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1

COMPUTATIONAL MODELING, SYNTHESIS, AND CHARACTERIZATION OF BaZr1-xYxO3-8 SOLID STATE PROTON CONDUCTOR  

SciTech Connect (OSTI)

During the second semiannual period we have carried out a series of QM calculations on the BaZr{sub 1-x}Y{sub x}H{sub x}O{sub 3} proton conductor to determine the equilibrium proton positions and corresponding energies. We find that the size of the crystal cell is very important for the identification of the equilibrium proton positions. To derive ReaxFF parameters for Pt-surfaces and for H-transfer in Y-doped BaZrO{sub 3}, we carried out QM-calculations on the structures and energies of relevant condensed phases and cluster systems. These data then served as a training set to optimize the ReaxFF parameters. ReaxFF for various bulk metals (Pt, Zr, and Y) and metal clusters (Pt) was developed. BaZr{sub 1-x}Y{sub x}O{sub 3-{delta}} with x = 0.2, 0.3, 0.4, 0.5 was synthesized using a modified Pechini method and characterization (X-ray diffraction, scanning electron microscopy, and impedance spectroscopy) of this material was performed. We find that a single perovskite phase is formed in BaZr{sub 1-x}Y{sub x}O{sub 3-{delta}}. The proton conductivity of BaZr{sub 1-x}Y{sub x}O{sub 3-{delta}} with x = 0.5 is significantly lower than the conductivity of the samples with Y-dopant concentrations of 0.1 and 0.2.

Boris Merinov; Claudio O. Dorso; William A. Goddard III; Jian Wu; Sossina Haile

2003-10-30T23:59:59.000Z

2

Strong blue and white photoluminescence emission of BaZrO{sub 3} undoped and lanthanide doped phosphor for light emitting diodes application  

SciTech Connect (OSTI)

In this paper, we report the obtained strong broadband blue photoluminescence (PL) emission centered at 427 nm for undoped BaZrO{sub 3} observed after 266 nm excitation of submicron crystals prepared by hydrothermal/calcinations method. This emission is enhanced with the introduction of Tm{sup 3+} ions and is stronger than the characteristic PL blue emission of such lanthanide. The proposed mechanism of relaxation for host lattice emission is based on the presence of oxygen vacancies produced during the synthesis process and the charge compensation due to the difference in the electron valence between dopant and substituted ion in the host. Brilliant white light emission with a color coordinate of (x=0.29, y=0.32) was observed by combining the blue PL emission from the host with the green and red PL emission from Tb{sup 3+} and Eu{sup 3+} ions, respectively. The color coordinate can be tuned by changing the ratio between blue, green and red band by changing the concentration of lanthanides. - Graphical abstract: Strong blue emission from undoped BaZrO{sub 3} phosphor and white light emission by doping with Tb{sup 3+} (green) and Eu{sup 3+} (red) after 266 nm excitation. Highlights: Black-Right-Pointing-Pointer Blue emission from BaZrO{sub 3} phosphor. Black-Right-Pointing-Pointer Blue emission enhanced with Tm{sup 3+}. Black-Right-Pointing-Pointer White light from BaZrO{sup 3+} phosphor.

Romero, V.H. [Centro de Investigaciones en Optica, A. P. 1-948, Leon Gto., 37160 (Mexico)] [Centro de Investigaciones en Optica, A. P. 1-948, Leon Gto., 37160 (Mexico); De la Rosa, E., E-mail: elder@cio.mx [Centro de Investigaciones en Optica, A. P. 1-948, Leon Gto., 37160 (Mexico); Salas, P. [Centro de Fisica Aplicada y Tecnologia Avanzada, Universidad Nacional Autonoma de Mexico, A.P. 1-1010, Queretaro, Qro. 76000 (Mexico)] [Centro de Fisica Aplicada y Tecnologia Avanzada, Universidad Nacional Autonoma de Mexico, A.P. 1-1010, Queretaro, Qro. 76000 (Mexico); Velazquez-Salazar, J.J. [Department of Physics and Astronomy, The University of Texas at San Antonio One UTSA Circle, San Antonio TX 78249 (United States)] [Department of Physics and Astronomy, The University of Texas at San Antonio One UTSA Circle, San Antonio TX 78249 (United States)

2012-12-15T23:59:59.000Z

3

Cation ordering transformations in Ba(Mg{sub 1/3}Ta{sub 2/3})O{sub 3}-BaZrO{sub 3} perovskite solid solutions  

SciTech Connect (OSTI)

The effect of the substitution of BaZrO{sub 3} on the cation ordering in Ba(Mg{sub 1/3}Ta{sub 2/3})O{sub 3} was studied using TEM and X-ray and neutron diffraction. Almost no solubility of Zr was found in the 1:2 ordered, trigonal structure of the Ba(Mg{sub 1/3}Ta{sub 2/3})O{sub 3} end-member (P{bar 3}m1), and a transformation to a 1:1 ordered, cubic (Fm{bar 3}m) phase with a = 2a{sub per} occurs for substitution levels between {approximately}10 and 25 mol% BaZrO{sub 3}. The structure of this Ba({beta}{prime}{sub 1/2}{beta}{double_prime}{sub 1/2})O{sub 3}-type phase consists of two distinct octahedral sites, {beta}{prime} and {beta}{double_prime}. The occupancies of the two cation positions, refined using the Rietveld method, were found to be consistent with a random site model in which {beta}{double_prime} is occupied by Ta, and {beta}{prime} by a random distribution of the remaining cations. The homogeneity range of the 1:1 solid solutions predicted by this model, Ba{l_brace}[Mg{sub (2{minus}y)/3} Ta{sub (1{minus}2y)/3} Zr{sub y}]{sub 1/2}[Ta]{sub 1/2}{r_brace}O{sub 3} (0.0 < y {le} 0.5), is in excellent agreement with that observed experimentally.

Chai, L.; Akbas, M.A.; Davies, P.K. [Univ. of Pennsylvania, Philadelphia, PA (United States). Dept. of Materials Science and Engineering] [Univ. of Pennsylvania, Philadelphia, PA (United States). Dept. of Materials Science and Engineering; Parise, J.B. [Univ. of New York, Stony Brook, NY (United States). Dept. of Earth and Space Sciences] [Univ. of New York, Stony Brook, NY (United States). Dept. of Earth and Space Sciences

1997-09-01T23:59:59.000Z

4

Characterization of the reaction products that develop in the processing of Al{sub 2}O{sub 3}/BaZrO{sub 3} laminated composites  

SciTech Connect (OSTI)

The absence of a chemical reaction at an interface is conventionally thought to be an important criterion in producing a tough ceramic matrix composite (CMC). As a result of this criterion, interphases in CMCs were chosen on the basis of their chemical reactivity. A weak interface results in crack deflection, crack bridging, and, in fiber-reinforced ceramics, fiber pullout, resulting in an increased fracture toughness. In this paper, the authors present microstructural observations on alumina (Al{sub 2}O{sub 3})-barium zirconate (BaZrO{sub 3}) laminated composites wherein the reaction products that develop during processing resulted in sharp interfaces and appear to be weak enough to deflect cracks. These in situ reaction products in Al{sub 2}O{sub 3}-BaZrO{sub 3} laminated composites were characterized with the use of a scanning electron microscope, an electron microprobe, and a transmission electron microscope. The phases that develop, ZrO{sub 2}, BaO{center_dot}Al{sub 2}O{sub 3}, and BaO{center_dot}6 Al{sub 2}O{sub 3}, produced sharp interfaces and are arranged in a sequence that could be predicted by using information from the phase diagram.

Gladysz, G.M. [Youngstown State Univ., OH (United States). Dept. of Chemical Engineering] [Youngstown State Univ., OH (United States). Dept. of Chemical Engineering; Schmuecker, M.; Schneider, H. [German Aerospace Establishment, Cologne (Germany)] [German Aerospace Establishment, Cologne (Germany); Chawla, K.K. [Univ. of Alabama, Birmingham, AL (United States). Dept. of Materials and Mechanical Engineering] [Univ. of Alabama, Birmingham, AL (United States). Dept. of Materials and Mechanical Engineering; Joslin, D.L.; Ferber, M.K. [Oak Ridge National Lab., TN (United States)] [Oak Ridge National Lab., TN (United States)

1998-04-01T23:59:59.000Z

5

Symmetry determination on Pb-free piezoceramic 0.5Ba(Zr{sub 0.2}Ti{sub 0.8})O{sub 3}-0.5(Ba{sub 0.7}Ca{sub 0.3})TiO{sub 3} using convergent beam electron diffraction method  

SciTech Connect (OSTI)

(1?x)(Ba(Zr{sub 0.2}Ti{sub 0.8})O{sub 3}-x(Ba{sub 0.7}Ca{sub 0.3})TiO{sub 3} (BZT-xBCT) Pb-free piezoceramic has been reported showing ultrahigh piezoelectric performance in its morphotropic phase boundary (MPB) region. However, the crystal structure characteristic for the MPB composition of BZT-xBCT is still under debate—between single orthorhombic phase and tetragonal + rhombohedral two phase mixture. In the present study, we perform the local symmetry determination on the MPB composition x = 0.5 using convergent beam electron diffraction analysis (CBED). Our CBED results from multiple zone axes suggest that there are two coexisting phases with the point group symmetries of 4?mm (tetragonal) and 3?m (rhombohedral) respectively, which agree with two phase mixture model. The strong piezoelectricity can thus be understood by considering the polarization rotation between tetragonal and rhombohedral phases by external field.

Gao, Jinghui, E-mail: gaojinghui@mail.xjtu.edu.cn; Zhong, Lisheng [Multi-Disciplinary Materials Research Center, State Key Lab of Electrical Insulation and Power Equipment and Frontier Institute of Science and Technology, Xi'an, 710049 (China); Zhang, Lixue; Xue, Dezhen [Multi-Disciplinary Materials Research Center, State Key Lab of Electrical Insulation and Power Equipment and Frontier Institute of Science and Technology, Xi'an, 710049 (China); State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an 710049 (China); Kimoto, Takayoshi [Ferroic Physics Group, National Institute for Materials Science, Tsukuba, 305-0047, Ibaraki (Japan); Song, Minghui [Electron Microscopy Group, National Institute for Materials Science, Tsukuba, 305-0047, Ibaraki (Japan); Ren, Xiaobing [Multi-Disciplinary Materials Research Center, State Key Lab of Electrical Insulation and Power Equipment and Frontier Institute of Science and Technology, Xi'an, 710049 (China); State Key Laboratory for Mechanical Behavior of Materials, Xi'an Jiaotong University, Xi'an 710049 (China); Ferroic Physics Group, National Institute for Materials Science, Tsukuba, 305-0047, Ibaraki (Japan)

2014-02-07T23:59:59.000Z

6

A comparative study of SrO and BaO doping to CeO{sub 2}-ZrO{sub 2}: Characteristic and its catalytic performance for three-way catalysts  

SciTech Connect (OSTI)

Graphical abstract: Display Omitted Highlights: ? The prepared materials have a face-centered cubic structure and nanosize particles. ?Comparing to CZB, aged CZS has 494 ?mol/g of OSC and 30 m{sup 2}/g of surface area. ? CZS and CZB have similar NO sorption and reductive properties and different H{sub 2} uptake. ? T{sub 50} of Pt-Rh/CZS/LA is as low as 199 °C for CO, 228 °C for NO, and 252 °C for C{sub 3}H{sub 8}. ? Pt-Rh/CZS/LA has wider working-window at 320 °C under different ? value. -- Abstract: Ceria-zirconia-strontia (Ce{sub 0.35}Zr{sub 0.55}Sr{sub 0.10}O{sub 1.9}) and ceria-zirconia-baria (Ce{sub 0.35}Zr{sub 0.55}Ba{sub 0.10}O{sub 1.9}) were synthesized using an oxidation-co-precipitation method with hydrogen peroxide (H{sub 2}O{sub 2}) as oxidant. The physical and chemical properties of the prepared materials were investigated using Brunauer–Emmett–Teller surface area characterization, transmission electron microscopy, X-ray diffraction, Raman spectra, X-ray photoelectron spectroscopy, and oxygen pulse reaction. The prepared materials were used in preparing three-way catalysts with low Pt and Rh content. Moreover, catalytic activities were evaluated at a fixed bed under a simulated gaseous mixture. The results are as follows: (1) the prepared materials have a face-centered cubic structure and are nano-sized; (2) aged Ce{sub 0.35}Zr{sub 0.55}Sr{sub 0.10}O{sub 1.9} has higher oxygen storage capacity (494 ?mol/g), better thermal stability (30 m{sup 2}/g), good low-temperature reducibility, and high hydrogen uptake after TPR-redox cycles; (3) the light-off temperature (T{sub 50}) of Pt-Rh/CZS/LA can be as low as 199 °C for CO, 228 °C for NO, and 252 °C for C{sub 3}H{sub 8}; and (4) Pt-Rh/CZS/LA has a fairly wide working-window.

Guo, Jiaxiu, E-mail: guojiaxiu@scu.edu.cn [College of Architecture and Environment, Sichuan University, Chengdu 610065 (China) [College of Architecture and Environment, Sichuan University, Chengdu 610065 (China); National Engineering Research Center for Flue Gas Desulfurization, Chengdu 610065 (China); Shi, Zhonghua, E-mail: shizhonghua@scu.edu.cn [College of Chemistry, Sichuan University, Chengdu 610064 (China)] [College of Chemistry, Sichuan University, Chengdu 610064 (China); Wu, Dongdong [College of Chemistry, Sichuan University, Chengdu 610064 (China)] [College of Chemistry, Sichuan University, Chengdu 610064 (China); Yin, Huaqiang [College of Architecture and Environment, Sichuan University, Chengdu 610065 (China) [College of Architecture and Environment, Sichuan University, Chengdu 610065 (China); National Engineering Research Center for Flue Gas Desulfurization, Chengdu 610065 (China); Gong, Maochu [College of Chemistry, Sichuan University, Chengdu 610064 (China)] [College of Chemistry, Sichuan University, Chengdu 610064 (China); Chen, Yaoqiang [College of Chemistry, Sichuan University, Chengdu 610064 (China) [College of Chemistry, Sichuan University, Chengdu 610064 (China); National Engineering Research Center for Flue Gas Desulfurization, Chengdu 610065 (China)

2013-02-15T23:59:59.000Z

7

Anode-supported tubular SOFCs based on BaZr0.1Ce0.7Y0.1Yb0.1O3?? electrolyte fabricated by dip coating  

SciTech Connect (OSTI)

Anode-supported tubular solid oxide fuel cells (SOFCs) based on a proton and oxide ion mixed conductor, BaZr{sub 0.1}Ce{sub 0.7}Y{sub 0.1}Yb{sub 0.1}O{sub 3 ? ?} (BZCYYb), have been fabricated using a dip coating and co-firing process. This new fabrication technique effectively reduced the Ohmic resistances of tubular cells to ~ 0.1 and ~ 0.3 ? cm{sup 2} at 750 and 600 °C, respectively. Typical tubular cells with Ni-BZCYYb anode, BZCYYb electrolyte, and La{sub 0.6}Sr{sub 0.4}Co{sub 0.2}Fe{sub 0.8}O{sub 3 ? ?} (LSCF)-BZCYYb composite cathode demonstrated much-improved performance, achieving peak power densities of 1.13, 0.81, 0.63, and 0.53 W cm{sup ? 2} at 750, 700, 650, and 600 °C, respectively, when humidified (3 v% water vapor) hydrogen was used as fuel and ambient air as oxidant.

Chen, Changcheng; Liu, Mingfei; Bai, Yaohui; Yang, Lei; Xie, Erqing; Liu, Meilin

2011-01-01T23:59:59.000Z

8

Preparation and dielectric properties of Ba{sub 0.95}Ca{sub 0.05}Ti{sub 0.8}Zr{sub 0.2}O{sub 3}-polyethersulfone composites  

SciTech Connect (OSTI)

We report the preparation and dielectric properties of ceramic-polymer composites using Ba{sub 0.95}Ca{sub 0.05}Ti{sub 0.8}Zr{sub 0.2}O{sub 3} (BCTZ) as a ceramic filler and polyethersulfone (PES) as a polymer matrix. The BCTZ powders were synthesized by a sol-gel method to fabricate BCZT-PES composites. The composites with various BCTZ volume fractions were prepared by a solution mixing and hot-pressing method. The composite with 50 vol % BCTZ showed high dielectric constant ({epsilon}=48.80) and low loss (tan {delta}=0.042) at 1 kHz and room temperature. Such excellent dielectric properties of the composites displayed an acceptable stability within a wide range of temperature (from 20 to 150 deg. C) and frequency (from 100 Hz to 100 kHz). The present work indicates that the BCTZ-PES composite can be a candidate for embedded capacitors.

Wang Fajun; Li Wen; Jiang Hongliu; Xue Mingshan; Lu Jinshan; Yao Junping [School of Materials Science and Engineering, Nanchang Hangkong University, Nanchang 330063 (China)

2010-02-15T23:59:59.000Z

9

Strong Enhancement of Flux Pinning in YBa2Cu3O7-? Multilayers with Columnar Defects Comprised of Self-Assembled BaZrO3  

SciTech Connect (OSTI)

Multilayer structures comprising YBa{sub 2}Cu{sub 3}O{sub 7-{delta}} (YBCO) films with columns of self-assembled BaZrO{sub 3} (BZO) nanodots with interlayers of CeO{sub 2} or pure YBa{sub 2}Cu{sub 3}O{sub 7-{delta}} were grown on rolling-assisted biaxially textured substrates (RABiTSs) using pulsed laser deposition. A significant enhancement of the critical current density (J{sub c}) was observed for the multilayers compared with a single layer of YBCO + BZO. J{sub c} varies as J{sub c}{approx}H{sup -{alpha}} with a of 0.27 for single layer of YBCO + BZO and 0.34 for both multilayered films. Enhancement of pinning in the multilayers is attributed to the presence of columnar defects comprised of self-assembled nanodots of BZO as well as planar CuO-type stacking defects arising as a result of interfacial reactions in the multilayers.

Kang, Sukill [ORNL; Leonard, Keith J [ORNL; Martin, Patrick M [ORNL; Li, Jing [ORNL; Goyal, Amit [ORNL

2007-01-01T23:59:59.000Z

10

WUSM RA Forum Grants & Contracts  

E-Print Network [OSTI]

1 WUSM RA Forum March 2006 Grants & Contracts #12;2 NIH Update #12;3 Beginning February 1, 2006, National Institute of Health (NIH) will stop sending summary statements and Peer Review Outcome letter NIH eRA Commons #12;4 Advantages to Registering in the NIH eRA Commons: · The NIH eRA Commons

Kroll, Kristen L.

11

Co.ra  

Office of Legacy Management (LM)

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12

Domain wall motion and electromechanical strain in lead-free piezoelectrics: Insight from the model system (1 ? x)Ba(Zr{sub 0.2}Ti{sub 0.8})O{sub 3}–x(Ba{sub 0.7}Ca{sub 0.3})TiO{sub 3} using in situ high-energy X-ray diffraction during application of electric fields  

SciTech Connect (OSTI)

The piezoelectric compositions (1 ? x)Ba(Zr{sub 0.2}Ti{sub 0.8})O{sub 3}–x(Ba{sub 0.7}Ca{sub 0.3})TiO{sub 3} (BZT-xBCT) span a model lead-free morphotropic phase boundary (MPB) between room temperature rhombohedral and tetragonal phases at approximately x?=?0.5. In the present work, in situ X-ray diffraction measurements during electric field application are used to elucidate the origin of electromechanical strain in several compositions spanning the tetragonal compositional range 0.6???x???0.9. As BCT concentration decreases towards the MPB, the tetragonal distortion (given by c/a-1) decreases concomitantly with an increase in 90° domain wall motion. The increase in observed macroscopic strain is predominantly attributed to the increased contribution from 90° domain wall motion. The results demonstrate that domain wall motion is a significant factor in achieving high strain and piezoelectric coefficients in lead-free polycrystalline piezoelectrics.

Tutuncu, Goknur [Department of Materials Science and Engineering, University of Florida, Gainesville, Florida 32611 (United States); Li, Binzhi [Department of Chemical Engineering and Materials Science, University of California, Davis, Davis, California 95616 (United States); Bowman, Keith [Illinois Institute of Technology, Armour College of Engineering, Chicago, Illinois 60616 (United States); School of Materials Engineering, Purdue University, West Lafayette, Indiana 47907 (United States); Jones, Jacob L., E-mail: JacobJones@ncsu.edu [Department of Materials Science and Engineering, North Carolina State University, Raleigh, North Carolina 27695 (United States)

2014-04-14T23:59:59.000Z

13

RA  

National Nuclear Security Administration (NNSA)

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14

eRA Training Team1 Terminations  

E-Print Network [OSTI]

eRA Training Team1 xTrain Terminations Electronic Research Administration Sponsored by: The National Institutes of Health, Office of Extramural Research March 2012 #12;eRA Training Team2 xTrain General Information xTrain Overview The following section provides general information on the xTrain

Baker, Chris I.

15

eRA Training Team1 Terminations  

E-Print Network [OSTI]

eRA Training Team1 xTrain Terminations Electronic Research Administration Sponsored by: The National Institutions of Health, Office of Extramural Research April 2010 #12;eRA Training Team2 xTrain General Information xTrain Overview The following section provides general information on the xTrain

Baker, Chris I.

16

The analysis of Ytrium doped BaZrO3  

Office of Scientific and Technical Information (OSTI)

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17

RAPID METHOD FOR DETERMINATION OF {sup 228}Ra IN WATER SAMPLES  

SciTech Connect (OSTI)

A new rapid method for the determination of {sup 228}Ra in natural water samples has been developed at the SRNL/EBL (Savannah River National Lab/ Environmental Bioassay Laboratory) that can be used for emergency response or routine samples. While gamma spectrometry can be employed with sufficient detection limits to determine {sup 228}Ra in solid samples (via {sup 228}Ac) , radiochemical methods that employ gas flow proportional counting techniques typically provide lower MDA (Minimal Detectable Activity) levels for the determination of {sup 228}Ra in water samples. Most radiochemical methods for {sup 228}Ra collect and purify {sup 228}Ra and allow for {sup 228}Ac daughter ingrowth for ~36 hours. In this new SRNL/EBL approach, {sup 228}Ac is collected and purified from the water sample without waiting to eliminate this delay. The sample preparation requires only about 4 hours so that {sup 228}Ra assay results on water samples can be achieved in < 6 hours. The method uses a rapid calcium carbonate precipitation enhanced with a small amount of phosphate added to enhance chemical yields (typically >90%), followed by rapid cation exchange removal of calcium. Lead, bismuth, uranium, thorium and protactinium isotopes are also removed by the cation exchange separation. {sup 228}Ac is eluted from the cation resin directly onto a DGA Resin cartridge attached to the bottom of the cation column to purify {sup 228}Ac. DGA Resin also removes lead and bismuth isotopes, along with Sr isotopes and {sup 90}Y. La is used to determine {sup 228}Ac chemical yield via ICP-MS, but {sup 133}Ba can also be used instead if ICP-MS assay is not available. Unlike some older methods, no lead or strontium holdback carriers or continual readjustment of sample pH is required.

Maxwell, S.

2012-09-05T23:59:59.000Z

18

Nuclear fusion as a probe for octupole deformation in $^{224}$Ra  

E-Print Network [OSTI]

$\\textit{Background}$: Nuclear fusion has been shown to be a perfect probe to study the different nuclear shapes. However, the possibility of testing octupole deformation of a nucleus with this tool has not been fully explored yet. The presence of a stactic octupole deformation in nuclei will enhanced a possible permanent electric dipole moment, leading to a possible demonstration of parity violation. $\\textit{Purpose}$: To check whether static octupole deformation or octupole vibration in fusion give qualitatively different results so that both situations can be experimentally disentangled. $\\textit{Method}$: Fusion cross sections are computed in the Coupled-Channels formalism making use of the Ingoing-Wave Boundary Conditions (IWBC) for the systems $^{16}$O+$^{144}$Ba and $^{16}$O+$^{224}$Ra. $\\textit{Results}$: Barrier distributions of the two considered schemes show different patterns. For the $^{224}$Ra case, the octupole deformation parameter is large enough to create a sizeable difference. $\\textit{Con...

Kumar, Raj; Vitturi, A

2015-01-01T23:59:59.000Z

19

(RA) Gila's Departments (RA) Jena's Departments BK Anesthesiology LN Biomedical Engineering  

E-Print Network [OSTI]

(RA) Gila's Departments (RA) Jena's Departments BK Anesthesiology LN Biomedical Engineering JC Biochemistry & Biophysics JC Biostatistics & Computational Biology BK Biomedical Genetics BK Brain & Cognitive Development & Disease AC Center for Oral Biology LN Center for Primary Care AB Center for Pediatric Biomedical

Mahon, Bradford Z.

20

Ra-226 radioassay of soil and tailings  

SciTech Connect (OSTI)

Studies of inactive uranium tailings piles have shown that tailings sands containing Ra-226 and other radionuclides may be dispersed by wind and water erosion, causing contamination of adjacent areas. To conduct an effective cleanup operation, it is necessary that boundaries of contamination be well defined. To accomplish this, data from surface gamma-ray surveys made under the Measurement Monitoring Program of the US DOE's Uranium Mill Tailings Remedial Action Project (UMTRAP) are first used to delineate a general outline of the contaminated area. Then, data from portable scintillometer surveys and from sealed-can gamma-ray analyses of soil samples are used to more precisely define the perimeter of Ra-226 contamination. These field measurements are supported by radiochemical analyses of randomly selected samples. Because of its adaptability to the widely varying chemical composition of the material in these samples, the complexing agent EDTA is used in a complexometric leaching procedure to analyze Ra-226. By this procedure, natural concentrations of Ra-226 in soil (approx. 1 pCi/g) can be measured routinely. The potential limit of detection is in the 0.1 to 0.5 pCi/g range. Details of the method, which includes leaching of radium followed by radon de-emanation, are described. Comparative data for various soil and tailings samples are presented.

Sabau, C.S.; Rayno, D.R.; Kretz, N.D.; Zelle, P.W.

1983-01-01T23:59:59.000Z

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21

Giant anelastic responses in (BaZrO -ZnO)-BaTiO  

E-Print Network [OSTI]

in the case of ceramic matrix composites which are usually synthesized via the solid-state reaction method. Porous interface and its brittleness nature are inevitable drawbacks for ceramic matrix composites, no experimental report is available (a)E-mail: lakes@engr.wisc.edu on ceramic matrix composites with negative

Lakes, Roderic

22

BA War & Society Module Information  

E-Print Network [OSTI]

BA War & Society Module Information 2014-2015 www.swansea.ac.uk/artsandhumanities Arts Studies BA War & Society BA War & Society The scope and scale of the BA (Hons) War and Society degree Theories of War 1 (compulsory) HUA102 War and Warfare in the Modern World (compulsory) HIH118 World History

Harman, Neal.A.

23

Galactic Evolution of Sr, Y, Zr: A Multiplicity of Nucleosynthetic Processes  

E-Print Network [OSTI]

We follow the Galactic enrichment of three easily observed light n-capture elements Sr,Y,and Zr.Input stellar yields have been first separated into their respective main and weak s-process,and r-process components.The s-process yields from AGB stars are computed,exploring a wide range of efficiencies of the major neutron source,13C,and covering both disk and halo metallicities.AGBs have been shown to reproduce the main s-component in the solar system.The concurrent weak s-process,which accounts for the major fraction of the light s-process isotopes in the solar system and occurs in massive stars by the operation of the 22Ne n-source,is discussed in detail.Neither the main s-,nor the weak s-components are shown to contribute significantly to the n-capture element abundances observed in unevolved halo stars.We present a detailed analysis of a large database of spectroscopic observations of Sr,Y,Zr, Ba,and Eu for Galactic stars at various metallicities.Spectroscopic observations of Sr,Y,and Zr to Ba and Eu abundance ratios versus metallicity provide useful diagnostics of the types of n-capture processes forming Sr,Y and Zr.The observed [Sr,Y,Zr/Ba,Eu] ratio is clearly not flat at low metallicities,as we would expect if Ba,Eu and Sr,Y,Zr all had the same r-process origin.We discuss our chemical evolution predictions, taking into account the interplay between different processes to produce Sr-Y-Zr.We find hints for a primary process in low-metallicity massive stars, different from the 'classical s-process' and from the 'classical r-process',that we tentatively define LEPP (Lighter Element Primary Process).This allows us to revise the estimates of the r-process contributions to the solar Sr,Y and Zr abundances,as well as of the contribution to the s-only isotopes 86Sr,87Sr,96Mo.

Claudia Travaglio; Roberto Gallino; Enrico Arnone; John Cowan; Faith Jordan; Chris Sneden

2003-10-07T23:59:59.000Z

24

R.A. Spicer -Publications. January, 2010 1 R.A. Spicer Publications -Articles, Papers and Books  

E-Print Network [OSTI]

2 108. Spicer, R.A., Ahlberg, A., Herman, A.B., Hofmann, C-C., Raikevich, M., Valdes, P -de Leon, M.P., Spicer, R.A., and Steart, D.C., In Press. Climatic reconstruction of two Pliocene Yakutia). Palaeogeography, Palaeoclimatolgy, Palaeoecology, 111. Moiseeva, M.G., Herman, A.B., and Spicer

Spicer, Robert A

25

Phase transformations in Cu-Zr multilayers  

SciTech Connect (OSTI)

A study of phase transformations is reported for Cu-rich, Cu-Zr multilayer foils synthesized using magnetron sputter deposition and annealed using a differential scanning calorimeter. The foils range in composition from 1.6 to 9.0 at% Zr and consist of alternate layers of polycrystalline Cu and Zr. Differential scanning calorimetry, X-ray analysis and electron microscopy were used to three distinct reactions in the foils: a mixing and an amorphization of the Cu and die Zr, a crystallization on of this amorphous phase to the metastable intermetallic Cu{sub 5l}Zr{sub l4}, and a transformation of the Cu{sub 5l}Zr{sub l4} phase into the equilibrium phase Cu{sub 9}Zr{sub 2}. The as-deposited layering remained stable during the first two reactions and then broke down in the third reaction as large grains of Cu{sub 9}Zr{sub 2} encompassed the smaller Cu grains. Heats of the reactions and activation energies of these reactions are measured and are compared to values reported for bulk samples. The measured heats provide evidence that amorphous Cu-Zr alloys phase separate and that mixing and short range ordering produce 3.5 times more heat than long range ordering produces when Ca and Zr react and form Cu{sub 5l}Zr{sub l4}.

Weihs, T.P.; Barbee, T.W. Jr.; Wall, M.A.

1993-04-01T23:59:59.000Z

26

RAPID DETERMINATION OF RA-226 IN ENVIRONMENTAL SAMPLES  

SciTech Connect (OSTI)

A new rapid method for the determination of {sup 226}Ra in environmental samples has been developed at the Savannah River Site Environmental Lab (Aiken, SC, USA) that can be used for emergency response or routine sample analyses. The need for rapid analyses in the event of a Radiological Dispersive Device or Improvised Nuclear Device event is well-known. In addition, the recent accident at Fukushima Nuclear Power Plant in March, 2011 reinforces the need to have rapid analyses for radionuclides in environmental samples in the event of a nuclear accident. {sup 226}Ra (T1/2 = 1,620 years) is one of the most toxic of the long-lived alpha-emitters present in the environment due to its long life and its tendency to concentrate in bones, which increases the internal radiation dose of individuals. The new method to determine {sup 226}Ra in environmental samples utilizes a rapid sodium hydroxide fusion method for solid samples, calcium carbonate precipitation to preconcentrate Ra, and rapid column separation steps to remove interferences. The column separation process uses cation exchange resin to remove large amounts of calcium, Sr Resin to remove barium and Ln Resin as a final purification step to remove {sup 225}Ac and potential interferences. The purified {sup 226}Ra sample test sources are prepared using barium sulfate microprecipitation in the presence of isopropanol for counting by alpha spectrometry. The method showed good chemical recoveries and effective removal of interferences. The determination of {sup 226}Ra in environmental samples can be performed in less than 16 h for vegetation, concrete, brick, soil, and air filter samples with excellent quality for emergency or routine analyses. The sample preparation work takes less than 6 h. {sup 225}Ra (T1/2 = 14.9 day) tracer is used and the {sup 225}Ra progeny {sup 217}At is used to determine chemical yield via alpha spectrometry. The rapid fusion technique is a rugged sample digestion method that ensures that any refractory radium particles are effectively digested. The preconcentration and column separation steps can also be applied to aqueous samples with good results.

Maxwell, S.

2012-01-03T23:59:59.000Z

27

Intermediate Major Full Major BUSIBA.I Intmd Business BA ARTHBA Art History BA  

E-Print Network [OSTI]

Studies HBS GEOSBS Geoscience BSG ESS.BA Exercise & Sport Sci BA GEOSHBS Geoscience HSG ESS.BS Exercise & Sport Sci BS GERMBA German BA ESS.HBS Exercise & Sport Sci HBS GERMHBA German HBA ESS.BS.T Exercise

Tipple, Brett

28

Simulation of Heat Treatment Distortion R.A. Hardin1  

E-Print Network [OSTI]

quenched in water and in oil. Unfortunately, due to the lack of documentation on the heat treatment processSimulation of Heat Treatment Distortion R.A. Hardin1 and C. Beckermann2 1 Research Engineer, 2 Abstract This paper gives an overview of the problem of heat treatment stress and distortion and a review

Beckermann, Christoph

29

NEWS & VIEWS X-RaY oPtiCS  

E-Print Network [OSTI]

NEWS & VIEWS X-RaY oPtiCS Clarity through a keyhole Janos Hajdu1,2 & Filipe R. n. C. maia2 are at 1 Stanford Synchrotron Radiation Laboratory, Stanford Linear Accelerator Center, 2575 Sand Hill Road, Menlo, as it does in conventional crystallography, but only on the wavelength used, the extent of ionization damage

Loss, Daniel

30

Audit Report: OAS-RA-L-13-01 | Department of Energy  

Energy Savers [EERE]

RA-L-13-01 Audit Report: OAS-RA-L-13-01 November 1, 2012 Implementation of the Department of Energy's Concentrating Solar Power Program The Department of Energy's (Department)...

31

BA Philosophy, Politics and Law  

E-Print Network [OSTI]

BA Philosophy, Politics and Law (PPL) Module Information 2013-2014 Arts and Humanities College of www.swansea.ac.uk/artsandhumanities Department of Politcial and Cultural Studies #12;PPL at Swansea Swansea offers one of only two PPL degrees in the UK. Building on the successfully launch of our PPE

Harman, Neal.A.

32

Bremsstrahlung emission during $?$-decay of $^{226}{\\rm Ra}$  

E-Print Network [OSTI]

We obtained the spectrum of probability of the bremsstrahlung emission accompanying the $\\alpha$-decay of $^{226}{\\rm Ra}$ (E$_{\\alpha}$=4.8 MeV) by measuring the $\\alpha$-$\\gamma$ coincidences and using the model presented in our previous study on the $\\alpha-$decay of $^{214}{\\rm Po}$ (E$_{\\alpha}$=7.7 MeV). We compare the experimental data with the quantum mechanical calculation and find a good agreement between theory and experiment. We discuss the differences between the photon spectra connected with the $\\alpha$-decay of the $^{226}{\\rm Ra}$ and $^{214}{\\rm Po}$ nuclei. For the two mentioned nuclei we analyze the bremsstrahlung emission contributions from the tunneling and external regions of the nucleus barrier into the total spectrum, and we find the destructive interference between these contributions. We also find that the emission of photons during tunneling of the $\\alpha$-particle gives an important contribution to the bremsstrahlung spectrum in the whole E$_{\\gamma}$ energy range of the studied $^{226}$Ra nucleus.

Giorgio Giardina; Giovanni Fazio; Giuseppe Mandaglio; Marina Manganaro; Serghei P. Maydanyuk; Vladislav S. Olkhovsky; Nikolay V. Eremin; Anton A. Paskhalov; Dmitry A. Smirnov; Carmelo Sacca

2008-04-16T23:59:59.000Z

33

Octupole collectivity in $^{220}$Rn and $^{224}$Ra  

E-Print Network [OSTI]

Collective properties of the radioactive nuclei $^{220}$Rn and $^{224}$Ra have been studied via Coulomb excitation of a $2.8$~A.MeV radioactive ion beam (RIB) incident upon $^{60}$Ni, $^{112,114}$Cd and $^{120}$Sn targets. The experiments took place at the REX-ISOLDE RIB facility, CERN. De-excitation $gamma$-ray yields following multiple-step Coulomb excitation were detected in coincidence with recoiling target nuclei in the Miniball spectrometer. For the first time, $B(E3;3^{+} ightarrow0^{+})$ values have been directly measured with a radioactive ion beam. In the process, $^{224}$Ra becomes the heaviest post-accelerated RIB to date at ISOLDE (with the possible exception of the quasi-stable $^{238}$U). The measurements presented in this thesis represent a tripling of the number of nuclei around $Zsimeq88$ and $Nsimeq134$, for which direct measurements of the octupole collectivity have been performed. The only previous measurements being for the relatively long-lived $^{226}$Ra. The $gamma$-ray yields, in con...

Gaffney, Liam Paul

34

Enhanced pinning in YBCO films with BaZrO3 nanoparticles  

DOE Patents [OSTI]

A process and composition of matter are provided and involve flux pinning in thin films of high temperature superconductive oxides such as YBCO by inclusion of particles including barium and a group 4 or group 5 metal, such as zirconium, in the thin film.

Driscoll, Judith L.; Foltyn, Stephen R.

2010-06-15T23:59:59.000Z

35

Superlattice Structure and Precipitates in O+ and Zr+ Ion Coimplanted...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

and Zr+ Ion Coimplanted SrTiO3: a Model Waste Form for 90Sr. Abstract: We investigate strontium titanate as a model waste form for 90Sr. Implantation with O+ and Zr+ ions, followed...

36

The Bayo Canyon/radioactive lanthanum (RaLa) program  

SciTech Connect (OSTI)

LANL conducted 254 radioactive lanthanum (RaLa) implosion experiments Sept. 1944-March 1962, in order to test implosion designs for nuclear weapons. High explosives surrounding common metals (surrogates for Pu) and a radioactive source containing up to several thousand curies of La, were involved in each experiment. The resulting cloud was deposited as fallout, often to distances of several miles. This report was prepared to summarize existing records as an aid in evaluating the off-site impact, if any, of this 18-year program. The report provides a historical setting for the program, which was conducted in Technical Area 10, Bayo Canyon about 3 miles east of Los Alamos. A description of the site is followed by a discussion of collateral experiments conducted in 1950 by US Air Force for developing an airborne detector for tracking atmospheric nuclear weapons tests. All known off-site data from the RaLa program are tabulated and discussed. Besides the radiolanthanum, other potential trace radioactive material that may have been present in the fallout is discussed and amounts estimated. Off-site safety considerations are discussed; a preliminary off-site dose assessment is made. Bibliographical data on 33 persons important to the program are presented as footnotes.

Dummer, J.E.; Taschner, J.C.; Courtright, C.C.

1996-04-01T23:59:59.000Z

37

BA Economics and BA Financial Economics Assessment Plan Program Learning Objectives  

E-Print Network [OSTI]

BA Economics and BA Financial Economics ­ Assessment Plan Program Learning Objectives The program will prepare graduates: 1. Understand the "economic way model economic decisions. 3. The ability to analyze historical and current events

Cantlon, Jessica F.

38

BaBar: Direct CPV Searches  

SciTech Connect (OSTI)

Some recent BaBar measurements of CP-violation charge asymmetries in B meson decays to charmless hadronic final states are presented.

Mir, L.M.; /LBL, Berkeley

2006-04-14T23:59:59.000Z

39

NOx Storage-Reduction Characteristics of Ba-Based Lean NOx Trap Catalysts Subjected to Simulated Road Aging  

SciTech Connect (OSTI)

Although Lean NO{sub x} Trap (LNT) catalyst technology has made significant strides in recent years, the issue of LNT durability remains problematic. Following on from our previous research concerning the effect of ceria addition on LNT preformance, in this study we focus on the role of ceria in ameliorating the deterioration of Ba-based LNT catalysts during aging. Indeed, we have observed that spectacular improvements in LNT durability can be achieved through the incorporation of CeO{sub 2}-ZrO{sub 2} into the LNT formulation, and, to a lesser extent, La-stabilized ceria.

Ji, Yaying [University of Kentucky; Fisk, Courtney [University of Kentucky; Easterling, Vencon [University of Kentucky; Graham, Uschi [University of Kentucky; Poole, Adam [University of Kentucky; Crocker, Mark [University of Kentucky; Choi, Jae-Soon [ORNL; Partridge Jr, William P [ORNL; Wilson, Karen [University of York, UK

2010-01-01T23:59:59.000Z

40

Academic Affairs Multidisciplinary Studies (BA) B700  

E-Print Network [OSTI]

of Architecture Architecture­5 year program (B Arch) B045 Architecture­Pre-Arch (BS in Env Des) B386 Construction Studies (BA) B875 College of Atmospheric & Geographic Sciences Environmental Sustainability (BA in Env Sustainability) Culture and Society B408 P161 Planning and Management B408 P516 Science and Natural Resources B

Oklahoma, University of

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


41

Setembro de 2014 Salvador/BA  

E-Print Network [OSTI]

PRĂ?-ANAIS Setembro de 2014 Salvador/BA 16 a 19SIMPĂ?SIO BRASILEIRO DE PESQUISA OPERACIONALSIMPĂ?SIO; Manufacturing systems. Main area: MP - Probabilistic Models #12;PRĂ?-ANAIS Setembro de 2014 Salvador/BA 16 a 19

Cruz, Frederico

42

Philosophy Honours (& BA Humanities and Social Science)  

E-Print Network [OSTI]

Philosophy Honours Handbook (& BA Humanities and Social Science) 2012/2013 Philosophy School of Philosophy, Psychology and Language Sciences University of Edinburgh #12;1 Philosophy Honours Handbook (& BA.......................................... 13 #12;2 1. Resources for Philosophy A complete list of the full-time academic staff in Philosophy

Edinburgh, University of

43

A correlation between soil descriptions and {sup 226}Ra concentrations in Florida soils  

SciTech Connect (OSTI)

The soil radium content in Florida is highly variable. The range in radium concentrations, where the samples involved in this study are concerned, is from 0.1 pCi/g to 18.5 pCi/g. Low {sup 226}Ra concentrations (0.1 to 5 pCi/g) are evidenced in sands, moderate concentrations (5 to 11 pCi/g) are found in silt and gravel, and high {sup 226}Ra concentrations (>11 pCi/g) are found in soil horizons with shell, clay, and strata with phosphate. Strata containing phosphate yields a high concentration of {sup 226}Ra. The information obtained in this study, soil descriptions with their corresponding {sup 226}Ra concentrations, comes from geological cores drilled by geotechnical consultants with gamma spectrometry analysis performed by high resolution gamma spectroscopy. Concentration; of {sup 226}Ra generally increase with depth. These cores are usually terminated at 20 feet deep, with some cores being shallower than this due to hitting bedrock or encountering the water table. These frequency distributions give the core-logging geologist an approximate concentration of {sup 226}Ra based on the description of the soil. Since the correlation of {sup 226}Ra and soil descriptions can be used as a tool in assigning indoor radon potential, this study is of importance to land managers, contractors, developers, and regulating agencies who are attempting to place standards on tracts of land with {sup 226}Ra concentration used as a criterion.

Harrison, D.P.

1992-12-31T23:59:59.000Z

44

Octupole deformation and Ra puzzle in reflection asymmetric covariant density functional theory  

E-Print Network [OSTI]

Reflection asymmetric covariant density functional theory(CDFT) based on the point-coupling interaction is established on a two-center harmonic-oscillator basis and applied to investigate the Ra puzzle, i.e., the anomalous enhancement of the residual proton-neutron interactions for Ra isotopes around N=135. The octupole deformation and shape evolution in the Ra and Rn isotopes are examined in the potential energy surfaces in(beta2, beta3) plane by the constrained reflection asymmetric calculations. The residual proton-neutron interactions extracted from the double difference of the binding energies for Ra isotopes are compared with the data as well as the axial and the triaxial calculations. It is found that the octupole deformation is responsible for the Ra puzzle in the microscopic CDFT.

L. F. Yu; P. W. Zhao; S. Q. Zhang; J. Meng

2012-11-03T23:59:59.000Z

45

Compression mode resonances in Zr-90  

E-Print Network [OSTI]

Compression mode resonances in 90Zr D. H. Youngblood, Y.-W. Lui, B. John,* Y. Tokimoto, H. L. Clark, and X. Chen Cyclotron Institute, Texas A&M University, College Station, Texas 77843, USA (Received 18 February 2004; published 20 May 2004..., JOHN, TOKIMOTO, CLARK, AND CHEN PHYSICAL REVIEW C 69, 054312 (2004) 054312-2 Fig. 2. The continuum distributions are similar over the en- tire energy range, whereas the angular distributions of the cross sections for the peak change...

Youngblood, David H.; Lui, YW; John, B.; Tokimoto, Y.; Clark, HL; Chen, X.

2004-01-01T23:59:59.000Z

46

Metrological Determination of Natural Radioactive Isotopes {sup 226}Ra, {sup 228}Ra and {sup 210}Pb by Means of Ge Detector  

SciTech Connect (OSTI)

A metrological method to determine the activity per mass unity (activity concentration) of {sup 226}Ra and {sup 210}Pb ({sup 238}U decay series) and {sup 228}Ra ({sup 232}Th series) by gamma-ray spectrometers based on hyper-pure coaxial germanium detector was developed. In the soil the {sup 22}Ra (half-life = 1600 years) exhibits the same level of radioactivity as {sup 238}U (half-life 4.5x10{sup 9} years) because of a natural phenomenon called secular equilibrium. {sup 226}Ra decays into {sup 222}Rn (half-life = 3.8 days), a radioactive inert gas. After several days, the {sup 222}Rn naturally decays to {sup 218}Po (half-life = 3 minutes), where finally {sup 210}Pb (half-life = 22 years) is produced. The metrological capability of high-resolution gamma-ray spectrometry for naturally occurring radionuclides at environmental levels is showed, with emphasis on the use of 2 mL standard sources volume in a glass ampoule. Source preparation and calibration procedures are described. Radionuclide standards in an activity range of 10 to 250 Bq/g were produced which can be applied in a variety of environmental sample analysis (water, plant material, sediment, etc.). Uncertainties for {sup 226}Ra and {sup 210}Pb around 3% (k = 1) were obtained.

Almeida, Maria Candida M. de; Delgado, Jose U.; Poledna, Roberto; Oliveira, Estela Maria de; Silva, Ronaldo L. da [Laboratorio Nacional de Metrologia das Radiacoes Ionizantes, Instituto de Radioprotecao e Dosimetria, Comissao Nacional de Energia Nuclear(SEMRA/LNMRI/IRD/CNEN) Av. Salvador Allende s/n, Recreio, Rio de Janeiro, CEP 22780-160, RJ (Brazil)

2008-08-07T23:59:59.000Z

47

PoPulation Differentiation anD raPiD evolution of egg Color in aCCorDanCe with Solar raDiation  

E-Print Network [OSTI]

PoPulation Differentiation anD raPiD evolution of egg Color in aCCorDanCe with Solar raDiation Davi, . Diferenciación entre Poblaciones y Evolución Rápida del Color de los Huevos de Acuerdo a la Radiación Solar Uy C P' R d Pm wb, ://www.j. m/I.. DOI: 10.1525/k.2008.07033DOI: 10.1525/k.2008.07033 Bird egg color

Lahti, David C.

48

Audit Report: OAS-RA-13-31 | Department of Energy  

Energy Savers [EERE]

3-31 Audit Report: OAS-RA-13-31 September 27, 2013 The Department of Energy's Hydrogen and Fuel Cells Program The Department of Energy spent approximately 1 billion over the last...

49

Ra, a naturally occurring isotope of the 238 U-series with a  

E-Print Network [OSTI]

for counting, liquid scintillation, or mass spectrometry at comparable activities, the simple setup, low cost- fiber and is continuously transferred to a scintillation cham- 226 Ra determination via the rate of 222

Paris-Sud XI, Université de

50

Audit Report: OAS-RA-12-12 | Department of Energy  

Energy Savers [EERE]

2-12 Audit Report: OAS-RA-12-12 May 22, 2012 The Department of Energy's Clean Cities Alternative Fuel Vehicle Grant Program Funded under the American Recovery and Reinvestment Act...

51

Examination Report: OAS-RA-13-01 | Department of Energy  

Energy Savers [EERE]

OAS-RA-13-01 October 9, 2012 California Energy Commission - Energy Efficiency and Conservation Block Grant Program Funds Provided by the American Recovery and Reinvestment Act of...

52

Examination Report: OAS-RA-13-12 | Department of Energy  

Energy Savers [EERE]

Report: OAS-RA-13-12 February 19, 2013 City of Los Angeles - Energy Efficiency and Conservation Block Grant Program Funds Provided by the American Recovery and Reinvestment Act of...

53

Examination Report: OAS-RA-13-02 | Department of Energy  

Office of Environmental Management (EM)

Report: OAS-RA-13-02 October 9, 2012 County of Los Angeles - Energy Efficiency and Conservation Block Grant Program Funds Provided by the American Recovery and Reinvestment Act of...

54

Audit Report: OAS-RA-11-12 | Department of Energy  

Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

Audit Report: OAS-RA-11-12 August 22, 2011 The Department of Energy's Weatherization Assistance Program under the American Recovery and Reinvestment Act in the State of Missouri...

55

Audit Report: OAS-RA-11-14 | Department of Energy  

Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

Audit Report: OAS-RA-11-14 August 25, 2011 The Department of Energy's Weatherization Assistance Program Funded under the American Recovery and Reinvestment Act for the Commonwealth...

56

Performance & Risk Assessment Community of Practice (P&RA CoP...  

Energy Savers [EERE]

an enduring data and modeling resource to minimize duplication of effort across DOE and train future generation of PA professionals In late 2013, the group was broadened as P&RA...

57

First In Vivo Evaluation of Liposome-encapsulated 223Ra as a Potential Alpha-particle-emitting Cancer Therapeutic Agent  

SciTech Connect (OSTI)

Liposomes carrying chemotherapeutics have had some success in cancer treatment and may be suitable carriers for therapeutic radionuclides. This study was designed to evaluate the biodistribution of and to estimate the radiation doses from the alpha emitter 223Ra loaded into pegylated liposomes in selected tissues. 223Ra was encapsulated in pegylated liposomal doxorubicin by ionophore-mediated loading. The biodistribution of liposomal 223Ra was compared to free cationic 223Ra in Balb/C mice. We showed that liposomal 223 Ra circulated in the blood with an initial half-time in excess of 24 hours, which agreed well with that reported for liposomal doxorubicin in rodents, while the blood half-time of cationic 223Ra was considerably less than one hour. When liposomal 223 Ra was catabolized, the released 223Ra was either excreted or taken up in the skeleton. This skeletal uptake increased up to 14 days after treatment, but did not reach the level seen with free 223Ra. Pre-treatment with non-radioactive liposomal doxorubicin 4 days in advance lessened the liver uptake of liposomal 223 Ra. Dose estimates showed that the spleen, followed by bone surfaces, received the highest absorbed doses. Liposomal 223 Ra was relatively stable in vivo and may have potential for radionuclide therapy and combination therapy with chemotherapeutic agents.

Jonasdottir, Thora J.; Fisher, Darrell R.; Borrebaek, Jorgen; Bruland, Oyvind S.; Larsen, Roy H.

2006-09-13T23:59:59.000Z

58

ccsd00001055 First principles study of the solubility of Zr in Al  

E-Print Network [OSTI]

ccsd­00001055 (version 1) : 22 Jan 2004 First principles study of the solubility of Zr in Al (Dated: January 22, 2004) The experimental solubility limit of Zr in Al is well-known. Al3Zr has a stable the solubility limit of Zr in Al for the stable as well as the metastable phase diagrams. The formation energies

59

Spectroscopy of Ba and Ba$^+$ deposits in solid xenon for barium tagging in nEXO  

E-Print Network [OSTI]

Progress on a method of barium tagging for the nEXO double beta decay experiment is reported. Absorption and emission spectra for deposits of barium atoms and ions in solid xenon matrices are presented. Excitation spectra for prominent emission lines, temperature dependence and bleaching of the fluorescence reveal the existence of different matrix sites. A regular series of sharp lines observed in Ba$^+$ deposits is identified with some type of barium hydride molecule. Lower limits for the fluorescence quantum efficiency of the principal Ba emission transition are reported. Under current conditions, an image of $\\le10^4$ Ba atoms can be obtained. Prospects for imaging single Ba atoms in solid xenon are discussed.

B. Mong; S. Cook; T. Walton; C. Chambers; A. Craycraft; C. Benitez-Medina; K. Hall; W. Fairbank Jr.; J. B. Albert; D. J. Auty; P. S. Barbeau; V. Basque; D. Beck; M. Breidenbach; T. Brunner; G. F. Cao; B. Cleveland; M. Coon; T. Daniels; S. J. Daugherty; R. DeVoe; T. Didberidze; J. Dilling; M. J. Dolinski; M. Dunford; L. Fabris; J. Farine; W. Feldmeier; P. Fierlinger; D. Fudenberg; G. Giroux; R. Gornea; K. Graham; G. Gratta; M. Heffner; M. Hughes; X. S. Jiang; T. N. Johnson; S. Johnston; A. Karelin; L. J. Kaufman; R. Killick; T. Koffas; S. Kravitz; R. Krucken; A. Kuchenkov; K. S. Kumar; D. S. Leonard; C. Licciardi; Y. H. Lin; J. Ling; R. MacLellan; M. G. Marino; D. Moore; A. Odian; I. Ostrovskiy; A. Piepke; A. Pocar; F. Retiere; P. C. Rowson; M. P. Rozo; A. Schubert; D. Sinclair; E. Smith; V. Stekhanov; M. Tarka; T. Tolba; K. Twelker; J. -L. Vuilleumier; J. Walton; M. Weber; L. J. Wen; U. Wichoski; L. Yang; Y. -R. Yen; Y. B. Zhao

2014-10-09T23:59:59.000Z

60

DFT STUDY REVISES INTERSTITIAL CONFIGURATIONS IN HCP Zr  

SciTech Connect (OSTI)

Analysis of experimental result on microstructure evolution in irradiated Zr and alloys has demonstrated that available knowledge on self-interstitial defects in Zr is in contradiction. We therefore have initiated an extensive theoretical and modeling program to clarify this issue. In this report we present first ab initio calculations results of single SIA configurations in Zr. We demonstrate importance of simulations cell size, applied exchange-correlation functional and simulated c/a ratio. The results obtained demonstrate clearly that the most stable configurations are in basal plane and provide some evidences for enhanced interstitial transport along basal planes. The results obtained will be used in generation a new interatomic potential for Zr to be used in large-scale atomistic modeling of mechanisms relevant for radiation-induced microstructure evolution.

Samolyuk, German D [ORNL; Golubov, Stanislav I [ORNL; Osetskiy, Yury N [ORNL; Stoller, Roger E [ORNL

2012-06-01T23:59:59.000Z

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


61

Audit Report: OAS-RA-12-12 | Department of Energy  

Energy Savers [EERE]

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Home Page on Google Bookmark EERE: Alternative Fuels Data Center Home Page on Delicious RankCombustionImprovement3--Logistical5/08 Attendance List1-02 Audit2-02 AuditRA-10-06 Audit22-07RA-12-12

62

Hadron Physics in BaBar  

SciTech Connect (OSTI)

Some recent results in hadron physics from the BaBar experiment are discussed. In particular, the observation of two new charmed states, the D*{sub sJ}{sup +}(2317) and the D*{sub sJ}{sup +}(2457), is described, and results are presented on the first measurement of the rare decay mode of the B meson, B{sup 0} {pi}{sup 0}{pi}{sup 0}.

Lafferty, G.D.; /Manchester U.

2005-08-29T23:59:59.000Z

63

New Spectroscopy at BaBar  

SciTech Connect (OSTI)

The Babar experiment at the SLAC B factory has accumulated a high luminosity that offers the possibility of systematic studies of quarkonium spectroscopy and of investigating rare new phenomena. Recent results in this field are presented. In recent times spectroscopy has become exciting again, after the discovery of new states that are not easily explained by conventional models. States such as the X(3872) and the Y(4260) could be new excited charmonium states, but require precise measurements for positive identification. The BaBar experiment [1] is installed at the asymmetric storage ring PEP-II. 90% of the data accumulated by BaBar are taken at the Y(4S) (10.58 GeV) and 10% just below (10.54 GeV). The BaBar detector includes a 5-layer, double-sided silicon vertex tracker and a 40-layer drift chamber in a 1.5 T solenoidal magnetic field, which detect charged particles and measures their momenta and ionization energy losses. Photons, electrons, and neutral hadrons are detected with a CsI(Tl)-crystal electromagnetic calorimeter. An internally reflecting ring-imaging Cherenkov is also used for particle id. Penetrating muon and neutral hadrons are identified by an array of resistive-plate chambers embedded in the steel of the flux return. The detector allows good track and vertex resolution, good particle id and good photon detection so it is especially suited for spectroscopy studies.

Mazzoni, M.A.; /INFN, Rome

2007-04-18T23:59:59.000Z

64

Supply of purified Th228 for Ra224 generators. Final CRADA Report .  

SciTech Connect (OSTI)

CRADA was terminated when it was determined that the Russians could not perform the terms of the subcontract. It became apparent that the Russians would not be a reliable source of Th228, as a precursor in the decay chain which leads to Ra224. Their government policies will prohibit the export of Th228 in quantities needed for commercial cancer therapy.

Ehst, D. A.; Nuclear Engineering Division

2009-10-02T23:59:59.000Z

65

George Feher (Photograph by R.A. Icaacson) Photosynthesis Research 55: 140, 1998.  

