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Sample records for atmospheric pressure atmospheric

  1. ARM - Measurement - Atmospheric pressure

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    pressure ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Atmospheric pressure The pressure exerted by the atmosphere as a consequence of gravitational attraction exerted upon the "column" of air lying directly above the point in question. Categories Atmospheric State Instruments The above measurement is considered scientifically relevant for the following instruments. Refer to the datastream

  2. ARM - Atmospheric Pressure

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ListAtmospheric Pressure Outreach Home Room News Publications Traditional Knowledge Kiosks Barrow, Alaska Tropical Western Pacific Site Tours Contacts Students Study Hall About ARM Global Warming FAQ Just for Fun Meet our Friends Cool Sites Teachers Teachers' Toolbox Lesson Plans Atmospheric Pressure Humans are subjected to the pressure produced by the weight of the gases of the atmosphere above us. The force exerted on a unit area of surface by the weight of the air above the surface is named

  3. NETL SOFC: Atmospheric Pressure Systems

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Atmospheric Pressure Systems ATMOSPHERIC PRESSURE SYSTEMS (INDUSTRY TEAMS)-This key technology focuses on the design, scaleup, and integration of the SOFC technology, ultimately resulting in atmospheric-pressure modules suitable to serve as the building blocks for distributed-generation, commercial, and utility-scale power systems. Activities include fabrication, testing, post-test analysis of cells; integrating cells into stacks; and the development and validation testing of progressively

  4. Atmospheric-pressure plasma jet

    DOE Patents [OSTI]

    Selwyn, Gary S. (Los Alamos, NM)

    1999-01-01

    Atmospheric-pressure plasma jet. A .gamma.-mode, resonant-cavity plasma discharge that can be operated at atmospheric pressure and near room temperature using 13.56 MHz rf power is described. Unlike plasma torches, the discharge produces a gas-phase effluent no hotter than 250.degree. C. at an applied power of about 300 W, and shows distinct non-thermal characteristics. In the simplest design, two concentric cylindrical electrodes are employed to generate a plasma in the annular region therebetween. A "jet" of long-lived metastable and reactive species that are capable of rapidly cleaning or etching metals and other materials is generated which extends up to 8 in. beyond the open end of the electrodes. Films and coatings may also be removed by these species. Arcing is prevented in the apparatus by using gas mixtures containing He, which limits ionization, by using high flow velocities, and by properly shaping the rf-powered electrode. Because of the atmospheric pressure operation, no ions survive for a sufficiently long distance beyond the active plasma discharge to bombard a workpiece, unlike low-pressure plasma sources and conventional plasma processing methods.

  5. Free Floating Atmospheric Pressure Ball Plasmas

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Free-Floating Atmospheric Pressure Ball Plasmas G. A. Wurden, Z. Wang, C. Ticos Los Alamos National Laboratory L Al NM 87545 USA Los Alamos, NM 87545 USA C. J. v. Wurden Los Alamos...

  6. Atmospheric Pressure Plasma Process And Applications

    SciTech Connect (OSTI)

    Peter C. Kong; Myrtle

    2006-09-01

    This paper provides a general discussion of atmospheric-pressure plasma generation, processes, and applications. There are two distinct categories of atmospheric-pressure plasmas: thermal and nonthermal. Thermal atmospheric-pressure plasmas include those produced in high intensity arcs, plasma torches, or in high intensity, high frequency discharges. Although nonthermal plasmas are at room temperatures, they are extremely effective in producing activated species, e.g., free radicals and excited state atoms. Thus, both thermal and nonthermal atmosphericpressure plasmas are finding applications in a wide variety of industrial processes, e.g. waste destruction, material recovery, extractive metallurgy, powder synthesis, and energy conversion. A brief discussion of recent plasma technology research and development activities at the Idaho National Laboratory is included.

  7. Large area atmospheric-pressure plasma jet

    DOE Patents [OSTI]

    Selwyn, Gary S. (Los Alamos, NM); Henins, Ivars (Los Alamos, NM); Babayan, Steve E. (Huntington Beach, CA); Hicks, Robert F. (Los Angeles, CA)

    2001-01-01

    Large area atmospheric-pressure plasma jet. A plasma discharge that can be operated at atmospheric pressure and near room temperature using 13.56 MHz rf power is described. Unlike plasma torches, the discharge produces a gas-phase effluent no hotter than 250.degree. C. at an applied power of about 300 W, and shows distinct non-thermal characteristics. In the simplest design, two planar, parallel electrodes are employed to generate a plasma in the volume therebetween. A "jet" of long-lived metastable and reactive species that are capable of rapidly cleaning or etching metals and other materials is generated which extends up to 8 in. beyond the open end of the electrodes. Films and coatings may also be removed by these species. Arcing is prevented in the apparatus by using gas mixtures containing He, which limits ionization, by using high flow velocities, and by properly spacing the rf-powered electrode. Because of the atmospheric pressure operation, there is a negligible density of ions surviving for a sufficiently long distance beyond the active plasma discharge to bombard a workpiece, unlike the situation for low-pressure plasma sources and conventional plasma processing methods.

  8. Free Floating Atmospheric Pressure Ball Plasmas | Princeton Plasma...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    7, 2008, 4:15pm to 5:30pm Colloquia MBG Auditorium Free Floating Atmospheric Pressure Ball Plasmas Dr. Glen Wurden Los Alamos National Laboratory Presentation: PDF icon Free...

  9. Atmospheric Pressure Deposition for Electrochromic Windows | Department of

    Office of Environmental Management (EM)

    Energy Atmospheric Pressure Deposition for Electrochromic Windows Atmospheric Pressure Deposition for Electrochromic Windows Emerging Technologies Project for the 2013 Building Technologies Office's Program Peer Review PDF icon emrgtech22_tenent_040413.pdf More Documents & Publications NREL senior scientist, Robert Tenent, Ph.D., with equipment for low cost processing (deposition) of window coatings materials. Dynamic Windows Low-Cost Solutions for Dynamic Window Material CX-003799:

  10. A comparison between characteristics of atmospheric-pressure plasma jets

    Office of Scientific and Technical Information (OSTI)

    sustained by nanosecond- and microsecond-pulse generators in helium (Journal Article) | SciTech Connect A comparison between characteristics of atmospheric-pressure plasma jets sustained by nanosecond- and microsecond-pulse generators in helium Citation Details In-Document Search Title: A comparison between characteristics of atmospheric-pressure plasma jets sustained by nanosecond- and microsecond-pulse generators in helium Power source is an important parameter that can affect the

  11. Atmospheric-pressure guided streamers for liposomal membrane disruption

    SciTech Connect (OSTI)

    Svarnas, P.; Aleiferis, Sp.; Matrali, S. H.; Gazeli, K.; Clement, F.; Antimisiaris, S. G.

    2012-12-24

    The potential to use liposomes (LIPs) as a cellular model in order to study interactions of cold atmospheric-pressure plasma with cells is herein investigated. Cold atmospheric-pressure plasma is formed by a dielectric-barrier discharge reactor. Large multilamellar vesicle liposomes, consisted of phosphatidylcholine and cholesterol, are prepared by the thin film hydration technique, to encapsulate a small hydrophilic dye, i.e., calcein. The plasma-induced release of calcein from liposomes is then used as a measure of liposome membrane integrity and, consequently, interaction between the cold atmospheric plasma and lipid bilayers. Physical mechanisms leading to membrane disruption are suggested, based on the plasma characterization including gas temperature calculation.

  12. Atmospheric pressure helium afterglow discharge detector for gas chromatography

    DOE Patents [OSTI]

    Rice, G.; D'Silva, A.P.; Fassel, V.A.

    1985-04-05

    An apparatus for providing a simple, low-frequency, electrodeless discharge system for atmospheric pressure afterglow generation. A single quartz tube through which a gas mixture is passed is extended beyond a concentric electrode positioned thereabout. A grounding rod is placed directly above the tube outlet to permit optical viewing of the discharge between the electrodes.

  13. Atmospheric pressure helium afterglow discharge detector for gas chromatography

    DOE Patents [OSTI]

    Rice, Gary (Gloucester, VA); D'Silva, Arthur P. (Ames, IA); Fassel, Velmer A. (Ames, IA)

    1986-05-06

    An apparatus for providing a simple, low-frequency electrodeless discharge system for atmospheric pressure afterglow generation. A single quartz tube through which a gas mixture is passed is extended beyond a concentric electrode positioned thereabout. A grounding rod is placed directly above the tube outlet to permit optical viewing of the discharge between the electrodes.

  14. Atmospheric pressure plasma analysis by modulated molecular beam mass spectrometry

    SciTech Connect (OSTI)

    Aranda Gonzalvo, Y.; Whitmore, T.D.; Rees, J.A.; Seymour, D.L.; Stoffels, E.

    2006-05-15

    Fractional number density measurements for a rf plasma 'needle' operating at atmospheric pressure have been obtained using a molecular beam mass spectrometer (MBMS) system designed for diagnostics of atmospheric plasmas. The MBMS system comprises three differentially pumped stages and a mass/energy analyzer and includes an automated beam-to-background measurement facility in the form of a software-controlled chopper mechanism. The automation of the beam modulation allows the neutral components in the plasma to be rapidly and accurately measured using the mass spectrometer by threshold ionization techniques. Data are reported for plasma generated by a needle plasma source operated using a helium/air mixture. In particular, data for the conversion of atmospheric oxygen and nitrogen into nitric oxide are discussed with reference to its significance for medical applications such as disinfecting wounds and dental cavities and for microsurgery.

  15. Cellular membrane collapse by atmospheric-pressure plasma jet

    SciTech Connect (OSTI)

    Kim, Kangil; Sik Yang, Sang E-mail: ssyang@ajou.ac.kr; Jun Ahn, Hak; Lee, Jong-Soo E-mail: ssyang@ajou.ac.kr; Lee, Jae-Hyeok; Kim, Jae-Ho

    2014-01-06

    Cellular membrane dysfunction caused by air plasma in cancer cells has been studied to exploit atmospheric-pressure plasma jets for cancer therapy. Here, we report that plasma jet treatment of cervical cancer HeLa cells increased electrical conductivity across the cellular lipid membrane and caused simultaneous lipid oxidation and cellular membrane collapse. We made this finding by employing a self-manufactured microelectrode chip. Furthermore, increased roughness of the cellular lipid membrane and sequential collapse of the membrane were observed by atomic force microscopy following plasma jet treatment. These results suggest that the cellular membrane catastrophe occurs via coincident altered electrical conductivity, lipid oxidation, and membrane roughening caused by an atmospheric-pressure plasma jet, possibly resulting in cellular vulnerability to reactive species generated from the plasma as well as cytotoxicity to cancer cells.

  16. Stable microwave coaxial cavity plasma system at atmospheric pressure

    SciTech Connect (OSTI)

    Song, H. [Department of Electrical and Computer Engineering, University of Colorado, Colorado Springs, Colorado 80918 (United States); Hong, J. M.; Lee, K. H. [Plasma Systems and Materials (PSM) Inc., Sungnam-Si, Gyonggi-Do 190-1 (Korea, Republic of); Choi, J. J. [Department of Radio Science and Engineering, Kwangwoon University, Nowon-Gu, Seoul 447-1 (Korea, Republic of)

    2008-05-15

    We present a systematic study of the development of a novel atmospheric microwave plasma system for material processing in the pressure range up to 760 torr and the microwave input power up to 6 kW. Atmospheric microwave plasma was reliably produced and sustained by using a cylindrical resonator with the TM{sub 011} cavity mode. The applicator and the microwave cavity, which is a cylindrical resonator, are carefully designed and optimized with the time dependent finite element Maxwell equation solver. The azimuthal apertures are placed at the maximum magnetic field positions between the cavity and the applicator to maximize the coupling efficiency into the microwave plasma at a resonant frequency of 2.45 GHz. The system consists of a magnetron power supply, a circulator, a directional coupler, a three-stub tuner, a dummy load, a coaxial cavity, and a central cavity. Design and construction of the resonant structures and diagnostics of atmospheric plasma using optical experiments are discussed in various ranges of pressure and microwave input power for different types of gases.

  17. Atmospheric Chemistry

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    competencies Atmospheric Chemistry Atmospheric Chemistry is the study of the composition of the atmosphere, the sources and fates of gases and particles in air, and changes induced...

  18. Electrical characteristics and formation mechanism of atmospheric pressure plasma jet

    SciTech Connect (OSTI)

    Liu, Lijuan; Zhang, Yu; Tian, Weijing; Meng, Ying; Ouyang, Jiting

    2014-06-16

    The behavior of atmospheric pressure plasma jet produced by a coplanar dielectric barrier discharge in helium in external electrostatic and magnetic field is investigated. Net negative charges in the plasma jet outside the tube were detected. The deflection of the plume in the external field was observed. The plasma jet is suggested to be formed by the electron beam from the temporal cathode which is accelerated by a longitudinal field induced by the surface charges on the dielectric tube or interface between the helium and ambient air. The helium flow is necessary for the jet formation in the surrounding air.

  19. Atmospheric-pressure plasma decontamination/sterilization chamber

    DOE Patents [OSTI]

    Herrmann, Hans W. (Los Alamos, NM); Selwyn, Gary S. (Los Alamos, NM)

    2001-01-01

    An atmospheric-pressure plasma decontamination/sterilization chamber is described. The apparatus is useful for decontaminating sensitive equipment and materials, such as electronics, optics and national treasures, which have been contaminated with chemical and/or biological warfare agents, such as anthrax, mustard blistering agent, VX nerve gas, and the like. There is currently no acceptable procedure for decontaminating such equipment. The apparatus may also be used for sterilization in the medical and food industries. Items to be decontaminated or sterilized are supported inside the chamber. Reactive gases containing atomic and metastable oxygen species are generated by an atmospheric-pressure plasma discharge in a He/O.sub.2 mixture and directed into the region of these items resulting in chemical reaction between the reactive species and organic substances. This reaction typically kills and/or neutralizes the contamination without damaging most equipment and materials. The plasma gases are recirculated through a closed-loop system to minimize the loss of helium and the possibility of escape of aerosolized harmful substances.

  20. Phenomena of oscillations in atmospheric pressure direct current glow discharges

    SciTech Connect (OSTI)

    Liu, Fu-cheng; Yan, Wen; Wang, De-zhen

    2013-12-15

    Self-sustained oscillations in a dc glow discharge with a semiconductor layer at atmospheric pressure were investigated by means of a one-dimensional fluid model. It is found that the dc glow discharge initially becomes unstable in the subnormal glow region and gives rise to oscillations of plasma parameters. A variety of oscillations with one or more frequencies have been observed under different conditions. The discharge oscillates between the glow discharge mode and the Townsend discharge mode in the oscillations with large amplitude while operates in the subnormal glow discharge mode all the while in the oscillations with small amplitude. Fourier Transform spectra of oscillations reveal the transition mechanism between different oscillations. The effects of semiconductor conductivity on the oscillation frequency of the dominant mode, gas voltage, as well as the discharge current have also been analyzed.

  1. Laser ablation electrospray ionization (LAESI) for atmospheric pressure, in vivo, and imaging mass spectrometry

    DOE Patents [OSTI]

    Vertes, Akos; Nemes, Peter

    2014-08-19

    The field of the invention is atmospheric pressure mass spectrometry (MS), and more specifically a process and apparatus which combine infrared laser ablation with electrospray ionization (ESI).

  2. Laser ablation electrospray ionization (LAESI) for atmospheric pressure, In vivo, and imaging mass spectrometry

    DOE Patents [OSTI]

    Vertes, Akos (Reston, VA); Nemes, Peter (Silver Spring, MD)

    2011-11-29

    The field of the invention is atmospheric pressure mass spectrometry (MS), and more specifically a process and apparatus which combine infrared laser ablation (LA) with electrospray ionization (ESI).

  3. Laser ablation electrospray ionization (LAESI) for atmospheric pressure, in vivo, and imaging mass spectrometry

    DOE Patents [OSTI]

    Vertes, Akos; Nemes, Peter

    2013-07-16

    The field of the invention is atmospheric pressure mass spectrometry (MS), and more specifically a process and apparatus which combine infrared laser ablation with electrospray ionization (ESI).

  4. Pulsed, atmospheric pressure plasma source for emission spectrometry

    DOE Patents [OSTI]

    Duan, Yixiang; Jin, Zhe; Su, Yongxuan

    2004-05-11

    A low-power, plasma source-based, portable molecular light emission generator/detector employing an atmospheric pressure pulsed-plasma for molecular fragmentation and excitation is described. The average power required for the operation of the plasma is between 0.02 W and 5 W. The features of the optical emission spectra obtained with the pulsed plasma source are significantly different from those obtained with direct current (dc) discharge higher power; for example, strong CH emission at 431.2 nm which is only weakly observed with dc plasma sources was observed, and the intense CN emission observed at 383-388 nm using dc plasma sources was weak in most cases. Strong CN emission was only observed using the present apparatus when compounds containing nitrogen, such as aniline were employed as samples. The present apparatus detects dimethylsulfoxide at 200 ppb using helium as the plasma gas by observing the emission band of the CH radical. When coupled with a gas chromatograph for separating components present in a sample to be analyzed, the present invention provides an apparatus for detecting the arrival of a particular component in the sample at the end of the chromatographic column and the identity thereof.

  5. Relation between plasma plume density and gas flow velocity in atmospheric pressure plasma

    SciTech Connect (OSTI)

    Yambe, Kiyoyuki; Taka, Shogo; Ogura, Kazuo [Graduate School of Science and Technology, Niigata University, Niigata 950-2181 (Japan)] [Graduate School of Science and Technology, Niigata University, Niigata 950-2181 (Japan)

    2014-04-15

    We have studied atmospheric pressure plasma generated using a quartz tube, helium gas, and copper foil electrode by applying RF high voltage. The atmospheric pressure plasma in the form of a bullet is released as a plume into the atmosphere. To study the properties of the plasma plume, the plasma plume current is estimated from the difference in currents on the circuit, and the drift velocity is measured using a photodetector. The relation of the plasma plume density n{sub plu}, which is estimated from the current and the drift velocity, and the gas flow velocity v{sub gas} is examined. It is found that the dependence of the density on the gas flow velocity has relations of n{sub plu} ? log(v{sub gas}). However, the plasma plume density in the laminar flow is higher than that in the turbulent flow. Consequently, in the laminar flow, the density increases with increasing the gas flow velocity.

  6. Striated microdischarges in an asymmetric barrier discharge in argon at atmospheric pressure

    SciTech Connect (OSTI)

    Hoder, Tomas; Loffhagen, Detlef; Wilke, Christian; Grosch, Helge; Schaefer, Jan; Weltmann, Klaus-Dieter; Brandenburg, Ronny

    2011-10-15

    The investigation of striated microdischarges in barrier discharges in argon at atmospheric pressure is reported. Microdischarges were investigated by means of electrical measurements correlated with intensified CCD camera imaging. The scaling law theory known from low-pressure glow discharge diagnostics was applied in order to describe and explain this phenomenon. The investigated microdischarge is characterized as a transient atmospheric-pressure glow discharge with a stratified column. It can be described by similarity parameters i/r{approx_equal}0.13 A/cm, pr{approx_equal}5 Torr cm, and 3<{lambda}/r<5 with the current i, pressure p, interval of subsequent striations {lambda}, and radius of the plasma channel r. An attempt to describe the mechanism of creation of a striated structure is given, based on an established model of the spatial electron relaxation.

  7. Sulfur capture by oil shale ashes under atmospheric and pressurized FBC conditions

    SciTech Connect (OSTI)

    Yrjas, K.P.; Hupa, M. [Aabo Akademi Univ., Turku (Finland). Dept. of Chemical Engineering; Kuelaots, I.; Ots, A. [Tallinn Technical Univ. (Estonia). Thermal Engineering Dept.

    1995-12-31

    When oil shale contains large quantities of limestone, a significant auto-absorption of sulfur is possible under suitable conditions. The sulfur capture by oil shale ashes has been studied using a pressurized thermogravimetric apparatus. The chosen experimental conditions were typical for atmospheric and pressurized fluidized bed combustion. The Ca/S molar ratios in the two oil shales studied were 8 (Estonian) and 10 (Israeli). The samples were first burned in a gas atmosphere containing O{sub 2} and N{sub 2} (and CO{sub 2} if pressurized). After the combustion step, SO{sub 2} was added and sulfation started. The results with the oil shales were compared to those obtained with an oil shale cyclone ash from the Narva power plant in Estonia. In general, the results from the sulfur capture experiments under both atmospheric and pressurized conditions showed that the oil shale cannot only capture its own sulfur but also significant amounts of additional sulfur of another fuel if the fuels are mixed together. For example from the runs at atmospheric pressure, the conversion of CaO to CaSO{sub 4} was about 70% for Israeli oil shale and about 55% for Estonian oil shale (850 C). For the cyclone ash the corresponding conversion was about 20%. In comparison it could be mentioned that under the same conditions the conversions of natural limestones are about 30%. The reason the cyclone ash was a poor sulfur absorbent was probably due to its temperature history. In Narva the oil shale was burned at a significantly higher temperature (1,400 C) than was used in the experiments (750 C and 850 C). This caused the ash to sinter and the reactive surface area of the cyclone ash was therefore decreased.

  8. Numerical simulation of torus breakdown to chaos in an atmospheric-pressure dielectric barrier discharge

    SciTech Connect (OSTI)

    Zhang, J.; Wang, Y. H.; Wang, D. Z. [Key Laboratory of Materials Modification by Laser, Electron, and Ion Beams, School of Physics and Optoelectronic Technology, Dalian University of Technology, Dalian 116024 (China)] [Key Laboratory of Materials Modification by Laser, Electron, and Ion Beams, School of Physics and Optoelectronic Technology, Dalian University of Technology, Dalian 116024 (China)

    2013-08-15

    Understanding the routes to chaos occurring in atmospheric-pressure dielectric barrier discharge systems by changing controlling parameters is very important to predict and control the dynamical behaviors. In this paper, a route of a quasiperiodic torus to chaos via the strange nonchaotic attractor is observed in an atmospheric-pressure dielectric barrier discharge driven by triangle-wave voltage. By increasing the driving frequency, the discharge system first bifurcates to a quasiperiodic torus from a stable single periodic state, and then torus and phase-locking periodic state appear and disappear alternately. In the meantime, the torus becomes increasingly wrinkling and stretching, and gradually approaches a fractal structure with the nonpositive largest Lyapunov exponent, i.e., a strange nonchaotic attractor. After that, the discharge system enters into chaotic state. If the driving frequency is further increased, another well known route of period-doubling bifurcation to chaos is also observed.

  9. Atmospheric-pressure air microplasma jets in aqueous media for the inactivation of Pseudomonas fluorescens cells

    SciTech Connect (OSTI)

    Zhang, Xianhui; Yang, Si-ze [Fujian Provincial Key Laboratory of Plasma and Magnetic Resonance, School of Physics and Mechanical and Electrical Engineering, Xiamen University, Xiamen, Fujian 361005 (China)] [Fujian Provincial Key Laboratory of Plasma and Magnetic Resonance, School of Physics and Mechanical and Electrical Engineering, Xiamen University, Xiamen, Fujian 361005 (China); Liu, Dongping [Fujian Provincial Key Laboratory of Plasma and Magnetic Resonance, School of Physics and Mechanical and Electrical Engineering, Xiamen University, Xiamen, Fujian 361005 (China) [Fujian Provincial Key Laboratory of Plasma and Magnetic Resonance, School of Physics and Mechanical and Electrical Engineering, Xiamen University, Xiamen, Fujian 361005 (China); School of Physics and Materials Engineering, Dalian Nationalities University, Dalian 116600 (China); Song, Ying [School of Physics and Materials Engineering, Dalian Nationalities University, Dalian 116600 (China) [School of Physics and Materials Engineering, Dalian Nationalities University, Dalian 116600 (China); School of Physics and Optoelectronic Technology, Dalian University of Technology, Dalian 116023 (China); Sun, Yue [School of Physics, Changchun University of Science and Technology, Changchun 130022 (China)] [School of Physics, Changchun University of Science and Technology, Changchun 130022 (China)

    2013-05-15

    The hollow fiber-based cold air microplasma jet array running at atmospheric pressure has been designed to inactivate Pseudomonas fluorescens (P. fluorescens) cells in vitro in aqueous media. The influences of electrode configurations, air flow rate, and applied voltage on the discharge characteristics of the single microplasma jet operating in aqueous media are presented, and the bactericidal efficiency of the hollow fibers-based and large-volume microplasma jet array is reported. Optical emission spectroscopy is utilized to identify excited species during the antibacterial testing of plasma in solutions. These well-aligned and rather stable air microplasma jets containing a variety of short-lived species, such as OH and O radicals and charged particles, are in direct contact with aqueous media and are very effective in killing P. fluorescens cells in aqueous media. This design shows its potential application for atmospheric pressure air plasma inactivation of bacteria cells in aqueous media.

  10. Free radicals induced in aqueous solution by non-contact atmospheric-pressure cold plasma

    SciTech Connect (OSTI)

    Tani, Atsushi; Fukui, Satoshi; Ono, Yusuke; Kitano, Katsuhisa; Ikawa, Satoshi

    2012-06-18

    To understand plasma-induced chemical processing in liquids, we investigated the formation of free radicals in aqueous solution exposed to different types of non-contact atmospheric-pressure helium plasma using the spin-trapping technique. Both hydroxyl radical (OH{center_dot}) and superoxide anion radical (O{sub 2}{sup -}{center_dot}) adducts were observed when neutral oxygen gas was additionally supplied to the plasma. In particular, O{sub 2}{sup -}{center_dot} can be dominantly induced in the solution via oxygen flow into the afterglow gas of helium plasma. This type of plasma treatment can potentially be used in medical applications to control infectious diseases, because the O{sub 2}{sup -}{center_dot} is crucial for sterilization of liquids via atmospheric-pressure plasma.

  11. Role of ambient dielectric in propagation of Ar atmospheric pressure nonequilibrium plasma jets

    SciTech Connect (OSTI)

    Song, Jian; Wang, Youyin; Yu, Daren; Tang, Jingfeng Wei, Liqiu; Ren, Chunsheng

    2015-05-15

    A single-electrode atmospheric pressure nonequilibrium plasma jet surrounded with different ambient dielectrics is investigated driven by AC power supply. Another three ambient dielectrics, distilled water, ethanol, and carbon tetrachloride, are adopted to compare with air. By examining electrical and optical characteristics, it was found that the molecular polarity of ambient dielectrics had its significant effect on the propagation of atmospheric pressure nonequilibrium plasma jets. When the polarization of molecules was enhanced, the discharge current and the bullet velocity were also increased. For nonpolar dielectric of carbon tetrachloride, this was mainly resulted from the electron polarization in the built-in electric field. For polar dielectrics of ethanol and distilled water, in addition to the electron polarization, orientation polarization was the main cause for the further increase in discharge current and bullet velocity.

  12. White light emission from silicon oxycarbide films prepared by using atmospheric pressure microplasma jet

    SciTech Connect (OSTI)

    Ding Yi; Shirai, Hajime

    2009-02-15

    An atmospheric pressure microplasma jet was employed as a deposition tool to fabricate silicon oxycarbide films from tetraethoxysilane-argon (Ar) mixture gas at room temperature. Resultant films exhibit intense visible emission under a 325 nm excitation which appears white to naked eyes in the range from {approx}1.75 to {approx}3.5 eV at room temperature. The origin of photoluminescence is attributed to the electron-hole pair recombination through neutral oxygen vacancies (NOVs) in the film. The density of NOV defects was found in the range from 3.48x10{sup 15} to 2.23x10{sup 16} cm{sup -3}. The photoluminescence quantum efficiencies were estimated to be 1.48%-4.15%. Present experiment results demonstrate that the silicon oxycarbide films prepared by using atmospheric pressure microplasma jet would be a competitive candidate for the development of white light emission devices.

  13. Energy density dependence of hydrogen combustion efficiency in atmospheric pressure microwave plasma

    SciTech Connect (OSTI)

    Yoshida, T.; Ezumi, N.; Sawada, K.; Tanaka, Y.; Tanaka, M.; Nishimura, K.

    2015-03-15

    The recovery of tritium in nuclear fusion plants is a key issue for safety. So far, the oxidation procedure using an atmospheric pressure plasma is expected to be part of the recovery method. In this study, in order to clarify the mechanism of hydrogen oxidation by plasma chemistry, we have investigated the dependence of hydrogen combustion efficiency on gas flow rate and input power in the atmospheric pressure microwave plasma. It has been found that the combustion efficiency depends on energy density of absorbed microwave power. Hence, the energy density is considered as a key parameter for combustion processes. Also neutral gas temperatures inside and outside the plasma were measured by an optical emission spectroscopy method and thermocouple. The result shows that the neutral gas temperature in the plasma is much higher than the outside temperature of plasma. The high neutral gas temperature may affect the combustion reaction. (authors)

  14. Processing materials inside an atmospheric-pressure radiofrequency nonthermal plasma discharge

    DOE Patents [OSTI]

    Selwyn, Gary S.; Henins, Ivars; Park, Jaeyoung; Herrmann, Hans W.

    2006-04-11

    Apparatus for the processing of materials involving placing a material either placed between an radio-frequency electrode and a ground electrode, or which is itself one of the electrodes. This is done in atmospheric pressure conditions. The apparatus effectively etches or cleans substrates, such as silicon wafers, or provides cleaning of spools and drums, and uses a gas containing an inert gas and a chemically reactive gas.

  15. ARM ARM Atmospheric Radiation Measurement Atmospheric Radiation...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Tom Ackerman Chief Scientist Tom Ackerman Chief Scientist ARM ARM Atmospheric Radiation Measurement Atmospheric Radiation Measurement Pacific Northwest National Laboratory Pacific ...

  16. Atmospheric pressure plasma jet with high-voltage power supply based on piezoelectric transformer

    SciTech Connect (OSTI)

    Babij, Micha?; Kowalski, Zbigniew W. Nitsch, Karol; Gotszalk, Teodor; Silberring, Jerzy

    2014-05-15

    The dielectric barrier discharge plasma jet, an example of the nonthermal atmospheric pressure plasma jet (APPJ), generates low-temperature plasmas that are suitable for the atomization of volatile species and can also be served as an ionization source for ambient mass and ion mobility spectrometry. A new design of APPJ for mass spectrometry has been built in our group. In these plasma sources magnetic transformers (MTs) and inductors are typically used in power supplies but they present several drawbacks that are even more evident when dealing with high-voltage normally used in APPJs. To overcome these disadvantages, high frequency generators with the absence of MT are proposed in the literature. However, in the case of miniaturized APPJs these conventional power converters, built of ferromagnetic cores and inductors or by means of LC resonant tank circuits, are not so useful as piezoelectric transformer (PT) based power converters due to bulky components and small efficiency. We made and examined a novel atmospheric pressure plasma jet with PT supplier served as ionization source for ambient mass spectrometry, and especially mobile spectrometry where miniaturization, integration of components, and clean plasma are required. The objective of this paper is to describe the concept, design, and implementation of this miniaturized piezoelectric transformer-based atmospheric pressure plasma jet.

  17. Production of stable, non-thermal atmospheric pressure rf capacitive plasmas using gases other than helium or neon

    DOE Patents [OSTI]

    Park, Jaeyoung; Henins, Ivars

    2005-06-21

    The present invention enables the production of stable, steady state, non-thermal atmospheric pressure rf capacitive .alpha.-mode plasmas using gases other than helium and neon. In particular, the current invention generates and maintains stable, steady-state, non-thermal atmospheric pressure rf .alpha.-mode plasmas using pure argon or argon with reactive gas mixtures, pure oxygen or air. By replacing rare and expensive helium with more readily available gases, this invention makes it more economical to use atmospheric pressure rf .alpha.-mode plasmas for various materials processing applications.

  18. ARM - Measurement - Atmospheric moisture

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    moisture ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Atmospheric moisture The moisture content of the air as indicated by several measurements including relative humidity, specific humidity, dewpoint, vapor pressure, water vapor mixing ratio, and water vapor density; note that precipitable water is a separate type. Categories Atmospheric State Instruments The above measurement is considered

  19. Spectroscopic characterization of rovibrational temperatures in atmospheric pressure He/CH{sub 4} plasmas

    SciTech Connect (OSTI)

    Moon, Se Youn; Kim, D. B.; Gweon, B.; Choe, W.

    2008-10-15

    Atmospheric pressure of helium (He) and methane (CH{sub 4}) mixture discharge characteristics are investigated using emission spectroscopic methods. Plasmas are produced in a radio frequency capacitively coupled device at atmospheric pressure in the ambient air. Without the CH{sub 4} gas introduced in the plasma, the emission spectrum exhibits typical helium discharge characteristics showing helium atomic lines with nitrogen molecular bands and oxygen atomic lines resulting from air impurities. Addition of a small amount (<1%) of CH{sub 4} to the supplied He results in the emission of CN (B{sup 2}{sigma}{sup +}-X{sup 2}{sigma}{sup +}: violet system) and CH (A{sup 2}{delta}-X{sup 2} product : 430 nm system) molecular bands. Analyzing the CN and CH diatomic molecular emission spectra, the vibrational temperature (T{sub vib}) and rotational temperature (T{sub rot}) are simultaneously obtained. As input power levels are raised from 20 W to 200 W, T{sub vib} and T{sub rot} are increased from 4230 K to 6310 K and from 340 K to 500 K, respectively. On the contrary, increasing the CH{sub 4} amount brings about the decrease of both temperatures because CH{sub 4} is harder to ionize than He. The emission intensities of CN and CH radicals, which are important in plasma processing, are also changed along with the temperature variation. From the results, the atmospheric pressure plasma shows strong nonequilibrium discharge properties, which may be effectively utilized for thermal damage free material treatments.

  20. An Open Port Sampling Interface for Liquid Introduction Atmospheric Pressure Ionization Mass Spectrometry

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Van Berkel, Gary J.; Kertesz, Vilmos

    2015-08-25

    RATIONALE: A simple method to introduce unprocessed samples into a solvent for rapid characterization by liquid introduction atmospheric pressure ionization mass spectrometry has been lacking. The continuous flow, self-cleaning open port sampling interface introduced here fills this void. METHODS: The open port sampling interface used a vertically aligned, co-axial tube arrangement enabling solvent delivery to the sampling end of the device through the tubing annulus and solvent aspiration down the center tube and into the mass spectrometer ionization source via the commercial APCI emitter probe. The solvent delivery rate to the interface was set to exceed the aspiration rate creatingmore » a continuous sampling interface along with a constant, self-cleaning spillover of solvent from the top of the probe. RESULTS: Using the open port sampling interface with positive ion mode APCI and a hybrid quadrupole time of flight mass spectrometer, rapid, direct sampling and analysis possibilities are exemplified with plastics, ballpoint and felt tip ink pens, skin, and vegetable oils. These results demonstrated that the open port sampling interface could be used as a simple, versatile and self-cleaning system to rapidly introduce multiple types of unprocessed, sometimes highly concentrated and complex, samples into a solvent flow stream for subsequent ionization and analysis by mass spectrometry. The basic setup presented here could be incorporated with any self-aspirating liquid introduction ionization source (e.g., ESI, APCI, APPI, ICP, etc.) or any type of atmospheric pressure sampling ready mass spectrometer system. CONCLUSIONS: The open port sampling interface provides a means to introduce and quickly analyze unprocessed solid or liquid samples with liquid introduction atmospheric pressure ionization source without fear of sampling interface or ionization source contamination.« less

  1. Soot surface temperature measurements in pure and diluted flames at atmospheric and elevated pressures

    SciTech Connect (OSTI)

    Berry Yelverton, T.L.; Roberts, W.L. [Department of Mechanical and Aerospace Engineering, Campus Box 7910, North Carolina State University, 3211 Broughton Hall, Raleigh, NC 27695 (United States)

    2008-10-15

    Soot surface temperature was measured in laminar jet diffusion flames at atmospheric and elevated pressures. The soot surface temperature was measured in flames at one, two, four, and eight atmospheres with both pure and diluted (using helium, argon, nitrogen, or carbon dioxide individually) ethylene fuels with a calibrated two-color soot pyrometry technique. These two dimensional temperature profiles of the soot aid in the analysis and understanding of soot production, leading to possible methods for reducing soot emission. Each flame investigated was at its smoke point, i.e., at the fuel flow rate where the overall soot production and oxidation rates are equal. The smoke point was chosen because it was desirable to have similar soot loadings for each flame. A second set of measurements were also taken where the fuel flow rate was held constant to compare with earlier work. These measurements show that overall flame temperature decreases with increasing pressure, with increasing pressure the position of peak temperature shifts to the tip of the flame, and the temperatures measured were approximately 10% lower than those calculated assuming equilibrium and neglecting radiation. (author)

  2. Role of secondary emission on discharge dynamics in an atmospheric pressure dielectric barrier discharge

    SciTech Connect (OSTI)

    Tay, W. H.; Kausik, S. S.; Yap, S. L.; Wong, C. S.

    2014-04-15

    The discharge dynamics in an atmospheric pressure dielectric barrier discharge (DBD) is studied in a DBD reactor consisting of a pair of stainless steel parallel plate electrodes. The DBD discharge has been generated by a 50?Hz ac high voltage power source. The high-speed intensified charge coupled device camera is used to capture the images of filaments occurring in the discharge gap. It is observed that frequent synchronous breakdown of micro discharges occurs across the discharge gap in the case of negative current pulse. The experimental results reveal that secondary emissions from the dielectric surface play a key role in the synchronous breakdown of plasma filaments.

