueous LiBr solutions. These results were then used to evaluate the feasibility of using the new working fluid in water heating applications showing limited potential.

  17. Atomic Collapse Observed

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative1 First Use of Energy for All Purposes (Fuel and Nonfuel), 2002; Level: National5Sales for4,645 3,625govInstrumentstdmadapInactiveVisiting the TWP TWPAlumni AlumniFederalAshley BoyleAn overhead viewAtom-split it

  18. Laser system for secondary cooling of {sup 87}Sr atoms

    SciTech Connect (OSTI)

    Khabarova, K Yu; Slyusarev, S N; Strelkin, S A; Belotelov, G S; Kostin, A S; Pal'chikov, Vitaly G; Kolachevsky, Nikolai N

    2012-11-30T23:59:59.000Z

    A laser system with a narrow generation line for secondary laser cooling of {sup 87}Sr atoms has been developed and investigated. It is planned to use ultracold {sup 87}Sr atoms loaded in an optical lattice in an optical frequency standard. To this end, a 689-nm semiconductor laser has been stabilised using an external reference ultrastable cavity with vibrational and temperature compensation near the critical point. The lasing spectral width was 80 Hz (averaging time 40 ms), and the frequency drift was at a level of 0.3 Hz s{sup -1}. Comparison of two independent laser systems yielded a minimum Allan deviation: 2 Multiplication-Sign 10{sup -14} for 300-s averaging. It is shown that this system satisfies all requirements necessary for secondary cooling of 87Sr atoms using the spectrally narrow {sup 1}S{sub 0} - {sup 3}P{sub 1} transition ({lambda} = 689 nm). (cooling of atoms)

  19. Enhancement of near-infrared absorption in graphene with metal gratings

    SciTech Connect (OSTI)

    Zhao, B.; Zhang, Z. M., E-mail: zhuomin.zhang@me.gatech.edu [G.W. Woodruff School of Mechanical Engineering, Georgia Institute of Technology, Atlanta, Georgia 30332 (United States); Zhao, J. M. [G.W. Woodruff School of Mechanical Engineering, Georgia Institute of Technology, Atlanta, Georgia 30332 (United States); School of Energy Science and Engineering, Harbin Institute of Technology, Harbin (China)

    2014-07-21T23:59:59.000Z

    Graphene has been demonstrated as a good candidate for ultrafast optoelectronic devices. However, graphene is essentially transparent in the visible and near infrared with an absorptivity of 2.3%, which has largely limited its application in photon detection. This Letter demonstrates that the absorptance in a monatomic graphene layer can be greatly enhanced to nearly 70%, thanks to the localized strong electric field resulting from magnetic resonances in deep metal gratings. Furthermore, the resonance frequency is essentially not affected by the additional graphene layer. The method presented here may benefit the design of next-generation graphene-based optical and optoelectronic devices.

  20. Jitter radiation in gamma-ray bursts and their afterglows: emission and self-absorption

    E-Print Network [OSTI]

    Jared Workman; Brian Morsony; Davide Lazzati; Mikhail Medvedev

    2008-01-23T23:59:59.000Z

    Relativistic electrons moving into a highly tangled magnetic field emit jitter radiation. We present a detailed computation of the jitter radiation spectrum, including self-absorption, for electrons inside Weibel-like shock generated magnetic fields. We apply our results to the case of the prompt and afterglow emission of gamma-ray bursts. We show that jitter emission can reproduce most of the observed features with some important differences with respect to standard synchrotron, especially in the frequency range between the self-absorption and the peak frequency. We discuss the similarities and differences between jitter and synchrotron and discuss experiments that can disentangle the two mechanisms.

  1. A Single-Photon Server with Just One Atom

    E-Print Network [OSTI]

    Markus Hijlkema; Bernhard Weber; Holger P. Specht; Simon C. Webster; Axel Kuhn; Gerhard Rempe

    2007-02-05T23:59:59.000Z

    Neutral atoms are ideal objects for the deterministic processing of quantum information. Entanglement operations have been performed by photon exchange or controlled collisions. Atom-photon interfaces were realized with single atoms in free space or strongly coupled to an optical cavity. A long standing challenge with neutral atoms, however, is to overcome the limited observation time. Without exception, quantum effects appeared only after ensemble averaging. Here we report on a single-photon source with one-and-only-one atom quasi permanently coupled to a high-finesse cavity. Quasi permanent refers to our ability to keep the atom long enough to, first, quantify the photon-emission statistics and, second, guarantee the subsequent performance as a single-photon server delivering up to 300,000 photons for up to 30 seconds. This is achieved by a unique combination of single-photon generation and atom cooling. Our scheme brings truly deterministic protocols of quantum information science with light and matter within reach.

  2. Atoms.inp Archive: Crystallographic Data from GSECARS

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Newville, Matthew

    The Atoms.inp Archive is a collection of crystallographic data for use in XAFS analysis. The crystallographic data is stored as atoms.inp files, which contain all the information necessary to describe the crystal, and can be used by the program ATOMS to generate feff.inp files. These files can then be used by the FEFF program [See http://leonardo.phys.washington.edu/feff/] to calculate a theoretical XAFS spectrum for the crystal. This archive exists because it can take a considerable amount of time to locate a suitable reference for a model structure to use for making theoretical XAFS standards. Even then, references sometimes give non-standard or incomplete crystallographic notation that ATOMS has difficulty interpreting. All of this means that getting a reliable atoms.inp file can take quite a bit of effort. It is hoped that this collection of well-documented and well-tested atoms.inp files will eliminate much of the work in creating theoretical XAFS standards from FEFF. [Taken from http://cars9.uchicago.edu/~newville/adb/]. The collection currently has more than 200 crystal structures, 2748 data files, and it continues to expand. The collection is related to the UWXAFS Project [http://depts.washington.edu/uwxafs/] and to the work of the Consortium for Advanced Radiation Sources (CARS). After searching the Archive, a user may also choose to run the web version of ATOMS software.

  3. Atomic Energy Commission Takes Over Responsibility for all Atomic...

    National Nuclear Security Administration (NNSA)

    Takes Over Responsibility for all Atomic Energy Programs | National Nuclear Security Administration Facebook Twitter Youtube Flickr RSS People Mission Managing the Stockpile...

  4. The use of solvent extraction in trace metal analysis by atomic absorption spectroscopy

    E-Print Network [OSTI]

    Eddy, Raymond Douglas

    1968-01-01T23:59:59.000Z

    . , reagen4 grade. NamHPOn ~ 7H-. . G T ' Till 68 08 Fe . ?. 0. 0003'Ii. S~ diun; di. hy;!i'cg=n phosphate, J. T. Baker, rcag?nt grade. F. W. 138. 00. Sodium tartrate, J. T. Baker, reagent grade. Nae04H40e 2HnO F. W. 250. 08 Fe = 0. 0002/0. d... the sta!&dards ;&ere prepared. The solutions werc pipeti, ed. into a 125&-ml pear-sba d. separatory funnel and. 5 ml of 41 reagen4 sclurion &;as added. '!ne rsixture was shaken for I'ive s&inutes. 'The layers were allowed to separate snd th or- ganic...

  5. atomic-absorption flame photometry: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    to modeling thermonuclear flames CiteSeer Summary: Turbulence-flame interactions of thermonuclear fusion flames occurring in Type Ia Supernovae were studied by means of...

  6. USE OF ZEEMAN ATOMIC ABSORPTION SPECTROSCOPY FOR THE MEASUREMENT OF MERCURY IN OIL SHALE GASES

    E-Print Network [OSTI]

    Girvin, D.G.

    2011-01-01T23:59:59.000Z

    A. Robb, and T. J. Spedding. Minor Elements in Oil Shale andOil-Shale Products. LERC RI 77-1, 1977. Bertine, K. K. andFrom A Simulated In-Situ Oil Shale Retort. In: Procedings of

  7. USE OF ZEEMAN ATOMIC ABSORPTION SPECTROSCOPY FOR THE MEASUREMENT OF MERCURY IN OIL SHALE GASES

    E-Print Network [OSTI]

    Girvin, D.G.

    2011-01-01T23:59:59.000Z

    W. A. Robb, and T. J. Spedding. Minor Elements in Oil Shaleand Oil-Shale Products. LERC RI 77-1, 1977. Bertine, K. K.From A Simulated In-Situ Oil Shale Retort. In: Procedings of

  8. USE OF ZEEMAN ATOMIC ABSORPTION SPECTROSCOPY FOR THE MEASUREMENT OF MERCURY IN OIL SHALE GASES

    E-Print Network [OSTI]

    Girvin, D.G.

    2011-01-01T23:59:59.000Z

    Minor Elements in Oil Shale and Oil-Shale Products. LERC RIChemistry of Tar Sands and Oil Shale, ACS, New Orleans.Constituent Analysis of Oil Shale and Solvent-Refined Coal

  9. NOx reduction by electron beam-produced nitrogen atom injection

    DOE Patents [OSTI]

    Penetrante, Bernardino M. (San Ramon, CA)

    2002-01-01T23:59:59.000Z

    Deactivated atomic nitrogen generated by an electron beam from a gas stream containing more than 99% N.sub.2 is injected at low temperatures into an engine exhaust to reduce NOx emissions. High NOx reduction efficiency is achieved with compact electron beam devices without use of a catalyst.

  10. Comprehensive online Atomic Database Management System (DBMS) with Highly Qualified Computing Capabilities

    E-Print Network [OSTI]

    Tahat, Amani

    2011-01-01T23:59:59.000Z

    The intensive need of atomic data is expanding continuously in a wide variety of applications (e.g. fusion energy and astrophysics, laser-produced, plasma researches, and plasma processing).This paper will introduce our ongoing research work to build a comprehensive, complete, up-to-date, user friendly and online atomic Database Management System (DBMS) namely called AIMS by using SQLite (http://www.sqlite.org/about.html)(8). Programming language tools and techniques will not be covered here. The system allows the generation of various atomic data based on professional online atomic calculators. The ongoing work is a step forward to bring detailed atomic model accessible to a wide community of laboratory and astrophysical plasma diagnostics. AIMS is a professional worldwide tool for supporting several educational purposes and can be considered as a complementary database of IAEA atomic databases. Moreover, it will be an exceptional strategy of incorporating the output data of several atomic codes to external ...

  11. Generator-absorber-heat exchange heat transfer apparatus and method and use thereof in a heat pump

    DOE Patents [OSTI]

    Phillips, Benjamin A. (Benton Harbor, MI); Zawacki, Thomas S. (St. Joseph, MI)

    1998-07-21T23:59:59.000Z

    Numerous embodiments and related methods for generator-absorber heat exchange (GAX) are disclosed, particularly for absorption heat pump systems. Such embodiments and related methods use, as the heat transfer medium, the working fluid of the absorption system taken from the generator at a location where the working fluid has a rich liquor concentration.

  12. Generator-absorber-heat exchange heat transfer apparatus and method and use thereof in a heat pump

    DOE Patents [OSTI]

    Phillips, B.A.; Zawacki, T.S.

    1998-07-21T23:59:59.000Z

    Numerous embodiments and related methods for generator-absorber heat exchange (GAX) are disclosed, particularly for absorption heat pump systems. Such embodiments and related methods use, as the heat transfer medium, the working fluid of the absorption system taken from the generator at a location where the working fluid has a rich liquor concentration. 5 figs.

  13. Quantum transport in ultracold atoms

    E-Print Network [OSTI]

    Chih-Chun Chien; Sebastiano Peotta; Massimiliano Di Ventra

    2015-04-11T23:59:59.000Z

    Ultracold atoms confined by engineered magnetic or optical potentials are ideal systems for studying phenomena otherwise difficult to realize or probe in the solid state because their atomic interaction strength, number of species, density, and geometry can be independently controlled. This review focuses on quantum transport phenomena in atomic gases that mirror and oftentimes either better elucidate or show fundamental differences with those observed in mesoscopic and nanoscopic systems. We discuss significant progress in performing transport experiments in atomic gases, contrast similarities and differences between transport in cold atoms and in condensed matter systems, and survey inspiring theoretical predictions that are difficult to verify in conventional setups. These results further demonstrate the versatility offered by atomic systems in the study of nonequilibrium phenomena and their promise for novel applications.

  14. Experimental Effects of Atomic Oxygen on the Development of an Electric Discharge Oxygen Iodine Laser

    E-Print Network [OSTI]

    Carroll, David L.

    state I. Conventionally, a two-phase (gas-liquid) chemistry singlet oxygen generator (SOG) producesExperimental Effects of Atomic Oxygen on the Development of an Electric Discharge Oxygen Iodine of the electric discharge iodine laser continues, the role of oxygen atoms downstream of the discharge region

  15. Nitrogen Dioxide Absorption and Sulfite Oxidation in Aqueous Sulfite

    E-Print Network [OSTI]

    Rochelle, Gary T.

    Nitrogen Dioxide Absorption and Sulfite Oxidation in Aqueous Sulfite C H E N H . S H E N A N D G by absorption in sulfite solution in existing scrubbers for desulfurization. Rates of NO2 absorption and sulfite absorption initiates sulfite oxidation in the presence of oxygen, and this study quantified the effect

  16. Simulating a 4-effect absorption chiller

    SciTech Connect (OSTI)

    Grossman, G. [Technion-Israel Inst. of Tech., Haifa (Israel). Dept. of Mechanical Engineering; Zaltash, A.; Adcock, P.W.; DeVault, R.C. [Oak Ridge National Lab., TN (United States). Energy Div.

    1995-06-01T23:59:59.000Z

    Absorption chillers are heat-operated refrigeration machines that operate on one of the earliest known principles of refrigeration. Current absorption chillers typically use either steam or a gas-fired burner as the energy source. All current gas-fired absorption cooling systems are based on the well known single-effect or double-effect cycles. To further improve utilization of the high temperature heat available from natural gas, a variety of triple-effect cycles have been proposed and are being developed that are capable of substantial performance improvement over equivalent double-effect cycles. This article describes a study that investigated the possibility of even further improving utilization of the high temperature heat available from natural gas combustion. During the study, performance simulation was conducted for a 4-effect lithium bromide/water cycle. From an environmental perspective, absorption chillers provide several benefits. They use absorption pairs (such as lithium bromide/water) as the working fluids, rather than chlorofluorocarbons or hydrochlorofluorocarbons, which contribute to ozone depletion and global warming.

  17. Atomic Inference from Weak Gravitational Lensing Data

    SciTech Connect (OSTI)

    Marshall, Phil; /KIPAC, Menlo Park

    2005-12-14T23:59:59.000Z

    We present a novel approach to reconstructing the projected mass distribution from the sparse and noisy weak gravitational lensing shear data. The reconstructions are regularized via the knowledge gained from numerical simulations of clusters, with trial mass distributions constructed from n NFW profile ellipsoidal components. The parameters of these ''atoms'' are distributed a priori as in the simulated clusters. Sampling the mass distributions from the atom parameter probability density function allows estimates of the properties of the mass distribution to be generated, with error bars. The appropriate number of atoms is inferred from the data itself via the Bayesian evidence, and is typically found to be small, reecting the quality of the data. Ensemble average mass maps are found to be robust to the details of the noise realization, and succeed in recovering the demonstration input mass distribution (from a realistic simulated cluster) over a wide range of scales. As an application of such a reliable mapping algorithm, we comment on the residuals of the reconstruction and the implications for predicting convergence and shear at specific points on the sky.

  18. The effects of pre-formed plasma on the generation and transport of fast electrons in relativistic laser-solid interactions

    E-Print Network [OSTI]

    Paradkar, Bhooshan S.

    2012-01-01T23:59:59.000Z

    Langdon. Absorption of ultra-intense laser pulses. Physicalproton generation in ultra-intense laser–solid interactions.heating in ultra high intensity laser-plasma interaction.

  19. Soft x-ray generation in gases with an ultrashort pulse laser

    SciTech Connect (OSTI)

    Ditmire, T.R.

    1996-01-08T23:59:59.000Z

    An experimental investigation of soft x-ray production resulting from the interaction of intense near infra-red laser radiation with gases is presented in this thesis. Specifically, soft x-ray generation through high order harmonic generation or exploiting intense inverse bremsstrahlung heating is examined. Most of these studies are conducted with femtosecond, terawatt class Cr:LiSrAlF{sub 6} (LiSAF) laser, though results derived from studies with other laser systems are presented as well. The majority of this work is devoted to experimental investigations, however, theoretical and computational models are developed to interpret the data. These studies are motivated by the possibility of utilizing the physics of intense laser/matter interactions as a potential compact source of bright x-rays. Consequently, the thrust of many of the experiments conducted is aimed at characterizing the x-rays produced for possible use in applications. In general, the studies of this manuscript fall into three categories. First, a unique 130 fs, 8 TW laser that is based on chirped pulse amplification, is described, and its performance is evaluated. The generation of x-rays through high order harmonics is then discussed with emphasis on characterizing and optimizing harmonic generation. Finally, the generation of strong, incoherent x-ray radiation by the intense irradiation of large (>1,000 atom) clusters in gas jets, is explored. The physics of laser energy absorption by clusters illuminated with intensities of 10{sup 15} to 10{sup 17} W/cm{sup 2} is considered in detail. X-ray spectroscopy of the hot plasmas that result from the irradiation of the clusters is conducted, and energy transport and kinetics issues in these plasmas are discussed.

  20. Phonon mediated electromagnetically induced absorption in hybrid opto-electro mechanical systems

    E-Print Network [OSTI]

    Kenan Qu; G. S. Agarwal

    2013-03-15T23:59:59.000Z

    We predict the existence of the electromagnetically induced absorption (EIA) in the double cavity configurations of the hybrid opto-electro mechanical systems (OEMS). We discuss the origin of the EIA in OEMS which exhibit the existence of an absorption peak within the transparency window. We provide analytical results for the width and the height of the EIA peak. The combination of the EIT and EIA is especially useful for photon switching applications. The EIA that we discuss is different from the one originally discovered by Lezama et al in atomic systems and can be understood in terms of the dynamics of three coupled oscillators (rather than two) under different conditions on the relaxation parameters. The EIA we report can also be realized in metamaterials and plasmonic structures.

  1. Dynamic polarizability of an atomic ion within a dense plasma

    SciTech Connect (OSTI)

    Basu, Joyee; Ray, Debasis [Department of Physics, Bengal Engineering and Science University, Shibpur, Howrah 711 103, West Bengal (India)

    2011-01-15T23:59:59.000Z

    We analyze the influence of plasma electron density on frequency-dependent linear field-response behavior of an atomic ion embedded in a dense plasma medium. The frequency-dependent atomic response, characterized by the dynamic dipole polarizability {alpha}{sub d}({omega}) as a function of the angular frequency {omega} of the time-dependent field, is estimated here up to the first pole of {alpha}{sub d}({omega}) on the {omega} axis (corresponding to the lowest resonance transition 1s{sup 2} {sup 1}S{yields}1s2p {sup 1}P) for the ground state 1s{sup 2} {sup 1}S of a two-electron atomic ion Ne{sup 8+} (Z = 10) at different plasma electron densities, as a typical example, employing the time-dependent coupled Hartree-Fock scheme within the framework of the ion-sphere model. It is observed that, owing to plasma density-induced enhancement of {alpha}{sub d}({omega}) at every {omega}, the pole position of {alpha}{sub d}({omega}) on the {omega} axis retracts toward the origin. This indicates a density-induced lowering (redshift) of the corresponding transition energy that conforms to experimentally observed trends. The polarizability calculation suggests a density-induced drop in the 1s{sup 2} {sup 1}S{yields}1s2p {sup 1}P absorption oscillator strength in the atomic ion within dense plasmas.

  2. Plasmon absorption modulator systems and methods

    SciTech Connect (OSTI)

    Kekatpure, Rohan Deodatta; Davids, Paul

    2014-07-15T23:59:59.000Z

    Plasmon absorption modulator systems and methods are disclosed. A plasmon absorption modulator system includes a semiconductor substrate, a plurality of quantum well layers stacked on a top surface of the semiconductor substrate, and a metal layer formed on a top surface of the stack of quantum well layers. A method for modulating plasmonic current includes enabling propagation of the plasmonic current along a metal layer, and applying a voltage across the stack of quantum well layers to cause absorption of a portion of energy of the plasmonic current by the stack of quantum well layers. A metamaterial switching system includes a semiconductor substrate, a plurality of quantum well layers stacked on a top surface of the semiconductor substrate, and at least one metamaterial structure formed on a top surface of the stack of quantum well layers.