E-Print Network [OSTI]

George Feher (Photograph by R.A. Icaacson) #12;Photosynthesis Research 55: 1­40, 1998. © 1998 of research in bacterial photosynthesis and the road leading to it: A personal account George Feher In this minireview I present a very personal account of my life and research in bacterial photosynthesis

Govindjee "Gov"

66

RaWMS -Random Walk based Lightweight Membership Service for Wireless Ad Hoc Networks  

E-Print Network [OSTI]

: Algorithms, Design Additional Key Words and Phrases: Ad Hoc Networks, Membership service, Random Walk 1. INTRODUCTION Context of this study. Membership services serve as essential building blocks in a varietyRaWMS - Random Walk based Lightweight Membership Service for Wireless Ad Hoc Networks ZIV BAR

Tomkins, Andrew

67

RA After Hours On Call (971) 246-1388 Your Guide to  

E-Print Network [OSTI]

for the resident to pick up at the move-in station. Laundry Laundry facilities are located on odd-numbered floors is on for an extended amount of time, please notify the Help desk or the RA on call. If you leave trash, abandoned

Latiolais, M. Paul

68

RaPID: THE END OF HEURISTIC PID TUNING Peter Van Overschee, Christiaan Moons, Wim Van Brempt  

E-Print Network [OSTI]

RaPID: THE END OF HEURISTIC PID TUNING Peter Van Overschee, Christiaan Moons, Wim Van Brempt Paul Vanvuchelen, Bart De Moor Abstract: RaPID (Robust Advanced PID Control) is a new and original engineer- ing tool for the design and implementation of optimal PID controllers. It integrates data acquisition

69

Targeting of Osseous Sites with Alpha-emitting Ra-223: Comparison with the Beta-emitter Sr-89 in Mice  

SciTech Connect (OSTI)

The bone-seeking property of and the potential to irradiate red marrow by the alpha-particle emitter Ra-223 (t1/2 = 11.43 d) were compared to those of the beta-emitter Sr-89 (t1/2 = 50.53 d). Methods: The biodistributions of Ra-223 and Sr-89 were studied in mice. Tissue uptakes were determined at 1 h, 6 h, 1 d, 3 d, and 14 d after intravenous administration. The potential redistribution of progeny from Ra-223 located in bone was investigated. Radiation absorbed doses were calculated for soft tissues and bone. Doses were also estimated for marrow-containing cavities assuming spheric geometries. Results: We found that both Sr-89 and Ra-223 selectively concentrated on bone surfaces relative to soft tissues. The measured bone uptake of Ra-223 was slightly higher than that of Sr-89. At the 24 h time-point, the femur uptake of Ra-223 was 40.1% of the administered activity per gram tissue. The uptake in spleen and most other soft tissues was higher for Ra-223 than for Sr-89. We observed rapid clearance of Ra-223 from soft tissues within the first 24 hours, but the bone surface uptake of Ra-223 increased with time up to 24 h. Among the soft tissues, the spleen had the greatest accumulation and retention of Ra-223. The femur-to-spleen ratio increased with time, from 6.4 at 6 h to 23.7 at 3 days after injections. We found little redistribution of Ra-223 daughter products away from bone (about 2% at 6 h and less than 1% detectable at 3 d). Estimates of dose to marrow-containing cavities showed that the Ra-223 alpha-emitter might have a marrow-sparing advantage compared to beta-emitters due to high linear-energy-transfer and short alpha range targeting osteoid surfaces. The alpha-emitters irradiate a smaller fraction of the marrow-containing volumes--sparing marrow and enhancing survival of marrow cells. At the same time, the bone surfaces receives a therapeutically effective radiation dose. Conclusion: The results of this study indicate that Ra-223 is a promising candidate for high linear-energy-transfer alpha-particle irradiation of cancer cells on bone surfaces. Radium-223 can, together with its daughter radionuclides, deliver an intense and highly localized field of radiation to bone surfaces with substantially less irradiation of healthy bone marrow dose compared to standard, bone-seeking beta-emitters such as Sr-89.

Henriksen, Gjermund; Fisher, Darrell R.; Roeske, John C.; Bruland, Oyvind S.; Larsen, Roy H.

2003-05-16T23:59:59.000Z

70

Characterization of Zr-Fe-Cu Alloys for an Inert Matrix Fuel for Nuclear Energy Applications  

E-Print Network [OSTI]

Cu had the largest melting temperature (886.3°C) while Zr-12Fe-10Cu had the smallest melting temperature (870°C). The third alloy, Zr-12Fe-15Cu, had a melting point just below that of Zr-12Fe-5Cu at 882.7°C. Light Flash Analysis (LFA...

Barnhart, Brian A.

2013-08-09T23:59:59.000Z

71

ccsd00001116 Nucleation of Al 3 Zr and Al 3 Sc in aluminum alloys  

E-Print Network [OSTI]

ccsd­00001116 (version 1) : 4 Feb 2004 Nucleation of Al 3 Zr and Al 3 Sc in aluminum alloys: from 4, 2004) Zr and Sc precipitate in aluminum alloys to form the compounds Al3Zr and Al3Sc which

72

Investigation of rare nuclear decays with BaF$_2$ crystal scintillator contaminated by radium  

E-Print Network [OSTI]

The radioactive contamination of a BaF$_2$ scintillation crystal with mass of 1.714 kg was measured over 101 hours in the low-background DAMA/R&D set-up deep underground (3600 m w.e.) at the Gran Sasso National Laboratories of INFN (LNGS, Italy). The half-life of $^{212}$Po (present in the crystal scintillator due to contamination by radium) was measured as $T_{1/2}(^{212}$Po) = 298.8$\\pm$0.8(stat.)$\\pm$1.4(syst.) ns by analysis of the events' pulse profiles. The $^{222}$Rn nuclide is known as 100% decaying via emission of $\\alpha$ particle with $T_{1/2}$ = 3.82 d; however, its $\\beta$ decay is also energetically allowed with $Q_\\beta = 24\\pm21$ keV. Search for decay chains of events with specific pulse shapes characteristic for $\\alpha$ or for $\\beta/\\gamma$ signals and with known energies and time differences allowed us to set, for the first time, the limit on the branching ratio of $^{222}$Rn relatively to $\\beta$ decay as $B_\\beta 8.0$ y). Half-life limits of $^{212}$Pb, $^{222}$Rn and $^{226}$Ra relatively to $2\\beta$ decays are also improved in comparison with the earlier results.

P. Belli; R. Bernabei; F. Cappella; V. Caracciolo; R. Cerulli; F. A. Danevich; A. Di Marco; A. Incicchitti; D. V. Poda; O. G. Polischuk; V. I. Tretyak

2014-07-22T23:59:59.000Z

73

Effect of BaO Morphology on NOx Abatement: NO Interaction with...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

BaO Morphology on NOx Abatement: NO Interaction with Unsupported and O-Supported BaO. Effect of BaO Morphology on NOx Abatement: NO Interaction with Unsupported and O-Supported...

74

Calculo Numerico (MS211) PROVA 1 (25/09/2012) Nome: RA: Turma  

E-Print Network [OSTI]

C´alculo Num´erico (MS211) PROVA 1 (25/09/2012) Nome: RA: Turma: Trabalhe com radianos e 4 d boa aproxima¸c~ao de uma solu¸c~ao pode ser encontrada atrav´es o m´etodo de Newton(-Raphson). Se for poss´ivel, execute duas itera¸c~oes do m´etodo de Newton(-Raphson) gr´aficamente para cada um dos

Sussner, Peter

75

Calculo Numerico (MS211) PROVA 1 (19/04/2010) Nome: RA: Turma  

E-Print Network [OSTI]

C´alculo Num´erico (MS211) PROVA 1 (19/04/2010) Nome: RA: Turma: Trabalhe com 4 d´igitos decimais desta equa¸c~ao utilizando o M´etodo de Newton- Raphson com x0 = 2.5 e precis~oes 1 = 2 = 10. [0.5 pts] (c) Se tomarmos x0 = 1.01 como ser´a o comportamento da sequ^encia gerada pelo M´etodo de

Sussner, Peter

76

Calculo Numerico (MS211) PROVA 1 (01/10/2013) Nome: RA: Turma: Y  

E-Print Network [OSTI]

] (c) Em qual dos m´etodos n´umericos que voc^e conhece geralmente se usa a fatora¸c~ao LU (com ou semC´alculo Num´erico (MS211) PROVA 1 (01/10/2013) Nome: RA: Turma: Y Trabalhe com radianos e 4 d = b fazendo todas as contas na maquina. Explicite as opera¸c~oes bin´arias que produzem erros num´ericos

Sussner, Peter

77

225-Ac and 223-Ra Production via 800 MeV Proton Irradiation of Natural Thorium Target  

E-Print Network [OSTI]

Cross sections for the formation of 225,227-Ac, 223,225-Ra, and 227-Th via the proton bombardment of natural thorium targets were measured at a nominal proton energy of 800 MeV. No earlier experimental cross section data for the production of 223,225-Ra, 227-Ac and 227-Th by this method were found in the literature. A comparison of theoretical predictions with the experimental data shows agreement within a factor of two. Results indicate that accelerator-based production of 225-Ac and 223-Ra is a viable production method.

J. W. Weidner; S. G. Mashnik; K. D. John; B. Ballard; E. R. Birnbaum; L. J. Bitteker; A. Couture; M. E. Fassbender; G. S. Goff; R. Gritzo; F. M. Hemez; W. Runde; J. L. Ullmann; L. E. Wolfsberg; F. M. Nortier

2012-04-10T23:59:59.000Z

78

A New Environmentally Friendly AL/ZR-Based Clay Stabilizer  

E-Print Network [OSTI]

Clay stabilizers are means to prevent fines migration and clay swelling, which are caused by the contact of formation with low salinity or high pH brines at high temperature. Previous clay stabilizers including: Al and Zr compounds and cationic...

El-Monier, Ilham Abdallah

2013-01-18T23:59:59.000Z

79

Correlation between corrosion performance and surface wettability in ZrTiCuNiBe bulk metallic glasses  

E-Print Network [OSTI]

Correlation between corrosion performance and surface wettability in ZrTiCuNiBe bulk metallic June 2010 The corrosion properties of two Zr-based bulk metallic glass, Zr41Ti14Cu12Ni10Be23 LM1 and Zr potential, LM1b showed superior corrosion resistance to LM1. Under identical sample preparation and testing

Zheng, Yufeng

80

FourYear Academic Plan 20122013 BA in Geology  

E-Print Network [OSTI]

FourYear Academic Plan 20122013 BA in Geology Internal Use Version Year 1 Year 2 Year 3 Year 4: Total UD Credits: 46 Total Credits: 120 3/19/12 #12;FourYear Academic Plan 20122013 BA in Geology

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


81

Roadmap: Paralegal Studies Bachelor of Arts [AS-BA-PLST  

E-Print Network [OSTI]

Roadmap: Paralegal Studies ­ Bachelor of Arts [AS-BA-PLST] College of Arts and Sciences Department of Sociology Catalog Year: 2013-2014 Page 1 of 3 | Last Updated: 7-May-13/LNHD This roadmap is a recommended on page 2 #12;Roadmap: Paralegal Studies ­ Bachelor of Arts [AS-BA-PLST] College of Arts and Sciences

Sheridan, Scott

82

Combined Honours BA Digital Journalism and Communication, Media, and Film  

E-Print Network [OSTI]

Combined Honours BA Digital Journalism and Communication, Media, and Film Are you looking in Digital Journalism (DJ) and Communication, Media, and Film (CMF) is for you. That's because our DJ Honours BA Digital Journalism and Communication, Media, and Film We look forward to meeting you! Student

83

ON THE MOTIVE OF A QUOTIENT VARIETY SEBASTIAN DEL BA ~  

E-Print Network [OSTI]

ON THE MOTIVE OF A QUOTIENT VARIETY SEBASTIAN DEL BA ~ NO ROLLIN AND VICENTE NAVARRO AZNAR En with the realization functors and Chow groups. Recently, in the case char k = 0, Guill'en and Navarro Aznar have given. DEL BA ~ NO ROLLIN AND V. NAVARRO AZNAR group, K 0 M k , these decompositions were considered by Denef

Politècnica de Catalunya, Universitat

84

Evidence of Eu{sup 2+} 4f electrons in the valence band spectra of EuTiO{sub 3} and EuZrO{sub 3}  

SciTech Connect (OSTI)

We report on optical band gap and valence electronic structure of two Eu{sup 2+}-based perovskites, EuTiO{sub 3} and EuZrO{sub 3} as revealed by diffuse optical scattering, electron energy loss spectroscopy, and valence-band x-ray photoelectron spectroscopy. The data show good agreement with the first-principles studies in which the top of the valence band structure is formed by the narrow Eu 4f{sup 7} electron band. The O 2p band shows the features similar to those of the Ba(Sr)TiO{sub 3} perovskites except that it is shifted to higher binding energies. Appearance of the Eu{sup 2+} 4f{sup 7} band is a reason for narrowing of the optical band gap in the title compounds as compared to their Sr-based analogues.

Kolodiazhnyi, T. [National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044 (Japan); Valant, M. [Materials Research Laboratory, University of Nova Gorica, Vipavska 13, 5000 Nova Gorica (Slovenia); Williams, J. R. [International Center for Young Scientists (ICYS), MANA, National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044 (Japan); Bugnet, M.; Botton, G. A. [Department of Materials Science and Engineering, McMaster University, Hamilton, Ontario L8S 4L7 (Canada); Ohashi, N. [International Center for Materials Nanoarchitectonics, MANA, National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044 (Japan); Sakka, Y. [National Institute for Materials Science, 1-2-1 Sengen, Tsukuba, Ibaraki 305-0047 (Japan)

2012-10-15T23:59:59.000Z

85

Body-specific representations of spatial location Tad T. Bruny b,a,  

E-Print Network [OSTI]

Body-specific representations of spatial location Tad T. Brunyé b,a, , Aaron Gardony b,a , Caroline

Patel, Aniruddh D.

86

Radioactive contamination of BaF2 crystal scintillator  

E-Print Network [OSTI]

Barium fluoride (BaF$_2$) crystal scintillators are promising detectors to search for double beta decay processes in $^{130}$Ba ($Q_{2{\\beta}}$ = 2619(3) keV) and $^{132}$Ba ($Q_{2{\\beta}}$ = 844(1) keV). The $^{130}$Ba isotope is of particular interest because of the indications on 2${\\beta}$ decay found in two geochemical experiments. The radioactive contamination of BaF$_2$ scintillation crystal with mass of 1.714 kg was measured over 113.4 hours in a low-background DAMA/R&D set-up deep underground (3600 m w.e.) at the Gran Sasso National Laboratories of INFN (LNGS, Italy). The half-life of $^{212}$Po (present in the crystal scintillator due to contamination by radium) was estimated as $T_{1/2}$ = 298.8 $\\pm$ 0.8(stat.) $\\pm$ 1.4(syst.) ns by analysis of the events pulse profiles.

O. G. Polischuk; P. Belli; R. Bernabei; F. Cappella; V. Caracciolo; R. Cerulli; A. Di Marco; F. A. Danevich; A. Incicchitti; D. V. Poda; V. I. Tretyak

2013-12-17T23:59:59.000Z

87

Radioactive contamination of BaF2 crystal scintillator  

E-Print Network [OSTI]

Barium fluoride (BaF$_2$) crystal scintillators are promising detectors to search for double beta decay processes in $^{130}$Ba ($Q_{2{\\beta}}$ = 2619(3) keV) and $^{132}$Ba ($Q_{2{\\beta}}$ = 844(1) keV). The $^{130}$Ba isotope is of particular interest because of the indications on 2${\\beta}$ decay found in two geochemical experiments. The radioactive contamination of BaF$_2$ scintillation crystal with mass of 1.714 kg was measured over 113.4 hours in a low-background DAMA/R&D set-up deep underground (3600 m w.e.) at the Gran Sasso National Laboratories of INFN (LNGS, Italy). The half-life of $^{212}$Po (present in the crystal scintillator due to contamination by radium) was estimated as $T_{1/2}$ = 298.8 $\\pm$ 0.8(stat.) $\\pm$ 1.4(syst.) ns by analysis of the events pulse profiles.

Polischuk, O G; Bernabei, R; Cappella, F; Caracciolo, V; Cerulli, R; Di Marco, A; Danevich, F A; Incicchitti, A; Poda, D V; Tretyak, V I

2013-01-01T23:59:59.000Z

88

Point defect energetics in the ZrNi and Zr2Ni intermetallics C.S. Moura a,b  

E-Print Network [OSTI]

and Nuclear Engineering, The Pennsylvania State University, University Park, PA 16802, USA c Materials Science-neighbor Zr atoms. Ă? 2001 Elsevier Science B.V. All rights reserved. 1. Introduction There has been great of these compounds is governed by the balance between the irradiation damage and the annealing response

Motta, Arthur T.

89

B.A and B.S. in Mathematics Program B.A. and B.S. Mathematics  

E-Print Network [OSTI]

B.A and B.S. in Mathematics Program B.A. and B.S. Mathematics Department(s) Mathematical Sciences.A. in the Mathematical Sciences will... 1. Demonstrate a solid understanding of differential (1A), integral (1B understanding of rigorous mathematical proof (reading and writing), and apply reasoning based on definitions

Hemmers, Oliver

90

Page 1 | B.A. in Chemistry | Academic Plan of Study Updated April 2014 B.A. in Chemistry  

E-Print Network [OSTI]

Page 1 | B.A. in Chemistry | Academic Plan of Study Updated April 2014 B.A. in Chemistry Academic Plan of Study College of Liberal Arts & Sciences Department of Chemistry chemistry.uncc.edu PROGRAM to declare the major. · Advising (For the Major): completed by your chemistry faculty advisor (please refer

Raja, Anita

91

Precipitation in cold-rolled Al–Sc–Zr and Al–Mn–Sc–Zr alloys prepared by powder metallurgy  

SciTech Connect (OSTI)

The effects of cold-rolling on thermal, mechanical and electrical properties, microstructure and recrystallization behaviour of the AlScZr and AlMnScZr alloys prepared by powder metallurgy were studied. The powder was produced by atomising in argon with 1% oxygen and then consolidated by hot extrusion at 350 °C. The electrical resistometry and microhardness together with differential scanning calorimetry measurements were compared with microstructure development observed by transmission and scanning electron microscopy, X-ray diffraction and electron backscatter diffraction. Fine (sub)grain structure developed and fine coherent Al{sub 3}Sc and/or Al{sub 3}(Sc,Zr) particles precipitated during extrusion at 350 °C in the alloys studied. Additional precipitation of the Al{sub 3}Sc and/or Al{sub 3}(Sc,Zr) particles and/or their coarsening was slightly facilitated by the previous cold rolling. The presence of Sc,Zr-containing particles has a significant antirecrystallization effect that prevents recrystallization at temperatures minimally up to 420 °C. The precipitation of the Al{sub 6}Mn- and/or Al{sub 6}(Mn,Fe) particles of a size ? 1.0 ?m at subgrain boundaries has also an essential antirecrystallization effect and totally suppresses recrystallization during 32 h long annealing at 550 °C. The texture development of the alloys seems to be affected by high solid solution strengthening by Mn. The precipitation of the Mn-containing alloy is highly enhanced by a cold rolling. The apparent activation energy of the Al{sub 3}Sc particles formation and/or coarsening and that of the Al{sub 6}Mn and/or Al{sub 6}(Mn,Fe) particle precipitation in the powder and in the compacted alloys were determined. The cold deformation has no effect on the apparent activation energy values of the Al{sub 3}Sc-phase and the Al{sub 6}Mn-phase precipitation. - Highlights: • The Mn, Sc and Zr additions to Al totally suppresses recrystallization at 550 °C. • The Sc,Zr-containing particle precipitation is slightly facilitated by cold rolling. • The Mn-containing particle precipitation is highly enhanced by cold rolling. • Cold rolling has no effect on activation energy of the Al{sub 3}Sc and Al{sub 6}Mn precipitation. • The texture development is affected by high solid solution strengthening by Mn.

Vlach, M., E-mail: martin.vlach@mff.cuni.cz [Charles University in Prague, Faculty of Mathematics and Physics, Ke Karlovu 3, CZ-121 16 Prague (Czech Republic); Stulikova, I.; Smola, B.; Kekule, T.; Kudrnova, H.; Danis, S. [Charles University in Prague, Faculty of Mathematics and Physics, Ke Karlovu 3, CZ-121 16 Prague (Czech Republic); Gemma, R. [King Abdullah University of Science and Technology (KAUST), Physical Sciences and Engineering Division, 23955-6900 Thuwal (Saudi Arabia); Ocenasek, V. [SVÚM a.s., Podnikatelská 565, CZ-190 11 Prague (Czech Republic); Malek, J. [Czech Technical University in Prague, Faculty of Mechanical Engineering, CZ-120 00 Prague (Czech Republic); Tanprayoon, D.; Neubert, V. [Institut für Materialprüfung und Werkstofftechnik, Freiberger Strasse 1, D-38678 Clausthal-Zellerfeld (Germany)

2013-12-15T23:59:59.000Z

92

Crystallization of Zr2PdxCu(1-x) and Zr2NixCu(1-x) Metallic Glass  

SciTech Connect (OSTI)

One interesting aspect of rretallic glasses is the numerous instances of the deviation of the phase selection from the amorphous state to thermodynamically stable phases during the crystallization process. Their devitrification pathways allow us to study the relationship between the original amorphous structure and their crystalline counter parts. Among the various factors of phase selections, size and electronic effects have been most extensively studied. Elucidating the phase selection process of a glassy alloy will be helpful to fill in the puzzle of the changes from disordered to ordered structures. In this thesis, Two model Zr{sub 2}Pd{sub x}Cu{sub (1-x)} and Zr{sub 2}Ni{sub x}Cu{sub (1-x)} (x = 0, 0.25, 0.5, 0.75 and 1) glassy systems were investigated since: (1) All of the samples can be made into a homogenous metallic glass; (2) The atomic radii differ from Pd to Cu is by 11%, while Ni has nearly the identical atomic size compare to Cu. Moreover, Pd and Ni differ by only one valence electron from Cu. Thus, these systems are ideal to test the idea of the effects of electronic structure and size factors; (3) The small number of components in these pseudo binary systems readily lend themselves to theoretical modeling. Using high temperature X-ray diffraction {HTXRD) and thermal analysis, topological, size, electronic, bond and chemical distribution factors on crystallization selections in Zr{sub 2}Pd{sub x}Cu{sub (1-x)} and Zr{sub 2}Ni{sub x}Cu{sub (1-x)} metallic glass have been explored. All Zr{sub 2}Pd{sub x}Cu{sub (1-x)} compositions share the same Cu11b phase with different pathways of meta-stable, icosahedral quasicrystalline phase (i-phase), and C16 phase formations. The quasicrystal phase formation is topologically related to the increasing icosahedral short range order (SRO) with Pd content in Zr{sub 2}Pd{sub x}Cu{sub (1·x)} system. Meta-stable C16 phase is competitive with C11b phase at x = 0.5, which is dominated by electronic structure rather than size effects. Cu-rich and Ni-rich compositions in Zr{sub 2}Ni{sub x}Cu{sub (1-x)} trend to divitrify to C11b or C16 phases respectively. In the proposed pseudo binary phase diagram, the domain of C16, C11b and co-existence phases are mainly related with the topology in the amorphous structure and formation enthalpies of crystalline phases.

Min Xu

2008-08-18T23:59:59.000Z

93

Physical properties of single crystalline BaSn{sub 5}  

SciTech Connect (OSTI)

We present a comprehensive study of the binary intermetallic superconductor, BaSn{sub 5}. High-quality single crystalline BaSn{sub 5} was grown out of a Sn flux. Detailed thermodynamic and transport measurements were performed to study BaSn{sub 5}'s normal and superconducting state properties. This material appears to be a strongly coupled, multiband superconductor. H{sub c2}(T) is almost isotropic. De Haas–van Alphen oscillations were observed and two effective masses were estimated from the FFT spectra. Hydrostatic pressure causes a decrease in the superconducting transition temperature at the rate of ??0.053?±?0.001?K/kbar.

Lin, Xiao; Budko, Sergey; Canfield, Paul

2012-01-30T23:59:59.000Z

94

Examination Report: OAS-RA-13-19 | Department of Energy  

Office of Environmental Management (EM)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr May Jun Jul(Summary) " ,"ClickPipelinesProvedDecember 2005DepartmentDecember U.S. Department of9 Examination Report: OAS-RA-13-19

95

Audit Special Report: OAS-RA-10-03 | Department of Energy  

Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Home Page on Google Bookmark EERE: Alternative Fuels Data Center Home Page on Delicious Rank EERE:Year in Review: Top Five EERE BlogAttachmentFlash2011-21 Audit Letter6-0136 AuditOAS-RA-10-03 Audit

96

Audit Report: OAS-RA-11-08 | Department of Energy  

Energy Savers [EERE]

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Home Page on Google Bookmark EERE: Alternative Fuels Data Center Home Page on Delicious RankCombustionImprovement3--Logistical5/08 Attendance List1-02 Audit2-02 AuditRA-10-06 Audit2 Audit4

97

Water-induced Bulk Ba(NO3)2 Formation From NO2 Exposed Thermally...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Bulk Ba(NO3)2 Formation From NO2 Exposed Thermally Aged BaOAl2O3. Water-induced Bulk Ba(NO3)2 Formation From NO2 Exposed Thermally Aged BaOAl2O3. Abstract: Phase changes in high...

98

D0-D0 Mixing at BaBar  

E-Print Network [OSTI]

The BaBar and Belle collaborations have recently found evidence for mixing within the D meson system. We present some of the mixing search techniques used by BaBar and their status as of the beginning of the summer 2007. These have culminated in a measurement in the K decay final state of the D that is inconsistent with the no-mixing hypothesis with a significance of 3.9 standard deviations.

A. Seiden

2007-10-05T23:59:59.000Z

99

Identification of phases in the interaction layer between U-Mo-Zr/Al and U-Mo-Zr/Al-Si  

SciTech Connect (OSTI)

Out-of-pile diffusion experiments were performed between U-7wt.% Mo-1wt.% Zr and Al or Al A356 (7,1wt.% Si) at 550 deg. C. In this work morphological characterization and phase identification on both interaction layer are presented. They were carried out by the use of different techniques: optical and scanning electron microscopy, X-Ray diffraction and WDS microanalysis. In the interaction layer U-7wt.% Mo-1wt.% Zr/Al, the phases UAl{sub 3}, UAl{sub 4}, Al{sub 20}Mo{sub 2}U and Al{sub 43}Mo{sub 4}U{sub 6} were identified. In the interaction layer U-7wt.% Mo-1wt.% Zr/Al A356, the phases U(Al, Si) with 25at.% Si and Si{sub 5}U{sub 3} were identified. This last phase, with a higher Si concentration, was identified with XRD Synchrotron radiation performed at the National Synchrotron Light Laboratory (LNLS), Campinas, Brasil. (author)

Varela, C.L. Komar; Arico, S.F.; Mirandou, M.; Balart, S.N. [Departamento Materiales, GIDAT, GAEN, CNEA, Avda. Gral Paz 1499, B1650KNA, San Martin (Argentina); Gribaudo, L.M. [Departamento Materiales, GIDAT, GAEN, CNEA, Avda. Gral Paz 1499, B1650KNA, San Martin (Argentina); CONICET, Avda. Rivadavia 1917, C1033AAJ, Buenos Aires (Argentina)

2008-07-15T23:59:59.000Z

100

Crystallization and glass formation in electron and laser beam irradiated Cu-Zr alloys  

SciTech Connect (OSTI)

Four Cu-Zr alloys, Cu/sub 56/Zr/sub 44/, Cu/sub 50/Zr/sub 50/, Cu/sub 47/Zr/sub 53/, and Cu/sub 33/Zr/sub 67/, were surface melted with electron and pulsed laser beams to compare their kinetics of nucleation, growth and glass formation. It was observed that the ease of glass formation increased in the order: Cu/sub 33/Zr/sub 67/, Cu/sub 47/Zr/sub 53/, Cu/sub 56/Zr/sub 44/, and Cu/sub 50/Zr/sub 50/. The nucleation and regrowth produced different metastable phases. At the equiatomic composition, the preferred phase is a CsCl-type (B2) BCC structure. As the composition deviates from this, the preferred phase is either orthorhombic or tetragonal with a much larger unit cell not previously reported in the literature. The maximum growth velocity of these metastable phases was found to be about 0.025 m/s. The slow kinetics are responsible for the ease of glass formation in these systems. 4 refs., 7 figs., 2 tabs.

Huang, J.S.; Kaufmann, E.N.; Wall, M.A.; Olsen, B.L.

1987-11-01T23:59:59.000Z

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


101

E-Print Network 3.0 - application zr-sn alloys Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

used... , Zr, Sn, ... Source: Zheng, Yufeng - Department of Advanced Materials and Nanotechnology, Peking University Collection: Materials Science ; Biology and Medicine 2...

102

Leptonic B Decays at BaBar  

SciTech Connect (OSTI)

The authors will present the most recent results on leptonic B decays B{sup {+-}(0)} {yields} K*{sup {+-}(0)} {nu}{bar {nu}} and B{sup {+-}} {yields} {mu}{sup {+-}}{nu}, based on the data collected by the BaBar detector at PEP-II, an asymmetric e{sup +}e{sup -} collider at the center of mass energy of the {Upsilon}(4S) resonance. Rare B decays have always been a standard probe for New Physics (NP) searches. The very low Standard Model (SM) rate of these decays often make them unaccessible with the present experimental datasets, unless NP effects enhance the rate up to the current experimental sensitivity. Moreover, as NP effects can modify the decay kinematic, particular attention must be payed in order to perform a model independent analysis. A B-Factory provides an unique environment where to investigate these processes. The high number of B{bar B} pairs produced by a B-Factory often allows to approach the needed experimental sensitivity. Moreover, the clean environment and the closed kinematic of the initial state enable to obtaining a very pure sample where to look for these decays.

Monorchio, Diego; /INFN, Naples /Naples U.

2011-09-13T23:59:59.000Z

103

Page 1 | B.A. in Middle Grades Education | Academic Plan of Study Updated March 2014 B.A. in Middle Grades Education  

E-Print Network [OSTI]

Page 1 | B.A. in Middle Grades Education | Academic Plan of Study Updated March 2014 B.A. in Middle 2 | B.A. in Middle Grades Education | Academic Plan of Study Updated March 2014 Middle Grades Grades Education Academic Plan of Study College of Education Department of Middle, Secondary and K-12

Raja, Anita

104

Studiengang Bachelor Studiengangsmoderator Zugangsinformationen Unterrichtssprache Fakultt Afrikanische Sprachen, Literaturen und Kunst B.A. Prof. D. Ibriszimow Deutsch 4  

E-Print Network [OSTI]

A Afrikanische Sprachen, Literaturen und Kunst B.A. Prof. D. Ibriszimow Deutsch 4 Angewandte Informatik B.A. Prof. D. Henrich Deutsch 1 Anglistik B.A. Prof. M. Steppat Deutsch 4 B Berufliche Bildung, Fachrichtung Metalltechnik B.A. Prof. U. Glatzel Deutsch Betriebswirtschaftslehre B.A. Prof. J. Sigloch Numerus Clausus

Schmidt, Matthias

105

Report on Characterization of U-10 wt.% Zr Alloy  

SciTech Connect (OSTI)

This report summarizes the chemical and structural characterization results for a U-10 wt.% Zr alloy to be used in an ultra-high burn-up nuclear fuel concept. The as-cast alloy material was received from Texas A and M University. Characterization and an initial heat treatment of the alloy material were conducted at Lawrence Livermore National Laboratory. The as-received ingot was sectioned for X-ray analysis, metallography, SEM, TEM, and heat treatments, as shown in Figure 1.

McKeown, J; Wall, M; Hsiung, L; Turchi, P

2012-03-01T23:59:59.000Z

106

Isoscalar Breathing Mode State in Zr-90 and Sn-116  

E-Print Network [OSTI]

PHYSICAL RKVIK% C VOLUIHE 21, NUMBER 4 Isoscalar breathing mode state in Zr and "Sn C. M. Rozsa, D. H. Youngblood, J. D. Bronson, Y.-%. Lui, and U. Garg Cyclotron Institute, Texas AckM University, College Station, Texas 77843 (Received 5..., BRONSON, LUI, AND GARG larger opening and served to catch some particles scattered from the first set. For measurements at 0', the beam was passed into the spectrograph and one set of brass defining slits with an open- ing of 6.4' horizontally by 3.V...

Rozsa, C. M.; Youngblood, David H.; Bronson, J. D.; Lui, YW; Garg, U.

1980-01-01T23:59:59.000Z

107

Site preferences of indium impurity atoms in intermetallics having Al3Ti and Al3Zr crystal structures  

E-Print Network [OSTI]

Site preferences of indium impurity atoms in intermetallics having Al3Ti and Al3Zr crystal-04843 (Metals Program) and Praveen Sinha Fund for Physics Research. L12 DO22 DO23 Cu3Au Al3Ti Al3Zr #12;Outline · Indium was doped in samples of Al3V and Al3Ti (Al3Ti structure) and Al3Zr (Al3Zr structure) by arc

Collins, Gary S.

108

Atomistic Studies of Cation Transport in Tetragonal ZrO2 During Zirconium Corrosion  

SciTech Connect (OSTI)

Zirconium alloys are the major fuel cladding materials in current reactors. The water-side corrosion is one of the major degradation mechanisms of these alloys. During corrosion the transport of oxidizing species in zirconium dioxide (ZrO2) determines the corrosion kinetics. Previously it has been argued that the outward diffusion of cation ions is important for forming protective oxides. In this work, the migration of Zr defects in tetragonal ZrO2 is studied with temperature accelerated dynamics and molecular dynamics simulations. The results show that Zr interstitials have anisotropic diffusion and migrate preferentially along the [001] or c direction in tetragonal ZrO2. The compressive stresses can increase the Zr interstitial migration barrier significantly. The migration barriers of some defect clusters can be much lower than those of point defects. The migration of Zr interstitials at some special grain boundaries is much slower than in a bulk oxide. The implications of these atomistic simulation results in the Zr corrosion are discussed.

Xian-Ming Bai; Yongfeng Zhang; Michael R. Tonks

2013-10-01T23:59:59.000Z

109

Transformation plasticity and thermoelastic behavior in ZrO2-containing ceramics  

E-Print Network [OSTI]

565 Transformation plasticity and thermoelastic behavior in ZrO2-containing ceramics A. H. Heuer plasticité de transformation dans ZrO2, qui est responsable de la ré- sistance mécanique et de la grande profit. Dans certaines conditions, cette transformation est réversible, autocatalytique et

Paris-Sud XI, Université de

110

NIH eRA System xTrain External Termination of Fellowships Quick Reference 1 January 27, 2011  

E-Print Network [OSTI]

NIH eRA System xTrain External Termination of Fellowships Quick Reference 1 January 27, 2011 Powering the Advancement of Science xTrain Termination of Fellowships Quick Reference Guide for Institution finds the Fellowship award to be terminated and selects the View Trainee Roster link. NOTE: Although

Baker, Chris I.

111

NIH eRA System xTrain Termination for Appointments Quick Reference 1 January 27, 2011  

E-Print Network [OSTI]

NIH eRA System xTrain Termination for Appointments Quick Reference 1 January 27, 2011 Powering the Advancement of Science xTrain Termination of Appointments Quick Reference Guide for Institution Users 1. The PD/PI Initiates a Termination Notice (TN) · The PD/PI locates the Trainee on the Trainee Roster

Baker, Chris I.

112

An experimental and numerical study of surface tension-driven melt flow R.A. Parsons a,, F. Nimmo a  

E-Print Network [OSTI]

An experimental and numerical study of surface tension-driven melt flow R.A. Parsons a,, F. Nimmo 2007 Abstract To determine the role of surface tension-driven melt migration in planetary bodies, we, surface tension causes the melt to relax back to a homogeneous distribution. Samples composed of 76 vol

Nimmo, Francis

113

1997 BNL Site Environmental Report E -1 Bari, R.A., Gordon, D., Moran, D., and Volkow, N.,  

E-Print Network [OSTI]

APPENDIX E 1997 BNL Site Environmental Report E - 1 Bari, R.A., Gordon, D., Moran, D., and Volkow, N., 1997. Report of the Ad Hoc Committee on Environmental, Safety, and Health Decision Making at Brookhaven National Laboratory (April 29, 1997). Brookhaven National Laboratory, 1997. Environmental

114

NIH Grants.gov and eRA Commons flowchart Electronic Application Process PreparationofApplicationSubmissiontoNIHApplicantRegistration  

E-Print Network [OSTI]

NIH Grants.gov and eRA Commons flowchart ­ Electronic Application Process Preparationof by the RO for Grant.gov, PI will be set up by the RO in eraCommons; AO (cannot submit to NIH) = Senior Research Administrator/Research Services Manager; SO (submit to NIH) = Research Services/ Grants Manager

115

Microfluidics for block polymer shells (DMR 0819860) SEED :H.A. Stone, R.A. Register and Janine Nunes  

E-Print Network [OSTI]

Microfluidics for block polymer shells (DMR 0819860) SEED :H.A. Stone, R.A. Register and Janine. We utilized microfluidic methods to investigate the role of geometric structures, e.g. thin spherical, microfluidic devices with two consecutive flow-focusing junctions were used to generate air bubble

Petta, Jason

116

25. Bialecki RA, Ostrowski ZP, Kassab AJ, Yin Q, Sciubba E (2002) Coupling FEM, BEM, and analyti-  

E-Print Network [OSTI]

(such as iron) form permanent magnets or are attracted to magnets. An everyday example of ferromagnetism25. Bialecki RA, Ostrowski ZP, Kassab AJ, Yin Q, Sciubba E (2002) Coupling FEM, BEM, and analyti, a ferrimagnetic mate- rial is one in which the magnetic moments of the atoms on different sublattices are opposed

Qin, Qinghua

117

Distributed Online Conditions Database of the BaBar Experiment  

SciTech Connect (OSTI)

This paper presents CDB - The distributed Conditions Database of the BaBar Experiment. CDB is the second major iteration of the database deployed in BaBar for production use as of October 2002. It replaced the original version of the database used through the first three years of the data taking. The new design and its implementation aims to improve the performance and scalability of the original database and addresses the emerging challenges of the distributed data production and analysis system of the Experiment.

Khan, A.; /Brunel U.; Gaponenko, I.A.; Brown, D.N.; /LBL, Berkeley

2011-11-21T23:59:59.000Z

118

BaTiO? based materials for piezoelectric and electro-optic applications  

E-Print Network [OSTI]

Ferroelectric materials are key to many modem technologies, in particular piezoelectric actuators and electro-optic modulators. BaTiO? is one of the most extensively studied ferroelectric materials. The use of BaTiO? for ...

Avrahami, Ytshak, 1969-

2003-01-01T23:59:59.000Z

119

E-Print Network 3.0 - apada em salvador-ba Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

do IguauPR Edgar Franco Gomes Medicina Veterinaria SalvadorBA Iraci... Costa Lopes Quimica So PauloSP Ana Gabriela de Oliveira Sardinha Cincias Naturais SalvadorBA...

120

Water-induced morphology changes in BaO/?-Al2O3 NOx storage...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

materials. Water-induced morphology changes in BaO?-Al2O3 NOx storage materials. Abstract: Exposure of NO2-saturated BaO?-Al2O3 NOx storage materials to H2O vapour...

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


121

Excellent Sulfur Resistance of Pt/BaO/CeO2 Lean NOx Trap Catalysts...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

NOx Trap Catalysts. Excellent Sulfur Resistance of PtBaOCeO2 Lean NOx Trap Catalysts. Abstract: In this work, we investigated the NOx storage behavior of Pt-BaOCeO2 catalysts,...

122

Isothermal oxidation behavior of ternary Zr-Nb-Y alloys at high temperature  

SciTech Connect (OSTI)

The effect of yttrium content on isothermal oxidation behavior of Zr-2,5%Nb-0,5%Y, Zr-2,5%Nb-1%Y Zr-2,5%Nb-1,5%Y alloy at high temperature has been studied. High temperature oxidation carried out at tube furnace in air at 600,700 and 800°C for 1 hour. Optical microscope is used for microstructure characterization of the alloy. Oxidized and un oxidized specimen was characterized by x-ray diffraction. In this study, kinetic oxidation of Zr-2,5%Nb with different Y content at high temperature has also been studied. Characterization by optical microscope showed that microstructure of Zr-Nb-Y alloys relatively unchanged and showed equiaxed microstructure. X-ray diffraction of the alloys depicted that the oxide scale formed during oxidation of zirconium alloys is monoclinic ZrO2 while unoxidised alloy showed two phase ? and ? phase. SEM-EDS examination shows that depletion of Zr composition took place under the oxide layer. Kinetic rate of oxidation of zirconium alloy showed that increasing oxidation temperature will increase oxidation rate but increasing yttrium content in the alloys will decrease oxidation rate.

Prajitno, Djoko Hadi, E-mail: djokohp@batan.go.id [Research Center for Nuclear Materials and Radiometry, Jl. Tamansari 71, Bandung 40132 (Indonesia); Soepriyanto, Syoni; Basuki, Eddy Agus [Metallurgy Engineering, Institute Technology Bandung, Jl. Ganesha 10, Bandung 40132 (Indonesia); Wiryolukito, Slameto [Materials Engineering, Institute Technology Bandung, Jl. Ganesha 10, Bandung 40132 (Indonesia)

2014-03-24T23:59:59.000Z

123

Morphology and Composition cycle of BaO/Al2O3 NSR Catalysts during...  

Broader source: Energy.gov (indexed) [DOE]

0 290 310 330 350 370 Chemical shiftppm 20wt% BaOAl2O3 Al2O3 8wt% BaOAl2O3 313 337 340.5 Morphology and Composition cycle of BaOAl 2 O 3 NSR Catalysts during NO 2 Uptake and...

124

BA in ECONOMICS (736020) MAP Sheet Department of Economics  

E-Print Network [OSTI]

BA in ECONOMICS (736020) MAP Sheet Department of Economics For students entering the degree program The Economics Department requires a minimum of 21 hours in the major to be taken in residency at BYU courses: complete the following with a grade of C- or better: Econ 110* Economics Principles and Problems

Olsen Jr., Dan R.

125

BA in ECONOMICS (736020) MAP Sheet Department of Economics  

E-Print Network [OSTI]

BA in ECONOMICS (736020) MAP Sheet Department of Economics For students entering the degree program from approved list from approved list Econ 110* from approved list personal choice The Economics: complete the following with a grade of C- or better: Econ 110* Economics Principles and Problems Econ 378

Olsen Jr., Dan R.

126

Structural phase transitions in BaPrO{sub 3}  

SciTech Connect (OSTI)

The crystal structures adopted by BaPrO{sub 3} at and above ambient temperature have been examined using a combination of synchrotron X-ray and neutron diffraction. BaPrO{sub 3} has been established to undergo a series of phase transitions from Pbnmorthorhombic{yields}Ibmmorthorhombic{yields}R3-bar crhombohedral{yields}Pm3-barm cubic. BaPrO{sub 3} is the second A{sup 2+}B{sup 4+}O{sub 3} perovskite found to adopt rhombohedral symmetry in preference to the I4/mcm tetragonal structure. Analysis of the octahedral tilting through the rhombohedral to cubic phase transition indicates that this transformation is continuous and tricritical in nature. The tricritical behaviour of this transition is likely to be a result of the competition between tetragonal and rhombohedral structures to be the preferred phase, with the rhombohedral symmetry adopted by BaPrO{sub 3} being stabilised by the unusually large B-site cation.

Saines, Paul J. [School of Chemistry, University of Sydney, Sydney, New South Wales 2006 (Australia); Kennedy, Brendan J. [School of Chemistry, University of Sydney, Sydney, New South Wales 2006 (Australia)], E-mail: b.kennedy@chem.usyd.edu.au; Smith, Ronald I. [ISIS Facility, Rutherford Appleton Laboratory, Chilton, Harwell Science and Innovation Campus, Didcot OX11 0QX (United Kingdom)

2009-04-02T23:59:59.000Z

127

BA Political Science Assessment Plan Program Learning Goals  

E-Print Network [OSTI]

BA Political Science ­ Assessment Plan Program Learning Goals Undergraduate students gain familiarity with American political behavior and institutions, the nature of politics in the rest of the world, and the sources of international conflict and cooperation. All students majoring in political science take

Cantlon, Jessica F.

128

Measurements of Form Factors with the BaBar Experiment  

SciTech Connect (OSTI)

Selected recent results on measurements of form factors by the BaBar Collaboration are reviewed, including e{sup +}e{sup -} {yields} {eta}{prime}{gamma}, leptonic and semileptonic charm decays from data collected at or near the {Upsilon}(4S) resonance.

Li, Selina Z.; /SLAC

2011-08-25T23:59:59.000Z

129

Roadmap: Philosophy -Bachelor of Arts [AS-BA-PHIL  

E-Print Network [OSTI]

Roadmap: Philosophy - Bachelor of Arts [AS-BA-PHIL] College of Arts and Sciences Department of Philosophy Catalog Year: 2013-2014 Page 1 of 3 | Last Updated: 22-Apr-13/LNHD This roadmap is a recommended Credit Hours] PHIL 11001 Introduction to Philosophy or PHIL11009 Principles of Thinking 3 Both courses

Sheridan, Scott

130

Roadmap: English Bachelor of Arts [AS-BA-ENG  

E-Print Network [OSTI]

Roadmap: English ­ Bachelor of Arts [AS-BA-ENG] College of Arts and Sciences Department of English Catalog Year: 2013-2014 Page 1 of 4 | Last Updated: 7-May-13/LNHD This roadmap is a recommended semester 5 on page 3 General Electives (upper division) 6 #12;Roadmap: English ­ Bachelor of Arts [AS

Sheridan, Scott

131

Roadmap: Art History Bachelor of Arts [CA-BA-ARTH  

E-Print Network [OSTI]

Roadmap: Art History ­ Bachelor of Arts [CA-BA-ARTH] College of the Arts School of Art Catalog Year: 2013­2014 Page 1 of 2 | Last Updated: 30-Apr-13/JS This roadmap is a recommended semester Elective (upper division) 3 Minor Requirements or General Electives 9 See note 2 on page 2 #12;Roadmap

Sheridan, Scott

132

Roadmap: Art History Bachelor of Arts [CA-BA-ARTH  

E-Print Network [OSTI]

Roadmap: Art History ­ Bachelor of Arts [CA-BA-ARTH] College of the Arts School of Art Catalog Year: 2012­2013 Page 1 of 2 | Last Updated: 29-May-12/JS This roadmap is a recommended semester Elective (upper division) 3 Minor Requirements or General Electives 9 See note 2 on page 2 #12;Roadmap

Sheridan, Scott

133

Roadmap: Biology -Bachelor of Arts [AS-BA-BSCI  

E-Print Network [OSTI]

Roadmap: Biology - Bachelor of Arts [AS-BA-BSCI] College of Arts and Sciences Department of Biological Sciences Catalog Year: 2012­2013 Page 1 of 3 | Last Updated: 2-May-12/LNHD This roadmap hours and minimum 42 upper- division credit hours #12;Roadmap: Biology - Bachelor of Arts [AS

Sheridan, Scott

134

B.A. DEGREE REQUIREMENTS FOR CHEMISTRY (CHEMISTRY TRACK)  

E-Print Network [OSTI]

B.A. DEGREE REQUIREMENTS FOR CHEMISTRY (CHEMISTRY TRACK) Requirements include 36 credits in chemistry core courses, 32 of which are taken in specific courses. Each student's course of study includes the following: 1.) Required Chemistry Core Courses CHE 106: General Chemistry Lecture I (3) CHE 116: General

Doyle, Robert

135

Roadmap: Chemistry Bachelor of Arts [AS-BA-CHEM  

E-Print Network [OSTI]

Roadmap: Chemistry ­ Bachelor of Arts [AS-BA-CHEM] College of Arts and Sciences Department of Chemistry and Biochemistry Catalog Year: 2012­2013 Page 1 of 3 | Last Updated: 24-May-12/LNHD This roadmap One: [15 Credit Hours] CHEM 10060 General Chemistry I or CHEM 10960 Honors General Chemistry 4

Sheridan, Scott

136

MAJOR TO CAREER GUIDE B.A. Chemistry  

E-Print Network [OSTI]

MAJOR TO CAREER GUIDE B.A. Chemistry College of Sciences www.unlv.edu/chemistry Mission of the College of Sciences The College of Sciences offers programs in life sciences, chemistry, geoscience: 702-895-2077 Campus Location: MPE-A 130 www.unlv.edu/sciences/advising About the Chemistry Career

Walker, Lawrence R.

137

Roadmap: Chemistry Bachelor of Arts [AS-BA-CHEM  

E-Print Network [OSTI]

Roadmap: Chemistry ­ Bachelor of Arts [AS-BA-CHEM] College of Arts and Sciences Department of Chemistry and Biochemistry Catalog Year: 2013-2014 Page 1 of 3 | Last Updated: 1-May-13/LNHD This roadmap One: [15 Credit Hours] CHEM 10060 General Chemistry I (4) and CHEM 10062 General Chemistry I

Sheridan, Scott

138

Combined Honours BA Digital Journalism and Communication, Media, and Film  

E-Print Network [OSTI]

Combined Honours BA Digital Journalism and Communication, Media, and Film Are you looking in Digital Journalism (DJ) and Communication, Media, and Film (CMF) is for you. That's because our DJ for a career combining your interests in media with a practical skill-set? If so, the Combined Honours program

139

Superconductivity in gallium-substituted Ba8Si46 clathrates  

E-Print Network [OSTI]

superconductor, with an onset at T-C approximate to 3.3 K. For x=10 and higher, no superconductivity was observed down to T=1.8 K. This represents a strong suppression of superconductivity with increasing Ga content, compared to Ba8Si46 with T-C approximate to 8...

Li, Yang; Zhang, Ruihong; Liu, Yang; Chen, Ning; Luo, Z. P.; Ma, Xingqiao; Cao, Guohui; Feng, Z. S.; Hu, Chia-Ren; Ross, Joseph H., Jr.

2007-01-01T23:59:59.000Z

140

Quantitative phase analysis of Mg:ZrO{sub 2} nanoparticles by Rietveld refinement method  

SciTech Connect (OSTI)

To quantify the structural phases of nanocrystalline ZrO{sub 2} doped with Mg ions of varying concentrations (3, 5, 10, 15 and 20%) and annealed at different temperatures. Magnesia doped zirconia was prepared by chemical co-precipitation method and annealed up to 1000°C. The monoclinic and tetragonal phases present in Mg:ZrO{sub 2} were quantified using Rietveld refinement analysis of the X-ray diffraction data and compared with the Direct method based on peak intensity calculations. Tetragonal phase was dominant in the 600°C annealed Mg:ZrO{sub 2} for all Mg concentrations.

Balaji, V., E-mail: thangadurai.p@gmail.com; Senthilkumaran, S., E-mail: thangadurai.p@gmail.com; Thangadurai, P., E-mail: thangadurai.p@gmail.com [Center for Nano Science and Technology, Pondicherry University, Puducherry- 605014 (India)

2014-04-24T23:59:59.000Z

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


141

Ternary ceramic alloys of Zr-Ce-Hf oxides  

DOE Patents [OSTI]

A ternary ceramic alloy is described which produces toughening of zirconia and zirconia composites through the stress transformation from tetragonal phase to monoclinic phase. This alloy, having the general formula Ce[sub x]Hf[sub y]Zr[sub 1[minus]x[minus]y]O[sub 2], is produced through the addition of appropriate amounts of ceria and hafnia to the zirconia. Typically, improved toughness is achieved with about 5 to about 15 mol % ceria and up to about 40 mol % hafnia. The preparation of alloys of these compositions are given together with data as to the densities, tetragonal phase content, hardness and fracture toughness. The alloys are useful in preparing zirconia bodies as well as reinforcing ceramic composites. 1 fig.

Becher, P.F.; Funkenbusch, E.F.

1990-11-20T23:59:59.000Z

142

Hysteretic electrical transport in BaTiO{sub 3}/Ba{sub 1?x}Sr{sub x}TiO{sub 3}/Ge heterostructures  

SciTech Connect (OSTI)

We present electrical transport measurements of heterostructures comprised of BaTiO{sub 3} and Ba{sub 1?x}Sr{sub x}TiO{sub 3} epitaxially grown on Ge. Sr alloying imparts compressive strain to the BaTiO{sub 3}, which enables the thermal expansion mismatch between BaTiO{sub 3} and Ge to be overcome to achieve c-axis oriented growth. The conduction bands of BaTiO{sub 3} and Ba{sub 1?x}Sr{sub x}TiO{sub 3} are nearly aligned with the conduction band of Ge, which facilitates electron transport. Electrical transport measurements through the dielectric stack exhibit rectifying behavior and hysteresis, where the latter is consistent with ferroelectric switching.

Ngai, J. H.; Kumah, D. P.; Walker, F. J. [Department of Applied Physics and Center for Research on Interface Structures and Phenomena, Yale University, 15 Prospect Street, New Haven, Connecticut 06520-8284 (United States); Ahn, C. H. [Department of Applied Physics and Center for Research on Interface Structures and Phenomena, Yale University, 15 Prospect Street, New Haven, Connecticut 06520-8284 (United States); Department of Mechanical Engineering and Materials Science, Yale University, 10 Hillhouse Avenue, New Haven, Connecticut 06520-8267 (United States)

2014-02-10T23:59:59.000Z

143

Proton-induced cross sections relevant to production of 225Ac and 223Ra in natural thorium targets below 200 MeV  

E-Print Network [OSTI]

Cross sections for 223,225Ra, 225Ac and 227Th production by the proton bombardment of natural thorium targets were measured at proton energies below 200 MeV. Our measurements are in good agreement with previously published data and offer a complete excitation function for 223,225Ra in the energy range above 90 MeV. Comparison of theoretical predictions with the experimental data shows reasonable-to-good agreement. Results indicate that accelerator-based production of 225Ac and 223Ra below 200 MeV is a viable production method.

J. W. Weidner; S. G. Mashnik; K. D. John; F. Hemez; B. Ballard; H. Bach; E. R. Birnbaum; L. J. Bitteker; A. Couture; D. Dry; M. E. Fassbender; M. S. Gulley; K. R. Jackman; J. L. Ullmann; L. E. Wolfsberg; F. M. Nortier

2012-05-15T23:59:59.000Z

144

Phase formation in Zr/Fe multilayers during Kr ion irradiation.  

SciTech Connect (OSTI)

A detailed study has been conducted of the effect of Kr ion irradiation on phase formation in Zr-Fe metallic multilayers, using the Intermediate Voltage Electron Microscopy (IVEM) at Argonne National Laboratory. Metallic multilayers were prepared with different overall compositions (near 50-50 and Fe-rich), and with different wavelengths (repetition thicknesses). These samples were irradiated with 300 keV Kr ions at various temperatures to investigate the final products, as well as the kinetics of phase formation. For the shorter wavelength samples, the final product was in all cases an amorphous Zr-Fe phase, in combination with Fe, while specially for the larger wavelength samples, in the Fe-rich samples the intermetallic compounds ZrFe{sub 2} and Zr{sub 3}Fe were formed in addition to the amorphous phase. The dose to full reaction decreases with temperature, and with wavelength in a manner consistent with a diffusion-controlled reaction.

Motta, A. T.

1998-01-29T23:59:59.000Z

145

Atomistic Modeling of Displacement Cascades in La2Zr2O7 Pyrochlore...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

static calculations. Citation: Chartier A, C Meis, JP Crocombette, LR Corrales, and WJ Weber.2003."Atomistic Modeling of Displacement Cascades in La2Zr2O7 Pyrochlore."Physical...

146

Analysis of the electronic structure of ZrO{sub 2} by Compton spectroscopy  

SciTech Connect (OSTI)

The electronic structure of ZrO{sub 2} is studied using the Compton scattering technique. The first-ever Compton profile measurement on polycrystalline ZrO{sub 2} was obtained using 59.54 keV gamma-rays emanating from the {sup 241}Am radioisotope. To explain the experimental data, we compute theoretical Compton profile values using the method of linear combination of atomic orbitals in the framework of density functional theory. The correlation scheme proposed by Perdew-Burke-Ernzerhof and the exchange scheme of Becke are considered. The ionic-model-based calculations for a number of configurations, i.e., Zr{sup +x}(O{sup -x/2}){sub 2} (0 {<=} x {<=} 2), are also performed to estimate the charge transfer on compound formation, and the study supports transfer of 1.5 electrons from Zr to O atoms.

Mahammad, F. M.; Mahammed, S. F. [University of Tikrit 42, Department of Physics (Iraq)] [University of Tikrit 42, Department of Physics (Iraq); Kumar, R.; Vijay, Y. K.; Sharma, B. K. [University of Rajasthan, Department of Physics (India)] [University of Rajasthan, Department of Physics (India); Sharma, G., E-mail: gsphysics@gmail.com [University of Kota, Department of Pure and Applied Physics (India)

2013-07-15T23:59:59.000Z

147

Oxygen impurity and microalloying effect in a Zr-based bulk metallic glass alloy  

E-Print Network [OSTI]

Oxygen impurity and microalloying effect in a Zr-based bulk metallic glass alloy C.T. Liu*, M composition Zr­10 at.%Al­5% Ti­17.9% Cu­14.6% Ni (BAM-11) was used to study the effects of oxygen impurities and microalloying on the microstructure and mechanical properties. Oxygen impurity at a level of 3000 appm

Pennycook, Steve

148

Process and properties of electroless Ni-Cu-P-ZrO{sub 2} nanocomposite coatings  

SciTech Connect (OSTI)

Highlights: Black-Right-Pointing-Pointer The Ni-P and Ni-P-Cu-ZrO{sub 2} coatings were produced by electroless technique. Black-Right-Pointing-Pointer The influence of copper and ZrO{sub 2} nanoparticles on Ni-P was studied. Black-Right-Pointing-Pointer Surface morphology, structure and electrochemical behavior were evaluated. Black-Right-Pointing-Pointer The Ni-Cu-P-ZrO{sub 2} and Ni-P-ZrO{sub 2} coatings are more resistant to corrosion than Ni-P. Black-Right-Pointing-Pointer Introduction of Cu and ZrO{sub 2} in the matrix aids to the enhancement of microhardness. -- Abstract: Electroless Ni-Cu-P-ZrO{sub 2} composite coating was successfully obtained on low carbon steel matrix by electroless plating technique. Coatings with different compositions were obtained by varying copper as ternary metal and nano sized zirconium oxide particles so as to obtain elevated corrosion resistant Ni-P coating. Microstructure, crystal structure and composition of deposits were analyzed by SEM, EDX and XRD techniques. The corrosion behavior of the deposits was studied by anodic polarization, Tafel plots and electrochemical impedance spectroscopy (EIS) in 3.5% sodium chloride solution. The ZrO{sub 2} incorporated Ni-P coating showed higher corrosion resistance than plain Ni-P. The introduction of copper metal into Ni-P-ZrO{sub 2} enhanced the protection ability against corrosion. The influence of copper metal and nanoparticles on microhardness of coatings was evaluated.

Ranganatha, S. [Department of Studies in Chemistry, School of Chemical Sciences, Kuvempu University, Shankaraghatta 577451, Shimoga, Karnataka (India)] [Department of Studies in Chemistry, School of Chemical Sciences, Kuvempu University, Shankaraghatta 577451, Shimoga, Karnataka (India); Venkatesha, T.V., E-mail: drtvvenkatesha@yahoo.co.uk [Department of Studies in Chemistry, School of Chemical Sciences, Kuvempu University, Shankaraghatta 577451, Shimoga, Karnataka (India); Vathsala, K. [Nanotribology Laboratory, Mechanical engineering department, Indian Institute of Science, Bangalore (India)] [Nanotribology Laboratory, Mechanical engineering department, Indian Institute of Science, Bangalore (India)

2012-03-15T23:59:59.000Z

149

In-Situ Control of BaZrO3 and BaSnO3 Nanorod Alignment and Microstructure in YBa2Cu3O7-x Thin Films by Strain Modulated Growth  

E-Print Network [OSTI]

military aircraft and naval applications to energy production by wind power, many types of power generation applications may operate under strenuous conditions, requiring current densities on the order of 105 A/cm2 while subjected to magnetic fields of 3...

Baca, Francisco Javier A.