  3. Plasma stability control using dielectric barriers in radio-frequency atmospheric pressure glow discharges

    SciTech Connect (OSTI)

    Shi, J. J.; Liu, D. W.; Kong, M. G.

    2006-08-21

    It is widely accepted that electrode insulation is unnecessary for generating radio-frequency (rf) atmospheric pressure glow discharges (APGDs). It is also known that rf APGDs with large discharge current are susceptible to the glow-to-arc transition. In this letter, a computational study is presented to demonstrate that dielectric barriers provide an effective control over unlimited current growth and allow rf APGDs to be operated at very high current densities with little danger of the glow-to-arc transition. Characteristics of electrode sheaths are used to show that the stability control is achieved by forcing the plasma-containing electrode unit to acquire positive differential conductivity.

  4. Pulsed microwave discharge in a capillary filled with atmospheric-pressure gas

    SciTech Connect (OSTI)

    Gritsinin, S. I.; Gushchin, P. A.; Davydov, A. M.; Ivanov, E. V.; Kossyi, I. A.

    2013-08-15

    A pulsed microwave coaxial capillary plasma source generating a thin plasma filament along the capillary axis in an atmospheric-pressure argon flow is described. The dynamics of filament formation is studied, and the parameters of the gas and plasma in the contraction region are determined. A physical model of discharge formation and propagation is proposed. The model is based on the assumption that, under the conditions in which the electric fields is substantially below the threshold value, the discharge operates in a specific form known as a self-sustained-non-self-sustained (SNS) microwave discharge.

  5. Development of a stable dielectric-barrier discharge enhanced laminar plasma jet generated at atmospheric pressure

    SciTech Connect (OSTI)

    Tang Jie; Li Shibo; Zhao Wei; Wang Yishan [State Key Laboratory of Transient Optics and Photonics, Xi'an Institute of Optics and Precision Mechanics of CAS, Xi'an (China); Duan Yixiang [State Key Laboratory of Transient Optics and Photonics, Xi'an Institute of Optics and Precision Mechanics of CAS, Xi'an (China); Research Center of Analytical Instrumentation, Sichuan University, Chengdu (China)

    2012-06-18

    A stable nonthermal laminar atmospheric-pressure plasma source equipped with dielectric-barrier discharge was developed to realize more efficient plasma generation, with the total energy consumption reduced to nearly 25% of the original. Temperature and emission spectra monitoring indicates that this plasma is uniform in the lateral direction of the jet core region. It is also found that this plasma contains not only abundant excited argon atoms but also sufficient excited N{sub 2} and OH. This is mainly resulted from the escape of abundant electrons from the exit, due to the sharp decrease of sustaining voltage and the coupling between ions and electrons.

  6. Selective killing of ovarian cancer cells through induction of apoptosis by nonequilibrium atmospheric pressure plasma

    SciTech Connect (OSTI)

    Iseki, Sachiko; Tanaka, Hiromasa; Kondo, Hiroki; Hori, Masaru; Nakamura, Kae; Hayashi, Moemi; Kajiyama, Hiroaki; Kikkawa, Fumitaka; Kano, Hiroyuki

    2012-03-12

    Two independent ovarian cancer cell lines and fibroblast controls were treated with nonequilibrium atmospheric pressure plasma (NEAPP). Most ovarian cancer cells were detached from the culture dish by continuous plasma treatment to a single spot on the dish. Next, the plasma source was applied over the whole dish using a robot arm. In vitro cell proliferation assays showed that plasma treatments significantly decreased proliferation rates of ovarian cancer cells compared to fibroblast cells. Flow cytometry and western blot analysis showed that plasma treatment of ovarian cancer cells induced apoptosis. NEAPP could be a promising tool for therapy for ovarian cancers.

  7. Atmospheric optical calibration system

    DOE Patents [OSTI]

    Hulstrom, Roland L. (Bloomfield, CO); Cannon, Theodore W. (Golden, CO)

    1988-01-01

    An atmospheric optical calibration system is provided to compare actual atmospheric optical conditions to standard atmospheric optical conditions on the basis of aerosol optical depth, relative air mass, and diffuse horizontal skylight to global horizontal photon flux ratio. An indicator can show the extent to which the actual conditions vary from standard conditions. Aerosol scattering and absorption properties, diffuse horizontal skylight to global horizontal photon flux ratio, and precipitable water vapor determined on a real-time basis for optical and pressure measurements are also used to generate a computer spectral model and for correcting actual performance response of a photovoltaic device to standard atmospheric optical condition response on a real-time basis as the device is being tested in actual outdoor conditions.

  8. Atmospheric optical calibration system

    DOE Patents [OSTI]

    Hulstrom, R.L.; Cannon, T.W.

    1988-10-25

    An atmospheric optical calibration system is provided to compare actual atmospheric optical conditions to standard atmospheric optical conditions on the basis of aerosol optical depth, relative air mass, and diffuse horizontal skylight to global horizontal photon flux ratio. An indicator can show the extent to which the actual conditions vary from standard conditions. Aerosol scattering and absorption properties, diffuse horizontal skylight to global horizontal photon flux ratio, and precipitable water vapor determined on a real-time basis for optical and pressure measurements are also used to generate a computer spectral model and for correcting actual performance response of a photovoltaic device to standard atmospheric optical condition response on a real-time basis as the device is being tested in actual outdoor conditions. 7 figs.

  9. Atmospheric Radiation Measurement Program

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Tom Ackerman Chief Scientist Tom Ackerman Chief Scientist ARM ARM Atmospheric Radiation Measurement Atmospheric Radiation Measurement WARNING WARNING Today is April 1 But that ...

  10. Influence of oxygen traces on an atmospheric-pressure radio-frequency capacitive argon plasma discharge

    SciTech Connect (OSTI)

    Li Shouzhe; Wu Qi; Yan Wen; Wang Dezhen [Key Laboratory of Materials Modification by Laser, Ion, Electron Beams, Dalian University of Technology, Ministry of Education, Dalian 116024 (China) and School of Physics and Optoelectronic Technology, Dalian University of Technology, Dalian 116024 (China); Uhm, Han S. [Kwangwoon Academy of Advanced Studies, Kwangwoon University, 447-1 Wolgye-dong, Nowon-gu, Seoul 137-701 (Korea, Republic of)

    2011-10-15

    An atmospheric-pressure capacitive discharge source driven by radio-frequency power supply at 13.56 MHz has been developed experimentally that is capable of producing a homogeneous and cold glow discharge in O{sub 2}/Ar. With respect to the influence of oxygen component when diluted into argon plasma discharge on the discharge characteristics, the measurements of the electrical parameters (impedance, phase angle, resistance, and reactance) are made systematically and the densities of the metastable and resonant state of argon are determined by means of optical emission spectroscopy (OES). It is shown that the admixture of oxygen into argon plasma not only changes the electric characteristics but also alters the optical emission spectra greatly due to strong interaction between the oxygen content and the argon in the plasma environment.

  11. Apparatus and method for atmospheric pressure reactive atom plasma processing for shaping of damage free surfaces

    DOE Patents [OSTI]

    Carr; Jeffrey W. (Livermore, CA)

    2009-03-31

    Fabrication apparatus and methods are disclosed for shaping and finishing difficult materials with no subsurface damage. The apparatus and methods use an atmospheric pressure mixed gas plasma discharge as a sub-aperture polisher of, for example, fused silica and single crystal silicon, silicon carbide and other materials. In one example, workpiece material is removed at the atomic level through reaction with fluorine atoms. In this example, these reactive species are produced by a noble gas plasma from trace constituent fluorocarbons or other fluorine containing gases added to the host argon matrix. The products of the reaction are gas phase compounds that flow from the surface of the workpiece, exposing fresh material to the etchant without condensation and redeposition on the newly created surface. The discharge provides a stable and predictable distribution of reactive species permitting the generation of a predetermined surface by translating the plasma across the workpiece along a calculated path.

  12. Electron density and temperature measurement by continuum radiation emitted from weakly ionized atmospheric pressure plasmas

    SciTech Connect (OSTI)

    Park, Sanghoo; Choe, Wonho, E-mail: wchoe@kaist.ac.kr [Department of Physics, Korea Advanced Institute of Science and Technology, 291 Daehak-ro, Yuseong-gu, Daejeon 305-701 (Korea, Republic of); Youn Moon, Se [High-enthalpy Plasma Research Center, Chonbuk National University, 567 Baekje-daero, Deokjin-gu, Jeonju 561-756 (Korea, Republic of); Park, Jaeyoung [5771 La Jolla Corona Drive, La Jolla, CA 92037 (United States)

    2014-02-24

    The electron-atom neutral bremsstrahlung continuum radiation emitted from weakly ionized plasmas is investigated for electron density and temperature diagnostics. The continuum spectrum in 4501000?nm emitted from the argon atmospheric pressure plasma is found to be in excellent agreement with the neutral bremsstrahlung formula with the electron-atom momentum transfer cross-section given by Popovi?. In 280450?nm, however, a large discrepancy between the measured and the neutral bremsstrahlung emissivities is observed. We find that without accounting for the radiative H{sub 2} dissociation continuum, the temperature, and density measurements would be largely wrong, so that it should be taken into account for accurate measurement.

  13. Statistical modelling of discharge behavior of atmospheric pressure dielectric barrier discharge

    SciTech Connect (OSTI)

    Tay, W. H.; Kausik, S. S.; Wong, C. S. Yap, S. L.; Muniandy, S. V.

    2014-11-15

    In this work, stochastic behavior of atmospheric pressure dielectric barrier discharge (DBD) has been investigated. The experiment is performed in a DBD reactor consisting of a pair of stainless steel parallel plate electrodes powered by a 50?Hz ac high voltage source. Current pulse amplitude distributions for different space gaps and the time separation between consecutive current pulses are studied. A probability distribution function is proposed to predict the experimental distribution function for the current pulse amplitudes and the occurrence of the transition regime of the pulse distribution. Breakdown voltage at different positions on the dielectric surface is suggested to be stochastic in nature. The simulated results based on the proposed distribution function agreed well with the experimental results and able to predict the regime of transition voltage. This model would be useful for the understanding of stochastic behaviors of DBD and the design of DBD device for effective operation and applications.

  14. Role of metastable atoms in the propagation of atmospheric pressure dielectric barrier discharge jets

    SciTech Connect (OSTI)

    Li Qing; Zhu Ximing; Li Jiangtao; Pu Yikang [Department of Engineering Physics, Tsinghua University, Beijing 100084 (China)

    2010-02-15

    In the experiment of plasma jets generated in a tube dielectric barrier discharge configuration, three distinguishable modes, namely, laminar, transition, and turbulent jet modes, have been identified. Flows of helium, neon, and argon gases shared the hydrodynamic law when their plasma jets spraying into ambient air of atmospheric pressure and room temperature. Aiming to reveal the basic processes, we propose that plasma jet length is mainly determined by reactions involving metastable atoms. These processes are responsible for the variation in plasma jet length versus gas flow rate and working gas species. To investigate this proposal in detail, we have obtained three significant experimental results, i.e., (1) the plasma jet lengths of helium, neon, and argon are different; (2) the plasma jet length of krypton slightly changes with gas flow rate, with three modes indistinguishable; and (3) there are large differences between optical emission spectra of helium, neon, argon, and krypton flow gases. These observations are in good agreement with our proposal.

  15. Effect of dielectric wall temperature on plasma plume in an argon atmospheric pressure discharge

    SciTech Connect (OSTI)

    Song, Jian; Huo, Yuxin; Wang, Youyin; Yu, Daren, E-mail: yudaren@hit.edu.cn [School of Energy Science and Engineering, Harbin Institute of Technology, Harbin 150001 (China); Tang, Jingfeng; Wei, Liqiu [Academy of Fundamental and Interdisciplinary Sciences, Harbin Institute of Technology, Harbin 150001 (China)

    2014-10-15

    In this letter, the effect of the dielectric wall temperature on the length and volume of an atmospheric pressure plasma jet (APPJ) is investigated using a single-electrode configuration driven with an AC power supply. To distinguish the APPJ status from the argon flow rate, the three modes, laminar, transition, and turbulent, are separated. When the dielectric wall is heated, the APPJ length and volume are enhanced. Also, the transition regions remarkably expand over a large range of flow rates. The results indicate that different factors contribute to the expansion of the transition region. The increase in the radial and axial velocities is the main cause of the expansion of the transition region to the low-velocity region. The expansion to the high-velocity region is dominantly induced by a change in the viscosity.

  16. On the magnetic field signal radiated by an atmospheric pressure room temperature plasma jet

    SciTech Connect (OSTI)

    Wu, S.; Huang, Q.; Wang, Z.; Lu, X. [State Key Laboratory of Advanced Electromagnetic Engineering and Technology, Huazhong University of Science and Technology, Wuhan, Hubei 430074 (China)

    2013-01-28

    In this paper, the magnetic field signal radiated from an atmospheric pressure room temperature plasma plume is measured. It's found that the magnetic field signal has similar waveform as the current carried by the plasma plume. By calibration of the magnetic field signal, the plasma plume current is obtained by measuring the magnetic field signal radiated by the plasma plume. In addition, it is found that, when gas flow modes changes from laminar regime to turbulence regime, the magnetic field signal waveforms appears different, it changes from a smooth curve to a curve with multiple spikes. Furthermore, it is confirmed that the plasma plume generated by a single electrode (without ground electrode) plasma jet device carries higher current than that with ground electrode.

  17. Non-equilibrium atmospheric pressure microplasma jet: An approach to endoscopic therapies

    SciTech Connect (OSTI)

    Zuo, Xiao; Wei, Yu; Wei Chen, Long; Dong Meng, Yue; Collaboration: Plasma Medicine Team

    2013-08-15

    Atmospheric pressure microplasma jet generated in a long hollow core optical fiber is studied to verify the potential feasibility of endoscopic therapies. Thermal damage and electric shock to the human body were suppressed by two technical methods, i.e., the high-voltage resistant flexible tube wrapped on the optical fiber and a power resistor of 100 k? connected between the power supply and the copper foil electrode. Optical emission spectra analysis indicated that many kinds of active radicals like excited atomic O and OH, were generated in the microplasma jet. In addition, the applications of the microplasma jet on sterilization and lung cancer cell apoptosis were presented. After 5 min of exposures to the microplasma jet, the cell viability and the bacillus subtilis replication decreased to about 3% and zero, respectively. More investigations are needed to improve the plasma-aided endoscopic therapies.

  18. Decomposition of toluene in a steady-state atmospheric-pressure glow discharge

    SciTech Connect (OSTI)

    Trushkin, A. N.; Grushin, M. E.; Kochetov, I. V.; Trushkin, N. I.; Akishev, Yu. S.

    2013-02-15

    Results are presented from experimental studies of decomposition of toluene (C{sub 6}H{sub 5}CH{sub 3}) in a polluted air flow by means of a steady-state atmospheric pressure glow discharge at different water vapor contents in the working gas. The experimental results on the degree of C{sub 6}H{sub 5}CH{sub 3} removal are compared with the results of computer simulations conducted in the framework of the developed kinetic model of plasma chemical decomposition of toluene in the N{sub 2}: O{sub 2}: H{sub 2}O gas mixture. A substantial influence of the gas flow humidity on toluene decomposition in the atmospheric pressure glow discharge is demonstrated. The main mechanisms of the influence of humidity on C{sub 6}H{sub 5}CH{sub 3} decomposition are determined. The existence of two stages in the process of toluene removal, which differ in their duration and the intensity of plasma chemical decomposition of C{sub 6}H{sub 5}CH{sub 3} is established. Based on the results of computer simulations, the composition of the products of plasma chemical reactions at the output of the reactor is analyzed as a function of the specific energy deposition and gas flow humidity. The existence of a catalytic cycle in which hydroxyl radical OH acts a catalyst and which substantially accelerates the recombination of oxygen atoms and suppression of ozone generation when the plasma-forming gas contains water vapor is established.

  19. Electrical studies and plasma characterization of an atmospheric pressure plasma jet operated at low frequency

    SciTech Connect (OSTI)

    Giuliani, L.; Xaubet, M.; Grondona, D.; Minotti, F.; Kelly, H.

    2013-06-15

    Low-temperature, high-pressure plasma jets have an extensive use in medical and biological applications. Much work has been devoted to study these applications while comparatively fewer studies appear to be directed to the discharge itself. In this work, in order to better understand the kind of electrical discharge and the plasma states existing in those devices, a study of the electrical characteristics of a typical plasma jet, operated at atmospheric pressure, using either air or argon, is reported. It is found that the experimentally determined electrical characteristics are consistent with the model of a thermal arc discharge, with a highly collisional cathode sheet. The only exception is the case of argon at the smallest electrode separation studied, around 1 mm in which case the discharge is better modeled as either a non-thermal arc or a high-pressure glow. Also, variations of the electrical behavior at different gas flow rates are interpreted, consistently with the arc model, in terms of the development of fluid turbulence in the external jet.

  20. Atmospheric Radiation Measurement Radiative Atmospheric Divergence...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    campaign is sponsored by the Atmospheric Radiation Measurement (ARM) Program, the largest global change research program within the U.S. Department of Energy's Office of Science. ...

  1. Influences of impedance matching network on pulse-modulated radio frequency atmospheric pressure glow discharges

    SciTech Connect (OSTI)

    Huo, W. G. [School of Physics and Optoelectronic Technology, Dalian University of Technology, Dalian 116023 (China); School of Physics and Electronic Technology, Liaoning Normal University, Dalian 116029 (China); Xu, K.; Sun, B.; Ding, Z. F. [School of Physics and Optoelectronic Technology, Dalian University of Technology, Dalian 116023 (China)

    2012-08-15

    Pulse-modulated RF atmospheric pressure glow discharges (APDGs) were investigated in recent years to reduce the thermal accumulation and extend the operation region of the stable alpha glow mode. Different pulse-modulated voltage and current waveforms were acquired in previous experiments, but no attention was paid to the interpretation. We investigated this issue and associated phenomenon via positive and negative feedback effects derived from varying the series capacitor in the inversely L-shaped matching network used in our pulse-modulated RF APGD source. The evolutions of pulse-modulated RF waveforms were found to be associated with the feedback region and the pulsed plasma absorbed RF power. In the positive feedback region, pulse-modulated RF APGDs are relatively stable. In the negative feedback region, wide spikes as well as undershoots occur in RF voltage and current waveforms and the plasma absorbed RF power. In case of a high RF power discharge with a low modulation frequency, the pulse-modulated RF APGD is extinguished and re-ignited due to the enhanced undershoot during the initial pulse phase. The pulse-modulated RF APGD can transit from positive to negative feedback region in a range of series capacitance. Experimental results are discussed by the aid of equivalent circuit, negative and positive feedback effects.

  2. Studies on gas breakdown in pulsed radio frequency atmospheric pressure glow discharges

    SciTech Connect (OSTI)

    Huo, W. G. [School of Physics and Optoelectronic Technology, Dalian University of Technology, Dalian 116023 (China) [School of Physics and Optoelectronic Technology, Dalian University of Technology, Dalian 116023 (China); School of Physics and Electronic Technology, Liaoning Normal University, Dalian 116029 (China); Jian, S. J.; Yao, J.; Ding, Z. F., E-mail: zfding@dlut.edu.cn [School of Physics and Optoelectronic Technology, Dalian University of Technology, Dalian 116023 (China)

    2014-05-15

    In pulsed RF atmospheric pressure glow discharges, the gas breakdown judged by the rapid drop in the amplitude of the pulsed RF voltage is no longer universally true. The steep increment of the plasma-absorbed RF power is proposed to determine the gas breakdown. The averaged plasma-absorbed RF power over a pulse period is used to evaluate effects of the preceding pulsed RF discharge on the breakdown voltage of the following one, finding that the breakdown voltage decreases with the increment in the averaged plasma-absorbed RF power under constant pulse duty ratio. Effects of the pulse off-time on the breakdown voltage and the breakdown delay time are also studied. The obtained dependence of the breakdown voltage on the pulse off-time is indicative of the transitional plasma diffusion processes in the afterglow. The breakdown voltage varies rapidly as the plasma diffuses fast in the region of moderate pulse off-time. The contribution of nitrogen atom recombination at the alumina surface is demonstrated in the prolonged memory effect on the breakdown delay time vs. the pulse off-time and experimentally validated by introducing a trace amount of nitrogen into argon at short and long pulse off-times.

  3. An experimental study of atmospheric pressure dielectric barrier discharge (DBD) in argon

    SciTech Connect (OSTI)

    Subedi, D. P.; Tyata, R. B.; Shrestha, R.; Wong, C. S.

    2014-03-05

    In this paper, experimental results on atmospheric pressure argon dielectric barrier discharge (DBD) have been presented. The discharge was generated using a high voltage (0 to 20 kV) power supply operating at frequency of 10 to 30 kHz and was studied by means of electrical and optical measurements. A homogeneous and steady discharge was observed between the electrodes with gap spacing from 1 mm to 3 mm and with a dielectric barrier of thickness 1.5 mm while argon gas is fed at a controlled flow rate of 2liter per min. The electron temperature (T{sub e}) and electron density (n{sub e}) of the plasma have been determined by means of optical emission spectroscopy. Our results show that the electron density is of the order of 10{sup 16} cm{sup ?3} while the electron temperature is estimated to be ? 1 eV. The homogeneity and non-thermal nature of the discharge were utilized in the investigation of the change in wettabilty of a polymer sample subjected to the treatment by the discharge. Contact angle analysis showed that the discharge was effective in improving the wettability of low density Polyethylene (LDPE) polymer sample after the treatment.

  4. Langmuir probe diagnostics of an atmospheric pressure, vortex-stabilized nitrogen plasma jet

    SciTech Connect (OSTI)

    Prevosto, L.; Mancinelli, B. R.; Kelly, H.

    2012-09-15

    Langmuir probe measurements in an atmospheric pressure direct current (dc) plasma jet are reported. Sweeping probes were used. The experiment was carried out using a dc non-transferred arc torch with a rod-type cathode and an anode of 5 mm diameter. The torch was operated at a nominal power level of 15 kW with a nitrogen flow rate of 25 Nl min{sup -1}. A flat ion saturation region was found in the current-voltage curve of the probe. The ion saturation current to a cylindrical probe in a high-pressure non local thermal equilibrium (LTE) plasma was modeled. Thermal effects and ionization/recombination processes inside the probe perturbed region were taken into account. Averaged radial profiles of the electron and heavy particle temperatures as well as the electron density were obtained. An electron temperature around 11 000 K, a heavy particle temperature around 9500 K and an electron density of about 4 Multiplication-Sign 10{sup 22} m{sup -3}, were found at the jet centre at 3.5 mm downstream from the torch exit. Large deviations from kinetic equilibrium were found throughout the plasma jet. The electron and heavy particle temperature profiles showed good agreement with those reported in the literature by using spectroscopic techniques. It was also found that the temperature radial profile based on LTE was very close to that of the electrons. The calculations have shown that this method is particularly useful for studying spraying-type plasma jets characterized by electron temperatures in the range 9000-14 000 K.

  5. Atmospheric pressure He-air plasma jet: Breakdown process and propagation phenomenon

    SciTech Connect (OSTI)

    Begum, Asma; Laroussi, Mounir; Pervez, Mohammad Rasel

    2013-06-15

    In this paper He-discharge (plasma jet/bullet) in atmospheric pressure air and its progression phenomenon has been studied experimentally using ICCD camera, optical emission spectroscopy (OES) and calibrated dielectric probe measurements. The repetitive nanosecond pulse has applied to a plasma pencil to generate discharge in the helium gas channel. The discharge propagation speed was measured from the ICCD images. The axial electric field distribution in the plasma jet is inferred from the optical emission spectroscopic data and from the probe measurement. The correlation between the jet velocities, jet length with the pulse duration is established. It shows that the plasma jet is not isolated from the input voltage along its propagation path. The discharge propagation speed, the electron density and the local and average electric field distribution along the plasma jet axis predicted from the experimental results are in good agreement with the data predicted by numerical simulation of the streamer propagation presented in different literatures. The ionization phenomenon of the discharge predicts the key ionization parameters, such as speed, peak electric field in the front, and electron density. The maximum local electric field measured by OES is 95 kV/cm at 1.3 cm of the jet axis, and average EF measured by probe is 24 kV/cm at the same place of the jet. The average and local electron density estimated are in the order of 10{sup 11} cm{sup -3} and it reaches to the maximum of 10{sup 12} cm{sup -3}.

  6. On-line coating of glass with tin oxide by atmospheric pressure chemical vapor deposition.

    SciTech Connect (OSTI)

    Allendorf, Mark D.; Sopko, J.F. (PPF Industries, Pittsburgh, PA); Houf, William G.; Chae, Yong Kee; McDaniel, Anthony H.; Li, M. (PPF Industries, Pittsburgh, PA); McCamy, J.W.

    2006-11-01

    Atmospheric pressure chemical vapor deposition (APCVD) of tin oxide is a very important manufacturing technique used in the production of low-emissivity glass. It is also the primary method used to provide wear-resistant coatings on glass containers. The complexity of these systems, which involve chemical reactions in both the gas phase and on the deposition surface, as well as complex fluid dynamics, makes process optimization and design of new coating reactors a very difficult task. In 2001 the U.S. Dept. of Energy Industrial Technologies Program Glass Industry of the Future Team funded a project to address the need for more accurate data concerning the tin oxide APCVD process. This report presents a case study of on-line APCVD using organometallic precursors, which are the primary reactants used in industrial coating processes. Research staff at Sandia National Laboratories in Livermore, CA, and the PPG Industries Glass Technology Center in Pittsburgh, PA collaborated to produce this work. In this report, we describe a detailed investigation of the factors controlling the growth of tin oxide films. The report begins with a discussion of the basic elements of the deposition chemistry, including gas-phase thermochemistry of tin species and mechanisms of chemical reactions involved in the decomposition of tin precursors. These results provide the basis for experimental investigations in which tin oxide growth rates were measured as a function of all major process variables. The experiments focused on growth from monobutyltintrichloride (MBTC) since this is one of the two primary precursors used industrially. There are almost no reliable growth-rate data available for this precursor. Robust models describing the growth rate as a function of these variables are derived from modeling of these data. Finally, the results are used to conduct computational fluid dynamic simulations of both pilot- and full-scale coating reactors. As a result, general conclusions are reached concerning the factors affecting the growth rate in on-line APCVD reactors. In addition, a substantial body of data was generated that can be used to model many different industrial tin oxide coating processes. These data include the most extensive compilation of thermochemistry for gas-phase tin-containing species as well as kinetic expressions describing tin oxide growth rates over a wide range of temperatures, pressures, and reactant concentrations.

  7. Final Report DE-FG02-00ER54583: "Physics of Atmospheric Pressure Glow Discharges" and "Nanoparticle Nucleation and Dynamics in Low-Pressure Plasmas"

    SciTech Connect (OSTI)

    Uwe Kortshagen; Joachim Heberlein; Steven L. Girshick

    2009-06-01

    This project was funded over two periods of three years each, with an additional year of no-cost extension. Research in the first funding period focused on the physics of uniform atmospheric pressure glow discharges, the second funding period was devoted to the study of the dynamics of nanometer-sized particles in plasmas.

  8. Community Atmosphere Model

    Energy Science and Technology Software Center (OSTI)

    2004-10-18

    The Community Atmosphere Model (CAM) is an atmospheric general circulation model that solves equations for atmospheric dynamics and physics. CAM is an outgrowth of the Community Climate Model at the National Center for Atmospheric Research (NCAR) and was developed as a joint collaborative effort between NCAR and several DOE laboratories, including LLNL. CAM contains several alternative approaches for advancing the atmospheric dynamics. One of these approaches uses a finite-volume method originally developed by personnel atmore » NASNGSFC, We have developed a scalable version of the finite-volume solver for massively parallel computing systems. FV-CAM is meant to be used in conjunction with the Community Atmosphere Model. It is not stand-alone.« less

  9. Laser schlieren deflectometry for temperature analysis of filamentary non-thermal atmospheric pressure plasma

    SciTech Connect (OSTI)

    Schaefer, J.; Foest, R.; Reuter, S.; Weltmann, K.-D.; Kewitz, T.; Sperka, J.

    2012-10-15

    The heat convection generated by micro filaments of a self-organized non-thermal atmospheric pressure plasma jet in Ar is characterized by employing laser schlieren deflectometry (LSD). It is demonstrated as a proof of principle, that the spatial and temporal changes of the refractive index n in the optical beam path related to the neutral gas temperature of the plasma jet can be monitored and evaluated simultaneously. The refraction of a laser beam in a high gradient field of n(r) with cylindrical symmetry is given for a general real refraction index profile. However, the usually applied Abel approach represents an ill-posed problem and in particular for this plasma configuration. A simple analytical model is proposed in order to minimize the statistical error. Based on that, the temperature profile, specifically the absolute temperature in the filament core, the FWHM, and the frequencies of the collective filament dynamics are obtained for non-stationary conditions. For a gas temperature of 700 K inside the filament, the presented model predicts maximum deflection angles of the laser beam of 0.3 mrad which is in accordance to the experimental results obtained with LSD. Furthermore, the experimentally obtained FWHM of the temperature profile produced by the filament at the end of capillary is (1.5 {+-} 0.2) mm, which is about 10 times wider than the visual radius of the filament. The obtained maximum temperature in the effluent is (450 {+-} 30) K and is in consistence with results of other techniques. The study demonstrates that LSD represents a useful low-cost method for monitoring the spatiotemporal behaviour of microdischarges and allows to uncover their dynamic characteristics, e.g., the temperature profile even for challenging diagnostic conditions such as moving thin discharge filaments. The method is not restricted to the miniaturized and self-organized plasma studied here. Instead, it can be readily applied to other configurations that produce measurable gradients of refractive index by local gas heating and opens new diagnostics prospects particularly for microplasmas.

  10. Ensemble Atmospheric Dispersion Modeling

    SciTech Connect (OSTI)

    Addis, R.P.

    2002-06-24

    Prognostic atmospheric dispersion models are used to generate consequence assessments, which assist decision-makers in the event of a release from a nuclear facility. Differences in the forecast wind fields generated by various meteorological agencies, differences in the transport and diffusion models, as well as differences in the way these models treat the release source term, result in differences in the resulting plumes. Even dispersion models using the same wind fields may produce substantially different plumes. This talk will address how ensemble techniques may be used to enable atmospheric modelers to provide decision-makers with a more realistic understanding of how both the atmosphere and the models behave.

  11. ARM - Measurement - Atmospheric temperature

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    temperature ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Atmospheric temperature The temperature indicated by a thermometer exposed to the air in a place sheltered from direct solar radiation. Categories Atmospheric State Instruments The above measurement is considered scientifically relevant for the following instruments. Refer to the datastream (netcdf) file headers of each instrument for a list

  12. ARM - Measurement - Atmospheric turbulence

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    turbulence ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Measurement : Atmospheric turbulence High frequency velocity fluctuations that lead to turbulent transport of momentum, heat, mositure, and passive scalars, and often expressed in terms of variances and covariances. Categories Atmospheric State, Surface Properties Instruments The above measurement is considered scientifically relevant for the following

  13. ARM - Atmospheric Heat Budget

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ListAtmospheric Heat Budget Outreach Home Room News Publications Traditional Knowledge Kiosks Barrow, Alaska Tropical Western Pacific Site Tours Contacts Students Study Hall About ARM Global Warming FAQ Just for Fun Meet our Friends Cool Sites Teachers Teachers' Toolbox Lesson Plans Atmospheric Heat Budget The average temperature of the earth has remained approximately constant at about 15 degrees Celsius during the past century. It is therefore in a state of radiative balance, emitting the same

  14. Nonlinear propagation of a high-power focused femtosecond laser pulse in air under atmospheric and reduced pressure

    SciTech Connect (OSTI)

    Geints, Yu E; Zemlyanov, A A; Ionin, Andrei A; Kudryashov, Sergei I; Seleznev, L V; Sinitsyn, D V; Sunchugasheva, E S

    2012-04-30

    This paper examines the propagation of focused femtosecond gigawatt laser pulses in air under normal and reduced pressure in the case of Kerr self-focusing and photoionisation of the medium. The influence of gas density on the beam dimensions and power and the electron density in the plasma column in the nonlinear focus zone of the laser beam has been studied experimentally and by numerical simulation. It has been shown that, in rarefied air, the radiation-induced reduction in the rate of plasma formation diminishes the blocking effect of the plasma on the growth of the beam intensity in the case of tight focusing. This allows higher power densities of ultrashort laser pulses to be reached in the focal waist region in comparison with beam self-focusing under atmospheric pressure.

  15. Atmospheric sampling glow discharge ionization source

    DOE Patents [OSTI]

    McLuckey, S.A.; Glish, G.L.

    1989-07-18

    An atmospheric sampling glow discharge ionization source that can be used in combination with an analytical instrument which operates at high vacuum, such as a mass spectrometer. The atmospheric sampling glow discharge ionization source comprises a chamber with at least one pair of electrodes disposed therein, an inlet for a gaseous sample to be analyzed and an outlet communicating with an analyzer which operates at subatmospheric pressure. The ionization chamber is maintained at a pressure below atmospheric pressure, and a voltage difference is applied across the electrodes to induce a glow discharge between the electrodes, so that molecules passing through the inlet are ionized by the glow discharge and directed into the analyzer. The ionization source accepts the sample under atmospheric pressure conditions and processes it directly into the high vacuum instrument, bridging the pressure gap and drawing off unwanted atmospheric gases. The invention also includes a method for analyzing a gaseous sample using the glow discharge ionization source described above. 3 figs.

  16. Atmospheric sampling glow discharge ionization source

    DOE Patents [OSTI]

    McLuckey, Scott A. (Oak Ridge, TN); Glish, Gary L. (Oak Ridge, TN)

    1989-01-01

    An atmospheric sampling glow discharge ionization source that can be used in combination with an analytical instrument which operates at high vacuum, such as a mass spectrometer. The atmospheric sampling glow discharge ionization source comprises a chamber with at least one pair of electrodes disposed therein, an inlet for a gaseous sample to be analyzed and an outlet communicating with an analyzer which operates at subatmospheric pressure. The ionization chamber is maintained at a pressure below atmospheric pressure, and a voltage difference is applied across the electrodes to induce a glow discharge between the electrodes, so that molecules passing through the inlet are ionized by the glow discharge and directed into the analyzer. The ionization source accepts the sample under atmospheric pressure conditions and processes it directly into the high vacuum instrument, bridging the pressure gap and drawing off unwanted atmospheric gases. The invention also includes a method for analyzing a gaseous sample using the glow discharge ionization source described above.

  17. Auto-ignition during instationary jet evolution of dimethyl ether (DME) in a high-pressure atmosphere

    SciTech Connect (OSTI)

    Fast, G.; Kuhn, D.; Class, A.G.; Maas, U.

    2009-01-15

    The auto-ignition process during transient injection of gaseous dimethyl ether (DME) in a constant high-pressure atmosphere is studied experimentally by laser-optical methods and compared with numerical calculations. With different non-intrusive measurement techniques jet properties and auto-ignition are investigated at high temporal and spatial resolution. The open jet penetrates a constant pressure oxidative atmosphere of up to 4 MPa. During the transient evolution, the fuel jet entrains air at up to 720 K. The subsequent auto-ignition of the ignitable part of the jet occurs simultaneously over a wide spatial extension. The ignition delay times are not affected by variation of the nozzle exit velocity. Thus, the low-temperature oxidation is slow compared with the shorter time scales of mixing, so that chemical kinetics is dominating the process. The typical two-stage ignition is resolved optically with high-speed shadowgraphy at a sampling rate of 10 kHz. The 2D fields of jet velocity and transient mixture fraction are measured phase-coupled with Particle Image Velocimetry (PIV) and Tracer Laser Induced Fluorescence (LIF) during the time-frame of ignition. The instationary Probability Density Functions (PDF) of mixture fraction are described very well by Beta functions within the complete area of the open jet. Additional 1D flamelet simulations of the auto-ignition process are computed with a detailed reaction mechanism for DME [S. Fischer, F. Dryer, H. Curran, Int. J. Chem. Kinet. 32 (12) (2000) 713-740; H. Curran, S. Fischer, F. Dryer, Int. J. Chem. Kinet. 32 (12) (2000) 741-759]. Calculated ignition delay times are in very good agreement with the measured mean ignition delay times of 3 ms. Supplemental flamelet simulations address the influence of DME and air temperature, pressure and strain. Underneath a critical strain rate the air temperature is identified to be the most sensitive factor on ignition delay time. (author)

  18. Research Update: Atmospheric pressure spatial atomic layer deposition of ZnO thin films: Reactors, doping, and devices

    SciTech Connect (OSTI)

    Hoye, Robert L. Z. E-mail: jld35@cam.ac.uk; MacManus-Driscoll, Judith L. E-mail: jld35@cam.ac.uk; Muoz-Rojas, David; Nelson, Shelby F.; Illiberi, Andrea; Poodt, Paul

    2015-04-01

    Atmospheric pressure spatial atomic layer deposition (AP-SALD) has recently emerged as an appealing technique for rapidly producing high quality oxides. Here, we focus on the use of AP-SALD to deposit functional ZnO thin films, particularly on the reactors used, the film properties, and the dopants that have been studied. We highlight how these films are advantageous for the performance of solar cells, organometal halide perovskite light emitting diodes, and thin-film transistors. Future AP-SALD technology will enable the commercial processing of thin films over large areas on a sheet-to-sheet and roll-to-roll basis, with new reactor designs emerging for flexible plastic and paper electronics.