  3. Absolute absorption spectroscopy based on molecule interferometry

    E-Print Network [OSTI]

    Stefan Nimmrichter; Klaus Hornberger; Hendrik Ulbricht; Markus Arndt

    2008-11-07T23:59:59.000Z

    We propose a new method to measure the absolute photon absorption cross section of neutral molecules in a molecular beam. It is independent of our knowledge of the particle beam density, nor does it rely on photo-induced fragmentation or ionization. The method is based on resolving the recoil resulting from photon absorption by means of near-field matter-wave interference, and it thus applies even to very dilute beams with low optical densities. Our discussion includes the possibility of internal state conversion as well as fluorescence. We assess the influence of various experimental uncertainties and show that the measurement of absolute absorption cross sections is conceivable with high precision and using existing technologies.

  4. On the local electronic and atomic structure of Ce{sub 1?x}Pr{sub x}O{sub 2??} epitaxial films on Si

    SciTech Connect (OSTI)

    Niu, Gang, E-mail: gang@ihp-microelectronics.com; Schubert, Markus Andreas; Zoellner, Marvin Hartwig [IHP, Im Technologiepark 25, 15236 Frankfurt (Oder) (Germany); D'Acapito, Francesco [Consiglio Nazionale delle Ricerche, Istituto Officina dei Materiali, Operative Group in Grenoble, c/o European Synchrotron Radiation Facility, B.P. 220, 38043 Grenoble (France); Schroeder, Thomas [IHP, Im Technologiepark 25, 15236 Frankfurt (Oder) (Germany); BTU Cottbus-Senftenberg, Konrad-Zuse-Str. 1, 03046 Cottbus (Germany); Boscherini, Federico [Consiglio Nazionale delle Ricerche, Istituto Officina dei Materiali, Operative Group in Grenoble, c/o European Synchrotron Radiation Facility, B.P. 220, 38043 Grenoble (France); Department of Physics and Astronomy, University of Bologna, via le C. Berti Pichat 6/2, 40127 Bologna (Italy)

    2014-09-28T23:59:59.000Z

    The local electronic and atomic structure of (111)-oriented, single crystalline mixed Ce{sub 1?x}Pr{sub x}O{sub 2??} (x?=?0, 0.1 and 0.6) epitaxial thin films on silicon substrates have been investigated in view of engineering redox properties of complex oxide films. Non-destructive X-ray absorption near edge structure reveals that Pr shows only +3 valence and Ce shows only nominal +4 valence in mixed oxides. Extended x-ray absorption fine structure (EXAFS) studies were performed at K edges of Ce and Pr using a specially designed monochromator system for high energy measurements. They demonstrate that the fluorite lattice of ceria (CeO{sub 2}) is almost not perturbed for x?=?0.1 sample, while higher Pr concentration (x?=?0.6) not only generates a higher disorder level (thus more disordered oxygen) but also causes a significant reduction of Ce–O interatomic distances. The valence states of the cations were also examined by techniques operating in highly reducing environments: scanning transmission electron microscopy-electron energy loss spectroscopy and X-ray photoemission spectroscopy; in these reducing environments, evidence for the presence of Ce{sup 3+} was clearly found for the higher Pr concentration. Thus, the introduction of Pr{sup 3+} into CeO{sub 2} strongly enhances the oxygen exchange properties of CeO{sub 2}. This improved oxygen mobility properties of CeO{sub 2} are attributed to the lattice disorder induced by Pr mixing in the CeO{sub 2} fluorite lattice, as demonstrated by EXAFS measurements. Thus, a comprehensive picture of the modifications of the atomic and electronic structure of Ce{sub 1?x}Pr{sub x}O{sub 2??} epitaxial films and their relation is obtained.

  5. Below gap optical absorption in GaAs driven by intense, single-cycle coherent transition radiation

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Goodfellow, J.; Fuchs, M.; Daranciang, D.; Ghimire, S.; Chen, F.; Loos, H.; Reis, D. A.; Fisher, A. S.; Lindenberg, A. M.

    2014-01-01T23:59:59.000Z

    Single-cycle terahertz fields generated by coherent transition radiation from a relativistic electron beam are used to study the high field optical response of single crystal GaAs. Large amplitude changes in the sub-band-gap optical absorption are induced and probed dynamically by measuring the absorption of a broad-band optical beam generated by transition radiation from the same electron bunch, providing an absolutely synchronized pump and probe geometry. This modification of the optical properties is consistent with strong-field-induced electroabsorption. These processes are pertinent to a wide range of nonlinear terahertz-driven light-matter interactions anticipated at accelerator-based sources.

  6. The 4000 A absorption system of formaldehyde

    E-Print Network [OSTI]

    Henderson, James Ralph

    1957-01-01T23:59:59.000Z

    THE $000 A ABSORPTION SYSTEM OF FORMALDEHYDE JAMES RALPH HENDERSON A Thesis Submitted to the Graduate School of the Agricultural and Mechanical College of Texas in partial fulfillment of the requirements for the degree of MASTER OF SCIENCE... May i 1957 Ma]or Subject: Physics THE 4000 A ABSORPTION SYSTEM OF FORMALDEHYDE A Thesis JAMES RALPH HENDERSON Approved as to style and content bye rlllan 0 OIllK e e ea o epar men May, l957 TABLE OF CONTENTS Page I. Introduction...

  7. Multi-plasmon absorption in graphene

    E-Print Network [OSTI]

    Marinko Jablan; Darrick E. Chang

    2015-01-21T23:59:59.000Z

    We show that graphene possesses a strong nonlinear optical response in the form of multi-plasmon absorption, with exciting implications in classical and quantum nonlinear optics. Specifically, we predict that graphene nano-ribbons can be used as saturable absorbers with low saturation intensity in the far-infrared and terahertz spectrum. Moreover, we predict that two-plasmon absorption and extreme localization of plasmon fields in graphene nano-disks can lead to a plasmon blockade effect, in which a single quantized plasmon strongly suppresses the possibility of exciting a second plasmon.

  8. Modified discrete random walk with absorption

    E-Print Network [OSTI]

    Theo van Uem

    2009-03-02T23:59:59.000Z

    We obtain expected number of arrivals, probability of arrival, absorption probabilities and expected time before absorption for a modified discrete random walk on the (sub)set of integers. In a [pqrs] random walk the particle can move one step forward or backward, stay for a moment in the same state or it can be absorbed immediately in the current state. M[pqrs] is a modified version, where probabilities on both sides of a multiple function barrier M are of different [pqrs] type.

  9. Anomalous Light Absorption by Small Particles

    E-Print Network [OSTI]

    Michael I. Tribelsky

    2009-12-18T23:59:59.000Z

    A new type of resonant light absorption by a small particle (nanocluster) is reported. The problem cannot be described within the commonly used dipole scattering approximation and should be studied with methods based upon the exact Mie solution. It is shown that the absorption cross-section has giant maxima realized at small values of the imaginary part of the complex dielectric permittivity of the particle. The maxima are situated in the vicinity of the plasmon (polariton) resonances and correspond to the regions where the dissipative damping equals the radiative one. The case is similar to the recently introduced anomalous scattering [PRL vol. 97, 263902 (2006)] and exhibits similar peculiarities.

  10. Laser isotope separation by multiple photon absorption

    DOE Patents [OSTI]

    Robinson, C. Paul (Los Alamos, NM); Rockwood, Stephen D. (Los Alamos, NM); Jensen, Reed J. (Los Alamos, NM); Lyman, John L. (Los Alamos, NM); Aldridge, III, Jack P. (Los Alamos, NM)

    1987-01-01T23:59:59.000Z

    Multiple photon absorption from an intense beam of infrared laser light may be used to induce selective chemical reactions in molecular species which result in isotope separation or enrichment. The molecular species must have a sufficient density of vibrational states in its vibrational manifold that, is the presence of sufficiently intense infrared laser light tuned to selectively excite only those molecules containing a particular isotope, multiple photon absorption can occur. By this technique, for example, intense CO.sub.2 laser light may be used to highly enrich .sup.34 S in natural SF.sub.6 and .sup.11 B in natural BCl.sub.3.

  11. Laser isotope separation by multiple photon absorption

    DOE Patents [OSTI]

    Robinson, C.P.; Rockwood, S.D.; Jensen, R.J.; Lyman, J.L.; Aldridge, J.P. III.

    1987-04-07T23:59:59.000Z

    Multiple photon absorption from an intense beam of infrared laser light may be used to induce selective chemical reactions in molecular species which result in isotope separation or enrichment. The molecular species must have a sufficient density of vibrational states in its vibrational manifold that, is the presence of sufficiently intense infrared laser light tuned to selectively excite only those molecules containing a particular isotope, multiple photon absorption can occur. By this technique, for example, intense CO[sub 2] laser light may be used to highly enrich [sup 34]S in natural SF[sub 6] and [sup 11]B in natural BCl[sub 3]. 8 figs.

  12. Towards simultaneous measurements of electronic and structural properties in ultra-fast x-ray free electron laser absorption spectroscopy experiments

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Gaudin, J.; Fourment, C.; Cho, B. I.; Engelhorn, K.; Galtier, E.; Harmand, M.; Leguay, P. M.; Lee, H. J.; Nagler, B.; Nakatsutsumi, M.; et al

    2014-04-17T23:59:59.000Z

    The rapidly growing ultrafast science with X-ray lasers unveils atomic scale processes with unprecedented time resolution bringing the so called “molecular movie” within reach. X-ray absorption spectroscopy is one of the most powerful x-ray techniques providing both local atomic order and electronic structure when coupled with ad-hoc theory. Collecting absorption spectra within few x-ray pulses is possible only in a dispersive setup. We demonstrate ultrafast time-resolved measurements of the LIII-edge x-ray absorption near-edge spectra of irreversibly laser excited Molybdenum using an average of only few x-ray pulses with a signal to noise ratio limited only by the saturation level ofmore »the detector. The simplicity of the experimental set-up makes this technique versatile and applicable for a wide range of pump-probe experiments, particularly in the case of non-reversible processes.« less

  13. Experimental protocol for high-fidelity heralded photon-to-atom quantum state transfer

    E-Print Network [OSTI]

    Christoph Kurz; Michael Schug; Pascal Eich; Jan Huwer; Philipp Müller; Jürgen Eschner

    2014-10-10T23:59:59.000Z

    A quantum network combines the benefits of quantum systems regarding secure information transmission and calculational speed-up by employing quantum coherence and entanglement to store, transmit, and process information. A promising platform for implementing such a network are atom-based quantum memories and processors, interconnected by photonic quantum channels. A crucial building block in this scenario is the conversion of quantum states between single photons and single atoms through controlled emission and absorption. Here we present an experimental protocol for photon-to-atom quantum state conversion, whereby the polarization state of an absorbed photon is mapped onto the spin state of a single absorbing atom with >95% fidelity, while successful conversion is heralded by a single emitted photon. Heralded high-fidelity conversion without affecting the converted state is a main experimental challenge, in order to make the transferred information reliably available for further operations. We record >80/s successful state transfer events out of 18,000/s repetitions.

  14. Bogoliubov theory and bosonic atoms

    E-Print Network [OSTI]

    Phan Thanh Nam

    2011-09-13T23:59:59.000Z

    We formulate the Bogoliubov variational principle in a mathematical framework similar to the generalized Hartree-Fock theory. Then we analyze the Bogoliubov theory for bosonic atoms in details. We discuss heuristically why the Bogoliubov energy should give the first correction to the leading energy of large bosonic atoms.

  15. Lyman- photometry: curve of growth determination, comparison to theoretical oscillator strength, and line absorption calculations at high temperature

    SciTech Connect (OSTI)

    Maki, R.G.; Michael, J.V.; Sutherland, J.W.

    1985-10-24T23:59:59.000Z

    Absolute concentrations of H atoms in the absorption region of an atomic resonance photometer have been accurately determined with a chemical kinetic technique that is based on the H + NO2 reaction. Subsequently, the curve of growth for the Lyman- transition (H(SP/sub 3/2,1/2/) reverse arrow H(SS/sub 1/2/)) has been determined with a resonance lamp that is essentially a microwave-driven electrodeless lamp plasma. Additional experiments have been performed in order to measure the temperature and (H) in the resonance lamp plasma. Thus, simplified theoretical calculations of the curve of growth could be made from first principles using no adjustable parameters. These calculations agreed with experiment within experimental error, and therefore, the theoretical oscillator strength, as calculated from the known wave functions for H, is experimentally confirmed for the H(SP/sub 3/2,1/2) reverse arrow H(SS/sub 1/2/) transition. Confidence can now be placed in line absorption calculations and, hence, in measurements of (H), at high absorber temperatures such as those encountered in flames, plasmas, and shock tubes where the atomic resonance absorption spectroscopic (aras) technique is commonly used. 25 references, 9 figures, 4 tables.

  16. In-situ control system for atomization

    DOE Patents [OSTI]

    Anderson, I.E.; Figliola, R.S.; Terpstra, R.L.

    1995-06-13T23:59:59.000Z

    Melt atomizing apparatus comprising a melt supply orifice for supplying the melt for atomization and gas supply orifices proximate the melt supply orifice for supplying atomizing gas to atomize the melt as an atomization spray is disclosed. The apparatus includes a sensor, such as an optical and/or audio sensor, for providing atomization spray data, and a control unit responsive to the sensed atomization spray data for controlling at least one of the atomizing gas pressure and an actuator to adjust the relative position of the gas supply orifice and melt supply in a manner to achieve a desired atomization spray. 3 figs.

  17. Spectral Emission of Moving Atom

    E-Print Network [OSTI]

    J. X. Zheng-Johansson

    2008-03-17T23:59:59.000Z

    A renewed analysis of the H.E. Ives and G.R. Stilwell's experiment on moving hydrogen canal rays (J. Opt. Soc. Am., 1938, v.28, 215) concludes that the spectral emission of a moving atom exhibits always a redshift which informs not the direction of the atom's motion. The conclusion is also evident from a simple energy relation: atomic spectral radiation is emitted as an orbiting electron consumes a portion of its internal energy on transiting to a lower-energy state which however has in a moving atom an additional energy gain; this results in a redshift in the emission frequency. Based on auxiliary experimental information and a scheme for de Broglie particle formation, we give a vigorous elucidation of the mechanism for deceleration radiation of atomic electron; the corresponding prediction of the redshift is in complete agreement with the Ives and Stilwell's experimental formula.

  18. Light Absorption by Secondary Organic Aerosol from ?-Pinene: Effects of Oxidants, Seed Aerosol Acidity, and Relative Humidity

    SciTech Connect (OSTI)

    Song, Chen; Gyawali, Madhu S.; Zaveri, Rahul A.; Shilling, John E.; Arnott, W. Patrick

    2013-10-25T23:59:59.000Z

    It is well known that light absorption from dust and black carbon aerosols has a warming effect on climate while light scattering from sulfate, nitrate, and sea salt aerosols has a cooling effect. However, there are large uncertainties associated with light absorption and scattering by different types of organic aerosols, especially in the near-UV and UV spectral regions. In this paper, we present the results from a systematic laboratory study focused on measuring light absorption by secondary organic aerosols (SOA) generated from ozonolysis or NO3 oxidation of ?-pinene in the presence of neutral and acidic sulfate seed aerosols. Light absorption was monitored using photoacoustic spectrometers at four different wavelengths: 355, 405, 532 and 870 nm. Light absorption at 355 and 405 nm was observed by SOA generated from oxidation of ?-pinene in the presence of acidic sulfate seed aerosols, under dry conditions. No absorption was observed when the relative humidity was elevated to greater than 27%, or in the presence of neutral sulfate seed aerosols. The light-absorbing compounds are speculated to be aldol condensation oligomers with organosulfate and organic nitrate groups. The results of this study also indicate that organic nitrates from ?-pinene SOA formed in the presence of neutral sulfate seed aerosols do not appear to absorb near-UV and UV radiation.

  19. Three- and four-nucleon absorption processes observed in the $K^-$-$^4$He reaction at rest

    E-Print Network [OSTI]

    T. Suzuki; H. Bhang; J. Chiba; S. Choi; Y. Fukuda; T. Hanaki; R. S. Hayano; M. Iio; T. Ishikawa; S. Ishimoto; T. Ishiwatari; K. Itahashi; M. Iwai; M. Iwasaki; P. Kienle; J. H. Kim; Y. Matsuda; H. Ohnishi; S. Okada; H. Outa; M. Sato; S. Suzuki; D. Tomono; E. Widmann; T. Yamazaki; H. Yim

    2010-09-26T23:59:59.000Z

    Correlations of back-to-back coincident $\\Lambda d$ and $\\Lambda t$ pairs from the stopped $K^-$ reaction on $^4$He had been investigated, thereby $\\Lambda d$ and $\\Lambda t$ branches of non-mesonic three- and four-nucleon absorption processes of antikaon at rest were identified as well-separable processes, respectively. The branching ratio of the three-nucleon process, ($^4$He-$K^-$)$_{atomic} \\rightarrow \\Lambda d "n"$, is estimated to be $(0.9 \\pm 0.1 (stat) \\pm 0.2 (syst)) \\times 10^{-3}$ from the normalized $\\Lambda d$ spectrum in a $\\Lambda d n$ final state, while the fraction of the four-nucleon process, ($^4$He-$K^-$)$_{atomic} \\rightarrow \\Lambda t$, is obtained to be $(3.1 \\pm 0.4 (stat) \\pm 0.5 (syst)) \\times 10^{-4}$ per stopped $K^-$.

  20. Supersonic coal water slurry fuel atomizer

    DOE Patents [OSTI]

    Becker, Frederick E. (Reading, MA); Smolensky, Leo A. (Concord, MA); Balsavich, John (Foxborough, MA)

    1991-01-01T23:59:59.000Z

    A supersonic coal water slurry atomizer utilizing supersonic gas velocities to atomize coal water slurry is provided wherein atomization occurs externally of the atomizer. The atomizer has a central tube defining a coal water slurry passageway surrounded by an annular sleeve defining an annular passageway for gas. A converging/diverging section is provided for accelerating gas in the annular passageway to supersonic velocities.

  1. Ab initio calculation of the electronic absorption spectrum of liquid water

    SciTech Connect (OSTI)

    Martiniano, Hugo F. M. C.; Galamba, Nuno [Grupo de Física Matemática da Universidade de Lisboa, Av. Professor Gama Pinto 2, 1649-003 Lisboa (Portugal)] [Grupo de Física Matemática da Universidade de Lisboa, Av. Professor Gama Pinto 2, 1649-003 Lisboa (Portugal); Cabral, Benedito J. Costa, E-mail: ben@cii.fc.ul.pt [Grupo de Física Matemática da Universidade de Lisboa, Av. Professor Gama Pinto 2, 1649-003 Lisboa (Portugal) [Grupo de Física Matemática da Universidade de Lisboa, Av. Professor Gama Pinto 2, 1649-003 Lisboa (Portugal); Departamento de Química e Bioquímica, Faculdade de Ciências, Universidade de Lisboa, 1749-016 Lisboa (Portugal); Instituto de Física da Universidade de São Paulo, CP 66318, 05314-970 São Paulo, SP (Brazil)

    2014-04-28T23:59:59.000Z

    The electronic absorption spectrum of liquid water was investigated by coupling a one-body energy decomposition scheme to configurations generated by classical and Born-Oppenheimer Molecular Dynamics (BOMD). A Frenkel exciton Hamiltonian formalism was adopted and the excitation energies in the liquid phase were calculated with the equation of motion coupled cluster with single and double excitations method. Molecular dynamics configurations were generated by different approaches. Classical MD were carried out with the TIP4P-Ew and AMOEBA force fields. The BLYP and BLYP-D3 exchange-correlation functionals were used in BOMD. Theoretical and experimental results for the electronic absorption spectrum of liquid water are in good agreement. Emphasis is placed on the relationship between the structure of liquid water predicted by the different models and the electronic absorption spectrum. The theoretical gas to liquid phase blue-shift of the peak positions of the electronic absorption spectrum is in good agreement with experiment. The overall shift is determined by a competition between the O–H stretching of the water monomer in liquid water that leads to a red-shift and polarization effects that induce a blue-shift. The results illustrate the importance of coupling many-body energy decomposition schemes to molecular dynamics configurations to carry out ab initio calculations of the electronic properties in liquid phase.