2009-11-20T23:59:59.000Z

150

Page 1 | B.A. in Earth Sciences | Academic Plan of Study Updated March 2014 B.A. in Earth Sciences  

E-Print Network [OSTI]

Page 1 | B.A. in Earth Sciences | Academic Plan of Study Updated March 2014 B.A. in Earth Sciences Academic Plan of Study College of Liberal Arts & Sciences Department of Geography & Earth Sciences geoearth. · Minimum Grades/GPA: minimum GPA is 2.0 · Teacher Licensure: YES in Earth Sciences. Students preparing

Raja, Anita

151

Page 1 | B.A. in Earth Sciences | Academic Plan of Study Updated April 2014 B.A. in Earth Sciences  

E-Print Network [OSTI]

Page 1 | B.A. in Earth Sciences | Academic Plan of Study Updated April 2014 B.A. in Earth Sciences Academic Plan of Study College of Liberal Arts & Sciences Department of Geography & Earth Sciences geoearth. · Minimum Grades/GPA: minimum GPA is 2.0 · Teacher Licensure: YES in Earth Sciences. Students preparing

Raja, Anita

152

Page 1 | B.A. in Special Education General Curriculum | Academic Plan of Study Updated May 2014 B.A. in Special Education (General Curriculum)  

E-Print Network [OSTI]

Page 1 | B.A. in Special Education ­ General Curriculum | Academic Plan of Study Updated May 2014 B.A. in Special Education (General Curriculum) Academic Plan of Study College of Education Department of Special Education and Child Development http://spcd.uncc.edu/ PROGRAM SUMMARY · Credit Hours: 120 hours

Raja, Anita

153

Page 1 | B.A. in Elementary Education | Academic Plan of Study Updated March 2014 B.A. in Elementary Education  

E-Print Network [OSTI]

Page 1 | B.A. in Elementary Education | Academic Plan of Study Updated March 2014 B.A. in Elementary Education Academic Plan of Study College of Education Department of Reading and Elementary Education education.uncc.edu/reel PROGRAM SUMMARY · Credit Hours: 120-121 · Concentrations: No · Declaring

Raja, Anita

154

Structural and chemical characterization of BaTiO{sub 3} nanorods  

SciTech Connect (OSTI)

Research highlights: {yields} Polycrystalline BaTiO{sub 3} nanorods were synthesized with EPD into AAO templates. {yields} Nanorods are composed of crystalline, nanosized grains with pseudo-cubic structure. {yields} Integrowth of hexagonal BaTiO{sub 3} polymorph within pseudo-cubic structure was observed. -- Abstract: An electron-microscopy investigation was performed on BaTiO{sub 3} nanorods that were processed by sol-gel electrophoretic deposition (EPD) into anodic aluminium oxide (AAO) membranes. The BaTiO{sub 3} nanorods grown within the template membranes had diameters ranging from 150 to 200 nm, with an average length of 10-50 {mu}m. By using various electron-microscopy techniques we showed that the processed BaTiO{sub 3} nanorods were homogeneous in their chemical composition. The BaTiO{sub 3} nanorods were always polycrystalline and were composed of well-crystallized, defect-free, pseudo-cubic BaTiO{sub 3} grains, ranging from 10 to 30 nm. No intergranular phases were observed between the BaTiO{sub 3} grains. A low-temperature hexagonal polymorph that is coherently intergrown with the BaTiO{sub 3} perovskite matrix was also observed as a minor phase. When annealing the AAO templates containing the BaTiO{sub 3} sol in an oxygen atmosphere the presence of the hexagonal polymorph was diminished.

Zagar, K.; Recnik, A.; Sturm, S. [Department for Nanostructured Materials, Jozef Stefan Institute, Jamova cesta 39, SI-1000 Ljubljana (Slovenia)] [Department for Nanostructured Materials, Jozef Stefan Institute, Jamova cesta 39, SI-1000 Ljubljana (Slovenia); Gajovic, A. [Molecular Physics Laboratory, Division of Materials Physics, Ruder Boskovic Institute, Bijenicka 54, HR-1002 Zagreb (Croatia)] [Molecular Physics Laboratory, Division of Materials Physics, Ruder Boskovic Institute, Bijenicka 54, HR-1002 Zagreb (Croatia); Ceh, M., E-mail: miran.ceh@ijs.si [Department for Nanostructured Materials, Jozef Stefan Institute, Jamova cesta 39, SI-1000 Ljubljana (Slovenia)

2011-03-15T23:59:59.000Z

155

High-Linear Energy Transfer Irradiation Targeted to Skeletal Metastases by the Alpha Emitter Ra-223: Adjuvant or Alternative to Conventional Modalities?  

SciTech Connect (OSTI)

The bone-seeking, alpha-particle emitting radiopharmaceutical Alpharadin, 223RaCl2 (t1/2 = 11.4 days) is under clinical development as a novel treatment for skeletal metastases from breast and prostate cancer. This paper summarizes the current status of preclinical and clinical research on 223RaCl2. Potential advantages of 223Ra to that of external beam irradiation or registered beta-emitting bone-seekers are discussed. Published data of 223Ra dosimetry in mice and a therapeutic study in a skeletal metastases model in nude rats have indicated significant therapeutic potential of bone-seeking alpha-emitters. This paper provides short-term and long-term results from the first clinical single dosage trial. We present data from a repeated dosage study of five consecutive injections of 50 kBq/kg bodyweight, once every third week, or two injections of 125 kBq/kg bodyweight, six weeks apart. Furthermore, preliminary results are given for a randomized phase II trial involving 64 patients with hormone-refractory prostate cancer and painful skeletal metastases who received four monthly injections of 223Ra or saline as an adjuvant to external beam radiotherapy. Also presented are preliminary dose estimates for 223Ra in humans. Results indicate that repeated dosing is feasible and that opportunities are available for combined treatment strategies.

Bruland, Oyvind S.; Nilsson, Sten; Fisher, Darrell R.; Larsen, Roy H.

2006-10-15T23:59:59.000Z

156

Ab initio study of radium monofluoride, RaF, as a candidate to search for P- and T,P- violation effects  

E-Print Network [OSTI]

Relativistic ab initio calculations have been performed to assess the suitability of RaF for experimental search of P- and T,P-violating interactions. The parameters of P- and T,P-odd terms of the spin-rotational Hamiltonian have been calculated for the ${^2}\\Sigma$ electronic ground state of RaF molecule. They include the parameter $W_a$, which is critical in experimental search for nuclear anapole moment and the parameters $W_d$ and $W_{\\rm SP}$ required to obtain restrictions on the electric dipole moment of the electron and T,P-odd scalar-pseudoscalar interactions, respectively. The parameter $X$ corresponding to the "volume effect" in the T,P$-$odd interaction of the $^{223}$Ra nuclear Schiff moment with electronic shells of RaF has also been computed. Spectroscopic and hyperfine structure constants for $^{223}$RaF and $^{223}$Ra$^+$ have been computed as well, demonstrating the accuracy of the methods employed.

A. D. Kudashov; A. N. Petrov; L. V. Skripnikov; N. S. Mosyagin; T. A. Isaev; R. Berger; A. V. Titov

2014-09-20T23:59:59.000Z

157

Superlattice Structure and Precipitates in O+ and Zr+ Ion Coimplanted SrTiO3: a Model Waste Form for 90Sr  

SciTech Connect (OSTI)

We investigate strontium titanate as a model waste form for 90Sr. Implantation with O+ and Zr+ ions, followed by annealing at 1423 K, was performed to simulate 90Sr to 90Zr decays. At low Zr concentrations, we observe formation of a ZrO-Sr superlattice structure. Ab initio calculations indicate that this atomic configuration is energetically favorable. At higher Zr concentrations, we observe precipitates of ZrO2 with a coherently strained interface, or a monolayer of disordered interfacial structure. Potential candidacy of 90SrTiO3 as a waste form for permanent disposal of 90Sr is discussed.

Jiang, Weilin; Van Ginhoven, Renee M.; Kovarik, Libor; Jaffe, John E.; Arey, Bruce W.

2012-07-13T23:59:59.000Z

158

The effects of zirconia morphology on methanol synthesis from COand H2 over Cu/ZrO2 catalysts: Part I -- Steady-State Studies  

SciTech Connect (OSTI)

The effect of zirconia phase on the activity and selectivityof Cu/ZrO2 for the hydrogenation of CO has been investigated. Relativelypure t-ZrO2 and m-ZrO2 were prepared with high surface areas (~; 145m2/g). Copper was then deposited onto the surface of these materials byeither incipient-wetness impregnation or deposition-precipitation. For afixed Cu surface area, Cu/m-ZrO2 was tenfold more active for methanolsynthesis than Cu/t-ZrO2 from a feed of 3/1 H2/CO at 3.0 MPa andtemperatures between 473 and 523 K. Cu/m-ZrO2 also exhibited a higherselectivity to methanol. Increasing the Cu surface area on m-ZrO2resulted in further improvement in activity with minimal change inselectivity. Methanol productivity increased linearly for both Cu/t-ZrO2and Cu/m-ZrO2 with increasing Cu surface area. The difference in inherentactivity of each phase paralleled the stronger and larger CO adsorptioncapacity of the Cu/m-ZrO2 as quantified by CO-TPD. The higher COadsorption capacity of Cu/m-ZrO2 is attributed to the presence of a highconcentration of anionic vacancies on the surface of m-ZrO2. Suchvacancies expose cus-Zr4+ cations, which act as Lewis acid centers andenhance the Bronsted acidity of adjacent Zr-OH groups. The presence ofcus-Zr4+ sites and adjacent Bronsted acidic Zr-OH groups contributes tothe adsorption of CO as HCOO-Zr groups, which are the initial precursorsto methanol.

Rhodes, Michael J.; Bell, Alexis T.

2005-03-21T23:59:59.000Z

159

Laboratory Results Area Lab ID Th-230 Ra-226 Pb-210 Po-210 U-238 ANSI Sum1  

E-Print Network [OSTI]

Laboratory Results Area Lab ID Th-230 Ra-226 Pb-210 Po-210 U-238 ANSI Sum1 Gamma Reading Area H Area I Confirmation 0405025-2 1.66 5.13 2.88 3.48 0.95 4.55 9741 Clear 11th Street 0405215-3 1.28 4.59 3.55 3.55 1.68 4.37 ++ Area K 0404284-2 14.8 43.4 17.4 13.8 10.6 80.8 15146 Estimated - lab

160

Melting temperatures of the ZrO{sub 2}-MOX system  

SciTech Connect (OSTI)

Severe accidents occurred at the Fukushima Daiichi Nuclear Power Plant Units 1-3 on March 11, 2011. MOX fuels were loaded in the Unit 3. For the thermal analysis of the severe accident, melting temperature and phase state of MOX corium were investigated. The simulated coriums were prepared from 4%Pu-containing MOX, 8%Pu-containing MOX and ZrO{sub 2}. Then X-ray diffraction, density and melting temperature measurements were carried out as a function of zirconium and plutonium contents. The cubic phase was observed in the 25%Zr-containing corium and the tetragonal phase was observed in the 50% and 75%Zr-containing coria. The lattice parameter and density monotonically changed with Pu content. Melting temperature increased with increasing Pu content; melting temperature were estimated to be 2932 K for 4%Pu MOX corium and 3012 K for 8%Pu MOX corium in the 25%ZrO{sub 2}-MOX system. The lowest melting temperature was observed for 50%Zr-containing corium. (authors)

Uchida, T.; Hirooka, S.; Kato, M.; Morimoto, K. [Japan Atomic Energy Agency, 4-33, Muramatsu, Tokai-mura, Naka-gun, Ibaraki 319-1194 (Japan); Sugata, H.; Shibata, K.; Sato, D. [Inspection Development Company, 4-33, Muramatsu, Tokai-mura, Naka-gun, Ibaraki 319-1194 (Japan)

2013-07-01T23:59:59.000Z

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
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161

Morphology and Composition cycle of BaO/Al2O3 NSR Catalysts during...  

Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

- PNNL Project 47120) Kinetic and Performance Studies of the Regeneration Phase of Model PtRhBa NOx Traps for Design and Optimization CLEERS Aftertreatment Modeling and Analysis...

162

Syntheses, crystal structures and characterizations of BaZn(SeO{sub 3}){sub 2} and BaZn(TeO{sub 3})Cl{sub 2}  

SciTech Connect (OSTI)

Two new barium zinc selenite and tellurite, namely, BaZn(SeO{sub 3}){sub 2} and BaZn(TeO{sub 3})Cl{sub 2}, have been synthesized by the solid state reaction. The structure of BaZn(SeO{sub 3}){sub 2} features double chains of [Zn(SeO{sub 3}){sub 2}]{sup 2-} anions composed of four- and eight-member rings which are alternatively along a-axis. The double chains of [Zn{sub 2}(TeO{sub 3}){sub 2}Cl{sub 3}]{sup 3-} anions in BaZn(TeO{sub 3})Cl{sub 2} are formed by Zn{sub 3}Te{sub 3} rings in which each tellurite group connects with three ZnO{sub 3}Cl tetrahedra. BaZn(SeO{sub 3}){sub 2} and BaZn(TeO{sub 3})Cl{sub 2} are wide bandgap semiconductors based on optical diffuse reflectance spectrum measurements. -- Graphical abstract: Two new barium zinc selenite and tellurite, namely, BaZn(SeO{sub 3}){sub 2} and BaZn(TeO{sub 3})Cl{sub 2}, have been synthesized by solid state reaction. The structure of BaZn(SeO{sub 3}){sub 2} features 1D double chains of [Zn(SeO{sub 3}){sub 2}]{sup 2-} anions composed of four- and eight-member rings which are alternatively along a-axis. The 1D double chains of [Zn{sub 2}(TeO{sub 3}){sub 2}Cl{sub 3}]{sup 3-} anions in BaZn(TeO{sub 3})Cl{sub 2} are formed by Zn{sub 3}Te{sub 3} rings in which each tellurite group connects with one ZnO{sub 3}Cl and two ZnO{sub 2}Cl{sub 2} tetrahedra. BaZn(SeO{sub 3}){sub 2} and BaZn(TeO{sub 3})Cl{sub 2} are wide bandgap semiconductors based on optical diffuse reflectance spectrum measurements.

Jiang Hailong [State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, and the Graduate School of the Chinese Academy of Sciences, Fuzhou 350002 (China); Feng Meiling [State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, and the Graduate School of the Chinese Academy of Sciences, Fuzhou 350002 (China); Mao Jianggao [State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, and the Graduate School of the Chinese Academy of Sciences, Fuzhou 350002 (China)]. E-mail: mjg@ms.fjirsm.ac.cn

2006-06-15T23:59:59.000Z

163

SeeBA Energiesysteme GmbH | Open Energy Information  

Open Energy Info (EERE)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Home Page on Google Bookmark EERE: Alternative Fuels Data Center Home Page on Office of Inspector GeneralDepartmentAUDIT REPORTOpenWende New EnergyAnatoliaScira Offshore EnergyLLCSeawindSeeBA

164

BA Tirunelveli Bundled Wind Project | Open Energy Information  

Open Energy Info (EERE)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Home Page on Google Bookmark EERE: Alternative Fuels Data Center Home5b9fcbce19 NoPublic Utilities Address: 160 EastMaine: EnergyAustin Energy Place: TexasAvoyellesdeA S Biogas AnlagenB9 EnergyB9BA

165

Low-lying Collective States in {sup 136}Ba  

SciTech Connect (OSTI)

Low-lying collective states in {sup 136}Ba were investigated with (n,n'{gamma}) techniques, including Doppler-shift attenuation lifetime measurements. The level spins, lifetimes, branching ratios, multipole-mixing ratios and transition strengths reveal candidates for symmetric-phonon states up to third order. The 2{sub ms}{sup +} mixed-symmetry state was confirmed as unfragmented and a candidate for a [2{sub 1}{sup +} x 2{sub ms}{sup +}]{sub 3}{sup +} two-phonon mixed-symmetry state is proposed.

Scheck, M. [Oliver Lodge Laboratory, University of Liverpool, Liverpool, GB (United Kingdom); Dept. of Physics and Astronomy, University of Kentucky, Lexington, KY (United States); Mukhopadhyay, S.; Crider, B.; Choudry, S. N.; Elhami, E.; Peters, E. E.; McEllistrem, M. T.; Orce, J. N. [Dept. of Physics and Astronomy, University of Kentucky, Lexington, KY (United States); Yates, S. W. [Dept. of Chemistry, University of Kentucky, Lexington, KY (United States); Dept. of Physics and Astronomy, University of Kentucky, Lexington, KY (United States)

2009-01-28T23:59:59.000Z

166

Formation of single-phase BaO nanoclusters. | EMSL  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr MayAtmospheric Optical Depth7-1D: Vegetation ProposedUsing ZirconiaPolicyFeasibilityFieldMinds" Give formsingle-phase BaO

167

Creep strength of niobium alloys, Nb-1%Zr and PWC-11  

SciTech Connect (OSTI)

A study is being conducted at NASA Lewis Research Center to determine the feasibility of using a carbide particle strengthened Nb-1% Zr base alloy to meet the anticipated temperature and creep resistance requirements of proposed near term space power systems. In order to provide information to aid in the determination of the suitability of the PWC-11 alloy as an alternative to Nb-1% Zr in space power systems this study investigated (1) the long-time high-vacuum creep behavior of the PWC-11 material and the Nb-1% Zr alloy, (2) the effect of prior stress-free thermal aging on this creep behavior, (3) the effect of electron beam (EB) welding on this creep behavior, and (4) the stability of creep strengthening carbide particles. 14 refs., 5 figs., 2 tabs.

Titran, R.H.

1990-01-01T23:59:59.000Z

168

Identification of a quasiparticle band in very neutron-rich {sup 104}Zr  

SciTech Connect (OSTI)

The high spin levels of a very neutron-rich {sup 104}Zr nucleus have been reinvestigated by measuring the prompt {gamma} rays in the spontaneous fission of {sup 252}Cf. The ground-state band has been confirmed. A new sideband has been identified with a band-head energy at 1928.7 keV. The projected shell model is employed to investigate the band structure of {sup 104}Zr. The results of calculated levels are in good agreement with the experimental data, and suggest that the new band in {sup 104}Zr may be based on the neutron {nu}5/2{sup -}[532] x {nu}3/2{sup +}[411] configuration.

Yeoh, E. Y.; Wang, J. G.; Ding, H. B.; Gu, L.; Xu, Q.; Xiao, Z. G. [Department of Physics, Tsinghua University, Beijing 100084 (China); Zhu, S. J. [Department of Physics, Tsinghua University, Beijing 100084 (China); Department of Physics, Vanderbilt University, Nashville, Tennessee 37235 (United States); Hamilton, J. H.; Ramayya, A. V.; Hwang, J. K.; Liu, S. H. [Department of Physics, Vanderbilt University, Nashville, Tennessee 37235 (United States); Liu, Y. X. [Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou 730000 (China); School of Science, Huzhou Teachers College, Huzhou 313000 (China); Sun, Y. [Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou 730000 (China); Department of Physics, Shanghai Jiao Tong University, Shanghai 200240 (China); Luo, Y. X. [Department of Physics, Vanderbilt University, Nashville, Tennessee 37235 (United States); Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Rasmussen, J. O.; Lee, I. Y. [Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States)

2010-08-15T23:59:59.000Z

169

Photocatalytic studies of Ho–Zr–O nano-composite with controllable composition and defects  

SciTech Connect (OSTI)

With the help of sol–gel method assisted by melting salt, a series of Ho–Zr–O nano-composite with controllable composition and defects have been successfully prepared. Characterization results show that the positions, intensity, and width of the X-ray diffraction peaks of the products have a regular variation with the increase of zirconium element which implies the gradual changes of crystal spacing and product size. At the same time, the molar ratios between holmium and zirconium ions are consistent with the chemical formula and both of them are uniformly distributed in products further showing the perfect formation of targeted materials. Optical properties reveal that diversified defect forms of Ho–Zr–O nano-composite lead to the different absorptions of visible light. Photocatalytic experiments demonstrate Zr{sub 0.8}Ho{sub 0.2}O{sub 2??} nano-crystals have excellent visible-light-responsive photocatalytic activities on some familiar dyes (e.g.: methylene blue and Rhodamine B) which results from the special defect structure, better absorption of visible light and larger specific surface area. It follows that Zr{sub 0.8}Ho{sub 0.2}O{sub 2??} nano-crystals are a new kind of visible-light-responsive photocatalysts with better prospects in conversion and utilization of solar energy. Also, the present melting salt assisted route might be generalized to synthesize other AxByOz composite oxide nano-crystals with more complicated structures. - Highlights: • Ho–Zr–O nano-composite with controllable composition and defects has been obtained. • Diversified defect forms of products lead to the different visible light absorption. • Zr{sub 0.8}Ho{sub 0.2}O{sub 2??} nano-crystals have excellent photocatalytic activities.

Du, Weimin, E-mail: duweimin75@gmail.com [College of Chemistry and Chemical Engineering, Anyang Normal University, Anyang, Henan 455000 (China); Zhao, Guoyan; Chang, Hongxun; Shi, Fei; Zhu, Zhaoqiang [College of Chemistry and Chemical Engineering, Anyang Normal University, Anyang, Henan 455000 (China); Qian, Xuefeng [School of Chemistry and Chemical Technology, Shanghai Jiao Tong University, Shanghai 200240 (China)

2013-09-15T23:59:59.000Z

170

{sup 226}Ra and {sup 231}Pa systematics of axial MORB, crustal residence ages, and magma chamber characteristics at 9--10{degree}N East Pacific Rise  

SciTech Connect (OSTI)

Mass spectrometric measurements of {sup 30}Th-22{sup 226}Ra and {sup 235}-U{sup 231}Pa disequilibria for axial basalts are used to determine crustal residence ages for MORB magma and investigate the temporal and spatial characteristics of axial magma chambers (AMC) at 9--10{degrees}N East Pacific Rise (EPR). Relative crustal residence ages can be calculated from variations in {sup 226}Ra/{sup 230}Th and {sup 231}Pa/{sup 235}U activity ratios for axial lavas, if (1) mantle sources and melting are uniform, and mantle transfer times are constant or rapid for axial N-MORB, and (2) {sup 231}Pa/{sup 235}U and {sup 226}Ra/{sup 230}Th in the melt are unaffected by shallow level fractional crystallization. Uniform Th, Sr, and Nd isotopic systematics and incompatible element ratios for N-MORB along the 9--10{degrees}N segment indicate that mantle sources and transfer times are similar. In addition, estimated bulk solid/melt partition coefficients for U, Th, and Pa are small, hence effects of fractional crystallization on {sup 231}Pa/{sup 235}U ratios for the melt are expected to be negligible. However, fractional crystallization of plagioclase in the AMC would lower {sup 226}Ra/{sup 230}Th ratios in the melt and produce a positive bias in {sup 226}Ra crustal residence ages for fractionated lavas.

Goldstein, S.J.; Murrell, M.T. [Los Alamos National Lab., NM (United States); Perfit, M.R. [Univ., of Florida, Gainesville, FL (United States). Dept. of Geology; Batiza, R. [Univ., of Hawaii, Honolulu, HI (United States); Fornari, D.J. [Woods Hole Oceanographic Institution, MA (United States). Dept. of Geology and Geophysics

1994-06-01T23:59:59.000Z

171

Silicon photodiode with selective Zr/Si coating for extreme ultraviolet spectral range  

SciTech Connect (OSTI)

The procedure of manufacturing silicon photodiodes with an integrated Zr/Si filter for extreme ultraviolet (EUV) spectral range is developed. A setup for measuring the sensitivity profile of detectors with spatial resolution better than 100 {mu}m is fabricated. The optical properties of silicon photodiodes in the EUV and visible spectral ranges are investigated. Some characteristics of SPD-100UV diodes with Zr/Si coating and without it, as well as of AXUV-100 diodes, are compared. In all types of detectors a narrow region beyond the operating aperture is found to be sensitive to the visible light. (photodetectors)

Aruev, P N; Barysheva, Mariya M; Ber, B Ya; Zabrodskaya, N V; Zabrodskii, V V; Lopatin, A Ya; Pestov, Alexey E; Petrenko, M V; Polkovnikov, V N; Salashchenko, Nikolai N; Sukhanov, V L; Chkhalo, Nikolai I

2012-10-31T23:59:59.000Z

172

Deformation Mechanisms in Tube Billets from Zr-1%Nb Alloy under Radial Forging  

SciTech Connect (OSTI)

Features of the deformation process by cold radial forging of tube billets from Zr-1%Nb alloy were reconstructed on the basis of X-ray data concerning their structure and texture. The cold radial forging intensifies grain fragmentation in the bulk of billet and increases significantly the latent hardening of potentially active slip systems, so that operation only of the single slip system becomes possible. As a result, in radially-forged billets unusual deformation and recrystallization textures arise. These textures differ from usual textures of {alpha}-Zr by the mutual inversion of crystallographic axes, aligned along the axis of tube.

Perlovich, Yuriy; Isaenkova, Margarita; Fesenko, Vladimir; Krymskaya, Olga [National Research Nuclear University 'Moscow Engineering Physics Institute', Kashirskoe shosse, 31, Moscow, 115409 (Russian Federation); Zavodchikov, Alexander [Perm Research Technological Institute, Hasan Heroes street, 41, Perm, 614990 (Russian Federation)

2011-05-04T23:59:59.000Z

173

Physical properties of epitaxial ZrN/MgO(001) layers grown by reactive magnetron sputtering  

SciTech Connect (OSTI)

Single-crystal ZrN films, 830 nm thick, are grown on MgO(001) at 450 °C by magnetically unbalanced reactive magnetron sputtering. The combination of high-resolution x-ray diffraction reciprocal lattice maps, high-resolution cross-sectional transmission electron microscopy, and selected-area electron diffraction shows that ZrN grows epitaxially on MgO(001) with a cube-on-cube orientational relationship, (001){sub ZrN}?(001){sub MgO} and [100]{sub ZrN}?[100]{sub MgO}. The layers are essentially fully relaxed with a lattice parameter of 0.4575 nm, in good agreement with reported results for bulk ZrN crystals. X-ray reflectivity results reveal that the films are completely dense with smooth surfaces (roughness = 1.3 nm, consistent with atomic-force microscopy analyses). Based on temperature-dependent electronic transport measurements, epitaxial ZrN/MgO(001) layers have a room-temperature resistivity ?{sub 300K} of 12.0 ??-cm, a temperature coefficient of resistivity between 100 and 300 K of 5.6 × 10{sup ?8}?-cm K{sup ?1}, a residual resistivity ?{sub o} below 30 K of 0.78 ??-cm (corresponding to a residual resistivity ratio ?{sub 300?}/?{sub 15K} = 15), and the layers exhibit a superconducting transition temperature of 10.4 K. The relatively high residual resistivity ratio, combined with long in-plane and out-of-plane x-ray coherence lengths, ?{sub ?} = 18 nm and ?{sub ?} = 161 nm, indicates high crystalline quality with low mosaicity. The reflectance of ZrN(001), as determined by variable-angle spectroscopic ellipsometry, decreases slowly from 95% at 1 eV to 90% at 2 eV with a reflectance edge at 3.04 eV. Interband transitions dominate the dielectric response above 2 eV. The ZrN(001) nanoindentation hardness and modulus are 22.7 ± 1.7 and 450 ± 25 GPa.

Mei, A. B.; Zhang, C.; Sardela, M.; Eckstein, J. N.; Rockett, A. [Departments of Materials Science, Physics, and the Materials Research Laboratory, University of Illinois, 104 South Goodwin, Urbana, Illinois 61801 (United States)] [Departments of Materials Science, Physics, and the Materials Research Laboratory, University of Illinois, 104 South Goodwin, Urbana, Illinois 61801 (United States); Howe, B. M. [Air Force Research Laboratory, Wright Patterson Air Force Base, Dayton, Ohio 45433-7817 (United States)] [Air Force Research Laboratory, Wright Patterson Air Force Base, Dayton, Ohio 45433-7817 (United States); Hultman, L. [Thin Film Physics Division, Department of Physics (IFM), Linköping University, SE-58183 Linköping (Sweden)] [Thin Film Physics Division, Department of Physics (IFM), Linköping University, SE-58183 Linköping (Sweden); Petrov, I.; Greene, J. E. [Departments of Materials Science, Physics, and the Materials Research Laboratory, University of Illinois, 104 South Goodwin, Urbana, Illinois 61801 and Thin Film Physics Division, Department of Physics (IFM), Linköping University, SE-58183 Linköping (Sweden)] [Departments of Materials Science, Physics, and the Materials Research Laboratory, University of Illinois, 104 South Goodwin, Urbana, Illinois 61801 and Thin Film Physics Division, Department of Physics (IFM), Linköping University, SE-58183 Linköping (Sweden)

2013-11-15T23:59:59.000Z

174

Am phases in the matrix of a U-Pu-Zr alloy with Np, Am, and rare-earth elements  

SciTech Connect (OSTI)

Phases and microstructures in the matrix of an as-cast U-Pu-Zr alloy with 3 wt% Am, 2% Np, and 8% rare-earth elements were characterized by scanning and transmission electron microscopy. The matrix consists primarily of two phases, both of which contain Am: ?-(U, Np, Pu, Am) (~70 at% U, 5% Np, 14% Pu, 1% Am, and 10% Zr) and ?-(U, Np, Pu, Am)Zr2 (~25% U, 2% Np, 10-15% Pu, 1-2% Am, and 55-60 at% Zr). These phases are similar to those in U-Pu-Zr alloys, although the Zr content in ?-(U, Np, Pu, Am) is higher than that in ?-(U, Pu) and the Zr content in ?-(U, Np, Pu, Am)Zr2 is lower than that in ?-UZr2. Nanocrystalline actinide oxides with structures similar to UO2 occurred in some areas, but may have formed by reactions with the atmosphere during sample handling. Planar features consisting of a central zone of ?-(U, Np, Pu, Am) bracketed by zones of ?-(U, Np, Pu, Am)Zr2 bound irregular polygons ranging in size from a few micrometers to a few tens of micrometers across. The rest of the matrix consists of elongated domains of ?-(U, Np, Pu, Am) and ?-(U, Np, Pu, Am)Zr2. Each of these domains is a few tens of nanometers across and a few hundred nanometers long. The domains display strong preferred orientations involving areas a few hundred nanometers to a few micrometers across.

Dawn E Janney; J. Rory Kennedy; James W. Madden; Thomas P. O'Holleran

2015-01-01T23:59:59.000Z

175

Diffusional Interaction between U – 10wt.% Zr and Fe at 903K, 923K and 953K  

SciTech Connect (OSTI)

U-Zr metallic fuels cladded in Fe-alloys are being considered for application in an advanced Sodium-Cooled Fast Reactor (SFR) that can recycle the U-Zr fuels and minimize the long-lived actinide waste. To understand the complex fuel-cladding chemical interaction between the U-Zr metallic fuel with Fe-alloys, a systematic multicomponent diffusion study was carried out using solid-to-solid diffusion couples. The U-10 wt.% Zr vs. pure Fe diffusion couples were assembled and annealed at temperatures, 903, 923 and 953K for 96 hours. Development of microstructure, phase constituents, and compositions developed during the thermal anneals were examined by scanning electron microscopy, transmission electron microscopy and X-ray energy dispersive spectroscopy. Complex microstructure consisting of several layers that include phases such as U6Fe, UFe2, ZrFe2, alpha-U, betha-U, Zr-precipitates, ?, e and ? were observed. Multi-phase layers were grouped based on phase constituents and microstructure, and the layer thicknesses were measured to calculate the growth constant and activation energy. The local average compositions through the interaction layer were systematically determined, and employed to construct semi-quantitative diffusion paths on isothermal U-Zr-Fe ternary phase diagrams at respective temperatures. The diffusion paths were examined to qualitatively estimate the diffusional behavior of individual components and their interactions. Furthermore, selected area diffraction analyses were carried out to determine, for the first time, the exact crystal structure and composition of ?, e and ?-phases. The ?, e and ?-phases were identified as Pnma(62) Fe(Zr,U), I4/mcm(140) Fe(Zr,U)2, and I4/mcm(140) U3(Zr,Fe), respectively.

K Y. Park; K. Huang; A. Ewh; Y.H. Sohn; B. H. Sencer; J. R. Kennedy

2015-01-01T23:59:59.000Z

176

ECONOMICS BA DEGREE MAJOR REQUIREMENTS FLOWCHART FOR ACADEMIC YEAR 2012-2013  

E-Print Network [OSTI]

ECONOMICS BA DEGREE MAJOR REQUIREMENTS FLOWCHART FOR ACADEMIC YEAR 2012-2013 (see http://www.catalog.sdes.ucf.edu/) All B.A. Economics majors will be required to take a minimum of seven (7) electives by choosing from the following: PREREQUISITES REQUIRED ECO 3223 Money and Banking ECO 3410 Mathematical Economics ECO 3703

Wu, Shin-Tson

177

Energy loss of relativistic heavy ions in matter B.A. Weaver*, A.J. Westphal  

E-Print Network [OSTI]

Energy loss of relativistic heavy ions in matter B.A. Weaver*, A.J. Westphal Space Sciences.50.Bw Keywords: Energy loss; Stopping power; Heavy ions 1. Introduction The theory of energy loss has.: + 1-510-642-9733; fax: + 1- 510-643-7629. E-mail address: weaver@curium.ssl.berkeley.edu (B.A. Weaver

Leung, Pui-Tak "Peter"

178

E-Print Network 3.0 - ag cd ba Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

, 15, 10, 5, and 0 nm . Device Thickness of BaAgITO nm EL max a nm L at 100 cdm2 lmW ext at 100 cd... Top-emitting organic light-emitting diodes with BaAgindium tin...

179

Roadmap: Classics Latin Concentration Bachelor of Arts [AS-BA-CLSS-LAT  

E-Print Network [OSTI]

Roadmap: Classics ­ Latin Concentration ­ Bachelor of Arts [AS-BA-CLSS-LAT] College of Arts Updated: 11-Jun-12/LNHD This roadmap is a recommended semester-by-semester plan of study for this major;Roadmap: Classics ­ Latin Concentration ­ Bachelor of Arts [AS-BA-CLSS-LAT] College of Arts and Sciences

Sheridan, Scott

180

Roadmap: German Literature, Culture and Translation Bachelor of Arts [AS-BA-GLCT  

E-Print Network [OSTI]

Roadmap: German Literature, Culture and Translation ­ Bachelor of Arts [AS-BA-GLCT] College of Arts Updated: 24-May12/LNHD This roadmap is a recommended semester-by-semester plan of study for this major;Roadmap: German Literature, Culture and Translation ­ Bachelor of Arts [AS-BA-GLCT] College of Arts

Sheridan, Scott

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


181

Preparation of BaTiO3 nanoparticles by combustion spray pyrolysis Sangjin Leea  

E-Print Network [OSTI]

], hydrothermal [6], and spray pyrolysis [7­9] have been developed to prepare stoichiometric, ultra- fine BaTiO3 process. Hydrothermal BaTiO3 powders [6] are usually a paraelectric cubic phase, which needs additional freedom from hydrocarbon-based chem- icals, and thus avoiding carbon-contamination problems. As a result

Messing, Gary L.

182

The effect of BaCO3 on the hydration of OPC and composite cements  

E-Print Network [OSTI]

The effect of BaCO3 on the hydration of OPC and composite cements Claire A. Utton* and Neil B of ordinary Portland cement (OPC) and up to 90% blast furnace slag (BFS), are used to encapsulate Intermediate. The effect of BaCO3 on the hydration properties of composite cements is being studied. This paper reports

Sheffield, University of

183

The Catalytic Chemistry of HCN+NO over Na- and Ba-Y, FAU: An...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

The Catalytic Chemistry of HCN+NO over Na- and Ba-Y, FAU: An In Situ FTIR and TPDTPR Study. The Catalytic Chemistry of HCN+NO over Na- and Ba-Y, FAU: An In Situ FTIR and TPDTPR...

184

A facile method for the preparation of Eu{sup 2+}-doped nanocrystalline BaFCl  

SciTech Connect (OSTI)

Graphical abstract: - Highlights: • A facile co-precipitation method for the preparation of Eu{sup 2+}-doped BaFCl. • Reduction of Eu{sup 3+} to Eu{sup 2+} by zinc granular under nitrogen flow. • Photoluminescence and cathodoluminescence spectroscopy of the as-prepared BaFCl:Eu{sup 2+}. • Temperature dependent photoluminescence properties of Eu{sup 2+} ions in BaFCl. - Abstract: A facile method for the preparation of Eu{sup 2+}-doped BaFCl is reported. The method is based on the co-precipitation of aqueous solutions of BaCl{sub 2} and NH{sub 4}F to yield BaFCl. The doping by europium in the 2+ oxidation state is realized by the reduction of Eu{sup 3+} to Eu{sup 2+} employing granular zinc in the BaCl{sub 2} solution under nitrogen. Powder X-ray diffraction and electron microscopy have been used to confirm the BaFCl phase and photoluminescence, in the temperature range of 2.5–290 K, and room-temperature cathodoluminescence spectra have been measured to characterize the Eu{sup 2+} ions in the sample.

Wang, Xianglei; Liu, Zhiqiang [School of Physical, Environmental and Mathematical Sciences, The University of New South Wales, UNSW Canberra (ADFA), Canberra, ACT 2600 (Australia); Stevens-Kalceff, Marion A. [School of Physics and Electron Microscope Unit, Mark Wainwright Analytical Centre, The University of New South Wales, Sydney, NSW 2052 (Australia); Riesen, Hans, E-mail: h.riesen@adfa.edu.au [School of Physical, Environmental and Mathematical Sciences, The University of New South Wales, UNSW Canberra (ADFA), Canberra, ACT 2600 (Australia)

2013-10-15T23:59:59.000Z

185

Submillimeter and microwave residual losses in epitaxial films of Y-Ba-Cu-O and Tl-Ca-Ba-Cu-O  

SciTech Connect (OSTI)

We have used a novel bolometric technique and a resonant technique to obtain accurate submillimeter and microwave residual loss data for epitaxial thin films of YBa{sub 2}Cu{sub 3}O{sub 7}, Tl{sub 2}Ca{sub 2}Ba{sub 2}Cu{sub 3}O{sub 10} and Tl{sub 2}CaBa{sub 2}Cu{sub 2}O{sub 8}. For all films we obtain good agreement between the submillimeter and microwave data, with the residual losses in both the Y-Ba-Cu-O and Tl-Ca-Ba-Cu-O films scaling approximately as frequency squared below {approximately} 1 THz. We are able to fit the losses in the Y-Ba-Cu-O films to a weakly coupled grain model for the a-b plane conductivity, in good agreement with results from a Kramers-Kronig analysis of the loss data. We observe strong phonon structure in the Tl-Ca-Ba-Cu-O films for frequencies between 2 and 21 THz, and are unable to fit these losses to the simple weakly coupled grain model. This is in strong contrast to the case for other high {Tc} superconductors such as YBa{sub 2}Cu{sub 3}O{sub 7}, where phonon structure observed in ceramic samples is absent in epitaxial oriented films and crystals because of the electronic screening due to the high conductivity of the a-b planes.

Miller, D.; Richards, P.L. [Lawrence Berkeley Lab., CA (United States); Garrison, S.M.; Newman, N. [Conductus, Inc., Sunnyvale, CA (United States); Eom, C.B.; Geballe, T.H. [Stanford Univ., CA (United States). Dept. of Applied Physics; Etemad, S.; Inam, A.; Venkatesan, T. [Bell Communications Research, Inc., Red Bank, NJ (United States); Martens, J.S. [Sandia National Labs., Albuquerque, NM (United States); Lee, W.Y. [International Business Machines Corp., San Jose, CA (United States); Bourne, L.C. [Superconductor Technologies, Inc., Santa Barbara, CA (United States)

1992-03-01T23:59:59.000Z

186

Modeling of Zircon (ZrSiO{sub 4}) and Zirconia (ZrO{sub 2}) using ADF-GUI Software  

SciTech Connect (OSTI)

Natural zircon (ZrSiO{sub 4}) has very high concentration of Uranium and Thorium of up to 5000 ppm. Radioactive decay process of alpha particles from these impurities affects some changes like several atomic displacements in the crystalline structure of zircon. The amount of track density caused by alpha particles decay process of these radioactive materials in zircon can be decreased with annealing temperatures from 700 deg. C to 980 deg. C. Recently it has been extensively studied as the possible candidate material for immobilization of fission products and actinides. Besides, zirconia (ZrO{sub 2}), product from natural zircon, is widely used in industrial field because it has excellent chemical and mechanical properties at high temperature. Dielectric constant of monoclinic, cubic and tetragonal ZrO{sub 2} can be found in the range of 22, 35 and 50 by computer simulation works. In recent years, atomistic simulations and modeling have been studied, because a lot of computational techniques can offer atomic-level approaching with minimum errors in estimations. One favorite methods is Density Functional Theory (DFT). In this study, ADF-GUI software from DFT will be used to calculate the frequency and absorption Intensity of zircon and zirconia molecules. The data from calculations will be verified with experimental works such as Raman Spectroscopy, AFM and XRD.

Lwin, Maung Tin Moe [Applied Radiation Laboratory, Department of Physics, Faculty of Science, University of Malaya, 50603 Kuala Lumpur (Malaysia); Amin, Yusoff Mohd; Kassim, Hasan Abu; Kamaluddin, Burhanuddin [Department of Physics, Faculty of Science, University of Malaya, 50603 Kuala Lumpur (Malaysia)

2010-07-07T23:59:59.000Z

187

Oklahoma State University Honors Degrees (May. 1969 -May, 2013) Barber Frank A. Chemistry (B.A.) AS MAY 1969  

E-Print Network [OSTI]

.A.) AS MAY 1976 McGuigan Patrick B. History (B.A.) AS MAY 1976 Holmes William J. Humanities (B.A.) AS MAY.S.) AS MAY 1969 Seebo Thomas C. II Political Science (B.A.) AS MAY 1970 Stewart Elisabeth French (B Charles E. Spanish (B.A.) AS DEC 1972 Miller Amanda K. English (B.S.) AS MAY 1973 Potts Jon R. III History

Veiga, Pedro Manuel Barbosa

188

Catalytic decomposition of Ba(NO3)2 on Pt(111)  

SciTech Connect (OSTI)

The decomposition of Ba(NO3)2 formed on BaO/Pt(111) (Pt(111) surface is partially covered by BaO) in the presence of CO was studied using temperature programmed desorption (TPD), infrared reflection absorption (IRA) and X-ray photoelectron (XP) spectroscopies. The exposure of BaO/Pt(111) to elevated NO2 pressure (1.0×10-4 Torr) at 450 K leads to the formation of Ba(NO3)2, chemisorbed O (OPt) and Pt-oxide-like domains. During TPD, the Ba(NO3)2 begins to thermally decompose near 490 K, releasing NO and NO2 with the maximum NOx desorption rate seen at 605 K. The OPt species formed following the exposure of BaO/Pt(111) to NO2 react with CO to release CO2 at 450 K. The consumption of OPt during CO oxidation initiates the migration of O from the Pt-oxide-like domains to the chemisorbed phase, where the CO oxidation reaction occurs. Therefore, the removal of OPt by CO leads to the reduction of oxidized Pt, and to the formation of metallic Pt(111) domains, where, subsequently, catalytic decomposition of Ba(NO3)2 can take place. The Pt-catalyzed decomposition of Ba(NO3)2 occurs readily at 450 K, a temperature much lower than the onset of the decomposition temperature of Ba(NO3)2 in the presence of oxidized Pt. This work was supported by the US Department of Energy Basic Energy Sciences' Chemical Sciences, Geosciences & Biosciences Division. Pacific Northwest National Laboratory is operated by Battelle for the US Department of Energy.

Mudiyanselage, Kumudu; Weaver, Jason F.; Szanyi, Janos

2011-04-07T23:59:59.000Z

189

Synthesis and magnetic properties of the double layer perovskite CeBaFe2O5+w  

E-Print Network [OSTI]

Synthesis and magnetic properties of the double layer perovskite CeBaFe2O5+w R. L. de Almeida,1 O The synthesis, crystallographic structure, and magnetic properties of polycrystalline single-phase samples of CeBaFe results on the successful prepara- tion and characterization of polycrystalline CeBaFe2O5+w samples. Ideal

de Lima, Oscar Ferreira

190

Hydrothermal Synthesis of Dy-Doped BaTiO3 Powders ERSIN E. OREN and A. CUNEYT TAS  

E-Print Network [OSTI]

. Hydrothermal processing sis method used and temperature, may exhibit four different of BaTiO3 powders has) are "ferroelectric." hydrothermal processing required a pH 12 in the aqueous BaTiO3 is of the tetragonal symmetryHydrothermal Synthesis of Dy-Doped BaTiO3 Powders ERSIN E. OREN and A. CUNEYT TAS Submicron

Tas, A. Cuneyt

191

Complexity of shear localization in a Zr-based bulk metallic glass  

E-Print Network [OSTI]

University of Aeronautics and Astronautics, Beijing 100191, China The compressive behaviour of a Zr. A significant advance occurred when compositions and copper mold casting method allowing for bulk material the consequence of) macroscopic shear banding remains unclear. It is therefore important to carry out in situ

192

Complexity of shear localization in a Zr-based bulk metallic glass  

E-Print Network [OSTI]

University of Aeronautics and Astronautics, Beijing 100191, China The compressive behaviour of a Zr. A significant advance occurred when compositions and copper mold casting method allowing for bulk material unclear. It is therefore important to carry out in situ observations of plastic deformation processes

193

Stress-corrosion fatiguecrack growth in a Zr-based bulk amorphous metal  

E-Print Network [OSTI]

Stress-corrosion fatigue­crack growth in a Zr-based bulk amorphous metal V. Schroeder 1 , R metallic glass; Amorphous metal; Fatigue; Stress corrosion; Crack growth 1. Introduction In recent years­crack growth resistance [1­5], its corresponding properties in the presence of a corrosive environment have

Ritchie, Robert

194

Phase Stability and Thermodynamic Assessment of the Np-Zr system  

E-Print Network [OSTI]

Metallic fuels have an important role to play in "fast breeder" Gen-IV type nuclear reactors, and U-Pu-Zr is one of the prototypical systems. Because of the variability in fuel chemistry during burn-up, it is important to understand the effect...

Bajaj, Saurabh

2012-02-14T23:59:59.000Z

195

Discovery of Critical Oxygen Content for Glass Formation in Zr80Pt20 Melt Spun Ribbons  

SciTech Connect (OSTI)

Zr{sub 80}Pt{sub 20} alloys may form meta-stable quasicrystals either during devitrification of an amorphous phase or directly upon cooling from a liquid depending on processing conditions. To date, little attention has been given to the role of oxygen on the glass formation or devitrification behavior of Zr-Pt and similar alloys. This study reveals that oxygen content during melt spinning indeed strongly influences the formation of the as-quenched structure. A critical amount of oxygen was found to be required to form amorphous ribbons at a fixed quench rate. At lower oxygen levels (i.e., <500 ppm mass), a fully crystallized is formed; the structure is composed mainly of meta-stable {beta}-Zr with a small fraction of a quasicrystalline phase. At higher oxygen levels, the as-quenched structure transitions to a fully amorphous structure ({approx}1000 ppm mass), and with further oxygen addition forms a mixture of amorphous and quasicrystalline ({approx}1500 ppm mass) or crystalline phases (>2500 ppm mass). Details regarding the structure of the meta-stable {beta}-Zr phase in the low-oxygen ribbons are provided along with a discussion of the structural similarity between this phase and the quasicrystal structure that formed in this alloy.

D.J. Sordelet; E.A. Rozhkova; X. Yang; M.J. Kramer

2004-09-30T23:59:59.000Z

196

Oxide Electronic Conductivity and Hydrogen Pickup Fraction in Zr alloys Adrien Coueta  

E-Print Network [OSTI]

hydrogen ingress can cause cladding embrittlement and limit cladding lifetime. However, mechanisticOxide Electronic Conductivity and Hydrogen Pickup Fraction in Zr alloys Adrien Coueta , Arthur T, 77818 Moret-sur-Loing, France INTRODUCTION The hydrogen pick-up during cladding corrosion is a critical

Motta, Arthur T.

197

Chemical Synthesis of Pure and Gd-doped CaZrO3 Powders  

E-Print Network [OSTI]

chemical synthesis techniques: (i) self-propagating combustion synthesis, and (ii) precipitation potential use as a high-temperature thermistor material.8 The electrical response of calcium zirconate (preChemical Synthesis of Pure and Gd-doped CaZrO3 Powders I. Erkin Gonenli a and A. CuĂ? neyt Tas b

Tas, A. Cuneyt

198

ACCEPTED MANUSCRIPT The behaviour of Rare-Earth Elements, Zr and Hf during biologically-mediated  

E-Print Network [OSTI]

ACCEPTED MANUSCRIPT ACCEPTED MANUSCRIPT 1 The behaviour of Rare-Earth Elements, Zr and Hf during.a,b* , Cangemi M.a , Brusca L.c , Madonia P.c , Saiano F.d , Zuddas P.e a) Department of Earth and Marine at the solid-liquid interface influencing the distribution of trace elements onto microbial surfaces. Since

199

Thermoluminescence of ZrSiO4 (zircon): A new dating method?  

E-Print Network [OSTI]

Thermoluminescence of ZrSiO4 (zircon): A new dating method? H.J. van Es a , D.I. Vainshtein a , A (TL) dating of sediments from the Quaternary. TL of zircon results predominantly from internal0168-583X(02)00627-4 #12;Heavily damaged grains significantly reduce the thermoluminescence (TL) light

Donoghue, Joseph

200

Defining the Proton Topology of the Zr6Based Metal-Organic Framework NU-1000  

E-Print Network [OSTI]

,16-19 heavy metal capture,20,21 sensing,12 ionic conductivity,22 toxic industrial chemical capture,23Defining the Proton Topology of the Zr6Based Metal-Organic Framework NU-1000 Nora Planas,, Joseph E of Science, King Abdulaziz University, Jeddah, Saudi Arabia *S Supporting Information ABSTRACT: Metal

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


201

High temperature ablation resistance of ZrNp reinforced W matrix composites  

E-Print Network [OSTI]

modulus of elasticity, good thermal shock resistance, stiffness and good high temperature strengthHigh temperature ablation resistance of ZrNp reinforced W matrix composites Malik Adeel Umer microscopy (SEM) For the purpose of improving the high temperature ablation resistance of tungsten

Hong, Soon Hyung

202

Recent BaBar Results on Hadron Spectroscopy  

SciTech Connect (OSTI)

Recent results from on hadronic spectroscopy are presented, based on data collected by the BaBar experiment between 1999 and 2004. The properties of the recently discovered D*{sub sJ}(2317){sup +} and D{sub sJ}(2460){sup +} states are studied: resonance parameters and ratios of decay rates are measured from continuum e{sup +}e{sup -} production, and production rates are measured from B decays. A search for the D*{sub sJ}(2632){sup +} state whose observation has been recently reported by the SELEX Collaboration, and a search for a charged partner of the charmonium-like X(3872) state, are performed, yielding negative results. Finally, extensive searches for several pentaquark candidates, both fully inclusive and in B decays, result in no positive evidence.

Robutti, E.; /INFN, Genoa

2005-08-29T23:59:59.000Z

203

Determination of transition frequencies in a single $^{138}$Ba$^{+}$ ion  

E-Print Network [OSTI]

Transition frequencies between low-lying energy levels in a single trapped $^{138}$Ba$^{+}$ ion have been measured with laser spectroscopy referenced to an optical frequency comb. By extracting the frequencies of one-photon and two-photon components of the line shape using an eight-level optical Bloch model, we achieved 0.1 MHz accuracy for the 5d $^{2}$D$_{3/2}$ - 6p $^{2}$P$_{1/2}$ and 6s $^{2}$S$_{1/2}$ - 5d $^{2}$D$_{3/2}$ transition frequencies, and 0.2 MHz for the 6s $^{2}$S$_{1/2}$ - 6p $^{2}$P$_{1/2}$ transition frequency.

Dijck, E A; Grier, A T; Jungmann, K; Mohanty, A; Valappol, N; Willmann, L

2015-01-01T23:59:59.000Z

204

Composition and grain size effects on the structural and mechanical properties of CuZr nanoglasses  

SciTech Connect (OSTI)

Nanoglasses (NGs), metallic glasses (MGs) with a nanoscale grain structure, have the potential to considerably increase the ductility of traditional MGs while retaining their outstanding mechanical properties. We investigated the effects of composition on the structural and mechanical properties of CuZr NG films with grain sizes between 3 to 15?nm using molecular dynamics simulations. Results indicate a transition from localized shear banding to homogeneous superplastic flow with decreasing grain size, although the critical average grain size depends on composition: 5?nm for Cu{sub 36}Zr{sub 64} and 3?nm for Cu{sub 64}Zr{sub 36}. The flow stress of the superplastic NG at different compositions follows the trend of the yield stress of the parent MG, i.e., Cu{sub 36}Zr{sub 64} yield/flow stress: 2.54?GPa/1.29?GPa and Cu{sub 64}Zr{sub 36} yield/flow stress: 3.57?GPa /1.58?GPa. Structural analysis indicates that the differences in mechanical behavior as a function of composition are rooted at the distinct statistics of prominent atomic Voronoi polyhedra. The mechanical behavior of NGs is also affected by the grain boundary thickness and the fraction of atoms at interfaces for a given average grain size. The results suggest that the composition dependence of the mechanical behavior of NGs follows that of their parent MGs, e.g., a stronger MG will generate a stronger NG, while the intrinsic tendency for homogeneous deformation occurring at small grain size is not affected by composition.

Adibi, Sara [Institute of High Performance Computing, A*STAR, 138632 Singapore (Singapore); Mechanical Engineering Department, National University of Singapore, 117576 Singapore (Singapore); Branicio, Paulo S., E-mail: branicio@ihpc.a-star.edu.sg; Zhang, Yong-Wei [Institute of High Performance Computing, A*STAR, 138632 Singapore (Singapore); Joshi, Shailendra P., E-mail: Shailendra@nus.edu.sg [Mechanical Engineering Department, National University of Singapore, 117576 Singapore (Singapore)

2014-07-28T23:59:59.000Z

205

Synthesis and crystal structure of new layered BaNaSc(BO{sub 3}){sub 2} and BaNaY(BO{sub 3}){sub 2} orthoborates  

SciTech Connect (OSTI)

Crystals of two new layered BaNaSc(BO{sub 3}){sub 2} (I) and BaNaY(BO{sub 3}){sub 2} (II) orthoborates are grown from the melt-solution by the spontaneous crystallization onto the platinum loop. Single crystal X-ray analysis showed that the compounds are isostructural with the space group R3-bar, a=5.23944(12) and 5.3338(2) A, and c=34.5919(11) and 35.8303(19) A for I and II, respectively, Z=6. The distinctive feature of the structure is the close-packed composite anion-cation (Ba,Na)(BO{sub 3}) layers. The layers are combined into the base building packages of two types: {l_brace}M{sup 3+}[Ba{sup 2+}(BO{sub 3}){sup 3-}]{sub 2}{r_brace}{sup +} and {l_brace}M{sup 3+}[Na{sup +}(BO{sub 3}){sup 3-}]{sub 2}{r_brace}{sup -}, where M is Sc or Y. Neutral-charge two-package (four-layer) blocks are stacked by the rhombohedral principle into twelve layers of the cubic packing. - Graphical abstract: The distinctive feature of new orthoborate crystals BaNaSc(BO{sub 3}){sub 2} and BaNaY(BO{sub 3}){sub 2} is the combination of base building packages of two types: {l_brace}M{sup 3+}[Ba{sup 2+}(BO{sub 3}){sup 3-}]{sub 2}{r_brace}{sup +} and {l_brace}M{sup 3+}[Na{sup +}(BO{sub 3}){sup 3-}]{sub 2}{r_brace}{sup -}, where M is Sc or Y.

Seryotkin, Yurii V., E-mail: yuvs@uiggm.nsc.r [Institute of Geology and Mineralogy RAS, 3, Koptyuga avenue, 630090 Novosibirsk (Russian Federation); Novosibirsk State University, 2, Pirogova street, 630090 Novosibirsk (Russian Federation); Bakakin, Vladimir V. [Institute of Inorganic Chemistry RAS, 3, Lavrentieva avenue, 630090 Novosibirsk (Russian Federation); Kokh, Aleksandr E.; Kononova, Nadezhda G. [Institute of Geology and Mineralogy RAS, 3, Koptyuga avenue, 630090 Novosibirsk (Russian Federation); Svetlyakova, Tatyana N. [Institute of Geology and Mineralogy RAS, 3, Koptyuga avenue, 630090 Novosibirsk (Russian Federation); Novosibirsk State University, 2, Pirogova street, 630090 Novosibirsk (Russian Federation); Kokh, Konstantin A. [Institute of Geology and Mineralogy RAS, 3, Koptyuga avenue, 630090 Novosibirsk (Russian Federation); Drebushchak, Tatyana N. [Novosibirsk State University, 2, Pirogova street, 630090 Novosibirsk (Russian Federation); Institute of Solid State Chemistry and Mechanochemistry RAS, 18, Kutateladze street, 630128 Novosibirsk (Russian Federation)

2010-05-15T23:59:59.000Z

206

Thermodynamic Model for the Solubility of Ba(SeO4, SO4) Precipitates  

SciTech Connect (OSTI)

Abstract: The solubility of Ba(SeO4, SO4) precipitates was determined as a function of the BaSeO4 mole fractions, ranging from 0.0015 to 0.3830, and time with an equilibration period extending to as long as 302 days. Equilibrium/steady state conditions in this system are reached in ? 65 days. Pitzer’s ion interaction model was used to calculate solid and aqueous phase activity coefficients. Thermodynamic analyses showed that the data do not satisfy Gibbs-Duhem equation, thereby demonstrating that a single-solid solution phase does not control both the selenate and sulfate concentrations. Our extensive data with log 10 [Ba] ranging from ?3.6 to ?5.9 mol kg?1, log 10 [SeO4] rangingfrom?3.6 to -5.2 mol kg?1, and log 10 [SO4] ranging from?4.0 to ?5.3 mol kg?1 can be explained with the formation of an ideal BaSeO4 solid solution phase that controls the selenium concentrations and a slightly disordered/less-crystalline BaSO4(s) (log 10𝐾?sp = ?9.5 instead of ?10.05 for barite) that controls the sulfate concentrations. In these experiments the BaSO4 component of the solid solution phase never reaches thermodynamic equilibrium with the aqueous phase. Thermodynamic interpretations of the data show that both the ideal BaSeO4 solid solution phase and less-crystalline BaSO4 (s) phase are in equilibrium with each other in the entire range of BaSeO 4 mole fractions investigated in this study.

Rai, D.; Felmy, Andrew R.; Moore, Dean A.; Kitamura, Akira; Yoshikawa, Hideki; Doi, Reisuke; Yoshida, Yasushi

2014-08-15T23:59:59.000Z

207

Comment on `Update of 40K and 226Ra and 232Th series $\\gamma$-to-dose conversion factors for soil'  

E-Print Network [OSTI]

A letter to the editor of the Journal of Environmental Radioactivity on the article: E. Gasser, A. Nachab, A. Nourreddine, Ch. Roy, and A. Sellam, `Update of 40K and 226Ra and 232Th series $\\gamma$-to-dose conversion factors for soil', J. Environ. Radioactiv. 138, 68-71 (2014), DOI: 10.1016/j.jenvrad.2014.08.002.

Malins, Alex; Saito, Kimiaki

2015-01-01T23:59:59.000Z

208

Heating Greenhouses1 D.E. Buffington, R.A. Bucklin, R.W. Henley and D.B. McConnell2  

E-Print Network [OSTI]

AE11 Heating Greenhouses1 D.E. Buffington, R.A. Bucklin, R.W. Henley and D.B. McConnell2 1 supplemental heat is required. Obviously there are many ways this can be accomplished from the standpoint of these factors be considered when selecting and installing a heating system. HEATING SYSTEMS Greenhouse heating

Watson, Craig A.