  19. Apparatus and method for enhanced chemical processing in high pressure and atmospheric plasmas produced by high frequency electromagnetic waves

    DOE Patents [OSTI]

    Efthimion, Philip C. (Bedminister, NJ); Helfritch, Dennis J. (Flemington, NJ)

    1989-11-28

    An apparatus and method for creating high temperature plasmas for enhanced chemical processing of gaseous fluids, toxic chemicals, and the like, at a wide range of pressures, especially at atmospheric and high pressures includes an electro-magnetic resonator cavity, preferably a reentrant cavity, and a wave guiding structure which connects an electro-magnetic source to the cavity. The cavity includes an intake port and an exhaust port, each having apertures in the conductive walls of the cavity sufficient for the intake of the gaseous fluids and for the discharge of the processed gaseous fluids. The apertures are sufficiently small to prevent the leakage of the electro-magnetic radiation from the cavity. Gaseous fluid flowing from the direction of the electro-magnetic source through the guiding wave structure and into the cavity acts on the plasma to push it away from the guiding wave structure and the electro-magnetic source. The gaseous fluid flow confines the high temperature plasma inside the cavity and allows complete chemical processing of the gaseous fluids at a wide range of pressures.

  20. Dynamics of plasma expansion and shockwave formation in femtosecond laser-ablated aluminum plumes in argon gas at atmospheric pressures

    SciTech Connect (OSTI)

    Miloshevsky, Alexander; Harilal, Sivanandan S.; Miloshevsky, Gennady Hassanein, Ahmed

    2014-04-15

    Plasma expansion with shockwave formation during laser ablation of materials in a background gasses is a complex process. The spatial and temporal evolution of pressure, temperature, density, and velocity fields is needed for its complete understanding. We have studied the expansion of femtosecond (fs) laser-ablated aluminum (Al) plumes in Argon (Ar) gas at 0.5 and 1 atmosphere (atm). The expansion of the plume is investigated experimentally using shadowgraphy and fast-gated imaging. The computational fluid dynamics (CFD) modeling is also carried out. The position of the shock front measured by shadowgraphy and fast-gated imaging is then compared to that obtained from the CFD modeling. The results from the three methods are found to be in good agreement, especially during the initial stage of plasma expansion. The computed time- and space-resolved fields of gas-dynamic parameters have provided valuable insights into the dynamics of plasma expansion and shockwave formation in fs-pulse ablated Al plumes in Ar gas at 0.5 and 1?atm. These results are compared to our previous data on nanosecond (ns) laser ablation of Al [S. S. Harilal et al., Phys. Plasmas 19, 083504 (2012)]. It is observed that both fs and ns plumes acquire a nearly spherical shape at the end of expansion in Ar gas at 1?atm. However, due to significantly lower pulse energy of the fs laser (5 mJ) compared to pulse energy of the ns laser (100 mJ) used in our studies, the values of pressure, temperature, mass density, and velocity are found to be smaller in the fs laser plume, and their time evolution occurs much faster on the same time scale. The oscillatory shock waves clearly visible in the ns plume are not observed in the internal region of the fs plume. These experimental and computational results provide a quantitative understanding of plasma expansion and shockwave formation in fs-pulse and ns-pulse laser ablated Al plumes in an ambient gas at atmospheric pressures.

  1. Differential atmospheric tritium sampler

    DOE Patents [OSTI]

    Griesbach, Otto A. (Langhorne, PA); Stencel, Joseph R. (Skillman, NJ)

    1990-01-01

    An atmospheric tritium sampler is provided which uses a carrier gas comprised of hydrogen gas and a diluting gas, mixed in a nonexplosive concentration. Sample air and carrier gas are drawn into and mixed in a manifold. A regulator meters the carrier gas flow to the manifold. The air sample/carrier gas mixture is pulled through a first moisture trap which adsorbs water from the air sample. The mixture then passes through a combustion chamber where hydrogen gas in the form of H.sub.2 or HT is combusted into water. The manufactured water is transported by the air stream to a second moisture trap where it is adsorbed. The air is then discharged back into the atmosphere by means of a pump.

  2. Differential atmospheric tritium sampler

    DOE Patents [OSTI]

    Griesbach, O.A.; Stencel, J.R.

    1987-10-02

    An atmospheric tritium sampler is provided which uses a carrier gas comprised of hydrogen gas and a diluting gas, mixed in a nonexplosive concentration. Sample air and carrier gas are drawn into and mixed in a manifold. A regulator meters the carrier gas flow to the manifold. The air sample/carrier gas mixture is pulled through a first moisture trap which adsorbs water from the air sample. The moisture then passes through a combustion chamber where hydrogen gas in the form of H/sub 2/ or HT is combusted into water. The manufactured water is transported by the air stream to a second moisture trap where it is adsorbed. The air is then discharged back into the atmosphere by means of a pump.

  3. ARM - Evolution of the Atmosphere

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ListEvolution of the Atmosphere Outreach Home Room News Publications Traditional Knowledge Kiosks Barrow, Alaska Tropical Western Pacific Site Tours Contacts Students Study Hall About ARM Global Warming FAQ Just for Fun Meet our Friends Cool Sites Teachers Teachers' Toolbox Lesson Plans Evolution of the Atmosphere The earth's atmosphere plays a crucial role in shaping the weather, climate, and life-supporting systems. However, the ocean and atmosphere are the earth's fluid outer layers and are

  4. ARM - Composition of the Atmosphere

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ListComposition of the Atmosphere Outreach Home Room News Publications Traditional Knowledge Kiosks Barrow, Alaska Tropical Western Pacific Site Tours Contacts Students Study Hall About ARM Global Warming FAQ Just for Fun Meet our Friends Cool Sites Teachers Teachers' Toolbox Lesson Plans Composition of the Atmosphere The atmosphere is 1000 kilometers above mean sea level. In fact, only about 1 percent of the total mass of the atmosphere is above an altitude of approximately 30 kilometers above

  5. A comparison between characteristics of atmospheric-pressure plasma jets sustained by nanosecond- and microsecond-pulse generators in helium

    SciTech Connect (OSTI)

    Zhang, Cheng; Shao, Tao Wang, Ruixue; Yan, Ping; Zhou, Zhongsheng; Zhou, Yixiao

    2014-10-15

    Power source is an important parameter that can affect the characteristics of atmospheric-pressure plasma jets (APPJs), because it can play a key role on the discharge characteristics and ionization process of APPJs. In this paper, the characteristics of helium APPJs sustained by both nanosecond-pulse and microsecond-pulse generators are compared from the aspects of plume length, discharge current, consumption power, energy, and optical emission spectrum. Experimental results showed that the pulsed APPJ was initiated near the high-voltage electrode with a small curvature radius, and then the stable helium APPJ could be observed when the applied voltage increased. Moreover, the discharge current of the nanosecond-pulse APPJ was larger than that of the microsecond-pulse APPJ. Furthermore, although the nanosecond-pulse generator consumed less energy than the microsecond-pulse generator, longer plume length, larger instantaneous power per pulse and stronger spectral line intensity could be obtained in the nanosecond-pulse excitation case. In addition, some discussion indicated that the rise time of the applied voltage could play a prominent role on the generation of APPJs.

  6. A dominant role of oxygen additive on cold atmospheric-pressure He + O{sub 2} plasmas

    SciTech Connect (OSTI)

    Yang, Aijun; Liu, Dingxin E-mail: xhw@mail.xjtu.edu.cn; Rong, Mingzhe; Wang, Xiaohua E-mail: xhw@mail.xjtu.edu.cn; Kong, Michael G.

    2014-08-15

    We present in this paper how oxygen additive impacts on the cold atmospheric-pressure helium plasmas by means of a one-dimensional fluid model. For the oxygen concentration [O{sub 2}]?>??0.1%, the influence of oxygen on the electron characteristics and the power dissipation becomes important, e.g., the electron density, the electron temperature in sheath, the electron-coupling power, and the sheath width decreasing by 1.6 to 16 folds with a two-log increase in [O{sub 2}] from 0.1% to 10%. Also the discharge mode evolves from the ? mode to the ? mode. The reactive oxygen species are found to peak in the narrow range of [O{sub 2}]?=?0.4%0.9% in the plasmas, similar to their power-coupling values. This applies to their wall fluxes except for those of O* and O{sub 2}{sup ?}. These two species have very short lifetimes, thus only when generated in boundary layers within several micrometers next to the electrode can contribute to the fluxes. The dominant reactive oxygen species and the corresponding main reactions are schematically presented, and their relations are quantified for selected applications.

  7. Influence of Penning effect on the plasma features in a non-equilibrium atmospheric pressure plasma jet

    SciTech Connect (OSTI)

    Chang, Zhengshi; Zhang, Guanjun; Jiang, Nan; Cao, Zexian

    2014-03-14

    Non-equilibrium atmospheric pressure plasma jet (APPJ) is a cold plasma source that promises various innovative applications. The influence of Penning effect on the formation, propagation, and other physical properties of the plasma bullets in APPJ remains a debatable topic. By using a 10?cm wide active electrode and a frequency of applied voltage down to 0.5?Hz, the Penning effect caused by preceding discharges can be excluded. It was found that the Penning effect originating in a preceding discharge helps build a conductive channel in the gas flow and provide seed electrons, thus the discharge can be maintained at a low voltage which in turn leads to a smaller propagation speed for the plasma bullet. Photographs from an intensified charge coupled device reveal that the annular structure of the plasma plume for He is irrelevant to the Penning ionization process arising from preceding discharges. By adding NH{sub 3} into Ar to introduce Penning effect, the originally filamentous discharge of Ar can display a rather extensive plasma plume in ambient as He. These results are helpful for the understanding of the behaviors of non-equilibrium APPJs generated under distinct conditions and for the design of plasma jet features, especially the spatial distribution and propagation speed, which are essential for application.

  8. Self-consistent fluid modeling and simulation on a pulsed microwave atmospheric-pressure argon plasma jet

    SciTech Connect (OSTI)

    Chen, Zhaoquan; Yin, Zhixiang Chen, Minggong; Hong, Lingli; Hu, Yelin; Huang, Yourui; Xia, Guangqing; Liu, Minghai; Kudryavtsev, A. A.

    2014-10-21

    In present study, a pulsed lower-power microwave-driven atmospheric-pressure argon plasma jet has been introduced with the type of coaxial transmission line resonator. The plasma jet plume is with room air temperature, even can be directly touched by human body without any hot harm. In order to study ionization process of the proposed plasma jet, a self-consistent hybrid fluid model is constructed in which Maxwell's equations are solved numerically by finite-difference time-domain method and a fluid model is used to study the characteristics of argon plasma evolution. With a Guass type input power function, the spatio-temporal distributions of the electron density, the electron temperature, the electric field, and the absorbed power density have been simulated, respectively. The simulation results suggest that the peak values of the electron temperature and the electric field are synchronous with the input pulsed microwave power but the maximum quantities of the electron density and the absorbed power density are lagged to the microwave power excitation. In addition, the pulsed plasma jet excited by the local enhanced electric field of surface plasmon polaritons should be the discharge mechanism of the proposed plasma jet.

  9. Analysis by oxygen atom number density measurement of high-speed hydrophilic treatment of polyimide using atmospheric pressure microwave plasma

    SciTech Connect (OSTI)

    Ono, S.

    2015-03-30

    This paper describes the fundamental experimental data of the plasma surface modification of the polyimide using atmospheric pressure microwave plasma source. The experimental results were discussed from the point of view of the radicals behavior, which significantly affects the modification mechanism. The purpose of the study is to examine how the value of the oxygen atom density will affect the hydrophilic treatment in the upstream region of the plasma where gas temperature is very high. The surface modification experiments were performed by setting the polyimide film sample in the downstream region of the plasma. The degree of the modification was measured by a water contact angle measurement. The water contact angle decreased less than 30 degrees within 1 second treatment time in the upstream region. Very high speed modification was observed. The reason of this high speed modification seems that the high density radical which contributes the surface modification exist in the upstream region of the plasma. This tendency is supposed to the measured relatively high electron density (~10{sup 15}cm{sup ?3}) at the center of the plasma. We used the electric heating catalytic probe method for oxygen radical measurement. An absolute value of oxygen radical density was determined by catalytic probe measurement and the results show that ~10{sup 15}cm{sup ?3} of the oxygen radical density in the upstream region and decreases toward downstream region. The experimental results of the relation of the oxygen radical density and hydrophilic modification of polyimide was discussed.

  10. An experimental study on sub-cooled flow boiling CHF of R134a at low pressure condition with atmospheric pressure (AP) plasma assisted surface modification

    SciTech Connect (OSTI)

    Kim, Seung Jun; Zou, Ling; Jones, Barclay G.

    2015-02-01

    In this study, sub-cooled flow boiling critical heat flux tests at low pressure were conducted in a rectangular flow channel with one uniformly heated surface, using simulant fluid R-134a as coolant. The experiments were conducted under the following conditions: (1) inlet pressure (P) of 400-800 kPa, (2) mass flux (G) of 124-248 kg/m2s, (3) inlet sub-cooling enthalpy (ΔHi) of 12~ 26 kJ/kg. Parametric trends of macroscopic system parameters (G, P, Hi) were examined by changing inlet conditions. Those trends were found to be generally consistent with previous understandings of CHF behavior at low pressure condition (i.e. reduced pressure less than 0.2). A fluid-to-fluid scaling model was utilized to convert the test data obtained with the simulant fluid (R-134a) into the prototypical fluid (water). The comparison between the converted CHF of equivalent water and CHF look-up table with same operation conditions were conducted, which showed good agreement. Furthermore, the effect of surface wettability on CHF was also investigated by applying atmospheric pressure plasma (AP-Plasma) treatment to modify the surface characteristic. With AP-Plasma treatment, the change of microscopic surface characteristic was measured in terms of static contact angle. The static contact angle was reduced from 80° on original non-treated surface to 15° on treated surface. An enhancement of 18% on CHF values under flow boiling conditions were observed on AP-Plasma treated surfaces compared to those on non-treated heating surfaces.

  11. On the physical processes ruling an atmospheric pressure air glow discharge operating in an intermediate current regime

    SciTech Connect (OSTI)

    Prevosto, L. Mancinelli, B.; Chamorro, J. C.; Cejas, E.; Kelly, H.

    2015-02-15

    Low-frequency (100?Hz), intermediate-current (50 to 200?mA) glow discharges were experimentally investigated in atmospheric pressure air between blunt copper electrodes. Voltagecurrent characteristics and images of the discharge for different inter-electrode distances are reported. A cathode-fall voltage close to 360?V and a current density at the cathode surface of about 11?A/cm{sup 2}, both independent of the discharge current, were found. The visible emissive structure of the discharge resembles to that of a typical low-pressure glow, thus suggesting a glow-like electric field distribution in the discharge. A kinetic model for the discharge ionization processes is also presented with the aim of identifying the main physical processes ruling the discharge behavior. The numerical results indicate the presence of a non-equilibrium plasma with rather high gas temperature (above 4000?K) leading to the production of components such as NO, O, and N which are usually absent in low-current glows. Hence, the ionization by electron-impact is replaced by associative ionization, which is independent of the reduced electric field. This leads to a negative current-voltage characteristic curve, in spite of the glow-like features of the discharge. On the other hand, several estimations show that the discharge seems to be stabilized by heat conduction; being thermally stable due to its reduced size. All the quoted results indicate that although this discharge regime might be considered to be close to an arc, it is still a glow discharge as demonstrated by its overall properties, supported also by the presence of thermal non-equilibrium.

  12. Atmospheric Pressure Plasma CVD of Amorphous Hydrogenated Silicon Carbonitride (a-SiCN:H) Films Using Triethylsilane and Nitrogen

    SciTech Connect (OSTI)

    Srinivasan Guruvenket; Steven Andrie; Mark Simon; Kyle W. Johnson; Robert A. Sailer

    2011-10-04

    Amorphous hydrogenated silicon carbonitride (a-SiCN:H) thin films are synthesized by atmospheric pressure plasma enhanced chemical vapor (AP-PECVD) deposition using the Surfx Atomflow{trademark} 250D APPJ source with triethylsilane (HSiEt{sub 3}, TES) and nitrogen as the precursor and the reactive gases, respectively. The effect of the substrate temperature (T{sub s}) on the growth characteristics and the properties of a-SiCN:H films was evaluated. The properties of the films were investigated via scanning electron microscopy (SEM), atomic force microscopy (AFM) for surface morphological analyses, Fourier transform infrared spectroscopy (FTIR), and X-ray photoelectron spectroscopy (XPS) for chemical and compositional analyses; spectroscopic ellipsometry for optical properties and thickness determination and nanoindentation to determine the mechanical properties of the a-SiCN:H films. Films deposited at low T{sub s} depict organic like features, while the films deposited at high T{sub s} depict ceramic like features. FTIR and XPS studies reveal that an increases in T{sub s} helps in the elimination of organic moieties and incorporation of nitrogen in the film. Films deposited at T{sub s} of 425 C have an index of refraction (n) of 1.84 and hardness (H) of 14.8 GPa. A decrease in the deposition rate between T{sub s} of 25 and 250 C and increase in deposition rate between T{sub s} of 250 and 425 C indicate that the growth of a-SiCN:H films at lower T{sub s} are surface reaction controlled, while at high temperatures film growth is mass-transport controlled. Based on the experimental results, a potential route for film growth is proposed.

  13. Atmospheric Radiation Measurement Climate Research Facility ...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Atmospheric Radiation Measurement Climate Research Facility Argonne scientists study ... for climate research to the Atmospheric Radiation Measurement (ARM) Climate Research ...

  14. Atmospheric Radiation Measurement Climate Research Facility ...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Atmospheric Radiation Measurement Climate Research Facility (ARM) Biological and ... BER Home About Research Facilities User Facilities Atmospheric Radiation Measurement ...

  15. ARM - Sources of Atmospheric Carbon

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Sources of Atmospheric Carbon Outreach Home Room News Publications Traditional Knowledge Kiosks Barrow, Alaska Tropical Western Pacific Site Tours Contacts Students Study Hall About ARM Global Warming FAQ Just for Fun Meet our Friends Cool Sites Teachers Teachers' Toolbox Lesson Plans Sources of Atmospheric Carbon Atmospheric carbon represented a steady state system, where influx equaled outflow, before the Industrial Revolution. Currently, it is no longer a steady state system because the

  16. ARM - Destination of Atmospheric Carbon

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Destination of Atmospheric Carbon Outreach Home Room News Publications Traditional Knowledge Kiosks Barrow, Alaska Tropical Western Pacific Site Tours Contacts Students Study Hall About ARM Global Warming FAQ Just for Fun Meet our Friends Cool Sites Teachers Teachers' Toolbox Lesson Plans Destination of Atmospheric Carbon Oceans: 92 gigatonnes [(Gt) 1 gigatonne = 1x1012 kilograms] are recycled annually from the atmosphere to the oceans. This carbon is used for biosynthesis or remains dissolved

  17. The quenching effect of hydrogen on the nitrogen in metastable state in atmospheric-pressure N{sub 2}-H{sub 2} microwave plasma torch

    SciTech Connect (OSTI)

    Li, Shou-Zhe, E-mail: lisz@dlut.edu.cn; Zhang, Xin; Chen, Chuan-Jie; Zhang, Jialiang [Key Laboratory of Materials Modification by Laser, Ion, Electron Beams (Dalian University of Technology), Ministry of Education, Dalian 116024 (China); School of Physics and Optoelectronic Technology, Dalian 116024 (China); Wang, Yong-Xing [College of Electrical Engineering, Dalian 116024 (China); Xia, Guang-Qing [School of Aeronautics and Astronautics, Dalian University of Technology, Dalian 116024 (China)

    2014-07-15

    The atmospheric-pressure microwave N{sub 2}-H{sub 2} plasma torch is generated and diagnosed by optical emission spectroscopy. It is found that a large amount of N atoms and NH radicals are generated in the plasma torch and the emission intensity of N{sub 2}{sup +} first negative band is the strongest over the spectra. The mixture of hydrogen in nitrogen plasma torch causes the morphology of the plasma discharge to change with appearance that the afterglow shrinks greatly and the emission intensity of N{sub 2}{sup +} first negative band decreases with more hydrogen mixed into nitrogen plasma. In atmospheric-pressure microwave-induced plasma torch, the hydrogen imposes a great influence on the characteristics of nitrogen plasma through the quenching effect of the hydrogen on the metastable state of N{sub 2}.

  18. Absolute atomic oxygen and nitrogen densities in radio-frequency driven atmospheric pressure cold plasmas: Synchrotron vacuum ultra-violet high-resolution Fourier-transform absorption measurements

    SciTech Connect (OSTI)

    Niemi, K.; O'Connell, D.; Gans, T.; Oliveira, N. de; Joyeux, D.; Nahon, L.; Booth, J. P.

    2013-07-15

    Reactive atomic species play a key role in emerging cold atmospheric pressure plasma applications, in particular, in plasma medicine. Absolute densities of atomic oxygen and atomic nitrogen were measured in a radio-frequency driven non-equilibrium plasma operated at atmospheric pressure using vacuum ultra-violet (VUV) absorption spectroscopy. The experiment was conducted on the DESIRS synchrotron beamline using a unique VUV Fourier-transform spectrometer. Measurements were carried out in plasmas operated in helium with air-like N{sub 2}/O{sub 2} (4:1) admixtures. A maximum in the O-atom concentration of (9.1 {+-} 0.7) Multiplication-Sign 10{sup 20} m{sup -3} was found at admixtures of 0.35 vol. %, while the N-atom concentration exhibits a maximum of (5.7 {+-} 0.4) Multiplication-Sign 10{sup 19} m{sup -3} at 0.1 vol. %.

  19. Polyport atmospheric gas sampler

    DOE Patents [OSTI]

    Guggenheim, S. Frederic (Teaneck, NJ)

    1995-01-01

    An atmospheric gas sampler with a multi-port valve which allows for multi, sequential sampling of air through a plurality of gas sampling tubes mounted in corresponding gas inlet ports. The gas sampler comprises a flow-through housing which defines a sampling chamber and includes a gas outlet port to accommodate a flow of gases through the housing. An apertured sample support plate defining the inlet ports extends across and encloses the sampling chamber and supports gas sampling tubes which depend into the sampling chamber and are secured across each of the inlet ports of the sample support plate in a flow-through relation to the flow of gases through the housing during sampling operations. A normally closed stopper means mounted on the sample support plate and operatively associated with each of the inlet ports blocks the flow of gases through the respective gas sampling tubes. A camming mechanism mounted on the sample support plate is adapted to rotate under and selectively lift open the stopper spring to accommodate a predetermined flow of gas through the respective gas sampling tubes when air is drawn from the housing through the outlet port.

  20. X-ray emission from a nanosecond-pulse discharge in an inhomogeneous electric field at atmospheric pressure

    SciTech Connect (OSTI)

    Zhang Cheng; Shao Tao; Ren Chengyan; Zhang Dongdong; Tarasenko, Victor; Kostyrya, Igor D.; Ma Hao; Yan Ping

    2012-12-15

    This paper describes experimental studies of the dependence of the X-ray intensity on the anode material in nanosecond high-voltage discharges. The discharges were generated by two nanosecond-pulse generators in atmospheric air with a highly inhomogeneous electric field by a tube-plate gap. The output pulse of the first generator (repetitive pulse generator) has a rise time of about 15 ns and a full width at half maximum of 30-40 ns. The output of the second generator (single pulse generator) has a rise time of about 0.3 ns and a full width at half maximum of 1 ns. The electrical characteristics and the X-ray emission of nanosecond-pulse discharge in atmospheric air are studied by the measurement of voltage-current waveforms, discharge images, X-ray count and dose. Our experimental results showed that the anode material rarely affects electrical characteristics, but it can significantly affect the X-ray density. Comparing the density of X-rays, it was shown that the highest x-rays density occurred in the diffuse discharge in repetitive pulse mode, then the spark discharge with a small air gap, and then the corona discharge with a large air gap, in which the X-ray density was the lowest. Therefore, it could be confirmed that the bremsstrahlung at the anode contributes to the X-ray emission from nanosecond-pulse discharges.

  1. Terrain-Responsive Atmospheric Code

    Energy Science and Technology Software Center (OSTI)

    1991-11-20

    The Terrain-Responsive Atmospheric Code (TRAC) is a real-time emergency response modeling capability designed to advise Emergency Managers of the path, timing, and projected impacts from an atmospheric release. TRAC evaluates the effects of both radiological and non-radiological hazardous substances, gases and particulates. Using available surface and upper air meteorological information, TRAC realistically treats complex sources and atmospheric conditions, such as those found in mountainous terrain. TRAC calculates atmospheric concentration, deposition, and dose for more thanmore »25,000 receptor locations within 80 km of the release point. Human-engineered output products support critical decisions on the type, location, and timing of protective actions for workers and the public during an emergency.« less

  2. Atmospheric science and power production

    SciTech Connect (OSTI)

    Randerson, D.

    1984-07-01

    This is the third in a series of scientific publications sponsored by the US Atomic Energy Commission and the two later organizations, the US Energy Research and Development Adminstration, and the US Department of Energy. The first book, Meteorology and Atomic Energy, was published in 1955; the second, in 1968. The present volume is designed to update and to expand upon many of the important concepts presented previously. However, the present edition draws heavily on recent contributions made by atmospheric science to the analysis of air quality and on results originating from research conducted and completed in the 1970s. Special emphasis is placed on how atmospheric science can contribute to solving problems relating to the fate of combustion products released into the atmosphere. The framework of this book is built around the concept of air-quality modeling. Fundamentals are addressed first to equip the reader with basic background information and to focus on available meteorological instrumentation and to emphasize the importance of data management procedures. Atmospheric physics and field experiments are described in detail to provide an overview of atmospheric boundary layer processes, of how air flows around obstacles, and of the mechanism of plume rise. Atmospheric chemistry and removal processes are also detailed to provide fundamental knowledge on how gases and particulate matter can be transformed while in the atmosphere and how they can be removed from the atmosphere. The book closes with a review of how air-quality models are being applied to solve a wide variety of problems. Separate analytics have been prepared for each chapter.

  3. Atmospheric Crude Oil Distillation Operable Capacity

    Gasoline and Diesel Fuel Update (EIA)

    (Barrels per Calendar Day) Data Series: Total Number of Operable Refineries Number of Operating Refineries Number of Idle Refineries Atmospheric Crude Oil Distillation Operable Capacity (B/CD) Atmospheric Crude Oil Distillation Operating Capacity (B/CD) Atmospheric Crude Oil Distillation Idle Capacity (B/CD) Atmospheric Crude Oil Distillation Operable Capacity (B/SD) Atmospheric Crude Oil Distillation Operating Capacity (B/SD) Atmospheric Crude Oil Distillation Idle Capacity (B/SD) Vacuum

  4. Electron density measurements of atmospheric-pressure non-thermal N{sub 2} plasma jet by Stark broadening and irradiance intensity methods

    SciTech Connect (OSTI)

    Xiao, Dezhi; Shen, Jie; Lan, Yan; Xie, Hongbing; Shu, Xingsheng; Meng, Yuedong; Li, Jiangang; Cheng, Cheng E-mail: paul.chu@cityu.edu.hk; Chu, Paul K. E-mail: paul.chu@cityu.edu.hk

    2014-05-15

    An atmospheric-pressure non-thermal plasma jet excited by high frequency alternating current using nitrogen is developed and the electron density in the active region of this plasma jet is investigated by two different methods using optical emission spectroscopy, Stark broadening, and irradiance intensity method. The irradiance intensity method shows that the average electron density is about 10{sup 20}/m{sup 3} which is slightly smaller than that by the Stark broadening method. However, the trend of the change in the electron density with input power obtained by these two methods is consistent.

  5. Working with SRNL - Our Facilities - Atmospheric Technologies...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The SRNL Atmospheric Technologies Center has extensive capabilities for world-wide meteorological forecasts and real-time atmospheric transport modeling and assessment. ...

  6. National Oceanic and Atmospheric Administration (NOAA) | Open...

    Open Energy Info (EERE)

    National Oceanic and Atmospheric Administration (NOAA) Jump to: navigation, search Logo: National Oceanic and Atmospheric Administration (NOAA) Name: National Oceanic and...

  7. Correcting radar range measurements for atmospheric propagation...

    Office of Scientific and Technical Information (OSTI)

    Correcting radar range measurements for atmospheric propagation effects. Citation Details In-Document Search Title: Correcting radar range measurements for atmospheric propagation...

  8. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion...

  9. Atmospheric Radiation Measurement Climate Research Facility Operations...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    6-001 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly ... DOESC-ARM-16-001 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  10. Atmospheric Radiation Measurement Program Climate Research Facility...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    1 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-12-001 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  11. Atmospheric Radiation Measurement Program Climate Research Facility...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    8 Atmospheric Radiation Measurement Program Climate Research Facility Operations Quarterly ... DOESC-ARM-11-008 Atmospheric Radiation Measurement Program Climate Research Facility ...

  12. Atmospheric Radiation Measurement Program Climate Research Facility...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    9 Atmospheric Radiation Measurement Program Climate Research Facility Operations Quarterly ... DOESC-ARM-10-029 Atmospheric Radiation Measurement Program Climate Research Facility ...

  13. Atmospheric Radiation Measurement (ARM) Climate Research Facility...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Atmospheric Radiation Measurement (ARM) Climate Research Facility and Atmospheric System Research (ASR) Science and Infrastructure Steering Committee CHARTER June 2012 DISCLAIMER ...

  14. Atmospheric Radiation Measurement Climate Research Facility ...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ... of Energy (DOE) established the Atmospheric Radiation Measurement (ARM) Program. ... Fiscal Year 2004 Budget Summary and User Statistics Atmospheric Radiation Measurement ...

  15. Atmospheric Radiation Measurement Program Climate Research Facility...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    2 Atmospheric Radiation Measurement Program Climate Research Facility Operations Quarterly ... DOESC-ARM-11-002 Atmospheric Radiation Measurement Program Climate Research Facility ...

  16. Atmospheric Radiation Measurement Climate Research Facility Operations...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    9 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-15-069 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  17. Atmospheric Radiation Measurement Program Climate Research Facility...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    2 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-11-022 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  18. Atmospheric Radiation Measurement Program Climate Research Facility...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    9 Atmospheric Radiation Measurement Program Climate Research Facility Operations Quarterly ... DOESC-ARM-11-019 Atmospheric Radiation Measurement Program Climate Research Facility ...

  19. Atmospheric Radiation Measurement Program Climate Research Facility...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    7 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-12-007 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  20. Improving the homogeneity of alternating current-drive atmospheric pressure dielectric barrier discharges in helium with an additional low-amplitude radio frequency power source: A numerical study

    SciTech Connect (OSTI)

    Wang Qi [Dalian Institute of Semiconductor Technology, School of Electronics Science and Technology, Dalian University of Technology, Dalian 116023 (China); Sun Jizhong; Zhang Jianhong; Wang Dezhen [School of Physics and Optoelectronic Technology, Dalian University of Technology, Dalian 116023 (China); Liu Liying [Department of Electrical Engineering, Shenyang Institute of Engineering, Shenyang 110136 (China)

    2013-04-15

    It was proposed in this paper that the homogeneity of the atmospheric pressure discharge driven by an ac power source could be improved by applying an auxiliary low-amplitude rf power source. To verify the idea, a two-dimensional fluid model then was applied to study the atmospheric discharges in helium driven by ac power, low-amplitude rf power, and combined ac and low-amplitude rf power, respectively. Simulation results confirmed that an auxiliary rf power could improve the homogeneity of a discharge driven by an ac power source. It was further found that there existed a threshold voltage of the rf power source leading to the transition from inhomogeneous to homogeneous discharge. As the frequency of the rf power source increased from 2 to 22 MHz, the magnitude of the threshold voltage dropped first rapidly and then to a constant value. When the frequency was over 13.56 MHz, the magnitude of the threshold voltage was smaller than one-sixth of the ac voltage amplitude under the simulated discharge parameters.

  1. Atmospheric Pressure Chemical Vapor Deposition of High Silica SiO2-TiO2 Antireflective Thin Films for Glass Based Solar Panels

    SciTech Connect (OSTI)

    Klobukowski, Erik R; Tenhaeff, Wyatt E; McCamy, James; Harris, Caroline; Narula, Chaitanya Kumar

    2013-01-01

    The atmospheric pressure chemical vapor deposition (APCVD) of SiO2-TiO2 thin films employing [[(tBuO)3Si]2O-Ti(OiPr)2], which can be prepared from commercially available materials, results in antireflective thin films on float glass under industrially relevant manufacturing conditions. It was found that while the deposition temperature had an effect on the SiO2:TiO2 ratio, the thickness was dependent on the time of deposition. This study shows that it is possible to use APCVD employing a single source precursor containing titanium and silicon to produce thin films on float glass with high SiO2:TiO2 ratios.

  2. Atmospheric Chemistry and Air Pollution

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Gaffney, Jeffrey S.; Marley, Nancy A.

    2003-01-01

    Atmospheric chemistry is an important discipline for understanding air pollution and its impacts. This mini-review gives a brief history of air pollution and presents an overview of some of the basic photochemistry involved in the production of ozone and other oxidants in the atmosphere. Urban air quality issues are reviewed with a specific focus on ozone and other oxidants, primary and secondary aerosols, alternative fuels, and the potential for chlorine releases to amplify oxidant chemistry in industrial areas. Regional air pollution issues such as acid rain, long-range transport of aerosols and visibility loss, and the connections of aerosols to ozonemore » and peroxyacetyl nitrate chemistry are examined. Finally, the potential impacts of air pollutants on the global-scale radiative balances of gases and aerosols are discussed briefly.« less

  3. Atmosphere to Electrons Program Overview

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Atmosphere to Electrons (A2e) Initiative Overview DOE Wind and Water Power Technologies Office January 2014 2 * Motivation for a new R&D framework * A2e initiative overview - Strategic planning framework - Management construct - Executive Management Committee (EMC) - National Laboratory Leadership * Strategic thrust area planning introduction * Program objectives * Open discussion of approach Overview Agenda 3 Wind energy today ..... * Multi-Billion dollar industry with involvement of

  4. DEFRA Global Atmosphere Dept | Open Energy Information

    Open Energy Info (EERE)

    Kingdom Zip: SW1E 6DE Product: Atmosphere research department of the UK Department of Food and Rural Affairs. References: DEFRA - Global Atmosphere Dept.1 This article is a...

  5. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused

  6. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused

  7. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused

  8. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Composition and Reactions of Atmospheric Aerosol Particles Print Wednesday, 29 June 2005 00:00 Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the

  9. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused

  10. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Composition and Reactions of Atmospheric Aerosol Particles Print Microscopic aerosol particles in the atmosphere contain carbonaceous components from mineral dust and combustion emissions released from around the world. How long these tiny particles remain in the atmosphere can have a huge impact on the global climate. Measurements based on high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused

  11. Quantitative determination of atmospheric hydroperoxyl radical

    DOE Patents [OSTI]

    Springston, Stephen R. (Upton, NY); Lloyd, Judith (Westbury, NY); Zheng, Jun (Stony Brook, NY)

    2007-10-23

    A method for the quantitative determination of atmospheric hydroperoxyl radical comprising: (a) contacting a liquid phase atmospheric sample with a chemiluminescent compound which luminesces on contact with hydroperoxyl radical; (b) determining luminescence intensity from the liquid phase atmospheric sample; and (c) comparing said luminescence intensity from the liquid phase atmospheric sample to a standard luminescence intensity for hydroperoxyl radical. An apparatus for automating the method is also included.

  12. Atmosphere to Electrons | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Research & Development » Atmosphere to Electrons Atmosphere to Electrons Atmosphere to Electrons Atmosphere to Electrons (A2e) is a multi-year U.S. Department of Energy (DOE) research initiative targeting significant reductions in the cost of wind energy through an improved understanding of the complex physics governing wind flow into and through wind farms. Better insight into the flow physics has the potential to reduce wind farm energy losses by up to 20%, to reduce annual operational

  13. Radar range measurements in the atmosphere. (Technical Report...

    Office of Scientific and Technical Information (OSTI)

    Radar range measurements in the atmosphere. Citation Details In-Document Search Title: Radar range measurements in the atmosphere. The earth's atmosphere affects the velocity of...

  14. Regional Ecosystem-Atmosphere CO2 Exchange Via Atmospheric Budgets

    SciTech Connect (OSTI)

    Davis, K.J.; Richardson, S.J.; Miles, N.L.