  2. Photoionization of the valence shells of the neutral tungsten atom

    E-Print Network [OSTI]

    Ballance, Connor P

    2015-01-01T23:59:59.000Z

    Results from large-scale theoretical cross section calculations for the total photoionization of the 4f, 5s, 5p and 6s orbitals of the neutral tungsten atom using the Dirac Coulomb R-matrix approximation (DARC: Dirac-Atomic R-matrix codes) are presented. Comparisons are made with previous theoretical methods and prior experimental measurements. In previous experiments a time-resolved dual laser approach was employed for the photo-absorption of metal vapours and photo-absorption measurements on tungsten in a solid, using synchrotron radiation. The lowest ground state level of neutral tungsten is $\\rm 5p^6 5d^4 6s^2 \\; {^5}D_{\\it J}$, with $\\it J$=0, and requires only a single dipole matrix for photoionization. To make a meaningful comparison with existing experimental measurements, we statistically average the large-scale theoretical PI cross sections from the levels associated with the ground state $\\rm 5p^6 5d^4 6s^2 \\; {^5}D_{\\it J}[{\\it J}=0,1,2,3,4]$ levels and the $\\rm 5d^56s \\; ^7S_3$ excited metastable...

  3. SUPPLY-SIDE OPTIMIZATION : MAXIMIZING ABSORPTIVE RATES

    E-Print Network [OSTI]

    Jumars, Pete

    and Piglet walked home thoughtfully together in the golden evening, and for a long time they were silent The World of Pooh INTRODUCTION The complexities of feeding behavior extend far beyond the simple priorities source of the material and energy for this escalation in heterotrophs with digestive tracts is absorption

  4. Absorption of solar radiation by solar neutrinos

    E-Print Network [OSTI]

    G. Duplancic; P. Minkowski; J. Trampetic

    2004-03-22T23:59:59.000Z

    We calculate the absorption probability of photons radiated from the surface of the Sun by a left-handed neutrino with definite mass and a typical momentum for which we choose |p_1|=0.2 MeV, producing a heavier right-handed antineutrino. Considering two transitions the \

  5. Corrosion inhibitor for aqueous ammonia absorption system

    DOE Patents [OSTI]

    Phillips, Benjamin A. (Benton Harbor, MI); Whitlow, Eugene P. (St. Joseph, MI)

    1998-09-22T23:59:59.000Z

    A method of inhibiting corrosion and the formation of hydrogen and thus improving absorption in an ammonia/water absorption refrigeration, air conditioning or heat pump system by maintaining the hydroxyl ion concentration of the aqueous ammonia working fluid within a selected range under anaerobic conditions at temperatures up to 425.degree. F. This hydroxyl ion concentration is maintained by introducing to the aqueous ammonia working fluid an inhibitor in an amount effective to produce a hydroxyl ion concentration corresponding to a normality of the inhibitor relative to the water content ranging from about 0.015 N to about 0.2 N at 25.degree. C. Also, working fluids for inhibiting the corrosion of carbon steel and resulting hydrogen formation and improving absorption in an ammonia/water absorption system under anaerobic conditions at up to 425.degree. F. The working fluids may be aqueous solutions of ammonia and a strong base or aqueous solutions of ammonia, a strong base, and a specified buffer.

  6. Corrosion inhibitor for aqueous ammonia absorption system

    DOE Patents [OSTI]

    Phillips, B.A.; Whitlow, E.P.

    1998-09-22T23:59:59.000Z

    A method is described for inhibiting corrosion and the formation of hydrogen and thus improving absorption in an ammonia/water absorption refrigeration, air conditioning or heat pump system by maintaining the hydroxyl ion concentration of the aqueous ammonia working fluid within a selected range under anaerobic conditions at temperatures up to 425 F. This hydroxyl ion concentration is maintained by introducing to the aqueous ammonia working fluid an inhibitor in an amount effective to produce a hydroxyl ion concentration corresponding to a normality of the inhibitor relative to the water content ranging from about 0.015 N to about 0.2 N at 25 C. Also, working fluids for inhibiting the corrosion of carbon steel and resulting hydrogen formation and improving absorption in an ammonia/water absorption system under anaerobic conditions at up to 425 F. The working fluids may be aqueous solutions of ammonia and a strong base or aqueous solutions of ammonia, a strong base, and a specified buffer. 5 figs.

  7. A high-flux BEC source for mobile atom interferometers

    E-Print Network [OSTI]

    Jan Rudolph; Waldemar Herr; Christoph Grzeschik; Tammo Sternke; Alexander Grote; Manuel Popp; Dennis Becker; Hauke Müntinga; Holger Ahlers; Achim Peters; Claus Lämmerzahl; Klaus Sengstock; Naceur Gaaloul; Wolfgang Ertmer; Ernst M. Rasel

    2015-06-16T23:59:59.000Z

    Quantum sensors based on coherent matter-waves are precise measurement devices whose ultimate accuracy is achieved with Bose-Einstein condensates (BEC) in extended free fall. This is ideally realized in microgravity environments such as drop towers, ballistic rockets and space platforms. However, the transition from lab-based BEC machines to robust and mobile sources with comparable performance is a challenging endeavor. Here we report on the realization of a miniaturized setup, generating a flux of $4 \\times 10^5$ quantum degenerate $^{87}$Rb atoms every 1.6$\\,$s. Ensembles of $1 \\times 10^5$ atoms can be produced at a 1$\\,$Hz rate. This is achieved by loading a cold atomic beam directly into a multi-layer atom chip that is designed for efficient transfer from laser-cooled to magnetically trapped clouds. The attained flux of degenerate atoms is on par with current lab-based BEC experiments while offering significantly higher repetition rates. Additionally, the flux is approaching those of current interferometers employing Raman-type velocity selection of laser-cooled atoms. The compact and robust design allows for mobile operation in a variety of demanding environments and paves the way for transportable high-precision quantum sensors.

  8. Mixed Rabi Jaynes-Cummings model of a three-level atom interacting with two quantized fields

    E-Print Network [OSTI]

    Boyan T. Torosov; Stefano Longhi; Giuseppe Della Valle

    2015-02-23T23:59:59.000Z

    The quantum Rabi model describes the ultrastrong interaction of a two-level atom coupled to a single quantized bosonic mode. As compared to the Jaynes-Cummings model, in the Rabi model the absorption and emission processes do not need to satisfy energy conservation and the usual rotating wave approximation (RWA) breaks down. As a result, the atom-field dynamics in the Hilbert space splits into two independent parity chains, exhibiting a collapse-revival pattern and exact periodic dynamics in the limit of degenerate atomic levels. Here we introduce a mixed Rabi Jaynes-Cummings model by considering a three-level atom interacting with two quantized bosonic fields, in which the RWA is made for one transition (with a weak atom-field coupling) but not for the other one (with an ultrastrong atom-field coupling). As a result, we show that the field in the weak coupled atomic transition can be used as a tool to control the atom-field dynamics of the other (strong coupled) transition, thus realizing an effective two-level quantum Rabi model with a controllable field. In particular, a periodic temporal dynamics of the atom-field state can be realized by appropriate tuning of the weak control field, even for non-degenerate atomic levels. A photonic simulator of the mixed Rabi Jaynes-Cummings model, based on light transport in evanescently-coupled optical waveguide lattices, is also briefly discussed.

  9. Generator-Absorber heat exchange transfer apparatus and method using an intermediate liquor

    DOE Patents [OSTI]

    Phillips, Benjamin A. (Benton Harbor, MI); Zawacki, Thomas S. (St. Joseph, MI)

    1996-11-05T23:59:59.000Z

    Numerous embodiments and related methods for generator-absorber heat exchange (GAX) are disclosed, particularly for absorption heat pump systems. Such embodiments and related methods use the working solution of the absorption system for the heat transfer medium where the working solution has an intermediate liquor concentration.

  10. Atomic cluster state build-up with macroscopic heralding

    SciTech Connect (OSTI)

    Metz, Jeremy; Schoen, Christian [Blackett Laboratory, Imperial College London, Prince Consort Road, London SW7 2BZ (United Kingdom); Beige, Almut [School of Physics and Astronomy, University of Leeds, Leeds LS2 9JT (United Kingdom)

    2007-11-15T23:59:59.000Z

    We describe a measurement-based state preparation scheme for the efficient build-up of cluster states in atom-cavity systems. As in a recent proposal for the generation of maximally entangled atom pairs [Metz et al., Phys. Rev. Lett. 97, 040503 (2006)], we use an electron shelving technique to avoid the necessity for the detection of single photons. Instead, the successful fusion of smaller into larger clusters is heralded by an easy-to-detect macroscopic fluorescence signal. High fidelities are achieved even in the vicinity of the bad cavity limit and are essentially independent of the concrete size of the system parameters.

  11. VOLUME 82, NUMBER 26 P HY S I CA L R E V I E W L E T T E R S 28 JUNE 1999 LaserDriven Atomic Pump

    E-Print Network [OSTI]

    , and by the wind force Fw caused by the reflection of conduction electrons from these atoms. Since F d usually, as schematically depicted in Fig. 1, by exerting on it the wind force Fw , due to the absorption of electron are driven by the direct force F d due to the external field that is locally modified at the atomic site

  12. VOLUME 82, NUMBER 26 P H Y S I C A L R E V I E W L E T T E R S 28 JUNE 1999 Laser-Driven Atomic Pump

    E-Print Network [OSTI]

    by the direct force Fd due to the external field that is locally modified at the atomic site, and by the wind in Fig. 1, by exerting on it the wind force Fw, due to the absorption of electron momenta. The direct force Fw caused by the reflection of conduction electrons from these atoms. Since Fd usually dominates

  13. Energetic neutral atoms as the explanation for the high velocity hydrogen around HD 209458b

    E-Print Network [OSTI]

    M. Holmström; A. Ekenbäck; F. Selsis; T. Penz; H. Lammer; P. Wurz

    2008-02-20T23:59:59.000Z

    Absorption in the stellar Lyman-$\\alpha$ (Ly-$\\alpha$) line observed during the transit of the extrasolar planet HD 209458b reveals high velocity atomic hydrogen at great distances from the planet. This has been interpreted as hydrogen atoms escaping from the exosphere of the planet, possibly undergoing hydrodynamic blow-off, being accelerated by stellar radiation pressure. However, around solar system planets the production of energetic neutral atoms from charge exchange between solar wind protons and neutral hydrogen from the exospheres has been observed, and should also occur at extrasolar planets. Here we show that the measured transit-associated Ly-$\\alpha$ absorption can be explained by the interaction between the exosphere of HD 209458b and the stellar wind, and that radiation pressure alone cannot explain the observation. This is the first observation of energetic neutral atoms outside the solar system. Since the stellar wind protons are the source of the observed energetic neutral atoms, this provides a completely new method of probing stellar wind conditions, and our model suggests a slow and hot stellar wind near HD 209458b at the time of the observation.

  14. Communication: Angular momentum alignment and fluorescence polarization of alkali atoms photodetached from helium nanodroplets

    SciTech Connect (OSTI)

    Hernando, Alberto; Beswick, J. Alberto; Halberstadt, Nadine [LCAR-IRSAMC, Université Toulouse 3 - Paul Sabatier and CNRS, 31062 Toulouse (France)] [LCAR-IRSAMC, Université Toulouse 3 - Paul Sabatier and CNRS, 31062 Toulouse (France)

    2013-12-14T23:59:59.000Z

    The theory of photofragments angular momentum polarization is applied to the photodetachment of an electronically excited alkali atom from a helium nanocluster (N = 200). The alignment of the electronic angular momentum of the bare excited alkali atoms produced is calculated quantum mechanically by solving the excited states coupled equations with potentials determined by density functional theory (DFT). Pronounced oscillations as a function of excitation energy are predicted for the case of Na@(He){sub 200}, in marked contrast with the absorption cross-section and angular distribution of the ejected atoms which are smooth functions of the energy. These oscillations are due to quantum interference between different coherently excited photodetachment pathways. Experimentally, these oscillations should be reflected in the fluorescence polarization and polarization-resolved photoelectron yield of the ejected atoms, which are proportional to the electronic angular momentum alignment. In addition, this result is much more general than the test case of NaHe{sub 200} studied here. It should be observable for larger droplets, for higher excited electronic states, and for other alkali as well as for alkali-earth atoms. Detection of these oscillations would show that the widely used pseudo-diatomic model can be valid beyond the prediction of absorption spectra and could help in interpreting parts of the dynamics, as already hinted by some experimental results on angular anisotropy of bare alkali fragments.

  15. Development of Updated ABsorption SIMulation Software (ABSIM)

    SciTech Connect (OSTI)

    Yang, Zhiyao [Purdue University, West Lafayette, IN; Tang, Xin [Purdue University, West Lafayette, IN; Qu, Ming [Purdue University, West Lafayette, IN; Abdelaziz, Omar [ORNL; Gluesenkamp, Kyle R [ORNL

    2014-01-01T23:59:59.000Z

    ABsorption SIMulation, ABSIM, was developed for the simulation of absorption systems by The Oak Ridge National Laboratory during 1980s and 1990s. ABSIM provides a platform for users to investigate various cycle configurations and working fluids, to calculate their operating parameters, to predict their performance, and to compare them with each other on a uniform basis. ABSIM is indeed a very useful and accurate tool for researchers to investigate various absorption systems. However, it has not been well maintained: it is incompatible with recent operating systems; the interface needs improved user-friendliness, and the system needs better parameter setting and debugging tools to help achieve convergence. Therefore, it is highly needed to update and improve ABSIM. The paper presents recent efforts to improve ABSIM s compatibility with current operating systems, user interface, and analysis capabilities. The paper details the features and functions of the newly updated ABSIM software. The new ABSIM still uses the previously validated calculation engine of the old ABSIM. The new graphic user interfaces (GUI) were developed in Qt, which is an open source license GUI software based on C++. XML was used as the database for data storage in the new ABSIM. The new ABSIM has been designed to be easily learned and used. It has enhanced editing and construction functions, plus enhanced analysis features including parametric tables, plotting, property plots, and master panels for debugging. A single effect water/LiBr absorption system is used as a case study in this paper to illustrate the features, capabilities, and functions of the new ABSIM. This case study was actually an example system available in the old ABSIM. The new version of ABSIM will be continuously developed to include additional subroutines for the components in liquid desiccant systems. The new ABSIM will be available to public for free. The ultimate goal of the new ABSIM is to allow it to become a simulation platform for both absorption heat pump and liquid desiccant systems.

  16. An Introduction to Multiphoton Ionization and Study of Ionization Rate of Hydrogen Atom

    SciTech Connect (OSTI)

    Shrestha, N.; Nakarmi, J. J.; Jha, L. N. [Central Department of Physics, Tribhuvan University, Kirtipur (Nepal)

    2009-04-19T23:59:59.000Z

    From a semiclassical point of view, we discuss the problem of nonlinear interaction between electromagnetic radiation and atoms. The time-dependent Schroedinger equation for single electron systems is solved using perturbative technique to obtain transition probability. We also discuss higher order perturbation used in multiple processes where two or more quanta are emitted instead of a single photon. The approach is based on the assumption that the perturbation is small. From the transition probability ionization rate and absorption, the cross-section of hydrogen atoms is calculated. Variation in photon energy and field strength is analyzed. Variation of cross-section with photon energy is discussed.

  17. Generation Planning (pbl/generation)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative1 First Use of Energy for All Purposes (Fuel and Nonfuel), 2002; Level: National5Sales for4,645U.S. DOEThe Bonneville Power AdministrationField8,Dist.Newof EnergyFundingGene ControlsCounselGeneral User Generation

  18. Measuring optical absorption coefficient of pure water in UV using the integrating cavity absorption meter. 

    E-Print Network [OSTI]

    Wang, Ling

    2008-10-10T23:59:59.000Z

    of the instrument is only several centimeters. The long effective total path length ensures a high sensitivity that enables the ICAM to measure liquid mediums with low absorption. Compared to the conventional transmission type of instruments that were used...

  19. Anticipating the atom: popular perceptions of atomic power before Hiroshima

    E-Print Network [OSTI]

    d'Emal, Jacques-Andre Christian

    1994-01-01T23:59:59.000Z

    Before Hiroshima made the Bomb an object of popular concern, possible implications and applications of atomic physics had been discussed in the public forum. The new science of X-rays and radium promised the possibilities of unlimited energy...

  20. Effect of Interatomic Separation on Entanglement Dynamics in a Two-Atom Two-Mode Model

    E-Print Network [OSTI]

    K. Sinha; N. I. Cummings; B. L. Hu

    2011-11-16T23:59:59.000Z

    We analyze the time evolution of quantum entanglement in a model consisting of two two-level atoms interacting with a two-mode electromagnetic field for a variety of initial states and interatomic separations. We study two specific atomic separations which give rise to symmetric atom-field couplings. For general atomic distances we consider a subset of initial states analytically, and then treat the more general situation numerically. We examine a variety of qualitative features such as entanglement sudden death, dynamical generation, protection, and transfer between subsystems. Our analysis shows a stark contrast in features of entanglement between the two special coupling schemes often considered; further, these features are uncharacteristic of those arising for general distances, due to the high degree of symmetry present in the special cases. The variety of behaviors in these two-mode cases suggest the importance of considering atomic separation carefully for any model where two atoms interact with a common field.

  1. Heterogeneous Catalysis on Atomically Dispersed Supported Metals...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Catalysis on Atomically Dispersed Supported Metals: CO2 Reduction on Multifunctional Pd Catalysts. Heterogeneous Catalysis on Atomically Dispersed Supported Metals: CO2 Reduction...

  2. Dynamics of production of iodine atoms by dissociation of iodides in a pulsed self-sustained discharge

    SciTech Connect (OSTI)

    Vagin, Nikolai P; Kochetov, Igor' V; Napartovich, A P; Yuryshev, Nikolai N

    2013-07-31T23:59:59.000Z

    Absorption at the laser transition has been used for the first time to assess the evolution of concentration of iodine atoms in a pulsed self-sustained discharge in mixtures of iodides with a buffer gas such as molecular nitrogen and helium. Dynamics of the iodine atom production is studied by the method of absorption spectroscopy. The dissociation of C{sub n}F{sub 2n+1}I and CnH{sub 2n+1}I (n = 1, 2) iodides is investigated. The energy required to produce atomic iodine is evaluated. The experimental data obtained for CF{sub 3}I are compared with the results of numerical simulations, their reasonable agreement being demonstrated. (active media)

  3. Influence of coherent Raman scattering on coherent population trapping in atomic sodium vapor

    SciTech Connect (OSTI)

    Wong, Vincent; Bennink, Ryan S.; Marino, Alberto M.; Boyd, Robert W.; Stroud, C.R. Jr.; Narducci, F.A. [Institute of Optics, University of Rochester, Rochester, New York 14627 (United States); EO Sensors Division, Naval Air Systems Command, Patuxent River, Maryland 20670 (United States)

    2004-11-01T23:59:59.000Z

    We study how coherent Stokes and anti-Stokes Raman scattering influence coherent population trapping. In an experiment using an atomic sodium vapor cell we observe induced transparency, induced absorption, and gain features, all of subnatural linewidth. The electromagnetically induced resonance is a peak or a dip depending on which side of the optical transition the fields are tuned to, and thus whether coherent anti-Stokes Raman scattering or coherent Stokes Raman scattering is the dominant process.

  4. The digestive adaptation of flying vertebrates: High intestinal paracellular absorption

    E-Print Network [OSTI]

    Mladenoff, David

    The digestive adaptation of flying vertebrates: High intestinal paracellular absorption compensates analysis. Significantly greater amplification of digestive surface area by villi in small birds, also in actively flying vertebrates. digestion gut morphometrics nutrient absorption paracellular uptake Birds have

  5. absorption cycle heat: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    drive compressor heat pump; (3) absorption heat pump; (4) high temperature heat powered compressor heat pump; (5) reverse absorption heat... Erickson, D. C. 1983-01-01 First Page...

  6. autonomous solar absorption: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    N; Teng, M; Cryan, M J 2012-01-01 4 WEATHER MODIFICATION BY CARBON DUST ABSORPTION OF SOLAR ENERGY Geosciences Websites Summary: WEATHER MODIFICATION BY CARBON DUST ABSORPTION...

  7. Infrared absorption spectra, radiative efficiencies, and global warming potentials

    E-Print Network [OSTI]

    Wirosoetisno, Djoko

    Infrared absorption spectra, radiative efficiencies, and global warming potentials absorption spectra, radiative efficiencies, and global warming potentials of perfluorocarbons: Comparison. (1995) and combined with atmospheric lifetimes from the literature to determine global warming

  8. absorption integrals measured: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    23 24 25 Next Page Last Page Topic Index 1 The development of an integrating cavity absorption meter to measure optical absorption of pure waters and suspended particulates Texas...