209

SPECIAL NOTES FOR NIH PROPOSALS--Postdocs Any NIH proposal requires an eRA Commons user name; request one at  

E-Print Network [OSTI]

SPECIAL NOTES FOR NIH PROPOSALS--Postdocs Any NIH proposal requires an eRA Commons user name and the SF424 R &R guide (you can skip ahead to section I-32 of the latter) [http://grants1.nih://grants1.nih.gov/grants/funding/424/index.htm#inst If you have concerns about your visa status eligibility

Bustamante, Carlos

210

H.C. DORLAND, N.J. BEUKES, J. GUTZMER, D.A.D. EVANS AND R.A. ARMSTRONG SOUTH AFRICAN JOURNAL OF GEOLOGY, 2006, VOLUME 109 PAGE 139-156  

E-Print Network [OSTI]

H.C. DORLAND, N.J. BEUKES, J. GUTZMER, D.A.D. EVANS AND R.A. ARMSTRONG SOUTH AFRICAN JOURNAL.evans@yale.edu R.A. Armstrong Research School of Earth Sciences, Australian National University, Canberra, Australia e-mail: Richard.Armstrong@anu.edu.au © 2006 March Geological Society of South Africa ABSTRACT

211

Methane Combustion over Pd/ZrO2/SiC, Pd/CeO2/SiC, Pd/Zr0.5Ce0.5O2/SiC Catalysts  

E-Print Network [OSTI]

1 Methane Combustion over Pd/ZrO2/SiC, Pd/CeO2/SiC, Pd/Zr0.5Ce0.5O2/SiC Catalysts Xiaoning Guo a Laboratory of Coal Conversion, Institute of Coal Chemistry, Taiyuan 030001, PR China b GREMI UMR6606 CNRS0.5O2 solid solution) modified Pd/SiC catalysts for methane combustion are studied. XRD and XPS

Paris-Sud XI, Université de

212

Ab initio investigation of phase stability of Y2Ti2O7 and Y2Zr2O7...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

to the defect-cotunnite state under high pressure. Citation: Xiao HY, F Gao, and WJ Weber.2009."Ab initio investigation of phase stability of Y2Ti2O7 and Y2Zr2O7 under high...

213

Pressure Induced Structural Transformation in Gd2Ti2O7 and Gd2Zr2O7...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

in determining the pressure induced phase transformation. Citation: Xiao HY, and WJ Weber.2011."Pressure Induced Structural Transformation in Gd2Ti2O7 and Gd2Zr2O7."Journal of...

214

Charge-trapping characteristics of fluorinated thin ZrO{sub 2} film for nonvolatile memory applications  

SciTech Connect (OSTI)

The effects of fluorine treatment on the charge-trapping characteristics of thin ZrO{sub 2} film are investigated by physical and electrical characterization techniques. The formation of silicate interlayer at the ZrO{sub 2}/SiO{sub 2} interface is effectively suppressed by fluorine passivation. However, excessive fluorine diffusion into the Si substrate deteriorates the quality of the SiO{sub 2}/Si interface. Compared with the ZrO{sub 2}-based memory devices with no or excessive fluorine treatment, the one with suitable fluorine-treatment time shows higher operating speed and better retention due to less resistance of built-in electric field (formed by trapped electrons) against electron injection from the substrate and smaller trap-assisted tunneling leakage, resulting from improved ZrO{sub 2}/SiO{sub 2} and SiO{sub 2}/Si interfaces.

Huang, X. D., E-mail: eexdhuang@gmail.com, E-mail: laip@eee.hku.hk [Key Laboratory of MEMS of the Ministry of Education, Southeast University, Nanjing 210096 (China); Shi, R. P.; Lai, P. T., E-mail: eexdhuang@gmail.com, E-mail: laip@eee.hku.hk [Department of Electrical and Electronic Engineering, The University of Hong Kong, Pokfulam Road, Hong Kong (China)

2014-04-21T23:59:59.000Z

215

Electrochemical corrosion behavior of biomedical Ti22Nb and Ti22Nb6Zr alloys in saline medium  

E-Print Network [OSTI]

Electrochemical corrosion behavior of biomedical Ti­22Nb and Ti­22Nb­6Zr alloys in saline medium B addition and potentiodynamic polarization on the microstructure and corrosion resistance of Ti­22Nb and Ti­22Nb­6Zr alloy samples.The corrosion tests were carried out in 0.9% NaCl at 37 8C and neutral p

Zheng, Yufeng

216

E-Print Network 3.0 - amikhte ba estefade Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

T0THSCVFMKTG major 2011-12.doc Summary: see page 2 for requirements. See an advisor with questions. 2 BA 396 is also offered online, usually... fall term. Check E-campus...

217

Water-induced morphology changes in BaO/?-Al2O3 NOx storage...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

materials: an FTIR, TPD, and time-resolved synchrotron XRD Water-induced morphology changes in BaO?-Al2O3 NOx storage materials: an FTIR, TPD, and time-resolved synchrotron...

218

The George R. Brown School of Engineering Degrees Offered: BA, MStat, MA, PhD  

E-Print Network [OSTI]

Introduction to Engineering Computation · STAT 310 Probability and Statistics · STAT 410 Introduction246 Statistics The George R. Brown School of Engineering Degrees Offered: BA, MStat, MA, PhD Course engineering, computational and applied mathematics, managerial studies, mathematics, political science

Richards-Kortum, Rebecca

219

The George R. Brown School of Engineering Degrees Offered: BA, MStat, MA, PhD  

E-Print Network [OSTI]

Introduction to Engineering Computation · STAT 310 Probability and Statistics · STAT 410 Introduction253 Statistics The George R. Brown School of Engineering Degrees Offered: BA, MStat, MA, PhD Course engineering, computational and applied mathematics, managerial studies, mathematics, political science

Richards-Kortum, Rebecca

220

Devitrification kinetics and phase selection mechanisms in Cu-Zr metallic glasses  

SciTech Connect (OSTI)

Metallic glasses have been a promising class of materials since their discovery in the 1960s. Indeed, remarkable chemical, mechanical and physical properties have attracted considerable attention, and several excellent reviews are available. Moreover, the special group of glass forming alloys known as the bulk metallic glasses (BMG) become amorphous solids even at relatively low cooling rates, allowing them to be cast in large cross sections, opening the scope of potential applications to include bulk forms and net shape structural applications. Recent studies have been reported for new bulk metallic glasses produced with lower cooling rates, from 0.1 to several hundred K/s. Some of the application products of BMGs include sporting goods, high performance springs and medical devices. Several rapid solidification techniques, including melt-spinning, atomization and surface melting have been developed to produce amorphous alloys. The aim of all these methods is to solidify the liquid phase rapidly enough to suppress the nucleation and growth of crystalline phases. Furthermore, the production of amorphous/crystalline composite (ACC) materials by partial crystallization of amorphous precursor has recently given rise to materials that provide better mechanical and magnetic properties than the monolithic amorphous or crystalline alloys. In addition, these advances illustrate the broad untapped potential of using the glassy state as an intermediate stage in the processing of new materials and nanostructures. These advances underlie the necessity of investigations on prediction and control of phase stability and microstructural dynamics during both solidification and devitrification processes. This research presented in this dissertation is mainly focused on Cu-Zr and Cu-Zr-Al alloy systems. The Cu-Zr binary system has high glass forming ability in a wide compositional range (35-70 at.% Cu). Thereby, Cu-Zr based alloys have attracted much attention according to fundamental research on the behaviors of glass forming alloys. Further motivation arising from the application of this system as a basis for many BMGs and ACC materials; the Cu-Zr system warrants this attention and offers great potential for the development of new materials. However, the prediction and control of microstructural evolution during devitrification remains challenging because of the complex devitrification behavior of the Cu-Zr binary alloy which is arising from the competition of metastable and stable phases and diversity of crystal structures. This dissertation details a systematic fundamental investigation into the mechanisms and kinetics of the various crystallization transformation processes involved in the overall devitrification response of Cu-Zr and Cu-Zr-Al glasses. Various isothermal and nonisothermal treatments are employed, and the structural response is characterized using bulk X-ray and thermal analysis methods as well as nanoscale microscopic analysis methods, revealing structural and chemical details down to the atomic-scale. By carefully combining techniques such as differential scanning calorimetry (DSC), in-situ synchrotron high energy X-ray diffraction (HEXRD), and transmission electron microscopy (TEM) to quantify the characterization transformations, this research has uncovered numerous details concerning the atomistic mechanisms of crystallization and has provided much new understanding related to the dominant phases, the overall reaction sequences, and the rate-controlling mechanisms. As such this work represents a substantial step forward in understanding these transformations and provides a clear framework for further progress toward ultimate application of controlled devitrification processing for the production of new materials with remarkable properties.

Kalay, Ilkay

2010-12-15T23:59:59.000Z

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
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to obtain the most current and comprehensive results.


221

DENSITY-FUNCTIONAL STUDY OF U-Mo AND U-Zr ALLOYS  

SciTech Connect (OSTI)

Density-functional theory previously used to describe phase equilibria in U-Zr alloys [A. Landa, P. Soederlind, P.E.A. Turchi, J. Alloys Comp. 478 (2009) 103-110] is extended to investigate the ground-state properties of U-Mo solid solutions. We discuss how the heat of formation in both alloys correlates with the charge transfer between the alloy components, and how the specific behavior of the density of states in the vicinity of the Fermi level promotes the stabilization of the U{sub 2}Mo compound. Our calculations prove that, due to the existence of a single {gamma}-phase over the typical fuel operation temperatures, {gamma}-U-Mo alloys should indeed have much lower constituent redistribution than {gamma}-U-Zr alloys for which binodal decomposition causes a high degree of constituent redistribution.

Landa, A; Soderlind, P; Turchi, P A

2010-11-01T23:59:59.000Z

222

Permeability of CoNbZr amorphous thin films over a wide frequency range  

SciTech Connect (OSTI)

CoNbZr amorphous films have attracted the attention of many researchers because of their high saturation magnetization, high permeability, low coercivity, and nearly zero magnetostriction. For these films to be used, one of the important magnetic properties is the behavior of the permeability over a wide frequency range. We have measured the permeability of a square-shaped magnetic film (13 mm x 55 mm) sputtered on a glass substrate from 1 MHz to 400 MHz using a stripline. Over 400 MHz, the permeability of the magnetic film was measured using a ring-shaped sample mounted in a coaxial fixture. The wall motion permeability of CoNbZr amorphous films decreases from 1 kHz to nearly zero at 1 MHz. The rotation permeability is constant to 100 MHz and ferromagnetic resonance is observed near 1 GHz.

Koyama, H.; Tsujimoto, H.; Shirae, K.

1987-09-01T23:59:59.000Z

223

Narrow Bandgap in beta-BaZn2As2 and Its Chemical Origins  

E-Print Network [OSTI]

Beta-BaZn2As2 is known to be a p-type semiconductor with the layered crystal structure similar to that of LaZnAsO, leading to the expectation that beta-BaZn2As2 and LaZnAsO have similar bandgaps; however, the bandgap of beta-BaZn2As2 (previously-reported value ~0.2 eV) is one order of magnitude smaller than that of LaZnAsO (1.5 eV). In this paper, the reliable bandgap value of beta-BaZn2As2 is determined to be 0.23 eV from the intrinsic region of the tem-perature dependence of electrical conductivity. The origins of this narrow bandgap are discussed based on the chemi-cal bonding nature probed by 6 keV hard X-ray photoemission spectroscopy, hybrid density functional calculations, and the ligand theory. One origin is the direct As-As hybridization between adjacent [ZnAs] layers, which leads to a secondary splitting of As 4p levels and raises the valence band maximum. The other is that the non-bonding Ba 5dx2-y2 orbitals form unexpectedly deep conduction band minimum (CBM) in beta-BaZn2As2 although the CBM of L...

Xiao, Zewen; Ueda, Shigenori; Toda, Yoshitake; Ran, Fan-Yong; Guo, Jiangang; Lei, Hechang; Matsuishi, Satoru; Hosono, Hideo; Kamiya, Toshio

2015-01-01T23:59:59.000Z

224

Ferroelectric and ferromagnetic properties in BaTiO{sub 3} thin films on Si (100)  

SciTech Connect (OSTI)

In this paper, we report on the epitaxial integration of room temperature lead-free ferroelectric BaTiO{sub 3} thin (?1050?nm) films on Si (100) substrates by pulsed laser deposition technique through a domain matching epitaxy paradigm. We employed MgO and TiN as buffer layers to create BaTiO{sub 3}/SrRuO{sub 3}/MgO/TiN/Si (100) heterostructures. C-axis oriented and cube-on-cube epitaxial BaTiO{sub 3} is formed on Si (100) as evidenced by the in-plane and out-of-plane x-ray diffraction, and transmission electron microscopy. X-ray photoemission spectroscopic measurements show that Ti is in 4(+) state. Polarization hysteresis measurements together with Raman spectroscopy and temperature-dependent x-ray diffraction confirm the room temperature ferroelectric nature of BaTiO{sub 3}. Furthermore, laser irradiation of BaTiO{sub 3} thin film is found to induce ferromagnetic-like behavior but affects adversely the ferroelectric characteristics. Laser irradiation induced ferromagnetic properties seem to originate from the creation of oxygen vacancies, whereas the pristine BaTiO{sub 3} shows diamagnetic behavior, as expected. This work has opened up the route for the integration of room temperature lead-free ferroelectric functional oxides on a silicon platform.

Singamaneni, Srinivasa Rao, E-mail: ssingam@ncsu.edu; Prater, John T. [Materials Science Division, Army Research Office, Research Triangle Park, North Carolina 27709 (United States); Department of Materials Science and Engineering, North Carolina State University, Raleigh, North Carolina 27695 (United States); Punugupati, Sandhyarani; Hunte, Frank; Narayan, Jagdish [Department of Materials Science and Engineering, North Carolina State University, Raleigh, North Carolina 27695 (United States)

2014-09-07T23:59:59.000Z

225

Influence of multiphonon excitations and transfer on the fusion of Ca+Zr  

E-Print Network [OSTI]

Fusion data for $^{48}$Ca+$^{90,96}$Zr are analyzed by coupled-channels calculations that are based on the M3Y+repulsion, double-folding potential. By applying a previously determined nuclear density of $^{48}$Ca, the neutron densities of the zirconium isotopes are adjusted to optimize the fit to the fusion data, whereas the proton densities are determined by electron scattering experiments. It is shown that the fusion data can be explained fairly well by including couplings to one- and two-phonon excitations of the reacting nuclei and to one- and two-nucleon transfer reactions but there is also some sensitivity to multiphonon excitations. The neutron skin thicknesses extracted for the two zirconium isotopes are consistent with anti-proton measurements. The densities of the zirconium isotopes are used together with the previously determined nuclear density of $^{40}$Ca to calculate the M3Y+repulsion potentials and predict the fusion cross sections of $^{40}$Ca+$^{90,96}$Zr. The predicted cross sections for $^{40}$Ca+$^{90}$Zr are in reasonable agreement with the data when the influence of multiphonon excitations and a modest transfer is considered. The prediction of the $^{40}$Ca+$^{96}$Zr fusion cross section, on the other hand, is poor and under-predicts the data by 30 to 40%. Although couplings to transfer channels with positive $Q$ values were expected to play an important role, they are not able to explain the data, primarily because the predicted Coulomb barrier is about 1.5 MeV too high. Possible reasons for this failure are discussed.

H. Esbensen; A. M. Stefanini

2014-04-16T23:59:59.000Z

226

Measurements of the CKM Angle Alpha at BaBar  

SciTech Connect (OSTI)

The authors present improved measurements of the branching fractions and CP-asymmetries fin the B{sup 0} {yields} {pi}{sup +}{pi}{sup -}, B{sup 0} {yields} {pi}{sup 0}{pi}{sup 0}, and B{sup +} {yields} {rho}{sup +}{rho}{sup 0} decays, which impact the determination of {alpha}. The combined branching fractions of B {yields} K{sub 1}(1270){pi} and B {yields} K{sub 1}(1400){pi} decays are measured for the first time and allow a novel determination of {alpha} in the B{sup 0} {yields} {alpha}{sub 1}(1260){sup {+-}}{pi}{sup {-+}} decay channel. These measurements are performed using the final dataset collected by the BaBar detector at the PEP-II B-factory. The primary goal of the experiments based at the B factories is to test the Cabibbo-Kobayashi-Maskawa (CKM) picture of CP violation in the standard model of electroweak interactions. This can be achieved by measuring the angles and sides of the Unitarity Triangle in a redundant way.

Stracka, Simone; /Milan U. /INFN, Milan; ,

2012-04-04T23:59:59.000Z

227

A Novel Zr-1Nb Alloy and a New Look at Hydriding  

SciTech Connect (OSTI)

A novel Zr-1Nb has begun development based on a working model that takes into account the hydrogen permeabilities for zirconium and niobium metals. The beta-Nb secondary phase particles (SPPs) in Zr-1Nb are believed to promote more rapid hydrogen dynamics in the alloy in comparison to other zirconium alloys. Furthermore, some hydrogen release is expected at the lower temperatures corresponding to outages when the partial pressure of H2 in the coolant is less. These characteristics lessen the negative synergism between corrosion and hydriding that is otherwise observed in cladding alloys without niobium. In accord with the working model, development of nanoscale precursors was initiated to enhance the performance of existing Zr-1Nb alloys. Their characteristics and properties can be compared to oxide-dispersion strengthened alloys, and material additions have been proposed to zirconium-based LWR cladding to guard further against hydriding and to fix the size of the SPPs for microstructure stability enhancements. A preparative route is being investigated that does not require mechanical alloying, and 10 nanometer molybdenum particles have been prepared which are part of the nanoscale precursors. If successful, the approach has implications for long term dry storage of used fuel and for new routes to nanoferritic and ODS alloys.

Robert D. Mariani; James I. Cole; Assel Aitkaliyeva

2013-09-01T23:59:59.000Z

228

Search for compounds of the NaBaR(BO{sub 3}){sub 2} family (R = La, Nd, Gd, and Yb) and the new NaBaYb(BO{sub 3}){sub 2} orthoborate  

SciTech Connect (OSTI)

A search for compounds of the NaBaR(BO{sub 3}){sub 2} composition (where R = La{sup 3+}, Nd{sup 3+}, Gd{sup 3+}, or Yb{sup 3+}) is performed by solid state synthesis and spontaneous crystallization. A new compound, NaBaYb(BO{sub 3}){sub 2}, is found in this series. It crystallizes in space group R3{sup -} and belongs to the family of sublayer complex orthoborates with isolated BO{sub 3} groups NaBaR(BO{sub 3}){sub 2} (R = Y, Sc, and Yb). Theoretical X-ray powder diffraction patterns of NaBaY(BO{sub 3}){sub 2}, NaBaSc(BO{sub 3}){sub 2}, and NaBaYb(BO{sub 3}){sub 2} are calculated based on single-crystal data.

Svetlyakova, T. N., E-mail: svetlyakovatn@gmail.com; Kokh, A. E.; Kononova, N. G. [Russian Academy of Sciences, Sobolev Institute of Geology and Mineralogy, Siberian Branch (Russian Federation)] [Russian Academy of Sciences, Sobolev Institute of Geology and Mineralogy, Siberian Branch (Russian Federation); Fedorov, P. P. [Russian Academy of Sciences, Prokhorov General Physics Institute (Russian Federation)] [Russian Academy of Sciences, Prokhorov General Physics Institute (Russian Federation); Rashchenko, S. V. [Russian Academy of Sciences, Sobolev Institute of Geology and Mineralogy, Siberian Branch (Russian Federation)] [Russian Academy of Sciences, Sobolev Institute of Geology and Mineralogy, Siberian Branch (Russian Federation); Maillard, A. [University of Metz and Supelec, Laboratoire Materiaux Optiques, Photonique et Systemes (France)] [University of Metz and Supelec, Laboratoire Materiaux Optiques, Photonique et Systemes (France)

2013-01-15T23:59:59.000Z

229

STM images showing the morphology of BaO film (7 MLleft and 80 MLright) formed by the direct evaporation of the BaO.  

E-Print Network [OSTI]

Spectroscopy and Diffraction Group, EMSL, PNNL Wayne Goodman Department of Chemistry, Texas A&M University alumina film with a buffer layer, and/or the BaO clusters can be formed via direct sublimation of metal of trimethylacetic acid molecules on reduced TiO2(110) surface." Physical Chemistry Chemical Physics 12

230

Page 1 | B.A. in Special Education Adapted Curriculum | Academic Plan of Study Updated May 2014 B.A. in Special Education (Adapted Curriculum)  

E-Print Network [OSTI]

Page 1 | B.A. in Special Education ­ Adapted Curriculum | Academic Plan of Study Updated May 2014 B ­ Adapted Curriculum | Academic Plan of Study Updated May 2014 Special Education - Adapted Curriculum Areas.A. in Special Education (Adapted Curriculum) Academic Plan of Study College of Education Department of Special

Raja, Anita

231

The new Hg-rich barium indium mercurides BaIn{sub x}Hg{sub 7?x} (x=3.1) and BaIn{sub x}Hg{sub 11?x} (x=0–2.8)  

SciTech Connect (OSTI)

The title compounds BaIn{sub x}Hg{sub 7?x} (x=3.1(1)) and BaIn{sub x}Hg{sub 11?x} (x=0–2.8) were synthesized from stoichiometric ratios of the elements in Ta crucibles. Their crystal structures have been determined using single crystal X-ray data. BaIn{sub x}Hg{sub 7?x} (x=3.1(1)) crystallizes in a new structure type (orthorhombic, oC16, space group Cmmm: a=512.02(1), b=1227.68(3), c=668.61(2) pm, Z=2, R1=0.0311). In the structure, the atoms of the three crystallographically different mixed In/Hg positions form planar nets of four-, six- and eight-membered rings. These nets are shifted against each other such that the four-membered rings form empty distorted cubes. The cubes are connected via common edges, corners and folded ladders, which are also found in BaIn{sub 2}/BaHg{sub 2} (KHg{sub 2} structure type) and BaIn (?-NaHg type). The Ba atoms are centered in the eight-membered rings and exhibit an overall coordination number of 20. The [BaM{sub 20}] polyhedra and twice as many distorted [M{sub 8}] cubes tesselate the space. BaIn{sub 2.8}Hg{sub 8.2} (cubic, cP36, space group Pm3{sup Ż}m, a=961.83(1) pm, Z=3, R1=0.0243) is the border compound of the phase width BaIn{sub x}Hg{sub 11?x} of the rare BaHg{sub 11} structure type. In the structure, ideal [M{sub 8}] cubes (at the corners of the unit cell) and BaM{sub 20} polyhedra (at the edges of the unit cell) represent the building blocks comparable to the other new In mercuride. In accordance with the increased In/Hg content, additional M-pure regions appear: the center of the unit cell contains a huge [Hg(1)M(2){sub 12}M(3,4){sub 32}] polyhedron, a Hg-centered cuboctahedron of In/Hg atoms surrounded by a capped cantellated cube of 32 additional M atoms. For both structure types, the bonding situation and the ‘coloring’, i.e. the In/Hg distribution of the polyanionic network, are discussed considering the different sizes of the atoms and the charge distribution (Bader AIM charges), which have been calculated within the framework of FP-LAPW density functional theory. - Graphical abstract: BaIn{sub 2.6}Hg{sub 4.4}: distorted cubes [(In/Hg){sub 8}] (green, like in BaHg{sub 11}), folded ladders (violet, like in BaIn, BaHg{sub 2} and BaIn{sub 2}) and Ba coordination polyhedra [Ba(In/Hg){sub 20}] (blue, like in BaHg{sub 11}). - Highlights: • The Hg-rich In-mercuride BaIn{sub 3.1}Hg{sub 3.9} crystallizes with a singular structure type. • The phase width of the BaHg{sub 11} structure in BaIn{sub x}Hg{sub 11-x} ends at x=2.8. • The relations of both compounds with other alkaline-earth mercurides are outlined. • The Hg/In coloring of the polyanion is discussed considering the structure features. • Bonding aspects are explored using band structure calculations.

Wendorff, Marco; Schwarz, Michael; Röhr, Caroline, E-mail: caroline@ruby.chemie.uni-freiburg.de

2013-07-15T23:59:59.000Z

232

RE/ZrO{sub 2} (RE = Sm, Eu) composite oxide nano-materials: Synthesis and applications in photocatalysis  

SciTech Connect (OSTI)

Graphical abstract: - Highlights: • RE/ZrO{sub 2} (RE = Sm, Eu) nano-materials have been successfully synthesized. • Defect and electron structures determine the absorption properties on visible light. • Nano-sized Zr{sub 0.8}Sm{sub 0.2}O{sub 2??} has good visible-light-responsive photocatalytic activities. • In the future, it can be used in wastewater treatment and environmental protection. - Abstract: Zirconia modified by Samarium/Europium, RE/ZrO{sub 2} (RE = Sm, Eu), composite oxide nano-materials have been successfully synthesized by improved sol–gel method. Characterization results show that X-ray diffraction (XRD) peaks of products gradually shift to the lower angle with the increase of rare earth which implies that the lattice distances of RE/ZrO{sub 2} nano-materials are gradually enlarged. Moreover, the molar ratios between zirconium and rare earth are consistent with the chemical formula and both of them are uniformly distributed in samples. Optical properties indicate that defect structures and electron configurations of RE/ZrO{sub 2} (RE = Sm, Eu) with single phase determine their absorption properties on visible light. Photocatalytic experiments indicate Zr{sub 0.8}Sm{sub 0.2}O{sub 2??} nano-crystals have excellent visible-light-responsive photocatalytic activities on Methylene blue and Rhodamine B which results from the special defect structure, suitable electronic configuration, and larger specific surface area. It follows that Zr{sub 0.8}Sm{sub 0.2}O{sub 2??} nano-crystals are new visible-light-responsive photocatalysts which can be applied in dye wastewater treatment and environmental protection in the future.

Du, Weimin, E-mail: duweimin75@gmail.com [College of Chemistry and Chemical Engineering, Anyang Normal University, Anyang, Henan 455002 (China); Zhu, Zhaoqiang [College of Chemistry and Chemical Engineering, Anyang Normal University, Anyang, Henan 455002 (China); College of Chemistry and Molecular Engineering, Zhengzhou University, Zhengzhou, Henan 450001 (China); Zhang, Xiaofen; Wang, Dacheng; Liu, Donghe [College of Chemistry and Chemical Engineering, Anyang Normal University, Anyang, Henan 455002 (China); Qian, Xuefeng [School of Chemistry and Chemical Technology, Shanghai Jiao Tong University, Shanghai 200240 (China); Du, Jimin, E-mail: djm@aynu.edu.cn [College of Chemistry and Chemical Engineering, Anyang Normal University, Anyang, Henan 455002 (China)

2013-10-15T23:59:59.000Z

233

Self-organization during growth of ZrN/SiN{sub x} multilayers by epitaxial lateral overgrowth  

SciTech Connect (OSTI)

ZrN/SiN{sub x} nanoscale multilayers were deposited on ZrN seed layers grown on top of MgO(001) substrates by dc magnetron sputtering with a constant ZrN thickness of 40 Ĺ and with an intended SiN{sub x} thickness of 2, 4, 6, 8, and 15 Ĺ at a substrate temperature of 800 °C and 6 Ĺ at 500 °C. The films were investigated by X-ray diffraction, high-resolution scanning transmission electron microscopy, and energy dispersive X-ray spectroscopy. The investigations show that the SiN{sub x} is amorphous and that the ZrN layers are crystalline. Growth of epitaxial cubic SiN{sub x}—known to take place on TiN(001)—on ZrN(001) is excluded to the monolayer resolution of this study. During the course of SiN{sub x} deposition, the material segregates to form surface precipitates in discontinuous layers for SiN{sub x} thicknesses ?6 Ĺ that coalesce into continuous layers for 8 and 15 Ĺ thickness at 800 °C, and for 6 Ĺ at 500 °C. The SiN{sub x} precipitates are aligned vertically. The ZrN layers in turn grow by epitaxial lateral overgrowth on the discontinuous SiN{sub x} in samples deposited at 800 °C with up to 6 Ĺ thick SiN{sub x} layers. Effectively a self-organized nanostructure can be grown consisting of strings of 1–3 nm large SiN{sub x} precipitates along apparent column boundaries in the epitaxial ZrN.

Fallqvist, A.; Fager, H.; Hultman, L.; Persson, P. O. Ĺ. [Thin Film Physics Division, Department of Physics, Chemistry and Biology (IFM), Linköping University, SE-581 83 Linköping (Sweden)] [Thin Film Physics Division, Department of Physics, Chemistry and Biology (IFM), Linköping University, SE-581 83 Linköping (Sweden); Ghafoor, N. [Nanostructured Materials, Department of Physics, Chemistry and Biology (IFM), Linköping University, SE-581 83 Linköping (Sweden)] [Nanostructured Materials, Department of Physics, Chemistry and Biology (IFM), Linköping University, SE-581 83 Linköping (Sweden)

2013-12-14T23:59:59.000Z

234

Synthesis and crystal structure of CuZrTiO{sub 5}-A new crystal structure type  

SciTech Connect (OSTI)

A new compound, CuZrTiO{sub 5}, was synthesized as strongly pleochroic green crystals from the oxides between 995 and 1010 deg. C, 1 atm. Its crystal structure was determined by single crystal XRD, resulting in R (F{sup 2}>2sigma(F{sup 2}))=0.032 and wR (all data)=0.079). CuZrTiO{sub 5} is orthorhombic, space group P2{sub 1}2{sub 1}2{sub 1}, a=3.5871(3) A, b=6.6968(4) A, c=14.6679(9) A, V=352.35(4) A{sup 3}, Z=4. The structure is topologically similar to In{sub 2}TiO{sub 5} but differs in space group and cation coordination. CuZrTiO{sub 5} has relatively regular TiO{sub 6} polyhedra, but coordination is 7+1 for Zr, and 4+2 for Cu due to the Jahn-Teller effect. Ordering of the long Cu-O bonds causes reduction in symmetry relative to In{sub 2}TiO{sub 5}. Layers of Cu alternate with Ti+Zr on (001), giving rise to a distinct cleavage. Bond valence sums on Ti and Zr are far from ideal, which appears due to the limited ability of this structural topology to avoid close next-nearest neighbour distances. - Graphical abstract: The new compound CuZrTiO{sub 5} is orthorhombic (P2{sub 1}2{sub 1}2{sub 1}), with a=3.5871(3) A, b=6.6968(4) A, c=14.6679(9) A. The structure, determined with single crystal XRD, represents a new crystal structure type that is a slight distortion of that of In{sub 2}TiO{sub 5} but differs in space group and cation coordination.

Troitzsch, Ulrike [Research School of Earth Sciences, Australian National University, Canberra ACT 0200 (Australia); Christy, Andrew G., E-mail: Andrew.Christy@anu.edu.a [Research School of Earth Sciences, Australian National University, Canberra ACT 0200 (Australia); Willis, Anthony C. [Research School of Chemistry, Australian National University, Canberra ACT 0200 (Australia); Ellis, David J. [Research School of Earth Sciences, Australian National University, Canberra ACT 0200 (Australia)

2010-03-15T23:59:59.000Z

235

KCP R.A'S  

National Nuclear Security Administration (NNSA)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr May Jun Jul(Summary) "ofEarlyEnergyDepartmentNational NuclearhasAdministration77NuclearSecurity Campus PreproposalJordan |

236

Microsoft Word - Ra-15  

Broader source: Energy.gov (indexed) [DOE]

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE:1 First Use of Energy for All Purposes (Fuel and Nonfuel),Feet) Year Jan Feb Mar Apr May Jun Jul(Summary) "ofEarly Careerlumens_placard-green.eps MoreWSRC-STI-2007-00250 Rev. 05 Oak RidgeBob Charrow Date:

237

Structure investigation with the (p,t) reaction on {sup 132,134}Ba nuclei  

SciTech Connect (OSTI)

The low-lying excited states in {sup 132,134}Ba isotopes have been studied with high-resolution (p,t) reactions. The experiments were performed at the Munich Q3D spectrograph with a 25-MeV proton beam and the 1.5-m-long focal plane detector. The high-resolution triton spectra allowed the observation of levels up to {approx}4 MeV. The experimental results revealed 75 excited states in {sup 134}Ba and 79 in {sup 132}Ba, many of them observed for the first time. The measured angular distributions compared with distorted-wave Born approximation calculations allowed spin assignments for these levels in most cases. The systematics of the monopole and quadrupole two-neutron transfer strengths is compared with the prediction of the interacting boson approximation model. The results indicate a transitional structure in {sup 132}Ba and {sup 134}Ba and contribute additional evidence in favor of a description between the U(5) and O(6) symmetries of the model.

Pascu, S.; Cata-Danil, Gh. [National Institute for Physics and Nuclear Engineering, RO-77125 Bucharest-Magurele (Romania); Physics Department, Politehnica University of Bucharest, RO-060042 Bucharest (Romania); Bucurescu, D. [National Institute for Physics and Nuclear Engineering, RO-77125 Bucharest-Magurele (Romania); Academy of Romanian Scientists, 54 Splaiul Independentei, RO-050094 Bucharest (Romania); Marginean, N.; Zamfir, N. V. [National Institute for Physics and Nuclear Engineering, RO-77125 Bucharest-Magurele (Romania); Mueller, C. [Physics Department, Politehnica University of Bucharest, RO-060042 Bucharest (Romania); Graw, G.; Gollwitzer, A.; Hofer, D.; Valnion, B. D. [Fakultaet fuer Physik der Universitaet Muenchen, D-85748 Garching (Germany)

2010-01-15T23:59:59.000Z

238

Significant increase of Curie temperature in nano-scale BaTiO{sub 3}  

SciTech Connect (OSTI)

The low Curie temperature (T{sub c}?=?130?°C) of bulk BaTiO{sub 3} greatly limits its applications. In this work, the phase structures of BaTiO{sub 3} nanoparticles with sizes ranging from 2.5?nm to 10?nm were studied at various temperatures by using aberration-corrected transmission electron microscopy (TEM) equipped with an in-situ heating holder. The results implied that each BaTiO{sub 3} nanoparticle was composed of different phases, and the ferroelectric ones were observed in the shells due to the complicated surface structure. The ferroelectric phases in BaTiO{sub 3} nanoparticles remained at 600?°C, suggesting a significant increase of T{sub c}. Based on the in-situ TEM results and the data reported by others, temperature-size phase diagrams for BaTiO{sub 3} particles and ceramics were proposed, showing that the phase transition became diffused and the T{sub c} obviously increased with decreasing size. The present work sheds light on the design and fabrication of advanced devices for high temperature applications.

Li, Yueliang; Liao, Zhenyu; Fang, Fang; Zhu, Jing, E-mail: jzhu@mail.tsinghua.edu.cn [National Center for Electron Microscopy in Beijing, School of Materials Science and Engineering, State Key Laboratory of New Ceramics and Fine Processing, Laboratory of Advanced Materials (MOE), Tsinghua University, Beijing 100084 (China); Wang, Xiaohui; Li, Longtu [State Key Laboratory of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing 100084 (China)

2014-11-03T23:59:59.000Z

239

Diffusion-governed-asymmetric growth of amorphous layer under solid-state reaction in Ni-Zr multilayers  

SciTech Connect (OSTI)

A molecular-dynamics simulation with an n-body potential was performed to study solid-state amorphization in the Ni-Zr system upon annealing at medium temperatures ranging from 300 to 600 C. The models for simulation were a Zr-Ni-Zr sandwich consisting of both hcp Zr and fcc Ni (001) atomic planes and a bilayer with a thin preset disordered interfacial layer, respectively, for revealing the detailed amorphization process and the growing kinetics of an amorphous layer upon solid-state reaction. The simulation results demonstrated, for the first time, that the atomic process proceeded through first diffusion, then alloying and eventually amorphization. In other words, amorphization was controlled by a diffusion-limited reaction and the growth kinetics of the amorphous layer followed exactly a t{sup 1/2} law. Another interesting finding was that the growing speeds of the amorphous layer exhibited an asymmetric behavior, i.e, the amorphous layer extended faster towards Ni lattice than that directed to Zr side. Besides, it was also found that an initiation of amorphization upon annealing was dependent to the interfacial textures, i.e., amorphization could take place when the interfaces were composed of the more open atomic planes, whereas it was suppressed if the interfaces were constructed with the close-packed planes of both lattices.

Liu, B.X.; Lai, W.S. [Tsinghua Univ., Beijing (China). Dept. of Materials Science and Engineering

1998-12-31T23:59:59.000Z

240

A new class of materials with promising thermoelectric properties: MNiSn (M=Ti, Zr, Hf)  

SciTech Connect (OSTI)

TiNiSn, ZrNiSn and HfNiSn are members of a large group of intermetallic compounds which crystallize in the cubic MgAgAs-type structure. Polycrystalline samples of these compounds have been prepared and investigated for their thermoelectric properties. With thermopowers of about {minus}200 {micro}V/K and resistivities of a few m{Omega}cm, power factors S{sup 2}/{rho} as high as 38 {micro}W/K{sup 2}cm were obtained at 700 K. These remarkably high power factors are, however, accompanied by a thermal conductivity, solid solutions Zr{sub 1{minus}x}Hf{sub x}NiSn, Zr{sub 1{minus}x}Ti{sub x}NiSn, and Hf{prime}{sub 1{minus}x}Ti{sub x}NiSn were formed. The figure of merit of Zr{sub 0.5}Hf{sub 0.5}NiSn at 700 K (ZT = 0.41) exceeds the end members ZrNiSn (ZT = 0.26) and HfNiSn (ZT = 0.22).

Hohl, H.; Ramirez, A.P.; Kaefer, W.; Fess, K.; Thurner, Ch.; Kloc, Ch.; Bucher, E.

1997-07-01T23:59:59.000Z

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


241

EXPLAINING THE Sr AND Ba SCATTER IN EXTREMELY METAL-POOR STARS  

SciTech Connect (OSTI)

Compilations of abundances of strontium and barium in extremely metal-poor stars show that an apparent cutoff is observed for [Sr/Ba] at [Fe/H] < -3.6 and large fluctuations for [Fe/H] > -3.6 with a clear upper bound depending on metallicity. We study the factors that place upper limits on the logarithmic ratio [Sr/Ba]. A model is developed in which the collapses of type II supernovae are found to reproduce many of the features seen in the data. This model is consistent with galactic chemical evolution constraints of light-element enrichment in metal-poor stars. Effects of turbulence in an explosive site have also been simulated, and are found to be important in explaining the large scatter observed in the [Sr/Ba] data.

Aoki, W.; Suda, T.; Boyd, R. N.; Kajino, T.; Famiano, M. A., E-mail: aoki.wako@nao.ac.jp, E-mail: takuma.suda@nao.ac.jp, E-mail: richard11boyde@comcast.net, E-mail: kajino@nao.ac.jp, E-mail: michael.famiano@wmich.edu [National Astronomical Observatory of Japan, 2-21-1 Mitaka, Tokyo 181-8588 (Japan)

2013-03-20T23:59:59.000Z

242

Field-effect BaTiO{sub 3}-Si solar cells  

SciTech Connect (OSTI)

Conventional solar cells make use of the spatial variation in electronic environment due to junctions for charge separation. We investigated field-effect BaTiO{sub 3}-Si solar cells that utilize the bound surface charges of BaTiO{sub 3} to separate charge carriers in silicon. Rectifying behavior and photovoltaic effect were observed on cells with forward polarization. Theoretical simulation indicated that the induced electric field due to BaTiO{sub 3} polarization could extend into the silicon layer, which is consistent with experimental observations. In addition, adjusting relevant parameters may optimize the electric field distribution. The cells are promising in terms of material selection, device design, and fabrication.

Wang, Wentao; Liu, Fude, E-mail: fordliu@hku.hk; Man Lau, Chor; Wang, Lei; Yang, Guandong; Zheng, Dawei [Department of Mechanical Engineering, The University of Hong Kong, Pokfulam Road, Hong Kong (China); Li, Zhigang [Department of Mechanical and Aerospace Engineering, The Hong Kong University of Science and Technology, Hong Kong (China)

2014-03-24T23:59:59.000Z

243

Microstructural evolutions in converting epitaxial Tl2Ba2CaCu2Ox thin films to epitaxial HgBa2CaCu2O6+delta thin films  

E-Print Network [OSTI]

Superconducting HgBa2CaCu2O6+delta (Hg-1212) thin films were obtained from Tl2Ba2CaCu2Ox (Tl-2212) precursor films using a cation-exchange process. In this process, Tl cations on the precursor lattice were thermally excited and then replaced with Hg...

Wu, Judy; Siegal, M. P.; Xie, Y. Y.; Aytug, T.; Fang, L.

2003-02-01T23:59:59.000Z

244

Electron microscopy of phase and structural transformations in soft magnetic nanocrystalline Fe-Zr-N films  

SciTech Connect (OSTI)

The effect of deposition conditions (film thickness) on the structure of soft magnetic Fe{sub 80-78}Zr{sub 10}N{sub 10-12} films formed by reactive magnetron deposition on a heat-resistant glass substrate has been investigated by analytical transmission electron microscopy, high-resolution electron microscopy, and diffraction analysis. The processes of evolution of the phase and structural state of films and the film-substrate interface upon annealing in the temperature range of 200-650 Degree-Sign C have been analyzed taking into account the thermodynamic, kinetic, and structural factors and the specific features of the nanocrystalline state.

Zhigalina, O. M., E-mail: zhigal@ns.crys.ras.ru; Khmelenin, D. N. [Russian Academy of Sciences, Shubnikov Institute of Crystallography (Russian Federation)] [Russian Academy of Sciences, Shubnikov Institute of Crystallography (Russian Federation); Sheftel', E. N.; Usmanova, G. Sh. [Russian Academy of Sciences, Baikov Institute of Metallurgy and Materials Science (Russian Federation)] [Russian Academy of Sciences, Baikov Institute of Metallurgy and Materials Science (Russian Federation); Vasil'ev, A. L. [Russian Academy of Sciences, Shubnikov Institute of Crystallography (Russian Federation)] [Russian Academy of Sciences, Shubnikov Institute of Crystallography (Russian Federation); Carlsson, A. [FEI Company (Netherlands)] [FEI Company (Netherlands)

2013-03-15T23:59:59.000Z

245

Beta-decay properties of Zr and Mo neutron-rich isotopes  

E-Print Network [OSTI]

Gamow-Teller strength distributions, beta-decay half-lives, and beta-delayed neutron emission are investigated in neutron-rich Zr and Mo isotopes within a deformed quasiparticle random-phase approximation. The approach is based on a self-consistent Skyrme Hartree-Fock mean field with pairing correlations and residual separable particle-hole and particle-particle forces. Comparison with recent measurements of half-lives stresses the important role that nuclear deformation plays in the description of beta-decay properties in this mass region.

P. Sarriguren; J. Pereira

2010-06-08T23:59:59.000Z

246

Microstructural Characterization and Shape Memory Response of Ni-Rich NiTiHf and NiTiZr High Temperature Shape Memory Alloys  

E-Print Network [OSTI]

NiTiHf and NiTiZr high temperature shape memory alloys (HTSMAs) have drawn a great deal of attention as cheaper alternatives to Pt, Pd and Au alloyed NiTi-based HTSMAs while NiTiZr alloys also providing at least 20% weight reduction then its Ni...

Evirgen, Alper

2014-08-14T23:59:59.000Z

247

EUREM 12, Brno, Czech Republic, July 9-14, 2000 P 257 High yield incorporation of ZrCl4 into single wall carbon nanotubes  

E-Print Network [OSTI]

in a furnace, held at temperature for 1hr and then furnace cooled. The specimens were characterised using) show the filling product obtained from as-supplied ZrCl4. Figure 1(a) shows an empty SWNT tip. Below beam. The average filling yield for `as-supplied' ZrCl4 was estimated to be between 20-30%. #12;P 258

Dunin-Borkowski, Rafal E.

248

13.21 Geochemistry of the Rare-Earth Element, Nb, Ta, Hf, and Zr Deposits RL Linnen, University of Western Ontario, London, ON, Canada  

E-Print Network [OSTI]

13.21 Geochemistry of the Rare-Earth Element, Nb, Ta, Hf, and Zr Deposits RL Linnen, University to Y, the rare- earth elements (REE, La to Lu), Zr, Hf, Nb, and Ta. The rare elements, Canada ĂŁ 2014 Elsevier Ltd. All rights reserved. 13.21.1 Introduction 543 13.21.1.1 Uses of Rare Elements

Chakhmouradian, Anton

249

Ab initio prediction of ordered ground-state structures in ZrO2-Y2O3 A. Predith,1  

E-Print Network [OSTI]

Institute of Technology, 77 Massachusetts Avenue, Cambridge, Massachusetts 02139, USA 2Department from yttrium and every Zr has seven oxygen first nearest neighbors. The Zr-O bond lengths and oxygen, 82.45.Xy I. INTRODUCTION Zirconia doped with yttria is a common oxygen ion con- ductor used in oxygen

Ceder, Gerbrand

250

Fundamental science investigations to develop a 6-MV laser triggered gas switch for ZR: first annual report.  

SciTech Connect (OSTI)

In October 2005, an intensive three-year Laser Triggered Gas Switch (LTGS) development program was initiated to investigate and solve observed performance and reliability issues with the LTGS for ZR. The approach taken has been one of mission-focused research: to revisit and reassess the design, to establish a fundamental understanding of LTGS operation and failure modes, and to test evolving operational hypotheses. This effort is aimed toward deploying an initial switch for ZR in 2007, on supporting rolling upgrades to ZR as the technology can be developed, and to prepare with scientific understanding for the even higher voltage switches anticipated needed for future high-yield accelerators. The ZR LTGS was identified as a potential area of concern quite early, but since initial assessments performed on a simplified Switch Test Bed (STB) at 5 MV showed 300-shot lifetimes on multiple switch builds, this component was judged acceptable. When the Z{sub 20} engineering module was brought online in October 2003 frequent flashovers of the plastic switch envelope were observed at the increased stresses required to compensate for the programmatically increased ZR load inductance. As of October 2006, there have been 1423 Z{sub 20} shots assessing a variety of LTGS designs. Numerous incremental and fundamental switch design modifications have been investigated. As we continue to investigate the LTGS, the basic science of plastic surface tracking, laser triggering, cascade breakdown, and optics degradation remain high-priority mission-focused research topics. Significant progress has been made and, while the switch does not yet achieve design requirements, we are on the path to develop successively better switches for rolling upgrade improvements to ZR. This report summarizes the work performed in FY 2006 by the large team. A high-level summary is followed by detailed individual topical reports.

Warne, Larry Kevin; Van Den Avyle, James A.; Lehr, Jane Marie; Rose, David (Voss Scientific, Albuquerque, NM); Krompholz, Hermann G. (Texas Tech University, Lubbock, TX); Vela, Russell (Texas Tech University, Lubbock, TX); Jorgenson, Roy Eberhardt; Timoshkin, Igor (University of Strathclyde, Glasgow, Scotland); Woodworth, Joseph Ray; Prestwich, Kenneth Randel (Voss Scientific, Albuquerque, NM); Krile, John (Texas Tech University, Lubbock, TX); Given, Martin (University of Strathclyde, Glasgow, Scotland); McKee, G. Randall; Rosenthal, Stephen Edgar; Struve, Kenneth William; Welch, Dale Robert (Voss Scientific, Albuquerque, NM); Benwell, Andrew L. (University of Missouri-Columbia, Columbia, Missouri); Kovaleski, Scott (University of Missouri-Columbia, Columbia, Missouri); LeChien, Keith, R.; Johnson, David (Titan Pulse Sciences Division); Fouracre, R.A. (University of Strathclyde, Glasgow, Scotland); Yeckel, Chris (University of Missouri-Columbia, Columbia, Missouri); Wakeland, Peter Eric (Ktech Corporation, Albuquerque, NM); Miller, A. R. (Titan Pulse Sciences Division); Hodge, Keith Conquest (Ktech Corporation, Albuquerque, NM); Pasik, Michael Francis; Savage, Mark Edward; Maenchen, John Eric; Curry, Randy D. (University of Missouri-Columbia, Columbia, Missouri); Feltz, Greg (Ktech Corporation, Albuquerque, NM); Bliss, David Emery; MacGregor, Scott (University of Strathclyde, Glasgow, Scotland); Corley, J. P. (Ktech Corporation, Albuquerque, NM); Anaya, Victor (Ktech Corporation, Albuquerque, NM); Wallace, Zachariah (Ktech Corporation, Albuquerque, NM); Thoma, Carsten (Voss Scientific, Albuquerque, NM); Neuber, Andreas. (Texas Tech University, Lubbock, TX)

2007-03-01T23:59:59.000Z

251

Energy Calibration of the BaBar EMC Using the Pi0 Invariant Mass Method  

SciTech Connect (OSTI)

The BaBar electromagnetic calorimeter energy calibration method was compared with the local and global peak iteration procedures, of Crystal Barrel and CLEO-II. An investigation was made of the possibility of {Upsilon}(4S) background reduction which could lead to increased statistics over a shorter time interval, for efficient calibration runs. The BaBar software package was used with unreconstructed data to study the energy response of the calorimeter, by utilizing the {pi}{sup 0} mass constraint on pairs of photon clusters.

Tanner, David J.; /Manchester U.

2007-04-06T23:59:59.000Z

252

The Radiation Dose Measurement System for the BaBar Electromagnetic Calorimeter  

SciTech Connect (OSTI)

An array of 116 p-channel radiation sensitive MOSFET transistors (RadFETs) has been operational for the past 6 years at the BaBar experiment at the PEP-II asymmetric B-Factory at the Stanford Linear Accelerator Center (SLAC). This system maps the integrated dose absorbed by different regions of the Electromagnetic Calorimeter (EMC) during the running of the experiment. We report on the design and implementation of the system and finally, the performance of the monitoring system during the last 6 years of BaBar data-taking.

Khan, A.; /Brunel U.; Meyer, W.T.; /Iowa State U.; Stelzer, J.; /Stanford U., Phys. Dept.; Yi, Jong; /Manchester U.

2006-08-14T23:59:59.000Z

253

Data:Edc9061a-dbcf-4e0b-a18a-7b38ef40ba47 | Open Energy Information  

Open Energy Info (EERE)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Home Page on Google Bookmark EERE: Alternative Fuels Data Center Home Pagec-01b596aa1744b55997c1cc NoEce78e10-0967-4d20-a270-53a70a3b054f NoEdc9061a-dbcf-4e0b-a18a-7b38ef40ba47 No revision has been

254

NOx uptake on alkaline earth oxides (BaO, MgO, CaO and SrO) supported...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

uptake on alkaline earth oxides (BaO, MgO, CaO and SrO) supported on ?-Al2O3. NOx uptake on alkaline earth oxides (BaO, MgO, CaO and SrO) supported on ?-Al2O3....

255

College of Charleston Major Roadmap: Religious Studies, B.A. | 2014-15 Page 1 MAJOR ROADMAP  

E-Print Network [OSTI]

College of Charleston Major Roadmap: Religious Studies, B.A. | 2014-15 Page 1 MAJOR ROADMAP Religious Studies, B.A. Catalog Year: 2014-15 This roadmap is a suggested semester-by-semester planning availability may vary from semester to semester. Roadmaps are not meant to cover every possibility

Kasman, Alex

256

Magnetic fabrics and fluid flow directions in hydrothermal systems. A case study in the Chaillac BaFFe deposits  

E-Print Network [OSTI]

of anisotropy of magnetic susceptibility (AMS) to describe the mineralizing process in hydrothermal systems. BaMagnetic fabrics and fluid flow directions in hydrothermal systems. A case study in the Chaillac Ba hydrothermal textures and tectonic structures have been described in veins, sinters, and sandstone cemented

Paris-Sud XI, Université de

257

PLAN OF STUDY Digital Media & Design SCHOOL OF FINE ARTS 2013-2014Catalog BA in DMD  

E-Print Network [OSTI]

PLAN OF STUDY ­ Digital Media & Design SCHOOL OF FINE ARTS 2013-2014Catalog BA in DMD ATTACH YOUR ______ _____ __ ______ ______ _____ __ ______ ______ _____ __ ______ ______ _____ __ ______ ______ _____ __ ______ ______ _____ __ ______ ______ _____ __ ______ ______ _____ __ ______ University of Connecticut DMD BA REQUIREMENTS: 51 credits DMD courses (21 credits): DMD 1000 (3) ­ Digital Foundation DMD 1030 (3) ­ Animation Lab DMD 2010 (3) ­ Digital Culture DMD 3050 (3) ­ Visible Language DMD

Alpay, S. Pamir

258

Effect of Y-211 particle size on the growth of single grain Y–Ba–Cu–O bulk superconductors  

E-Print Network [OSTI]

The engineering of fine Y2Ba1Cu1O5 (Y-211) inclusions of average particle size 1?2 ?m within the continuous, superconducting YBa2Cu3O7?? (Y-123) phase matrix of single-grain, bulk high temperature Y–Ba–Cu–O (YBCO) superconductors is fundamental...

Thoma, Max; Shi, Yunhua; Dennis, Tony; Durrell, John; Cardwell, David

2014-12-01T23:59:59.000Z

259

Intrinsic nanostructure in Zr2 xFe4Si16 y (x = 0.81, y = 6.06)  

SciTech Connect (OSTI)

We present a study of the crystal structure and physical properties of single crystals of a new Fe-based ternary compound, Zr2 xFe4Si16 y (x = 0.81, y = 6.06). Zr1.19Fe4Si9.94 is a layered compound, where stoichiometric -FeSi2-derived slabs are separated by Zr-Si planes with substantial numbers of vacancies. High resolution transmission electron microscopy (HRTEM) experiments show that these Zr-Si layers consist of 3.5 nm domains where the Zr and Si vacancies are ordered within a supercell sixteen times the volume of the stoichiometric cell. Within these domains, the occupancies of the Zr and Si sites obey symmetry rules that permit only certain compositions, none of which by themselves reproduce the average composition found in x-ray diffraction experiments. Magnetic susceptibility and magnetization measurements reveal a small but appreciable number of magnetic moments that remain freely fluctuating to 1.8 K, while neutron diffraction confirms the absence of bulk magnetic order with a moment of 0.2 B or larger down to 1.5 K. Electrical resistivity measurements find that Zr1.19Fe4Si9.94 is metallic, and the modest value of the Sommerfeld coefficient of the specific heat = C/T suggests that quasi-particle masses are not particularly strongly enhanced. The onset of superconductivity at Tc 6 K results in a partial resistive transition and a small Meissner signal, although a bulk-like transition is found in the specific heat. Sharp peaks in the ac susceptibility signal the interplay of the normal skin depth and the London penetration depth, typical of a system in which nano-sized superconducting grains are separated by a non-superconducting host. Ultra low field differential magnetic susceptibility measurements reveal the presence of a surprisingly large number of trace magnetic and superconducting phases, suggesting that the Zr-Fe-Si ternary system could be a potentially rich source of new bulk superconductors.

Smith, G J [Stony Brook University, Department of Physics and Astronomy; Simonson, Jack [Stony Brook University (SUNY); Prozorov, R. [Ames Laboratory and Iowa State University; Zhu, Y [Brookhaven National Laboratory (BNL); Aronson, M. [Stony Brook University, Department of Physics and Astronomy

2014-01-01T23:59:59.000Z

260

Preliminary study of niobium alloy contamination by transport through helium. [Nb-1Zr; Sm-Co; Hiperco 50 steel; alumina  

SciTech Connect (OSTI)

Preliminary tests were conducted to determine if interstitial element transport through a circulating helium working fluid was a potential problem in Brayton and Stirling space power systems. Test specimens exposed to a thermal gradient for up to 3000 h included Nb-1%Zr, a Sm-Co alloy, Hiperco 50 steel, and alumina to simulate various engine components of the Brayton and Stirling systems. Results indicate that helium transport of interstitial contaminants can be minimized over a 7-y life with monometallic Nb-1%Zr design. Exposure with other materials indicated a potential for interstitial contaminant transport.

Scheuermann, C.M.; Moore, T.J.; Wheeler, D.R.

1987-01-12T23:59:59.000Z

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261

Repetitive Ultra-low Stress Induced Nanocrystallization in Amorphous Cu?Zr?Al Alloy Evidenced by in situ Nanoindentation  

E-Print Network [OSTI]

?Zr?Al Alloy Evidenced by in situ Nanoindentation Y. Liu a , J. Jian b , J.H. Lee b , C. Wang cd , Q.P. Cao cd , C. Gutierrez e , H. Wang ab , J.Z. Jiang cd & X. Zhang ae a Department of Materials Science and Engineering, Texas A&M University, College Station.... To cite this article: Y. Liu, J. Jian, J.H. Lee, C. Wang, Q.P. Cao, C. Gutierrez, H. Wang, J.Z. Jiang & X. Zhang (2014) Repetitive Ultra-low Stress Induced Nanocrystallization in Amorphous Cu?Zr?Al Alloy Evidenced by in situ Nanoindentation, Materials...

Liu, Y.; Jian, J.; Lee, J. H.; Wang, C.; Cao, Q. P.; Gutierrez, C.; Wang, H.; Jiang, J. Z.; Zhang, X.

2014-05-12T23:59:59.000Z

262

Interface control of ferroelectricity in LaNiO{sub 3}-BaTiO{sub 3} superlattices  

SciTech Connect (OSTI)

LaNiO{sub 3}-BaTiO{sub 3} superlattices with different types of interfaces are studied from first-principles density-functional theory. It is revealed that the ferroelectricity in the superlattice with (NiO{sub 2}){sup ?}/(BaO){sup 0} interfaces is enhanced from that of the superlattice with (LaO){sup +}/(TiO{sub 2}){sup 0} interfaces. The origin lies at the polar discontinuity at the interface, which makes the holes localized within the (NiO{sub 2}){sup ?}/(BaO){sup 0} interface, but drives a penetration of electrons into BaTiO{sub 3} component near (LaO){sup +}/(TiO{sub 2}){sup 0} interface. Our calculations demonstrate an effective avenue to the robust ferroelectricity in BaTiO{sub 3} ultrathin films.

Wu, Yin-Zhong, E-mail: yzwu@cslg.edu.cn [Jiangsu Laboratory of Advanced Functional Materials and Physics Department, Changshu Institute of Technology, Changshu 215500 (China); School of Mathematics and Physics, Suzhou University of Science and Technology, Suzhou 215009 (China); Lu, Hai-Shuang; Cai, Tian-Yi; Ju, Sheng, E-mail: jusheng@suda.edu.cn [Department of Physics and Jiangsu Key Laboratory of Thin Films, Soochow University, Suzhou 215006 (China)

2014-08-15T23:59:59.000Z

263

Biotechnol. Appl. Biochem. (2005) 42, 119131 (Printed in Great Britain) doi:10.1042/BA20040207 119 Clonal evolution of stem and differentiated cells can be  

E-Print Network [OSTI]

Biotechnol. Appl. Biochem. (2005) 42, 119­131 (Printed in Great Britain) doi:10.1042/BA20040207 119

Zandstra, Peter W.

264

Synthesis of ZrO{sub 2} nanoparticles by hydrothermal treatment  

SciTech Connect (OSTI)

Zirconium oxide (zirconia, ZrO{sub 2}) is the most common material used for electrolyte of solid oxide fuel cells (SOFCs). Zirconia has attracted attention for applications in optical coatings, buffer layers for growing superconductors, thermal-shield, corrosion resistant coatings, ionic conductors, and oxygen sensors, and for potential applications including transparent optical devices and electrochemical capacitor electrodes, fuel cells, catalysts, and advanced ceramics. In this work, zirconia particles were synthesized from ZrCl{sub 4} precursor with hydrothermal treatment in a batch reactor. Hydrothermal treatment may allow obtaining nanoparticles and sintered materials with controlled chemical and structural characteristics. Hydrothermal treatment was carried out at temperatures of 150 – 200°C with precursor concentration of 0.1 – 0.5 M. Zirconia particles obtained from this treatment were analyzed by using SEM, PSD and XRD to characterize the morphology, particle size distribution, and crystallinity, respectively. Based on the analysis, the size of zirconia particles were around 200 nm and it became smaller with decreasing precursor concentration. The increasing temperature caused the particles formed having uniform size. Zirconia particles formed by hydrothermal treatment were monoclinic, tetragonal and cubic crystal.