    2007-03-07

    Inversions of atmospheric CO2 mixing ratio measurements to determine CO2 sources and sinks are typically limited to coarse spatial and temporal resolution. This limits our ability to evaluate efforts to upscale chamber- and stand-level CO2 flux measurements to regional scales, where coherent climate and ecosystem mechanisms govern the carbon cycle. As a step towards the goal of implementing atmospheric budget or inversion methodology on a regional scale, a network of five relatively inexpensive CO2 mixing ratio measurement systems was deployed on towers in northern Wisconsin. Four systems were distributed on a circle of roughly 150-km radius, surrounding one centrally located system at the WLEF tower near Park Falls, WI. All measurements were taken at a height of 76 m AGL. The systems used single-cell infrared CO2 analyzers (Licor, model LI-820) rather than the siginificantly more costly two-cell models, and were calibrated every two hours using four samples known to within 0.2 ppm CO2. Tests prior to deployment in which the systems sampled the same air indicate the precision of the systems to be better than 0.3 ppm and the accuracy, based on the difference between the daily mean of one system and a co-located NOAA-ESRL system, is consistently better than 0.3 ppm. We demonstrate the utility of the network in two ways. We interpret regional CO2 differences using a Lagrangian parcel approach. The difference in the CO2 mixing ratios across the network is at least 2?3 ppm, which is large compared to the accuracy and precision of the systems. Fluxes estimated assuming Lagrangian parcel transport are of the same sign and magnitude as eddy-covariance flux measurements at the centrally-located WLEF tower. These results indicate that the network will be useful in a full inversion model. Second, we present a case study involving a frontal passage through the region. The progression of a front across the network is evident; changes as large as four ppm in one minute are captured. Influence functions, derived using a Lagrangian Particle Dispersion model driven by the CSU Regional Atmospheric Modeling System and nudged to NCEP reanalysis meteorological fields, are used to determine source regions for the towers. The influence functions are combined with satellite vegetation observations to interpret the observed trends in CO2 concentration. Full inversions will combine these elements in a more formal analytic framework.

  15. Modeling of plasma chemistry in an atmospheric pressure Ar/NH{sub 3} cylindrical dielectric barrier discharge described using the one-dimensional fluid model

    SciTech Connect (OSTI)

    Li Zhi [School of Science, University of Science and Technology Liaoning, Anshan 114051 (China); School of Physics and Optoelectronic Engineering, Dalian University of Technology, Dalian 116024 (China); Zhao Zhen [School of Chemistry and Life Science, Anshan Normal University, Anshan 114007 (China); School of Chemical Engineering, University of Science and Technology Liaoning, Anshan 114051 (China); Li Xuehui [Physical Science and Technical College, Dalian University, Dalian 116622 (China)

    2013-01-15

    The keynote of our research is to study the gas phase chemistry in an atmospheric pressure Ar/NH{sub 3} cylindrical dielectric barrier discharge, which is very important to produce the iron-nitride magnetic fluid. For this purpose, a home-made one dimensional fluid model with the Scharfetter-Gummel method has been developed. The equations solved are the particle balances, assuming a drift-diffusion approximation for the fluxes, and the electron energy equation. The self-consistent electric field is obtained by the simultaneous solution of Poisson's equation. The simulations were carried out for the different ammonia concentrations (2%, 3.5%, and 7%), at a voltage of 1 kV, and a driving frequency of 20 kHz. It concluded that the major ion products of Ar are Ar{sup +} and Ar{sub 2}{sup +}. Ar{sup +} is the most important positive ions, followed by Ar{sub 2}{sup +}. It is shown that the NH{sup +} density is smaller than that of the other ammonia ions. The density of NH{sub 4}{sup +} is more than that of the other ammonia ions when the ammonia concentration increased. The diffuse mode can be established after the discharge was ignited, and the mode changes to filamentary mode with an increase in ammonia concentration.

  16. Characteristics of atmospheric-pressure non-thermal N{sub 2} and N{sub 2}/O{sub 2} gas mixture plasma jet

    SciTech Connect (OSTI)

    Xiao, Dezhi; Shen, Jie; Lan, Yan; Xie, Hongbing; Shu, Xingsheng; Meng, Yuedong; Li, Jiangang; Cheng, Cheng E-mail: paul.chu@cityu.edu.hk; Chu, Paul K. E-mail: paul.chu@cityu.edu.hk

    2014-01-21

    An atmospheric-pressure non-thermal plasma jet driven by high frequency alternating current and operating on N{sub 2} and N{sub 2}/O{sub 2} gas mixture is investigated. The plasma jet can reach 55?mm in length at a gas flow rate of 2500?l/h. The gas temperature at a distance of 4?mm from the nozzle is close to room temperature. Optical emission spectroscopy is employed to investigate the important plasma parameters such as the excited species, rotational temperature, vibrational temperature, and excitation temperature under different discharge conditions. The results show that the plasma source operates under non-equilibrium conditions. The absolute irradiance intensity of the vibrational band N{sub 2}(C-B) in the active region is measured. Taking into account the irradiance intensity of N{sub 2}(C-B,0-0) and N{sub 2}(B-X,0-0) as well as measured current, the electron density, which is determined by considering direct and step-wise electron impact excitation of nitrogen emission, reaches a maximum value of 5.6??10{sup 20}/m{sup 3}.

  17. Broadband Outdoor Radiometer Callibration Process for the Atmospheric...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Broadband Outdoor Radiometer Calibration Process for the Atmospheric Radiation Measurement ... Broadband Outdoor Radiometer Calibration Process for the Atmospheric Radiation Measurement ...

  18. National Oceanic and Atmospheric Administration, Honolulu, Hawaii |

    Office of Environmental Management (EM)

    Department of Energy Oceanic and Atmospheric Administration, Honolulu, Hawaii National Oceanic and Atmospheric Administration, Honolulu, Hawaii Photo of a Staff Residence at the Pacific Tsunami Warning Center in Hawaii The staff residences at the Pacific Tsunami Warning Center in Hawaii now have solar water heating systems funded by the Federal Energy Management Program (FEMP). The Center is part of the Department of Commerce's National Oceanic and Atmospheric Administration (DOC-NOAA). New

  19. Composition and Reactions of Atmospheric Aerosol Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    high-resolution scanning transmission x-ray images obtained at the ALS have revealed chemical reactions on and in atmospheric aerosol particles that caused particle growth while...

  20. Precision Determination of Atmospheric Extinction at Optical...

    Office of Scientific and Technical Information (OSTI)

    a technique to implement a new strategy to directly measure variations of atmospheric transmittance at optical wavelengths and application of these measurements to calibration...

  1. Atmospheric Dispersion Modeling in Safety Analyses; GENII

    Office of Environmental Management (EM)

    part of GENII) 5 GENII Acute Atmospheric Transport Straight-line (centerline) Gaussian plume for individuals For short duration releases (2 hours) Single source...

  2. Atmosphere to Electrons Program Overview Presentation

    Broader source: Energy.gov [DOE]

    This presentation provides an introduction to the Atmosphere to Electrons (A2e) initiative, including objectives, program areas, and a general timeline of activities.

  3. Precision Determination of Atmospheric Extinction at Optical...

    Office of Scientific and Technical Information (OSTI)

    spectra by their characteristic dependences on wavelength and airmass. State-of-the-art models of atmospheric radiation transport and modern codes are used to accurately...

  4. An Instrumentation Complex for Atmospheric Radiation Measurements...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Instrumentation Complex for Atmospheric Radiation Measurements in Siberia S. M. Sakerin, F. V. Dorofeev, D. M. Kabanov, V. S. Kozlov, M. V. Panchenko, Yu. A. Pkhalagov, V. V. ...

  5. Session Papers Atmospheric Radiation Measurement Program- Unmanned...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Session Papers Atmospheric Radiation Measurement Program- Unmanned Aerospace Vehicle: The Follow-On Phase J. Vitko, Jr. ARM-UAV Technical Director Sandia National Laboratories ...

  6. Atmospheric Radiation Measurement Tropical Warm Pool International...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    The Tropical Warm Pool - International Cloud Experiment (TWP-ICE) was a collaborative effort led by the U.S. Department of Energy's Atmospheric Radiation Measurement (ARM) Program ...

  7. Atmospheric Radiation Measurement Convective and Orographically...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Convective and Orographically Induced Precipitation Study The U.S. Department of Energy's Atmospheric Radiation Measurement (ARM) Climate Research Facility is providing the ARM ...

  8. Parametric study of atmospheric pressure microwave-induced Ar/O{sub 2} plasmas and the ambient air effect on the plasma

    SciTech Connect (OSTI)

    Moon, Se Youn; Choe, W.

    2006-10-15

    A torch type microwave-induced afterglow plasma was produced at atmospheric pressure using an open-ended fused silica concentric double tube assisted by Ar and O{sub 2} supply gases. The plasma emerged from the end of the discharge tube and was exposed to ambient air. A parametric study of the plasma characteristics was performed by measuring the temperature, density, and plasma volume as the operational parameters such as microwave power, gas flow rate, and its composition were varied. The excitation temperature (T{sub exc}) obtained from the Ar I emission spectrum ranged from 3010 to 4350 K and the rotational temperature (T{sub rot}) measured from the OH and O{sub 2} diatomic molecular spectra ranged from 2250 to 3550 K. The electron density (n{sub e}) from the H{sub {beta}} Stark broadening width at the plasma core was in the range of 6.6 to 7.6x10{sup 14} cm{sup -3}. The two-dimensional distribution of T{sub exc} and T{sub rot} was also obtained. Experiments while varying the Ar and O{sub 2} gas flow rate and the O{sub 2}/Ar ratio showed that n{sub e} was reduced but T{sub exc} was increased as the O{sub 2} flow rate was increased. Using an additional dielectric tube for shielding the plasma from the ambient air demonstrated a significantly enlarged plasma length and lower T{sub rot} due to the nitrogen entrainment, as compared to the unshielded case.

  9. SULI Intern: Atmospheric Science | Argonne National Laboratory

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Atmospheric Science Share Hear how Argonne intern Jane Pan helped scientists accurately represent atmospheric conditions in computer models and forecasts. Browse By - Any - Energy -Energy efficiency --Vehicles ---Alternative fuels ---Automotive engineering ---Diesel ---Electric drive technology ---Hybrid & electric vehicles ---Hydrogen & fuel cells ---Internal combustion ---Powertrain research --Building design ---Construction --Manufacturing -Energy sources --Renewable energy

  10. NREL: Process Development and Integration Laboratory - Atmospheric

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Processing Platform Capabilities Atmospheric Processing Platform Capabilities The Atmospheric Processing platform in the Process Development and Integration Laboratory offers powerful capabilities with integrated tools for depositing, processing, and characterizing photovoltaic materials and devices. In particular, this platform focuses on different methods to deposit ("write") materials onto a variety of substrates and then further process into optoelectronic materials using rapid

  11. Atmospheric transmittance model for photosynthetically active radiation

    SciTech Connect (OSTI)

    Paulescu, Marius; Stefu, Nicoleta; Gravila, Paul; Paulescu, Eugenia; Boata, Remus; Pacurar, Angel; Mares, Oana; Pop, Nicolina; Calinoiu, Delia

    2013-11-13

    A parametric model of the atmospheric transmittance in the PAR band is presented. The model can be straightforwardly applied for calculating the beam, diffuse and global components of the PAR solar irradiance. The required inputs are: air pressure, ozone, water vapor and nitrogen dioxide column content, ngstrm's turbidity coefficient and single scattering albedo. Comparison with other models and ground measured data shows a reasonable level of accuracy for this model, making it suitable for practical applications. From the computational point of view the calculus is condensed into simple algebra which is a noticeable advantage. For users interested in speed-intensive computation of the effective PAR solar irradiance, a PC program based on the parametric equations along with a user guide are available online at http://solar.physics.uvt.ro/srms.

  12. SWiFT site atmospheric characterization

    SciTech Connect (OSTI)

    Kelley, Christopher Lee; Ennis, Brandon Lee

    2016-01-01

    Historical meteorological tall tower data are analyzed from the Texas Tech University 200 m tower to characterize the atmospheric trends of the Scaled Wind Farm Technologies (SWiFT) site. In this report the data are analyzed to reveal bulk atmospheric trends, temporal trends and correlations of atmospheric variables. Through this analysis for the SWiFT turbines the site International Electrotechnical Commission (IEC) classification is determined to be class III-C. Averages and distributions of atmospheric variables are shown, revealing large fluctuations and the importance of understanding the actual site trends as opposed to simply using averages. The site is significantly directional with the average wind speed from the south, and particularly so in summer and fall. Site temporal trends are analyzed from both seasonal (time of the year) to daily (hour of the day) perspectives. Atmospheric stability is seen to vary most with time of day and less with time of year. Turbulence intensity is highly correlated with stability, and typical daytime unstable conditions see double the level of turbulence intensity versus that experienced during the average stable night. Shear, veer and atmospheric stability correlations are shown, where shear and veer are both highest for stable atmospheric conditions. An analysis of the Texas Tech University tower anemometer measurements is performed which reveals the extent of the tower shadow effects and sonic tilt misalignment.

  13. Pavlos Kollias Associate Professor Department of Atmospheric...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Pavlos Kollias Associate Professor Department of Atmospheric and Oceanic Sciences, McGill University Room 817, Burnside Hall, 805 Sherbrooke Street West, Montreal, Quebec, H3A 0B9...

  14. Operating Experience Level 3, Atmospheric Dispersion Parameter...

    Broader source: Energy.gov (indexed) [DOE]

    5 OE-3 2015-02: Atmospheric Dispersion Parameter (xQ) for Calculation of Co-located Worker Dose This Operating Experience Level 3 (OE-3) document informs the complex of the...

  15. Impact of atmospheric refraction: how deeply can we probe exo-earth's atmospheres during primary eclipse observations?

    SciTech Connect (OSTI)

    Btrmieux, Yan; Kaltenegger, Lisa

    2014-08-10

    Most models used to predict or fit exoplanet transmission spectra do not include all the effects of atmospheric refraction. Namely, the angular size of the star with respect to the planet can limit the lowest altitude, or highest density and pressure, probed during primary eclipses as no rays passing below this critical altitude can reach the observer. We discuss this geometrical effect of refraction for all exoplanets and tabulate the critical altitude, density, and pressure for an exoplanet identical to Earth with a 1 bar N{sub 2}/O{sub 2} atmosphere as a function of both the incident stellar flux (Venus, Earth, and Mars-like) at the top of the atmosphere and the spectral type (O5-M9) of the host star. We show that such a habitable exo-Earth can be probed to a surface pressure of 1 bar only around the coolest stars. We present 0.4-5.0 ?m model transmission spectra of Earth's atmosphere viewed as a transiting exoplanet, and show how atmospheric refraction modifies the transmission spectrum depending on the spectral type of the host star. We demonstrate that refraction is another phenomenon that can potentially explain flat transmission spectra over some spectral regions.

  16. Analysis and experimental study on formation conditions of large-scale barrier-free diffuse atmospheric pressure air plasmas in repetitive pulse mode

    SciTech Connect (OSTI)

    Li, Lee Liu, Lun; Liu, Yun-Long; Bin, Yu; Ge, Ya-Feng; Lin, Fo-Chang

    2014-01-14

    Atmospheric air diffuse plasmas have enormous application potential in various fields of science and technology. Without dielectric barrier, generating large-scale air diffuse plasmas is always a challenging issue. This paper discusses and analyses the formation mechanism of cold homogenous plasma. It is proposed that generating stable diffuse atmospheric plasmas in open air should meet the three conditions: high transient power with low average power, excitation in low average E-field with locally high E-field region, and multiple overlapping electron avalanches. Accordingly, an experimental configuration of generating large-scale barrier-free diffuse air plasmas is designed. Based on runaway electron theory, a low duty-ratio, high voltage repetitive nanosecond pulse generator is chosen as a discharge excitation source. Using the wire-electrodes with small curvature radius, the gaps with highly non-uniform E-field are structured. Experimental results show that the volume-scaleable, barrier-free, homogeneous air non-thermal plasmas have been obtained between the gap spacing with the copper-wire electrodes. The area of air cold plasmas has been up to hundreds of square centimeters. The proposed formation conditions of large-scale barrier-free diffuse air plasmas are proved to be reasonable and feasible.

  17. Atmospheric State, Cloud Microphysics and Radiative Flux

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Mace, Gerald

    2008-01-15

    Atmospheric thermodynamics, cloud properties, radiative fluxes and radiative heating rates for the ARM Southern Great Plains (SGP) site. The data represent a characterization of the physical state of the atmospheric column compiled on a five-minute temporal and 90m vertical grid. Sources for this information include raw measurements, cloud property and radiative retrievals, retrievals and derived variables from other third-party sources, and radiative calculations using the derived quantities.

  18. Air Activation Following an Atmospheric Explosion

    SciTech Connect (OSTI)

    Lowrey, Justin D.; McIntyre, Justin I.; Prichard, Andrew W.; Gesh, Christopher J.

    2013-03-13

    In addition to thermal radiation and fission products, nuclear explosions result in a very high flux of unfissioned neutrons. Within an atmospheric nuclear explosion, these neutrons can activate the various elemental components of natural air, potentially adding to the radioactive signature of the event as a whole. The goal of this work is to make an order-of-magnitude estimate of the total amount of air activation products that can result from an atmospheric nuclear explosion.

  19. Atmospheric and Climate Science | Argonne National Laboratory

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Atmospheric and Climate Science Argonne research in aerosols, micro-meteorology, remote sensing, and atmospheric chemistry combined with our scalable, portable, high-performance climate and weather applications offer a unique look at the complexities of a dynamic planet. Changes in climate can affect biodiversity, the cost of food, our health, and even whole economies. Argonne is developing computational models and tools designed to shed light on complex biological processes and their economic,

  20. Atmospheric State, Cloud Microphysics and Radiative Flux

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Mace, Gerald

    Atmospheric thermodynamics, cloud properties, radiative fluxes and radiative heating rates for the ARM Southern Great Plains (SGP) site. The data represent a characterization of the physical state of the atmospheric column compiled on a five-minute temporal and 90m vertical grid. Sources for this information include raw measurements, cloud property and radiative retrievals, retrievals and derived variables from other third-party sources, and radiative calculations using the derived quantities.

  1. Atmospheric Neutrinos in the MINOS Far Detector

    SciTech Connect (OSTI)

    Howcroft, Caius L.F.

    2004-12-01

    The phenomenon of flavour oscillations of neutrinos created in the atmosphere was first reported by the Super-Kamiokande collaboration in 1998 and since then has been confirmed by Soudan 2 and MACRO. The MINOS Far Detector is the first magnetized neutrino detector able to study atmospheric neutrino oscillations. Although it was designed to detect neutrinos from the NuMI beam, it provides a unique opportunity to measure the oscillation parameters for neutrinos and anti-neutrinos independently. The MINOS Far Detector was completed in August 2003 and since then has collected 2.52 kton-years of atmospheric data. Atmospheric neutrino interactions contained within the volume of the detector are separated from the dominant background from cosmic ray muons. Thirty seven events are selected with an estimated background contamination of less than 10%. Using the detector's magnetic field, 17 neutrino events and 6 anti-neutrino events are identified, 14 events have ambiguous charge. The neutrino oscillation parameters for {nu}{sub {mu}} and {bar {nu}}{sub {mu}} are studied using a maximum likelihood analysis. The measurement does not place constraining limits on the neutrino oscillation parameters due to the limited statistics of the data set analysed. However, this thesis represents the first observation of charge separated atmospheric neutrino interactions. It also details the techniques developed to perform atmospheric neutrino analyses in the MINOS Far Detector.

  2. Radon Measurements of Atmospheric Mixing (RAMIX) 2006-2014 Final...

    Office of Scientific and Technical Information (OSTI)

    Title: Radon Measurements of Atmospheric Mixing (RAMIX) 2006-2014 Final Campaign Summary ... estimates of regional land-atmosphere carbon exchange (i.e., estimates based on ...

  3. Global Atmospheric Pollution Forum Air Pollutant Emission Inventory...

    Open Energy Info (EERE)

    Atmospheric Pollution Forum Air Pollutant Emission Inventory Jump to: navigation, search Tool Summary LAUNCH TOOL Name: Global Atmospheric Pollution (GAP) Forum Air Pollutant...

  4. Radar range measurements in the atmosphere. (Technical Report...

    Office of Scientific and Technical Information (OSTI)

    Radar range measurements in the atmosphere. Citation Details In-Document Search Title: Radar range measurements in the atmosphere. You are accessing a document from the...

  5. Simulation and Theory of Ions at Atmospherically Relevant Aqueous...

    Office of Scientific and Technical Information (OSTI)

    Simulation and Theory of Ions at Atmospherically Relevant Aqueous Liquid-Air Interfaces Citation Details In-Document Search Title: Simulation and Theory of Ions at Atmospherically...

  6. A marine biogenic source of atmospheric ice-nucleating particles...

    Office of Scientific and Technical Information (OSTI)

    A marine biogenic source of atmospheric ice-nucleating particles Citation Details In-Document Search Title: A marine biogenic source of atmospheric ice-nucleating particles The ...

  7. Model-Observation "Data Cubes" for the DOE Atmospheric Radiation...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Model-Observation "Data Cubes" for the DOE Atmospheric Radiation Measurement Facility's ... Program through its Atmospheric Radiation Measurement Facility. 2. Data Cube ...

  8. Posters Single-Column Model for Atmospheric Radiation Measurement...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Posters Single-Column Model for AtmosphericRadiation Measurement Sites: Model Development ... Using observational data obtained from the Oklahoma Atmospheric Radiation Measurement ...

  9. A U. S. Department of Energy User Facility Atmospheric Radiation

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    S. Department of Energy User Facility AtmosphericRadiationMeasurement Climate Research Facility U.S. Department of Energy Atmospheric Radiation Measurement Program DOESC-ARM...

  10. Session Papers Quality Measurement Experiments Within the Atmospheric...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Quality Measurement Experiments Within the Atmospheric Radiation Measurement Program N. E. ... Introduction The general goal of the Atmospheric RadiationMeasurement (ARM) Program is to ...

  11. Modeling Workflow for the DOE Atmospheric Radiation Measurement...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Workflow for the DOE Atmospheric Radiation Measurement Facility's LES ARM Symbiotic ... and Environmental Research Program through its Atmospheric Radiation Measurement Facility. ...

  12. ARMlUnmanned Air VehiclelSatelites The Atmospheric Radiation...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ARMlUnmanned Air VehiclelSatelites The Atmospheric Radiation Measurement Unmanned ... This program has its origins in the Atmospheric RadiationMeasurement (ARM) Program's long ...

  13. DOE/SC-ARM-020 Atmospheric Radiation Measurement Climate Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    20 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-020 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  14. Posters Objective Analysis Schemes to Monitor Atmospheric Radiation...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Objective Analysis Schemes to Monitor AtmosphericRadiation Measurement Data in Near ... large networks of instruments such as the AtmosphericRadiation Measurement (ARM) Program. ...

  15. Style Guide Atmospheric Radiation Measurement (ARM) Climate Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Style Guide Atmospheric Radiation Measurement (ARM) Climate Research Facility March 2013 Style Guide Atmospheric Radiation Measurement Climate Research Facility March 2013 Work ...

  16. A Decade of Atmospheric Research in the Tropical Western Pacific...

    Office of Science (SC) Website

    The Atmospheric Radiation Measurement (ARM) Climate Research Facility has three user ... The Science The Department of Energy's Atmospheric Radiation Measurement (ARM) Climate ...

  17. Multi-scale Atmospheric Modeling of Green House Gas Dispersion in Complex Terrain. Atmospheric Methane at Four Corners

    SciTech Connect (OSTI)

    Costigan, Keeley Rochelle; Dubey, Manvendra Krishna

    2015-07-10

    Atmospheric models are compared in collaboration with LANL and the University of Michigan to understand emissions and the condition of the atmosphere from a model perspective.

  18. Controlled atmosphere for fabrication of cermet electrodes

    DOE Patents [OSTI]

    Ray, Siba P. (Murrysville, PA); Woods, Robert W. (New Kensington, PA)

    1998-01-01

    A process for making an inert electrode composite wherein a metal oxide and a metal are reacted in a gaseous atmosphere at an elevated temperature of at least about 750.degree. C. The metal oxide is at least one of the nickel, iron, tin, zinc and zirconium oxides and the metal is copper, silver, a mixture of copper and silver or a copper-silver alloy. The gaseous atmosphere has an oxygen content that is controlled at about 5-3000 ppm in order to obtain a desired composition in the resulting composite.

  19. Our Dusty Atmosphere | Department of Energy

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Dusty Atmosphere Our Dusty Atmosphere September 6, 2011 - 4:26pm Addthis A heavy layer of air pollution, a mix of aerosol particles and vapors, obscures the view over Mexico City. Two studies by the Pacific Northwest National Laboratory show the importance of including the small-scale effects of aerosols in climate modeling. | Image courtesy of PNNL A heavy layer of air pollution, a mix of aerosol particles and vapors, obscures the view over Mexico City. Two studies by the Pacific Northwest

  20. Controlled atmosphere for fabrication of cermet electrodes

    DOE Patents [OSTI]

    Ray, S.P.; Woods, R.W.

    1998-08-11

    A process is disclosed for making an inert electrode composite wherein a metal oxide and a metal are reacted in a gaseous atmosphere at an elevated temperature of at least about 750 C. The metal oxide is at least one of the nickel, iron, tin, zinc and zirconium oxides and the metal is copper, silver, a mixture of copper and silver or a copper-silver alloy. The gaseous atmosphere has an oxygen content that is controlled at about 5--3000 ppm in order to obtain a desired composition in the resulting composite. 2 figs.

  1. Temperature measurement of an atmospheric pressure arc discharge plasma jet using the diatomic CN (B {sup 2}{sigma}{sup +}-X {sup 2}{sigma}{sup +}, violet system) molecular spectra

    SciTech Connect (OSTI)

    Moon, Se Youn; Kim, D. B.; Gweon, B.; Choe, W.

    2009-03-01

    The CN (B {sup 2}{sigma}{sup +}-X {sup 2}{sigma}{sup +}) molecular emission spectrum is used to measure both the vibrational and rotational temperatures in atmospheric pressure arc jet discharges. The vibrational and rotational temperature effects on the synthetic diatomic molecular spectra were investigated from the (v{sup '},v{sup ''})=(0,0) band to the (5,5) band. The temperatures obtained from the synthetic spectra compared with the experimental result of a low-frequency arc discharge show a vibrational temperature of (4250-5010) K and a rotational temperature of (3760-3980) K for the input power in the range of (80-280) W. As the (0,0) band is isolated from other vibrational transition bands, determination of the rotational temperature is possible based only on the (0,0) band, which simplifies the temperature measurement. From the result, it was found that the CN molecular spectrum can be used as a thermometer for atmospheric pressure plasmas containing carbon and nitrogen.

  2. Atmosphere contamination following repainting of a human hyperbaric chamber complex

    SciTech Connect (OSTI)

    Lillo, R.S.; Morris, J.W.; Caldwell, J.M.; Balk, D.M.; Flynn, E.T. )

    1990-09-01

    The Naval Medical Research Institute currently conducts hyperbaric research in a Man-Rated Chamber Complex (MRCC) originally installed in 1977. Significant engineering alterations to the MRCC and rusting of some of its interior sections necessitated repainting, which was completed in 1988. Great care was taken in selecting an appropriate paint (polyamide epoxy) and in ensuring correct application and curing procedures. Only very low levels of hydrocarbons were found in the MRCC atmosphere before initial pressurization after painting and curing. After pressurization, however, significant chemical contamination was found. The primary contaminants were aromatic hydrocarbons: xylenes (which were a major component of both the primer and topcoat paint) and ethyl benzene. The role that pressure played in stimulating off-gassing from the paint is not clear; the off-gassing rate was observed to be similar over a large range in chamber pressures from 1.6 to 31.0 atm abs. Scrubbing the chamber atmosphere with the chemical absorbent Purafil was effective in removing the contaminants. Contamination has been observed to slowly decline with chamber use and is expected to continue to improve with time. However, this contamination experience emphasizes the need for a high precision gas analysis program at any diving facility to ensure the safety of the breathing gas and chamber atmosphere.

  3. Connectivity To Atmospheric Release Advisory Capability

    Broader source: Directives, Delegations, and Requirements [Office of Management (MA)]

    2001-02-26

    To establish DOE and NNSA connectivity to Atmospheric Release Advisory Capability (ARAC) for sites and facilities that have the potential for releasing hazardous materials sufficient to generate certain emergency declarations and to promote efficient use of resources for consequence assessment activities at DOE sites, facilities, operations, and activities in planning for and responding to emergency events. No cancellations.

  4. Application of lidar to current atmospheric topics

    SciTech Connect (OSTI)

    Sedlacek, A.J. III

    1996-12-31

    The goal of the conference was to address the various applications of lidar to topics of interest in the atmospheric community. Specifically, with the development of frequency-agile, all solid state laser systems, high-quantum-efficiency detectors, increased computational power along with new and more powerful algorithms, and novel detection schemes, the application of lidar to both old and new problems has expanded. This expansion is evidenced by the contributions to the proceedings, which demonstrate the progress made on a variety of atmospheric remote sensing problems, both theoretically and experimentally. The first session focused on aerosol, ozone, and temperature profile measurements from ground-based units. The second session, Chemical Detection, provided applications of lidar to the detection of atmospheric pollutants. Papers in the third session, Wind and Turbulence Measurements, described the Multi-center Airborne Coherent Atmospheric Wind Sensor (MACAWS) experiments, Doppler techniques for ground-based wind profiling and mesopause radial wind and temperature measurements utilizing a frequency-agile lidar system. The papers in the last two sessions, Recent Advanced in Lidar Technology and Techniques and Advanced Operational Lidars, provided insights into novel approaches, materials, and techniques that would be of value to the lidar community. Papers have been processed separately for inclusion on the data base.

  5. Atmospheric Science: Solving Challenges of Climate Change

    SciTech Connect (OSTI)

    Geffen, Charlette

    2015-08-05

    PNNLs atmospheric science research provides data required to make decisions about challenges presented by climate change: Where to site power plants, how to manage water resources, how to prepare for severe weather events and more. Our expertise in fundamental observations and modeling is recognized among the national labs and the world.

  6. CHARACTERIZATION OF CLOUDS IN TITAN'S TROPICAL ATMOSPHERE

    SciTech Connect (OSTI)

    Griffith, Caitlin A.; Penteado, Paulo; Rodriguez, Sebastien; Baines, Kevin H.; Buratti, Bonnie; Sotin, Christophe; Clark, Roger; Nicholson, Phil; Jaumann, Ralf

    2009-09-10

    Images of Titan's clouds, possible over the past 10 years, indicate primarily discrete convective methane clouds near the south and north poles and an immense stratiform cloud, likely composed of ethane, around the north pole. Here we present spectral images from Cassini's Visual Mapping Infrared Spectrometer that reveal the increasing presence of clouds in Titan's tropical atmosphere. Radiative transfer analyses indicate similarities between summer polar and tropical methane clouds. Like their southern counterparts, tropical clouds consist of particles exceeding 5 {mu}m. They display discrete structures suggestive of convective cumuli. They prevail at a specific latitude band between 8 deg. - 20 deg. S, indicative of a circulation origin and the beginning of a circulation turnover. Yet, unlike the high latitude clouds that often reach 45 km altitude, these discrete tropical clouds, so far, remain capped to altitudes below 26 km. Such low convective clouds are consistent with the highly stable atmospheric conditions measured at the Huygens landing site. Their characteristics suggest that Titan's tropical atmosphere has a dry climate unlike the south polar atmosphere, and despite the numerous washes that carve the tropical landscape.

  7. ANALYTICAL MODELS OF EXOPLANETARY ATMOSPHERES. I. ATMOSPHERIC DYNAMICS VIA THE SHALLOW WATER SYSTEM

    SciTech Connect (OSTI)

    Heng, Kevin; Workman, Jared E-mail: jworkman@coloradomesa.edu

    2014-08-01

    Within the context of exoplanetary atmospheres, we present a comprehensive linear analysis of forced, damped, magnetized shallow water systems, exploring the effects of dimensionality, geometry (Cartesian, pseudo-spherical, and spherical), rotation, magnetic tension, and hydrodynamic and magnetic sources of friction. Across a broad range of conditions, we find that the key governing equation for atmospheres and quantum harmonic oscillators are identical, even when forcing (stellar irradiation), sources of friction (molecular viscosity, Rayleigh drag, and magnetic drag), and magnetic tension are included. The global atmospheric structure is largely controlled by a single key parameter that involves the Rossby and Prandtl numbers. This near-universality breaks down when either molecular viscosity or magnetic drag acts non-uniformly across latitude or a poloidal magnetic field is present, suggesting that these effects will introduce qualitative changes to the familiar chevron-shaped feature witnessed in simulations of atmospheric circulation. We also find that hydrodynamic and magnetic sources of friction have dissimilar phase signatures and affect the flow in fundamentally different ways, implying that using Rayleigh drag to mimic magnetic drag is inaccurate. We exhaustively lay down the theoretical formalism (dispersion relations, governing equations, and time-dependent wave solutions) for a broad suite of models. In all situations, we derive the steady state of an atmosphere, which is relevant to interpreting infrared phase and eclipse maps of exoplanetary atmospheres. We elucidate a pinching effect that confines the atmospheric structure to be near the equator. Our suite of analytical models may be used to develop decisively physical intuition and as a reference point for three-dimensional magnetohydrodynamic simulations of atmospheric circulation.

  8. Perspective: Water cluster mediated atmospheric chemistry

    SciTech Connect (OSTI)

    Vaida, Veronica

    2011-07-14

    The importance of water in atmospheric and environmental chemistry initiated recent studies with results documenting catalysis, suppression and anti-catalysis of thermal and photochemical reactions due to hydrogen bonding of reagents with water. Water, even one water molecule in binary complexes, has been shown by quantum chemistry to stabilize the transition state and lower its energy. However, new results underscore the need to evaluate the relative competing rates between reaction and dissipation to elucidate the role of water in chemistry. Water clusters have been used successfully as models for reactions in gas-phase, in aqueous condensed phases and at aqueous surfaces. Opportunities for experimental and theoretical chemical physics to make fundamental new discoveries abound. Work in this field is timely given the importance of water in atmospheric and environmental chemistry.

  9. Pulsed atmospheric fluidized bed combustor apparatus

    DOE Patents [OSTI]

    Mansour, Momtaz N. (Columbia, MD)

    1993-10-26

    A pulsed atmospheric fluidized bed reactor system is disclosed and claimed along with a process for utilization of same for the combustion of, e.g. high sulfur content coal. The system affords a economical, ecologically acceptable alternative to oil and gas fired combustors. The apparatus may also be employed for endothermic reaction, combustion of waste products, e.g., organic and medical waste, drying materials, heating air, calcining and the like.

  10. Atmosphere to Electrons Initiative Takes Shape

    Broader source: Energy.gov [DOE]

    Since DOE launched its Atmosphere to Electrons (A2e) Initiative last July, the A2e executive committee has been developing a comprehensive approach for working with multiple stakeholders (industry, national laboratories, international experts, and universities) over the next 5- to 7 years. In February, they held an external merit review to lay the groundwork for an A2e multi-year strategic research plan.

  11. Emerging Technology for Measuring Atmospheric Aerosol Properties

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Technology for Measuring Atmospheric Aerosol Properties Bruce Gandrud Greg Kok Droplet Measurement Technologies Darrel Baumgardner Centro de Ciencias de la Atmósfera Universidad Nacional Autónoma de México Acknowledgements * The DMT staff * Bob Bluth and Haflidi Jonsson * Pat Arnott * Greg Roberts and Thanos Nenes * Dave Fahey, Shuka Schwarz and Ru-Shan Gao * NSF, NASA, ONR, NOAA and DOE Introducing Droplet Measurement Technologies * Founded in 1987 * Specializing in aerosol and cloud

  12. Atmospheric and combustion chemistry of dimethyl ether

    SciTech Connect (OSTI)

    Nielsen, O.J.; Egsgaard, H.; Larsen, E.; Sehested, J.; Wallington, T.J.

    1997-12-31

    It has been demonstrated that dimethyl ether (DME) is an ideal diesel fuel alternative. DME, CH{sub 3}OCH{sub 3}, combines good fuel properties with low exhaust emissions and low combustion noise. Large scale production of this fuel can take place using a single step catalytic process converting CH{sub 4} to DME. The fate of DME in the atmosphere has previously been studied. The atmospheric degradation is initiated by the reaction with hydroxyl radicals, which is also a common feature of combustion processes. Spectrokinetic investigations and product analysis were used to demonstrate that the intermediate oxy radical, CH{sub 3}OCH{sub 2}O, exhibits a novel reaction pathway of hydrogen atom ejection. The application of tandem mass spectrometry to chemi-ions based on supersonic molecular beam sampling has recently been demonstrated. The highly reactive ionic intermediates are sampled directly from the flame and identified by collision activation mass spectrometry and ion-molecule reactions. The mass spectrum reflects the distribution of the intermediates in the flame. The atmospheric degradation of DME as well as the unique fuel properties of a oxygen containing compound will be discussed.

  13. Formation and consumption of NO in H{sub 2} + O{sub 2} + N{sub 2} flames doped with NO or NH{sub 3} at atmospheric pressure

    SciTech Connect (OSTI)

    Shmakov, A.G.; Chernov, A.A.; Knyazkov, D.A.; Bolshova, T.A.; Korobeinichev, O.P.; Rybitskaya, I.V.; Konnov, A.A.