  9. CO2 Capture by Absorption with Potassium Carbonate

    E-Print Network [OSTI]

    Rochelle, Gary T.

    CO2 Capture by Absorption with Potassium Carbonate First Quarterly Report 2007 Quarterly Progress of this work is to improve the process for CO2 capture by alkanolamine absorption/stripping by developing

  10. CO2 Capture by Absorption with Potassium Carbonate

    E-Print Network [OSTI]

    Rochelle, Gary T.

    CO2 Capture by Absorption with Potassium Carbonate Fourth Quarterly Report 2006 Quarterly Progress of this work is to improve the process for CO2 capture by alkanolamine absorption/stripping by developing

  11. Imaging atoms in 3-D

    ScienceCinema (OSTI)

    Ercius, Peter

    2014-06-27T23:59:59.000Z

    Berkeley Lab's Peter Ercius discusses "Imaging atoms in 3-D" in this Oct. 28, 2013 talk, which is part of a Science at the Theater event entitled Eight Big Ideas

  12. Imaging atoms in 3-D

    SciTech Connect (OSTI)

    Ercius, Peter

    2013-10-31T23:59:59.000Z

    Berkeley Lab's Peter Ercius discusses "Imaging atoms in 3-D" in this Oct. 28, 2013 talk, which is part of a Science at the Theater event entitled Eight Big Ideas

  13. Topological Insulators and Metals in Atomic Optical Lattices

    E-Print Network [OSTI]

    Tudor D. Stanescu; Victor Galitski; J. Y. Vaishnav; Charles W. Clark; S. Das Sarma

    2009-01-26T23:59:59.000Z

    We propose the realization of topological quantum states with cold atoms trapped in an optical lattice. We discuss an experimental setup that generates a two-dimensional hexagonal lattice in the presence of a light-induced periodic vector potential, which represents a realization of the Haldane model with cold atoms. We determine theoretically the conditions necessary for observing the topological states and show that two of the key conditions are: 1) the realization of sharp boundaries and 2) the minimization of any smoothly varying component of the confining potential. We argue that, unlike their condensed matter counterparts, cold atom topological quantum states can be i) "seen", by mapping out the characteristic chiral edge states, and ii) controlled, by controlling the periodic vector potential and the properties of the confining potential.

  14. Cooling atom-cavity systems into entangled states

    E-Print Network [OSTI]

    J. Busch; S. De; S. S. Ivanov; B. T. Torosov; T. P. Spiller; A. Beige

    2011-05-25T23:59:59.000Z

    Generating entanglement by simply cooling a system into a stationary state which is highly entangled has many advantages. Schemes based on this idea are robust against parameter fluctuations, tolerate relatively large spontaneous decay rates, and achieve high fidelities independent of their initial state. A possible implementation of this idea in atom-cavity systems has recently been proposed by Kastoryano et al. [Phys. Rev. Lett. 106, 090502 (2011)]. Here we propose an improved entanglement cooling scheme for two atoms inside an optical cavity which achieves higher fidelities for comparable single-atom cooperativity parameters C. For example, we predict fidelities above 90% even for C as low as 20 without requiring individual laser addressing and without having to detect photons.

  15. Integrated vacuum absorption steam cycle gas separation

    DOE Patents [OSTI]

    Chen, Shiaguo (Champaign, IL); Lu, Yonggi (Urbana, IL); Rostam-Abadi, Massoud (Champaign, IL)

    2011-11-22T23:59:59.000Z

    Methods and systems for separating a targeted gas from a gas stream emitted from a power plant. The gas stream is brought into contact with an absorption solution to preferentially absorb the targeted gas to be separated from the gas stream so that an absorbed gas is present within the absorption solution. This provides a gas-rich solution, which is introduced into a stripper. Low pressure exhaust steam from a low pressure steam turbine of the power plant is injected into the stripper with the gas-rich solution. The absorbed gas from the gas-rich solution is stripped in the stripper using the injected low pressure steam to provide a gas stream containing the targeted gas. The stripper is at or near vacuum. Water vapor in a gas stream from the stripper is condensed in a condenser operating at a pressure lower than the stripper to concentrate the targeted gas. Condensed water is separated from the concentrated targeted gas.

  16. Recent Progress in ultracold atoms

    E-Print Network [OSTI]

    Baltisberger, Jay H.

    , cold gas experiments 2. How to make a BEC out of fermions 3. Recent Progress: Controlling Interaction (Feshbach Resonance) 4. From BCS to BEC: Rotating trap and spin- polarized condensates. 5. Future research and Einstein What is Bose-Einstein condensation (BEC)? #12;300 K to 1 mK 109 atoms 1 mK to 1 mK 108 106 atoms

  17. DEVELOPMENT OF SOLAR DRIVEN ABSORPTION AIR CONDITIONERS AND HEAT PUMPS

    E-Print Network [OSTI]

    Dao, K.

    2013-01-01T23:59:59.000Z

    ROAD BERKELEY, CALIFORNIA OBJECTIVE AND APPROACH The objective of this project is the development of absorption refrigeration systems for solar

  18. Absorptive Recycle of Distillation Waste Heat

    E-Print Network [OSTI]

    Erickson, D. C.; Lutz, E. J., Jr.

    1982-01-01T23:59:59.000Z

    ABSORPTIVE RECYCLE OF DISTILLATION WASTE HEAT Donald C. Erickson and Edward J. Lutz Jr. Energy Concepts Company Annapolis, Maryland ABSTRACT When the heat source available to a distillation process is at a significantly higher temperature... which conserve 60 to 70%. Also, there are ver sions which incorporate separate low tem perature waste heat streams and thereby conserve over 90% of the required dis tillation energy. The main limitations of the R/AHP are the need for sufficient...

  19. Intensity dependence narrowing of electromagnetically induced absorption in a Doppler-broadened medium

    SciTech Connect (OSTI)

    Dimitrijevic, J.; Arsenovic, D.; Jelenkovic, B. M. [Institute of Physics, 11080 Belgrade (Serbia)

    2007-07-15T23:59:59.000Z

    In this paper, we present a theoretical model for studying the interaction between linearly polarized laser light and near-degenerated Zeeman sublevels for a multiple V-type atomic system of {sup 2}S{sub 1/2}F{sub g}=2{yields}{sup 2}P{sub 3/2}F{sub e}=3 transition in {sup 87}Rb. We have calculated the laser absorption in a Hanle configuration, as well as the amplitudes and the widths of electromagnetically induced absorption (EIA) in the range of laser intensities from 0.01 to 40 mW/cm{sup 2}. Our results, showing nonvanishing EIA amplitude, a nonmonotonic increase of the EIA width for the increase of laser intensity, and pronounced shape differences of the Hanle EIA curves at different laser intensities, are in good agreement with recent experimental results. We have found that the EIA behaves differently than the electromagnetically induced transparency (EIT) as a function of the laser intensity. Both the amplitude and width of the EIA have narrow maximums at 1 to 2 mW/cm{sup 2}. We have shown the strong influence of Doppler broadening of atomic transition on Hanle resonances and have suggested the explanation of it.

  20. The Nature of Interstellar Gas toward the Pleiades Revealed in Absorption Lines

    E-Print Network [OSTI]

    A. M. Ritchey; M. Martinez; K. Pan; S. R. Federman; D. L. Lambert

    2006-06-27T23:59:59.000Z

    We present high-resolution, high signal to noise absorption-line observations of CN, Ca II, Ca I, CH^+, and CH along twenty lines of sight toward members of the Pleiades. The acquired data enable the most detailed study to date of the interaction between cluster stars and the surrounding interstellar gas. Total equivalent widths are consistent with previous investigations except where weaker features are detected owing to our greater sensitivity. Mean b-values for the molecular species indicate that toward most of the Pleiades CH is associated with the production of CH^+ rather than CN. An analysis of radial velocities reveals a kinematic distinction between ionized atomic gas and molecular and neutral gas. Molecular components are found with velocities in the local standard of rest of either ~ +7 km s^-1 or ~ +9.5 km s^-1, with the higher-velocity components associated with the strongest absorption. Atomic gas traced by Ca II shows a strong central component at v_LSR ~ +7 km s^-1 exhibiting velocity gradients indicative of cloud-cluster interactions. Gas density estimates derived from measured CH/CH^+ column density ratios show good agreement with those inferred from H_2 rotational populations, yielding typical values of n ~ 50 cm^-3. Our models do not include the important time-dependent effects on CH^+ formation which may ultimately be needed to extract physical conditions in these clouds.

  1. Split-flow regeneration in absorptive air separation

    DOE Patents [OSTI]

    Weimer, Robert F. (Allentown, PA)

    1987-01-01T23:59:59.000Z

    A chemical absorptive separation of air in multiple stage of absorption and desorption is performed with partial recycle of absorbent between stages of desorption necessary to match equilibrium conditions in the various stages of absorption. This allows reduced absorbent flow, reduced energy demand and reduced capital costs.

  2. Split-flow regeneration in absorptive air separation

    DOE Patents [OSTI]

    Weimer, R.F.

    1987-11-24T23:59:59.000Z

    A chemical absorptive separation of air in multiple stage of absorption and desorption is performed with partial recycle of absorbent between stages of desorption necessary to match equilibrium conditions in the various stages of absorption. This allows reduced absorbent flow, reduced energy demand and reduced capital costs. 4 figs.

  3. Chukwuemeka I. Okoye Carbon Dioxide Solubility and Absorption Rate in

    E-Print Network [OSTI]

    Rochelle, Gary T.

    Copyright by Chukwuemeka I. Okoye 2005 #12;Carbon Dioxide Solubility and Absorption Rate _______________________ Nicholas A. Peppas #12;Carbon Dioxide Solubility and Absorption Rate in Monoethanolamine/Piperazine/H2O for. #12;iii Carbon Dioxide Solubility and Absorption Rate in Monoethanolamine/Piperazine/H2O

  4. On the Absorption and Emission Properties of Interstellar Grains

    E-Print Network [OSTI]

    Aigen Li

    2005-03-25T23:59:59.000Z

    Our current understanding of the absorption and emission properties of interstellar grains are reviewed. The constraints placed by the Kramers-Kronig relation on the wavelength-dependence and the maximum allowable quantity of the dust absorption are discussed. Comparisons of the opacities (mass absorption coefficients) derived from interstellar dust models with those directly estimated from observations are presented.

  5. CO2 Capture by Absorption with Potassium Carbonate

    E-Print Network [OSTI]

    Rochelle, Gary T.

    CO2 Capture by Absorption with Potassium Carbonate Third Quarterly Report 2005 Quarterly Progress absorption/stripping by developing an alternative solvent, aqueous K2CO3 promoted by piperazine. Modeling.................................................................................................................................. 11 Task 1 ­ Modeling Performance of Absorption/Stripping of CO2 with Aqueous K2CO3 Promoted

  6. CO2 Capture by Absorption with Potassium Carbonate

    E-Print Network [OSTI]

    Rochelle, Gary T.

    CO2 Capture by Absorption with Potassium Carbonate First Quarterly Report 2006 Quarterly Progress the process for CO2 capture by alkanolamine absorption/stripping by developing an alternative solvent, aqueous.................................................................................................................................... 8 Task 1 ­ Modeling Performance of Absorption/Stripping of CO2 with Aqueous K2CO3 Promoted

  7. CO2 Capture by Absorption with Potassium Carbonate

    E-Print Network [OSTI]

    Rochelle, Gary T.

    CO2 Capture by Absorption with Potassium Carbonate Third Quarterly Report 2006 Quarterly Progress of this work is to improve the process for CO2 capture by alkanolamine absorption/stripping by developing...................................................................................................................................11 Task 1 ­ Modeling Performance of Absorption/Stripping of CO2 with Aqueous K2CO3 Promoted

  8. CO2 Capture by Absorption with Potassium Carbonate

    E-Print Network [OSTI]

    Rochelle, Gary T.

    CO2 Capture by Absorption with Potassium Carbonate Second Quarterly Report 2006 Quarterly Progress of this work is to improve the process for CO2 capture by alkanolamine absorption/stripping by developing.................................................................................................................................. 10 Task 1 ­ Modeling Performance of Absorption/Stripping of CO2 with Aqueous K2CO3 Promoted

  9. Application of Quantitative Fluorescence and Absorption-Edge

    E-Print Network [OSTI]

    Sparks, Donald L.

    Application of Quantitative Fluorescence and Absorption-Edge Computed Microtomography to Image, Chicago, Illinois 60637 This paper shows that synchrotron-based fluorescence and absorption-edge computed, which had a well-correlated metal coating. Absorption-edge CMT showed the three-dimensional distribution

  10. The role of solar absorption in climate and climate change

    E-Print Network [OSTI]

    1 The role of solar absorption in climate and climate change William Collins UC Berkeley Research Boulder, Colorado, USA #12;2 Prior Research on Absorption and Climate Field Experiments: · Central · Climate with enhanced cloud absorption Synthesis of models and aerosol observations: · Development

  11. CO2 Capture by Absorption with Potassium Carbonate

    E-Print Network [OSTI]

    Rochelle, Gary T.

    CO2 Capture by Absorption with Potassium Carbonate Fourth Quarterly Report 2005 Quarterly Progress absorption/stripping by developing an alternative solvent, aqueous K2CO3 promoted by piperazine. In Campaign.................................................................................................................................... 9 Task 1 ­ Modeling Performance of Absorption/Stripping of CO2 with Aqueous K2CO3 Promoted

  12. Absorption of Carbon Dioxide in Aqueous Piperazine/Methyldiethanolamine

    E-Print Network [OSTI]

    Rochelle, Gary T.

    Absorption of Carbon Dioxide in Aqueous Piperazine/Methyldiethanolamine Sanjay Bishnoi and Gary T dioxide absorption in 0.6 M piperazine PZ r4 M methyldiethanolamine ( )MDEA was measured in a wetted wall loading. The absorption rate did not follow pseudo first-order beha®ior except at ®ery low loading. All

  13. Absorption of solar radiation by the cloudy atmosphere: Further interpretations of collocated aircraft measurements

    E-Print Network [OSTI]

    1999-01-01T23:59:59.000Z

    J. Vitko Jr. , Absorption of solar radiation by the cloudyet al. , Absorption of solar radiation by clouds: Observa-1999 Absorption of solar radiation by the cloudy atmosphere:

  14. ISO-LWS observations of C+ and O lines in absorption toward SgrB2

    E-Print Network [OSTI]

    Charlotte Vastel; Edward Polehampton; Jean-Paul Baluteau; Bruce Swinyard; Emmanuel Caux; Pierre Cox

    2002-08-09T23:59:59.000Z

    High spectral resolution ISO-LWS observations of the [OI] 63.2 and 145.5 microns and [CII] 157.7 microns fine structure lines are presented for the center of the Sagittarius B2 complex (SgrB2). Both the [OI] 63.2 microns and the [CII] 157.7 microns lines are detected in absorption. Using observations of the CO isotopes and of the HI lines, absorption components can be associated with many clouds along the Sgr B2 line of sight. From these data, we were able to disentangle three different layers, as predicted by PDR models, which contain atomic oxygen. We derive lower limits for the column densities of C and O. The fact that the [CII] 157.7 microns line is detected in absorption implies that the main cooling line of the interstellar medium can be optically thick especially in the direction of large star-forming complexes or in the nuclei of galaxies. This could partially account for the deficiency in the [CII] 157.7 microns line which has been recently found toward infrared bright galaxies in ISO data.

  15. Improvement of the Performance for an Absorption Refrigeration System with Lithium bromide-water as Refrigerant by Increasing Absorption Pressure

    E-Print Network [OSTI]

    Xie, G.; Sheng, G.; Li, G.; Pan, S.

    2006-01-01T23:59:59.000Z

    ICEBO2006, Shenzhen, China HVAC Technologies for Energy Efficiency, Vol. IV-10-4 Improvement of the Performance for an Absorption Refrigerating System with Lithium bromide-water as Refrigerant by Increasing Absorption... in order to lay a theoretical foundation of improving the performance of whole LBAC. 2. THE PRINCIPLE OF ENHANCING ABSORPTION EFFICIENCY OF THE ABSORBER It is well known that the absorption of ICEBO2006, Shenzhen, China HVAC...

  16. Asymmetric perfectly matched layer for the absorption of waves

    SciTech Connect (OSTI)

    Vay, Jean-Luc

    2002-02-10T23:59:59.000Z

    The Perfectly Matched Layer (PML) has become a standard for comparison in the techniques that have been developed to close the system of Maxwell equations (more generally wave equations) when simulating an open system. The original Berenger PML formulation relies on a split version of Maxwell equations with numerical electric and magnetic conductivities. They present here an extension of this formulation which introduces counterparts of the electric and magnetic conductivities affecting the term which is spatially differentiated in the equations. they phase velocity along each direction is also multiplied by an additional coefficient. They show that, under certain constraints on the additional numerical coefficients, this ''medium'' does not generate any reflection at any angle and any frequency and is then a Perfectly Matched Layer. Technically it is a super-set of Berenger's PML to which it reduces for a specific set of parameters and like it, it is anisotropic. However, unlike the PML, it introduces some asymmetry in the absorption rate and is therefore labeled an APML for Asymmetric Perfectly Matched Layer. They present here the numerical considerations that have led them to introduce such a medium as well as its theory. Several finite-different numerical implementations are derived (in one, two and three dimensions) and the performance of the APML is contrasted with that of the PML in one and two dimensions. Using plane wave analysis, they show that the APML implementations lead to higher absorption rates than the considered PML implementations. Although they have considered in this paper the finite-different discretization of Maxwell-like equations only, the APML system of equations may be used with other discretization schemes, such as finite-elements, and may be applied to other equations, for applications beyond electromagnetics.

  17. Light-induced gauge fields for ultracold atoms

    E-Print Network [OSTI]

    N. Goldman; G. Juzeliunas; P. Ohberg; I. B. Spielman

    2014-12-12T23:59:59.000Z

    Gauge fields are central in our modern understanding of physics at all scales. At the highest energy scales known, the microscopic universe is governed by particles interacting with each other through the exchange of gauge bosons. At the largest length scales, our universe is ruled by gravity, whose gauge structure suggests the existence of a particle - the graviton - that mediates the gravitational force. At the mesoscopic scale, solid-state systems are subjected to gauge fields of different nature: materials can be immersed in external electromagnetic fields, but they can also feature emerging gauge fields in their low-energy description. In this review, we focus on another kind of gauge field: those engineered in systems of ultracold neutral atoms. In these setups, atoms are suitably coupled to laser fields that generate effective gauge potentials in their description. Neutral atoms "feeling" laser-induced gauge potentials can potentially mimic the behavior of an electron gas subjected to a magnetic field, but also, the interaction of elementary particles with non-Abelian gauge fields. Here, we review different realized and proposed techniques for creating gauge potentials - both Abelian and non-Abelian - in atomic systems and discuss their implication in the context of quantum simulation. While most of these setups concern the realization of background and classical gauge potentials, we conclude with more exotic proposals where these synthetic fields might be made dynamical, in view of simulating interacting gauge theories with cold atoms.

  18. A high-flux BEC source for mobile atom interferometers

    E-Print Network [OSTI]

    Jan Rudolph; Waldemar Herr; Christoph Grzeschik; Tammo Sternke; Alexander Grote; Manuel Popp; Dennis Becker; Hauke Müntinga; Holger Ahlers; Achim Peters; Claus Lämmerzahl; Klaus Sengstock; Naceur Gaaloul; Wolfgang Ertmer; Ernst M. Rasel

    2015-01-02T23:59:59.000Z

    Quantum sensors based on coherent matter-waves are precise measurement devices whose ultimate accuracy is achieved with Bose-Einstein condensates (BEC) in extended free fall. This is ideally realized in microgravity environments such as drop towers, ballistic rockets and space platforms. However, the transition from lab-based BEC machines to robust and mobile sources with comparable performance is a technological challenge. Here we report on the realization of a miniaturized setup, generating a flux of $4 \\times 10^5$ quantum degenerate $^{87}$Rb atoms every 1.6 s. Ensembles of $1 \\times 10^5$ atoms can be produced at a 1 Hz rate. This is achieved by loading a cold atomic beam directly into a multi-layer atom chip that is designed for efficient transfer from laser-cooled to magnetically trapped clouds. The attained flux of degenerate atoms is on par with current lab-based experiments while offering significantly higher repetition rates. The compact and robust design allows for mobile operation in a variety of demanding environments and paves the way for portable high-precision quantum sensors.