Machmudah, Siti, E-mail: machmudah@chem-eng.its.ac.id; Widiyastuti, W., E-mail: machmudah@chem-eng.its.ac.id; Prastuti, Okky Putri, E-mail: machmudah@chem-eng.its.ac.id; Nurtono, Tantular, E-mail: machmudah@chem-eng.its.ac.id; Winardi, Sugeng, E-mail: machmudah@chem-eng.its.ac.id [Chemical Engineering Department, Sepuluh Nopember Institute of Technology, Surabaya 60111 (Indonesia); Wahyudiono,; Kanda, Hideki; Goto, Motonobu [Department of Chemical Engineering, Nagoya University, Nagoya 464-8603 (Japan)

2014-02-24T23:59:59.000Z

265

Dissociation of trimethylgallium on the ZrB{sub 2}(0001) surface  

SciTech Connect (OSTI)

X-ray photoelectron spectroscopy and reflection absorption infrared spectroscopy (RAIRS) have been used to study the dissociative adsorption of trimethylgallium (TMG) on the ZrB{sub 2}(0001) surface. Spectra were obtained as a function of annealing temperature following TMG exposure at temperatures of 95 and 300 K, and also as a function of TMG exposure for a surface temperature of 300 K. After annealing above 220 K, a significant decrease in the relative concentration of carbon and gallium occurred accompanied by a shift of ?0.2 eV in the Ga 2p{sub 3/2} binding energy. The RAIR spectra show that after annealing to ?220 K, only one CH{sub 3} deformation band at 1196 cm{sup ?1} remains, the intensity of which is considerably decreased indicating loss of at least one methyl group from TMG. Further annealing leads to the sequential loss of the other methyl groups. The first methyl desorbs while the last two dissociate to deposit two C atoms per TMG molecule onto the ZrB{sub 2} surface.

Manandhar, Kedar; Trenary, Michael [Department of Chemistry, University of Illinois at Chicago, 845W Taylor St., Chicago, Illinois 60607 (United States)] [Department of Chemistry, University of Illinois at Chicago, 845W Taylor St., Chicago, Illinois 60607 (United States); Otani, Shigeki [National Institute for Material Science, 1-1 Namiki, Tsukuba-shi, Ibaraki 305-0044 (Japan)] [National Institute for Material Science, 1-1 Namiki, Tsukuba-shi, Ibaraki 305-0044 (Japan); Zapol, Peter [Materials Science Division, Argonne National Laboratory, 9700 S. Cass Ave., Argonne, Illinois 60439 (United States)] [Materials Science Division, Argonne National Laboratory, 9700 S. Cass Ave., Argonne, Illinois 60439 (United States)

2013-11-15T23:59:59.000Z

266

New Insights into Reaction Mechanisms of Ethanol Steam Reforming on Co-ZrO2  

SciTech Connect (OSTI)

The reaction pathway of ethanol steam reforming on Co-ZrO2 has been identified and the active sites associated with each step are proposed. Ethanol is converted to acetaldehyde and then to acetone, followed by acetone steam reforming. More than 90% carbon was found to follow this reaction pathway. N2-Sorption, X-ray Diffraction (XRD), Temperature Programmed Reduction (TPR), in situ X-ray Photoelectron Spectroscopy (XPS), Transmission Electron Microscopy, as well as theoretical Density Functional Theory (DFT) calculations have been employed to identify the structure and functionality of the catalysts, which was further used to correlate their performance in ESR. It was found that metallic cobalt is mainly responsible for the acetone steam reforming reactions; while, CoO and basic sites on the support play a key role in converting ethanol to acetone via dehydrogenation and condensation/ketonization reaction pathways. The current work provides fundamental understanding of the ethanol steam reforming reaction mechanisms on Co-ZrO2 catalysts and sheds light on the rational design of selective and durable ethanol steam reforming catalysts.

Sun, Junming; Karim, Ayman M.; Mei, Donghai; Engelhard, Mark H.; Bao, Xinhe; Wang, Yong

2015-01-01T23:59:59.000Z

267

Synthesis and characterization of rare earth doped ZrO{sub 2} nanophosphors  

SciTech Connect (OSTI)

In this paper, we reports synthesis, characterization and thermoluminescence (TL) glow curves of europium and dysprosium activated zirconium dioxide (ZrO{sub 2}: Eu{sup 3+}, Dy{sup 3+}) phosphor with variable concentration of europium and fixed concentration of dysprosium. The sample was prepared by the Solid state method; thereafter, the TL glow curves were recorded for different concentration of europium with 20 min UV exposure at a heating rate of 6.7°C/s. The trapping parameters for synthesized phosphors of ZrO{sub 2}: Eu{sup 3+}, Dy{sup 3+} have been calculated by using a peak shape method. The sample was characterized for structural analysis by XRD (X-ray diffraction) and morphological analysis by FEGSEM (field emission gun scanning electron microscope) and FTIR (Fourier transform infrared spectroscopy). The effect of variable europium concentration and fixed dysprosium concentration on TL studies were interpreted and the formation of trap depth and reproducibility of prepared phosphor were analyzed by TL glow curves. The peak temperature on TL less than 200°C shows the formation of deep trapping in prepared sample. The high temperature peak shows the less fading and more stability in prepared sample.

Agrawal, Sadhana, E-mail: sagrawal.phy@nitrr.ac.in, E-mail: jsvikasdubey@gmail.com; Dubey, Vikas, E-mail: sagrawal.phy@nitrr.ac.in, E-mail: jsvikasdubey@gmail.com [Department of Physics, National Institute of Technology, Raipur (C.G.) (India)

2014-10-24T23:59:59.000Z

268

Precipitation in a Cu–Cr–Zr–Mg alloy during aging  

SciTech Connect (OSTI)

The precipitation processes in a Cu-0.69Cr-0.10Zr-0.02Mg alloy aged at 450 °C and 550 °C have been investigated by transmission electron microscopy and high resolution transmission electron microscopy. The precipitation sequence in this alloy aged at 450 °C is: supersaturated solid solution ? Guinier–Preston zone (fcc Cr-rich phase) ? ordered fcc Cr-rich phase ? ordered bcc Cr-rich phase. The precipitation sequence in this alloy aged at 550 °C is: supersaturated solid solution ? ordered fcc Cr-rich phase ? ordered bcc Cr-rich phase. In the evolution of decomposition, the orientation relationship between the precipitates and the Cu matrix changes from cube-on-cube to Nishiyama–Wassermann orientation. The ordering of Cr-rich precipitates facilitates the formation of the bcc precipitates and promotes the development of Nishiyama–Wassermann orientation. - Highlights: • Two different precipitation sequences in the Cu–Cr–Zr–Mg alloy are proposed. • The changes in orientation relationship of the precipitates are presented. • The roles of ordering and coherent interface of the precipitates are discussed.

Cheng, J.Y., E-mail: bigchengjianyi@163.com; Shen, B.; Yu, F.X.

2013-07-15T23:59:59.000Z

269

Nonequilibrium quasiparticle relaxation dynamics in single crystals of hole- and electron-doped BaFe[subscript 2]As[subscript 2  

E-Print Network [OSTI]

We report on the nonequilibrium quasiparticle dynamics in BaFe[subscript 2]As[subscript 2] on both the hole-doped (Ba[subscript 1?x]K[subscript x]Fe[subscript 2]As[subscript 2]) and electron-doped (BaFe[subscript ...

Torchinsky, Darius Hosseinzadeh

270

CASIS: A System for Concept-Aware Social Image Search Ba Quan Truong  

E-Print Network [OSTI]

CASIS: A System for Concept-Aware Social Image Search Ba Quan Truong bqtruong@ntu.edu.sg Aixin Sun axsun@ntu.edu.sg Sourav S. Bhowmick assourav@ntu.edu.sg School of Computer Engineering, Nanyang the opportunity of building effective tag-based social image retrieval systems. In contrast to content-based image

Aixin, Sun

271

Influence of Ba content on grain size and dynamics of crystallization in barium ferrite thin films  

E-Print Network [OSTI]

Influence of Ba content on grain size and dynamics of crystallization in barium ferrite thin films of the crystallization process, which ultimately determines the grain size, were studied in barium ferrite thin films. Rapid thermal annealing was used to crystallize the amorphous as-deposited barium ferrite films

Laughlin, David E.

272

Search for Physics Beyond the Standard Model at BaBar and Belle  

E-Print Network [OSTI]

Recent results on the search for new physics at BaBar and Belle B-factories are presented. The search for a light Higgs boson produced in the decay of different Y resonances is shown. In addition, recent measurements aimed to discover invisible final states produced by new physics mechanisms beyond the standard model are presented.

G. Calderini

2012-04-19T23:59:59.000Z

273

Computer Science Major Worksheet B.A. Degree Student: _______________________ ID#___________ Catalog:_________ Advisor _____________  

E-Print Network [OSTI]

10/15/2012 Computer Science Major Worksheet ­ B.A. Degree Student: _______________________ ID#___________ Catalog:_________ Advisor _____________ Computer Science Required Courses Cr. Semester Gr. CSci 160 Computer Science I 4 CSci 161 Computer Science II 4 CSci 230 Systems Programming 3 CSci 242 Algo. & Data

Delene, David J.

274

NAME__________________________________ REQUIREMENTS FOR THE B.A. DEGREE IN COMPUTER SCIENCE  

E-Print Network [OSTI]

NAME__________________________________ REQUIREMENTS FOR THE B.A. DEGREE IN COMPUTER SCIENCE (effective entering class Fall 2013) 1) REQUIRED COMPUTER SCIENCE COURSES (Total of 47 CS credit hours) * COS.00 or greater as must the overall GPA. February 18, 2013 #12;Computer Science Summary Total Total CS Hrs Hrs Q

Thomas, Andrew

275

Roadmap: Political Science American Politics Bachelor of Arts [AS-BA-POL-APOL  

E-Print Network [OSTI]

Roadmap: Political Science ­ American Politics ­ Bachelor of Arts [AS-BA-POL-APOL] College of Arts and Sciences Department of Political Science Catalog Year: 2013-2014 Page 1 of 3 | Last Updated: 30-Sept-13 Important Notes Semester One: [14-17 Credit Hours] POL 10100 American Politics or POL 10300 Public Policy 3

Sheridan, Scott

276

BA Political Economy Political Economy caters for students who wish to understand the  

E-Print Network [OSTI]

BA Political Economy Political Economy caters for students who wish to understand the political to offer such a programme. www.birmingham.ac.uk/polsis Department of Political Science and International.birmingham.ac.uk/international/ students/country Programme Structure First Year Required modules: Foundations of Politics; Introduction

Miall, Chris

277

Roadmap: Political Science American Politics Bachelor of Arts [AS-BA-POL-APOL  

E-Print Network [OSTI]

Roadmap: Political Science ­ American Politics ­ Bachelor of Arts [AS-BA-POL-APOL] College of Arts and Sciences Department of Political Science Catalog Year: 2012­2013 Page 1 of 3 | Last Updated: 20-Apr-12/LNHD Important Notes Semester One: [14-17 Credit Hours] POL 10100 American Politics or POL 10300 Public Policy 3

Sheridan, Scott

278

Roadmap: Political Science General -Bachelor of Arts [AS-BA-POL-GENL  

E-Print Network [OSTI]

Roadmap: Political Science ­ General - Bachelor of Arts [AS-BA-POL-GENL] College of Arts and Sciences Department of Political Science Catalog Year: 2013-2014 Page 1 of 3 | Last Updated: 30-Sept-13 Important Notes Semester One: [14-17 Credit Hours] POL 10100 American Politics or POL 10300 Public Policy 3

Sheridan, Scott

279

Roadmap: Political Science General -Bachelor of Arts [AS-BA-POL-GENL  

E-Print Network [OSTI]

Roadmap: Political Science ­ General - Bachelor of Arts [AS-BA-POL-GENL] College of Arts and Sciences Department of Political Science Catalog Year: 2012­2013 Page 1 of 3 | Last Updated: 8-May-12/LNHD Important Notes Semester One: [14-17 Credit Hours] POL 10100 American Politics or POL 10300 Public Policy 3

Sheridan, Scott

280

BA in POLITICAL SCIENCE (735121) MAP Sheet Department of Political Science  

E-Print Network [OSTI]

BA in POLITICAL SCIENCE (735121) MAP Sheet Department of Political Science For students entering approved list from approved list Poli 328* from approved list personal choice · 27 hours of political, or 270): a. Political Philosophy: Poli 201 Western Political Heritage 1 Poli 202 Western Political

Olsen Jr., Dan R.

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
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281

Roadmap: Political Science Public Policy Bachelor of Arts [AS-BA-POL-PPOL  

E-Print Network [OSTI]

Roadmap: Political Science ­ Public Policy ­ Bachelor of Arts [AS-BA-POL-PPOL] College of Arts and Sciences Department of Political Science Catalog Year: 2012­2013 Page 1 of 3 | Last Updated: 8-May-12/LNHD Important Notes Semester One: [14-17 Credit Hours] POL 10100 American Politics or POL 10300 Public Policy 3

Sheridan, Scott

282

Roadmap: Political Science Public Policy Bachelor of Arts [AS-BA-POL-PPOL  

E-Print Network [OSTI]

Roadmap: Political Science ­ Public Policy ­ Bachelor of Arts [AS-BA-POL-PPOL] College of Arts and Sciences Department of Political Science Catalog Year: 2013-2014 Page 1 of 3 | Last Updated: 30-Sept-13 Important Notes Semester One: [14-17 Credit Hours] POL 10100 American Politics or POL 10300 Public Policy 3

Sheridan, Scott

283

BA Political Science This is one of our most popular degree programmes. It provides  

E-Print Network [OSTI]

BA Political Science This is one of our most popular degree programmes. It provides you with a thorough grounding in the main approaches, theories and debates in Political Science, as well as allowing to you. www.birmingham.ac.uk/polsis Department of Political Science and International Studies (POLSIS

Miall, Chris

284

Spectroscopy, polarization and nonadiabatic dynamics of electronically excited Ba(Ar)n clusters: Theory and experiment  

E-Print Network [OSTI]

Spectroscopy, polarization and nonadiabatic dynamics of electronically excited Ba(Ar)n clusters, France Received 13 September 1995; accepted 17 November 1995 Molecular Dynamics simulations using, a comprehensive picture of the excited state dynamics is given. It is found that upon excitation, energy

Krylov, Anna I.

285

Roadmap: Communication Studies Public Communication Bachelor of Arts [CI-BA-COMM-PCMM  

E-Print Network [OSTI]

Roadmap: Communication Studies ­ Public Communication ­ Bachelor of Arts [CI-BA-COMM-PCMM] College of Communication and Information School of Communication Studies Catalog Year: 2012­2013 Page 1 of 3 | Last Updated Major GPA Important Notes Semester One: [16 Credit Hours] COMM 15000 Introduction to Human Communication

Sheridan, Scott

286

Roadmap: Communication Studies -Applied Communication -Bachelor of Arts [CI-BA-COMM-APCO  

E-Print Network [OSTI]

Roadmap: Communication Studies - Applied Communication - Bachelor of Arts [CI-BA-COMM-APCO] College of Communication and Information School of Communication Studies Catalog Year: 2012­2013 Page 1 of 3 | Last Updated Major GPA Important Notes Semester One: [16 Credit Hours] COMM 15000 Introduction to Human Communication

Sheridan, Scott

287

6/06/09 BA in General Biology Bachelor of Arts in General Biology  

E-Print Network [OSTI]

6/06/09 BA in General Biology Bachelor of Arts in General Biology Department of Biology College of Science and Engineering Undergraduate Programs Students majoring in the General Biology degree program are required to complete 57 units in the major. In addition to the biological science courses, it includes

288

BA (Hons) Business Management (In-Company) Degree Information for Prospective Sponsoring Companies  

E-Print Network [OSTI]

BA (Hons) Business Management (In-Company) Degree Information for Prospective Sponsoring Companies) Business Management (In-Company) degree, which is based at Nottingham Business School, is aimed of the programme is full time at the Business School but students then spend the next two years in a company

Evans, Paul

289

Roadmap: Theatre Studies Theatre and Society-Bachelor of Arts [CA-BA-THEA-THSO  

E-Print Network [OSTI]

Roadmap: Theatre Studies ­ Theatre and Society- Bachelor of Arts [CA-BA-THEA-THSO] College This roadmap is a recommended semester-by-semester plan of study for this major. However, courses Requirement 3 Kent Core Requirement 3 General Elective (upper division) 3 See note 2 on page 3 #12;Roadmap

Sheridan, Scott

290

Roadmap: Criminology and Justice Studies Corrections Bachelor of Arts [AS-BA-CRJU-CORR  

E-Print Network [OSTI]

Roadmap: Criminology and Justice Studies ­ Corrections ­ Bachelor of Arts [AS-BA-CRJU-CORR] College/LNHD This roadmap is a recommended semester-by-semester plan of study for this major. However, courses Hours] JUS 46792 Internship 0-6 Recommended but not required #12;Roadmap: Criminology and Justice

Sheridan, Scott

291

Roadmap: Criminology and Justice Studies Policing Bachelor of Arts [AS-BA-CRJU-POLG  

E-Print Network [OSTI]

Roadmap: Criminology and Justice Studies ­ Policing ­ Bachelor of Arts [AS-BA-CRJU-POLG] College/LNHD This roadmap is a recommended semester-by-semester plan of study for this major. However, courses Elective 3 See note 3 on page 2 General Electives (upper division) 9 #12;Roadmap: Criminology

Sheridan, Scott

292

Revised version of J Gen Physiol: 200709771 MOLECULAR DETERMINANT FOR SPECIFIC Ca/Ba  

E-Print Network [OSTI]

1 Revised version of J Gen Physiol: 200709771 MOLECULAR DETERMINANT FOR SPECIFIC Ca/Ba SELECTIVITY PROFILES OF LOW AND HIGH THRESHOLD Ca2+ CHANNELS Thierry Cens, Matthieu Rousset, Andrey Kajava & Pierre-1559; E-mail: Pierre.charnet@crbm.cnrs.fr Running title: Divalent cation selection in LVA/HVA Ca2

Boyer, Edmond

293

Computer Science B.A. Degree Curriculum Chart: 2013-2014  

E-Print Network [OSTI]

Computer Science B.A. Degree Curriculum Chart: 2013-2014 http://ua.soe.ucsc.edu · advising Comparative Programming Languages CMPS 115 Software Methodology CMPS 122 Computer Security CMPS 140 Artificial Intelligence CMPS 160 Computer Graphics CMPS 180 Database Systems CMPE 110 Computer Architecture 2. Students

Stuart, Josh

294

Computer Science B.A. Degree 2014-2015 Curriculum Chart  

E-Print Network [OSTI]

Computer Science B.A. Degree 2014-2015 Curriculum Chart CMPS 12B/M Data Structures *CMPS 13H to Prog: Java CMPS 11 Intermediate Programming *CMPE 13/L Computer Systems and C Programming OR OR *CMPE to Analysis of Algorithms CMPS 140 Artificial Intelligence CMPS 104A Compiler Design CMPS 160 Computer

Stuart, Josh

295

Internal conversion coefficients in (134)Cs, (137)Ba, and (139)La: A precise test of theory  

E-Print Network [OSTI]

Recently we measured the ratio of K-shell internal conversion coefficients, alpha(K), for the 127.5-keV E3 transition in (134)Cs and the 661.7-keV M4 transition in (137)Ba. We here report a measurement of the 165.9-keV M1 transition in (139)La...

Nica, N.; Hardy, John C.; Iacob, V. E.; Balonek, C.; Trzhaskovskaya, M. B.

2008-01-01T23:59:59.000Z

296

Department of Mechanical Engineering University of Bath, Bath BA2 7AY, UK  

E-Print Network [OSTI]

. The balance between activities has shifted through the years with an increasing emphasis on research), and today as City of Bristol College #12;Department of Mechanical Engineering University of Bath, Bath BA2 7 vision and energy. Ted retired in 1987, and was succeeded as Director by Cliff Burrows. In 1992 Kevin

Burton, Geoffrey R.

297

BA in CHEMISTRY (692827) MAP Sheet Department of Chemistry and Biochemistry  

E-Print Network [OSTI]

BA in CHEMISTRY (692827) MAP Sheet Department of Chemistry and Biochemistry For students entering Chemistry and Biochemistry Department requires the final 10 hours of required chemistry credit to be taken for graduation. Complete the following: Chem 111* Honors Principles of Chemistry Chem 112 Principles of Chemistry

Seamons, Kent E.

298

BA in CHEMISTRY (692827) MAP Sheet Department of Chemistry and Biochemistry  

E-Print Network [OSTI]

BA in CHEMISTRY (692827) MAP Sheet Department of Chemistry and Biochemistry For students entering in major courses. --The Chemistry and Biochemistry Department requires the final 10 hours of required chemistry credit to be taken in residence at BYU for this degree program. These hours may also go toward BYU

Seamons, Kent E.

299

B.A. Master of Architecture Plan (173 credits) Year 1 (32-33 credits)  

E-Print Network [OSTI]

B.A. ­ Master of Architecture Plan (173 credits) Year 1 (32-33 credits) Fall (16 credits) Spring (16-17 credits) ARCH 103 Introduction to Architecture (3) BDS 102 Thinking & Making Studio II (3) ARCH Culture of Building Technology (3) ARCH 630 Theory & Context (3) ARCH 530 Environmental Systems I (3

300

The George R. Brown School of Engineering Degrees Offered: BA, MStat, MA, PhD  

E-Print Network [OSTI]

211Introduction to Engineering Computation · STAT310Probability and Statistics · STAT410Introduction263 Statistics The George R. Brown School of Engineering Degrees Offered: BA, MStat, MA, PhD Course engineering, computational and applied mathematics, managerial studies, mathematics, political science

Richards-Kortum, Rebecca

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


301

PHENOLOGY AND BROWN-HEADED COWBIRD PARASITISM B.A., University of Colorado, 2003  

E-Print Network [OSTI]

PHENOLOGY AND BROWN-HEADED COWBIRD PARASITISM by TY TUFF B.A., University of Colorado, 2003 A thesis submitted to the Faculty of the Graduate School of the University of Colorado in partial, to evaluate the impact of parasitism on two local hosts in the Colorado Front Range: the primary host

Hammerton, James

302

Atomistic Study of Doped BaCeO3: Dopant Site-Selectivity and Cation Nonstoichiometry  

E-Print Network [OSTI]

of Technology, Pasadena, California 91125, and Materials Chemistry Group, Chemistry DiVision, Uni, the trivalent dopants are assumed to occupy the Ce4+ -site, which introduces oxygen vacancies partitioning over both Ba and Ce sites. Such partitioning reduces the concentration of oxygen vacancies, which

Haile, Sossina M.

303

Synthesis and Structure Determination of Ferromagnetic Semiconductors LaAMnSnO6 (A = Sr Ba)  

SciTech Connect (OSTI)

LaAMnSnO{sub 6} (A = Sr, Ba) have been synthesized by high temperature solid-state reactions under dynamic 1% H{sub 2}/Ar flow. Rietveld refinements on room temperature powder X-ray diffraction data indicate that LaSrMnSnO{sub 6} crystallizes in the GdFeO{sub 3}-structure, with space group Pnma and, combined with transmission electron microscopy, LaBaMnSnO{sub 6} in Imma. Both space groups are common in disordered double-perovskites. The Mn{sup 3+} and Sn{sup 4+} ions whose valence states were confirmed by X-ray absorption spectroscopy, are completely disordered over the B-sites and the BO{sub 6} octahedra are slightly distorted. LaAMnSnO{sub 6} are ferromagnetic semiconductors with a T{sub C} = 83 K for the Sr- and 66 K for the Ba-compound. The title compounds, together with the previously reported LaCaMnSnO{sub 6} provide an interesting example of progression from Pnma to Imma as the tolerance factor increases. An analysis of the relationship between space group and tolerance factor for the series LaAMnMO{sub 6} (A = Ca, Sr, Ba; M = Sn, Ru) provides a better understanding of the symmetry determination for double perovskites.

T Yang; T Perkisas; J Hadermann; M Croft; A Ignatov; M Greenblatt

2011-12-31T23:59:59.000Z

304

Test of internal-conversion theory with measurements in Cs-134 and Ba-137  

E-Print Network [OSTI]

We have measured the ratio of K-shell internal conversion coefficients, alpha(K), for the 127.5-keV E3 transition in Cs-134 and the 661.7-keV M4 transition in Ba-137. Previous measurements of these alpha(K) values led to a ratio that differed from...

Nica, N.; Hardy, John C.; Iacob, V. E.; Rockwell, W. E.; Trzhaskovskaya, M. B.

2007-01-01T23:59:59.000Z

305

Magnetic properties of HITPERM ,,Fe,Co...88Zr7B4Cu1 magnets M. A. Willard,a)  

E-Print Network [OSTI]

power applications requires new bulk soft magnetic materials that 1 are capable of operating at higher magnetization that persists to the phase transformation at 980 °C. Alternating current permeability experiments nanocrystalline Fe­Si­B­Nb­Cu alloys and nanocrystalline Fe­M­B­Cu M Zr, Nb, Hf, etc. alloys have been optimized

Laughlin, David E.

306

Precipitation and Thermal Fatigue in Ni-Ti-Zr Shape Memory Alloy Thin Films by Combinatorial nanoCalorimetry  

E-Print Network [OSTI]

- elastic martensitic phase transformation. They demonstrate enhanced power density compared to other associated with the transformation hysteresis by alloying tertiary components [6,7]. Ni-Ti-Zr is seen as one transformation. The response of the samples to heat treatments depends on composition and is controlled

307

Effect of La2Zr2O7 on Interfacial Resistance in Solid Oxide J. R. Smith,a  

E-Print Network [OSTI]

Effect of La2Zr2O7 on Interfacial Resistance in Solid Oxide Fuel Cells A. Chen,a J. R. Smith,a K. L manuscript received August 9, 2010. Published September 14, 2010. Solid oxide fuel cells SOFC are energy to gas phase transport in porous media, is controlled by optimizing electrode mi- crostructures

Florida, University of

308

Kinetic Modeling of Slurry Propylene Polymerization using rac-Et(Ind)2ZrCl2/MAO  

E-Print Network [OSTI]

by the isospecific metallocene rac-Et(Ind)2ZrCl2/MAO was investigated using a semi-batch reactor. A full factorial using a systematic optimization strategy. The model predicts that the insertion of the first propylene such understanding and affords opportunities for optimization. Thermoplastic industries for polypropylene (PP

309

First-principles study of the stability and migration of Kr, I and Xe in ZrO2  

SciTech Connect (OSTI)

The stability and migration of Kr, I and Xe in bulk ZrO2 and on the ZrO2 (1 1 1) surface have been studied by standard density functional theory (DFT) and the DFT-D2 method that corrects for the van der Waals interaction. Both methods show that Kr and Xe prefer to incorporate in the bulk phase rather than adsorb on the surface, and Xe is very mobile in the bulk state. For Kr and Xe adsorption on the surface, van der Waals interaction dominates, causing the weak interaction between the adsorbate and substrate. Iodine is found to have comparable stability in both phases and forms I O bonds with strong covalency. It exhibits higher mobility on the surface than in the bulk ZrO2, and diffusion from bulk-like state to surface state is an exothermic process. The fission product behavior in ZrO2 is shown to be a complicated synergetic effect of fission product atomic size, electron negativity, occupation site and phase structure of the host.

Xiao, Haiyan [University of Tennessee, Knoxville (UTK); Weber, William J [ORNL; Zhang, Yanwen [ORNL

2014-01-01T23:59:59.000Z

310

Thermodynamic model for the solubility of BaSeO4(cr) in the aqueous Ba2+-SeO42--Na+-H+-OH--H2O system: Extending to high selenate concentrations  

SciTech Connect (OSTI)

The solubility of Ba(SeO4, SO4) precipitates was determined as a function of the BaSeO4 mole fractions, ranging from 0.0015 to 0.3830, and time with an equilibration period extending to as long as 302 days. Equilibrium/steady state conditions in this system are reached in ? 65 days. Pitzer’s ion interaction model was used to calculate solid and aqueous phase activity coefficients. Thermodynamic analyses showed that the data do not satisfy Gibbs-Duhem equation, thereby demonstrating that a single-solid solution phase does not control both the selenate and sulfate concentrations. Our extensive data with log10 [Ba]) ranging from -3.6 to -5.9 mol.kg-1, log10 [SeO4]) ranging from -3.6 to -5.2 mol.kg-1, and log10 [SO4] ranging from -4.0 to -5.3 mol.kg-1 can be explained with the formation of an ideal BaSeO4 solid solution phase that controls the selenium concentrations and a slightly disordered/less-crystalline BaSO4(s) (log10 K0sp = -9.5 instead of -10.05 for barite) that controls the sulfate concentrations. In these experiments the BaSO4 component of the solid solution phase never reaches thermodynamic equilibrium with the aqueous phase. Thermodynamic interpretations of the data show that both the ideal BaSeO4 solid solution phase and less-crystalline BaSO4(s) phase are in equilibrium with each other in the entire range of BaSeO4 mole fractions investigated in this study.

Rai, Dhanpat; Felmy, Andrew R.; Moore, Dean A.; Kitamura, Akira; Yoshikawa, Hideki; Doi, Reisuke; Yoshida, Yasushi

2014-09-15T23:59:59.000Z

311

Electric transport properties of the pentatelluride materials HfTe{sub 5} and ZrTe{sub 5}  

SciTech Connect (OSTI)

The authors have measured the resistivity and thermopower of single crystals as well as polycrystalline pressed powders of the low-dimensional pentatelluride materials: HfTe{sub 5} and ZrTe{sub 5}. They have performed these measurements as a function of temperature between 5K and 320K. In the single crystals there is a peak in the resistivity for both materials at a peak temperature, T{sub p} where T{sub p} {approx} 80K for HfTe{sub 5} and T{sub p} {approx} 145K for ZrTe{sub 5}. Both materials exhibit a large p-type thermopower around room temperature which undergoes a change to n-type below the peak. These data are similar to behavior observed previously in these materials. They have also synthesized pressed powders of polycrystalline pentatelluride materials, HfTe{sub 5} and ZrTe{sub 5}. They have measured the resistivity and thermopower of these polycrystalline materials as a function of temperature between 5K and 320K. For the polycrystalline material, the room temperature thermopower for each of these materials is relatively high, +95 {micro}V/K and +65 {micro}V/K for HfTe{sub 5} and ZrTe{sub 5}, respectively. These values compare closely to thermopower values for single crystals of these materials. At 77 K, the thermopower is +55 {micro}V/K for HfTe{sub 5} and +35 {micro}V/K for ZrTe{sub 5}. In fact, the thermopower for the polycrystals decreases monotonically with temperature to T {approx} 5K, thus exhibiting p-type behavior over the entire range of temperature. As expected, the resistivity for the polycrystals is higher than the single crystal material, with values of 430 m{Omega}-cm and 24 m{Omega}-cm for HfTe{sub 5} and ZrTe{sub 5} respectively, compared to single crystal values of 0.35 m{Omega}-cm (HfTe{sub 5}) and 1.0 m{Omega}-cm (ZrTe{sub 5}). The authors have found that the peak in the resistivity evident in both single crystal materials is absent in these polycrystalline materials. They will discuss these materials in relation to their potential as candidates for thermoelectric applications.

Tritt, T.M.; Wilson, M.L.; Littleton, R.L. [and others

1997-07-01T23:59:59.000Z

312

Intrinsic Nanostructure in Zr2-xFe4Si16-y (x=0.81, y=6.06)  

SciTech Connect (OSTI)

We present a study of the crystal structure and physical properties of single crystals of a new Fe-based ternary compound, Zr2?x Fe4Si16?y(x=0.81,y=6.06). Zr1.19 Fe4Si9.94 is a layered compound, where stoichiometric ?-FeSi2-derived slabs are separated by Zr-Si planes with substantial numbers of vacancies. High resolution transmission electron microscopy (HRTEM) experiments show that these Zr-Si layers consist of 3.5nm domains where the Zrand Si vacancies are ordered within a supercell sixteen times the volume of the stoichiometric cell. Within these domains, the occupancies of the Zr and Si sites obey symmetry rules that permit only certain compositions, none of which by themselves reproduce the average composition found in x-ray diffraction experiments. Magnetic susceptibility and magnetization measurements reveal a small but appreciable number of magnetic moments that remain freely fluctuating to 1.8K, while neutron diffraction confirms the absence of bulk magnetic order with a moment of 0.2? B or larger down to 1.5K. Electrical resistivity measurements find that Zr1.19Fe4Si9.94 is metallic, and the modest value of the Sommerfeld coefficient of the specific heat ? = C/T suggests that quasi-particle masses are not particularly strongly enhanced. The onset of superconductivity at Tc 6K results in a partial resistive transition and a small Meissner signal, although a bulk-like transition is found in the specific heat. Sharp peaks in the ac susceptibility signal the interplay of the normal skin depth and the London penetration depth, typical of a system in which nano-sized superconducting grains are separated by a on-superconducting host. Ultra low field differential magnetic susceptibility measurements reveal the presence of a surprisingly large number of trace magnetic and superconducting phases, suggesting that the Zr-Fe-Si ternary system could be a potentially rich source of new bulk superconductor.

Smith, G J [Stony Brook University; Simonson, J W [Stony Brook University; Orvis, T [Stony Brook University; Marques, C [Stony Brook University; Grose, J E [Stony Brook University; Kistner-Morris, J J [Stony Brook University; Wu, L [Brookhaven National Laboratory; Cho, Kyuil [Ames Laboratory; Kim, Hyong june [Ames Laboratory; Tanatar, Makariy A [Ames Laboratory; Garlea, V O [Oak Ridge National Laboratory; Prozorov, Ruslan [Ames Laboratory; Zhu, Y [Brookhaven National Laboratory; Aronson, M C [Stony Brook University

2014-09-17T23:59:59.000Z

313

Pre- and post-irradiation characterization and properties measurements of ZrC coated surrogate TRISO particles  

SciTech Connect (OSTI)

Zirconium carbide is a candidate to either replace or supplement silicon carbide as a coating material in TRISO fuel particles for high temperature gas-cooled reactor fuels. Six sets of ZrC coated surrogate microsphere samples, fabricated by the Japan Atomic Energy Agency using the fluidized bed chemical vapor deposition method, were irradiated in the High Flux Isotope Reactor at the Oak Ridge National Laboratory. These developmental samples available for the irradiation experiment were in conditions of either as-fabricated coated particles or particles that had been heat-treated to simulate the fuel compacting process. Five sets of samples were composed of nominally stoichiometric compositions, with the sixth being richer in carbon (C/Zr = 1.4). The samples were irradiated at 800 and 1250 C with fast neutron fluences of 2 and 6 dpa. Post-irradiation, the samples were retrieved from the irradiation capsules followed by microstructural examination performed at the Oak Ridge National Laboratory's Low Activation Materials Development and Analysis Laboratory. This work was supported by the US Department of Energy Office of Nuclear Energy's Advanced Gas Reactor program as part of International Nuclear Energy Research Initiative collaboration with Japan. This report includes progress from that INERI collaboration, as well as results of some follow-up examination of the irradiated specimens. Post-irradiation examination items included microstructural characterization, and nanoindentation hardness/modulus measurements. The examinations revealed grain size enhancement and softening as the primary effects of both heat-treatment and irradiation in stoichiometric ZrC with a non-layered, homogeneous grain structure, raising serious concerns on the mechanical suitability of these particular developmental coatings as a replacement for SiC in TRISO fuel. Samples with either free carbon or carbon-rich layers dispersed in the ZrC coatings experienced negligible grain size enhancement during both heat treatment and irradiation. However, these samples experienced irradiation induced softening similar to stoichiometric ZrC samples.

Vasudevamurthy, Gokul [ORNL; Katoh, Yutai [ORNL; Hunn, John D [ORNL; Snead, Lance Lewis [ORNL

2010-09-01T23:59:59.000Z

314

On the densification of cubic ZrO{sub 2} nanocondensates by capillarity force and turbostratic C–Si–H multiple shell  

SciTech Connect (OSTI)

A turbostratic C–Si–H lamellar phase with 0.35–0.39 nm interspacing and ZrO{sub 2} condensates having cubic (c), tetragonal and monoclinic structures stabilized by increasing particle size were synthesized by pulsed laser ablation on Zr plate in TEOS and characterized by X-ray/electron diffraction and optical spectroscopy. The c-ZrO{sub 2} phase ca. 10% denser than the ambient lattice was stabilized as 3–10 nm sized cubo-octahedral nanoparticles but as abnormal large-sized (up to 30 nm) ones when encapsulated by the C{sub 1?x}Si{sub x}:H multiple shell with defective graphite-like structure units to exert an effective compressive stress. The potential application of such core–shell nanostructure with enhanced binding of Zr and O ions and implication for natural dynamic occurrence of the C{sub 1?x}Si{sub x}:H phase are addressed. - Graphical abstract: Lattice image of a typical cubic-ZrO{sub 2} particle densified by the turbostratic Si{sub x}C{sub 1?x}:H shell. Highlights: ? Turbostratic C–Si–H lamellar phase and ZrO{sub 2} condensates were synthesized by PLA. ? The c-ZrO{sub 2} phase ca. 10% denser than the ambient lattice was stabilized as 3–10 nm. ? The c-ZrO{sub 2} particles up to 30 nm were densified when encapsulated by the C{sub 1?x}Si{sub x}:H multiple shell. ? Tight ion binding of the c-ZrO{sub 2} due to capillarity force and turbostratic shell.

Wu, Chao-Hsien [Department of Materials and Optoelectronic Science, National Sun Yat-sen University, Kaohsiung 80424, Taiwan, ROC (China); Chen, Shuei-Yuan [Department of Mechanical and Automation Engineering, I-Shou University, Kaohsiung 84001, Taiwan, ROC (China); Shen, Pouyan, E-mail: pshen@mail.nsysu.edu.tw [Department of Materials and Optoelectronic Science, National Sun Yat-sen University, Kaohsiung 80424, Taiwan, ROC (China)

2013-04-15T23:59:59.000Z

315

Synthesis, structural and magnetic characterisation of the fully fluorinated compound 6H-BaFeO{sub 2}F  

SciTech Connect (OSTI)

The compound 6H-BaFeO{sub 2}F (P6{sub 3}/mmc) was synthesised by the low temperature fluorination of 6H-BaFeO{sub 3-d} using polyvinylidenedifluoride (PVDF) as a fluorination agent. Structural characterisation by XRD and NPD suggests that the local positions of the oxygen and fluorine atoms vary with no evidence for ordering on the anion sites. This compound shows antiferromagnetic ordering at room temperature with antiparallel alignment of the magnetic moments along the c-axis. The use of PVDF also allows the possibility of tuning the fluorine content in materials of composition 6H-BaFeO{sub 3-d}F{sub y} to any value of 0BaFeO{sub 2}F. Highlights: Black-Right-Pointing-Pointer The crystal structure of the hexagonal perovskite phase 6H-BaFeO{sub 2}F. Black-Right-Pointing-Pointer H-BaFeO{sub 2}F and 6H-BaFeO{sub 3-d}F{sub y} were prepared via low temperature fluorination using PVDF. Black-Right-Pointing-Pointer A structural investigation of the compounds BaFeO{sub 2}F is presented in detail. Black-Right-Pointing-Pointer This analysis suggests differences for the local coordination of O{sup 2-} and F{sup -} anions. Black-Right-Pointing-Pointer H-BaFeO{sub 2}F shows antiferromagnetic ordering at 300 K. Black-Right-Pointing-Pointer The magnetic moments align parallel to the a-axis.

Clemens, Oliver, E-mail: oliverclemens@online.de [School of Chemistry, University of Birmingham, Birmingham B15 2TT (United Kingdom)] [School of Chemistry, University of Birmingham, Birmingham B15 2TT (United Kingdom); Wright, Adrian J.; Berry, Frank J. [School of Chemistry, University of Birmingham, Birmingham B15 2TT (United Kingdom)] [School of Chemistry, University of Birmingham, Birmingham B15 2TT (United Kingdom); Smith, Ronald I. [ISIS Facility, Rutherford Appleton Laboratory, Harwell Oxford, Didcot, OX11 0QX (United Kingdom)] [ISIS Facility, Rutherford Appleton Laboratory, Harwell Oxford, Didcot, OX11 0QX (United Kingdom); Slater, Peter R. [School of Chemistry, University of Birmingham, Birmingham B15 2TT (United Kingdom)] [School of Chemistry, University of Birmingham, Birmingham B15 2TT (United Kingdom)

2013-02-15T23:59:59.000Z

316

Isoscalar giant dipole resonance in Zr-90, Sn-116, and Pb-208  

E-Print Network [OSTI]

0.26a 0.545b 43.3 61.4 7.75 0.567 aReference @13#. bReference @19#. Isoscalar giant dipole resonanc H. L. Clark, Y.-W. Lui Cyclotron Institute, Texas A&M University ~Received 30 August 2000; Strength functions for isoscalar dipole excitations... density for the ISGDR is @6# r~r !52b1 /RA3@3r2d/dr110r25/3^r2&d/dr1e~rd2/dr2 14d/dr !#ro~r !. For one state which exhausts the energy weighted sum rule @6# ?2001 The American Physical Society1 inelasti e RAPID COMMUNICATIONS H. L. CLARK, Y.-W. LUI...

Clark, HL; Lui, YW; Youngblood, David H.

2001-01-01T23:59:59.000Z

317

Synthesis, structural and magnetic characterisation of the fluorinated compound 15R-BaFeO{sub 2}F  

SciTech Connect (OSTI)

The compounds 15R-BaFeO{sub 2}F and 15R-BaFeO{sub 2.27}F{sub 0.5} have been synthesised by the low temperature fluorination of 15R-BaFeO{sub 3?d}F{sub 0.2} using polyvinylidenedifluoride (PVDF) as a fluorination agent. The materials have been structurally characterised by Rietveld analysis of the X-ray- and HRPD-powder neutron diffraction data. A detailed analysis of bond valence sums suggests that the oxide and fluoride ions order on the different anion sites. A reinvestigation of our recently published structure (Clemens et al., 2013) [34] of 6H-BaFeO{sub 2}F is also reported and incorporation of fluoride in h-type layers is also confirmed in this compound. The magnetic moments for 15R-BaFeO{sub 2}F and 15R-BaFeO{sub 2.25}F{sub 0.5} align in the a/b-plane with antiferromagnetic alignment of the moments between adjacent layers, and are flipped by 90° as compared to the precursor compound. 15R-BaFeO{sub 2}F exhibits very robust antiferromagnetism with a Néel temperature between 300 and 400 °C. - Graphical abstract: The crystal and magnetic structure of the perovskite phase 15R-BaFeO{sub 2}F. - Highlights: • 15R-BaFeO{sub 2}F and 15R-BaFeO{sub 2.27}F{sub 0.5}were prepared via low temperature fluorination using PVDF. • A structural investigation of the compounds BaFeO{sub 2}F is presented in detail. • This analysis suggests ordering of O{sup 2?} and F{sup ?} anions between different layers. • 15R-BaFeO{sub 2}F shows antiferromagnetic ordering at 300 K with T{sub N} ?300–400 °C. • The magnetic moments align in the a/b-plane.

Clemens, Oliver, E-mail: oliverclemens@online.de [School of Chemistry, The University of Birmingham, Birmingham B15 2TT (United Kingdom); Berry, Frank J. [School of Chemistry, The University of Birmingham, Birmingham B15 2TT (United Kingdom); Bauer, Jessica [Anorganische Festkörperchemie, Universität des Saarlandes, Am Markt, Zeile 3, 66125 Saarbrücken (Germany); Wright, Adrian J. [School of Chemistry, The University of Birmingham, Birmingham B15 2TT (United Kingdom); Knight, Kevin S. [ISIS Facility, Rutherford Appleton Laboratory, Harwell Oxford, Didcot OX11 0QX (United Kingdom); Slater, Peter R. [School of Chemistry, The University of Birmingham, Birmingham B15 2TT (United Kingdom)

2013-07-15T23:59:59.000Z

318

Investigation of oxygen point defects in cubic ZrO2 by density functional theory  

SciTech Connect (OSTI)

The energetics of formation and migration of the oxygen vacancy and interstitial in cubic ZrO2 are investigated by density functional theory calculations. In an O-rich environment, the negatively charged oxygen interstitial is the most dominant defect whereas, the positively charged oxygen vacancy is the most dominant defect under O-poor conditions. Oxygen interstitial migration occurs by the interstitialcy and the direct interstitial mechanisms, with calculated migration energy barriers of 2.94 eV and 2.15 eV, respectively. For the oxygen vacancy, diffusion is preferred along the <100> direction, and the calculated energy barriers are 0.26 eV for , 0.27 eV for and 0.54 eV for . These results indicate that oxygen diffusivity is higher through the vacancy-migration mechanism.

Liu, Bin [ORNL] [ORNL; Xiao, Haiyan [University of Tennessee, Knoxville (UTK)] [University of Tennessee, Knoxville (UTK); Zhang, Yanwen [ORNL] [ORNL; Aidhy, Dilpuneet S [ORNL] [ORNL; Weber, William J [ORNL] [ORNL

2014-01-01T23:59:59.000Z

319

Rapid Relaxation and Embrittlement of Zr-based Bulk Metallic Glasses by Electropulsing  

SciTech Connect (OSTI)

Mechanical relaxation and embrittlement of Zr52.5Cu17.9Ni14.6Al10Ti5 bulk metallic glasses were achieved rapidly by the direct current electropulsing treatment. The temperature profile was recorded by an infrared camera and it was found to be non-uniform in the treated specimen. Specifically, temperatures below the glass transition temperature, near and above the crystallization temperature could be ach- ieved, respectively, at different locations in the same treated specimen. Two sets of nanoindentation were conducted. While the first set investigated the mechanical properties of three individually elec- tropulsed specimens with different conditions, the second set indented a single treated specimen along its temperature gradient. Both sets of indentation revealed that by Joule heating to different tempera- tures, relaxation, embrittlement, and crystallization were significantly accelerated by electrical pulses. Results suggest that electropulsing provides an opportunity to simultaneously achieve plastic forming and mechanical property control of metallic glasses.

Yiu, P [Department of Materials Science and Engineering, National Taiwan University, Taipei 106, Taiwan; Chen, Y. C. [National Taiwan University of Science & Technology; Chu, J. P. [National Taiwan Ocean University; Chang, S Y [National Chung Hsing University; Bei, Hongbin [ORNL; Jang, J. S.C. [National Central University, Jhongli 32001, Taiwan; Hsueh, C. H. [Department of Materials Science and Engineering, National Taiwan University, Taipei 106, Taiwan

2013-01-01T23:59:59.000Z

320

Gamow-Teller response in deformed even and odd neutron-rich Zr and Mo isotopes  

E-Print Network [OSTI]

Beta-decay properties of neutron-rich Zr and Mo isotopes are investigated within a microscopic theoretical approach based on the proton-neutron quasiparticle random-phase approximation. The underlying mean field is described self-consistently from deformed Skyrme Hartree-Fock calculations with pairing correlations. Residual separable particle-hole and particle-particle forces are also included in the formalism. The structural evolution in these isotopic chains including both even and odd isotopes is analyzed in terms of the equilibrium deformed shapes. Gamow-Teller strength distributions, beta-decay half-lives, and beta-delayed neutron-emission probabilities are studied, stressing their relevance to describe the path of the nucleosynthesis rapid neutron capture process.

P. Sarriguren; A. Algora; J. Pereira

2014-03-05T23:59:59.000Z

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
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they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
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321

Current scaling of axially radiated power in dynamic hohlraums and dynamic hohlraum load design for ZR.  

SciTech Connect (OSTI)

We present designs for dynamic hohlraum z-pinch loads on the 28 MA, 140 ns driver ZR. The scaling of axially radiated power with current in dynamic hohlraums is reviewed. With adequate stability on ZR this scaling indicates that 30 TW of axially radiated power should be possible. The performance of the dynamic hohlraum load on the 20 MA, 100 ns driver Z is extensively reviewed. The baseline z-pinch load on Z is a nested tungsten wire array imploding onto on-axis foam. Data from a variety of x-ray diagnostics fielded on Z are presented. These diagnostics include x-ray diodes, bolometers, fast x-ray imaging cameras, and crystal spectrometers. Analysis of these data indicates that the peak dynamic radiation temperature on Z is between 250 and 300 eV from a diameter less than 1 mm. Radiation from the dynamic hohlraum itself or from a radiatively driven pellet within the dynamic hohlraum has been used to probe a variety of matter associated with the dynamic hohlraum: the tungsten z-pinch itself, tungsten sliding across the end-on apertures, a titanium foil over the end aperture, and a silicon aerogel end cap. Data showing the existence of asymmetry in radiation emanating from the two ends of the dynamic hohlraum is presented, along with data showing load configurations that mitigate this asymmetry. 1D simulations of the dynamic hohlraum implosion are presented and compared to experimental data. The simulations provide insight into the dynamic hohlraum behavior but are not necessarily a reliable design tool because of the inherently 3D behavior of the imploding nested tungsten wire arrays.

Mock, Raymond Cecil; Nash, Thomas J.; Sanford, Thomas W. L.

2007-03-01T23:59:59.000Z

322

Data:3a9b7691-e6ba-4286-9cce-e755902ae9ba | Open Energy Information  

Open Energy Info (EERE)

AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Home Page on Google Bookmark EERE: Alternative Fuels Data Center Home Page on Office of48d9ff47edf3 Noc7e1a8ffef-15f046e6d97e No revisionfb5101c21c4f No revision has beene755902ae9ba No revision

323

Phase characterization and grain size effects of nanophase Y{sub 2}O{sub 3}, ZrO{sub 2} and Y{sub 2}O{sub 3}-ZrO{sub 2} composites produced by the gas-phase condensation technique  

SciTech Connect (OSTI)

Nanophase (n-) ZrO{sub 2} was produce in its pure and partially stabilized form by the gas-phase condensation method. The material was examined by x-ray diffraction and Raman scattering to obtain information on the structural evolution of the material during sintering. Two types of Y{sub 2}O{sub 3} doped ZrO{sub 2} doped ZrO{sub 2} nanophase materials were made, one by co-deposition of n-Y{sub 2}O{sub 3} and n-ZrO{sub 2}. We have determined that the co-deposition process is the most effect means of doping the n-ZrO{sub 2}.

Foster, C.M.; Bai, G.R. [Argonne National Lab., IL (United States); Parker, J.C.; Ali, M.N. [Nanophase Technologies Corp., Darien, IL (United States)

1992-12-01T23:59:59.000Z

324

Phase characterization and grain size effects of nanophase Y[sub 2]O[sub 3], ZrO[sub 2] and Y[sub 2]O[sub 3]-ZrO[sub 2] composites produced by the gas-phase condensation technique  

SciTech Connect (OSTI)

Nanophase (n-) ZrO[sub 2] was produce in its pure and partially stabilized form by the gas-phase condensation method. The material was examined by x-ray diffraction and Raman scattering to obtain information on the structural evolution of the material during sintering. Two types of Y[sub 2]O[sub 3] doped ZrO[sub 2] doped ZrO[sub 2] nanophase materials were made, one by co-deposition of n-Y[sub 2]O[sub 3] and n-ZrO[sub 2]. We have determined that the co-deposition process is the most effect means of doping the n-ZrO[sub 2].

Foster, C.M.; Bai, G.R. (Argonne National Lab., IL (United States)); Parker, J.C.; Ali, M.N. (Nanophase Technologies Corp., Darien, IL (United States))

1992-12-01T23:59:59.000Z

325

Sympathetic cooling of the Ba{sup +} ion by collisions with ultracold Rb atoms: Theoretical prospects  

SciTech Connect (OSTI)

State-of-the-art ab initio techniques have been applied to compute the potential energy curves of the (BaRb){sup +} molecular ion in the Born-Oppenheimer approximation for the singlet and triplet states dissociating into the ground-state {sup 1}S Rb{sup +} ion and the Ba atom in the ground {sup 1}S state or the lowest singlet or triplet d excited states, and for the singlet and triplet states dissociating into the ground-state {sup 2}S Rb atom and the ground-state {sup 2}S Ba{sup +} ion. The ground-state potential energy was obtained with the coupled-cluster method restricted to single, double, and nonperturbative triple excitations. The first triplet states in the {Sigma}, {Pi}, and {Delta} symmetries were computed with the restricted open-shell coupled-cluster method restricted to single, double, and nonperturbative triple excitations. All other excited-state potential energy curves were computed using the equation of motion approach within the coupled-cluster singles, doubles, and linear triples framework. The long-range coefficients describing the electrostatic, induction, and dispersion interactions at large interatomic distances are also reported. The electric transition dipole moments governing the x {sup 1{Sigma}{yields}1{Sigma}},{sup 1{Pi}} transitions have been obtained as the first residue of the polarization propagator computed with the linear response coupled-cluster method restricted to single and double excitations. Nonadiabatic radial and angular coupling matrix elements as well as the spin-orbit coupling matrix elements have been evaluated using the multireference configuration-interaction method restricted to single and double excitations with a large active space. With these couplings, the spin-orbit-coupled (relativistic) potential energy curves for the 0{sup +} and 1 states relevant for the running experiments have been obtained. Finally, relativistic transition moments and nonadiabatic coupling matrix elements were obtained from the nonrelativistic results and spin-orbit eigenvectors. The electronic structure input has been employed in the single-channel scattering calculations of the collisional cross sections between the Ba{sup +} ion and Rb atom. Both nonrelativistic and relativistic potentials were used in these calculations. Our results show that the inelastic cross section corresponding to the charge transfer from the Rb atom to the Ba{sup +} ion is much smaller than the elastic one over a wide range of energies up to 1 mK. This suggests that sympathetic cooling of the Ba{sup +} ion by collisions with ultracold Rb atoms should be possible.

Krych, Michal; Skomorowski, Wojciech; Pawlowski, Filip; Moszynski, Robert; Idziaszek, Zbigniew [Institute of Theoretical Physics, Department of Physics, University of Warsaw, Hoza 69, 00-681 Warsaw (Poland) and Quantum Chemistry Laboratory, Department of Chemistry, University of Warsaw, Pasteura 1, 02-093 Warsaw (Poland); Quantum Chemistry Laboratory, Department of Chemistry, University of Warsaw, Pasteura 1, 02-093 Warsaw (Poland); Institute of Theoretical Physics, Department of Physics, University of Warsaw, Hoza 69, 00-681 Warsaw (Poland) and Institut de Physique de Rennes, UMR 6251 du CNRS and Universite de Rennes I, F-35042 Rennes Cedex (France)

2011-03-15T23:59:59.000Z

326

EffectsofTransitionMetalSubstitutionsontheIncommensurabilityandSpinFluctuationsinBaFe2As2byElasticandInelasticNeutronScattering  

SciTech Connect (OSTI)

Thespin uctuationspectrafromnonsuperconductingCu-substituted,andsuperconductingCo-substituted,BaFe2As2arecomparedquantitativelybyinelasticneutronscatteringmeasurementsandarefoundtobeindistinguishable.Whereasdiffractionstudiesshowtheappearanceofincommensu-ratespin-densitywaveorderinCoandNisubstitutedsamples,themagneticphasediagramforCusubstitutiondoesnotdisplayincommensurateorder,demonstratingthatsimpleelectroncountingbasedonrigid-bandconceptsisinvalid.Theseresults,supportedbytheoreticalcalculations,suggestthatsubstitu-tionalimpurityeffectsintheFeplaneplayasigni cantroleincontrollingmagnetismandtheappearanceofsuperconductivity,withCudistinguishedbyenhancedimpurityscatteringandsplit-bandbehavior.

Kim, M. G. [Ames Laboratory and Iowa State University; Lamsal, J. [Ames Laboratory and Iowa State University; Heitmann, T. W. [University of Missouri; Tucker, G. S. [Ames Laboratory and Iowa State University; Pratt, Daniel [Ames Laboratory and Iowa State University; Khan, S. N. [Ames Laboratory; Lee, Y. B. [Ames Laboratory and Iowa State University; Alam, A. [Ames Laboratory; Thaler, A. [Ames Laboratory and Iowa State University; Ni, N [Ames Laboratory and Iowa State University; Ran, S. [Ames Laboratory and Iowa State University; Budko, S L [Ames Laboratory and Iowa State University; Marty, Karol J [ORNL; Lumsden, Mark D [ORNL; Canfield, Paul [Ames Laboratory and Iowa State University; Harmon, B. N. [Ames Laboratory; Johnson, D. D. [Ames Laboratory and Iowa State University; Kreyssig, A. [Ames Laboratory and Iowa State University; Mcqueeney, R J [Ames Laboratory and Iowa State University; Goldman, A. I. [Ames Laboratory and Iowa State University

2012-01-01T23:59:59.000Z

327

Infrared-optical spectroscopy of transparent conducting perovskite (La,Ba)SnO{sub 3} thin films  

SciTech Connect (OSTI)

We have performed optical transmission, reflection, spectroscopic ellipsometry, and Hall effect measurements on the electron-doped La{sub x}Ba{sub 1–x}SnO{sub 3} (x?=?0.04) transparent thin films. From the infrared Drude response and plasma frequency analysis we determine the effective mass of the conducting electron m*?=?0.35m{sub 0}. In the visible-UV region the optical band gap shifts to high energy in (La,Ba)SnO{sub 3} by 0.18?eV compared with undoped BaSnO{sub 3} which, in the context of the Burstein-Moss analysis, is consistent with the infrared-m*. m* of BaSnO{sub 3} is compared with other existing transparent conducting oxides (TCO), and implication on search for high-mobility TCO compounds is discussed.

Seo, Dongmin; Yu, Kwangnam; Jun Chang, Young; Choi, E. J., E-mail: echoi@uos.ac.kr [Department of Physics, University of Seoul, Seoul 130-743 (Korea, Republic of); Sohn, Egon; Hoon Kim, Kee [Center for Novel States of Complex Materials Research, Department of Physics and Astronomy, Seoul National University, Seoul 151-747 (Korea, Republic of)

2014-01-13T23:59:59.000Z

328

An, Yanming, Professor, Languages. BA, 1982, MA, 1985, Fudan University (China); PhD, University of Michigan,  

E-Print Network [OSTI]

, 1997 Andrews, Phillip A., Assistant Professor, Military Leadership; Major, U.S. Army. BA, University, 1978, PhD, 1985, University of Connecticut Armstrong, James B., Adjunct Professor, School

Stuart, Steven J.

329

Angle-resolved photoemission spectroscopy study of HgBa[subscript 2]CuO[subscript 4+?  

E-Print Network [OSTI]

HgBa[subscript 2]CuO[subscript 4+?]. (Hg1201) has been shown to be a model cuprate for scattering, optical, and transport experiments, but angle-resolved photoemission spectroscopy (ARPES) data are still lacking owing to ...

Chan, M. K.