    2010-03-15

    Flat premixed burner-stabilized H{sub 2} + O{sub 2} + N{sub 2} flames, neat or doped with 300-1000 ppm of NO or NH{sub 3}, were studied experimentally using molecular-beam mass-spectrometry and simulated numerically. Spatial profiles of temperature and concentrations of stable species, H{sub 2}, O{sub 2}, H{sub 2}O, NO, NH{sub 3}, and of H and OH radicals obtained at atmospheric pressure in lean ({phi} = 0.47), near-stoichiometric ({phi} = 1.1) and rich ({phi} = 2.0) flames are reported. Good agreement between measured and calculated structure of lean and near-stoichiometric flames was found. Significant discrepancy between simulated and measured profiles of NO concentration was observed in the rich flames. Sensitivity and reaction path analyses revealed reactions responsible for the discrepancy. Modification to the model was proposed to improve an overall agreement with the experiment. (author)

  14. Atmospheric Radiation Measurement Program Science Plan

    SciTech Connect (OSTI)

    Ackerman, T

    2004-10-31

    The Atmospheric Radiation Measurement (ARM) Program has matured into one of the key programs in the U.S. Climate Change Science Program. The ARM Program has achieved considerable scientific success in a broad range of activities, including site and instrument development, atmospheric radiative transfer, aerosol science, determination of cloud properties, cloud modeling, and cloud parameterization testing and development. The focus of ARM science has naturally shifted during the last few years to an increasing emphasis on modeling and parameterization studies to take advantage of the long time series of data now available. During the next 5 years, the principal focus of the ARM science program will be to: Maintain the data record at the fixed ARM sites for at least the next five years. Improve significantly our understanding of and ability to parameterize the 3-D cloud-radiation problem at scales from the local atmospheric column to the global climate model (GCM) grid square. Continue developing techniques to retrieve the properties of all clouds, with a special focus on ice clouds and mixed-phase clouds. Develop a focused research effort on the indirect aerosol problem that spans observations, physical models, and climate model parameterizations. Implement and evaluate an operational methodology to calculate broad-band heating rates in the atmospheric columns at the ARM sites. Develop and implement methodologies to use ARM data more effectively to test atmospheric models, both at the cloud-resolving model scale and the GCM scale. Use these methodologies to diagnose cloud parameterization performance and then refine these parameterizations to improve the accuracy of climate model simulations. In addition, the ARM Program is actively developing a new ARM Mobile Facility (AMF) that will be available for short deployments (several months to a year or more) in climatically important regions. The AMF will have much of the same instrumentation as the remote facilities at ARM's Tropical Western Pacific and the North Slope of Alaska sites. Over time, this new facility will extend ARM science to a much broader range of conditions for model testing.

  15. Atmosphere to Electrons: Enabling the Wind Plant of Tomorrow

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Atmosphere to Electrons Enabling the Wind Plant of Tomorrow 2 Atmosphere to Electrons Enabling the Wind Plant of Tomorrow The U.S. Department of Energy's (DOE's) Atmosphere to Electrons (A2e) research initiative is focused on improving the performance and reliability of wind plants by establishing an unprecedented under- standing of how the Earth's atmosphere interacts with the wind plants and developing innovative technologies to maximize energy extraction from the wind. The A2e initiative

  16. DOE - NNSA/NFO -- Photo Library Atmospheric Testing

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Atmospheric NNSA/NFO Language Options U.S. DOE/NNSA - Nevada Field Office Photo Library - Atmospheric Testing A total of 100 atmospheric tests were conducted at the Nevada Test Site. These tests were conducted to provide information on weapons effects, effects of the height of burst on overpressure, and information on nuclear phenomena to improve the design of nuclear weapons. Atmospheric testing ceased for good in 1963, after which nuclear testing moved underground. Instructions: Click the

  17. Atmosphere to Electrons: Enabling the Wind Plant of Tomorrow | Department

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    of Energy Atmosphere to Electrons: Enabling the Wind Plant of Tomorrow Atmosphere to Electrons: Enabling the Wind Plant of Tomorrow a2e-fact-sheet-cover-thumbnail.jpg The U.S. Department of Energy's (DOE's) Atmosphere to Electrons (A2e) research initiative is focused on improving the performance and reliability of wind plants by establishing an unprecedented understanding of how the Earth's atmosphere interacts with the wind plants and developing innovative technologies to maximize energy

  18. Dynamic characteristic of intense short microwave propagation in an atmosphere

    SciTech Connect (OSTI)

    Yee, J.H.; Alvarez, R.A.; Mayhall, D.J.; Madsen, N.K.; Cabayan, H.S.

    1983-07-01

    The dynamic behavior of an intense microwave pulse which propagates through the atmosphere will be presented. Our theoretical results are obtained by solving Maxwell's equations, together with the electron fluid equations. Our calculations show that although large portions of the initial energy are absorbed by the electrons that are created through the avalanche process, a significant amount of energy is still able to reach the earth's surface. The amount of energy that reaches the earth's surface as a function of initial energy and wave shape after having propagated through 100 km in the atmosphere are investigated. Results for the air breakdown threshold intensity as a function of the pressure for different pulse widths and different frequencies will also be presented. In addition, we will present a comparison between the theoretical and the experimental results for the pulse shape of a short microwave pulse after it has traveled through a rectangular wave guide which contains a section of air. 23 references, 9 figures.

  19. Nonlinear symmetric stability of planetary atmospheres

    SciTech Connect (OSTI)

    Bowman, J.C.; Shepherd, T.G.

    1994-11-01

    The energy-Casimir method is applied to the problem of symmetric stability in the context of a compressible, hydrostatic planetary atmosphere with a general equation of state. Linear stability criteria for symmetric disturbances to a zonally symmetric baroclinic flow are obtained. In the special case of a perfect gas the results of Stevens (1983) are recovered. Nonlinear stability conditions are also obtained that, in addition to implying linear stability, provide an upper bound on a certain positive-definite measure of disturbance amplitude.

  20. Explosive Release Atmospheric Dispersal 3.2

    Energy Science and Technology Software Center (OSTI)

    2001-06-26

    ERAD (Explosive Release Atmospheric Dispersal) is a 3D numerical transport and diffusion model, used to model the consequences associated with the buoyant (or nonbuoyant) dispersal of radioactive material It incorporates an integral plume rise model to simulate the buoyant rise of heated gases following an explosive detonation. treating buoyancy effects from time zero onward, eliminating the need for the stabilized doud assumption, and enabling the penetration of inversions. Modeling of the atmospheric boundary layer usesmore » contemporary parameterization based on scaling theories derived from observational, laboratory and numerical studies. A Monte Carlo stochastic process simulates particle dispersion. Results were validated for both dose and deposition against measurements taken during Operation Roller Coaster (a joint US-UK test performed at NTS). Meteorology is defined using a single vertical sounding containing wind speed and direction and temperature as a function of height. Post processing applies 50-year CEDE DCFs (either ICRP 26 or 60) to determine the contribution of the relevant dose pathways (inhalation, submersion, and ground shine) as well as the total dose received. Dose and deposition contours are overlaid on a fully integrated worldwide GIS and tabulates hearth effects (fatalities and casualties) to resident population. The software runs on a laptop and takes less than 2 minutes to process. The Municipal version of ERAD does not include the ability to model the mitigation effects of aqueous foam.« less

  1. Cold atmospheric plasma in cancer therapy

    SciTech Connect (OSTI)

    Keidar, Michael; Shashurin, Alex; Volotskova, Olga; Ann Stepp, Mary; Srinivasan, Priya; Sandler, Anthony; Trink, Barry

    2013-05-15

    Recent progress in atmospheric plasmas has led to the creation of cold plasmas with ion temperature close to room temperature. This paper outlines recent progress in understanding of cold plasma physics as well as application of cold atmospheric plasma (CAP) in cancer therapy. Varieties of novel plasma diagnostic techniques were developed recently in a quest to understand physics of CAP. It was established that the streamer head charge is about 10{sup 8} electrons, the electrical field in the head vicinity is about 10{sup 7} V/m, and the electron density of the streamer column is about 10{sup 19} m{sup ?3}. Both in-vitro and in-vivo studies of CAP action on cancer were performed. It was shown that the cold plasma application selectively eradicates cancer cells in-vitro without damaging normal cells and significantly reduces tumor size in-vivo. Studies indicate that the mechanism of action of cold plasma on cancer cells is related to generation of reactive oxygen species with possible induction of the apoptosis pathway. It is also shown that the cancer cells are more susceptible to the effects of CAP because a greater percentage of cells are in the S phase of the cell cycle.

  2. Aeras: A next generation global atmosphere model

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Spotz, William F.; Smith, Thomas M.; Demeshko, Irina P.; Fike, Jeffrey A.

    2015-06-01

    Sandia National Laboratories is developing a new global atmosphere model named Aeras that is performance portable and supports the quantification of uncertainties. These next-generation capabilities are enabled by building Aeras on top of Albany, a code base that supports the rapid development of scientific application codes while leveraging Sandia's foundational mathematics and computer science packages in Trilinos and Dakota. Embedded uncertainty quantification (UQ) is an original design capability of Albany, and performance portability is a recent upgrade. Other required features, such as shell-type elements, spectral elements, efficient explicit and semi-implicit time-stepping, transient sensitivity analysis, and concurrent ensembles, were not componentsmore » of Albany as the project began, and have been (or are being) added by the Aeras team. We present early UQ and performance portability results for the shallow water equations.« less

  3. Aeras: A next generation global atmosphere model

    SciTech Connect (OSTI)

    Spotz, William F.; Smith, Thomas M.; Demeshko, Irina P.; Fike, Jeffrey A.

    2015-06-01

    Sandia National Laboratories is developing a new global atmosphere model named Aeras that is performance portable and supports the quantification of uncertainties. These next-generation capabilities are enabled by building Aeras on top of Albany, a code base that supports the rapid development of scientific application codes while leveraging Sandia's foundational mathematics and computer science packages in Trilinos and Dakota. Embedded uncertainty quantification (UQ) is an original design capability of Albany, and performance portability is a recent upgrade. Other required features, such as shell-type elements, spectral elements, efficient explicit and semi-implicit time-stepping, transient sensitivity analysis, and concurrent ensembles, were not components of Albany as the project began, and have been (or are being) added by the Aeras team. We present early UQ and performance portability results for the shallow water equations.

  4. Emulation to simulate low resolution atmospheric data

    SciTech Connect (OSTI)

    Hebbur Venkata Subba Rao, Vishwas [ORNL; Archibald, Richard K [ORNL; Evans, Katherine J [ORNL

    2012-08-01

    Climate simulations require significant compute power, they are complex and therefore it is time consuming to simulate them. We have developed an emulator to simulate unknown climate datasets. The emulator uses stochastic collocation and multi-dimensional in- terpolation to simulate the datasets. We have used the emulator to determine various physical quantities such as temperature, short and long wave cloud forcing, zonal winds etc. The emulation gives results which are very close to those obtained by simulations. The emulator was tested on 2 degree atmospheric datasets. The work evaluates the pros and cons of evaluating the mean first and inter- polating and vice versa. To determine the physical quantities, we have assumed them to be a function of time, longitude, latitude and a random parameter. We have looked at parameters that govern high stable clouds, low stable clouds, timescale for convection etc. The emulator is especially useful as it requires negligible compute times when compared to the simulation itself.

  5. Atmospheric Dispersion Effects in Weak Lensing Measurements

    SciTech Connect (OSTI)

    Plazas, Andrs Alejandro; Bernstein, Gary

    2012-10-01

    The wavelength dependence of atmospheric refraction causes elongation of finite-bandwidth images along the elevation vector, which produces spurious signals in weak gravitational lensing shear measurements unless this atmospheric dispersion is calibrated and removed to high precision. Because astrometric solutions and PSF characteristics are typically calibrated from stellar images, differences between the reference stars' spectra and the galaxies' spectra will leave residual errors in both the astrometric positions (dr) and in the second moment (width) of the wavelength-averaged PSF (dv) for galaxies.We estimate the level of dv that will induce spurious weak lensing signals in PSF-corrected galaxy shapes that exceed the statistical errors of the DES and the LSST cosmic-shear experiments. We also estimate the dr signals that will produce unacceptable spurious distortions after stacking of exposures taken at different airmasses and hour angles. We also calculate the errors in the griz bands, and find that dispersion systematics, uncorrected, are up to 6 and 2 times larger in g and r bands,respectively, than the requirements for the DES error budget, but can be safely ignored in i and z bands. For the LSST requirements, the factors are about 30, 10, and 3 in g, r, and i bands,respectively. We find that a simple correction linear in galaxy color is accurate enough to reduce dispersion shear systematics to insignificant levels in the r band for DES and i band for LSST,but still as much as 5 times than the requirements for LSST r-band observations. More complex corrections will likely be able to reduce the systematic cosmic-shear errors below statistical errors for LSST r band. But g-band effects remain large enough that it seems likely that induced systematics will dominate the statistical errors of both surveys, and cosmic-shear measurements should rely on the redder bands.

  6. Atmospheric Dispersion Effects in Weak Lensing Measurements

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Plazas, Andrés Alejandro; Bernstein, Gary

    2012-10-01

    The wavelength dependence of atmospheric refraction causes elongation of finite-bandwidth images along the elevation vector, which produces spurious signals in weak gravitational lensing shear measurements unless this atmospheric dispersion is calibrated and removed to high precision. Because astrometric solutions and PSF characteristics are typically calibrated from stellar images, differences between the reference stars' spectra and the galaxies' spectra will leave residual errors in both the astrometric positions (dr) and in the second moment (width) of the wavelength-averaged PSF (dv) for galaxies.We estimate the level of dv that will induce spurious weak lensing signals in PSF-corrected galaxy shapes that exceed themore »statistical errors of the DES and the LSST cosmic-shear experiments. We also estimate the dr signals that will produce unacceptable spurious distortions after stacking of exposures taken at different airmasses and hour angles. We also calculate the errors in the griz bands, and find that dispersion systematics, uncorrected, are up to 6 and 2 times larger in g and r bands,respectively, than the requirements for the DES error budget, but can be safely ignored in i and z bands. For the LSST requirements, the factors are about 30, 10, and 3 in g, r, and i bands,respectively. We find that a simple correction linear in galaxy color is accurate enough to reduce dispersion shear systematics to insignificant levels in the r band for DES and i band for LSST,but still as much as 5 times than the requirements for LSST r-band observations. More complex corrections will likely be able to reduce the systematic cosmic-shear errors below statistical errors for LSST r band. But g-band effects remain large enough that it seems likely that induced systematics will dominate the statistical errors of both surveys, and cosmic-shear measurements should rely on the redder bands.« less

  7. Oxygen detected in atmosphere of Saturn's moon Dione

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Oxygen detected in atmosphere of Saturn's moon Dione Oxygen detected in atmosphere of Saturn's moon Dione Scientists and an international research team have announced discovery of molecular oxygen ions in the upper-most atmosphere of Dione. March 3, 2012 Los Alamos National Laboratory sits on top of a once-remote mesa in northern New Mexico with the Jemez mountains as a backdrop to research and innovation covering multi-disciplines from bioscience, sustainable energy sources, to plasma physics

  8. Clear Skies S. A. Clough Atmospheric and Environmental Research, Inc.

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    S. A. Clough Atmospheric and Environmental Research, Inc. Cambridge, MA 02139 The objective of this research effort is to develop radiative transfer models that are consistent with Atmospheric Radiation Measurement (ARM) Program spectral radiance measurements for clear and cloudy atmospheres. Our approach is to develop the model physics and related databases with a line-by-line model in the context of available spectral radiance measurements. The line-by- line mode! then functions as an

  9. ARM - PI Product - Atmospheric State, Cloud Microphysics & Radiative Flux

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ProductsAtmospheric State, Cloud Microphysics & Radiative Flux ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send PI Product : Atmospheric State, Cloud Microphysics & Radiative Flux [ ARM Principal Investigator (PI) Data Product ] Atmospheric thermodynamics, cloud properties, radiative fluxes and radiative heating rates for the ARM Southern Great Plains (SGP) site. The data represent a characterization of the

  10. ARM - Amount of Greenhouse Gases in the Global Atmosphere

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    PlansAmount of Greenhouse Gases in the Global Atmosphere Outreach Home Room News Publications Traditional Knowledge Kiosks Barrow, Alaska Tropical Western Pacific Site Tours Contacts Students Study Hall About ARM Global Warming FAQ Just for Fun Meet our Friends Cool Sites Teachers Teachers' Toolbox Lesson Plans Amount of Greenhouse Gases in the Global Atmosphere Objective The objective is to feel the changes of the amounts of greenhouse gases in the global atmosphere. Materials Each group of

  11. On the use of the double floating probe method to infer the difference between the electron and the heavy particles temperatures in an atmospheric pressure, vortex-stabilized nitrogen plasma jet

    SciTech Connect (OSTI)

    Prevosto, L. Mancinelli, B. R.; Kelly, H.; Instituto de Fsica del Plasma , Departamento de Fsica, Facultad de Ciencias Exactas y Naturales Ciudad Universitaria Pab. I, 1428 Buenos Aires

    2014-05-15

    Sweeping double probe measurements in an atmospheric pressure direct current vortex-stabilized plasma jet are reported (plasma conditions: 100 A discharge current, N{sub 2} gas flow rate of 25 Nl/min, thoriated tungsten rod-type cathode, copper anode with 5 mm inner diameter). The interpretation of the double probe characteristic was based on a generalization of the standard double floating probe formulae for non-uniform plasmas coupled to a non-equilibrium plasma composition model. Perturbations caused by the current to the probe together with collisional and thermal processes inside the probe perturbed region were taken into account. Radial values of the average electron and heavy particle temperatures as well as the electron density were obtained. The calculation of the temperature values did not require any specific assumption about a temperature relationship between different particle species. An electron temperature of 10?900 900 K, a heavy particle temperature of 9300 900 K, and an electron density of about 3.5 10{sup 22} m{sup ?3} were found at the jet centre at 3.5 mm downstream from the torch exit. Large deviations from kinetic equilibrium were found toward the outer border of the plasma jet. These results showed good agreement with those previously reported by the authors by using a single probe technique. The calculations have shown that this method is particularly useful for studying spraying-type plasma torches operated at power levels of about 15 kW.

  12. Quantitative infrared absorption cross sections of isoprene for atmospheric measurements

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Brauer, C. S.; Blake, T. A.; Guenther, A. B.; Sharpe, S. W.; Sams, R. L.; Johnson, T. J.

    2014-11-19

    Isoprene (C5H8, 2-methyl-1,3-butadiene) is a volatile organic compound (VOC) and is one of the primary contributors to annual global VOC emissions. Isoprene is produced primarily by vegetation as well as anthropogenic sources, and its OH- and O3-initiated oxidations are a major source of atmospheric oxygenated organics. Few quantitative infrared studies have been reported for isoprene, limiting the ability to quantify isoprene emissions via remote or in situ infrared detection. We thus report absorption cross sections and integrated band intensities for isoprene in the 600–6500 cm-1 region. The pressure-broadened (1 atmosphere N2) spectra were recorded at 278, 298, and 323 Kmore » in a 19.94 cm path-length cell at 0.112 cm-1 resolution, using a Bruker IFS 66v/S Fourier transform infrared (FTIR) spectrometer. Composite spectra are derived from a minimum of seven isoprene sample pressures, each at one of three temperatures, and the number densities are normalized to 296 K and 1 atm.« less

  13. Atmospheric gradients and the stability of expanding jets. [Astrophysics

    SciTech Connect (OSTI)

    Hardee, P.E.; Koupelis, T.; Norman, M.L.; Clarke, D.A. Illinois, University, Urbana )

    1991-05-01

    Numerical simulations of adiabatically expanding slab jets in initial static pressure balance with an external atmosphere have been performed and compared to predictions made by a linear analysis of the stability of expanding jets. It is found that jets are stabilized by jet expansion as predicted by the linear analysis. It is also found that an expanding jet can be destabilized by a positive temperature gradient or temperature jump in the surrounding medium which lowers the Mach number defined by the external sound speed. A temperature gradient or jump is more destabilizing than would be predicted by a linear stability analysis. The enhanced instability compared to an isothermal atmosphere with identical pressure gradient is a result of the reduced external Mach number and a result of a higher jet density relative to the density in the external medium and higher ram speed. Other differences between predictions made by the linear theory and the simulations can be understood qualitatively as a result of a change in wave speed as the wave amplitude increases. 12 refs.

  14. Good Is Not Enough: Improving Measurements of Atmospheric Particles

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    scatter sunlight, with other particle properties. These properties include particle size, chemical composition, and ability to soak up atmospheric water. By linking these...

  15. Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    tmospheric R R esearch esearch 4STAR: 4STAR: Spectrometer Spectrometer for for Sky Sky - - Scanning Scanning , , Sun Sun - - Tracking Tracking Atmospheric Research...

  16. Simulation of atmospheric temperature effects on cosmic ray muon flux

    SciTech Connect (OSTI)

    Tognini, Stefano Castro; Gomes, Ricardo Avelino

    2015-05-15

    The collision between a cosmic ray and an atmosphere nucleus produces a set of secondary particles, which will decay or interact with other atmosphere elements. This set of events produced a primary particle is known as an extensive air shower (EAS) and is composed by a muonic, a hadronic and an electromagnetic component. The muonic flux, produced mainly by pions and kaons decays, has a dependency with the atmospheres effective temperature: an increase in the effective temperature results in a lower density profile, which decreases the probability of pions and kaons to interact with the atmosphere and, consequently, resulting in a major number of meson decays. Such correlation between the muon flux and the atmospheres effective temperature was measured by a set of experiments, such as AMANDA, Borexino, MACRO and MINOS. This phenomena can be investigated by simulating the final muon flux produced by two different parameterizations of the isothermal atmospheric model in CORSIKA, where each parameterization is described by a depth function which can be related to the muon flux in the same way that the muon flux is related to the temperature. This research checks the agreement among different high energy hadronic interactions models and the physical expected behavior of the atmosphere temperature effect by analyzing a set of variables, such as the height of the primary interaction and the difference in the muon flux.

  17. An ensemble constrained variational analysis of atmospheric forcing...

    Office of Scientific and Technical Information (OSTI)

    Journal Article: An ensemble constrained variational analysis of atmospheric forcing data and its application to evaluate clouds in CAM5: Ensemble 3DCVA and Its Application ...

  18. Posters Scanning Raman Lidar Measurements of Atmospheric Water...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Program (ARM) is to develop a better understanding of the atmospheric radiative balance in order to improve the parameterization of radiative processes in general...

  19. Atmospheric Dispersion Parameter (x/Q) for Calculation of Co...

    Energy Savers [EERE]

    Nuclear facilities that are potentially affected by the situation described above should review their atmospheric dispersion assumptions and NSRD- 2015-TD01. Attachment E of...

  20. Estimating atmospheric parameters and reducing noise for multispectral imaging

    DOE Patents [OSTI]

    Conger, James Lynn

    2014-02-25

    A method and system for estimating atmospheric radiance and transmittance. An atmospheric estimation system is divided into a first phase and a second phase. The first phase inputs an observed multispectral image and an initial estimate of the atmospheric radiance and transmittance for each spectral band and calculates the atmospheric radiance and transmittance for each spectral band, which can be used to generate a "corrected" multispectral image that is an estimate of the surface multispectral image. The second phase inputs the observed multispectral image and the surface multispectral image that was generated by the first phase and removes noise from the surface multispectral image by smoothing out change in average deviations of temperatures.

  1. Atmospheric Correction of Satellite Signal in Solar Domain: ...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Atmospheric Correction of Satellite Signal in Solar Domain: Impact of Improved Molecular Spectroscopy A. P. Trishchenko Canada Centre for Remote Sensing Ottawa, Ontario, Canada B....

  2. Technical Sessions M. C. MacCracken Atmospheric amj Geophysical...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    ... system, including treatment of the deep ocean and horizontal transport by ocean currents 4 Separate, uncoupled, and limited treatment of atmospheric composition, chemical ...

  3. NSRD-2015-TD01, Technical Report for Calculations of Atmospheric...

    Broader source: Energy.gov (indexed) [DOE]

    an evaluation of the technical bases for the default value for the atmospheric dispersion parameter Q. This parameter appears in the calculation of radiological dose at...

  4. ARM - Field Campaign - Evaluation of Routine Atmospheric Sounding...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    of Routine Atmospheric Sounding Measurements using Unmanned Systems (ERASMUS) Campaign Links ERASMUS Backgrounder News & Press Images Comments? We would love to hear from...

  5. A Framework for Integrated Modeling of Perturbations in Atmospheres...

    Office of Scientific and Technical Information (OSTI)

    Conjunction Tracking (IMPACT) Citation Details In-Document Search Title: A Framework for Integrated Modeling of Perturbations in Atmospheres for Conjunction Tracking (IMPACT) ...

  6. Radon Measurements of Atmospheric Mixing (RAMIX) 2006-2014 Final...

    Office of Scientific and Technical Information (OSTI)

    Publisher: DOE ARM Climate Research Facility, Pacific Northwest National Laboratory; Richland, Washington. Research Org: DOE Office of Science Atmospheric Radiation Measurement ...

  7. Duplex Rules June 2010 Atmospheric Radiation Measurement Climate...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Duplex Rules June 2010 Atmospheric Radiation Measurement Climate Research Facility North Slope of AlaskaAdjacent Arctic Ocean (ACRFNSAAAO) Duplex Rules Who can stay in the ...

  8. Description of Atmospheric Conditions at the Pierre Auger Observatory using the Global Data Assimilation System (GDAS)

    SciTech Connect (OSTI)

    Abreu, P.; Aglietta, M.; Ahlers, M.; Ahn, E.J.; Albuquerque, I.F.M.; Allard, D.; Allekotte, I.; Allen, J.; Allison, P.; Almela, A.; Alvarez Castillo, J.; /Mexico U., ICN /Santiago de Compostela U.

    2012-01-01

    Atmospheric conditions at the site of a cosmic ray observatory must be known for reconstructing observed extensive air showers. The Global Data Assimilation System (GDAS) is a global atmospheric model predicated on meteorological measurements and numerical weather predictions. GDAS provides altitude-dependent profiles of the main state variables of the atmosphere like temperature, pressure, and humidity. The original data and their application to the air shower reconstruction of the Pierre Auger Observatory are described. By comparisons with radiosonde and weather station measurements obtained on-site in Malargue and averaged monthly models, the utility of the GDAS data is shown.

  9. Atmospheric Pressure Deposition for Electrochromic Windows

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    ... Consultant * Alan Goodrich, NREL Strategic Analysis Center, Cost Modeling * Rob Moore, Dennis Nordlund, Tsu-Chien Weng, SLAC National Accelerator Laboratory Technology ...

  10. Photochemistry in terrestrial exoplanet atmospheres. III. Photochemistry and thermochemistry in thick atmospheres on super Earths and mini Neptunes

    SciTech Connect (OSTI)

    Hu, Renyu; Seager, Sara

    2014-03-20

    Some super Earths and mini Neptunes will likely have thick atmospheres that are not H{sub 2}-dominated. We have developed a photochemistry-thermochemistry kinetic-transport model for exploring the compositions of thick atmospheres on super Earths and mini Neptunes, applicable for both H{sub 2}-dominated atmospheres and non-H{sub 2}-dominated atmospheres. Using this model to study thick atmospheres for wide ranges of temperatures and elemental abundances, we classify them into hydrogen-rich atmospheres, water-rich atmospheres, oxygen-rich atmospheres, and hydrocarbon-rich atmospheres. We find that carbon has to be in the form of CO{sub 2} rather than CH{sub 4} or CO in a H{sub 2}-depleted water-dominated thick atmosphere and that the preferred loss of light elements from an oxygen-poor carbon-rich atmosphere leads to the formation of unsaturated hydrocarbons (C{sub 2}H{sub 2} and C{sub 2}H{sub 4}). We apply our self-consistent atmosphere models to compute spectra and diagnostic features for known transiting low-mass exoplanets GJ 1214 b, HD 97658 b, and 55 Cnc e. For GJ 1214 b, we find that (1) C{sub 2}H{sub 2} features at 1.0 and 1.5 ?m in transmission and C{sub 2}H{sub 2} and C{sub 2}H{sub 4} features at 9-14 ?m in thermal emission are diagnostic for hydrocarbon-rich atmospheres; (2) a detection of water-vapor features and a confirmation of the nonexistence of methane features would provide sufficient evidence for a water-dominated atmosphere. In general, our simulations show that chemical stability has to be taken into account when interpreting the spectrum of a super Earth/mini Neptune. Water-dominated atmospheres only exist for carbon to oxygen ratios much lower than the solar ratio, suggesting that this kind of atmospheres could be rare.

  11. Steam atmosphere drying exhaust steam recompression system

    DOE Patents [OSTI]

    Becker, Frederick E. (Reading, MA); Smolensky, Leo A. (Concord, MA); Doyle, Edward F. (Dedham, MA); DiBella, Francis A. (Roslindale, MA)

    1994-01-01

    This invention relates to a heated steam atmosphere drying system comprising dryer in combination with an exhaust recompression system which is extremely energy efficient and eliminates dangers known to air dryers. The system uses superheated steam as the drying medium, which recirculated through the system where its heat of evaporation and heat of compression is recovered, thereby providing a constant source of heat to the drying chamber. The dryer has inlets whereby feedstock and superheated steam are fed therein. High heat transfer and drying rates are achieved by intimate contact of the superheated steam with the particles being dried The dryer comprises a vessel which enables the feedstock and steam to enter recirculate together. When the feedstock becomes dry it will exit the dryer with the steam and become separated from the steam through the use of a curvilinear louver separator (CLS). The CLS enables removal of fine and ultrafine particles from the dryer. Water vapor separated from the particles in the CLS as superheated steam, may then be recovered and recirculated as steam through the use of a compressor to either directly or indirectly heat the dryer, and a heat exchanger or a heater to directly provide heat to the dryer. This system not only provides a very efficient heat transfer system but results in a minimum carry-over of ultrafine particles thereby eliminating any explosive hazard.

  12. Steam atmosphere drying exhaust steam recompression system

    DOE Patents [OSTI]

    Becker, F.E.; Smolensky, L.A.; Doyle, E.F.; DiBella, F.A.

    1994-03-08

    This invention relates to a heated steam atmosphere drying system comprising dryer in combination with an exhaust recompression system which is extremely energy efficient and eliminates dangers known to air dryers. The system uses superheated steam as the drying medium, which recirculates through the system where its heat of evaporation and heat of compression is recovered, thereby providing a constant source of heat to the drying chamber. The dryer has inlets whereby feedstock and superheated steam are fed therein. High heat transfer and drying rates are achieved by intimate contact of the superheated steam with the particles being dried. The dryer comprises a vessel which enables the feedstock and steam to enter and recirculate together. When the feedstock becomes dry it will exit the dryer with the steam and become separated from the steam through the use of a curvilinear louver separator (CLS). The CLS enables removal of fine and ultrafine particles from the dryer. Water vapor separated from the particles in the CLS as superheated steam, may then be recovered and recirculated as steam through the use of a compressor to either directly or indirectly heat the dryer, and a heat exchanger or a heater to directly provide heat to the dryer. This system not only provides a very efficient heat transfer system but results in a minimum carry-over of ultrafine particles thereby eliminating any explosive hazard. 17 figures.

  13. Antineutrino Oscillations in the Atmospheric Sector

    SciTech Connect (OSTI)

    Himmel, Alexander I.; /Caltech

    2011-05-01

    This thesis presents measurements of the oscillations of muon antineutrinos in the atmospheric sector, where world knowledge of antineutrino oscillations lags well behind the knowledge of neutrinos, as well as a search for {nu}{sub {mu}} {yields} {bar {nu}}{sub {mu}} transitions. Differences between neutrino and antineutrino oscillations could be a sign of physics beyond the Standard Model, including non-standard matter interactions or the violation of CPT symmetry. These measurements leverage the sign-selecting capabilities of the magnetized steel-scintillator MINOS detectors to analyze antineutrinos from the NuMI beam, both when it is in neutrino-mode and when it is in antineutrino-mode. Antineutrino oscillations are observed at |{Delta}{bar m}{sub atm}{sup 2}| = (3.36{sub -0.40}{sup +0.46}(stat) {+-} 0.06(syst)) x 10{sup -3} eV{sup 2} and sin{sup 2}(2{bar {theta}}{sub 23}) = 0.860{sub -0.12}{sup +0.11}(stat) {+-} 0.01(syst). The oscillation parameters measured for antineutrinos and those measured by MINOS for neutrinos differ by a large enough margin that the chance of obtaining two values as discrepant as those observed is only 2%, assuming the two measurements arise from the same underlying mechanism, with the same parameter values. No evidence is seen for neutrino-to-antineutrino transitions.

  14. Thermal shallow water models of geostrophic turbulence in Jovian atmospheres

    SciTech Connect (OSTI)

    Warneford, Emma S. Dellar, Paul J.

    2014-01-15

    Conventional shallow water theory successfully reproduces many key features of the Jovian atmosphere: a mixture of coherent vortices and stable, large-scale, zonal jets whose amplitude decreases with distance from the equator. However, both freely decaying and forced-dissipative simulations of the shallow water equations in Jovian parameter regimes invariably yield retrograde equatorial jets, while Jupiter itself has a strong prograde equatorial jet. Simulations by Scott and Polvani [Equatorial superrotation in shallow atmospheres, Geophys. Res. Lett. 35, L24202 (2008)] have produced prograde equatorial jets through the addition of a model for radiative relaxation in the shallow water height equation. However, their model does not conserve mass or momentum in the active layer, and produces mid-latitude jets much weaker than the equatorial jet. We present the thermal shallow water equations as an alternative model for Jovian atmospheres. These equations permit horizontal variations in the thermodynamic properties of the fluid within the active layer. We incorporate a radiative relaxation term in the separate temperature equation, leaving the mass and momentum conservation equations untouched. Simulations of this model in the Jovian regime yield a strong prograde equatorial jet, and larger amplitude mid-latitude jets than the Scott and Polvani model. For both models, the slope of the non-zonal energy spectra is consistent with the classic Kolmogorov scaling, and the slope of the zonal energy spectra is consistent with the much steeper spectrum observed for Jupiter. We also perform simulations of the thermal shallow water equations for Neptunian parameter values, with a radiative relaxation time scale calculated for the same 25 mbar pressure level we used for Jupiter. These Neptunian simulations reproduce the broad, retrograde equatorial jet and prograde mid-latitude jets seen in observations. The much longer radiative time scale for the colder planet Neptune explains the transition from a prograde to a retrograde equatorial jet, while the broader jets are due to the deformation radius being a larger fraction of the planetary radius.

  15. Atmospheric process evaluation of mobile source emissions

    SciTech Connect (OSTI)

    1995-07-01

    During the past two decades there has been a considerable effort in the US to develop and introduce an alternative to the use of gasoline and conventional diesel fuel for transportation. The primary motives for this effort have been twofold: energy security and improvement in air quality, most notably ozone, or smog. The anticipated improvement in air quality is associated with a decrease in the atmospheric reactivity, and sometimes a decrease in the mass emission rate, of the organic gas and NO{sub x} emissions from alternative fuels when compared to conventional transportation fuels. Quantification of these air quality impacts is a prerequisite to decisions on adopting alternative fuels. The purpose of this report is to present a critical review of the procedures and data base used to assess the impact on ambient air quality of mobile source emissions from alternative and conventional transportation fuels and to make recommendations as to how this process can be improved. Alternative transportation fuels are defined as methanol, ethanol, CNG, LPG, and reformulated gasoline. Most of the discussion centers on light-duty AFVs operating on these fuels. Other advanced transportation technologies and fuels such as hydrogen, electric vehicles, and fuel cells, will not be discussed. However, the issues raised herein can also be applied to these technologies and other classes of vehicles, such as heavy-duty diesels (HDDs). An evaluation of the overall impact of AFVs on society requires consideration of a number of complex issues. It involves the development of new vehicle technology associated with engines, fuel systems, and emission control technology; the implementation of the necessary fuel infrastructure; and an appropriate understanding of the economic, health, safety, and environmental impacts associated with the use of these fuels. This report addresses the steps necessary to properly evaluate the impact of AFVs on ozone air quality.

  16. Strategic Environmental Research and Development Program: Atmospheric Remote Sensing and Assessment Program -- Final Report. Part 1: The lower atmosphere

    SciTech Connect (OSTI)

    Tooman, T.P.

    1997-01-01

    This report documents work done between FY91 and FY95 for the lower atmospheric portion of the joint Department of Defense (DoD) and Department of Energy (DOE) Atmospheric Remote Sensing and Assessment Program (ARSAP) within the Strategic Environmental Research and Development Program (SERDP). The work focused on (1) developing new measurement capabilities and (2) measuring atmospheric heating in a well-defined layer and then relating it to cloud properties an water vapor content. Seven new instruments were develop3ed for use with Unmanned Aerospace Vehicles (UAVs) as the host platform for flux, radiance, cloud, and water vapor measurements. Four major field campaigns were undertaken to use these new as well as existing instruments to make critically needed atmospheric measurements. Scientific results include the profiling of clear sky fluxes from near surface to 14 km and the strong indication of cloudy atmosphere absorption of solar radiation considerably greater than predicted by extant models.