  19. A high-flux BEC source for mobile atom interferometers

    E-Print Network [OSTI]

    Rudolph, Jan; Grzeschik, Christoph; Sternke, Tammo; Grote, Alexander; Popp, Manuel; Becker, Dennis; Müntinga, Hauke; Ahlers, Holger; Peters, Achim; Lämmerzahl, Claus; Sengstock, Klaus; Gaaloul, Naceur; Ertmer, Wolfgang; Rasel, Ernst M

    2015-01-01T23:59:59.000Z

    Quantum sensors based on coherent matter-waves are precise measurement devices whose ultimate accuracy is achieved with Bose-Einstein condensates (BEC) in extended free fall. This is ideally realized in microgravity environments such as drop towers, ballistic rockets and space platforms. However, the transition from lab-based BEC machines to robust and mobile sources with comparable performance is a technological challenge. Here we report on the realization of a miniaturized setup, generating a flux of $4 \\times 10^5$ quantum degenerate $^{87}$Rb atoms every 1.6 s. Ensembles of $1 \\times 10^5$ atoms can be produced at a 1 Hz rate. This is achieved by loading a cold atomic beam directly into a multi-layer atom chip that is designed for efficient transfer from laser-cooled to magnetically trapped clouds. The attained flux of degenerate atoms is on par with current lab-based experiments while offering significantly higher repetition rates. The compact and robust design allows for mobile operation in a variety of...

  20. HRTEM Imaging of Atoms at Sub-Angstrom Resolution

    SciTech Connect (OSTI)

    O'Keefe, Michael A.; Allard, Lawrence F.; Blom, Douglas A.

    2005-04-06T23:59:59.000Z

    John Cowley and his group at Arizona State University pioneered the use of transmission electron microscopy (TEM) for high-resolution imaging. Images were achieved three decades ago showing the crystal unit cell content at better than 4 Angstrom resolution. This achievement enabled researchers to pinpoint the positions of heavy atom columns within the unit cell. Lighter atoms appear as resolution is improved to sub-Angstrom levels. Currently, advanced microscopes can image the columns of the light atoms (carbon, oxygen, nitrogen) that are present in many complex structures, and even the lithium atoms present in some battery materials. Sub-Angstrom imaging, initially achieved by focal-series reconstruction of the specimen exit surface wave, will become common place for next-generation electron microscopes with CS-corrected lenses and monochromated electron beams. Resolution can be quantified in terms of peak separation and inter-peak minimum, but the limits imposed on the attainable resolution by the properties of the micro-scope specimen need to be considered. At extreme resolution the ''size'' of atoms can mean that they will not be resolved even when spaced farther apart than the resolution of the microscope.

  1. Accelerometer using atomic waves for space applications

    E-Print Network [OSTI]

    of Bose-Einstein condensation (BEC) of a dilute gas of trapped atoms in a single quantum state [18, 19, 20 of such devices in the field of navigation, surveying and analysis of earth structures. Matter-wave interferometry that the use of Bose-Einstein condensed atoms will bring the science of atom optics, and in particular atom

  2. Atomic Cascade in Muonic and Hadronic Hydrogen Atoms

    E-Print Network [OSTI]

    T. S. Jensen; V. P. Popov; V. N. Pomerantsev

    2007-12-18T23:59:59.000Z

    The atomic cascade in $\\mu^- p$ and $\\pi^- p$ atoms has been studied with the improved version of the extended cascade model in which new quantum mechanical calculations of the differential and integral cross sections of the elastic scattering, Stark transitions and Coulomb de-excitation have been included for the principal quantum number values $n\\le 8$ and the relative energies $E \\ge 0.01$ eV. The $X$-ray yields and kinetic energy distributions are compared with the experimental data.

  3. Quantum Electrodynamics of Atomic Resonances

    E-Print Network [OSTI]

    Miguel Ballesteros; Jérémy Faupin; Jürg Fröhlich; Baptiste Schubnel

    2015-03-09T23:59:59.000Z

    A simple model of an atom interacting with the quantized electromagnetic field is studied. The atom has a finite mass $m$, finitely many excited states and an electric dipole moment, $\\vec{d}_0 = -\\lambda_{0} \\vec{d}$, where $\\| d^{i}\\| = 1,$ $ i=1,2,3,$ and $\\lambda_0$ is proportional to the elementary electric charge. The interaction of the atom with the radiation field is described with the help of the Ritz Hamiltonian, $-\\vec{d}_0\\cdot \\vec{E}$, where $\\vec{E}$ is the electric field, cut off at large frequencies. A mathematical study of the Lamb shift, the decay channels and the life times of the excited states of the atom is presented. It is rigorously proven that these quantities are analytic functions of the momentum $\\vec{p}$ of the atom and of the coupling constant $\\lambda_0$, provided $|\\vec{p}| < mc$ and $| \\Im\\vec{p} |$ and $| \\lambda_{0} |$ are sufficiently small. The proof relies on a somewhat novel inductive construction involving a sequence of `smooth Feshbach-Schur maps' applied to a complex dilatation of the original Hamiltonian, which yields an algorithm for the calculation of resonance energies that converges super-exponentially fast.

  4. Electromagnetic scattering and absorption by aerosol agglomerates

    SciTech Connect (OSTI)

    Chen, Hsingyi.

    1989-01-01T23:59:59.000Z

    Calculation of scattering and absorption by smoke aerosols is required in many applications, including characterization of atmospheric aerosols, prediction of climatic impact of smoke, evaluation of smoke effectiveness in obscuration, calculation of heat transfer from flames, and evaluation of various scenarios of nuclear winter. In this dissertation two procedures were developed to accurately make these calculations utilizing realistic models of smoke agglomerates including oriented chains and fractal geometries. First the Iterative Extended Boundary Condition Method (IEBCM) was utilized to calculate the electromagnetic (EM) scattering and absorption of elongated aerosol particles. The computation efficiency and capability of IEBCM were improved by implementing the sectioning and the segmentation procedures. The sectioning procedure resulted in improving the computational efficiency and the segmentation method made it possible to make calculations for particles with aspect ratios as high as 250. The other procedure employed the Volume Integral Equation Formulation (VIEF) to compute the EM scattering and absorption by agglomerates of complex geometries. The validity of the procedure was checked first by comparing the obtained results with those obtained from the Mie solution for a spherical object and with the IEBCM for nonspherical objects. The comparison between results showed excellent agreement and hence validated the accuracy of the VIEF. The VIEF solution was then used to make calculations for five types of fractal agglomerates of smoke aerosol particles with fractal dimensions in the range from 1.7 to 1.9. The results obtained were compared with those based on the fractal theory recently published by Berry and Percival, and some differences were observed.

  5. Degeneracy Breaking of Hydrogen Atom

    E-Print Network [OSTI]

    Agung Trisetyarso; Pantur Silaban

    2014-11-21T23:59:59.000Z

    The three dimensional rotation group, SO(3), is a symmetry group of the normal hydrogen atom. Each reducible representation of this group can be associated with a degenerate energy level. If this atom is placed in an external magnetic field, the interaction between the orbital magnetic moment with this field will lead to a symmetry breaking where the symmetry group of the atom is a new group distinct from the SO(3) group. This phenomenon describes the normal Zeeman effect, where a degenerate energy level splits into several new energy levels. It is explicitly shown that each of the new energy levels can be associated with an irreducible representation of the new symmetry group.

  6. Atomizing, continuous, water monitoring module

    DOE Patents [OSTI]

    Thompson, Cyril V. (Knoxville, TN); Wise, Marcus B. (Kingston, TN)

    1997-01-01T23:59:59.000Z

    A system for continuously analyzing volatile constituents of a liquid is described. The system contains a pump for continuously pumping the liquid to be tested at a predetermined flow rate into an extracting container through a liquid directing tube having an orifice at one end and positioned to direct the liquid into the extracting container at a flow rate sufficient to atomize the liquid within the extracting container. A continuous supply of helium carrier gas at a predetermined flow rate is directed through a tube into the extracting container and co-mingled with the atomized liquid to extract the volatile constituents contained within the atomized liquid. The helium containing the extracted volatile constituents flows out of the extracting container into a mass spectrometer for an analysis of the volatile constituents of the liquid.

  7. Atomizing, continuous, water monitoring module

    DOE Patents [OSTI]

    Thompson, C.V.; Wise, M.B.

    1997-07-08T23:59:59.000Z

    A system for continuously analyzing volatile constituents of a liquid is described. The system contains a pump for continuously pumping the liquid to be tested at a predetermined flow rate into an extracting container through a liquid directing tube having an orifice at one end and positioned to direct the liquid into the extracting container at a flow rate sufficient to atomize the liquid within the extracting container. A continuous supply of helium carrier gas at a predetermined flow rate is directed through a tube into the extracting container and co-mingled with the atomized liquid to extract the volatile constituents contained within the atomized liquid. The helium containing the extracted volatile constituents flows out of the extracting container into a mass spectrometer for an analysis of the volatile constituents of the liquid. 3 figs.

  8. Cross section for charmonium absorption by nucleons

    E-Print Network [OSTI]

    Liu, W.; Ko, Che Ming; Lin, ZW.

    2002-01-01T23:59:59.000Z

    July 2001; publishe The cross section for J/c absorption by nucleons is with empirical particle masses, which has been used previousl by pion and r meson. Including both two-body and three-bod of 1 GeV at interaction vertices involving charm hadrons... and is consistent with that extracted from J/c productio DOI: 10.1103/PhysRevC.65.015203 PAC I. INTRODUCTION Two main mechanisms for J/c suppression observed in relativistic heavy ion collisions @1# are the dissociation by the quark-gluon plasma @2...

  9. Distributed Bragg Reflectors With Reduced Optical Absorption

    DOE Patents [OSTI]

    Klem, John F. (Albuquerque, NM)

    2005-08-16T23:59:59.000Z

    A new class of distributed Bragg reflectors has been developed. These distributed Bragg reflectors comprise interlayers positioned between sets of high-index and low-index quarter-wave plates. The presence of these interlayers is to reduce photon absorption resulting from spatially indirect photon-assisted electronic transitions between the high-index and low-index quarter wave plates. The distributed Bragg reflectors have applications for use in vertical-cavity surface-emitting lasers for use at 1.55 .mu.m and at other wavelengths of interest.

  10. Absorption of the $?$ and $?$ Mesons in Nuclei

    E-Print Network [OSTI]

    M. H. Wood; R. Nasseripour; M. Paolone; C. Djalali; D. P. Weygand; the CLAS Collaboration

    2010-06-17T23:59:59.000Z

    Due to their long lifetimes, the $\\omega$ and $\\phi$ mesons are the ideal candidates for the study of possible modifications of the in-medium meson-nucleon interaction through their absorption inside the nucleus. During the E01-112 experiment at the Thomas Jefferson National Accelerator Facility, the mesons were photoproduced from $^{2}$H, C, Ti, Fe, and Pb targets. This paper reports the first measurement of the ratio of nuclear transparencies for the $e^{+}e^{-}$ channel. The ratios indicate larger in-medium widths compared with what have been reported in other reaction channels.

  11. Absorption Heat Pump Basics | Department of Energy

    Broader source: Energy.gov (indexed) [DOE]

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative1 First Use of Energy for All Purposes (Fuel and Nonfuel), 2002; Level: National5Sales for4,645 3,625 1,006 492 742 33Frequently20,000 RussianBy:Whether you're a16-17, 201529, 2015 8:00AM EDT toTheWith693Absorption

  12. SMB, X-ray Absorption Spectroscopy

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative1 First Use of Energy for All Purposes (Fuel and Nonfuel), 2002; Level:Energy: Grid Integration Redefining What's PossibleRadiation Protection245C Unlimited ReleaseWelcome to theAbsorption Spectroscopy X-ray

  13. Secondary atomization of coal-water fuels for gas turbine applications: Final report

    SciTech Connect (OSTI)

    Yu, T.U.; Kang, S.W.; Beer, J.M.

    1988-12-01T23:59:59.000Z

    The main research objective was to determine the effectiveness of the CWF treatments on atomization quality when applied to an ultrafine coal-water fuel (solids loading reduced to 50%) and to gas turbine operating conditions (atomization at elevated pressures). Three fuel treatment techniques were studied: (1) heating of CWF under pressure to produce steam as the pressure drops during passage of the CWF through the atomizer nozzle, (2) absorption of CO/sub 2/ gas in the CWF to produce a similar effect, and (3) a combination of the two treatments above. These techniques were expected to produce secondary atomization, that is, disruptive shattering of CWF droplets subsequent to their leaving the atomizing nozzle, and to lead to better burnout and finer fly ash size distribution. A parallel objective was to present quantitative information on the spray characteristics (mean droplet size, radial distribution of droplet size, and spray shape) of CWF with and without fuel treatment, applicable to the design of CWF-burning gas turbine combustors. The experiments included laser diffraction droplet size measurements and high-speed photographic studies in the MIT Spray Test Facility to determine mean droplet size (mass median diameter), droplet size distribution, and spray shape and angle. Three systems of atomized sprays were studied: (1) water sprays heated to a range of temperatures at atmospheric pressure; (2) CWF sprays heated at atmospheric pressure to different temperatures; and (3) sprays at elevated pressure. 31 refs., 47 figs., 1 tab.

  14. Ionization and dissociation dynamics of vinyl bromide probed by femtosecond extreme ultraviolet transient absorption spectroscopy

    SciTech Connect (OSTI)

    Lin, Ming-Fu; Neumark, Daniel M. [Ultrafast X-ray Science Laboratory, Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States) [Ultrafast X-ray Science Laboratory, Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Department of Chemistry, University of California, Berkeley, California 94720 (United States); Gessner, Oliver [Ultrafast X-ray Science Laboratory, Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States)] [Ultrafast X-ray Science Laboratory, Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Leone, Stephen R. [Ultrafast X-ray Science Laboratory, Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States) [Ultrafast X-ray Science Laboratory, Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Department of Chemistry, University of California, Berkeley, California 94720 (United States); Department of Physics, University of California, Berkeley, California 94720 (United States)

    2014-02-14T23:59:59.000Z

    Strong-field induced ionization and dissociation dynamics of vinyl bromide, CH{sub 2}=CHBr, are probed using femtosecond extreme ultraviolet (XUV) transient absorption spectroscopy. Strong-field ionization is initiated with an intense femtosecond, near infrared (NIR, 775 nm) laser field. Femtosecond XUV pulses covering the photon energy range of 50-72 eV probe the subsequent dynamics by measuring the time-dependent spectroscopic features associated with transitions of the Br (3d) inner-shell electrons to vacancies in molecular and atomic valence orbitals. Spectral signatures are observed for the depletion of neutral C{sub 2}H{sub 3}Br, the formation of C{sub 2}H{sub 3}Br{sup +} ions in their ground (X{sup ~}) and first excited (A{sup ~}) states, the production of C{sub 2}H{sub 3}Br{sup ++} ions, and the appearance of neutral Br ({sup 2}P{sub 3/2}) atoms by dissociative ionization. The formation of free Br ({sup 2}P{sub 3/2}) atoms occurs on a timescale of 330 ± 150 fs. The ionic A{sup ~} state exhibits a time-dependent XUV absorption energy shift of ?0.4 eV within the time window of the atomic Br formation. The yield of Br atoms correlates with the yield of parent ions in the A{sup ~} state as a function of NIR peak intensity. The observations suggest that a fraction of vibrationally excited C{sub 2}H{sub 3}Br{sup +} (A{sup ~}) ions undergoes intramolecular vibrational energy redistribution followed by the C–Br bond dissociation. The C{sub 2}H{sub 3}Br{sup +} (X{sup ~}) products and the majority of the C{sub 2}H{sub 3}Br{sup ++} ions are relatively stable due to a deeper potential well and a high dissociation barrier, respectively. The results offer powerful new insights about orbital-specific electronic processes in high field ionization, coupled vibrational relaxation and dissociation dynamics, and the correlation of valence hole-state location and dissociation in polyatomic molecules, all probed simultaneously by ultrafast table-top XUV spectroscopy.

  15. Understanding and Managing Generation Y

    E-Print Network [OSTI]

    Wallace, Kevin

    2007-12-14T23:59:59.000Z

    There are four generations in the workplace today; they consist of the Silent Generation, Baby Boom Generation, Generation X, and Generation Y. Generation Y, being the newest generation, is the least understood generation although marketers...

  16. Nanoplasmonic Lattices for Ultracold atoms

    E-Print Network [OSTI]

    M. Gullans; T. Tiecke; D. E. Chang; J. Feist; J. D. Thompson; J. I. Cirac; P. Zoller; M. D. Lukin

    2014-07-25T23:59:59.000Z

    We propose to use sub-wavelength confinement of light associated with the near field of plasmonic systems to create nanoscale optical lattices for ultracold atoms. Our approach combines the unique coherence properties of isolated atoms with the sub-wavelength manipulation and strong light-matter interaction associated with nano-plasmonic systems. It allows one to considerably increase the energy scales in the realization of Hubbard models and to engineer effective long-range interactions in coherent and dissipative many-body dynamics. Realistic imperfections and potential applications are discussed.

  17. Relativistic effects in photoionization time delay near the Cooper minimum of noble gas atoms

    E-Print Network [OSTI]

    Kheifets, Anatoli

    of the photoelectron wave- packet upon absorption of a short electromagnetic pulse. This delay is very short such as the kinetic energy (attosecond streak camera), the momentum vector (an- gular streaking attoclock be performed using the time delay in the 1s subshell of He [8]. The high har- monics generation (HHG) technique

  18. An ultra-bright atom laser

    E-Print Network [OSTI]

    V. Bolpasi; N. K. Efremidis; M. J. Morrissey; P. Condylis; D. Sahagun; M. Baker; W. von Klitzing

    2013-11-25T23:59:59.000Z

    We present a novel, ultra-bright atom-laser and ultra-cold thermal atom beam. Using rf-radiation we strongly couple the magnetic hyperfine levels of 87Rb atoms in a magnetically trapped Bose-Einstein condensate. At low rf-frequencies gravity opens a small hole in the trapping potenital and a well collimated, extremely bright atom laser emerges from just below the condensate. As opposed to traditional atom lasers based on weak coupling, this technique allows us to outcouple atoms at an arbitrarily large rate. We demonstrate an increase in flux per atom in the BEC by a factor of sixteen compared to the brightest quasi-continuous atom laser. Furthermore, we produce by two orders of magnitude the coldest thermal atom beam to date (200 nK).

  19. Generator-absorber-heat exchange heat transfer apparatus and method and use thereof in a heat pump

    DOE Patents [OSTI]

    Phillips, Benjamin A. (Benton Harbor, MI); Zawacki, Thomas S. (St. Joseph, MI)

    1996-12-03T23:59:59.000Z

    Numerous embodiments and related methods for generator-absorber heat exchange (GAX) are disclosed, particularly for absorption heat pump systems. Such embodiments and related methods use the working solution of the absorption system for the heat transfer medium. A combination of weak and rich liquor working solution is used as the heat transfer medium.

  20. Narrowband Biphotons: Generation, Manipulation, and Applications

    E-Print Network [OSTI]

    Chih-Sung Chuu; Shengwang Du

    2015-03-14T23:59:59.000Z

    In this chapter, we review recent advances in generating narrowband biphotons with long coherence time using spontaneous parametric interaction in monolithic cavity with cluster effect as well as in cold atoms with electromagnetically induced transparency. Engineering and manipulating the temporal waveforms of these long biphotons provide efficient means for controlling light-matter quantum interaction at the single-photon level. We also review recent experiments using temporally long biphotons and single photons.

  1. ELECTRONIC SPUTTERING: FROM ATOMIC PHYSICS

    E-Print Network [OSTI]

    Johnson, Robert E.

    ELECTRONIC SPUTTERING: FROM ATOMIC PHYSICS TO CONTINUUM MECHANICS Ejection of simple and complex molecules from surfaces probes the response of condensed matter to electronic excitations and has and Engineering Physics at the University of Virginia, Charlottesville. Bo Sundqvist holds the Chair in Ion

  2. Photoabsorption by Ions and Atoms

    SciTech Connect (OSTI)

    Manson, Steven T. [Department of Physics and Astronomy, Georgia State University, Atlanta, Georgia 30303 (United States)

    2004-12-01T23:59:59.000Z

    Recent progress in theoretical and experimental investigations of photoabsorption by atoms and ions is presented. Specifically, examples of near-chaotic behavior in photoionization of positive ions, low-energy manifestations of nondipole effects, high-energy breakdown of the single particle picture and new phenomenology uncovered in the inner-shell photoabsorption by negative ions are discussed.