330

The elastic and piezoelectric properties of tungsten bronze ferroelectric crystals ,,Sr0.7Ba0.3...2NaNb5O15 and ,,Sr0.3Ba0.7...2NaNb5O15  

E-Print Network [OSTI]

The elastic and piezoelectric properties of tungsten bronze ferroelectric crystals ,,Sr0.7Ba0 and piezoelectric constants of tungsten bronze ferroelectric crystals Sr0.7Ba0.3 2NaNb5O15 SBNN70 and Sr0.3Ba0.7 2Na. INTRODUCTION Ferroelectric crystals with tungsten bronze structure are another attractive family beside

Cao, Wenwu

331

Single crystal growth and characterization of the large-unit-cell compound Cu13Ba  

SciTech Connect (OSTI)

Single crystals of Cu13Ba were successfully grown out of Ba–Cu self flux. Temperature dependent magnetization, M (T ), electrical resistivity, ?(T)?(T), and specific heat, Cp(T)Cp(T), data are reported. Isothermal magnetization measurements, M(H)M(H), show clear de Haas-van Alphen oscillations at T = 2 K for applied fields as low as View the MathML source?0H=1T. An anomalous behavior of the magnetic susceptibility is observed up to T ? 50 K reflecting the effect of de Haas-van Alphen oscillations at fairly high temperatures. The field- and temperature-dependencies of the magnetization indicate the presence of diluted magnetic impurities with a concentration of the order of 0.01 at.%. Accordingly, the minimum and lower temperature rise observed in the electrical resistivity at and below T = 15 K is attributed to the Kondo-impurity effect.

Jesche, Anton [Ames Laboratory; Budko, Serguei L. [Ames Laboratory; Canfield, Paul C. [Ames Laboratory

2013-10-31T23:59:59.000Z

332

Effect of 3d doping on the electronic structure of BaFe2As2  

SciTech Connect (OSTI)

The electronic structure of BaFe2As2 doped with Co, Ni and Cu has been studied by a variety of experimental and theoretical methods, but a clear picture of the dopant 3d states has not yet emerged. Herein we provide experimental evidence of the distribution of Co, Ni and Cu 3d states in the valence band. We conclude that the Co and Ni 3d states provide additional free carriers to the Fermi level, while the Cu 3d states are found at the bottom of the valence band in a localized 3d10 shell. These findings help shed light on why superconductivity can occur in BaFe2As2 doped with Co and Ni but not Cu.

McLeod, John A.; Buling, A.; Green, R.J.; Boyko, T.D.; Skorikov, N.A.; Kurmaev, E.Z.; Neumann, M.; Finkelstein, L.D.; Ni, Ni; Thaler, Alexander; Budko, Serguei L.; Canfield, Paul; Moewes, A.

2012-04-25T23:59:59.000Z

333

Superconductivity at 34 K in the K/Ba/Bi/O system  

SciTech Connect (OSTI)

The critical temperature for superconductivity in the (Ba, K)BiO{sub 3} system has been increased to 34 K. With each such increase of T{sub c} in a system containing no copper it becomes increasingly likely that the mechanisms for superconductivity in the Bi-based and the Cu-based oxide superconductors are very closely related to each other. Since the (Ba, K)BiO{sub 3} superconductors possess the cubic perovskite structure, the mechanism for high T{sub c} would then not related directly to the two-dimensional character of the copper oxide superconductors or to the magnetism in such systems. 12 refs., 1 fig.

Jones, N.L.; Parise, J.B.; Flippen, R.B.; Sleight, A.W. (E.I. DuPont de Nemours and Co., Wilmington, DE (USA))

1989-02-01T23:59:59.000Z

334

Optical properties of Pr-doped BaY{sub 2}F{sub 8}  

SciTech Connect (OSTI)

Crystalline samples of Pr-doped BaY{sub 2}F{sub 8} (BaYF) were prepared by zone melting technique. The pure phase obtained was identified by X-ray diffraction measurement. Optical absorption result was evaluated and it showed that the formation of the absorption bands can be connected to color centers generated by radiation in the matrix. Radioluminescence emission measurements after excitation by X-ray showed that the material exhibited components responsible for long lasting phosphorescence. Short decay times were also evaluated, the measurements showed a fast component around 70?ns associated to the 4f{sup 1}5d{sup 1} ? 4f{sup 2} transition of the Pr{sup 3+} ion. The Thermoluminescence (TL) results indicate the presence of two trapping centers.

Andrade, Adriano B., E-mail: abandrade1@gmail.com; Mello, Ana C. S. de; Valerio, Mário E. G. [Physics Department, Federal University of Sergipe, 49100-000 Săo Cristovăo, SE (Brazil); Rezende, Marcos V. dos S. [Physics Department, Federal University of Sergipe, 49500-000 Itabaiana, SE (Brazil); Baldochi, Sonia L. [IPEN-CNEN/SP, CEP 11049, 05422-970 Săo Paulo, SP (Brazil)

2014-08-07T23:59:59.000Z

335

A study of the anodic polarization behavior of Zr(50)Cu(40-x)Al(10)Pd(x) BMG with scanning Auger microanalysis  

SciTech Connect (OSTI)

The anodic-polarization behaviors of Zr50Cu40-XAl10PdX (x = 0 and 7 atomic %) BMGs were investigated in 0.6 M NaCl electrolytes. Initial anodic polarization of both alloys yielded regions where small increases in the applied potential induced significant increases in the current density. Continued polarization of both BMGs resulted in diffusion controlled regimes. However, the limiting diffusion current density of Zr50Cu33Al10Pd7 was higher than that of Zr50Cu40Al10. Scanning Auger microanalysis was used to investigate the oxide formed during polarization and to analyze the chemistry within corrosion pits. The pits formed on both BMGs were enriched with Cu and Cl. Corrosion pits on Zr50Cu33Al10Pd7 were additionally enriched with Pd. A corrosion mechanism relating to the formation of CuCl and Cu2O is proposed based on both the polarization and microanalysis results.

Green, Brandice [ORNL; Meyer III, Harry M [ORNL; Benson, Roberto S [ORNL; Yokoyama, Y [Institute for Materials Research; Liaw, Peter K [University of Tennessee, Knoxville (UTK); Liu, Chain T [ORNL

2008-01-01T23:59:59.000Z

336

All undergraduate/Bachelor degrees BSc/BA/BEng/MEng 13,000 Childhood Studies MA 12,500  

E-Print Network [OSTI]

All undergraduate/Bachelor degrees BSc/BA/BEng/MEng ÂŁ13,000 Childhood Studies MA ÂŁ12,500 Developmental and Therapeutic Play MA/PGDip/PGCert ÂŁ12,500 Health Care Management MSc ÂŁ13,000 Public Health/BA/BEng/MEng ÂŁ11,750 Ancient Egyptian Culture MA ÂŁ12,500 Ancient History & Classical Culture MA ÂŁ12,500 Ancient

Harman, Neal.A.

337

Zinc ferrite nanoparticles as MRI contrast agentsw Carlos Ba rcena,a  

E-Print Network [OSTI]

Zinc ferrite nanoparticles as MRI contrast agentsw Carlos Ba´ rcena,a Amandeep K. Sra,a Girija S, a series of spinel-structured ferrites, MFe2O4 (M = Mn2+ , Fe2+ , Co2+ , Ni2+ ), were reported as novel MRI.e., Mn2+ occupies both A and B sites), whereas the other metal ferrites have an inverse spinel structure

Gao, Jinming

338

Lifshitz Transition and Chemical Instabilities in Ba1 xKxFe2As2 Superconductors  

SciTech Connect (OSTI)

Forsolid-solutionBa1 xKxFe2As2FermisurfaceevolutionismappedviaBlochspectralfunctionscalculatedusingdensityfunctionaltheoryimplementedinKorringa-Kohn-Rostokermultiplescatteringtheorywiththecoherent-potentialapproximation.Spectralfunctionsrevealelectronicdispersion,topology,orbitalcharacter,andbroadening(electron-lifetimeeffects)duetochemicaldisorder.Dissolutionofelectroncylindersoccursnearx 0.9withanonuniform,topological(Lifshitz)transition,reducingtheinterbandinteractions;yetthedispersionmaintainsitsdxzordyzcharacter.Formationenergiesindicatealloyingatx 0.35,asobserved,andatendencyforsegregationontheK-rich(x>0.6)side,explainingthedifficultyofcontrollingsamplequalityandtheconflictingresultsbetweencharacterizedelectronicstructures.OurresultsrevealFermisurfacetransitionsinalloyedsamplesthatinfluencestonodalsuperconductivityandsuggesttheoriginfordeviationsofcommontrendsinFe-basedsuperconductors,suchasBud ko-Ni-Canfieldscaling.

Khan, Suffian N. [University of Illinois, Urbana-Champaign] [University of Illinois, Urbana-Champaign; Johnson, Duane D. [University of Illinois, Urbana-Champaign] [University of Illinois, Urbana-Champaign

2014-01-01T23:59:59.000Z

339

Brazing ZrO{sub 2} ceramic to Ti–6Al–4V alloy using NiCrSiB amorphous filler foil: Interfacial microstructure and joint properties  

SciTech Connect (OSTI)

Reliable brazing of ZrO{sub 2} ceramic and Ti–6Al–4V alloy was achieved using NiCrSiB amorphous filler foil. The interfacial microstructure of ZrO{sub 2}/Ti–6Al–4V joints was characterized by scanning electron microscope, energy dispersive spectrometer and micro-focused X-ray diffractometer. The effects of brazing temperature on the interfacial microstructure and joining properties of brazed joints were investigated in detail. Active Ti of Ti–6Al–4V alloy dissolved into molten filler metal and reacted with ZrO{sub 2} ceramic to form a continuous TiO reaction layer, which played an important role in brazing. Various reaction phases including Ti{sub 2}Ni, Ti{sub 5}Si{sub 3} and ?-Ti were formed in brazed joints. With an increasing of brazing temperature, the TiO layer thickened gradually while the Ti{sub 2}Ni amount reduced. Shear test indicated that brazed joints tend to fracture at the interface between ZrO{sub 2} ceramic and brazing seam or Ti{sub 2}Ni intermetallic layer. The maximum average shear strength reached 284.6 MPa when brazed at 1025 °C for 10 min. - Graphical Abstract: Interfacial microstructure of ZrO{sub 2}/TC4 joint brazed using NiCrSiB amorphous filler foil was: ZrO{sub 2}/TiO/Ti{sub 2}Ni + ?-Ti + Ti{sub 5}Si{sub 3}/?-Ti/Widmanstätten structure/TC4. - Highlights: • Brazing of ZrO{sub 2} ceramic and Ti-6Al-4V alloy was achieved. • Interfacial microstructure was TiO/Ti{sub 2}Ni + ? + Ti{sub 5}Si{sub 3}/?/Widmanstätten structure. • The formation of TiO produced the darkening effect of ZrO{sub 2} ceramic. • The highest joining strength of 284.6MPa was obtained.

Cao, J., E-mail: cao_jian@hit.edu.cn [Shandong Provincial Key Laboratory of Special Welding Technology, Harbin Institute of Technology at Weihai, Weihai 264209 (China); State Key Laboratory of Advanced Welding and Joining, Harbin Institute of Technology, Harbin 150001 (China); Song, X.G., E-mail: song_xiaoguohit@yahoo.com.cn [Shandong Provincial Key Laboratory of Special Welding Technology, Harbin Institute of Technology at Weihai, Weihai 264209 (China); State Key Laboratory of Advanced Welding and Joining, Harbin Institute of Technology, Harbin 150001 (China); Li, C., E-mail: li_chun1989@yahoo.cn [State Key Laboratory of Advanced Welding and Joining, Harbin Institute of Technology, Harbin 150001 (China); Zhao, L.Y., E-mail: Zhao_ly@163.com [State Key Laboratory of Advanced Welding and Joining, Harbin Institute of Technology, Harbin 150001 (China); Feng, J.C., E-mail: feng_jicai@163.com [Shandong Provincial Key Laboratory of Special Welding Technology, Harbin Institute of Technology at Weihai, Weihai 264209 (China); State Key Laboratory of Advanced Welding and Joining, Harbin Institute of Technology, Harbin 150001 (China)

2013-07-15T23:59:59.000Z

340

Two- and Three-Body Charmless B Decays at BaBar  

SciTech Connect (OSTI)

We report recent measurements of rare charmless B decays performed by BaBar. The results are based on the final BaBar dataset of 424 fb{sup -1} collected at the PEP-II B-factory based at the SLAC National Accelerator Laboratory. The study of rare B decays is a key ingredient to meet two of the main goals of the B-factories: assessing the validity of the Cabibbo-Kobayashi-Maskawa (CKM) picture of CP-violation by precisely measuring the elements of the Unitarity Triangle (UT), and searching for hints of New Physics (NP), or otherwise constraining NP scenarios, in processes which are suppressed in the Standard Model (SM). In loop processes, in particular, NP at some higher energy scale may manifest itself in the low energy effective theory as new couplings, such as those introduced by new very massive virtual particles in the loop. In NP searches hadronic uncertainties can play a major role, expecially for branching fraction measurements. Many theoretical uncertainties cancel in ratios of amplitudes, and most NP probes are therefore of this kind. In the following sections we report recent measurements, performed by the BaBar Collaboration, that are relevant to NP searches in charmless hadronic B decays.

Stracka, Simone; /Milan U. /INFN, Milan; ,

2012-04-05T23:59:59.000Z

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341

Hydrostatic pressure (8 GPa) dependence of electrical resistivity of BaCo{sub 2}As{sub 2} single crystal  

SciTech Connect (OSTI)

Graphical abstract: - Highlights: • Single crystals of BaCo{sub 2}As{sub 2} were grown by CoAs self-flux method. • We have studied pressure effects (8 GPa) on dc electrical resistivity of BaCo{sub 2}As{sub 2}. • On applied external pressure BaCo{sub 2}As{sub 2} remains a metallic state up to 8 GPa. • Superconductivity is absent in BaCo{sub 2}As{sub 2} because of its proximity to ferromagnetism. - Abstract: The pressure dependence of the electrical resistivity of BaCo{sub 2}As{sub 2} single crystal as a function of temperature was measured at ambient and high pressures up to 8 GPa for the first time using cubic anvil high pressure cell. It is observed that at room temperature the resistivity monotonically decreases with increasing pressure and it remains in the metallic state even at an applied pressure of 8 GPa. From the temperature dependence of the resistivity measurements under pressure, we found that superconductivity is absent up to 8 GPa. The value of the electron's scattering factor (A) is found to be large at ambient pressure and it decreases with the application of pressure, indicating that the substantial electron correlation effect of BaCo{sub 2}As{sub 2} is reduced under pressure, revealing a dramatic change of density of states at the Fermi energy.

Ganguli, Chandreyee; Matsubayashi, Kazuyuki; Ohgushi, Kenya [Institute for Solid State Physics, The University of Tokyo, Kashiwanoha, Kashiwa, Chiba 277-8581 (Japan); Uwatoko, Yoshiya, E-mail: uwatoko@issp.u-tokyo.ac.jp [Institute for Solid State Physics, The University of Tokyo, Kashiwanoha, Kashiwa, Chiba 277-8581 (Japan); Kanagaraj, Moorthi [Centre for High Pressure Research, School of Physics, Bharathidasan University, Tiruchirappalli 620024 (India); Arumugam, Sonachalam, E-mail: sarumugam1963@yahoo.com [Centre for High Pressure Research, School of Physics, Bharathidasan University, Tiruchirappalli 620024 (India)

2013-10-15T23:59:59.000Z

342

Characterization of self-propagating formation reactions in Ni/Zr multilayered foils using reaction heats, velocities, and temperature-time profiles  

DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

We report on intermetallic formation reactions in vapor-deposited multilayered foils of Ni/Zr with 70 nm bilayers and overall atomic ratios of Ni:Zr, 2 Ni:Zr, and 7 Ni:2 Zr. The sequence of alloy phase formation and the stored energy is evaluated at slow heating rates (~1 K/s) using differential scanning calorimetry (DSC) traces to 725şC. All three chemistries initially form a Ni-Zr amorphous phase which crystallizes first to the intermetallic NiZr. The heat of reaction to the final phase is 34-36 kJ/mol atom for all chemistries. Intermetallic formation reactions are also studied at rapid heating rates (greater than 105 K/s) in high temperature, self-propagating reactions which can be ignited in these foils by an electric spark. We find that reaction velocities and maximum reaction temperatures (Tmax) are largely independent of foil chemistry at 0.6 ± 0.1 m/s and 1220 ± 50 K, respectively, and that the measured Tmax is more than 200 K lower than predicted adiabatic temperatures (Tad). The difference between Tmax and Tad is explained by the prediction that transformation to the final intermetallic phases occurs after Tmax and results in the release of 20-30 % of the total heat of reaction and a delay in rapid cooling.

Barron, S. C.; Knepper, R.; Walker, N.; Weihs, T. P.

2011-01-11T23:59:59.000Z

343

Behavior of the electroless composite films plated from a Ni-P bath with metallic dispersion of Zr and Nb powders  

SciTech Connect (OSTI)

An electroless Ni-Zr-P composite film and a Ni-Nb-P composite film were plated and their heat-treating behaviors were investigated. The addition of 20g dm/sup -3/ of metallic powder resulted in a composite film that contained 21.2 weight percent (w/o) of Zr. (13.8 atom percent (a/o)), or 4.8 w/o of Nb. (2.9 a/o), respectively. Both metallic powders were dispersed uniformly throughout the film. The metallic Ni formed by the crystallization on the Ni-P matrix diffused into the metallic powders, and the amorphous Ni-Zr and Ni-Nb phases were formed by heat-treatment at 500/sup 0/ or 300/sup 0/C. Some parts of the amorphous Ni-Zr phases and the metallic Ni phases combined to form intermetallic compounds by heat-treatment at 600/sup 0/C. The nickel-rich parts of the amorphous Ni-Nb phase were converted into a metastable Ni-Nb phase (zeta phase) or a Ni-Nb solid solution by heat-treatment at 700/sup 0/C. The longer heating time at 400/sup 0/C increased the amount of the Ni-Zr amorphous phase: however, it decreased the reactivity of the amorphous Ni-Zr phase. The same heat-treatment of 400/sup 0/C did not give the considerable change on the amorphous Ni-Nb phase.

Osaka, T.; Koiwa, I.; Usuda, M.; Arai, K.; Saito, I.

1989-04-01T23:59:59.000Z

344

Characterization of Ceramic Plasma-Sprayed Coatings, and Interaction Studies Between U-Zr Fuel and Ceramic Coated Interface at an Elevated Temperature  

SciTech Connect (OSTI)

Candidate coating materials for re-usable metallic nuclear fuel crucibles, HfN, TiC, ZrC, and Y2O3, were plasma-sprayed onto niobium substrates. The coating microstructure and the thermal cycling behavior were characterized, and U-Zr melt interaction studies carried out. The Y2O3 coating layer had a uniform thickness and was well consolidated with a few small pores scattered throughout. While the HfN coating was not well consolidated with a considerable amount of porosity, but showed somewhat uniform thickness. Thermal cycling tests on the HfN, TiC, ZrC, and Y2O3 coatings showed good cycling characteristics with no interconnected cracks forming even after 20 cycles. Interaction studies done on the coated samples by dipping into a U-20wt.%Zr melt indicated that HfN and Y2O3 did not form significant reaction layers between the melt and the coating while the TiC and the ZrC coatings were significantly degraded. Y2O3 exhibited the most promising performance among HfN, TiC, ZrC, and Y2O3 coatings.

Ki Hwan Kim; Chong Tak Lee; R. S. Fielding; J. R. Kennedy

2011-08-01T23:59:59.000Z

345

Phase Characteristics of a Number of U-Pu-Am-Np-Zr Metallic Alloys for Use as Fast Reactor Fuels  

SciTech Connect (OSTI)

Metallic fuel alloys consisting of uranium, plutonium, and zirconium with minor additions of americium and neptunium are under evaluation for potential use to transmute long-lived transuranic actinide isotopes in fast reactors. A series of test designs for the Advanced Fuel Cycle Initiative (AFCI) have been irradiated in the Advanced Test Reactor (ATR), designated as the AFC-1 and AFC-2 designs. Metal fuel compositions in these designs have included varying amounts of U, Pu, Zr, and minor actinides (Am, Np). Investigations into the phase behavior and relationships based on the alloy constituents have been conducted using x-ray diffraction and differential thermal analysis. Results of these investigations, along with proposed relationships between observed behavior and alloy composition, are provided. In general, observed behaviors can be predicted by a ternary U-Pu-Zr phase diagram, with transition temperatures being most dependent on U content. Furthermore, the enthalpy associated with transitions is strongly dependent on the as-cast microstructural characteristics.

Douglas E. Burkes; J. Rory Kennedy; Thomas Hartmann; Cynthia A. Papesch; Denis D. Keiser, Jr.

2010-01-01T23:59:59.000Z

346

Quarkonium Spectroscopy And Search for New States at BaBar  

SciTech Connect (OSTI)

The BaBar experiment at the PEP-II B-factory gives excellent opportunities for the quarkonium spectroscopy. Investigation of the properties of new states like the X(3872), Y(3940) and Y(4260) are performed aiming to understand their nature. Recent BaBar results will be presented in this paper. At the B-factories charmonium and charmonium-like states are copiously produced via several mechanisms: in B decay (color suppressed b {yields} c transition), double charmonium production (e{sup +}e{sup -} {yields} c{bar c} + c{bar c}), two photons production ({gamma}*{gamma}* {yields} c{bar c}, where the c{bar c} state has positive C-parity) and in initial state radiation (ISR) when the e{sup {+-}} in its initial state emits a photon lowering the effective center of mass energy of the e{sup +}e{sup -} interaction (e{sup +}e{sup -} {yields} {gamma}{sub ISR} + c{bar c}, where the charmonium state has the quantum numbers J{sup PC} = 1{sup -2}). Many new states have been recently discovered at the B-factories, BaBar and Belle, above the D{bar D} threshold in the charmonium energy region. While some of them appear to be consistent with conventional c{sub c} states others do not fit with any expectation. Several interpretations for these states have been proposed: for some of them the mass values suggest that they could be conventional charmonia, but also other interpretations like D{sup 0}{bar D}*{sup 0} molecule or diquark-antidiquark states among many other models have been advanced. Reviews can be found in Refs. [1][2]. In all cases the picture is not completely clear. This situation could be remedied by a coherent search of the decay pattern to D{bar D}, search for production in two-photon fusion and ISR, and of course improving the statistical precision upon the current measurements. The BaBar experiment at the PEP-II asymmetric collider, designed to perform precision measurement of CP violation in the B meson system, has an extensive quarkonium spectroscopy program. Recent BaBar outcomes on the X(3872) and Y(4260) and a new result on the Y(3940) are reported here.

Cibinetto, G.

2011-11-04T23:59:59.000Z

347

Thermal conductivity profile determination in proton-irradiated ZrC by spatial and frequency scanning thermal wave methods  

SciTech Connect (OSTI)

Using complementary thermal wave methods, the irradiation damaged region of zirconium carbide (ZrC) is characterized by quantifiably profiling the thermophysical property degradation. The ZrC sample was irradiated by a 2.6 MeV proton beam at 600 °C to a dose of 1.75 displacements per atom. Spatial scanning techniques including scanning thermal microscopy (SThM), lock-in infrared thermography (lock-in IRT), and photothermal radiometry (PTR) were used to directly map the in-depth profile of thermal conductivity on a cross section of the ZrC sample. The advantages and limitations of each system are discussed and compared, finding consistent results from all techniques. SThM provides the best resolution finding a very uniform thermal conductivity envelope in the damaged region measuring ?52 ± 2 ?m deep. Frequency-based scanning PTR provides quantification of the thermal parameters of the sample using the SThM measured profile to provide validation of a heating model. Measured irradiated and virgin thermal conductivities are found to be 11.9 ± 0.5 W m{sup ?1} K{sup ?1} and 26.7 ±1 W m{sup ?1} K{sup ?1}, respectively. A thermal resistance evidenced in the frequency spectra of the PTR results was calculated to be (1.58 ± 0.1) × 10{sup ?6} m{sup 2} K W{sup ?1}. The measured thermal conductivity values compare well with the thermal conductivity extracted from the SThM calibrated signal and the spatially scanned PTR. Combined spatial and frequency scanning techniques are shown to provide a valuable, complementary combination for thermal property characterization of proton-irradiated ZrC. Such methodology could be useful for other studies of ion-irradiated materials.

Jensen, C. [GRESPI, Multiscale Thermophysics Lab., Université de Reims Champagne-Ardenne URCA, Moulin de la Housse BP 1039, Reims 51687 (France) [GRESPI, Multiscale Thermophysics Lab., Université de Reims Champagne-Ardenne URCA, Moulin de la Housse BP 1039, Reims 51687 (France); Department of Mechanical and Aerospace Engineering, Utah State University, Logan, Utah 84322 (United States); Chirtoc, M.; Horny, N.; Antoniow, J. S.; Pron, H. [GRESPI, Multiscale Thermophysics Lab., Université de Reims Champagne-Ardenne URCA, Moulin de la Housse BP 1039, Reims 51687 (France)] [GRESPI, Multiscale Thermophysics Lab., Université de Reims Champagne-Ardenne URCA, Moulin de la Housse BP 1039, Reims 51687 (France); Ban, H. [Department of Mechanical and Aerospace Engineering, Utah State University, Logan, Utah 84322 (United States)] [Department of Mechanical and Aerospace Engineering, Utah State University, Logan, Utah 84322 (United States)

2013-10-07T23:59:59.000Z

348

The new barium zinc mercurides Ba{sub 3}ZnHg{sub 10} and BaZn{sub 0.6}Hg{sub 3.4} - Synthesis, crystal and electronic structure  

SciTech Connect (OSTI)

The title compounds Ba{sub 3}ZnHg{sub 10} and BaZn{sub 0.6}Hg{sub 3.4} were synthesized from stoichiometric ratios of the elements in Ta crucibles. Their crystal structures, which both represent new structure types, have been determined using single crystal X-ray data. The structure of Ba{sub 3}ZnHg{sub 10} (orthorhombic, oP28, space group Pmmn, a=701.2(3), b=1706.9(8), c=627.3(3)pm, Z=2, R1=0.0657) contains folded 4{sup 4} Hg nets, where the meshes form the bases of flat rectangular pyramids resembling the structure of BaAl{sub 4}. The flat pyramids are connected via Hg-Zn/Hg bonds, leaving large channels at the folds, in which Ba(1) and Hg(2) atoms alternate. Whereas the remaining Hg/Zn atoms form a covalent 3D network of three- to five-bonded atoms with short M-M distances (273-301 pm; CN 9-11), the Hg(2) atoms in the channels adopt a comparatively large coordination number of 12 and increased distances (317-348 pm) to their Zn/Hg neighbours. In the structure of BaZn{sub 0.6}Hg{sub 3.4} (cubic, cI320, space group I4{sup Macron }3d, a=2025.50(7) pm, Z=64, R1=0.0440), with a chemical composition not much different from that of Ba{sub 3}ZnHg{sub 10}, the Zn/Hg atoms of the mixed positions M(1/2) are arranged in an slightly distorted primitive cubic lattice with a 4 Multiplication-Sign 4 Multiplication-Sign 4 subcell relation to the unit cell. The 24 of the originating 64 cubes contain planar cis tetramers Hg(5,6){sub 4} with Hg in a nearly trigonal planar or tetrahedral coordination. In another 24 of the small cubes, two opposing faces are decorated by Hg(3,4){sub 2} dumbbells, two by Ba(2) atoms respectively. The third type of small cubes are centered by Ba(1) atoms only. The complex 3D polyanionic Hg/Zn network thus formed is compared with the Hg partial structure in Rb{sub 3}Hg{sub 20} applying a group-subgroup relation. Despite their different overall structures, the connectivity of the negatively charged Hg atoms, the rather metallic Zn bonding characteristic (as obtained from FP-LAPW band structure calculations) and the coordination number of 16 for all Ba cations relate the two title compounds. - Graphical abstract: Six of the 64 small sub-cubes of three types (A, B, C) forming the unit cell of the Hg-rich mercuride BaZn{sub 0.6}Hg{sub 3.4}. Highlights: Black-Right-Pointing-Pointer Two new Hg-rich Ba mercurides, both synthesized from the elements in pure phase. Black-Right-Pointing-Pointer BaZn{sub 0.6}HgG{sub 3.4} and Ba{sub 3}ZnHg{sub 10} with new complex structure types. Black-Right-Pointing-Pointer Structure relation to other complex cubic intermetallics. Black-Right-Pointing-Pointer Discussion of covalent and metallic bonding aspects, as found by the structure features and band structure calculations.

Schwarz, Michael; Wendorff, Marco [Institut fuer Anorganische und Analytische Chemie, University of Freiburg, Albertstr. 21, D-79104 Freiburg (Germany)] [Institut fuer Anorganische und Analytische Chemie, University of Freiburg, Albertstr. 21, D-79104 Freiburg (Germany); Roehr, Caroline, E-mail: caroline@ruby.chemie.uni-freiburg.de [Institut fuer Anorganische und Analytische Chemie, University of Freiburg, Albertstr. 21, D-79104 Freiburg (Germany)] [Institut fuer Anorganische und Analytische Chemie, University of Freiburg, Albertstr. 21, D-79104 Freiburg (Germany)

2012-12-15T23:59:59.000Z

349

Dynamic study on fusion reactions for $^{40,48}$Ca+$^{90,96}$Zr around Coulomb barrier  

E-Print Network [OSTI]

By using the updated improved Quantum Molecular Dynamics model in which a surface-symmetry potential term has been introduced for the first time, the excitation functions for fusion reactions of $^{40,48}$Ca+$^{90,96}$Zr at energies around the Coulomb barrier have been studied. The experimental data of the fusion cross sections for $^{40}$Ca+$^{90,96}$Zr have been reproduced remarkably well without introducing any new parameters. The fusion cross sections for the neutron-rich fusion reactions of $^{48}$Ca+$^{90,96}$Zr around the Coulomb barrier are predicted to be enhanced compared with a non-neutron-rich fusion reaction. In order to clarify the mechanism of the enhancement of the fusion cross sections for neutron-rich nuclear fusions, we pay a great attention to study the dynamic lowering of the Coulomb barrier during a neck formation. The isospin effect on the barrier lowering is investigated. It is interesting that the effect of the projectile and target nuclear structure on fusion dynamics can be revealed to a certain extent in our approach. The time evolution of the N/Z ratio at the neck region has been firstly illustrated. A large enhancement of the N/Z ratio at neck region for neutron-rich nuclear fusion reactions is found.

Ning Wang; Xizhen Wu; Zhuxia Li

2003-01-09T23:59:59.000Z

350

85R.A. Calvo and S.K. D'Mello (eds.), New Perspectives on Affect and Learning Technologies, Explorations in the Learning Sciences, Instructional Systems and Performance Technologies 3,  

E-Print Network [OSTI]

85R.A. Calvo and S.K. D'Mello (eds.), New Perspectives on Affect and Learning Technologies to which he or she is motivated to continue with the learning process (Kort, Reilly, & Picard, 2001; Picard work (Arroyo, Woolf, Royer, & Tai, 2009; Chaffar & Frasson, 2004; D'Mello et al., 2008; Forbes- Riley

Young, R. Michael

351

Citation: Myers, R.A. and C.A. Ottensmeyer.(2005, in press). Extinction Risk in Marine Species. in Norse, E.A. and L.B. Crowder, eds. Marine Conservation Biology: The Science of Maintaining the Sea's Biodiversity. Island  

E-Print Network [OSTI]

Citation: Myers, R.A. and C.A. Ottensmeyer.(2005, in press). Extinction Risk in Marine Species's Biodiversity. Island Press, Washington DC (USA) Chapter 5 Extinction Risk in Marine Species Ransom A. Myers C resources seemed inexhaustible, its capacity boundless. Marine species have even been considered "extinction

Myers, Ransom A.

352

Tsovaltzi, D., Weinberger, A., Scheuer, O., Dragon, T. & McLaren, B.M., (2012). Argument diagrams in Facebook: Facilitating the formation of scientifically sound opinions. In: A. Ra-  

E-Print Network [OSTI]

in Facebook: Facilitating the formation of scientifically sound opinions. In: A. Ra- venscroft, S. Lindstaedt in Facebook: Facilitating the Formation of Scientifically Sound Opinions Dimitra Tsovaltzi, Armin Weinberger Dimitra.tsovalzi@mx.uni-saarland.de Students use Facebook to organize their classroom experiences [1

McLaren, Bruce Martin

2012-01-01T23:59:59.000Z

353

Observation of the chiral magnetic effect in ZrTe5  

E-Print Network [OSTI]

The chiral magnetic effect is the generation of electric current induced by chirality imbalance in the presence of magnetic field. It is a macroscopic manifestation of the quantum anomaly in relativistic field theory of chiral fermions (massless spin $1/2$ particles with a definite projection of spin on momentum) -- a dramatic phenomenon arising from a collective motion of particles and antiparticles in the Dirac sea. The recent discovery of Dirac semimetals with chiral quasi-particles opens a fascinating possibility to study this phenomenon in condensed matter experiments. Here we report on the first observation of chiral magnetic effect through the measurement of magneto-transport in zirconium pentatelluride, ZrTe_5. Our angle-resolved photoemission spectroscopy experiments show that this material's electronic structure is consistent with a 3D Dirac semimetal. We observe a large negative magnetoresistance when magnetic field is parallel with the current. The measured quadratic field dependence of the magnetoconductance is a clear indication of the chiral magnetic effect. The observed phenomenon stems from the effective transmutation of Dirac semimetal into a Weyl semimetal induced by the parallel electric and magnetic fields that represent a topologically nontrivial gauge field background.

Qiang Li; Dmitri E. Kharzeev; Cheng Zhang; Yuan Huang; I. Pletikosic; A. V. Fedorov; R. D. Zhong; J. A. Schneeloch; G. D. Gu; T. Valla

2014-12-19T23:59:59.000Z

354

Memory functions of nanocrystalline cadmium selenide embedded ZrHfO high-k dielectric stack  

SciTech Connect (OSTI)

Metal-oxide-semiconductor capacitors made of the nanocrystalline cadmium selenide nc-CdSe embedded Zr-doped HfO{sub 2} high-k stack on the p-type silicon wafer have been fabricated and studied for their charge trapping, detrapping, and retention characteristics. Both holes and electrons can be trapped to the nanocrystal-embedded dielectric stack depending on the polarity of the applied gate voltage. With the same magnitude of applied gate voltage, the sample can trap more holes than electrons. A small amount of holes are loosely trapped at the nc-CdSe/high-k interface and the remaining holes are strongly trapped to the bulk nanocrystalline CdSe site. Charges trapped to the nanocrystals caused the Coulomb blockade effect in the leakage current vs. voltage curve, which is not observed in the control sample. The addition of the nanocrystals to the dielectric film changed the defect density and the physical thickness, which are reflected on the leakage current and the breakdown voltage. More than half of the originally trapped holes can be retained in the embedded nanocrystals for more than 10 yr. The nanocrystalline CdSe embedded high-k stack is a useful gate dielectric for this nonvolatile memory device.

Lin, Chi-Chou; Kuo, Yue [Thin Film Nano and Microelectronics Research Laboratory, Artie McFerrin Department of Chemical Engineering, Texas A and M University, College Station, Texas 77843-3122 (United States)

2014-02-28T23:59:59.000Z

355

Characterization of ternary compounds in the BaO:Fe{sub 2}O{sub 3}:TiO{sub 2} system: Ba{sub 6}Fe{sub 45}Ti{sub 17}O{sub 106} and BaFe{sub 11}Ti{sub 3}O{sub 23}  

SciTech Connect (OSTI)

Single crystals of Ba{sub 6}Fe{sub 45}Ti{sub 17}O{sub 106} and BaFe{sub 11}Ti{sub 3}O{sub 23} were obtained as major and minor coproducts, respectively, by slow-cooling an off-stoichiometric BaO:Fe{sub 2}O{sub 3}:TiO{sub 2} melt. The former compound exhibits variable stoichiometry, Ba{sub 6}Fe{sub 48{minus}x}Ti{sub 14+x}O{sub 106}, with the Fe:Ti ratio dependent upon the partial pressure of oxygen. The value of x corresponds to the equivalents of reduction that occur to maintain electroneutrality as the Ti-content increases. When prepared in air, this phase occurs at x = 3 with the stoichiometry Ba{sub 6}Fe{sub 45}Ti{sub 17}O{sub 106}, while in 100% oxygen the x-value approaches zero with the resulting stoichiometry Ba{sub 6}Fe{sub 48}Ti{sub 14}O{sub 106} (all Fe{sup 3+} and Ti{sup 4+}). The structures of Ba{sub 6}Fe{sub 45}Ti{sub 17}O{sub 106} and BaFe{sub 11}Ti{sub 3}O{sub 23} were solved using single-crystal X-ray diffraction methods. Ba{sub 6}Fe{sub 45}Ti{sub 17}O{sub 106} was prepared in polycrystalline form, and further structural details, including accurate Fe/Ti occupancy factors, were determined by a combined refinement using neutron and synchrotron powder diffraction data. (Ba{sub 6}Fe{sub 45}Ti{sub 17}O{sub 106}: Space group C2/m (No 12); a = 19.390(1) {angstrom}, b = 20.260(1) {angstrom}, c = 10.076(1) {angstrom}, {beta} = 105.27(1){degree}; V = 3818.5(3) {angstrom}{sup 3}; Z = 2; {rho}{sub calc} = 5.08 g/cm{sup 3}. Ba{sub 6}Fe{sub 11}Ti{sub 3}O{sub 23}: Space group C2/c (No 15); a = 19.56(1) {angstrom}, b = 8.6614(7) {angstrom}, c = 10.120(1) {angstrom}, {beta} = 105.62(1){degree}; V = 1651.1(3) {angstrom}{sup 3}; Z = 4; {rho}{sub calc} = 5.08 g/cm{sup 3}.) The magnetic behavior of Ba{sub 6}Fe{sub 45}Ti{sub 17}O{sub 106} above room temperature up to 1073 K was found to obey the Curie-Weiss law, which indicated a small effective magnetic moment (34 {mu}{sub B} per mole Ba{sub 6}Fe{sub 45}Ti{sub 17}O{sub 106}) and a large negative temperature intercept ({minus}806 K). Electrical resistivity measurements between room temperature and 120 K revealed nonmetallic behavior with an activation energy on the order of 0.17 eV. At 347 MHz under ambient conditions, Ba{sub 6}Fe{sub 45}Ti{sub 17}O{sub 106} exhibited a relative permittivity of 24 and a dielectric loss tangent of 0.10.

Vanderah, T.A.; Wong-Ng, W.; Toby, B.H.; Shull, R.D.; Roth, R.S. [National Inst. of Standards and Technology, Gaithersburg, MD (United States). Materials Science and Engineering Lab.] [National Inst. of Standards and Technology, Gaithersburg, MD (United States). Materials Science and Engineering Lab.; Browning, V.M. [Naval Research Lab., Washington, DC (United States)] [Naval Research Lab., Washington, DC (United States); Geyer, R.G. [National Inst. of Standards and Technology, Boulder, CO (United States)] [National Inst. of Standards and Technology, Boulder, CO (United States)

1999-03-01T23:59:59.000Z

356

TOPIC TIME LOCATION CATEGORY TITLE AUTHORS INSTITUTION Advanced Energy Systems 10:15 to 10:35 AM BA1180 CSME  

E-Print Network [OSTI]

microorganisms P. Graham, D.Sinton University of Toronto Advanced Energy Systems 2:35 to 2:55 PM BA1180 CSME

357

Synthesis, crystal structure, and properties of the rhombohedral modification of the thiospinel CuZr{sub 1.86(1)}S{sub 4}  

SciTech Connect (OSTI)

The rhombohedral modification of the thiospinel, CuZr{sub 1.86(1)}S{sub 4}, has been synthesized by the reaction of the constituent elements in an alkali metal halide flux and structurally characterized by single crystal X-ray diffraction techniques. The title compound crystallizes in the rhombohedral space group D{sub 3d}{sup 5}-R3-barm (no. 166, a=7.3552(2) A, c=35.832(2) A, V=1678.76(13) A{sup 3}, Z=12, and R/wR=0.0239/0.0624). The structure is composed of close packed S layers, with a stacking order of ...ABCBCABABCACAB....along the c axis. The Zr and Cu atoms occupy the octahedral and tetrahedral holes between S layers, respectively. Three different kinds of S-M-S layers exist in the structure: layer I has fully occupied Zr and Cu sites, layer II has fully occupied Zr sites but no Cu, and layer III has partially occupied Zr and fully occupied Cu sites. Transport and optical properties indicate that the title compound is a small band gap (1.26 eV) n-type semiconductor. - Graphical abstract: The projected view of the rhombohedral modification, CuZr{sub 1.86(1)}S{sub 4}, down the [100] direction. Large letters denote the packing sequence of the S atoms (yellow circles) along the c axis. Zr (black circles) and Cu (red circles) atoms occupy the octahedral and tetrahedral holes, respectively, between close packed S layers.

Dong, Yongkwan [Baker Laboratory, Department of Chemistry, Cornell University, Ithaca, NY 14853-1301 (United States); McGuire, Michael A. [Department of Physics, Cornell University, Ithaca, NY 14853-1301 (United States); Yun, Hoseop, E-mail: hsyun@ajou.ac.k [Division of Energy Research System and Department of Chemistry, Ajou University, Suwon 442-749 (Korea, Republic of); DiSalvo, Francis J., E-mail: fjd3@cornell.ed [Baker Laboratory, Department of Chemistry, Cornell University, Ithaca, NY 14853-1301 (United States)

2010-03-15T23:59:59.000Z

358

Neutron scattering investigation of the magnetic order in single crystalline BaFe2As2  

SciTech Connect (OSTI)

The magnetic structure of BaFe{sub 2}As{sub 2} was determined from polycrystalline neutron diffraction measurements soon after the ThCr{sub 2}Si{sub 2}-type FeAs-based superconductors were discovered. Both the moment direction and the in-plane antiferromagnetic wavevector are along the longer a-axis of the orthorhombic unit cell. There is only one combined magnetostructural transition at {approx}140 K. However, a later single-crystal neutron diffraction work reported contradicting results. Here, we show neutron diffraction results from a single-crystal sample, grown by a self-flux method, that support the original polycrystalline work.

Bao, Wei [Los Alamos National Laboratory; Qiu, Y [NIST; Kofu, M [UNIV OF VA; Lee, S - H [UNIV OF VA; Chang, S [NIST; Wu, T [HEFEI NAT. LAB.; Wu, G [HEFEI NAT. LAB; Chen, X H [HEFEI NAT. LAB

2008-01-01T23:59:59.000Z

359

BaBar Results on E+ E- ---> P Anti-P By Means of ISR  

SciTech Connect (OSTI)

BaBar has measured with unprecedented accuracy the e{sup +}e{sup -} {yields} p{bar p} cross section from the threshold up to Q{sub p{bar p}}{sup 2} {approx} 20 GeV{sup 2}/c{sup 4}, finding out an unexpected cross section, with plateaux and negative steps. Evidence for a ratio |G{sub E}/G{sub M}| > 1 has also been found as well as a sudden variation in |G{sub M}| just above the threshold.

Ferroli, Rinaldo Baldini; /Enrico Fermi Ctr., Rome /Frascati

2006-02-21T23:59:59.000Z

360

Search for LFV in Tau- to L- L+ L- Decays at BaBar  

SciTech Connect (OSTI)

We report the results of search for the neutrinoless lepton-flavor violating decay of the tau lepton into three charged leptons, performed using 376 fb{sup -1} of data collected at an e{sup +}e{sup -} center-of-mass energy around 10.58 GeV with the BaBar detector at the PEP-II. In all six decay modes considered, the number of events found in data are compatible with the background expectations. Upper limits on the branching fractions are set in the range (4-8) x 10{sup -8} at 90% confidence level.

Giorgi, Marcello A.; /Pisa U. /INFN, Pisa

2011-11-30T23:59:59.000Z

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361

Localization of vacancies and mobility of lithium ions in Li{sub 2}ZrO{sub 3} as obtained by {sup 6,7}Li NMR  

SciTech Connect (OSTI)

The {sup 6,7}Li NMR spectra and the {sup 7}Li spin–lattice relaxation rate were measured on polycrystalline samples of Li{sub 2}ZrO{sub 3}, synthesized at 1050 K and 1300 K. The {sup 7}Li NMR lines were attributed to corresponding structural positions of lithium Li1 and Li2 by comparing the EFG components with those obtained in the first-principles calculations of the charge density in Li{sub 2}ZrO{sub 3}. For both samples the line width of the central {sup 7}Li transition and the spin–lattice relaxation time decrease abruptly at the temperature increasing above ?500 K, whereas the EFG parameters are averaged (??{sub Q}?=42 (5) kHz) owing to thermally activated diffusion of lithium ions. - Graphical abstract: Path of lithium ion hopping in lithium zirconate Li{sub 2}ZrO{sub 3}. - Highlights: • Polycrystalline samples Li{sub 2}ZrO{sub 3} with monoclinic crystal structure synthesized at different temperatures were investigated by {sup 6,7}Li NMR spectroscopy. • Two {sup 6,7}Li NMR lines were attributed to the specific structural positions Li1 and Li2. • The distribution of vacancies was clarified for both lithium sites. • The activation energy and pathways of lithium diffusion in Li{sub 2}ZrO{sub 3} were defined.

Baklanova, Ya. V., E-mail: baklanovay@ihim.uran.ru [Institute of Solid State Chemistry, Ural Branch of the Russian Academy of Sciences, 91 Pervomaiskaya str., 620990 Ekaterinburg (Russian Federation); Arapova, I. Yu.; Buzlukov, A.L.; Gerashenko, A.P.; Verkhovskii, S.V.; Mikhalev, K.N. [Institute of Metal Physics, Ural Branch of the Russian Academy of Sciences, 18 Kovalevskaya str., 620990 Ekaterinburg (Russian Federation); Denisova, T.A.; Shein, I.R.; Maksimova, L.G. [Institute of Solid State Chemistry, Ural Branch of the Russian Academy of Sciences, 91 Pervomaiskaya str., 620990 Ekaterinburg (Russian Federation)

2013-12-15T23:59:59.000Z

362

Interfacial analysis of the ex-situ reinforced phase of a laser spot welded Zr-based bulk metallic glass composite  

SciTech Connect (OSTI)

To study the interfacial reaction of the ex-situ reinforced phase (Ta) of a Zr-based ((Zr{sub 48}Cu{sub 36}Al{sub 8}Ag{sub 8})Si{sub 0.75} + Ta{sub 5}) bulk metallic glass composite after laser spot welding, the interfacial regions of the reinforced phases located at specific zones in the welds including the parent material, weld fusion zone and heat affected zone were investigated. Specimen preparation from the specific zones for transmission electron microscopy analysis was performed using the focused ion beam technique. The test results showed that the reinforced phases in the parent material, weld fusion zone and heat affected zone were all covered by an interfacial layer. From microstructure analysis, and referring to the phase diagram, it was clear that the thin layers are an intermetallic compound ZrCu phase. However, due to their different formation processes, those layers show the different morphologies or thicknesses. - Highlights: • An ex-situ Zr-based BMG composite was laser spot welded. • The interfacial regions of the RPs located at PM, WFZ and HAZ were investigated. • The RPs in the PM, WFZ and HAZ were all covered by a ZrCu interfacial layer. • Due to different formation processes, those layers show the different morphology.

Wang, Huei-Sen, E-mail: huei@isu.edu.tw [Department of Materials Science and Engineering, I-Shou University, Kaohsiung, 84001, Taiwan (China); Department of Chemical and Materials Engineering, National University of Kaohsiung, 81148, Kaohsiung, Taiwan (China); Chen, Hou-Guang [Department of Materials Science and Engineering, I-Shou University, Kaohsiung, 84001, Taiwan (China); Jang, Jason Shian-Ching [Institute of Materials Science and Engineering and Department of Mechanical Engineering, National Central University, Chung-Li 32001, Taiwan (China); Lin, Dong-Yih [Department of Chemical and Materials Engineering, National University of Kaohsiung, 81148, Kaohsiung, Taiwan (China); Gu, Jhen-Wang [Department of Materials Science and Engineering, I-Shou University, Kaohsiung, 84001, Taiwan (China)

2013-12-15T23:59:59.000Z

363

Synthesis, Crystal Structure, and Properties of the Rhomboheral Modification of the Thiospinel CuZr1.86(1)S4  

SciTech Connect (OSTI)

The rhombohedral modification of the thiospinel, CuZr{sub 1.86(1)}S{sub 4}, has been synthesized by the reaction of the constituent elements in an alkali metal halide flux and structurally characterized by single crystal X-ray diffraction techniques. The title compound crystallizes in the rhombohedral space group D{sub 3d}{sup 5}-R{bar 3}m (166, a=7.3552(2) {angstrom}, c=35.832(2) {angstrom}, V=1678.76(13) {angstrom}{sup 3}, Z=12, and R/wR=0.0239/0.0624). The structure is composed of close packed S layers, with a stacking order of ABCBCABABCACAB along the c axis. The Zr and Cu atoms occupy the octahedral and tetrahedral holes between S layers, respectively. Three different kinds of S-M-S layers exist in the structure: layer I has fully occupied Zr and Cu sites, layer II has fully occupied Zr sites but no Cu, and layer III has partially occupied Zr and fully occupied Cu sites. Transport and optical properties indicate that the title compound is a small band gap (1.26 eV) n-type semiconductor.

Dong, Yongkwan [Cornell University; McGuire, Michael A [ORNL; Hoseop, Yun [Ajou University, Suwon, South Korea; DiSalvo, Francis J. [Cornell University

2009-01-01T23:59:59.000Z

364

High temperature crystal structures and superionic properties of SrCl{sub 2}, SrBr{sub 2}, BaCl{sub 2} and BaBr{sub 2}  

SciTech Connect (OSTI)

The structural properties of the binary alkaline-earth halides SrCl{sub 2}, SrBr{sub 2}, BaCl{sub 2} and BaBr{sub 2} have been investigated from ambient temperature up to close to their melting points, using the neutron powder diffraction technique. Fluorite-structured SrCl{sub 2} undergoes a gradual transition to a superionic phase at 900-1100 K, characterised by an increasing concentration of anion Frenkel defects. At a temperature of 920(3) K, the tetragonal phase of SrBr{sub 2} undergoes a first-order transition to a cubic fluorite phase. This high temperature phase shows the presence of extensive disorder within the anion sublattice, which differs from that found in superionic SrCl{sub 2}. BaCl{sub 2} and BaBr{sub 2} both adopt the cotunnite crystal structure under ambient conditions. BaCl{sub 2} undergoes a first-order structural transition at 917(5) K to a disordered fluorite-structured phase. The relationship between the (disordered) crystal structures and the ionic conductivity behaviour is discussed and the influence of the size of the mobile anion on the superionic behaviour is explored. - Graphical abstract: Anomalous behaviour of the lattice expansion of SrCl{sub 2} at temperatures of {approx}1000 K is associated with the gradual transition to a superionic phase, whilst SrBr{sub 2} undergoes a first-order structural transition ({beta}{yields}{alpha}) to a fluorite-structured superionic phase at 920(3) K. Highlights: > Anomalous behaviour of the lattice expansion of SrCl{sub 2} occurs at temperatures {approx}1000 K. > Crystal structure of {beta}-SrBr{sub 2} is described in detail. > On heating, SrBr{sub 2} and BaCl{sub 2} transform to a fluorite-structured superionic phase. > Temperature dependence of the BaCl{sub 2} and BaBr{sub 2} structures is presented. > Nature of the superionic phases within the alkaline-earth halides is discussed.

Hull, Stephen, E-mail: stephen.hull@stfc.ac.uk [The ISIS Facility, STFC Rutherford Appleton Laboratory, Chilton, Didcot, Oxfordshire OX11 0QX (United Kingdom); Norberg, Stefan T. [The ISIS Facility, STFC Rutherford Appleton Laboratory, Chilton, Didcot, Oxfordshire OX11 0QX (United Kingdom); Department of Chemical and Biological Engineering, Chalmers University of Technology, SE-412 96 Gothenburg (Sweden); Ahmed, Istaq; Eriksson, Sten G. [Department of Chemical and Biological Engineering, Chalmers University of Technology, SE-412 96 Gothenburg (Sweden); Mohn, Chris E. [Department of Chemistry and Centre for Materials Science and Nanotechnology, University of Oslo, P.O. Box 1033 Blindern, N-0315 Oslo (Norway)

2011-11-15T23:59:59.000Z

365

Effect of high strain rates on peak stress in a Zr-based bulk metallic glass  

SciTech Connect (OSTI)

The mechanical behavior of Zr{sub 41.25}Ti{sub 13.75}Cu{sub 12.5}Ni{sub 10}Be{sub 22.5} (LM-1) has been extensively characterized under quasistatic loading conditions; however, its mechanical behavior under dynamic loading conditions is currently not well understood. A Split-Hopkinson pressure bar (SHPB) and a single-stage gas gun are employed to characterize the mechanical behavior of LM-1 in the strain-rate regime of 10{sup 2}-10{sup 5}/s. The SHPB experiments are conducted with a tapered insert design to mitigate the effects of stress concentrations and preferential failure at the specimen-insert interface. The higher strain-rate plate-impact compression-and-shear experiments are conducted by impacting a thick tungsten carbide (WC) flyer plate with a sandwich sample comprising a thin bulk metallic glass specimen between two thicker WC target plates. Specimens employed in the SHPB experiments failed in the gage-section at a peak stress of approximately 1.8 GPa. Specimens in the high strain-rate plate-impact experiments exhibited a flow stress in shear of approximately 0.9 GPa, regardless of the shear strain-rate. The flow stress under the plate-impact conditions was converted to an equivalent flow stress under uniaxial compression by assuming a von Mises-like material behavior and accounting for the plane strain conditions. The results of these experiments, when compared to the previous work conducted at quasistatic loading rates, indicate that the peak stress of LM-1 is essentially strain rate independent over the strain-rate range up to 10{sup 5}/s.

Sunny, George; Yuan Fuping; Prakash, Vikas [Department of Mechanical and Aerospace Engineering, Case Western Reserve University, Cleveland, Ohio 44106-7222 (United States); Lewandowski, John [Department of Materials Science and Engineering, Case Western Reserve University, Cleveland, Ohio 44106-7222 (United States)

2008-11-01T23:59:59.000Z

366

Avoided Quantum Criticality and Magnetoelastic Coupling in BaFe2-xNixAs2  

DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

We study the structural and magnetic orders in electron-doped BaFe2?xNixAs2 by high-resolution synchrotron x-ray and neutron scatterings. Upon Ni doping x, the nearly simultaneous tetragonal-to-orthorhombic structural (Ts) and antiferromagnetic (TN) phase transitions in BaFe2As2 are gradually suppressed and separated, resulting in Ts>TN with increasing x, as was previously observed. However, the temperature separation between Ts and TN decreases with increasing x for x?0.065, tending toward a quantum bicritical point near optimal superconductivity at x?0.1. The zero-temperature transition is preempted by the formation of a secondary incommensurate magnetic phase in the region 0.088?x?0.104, resulting in a finite value of TN?Tc+10??K above the superconducting dome around x?0.1. Our results imply an avoided quantum critical point, which is expected to strongly influence the properties of both the normal and superconducting states.

Lu, Xingye; Gretarsson, H.; Zhang, Rui; Liu, Xuerong; Luo, Huiqian; Tian, Wei; Laver, Mark; Yamani, Z.; Kim, Young-June; Nevidomskyy, A. H.; Si, Qimiao; Dai, Pengcheng

2013-06-01T23:59:59.000Z

367

Influence of deposition pressure and pulsed dc sputtering on pumping properties of Ti-Zr-V nonevaporable getter films  

SciTech Connect (OSTI)

The performance of a UHV vessel can be improved with a new CERN technology nonevaporable getter (NEG) coating, which is already widely used for accelerator vacuum chambers. Better understanding of the processes involved in NEG film deposition, activation, and poisoning should allow optimization and engineering of the film properties, which are necessary for a particular application. Ti-Zr-V NEG films were created by magnetron sputtering from a single Ti-Zr-V target, and the NEG performance and morphology dependence on deposition pressure, sputtering conditions, and substrate surface roughness have been investigated. It was found that the average grain size of the Ti-Zr-V film was 5-6 nm and was broadly independent of the substrate material and deposition conditions. However, film topography and density were shown to depend very much on the substrate surface roughness and deposition conditions. Rough substrates, high working pressures, and the absence of ion bombardment produced open columnar structures, whereas smooth substrates, ion assistance, and low pressures produced much denser layers. X-ray photoelectron spectroscopy studies have shown that full regeneration occurred at 300 degree sign C but film activation started at temperatures of as low as 160 degree sign C. The CO sticking probability reaches its maximum after activation at 250 degree sign C and is found to be up to 0.3 with a pumping capacity in the range of 0.8-1.2 ML. The samples activated at 160 degree sign C have a reduced pumping speed and capacity by an order of magnitude.

Malyshev, O. B.; Valizadeh, R.; Colligon, J. S.; Hannah, A.; Middleman, K. J.; Patel, S.; Vishnyakov, V. M. [ASTeC Vacuum Science Group, STFC Daresbury Laboratory, Warrington WA4 4AD (United Kingdom); Department of Chemistry, Manchester Metropolitan University Manchester M1 5GD (United Kingdom); ASTeC Vacuum Science Group, STFC Daresbury Laboratory, Warrington WA4 4AD (United Kingdom); Department of Chemistry, Manchester Metropolitan University, Manchester, M1 5GD (United Kingdom)

2009-05-15T23:59:59.000Z

368

Controlling internal barrier in low loss BaTiO3 supercapacitors U-C. Chung, C. Elissalde, S. Mornet and M. Maglione  

E-Print Network [OSTI]

1 Controlling internal barrier in low loss BaTiO3 supercapacitors U-C. Chung, C. Elissalde, S Supercapacitor behavior has been reported in a number of oxides including reduced BaTiO3 ferroelectric ceramics to process bulk composites having supercapacitor features with low dielectric losses and temperature

Boyer, Edmond

369

Evidence for a phosphorylation-independent role for Ser 32 and 36 in proteasome inhibitor-resistant (PIR) InBa degradation in B cells  

E-Print Network [OSTI]

-resistant (PIR) InBa degradation in B cells Shelby O'Connor, Stephanie Markovina, Shigeki MiyamotoT Program is maintained through proteasome inhibitor-resistant (PIR) InBa degradation in a manner that requires Ser 32 whether dual phosphorylation of Ser 32 and 36 was required for PIR degradation. Through mutagenesis

Miyamoto, Shigeki

370

Studies on catalytic and structural properties of BaRuO3 type perovskite1 material for diesel soot oxidation2  

E-Print Network [OSTI]

1 Studies on catalytic and structural properties of BaRuO3 type perovskite1 material for diesel by co-precipitation24 method and its catalytic activity has been tested for diesel soot oxidation processes and vehicle exhaust.33 Key words: BaRuO3, perovskite, diesel soot oxidation, vehicular exhaust

Paris-Sud XI, Université de

371

Guided wave absorption and uorescence in epitaxial Er:BaTiO3 on MgO D.M. Gilla,*, G.M. Fordb  

E-Print Network [OSTI]

. Keywords: Er:BaTiO3; Fluorescence; Luminescence 1. Introduction The development of low-cost composite waveguides fabricated in erbium-doped thin-®lm epitaxial BaTiO3. Luminescence transient measurements indicate strategies toward the realization of this type of opto-electronic circuit. Proposed designs of hybrid opto

Ho, Seng-Tiong

372

Page 1 | B.A. in Special Education (General Curriculum) and Elementary Education (K-6) Dual Major | Academic Plan of Study  

E-Print Network [OSTI]

| Academic Plan of Study Updated May 2014 B.A. in Special Education (General Curriculum) and ElementaryPage 1 | B.A. in Special Education (General Curriculum) and Elementary Education (K-6) Dual Major Education (K-6) Dual Program Academic Plan of Study College of Education Department of Special Education

Raja, Anita

373

Mechanism of Cation Exchange Process for Epitaxy of Superconducting HgBa2CaCu2O6 Films and Passive Microwave Devices  

E-Print Network [OSTI]

cations into, the lattice of epitaxial Tl2Ba2CaCu2O8 (Tl-2212) or TlBa2CaCu2O7 (Tl-1212) precursor films. Aiming at the remained issues in understanding the mechanism of the cation exchange (CE) process, this thesis work has studied the reversibility of CE...