  17. Recuperated atmosphere SOFC/gas turbine hybrid cycle

    DOE Patents [OSTI]

    Lundberg, Wayne (Pittsburgh, PA)

    2010-08-24

    A method of operating an atmospheric-pressure solid oxide fuel cell generator (6) in combination with a gas turbine comprising a compressor (1) and expander (2) where an inlet oxidant (20) is passed through the compressor (1) and exits as a first stream (60) and a second stream (62) the first stream passing through a flow control valve (56) to control flow and then through a heat exchanger (54) followed by mixing with the second stream (62) where the mixed streams are passed through a combustor (8) and expander (2) and the first heat exchanger for temperature control before entry into the solid oxide fuel cell generator (6), which generator (6) is also supplied with fuel (40).

  18. Recuperated atmospheric SOFC/gas turbine hybrid cycle

    DOE Patents [OSTI]

    Lundberg, Wayne

    2010-05-04

    A method of operating an atmospheric-pressure solid oxide fuel cell generator (6) in combination with a gas turbine comprising a compressor (1) and expander (2) where an inlet oxidant (20) is passed through the compressor (1) and exits as a first stream (60) and a second stream (62) the first stream passing through a flow control valve (56) to control flow and then through a heat exchanger (54) followed by mixing with the second stream (62) where the mixed streams are passed through a combustor (8) and expander (2) and the first heat exchanger for temperature control before entry into the solid oxide fuel cell generator (6), which generator (6) is also supplied with fuel (40).

  19. Clean coal reference plants: Atmospheric CFB. Topical report, Task 1

    SciTech Connect (OSTI)

    Rubow, L.N.; Harvey, L.E.; Buchanan, T.L.; Carpenter, R.G.; Hyre, M.R.; Zaharchuk, R.

    1992-06-01

    The Clean Coal Technology Demonstration Program is a government and industry cofunded technology development effort to demonstrate a new generation of innovative coal utilization processes in a series of full-scale facilities. The goal of the program is to provide the US energy marketplace with a number of advanced, more efficient and environmentally responsive coal-using technologies. The Morgantown Energy Technology Center (METC) has the responsibility for monitoring the CCT Projects within certain technology categories, which correspond to the center`s areas of technology development, including atmospheric fluidized bed combustion, pressurized fluidized bed combustion, integrated gasification combined cycle, mild gasification, and industrial applications. A measure of success in the CCT program will be the commercial acceptance of the new technologies being demonstrated. The dissemination of project information to potential users is being accomplished by producing a series of reference plant designs which will provide the users a basis for the selection of technologies applicable to their future energy requirements. As a part of DOE`s monitoring and evaluation of the CCT Projects, Gilbert/Commonwealth (G/C) has been contracted to assist in this effort by producing the design of a commercial size Reference Plant, utilizing technologies developed in the CCT Program. This report, the first in a series, describes the design of a 400 MW electric power plant, utilizing an atmospheric pressure, circulating fluidized bed combustor (ACFB) similar to the one which was demonstrated at Colorado-Ute`s Nucla station, funded in Round 1 of the CCT Program. The intent of the reference plant design effort was to portray a commercial power plant with attributes considered important to the utility industry. The logical choice for the ACFB combustor was Pyropower since they supplied the ACFB for the Nucla Project.

  20. ARM - Field Campaign - 2013 Lower Atmospheric Boundary Layer Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaigns2013 Lower Atmospheric Boundary Layer Experiment ARM Data Discovery Browse Data Related Campaigns Lower Atmospheric Boundary Layer Experiment 2012.09.17, Turner, SGP Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : 2013 Lower Atmospheric Boundary Layer Experiment 2013.05.28 - 2013.07.01 Lead Scientist : David Turner For data sets, see below. Abstract Instruments were deployed at the SGP Central Facility to investigate how

  1. ARM - Field Campaign - Lower Atmospheric Boundary Layer Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsLower Atmospheric Boundary Layer Experiment Campaign Links LABLE Website Field Campaign Report ARM Data Discovery Browse Data Related Campaigns 2013 Lower Atmospheric Boundary Layer Experiment 2013.05.28, Turner, SGP Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : Lower Atmospheric Boundary Layer Experiment 2012.09.17 - 2012.11.13 Lead Scientist : David Turner For data sets, see below. Abstract Boundary layer turbulence is

  2. ARM - Field Campaign - Radon Measurements of Atmospheric Mixing (RAMIX

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    2008) govCampaignsRadon Measurements of Atmospheric Mixing (RAMIX 2008) ARM Data Discovery Browse Data Related Campaigns Radon Measurements of Atmospheric Mixing (RAMIX) 2006.11.01, Fischer, SGP Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : Radon Measurements of Atmospheric Mixing (RAMIX 2008) 2008.04.01 - 2009.03.31 Lead Scientist : Marc Fischer For data sets, see below. Abstract At present, uncertainty in vertical mixing

  3. JGR-Atmospheres Papers from the RADAGAST Research Team

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    JGR-Atmospheres Papers from the RADAGAST Research Team Bharmal, N.A., A. Slingo, G.J. Robinson, and J.J. Settle, 2009: Simulation of surface and top of atmosphere thermal fluxes and radiances from the RADAGAST experiment. Journal of Geophysical Research-Atmospheres, 114, doi:10.1029/2008JD010504, in press. Kollias, P., M.A. Miller, K.L. Johnson, M.P. Jensen, and D.T. Troyan, 2009: Cloud, thermodynamic, and precipitation observations in West Africa during 2006. Journal of Geophysical Research-

  4. Airborne Instrumentation Needs for Climate and Atmospheric Research

    SciTech Connect (OSTI)

    McFarquhar, Greg; Schmid, Beat; Korolev, Alexei; Ogren, John A.; Russell, P. B.; Tomlinson, Jason M.; Turner, David D.; Wiscombe, Warren J.

    2011-10-06

    Observational data are of fundamental importance for advances in climate and atmospheric research. Advances in atmospheric science are being made not only through the use of ground-based and space-based observations, but also through the use of in-situ and remote sensing observations acquired on instrumented aircraft. In order for us to enhance our knowledge of atmospheric processes, it is imperative that efforts be made to improve our understanding of the operating characteristics of current instrumentation and of the caveats and uncertainties in data acquired by current probes, as well as to develop improved observing methodologies for acquisition of airborne data.

  5. Fehner and Gosling, Atmospheric Nuclear Weapons Testing, 1951-1963.

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Battlefield of the Cold War: The Nevada Test Site, Volume I | Department of Energy Atmospheric Nuclear Weapons Testing, 1951-1963. Battlefield of the Cold War: The Nevada Test Site, Volume I Fehner and Gosling, Atmospheric Nuclear Weapons Testing, 1951-1963. Battlefield of the Cold War: The Nevada Test Site, Volume I Terrence R. Fehner and F.G. Gosling. Atmospheric Nuclear Weapons Testing, 1951-1963. Battlefield of the Cold War: The Nevada Test Site, Volume I (pdf). DOE/MA-0003. Washington,

  6. Computer support to run models of the atmosphere. Final report

    SciTech Connect (OSTI)

    Fung, I.

    1996-08-30

    This research is focused on a better quantification of the variations in CO{sub 2} exchanges between the atmosphere and biosphere and the factors responsible for these exchangers. The principal approach is to infer the variations in the exchanges from variations in the atmospheric CO{sub 2} distribution. The principal tool involves using a global three-dimensional tracer transport model to advect and convect CO{sub 2} in the atmosphere. The tracer model the authors used was developed at the Goddard institute for Space Studies (GISS) and is derived from the GISS atmospheric general circulation model. A special run of the GCM is made to save high-frequency winds and mixing statistics for the tracer model.

  7. PNNL: Atmospheric Sciences & Global Change Search for Staff

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Atmospheric Science & Global Change Search for Staff Search for an ASGC staff member (Last, First) Search Search for staff member by Group View Alphabetical List of all ASGC Staff...

  8. Integrated Study of MFRSR-derived Parameters of Atmospheric Aerosols...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Program CART site, in Remote Sensing of Clouds and the Atmosphere VI, K. Schafer, O. Lado- Bordowsky, A. Comeron, M. R. Carleer, J. S. Fender, Editors, Proc. SPIE Vol. 4539,...

  9. North America's net terrestrial CO2 exchange with the atmosphere...

    Office of Scientific and Technical Information (OSTI)

    a synthesis of net land-atmosphere CO2 exchange for North America (Canada, United States, and Mexico) over the period 1990-2009. Only CO2 is considered, not methane or...

  10. ARM - Field Campaign - Cross-Scale Land-Atmosphere Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    would love to hear from you Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : Cross-Scale Land-Atmosphere Experiment 2016.09.01 - 2019.05.31 Lead Scientist :...

  11. The Atmosphere as a Laboratory: Aerosols, Air Quality, and Climate...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    to 11:00am Science On Saturday MBG Auditorium The Atmosphere as a Laboratory: Aerosols, Air Quality, and Climate Peter DeCarlo, Assistant Professor of Environmental Engineering...

  12. Atmospheric Radiation Measurement Program Facilities Newsletter - September 1999

    SciTech Connect (OSTI)

    Holdridge, D. J., ed

    1999-09-27

    The Atmospheric Radiation Measurement Program September 1999 Facilities Newsletter discusses the several Intensive Observation Periods (IOPs) that the ARM SGP CART site will host in the near future. Two projects of note are the International Pyrgeometer Intercomparison and the Fall Single Column Model (SCM)/Nocturnal Boundary Layer (NBL) IOP. Both projects will bring many US and international scientists to the SGP CART site to participate in atmospheric research.

  13. Technical Sessions B. E. Manner National Oceanic and Atmospheric Administration

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    B. E. Manner National Oceanic and Atmospheric Administration Wave Propagation Laboratory 130ulder, CO 80303 The Atmospheric Radiation Measurement (ARM) pirog ram goals are ambitious, and its schedule is demanding. Many of the instruments, proposed for operations at the first Cloud and Radiation Testbed (CART) site as early alS 1992 represent emerging technology and exist only as :special research prototypes. Therefore, an important preparatory step for ARM was an intensive field project in

  14. ARM - Field Campaign - ASSIST: Atmospheric Sounder Spectrometer for

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Infrared Spectral Technology govCampaignsASSIST: Atmospheric Sounder Spectrometer for Infrared Spectral Technology ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : ASSIST: Atmospheric Sounder Spectrometer for Infrared Spectral Technology 2008.07.08 - 2008.07.18 Lead Scientist : Michael Howard For data sets, see below. Abstract Goals of assist were to intercompare radiance spectra and profile retrievals

  15. PRECISION DETERMINATION OF ATMOSPHERIC EXTINCTION AT OPTICAL AND

    Office of Scientific and Technical Information (OSTI)

    NEAR-INFRARED WAVELENGTHS (Journal Article) | SciTech Connect PRECISION DETERMINATION OF ATMOSPHERIC EXTINCTION AT OPTICAL AND NEAR-INFRARED WAVELENGTHS Citation Details In-Document Search Title: PRECISION DETERMINATION OF ATMOSPHERIC EXTINCTION AT OPTICAL AND NEAR-INFRARED WAVELENGTHS The science goals for future ground-based all-sky surveys, such as the Dark Energy Survey, PanSTARRS, and the Large Synoptic Survey Telescope, require calibration of broadband photometry that is stable in time

  16. A Framework for Integrated Modeling of Perturbations in Atmospheres for

    Office of Scientific and Technical Information (OSTI)

    Conjunction Tracking (IMPACT) (Conference) | SciTech Connect Framework for Integrated Modeling of Perturbations in Atmospheres for Conjunction Tracking (IMPACT) Citation Details In-Document Search Title: A Framework for Integrated Modeling of Perturbations in Atmospheres for Conjunction Tracking (IMPACT) Authors: Linares, Richard [1] ; Klimenko, Alexei V. [1] ; Brennan, Sean M. [1] ; Godinez Vazquez, Humberto C. [1] ; Higdon, David M. [1] ; Koller, Josef [1] ; Lawrence, Earl C. [1] ; Palmer,

  17. Carbonyl sulfide: potential agent of atmospheric sulfur corrosion

    SciTech Connect (OSTI)

    Graedel, T.E.; Kammlott, G.W.; Franey, J.P.

    1981-05-08

    Laboratory exposure experiments demonstrate that carbonyl sulfide in wet air corrodes copper at 22/sup 0/C at a rate that is approximately linear with total exposure (the product of exposure time and carbonyl sulfide concentration). The corrosion rate is similar to that of hydrogen sulfide, a widely recognized corrodant. The much greater average atmospheric abundance of carbonyl sulfide compared with that of hydrogen sulfide or sulfur dioxide suggests that carbonyl sulfide may be a major agent of atmospheric sulfur corrosion.

  18. DOE/ER-0441 Atmospheric Radiation Measurement Plan - February 1990

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    1 Atmospheric Radiation Measurement Program Plan ARM Program Plan Forward In 1978 the Department of Energy initiated the Carbon Dioxide Research Program to address climate change from the increasing concentration of carbon dioxide in the atmosphere. Over the years the Program has studied the many facets of the issue, from the carbon cycle, the climate diagnostics, the vegetative effects, to the societal impacts. The Program is presently the Department's principal entry in the U.S. Global Change

  19. Diesel and Gasoline Engine Emissions: Characterization of Atmosphere

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Composition and Health Responses to Inhaled Emissions | Department of Energy and Gasoline Engine Emissions: Characterization of Atmosphere Composition and Health Responses to Inhaled Emissions Diesel and Gasoline Engine Emissions: Characterization of Atmosphere Composition and Health Responses to Inhaled Emissions 2005 Diesel Engine Emissions Reduction (DEER) Conference Presentations and Posters PDF icon 2005_deer_mcdonald.pdf More Documents & Publications The Effect of Changes in Diesel

  20. INFERENCE OF INHOMOGENEOUS CLOUDS IN AN EXOPLANET ATMOSPHERE

    SciTech Connect (OSTI)

    Demory, Brice-Olivier; De Wit, Julien; Lewis, Nikole; Zsom, Andras; Seager, Sara; Fortney, Jonathan; Knutson, Heather; Desert, Jean-Michel; Heng, Kevin; Madhusudhan, Nikku; Gillon, Michael; Barclay, Thomas; Cowan, Nicolas B.

    2013-10-20

    We present new visible and infrared observations of the hot Jupiter Kepler-7b to determine its atmospheric properties. Our analysis allows us to (1) refine Kepler-7b's relatively large geometric albedo of Ag = 0.35 0.02, (2) place upper limits on Kepler-7b thermal emission that remains undetected in both Spitzer bandpasses and (3) report a westward shift in the Kepler optical phase curve. We argue that Kepler-7b's visible flux cannot be due to thermal emission or Rayleigh scattering from H{sub 2} molecules. We therefore conclude that high altitude, optically reflective clouds located west from the substellar point are present in its atmosphere. We find that a silicate-based cloud composition is a possible candidate. Kepler-7b exhibits several properties that may make it particularly amenable to cloud formation in its upper atmosphere. These include a hot deep atmosphere that avoids a cloud cold trap, very low surface gravity to suppress cloud sedimentation, and a planetary equilibrium temperature in a range that allows for silicate clouds to potentially form in the visible atmosphere probed by Kepler. Our analysis does not only present evidence of optically thick clouds on Kepler-7b but also yields the first map of clouds in an exoplanet atmosphere.

  1. DOE/SC-ARM-13-013 Atmospheric Radiation Measurement Climate Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    3 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-13-013 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  2. DOE/SC-ARM-14-025 Atmospheric Radiation Measurement Climate Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    5 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-14-025 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  3. DOE/SC-ARM-15-037 Atmospheric Radiation Measurement Climate Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    7 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-15-037 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  4. DOE/SC-ARM-12-021 Atmospheric Radiation Measurement Climate Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    1 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-12-021 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  5. DOE/SC-ARM-14-007 Atmospheric Radiation Measurement Climate Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    7 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-14-007 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  6. DOE/SC-ARM-15-018 Atmospheric Radiation Measurement Climate Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    8 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-15-018 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  7. FACT SHEET U.S. Department of Energy Atmospheric Radiation Measurement...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Atmospheric Radiation Measurement Climate Research Facility The Atmospheric Radiation Measurement (ARM) Climate Research Facility is a key component of the U.S. Department of ...

  8. DOE/SC-ARM-14-019 Atmospheric Radiation Measurement Climate Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    9 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-14-019 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  9. DOE/SC-ARM-15-001 Atmospheric Radiation Measurement Climate Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    1 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-15-001 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  10. DOE/SC-ARM-14-001 Atmospheric Radiation Measurement Climate Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    1 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-14-001 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  11. DOE/SC-ARM-13-007 Atmospheric Radiation Measurement Climate Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    7 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-13-007 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  12. DOE/SC-ARM-12-015 Atmospheric Radiation Measurement Climate Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    5 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-12-015 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  13. DOE/SC-ARM-13-001 Atmospheric Radiation Measurement Climate Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    1 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-13-001 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  14. DOE/SC-ARM-13-020 Atmospheric Radiation Measurement Climate Research...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    0 Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report ... DOESC-ARM-13-020 Atmospheric Radiation Measurement Climate Research Facility Operations ...

  15. Investigation on coal pyrolysis in CO{sub 2} atmosphere

    SciTech Connect (OSTI)

    Lunbo Duan; Changsui Zhao; Wu Zhou; Chengrui Qu; Xiaoping Chen [Institute for Thermal Power Engineering of Southeast University, Nanjing (China)

    2009-07-15

    Considerable studies have been reported on the coal pyrolysis process and the formation of SO{sub 2} and NOx processors such as H{sub 2}S, COS, SO{sub 2}, HCN, and NH{sub 3} in inert atmospheres. Similar studies in CO{sub 2} atmosphere also need to be accomplished for better understanding of the combustion characteristics and the SO{sub 2}/NOx formation mechanism of oxy-fuel combustion, which is one of the most important technologies for CO{sub 2} capture. In this study, thermogravimetry coupled with Fourier Transform Infrared (TG-FTIR) analysis was employed to measure the volatile yield and gas evolution features during coal pyrolysis process in CO{sub 2} atmosphere. Results show that replacing N{sub 2} with CO{sub 2} does not influence the starting temperature of volatile release but seems to enhance the volatile releasing rate even at 480{sup o}C. At about 760{sup o}C, CO{sub 2} prevents the calcite from decomposing. In CO{sub 2} atmosphere, the volatile yield increases as the temperature increases and decreases as the heating rate increases. COS is monitored during coal pyrolysis in CO{sub 2} atmosphere while there are only H{sub 2}S and SO{sub 2} formed in N{sub 2} atmosphere. The COS is most likely formed by the reaction between CO{sub 2} and H{sub 2}S. No NH{sub 3} was monitored in this study. In CO{sub 2} atmosphere, the gasification of char elevates the conversion of char-N to HCN. The HCN yield increases as the temperature increases and decreases as the heating rate increases. 20 refs., 13 figs., 3 tabs.

  16. Atmospheric Radiation Measurement Program facilities newsletter, November 2002.

    SciTech Connect (OSTI)

    Holdridge, D. J.

    2002-12-03

    Fall 2002 Intensive Operation Periods: Single Column Model and Unmanned Aerospace Vehicle--In an Intensive Operation Period (IOP) on November 3-23, 2002, researchers at the SGP CART site are collecting a detailed data set for use in improving the Single Column Model (SCM), a scaled-down climate model. The SCM represents one vertical column of air above Earth's surface and requires less computation time than a full-scale global climate model. Researchers first use the SCM to efficiently improve submodels of clouds, solar radiation transfer, and atmosphere-surface interactions, then implement the results in large-scale global models. With measured values for a starting point, the SCM predicts atmospheric variables during prescribed time periods. A computer calculates values for such quantities as the amount of solar radiation reaching the surface and predicts how clouds will evolve and interact with incoming light from the sun. Researchers compare the SCM's predictions with actual measurements made during the IOP, then adjust the submodels to make predictions more reliable. A second IOP conducted concurrently with the SCM IOP involves high-altitude, long-duration aircraft flights. The original plan was to use an unmanned aerospace vehicle (UAV), but the National Aeronautics and Space Administration (NASA) aircraft Proteus will be substituted because all UAVs have been deployed elsewhere. The UAV is a small, instrument-equipped, remote-control plane that is operated from the ground by a computer. The Proteus is a manned aircraft, originally designed to carry telecommunications relay equipment, that can be reconfigured for uses such as reconnaissance and surveillance, commercial imaging, launching of small space satellites, and atmospheric research. The plane is designed for two on-board pilots in a pressurized cabin, flying to altitudes up to 65,000 feet for as long as 18 hours. The Proteus has a variable wingspan of 77-92 feet and is 56 feet long. The plane can carry up to 7,260 pounds of equipment, making it a versatile research tool. The Proteus is making measurements at the very top of the cirrus cloud layer to characterize structures of these clouds. These new measurements will provide more accurate, more abundant data for use in improving the representation of clouds in the SCM. 2002-2003 Winter Weather Forecast--Top climate forecasters at the National Oceanic and Atmospheric Administration's (NOAA's) Climate Prediction Center say that an El Nino condition in the tropical Pacific Ocean will influence our winter weather this year. Although this El Nino is not as strong as the event of the 1997-1998 winter season, the United States will nevertheless experience some atypical weather. Strong impacts could be felt in several areas. Nationally, forecasters are predicting warmer-than-average temperatures over the northern tier of states and wetter-than-average conditions in the southern tier of states during the 2002-2003 winter season. Kansas residents should expect warmer and wetter conditions, while Oklahoma will be wetter than average.

  17. Characteristic emission enhancement in the atmosphere with Rn trace using metal assisted LIBS

    SciTech Connect (OSTI)

    Hashemi, M. M.; Parvin, P. Moosakhani, A.; Mortazavi, S. Z.; Reyhani, A.; Majdabadi, A.; Abachi, S.

    2014-06-15

    Several characteristic emission lines from the metal targets (Cu, Zn and Pb) were investigated in trace presence of radon gas in the atmospheric air, using Q-SW Nd:YAG laser induced plasma inside a control chamber. The emission lines of metal species are noticeably enhanced in (Rn+air), relative to those in the synthetic air alone. Similar spectra were also taken in various sub-atmospheric environments in order to determine the optimum pressure for enhancement. Solid-state nuclear track detectors were also employed to count the tracks due to alpha particles for the activity assessment.

  18. Atmospheric sensing for the H.E.S.S. array

    SciTech Connect (OSTI)

    Aye, K.-M.; Brown, A.M.; Chadwick, P.M.; Hadjichristidis, C.; Latham, I.J.; Le Gallou, R.; McComb, T.J.L.; Nolan, S.J.; Noutsos, A.; Orford, K.J.; Osborne, J.L.; Rayner, S.M.

    2005-02-21

    Several atmospheric monitoring instruments have been installed at the H.E.S.S. gamma-ray observatory in Namibia. Firstly, Heitronics KT19 infrared radiometers, aligned paraxially with the H.E.S.S. telescopes, measure the infrared radiation of the water molecules. These allow us to detect clouds crossing the telescopes' field of view and to estimate the humidity present in the atmosphere. For a general estimate of the atmosphere's transmittance, i.e. the detection of any light-attenuating aerosols, a ceilometer, which is a LIDAR with built-in atmospheric data reduction code, is being used. It will be complemented soon by an instrument which will measure the transmissivity of the atmosphere at different wavelengths up to 500m above the ground. The overall status of the weather is monitored by a fully automated weatherstation. This paper describes the setup, the data analysis and how this will be used in order to improve the knowledge of the telescopes' effective collection area.

  19. Atmospheric gas supersaturation: educational and research needs

    SciTech Connect (OSTI)

    Bouck, G.R.; D'Aoust, B.; Ebel, W.J.; Rulifson, R.

    1980-11-01

    There still is need for research on gas supersaturation as it relates to gas bubble disease. Better methods are required for both measurement and treatment of gas-supersaturated water. We must understand more about physiological and ecosystem responses to high gas pressures if existing tolerance data for individual species are to be applied accurately to field or fish-cultural situations. A better training program is needed for scientists, engineers, and facility operators involved in the monitoring and mitigation of gas-supersaturated waters.

  20. Atmospheric benzenoid emissions from plants rival those from fossil fuels

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Misztal, P. K.; Hewitt, C. N.; Wildt, J.; Blande, J. D.; Eller, A. S.D.; Fares, S.; Gentner, D. R.; Gilman, J. B.; Graus, M.; Greenberg, J.; et al

    2015-07-13

    Despite the known biochemical production of a range of aromatic compounds by plants and the presence of benzenoids in floral scents, the emissions of only a few benzenoid compounds have been reported from the biosphere to the atmosphere. Here, using evidence from measurements at aircraft, ecosystem, tree, branch and leaf scales, with complementary isotopic labeling experiments, we show that vegetation (leaves, flowers, and phytoplankton) emits a wide variety of benzenoid compounds to the atmosphere at substantial rates. Controlled environment experiments show that plants are able to alter their metabolism to produce and release many benzenoids under stress conditions. The functionsmore » of these compounds remain unclear but may be related to chemical communication and protection against stress. We estimate the total global secondary organic aerosol potential from biogenic benzenoids to be similar to that from anthropogenic benzenoids (~10 Tg y-1), pointing to the importance of these natural emissions in atmospheric physics and chemistry.« less

  1. Atmospheric dispersion modeling: Challenges of the Fukushima Daiichi response

    SciTech Connect (OSTI)

    Sugiyama, Gayle; Nasstrom, John; Pobanz, Brenda; Foster, Kevin; Simpson, Matthew; Vogt, Phil; Aluzzi, Fernando; Homann, Steve

    2012-05-01

    In this research, the U.S. Department of Energy’s (DOE) National Atmospheric Release Advisory Center (NARAC) provided a wide range of predictions and analyses as part of the response to the Fukushima Daiichi Nuclear Power Plant accident including: daily Japanese weather forecasts and atmospheric transport predictions to inform planning for field monitoring operations and to provide U.S. government agencies with ongoing situational awareness of meteorological conditions; estimates of possible dose in Japan based on hypothetical U.S. Nuclear Regulatory Commission scenarios of potential radionuclide releases to support protective action planning for U.S. citizens; predictions of possible plume arrival times and dose levels at U.S. locations; and source estimation and plume model refinement based on atmospheric dispersion modeling and available monitoring data.

  2. An active atmospheric methane sink in high Arctic mineral cryosols

    SciTech Connect (OSTI)

    Lau, Maggie C.Y.; Stackhouse, B.; Layton, Alice C.; Chauhan, Archana; Vishnivetskaya, T. A.; Chourey, Karuna; Mykytczuk, N. C.S.; Bennett, Phil C.; Lamarche-Gagnon, G.; Burton, N.; Renholm, J.; Hettich, R. L.; Pollard, W. H.; Omelon, C. R.; Medvigy, David M.; Pffifner, Susan M.; Whyte, L. G.; Onstott, T. C.

    2015-04-14

    The transition of Arctic carbon-rich cryosols into methane (CH?)-emitting wetlands due to global warming is a rising concern. However, the spatially predominant mineral cryosols and their CH? emission potential are poorly understood. Fluxes measured in situ and estimated under laboratory conditions coupled with -omics analysis indicate (1) mineral cryosols in the Canadian high Arctic contain atmospheric CH?-oxidizing bacteria; (2) the atmospheric CH? uptake flux increases with ground temperature; and, as a result, (3) the atmospheric CH? sink strength will increase by a factor of 5-30 as the Arctic warms by 5-15 C over a century. We demonstrated that acidic mineral cryosols have previously unrecognized potential of negative CH? feedback.

  3. An active atmospheric methane sink in high Arctic mineral cryosols

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Lau, Maggie C.Y.; Stackhouse, B.; Layton, Alice C.; Chauhan, Archana; Vishnivetskaya, T. A.; Chourey, Karuna; Mykytczuk, N. C.S.; Bennett, Phil C.; Lamarche-Gagnon, G.; Burton, N.; et al

    2015-04-14

    The transition of Arctic carbon-rich cryosols into methane (CH₄)-emitting wetlands due to global warming is a rising concern. However, the spatially predominant mineral cryosols and their CH₄ emission potential are poorly understood. Fluxes measured in situ and estimated under laboratory conditions coupled with -omics analysis indicate (1) mineral cryosols in the Canadian high Arctic contain atmospheric CH₄-oxidizing bacteria; (2) the atmospheric CH⁺ uptake flux increases with ground temperature; and, as a result, (3) the atmospheric CH₄ sink strength will increase by a factor of 5-30 as the Arctic warms by 5-15 °C over a century. We demonstrated that acidic mineralmore » cryosols have previously unrecognized potential of negative CH₄ feedback.« less

  4. Atmospheric benzenoid emissions from plants rival those from fossil fuels

    SciTech Connect (OSTI)

    Misztal, P. K.; Hewitt, C. N.; Wildt, J.; Blande, J. D.; Eller, A. S.D.; Fares, S.; Gentner, D. R.; Gilman, J. B.; Graus, M.; Greenberg, J.; Guenther, A. B.; Hansel, A.; Harley, P.; Huang, M.; Jardine, K.; Karl, T.; Kaser, L.; Keutsch, F. N.; Kiendler-Scharr, A.; Kleist, E.; Lerner, B. M.; Li, T.; Mak, J.; Nlscher, A. C.; Schnitzhofer, R.; Sinha, V.; Thornton, B.; Warneke, C.; Wegener, F.; Werner, C.; Williams, J.; Worton, D. R.; Yassaa, N.; Goldstein, A. H.

    2015-07-13

    Despite the known biochemical production of a range of aromatic compounds by plants and the presence of benzenoids in floral scents, the emissions of only a few benzenoid compounds have been reported from the biosphere to the atmosphere. Here, using evidence from measurements at aircraft, ecosystem, tree, branch and leaf scales, with complementary isotopic labeling experiments, we show that vegetation (leaves, flowers, and phytoplankton) emits a wide variety of benzenoid compounds to the atmosphere at substantial rates. Controlled environment experiments show that plants are able to alter their metabolism to produce and release many benzenoids under stress conditions. The functions of these compounds remain unclear but may be related to chemical communication and protection against stress. We estimate the total global secondary organic aerosol potential from biogenic benzenoids to be similar to that from anthropogenic benzenoids (~10 Tg y-1), pointing to the importance of these natural emissions in atmospheric physics and chemistry.

  5. ChEAS Data: The Chequamegon Ecosystem Atmosphere Study

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Davis, Kenneth J. [Penn State

    The Chequamegon Ecosystem-Atmosphere Study (ChEAS) is a multi-organizational research effort studying biosphere/atmosphere interactions within a northern mixed forest in Northern Wisconsin. A primary goal is to understand the processes controlling forest-atmosphere exchange of carbon dioxide and the response of these processes to climate change. Another primary goal is to bridge the gap between canopy-scale flux measurements and the global CO2 flask sampling network. The ChEAS flux towers participate in AmeriFlux, and the region is an EOS-validation site. The WLEF tower is a NOAA-CMDL CO2 sampling site. ChEAS sites are primarily located within or near the Chequamegon-Nicolet National Forest in northern Wisconsin, with one site in the Ottawa National Forest in the upper peninsula of Michigan. Current studies observe forest/atmosphere exchange of carbon dioxide at canopy and regional scales, forest floor respiration, photosynthesis and transpiration at the leaf level and use models to scale to canopy and regional levels. EOS-validation studies quantitatively assess the land cover of the area using remote sensing and conduct extensive ground truthing of new remote sensing data (i.e. ASTER and MODIS). Atmospheric remote sensing work is aimed at understanding atmospheric boundary layer dynamics, the role of entrainment in regulating the carbon dioxide mixing ratio profiles through the lower troposphere, and feedback between boundary layer dynamics and vegetation (especially via the hydrologic cycle). Airborne studies have included include balloon, kite and aircraft observations of the CO2 profile in the troposphere.

  6. ARESE (ARM Enhanced Shortwave Experiment) Science Plan [Atmospheric Radiation Program

    SciTech Connect (OSTI)

    Valero, F.P.J.; Schwartz, S.E.; Cess, R.D.; Ramanathan, V.; Collins, W.D.; Minnis, P.; Ackerman, T.P.; Vitko, J.; Tooman, T.P.

    1995-09-27

    Several recent studies have indicated that cloudy atmospheres may absorb significantly more solar radiation than currently predicted by models. The magnitude of this excess atmospheric absorption, is about 50% more than currently predicted and would have major impact on our understanding of atmospheric heating. Incorporation of this excess heating into existing general circulation models also appears to ameliorate some significant shortcomings of these models, most notably a tendency to overpredict the amount of radiant energy going into the oceans and to underpredict the tropopause temperature. However, some earlier studies do not show this excess absorption and an underlying physical mechanism that would give rise to such absorption has yet to be defined. Given the importance of this issue, the Department of Energy's (DOE) Atmospheric Radiation Measurement (ARM) program is sponsoring the ARM Enhanced Shortwave Experiment (ARESE) to study the absorption of solar radiation by clear and cloudy atmospheres. The experimental results will be compared with model calculations. Measurements will be conducted using three aircraft platforms (ARM-UAV Egrett, NASA ER-2, and an instrumented Twin Otter), as well as satellites and the ARM central and extended facilities in North Central Oklahoma. The project will occur over a four week period beginning in late September, 1995. Spectral broadband, partial bandpass, and narrow bandpass (10nm) solar radiative fluxes will be measured at different altitudes and at the surface with the objective to determine directly the magnitude and spectral characteristics of the absorption of shortwave radiation by the atmosphere (clear and cloudy). Narrow spectral channels selected to coincide with absorption by liquid water and ice will help in identifying the process of absorption of radiation. Additionally, information such as water vapor profiles, aerosol optical depths, cloud structure and ozone profiles, needed to use as input in radiative transfer calculations, will be acquired using the aircraft and surface facilities available to ARESE. This document outlines the scientific approach and measurement requirements of the project.

  7. ATMOSPHERIC CIRCULATION OF BROWN DWARFS: JETS, VORTICES, AND TIME VARIABILITY

    SciTech Connect (OSTI)

    Zhang, Xi; Showman, Adam P.

    2014-06-10

    A variety of observational evidence demonstrates that brown dwarfs exhibit active atmospheric circulations. In this study we use a shallow-water model to investigate the global atmospheric dynamics in the stratified layer overlying the convective zone on these rapidly rotating objects. We show that the existence and properties of the atmospheric circulation crucially depend on key parameters including the energy injection rate and radiative timescale. Under conditions of strong internal heat flux and weak radiative dissipation, a banded flow pattern comprised of east-west jet streams spontaneously emerges from the interaction of atmospheric turbulence with the planetary rotation. In contrast, when the internal heat flux is weak and/or radiative dissipation is strong, turbulence injected into the atmosphere damps before it can self-organize into jets, leading to a flow dominated by transient eddies and isotropic turbulence instead. The simulation results are not very sensitive to the form of the forcing. Based on the location of the transition between jet-dominated and eddy-dominated regimes, we suggest that many brown dwarfs may exhibit atmospheric circulations dominated by eddies and turbulence (rather than jets) due to the strong radiative damping on these worlds, but a jet structure is also possible under some realistic conditions. Our simulated light curves capture important features from observed infrared light curves of brown dwarfs, including amplitude variations of a few percent and shapes that fluctuate between single-peak and multi-peak structures. More broadly, our work shows that the shallow-water system provides a useful tool to illuminate fundamental aspects of the dynamics on these worlds.

  8. 2010 Atmospheric System Research (ASR) Science Team Meeting Summary

    SciTech Connect (OSTI)

    Dupont, DL

    2011-05-04

    This document contains the summaries of papers presented in poster format at the March 2010 Atmospheric System Research Science Team Meeting held in Bethesda, Maryland. More than 260 posters were presented during the Science Team Meeting. Posters were sorted into the following subject areas: aerosol-cloud-radiation interactions, aerosol properties, atmospheric state and surface, cloud properties, field campaigns, infrastructure and outreach, instruments, modeling, and radiation. To put these posters in context, the status of ASR at the time of the meeting is provided here.

  9. ARM - Field Campaign - The MOSAiC Atmosphere

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    govCampaignsThe MOSAiC Atmosphere Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : The MOSAiC Atmosphere 2019.09.01 - 2020.10.31 Lead Scientist : Matthew Shupe Abstract Arctic climate change is amplified relative to global change and is embodied by a dramatic decline in the perennial sea-ice pack. These cryospheric transitions carry significant implications for regional resource development, geopolitics, and global climate patterns.

  10. Lower Atmospheric Boundary Layer Experiment (LABLE) Final Campaign Report

    SciTech Connect (OSTI)

    Klein, P; Bonin, TA; Newman, JF; Turner, DD; Chilson, P; Blumberg, WG; Mishra, S; Wainwright, CE; Carney, M; Jacobsen, EP; Wharton, S

    2015-11-01

    The Lower Atmospheric Boundary Layer Experiment (LABLE) included two measurement campaigns conducted at the Atmospheric Radiation Measurement (ARM) Southern Great Plains site in Oklahoma during 2012 and 2013. LABLE was designed as a multi-phase, low-cost collaboration among the University of Oklahoma, the National Severe Storms Laboratory, Lawrence Livermore National Laboratory, and the ARM program. A unique aspect was the role of graduate students in LABLE. They served as principal investigators and took the lead in designing and conducting experiments using different sampling strategies to best resolve boundary-layer phenomena.