  3. Diagnostic probes for particle and molecule distributions in laser-generated plumes

    SciTech Connect (OSTI)

    Kimbrell, S.M.

    1990-10-17T23:59:59.000Z

    Laser microprobe analysis (LMA) offers good spatial and depth resolution for solid sampling of virtually any material. Coupled with numerous optical spectroscopic and mass spectrometric detection methods, LMA is a powerful analytical tool. Yet, fundamental understanding of the interaction between the laser and the sample surface leading to the formation of the high temperature plasma (plume) is far from complete. To better understand the process of plume formation, an imaging method based on acousto-optic laser beam deflection has been coupled with light scattering methods and absorption methods to record temporal and spatial maps of the particle and molecule distributions in the plume with good resolution. Because particles can make up a major fraction of the vaporized material under certain operating conditions, they can reflect a large loss of atomic signal for elemental analysis, even when using auxiliary excitation to further vaporized the particles. Characterization of the particle size distributions in plumes should provide insight into the vaporization process and information necessary for studies of efficient particle transfer. Light scattering methods for particle size analysis based on the Mie Theory are used to determine the size of particles in single laser-generated plumes. The methods used, polarization ratio method and dissymmetry ratio method, provide good estimates of particle size with good spatial and temporal resolution for this highly transient system. Large particles, on the order of 0.02-0.2{mu}m in radius, were observed arising directly from the sample surface and from condensation.

  4. Realization of a superconducting atom chip

    E-Print Network [OSTI]

    Thomas Nirrengarten; Angie Qarry; Cédric Roux; Andreas Emmert; Gilles Nogues; Michel Brune; Jean-Michel Raimond; Serge Haroche

    2006-10-09T23:59:59.000Z

    We have trapped rubidium atoms in the magnetic field produced by a superconducting atom chip operated at liquid Helium temperatures. Up to $8.2\\cdot 10^5$ atoms are held in a Ioffe-Pritchard trap at a distance of 440 $\\mu$m from the chip surface, with a temperature of 40 $\\mu$K. The trap lifetime reaches 115 s at low atomic densities. These results open the way to the exploration of atom--surface interactions and coherent atomic transport in a superconducting environment, whose properties are radically different from normal metals at room temperature.

  5. 21cm Absorption by Compact Hydrogen Disks Around Black Holes in Radio-Loud Nuclei of Galaxies

    E-Print Network [OSTI]

    Abraham Loeb

    2008-02-19T23:59:59.000Z

    The clumpy maser disks observed in some galactic nuclei mark the outskirts of the accretion disk that fuels the central black hole and provide a potential site of nuclear star formation. Unfortunately, most of the gas in maser disks is currently not being probed; large maser gains favor paths that are characterized by a small velocity gradient and require rare edge-on orientations of the disk. Here we propose a method for mapping the atomic hydrogen distribution in nuclear disks through its 21cm absorption against the radio continuum glow around the central black hole. In NGC 4258, the 21cm optical depth may approach unity for high angular-resolution (VLBI) imaging of coherent clumps which are dominated by thermal broadening and have the column density inferred from X-ray absorption data, ~10^{23}/cm^2. Spreading the 21cm absorption over the full rotation velocity width of the material in front of the narrow radio jets gives a mean optical depth of ~0.1. Spectroscopic searches for the 21cm absorption feature in other galaxies can be used to identify the large population of inclined gaseous disks which are not masing in our direction. Follow-up imaging of 21cm silhouettes of accelerating clumps within these disks can in turn be used to measure cosmological distances.

  6. Remote atom entanglement in a fiber-connected three-atom system

    E-Print Network [OSTI]

    Guo Yan-Qing; Chen Jing; Song He-Shan

    2008-05-28T23:59:59.000Z

    An Ising-type atom-atom interaction is obtained in a fiber-connected three-atom system. The interaction is effective when $\\Delta\\approx \\gamma _{0}\\gg g$. The preparations of remote two-atom and three-atom entanglement governed by this interaction are discussed in specific parameters region. The overall two-atom entanglement is very small because of the existence of the third atom. However, the three-atom entanglement can reach a maximum very close to 1.

  7. A solenoidal synthetic field and the non-Abelian Aharonov-Bohm effects in neutral atoms

    E-Print Network [OSTI]

    Ming-Xia Huo; Nie Wei; David A. W. Hutchinson; Leong Chuan Kwek

    2014-08-11T23:59:59.000Z

    Cold neutral atoms provide a versatile and controllable platform for emulating various quantum systems. Despite efforts to develop artificial gauge fields in these systems, realizing a unique ideal-solenoid-shaped magnetic field within the quantum domain in any real-world physical system remains elusive. Here we propose a scheme to generate a "hairline" solenoid with an extremely small size around 1 micrometer which is smaller than the typical coherence length in cold atoms. Correspondingly, interference effects will play a role in transport. Despite the small size, the magnetic flux imposed on the atoms is very large thanks to the very strong field generated inside the solenoid. By arranging different sets of Laguerre-Gauss (LG) lasers, the generation of Abelian and non-Abelian SU(2) lattice gauge fields is proposed for neutral atoms in ring- and square-shaped optical lattices. As an application, interference patterns of the magnetic type-I Aharonov-Bohm (AB) effect are obtained by evolving atoms along a circle over several tens of lattice cells. During the evolution, the quantum coherence is maintained and the atoms are exposed to a large magnetic flux. The scheme requires only standard optical access, and is robust to weak particle interactions.

  8. Development and proof-testing of advanced absorption refrigeration cycle concepts

    SciTech Connect (OSTI)

    Modahl, R.J.; Hayes, F.C. (Trane Co., La Crosse, WI (United States). Applied Unitary/Refrigeration Systems Div.)

    1992-03-01T23:59:59.000Z

    The overall objectives of this project are to evaluate, develop, and proof-test advanced absorption refrigeration cycles that are applicable to residential and commercial heat pumps for space conditioning. The heat pump system is to be direct-fired with natural gas and is to use absorption working fluids whose properties are known. Target coefficients of performance (COPs) are 1.6 at 47{degrees}F and 1.2 at 17{degrees} in the heating mode, and 0.7 at 95{degree}F in the cooling mode, including the effect of flue losses. The project is divided into three phases. Phase I entailed the analytical evaluation of advanced cycles and included the selection of preferred concepts for further development. Phase II involves the development and testing of critical components and of a complete laboratory breadboard version of the selected system. Phase III calls for the development of a prototype unit and is contingent on the successful completion of Phase II. This report covers Phase I work on the project. In Phase 1, 24 advanced absorption cycle/fluid combinations were evaluated, and computer models were developed to predict system performance. COP, theoretical pump power, and internal heat exchange were calculated for each system, and these calculations were used as indicators of operating and installed costs in order to rank the relative promise of each system. The highest ranking systems involve the cycle concept of absorber/generator heat exchange, generator heat exchanger/absorber heat exchange, regeneration, and resorption/desorption, in combination with the NH{sub 3}/H{sub 2}O/LiBr ternary absorption fluid mixture or with the NH{sub 3}/H{sub 2}O binary solution. Based upon these conclusions, the recommendation was made to proceed to Phase II, the laboratory breadboard proof-of- concept.

  9. Enhanced light absorption of solar cells and photodetectors by diffraction

    DOE Patents [OSTI]

    Zaidi, Saleem H.; Gee, James M.

    2005-02-22T23:59:59.000Z

    Enhanced light absorption of solar cells and photodetectors by diffraction is described. Triangular, rectangular, and blazed subwavelength periodic structures are shown to improve performance of solar cells. Surface reflection can be tailored for either broadband, or narrow-band spectral absorption. Enhanced absorption is achieved by efficient optical coupling into obliquely propagating transmitted diffraction orders. Subwavelength one-dimensional structures are designed for polarization-dependent, wavelength-selective absorption in solar cells and photodetectors, while two-dimensional structures are designed for polarization-independent, wavelength-selective absorption therein. Suitable one and two-dimensional subwavelength periodic structures can also be designed for broadband spectral absorption in solar cells and photodetectors. If reactive ion etching (RIE) processes are used to form the grating, RIE-induced surface damage in subwavelength structures can be repaired by forming junctions using ion implantation methods. RIE-induced surface damage can also be removed by post RIE wet-chemical etching treatments.

  10. Influence of laser beam profile on electromagnetically induced absorption

    SciTech Connect (OSTI)

    Cuk, S. M.; Radonjic, M.; Krmpot, A. J.; Nikolic, S. N.; Grujic, Z. D.; Jelenkovic, B. M. [Institute of Physics, University of Belgrade, Pregrevica 118, 11080 Belgrade (Serbia)

    2010-12-15T23:59:59.000Z

    We compared, experimentally and theoretically, Hanle electromagnetically induced absorption (EIA) obtained using Gaussian and {Pi}-shaped laser beams 3 mm in diameter. The study was done by measuring the transmission of a laser locked to the F{sub g}=2{yields}F{sub e}=3 transition at the D{sub 2} line of {sup 87}Rb in a vacuum cell. EIA linewidths obtained for the two laser profiles were significantly different in the range of laser intensities 1-4 mW/cm{sup 2}. EIA with the {Pi}-shaped laser beam has a broad intensity maximum and linewidths larger than those obtained with the Gaussian beam profile. We also studied Hanle EIA by measuring the transmission of selected segments of the entire laser beam by placing a small movable aperture in front of the detector. Waveforms so obtained in Hanle EIA resonances were strongly influenced both by the radial distance of the transmitted segment from the beam center and by the radial profile of the laser beam. We show that outer regions of Gaussian beam, and central regions of the {Pi}-shaped beam generate the narrowest lines. The different behaviors of EIA owing to different beam profiles revealed by both theory and experiment indicate the importance of the radial profile of the laser beam for proper modeling of coherent effects in alkali metal vapors.

  11. Local versus global electronic properties of chalcopyrite alloys: X-ray absorption spectroscopy and ab initio calculations

    SciTech Connect (OSTI)

    Sarmiento-Pérez, Rafael; Botti, Silvana, E-mail: silvana.botti@univ-lyon1.fr [Institut Lumière Matière and ETSF, UMR5306 Université Lyon 1-CNRS, Université de Lyon, F-69622 Villeurbanne Cedex (France); Schnohr, Claudia S., E-mail: c.schnohr@uni-jena.de [Institut für Festkörperphysik, Friedrich-Schiller-Universität Jena, Max-Wien-Platz 1, 07743 Jena (Germany); Lauermann, Iver [Helmholtz-Zentrum Berlin für Materialien und Energie, Hahn-Meitner Platz 1, 14109 Berlin (Germany); Rubio, Angel [Nano-Bio Spectroscopy Group and ETSF Scientific Development Centre, Departamento de Física de Materiales, Centro de Física de Materiales CSIC-MPC and DIPC, Universidad del País Vasco UPV/EHU, Avenida de Tolosa 72, E-20018 San Sebastián (Spain); Fritz Haber Institute, Max Planck Society, Faradayweg 4-6, 14195 Berlin (Germany); Johnson, Benjamin, E-mail: benjamin.johnson@alumni.tu-berlin.de [Fritz Haber Institute, Max Planck Society, Faradayweg 4-6, 14195 Berlin (Germany)

    2014-09-07T23:59:59.000Z

    Element-specific unoccupied electronic states of Cu(In, Ga)S{sub 2} were studied as a function of the In/Ga ratio by combining X-ray absorption spectroscopy with density functional theory calculations. The S absorption edge shifts with changing In/Ga ratio as expected from the variation of the band gap. In contrast, the cation edge positions are largely independent of composition despite the changing band gap. This unexpected behavior is well reproduced by our calculations and originates from the dependence of the electronic states on the local atomic environment. The changing band gap arises from a changing spatial average of these localized states with changing alloy composition.

  12. Commercialization of Industrialized Absorption Heat Pumps in the US

    E-Print Network [OSTI]

    Pettigrew, M. G.

    COMMERCIALIZATION OF INDUSTRIAL ABSORPTION HEAT PUMPS IN THE US MALCOLM G. PETTIGREW LITWIN ENGINEERS &CONSTRUCTORS, INC. HOUSTON, ABSTRACT The recovery of waste heat through absorption heat pumping is quite appeal ing to U.S. industry.... However, although this technology has been successfully applied in Europe and Japan, a cauti ous atmosphere wi 11 continue to prevail in the U.S. until the first absorption heat pump is built and successfully demonstrates it's viability...

  13. absorption spectrometry configurations: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    recurrence satisfied by the Stirling numbers of the second kind. Abrams, Aaron; Hower, Valerie 2010-01-01 74 Nonlinear Coherent Perfect Absorption CERN Preprints Summary:...

  14. absorption heat pumps: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Heating capacity k jet nozzle Closed Cycles: AbsorptionAdsorption heat pump thermal compressor driven by waste heat1 Industrial heat pumps in Germany - potentials,...

  15. absorption heat pump: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Heating capacity k jet nozzle Closed Cycles: AbsorptionAdsorption heat pump thermal compressor driven by waste heat1 Industrial heat pumps in Germany - potentials,...

  16. Capturing All the Light: Panchromatic Visible Absorption for...

    Office of Science (SC) Website

    Capturing All the Light: Panchromatic Visible Absorption for Solar Photoconversion Basic Energy Sciences (BES) BES Home About Research Facilities Science Highlights Benefits of BES...

  17. Geothermal: Sponsored by OSTI -- Chapter 13. Absorption Refrigeration

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    3. Absorption Refrigeration Geothermal Technologies Legacy Collection HelpFAQ | Site Map | Contact Us HomeBasic Search About Publications Advanced Search New Hot Docs News...

  18. absorption solar receiver: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    which exhibit a broadband absorption enhancement over 2 An Air-Based Cavity-Receiver for Solar Trough Concentrators Roman Bader Renewable Energy Websites Summary: for a heat...

  19. Absorption of Foliar-Applied Nitrogen by Cotton

    E-Print Network [OSTI]

    Oosterhuis, Derrick M

    2009-01-01T23:59:59.000Z

    on the epicuticular wax composition and ultrastructure ofleaf age, epicuticular wax, and nitrogen-15 absorption. Cropleaf cuticle and epicuticular wax as described by Oosterhuis

  20. absorption spectrometry feasibility: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption is induced by tunable laser excitation Maier, John Paul 5 FEASIBILITY OF SOLAR-FIRED, COMPRESSOR-ASSISTED Energy Storage, Conversion and Utilization Websites...

  1. Absorption Mode FT-ICR Mass Spectrometry Imaging. | EMSL

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Mass Spectrometry Imaging. Absorption Mode FT-ICR Mass Spectrometry Imaging. Abstract: Fourier transform ion cyclotron resonance mass spectrometry offers the highest mass resolving...

  2. absorption diffusion physical: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    of Low Temperature Physics, Vol. 72, Nos. 56, 1988 Pressure Diffusion and Sound Absorption in Physics Websites Summary: of the usual transport coefficients (viscosity...

  3. absorption coefficient based: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    22 23 24 25 Next Page Last Page Topic Index 1 Lifshitz tails for the Interband Light Absorption Coefficient Mathematics Websites Summary: Lifshitz tails for the Interband Light...

  4. Black holes and the absorption rate of cosmological scalar fields

    E-Print Network [OSTI]

    L. Arturo Urena-Lopez; Lizbeth M. Fernandez

    2011-07-15T23:59:59.000Z

    We study the absorption of a massless scalar field by a static black hole. Using the continuity equation that arises from the Klein-Gordon equation, it is possible to define a normalized absorption rate $\\Gamma(t)$ for the scalar field as it falls into the black hole. It is found that the absorption mainly depends upon the characteristics wavelengths involved in the physical system: the mean wavenumber and the width of the wave packet, but that it is insensitive to the scalar field's strength. By taking a limiting procedure, we determine the minimum absorption fraction of the scalar field's mass by the black hole, which is around 50%.

  5. Absorption Lengths in the Holographic Plasma

    E-Print Network [OSTI]

    Irene Amado; Carlos Hoyos; Karl Landsteiner; Sergio Montero

    2007-07-11T23:59:59.000Z

    We consider the effect of a periodic perturbation with frequency $\\omega$ on the holographic N=4 plasma represented by the planar AdS black hole. The response of the system is given by exponentially decaying waves. The corresponding complex wave numbers can be found by solving wave equations in the AdS black hole background with infalling boundary conditions on the horizon in an analogous way as in the calculation of quasinormal modes. The complex momentum eigenvalues have an interpretation as poles of the retarded Green's functions, where the inverse of the imaginary part gives an absorption length $\\lambda$. At zero frequency we obtain the screening length for a static field. These are directly related to the glueball masses in the dimensionally reduced theory. We also point out that the longest screening length corresponds to an operator with non-vanishing R-charge and thus does not have an interpretation as a QCD3 glueball.

  6. Performance bound for quantum absorption refrigerators

    E-Print Network [OSTI]

    Luis A. Correa; José P. Palao; Gerardo Adesso; Daniel Alonso

    2013-04-29T23:59:59.000Z

    An implementation of quantum absorption chillers with three qubits has been recently proposed, that is ideally able to reach the Carnot performance regime. Here we study the working efficiency of such self-contained refrigerators, adopting a consistent treatment of dissipation effects. We demonstrate that the coefficient of performance at maximum cooling power is upper bounded by 3/4 of the Carnot performance. The result is independent of the details of the system and the equilibrium temperatures of the external baths. We provide design prescriptions that saturate the bound in the limit of a large difference between the operating temperatures. Our study suggests that delocalized dissipation, which must be taken into account for a proper modelling of the machine-baths interaction, is a fundamental source of irreversibility which prevents the refrigerator from approaching the Carnot performance arbitrarily closely in practice. The potential role of quantum correlations in the operation of these machines is also investigated.

  7. Counterflow absorber for an absorption refrigeration system

    DOE Patents [OSTI]

    Reimann, Robert C. (Lafayette, NY)

    1984-01-01T23:59:59.000Z

    An air-cooled, vertical tube absorber for an absorption refrigeration system is disclosed. Strong absorbent solution is supplied to the top of the absorber and refrigerant vapor is supplied to the bottom of the absorber to create a direct counterflow of refrigerant vapor and absorbent solution in the absorber. The refrigeration system is designed so that the volume flow rate of refrigerant vapor in the tubes of the absorber is sufficient to create a substantially direct counterflow along the entire length of each tube in the absorber. This provides several advantages for the absorber such as higher efficiency and improved heat transfer characteristics, and allows improved purging of non-condensibles from the absorber.

  8. Multi-stage quantum absorption heat pumps

    E-Print Network [OSTI]

    Luis A. Correa

    2014-01-16T23:59:59.000Z

    It is well known that heat pumps, while being all limited by the same basic thermodynamic laws, may find realization on systems as "small" and "quantum" as a three-level maser. In order to quantitatively assess how the performance of these devices scales with their size, we design generalized $N$-dimensional ideal heat pumps by merging $N-2$ elementary three-level stages. We set them to operate in the absorption chiller mode between given hot and cold baths, and study their maximum achievable cooling power and the corresponding efficiency as a function of $N$. While the efficiency at maximum power is roughly size-independent, the power itself slightly increases with the dimension, quickly saturating to a constant. Thus, interestingly, scaling up autonomous quantum heat pumps does not render a significant enhancement beyond the optimal double-stage configuration.

  9. Gas separation using ultrasound and light absorption

    DOE Patents [OSTI]

    Sinha, Dipen N. (Los Alamos, NM)

    2012-07-31T23:59:59.000Z

    An apparatus and method for separating a chosen gas from a mixture of gases having no moving parts and utilizing no chemical processing is described. The separation of particulates from fluid carriers thereof has been observed using ultrasound. In a similar manner, molecular species may be separated from carrier species. It is also known that light-induced drift may separate light-absorbing species from carrier species. Therefore, the combination of temporally pulsed absorption of light with ultrasonic concentration is expected to significantly increase the efficiency of separation by ultrasonic concentration alone. Additionally, breaking the spatial symmetry of a cylindrical acoustic concentrator decreases the spatial distribution of the concentrated particles, and increases the concentration efficiency.