Zhao, Hua

2007-12-17T23:59:59.000Z

374

Two-Dimensional Polaronic Behavior in the Binary Oxides m-HfO2 and m-ZrO2  

SciTech Connect (OSTI)

We demonstrate that the three-dimensional (3D) binary monoclinic oxides HfO{sub 2} and ZrO{sub 2} exhibit quasi-2D polaron localization and conductivity, which results from a small difference in the coordination of two oxygen sublattices in these materials. The transition between a 2D large polaron into a zero-dimensional small polaron state requires overcoming a small energetic barrier. These results demonstrate how a small asymmetry in the lattice structure can determine the qualitative character of polaron localization and significantly broaden the realm of quasi-2D polaron systems.

McKenna, K. P.; Wolf, M. J.; Shluger, A. L.; Lany, S.; Zunger, A.

2012-03-16T23:59:59.000Z

375

Electron-Transport Properties of Amorphous (Zr0.64ni0.36)1-Xalx Alloys  

E-Print Network [OSTI]

PHYSICAL REVIEW B VOLUME 39, NUMBER 17 15 JUNE 1989-I Electron transport properties of amorphous (Zro 64Nio 36), ?Al?alloys A. K. Bhatnagar, ' R. Pan, and D. G. Naugle Department ofPhysics, Texas Ad'cM Uniuersity, College Station, Texas 77843...-4242 (Received 28 November 1988; revised manuscript received 16 March 1989) Measurements of the electrical resistivity p(T), thermopower S(T), and Hall coe%cient RH for a series of rapidly quenched Zr-Ni-Al alloys are reported for concentrations from x =0 to 0...

BHATNAGAR, AK; PAN, R.; Naugle, Donald G.

1989-01-01T23:59:59.000Z

376

The structural and mechanical properties of a Cu??Zr??(at. %) alloy processed by High-Velocity-Injection (HVI)  

E-Print Network [OSTI]

/vacuum coupled pressure gradient. The molten jet rapidly solidifies, as it is in good thermal contact wi th the cir- cular walls of the copper channel. This process (melting and injection) is carried out in inert protective atmospheres (helium). The samples... produced are in the form of cylindrical rods with large length to diameter ratios (40:1). The samples exhibit a good sur- face finish and are of high density. The structural and mechanical characterization of the Cu6 Zr 0(at. %%u) samples produced...

Hays, Charles C.

1986-01-01T23:59:59.000Z

377

Negative Thermal Expansion in ZrW{sub 2}O{sub 8}: Mechanisms, Rigid Unit Modes, and Neutron Total Scattering  

SciTech Connect (OSTI)

The local structure of the low-temperature ordered phase of the negative thermal expansion (NTE) material ZrW{sub 2}O{sub 8} has been investigated by reverse Monte Carlo (RMC) modeling of neutron total scattering data. We obtain, for the first time, quantitative measurements of the extent to which the WO{sub 4} and ZrO{sub 6} polyhedra move as rigid units, and we show that these values are consistent with the predictions of rigid unit mode theory. We suggest that rigid unit modes are associated with the NTE. Our results do not support a recent interpretation of x-ray-absorption fine structure spectroscopy data in terms of a larger rigid structural component involving the Zr-O-W linkage.

Tucker, Matthew G. [Department of Earth Sciences, University of Cambridge, Downing Street, Cambridge CB2 3EQ (United Kingdom); ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot, Oxon OX11 0QX (United Kingdom); Goodwin, Andrew L.; Dove, Martin T. [Department of Earth Sciences, University of Cambridge, Downing Street, Cambridge CB2 3EQ (United Kingdom); Keen, David A. [Physics Department, Oxford University, Clarendon Laboratory, Parks Road, Oxford OX1 3PU (United Kingdom); ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot, Oxon OX11 0QX (United Kingdom); Wells, Stephen A. [Biological Physics, Bateman Physical Sciences Building, Arizona State University, Tempe, Arizona 85287-1504 (United States); Evans, John S.O. [Department of Chemistry, University Science Laboratories, South Road, Durham DH1 3LE (United Kingdom)

2005-12-16T23:59:59.000Z

378

11196. Proposed by Mohammad Hossein Mehrabi, Iran University of Science and Technology, Tehran, Iran. Let A and B be real n n matrices. Show that if AB -BA is invertible and A2  

E-Print Network [OSTI]

11196. Proposed by Mohammad Hossein Mehrabi, Iran University of Science and Technology, Tehran, Iran. Let A and B be real n Ă? n matrices. Show that if AB - BA is invertible and A2 + B2 = 3(AB - BA

Heckman, Christopher Carl

379

Characterization of self-propagating formation reactions in Ni/Zr multilayered foils using reaction heats, velocities, and temperature-time profiles  

SciTech Connect (OSTI)

We report on intermetallic formation reactions in vapor-deposited multilayered foils of Ni/Zr with 70 nm bilayers and overall atomic ratios of Ni:Zr, 2 Ni:Zr, and 7 Ni:2 Zr. The sequence of alloy phase formation and the stored energy is evaluated at slow heating rates (~1 K/s) using differential scanning calorimetry (DSC) traces to 725şC. All three chemistries initially form a Ni-Zr amorphous phase which crystallizes first to the intermetallic NiZr. The heat of reaction to the final phase is 34-36 kJ/mol atom for all chemistries. Intermetallic formation reactions are also studied at rapid heating rates (greater than 105 K/s) in high temperature, self-propagating reactions which can be ignited in these foils by an electric spark. We find that reaction velocities and maximum reaction temperatures (Tmax) are largely independent of foil chemistry at 0.6 ± 0.1 m/s and 1220 ± 50 K, respectively, and that the measured Tmax is more than 200 K lower than predicted adiabatic temperatures (Tad). The difference between Tmax and Tad is explained by the prediction that transformation to the final intermetallic phases occurs after Tmax and results in the release of 20-30 % of the total heat of reaction and a delay in rapid cooling.

Barron, S. C.; Knepper, R.; Walker, N.; Weihs, T. P.

2011-01-11T23:59:59.000Z

380

First principle study of elastic and thermodynamic properties of ZrZn{sub 2} and HfZn{sub 2} under high pressure  

SciTech Connect (OSTI)

A comprehensive investigation of the structural, elastic, and thermodynamic properties for Laves-phases ZrZn{sub 2} and HfZn{sub 2} are conducted using density functional total energy calculations combined with the quasi-harmonic Debye model. The optimized lattice parameters of ZrZn{sub 2} and HfZn{sub 2} compare well with available experimental values. We estimated the mechanical behaviors of both compounds under compression, including mechanical stability, Young's modulus, Poisson's ratio, ductility, and anisotropy. Additionally, the thermodynamic properties as a function of pressure and temperature are analyzed and found to be in good agreement with the corresponding experimental data.

Sun, Na; Zhang, Xinyu, E-mail: jiaqianqin@gmail.com; Ning, Jinliang; Zhang, Suhong; Liang, Shunxing; Ma, Mingzhen; Liu, Riping [State Key Laboratory of Metastable Materials Science and Technology, Yanshan University, Qinhuangdao 066004 (China); Qin, Jiaqian, E-mail: jiaqianqin@gmail.com [Metallurgy and Materials Science Research Institute, Chulalongkorn University, Bangkok 10330 (Thailand)

2014-02-28T23:59:59.000Z

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


381

Usefulness of gel-casting method in the fabrication of nonstoichiometric CaZrO{sub 3}-based electrolytes for high temperature application  

SciTech Connect (OSTI)

Hydrogels obtained from lower toxicity monomers of N-(hydroxymethyl)acrylamide and N,N'-methylenebisacrylamide were applied to form nonstoichiometric CaZrO{sub 3}-based electrolytes. A coprecipitation-calcination method with ((NH{sub 4}){sub 2}C{sub 2}O{sub 4}) in concentrated NH{sub 3} aqueous solution was used to synthesise CaZrO{sub 3} involving 51 mol.% CaO (CZ-51) powder. The gas-tight CaZrO{sub 3}-based rods were prepared by the gel-casting method with 45 vol.% suspension and then sintered at 1500 deg. C-2 h. It was found that in low oxygen partial pressure, the nonstoichiometric CaZrO{sub 3} obtained by gel-casting method were pure oxide ion conductors. These samples exhibited comparable electrical conductivity values to isostatically compressed pellets starting from the same powder. The results of experiments on thermochemical stability of CZ-51 gel-cast shapes at high temperatures in air or gas mixtures involving 2-50 vol.% H{sub 2}, as well as the corrosion resistance in exhaust gases from a self-ignition engine were also presented and discussed. The thermal resistance of CaZrO{sub 3} obtained rods against molten nickel or iron was also examined. Based upon these investigations, it is evident that only in hydrogen-rich gas atmospheres can the stability of CaZrO{sub 3} shapes be limited due to the presence of CaO precipitation as a second phase. The nonstoichiometric CaZrO{sub 3} (CZ-51) gel-cast materials were also tested in solid galvanic cells, designed to study thermodynamic properties of oxide materials, important for SOFC and energy technology devices. In this way, the Gibbs energy of NiM{sub 2}O{sub 4}, M = Cr, Fe, at 650-1000 deg. C was determined. The CaZrO{sub 3} involving 51 mol.% CaO gel-cast sintered shapes seems to be promising solid electrolytes for electrochemical oxygen probes in control of metal processing and thermodynamic studies of materials important for the development of the energy industry.

Dudek, Magdalena [AGH - University of Science and Technology, Faculty of Energy and Fuels, 30-059 Cracow (Poland)

2009-09-15T23:59:59.000Z

382

Fission gas bubble nucleated cavitational swelling of the alpha-uranium phase of irradiated U-Pu-Zr fuel  

SciTech Connect (OSTI)

Cavitational swelling has been identified as a potential swelling mechanism for the alpha uranium phase of irradiated U-Pu-Zr metal fuels for the Integral Fast Reactor being developed at Argonne National Laboratory. The trends of U-Pu-Zr swelling data prior to fuel cladding contact can be interpreted in terms of unrestrained cavitational driven swelling. It is theorized that the swelling mechanisms at work in the alpha uranium phase can be modeled by single vacancy and single interstitial kinetics with intergranular gas bubbles providing the void nuclei, avoiding the use of complicated defect interaction terms required for the calculation of void nucleation. The focus of the kinetics of fission gas evolution as it relates to cavitational swelling is prior to the formation of a significant amount of interconnected porosity and is on the development of small intergranular gas bubbles which can act as void nuclei. Calculations for the evolution of intergranular fission gas bubbles show that they provide critical cavity sizes (i.e., the size above which the cavity will grow by bias-driven vacancy flux) consistent with the observed incubation dose for the onset of rapid swelling and gas release.

Rest, J.

1992-04-01T23:59:59.000Z

383

Electron-stimulated desorption from polished and vacuum fired 316LN stainless steel coated with Ti-Zr-Hf-V  

SciTech Connect (OSTI)

In this study, two identical 316LN stainless steel tubular samples, which had previously been polished and vacuum-fired and then used for the electron-stimulated desorption (ESD) experiments, were coated with Ti-Zr-Hf-V with different morphologies: columnar and dense. ESD measurement results after nonevaporable getter (NEG) activation to 150, 180, 250, and 350?°C indicated that the values for the ESD yields are significantly (2–20 times) lower than the data from our previous study with similar coatings on nonvacuum-fired samples. Based on these results, the lowest pressure and best long-term performance in particle accelerators will be achieved with a vacuum-fired vacuum chamber coated with dense Ti-Zr-Hf-V coating activated at 180?°C. This is likely due to the following facts: after NEG activation, the hydrogen concentration inside the NEG was lower than in the bulk stainless steel substrate; the NEG coating created a barrier for gas diffusion from the sample bulk to vacuum; the dense NEG coating performed better as a barrier than the columnar NEG coating.

Malyshev, Oleg B., E-mail: oleg.malyshev@stfc.ac.uk; Valizadeh, Reza; Hogan, Benjamin T.; Hannah, Adrian N. [ASTeC, STFC Daresbury Laboratory, Daresbury, Warrington, WA4 4AD Cheshire (United Kingdom)

2014-11-01T23:59:59.000Z

384

Experimental study of the low-lying structure of {sup 94}Zr with the (n,n{sup '}{gamma}) reaction  

SciTech Connect (OSTI)

The low-lying structure of {sub 40}{sup 94}Zr was studied with the (n,n{sup '}{gamma}) reaction, and a level scheme was established based on excitation function and {gamma}{gamma} coincidence measurements. Branching ratios, multipole mixing ratios, and spin assignments were determined from angular distribution measurements. Lifetimes of levels up to 3.4 MeV were measured by the Doppler-shift attenuation method, and for many transitions the reduced transition probabilities were determined. In addition to the anomalous 2{sub 2}{sup +} state, which has a larger B(E2;2{sub 2}{sup +}{yields}0{sub 1}{sup +}) value than the B(E2;2{sub 1}{sup +}{yields}0{sub 1}{sup +}), the experimental results revealed interesting and unusual properties of the low-lying states in {sup 94}Zr. In a simple interpretation, the excited states are classified in two distinct categories, i.e., those populating the 2{sub 2}{sup +} state and those decaying to the 2{sub 1}{sup +} state.

Elhami, E.; Orce, J. N.; Scheck, M.; Mukhopadhyay, S.; Choudry, S. N.; McEllistrem, M. T. [Department of Physics and Astronomy, University of Kentucky, Lexington, Kentucky 40506-0055 (United States); Yates, S. W. [Department of Physics and Astronomy, University of Kentucky, Lexington, Kentucky 40506-0055 (United States); Department of Chemistry, University of Kentucky, Lexington, Kentucky 40506-0055 (United States); Angell, C.; Boswell, M.; Karwowski, H. J. [Department of Physics and Astronomy, University of North Carolina, Chapel Hill, North Carolina 27599-3255 (United States); Triangle Universities Nuclear Laboratory (TUNL), Durham, North Carolina 27708 (United States); Fallin, B.; Howell, C. R.; Hutcheson, A.; Parpottas, Y.; Tonchev, A. P.; Tornow, W. [Triangle Universities Nuclear Laboratory (TUNL), Durham, North Carolina 27708 (United States); Department of Physics, Duke University, Durham, North Carolina 27708-0308 (United States); Kelley, J. H. [Triangle Universities Nuclear Laboratory (TUNL), Durham, North Carolina 27708 (United States); Department of Physics, North Carolina State University, Raleigh, North Carolina 27695-8202 (United States)

2008-12-15T23:59:59.000Z

385

High temperature oxidation behavior of austenitic stainless steel AISI 304 in steam of nanofluids contain nanoparticle ZrO2  

SciTech Connect (OSTI)

The objective of this study is to evaluate high temperature oxidation behavior of austenitic stainless steel SS 304 in steam of nanofluids contain nanoparticle ZrO{sub 2}. The oxidation was performed at high temperatures ranging from 600 to 800°C. The oxidation time was 60 minutes. After oxidation the surface of the samples was analyzed by different methods including, optical microscope, scanning electron microscope (SEM) and X-ray diffraction (XRD). X-ray diffraction examination show that the oxide scale formed during oxidation of stainless steel AISI 304 alloys is dominated by iron oxide, Fe{sub 2}O{sub 3}. Minor element such as Cr{sub 2}O{sub 3} is also appeared in the diffraction pattern. Characterization by optical microscope showed that cross section microstructure of stainless steel changed after oxidized with the oxide scale on the surface stainless steels. SEM and x-ray diffraction examination show that the oxide of ZrO{sub 2} appeared on the surface of stainless steel. Kinetic rate of oxidation of austenite stainless steel AISI 304 showed that increasing oxidation temperature and time will increase oxidation rate.

Prajitno, Djoko Hadi, E-mail: djokohp@batan.go.id; Syarif, Dani Gustaman, E-mail: djokohp@batan.go.id [Research Center for Nuclear Materials and Radiometry, Jl. Tamansari 71, Bandung 40132 (Indonesia)

2014-03-24T23:59:59.000Z

386

Hysteresis analysis of CoTi substituted M-type BaSr hexagonal ferrite Charanjeet Singh a,  

E-Print Network [OSTI]

Hysteresis analysis of Co­Ti substituted M-type Ba­Sr hexagonal ferrite Charanjeet Singh a, , S.5Sr0.5CoxTixFe(12 - 2x)O19 ferrite have been investigated by XRD, SEM and VSM. XRD and SEM confirm M ferrites are known for their strong uniaxial magne- tocrystalline anisotropy with ease of magnetization

Koledintseva, Marina Y.

387

Computer Science Educational Effectiveness Assessment Plan Page 1 of 23 B.S., B.A, Minor in Computer Science  

E-Print Network [OSTI]

Computer Science Educational Effectiveness Assessment Plan Page 1 of 23 B.S., B.A, Minor in Computer Science Educational Effectiveness Assessment Plan Version 1.3 Adopted by The Computer Science of Academic Affairs: #12;Computer Science Educational Effectiveness Assessment Plan Page 2 of 23 TABLE

Mock, Kenrick

388

Office of the Faculty of Engineering Syllabus for the Degree Project for the B.A. in Industrial Design  

E-Print Network [OSTI]

Office of the Faculty of Engineering Syllabus for the Degree Project for the B.A. in Industrial Design Approved by the Board of the Faculty of Engineering on 2nd March 2009 and valid from 1 st January of compulsory courses that can be accredited to the degree of Bachelor of Arts in Industrial Design. Exemption

389

Hall-Coefficient for Oriented Tl2ba2cacu2o8+delta Thin-Films  

E-Print Network [OSTI]

Measurements of the Hall coefficient and resistivity for highly oriented Tl2Ba2CaCu2O8+delta thin films are reported. The temperature dependence of cotTHETA(H), where THETA(H) is the normal-state Hall angle, for a single-phase (2:2:1:2) film sample...

WANG, PS; WILLIAMS, JC; RATHNAYAKA, KDD; HENNINGS, BD; Naugle, Donald G.; KAISER, AB.

1993-01-01T23:59:59.000Z

390

Philosophy, Politics & Law BA-MA A master degree adds problem-solving abilities in new and unfamiliar environments within  

E-Print Network [OSTI]

Philosophy, Politics & Law BA-MA A master degree adds problem-solving abilities in new and students of philosophy are well prepared, but also an area which is often intellectually interesting. "...The law is not only a career that interests many philosophers and philosophy students; it is also

Suzuki, Masatsugu

391

Roadmap: Pan-African Studies Pan-African Studies Bachelor of Arts [AS-BA-PAS-PAS  

E-Print Network [OSTI]

Roadmap: Pan-African Studies ­ Pan-African Studies ­ Bachelor of Arts [AS-BA-PAS-PAS] College: 22-Apr-13/LNHD This roadmap is a recommended semester-by-semester plan of study for this major Non-PAS Elective 3 General Elective (upper division) 9 #12;Roadmap: Pan-African Studies ­ Pan

Sheridan, Scott

392

Electron irradiation of Co, Ni, and P-doped BaFe2As2type iron-based superconductors  

E-Print Network [OSTI]

± superconductivity in the multiband iron-based superconductors [1, 2], with a sign-changing order parameter betweenElectron irradiation of Co, Ni, and P-doped BaFe2As2­type iron-based superconductors Cornelis-scale point-like disorder on superconductivity in these materials [5, 6]. In particular, interband scattering

Paris-Sud XI, Université de

393

HYDROTHERMAL PROCESSING OF BaTiO 3/POLYMER FILMS Elliott B. Slamovich and Ilhan A. Aksay  

E-Print Network [OSTI]

HYDROTHERMAL PROCESSING OF BaTiO 3/POLYMER FILMS Elliott B. Slamovich and Ilhan A. Aksay Department temperature used in hydrothermal processing. BACKGROUND Over the last decade efforts have increased to develop hydrothermal processing not only to fabricate ceramics, but also to form thin film composites containing

Aksay, Ilhan A.

394

Draft Version 9 BA 290N-3, ME 290H, INFOSYS 290P-5 and CCA UDIST-300-14  

E-Print Network [OSTI]

Objectives: The focus of the course is on innovation processes for sustainable products, from product sustainability means, how companies are approaching it, and a process for generating sustainable solutions1 Draft Version 9 BA 290N-3, ME 290H, INFOSYS 290P-5 and CCA UDIST-300-14 Design for Sustainability

Agogino, Alice M.

395

La-doped BaTiO{sub 3} heterostructures: Compensating the polarization discontinuity  

SciTech Connect (OSTI)

We demonstrate a route to manipulate the polarization and internal electric field of a complex oxide heterostructure using a layering sequence based on the LaAlO{sub 3}-SrTiO{sub 3} interface. By combining sensitive atomic-level mapping of the structure using direct x-ray phase-retrieval methods with theoretical modeling of the electrostatic charge and polarization, we have devised a novel single-domain polar heterostructure. We find that ionic rearrangement results in strain and free energy minimization, and eliminates the polarization discontinuity leading to a two-fold increase of the spontaneous polarization towards the surface of an ultra-thin single-domain BaTiO{sub 3} film.

Kumah, D. P.; Clarke, R., E-mail: royc@umich.edu [Applied Physics Program, University of Michigan, Ann Arbor, Michigan 48109 (United States); Yacoby, Y. [Racah Institute of Physics, Hebrew University, Jerusalem 91904 (Israel); Pauli, S. A.; Willmott, P. R. [Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen PSI (Switzerland)

2013-12-01T23:59:59.000Z

396

Microscopic description of spherical to {gamma}-soft shape transitions in Ba and Xe nuclei  

SciTech Connect (OSTI)

The rapid transition between spherical and {gamma}-soft shapes in Ba and Xe nuclei in the mass region A>=130 is analyzed using excitation spectra and collective wave functions obtained by diagonalization of a five-dimensional Hamiltonian for quadrupole vibrational and rotational degrees of freedom, with parameters determined by constrained self-consistent relativistic mean-field calculations for triaxial shapes. The results reproduce the characteristic evolution of excitation spectra and E2 transition probabilities, and in general, a good agreement with available data is obtained. The calculated spectra display fingerprints of a second-order shape phase transition that can approximately be described by analytic solutions corresponding to the E(5) dynamical symmetry.

Li, Z. P. [State Key Laboratory of Nuclear Physics and Technology, School of Physics, Peking University, Beijing 100871 (China); Physics Department, Faculty of Science, University of Zagreb, 10000 Zagreb (Croatia); Niksic, T.; Vretenar, D. [Physics Department, Faculty of Science, University of Zagreb, 10000 Zagreb (Croatia); Meng, J. [State Key Laboratory of Nuclear Physics and Technology, School of Physics, Peking University, Beijing 100871 (China); School of Physics and Nuclear Energy Engineering, Beihang University, Beijing 100191 (China)

2010-03-15T23:59:59.000Z

397

Investigation of novel decay B _____ ____(2S)____K at BaBar  

SciTech Connect (OSTI)

We investigate the undocumented B meson decay, B{sup +} {yields} {Psi}(2S){omega}K{sup +}. The data were collected with the BaBar detector at the SLAC PEP-II asymmetric-energy e{sup +}e{sup -} collier operating at the {gamma}(4S) resonance, a center-of-mass energy of 10.58 GeV/c{sup 2}. The {gamma}(4S) resonance primarily decays to pairs of B-mesons. The BaBar collaboration at the PEP-II ring was located at the SLAC National Accelerator Laboratory and was designed to study the collisions of positrons and electrons. The e{sup -}e{sup +} pairs collide at asymmetric energies, resulting in a center of mass which is traveling at relativistic speeds. The resulting time dilation allows the decaying particles to travel large distances through the detector before undergoing their rapid decays, a process that occurs in the in the center of mass frame over extremely small distances. As they travel through silicon vertex trackers, a drift chamber, a Cerenkov radiation detector and finally an electromagnetic calorimeter, we measure the charge, energy, momentum, and particle identification in order to reconstruct the decays that have occurred. While all well understood mesons currently fall into the qq model, the quark model has no a priori exclusion of higher configuration states such as qqqq which has led experimentalists and theorists alike to seek evidence supporting the existence of such states. Currently, there are hundreds of known decay modes of the B mesons cataloged by the Particle Data Group, but collectively they only account for approximately 60% of the B branching fraction and it is possible that many more exist.

Schalch, Jacob; /Oberlin Coll. /SLAC

2011-06-22T23:59:59.000Z

398

Precipitation method for barium metaborate (BaB{sub 2}O{sub 4}) synthesis from borax solution  

SciTech Connect (OSTI)

In this study, barium metaborate (BaB{sub 2}O{sub 4}, BMB) synthesis from the borax solution was carried out. BMB currently is used in production of ceramic glazes, luminophors, oxide cathodes as well as additives to pigments for aqueous emulsion paints and also ??BaB{sub 2}O{sub 4} single crystals are the best candidate for fabrication of solid-state UV lasers operating at a wavelength of 200 nm due to excellent nonlinear optical properties. In the present study, synthesis was carried out from the borax solution (Na{sub 2}B{sub 4}O{sub 7?}10H{sub 2}O, BDH) and barium chloride (BaCI{sub 2?}2H{sub 2}O, Ba) in the glass-batch reactor with stirring. The effect of, times (5-15 min), molar ratio [stoich.ration (1.0:2.0), 1.25:2.0, 1.5:2.0, 2.5:2:0, 3.0:2.0, 3.5:2.0,4.0:2.0, 5.0:2.0] and also crystallization time (2-6 hour) on the BMB yield (%) was investigated at 80 °C reaction temperature. It is found that, BMB precipitation synthesis with 90 % yield can be performed from 0.50 molar ration (BDH:Ba), under 80 °C, 15 minute, and 6 hours crystallization time. The structural properties of BMB powders were characterized by using XRD, FT-IR and DTA-TG instrumental analysis technique.

Ak?ener, Eymen; Figen, Aysel Kantürk; Pi?kin, Sabriye [Yildiz Technical University, Chem. Eng. Dept., Davutpasa Campus, 34210, Istanbul (Turkey)

2013-12-16T23:59:59.000Z

399

COMPARISON OF THE CORROSION BEHAVIOR OF A BULK AMORPHOUS METAL, Zr41.2Ti13.8Cu12.5Ni10Be22.5,  

E-Print Network [OSTI]

COMPARISON OF THE CORROSION BEHAVIOR OF A BULK AMORPHOUS METAL, Zr41.2Ti13.8Cu12.5Ni10Be22 exhibit excellent corrosion resistance (4­7), which has been explained in terms of their structural researchers attribute "good corrosion resistance" to the entire class of amorphous metals. It is this point

Ritchie, Robert

400

From fluorite to pyrochlore: Characterisation of local and average structure of neodymium zirconate, Nd{sub 2}Zr{sub 2}O{sub 7}  

SciTech Connect (OSTI)

The structural characterisation of Nd{sub 2}Zr{sub 2}O{sub 7} prepared via a precursor route was performed using a combination of local and average structure probes (neutron total scattering, X-ray and neutron diffraction). We present the first total scattering and reverse Monte Carlo (RMC) modelling study of Nd{sub 2}Zr{sub 2}O{sub 7}, which provides compelling evidence for the adoption of a disordered fluorite-type structure by Nd{sub 2}Zr{sub 2}O{sub 7} prepared by a low-temperature precursor route. Annealing the material at high temperatures leads to a transformation to a pyrochlore-type structure; however, Rietveld refinement using powder neutron diffraction data shows that the oxygen sublattice retains a degree of disorder. - Graphical abstract: Display Omitted - Highlights: • The first total scattering and RMC modelling study of Nd{sub 2}Zr{sub 2}O{sub 7}. • Demonstration that the synthetic route influences the crystal structure adopted. • Insight into the importance of total scattering in studies of complex superstructures, especially for nano-sized materials.

Payne, Julia L. [Department of Chemistry, Durham University, South Road, Durham DH1 3LE (United Kingdom); Tucker, Matthew G. [ISIS Facility, Rutherford Appleton Laboratory, Didcot, Oxfordshire OX11 0QX (United Kingdom); Evans, Ivana Radosavljevi?, E-mail: ivana.radosavljevic@durham.ac.uk [Department of Chemistry, Durham University, South Road, Durham DH1 3LE (United Kingdom)

2013-09-15T23:59:59.000Z

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


401

Growth and Properties of (001)-oriented Pb(Zr?.??Ti?.??)O?/LaNiO? Films on Si(001) Substrates with TiN Buffer Layers  

E-Print Network [OSTI]

Pulsed laser deposition has been used to grow Pb(Zr?.??Ti?.??)O? (PZT)/LaNiO? (LNO) heterostructures with restricted crystallographic orientations on bare Si(001) and SiO?-coated Si(001) substrates, using TiN buffer layers. ...

Zhu, Tie-Jun

402

A thermokinetic model describing the vaporization behavior of U{sub x}Zr{sub 1-x}C{sub 1-y} in hydrogen  

SciTech Connect (OSTI)

This paper describes the thermodynamics and kinetics of the corrosion of U{sub x}Zr{sub 1-x}C{sub 1-y} in hydrogen gas. It describes how corrosion rates are influenced by variables such as pressure, temperature, and gas flow rate. A model is developed which agrees with experimental steady-state corrosion rates at 1 atm between 2670 and 3100 K. It is shown that under steady-state conditions the corrosion flux is rate limited by the vapor phase transport of Zr(g) away from the solid surface to the bulk gas stream where the partial pressure of Zr(g) is determined by the congruently vaporizing surface composition. Extrapolation of the model to higher pressures indicates that Zr(g) transport should also be rate limiting at higher pressures but the corrosion rate should decrease slightly with increased hydrogen pressure due to reduced gaseous diffusion rates. The model predicts that the corrosion rate will increase as the square root of gas velocity for a given temperature and pressure. Calculations demonstrating the effects of gas velocity are in agreement with experimental studies.

Butt, D.P

1993-05-01T23:59:59.000Z

403

A thermokinetic model describing the vaporization behavior of U[sub x]Zr[sub 1-x]C[sub 1-y] in hydrogen  

SciTech Connect (OSTI)

This paper describes the thermodynamics and kinetics of the corrosion of U[sub x]Zr[sub 1-x]C[sub 1-y] in hydrogen gas. It describes how corrosion rates are influenced by variables such as pressure, temperature, and gas flow rate. A model is developed which agrees with experimental steady-state corrosion rates at 1 atm between 2670 and 3100 K. It is shown that under steady-state conditions the corrosion flux is rate limited by the vapor phase transport of Zr(g) away from the solid surface to the bulk gas stream where the partial pressure of Zr(g) is determined by the congruently vaporizing surface composition. Extrapolation of the model to higher pressures indicates that Zr(g) transport should also be rate limiting at higher pressures but the corrosion rate should decrease slightly with increased hydrogen pressure due to reduced gaseous diffusion rates. The model predicts that the corrosion rate will increase as the square root of gas velocity for a given temperature and pressure. Calculations demonstrating the effects of gas velocity are in agreement with experimental studies.

Butt, D.P.

1993-01-01T23:59:59.000Z

404

Giant dielectric response in Pb,,Zr,Ti...O3Pb2Ru2O6.5 all-ceramic percolative composite  

E-Print Network [OSTI]

Giant dielectric response in Pb,,Zr,Ti...O3­Pb2Ru2O6.5 all-ceramic percolative composite Vid Bobnar response of a composite comprising a conductive filler embedded in a dielectric matrix--the effective­9 and inorganic composites comprising metal particles dis- persed in a dielectric matrix10­14 have been developed

Bobnar, Vid

405

PVP-Assisted ZrO2 coating on LiMn2O4 spinel cathode nanoparticles prepared by MnO2 nanowire templates  

E-Print Network [OSTI]

solution. Upon annealing at 600 °C in air, an amorphous ZrO2 nanoscale coating layer was obtained [5­10]. Although Li-ion batteries are attractive power-storage devices that have high energy density metal oxide coatings have been reported, studies to improve both the rate capabilities of spinel LiMn2O4

Cho, Jaephil

406

First-principles phase diagram calculations for the HfCTiC, ZrCTiC, and HfCZrC solid O. Adjaoud,1,*,  

E-Print Network [OSTI]

Transition metal carbides, including the NaCl-structured group IV Ti, Zr, and Hf carbides, have extremely of oxidizing agents, and retain good corrosion resistance to high temperature.1,5,6 The transition-metal high melting points and are therefore referred to collectively as the "refractory carbides

Steinle-Neumann, Gerd

407

A Novel Combustion Synthesis Preparation of CuO/ZnO/ZrO2/Pd for Oxidative Hydrogen Production from Methanol  

E-Print Network [OSTI]

cells using hydrogen as fuel are efficient, quiet, and have near zero harmful emissions. Elemental fuel cells that use precious metal catalysts such as platinum require hydrogen fuel which contains lessA Novel Combustion Synthesis Preparation of CuO/ZnO/ZrO2/Pd for Oxidative Hydrogen Production from

Mukasyan, Alexander

408

The ternary silicide ZrPd{sub 3}Si{sub 3}, a stacking variant of the {alpha}-FeSi{sub 2} and Re{sub 3}B structure types  

SciTech Connect (OSTI)

The ternary zirconium palladium silicide ZrPd{sub 3}Si{sub 3} has been synthesized by arc-melting of the elemental components. It adopts a new structure type and crystallizes in the orthorhombic space group Cmcm with a = 3.8127(4){angstrom}, b = 15.551(1){angstrom}, c = 7.0390(5){angstrom}, and Z = 4 (Pearson symbol oC28). The structure can be regarded as being built up of Re{sub 3}B-type slabs of composition Pd{sub 3}Si alternating with {alpha}-FeSi{sub 2} slabs of composition ZrSi{sub 2}. Notable features include the presence of Si{sub 2} pairs, square pyramidal and tetrahedral coordination of Pd centers by Si atoms, an unusual distorted cubic coordination of the Zr atoms by the Si{sub 2} pairs, and an extensive network of Zr-Zr, Zr-Pd, and Pd-Pd metal-metal bonds. ZrPd{sub 3}Si{sub 3} is weakly metallic with a room-temperature resistivity of 1.7 x 10{sup {minus}3} {Omega} cm. Extended Hueckel band structure calculations confirm the metallic behavior; support the simultaneous existence of strong metal-metal, metal-nonmetal, and nonmetal-nonmetal bonding; and suggest a reduced state for the Pd atoms resulting from electron transfer from the Si atoms.

Wang, M.; Mar, A.

1999-11-01T23:59:59.000Z

409

Ab initio molecular dynamics simulations of ion-solid interactions in Gd2Zr2O7 and Gd2Ti2O7  

SciTech Connect (OSTI)

The development of ab initio molecular dynamics (AIMD) method has made it a powerful tool in describing ion-solid interactions in materials, with identification determination of threshold displacement energies with ab initio accuracy, and prediction of new mechanism for defect generation and new defective states that are different from classical molecular dynamics (MD) simulations. In the present work, this method is employed to study the low energy recoil events in Gd2Zr2O7 and Gd2Ti2O7. The weighted average threshold displacement energies in Gd2Zr2O7 are determined to be 38.8 eV for Gd, 41.4 eV for Zr, 18.6 eV for O48f, and 15.6 eV for O8b, which are smaller than the respective values of 41.8, >53.8, 22.6 and 16.2 eV in Gd2Ti2O7. It reveals that all the ions in Gd2Zr2O7 are more easily displaced than those in Gd2Ti2O7, and anion order-disorder are more likely to be involved in the displacement events than cation disordering. The average charge transfer from the primary knock-on atom to its neighbors is estimated to be ~0.15, ~0.11-0.27 and ~0.1-0.13 |e| for Gd, Zr (or Ti), and O, respectively. Negligence of the charge transfer in the interatomic potentials may result in the larger threshold displacement energies in classical MD.

Wang, X J [University of Electronic Science and Technology of China (UESTC); Xiao, Haiyan [University of Tennessee, Knoxville (UTK); Zu, X T [University of Electronic Science and Technology of China (UESTC); Zhang, Yanwen [ORNL; Weber, William J [ORNL

2013-01-01T23:59:59.000Z

410

Use of Sm-123 + Sm-211 Mixed-powder Buffers to Assist the Growth of SmBCO and ZrO2-doped SmBCO Single Grain, Bulk Superconductors  

E-Print Network [OSTI]

. Murakami, and I. Hirabayashi, "High critical current density in RE–Ba–Cu–O bulk superconductors with very fine RE2BaCuO5 particles," Physica C: Superconductivity, vol. 412-414, no. 1, pp. 557–565, Oct. 2004. [4] H. S. Chauhan, and M. Murakami, "Hot... )–Ba–Cu–O superconductors," Nature Materials, vol. 4, pp. 476 - 480, Jun. 2005. [7] N. H. Babu, K. Iida, Y. Shi, and D. A. Cardwell, "Processing of high performance (LRE)-Ba–Cu–O large, single-grain bulk superconductors in air," Physica C: Superconductivity, vol. 445...

Zhao, Wen; Shi, Yunhua; Dennis, Anthony R.; Cardwell, David A.

2014-12-18T23:59:59.000Z

411

JOURNAL DE PHYSIQUE Colfoque Cl, supplkrnent au no 4, Tome 38, Auril 1977, page Cl-333 METAL-OXIDES COMPOSITES FOR BaFe,,Ol PERMANENT MAGNETS  

E-Print Network [OSTI]

the possibility of producing composites of Ba ferrite with various metals such as cobalt, nickel, iron, copper of a CO deposit with preferential orientation obtained by chemical reduction and electrodeposition. 2. CO

Paris-Sud XI, Université de

412

Is the Communicative Language Teaching Approach More Effective Than the Grammar Translation Method at Teaching the Ba-Construction in Mandarin Chinese to American Undergraduate Students?  

E-Print Network [OSTI]

(CLT) with that of Grammar Translation Method (GT) at teaching Chinese as a foreign language (CFL). The present study fills this gap. The purpose of this study is to investigate quantitatively which method is more effective at teaching the ba...

Wang, Jun

2013-12-31T23:59:59.000Z

413

Structural and magnetic properties and superconductivity in Ba(Fe{sub 1-x}TM{sub x}){sub 2}As{sub 2}  

SciTech Connect (OSTI)

We studied the effects on structural and magnetic phase transitions and the emergence of superconductivity in transition metal substituted BaFe{sub 2}As{sub 2}. We grew four series of Ba(Fe{sub 1-x}TM{sub x}){sub 2}As{sub 2} (TM=Ru, Mn, Co+Cr and Co+Mn) and characterized them by crystallographic, magnetic and transport measurements. We also subjected Ba(Fe{sub 1-x}Cr{sub x}){sub 2}As{sub 2} and Ba(Fe{sub 1-x}Co{sub x}){sub 2}As{sub 2} to heat treatment to explore what changes might be induced.

Thaler, Alexander

2012-07-23T23:59:59.000Z

414

Single-crystal neutron diffraction studies on Ni-based metal-pnictide superconductor BaNi2As2  

SciTech Connect (OSTI)

We report the results of single-crystal neutron diffraction studies of the superconductor BaNi{sub 2}As{sub 2}. The experiments were performed on a tiny crystal of mass 0.8 mg at several temperatures between 20 and 200 K using the Single Crystal Diffractometer, SCD, at the Los Alamos Neutron Science Center. Above 130 K, BaNi{sub 2}As{sub 2} crystallizes in the tetragonal ThCr{sub 2}Si{sub 2} structure. Our neutron diffraction data corroborate a first-order structural transition around 130 K with a relatively large hysteresis of about 10K, in agreement with observations from bulk studies. The anisotropic thermal displacement coefficients are enhanced along c-axis approaching the transition, and a splitting is observed for in-plane type reflections below the transition, which is evidence for a change in crystal structure.

Kothapalli, Karunakar [Los Alamos National Laboratory; Ronning, F [Los Alamos National Laboratory; Bauer, E D [Los Alamos National Laboratory; Schultz, A J [Los Alamos National Laboratory; Nakotte, Heinz [Los Alamos National Laboratory

2009-01-01T23:59:59.000Z

415

Two-dimensional resonant magnetic excitation in BaFe1.84Co0.16As2  

SciTech Connect (OSTI)

Inelastic neutron scattering measurements on single crystals of superconducting BaFe1.84Co0.16As2 clearly reveal a magnetic excitation located at wavevectors (1/2 1/2 L) in tetragonal notation. The scattering is much broader in L than are spin waves observed in the parent compound BaFe2As2 indicating that the excitations in the superconducting material are more two-dimensional in nature. The excitation appears gapless for T > TC and becomes gapped on cooling below TC. The observed gap energy is approximately 9.6 meV corresponding to 5 kBTC which is remarkably similar to the canonical value for the resonance energy in the cuprates.

Lumsden, Mark D [ORNL; Christianson, Andrew D [ORNL; Parshall, Daniel [ORNL; Stone, Matthew B [ORNL; Nagler, Stephen E [ORNL; Mook Jr, Herbert A [ORNL; Lokshin, Konstantin A [ORNL; Egami, Takeshi [ORNL; Abernathy, Douglas L [ORNL; Goremychkin, E. A. [ISIS Facility, Rutherford Appleton Laboratory; Osborn, R. [Argonne National Laboratory (ANL); McGuire, Michael A [ORNL; Safa-Sefat, Athena [ORNL; Jin, Rongying [ORNL; Sales, Brian C [ORNL; Mandrus, David [ORNL

2009-01-01T23:59:59.000Z

416

Coherency strain enhanced dielectric-temperature property of rare-earth doped BaTiO{sub 3}  

SciTech Connect (OSTI)

Core/shell-grained BaTiO{sub 3} samples were prepared with addition of rare earth elements. The core/shell interface was semi-coherent, and many misfit dislocations formed in Dy-doped samples. In contrast, a coherent interface and few dislocations were observed in Ho- and Er-doped samples. Dy-doped samples exhibited poor temperature stability, showing a peak with no frequency dispersion. Ho- and Er-doped samples exhibited a broad curve with frequency dispersion. This improved temperature stability is attributed to the coherency strain, which leads to the formation of polar nano-regions in the shell. Coherency at the core/shell interface is critical to improve the temperature stability of core/shell-structured BaTiO{sub 3}.

Jeon, Sang-Chae; Kang, Suk-Joong L. [Materials Interface Laboratory, Department of Materials Science and Engineering, Korea Advanced Institute of Science and Technology, 373-1, Guseong-dong, Yuseong-gu, Daejeon 305-701 (Korea, Republic of)] [Materials Interface Laboratory, Department of Materials Science and Engineering, Korea Advanced Institute of Science and Technology, 373-1, Guseong-dong, Yuseong-gu, Daejeon 305-701 (Korea, Republic of)

2013-03-18T23:59:59.000Z

417

Phase, Dielectric and Ferroelectric Properties of Microwave Sintered La and Ca Modified BaTiO{sub 3} Ceramics  

SciTech Connect (OSTI)

Lanthanum and calcium modified barium titanate, Ba{sub (1-x)}La{sub x}Ti{sub (1-x/4)}O{sub 3}/BLT and Ba({sub 1-x})Ca{sub x}TiO{sub 3}/BCT, where x = 0.02, ferroelectric ceramic samples were synthesized in single perovskite phase by microwave processing technique. Sintering temperature was optimized at 1100 deg. C for 1h. Presence of pore free micron size uniform grains suggested the advantage of using microwave sintering process. Transition temperature (T{sub c}) decreases with the substitution of La content in BT system. Temperature coefficient of capacitance is negligible from RT temperature to 75 deg. C for BLT ceramic samples. Polarization vs. electric field (P-E) hysteresis loop study confirms the ferroelectric nature of the modified BT ceramic samples.

Sonia, S.; Patel, R. K. [Department of Chemistry, National Institute of Technology, Rourkela - 769008 (India); Kumar, P. [Department of Physics, National Institute of Technology, Rourkela - 769008 (India); Prakash, Chandra [Directorate of IE and IPR, DRDO, DRDO Bhawan, New Delhi-110105 (India); Agrawal, D. K. [Materials Research Laboratory, Pennsylvania State University, University Park, PA 16802 (United States)

2011-11-22T23:59:59.000Z

418

Heat capacity of the site-diluted spin dimer system Ba?(Mn1-xVx)?O?  

DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

Heat-capacity and susceptibility measurements have been performed on the diluted spin dimer compound Ba?(Mn1-xVx)?O?. The parent compound Ba?Mn?O? is a spin dimer system based on pairs of antiferromagnetically coupled S=1, 3d˛ Mn?? ions such that the zero-field ground state is a product of singlets. Substitution of nonmagnetic S=0, 3d? V?? ions leads to an interacting network of unpaired Mn moments, the low-temperature properties of which are explored in the limit of small concentrations 0?x?0.05. The zero-field heat capacity of this diluted system reveals a progressive removal of magnetic entropy over an extended range of temperatures, with no evidence for a phase transition. The concentration dependence does not conform to expectations for a spin-glass state. Rather, the data suggest a low-temperature random singlet phase, reflecting the hierarchy of exchange energies found in this system.

Samulon, E. C.; Shapiro, M. C.; Fisher, I. R.

2011-08-01T23:59:59.000Z

419

APS/123-QED Evidence for nodeless energy gaps in hole-doped Ba0.68K0.32Fe2As2  

E-Print Network [OSTI]

Institute - Heisenbergstrasse 1, D-70569 Stuttgart, Germany 3 Institute of Science and Technology for Opto-doped Ba0.68K0.32Fe2As2 superconductor: NMR study in a clean single crystal Z. Li,1 D. L. Sun,2 C. T. Lin,2) Abstract We report 75As NMR studies on a very clean hole-doped single crystal Ba0.68K0.32Fe2As2 (Tc = 38

Hu, Jiangping

420

High field nuclear magnetic resonance in transition metal substituted BaFe{sub 2}As{sub 2}  

SciTech Connect (OSTI)

We report high field {sup 75}As nuclear magnetic resonance (NMR) measurements on Co and Cu substituted BaFe{sub 2}As{sub 2} single crystals displaying same structural/magnetic transition T{sub 0}?128??K. From our anisotropy studies in the paramagnetic state, we strikingly found virtually identical quadrupolar splitting and consequently the quadrupole frequency ?{sub Q}?2.57(1)??MHz for both compounds, despite the claim that each Cu delivers 2 extra 3d electrons in BaFe{sub 2}As{sub 2} compared to Co substitution. These results allow us to conclude that a subtle change in the crystallographic structure, particularly in the Fe–As tetrahedra, must be the most probable tuning parameter to determine T{sub 0} in this class of superconductors rather than electronic doping. Furthermore, our NMR data around T{sub 0} suggest coexistence of tetragonal/paramagnetic and orthorhombic/antiferromagnetic phases between the structural and the spin density wave magnetic phase transitions, similarly to what was reported for K-doped BaFe{sub 2}As{sub 2} [Urbano et al., Phys. Rev. Lett. 105, 107001 (2010)].

Garitezi, T. M., E-mail: thalesmg@ifi.unicamp.br; Lesseux, G. G.; Rosa, P. F. S.; Adriano, C.; Pagliuso, P. G.; Urbano, R. R. [Instituto de Física “Gleb Wataghin,” UNICAMP, Campinas, SP 13083-859 (Brazil); Reyes, A. P.; Kuhns, P. L. [National High Magnetic Field Laboratory, FSU, Tallahassee, Florida 32306-4005 (United States)

2014-05-07T23:59:59.000Z

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


421

Structural and magnetic properties of the Kagome antiferromagnet YbBaCo{sub 4}O{sub 7}  

SciTech Connect (OSTI)

The mixed-valent compound YbBaCo{sub 4}O{sub 7} is built up of Kagome sheets of CoO{sub 4} tetrahedra, linked in the third dimension by a triangular layer of CoO{sub 4} tetrahedra in an analogous fashion to that found in the known geometrically frustrated magnets such as pyrochlores and SrCr{sub 9} {sub x} Ga{sub 12-9} {sub x} O{sub 19} (SCGO). We have undertaken a study of the structural and magnetic properties of this compound using combined high-resolution powder neutron and synchrotron X-ray diffraction. YbBaCo{sub 4}O{sub 7} undergoes a first-order trigonal{sup {yields}}orthorhombic phase transition at 175 K. We show that this transition occurs as a response to a markedly underbonded Ba{sup 2+} site in the high-temperature phase and does not appear to involve charge ordering of Co{sup 2+}/Co{sup 3+} ions in the tetrahedra. The symmetry lowering relieves the geometric frustration of the structure, and a long-range-ordered 3-D antiferromagnetic state develops below 80 K.

Huq, A. [Intense Pulsed Neutron Source, Argonne National Laboratory, 9700 S. Cass Ave., Argonne, IL 60439 (United States); Mitchell, J.F. [Materials Science Division, Argonne National Laboratory, 9700 S. Cass Ave., Argonne, IL 60439 (United States)]. E-mail: mitchell@anl.gov; Zheng, H. [Materials Science Division, Argonne National Laboratory, 9700 S. Cass Ave., Argonne, IL 60439 (United States); Chapon, L.C. [ISIS Facility, Rutherford Appleton Laboratory-CCLRC, Chilton, Didcot, Oxfordshire, OX11 0QX (United Kingdom); Radaelli, P.G. [ISIS Facility, Rutherford Appleton Laboratory-CCLRC, Chilton, Didcot, Oxfordshire, OX11 0QX (United Kingdom); Knight, K.S. [ISIS Facility, Rutherford Appleton Laboratory-CCLRC, Chilton, Didcot, Oxfordshire, OX11 0QX (United Kingdom); Stephens, P.W. [Department of Physics and Astronomy, SUNY Stonybrook, NY 11794 (United States)

2006-04-15T23:59:59.000Z

422

First order phase transition and superconductivity in BaNi2As2 single crystals  

SciTech Connect (OSTI)

We report the synthesis and physical properties of single crystals of stoichiometric BaNi{sub 2}As{sub 2} which crystallizes in the ThCr{sub 2}Si{sub 2} structure type with lattice parameters a = 4.112(4) {angstrom} and c = 11.54(2) {angstrom}. Resistivity and heat capacity show a first order phase transition at T{sub 0} = 130 K with a thermal hysteresis of 7 K. The Hall coefficient is weakly temperature dependent from room temperature to 2 K where it has a value of -4 x 10{sup -10} {Omega}-cm/Oe. Resist.ivity, ac-susceptibility, and heat capacity find evidence for bulk superconductivity at T{sub c} = 0.7 K. The Sommerfeld coefficient at T{sub c} is 11.6 {+-} 0.9 mJ/ molK{sup 2}. The upper critical field is anisotropic with initial slopes of dH{sub c2}{sup c}/dT = -0.19 T/K and dH{sub c2}{sup ab}/dT = -0.40 T/K, as determined by resistivity.

Ronning, F [Los Alamos National Laboratory; Kurita, N [Los Alamos National Laboratory; Bauer, E D [Los Alamos National Laboratory; Scott, B L [Los Alamos National Laboratory; Park, T [Los Alamos National Laboratory; Klimczuk, T [Los Alamos National Laboratory; Movshovich, R [Los Alamos National Laboratory; Thompson, J D [Los Alamos National Laboratory

2008-01-01T23:59:59.000Z

423

Cross-section measurement of the $^{130}$Ba(p,$?$)$^{131}$La reaction for $?$-process nucleosynthesis  

E-Print Network [OSTI]

A measurement of total cross-section values of the $^{130}$Ba(p,$\\gamma$)$^{131}$La reaction at low proton energies allows a stringent test of statistical model predictions with different proton+nucleus optical model potentials. Since no experimental data are available for proton-capture reactions in this mass region around A~$\\approx$~130, this measurement can be an important input to test the global applicability of proton+nucleus optical model potentials. The total reaction cross-section values were measured by means of the activation method. After the irradiation with protons, the reaction yield was determined by use of $\\gamma$-ray spectroscopy using two clover-type high-purity germanium detectors. In total, cross-section values for eight different proton energies could be determined in the energy range between 3.6 MeV $\\leq E_p \\leq$ 5.0 MeV, thus, inside the astrophysically relevant energy region. The measured cross-section values were compared to Hauser-Feshbach calculations using the statistical model codes TALYS and SMARAGD with different proton+nucleus optical model potentials. With the semi-microscopic JLM proton+nucleus optical model potential used in the SMARAGD code, the absolute cross-section values are reproduced well, but the energy dependence is too steep at the lowest energies. The best description is given by a TALYS calculation using the semi-microscopic Bauge proton+nucleus optical model potential using a constant renormalization factor.

L. Netterdon; A. Endres; G. G. Kiss; J. Mayer; T. Rauscher; P. Scholz; K. Sonnabend; Zs. Török; A. Zilges

2014-09-27T23:59:59.000Z

424

Structural feature controlling superconductivity in compressed BaFe{sub 2}As{sub 2}  

SciTech Connect (OSTI)

Superconductivity can be induced with the application of pressure but it disappears eventually upon heavy compression in the iron-based parent compound BaFe{sub 2}As{sub 2}. Structural evolution with pressure is used to understand this behavior. By performing synchrotron X-ray powder diffraction measurements with diamond anvil cells up to 26.1?GPa, we find an anomalous behavior of the lattice parameter with a S shape along the a axis but a monotonic decrease in the c-axis lattice parameter with increasing pressure. The close relationship between the axial ratio c/a and the superconducting transition temperature T{sub c} is established for this parent compound. The c/a ratio is suggested to be a measure of the spin fluctuation strength. The reduction of T{sub c} with the further increase of pressure is a result of the pressure-driven weakness of the spin-fluctuation strength in this material.

Yang, Wenge, E-mail: wyang@ciw.edu [Center for High Pressure Science and Technology Advanced Research, Shanghai 201203 (China); High Pressure Synergetic Consortium, Geophysical Laboratory, Carnegie Institution of Washington, Argonne, Illinois 60439 (United States); Jia, Feng-Jiang [Key Laboratory of Materials Physics and Center for Energy Matter in Extreme Environments, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei 230031 (China); Tang, Ling-Yun [Center for High Pressure Science and Technology Advanced Research, Shanghai 201203 (China); Department of Physics, South China University of Technology, Guangzhou 510640 (China); Tao, Qian; Xu, Zhu-An [Department of Physics, Zhejiang University, Hangzhou 310027 (China); Chen, Xiao-Jia, E-mail: xjchen@ciw.edu [Center for High Pressure Science and Technology Advanced Research, Shanghai 201203 (China); Key Laboratory of Materials Physics and Center for Energy Matter in Extreme Environments, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei 230031 (China); Geophysical Laboratory, Carnegie Institution of Washington, Washington, DC 20015 (United States)

2014-02-28T23:59:59.000Z

425

High temperature superconductor step-edge Josephson junctions using Ti-Ca-Ba-Cu-O  

SciTech Connect (OSTI)

A process is disclosed for formulating non-hysteretic and hysteretic Josephson junctions using HTS materials which results in junctions having the ability to operate at high temperatures while maintaining high uniformity and quality. The non-hysteretic Josephson junction is formed by step-etching a LaAlO[sub 3] crystal substrate and then depositing a thin film of TlCaBaCuO on the substrate, covering the step, and forming a grain boundary at the step and a subsequent Josephson junction. Once the non-hysteretic junction is formed the next step to form the hysteretic Josephson junction is to add capacitance to the system. In the current embodiment, this is accomplished by adding a thin dielectric layer, LaA1O[sub 3], followed by a cap layer of a normal metal where the cap layer is formed by first depositing a thin layer of titanium (Ti) followed by a layer of gold (Au). The dielectric layer and the normal metal cap are patterned to the desired geometry. 8 figs.

Ginley, D.S.; Hietala, V.M.; Hohenwarter, G.K.G.; Martens, J.S.; Plut, T.A.; Tigges, C.P.; Vawter, G.A.; Zipperian, T.E.

1994-10-25T23:59:59.000Z

426

High temperature superconductor step-edge Josephson junctions using Ti-Ca-Ba-Cu-O  

SciTech Connect (OSTI)

A process for formulating non-hysteretic and hysteretic Josephson junctions using HTS materials which results in junctions having the ability to operate at high temperatures while maintaining high uniformity and quality. The non-hysteretic Josephson junction is formed by step-etching a LaAlO.sub.3 crystal substrate and then depositing a thin film of TlCaBaCuO on the substrate, covering the step, and forming a grain boundary at the step and a subsequent Josephson junction. Once the non-hysteretic junction is formed the next step to form the hysteretic Josephson junction is to add capacitance to the system. In the current embodiment, this is accomplished by adding a thin dielectric layer, LaA1O.sub.3, followed by a cap layer of a normal metal where the cap layer is formed by first depositing a thin layer of titanium (Ti) followed by a layer of gold (Au). The dielectric layer and the normal metal cap are patterned to the desired geometry.

Ginley, David S. (Evergreen, CO); Hietala, Vincent M. (Placitas, NM); Hohenwarter, Gert K. G. (Madison, WI); Martens, Jon S. (Sunnyvale, CA); Plut, Thomas A. (Albuquerque, NM); Tigges, Chris P. (Albuquerque, NM); Vawter, Gregory A. (Albuquerque, NM); Zipperian, Thomas E. (Albuquerque, NM)

1994-10-25T23:59:59.000Z

427

Multiphonon states in {sub 56}{sup 136}Ba{sub 80}  

SciTech Connect (OSTI)

Low-lying multiphonon states in {sup 136}Ba have been populated with the inelastic neutron scattering reaction. Excitation functions were performed at neutron energies from 2.2 to 3.9 MeV, and {gamma}-ray angular distributions were measured at 2.5, 3.0, and 3.5 MeV. Lifetimes have been determined using the Doppler-shift attenuation method, and electromagnetic transition rates have been deduced. The previously assigned 2{sub 1,ms}{sup +} mixed-symmetry state at 2128.9 keV has been confirmed and is not greatly fragmented. For the first time in the N=80 isotones, a 3{sub 2,ms}{sup +} two-phonon mixed-symmetry state is proposed. In addition, the 2{sub 5}{sup +} and the 4{sub 3}{sup +} levels at 2222.7 and 2356.4 keV, respectively, decay with large B(M1) values to the two-phonon 2{sub 2}{sup +} and 4{sub 1}{sup +} states, respectively, which suggests two-phonon mixed-symmetric character. Their excitation energies, however, are not consistent with this interpretation.

Mukhopadhyay, S.; Scheck, M.; Crider, B.; Choudry, S. N.; Elhami, E.; McEllistrem, M. T.; Orce, J. N. [Department of Physics and Astronomy, University of Kentucky, Lexington, Kentucky 40506-0055 (United States); Peters, E. [Department of Chemistry, University of Kentucky, Lexington, Kentucky 40506-0055 (United States); Yates, S. W. [Department of Physics and Astronomy, University of Kentucky, Lexington, Kentucky 40506-0055 (United States); Department of Chemistry, University of Kentucky, Lexington, Kentucky 40506-0055 (United States)

2008-09-15T23:59:59.000Z

428

Specification of CuCrZr Alloy Properties after Various Thermo-Mechanical Treatments and Design Allowables including Neutron Irradiation Effects  

SciTech Connect (OSTI)

Precipitation hardened CuCrZr alloy is a promising heat sink and functional material for various applica- tions in ITER, for example the first wall, blanket electrical attachment, divertor, and heating systems. Three types of thermo-mechanical treatment were identified as most promising for the various applica- tions in ITER: solution annealing, cold working and ageing; solution annealing and ageing; solution annealing and ageing at non-optimal condition due to specific manufacturing processes for engineer- ing-scale components. The available data for these three types of treatments were assessed and mini- mum tensile properties were determined based on recommendation of Structural Design Criteria for the ITER In-vessel Components. The available data for these heat treatments were analyzed for assess- ment of neutron irradiation effect. Using the definitions of the ITER Structural Design Criteria the design allowable stress intensity values are proposed for CuCrZr alloy after various heat treatments.