  11. PHOTOCHEMISTRY IN TERRESTRIAL EXOPLANET ATMOSPHERES. II. H{sub 2}S AND SO{sub 2} PHOTOCHEMISTRY IN ANOXIC ATMOSPHERES

    SciTech Connect (OSTI)

    Hu Renyu; Seager, Sara; Bains, William

    2013-05-20

    Sulfur gases are common components in the volcanic and biological emission on Earth, and are expected to be important input gases for atmospheres on terrestrial exoplanets. We study the atmospheric composition and the spectra of terrestrial exoplanets with sulfur compounds (i.e., H{sub 2}S and SO{sub 2}) emitted from their surfaces. We use a comprehensive one-dimensional photochemistry model and radiative transfer model to investigate the sulfur chemistry in atmospheres ranging from reducing to oxidizing. The most important finding is that both H{sub 2}S and SO{sub 2} are chemically short-lived in virtually all types of atmospheres on terrestrial exoplanets, based on models of H{sub 2}, N{sub 2}, and CO{sub 2} atmospheres. This implies that direct detection of surface sulfur emission is unlikely, as their surface emission rates need to be extremely high (>1000 times Earth's volcanic sulfur emission) for these gases to build up to a detectable level. We also find that sulfur compounds emitted from the surface lead to photochemical formation of elemental sulfur and sulfuric acid in the atmosphere, which would condense to form aerosols if saturated. For terrestrial exoplanets in the habitable zone of Sun-like stars or M stars, Earth-like sulfur emission rates result in optically thick haze composed of elemental sulfur in reducing H{sub 2}-dominated atmospheres for a wide range of particle diameters (0.1-1 {mu}m), which is assumed as a free parameter in our simulations. In oxidized atmospheres composed of N{sub 2} and CO{sub 2}, optically thick haze, composed of elemental sulfur aerosols (S{sub 8}) or sulfuric acid aerosols (H{sub 2}SO{sub 4}), will form if the surface sulfur emission is two orders of magnitude more than the volcanic sulfur emission of Earth. Although direct detection of H{sub 2}S and SO{sub 2} by their spectral features is unlikely, their emission might be inferred by observing aerosol-related features in reflected light with future generation space telescopes.

  12. Excitation of electron Langmuir frequency harmonics in the solar atmosphere

    SciTech Connect (OSTI)

    Fomichev, V. V.; Fainshtein, S. M.; Chernov, G. P.

    2013-05-15

    An alternative mechanism for the excitation of electron Langmuir frequency harmonics as a result of the development of explosive instability in a weakly relativistic beam-plasma system in the solar atmosphere is proposed. The efficiency of the new mechanism as compared to the previously discussed ones is analyzed.

  13. Connectivity to National Atmospheric Release Advisory Center (NARAC)

    Broader source: Directives, Delegations, and Requirements [Office of Management (MA)]

    2003-08-11

    To establish requirements for connectivity with the National Atmospheric Release Advisory Center (NARAC) at Lawrence Livermore National Laboratory for all DOE and NNSA sites and facilities with potential for hazardous materials releases at levels that require emergency response. The requirements of this Notice have been incorporated into DOE O 151.1C, Comprehensive Emergency Management System, dated 11-2-05. No cancellations.

  14. LARGE ABUNDANCES OF POLYCYCLIC AROMATIC HYDROCARBONS IN TITAN'S UPPER ATMOSPHERE

    SciTech Connect (OSTI)

    Lopez-Puertas, M.; Funke, B.; Garcia-Comas, M.; Dinelli, B. M.; Adriani, A.; D'Aversa, E.; Moriconi, M. L.; Boersma, C.; Allamandola, L. J.

    2013-06-20

    In this paper, we analyze the strong unidentified emission near 3.28 {mu}m in Titan's upper daytime atmosphere recently discovered by Dinelli et al. We have studied it by using the NASA Ames PAH IR Spectroscopic Database. The polycyclic aromatic hydrocarbons (PAHs), after absorbing UV solar radiation, are able to emit strongly near 3.3 {mu}m. By using current models for the redistribution of the absorbed UV energy, we have explained the observed spectral feature and have derived the vertical distribution of PAH abundances in Titan's upper atmosphere. PAHs have been found to be present in large concentrations, about (2-3) Multiplication-Sign 10{sup 4} particles cm{sup -3}. The identified PAHs have 9-96 carbons, with a concentration-weighted average of 34 carbons. The mean mass is {approx}430 u; the mean area is about 0.53 nm{sup 2}; they are formed by 10-11 rings on average, and about one-third of them contain nitrogen atoms. Recently, benzene together with light aromatic species as well as small concentrations of heavy positive and negative ions have been detected in Titan's upper atmosphere. We suggest that the large concentrations of PAHs found here are the neutral counterpart of those positive and negative ions, which hence supports the theory that the origin of Titan main haze layer is located in the upper atmosphere.

  15. Atmospheric Radiation Measurement Climate Research Facility (ACRF) Annual Report 2008

    SciTech Connect (OSTI)

    LR Roeder

    2008-12-01

    The Importance of Clouds and Radiation for Climate Change: The Earths surface temperature is determined by the balance between incoming solar radiation and thermal (or infrared) radiation emitted by the Earth back to space. Changes in atmospheric composition, including greenhouse gases, clouds, and aerosols, can alter this balance and produce significant climate change. Global climate models (GCMs) are the primary tool for quantifying future climate change; however, there remain significant uncertainties in the GCM treatment of clouds, aerosol, and their effects on the Earths energy balance. In 1989, the U.S. Department of Energy (DOE) Office of Science created the Atmospheric Radiation Measurement (ARM) Program to address scientific uncertainties related to global climate change, with a specific focus on the crucial role of clouds and their influence on the transfer of radiation in the atmosphere. To reduce these scientific uncertainties, the ARM Program uses a unique twopronged approach: The ARM Climate Research Facility, a scientific user facility for obtaining long-term measurements of radiative fluxes, cloud and aerosol properties, and related atmospheric characteristics in diverse climate regimes; and The ARM Science Program, focused on the analysis of ACRF and other data to address climate science issues associated with clouds, aerosols, and radiation, and to improve GCMs. This report provides an overview of each of these components and a sample of achievements for each in fiscal year (FY) 2008.

  16. Program Abstracts: Formation and Growth of Atmospheric Aerosols

    SciTech Connect (OSTI)

    Peter H. McMurry; Markku Kulmala

    2006-09-07

    DOE provided $11,000 to sponsor the Workshop on New Particle Formation in the Atmosphere, which was held at The Riverwood Inn and Conference Center near Minneapolis, MN from September 7 to 9, 2006. Recent work has shown that new particle formation is an important atmospheric process that must be better understood due to its impact on cloud cover and the Earth's radiation balance. The conference was an informal gathering of atmospheric and basic scientists with expertise pertinent to this topic. The workshop included discussions of: atmospheric modeling; computational chemistry pertinent to clustering; ions and ion induced nucleation; basic laboratory and theoretical studies of nucleation; studies on neutral molecular clusters; interactions of organic compounds and sulfuric acid; composition of freshly nucleated particles. Fifty six scientists attended the conference. They included 27 senior scientists, 9 younger independent scientists (assistant professor or young associate professor level), 7 postdocs, 13 graduate students, 10 women, 35 North Americans (34 from the U.S.), 1 Asian, and 20 Europeans. This was an excellent informal workshop on an important topic. An effort was made to include individuals from communities that do not regularly interact. A number of participants have provided informal feedback indicating that the workshop led to research ideas and possible future collaborations.

  17. National Atmospheric Release Advisory Center | National Nuclear Security

    National Nuclear Security Administration (NNSA)

    Administration Atmospheric Release Advisory Center | National Nuclear Security Administration Facebook Twitter Youtube Flickr RSS People Mission Managing the Stockpile Preventing Proliferation Powering the Nuclear Navy Emergency Response Recapitalizing Our Infrastructure Countering Nuclear Terrorism About Our Programs Our History Who We Are Our Leadership Our Locations Budget Our Operations Library Bios Congressional Testimony Fact Sheets Newsletters Press Releases Photo Gallery Jobs Apply

  18. THE LOS ALAMOS NATIONAL LABORATORY ATMOSPHERIC TRANSPORT AND DIFFUSION MODELS

    SciTech Connect (OSTI)

    M. WILLIAMS

    1999-08-01

    The LANL atmospheric transport and diffusion models are composed of two state-of-the-art computer codes. The first is an atmospheric wind model called HOThlAC, Higher Order Turbulence Model for Atmospheric circulations. HOTMAC generates wind and turbulence fields by solving a set of atmospheric dynamic equations. The second is an atmospheric diffusion model called RAPTAD, Random Particle Transport And Diffusion. RAPTAD uses the wind and turbulence output from HOTMAC to compute particle trajectories and concentration at any location downwind from a source. Both of these models, originally developed as research codes on supercomputers, have been modified to run on microcomputers. Because the capability of microcomputers is advancing so rapidly, the expectation is that they will eventually become as good as today's supercomputers. Now both models are run on desktop or deskside computers, such as an IBM PC/AT with an Opus Pm 350-32 bit coprocessor board and a SUN workstation. Codes have also been modified so that high level graphics, NCAR Graphics, of the output from both models are displayed on the desktop computer monitors and plotted on a laser printer. Two programs, HOTPLT and RAPLOT, produce wind vector plots of the output from HOTMAC and particle trajectory plots of the output from RAPTAD, respectively. A third CONPLT provides concentration contour plots. Section II describes step-by-step operational procedures, specifically for a SUN-4 desk side computer, on how to run main programs HOTMAC and RAPTAD, and graphics programs to display the results. Governing equations, boundary conditions and initial values of HOTMAC and RAPTAD are discussed in Section III. Finite-difference representations of the governing equations, numerical solution procedures, and a grid system are given in Section IV.

  19. High Resolution Atmospheric Modeling for Wind Energy Applications

    SciTech Connect (OSTI)

    Simpson, M; Bulaevskaya, V; Glascoe, L; Singer, M

    2010-03-18

    The ability of the WRF atmospheric model to forecast wind speed over the Nysted wind park was investigated as a function of time. It was found that in the time period we considered (August 1-19, 2008), the model is able to predict wind speeds reasonably accurately for 48 hours ahead, but that its forecast skill deteriorates rapidly after 48 hours. In addition, a preliminary analysis was carried out to investigate the impact of vertical grid resolution on the forecast skill. Our preliminary finding is that increasing vertical grid resolution does not have a significant impact on the forecast skill of the WRF model over Nysted wind park during the period we considered. Additional simulations during this period, as well as during other time periods, will be run in order to validate the results presented here. Wind speed is a difficult parameter to forecast due the interaction of large and small length scale forcing. To accurately forecast the wind speed at a given location, the model must correctly forecast the movement and strength of synoptic systems, as well as the local influence of topography / land use on the wind speed. For example, small deviations in the forecast track or strength of a large-scale low pressure system can result in significant forecast errors for local wind speeds. The purpose of this study is to provide a preliminary baseline of a high-resolution limited area model forecast performance against observations from the Nysted wind park. Validating the numerical weather prediction model performance for past forecasts will give a reasonable measure of expected forecast skill over the Nysted wind park. Also, since the Nysted Wind Park is over water and some distance from the influence of terrain, the impact of high vertical grid spacing for wind speed forecast skill will also be investigated.

  20. Study of the atmospheric chemistry of radon progeny in laboratory and real indoor atmospheres. Final project report

    SciTech Connect (OSTI)

    Hopke, P.K.

    1996-09-01

    This report completes Clarkson University`s study of the chemical and physical behavior of the {sup 218}Po atom immediately following its formation by the alpha decay of radon. Because small changes in size for activity in the sub-10 nm size range result in large changes in the delivered dose per unit exposure, this behavior must be understood if the exposure to radon progeny and it dose to the cells in the respiratory tract are to be fully assessed. In order to pursue this general goal, two areas of radon progeny behavior are being pursued; laboratory studies under controlled conditions to better understand the fundamental physical and chemical processes that affect the progeny`s atmospheric behavior and studies in actual indoor environments to develop a better assessment of the exposure of the occupants of that space to the size and concentration of the indoor radioactive aerosol. Thus, two sets of specific goals have been established for this project. The specific tasks of the controlled laboratory studies are (1) Determine the formation rates of {circ}OH radicals formed by the radiolysis of air following radon decay; (2) Examine the formation of particles by the radiolytic oxidation of substances like SO{sub 2}, ethylene, and H{sub 2}S to lower vapor pressure compounds and determine the role of gas phase additives such as H{sub 2}O and NH{sub 3} in determining the particle size; (3) Measure the rate of ion-induced nucleation using a thermal diffusion cloud chamber, and (4) Measure the neutralization rate of {sup 218}PoO{sub x}{sup +} in O{sub 2} at low radon concentrations.

  1. Constraining the atmospheric composition of the day-night terminators of HD 189733b: Atmospheric retrieval with aerosols

    SciTech Connect (OSTI)

    Lee, Jae-Min; Irwin, Patrick G. J.; Fletcher, Leigh N.; Barstow, Joanna K.; Heng, Kevin

    2014-07-01

    A number of observations have shown that Rayleigh scattering by aerosols dominates the transmission spectrum of HD 189733b at wavelengths shortward of 1 ?m. In this study, we retrieve a range of aerosol distributions consistent with transmission spectroscopy between 0.3-24 ?m that were recently re-analyzed by Pont et al. To constrain the particle size and the optical depth of the aerosol layer, we investigate the degeneracies between aerosol composition, temperature, planetary radius, and molecular abundances that prevent unique solutions for transit spectroscopy. Assuming that the aerosol is composed of MgSiO{sub 3}, we suggest that a vertically uniform aerosol layer over all pressures with a monodisperse particle size smaller than about 0.1 ?m and an optical depth in the range 0.002-0.02 at 1 ?m provides statistically meaningful solutions for the day/night terminator regions of HD 189733b. Generally, we find that a uniform aerosol layer provide adequate fits to the data if the optical depth is less than 0.1 and the particle size is smaller than 0.1 ?m, irrespective of the atmospheric temperature, planetary radius, aerosol composition, and gaseous molecules. Strong constraints on the aerosol properties are provided by spectra at wavelengths shortward of 1 ?m as well as longward of 8 ?m, if the aerosol material has absorption features in this region. We show that these are the optimal wavelengths for quantifying the effects of aerosols, which may guide the design of future space observations. The present investigation indicates that the current data offer sufficient information to constrain some of the aerosol properties of HD189733b, but the chemistry in the terminator regions remains uncertain.

  2. New analysis indicates no thermal inversion in the atmosphere of HD 209458b

    SciTech Connect (OSTI)

    Diamond-Lowe, Hannah; Stevenson, Kevin B.; Bean, Jacob L.; Line, Michael R.; Fortney, Jonathan J.

    2014-11-20

    An important focus of exoplanet research is the determination of the atmospheric temperature structure of strongly irradiated gas giant planets, or hot Jupiters. HD 209458b is the prototypical exoplanet for atmospheric thermal inversions, but this assertion does not take into account recently obtained data or newer data reduction techniques. We reexamine this claim by investigating all publicly available Spitzer Space Telescope secondary-eclipse photometric data of HD 209458b and performing a self-consistent analysis. We employ data reduction techniques that minimize stellar centroid variations, apply sophisticated models to known Spitzer systematics, and account for time-correlated noise in the data. We derive new secondary-eclipse depths of 0.119% 0.007%, 0.123% 0.006%, 0.134% 0.035%, and 0.215% 0.008% in the 3.6, 4.5, 5.8, and 8.0 ?m bandpasses, respectively. We feed these results into a Bayesian atmospheric retrieval analysis and determine that it is unnecessary to invoke a thermal inversion to explain our secondary-eclipse depths. The data are well fitted by a temperature model that decreases monotonically between pressure levels of 1 and 0.01 bars. We conclude that there is no evidence for a thermal inversion in the atmosphere of HD 209458b.

  3. Atmospheric Radiation Measurement Program facilities newsletter, April 2000

    SciTech Connect (OSTI)

    Sisterson, D. L.

    2000-05-05

    This issue of the Atmospheric Radiation Measurement Program (ARM Program) monthly newsletter is about the ARM Program goal to improve scientific understanding of the interactions of sunlight (solar radiation) with the atmosphere, then incorporate this understanding into computer models of climate change. To model climate accurately all around the globe, a variety of data must be collected from many locations on Earth. For its Cloud and Radiation Testbed (CART) sites, ARM chose locations in the US Southern Great Plains, the North Slope of Alaska, and the Tropical Western Pacific Ocean to represent different climate types around the world. In this newsletter they consider the North Slope of Alaska site, with locations at Barrow and Atqasuk, Alaska.

  4. The Atmospheric Muon Charge Ratio at the MINOS Near Detector

    SciTech Connect (OSTI)

    de Jong, J.K.; /IIT, Chicago /Oxford U.

    2011-11-01

    The magnetized MINOS near detector can accurately determine the charge sign of atmospheric muons, this facilitates a measurement of the atmospheric muon charge ratio. To reduce the systematic error associated with geometric bias and acceptance we have combined equal periods of data obtained with opposite magnetic field polarities. We report a charge ratio of 1.2666 {+-} 0.0015(stat.){sub -0.0088}{sup +0.0096}(syst.) at a mean E{sub {mu},0{sup cos}}({theta}) = 63 GeV. This measurement is consistent with the world average but significantly lower than the earlier observation at the MINOS far detector. This increase is shown to be consistent with the hypothesis that a greater fraction of the observed muons arise from kaon decay within the cosmic ray shower.

  5. National Atmospheric Release Advisory Center (NARAC) Capabilities for Homeland Security

    SciTech Connect (OSTI)

    Sugiyama, G; Nasstrom, J; Baskett, R; Simpson, M

    2010-03-08

    The Department of Energy's National Atmospheric Release Advisory Center (NARAC) provides critical information during hazardous airborne releases as part of an integrated national preparedness and response strategy. Located at Lawrence Livermore National Laboratory, NARAC provides 24/7 tools and expert services to map the spread of hazardous material accidentally or intentionally released into the atmosphere. NARAC graphical products show affected areas and populations, potential casualties, and health effect or protective action guideline levels. LLNL experts produce quality-assured analyses based on field data to assist decision makers and responders. NARAC staff and collaborators conduct research and development into new science, tools, capabilities, and technologies in strategically important areas related to airborne transport and fate modeling and emergency response. This paper provides a brief overview of some of NARAC's activities, capabilities, and research and development.

  6. Atmospheric Science Program. Summaries of research in FY 1994

    SciTech Connect (OSTI)

    1995-06-01

    This report provides descriptions for all projects funded by ESD under annual contracts in FY 1994. Each description contains the project`s title; three-year funding history (in thousands of dollars); the contract period over which the funding applies; the name(s) of the principal investigator(s); the institution(s) conducting the projects; and the project`s objectives, products, approach, and results to date (for most projects older than one year). Project descriptions are categorized within the report according to program areas: atmospheric chemistry, atmospheric dynamics, and support operations. Within these categories, the descriptions are ordered alphabetically by principal investigator. Each program area is preceded by a brief text that defines the program area, states it goals and objectives, lists principal research questions, and identifies program managers. Appendixes provide the addresses and telephone numbers of the principal investigators and define the acronyms used.

  7. Unintended consequences of atmospheric injection of sulphate aerosols.

    SciTech Connect (OSTI)

    Brady, Patrick Vane; Kobos, Peter Holmes; Goldstein, Barry

    2010-10-01

    Most climate scientists believe that climate geoengineering is best considered as a potential complement to the mitigation of CO{sub 2} emissions, rather than as an alternative to it. Strong mitigation could achieve the equivalent of up to -4Wm{sup -2} radiative forcing on the century timescale, relative to a worst case scenario for rising CO{sub 2}. However, to tackle the remaining 3Wm{sup -2}, which are likely even in a best case scenario of strongly mitigated CO{sub 2} releases, a number of geoengineering options show promise. Injecting stratospheric aerosols is one of the least expensive and, potentially, most effective approaches and for that reason an examination of the possible unintended consequences of the implementation of atmospheric injections of sulphate aerosols was made. Chief among these are: reductions in rainfall, slowing of atmospheric ozone rebound, and differential changes in weather patterns. At the same time, there will be an increase in plant productivity. Lastly, because atmospheric sulphate injection would not mitigate ocean acidification, another side effect of fossil fuel burning, it would provide only a partial solution. Future research should aim at ameliorating the possible negative unintended consequences of atmospheric injections of sulphate injection. This might include modeling the optimum rate and particle type and size of aerosol injection, as well as the latitudinal, longitudinal and altitude of injection sites, to balance radiative forcing to decrease negative regional impacts. Similarly, future research might include modeling the optimum rate of decrease and location of injection sites to be closed to reduce or slow rapid warming upon aerosol injection cessation. A fruitful area for future research might be system modeling to enhance the possible positive increases in agricultural productivity. All such modeling must be supported by data collection and laboratory and field testing to enable iterative modeling to increase the accuracy and precision of the models, while reducing epistemic uncertainties.

  8. T AMS ARAC (Atmospheric Release Advisory Capability) NEST RAP

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    T AMS ARAC (Atmospheric Release Advisory Capability) NEST RAP . . INTRODUCTION ARAC ARAC he Department of Energy's (DOE) National Nuclear Security Administration (NNSA) has the world's leading scientists, engineers and technicians from over 50 years of managing the nation's nuclear weapons program. When the need arises, DOE is prepared to respond immediately to any type of radiological accident or incident anywhere in the world with the following seven radiological emergency response assets.

  9. ARM - Publications: Science Team Meeting Documents: Atmospheric Modes of

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Drizzling Stratus at the ARM SGP Site Atmospheric Modes of Drizzling Stratus at the ARM SGP Site Kollias, Pavlos RSMAS/University of Miami Albrecht, Bruce University of Miami The representation of boundary layer clouds in GCMs remains a source of uncertainty in climate simulations. The cloud amount in the boundary layer is sensitive to the boundary layer scheme. Furthermore, little is known on the climatology of drizzling or precipitating boundary layer clouds, their seasonal variability and

  10. Hierardlicsl Diagnosis V. V. Zuev Institute of Atmospheric Optics

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Hierardlicsl Diagnosis V. V. Zuev Institute of Atmospheric Optics Siberian Branch of the Russian Academy of Sciences Tomsk, Russia Systematic observations of the earth's ozone layer over the last ten years indicate a steady decrease of ozone content in the stratospheric maximum and, on the contrary, a increase of ozone concentrations in the troposphere. This trend is illustrated clearly by the results of 20 years' observations of high-altitude ozone concentration distribution in the troposphere

  11. MONTE CARLO SIMULATION OF METASTABLE OXYGEN PHOTOCHEMISTRY IN COMETARY ATMOSPHERES

    SciTech Connect (OSTI)

    Bisikalo, D. V.; Shematovich, V. I. [Institute of Astronomy of the Russian Academy of Sciences, Moscow (Russian Federation); Grard, J.-C.; Hubert, B. [Laboratory for Planetary and Atmospheric Physics (LPAP), University of Lige, Lige (Belgium); Jehin, E.; Decock, A. [Origines Cosmologiques et Astrophysiques (ORCA), University of Lige (Belgium); Hutsemkers, D. [Extragalactic Astrophysics and Space Observations (EASO), University of Lige (Belgium); Manfroid, J., E-mail: B.Hubert@ulg.ac.be [High Energy Astrophysics Group (GAPHE), University of Lige (Belgium)

    2015-01-01

    Cometary atmospheres are produced by the outgassing of material, mainly H{sub 2}O, CO, and CO{sub 2} from the nucleus of the comet under the energy input from the Sun. Subsequent photochemical processes lead to the production of other species generally absent from the nucleus, such as OH. Although all comets are different, they all have a highly rarefied atmosphere, which is an ideal environment for nonthermal photochemical processes to take place and influence the detailed state of the atmosphere. We develop a Monte Carlo model of the coma photochemistry. We compute the energy distribution functions (EDF) of the metastable O({sup 1}D) and O({sup 1}S) species and obtain the red (630nm) and green (557.7nm) spectral line shapes of the full coma, consistent with the computed EDFs and the expansion velocity. We show that both species have a severely non-Maxwellian EDF, that results in broad spectral lines and the suprathermal broadening dominates due to the expansion motion. We apply our model to the atmosphere of comet C/1996 B2 (Hyakutake) and 103P/Hartley 2. The computed width of the green line, expressed in terms of speed, is lower than that of the red line. This result is comparable to previous theoretical analyses, but in disagreement with observations. We explain that the spectral line shape does not only depend on the exothermicity of the photochemical production mechanisms, but also on thermalization, due to elastic collisions, reducing the width of the emission line coming from the O({sup 1}D) level, which has a longer lifetime.

  12. Evaluation of Routine Atmospheric Sounding Measurements Using Unmanned Systems

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Routine Atmospheric Sounding Measurements Using Unmanned Systems but also to understand the different processes involved in a cloud's life cycle by providing measurements complimentary to those concurrently obtained by instruments stationed at the third ARM Mobile Facility (AMF3) at Oliktok Point. ERASMUS will supply data to address the following science questions: * How does temperature and humidity evolve during transitions between clear and cloudy skies? * How do aerosol properties vary with

  13. Interactive Uses of the NSDL: .Atmospheric Visualization Collection

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Interactive Uses of the NSDL: Atmospheric Visualization Collection C. M. Klaus, E. N. Vernon, T. McCollum, T. R. Gobble, H. M. Anthony, and D. Johnson Argonne National Laboratory Argonne, Illinois K. Andrew Eastern Illinois University Charleston, Illinois G. G. Mace University of Utah Salt Lake City, Utah C. P. Bahrmann University of Oklahoma Norman, Oklahoma User Interfaces The National Science Digital Library (NSDL) has three user interfaces for accessing data images. 1. The Geophysical Focus

  14. Pulsed atmospheric fluidized bed combustor apparatus and process

    DOE Patents [OSTI]

    Mansour, Momtaz N. (Columbia, MD)

    1992-01-01

    A pulsed atmospheric fluidized bed reactor system is disclosed and claimed along with a process for utilization of same for the combustion of, e.g. high sulfur content coal. The system affords a economical, ecologically acceptable alternative to oil and gas fired combustors. The apparatus may also be employed for endothermic reaction, combustion of waste products, e.g. organic and medical waste, drying, calcining and the like.

  15. Atmospheric Sciences Program summaries of research in FY 1993

    SciTech Connect (OSTI)

    Not Available

    1993-11-01

    This document describes the activities and products of the Atmospheric Science Program of the Environmental Sciences Division, Office of Health and Environmental Research, Office of Energy Research, in FY 1993. Each description contains the project`s title; three-year funding history; the contract period over which the funding applies; the name(s) of the principal investigator(s); the institution(s) conducting the projects; and the project`s objectives, products, approach, and results to date. Project descriptions are categorized within the report according to program areas: atmospheric chemistry, atmospheric dynamics, and support operations. Within these categories, the descriptions are ordered alphabetically by principal investigator. Each program area is preceded by a brief text that defines the program area, states its goals and objectives, lists principal research questions, and identifies program managers. Appendixes provide the addresses and telephone numbers of the principal investigators and define the acronyms used. This document has been indexed to aid the reader in locating research topics, participants, and research institutions in the text and the project descriptions. Comprehensive subject, principal investigator, and institution indexes are provided at the end of the text for this purpose. The comprehensive subject index includes keywords from the introduction and chapter texts in addition to those from the project descriptions.

  16. Critical review of studies on atmospheric dispersion in coastal regions

    SciTech Connect (OSTI)

    Shearer, D.L.; Kaleel, R.J.

    1982-09-01

    This study effort was required as a preliminary step prior to initiation of field measurements of atmospheric dispersion in coastal regions. The Nuclear Regulatory Commission (NRC) is in the process of planning an extensive field measurement program to generate data which will serve as improved data bases for licensing decisions, confirmation of regulations, standards, and guides, and for site characterizations. The study being reported here is an effort directed to obtaining as much information as is possible from existing studies that is relevant toward NRC's objectives. For this study, reports covering research and meteorological measurements conducted for industrial purposes, utility needs, military objectives, and academic studies were obtained and critically reviewed in light of NRC's current data needs. This report provides an interpretation of the extent of existing usable information, an indication of the potential for tailoring existing research toward current NRC information needs, and recommendations for several follow-on studies which could provide valuable additional information through reanalysis of the data. Recommendations are also offered regarding new measurement programs. Emphasis is placed on the identification and acquisition of data from atmospheric tracer studies conducted in coastal regions. A total of 225 references were identified which deal with the coastal atmosphere, including meteorological and tracer measurement programs, theoretical descriptions of the relevant processes, and dispersion models.

  17. Retention of elemental mercury in fly ashes in different atmospheres

    SciTech Connect (OSTI)

    M.A. Lopez-Anton; M. Diaz-Somoano; M.R. Martinez-Tarazona

    2007-01-15

    Mercury is an extremely volatile element, which is emitted from coal combustion to the environment mostly in the vapor phase. To avoid the environmental problems that the toxic species of this element may cause, control technologies for the removal of mercury are necessary. Recent research has shown that certain fly ash materials have an affinity for mercury. Moreover, it has been observed that fly ashes may catalyze the oxidation of elemental mercury and facilitate its capture. However, the exact nature of Hg-fly ash interactions is still unknown, and mercury oxidation through fly ash needs to be investigated more thoroughly. In this work, the influence of a gas atmosphere on the retention of elemental mercury on fly ashes of different characteristics was evaluated. The retention capacity was estimated comparatively in inert and two gas atmospheres containing species present in coal gasification and coal combustion. Fly ashes produced in two pulverized coal combustion (PCC) plants, produced from coals of different rank (CTA and CTSR), and a fly ash (CTP) produced in a fluidized bed combustion (FBC) plant were used as raw materials. The mercury retention capacity of these fly ashes was compared to the retention obtained in different activated carbons. Although the capture of mercury is very similar in the gasification atmosphere and N{sub 2}, it is much more efficient in a coal combustion retention, being greater in fly ashes from PCC than those from FBC plants. 22 refs., 6 figs., 3 tabs.

  18. VOCALS: The VAMOS Ocean-Cloud-Atmosphere-Land Study

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    Wood, Robert [VOCALS-REx PI, University of Washington; Bretherton, Christopher [GEWEX/GCSS Representative, University of Washington; Huebert, Barry [SOLAS Representative, University of Hawaii; Mechoso, Roberto C. [VOCALS Science Working Group Chair, UCLA; Weller, Robert [Woods Hole Oceanographic Institution

    VOCALS (VAMOS* Ocean-Cloud-Atmosphere-Land Study) is an international CLIVAR program the major goal of which is to develop and promote scientific activities leading to improved understanding of the Southeast Pacific (SEP) coupled ocean-atmosphere-land system on diurnal to inter-annual timescales. The principal program objectives are: 1) the improved understanding and regional/global model representation of aerosol indirect effects over the SEP; 2) the elimination of systematic errors in the region of coupled atmospheric-ocean general circulation models, and improved model simulations and predictions of the coupled climate in the SEP and global impacts of the system variability. VOCALS is organized into two tightly coordinated components: 1) a Regional Experiment (VOCALSREx), and 2) a Modeling Program (VOCALS-Mod). Extended observations (e.g. IMET buoy, satellites, EPIC/PACS cruises) will provide important additional contextual datasets that help to link the field and the modeling components. The coordination through VOCALS of observational and modeling efforts (Fig. 3) will accelerate the rate at which field data can be used to improve simulations and predictions of the tropical climate variability [Copied from the Vocals Program Summary of June 2007, available as a link from the VOCALS web at http://www.eol.ucar.edu/projects/vocals/]. The CLIVAR sponsored program to under which VOCALS falls is VAMOS, which stands for Variability of the American Monsoon Systems.

  19. Atmospheric Rivers Coming to a Cloud Near You (Other) | SciTech...

    Office of Scientific and Technical Information (OSTI)

    Other: Atmospheric Rivers Coming to a Cloud Near You Citation Details In-Document Search Title: Atmospheric Rivers Coming to a Cloud Near You You are accessing a document from...

  20. About EffectiveŽ Height of the Aerosol Atmosphere in Visible and IR Wavelength Range

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    "Effective" Height of the Aerosol Atmosphere in Visible and IR Wavelength Range V. N. Uzhegov, D. M. Kabanov, M. V. Panchenko, Yu. A. Pkhalagov, and S. M. Sakerin Institute of Atmospheric Optics Tomsk, Russia Introduction Aerosol component of the atmosphere is one of the important factors affecting the radiation budget of the space - atmosphere - underlying surface system in visible and infrared (IR) wavelength ranges. It is extremely important to take into account the contribution of

  1. The mean climate of the Community Atmosphere Model (CAM4) in forced SST and

    Office of Scientific and Technical Information (OSTI)

    fully coupled experiments (Journal Article) | SciTech Connect Journal Article: The mean climate of the Community Atmosphere Model (CAM4) in forced SST and fully coupled experiments Citation Details In-Document Search Title: The mean climate of the Community Atmosphere Model (CAM4) in forced SST and fully coupled experiments The Community Atmosphere Model, version 4 (CAM4) was released as the atmosphere component of the Community Climate System Model, version 4 (CCSM4) and is described. The

  2. Quantitative infrared absorption cross-sections of isoprene for atmospheric measurements

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Brauer, C. S.; Blake, T. A.; Guenther, A. B.; Sams, R. L.; Johnson, T. J.

    2014-04-25

    Isoprene (C5H8, 2-methyl-1,3-butadiene) is a volatile organic compound (VOC) that is one of the primary contributors to annual global VOC emissions. Produced by vegetation as well as anthropogenic sources, the OH- and O3-initiated oxidations of isoprene are a major source of atmospheric oxygenated organics. Few quantitative infrared studies have been reported for isoprene, however, limiting the ability to quantify isoprene emissions via stand-off infrared or in situ detection. We thus report absorption coefficients and integrated band intensities for isoprene in the 600–6500 cm−1 region. The pressure-broadened (1 atmosphere N2) spectra were recorded at 278, 298 and 323 K in amore » 19.94 cm path length cell at 0.112 cm−1 resolution, using a Bruker 66v FTIR. Composite spectra are derived from a minimum of seven isoprene sample pressures at each temperature and the number densities are normalized to 296 K and 1 atmosphere.« less

  3. Magnetohydrostatic equilibrium. II. Three-dimensional multiple open magnetic flux tubes in the stratified solar atmosphere

    SciTech Connect (OSTI)

    Gent, F. A.; Erdlyi, R.; Fedun, V.

    2014-07-01

    A system of multiple open magnetic flux tubes spanning the solar photosphere and lower corona is modeled analytically, within a realistic stratified atmosphere subject to solar gravity. This extends results for a single magnetic flux tube in magnetohydrostatic equilibrium, described in Gent et al. Self-similar magnetic flux tubes are combined to form magnetic structures, which are consistent with high-resolution observations. The observational evidence supports the existence of strands of open flux tubes and loops persisting in a relatively steady state. Self-similar magnetic flux tubes, for which an analytic solution to the plasma density and pressure distribution is possible, are combined. We calculate the appropriate balancing forces, applying to the equations of momentum and energy conservation to preserve equilibrium. Multiplex flux tube configurations are observed to remain relatively stable for up to a day or more, and it is our aim to apply our model as the background condition for numerical studies of energy transport mechanisms from the solar surface to the corona. We apply magnetic field strength, plasma density, pressure, and temperature distributions consistent with observational and theoretical estimates for the lower solar atmosphere. Although each flux tube is identical in construction apart from the location of the radial axis, combinations can be applied to generate a non-axisymmetric magnetic field with multiple non-uniform flux tubes. This is a considerable step forward in modeling the realistic magnetized three-dimensional equilibria of the solar atmosphere.

  4. Magnetospheric structure and atmospheric Joule heating of habitable planets orbiting M-dwarf stars

    SciTech Connect (OSTI)

    Cohen, O.; Drake, J. J.; Garraffo, C.; Poppenhaeger, K.; Glocer, A.; Ridley, A. J.; Gombosi, T. I.

    2014-07-20

    We study the magnetospheric structure and the ionospheric Joule Heating of planets orbiting M-dwarf stars in the habitable zone using a set of magnetohydrodynamic models. The stellar wind solution is used to drive a model for the planetary magnetosphere, which is coupled with a model for the planetary ionosphere. Our simulations reveal that the space environment around close-in habitable planets is extreme, and the stellar wind plasma conditions change from sub- to super-Alfvnic along the planetary orbit. As a result, the magnetospheric structure changes dramatically with a bow shock forming in the super-Alfvnic sectors, while no bow shock forms in the sub-Alfvnic sectors. The planets reside most of the time in the sub-Alfvnic sectors with poor atmospheric protection. A significant amount of Joule Heating is provided at the top of the atmosphere as a result of the intense stellar wind. For the steady-state solution, the heating is about 0.1%-3% of the total incoming stellar irradiation, and it is enhanced by 50% for the time-dependent case. The significant Joule Heating obtained here should be considered in models for the atmospheres of habitable planets in terms of the thickness of the atmosphere, the top-side temperature and density, the boundary conditions for the atmospheric pressure, and particle radiation and transport. Here we assume constant ionospheric Pedersen conductance similar to that of the Earth. The conductance could be greater due to the intense EUV radiation leading to smaller heating rates. We plan to quantify the ionospheric conductance in future study.