  10. J/$?$ absorption in a multicomponent hadron gas

    E-Print Network [OSTI]

    Dariusz Prorok; Ludwik Turko; David Blaschke

    2008-08-04T23:59:59.000Z

    A model for anomalous $J/\\Psi$ suppression in high energy heavy ion collisions is presented. As the additional suppression mechanism beyond standard nuclear absorption inelastic $J/\\Psi$ scattering with hadronic matter is considered. Hadronic matter is modeled as an evolving multi-component gas of point-like non-interacting particles (MCHG). Estimates for the sound velocity of the MCHG are given and the equation of state is compared with Lattice QCD data in the vicinity of the deconfinement phase transition. The approximate cooling pattern caused by longitudinal expansion is presented. It is shown that under these conditions the resulting $J/\\Psi$ suppression pattern agrees well with NA38 and NA50 data.

  11. Moøller polarimetry with polarized atomic hydrogen at MESA

    SciTech Connect (OSTI)

    Bartolomé, P. Aguar; Aulenbacher, K.; Tyukin, V. [Institut für Kernphysik, Johannes Gutenberg-University, D-55099 Mainz (Germany)

    2013-11-07T23:59:59.000Z

    A new generation of parity violation (PV) electron scattering experiments are planned to be carried out at the Institut für Kernphysik in Mainz. These experiments will be performed at low energies of 100-200 MeV using the new accelerator MESA (Mainz Energy recovering Superconducting Accelerator). One of the main challenges of such experiments is to achieve an accuracy in beam polarization measurements that must be below 0.5%. This very high accuracy can be reached using polarized atomic hydrogen gas, stored in an ultra-cold magnetic trap, as the target for electron beam polarimetry based on Mo/ller scattering. Electron spin-polarized atomic hydrogen can be stored at high densities of 10{sup 16} cm{sup ?2}, over relatively long time periods, in a high magnetic field (8T) and at low temperatures (0.3K). The gradient force splits the ground state of the hydrogen into four states with different energies. Atoms in the low energy states are trapped in the strong magnetic field region whereas the high energy states are repelled and pumped away. The physics of ultra-cold atomic hydrogen in magnetic traps and the status of the Mainz Hydro-Mo/ller project will be presented.

  12. Laser sustained discharge nozzle apparatus for the production of an intense beam of high kinetic energy atomic species

    DOE Patents [OSTI]

    Cross, J.B.; Cremers, D.A.

    1986-01-10T23:59:59.000Z

    Laser sustained discharge apparatus for the production of intense beams of high kinetic energy atomic species is described. A portion of the plasma resulting from a laser sustained continuous optical discharge which generates energetic atomic species from a gaseous source thereof is expanded through a nozzle into a region of low pressure. The expanded plasma contains a significant concentration of the high kinetic energy atomic species which may be used to investigate the interaction of surfaces therewith. In particular, O-atoms having velocities in excess of 3.5 km/s can be generated for the purpose of studying their interaction with materials in order to develop protective materials for spacecraft which are exposed to such energetic O-atoms during operation in low earth orbit.

  13. Distinct local structure of nanoparticles and nanowires of V{sub 2}O{sub 5} probed by x-ray absorption spectroscopy

    SciTech Connect (OSTI)

    Joseph, B.; Maugeri, L.; Bendele, M.; Saini, N. L., E-mail: Naurang.Saini@roma1.infn.it [Dipartimento di Fisica, Universitá di Roma “La Sapienza” - P. le Aldo Moro 2, 00185 Roma (Italy); Iadecola, A. [Dipartimento di Fisica, Universitá di Roma “La Sapienza” - P. le Aldo Moro 2, 00185 Roma (Italy) [Dipartimento di Fisica, Universitá di Roma “La Sapienza” - P. le Aldo Moro 2, 00185 Roma (Italy); Elettra, Sincrotrone Trieste, Strada Statale 14, Km 163.5, Basovizza, Trieste (Italy); Okubo, M.; Li, H.; Zhou, H. [National Institute of Advanced Industrial Science and Technology (AIST), Umezono 1-1-1, Tsukuba 305-8568 (Japan)] [National Institute of Advanced Industrial Science and Technology (AIST), Umezono 1-1-1, Tsukuba 305-8568 (Japan); Mizokawa, T. [Department of Physics, University of Tokyo, 5-1-5 Kashiwanoha, Kashiwa, Chiba 277-8561 (Japan) [Department of Physics, University of Tokyo, 5-1-5 Kashiwanoha, Kashiwa, Chiba 277-8561 (Japan); Department of Complexity Science and Engineering, University of Tokyo, 5-1-5 Kashiwanoha, Kashiwa, Chiba 277-8561 (Japan)

    2013-12-16T23:59:59.000Z

    We have used V K-edge x-ray absorption spectroscopy to study local structures of bulk, nanoparticles and nanowires of V{sub 2}O{sub 5}. The extended x-ray absorption fine structure measurements show different local displacements in the three morphologically different V{sub 2}O{sub 5} samples. It is found that the nanowires have a significantly ordered chain structure in comparison to the V{sub 2}O{sub 5} bulk. In contrast, nanoparticles have larger interlayer disorder. The x-ray absorption near-edge structure spectra show different electronic structure that appears to be related with the local atomic disorder in the three V{sub 2}O{sub 5} samples.

  14. Role of atomic collisions in fusion

    SciTech Connect (OSTI)

    Post, D.E.

    1982-04-01T23:59:59.000Z

    Atomic physics issues have played a large role in controlled fusion research. A general discussion of the present role of atomic processes in both magnetic and inertial controlled fusion work is presented.

  15. Preliminary steps to the Atomic Energy Commission

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    program to the newly created Atomic Energy Commission. He had succeeded in ending the war, but the transition to peacetime use of atomic energy was not something the Army was...

  16. Sub-Doppler and subnatural narrowing of an absorption line induced by interacting dark resonances in a tripod system

    SciTech Connect (OSTI)

    Goren, C.; Rosenbluh, M. [Department of Physics, Bar-Ilan University, Ramat Gan 52900 (Israel); Wilson-Gordon, A.D.; Friedmann, H. [Department of Chemistry, Bar-Ilan University, Ramat Gan 52900 (Israel)

    2004-06-01T23:59:59.000Z

    A method is presented for obtaining sub-Doppler and subnatural narrowing and increased absorption of a spectral line. The ultranarrow spectral line is confined between two closely spaced electromagnetically induced transparency windows in a nearly degenerate tripod atomic system formed by an F{sub g}=1{yields}F{sub e}=0 transition, split by a magnetic field. The system is driven by a {sigma}-polarized pump and probed by a tunable {pi}-polarized laser. It can be used to measure small magnetic fields and also as a magneto-optic switch.

  17. atomic kitteni lauljatar: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    with atomic and molecular matter waves is a rich branch of atomic physics and quantum optics. It started with atom diffraction from crystal surfaces and the separated oscillatory...

  18. atoms barrasiye barhamkoneshhaye: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    with atomic and molecular matter waves is a rich branch of atomic physics and quantum optics. It started with atom diffraction from crystal surfaces and the separated oscillatory...

  19. atomic mass spectrometry: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Negative *) Atomic composition Graham, Nick 3 Prospects in Analytical Atomic Spectrometry CERN Preprints Summary: Tendencies in five main branches of atomic spectrometry...

  20. Institute for Atom-Efficient Chemical Transformations Energy...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    adsorbed in a zirconium oxide nanobowl. The brown atoms are surface oxygen and the coral atoms are zirconium. Carbon, oxygen, and hydrogen atoms of fructose molecules are...

  1. Towards a high-precision atomic gyroscope

    E-Print Network [OSTI]

    Van Camp, Mackenzie A. (Mackenzie Anne)

    2013-01-01T23:59:59.000Z

    In this thesis, I report on the design and construction of the Rubidium Atomic Gyroscope Experiment (RAGE) at Draper Lab.

  2. Atomic Ordering Enhanced Electrocatalytic Activity of Nanoalloys...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Ordering Enhanced Electrocatalytic Activity of Nanoalloys for Oxygen Reduction Reaction. Atomic Ordering Enhanced Electrocatalytic Activity of Nanoalloys for Oxygen Reduction...

  3. Resonant subharmonic absorption and second-harmonic generation by a fluctuating nonlinear oscillator

    E-Print Network [OSTI]

    Dykman, Mark

    energy E or, equivalently, on the vibration amplitude . For a fluctuating oscillator the energy varies theoretically, numerically, and with an analog elec- tronic circuit model. The system studied has often been oscillator. The eigen- frequency of the vibrations of a nonlinear oscillator (E) depends on the oscillator

  4. Generation gaps in engineering?

    E-Print Network [OSTI]

    Kim, David J. (David Jinwoo)

    2008-01-01T23:59:59.000Z

    There is much enthusiastic debate on the topic of generation gaps in the workplace today; what the generational differences are, how to address the apparent challenges, and if the generations themselves are even real. ...

  5. Influence of plasma parameters on the absorption coefficient of alpha particles to lower hybrid waves in tokamaks

    SciTech Connect (OSTI)

    Wang, J.; Zhang, X., E-mail: zhangxm@ecust.edu.cn; Yu, L.; Zhao, X. [East China University of Science and Technology, Department of Physics (China)

    2014-12-15T23:59:59.000Z

    In tokamaks, fusion generated ? particles may absorb lower hybrid (LH) wave energy, thus reducing the LH current drive efficiency. The absorption coefficient ?{sub ?} of LH waves due to ? particles changing with some typical parameters is calculated in this paper. Results show that ?{sub ?} increases with the parallel refraction index n{sub ?}, while decreases with the frequency of LH waves ? over a wide range. Higher background plasma temperature and toroidal magnetic field will increase the absorption. The absorption coefficient ?{sub ?} increases with n{sub e} when n{sub e} ? 8 × 10{sup 19} m{sup ?3}, while decreases with n{sub e} when n{sub e} becomes larger, and there is a peak value of ?{sub ?} when n{sub e} ? 8 × 10{sup 19} m{sup ?1} for the ITER-like scenario. The influence of spectral broadening in parametric decay instabilities on the absorption coefficient is evaluated. The value of ?{sub ?} with n{sub ?} being 2.5 is almost two times larger than that with n{sub ?} being 2.0 and is even lager in the case of 2.9, which will obviously increase the absorption of the LH power by alpha particles.

  6. Chaotic Behaviour of Atomic Energy Levels

    E-Print Network [OSTI]

    A. Yilmaz; G. Hacibekiroglu; E. Bolcal; Y. Polatoglu

    2008-04-01T23:59:59.000Z

    The authors of this paper studied Schrodinger wave equation to investiagate the chaotic behavior of atomic energy levels in relation with three quantum numbers n, l, m by means of derived inequality. It could give rise to the siplitting of atomic spectral lines. Keywords: Chaos, Schrodinger wave equation, atomic energy levels

  7. Riso Report No. Danish Atomic Energy Commission

    E-Print Network [OSTI]

    Jagiellonski Institute of Physics Krakow, Poland and P. A. Lindgård Mogensen The Danish Atomic EnergyfM O o 8- OL '·O c/i Riso Report No. Danish Atomic Energy Commission Research Establishment Riso/t on exchangefrom: Library, Danish Atomic Energy Commission, Risd, Roskilde, Denmark #12;May, 1966 Ris6 Report No

  8. The Future of Atomic Energy

    DOE R&D Accomplishments [OSTI]

    Fermi, E.

    1946-05-27T23:59:59.000Z

    There is definitely a technical possibility that atomic power may gradually develop into one of the principal sources of useful power. If this expectation will prove correct, great advantages can be expected to come from the fact that the weight of the fuel is almost negligible. This feature may be particularly valuable for making power available to regions of difficult access and far from deposits of coal. It also may prove a great asset in mobile power units for example in a power plant for ship propulsion. On the negative side there are some technical limitations to be applicability of atomic power of which perhaps the most serious is the impossibility of constructing light power units; also there will be some peculiar difficulties in operating atomic plants, as for example the necessity of handling highly radioactive substances which will necessitate, at least for some considerable period, the use of specially skilled personnel for the operation. But the chief obstacle in the way of developing atomic power will be the difficulty of organizing a large scale industrial development in an internationally safe way. This presents actually problems much more difficult to solve than any of the technical developments that are necessary, It will require an unusual amount of statesmanship to balance properly the necessity of allaying the international suspicion that arises from withholding technical secrets against the obvious danger of dumping the details of the procedures for an extremely dangerous new method of warfare on a world that may not yet be prepared to renounce war. Furthermore, the proper balance should be found in the relatively short time that will elapse before the 'secrets' will naturally become open knowledge by rediscovery on part of the scientists and engineers of other countries.

  9. Small Generator Aggregation (Maine)

    Broader source: Energy.gov [DOE]

    This section establishes requirements for electricity providers to purchase electricity from small generators, with the goal of ensuring that small electricity generators (those with a nameplate...

  10. Off-resonance energy absorption in a linear Paul trap due to mass selective resonant quenching

    SciTech Connect (OSTI)

    Sivarajah, I.; Goodman, D. S.; Wells, J. E.; Smith, W. W. [Department of Physics, University of Connecticut, Storrs, Connecticut 06269 (United States)] [Department of Physics, University of Connecticut, Storrs, Connecticut 06269 (United States); Narducci, F. A. [Naval Air Systems Command, EO Sensors Division, Bldg 2187, Suite 3190 Patuxent River, Maryland 20670 (United States)] [Naval Air Systems Command, EO Sensors Division, Bldg 2187, Suite 3190 Patuxent River, Maryland 20670 (United States)

    2013-11-15T23:59:59.000Z

    Linear Paul traps (LPT) are used in many experimental studies such as mass spectrometry, atom-ion collisions, and ion-molecule reactions. Mass selective resonant quenching (MSRQ) is implemented in LPT either to identify a charged particle's mass or to remove unwanted ions from a controlled experimental environment. In the latter case, MSRQ can introduce undesired heating to co-trapped ions of different mass, whose secular motion is off resonance with the quenching ac field, which we call off-resonance energy absorption (OREA). We present simulations and experimental evidence that show that the OREA increases exponentially with the number of ions loaded into the trap and with the amplitude of the off-resonance external ac field.

  11. High resolution laser induced fluorescence Doppler velocimetry utilizing saturated absorption spectroscopy

    SciTech Connect (OSTI)

    Aramaki, Mitsutoshi [Department of Electrical Engineering and Computer Science, Nagoya University, Nagoya 464-8603 (Japan); Ogiwara, Kohei; Etoh, Shuzo [Interdisciplinary Graduate School of Engineering Sciences, Kyushu University, Kasuga 816-8580 (Japan); Yoshimura, Shinji [National Institute for Fusion Science, Toki 509-5292 (Japan); Tanaka, Masayoshi Y. [Department of Advanced Energy Engineering Science, Kyushu University, Kasuga 816-8580 (Japan)

    2009-05-15T23:59:59.000Z

    A high resolution laser induced fluorescence (LIF) system has been developed to measure the flow velocity field of neutral particles in an electron-cyclotron-resonance argon plasma. The flow velocity has been determined by the Doppler shift of the LIF spectrum, which is proportional to the velocity distribution function. Very high accuracy in velocity determination has been achieved by installing a saturated absorption spectroscopy unit into the LIF system, where the absolute value and scale of laser wavelength are determined by using the Lamb dip and the fringes of a Fabry-Perot interferometer. The minimum detectable flow velocity of a newly developed LIF system is {+-}2 m/s, and this performance remains unchanged in a long-time experiment. From the radial measurements of LIF spectra of argon metastable atoms, it is found that there exists an inward flow of neutral particles associated with neutral depletion.

  12. Temperature and number evolution of cold cesium atoms inside a glass cell

    E-Print Network [OSTI]

    Huang, J Q; Wang, S G; Wang, Z B; Wang, L J

    2015-01-01T23:59:59.000Z

    We report an experimental study on the temperature and number evolution of the cold cesium atoms diffusively cooled inside a wall-coated glass cell by measuring the absorption profile of the 62S1/2 (F=4)-62P3/2 (F'=5) transition line with a weak probe laser in the evolution process. We found that the temperature of the cold atoms first gradually decreases from 16 mK to 9 mK, and then rapidly increases. A theoretical model of the number evolution is built, which includes the temperature of the cold atoms and the fraction p of the cold cesium atoms elastically reflected by the cell wall. The theoretical model is consistent with the experimental result very well, and the fraction p is obtained to be (0.58 +/- 0.03), which reveals that the cold cesium atoms are not all heated to the ambient temperature by a single collision with the cell wall.

  13. NAAP Hydrogen Atom 1/9 The Hydrogen Atom Student Guide

    E-Print Network [OSTI]

    Farritor, Shane

    Name: NAAP ­ Hydrogen Atom 1/9 The Hydrogen Atom ­ Student Guide Background Material Carefully read and the Quantum model represent the Hydrogen atom. In some cases they both describe things in the same way frequency, smaller energy, and the same velocity through space as a blue photon". #12;NAAP ­Hydrogen Atom 2

  14. Fast transport, atom sample splitting and single-atom qubit supply in two-dimensional arrays

    E-Print Network [OSTI]

    Birkl, Gerhard

    Fast transport, atom sample splitting and single-atom qubit supply in two-dimensional arrays architecture for neutral atom quantum information processing, quantum simulation and the manipulation of ultra-cold implemented functions. We introduce piezo-actuator-based transport of atom ensembles over distances of more

  15. Light pulse in {Lambda}-type cold-atom gases

    SciTech Connect (OSTI)

    Wei Ran; Deng Youjin; Chen Shuai; Chen Zengbing; Pan Jianwei [Hefei National Laboratory for Physical Sciences at Microscale and Department of Modern Physics, University of Science and Technology of China, Hefei, Anhui 230026 (China); Zhao Bo [Institute for Theoretical physics, University of Innsbruck, A-6020 Innsbruck (Austria); Institute for Quantum Optics and Quantum Information of the Austrian Academy of Science, A-6020 Innsbruck (Austria)

    2010-04-15T23:59:59.000Z

    We investigate the behavior of the light pulse in {Lambda}-type cold-atom gases with two counter-propagating control lights with equal strength by directly simulating the dynamic equations and exploring the dispersion relation. Our analysis shows that, depending on the length L{sub 0} of the stored wave packet and the decay rate {gamma} of ground-spin coherence, the recreated light can behave differently. For long L{sub 0} and/or large {gamma}, a stationary light pulse is produced, while two propagating light pulses appear for short L{sub 0} and/or small {gamma}. In the {gamma}{yields}0 limit, the light always splits into two propagating pulses for a sufficiently long time. This scenario agrees with a recent experiment [Y.-W. Lin et al., Phys. Rev. Lett. 102, 213601 (2009)] where two propagating light pulses are generated in laser-cooled cold-atom ensembles.

  16. Ab initio curved-wave x-ray-absorption fine structure

    SciTech Connect (OSTI)

    Mustre de Leon, J.; Rehr, J.J.; Zabinsky, S.I. (Department of Physics, FM-15, University of Washington, Seattle, Washington (USA)); Albers, R.C. (Theoretical Division, Los Alamos National Laboratory, Los Alamos, New Mexico (USA))

    1991-09-01T23:59:59.000Z

    The most important elements of {ital ab} {ital initio} calculations of x-ray-absorption fine structure (XAFS) are studied. To obtain accurate results without {ital ad} {ital hoc} adjustable parameters, we find it essential to include (i) curved-wave effects, (ii) a complex, energy-dependent self-energy, (iii) an approximate molecular potential, and (iv) a fixed energy reference for the photoelectron wave number. Based on these findings, an automated code has been developed for {ital ab} {ital initio} calculations of single-scattering XAFS, in which curved-wave effects are treated exactly in terms of effective backscattering amplitudes, inelastic losses and self-energy shifts are incorporated with use of a Hedin-Lundqvist self-energy, an automated relativistic overlapping-atom muffin-tin potential is used, and the energy threshold is estimated from electron-gas theory. The efficiency of the code is made possible by analytic expressions for the Hedin-Lundqvist self-energy. This code replaces existing tables of XAFS phases and scattering amplitudes and yields reliable theoretical XAFS standards for arbitrary pairs of atoms throughout the Periodic Table ({ital Z}{le}94). These results are comparable to those from self-consistent calculations and are valid to within about 20 eV of the absorption edge. Comparisons with experiment are presented for Cu, Ge, Pt, Br{sub 2}, and GeCl{sub 4}. The calculated XAFS amplitudes are found to be accurate to within 15%; XAFS phases are accurate to within 0.2 rad; and nearest-neighbor distances are typically accurate to within 0.02 A.