Barabash, Vladimir [ITER Organization, Saint Paul Lez Durance, France] [ITER Organization, Saint Paul Lez Durance, France; Kalinin, G. M. [RDIPE, P.O. Box 788, 101000 Moscow, Russia] [RDIPE, P.O. Box 788, 101000 Moscow, Russia; Fabritsiev, Sergei A. [D.V. Efremov Scientific Research Institute, St. Petersburg, Russia] [D.V. Efremov Scientific Research Institute, St. Petersburg, Russia; Zinkle, Steven J [ORNL] [ORNL

2012-01-01T23:59:59.000Z

429

Surface Passivation of Nanoporous TiO2 via Atomic Layer Deposition of ZrO2 for Solid-State Dye-Sensitized Solar Cell Applications  

E-Print Network [OSTI]

to the spiro-OMeTAD. Introduction Dye-sensitized solar cells (DSCs) based on mesoporous titania and liquidSurface Passivation of Nanoporous TiO2 via Atomic Layer Deposition of ZrO2 for Solid-State Dye-Sensitized Solar Cell Applications Tina C. Li, Ma´rcio S. Go´es,,§ Francisco Fabregat-Santiago,*, Juan Bisquert

430

Thermodynamic Assessment of Hot Corrosion Mechanisms of Superalloys Hastelloy N and Haynes 242 in Eutectic Mixture of Molten Salts KF and ZrF4  

SciTech Connect (OSTI)

The KF - ZrF4 system was considered for the application as a heat exchange agent in molten salt nuclear reactors (MSRs) beginning with the work carried out at ORNL in early fifties. Based on a combination of excellent properties such as thermal conductivity, viscosity in the molten state, and other thermo-physical and rheological properties, it was selected as one of possible candidates for the nuclear reactor secondary heat exchanger loop.

Michael V. Glazoff

2012-02-01T23:59:59.000Z

431

Influence of crystalline phase and defects in the ZrO{sub 2} nanoparticles synthesized by thermal plasma route on its photocatalytic properties  

SciTech Connect (OSTI)

Graphical abstract: Thermal plasma synthesized nanophase zirconia showing the blue shift in the band gap of monoclinic phase as found from the photoabsorption spectroscopy was found to be the dominant parameter for the enhancement in its photocatalytic activity. The existence of different defect states and their concentration in as synthesized samples also inferred from the photoabsorption measurements were also found to be responsible for the enhanced photocatalytic activity of the samples. Highlights: ? Phase controlled structural formation of nanophase ZrO{sub 2} by thermal plasma route. ? Enhanced photocatalytic degradation rate of methylene blue dye. ? The blue shift in the band gap of monoclinic phase of nanocrystalline ZrO{sub 2}. ? Existence of different defect states in the as synthesized nano phase ZrO{sub 2}. ? Several competing processes which controls the photocatalytic degradation rate. -- Abstract: The photocatalytic activity of pure ZrO{sub 2} samples, prepared by a thermal plasma route, and characterized by X-ray diffraction technique was tested for the degradation of methylene blue, which is known to be a hazardous dye. Although, all these samples synthesized at different operating pressures of the thermal plasma reactor showed the photocatalytic activity; the sample synthesized at 1.33 bar of operating pressure showed the highest photocatalytic activity. The blue shift in the band gap of monoclinic phase, as observed from the photo-absorption spectroscopy, may be attributed to the enhanced photocatalytic activity. The existence of different defect states and their concentration as, inferred from the photo-absorption measurements were also found to be responsible for the enhanced photocatalytic activity of the as synthesized samples.

Nawale, Ashok B.; Kanhe, Nilesh S.; Bhoraskar, S.V. [Department of Physics, University of Pune, Pune 411007 (India)] [Department of Physics, University of Pune, Pune 411007 (India); Mathe, V.L., E-mail: vlmathe@physics.unipune.ac.in [Department of Physics, University of Pune, Pune 411007 (India); Das, A.K. [Laser and Plasma Technology Division, Bhabha Atomic Research Centre, Trombay, Mumbai 400085 (India)] [Laser and Plasma Technology Division, Bhabha Atomic Research Centre, Trombay, Mumbai 400085 (India)

2012-11-15T23:59:59.000Z

432

Low thermal expansion behavior and thermal durability of ZrTiO4Al2TiO5Fe2O3 ceramics between 750 and 1400  

E-Print Network [OSTI]

2002 Abstract The thermal-shock-resistant materials in the system Al2TiO5­ZrTiO4 (ZAT) were synthesized Aluminum titanate (Al2TiO5) is well-known as an excellent thermal shock-resistant material, resulting from. All rights reserved. Keywords: Al2TiO5; Thermal expansion; Thermal shock resistance 1. Introduction

Cao, Guozhong

433

A Method to Increase Current Density in a Mono Element Internal Tin Processed Superconductor Utilizing Zr Oxide to Refine Grain Size  

SciTech Connect (OSTI)

The effect of Oxygen on (Nb1Zr)3Sn multifilament conductors manufactured by the Mono Element Internal Tin (MEIT) process was explored to improve the current density by refining the grain size. This followed work first done by General Electric on the Nb3Sn tape process. Techniques to fabricate the more difficult Nb1Zr composites are described and allowed fabrication of long lengths of .254 mm diameter wire from an 88.9 mm diameter billet. Oxygen was incorporated through the use of SnO2 mixed with tin powder and incorporated into the core. These were compared to samples with Ti+Sn and Cu+Sn cores. Heat treatments covered the range of 700 C to 1000 C. Current density vs. H, grain size, and reaction percentages are provided for the materials tested. The Oxygen gave superior results in the temperature range of 815-1000 C. It also stabilized the filament geometry of the array in comparison to the other additions at the higher temperatures. At 815 C a peak in layer Jc yielded values of 2537 A/mm2 at 12 T and 1353 A/mm2 at 15T, 8-22% and 30-73% greater respectively than 700 C values. Results with Oxygen at high temperature show the possibility of high speed continuous reaction of the composite versus the current batch or react in place methods. In general the Ti additions gave superior results at the lower reaction temperature. Future work is suggested to determine if the 815 C reaction temperature can lead to higher current density in high tin (Nb1Zr+Ox)3Sn conductors. A second technique incorporated oxygen directly into the Nb1Zr rods through heat treatment with Nb2O5 at 1100 C for 100 hours in vacuum prior to extrusion. The majority of the filaments reduced properly in the composite but some local variations in hardness led to breakage at smaller diameters.

Bruce A. Zeitlin, Eric Gregory

2008-04-07T23:59:59.000Z

434

Thermal stability of Al- and Zr-doped HfO{sub 2} thin films grown by direct current magnetron sputtering  

SciTech Connect (OSTI)

Ultrathin HfO{sub 2} dielectric films doped with Al and Zr were grown on p-type Si(100) substrates by dc magnetron sputtering, and their microstructural and electrical properties were examined. Compositions and chemical states of the dielectric films were analyzed by Rutherford backscattering spectrometry and x-ray photoelectron spectroscopy. The HfO{sub 2} films doped with Zr were crystallized even from the as-deposited state, however, the crystallization temperature of the HfO{sub 2} film doped with 16% Al{sub 2}O{sub 3} was delayed up to 900 deg. C. As the annealing temperature increases, high-resolution transmission electron microscopy analyses of all doped HfO{sub 2} films showed an increase of the interfacial layer thickness due to the diffusion of small partial pressure of oxygen in annealing ambient. Our results also showed that the addition of Al{sub 2}O{sub 3} to 14% is not useful for blocking the oxygen diffusion through the (HfO{sub 2}){sub 0.86}(Al{sub 2}O{sub 3}){sub 0.14} film. From the capacitance-voltage measurements, the dielectric constants of the Al- and Zr-doped HfO{sub 2} thin films were measured to be 18.7 and 7.6, respectively.

Hong, Yeong-Eui; Kim, Yong-Seok; Do, Kihoon; Lee, Dongwon; Ko, Dae-Hong; Ku, Ja-Hum; Kim, Hyoungsub [Department of Ceramic Engineering, Yonsei University, 134 Shinchon-Dong, Seodaemoon-Ku, Seoul 120-749 (Korea, Republic of); Semiconductor R and D Division, Samsung Electronics Co, Ltd., San no. 24, Nongseo-Ri, Kiheung-Eup, Yongin-City, Kyunggi-Do 449-711 (Korea, Republic of); Department of Advanced Materials Engineering, Sungkyunkwan University, 300 Chunchun-Dong, Jangan-Ku, Suwon 440-746 (Korea, Republic of)

2005-09-15T23:59:59.000Z

435

First-principles study of structural, electronic, vibrational, dielectric and elastic properties of tetragonal Ba{sub 2}YTaO{sub 6}  

SciTech Connect (OSTI)

We report first-principles study of structural, electronic, vibrational, dielectric, and elastic properties of Ba{sub 2}YTaO{sub 6}, a pinning material in high temperature superconductors (HTS), by using density functional theory. By using different exchange-correlation potentials, the accuracy of the calculated lattice constants of Ba{sub 2}YTaO{sub 6} has been achieved with GGA-RPBE, since many important physical quantities crucially depend on change in volume. We have calculated the electronic band structure dispersion, total and partial density of states to study the band gap origin and found that Ba{sub 2}YTaO{sub 6} is an insulator with a direct band gap of 3.50?eV. From Mulliken population and charge density studies, we conclude that Ba{sub 2}YTaO{sub 6} have a mixed ionic-covalent character. Moreover, the vibrational properties, born effective charges, and the dielectric permittivity tensor have been calculated using linear response method. Vibrational spectrum determined through our calculations agrees well with the observed Raman spectrum, and allows assignment of symmetry labels to modes. We perform a detailed analysis of the contribution of the various infrared-active modes to the static dielectric constant to explain its anisotropy, while electronic dielectric tensor of Ba{sub 2}YTaO{sub 6} is nearly isotropic, and found that static dielectric constant is in good agreement with experimental value. The six independent elastic constants were calculated and found that tetragonal Ba{sub 2}YTaO{sub 6} is mechanically stable. Other elastic properties, including bulk modulus, shear modulus, Young's modulus, Poisson's ratio, and elastic anisotropy ratios are also investigated and found that Poisson's ratio and Young's modulus of Ba{sub 2}YTaO{sub 6} are similar to that of other pinning materials in HTS.

Ganeshraj, C.; Santhosh, P. N., E-mail: santhosh@physics.iitm.ac.in [Low Temperature Physics Laboratory, Department of Physics, Indian Institute of Technology Madras, Chennai 600 036, Tamil Nadu (India)

2014-10-14T23:59:59.000Z

436

Fluorine sites in glasses and transparent glass-ceramics of the system Na{sub 2}O/K{sub 2}O/Al{sub 2}O{sub 3}/SiO{sub 2}/BaF{sub 2}  

SciTech Connect (OSTI)

The transparent glass-ceramics obtained in the silicate system Na{sub 2}O/K{sub 2}O/SiO{sub 2}/BaF{sub 2} show homogeneously dispersed BaF{sub 2} nano crystals with a narrow size distribution. The X-ray diffraction and the nuclear magnetic resonance spectroscopy were applied to glasses and the respective glass-ceramics in order to clarify the crystallization mechanism and the role of fluorine during crystallization. With an increasing annealing time, the concentration and also the number of crystals remain approximately constant. With an increasing annealing temperature, the crystalline fraction increases until a saturation limit is reached, while the number of crystals decreases and the size of the crystals increases. Fluoride in the glassy network occurs as Al-F-Ba, Al-F-Na and also as Ba-F structures. The latter are transformed into crystalline BaF{sub 2} and fluoride is removed from the Al-F-Ba/Na bonds. However, some fluorine is still present in the glassy phase after the crystallization. -- Graphical abstract: The X-ray diffraction and the nuclear magnetic resonance spectroscopy were applied to glasses in the silicate system Na{sub 2}O/K{sub 2}O/SiO{sub 2}/BaF{sub 2} and the respective glass-ceramics with BaF{sub 2} nano crystals in order to clarify the crystallization mechanism and the role of fluorine during crystallization. Display Omitted Research highlights: {yields} BaF{sub 2} nano crystals are precipitated from a silicate glass system. {yields} Ostwald ripening during the late stage of crystallization does not occur. {yields} Fluorine in the glass is coordinated with Ba as well as Al together with Ba or Na.{yields} In the glass-ceramics, the residual fluorine is coordinated as Al-F-Ba/Na.

Bocker, Christian, E-mail: christian.bocker@uni-jena.d [Otto-Schott-Institut, Jena University, Fraunhoferstr. 6, 07743 Jena (Germany); Munoz, Francisco; Duran, Alicia [Instituto de Ceramica y Vidrio (CSIC), Kelsen 5, 28049 Madrid (Spain); Ruessel, Christian [Otto-Schott-Institut, Jena University, Fraunhoferstr. 6, 07743 Jena (Germany)

2011-02-15T23:59:59.000Z

437

Mercury nonstoichiometry of the Hg1-xBa2CuO4+ superconductor and the P(Hg)-P(O2)-T phase diagram of the Hg-Ba-Cu-O system.  

E-Print Network [OSTI]

1 Mercury nonstoichiometry of the Hg1-xBa2CuO4+ superconductor and the P(Hg)-P(O2)-T phase diagram-nonstoichiometry and exists in a certain P(Hg), P(O2) and T range. Mercury nonstoichiometry of Hg-1201 was investigated in the 923 T 1095 K; 2.0 P(Hg) 8.4 atm; 0.09 P(O2) 0.86 atm ranges. It was found that the mercury

Rudnyi, Evgenii B.

438

Correlation between upconversion photoluminescence and dielectric response in Ba-substituted (Sr{sub 1?x}Ba{sub x}){sub 4}(La{sub 0.85}Ho{sub 0.025}Yb{sub 0.125}){sub 2}Ti{sub 4}Nb{sub 6}O{sub 30}  

SciTech Connect (OSTI)

The filled tetragonal tungsten bronze (Sr{sub 1?x}Ba{sub x}){sub 4}(La{sub 0.85}Ho{sub 0.025}Yb{sub 0.125}){sub 2}Ti{sub 4}Nb{sub 6}O{sub 30} (SBLTNx: Ho-Yb) ceramics with different Ba substitution levels (x) are prepared. The upconversion photoluminescence (UC-PL) and dielectric permittivity are investigated. The substitution of Sr{sup 2+} ions at the A{sub 2}-sites by larger Ba{sup 2+} ions results in substantial variation of the UC-PL intensity as a function of substitution level x. Furthermore, the dielectric response to the substitution of Sr{sup 2+} by Ba{sup 2+} suggests a close correlation between the UC-PL intensity and dielectric permittivity. The origin for this correlation is discussed based on the random stress field (RSF) model.

Wei, T., E-mail: weitong.nju@gmail.com [College of Science, Civil Aviation University of China, Tianjin 300300 (China); Laboratory of Solid State Microstructures, Nanjing University, Nanjing 210093 (China); Wang, X. D. [College of Science, Civil Aviation University of China, Tianjin 300300 (China); Zhao, C. Z. [School of Electronics and Information Engineering, Tianjin Polytechnic University, Tianjin 300160 (China); Liu, M. F.; Liu, J. M., E-mail: liujm@nju.edu.cn [Laboratory of Solid State Microstructures, Nanjing University, Nanjing 210093 (China)

2014-06-30T23:59:59.000Z

439

Laser patterning and preferential orientation of two-dimensional planar {beta}-BaB{sub 2}O{sub 4} crystals on the glass surface  

SciTech Connect (OSTI)

The laser-induced crystallization method is applied to pattern two-dimensional planar {beta}-BaB{sub 2}O{sub 4} crystals on the surface of Sm{sub 2}O{sub 3}-BaO-B{sub 2}O{sub 3} glass. By scanning Yb:YVO{sub 4} fiber lasers (wavelength: 1080 nm) continuously with a small step (0.5 {mu}m) between laser irradiated areas, homogeneous planar {beta}-BaB{sub 2}O{sub 4} crystals are patterned successfully, and a preferential growth orientation of {beta}-BaB{sub 2}O{sub 4} crystals is confirmed from linearly polarized micro-Raman scattering spectrum and second harmonic intensity measurements. It is found that the crystal growth direction is perpendicular to the laser scanning direction. This relation, i.e., the perpendicular relation, is different from the behavior in discrete crystal line patterning, where the crystal growth direction is consistent with the laser scanning direction. The present study proposes the possibility of the control of crystal growth direction in laser-induced crystallization in glasses. - Graphical abstract: This figure shows confocal scanning laser microscope and polarized optical microscope photographs for {beta}-BaB{sub 2}O{sub 4} crystals obtained by laser irradiations. The laser scanning was repeated with a step of 0.5 {mu}m between the lines using the condition of the power of P=0.8 W and a laser scanning speed of S=8 {mu}m/s. It is suggested that {beta}-BaB{sub 2}O{sub 4} crystals in the overlapped laser-irradiated region are highly oriented and the c-axis direction of {beta}-BaB{sub 2}O{sub 4} crystals is perpendicular to the laser scanning direction. Highlights: Black-Right-Pointing-Pointer Laser-induced crystallization method is applied to pattern {beta}-BaB{sub 2}O{sub 4} crystals. Black-Right-Pointing-Pointer Two-dimensional planar crystals are patterned on the glass surface. Black-Right-Pointing-Pointer Preferential growth orientation of {beta}-BaB{sub 2}O{sub 4} crystals is confirmed. Black-Right-Pointing-Pointer Crystal growth direction is perpendicular to the laser scanning direction.

Suzuki, F.; Ogawa, K.; Honma, T. [Department of Materials Science and Technology, Nagaoka University of Technology, 1603-1 Kamitomioka-cho, Nagaoka 940-2188 (Japan); Komatsu, T., E-mail: komatsu@mst.nagaokaut.ac.jp [Department of Materials Science and Technology, Nagaoka University of Technology, 1603-1 Kamitomioka-cho, Nagaoka 940-2188 (Japan)

2012-01-15T23:59:59.000Z

440

Shell Model Monte Carlo method in the $pn$-formalism and applications to the Zr and Mo isotopes  

E-Print Network [OSTI]

We report on the development of a new shell-model Monte Carlo algorithm which uses the proton-neutron formalism. Shell model Monte Carlo methods, within the isospin formulation, have been successfully used in large-scale shell-model calculations. Motivation for this work is to extend the feasibility of these methods to shell-model studies involving non-identical proton and neutron valence spaces. We show the viability of the new approach with some test results. Finally, we use a realistic nucleon-nucleon interaction in the model space described by (1p_1/2,0g_9/2) proton and (1d_5/2,2s_1/2,1d_3/2,0g_7/2,0h_11/2) neutron orbitals above the Sr-88 core to calculate ground-state energies, binding energies, B(E2) strengths, and to study pairing properties of the even-even 90-104 Zr and 92-106 Mo isotope chains.

C. Ozen; D. J. Dean

2005-08-05T23:59:59.000Z

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
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441

(Sr,Ba)(Si,Ge){sub 2} for thin-film solar-cell applications: First-principles study  

SciTech Connect (OSTI)

In order to meet the increasing demand for electric power generation from solar energy conversion, the development of efficient light absorber materials has been awaited. To this end, the electronic and optical properties of advanced alkaline-earth-metals disilicides and digermanides (SrSi{sub 2}, BaSi{sub 2}, SrGe{sub 2}, and BaGe{sub 2}) are studied by means of the density functional theory using HSE06 exchange-correlation energy functional. Our calculations show that all these orthorhombic structured compounds have fundamental indirect band gaps in the range E{sub g} ? 0.89–1.25 eV, which is suitable for solar cell applications. The estimated lattice parameters and band gaps are in good agreement with experiments. Our calculations show that the electronic band structures of all four compounds are very similar except in the vicinity of the ?-point. The valence band of these compounds is made up by Si(Ge)-p states, whereas the conduction band is composed of Sr(Ba)-d states. Their band alignments are carefully determined by estimating the work function of each compound using slab model. The optical properties are discussed in terms of the complex dielectric function ?(?)?=??{sub 1}(?)?+?i?{sub 2}(?). The static and high-frequency dielectric constants are calculated, taking into account the ionic contribution. The absorption coefficient ?(?) demonstrates that a low energy dispersion of the conduction band, which results in a flat conduction band minimum, leads to large optical activity in these compounds. Therefore, alkaline-earth-metals disilicides and digermanides possess great potential as light absorbers for applications in thin-film solar cell technologies.

Kumar, Mukesh, E-mail: Kumar.Mukesh@nims.go.jp, E-mail: mkgarg79@gmail.com [Environmental Remediation Materials Unit, National Institute for Materials Science, Ibaraki 305-0044 (Japan); Umezawa, Naoto [Environmental Remediation Materials Unit, National Institute for Materials Science, Ibaraki 305-0044 (Japan); PRESTO, Japan Science and Technology Agency (JST), 4-1-8 Honcho Kawaguchi, Saitama 332-0012 (Japan); TU-NIMS Joint Research Center, School of Materials Science and Engineering, Tianjin University, 92 Weijin Road, Nankai District, Tianjin (China); Imai, Motoharu [Superconducting Properties Unit, National Institute for Materials Science, Ibaraki 305-0047 (Japan)

2014-05-28T23:59:59.000Z

442

A conversion route towards tubular SiO{sub 2} using rod-like BaSiF{sub 6} as a novel template  

SciTech Connect (OSTI)

A simple hydrothermal reaction between Ba(NO{sub 3}){sub 2} and K{sub 2}SiF{sub 6} results in the formation of 1D rod-like BaSiF{sub 6}. The BaSiF{sub 6} rods can act as efficient precursors for production of tubular SiO{sub 2} by hydrothermal reaction in alkaline solutions. Powder X-ray diffraction (XRD), X-ray photoelectron spectra (XPS), transmission electron microscopy (TEM), high resolution electron microscopy (HRTEM), and field emission scanning electron microscopy (FESEM) were used to characterize the phase and morphology of the final product. The experiments indicated the amount of NaOH, reaction temperature, and reaction time played important roles in the transformation process. A possible growth mechanism of tubular silica was proposed. - Graphical abstract: Tubular silica was prepared via a hydrothermal reaction between BaSiF{sub 6} and NaOH, in which BaSiF{sub 6} nanorods act as both a physical and chemical template. It was found that the amount of NaOH, reaction temperature, and reaction time played important roles in this transformation process.

Zhong Haoxiang; Huang Qingli; Ma Yingli [Coordination Chemistry Institute, State Key Laboratory of Coordination Chemistry, Nanjing National Laboratory of Microstructures, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing 210093 (China); Hong Jianming [Analytic Center of Nanjing University, Jiangsu, Nanjing 210093 (China); Chen Xuetai, E-mail: xtchen@netra.nju.edu.c [Coordination Chemistry Institute, State Key Laboratory of Coordination Chemistry, Nanjing National Laboratory of Microstructures, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing 210093 (China); Xue Ziling [Department of Chemistry, University of Tennessee, Knoxville, Tennessee 37996-1600 (United States)

2009-07-15T23:59:59.000Z

443

Synthesis of BaTiO[subscript 3]-20wt%CoFe[subscript 2]O[subscript 4] Nanocomposites via Spark Plasma Sintering  

SciTech Connect (OSTI)

Barium titanate-20wt% cobalt ferrite (BaTiO{sub 3}-20wt%CoFe{sub 2}O{sub 4}) nanocomposites were sintered from nanocrystalline BaTiO{sub 3} and CoFe{sub 2}O{sub 4} powders using spark plasma sintering (SPS) and pressureless sintering (PS) techniques. Using SPS, dense polycrystalline composites were obtained at a sintering temperature as low as 860 C and a time of 5 min whereas PS required a higher sintering temperature (1150 C) and time (120 min) to obtain similarly dense composites. Microstructural analysis of the composites showed that both the techniques retained nanocrystalline grain sizes after sintering. High resolution X-ray diffraction measurements revealed that the BaTiO{sub 3}-20wt%CoFe{sub 2}O{sub 4} composites sintered by the SPS technique did not exhibit formation of any new phase(s) due to reaction between the BaTiO{sub 3} and CoFe{sub 2}O{sub 4} phases during sintering. However, the PS technique resulted in the formation of additional phases (other than the BaTiO{sub 3} and CoFe{sub 2}O{sub 4} phases) in the composites. While the composites synthesized by SPS were of superior phase-purity, evidence of Fe diffusion from the spinel to the perovskite phase was found from X-ray diffraction and permittivity measurements.

Ghosh, Dipankar; Han, Hyuksu; Nino, Juan C.; Subhash, Ghatu; Jones, Jacob L. (Florida)

2012-10-23T23:59:59.000Z

444

Synthesis, structural characterization and properties of SrAl{sub 4?x}Ge{sub x}, BaAl{sub 4?x}Ge{sub x}, and EuAl{sub 4?x}Ge{sub x} (x?0.3–0.4)—Rare examples of electron-rich phases with the BaAl{sub 4} structure type  

SciTech Connect (OSTI)

Three solid solutions with the general formula AEAl{sub 4?x}Ge{sub x} (AE=Eu, Sr, Ba; 0.32(1)?x?0.41(1)) have been synthesized via the aluminum self-flux method, and their crystal structures have been established from powder and single-crystal X-ray diffraction. They are isotypic and crystallize with the well-known BaAl{sub 4} structure type, adopted by the three AEAl{sub 4} end members. In all structures, Ge substitutes Al only at the 4e Wyckoff site. Results from X-rays photoelectron spectroscopy on EuAl{sub 4?x}Ge{sub x} and EuAl{sub 4} indicate that the interactions between the Eu{sup 2+} cations and the polyanionic framework are enhanced in the Ge-doped structure, despite the slightly elevated Fermi level. Magnetic susceptibility measurements confirm the local moment magnetism, expected for the [Xe]4f{sup 7} electronic configuration of Eu{sup 2+} and suggest strong ferromagnetic interactions at cryogenic temperatures. Resistivity data from single-crystalline samples show differences between the title compounds, implying different bonding characteristics despite the close Debye temperatures. A brief discussion on the observed electron count and homogeneity ranges for AEAl{sub 4?x}Ge{sub x} (AE=Eu, Sr, Ba) is also presented. - Graphical abstract: AEAl{sub 4?x}Ge{sub x} (AE=Eu, Sr, Ba; 0.32(1)?x?0.41(1)), three “electron-rich” phases with BaAl{sub 4} structure type have been synthesized and characterized. Display Omitted - Highlights: • Three BaAl{sub 4}-type ternary aluminum germanides have been synthesized with Eu, Sr and Ba. • Eu, Sr and Ba cations have no apparent influence on the solubility of Ge. • The Ge atoms substitute Al on one of two framework sites, thereby strengthening the interactions between the cations and the polyanionic framework.

Zhang, Jiliang; Bobev, Svilen, E-mail: bobev@udel.edu

2013-09-15T23:59:59.000Z

445

Quantum Oscillations in the Parent pnictide BaFe2As2 : Itinerant Electrons in the Reconstructed State  

SciTech Connect (OSTI)

We report quantum oscillation measurements that enable the direct observation of the Fermi surface of the low temperature ground state of BaFe{sub 2}As{sub 2}. From these measurements we characterize the low energy excitations, revealing that the Fermi surface is reconstructed in the antiferromagnetic state, but leaving itinerant electrons in its wake. The present measurements are consistent with a conventional band folding picture of the antiferromagnetic ground state, placing important limits on the topology and size of the Fermi surface.

Analytis, J.G.

2010-05-26T23:59:59.000Z

446

Zn-Doping Dependence of Stripe Order in La1.905Ba0.095CuO4  

SciTech Connect (OSTI)

The effect of Zn-doping on the stripe order in La{sub 1.905}Ba{sub 0.095}CuO{sub 4} has been studied by means of x-ray and neutron diffraction as well as magnetization measurements. While 1% Zn leads to an increase of the spin stripe order, it unexpectedly causes a wipe out of the visibility of the charge stripe order. A magnetic field of 10 Tesla applied along the c-axis has no reversing effect on the charge order. We compare this observation with the Zn-doping dependence of the crystal structure, superconductivity, and normal state magnetism.

Hucker, M.; Zimmermann, M.v.; Xu, Z.J.; Wen, J.S.; Gu, G.D.; Tian, W.; Zarestky, J.; Tranquada, J.M.

2011-04-01T23:59:59.000Z

447

Data:Edad1fff-07ba-49cd-9054-e492ad88936d | Open Energy Information  

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448

Data:209b4880-04bc-4f18-9295-39ba0506f055 | Open Energy Information  

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449

Data:6133353e-33af-4276-a282-3daf0dd8a3ba | Open Energy Information  

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AFDC Printable Version Share this resource Send a link to EERE: Alternative Fuels Data Center Home Page to someone by E-mail Share EERE: Alternative Fuels Data Center Home Page on Facebook Tweet about EERE: Alternative Fuels Data Center Home Page on Twitter Bookmark EERE: Alternative Fuels Data Center Home Page on Google Bookmark EERE: Alternative Fuels Data Center Home Page on Office695810186 No revision has been approved for thisbade-2c5cfacaa2ee No revisiondaf0dd8a3ba No revision has been

450

Data:96050660-269e-4d31-a760-777ba27065d9 | Open Energy Information  

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451

Data:7ebeffe5-fb88-45f8-8376-6ba307047cb9 | Open Energy Information  

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452

Data:856cce9a-2857-4c92-afff-3d562710ba6d | Open Energy Information  

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453

Data:3dfe9516-886e-413a-baed-ae8390939e0b | Open Energy Information  

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454

Highly uniform bipolar resistive switching characteristics in TiO{sub 2}/BaTiO{sub 3}/TiO{sub 2} multilayer  

SciTech Connect (OSTI)

Nanoscale multilayer structure TiO{sub 2}/BaTiO{sub 3}/TiO{sub 2} has been fabricated on Pt/Ti/SiO{sub 2}/Si substrate by chemical solution deposition method. Highly uniform bipolar resistive switching (BRS) characteristics have been observed in Pt/TiO{sub 2}/BaTiO{sub 3}/TiO{sub 2}/Pt cells. Analysis of the current-voltage relationship demonstrates that the space-charge-limited current conduction controlled by the localized oxygen vacancies should be important to the resistive switching behavior. X-ray photoelectron spectroscopy results indicated that oxygen vacancies in TiO{sub 2} play a crucial role in the resistive switching phenomenon and the introduced TiO{sub 2}/BaTiO{sub 3} interfaces result in the high uniformity of bipolar resistive switching characteristics.

Ma, W. J.; Zhang, X. Y.; Wang, Ying; Zheng, Yue, E-mail: zhengy35@mail.sysu.edu.cn, E-mail: wangbiao@mail.sysu.edu.cn [State Key Laboratory of Optoelectronic Materials and Technologies, School of Physics and Engineering, Sun Yat-Sen University, 510275 Guangzhou (China) [State Key Laboratory of Optoelectronic Materials and Technologies, School of Physics and Engineering, Sun Yat-Sen University, 510275 Guangzhou (China); Micro and Nano Physics and Mechanics Research Laboratory, School of Physics and Engineering, Sun Yat-Sen University, 510275 Guangzhou (China); Lin, S. P. [Micro and Nano Physics and Mechanics Research Laboratory, School of Physics and Engineering, Sun Yat-Sen University, 510275 Guangzhou (China) [Micro and Nano Physics and Mechanics Research Laboratory, School of Physics and Engineering, Sun Yat-Sen University, 510275 Guangzhou (China); Sino-French Institute of Nuclear Engineering and Technology, Zhuhai Campus, Sun Yat-Sen University, Zhuhai 519082 (China); Luo, J. M.; Wang, B., E-mail: zhengy35@mail.sysu.edu.cn, E-mail: wangbiao@mail.sysu.edu.cn [State Key Laboratory of Optoelectronic Materials and Technologies, School of Physics and Engineering, Sun Yat-Sen University, 510275 Guangzhou (China); Li, Z. X. [Micro and Nano Physics and Mechanics Research Laboratory, School of Physics and Engineering, Sun Yat-Sen University, 510275 Guangzhou (China)] [Micro and Nano Physics and Mechanics Research Laboratory, School of Physics and Engineering, Sun Yat-Sen University, 510275 Guangzhou (China)

2013-12-23T23:59:59.000Z

455

X-ray and neutron powder diffraction studies of Ba(Nd{sub x}Y{sub 2-x})CuO{sub 5}  

SciTech Connect (OSTI)

Ba(R,R'){sub 2}CuO{sub 5} (R,R'=lanthanides and Y) plays an important role as a flux-pinning agent in enhancing the superconducting properties of the Ba{sub 2}(R,R')Cu{sub 3}O{sub 6+x} (R,R'=lanthanides and Y) coated conductors. Using X-ray diffraction and neutron diffraction, we found that the Ba(Nd{sub x}Y{sub 2-x})CuO{sub 5} solid solution adopts two structure types. In the Nd-rich region (1.8{<=}x{<=}2.0), the materials are of brown color (commonly referred to as the 'brown phase'), and the structure is tetragonal with space group I4/mbm (no. 127). In the Y-rich region (0.0{<=}x{<=}1.4), the materials are green (commonly referred to as the 'green phase') and the structure is orthorhombic with space group Pnma (no. 62). A two-phase region (1.4Ba(Nd{sub x}Y{sub 2-x})CuO{sub 5} (isostructural to BaY{sub 2}CuO{sub 5}), are discussed in this paper. - Graphical abstract: Perspective view of the 'green phase' Ba(Nd{sub x}Y{sub 2-x})CuO{sub 5} structure along the b-axis, showing the isolated square pyramids of [CuO{sub 5}] and the trigonal prisms, RO{sub 7}, around the lanthanide sites.

Liu, G. [Ceramics Division, National Institute of Standards and Technology (NIST), Gaithersburg, MD 20899 (United States); Huang, Q. [NIST Center for Neutron Research, Naperville, IL 60563 (United States); Kaduk, J.A. [INEOS Technologies, Naperville, IL 60563 (United States); Yang, Z. [Yunnan Normal University, Kunming 650092 (China); Lucas, C. [Chemistry and Biochemistry Department, University of Maryland, College Park, MD 20742 (United States); Wong-Ng, W. [Ceramics Division, National Institute of Standards and Technology (NIST), Gaithersburg, MD 20899 (United States)], E-mail: Winnie.wong-ng@nist.gov

2008-12-15T23:59:59.000Z

456

Competition between stripe and checkerboard magnetic instabilities in Mn-doped BaFe2As2  

SciTech Connect (OSTI)

The appearance of unconventional superconductivity often requires the suppression of an antiferromagnetic (AFM) ordered state by tuning the chemical composition. In BaFe2As2, the AFM ordered state is driven by Fermi surface nesting, resulting in stripe magnetic ordering with propagation vector Qstripe = (; 0) (in Fe square lattice notation). Co substitution acts as an electron donor that destabilizes the nesting condition,1 leading to suppression of the stripe AFM ordering2 and the appearance of superconductivity.3,4 Mn is nominally the hole-doping counterpart of Co which should also detune the Fermi surface nesting, but it is not a superconductor.5 Here we report that Mn doping does not act solely as a hole donor, but instead introduces strong spin uctuations at a wavevector (; ) that is unrelated to the Fermi surface topology of BaFe2As2. Spin uctuations at (; ) and (; 0) coexist, suggesting the Mn dopants act as local magnetic impurities that polarize neighbouring Fe/Mn spins, potentially disrupting superconductivity.

Pratt, Daniel [Ames Laboratory and Iowa State University; Kim, M. G. [Ames Laboratory and Iowa State University; Ran, S. [Ames Laboratory and Iowa State University; Thaler, A. [Ames Laboratory and Iowa State University; Granroth, Garrett E [ORNL; Marty, Karol J [ORNL; Tian, W. [University of Tennessee, Knoxville (UTK); Zarestky, J. L. [Ames Laboratory and Iowa State University; Lumsden, Mark D [ORNL; Budko, S L [Ames Laboratory and Iowa State University; Canfield, P. C. [Ames Laboratory; Goldman, A. I. [Ames Laboratory and Iowa State University; Mcqueeney, R J [Ames Laboratory and Iowa State University; Tucker, G. S. [Ames Laboratory and Iowa State University

2012-01-01T23:59:59.000Z

457

Magnetically polarized Ir dopant atoms in superconducting Ba(Fe1?xIrx)2As2  

SciTech Connect (OSTI)

We investigate the magnetic polarization of the Ir 5d dopant states in the pnictide superconductor Ba(Fe1?xIrx)2As2 with x=0.027(2) using Ir L3 edge x-ray resonant magnetic scattering (XRMS). Despite the fact that doping partially suppresses the antiferromagnetic transition, we find that magnetic order survives around the Ir dopant sites. The Ir states are magnetically polarized with commensurate stripe-like antiferromagnetic order and long correlations lengths, ?mag>2800 and >850 Ĺ, in the ab plane and along the c axis, respectively, driven by their interaction with the Fe spins. This Ir magnetic order persists up to the Néel transition of the majority Fe spins at TN=74(2) K. At 5 K we find that magnetic order coexists microscopically with superconductivity in Ba(Fe1?xIrx)2As2. The energy dependence of the XRMS through the Ir L3 edge shows a non-Lorentzian line shape, which we explain in terms of interference between Ir resonant scattering and Fe nonresonant magnetic scattering.

Dean, M.P.M.; Kim, M.G.; Kreyssig, A.; Kim, J.W.; Liu, X.; Ryan, P.J.; Thaler, A.; Budko, S.L.; Strassheim, W.; Canfield, P.C.; Hill, J.P.; Goldman, A.I.

2012-04-25T23:59:59.000Z

458

Inclusion property of Cs, Sr, and Ba impurities in LiCl crystal formed by layer-melt crystallization  

SciTech Connect (OSTI)

Pyroprocessing is one of the promising technologies enabling the recycling of spent nuclear fuels from a commercial light water reactor (LWR). In general, pyroprocessing uses dry molten salts as electrolytes. In particular, LiCl waste salt after pyroprocessing contains highly radioactive I/II group fission products mainly composed of Cs, Sr, and Ba impurities. Therefore, it is beneficial to reuse LiCl salt in the pyroprocessing as an electrolyte for economic and environmental issues. Herein, to understand the inclusion property of impurities within LiCl crystal, the physical properties such as lattice parameter change, bulk modulus, and substitution enthalpy of a LiCl crystal having 0-6 at% Cs{sup +} or Ba{sup 2+} impurities under existence of 1 at% Sr{sup 2+} impurity were calculated via the first-principles density functional theory. The substitution enthalpy of LiCl crystals having 1 at% Sr{sup 2+} showed slightly decreased value than those without Sr{sup 2+} impurity. Therefore, through the substitution enthalpy calculation, it is expected that impurities will be incorporated within LiCl crystal as co-existed form rather than as a single component form. (authors)

Choi, Jung-Hoon; Cho, Yung-Zun; Lee, Tae-Kyo; Eun, Hee-Chul; Kim, Jun-Hong; Park, Hwan-Seo; Kim, In-Tae; Park, Geun-Il [Nuclear Fuel Cycle Waste Treatment Research Division, Korea Atomic Energy Research Institute, Daejeon, 305-353 (Korea, Republic of)

2013-07-01T23:59:59.000Z

459

Growth-induced non-planar magnetic anisotropy in FeCoZr-CaF{sub 2} nanogranular films: Structural and magnetic characterization  

SciTech Connect (OSTI)

The relation between nanoscale structure, local atomic order and magnetic properties of (FeCoZr){sub x}(CaF{sub 2}){sub 100?x} (29???x???73 at.?%) granular films is studied as a function of metal/insulator fraction ratio. The films of a thickness of 1–6??m were deposited on Al-foils and glass-ceramic substrates, by ion sputtering of targets of different metal/insulator contents. Structural characterization with X-ray and electron diffraction as well as transmission electron microscopy revealed that the films are composed of isolated nanocrystalline bcc ?-FeCo(Zr) alloy and insulating fcc CaF{sub 2} matrix. They grow in a columnar structure, where elongated metallic nanograins are arranged on top of each other within the columns almost normal to the substrate surface. Mössbauer spectroscopy and magnetometry results indicate that their easy magnetization axes are oriented at an angle of 65°–74° to the surface in films with x between 46 and 74, above the electrical percolation threshold, which is attributed to the growth-induced shape anisotropy. Interatomic distances characteristic for metallic state of ?-FeCo(Zr) nanograins were revealed by X-ray Absorption Spectroscopy. The results show a lack of surface oxidation of the alloy nanograins, so the growth-induced orientation of nanograins in the films cannot be attributed to this effect. The study is among the first to report a growth-induced non-planar magnetic anisotropy in metal/insulator granular films above the percolation threshold and to reveal the origin of it.

Kasiuk, J. V.; Fedotova, J. A. [NC PHEP Belarusian State University, 220040 Minsk (Belarus); Przewoznik, J., E-mail: januszp@agh.edu.pl; Zukrowski, J.; Sikora, M.; Kapusta, Cz. [Department of Solid State Physics, Faculty of Physics and Applied Computer Science, AGH University of Science and Technology, al. Mickiewicza 30, 30-059 Krakow (Poland); Grce, A. [VIN?A Institute of Nuclear Sciences, Belgrade University, P.O. Box 522, 11001 Belgrade (Serbia); Milosavljevi?, M. [VIN?A Institute of Nuclear Sciences, Belgrade University, P.O. Box 522, 11001 Belgrade (Serbia); Advanced Technology Institute, Faculty of Engineering and Physical Sciences, University of Surrey, Guildford, Surrey GU2 7XH (United Kingdom)

2014-07-28T23:59:59.000Z

460

Pion-nucleus elastic scattering on 12C, 40Ca, 90Zr, and 208Pb at 400 and 500 MeV  

E-Print Network [OSTI]

Pion-nucleus elastic scattering at energies above the Delta(1232) resonance is studied using both pi+ and pi- beams on 12C, 40Ca, 90Zr, and 208Pb. The present data provide an opportunity to study the interaction of pions with nuclei at energies where second-order corrections to impulse approximation calculations should be small. The results are compared with other data sets at similar energies, and with four different first-order impulse approximation calculations. Significant disagreement exists between the calculations and the data from this experiment.

George Kahrimanis; George Burleson; C. M. Chen; B. C. Clark; Kalvir Dhuga; D. J. Ernst; J. A. Faucett; H. T. Fortune; S. Hama; Ahmed Hussein; M. F. Jiang; K. W. Johnson; L. Kurth Kerr; Scott Mathews; John McGill; C. Fred Moore; Shaul Mordechai; Christopher L. Morris; John O'Donnell; Mike Snell; Mohini Rawool-Sullivan; L. Ray; Charles Whitley; Allen L. Williams

1997-02-25T23:59:59.000Z

Note: This page contains sample records for the topic "ba ra zr" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


461

Thickness dependence of magnetoelectric response for composites of Pb(Zr{sub 0.52}Ti{sub 0.48})O{sub 3} films on CoFe{sub 2}O{sub 4} ceramic substrates  

SciTech Connect (OSTI)

Using chemical solution spin-coating we grew Pb(Zr{sub 0.52}Ti{sub 0.48})O{sub 3} films of different thicknesses on highly dense CoFe{sub 2}O{sub 4} ceramics. X-ray diffraction revealed no other phases except Pb(Zr{sub 0.52}Ti{sub 0.48})O{sub 3} and CoFe{sub 2}O{sub 4}. In many of these samples we observed typical ferroelectric hysteresis loops, butterfly-shaped piezoelectric strains, and the magnetic-field-dependent magnetostriction. These behaviors caused appreciable magnetoelectric responses based on magnetic-mechanical-electric coupling. Our results indicated that the thickness of the Pb(Zr{sub 0.52}Ti{sub 0.48})O{sub 3} film was important in obtaining strong magnetoelectric coupling.

Wang, Jing, E-mail: wang-jing@nuaa.edu.cn; Zhu, Kongjun [State Key Laboratory of Mechanics and Control of Mechanical Structures, College of Aerospace Engineering, Nanjing University of Aeronautics and Astronautics, Nanjing 210016 (China); Wu, Xia; Deng, Chaoyong [School of Electronics and Information Engineering, Guizhou University, Guiyang 550025 (China); Peng, Renci; Wang, Jianjun [School of Materials Science and Engineering, and State Key Lab of New Ceramics and Fine Processing, Tsinghua University, Beijing 100084 (China)

2014-08-15T23:59:59.000Z

462

Synthesis and nonlinear optical properties of BaTi(BO{sub 3}){sub 2} and Ba{sub 3}Ti{sub 3}O{sub 6}(BO{sub 3}){sub 2} crystals in glasses with high TiO{sub 2} contents  

SciTech Connect (OSTI)

The ternary BaO-TiO{sub 2}-B{sub 2}O{sub 3} glasses containing a large amount of TiO{sub 2} (20-40mol%) are prepared, and their optical basicities ({lambda}), the formation, structural features and second-order optical nonlinearities of BaTi(BO{sub 3}){sub 2} and Ba{sub 3}Ti{sub 3}O{sub 6}(BO{sub 3}){sub 2} crystals are examined to develop new nonlinear optical materials. It is found that the glasses with high TiO{sub 2} contents of 30-40mol% show large optical basicities of {lambda}=0.81-0.87, suggesting the high polarizabity of TiO{sub n} polyhedra (n=4-6) in the glasses. BaTi(BO{sub 3}){sub 2} and Ba{sub 3}Ti{sub 3}O{sub 6}(BO{sub 3}){sub 2} crystals are found to be formed as main crystalline phases in the glasses. It is found that BaTi(BO{sub 3}){sub 2} crystals tend to orient at the surface of crystallized glasses. The new XRD pattern for the Ba{sub 3}Ti{sub 3}O{sub 6}(BO{sub 3}){sub 2} phase is proposed through Rietvelt analysis. The second harmonic intensities of crystallized glasses were found to be 0.8 times as large as {alpha}-quartz powders, i.e., I{sup 2{omega}}(sample)/I{sup 2{omega}}({alpha}-quartz)=0.8, for the sample with BaTi(BO{sub 3}){sub 2} crystals and to be I{sup 2{omega}}(sample)/I{sup 2{omega}}({alpha}-quartz)=68 for the sample with Ba{sub 3}Ti{sub 3}O{sub 6}(BO{sub 3}){sub 2} crystals. The Raman scattering spectra for these two crystalline phases are measured for the first time and their structural features are discussed.

Kosaka, Shinji [Department of Chemistry, Nagaoka University of Technology, 1603-1Kamitomioka-cho, Nagaoka 940-2188 (Japan); Benino, Yasuhiko [Department of Chemistry, Nagaoka University of Technology, 1603-1Kamitomioka-cho, Nagaoka 940-2188 (Japan); Fujiwara, Takumi [Department of Chemistry, Nagaoka University of Technology, 1603-1Kamitomioka-cho, Nagaoka 940-2188 (Japan); Dimitrov, Vesselin [Department of Silicate Technology, University of Chemical Technology and Metallurgy, 8 Kl, Ohridki Blvd., Sofia 1756 (Bulgaria); Komatsu, Takayuki [Department of Chemistry, Nagaoka University of Technology, 1603-1Kamitomioka-cho, Nagaoka 940-2188 (Japan)]. E-mail: komatsu@chem.nagaokaut.ac.jp

2005-06-15T23:59:59.000Z

463

B.A. GEOLOGY CHECKLIST of required courses for major Courses in Natural Sciences: 5-6 courses, 18 credits minimum*  

E-Print Network [OSTI]

B.A. GEOLOGY CHECKLIST of required courses for major Courses in Natural Sciences: 5-6 courses, 18 year, either semester *COURSES MUST BE SELECTED WITH CONSULTATION AND APPROVAL OF A GEOLOGY FACULTY or 4th year, either semester Introductory Geology Courses: 3 courses, 11-12 credits Course Credits When

Massachusetts at Amherst, University of

464

New oxyfluoride glass with high fluorine content and laser patterning of nonlinear optical BaAlBO{sub 3}F{sub 2} single crystal line  

SciTech Connect (OSTI)

A new oxyfluoride glass of 50BaF{sub 2}-25Al{sub 2}O{sub 3}-25B{sub 2}O{sub 3} (mol. %) with a large fraction of fluorine, i.e., F/(F + O) = 0.4, was prepared using a conventional melt-quenching method in order to synthesize new glass-ceramics containing nonlinear optical oxyfluoride crystals. The refractive index at 632.8 nm and ultra-violet cutoff wavelength of the glass were 1.564 and {approx}200 nm, respectively. Eu{sup 3+} ions in the glass showed a high quantum yield of 88% in the photoluminescence spectrum in the visible region. BaAlBO{sub 3}F{sub 2} crystals (size: 50-100 nm) showing second harmonic generations were formed through the crystallization of the glass. Lines consisting of BaAlBO{sub 3}F{sub 2} crystals were patterned successfully on the glass surface by laser irradiations (Yb:YVO{sub 4} laser with a wavelength of 1080 nm, laser power of 1.1 W, scanning speed of 8 {mu}m/s). High resolution transmission electron microscope observations combined with a focused ion beam technique indicate that BaAlBO{sub 3}F{sub 2} crystals are highly oriented just like a single crystal. The present study proposes that the new oxyfluoride glass and glass-ceramics prepared have a high potential for optical device applications.

Shionozaki, K.; Honma, T.; Komatsu, T. [Department of Materials Science and Technology, Nagaoka University of Technology, 1603-1 Kamitomioka-cho, Nagaoka 940-2188 (Japan)

2012-11-01T23:59:59.000Z

465

Effect of strain on tunability in Ba0.60Sr0.40TiO3 thin films on PtSi substrates  

E-Print Network [OSTI]

Effect of strain on tunability in Ba0.60Sr0.40TiO3 thin films on Pt­Si substrates D. M. Potrepkaa, M. W. Cole, and W. D. Nothwang Weapons & Materials Research Directorate, Active Materials Research discussed the effects that postannealing in oxygen can have to overcome limits on oxygen diffusion

Alpay, S. Pamir

466

Political Science Sample 4-5 Year Study Plan for Doctoral Program Current catalog for student with B.A., major field International Relations with minor fields  

E-Print Network [OSTI]

Political Science Sample 4-5 Year Study Plan for Doctoral Program Current catalog for student with B.A., major field International Relations with minor fields Comparative Politics and Political Politics PSC 710r Proseminar in American Politics Year One: Semester 2 PSC 702 Advanced Quantitative

Ahmad, Sajjad

467

COEXTRUSION OF TPU AND BaSO4 FILLED MEDICAL-GRADE TPU Guangyu Lu, Dilhan M. Kalyon, Iskender Yilgor* and Emel Yilgor*  

E-Print Network [OSTI]

the partial cross-section of stripe tubing that was extruded with unfilled TPU (matrix) and 20% BaSO4 filled TPU suspension (stripe) extruded at the same temperature, 210°C. The difference in viscosities between to be 0.64 using the method of Ouchiyama and Tanaka (6, 7). A Harrel single screw coextrusion system

468

Essential Studies Worksheet B.A. with major in Computer Science I. Communication 9 Credits (6 credits writing and 3 credits Oral Communication)  

E-Print Network [OSTI]

Essential Studies Worksheet ­ B.A. with major in Computer Science I. Communication 9 Credits (6 credits writing and 3 credits Oral Communication) Special Emphasis Area: Course: Credits: Semester Special Emphasis Area requirements that may fall outside of Communication, Social Sciences, Arts

Delene, David J.

469

SAMPLE PROGRAMSAMPLE PROGRAMSAMPLE PROGRAMSAMPLE PROGRAM PHILOSOPHY & RELIGION B.A.PHILOSOPHY & RELIGION B.A.PHILOSOPHY & RELIGION B.A.PHILOSOPHY & RELIGION B.A.  

E-Print Network [OSTI]

SAMPLE PROGRAMSAMPLE PROGRAMSAMPLE PROGRAMSAMPLE PROGRAM PHILOSOPHY & RELIGION B.A.PHILOSOPHY & RELIGION B.A.PHILOSOPHY & RELIGION B.A.PHILOSOPHY & RELIGION B.A. 2005: Philosophy & Religion Elective ** 3 MATH 156: College Algebra 3 and MATH 157: Plane Trigonometry 2 or MATH

Gering, Jon C.

470

Greenhouse Heating Checklist1 R. A. Bucklin, P. H. Jones, B.A. Barmby, D. B. McConnell, and R. W. Henley2  

E-Print Network [OSTI]

CIR791 Greenhouse Heating Checklist1 R. A. Bucklin, P. H. Jones, B.A. Barmby, D. B. Mc heating is the union of an appropriate heat source and an efficient heat distribu- tion system. The best greenhouse heat source in the world is useless if the heat cannot be transferred to the plant environment

Watson, Craig A.

471

Degrees Offered: BA, BSME, BSMS, MAE, MME, MMS, Studies in mechanical engineering can lead to specialization in one or more of  

E-Print Network [OSTI]

fluid mechanics and fluid­structure interactions,stochastic mechanics,fluid dynamics,heat transfer1 Degrees Offered: BA, BSME, BSMS, MAE, MME, MMS, MS, PhD Studies in mechanical engineering can lead to specialization in one or more of a diverse set of areas, including mechanics, computational

Richards-Kortum, Rebecca

472

A phenomenological thermodynamic potential for BaTiO3 single crystals Department of Materials Science and Engineering, The Pennsylvania State University, University Park,  

E-Print Network [OSTI]

A phenomenological thermodynamic potential for BaTiO3 single crystals Y. L. Lia Department; accepted 4 August 2005; published online 16 September 2005 A phenomenological thermodynamic potential is to con- struct such a thermodynamic potential. II. PHENOMENOLOGICAL THERMODYNAMIC POTENTIAL

Chen, Long-Qing

473

Oxygen-related dielectric relaxation and leakage characteristics of Pt,,Ba,Sr...TiO3 Pt thin-film capacitors  

E-Print Network [OSTI]

Oxygen-related dielectric relaxation and leakage characteristics of Pt�,,Ba,Sr...TiO3 �Pt thin to the postannealing temperature in oxygen and nitrogen atmosphere. High leakage currents and low-frequency dielectric and subsequently annealed in oxygen at 350 °C. Such results are related to the mobile oxygen ions and oxygen

Cao, Wenwu

474

Light-induced oxygen-ordering dynamics in ,,Y,Pr...Ba2Cu3O6.7: A Raman spectroscopy and Monte Carlo study  

E-Print Network [OSTI]

Light-induced oxygen-ordering dynamics in ,,Y,Pr...Ba2Cu3O6.7: A Raman spectroscopy and Monte Carlo energy barrier which impedes oxygen movement in the plane unless the oxygen atoms are excited by light for oxygen reordering in the chain plane being at the origin of Raman photobleaching and related effects. DOI

Nabben, Reinhard

475

Nesting between hole and electron pockets in Ba(Fe1-xCox)2As2 (x=00.3) observed with angle-resolved photoemission  

E-Print Network [OSTI]

Nesting between hole and electron pockets in Ba(Fe1-xCox)2As2 (x=0­0.3) observed with angle and electrons is smaller than predicted by theory. Finally, we discuss the quality of nesting in the different regions of the phase diagram. The presence of the third hole pocket significantly weakens the nesting at x

Paris-Sud 11, Université de

476

Single Phase Melt Processed Powellite (Ba,Ca) MoO{sub 4} For The Immobilization Of Mo-Rich Nuclear Waste  

SciTech Connect (OSTI)

Crystalline and glass composite materials are currently being investigated for the immobilization of combined High Level Waste (HLW) streams resulting from potential commercial fuel reprocessing scenarios. Several of these potential waste streams contain elevated levels of transition metal elements such as molybdenum (Mo). Molybdenum has limited solubility in typical silicate glasses used for nuclear waste immobilization. Under certain chemical and controlled cooling conditions, a powellite (Ba,Ca)MoO{sub 4} crystalline structure can be formed by reaction with alkaline earth elements. In this study, single phase BaMoO{sub 4} and CaMoO{sub 4} were formed from carbonate and oxide precursors demonstrating the viability of Mo incorporation into glass, crystalline or glass composite materials by a melt and crystallization process. X-ray diffraction, photoluminescence, and Raman spectroscopy indicated a long range ordered crystalline structure. In-situ electron irradiation studies indicated that both CaMoO{sub 4} and BaMoO{sub 4} powellite phases exhibit radiation stability up to 1000 years at anticipated doses with a crystalline to amorphous transition observed after 1 X 10{sup 13} Gy. Aqueous durability determined from product consistency tests (PCT) showed low normalized release rates for Ba, Ca, and Mo (<0.05 g/m{sup 2}).

Brinkman, Kyle [Savannah River Site (SRS), Aiken, SC (United States); Marra, James [Savannah River Site (SRS), Aiken, SC (United States); Fox, Kevin [Savannah River Site (SRS), Aiken, SC (United States); Reppert, Jason [Savannah River Site (SRS), Aiken, SC (United States); Crum, Jarrod [Paci fic Northwest National Laboratory , Richland, WA (United States); Tang, Ming [Los Alamos National Laboratory , Los Alamos, NM (United States)

2012-09-17T23:59:59.000Z

477

X-Ray Storage Luminescence of BaFCl:Eu2+ Single Crystals Nomadics, Inc., 1024 South InnoVation Way, Stillwater, Oklahoma 74074  

E-Print Network [OSTI]

X-Ray Storage Luminescence of BaFCl:Eu2+ Single Crystals Wei Chen* Nomadics, Inc., 1024 South InnoVed: January 18, 2005; In Final Form: March 22, 2005 Temperature behaviors of X-ray luminescence (XL might not be oxidized to Eu3+ upon X-ray or -irradiation. Instead, the color centers, Cl excitons

Chen, Reuven

478

Unconventional Electronic Reconstruction in Undoped (Ba,Sr)Fe2As2 Across the Spin Density Wave Transition  

SciTech Connect (OSTI)

Through a systematic high-resolution angle-resolved photoemission study of the iron pnictide compounds (Ba,Sr)Fe{sub 2}As{sub 2}, we show that the electronic structures of these compounds are significantly reconstructed across the spin density wave transition, which cannot be described by a simple folding scenario of conventional density wave ordering. Moreover, we find that LDA calculations with an incorporated suppressed magnetic moment of 0.5{mu}{sub B} can match well the details in the reconstructed electronic structure, suggesting that the nature of magnetism in the pnictides is more itinerant than local, while the origin of suppressed magnetic moment remains an important issue for future investigations.

Yi, M.

2010-06-02T23:59:59.000Z

479

Coexistence of the spini-density-wave and superconductivity in the Ba1-xKxFe2As2  

SciTech Connect (OSTI)

The relation between the spin-density-wave (SDW) and superconducting order is a central topic in current research on the FeAs-based high T{sub c} superconductors. Conflicting results exist in the LaFeAs(O,F)-class of materials, for which whether the SDW and superconductivity are mutually exclusive or they can coexist has not been settled. Here we show that for the (Ba,K)Fe{sub 2}As{sub 2} system, the SDW and superconductivity can coexist in an extended range of compositions. The availability of single crystalline samples and high value of the energy gaps would make the materials a model system to investigate the high T{sub c} ferropnictide superconductivity.

Bao, Wei [Los Alamos National Laboratory; Chen, H [HEFEI NAT. LAB; Ren, Y [ANL; Qiu, Y [NIST CENTER FOR NEUTRON; Liu, R [HEFEI NAT. LAB.; Wu, G H [HEFEI NAT. LAB; Wu, T [HEFEI NAT. LAB.; Xie, Y L [HEFEI NAT. LAB; Wang, F [HEFEI NAT. LAB.; Huang, Q [NIST CENTER FOR NEUTRON; Chen, X H [HEFEI NAT. LAB

2008-01-01T23:59:59.000Z

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