  17. LATTICE DYNAMICS NUCLEAR RESONANCE ABSORPTION OF GAMMA-RADIATION

    E-Print Network [OSTI]

    Paris-Sud XI, Université de

    LATTICE DYNAMICS NUCLEAR RESONANCE ABSORPTION OF GAMMA-RADIATION AND COHERENT DECAY MODES Institut effets de correlation de paires. Abstract. -The cross-section for nuclear resonance absorption of gamma-radiation rksonnante des radiations gamma est en gBneral calculee en negligeant I'influence des phenomknes de coherence

  18. Laser Locking with Doppler-free Saturated Absorption Spectroscopy

    E-Print Network [OSTI]

    Novikova, Irina

    - 1 - Laser Locking with Doppler-free Saturated Absorption Spectroscopy Paul L. Stubbs, Advisor the frequency of a 795 nm diode laser using a saturated absorption spectroscopy method. Laser locking in AMO physics is done to stabilize the frequency of lasers used in the laboratory in order to make results more

  19. Optical absorption and ionization of silicate glasses Leonid B. Glebov

    E-Print Network [OSTI]

    Glebov, Leon

    Optical absorption and ionization of silicate glasses Leonid B. Glebov School of Optics and hydroxyl), and induced (color centers) absorption of multicomponent silicate glasses in UV, visible-photon ionization was detected in alkaline-silicate glasses exposed to high-power laser radiation in nano

  20. Simulations of solar cell absorption enhancement using resonant modes

    E-Print Network [OSTI]

    Grandidier, Jonathan

    Simulations of solar cell absorption enhancement using resonant modes of a nanosphere array Jonathan Grandidier Michael G. Deceglie Dennis M. Callahan Harry A. Atwater #12;Simulations of solar cell for enhancing the absorption of thin-film amorphous silicon solar cells using periodic arrangements of resonant

  1. Quantum of optical absorption in two-dimensional semiconductors

    E-Print Network [OSTI]

    California at Irvine, University of

    Quantum of optical absorption in two-dimensional semiconductors Hui Fanga,b,c , Hans A. Bechteld semiconductor, where is the fine structure con- stant and nc is an optical local field correction factor quantitative examination of the intrinsic absorption properties of free-standing 2D semiconductor thin films

  2. Infrared absorption spectra, radiative efficiencies, and global warming potentials

    E-Print Network [OSTI]

    Wirosoetisno, Djoko

    Infrared absorption spectra, radiative efficiencies, and global warming potentials of newly.mdpi.com/journal/atmosphere Article Infrared Absorption Spectra, Radiative Efficiencies, and Global Warming Potentials of Newly of 600­1730 cm-1 . These spectra are then used to calculate the radiative efficiencies and global warming

  3. absorption spectroscopy: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption spectroscopy First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Relic Neutrino Absorption...

  4. absorption difference spectra: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption difference spectra First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Absorption Spectra of...

  5. absorption spectroscopy aas: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption spectroscopy aas First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Relic Neutrino Absorption...

  6. affect intestinal absorption: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    affect intestinal absorption First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Intestinal Absorption and...

  7. absorption tissue distribution: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption tissue distribution First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Absorption and...

  8. absorption features dust: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption features dust First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Silicon carbide absorption...

  9. absorption spectrophotometric studies: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption spectrophotometric studies First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Light absorption...

  10. absorption intestinal: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption intestinal First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Intestinal Absorption and...

  11. acid absorption acceleration: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption acceleration First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Digestion and absorption of...

  12. absorption model: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption model First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Two models for absorption by coloured...

  13. active potassium absorption: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    active potassium absorption First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 CO2 Capture by Absorption...

  14. absorption spectroscopy exafs: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption spectroscopy exafs First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Extended Xray Absorption...

  15. anomalous light absorption: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    anomalous light absorption First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Anomalous Light Absorption...

  16. absorption cross section: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption cross section First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 ? absorption cross sections...

  17. absorption line quasars: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption line quasars First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Quasar Absorption Lines...

  18. absorption spectroscopy studies: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption spectroscopy studies First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 On Automatic Absorption...

  19. absorption lines ii: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption lines ii First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 ABSORPTION LINE SURVEY OF H 3...

  20. absorption spectroscopic analysis: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption spectroscopic analysis First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 X-ray Absorption...

  1. absorption spectra: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption spectra First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Absorption Spectra of Astaxanthin...

  2. absorption line quasar: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption line quasar First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Quasar Absorption Lines...

  3. absorption process tcap: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption process tcap First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Two-photon Absorption Process...

  4. absorption line systems: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption line systems First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Clustering of absorption line...

  5. absorption band substructure: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption band substructure First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 THE ABSORPTION BAND EDGE...

  6. alpha absorption systems: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    absorption systems First Page Previous Page 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 Next Page Last Page Topic Index 1 Lyman alpha Absorption Systems and...

  7. Absorption of surface acoustic waves by topological insulator thin films

    SciTech Connect (OSTI)

    Li, L. L., E-mail: lllihfcas@foxmail.com [Key Laboratory of Materials Physics, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei 230031 (China); Xu, W., E-mail: wenxu-issp@aliyun.com [Key Laboratory of Materials Physics, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei 230031 (China); Department of Physics, Yunnan University, Kunming 650091 (China)

    2014-08-11T23:59:59.000Z

    We present a theoretical study on the absorption of the surface acoustic waves (SAWs) by Dirac electrons in topological insulator (TI) thin films (TITFs). We find that due to momentum and energy conservation laws, the absorption of the SAWs in TITFs can only be achieved via intra-band electronic transitions. The strong absorption can be observed up to sub-terahertz frequencies. With increasing temperature, the absorption intensity increases significantly and the cut-off frequency is blue-shifted. More interestingly, we find that the absorption of the SAWs by the TITFs can be markedly enhanced by the tunable subgap in the Dirac energy spectrum of the TI surface states. Such a subgap is absent in conventional two-dimensional electron gases (2DEGs) and in the gapless Dirac 2DEG such as graphene. This study is pertinent to the exploration of the acoustic properties of TIs and to potential application of TIs as tunable SAW devices working at hypersonic frequencies.

  8. Electromagnetically induced absorption due to transfer of coherence and to transfer of population

    SciTech Connect (OSTI)

    Goren, C.; Rosenbluh, M. [Department of Physics, Bar-Ilan University, Ramat Gan 52900 (Israel); Wilson-Gordon, A.D.; Friedmann, H. [Department of Chemistry, Bar-Ilan University, Ramat Gan 52900 (Israel)

    2003-03-01T23:59:59.000Z

    The absorption spectrum of a weak probe, interacting with a driven degenerate two-level atomic system, whose ground and excited hyperfine states are F{sub g,e}, can exhibit narrow peaks at line center. When the pump and probe polarizations are different, F{sub e}=F{sub g}+1 and F{sub g}>0, the electromagnetically induced absorption (EIA) peak has been shown to be due to the transfer of coherence (TOC) between the excited and ground states via spontaneous decay. We give a detailed explanation of why the TOC that leads to EIA (EIA-TOC) can only take place when ground-state population trapping does not occur, that is, when F{sub e}=F{sub g}+1. We also explain why EIA-TOC is observed in open systems. We show that EIA can also occur when the pump and probe polarizations are identical and F{sub e}=F{sub g}+1. This EIA is analogous to an effect that occurs in simple two-level systems when the collisional transfer of population (TOP) from the ground state to a reservoir is greater than that from the excited state. For a degenerate two-level system, the reservoir consists of the Zeeman sublevels of the ground hyperfine state, and of other nearby hyperfine states that do not interact with the pump. We will also discuss the four-wave mixing spectrum under the conditions where EIA-TOC and EIA-TOP occur.

  9. A wavelet analysis for the X-ray absorption spectra of molecules

    SciTech Connect (OSTI)

    Penfold, T. J. [Ecole polytechnique Federale de Lausanne, Laboratoire de spectroscopie ultrarapide, ISIC, FSB-BSP, CH-1015 Lausanne (Switzerland); Ecole polytechnique Federale de Lausanne, Laboratoire de chimie et biochimie computationnelles, ISIC, FSB-BCH, CH-1015 Lausanne (Switzerland); SwissFEL, Paul Scherrer Inst, CH-5232 Villigen (Switzerland); Tavernelli, I.; Rothlisberger, U. [Ecole polytechnique Federale de Lausanne, Laboratoire de chimie et biochimie computationnelles, ISIC, FSB-BCH, CH-1015 Lausanne (Switzerland); Milne, C. J.; Abela, R. [SwissFEL, Paul Scherrer Inst, CH-5232 Villigen (Switzerland); Reinhard, M.; Nahhas, A. El; Chergui, M. [Ecole polytechnique Federale de Lausanne, Laboratoire de spectroscopie ultrarapide, ISIC, FSB-BSP, CH-1015 Lausanne (Switzerland)

    2013-01-07T23:59:59.000Z

    We present a Wavelet transform analysis for the X-ray absorption spectra of molecules. In contrast to the traditionally used Fourier transform approach, this analysis yields a 2D correlation plot in both R- and k-space. As a consequence, it is possible to distinguish between different scattering pathways at the same distance from the absorbing atom and between the contributions of single and multiple scattering events, making an unambiguous assignment of the fine structure oscillations for complex systems possible. We apply this to two previously studied transition metal complexes, namely iron hexacyanide in both its ferric and ferrous form, and a rhenium diimine complex, [ReX(CO){sub 3}(bpy)], where X = Br, Cl, or ethyl pyridine (Etpy). Our results demonstrate the potential advantages of using this approach and they highlight the importance of multiple scattering, and specifically the focusing phenomenon to the extended X-ray absorption fine structure (EXAFS) spectra of these complexes. We also shed light on the low sensitivity of the EXAFS spectrum to the Re-X scattering pathway.

  10. Calculation of the spatial resolution in two-photon absorption spectroscopy applied to plasma diagnosis

    SciTech Connect (OSTI)

    Garcia-Lechuga, M. [Departamento de Física Teórica, Atómica y Óptica, Universidad de Valladolid, 47011-Valladolid (Spain); Laser Processing Group, Instituto de Óptica “Daza de Valdés,” CSIC, 28006-Madrid (Spain); Fuentes, L. M. [Departamento de Física Aplicada, Universidad de Valladolid, 47011-Valladolid (Spain); Grützmacher, K.; Pérez, C., E-mail: concha@opt.uva.es; Rosa, M. I. de la [Departamento de Física Teórica, Atómica y Óptica, Universidad de Valladolid, 47011-Valladolid (Spain)

    2014-10-07T23:59:59.000Z

    We report a detailed characterization of the spatial resolution provided by two-photon absorption spectroscopy suited for plasma diagnosis via the 1S-2S transition of atomic hydrogen for optogalvanic detection and laser induced fluorescence (LIF). A precise knowledge of the spatial resolution is crucial for a correct interpretation of measurements, if the plasma parameters to be analysed undergo strong spatial variations. The present study is based on a novel approach which provides a reliable and realistic determination of the spatial resolution. Measured irradiance distribution of laser beam waists in the overlap volume, provided by a high resolution UV camera, are employed to resolve coupled rate equations accounting for two-photon excitation, fluorescence decay and ionization. The resulting three-dimensional yield distributions reveal in detail the spatial resolution for optogalvanic and LIF detection and related saturation due to depletion. Two-photon absorption profiles broader than the Fourier transform-limited laser bandwidth are also incorporated in the calculations. The approach allows an accurate analysis of the spatial resolution present in recent and future measurements.

  11. Ultracold Atoms: How Quantum Field Theory Invaded Atomic Physics

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative1 First Use of Energy for All Purposes (Fuel and Nonfuel), 2002; Level:Energy: Grid Integration Redefining What'sis Taking Over OurThe Iron Spin TransitionProgram |Frank CasellaEnergyUltracold Atoms: How Quantum

  12. Engineering Atomic Quantum Reservoirs for Photons

    E-Print Network [OSTI]

    Susanne Pielawa; Luiz Davidovich; David Vitali; Giovanna Morigi

    2010-04-06T23:59:59.000Z

    We present protocols for creating entangled states of two modes of the electromagnetic field, by using a beam of atoms crossing microwave resonators. The atoms are driven by a transverse, classical field and pump correlated photons into (i) two modes of a cavity and (ii) the modes of two distant cavities. The protocols are based on a stochastic dynamics, characterized by random arrival times of the atoms and by random interaction times between atoms and cavity modes. The resulting effective model yields a master equation, whose steady state is an entangled state of the cavity modes. In this respect, the atoms act like a quantum reservoir, pulling the cavity modes into an entangled, Einstein-Podolski-Rosen (EPR) state, whose degree of entanglement is controlled by the intensity and the frequency of the transverse field. This scheme is robust against stochastic fluctuations in the atomic beam, and it does not require atomic detection nor velocity selection.

  13. Engineering Atomic Quantum Reservoirs for Photons

    E-Print Network [OSTI]

    Pielawa, Susanne; Vitali, David; Morigi, Giovanna

    2010-01-01T23:59:59.000Z

    We present protocols for creating entangled states of two modes of the electromagnetic field, by using a beam of atoms crossing microwave resonators. The atoms are driven by a transverse, classical field and pump correlated photons into (i) two modes of a cavity and (ii) the modes of two distant cavities. The protocols are based on a stochastic dynamics, characterized by random arrival times of the atoms and by random interaction times between atoms and cavity modes. The resulting effective model yields a master equation, whose steady state is an entangled state of the cavity modes. In this respect, the atoms act like a quantum reservoir, pulling the cavity modes into an entangled, Einstein-Podolski-Rosen (EPR) state, whose degree of entanglement is controlled by the intensity and the frequency of the transverse field. This scheme is robust against stochastic fluctuations in the atomic beam, and it does not require atomic detection nor velocity selection.

  14. atomic recoil laser: Topics by E-print Network

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Atomic Recoil Laser Quantum Physics (arXiv) Summary: We formulate a wave atom optics theory of the Collective Atomic Recoil Laser, where the atomic center-of-mass motion...

  15. Design of a dual species atom interferometer for space

    E-Print Network [OSTI]

    Thilo Schuldt; Christian Schubert; Markus Krutzik; Lluis Gesa Bote; Naceur Gaaloul; Jonas Hartwig; Holger Ahlers; Waldemar Herr; Katerine Posso-Trujillo; Jan Rudolph; Stephan Seidel; Thijs Wendrich; Wolfgang Ertmer; Sven Herrmann; André Kubelka-Lange; Alexander Milke; Benny Rievers; Emanuele Rocco; Andrew Hinton; Kai Bongs; Markus Oswald; Matthias Franz; Matthias Hauth; Achim Peters; Ahmad Bawamia; Andreas Wicht; Baptiste Battelier; Andrea Bertoldi; Philippe Bouyer; Arnaud Landragin; Didier Massonnet; Thomas Lévèque; Andre Wenzlawski; Ortwin Hellmig; Patrick Windpassinger; Klaus Sengstock; Wolf von Klitzing; Chris Chaloner; David Summers; Philip Ireland; Ignacio Mateos; Carlos F. Sopuerta; Fiodor Sorrentino; Guglielmo M. Tino; Michael Williams; Christian Trenkel; Domenico Gerardi; Michael Chwalla; Johannes Burkhardt; Ulrich Johann; Astrid Heske; Eric Wille; Martin Gehler; Luigi Cacciapuoti; Norman Gürlebeck; Claus Braxmaier; Ernst Rasel

    2014-12-08T23:59:59.000Z

    Atom interferometers have a multitude of proposed applications in space including precise measurements of the Earth's gravitational field, in navigation & ranging, and in fundamental physics such as tests of the weak equivalence principle (WEP) and gravitational wave detection. While atom interferometers are realized routinely in ground-based laboratories, current efforts aim at the development of a space compatible design optimized with respect to dimensions, weight, power consumption, mechanical robustness and radiation hardness. In this paper, we present a design of a high-sensitivity differential dual species $^{85}$Rb/$^{87}$Rb atom interferometer for space, including physics package, laser system, electronics and software. The physics package comprises the atom source consisting of dispensers and a 2D magneto-optical trap (MOT), the science chamber with a 3D-MOT, a magnetic trap based on an atom chip and an optical dipole trap (ODT) used for Bose-Einstein condensate (BEC) creation and interferometry, the detection unit, the vacuum system for $10^{-11}$ mbar ultra-high vacuum generation, and the high-suppression factor magnetic shielding as well as the thermal control system. The laser system is based on a hybrid approach using fiber-based telecom components and high-power laser diode technology and includes all laser sources for 2D-MOT, 3D-MOT, ODT, interferometry and detection. Manipulation and switching of the laser beams is carried out on an optical bench using Zerodur bonding technology. The instrument consists of 9 units with an overall mass of 221 kg, an average power consumption of 608 W (819 W peak), and a volume of 470 liters which would well fit on a satellite to be launched with a Soyuz rocket, as system studies have shown.

  16. Corona enhanced absorption of SO sub 2 /NO sub x

    SciTech Connect (OSTI)

    Dhali, S.K.

    1990-11-01T23:59:59.000Z

    This report contains results of an investigation of plasma-assisted oxidation of SO{sub 2} to SO{sub 3}. The SO{sub 3} is a more desirable by-product of flue gas than SO{sub 2} because it easily dissolves in water and can be reacted with lime to form gypsum. A coaxial dielectric-barrier discharge is used to generate an air plasma to carry out the reaction. The dielectric-barrier discharge,which is an interrupted discharge, is very efficient in producing atomic oxygen and requires a simple form of excitation. We have observed a significant reduction (over 75%) in the SO{sub 2} concentration using this technique. The simulation results indicate that about 99% of the SO{sub 2} can be oxidized with UV-irradiation along with plasma oxidation and that NO{sub x} can be reduced to N{sub 2} in the presence of an air plasma. The results of varying the gas composition, the gas pressure, and the gas flow are also reported. 18 refs., 8 figs.

  17. Cost reduction in absorption chillers: Phase 2

    SciTech Connect (OSTI)

    Leigh, R.W.

    1989-02-01T23:59:59.000Z

    A research program at Brookhaven National Laboratory (BNL) has addressed the possibility of dramatically lowering the first costs of absorption chillers through lowered material intensity and the use of lower cost materials, primarily in the heat exchangers which make up the bulk of the operating components of these systems. This must be done while retaining the best performance characteristics available today, a gross design point coefficient of performance (COP) of 1.3 and a net design (seasonal) average COP of 1.0 (0.90) in a directly fired, double effect unit. We have investigated several possible routes to these goals, and here report on these findings, focusing on the areas that appear most promising. The candidate technologies include the use of polymer film heat exchangers in several applications, the use of thin strips of new, corrosion resistant alloys to replace thicker, less impervious metals in applications exposed to gas flames, and copper or cupro-nickel foils in contact with system water. The use of such materials is only possible in the context of new heat exchanger and system designs, which are also discussed. To lend focus, we have concentrated on a directly fired double effect system providing capacity only. If successful, these techniques will also find wide applicability in heat pumps, cogeneration systems, solar cooling, heat recovery and chemical process heat transfer. 46 refs., 24 figs., 22 tabs.

  18. Generation to Generation: The Heart of Family Medicine

    E-Print Network [OSTI]

    Winter, Robin O

    2012-01-01T23:59:59.000Z

    Ageism in the Workplace. Generations Spring, 5. Westman,of caring for multiple generations simultaneously. StronglyGeneration to Generation: The Heart of Family Medicine

  19. Gamma ray generator

    DOE Patents [OSTI]

    Firestone, Richard B; Reijonen, Jani

    2014-05-27T23:59:59.000Z

    An embodiment of a gamma ray generator includes a neutron generator and a moderator. The moderator is coupled to the neutron generator. The moderator includes a neutron capture material. In operation, the neutron generator produces neutrons and the neutron capture material captures at least some of the neutrons to produces gamma rays. An application of the gamma ray generator is as a source of gamma rays for calibration of gamma ray detectors.

  20. Atomic Structure Calculations from the Los Alamos Atomic Physics Codes

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Cowan, R. D.

    The well known Hartree-Fock method of R.D. Cowan, developed at Los Alamos National Laboratory, is used for the atomic structure calculations. Electron impact excitation cross sections are calculated using either the distorted wave approximation (DWA) or the first order many body theory (FOMBT). Electron impact ionization cross sections can be calculated using the scaled hydrogenic method developed by Sampson and co-workers, the binary encounter method or the distorted wave method. Photoionization cross sections and, where appropriate, autoionizations are also calculated. Original manuals for the atomic structure code, the collisional excitation code, and the ionization code, are available from this website. Using the specialized interface, you will be able to define the ionization stage of an element and pick the initial and final configurations. You will be led through a series of web pages ending with a display of results in the form of cross sections, collision strengths or rates coefficients. Results are available in tabular and graphic form.