  5. Untangling the Chemical Evolution of Titan's Atmosphere and Surface -- From Homogeneous to Heterogeneous Chemistry

    SciTech Connect (OSTI)

    Kaiser, Ralf I.; Maksyutenko, Pavlo; Ennis, Courtney; Zhang, Fangtong; Gu, Xibin; Krishtal, Sergey P.; Mebel, Alexander M.; Kostko, Oleg; Ahmed, Musahid

    2010-03-16

    The arrival of the Cassini-Huygens probe at Saturn's moon Titan - the only Solar System body besides Earth and Venus with a solid surface and a thick atmosphere with a pressure of 1.4 atm at surface level - in 2004 opened up a new chapter in the history of Solar System exploration. The mission revealed Titan as a world with striking Earth-like landscapes involving hydrocarbon lakes and seas as well as sand dunes and lava-like features interspersed with craters and icy mountains of hitherto unknown chemical composition. The discovery of a dynamic atmosphere and active weather system illustrates further the similarities between Titan and Earth. The aerosol-based haze layers, which give Titan its orange-brownish color, are not only Titan's most prominent optically visible features, but also play a crucial role in determining Titan's thermal structure and chemistry. These smog-like haze layers are thought to be very similar to those that were present in Earth's atmosphere before life developed more than 3.8 billion years ago, absorbing the destructive ultraviolet radiation from the Sun, thus acting as 'prebiotic ozone' to preserve astrobiologically important molecules on Titan. Compared to Earth, Titan's low surface temperature of 94 K and the absence of liquid water preclude the evolution of biological chemistry as we know it. Exactly because of these low temperatures, Titan provides us with a unique prebiotic 'atmospheric laboratory' yielding vital clues - at the frozen stage - on the likely chemical composition of the atmosphere of the primitive Earth. However, the underlying chemical processes, which initiate the haze formation from simple molecules, have been not understood well to date.

  6. Enhanced transportation of energetic electrons in dual-frequency atmospheric microplasmas

    SciTech Connect (OSTI)

    Kwon, H. C.; Kim, H. Y.; Won, I. H.; Lee, H. Wk.; Shin, H. K.; Lee, J. K.

    2013-02-15

    A comparative study of electron kinetics between single-frequency (SF) microplasmas and their equivalent dual-frequency (DF) microplasmas with matching effective frequencies in atmospheric-pressure helium discharges was performed using particle-in-cell simulation with a Monte Carlo collision. The effective-frequency concept helps in analyzing DF microplasmas in a fashion similar to SF microplasmas with effective parameters. In this study, the plasma characteristics such as the plasma potential, density, and electron energy probability functions of the SF microplasma and its DF counterpart were almost the same. However, the oscillating sheath edge was pushed further into the electrode for a substantial fraction of the time and the sheath width decreased in DF microplasmas. As a result, the transportation of the energetic electrons ({epsilon} > 4 eV) usable for tailoring the surface chemistry in atmospheric microplasmas is enhanced in DF microplasmas as compared to SF microplasmas.

  7. Abiotic ozone and oxygen in atmospheres similar to prebiotic Earth

    SciTech Connect (OSTI)

    Domagal-Goldman, Shawn D.; Segura, Antgona; Claire, Mark W.; Robinson, Tyler D.; Meadows, Victoria S.

    2014-09-10

    The search for life on planets outside our solar system will use spectroscopic identification of atmospheric biosignatures. The most robust remotely detectable potential biosignature is considered to be the detection of oxygen (O{sub 2}) or ozone (O{sub 3}) simultaneous to methane (CH{sub 4}) at levels indicating fluxes from the planetary surface in excess of those that could be produced abiotically. Here we use an altitude-dependent photochemical model with the enhanced lower boundary conditions necessary to carefully explore abiotic O{sub 2} and O{sub 3} production on lifeless planets with a wide variety of volcanic gas fluxes and stellar energy distributions. On some of these worlds, we predict limited O{sub 2} and O{sub 3} buildup, caused by fast chemical production of these gases. This results in detectable abiotic O{sub 3} and CH{sub 4} features in the UV-visible, but no detectable abiotic O{sub 2} features. Thus, simultaneous detection of O{sub 3} and CH{sub 4} by a UV-visible mission is not a strong biosignature without proper contextual information. Discrimination between biological and abiotic sources of O{sub 2} and O{sub 3} is possible through analysis of the stellar and atmospheric contextparticularly redox state and O atom inventoryof the planet in question. Specifically, understanding the spectral characteristics of the star and obtaining a broad wavelength range for planetary spectra should allow more robust identification of false positives for life. This highlights the importance of wide spectral coverage for future exoplanet characterization missions. Specifically, discrimination between true and false positives may require spectral observations that extend into infrared wavelengths and provide contextual information on the planet's atmospheric chemistry.

  8. Atmospheric characterization of the hot Jupiter Kepler-13Ab

    SciTech Connect (OSTI)

    Shporer, Avi; O'Rourke, Joseph G.; Knutson, Heather A.; Szab, Gyula M.; Zhao, Ming; Burrows, Adam; Fortney, Jonathan; Agol, Eric; Cowan, Nicolas B.; Desert, Jean-Michel; Howard, Andrew W.; Isaacson, Howard; Lewis, Nikole K.; Showman, Adam P.; Todorov, Kamen O.

    2014-06-10

    Kepler-13Ab (= KOI-13.01) is a unique transiting hot Jupiter. It is one of very few known short-period planets orbiting a hot A-type star, making it one of the hottest planets currently known. The availability of Kepler data allows us to measure the planet's occultation (secondary eclipse) and phase curve in the optical, which we combine with occultations observed by warm Spitzer at 4.5 ?m and 3.6 ?m and a ground-based occultation observation in the K{sub s} band (2.1 ?m). We derive a day-side hemisphere temperature of 2750 160 K as the effective temperature of a black body showing the same occultation depths. Comparing the occultation depths with one-dimensional planetary atmosphere models suggests the presence of an atmospheric temperature inversion. Our analysis shows evidence for a relatively high geometric albedo, A {sub g} = 0.33{sub ?0.06}{sup +0.04}. While measured with a simplistic method, a high A {sub g} is supported also by the fact that the one-dimensional atmosphere models underestimate the occultation depth in the optical. We use stellar spectra to determine the dilution, in the four wide bands where occultation was measured, due to the visual stellar binary companion 1.''15 0.''05 away. The revised stellar parameters measured using these spectra are combined with other measurements, leading to revised planetary mass and radius estimates of M{sub p} = 4.94-8.09 M {sub J} and R{sub p} = 1.406 0.038 R {sub J}. Finally, we measure a Kepler midoccultation time that is 34.0 6.9 s earlier than expected based on the midtransit time and the delay due to light-travel time and discuss possible scenarios.

  9. Optical remote diagnostics of atmospheric propagating beams of ionizing radiation

    DOE Patents [OSTI]

    Karl, Jr., Robert R. (Los Alamos, NM)

    1990-01-01

    Data is obtained for use in diagnosing the characteristics of a beam of ionizing radiation, such as charged particle beams, neutral particle beams, and gamma ray beams. In one embodiment the beam is emitted through the atmosphere and produces nitrogen fluorescence during passage through air. The nitrogen fluorescence is detected along the beam path to provide an intensity from which various beam characteristics can be calculated from known tabulations. Optical detecting equipment is preferably located orthogonal to the beam path at a distance effective to include the entire beam path in the equipment field of view.

  10. Motion characteristics of long ac arcs in atmospheric air

    SciTech Connect (OSTI)

    Gu Shanqiang; He Jinliang; Zeng Rong; Zhang Bo; Xu Guozheng; Chen Weijiang

    2007-01-29

    Experiments on the motion of long alternating current arcs in atmospheric air show that the anode and cathode arc roots have different motion characteristics because of different formation mechanisms. During a half cycle of the arc current, the anode arc root moves towards the direction of magnetic force and occasionally has a jumping motion, while the cathode arc root moves sufficiently slow to consider it stationary and hardly has any jump. The arc column has a complex shape and moves under the drive of the magnetic force and is also quickened by the lower arc root.

  11. Gross Input to Atmospheric Crude Oil Distillation Units

    Gasoline and Diesel Fuel Update (EIA)

    Day) Process: Gross Input to Atmospheric Crude Oil Dist. Units Operable Capacity (Calendar Day) Operating Capacity Idle Operable Capacity Operable Utilization Rate Period: Monthly Annual Download Series History Download Series History Definitions, Sources & Notes Definitions, Sources & Notes Show Data By: Process Area Jul-15 Aug-15 Sep-15 Oct-15 Nov-15 Dec-15 View History U.S. 17,178 16,963 16,394 15,690 16,673 16,848 1985-2015 PADD 1 1,192 1,196 1,063 1,133 1,190 1,136 1985-2015 East

  12. COLLOQUIUM: Toward a Better Understanding of the Solar Atmosphere:

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Combining Observations and Numerical Modeling | Princeton Plasma Physics Lab September 21, 2015, 4:00pm to 5:30pm Colloquia MBG Auditorium COLLOQUIUM: Toward a Better Understanding of the Solar Atmosphere: Combining Observations and Numerical Modeling Dr. Bart De Pontieu Solar and Astrophysics Laboratory, Lockheed Martin, Inc. Presentation: File MC21SEP2015_BDePontieu_PPT.pptx The study of the Sun, our nearest star, is making rapid progress, through a combination of a host of new space-based

  13. Gap-dependent transitions of atmospheric microplasma in open air

    SciTech Connect (OSTI)

    Chu, Hong-Yu; Huang, Bo-Shiun

    2011-04-15

    We report on the gap dependence of the planar atmospheric microplasma in air. We investigate the transitions of the dielectric barrier discharge in open air, including the random walk filaments (plasma columns), localized filaments, stochastic filaments, and diffuse discharge. A star-shaped filamentary discharge pattern is observed after the formation of the localized filaments. The liquid drops found on the dielectric surface further become a confining pattern for star-shaped discharge. We also demonstrate the applications of the insulating pattern for the use of the plasma display in open air by the handwritten characters with UV adhesive.

  14. Atmospheric Trace Gases from the Carbon Dioxide Information Analysis Center (CDIAC)

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    CDIAC products are indexed and searchable through a customized interface powered by ORNL's Mercury search engine. Products include numeric data packages, publications, trend data, atlases, models, etc. and can be searched for by subject area, keywords, authors, product numbers, time periods, collection sites, spatial references, etc. Some of the collections may also be included in the CDIAC publication, Trends Online: A Compendium of Global Change Data. Most data sets, many with numerous data files, are free to download from CDIAC's ftp area. The collections under the CDIAC heading of Atmospheric Trace Gases include: Atmospheric Carbon Dioxide, Atmospheric Methane, Atmospheric Carbon Monoxide, Atmospheric Hydrogen, Isotopes in Greenhouse Gases, Radionuclides, Aerosols, and Other Trace Gases.

  15. On the numerical treatment of problems in atmospheric chemistry

    SciTech Connect (OSTI)

    Aro, C.J.

    1995-09-01

    Atmospheric chemical-radiative-transport (CRT) models are vital in performing research on atmospheric chemical change. Even with the enormous computing capability delivered by massively parallel systems, extended three dimensional CRT simulations are still not computationally feasible. The major obstacle in a CRT model is the nonlinear ODE system describing the chemical kinetics in the model. These ODE systems are usually very stiff and account for anywhere from 75% to 90% of the CPU time required to run a CRT model. In this study, a simple explicit class of time stepping method is developed and demonstrated to be useful in treating chemical ODE systems without the use of a Jacobian matrix. These methods, called preconditioned time differencing methods, are tested on small mathematically idealized problems, box model problems, and full 2-D and 3-D CRT models. The methods are found to be both fast and memory efficient. Studies are performed on both vector and parallel systems. The preconditioned time differencing methods are established as a viable alternative to the more common backward differentiation formulas in terms of CPU speed across architectural platforms.

  16. Atmospheric Dispersion Modeling: Challenges of the Fukushima Daiichi Response

    SciTech Connect (OSTI)

    Sugiyama, Gayle; Nasstrom, John; Pobanz, Brenda; Foster, Kevin; Simpson, Matthew; Vogt, Phil; Aluzzi, Fernando; Homann, Steve

    2012-05-01

    The U.S. Department of Energy’s (DOE) National Atmospheric Release Advisory Center (NARAC) provided a wide range of predictions and analyses as part of the response to the Fukushima Daiichi Nuclear Power Plant accident. This work encompassed: weather forecasts and atmospheric transport predictions, estimates of possible dose in Japan based on hypothetical U.S. Nuclear Regulatory Commission scenarios of potential radionuclide releases, predictions of possible plume arrival times and dose levels at U.S. locations, and source estimation and plume model refinement. An overview of NARAC response activities is provided, along with a more in-depth discussion of some of NARAC’s preliminary source reconstruction analyses. NARAC optimized the overall agreement of model predictions to dose rate measurements using statistical comparisons of data and model values paired in space and time. Estimated emission rates varied depending on the choice of release assumptions (e.g., time-varying vs. constant release rates), the radionuclide mix, meteorology, and/or the radiological data used in the analysis. Results were found to be consistent with other studies within expected uncertainties, despite the application of different source estimation methodologies and the use of significantly different radiological measurement data. A discussion of some of the operational and scientific challenges encountered during the response, along with recommendations for future work, is provided.

  17. Experimental studies on atmospheric Stirling engine NAS-2

    SciTech Connect (OSTI)

    Watanabe, Hiroichi; Isshiki, Naotsugu; Ohtomo, Michihiro

    1996-12-31

    Atmospheric hot air Stirling engine NAS-1 and 2 have a simple flat rubber sheet diaphragm as their power piston, and they have been experimentally studied at Nihon University for several years continuously, with the target of to get more than 100 watts shaft power by atmospheric air with simple construction and cheap material. The first NAS-1 was intended to be a solar heated engine using television glass and wood for cheap cost, but it failed by thermal break of glass, so the improved NAS-2 is changed to be heated by gas burner, using metallic materials in all parts except rubber power piston. Other than this rubber sheet diaphragm, NAS-2 has many features as using James Watt crank mechanism, high finny copper tube for conventional commercial heat exchanger, and two kinds of hot gas heaters, etc. About the rubber sheet for the power piston, the thickness of the sheet was changed from 2 mm to 6 mm gradually to known what thickness is best, and it is found that about 5 mm is best for this engine. After trying many improvements on this engine, NAS-2 has produced about 130 watt shaft power with indicated power of 350 watt at 1994. In this paper detail of many features, history, results and experiments of these NAS engines are reported.

  18. Multi-center airborne coherent atmospheric wind sensor (MACAWS)

    SciTech Connect (OSTI)

    Rothermel, J.; Menzies, R.T.; Tratt, D.M.

    1996-11-01

    The Multi-center Airborne Coherent Atmospheric Wind Sensor (MACAWS) is an airborne scanning coherent Doppler lidar designed to acquire remote multi-dimensional measurements of winds and absolute aerosol backscatter in the troposphere and lower stratosphere. These measurements enable study of atmospheric dynamic processes and features at scales of motion that may be undersampled by, or may be beyond the capability of, existing or planned sensors. MACAWS capabilities enable more realistic assessments of concepts in global tropospheric wind measurement with satellite Doppler lidar, as well as a unique capability to validate the NASA Scatterometer currently scheduled for launch in late 1996. MACAWS consists of a Joule-class CO{sub 2} coherent Doppler lidar on a ruggedized optical table, a programmable scanner to direct the lidar beam in the desired direction, and a dedicated inertial navigation system to account for variable aircraft attitude and speed. MACAWS was flown for the first time in September 1995, over the eastern Pacific Ocean and western US. 33 refs., 2 figs.

  19. Characterization of extreme precipitation within atmospheric river events over California

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Jeon, S.; Prabhat,; Byna, S.; Gu, J.; Collins, W. D.; Wehner, M. F.

    2015-11-17

    Atmospheric rivers (ARs) are large, spatially coherent weather systems with high concentrations of elevated water vapor. These systems often cause severe downpours and flooding over the western coastal United States – and with the availability of more atmospheric moisture in the future under global warming we expect ARs to play an important role as potential causes of extreme precipitation changes. Therefore, we aim to investigate changes in extreme precipitation properties correlated with AR events in a warmer climate, which are large-scale meteorological patterns affecting the weather and climate of California. We have recently developed the TECA (Toolkit for Extreme Climatemore » Analysis) software for automatically identifying and tracking features in climate data sets. Specifically, we can now identify ARs that make landfall on the western coast of North America. Based on this detection procedure, we can investigate the impact of ARs by exploring the spatial extent of AR precipitation using climate model (CMIP5) simulations and characterize spatial patterns of dependence for future projections between AR precipitation extremes under climate change within the statistical framework. Our results show that AR events in the future RCP (Representative Concentration Pathway)8.5 scenario (2076–2100) tend to produce heavier rainfall with higher frequency and longer days than events from the historical run (1981–2005). We also find that the dependence between extreme precipitation events has a shorter spatial range, within localized areas in California, under the high future emissions scenario than under the historical run.« less

  20. Design of a differential radiometer for atmospheric radiative flux measurements

    SciTech Connect (OSTI)

    LaDelfe, P.C.; Weber, P.G.; Rodriguez, C.W.

    1994-11-01

    The Hemispherical Optimized NEt Radiometer (HONER) is an instrument under development at the Los Alamos National Laboratory for deployment on an unmanned aerospace vehicle as part of the Atmospheric Radiation Measurements (ARM/UAV) program. HONER is a differential radiometer which will measure the difference between the total upwelling and downwelling fluxes and is intended to provide a means of measuring the atmospheric radiative flux divergence. Unlike existing instruments which measure the upwelling and downwelling fluxes separately, HONER will achieve an optical difference by chopping the two fluxes alternately onto a common pyroelectric detector. HONER will provide data resolved into two spectral bands; one covering the solar dominated region from less than 0.4 micrometer to approximately 4.5 micrometers and the other covering the region from approximately 4.5 micrometers to greater than 50 micrometers, dominated by thermal radiation. The means of separating the spectral regions guarantees seamless summation to calculate the total flux. The fields-of-view are near-hemispherical, upward and downward. The instrument can be converted, in flight, from the differential mode to absolute mode, measuring the upwelling and downwelling fluxes separately and simultaneously. The instrument also features continuous calibration from on-board sources. We will describe the design and operation of the sensor head and the on-board reference sources as well as the means of deployment.

  1. Atmospheric Radiation Measurement Program facilities newsletter, January 2000

    SciTech Connect (OSTI)

    Sisterson, D.L.

    2000-02-16

    The subject of this newsletter is the ARM unmanned aerospace vehicle program. The ARM Program's focus is on climate research, specifically research related to solar radiation and its interaction with clouds. The SGP CART site contains highly sophisticated surface instrumentation, but even these instruments cannot gather some crucial climate data from high in the atmosphere. The Department of Energy and the Department of Defense joined together to use a high-tech, high-altitude, long-endurance class of unmanned aircraft known as the unmanned aerospace vehicle (UAV). A UAV is a small, lightweight airplane that is controlled remotely from the ground. A pilot sits in a ground-based cockpit and flies the aircraft as if he were actually on board. The UAV can also fly completely on its own through the use of preprogrammed computer flight routines. The ARM UAV is fitted with payload instruments developed to make highly accurate measurements of atmospheric flux, radiance, and clouds. Using a UAV is beneficial to climate research in many ways. The UAV puts the instrumentation within the environment being studied and gives scientists direct measurements, in contrast to indirect measurements from satellites orbiting high above Earth. The data collected by UAVs can be used to verify and calibrate measurements and calculated values from satellites, therefore making satellite data more useful and valuable to researchers.

  2. A review of wind field models for atmospheric transport

    SciTech Connect (OSTI)

    Ramsdell, J.V. Jr.; Skyllingstad, E.D.

    1993-06-01

    The primary objective of the Hanford Environmental Dose Reconstruction (HEDR) Project is to estimate the radiation dose that individuals could have received as a result of emissions since 1944 from the US Department of Energy`s (DOE) Hanford Site near Richland, Washington. The HEDR Project is developing a computer code to estimate these doses and their uncertainties. The code, known as the HEDR integrated Code (HEDRIC), consists of four separate component codes. One of the component codes, called the Regional Atmospheric Transport Code for Hanford Emission Tracking (RATCHET) combines meteorological and release data to estimate time-integrated air concentrations and surface contamination at specific locations in the vicinity of the Hanford Site. The RATCHET domain covers approximately 75,000 square miles, extending from the crest of the Cascade Mountains on the west to the eastern edge of the Idaho panhandle and from central Oregon on the south to the Canadian border. This letter report explains the procedures in RATCHET that transform observed wind data into the wind fields used in atmospheric transport calculations. It also describes and evaluates alternative procedures not selected for use in RATCHET.

  3. The oceanic cycle and global atmospheric budget of carbonyl sulfide

    SciTech Connect (OSTI)

    Weiss, P.S.

    1994-12-31

    A significant portion of stratospheric air chemistry is influenced by the existence of carbonyl sulfide (COS). This ubiquitous sulfur gas represents a major source of sulfur to the stratosphere where it is converted to sulfuric acid aerosol particles. Stratospheric aerosols are climatically important because they scatter incoming solar radiation back to space and are able to increase the catalytic destruction of ozone through gas phase reactions on particle surfaces. COS is primarily formed at the surface of the earth, in both marine and terrestrial environments, and is strongly linked to natural biological processes. However, many gaps in the understanding of the global COS cycle still exist, which has led to a global atmospheric budget that is out of balance by a factor of two or more, and a lack of understanding of how human activity has affected the cycling of this gas. The goal of this study was to focus on COS in the marine environment by investigating production/destruction mechanisms and recalculating the ocean-atmosphere flux.

  4. Atmospheric mercury (Hg) in the Adirondacks: Concentrations and sources

    SciTech Connect (OSTI)

    Hyun-Deok Choi; Thomas M. Holsen; Philip K. Hopke

    2008-08-15

    Hourly averaged gaseous elemental Hg (GEM) concentrations and hourly integrated reactive gaseous Hg (RGM), and particulate Hg (HgP) concentrations in the ambient air were measured at Huntington Forest in the Adirondacks, New York from June 2006 to May 2007. The average concentrations of GEM, RGM, and HgP were 1.4 {+-} 0.4 ng m{sup -3}, 1.8 {+-} 2.2 pg m{sup -3}, and 3.2 {+-} 3.7 pg m{sup -3}, respectively. RGM represents <3.5% of total atmospheric Hg or total gaseous Hg (TGM: GEM + RGM) and HgP represents <3.0% of the total atmospheric Hg. The highest mean concentrations of GEM, RGM, and HgP were measured during winter and summer whereas the lowest mean concentrations were measured during spring and fall. Significant diurnal patterns were apparent in warm seasons for all species whereas diurnal patterns were weak in cold seasons. RGM was better correlated with ozone concentration and temperature in both warm than the other species. Potential source contribution function (PSCF) analysis was applied to identify possible Hg sources. This method identified areas in Pennsylvania, West Virginia, Ohio, Kentucky, Texas, Indiana, and Missouri, which coincided well with sources reported in a 2002 U.S. mercury emissions inventory. 51 refs., 7 figs., 1 tab.

  5. NUCLEAR POWERED CO2 CAPTURE FROM THE ATMOSPHERE

    SciTech Connect (OSTI)

    Sherman, S

    2008-09-22

    A process for capturing CO{sub 2} from the atmosphere was recently proposed. This process uses a closed cycle of sodium and calcium hydroxide, carbonate, and oxide transformations to capture dilute CO{sub 2} from the atmosphere and to generate a concentrated stream of CO{sub 2} that is amenable to sequestration or subsequent chemical transformations. In one of the process steps, a fossil-fueled lime kiln is needed, which reduces the net CO{sub 2} capture of the process. It is proposed to replace the fossil-fueled lime kiln with a modified kiln heated by a high-temperature nuclear reactor. This will have the effect of eliminating the use of fossil fuels for the process and increasing the net CO{sub 2} capture. Although the process is suitable to support sequestration, the use of a nuclear power source for the process provides additional capabilities, and the captured CO{sub 2} may be combined with nuclear-produced hydrogen to produce liquid fuels via Fischer-Tropsch synthesis or other technologies. Conceivably, such plants would be carbon-neutral, and could be placed virtually anywhere without being tied to fossil fuel sources or geological sequestration sites.

  6. Zeroing and testing units developed for Gerdien atmospheric ion detectors

    SciTech Connect (OSTI)

    Kolarz, P.; Marinkovic, B.P.; Filipovic, D.M.

    2005-04-01

    Low current measurements in atmospheric ion detection using a Gerdien condenser are subjected to numerous sources of error. Zeroing and testing units described in this article, connected as modules to this type of detector, enable some of these errors to be found and eliminated. The zeroing unit provides digital compensation of the zero drift with a digital sample and hold circuit of 12-bit resolution. It overcomes difficulties related to zero drift and techniques used in the zero conductivity determination when the accelerating potential or airflow rate are zero. The testing unit is a current reference of nominally 10{sup -12} A intended for testing and correcting the system on current leakage and other measuring deviations due to changes in atmospheric parameters. This unit is an independent battery-powered module, which provides a charge of 10{sup -12} C per cycle (frequency of order 1 Hz) to the collecting electrode. The control of Gerdien devices is substantially simplified using the zeroing and testing units realized here. Both units are used during 'zero conductivity' regime only.

  7. Materials, methods and devices to detect and quantify water vapor concentrations in an atmosphere

    DOE Patents [OSTI]

    Allendorf, Mark D; Robinson, Alex L

    2014-12-09

    We have demonstrated that a surface acoustic wave (SAW) sensor coated with a nanoporous framework material (NFM) film can perform ultrasensitive water vapor detection at concentrations in air from 0.05 to 12,000 ppmv at 1 atmosphere pressure. The method is extendable to other MEMS-based sensors, such as microcantilevers, or to quartz crystal microbalance sensors. We identify a specific NFM that provides high sensitivity and selectivity to water vapor. However, our approach is generalizable to detection of other species using NFM to provide sensitivity and selectivity.

  8. The Atmospheric Dynamics Mission on the International Space Station--A new technique for observing winds in the atmosphere

    SciTech Connect (OSTI)

    Ingmann, P.; Readings, C. J.; Knott, K.

    1999-01-22

    For the post-2000 time-frame two general classes of Earth Observation missions have been identified to address user requirements (see e.g. ESA, 1995), namely Earth Watch and Earth Explorer missions. One of the candidate Earth Explorer Missions selected for Phase A study is the Atmospheric Dynamics Mission which is intended to exploit a Doppler wind lidar, ALADIN, to measure winds in clear air (ESA, 1995 and ESA, 1996). It is being studied as a candidate for flight on the International Space Station (ISS) as an externally attached payload. The primary, long-term objective of the Atmospheric Dynamics Mission is to provide observations of wind profiles (e.g. radial wind component). Such data would be assimilated into numerical forecasting models leading to an improvement in objective analyses and hence in Numerical Weather Prediction. The mission would also provide data needed to address some of the key concerns of the World Climate Research Programme (WCRP) i.e. quantification of climate variability, validation and improvement of numerical models and process studies relevant to climate change. The newly acquired data would also help realize some of the objectives of the Global Climate Observing System (GCOS)

  9. Pre/post-strike atmospheric assessment system (PAAS)

    SciTech Connect (OSTI)

    Peglow, S. G., LLNL; Molitoris, J. D., LLNL

    1997-02-03

    The Pre/Post-Strike Atmospheric Assessment System was proposed to show the importance of local meteorological conditions in the vicinity of a site suspected of storing or producing toxic agents and demonstrate a technology to measure these conditions, specifically wind fields. The ability to predict the collateral effects resulting from an attack on a facility containing hazardous materials is crucial to conducting effective military operations. Our study approach utilized a combination of field measurements with dispersion modeling to better understand which variables in terrain and weather were most important to collateral damage predictions. To develop the PAAS wind-sensing technology, we utilized a combination of emergent and available technology from micro-Doppler and highly coherent laser systems. The method used for wind sensing is to probe the atmosphere with a highly coherent laser beam. As the beam probes, light is back-scattered from particles entrained in the air to the lidar transceiver and detected by the instrument. Any motion of the aerosols with a component along the beam axis leads to a Doppler shift of the received light. Scanning in a conical fashion about the zenith results in a more accurate and two-dimensional measurement of the wind velocity. The major milestones in the benchtop system development were to verify the design by demonstrating the technique in the laboratory, then scale the design down to a size consistent with a demonstrator unit which could be built to take data in the field. The micro-Doppler heterodyne system we developed determines absolute motion by optically mixing a reference beam with the return signal and has shown motion sensitivity to better than 1 cm/s. This report describes the rationale, technical approach and laboratory testing undertaken to demonstrate the feasibility and utility of a system to provide local meteorological data and predict atmospheric particulate motion. The work described herein was funded by the Laboratory Science and Technology Office as a part of the 1996 Laboratory Directed Research and Development Program at Lawrence Livermore National Laboratory.

  10. Current state of atmospheric fluidized-bed combustion technology

    SciTech Connect (OSTI)

    Not Available

    1989-01-01

    This paper examines atmospheric fluidized-bed combustion (AFBC) technology, a coal burning method that has several environmental and technical advantages over the more conventional technologies, such as pulverized-coal methods. The AFBC approach injects an air stream into a boiler in such a way that it mixes with solid fuel and sorbent to create a dense phase region or fluidized bed. This method makes it possible to use a much wider range of low-quality fuels and to burn them at lower temperatures with less pollutant by-product. The paper presents a comprehensive overview of AFBC technology to date. It includes worldwide development of this technology since the 1950s necessary to meet ever-stricter emissions requirements while providing greater fuel flexibility.

  11. Regional forecasting with global atmospheric models; Third year report

    SciTech Connect (OSTI)

    Crowley, T.J.; North, G.R.; Smith, N.R.

    1994-05-01

    This report was prepared by the Applied Research Corporation (ARC), College Station, Texas, under subcontract to Pacific Northwest Laboratory (PNL) as part of a global climate studies task. The task supports site characterization work required for the selection of a potential high-level nuclear waste repository and is part of the Performance Assessment Scientific Support (PASS) Program at PNL. The work is under the overall direction of the Office of Civilian Radioactive Waste Management (OCRWM), US Department of Energy Headquarters, Washington, DC. The scope of the report is to present the results of the third year`s work on the atmospheric modeling part of the global climate studies task. The development testing of computer models and initial results are discussed. The appendices contain several studies that provide supporting information and guidance to the modeling work and further details on computer model development. Complete documentation of the models, including user information, will be prepared under separate reports and manuals.

  12. A Doppler lidar for measuring winds in the middle atmosphere

    SciTech Connect (OSTI)

    Chanin, M.L.; Garnier, A.; Hauchecorne, A.; Porteneuve, J. )

    1989-11-01

    The possibility of measuring winds in the middle atmosphere with a Doppler lidar has just been demonstrated. It is aimed at studying the wave-mean flow interaction, when used is association with the Rayleigh lidar providing density and temperature profiles and their fluctuations. The new Doppler lidar relies on the Rayleigh scattering from air molecules is designed to cover the height range 25-60 km, a region where radars cannot operate. The Doppler shift to the backscattered echo is measured by inter-comparing the signal detected through each of the two high-resolution, narrow band-pass Fabry-Perot interferometers tuned on either side of the emitted laser line.

  13. Doppler lidar for measurement of atmospheric wind fields

    SciTech Connect (OSTI)

    Menzies, R.T. )

    1991-01-01

    Measurements of wind fields in the earth's troposphere with daily global coverage is widely considered as a significant advance for forecasting and transport studies. For optimal use by NWP (Numerical Weather Prediction) models the horizontal and vertical resolutions should be approximately 100 km and 1 km, respectively. For boundary layer studies vertical resolution of a few hundred meters seems essential. Earth-orbiting Doppler lidar has a unique capability to measure global winds in the troposphere with the high vertical resolution required. The lidar approach depends on transmission of pulses with high spectral purity and backscattering from the atmospheric aerosol particles or layered clouds to provide a return signal. Recent field measurement campaigns using NASA research aircraft have resulted in collection of aerosol and cloud data which can be used to optimize the Doppler lidar instrument design and measurement strategy. 5 refs.

  14. Method of reducing chlorofluorocarbon refrigerant emissons to the atmosphere

    DOE Patents [OSTI]

    DeVault, Robert C. (Knoxville, TN); Fairchild, Phillip D. (Clinton, TN); Biermann, Wendell J. (Fayetteville, NY)

    1990-01-01

    A method is disclosed for reducing chloroflurocarbon (CFC) refrigerant emissions during removal or transfer or refrigerants from a vapor compression cooling system or heat pump which comprises contacting the refrigerant with a suitable sorbent material. The sorbent material allows for the storage and retention or the chlorofluorocarbon in non-gaseous form so that it does not tend to escape to the atmosphere where it would cause harm by contributing to ozone depletion. In other aspects of the invention, contacting of CFC refrigerants with sorbent material allows for purification and recycling of used refrigerant, and a device containing stored sorbent material can be employed in the detection of refrigerant leakage in a cooling system or heat pump.

  15. ATOMIC CARBON IN THE UPPER ATMOSPHERE OF TITAN

    SciTech Connect (OSTI)

    Zhang, X.; Yung, Y. L.; Ajello, J. M.

    2010-01-01

    The atomic carbon emission C I line feature at 1657 A ({sup 3} P {sup 0} {sub J}-{sup 3} P{sub J} ) in the upper atmosphere of Titan is first identified from the airglow spectra obtained by the Cassini Ultra-violet Imaging Spectrograph. A one-dimensional photochemical model of Titan is used to study the photochemistry of atomic carbon on Titan. Reaction between CH and atomic hydrogen is the major source of atomic carbon, and reactions with hydrocarbons (C{sub 2}H{sub 2} and C{sub 2}H{sub 4}) are the most important loss processes. Resonance scattering of sunlight by atomic carbon is the dominant emission mechanism. The emission intensity calculations based on model results show good agreement with the observations.

  16. Collision--induced absorption in dense atmospheres of cool stars

    SciTech Connect (OSTI)

    Borysow, Aleksandra; Joergensen, Uffe Graae

    1999-04-01

    In the atmosphere of the Sun the major interaction between the matter and the radiation is through light absorption by ions (predominantly the negative ion of hydrogen atoms), neutral atoms and a small amount of polar molecules. The majority of stars in the universe are, however, cooler and denser than our Sun, and for a large fraction of these, the above absorption processes are very weak. Here, collision-induced absorption (CIA) becomes the dominant opacity source. The radiation is absorbed during very short mutual passages ('collisions') of two non-polar molecules (and/or atoms), while their electric charge distributions are temporarily distorted which gives rise to a transient dipole moment. We present here a review of the present-day knowledge about the impact of collision-induced absorption processes on the structure and the spectrum of such stars.

  17. A General Investigation of Optimized Atmospheric Sample Duration

    SciTech Connect (OSTI)

    Eslinger, Paul W.; Miley, Harry S.

    2012-11-28

    ABSTRACT The International Monitoring System (IMS) consists of up to 80 aerosol and xenon monitoring systems spaced around the world that have collection systems sensitive enough to detect nuclear releases from underground nuclear tests at great distances (CTBT 1996; CTBTO 2011). Although a few of the IMS radionuclide stations are closer together than 1,000 km (such as the stations in Kuwait and Iran), many of them are 2,000 km or more apart. In the absence of a scientific basis for optimizing the duration of atmospheric sampling, historically scientists used a integration times from 24 hours to 14 days for radionuclides (Thomas et al. 1977). This was entirely adequate in the past because the sources of signals were far away and large, meaning that they were smeared over many days by the time they had travelled 10,000 km. The Fukushima event pointed out the unacceptable delay time (72 hours) between the start of sample acquisition and final data being shipped. A scientific basis for selecting a sample duration time is needed. This report considers plume migration of a nondecaying tracer using archived atmospheric data for 2011 in the HYSPLIT (Draxler and Hess 1998; HYSPLIT 2011) transport model. We present two related results: the temporal duration of the majority of the plume as a function of distance and the behavior of the maximum plume concentration as a function of sample collection duration and distance. The modeled plume behavior can then be combined with external information about sampler design to optimize sample durations in a sampling network.

  18. Atmospheric Inverse Estimates of Methane Emissions from Central California

    SciTech Connect (OSTI)

    Zhao, Chuanfeng; Andrews, Arlyn E.; Bianco, Laura; Eluszkiewicz, Janusz; Hirsch, Adam; MacDonald, Clinton; Nehrkorn, Thomas; Fischer, Marc L.

    2008-11-21

    Methane mixing ratios measured at a tall-tower are compared to model predictions to estimate surface emissions of CH{sub 4} in Central California for October-December 2007 using an inverse technique. Predicted CH{sub 4} mixing ratios are calculated based on spatially resolved a priori CH{sub 4} emissions and simulated atmospheric trajectories. The atmospheric trajectories, along with surface footprints, are computed using the Weather Research and Forecast (WRF) coupled to the Stochastic Time-Inverted Lagrangian Transport (STILT) model. An uncertainty analysis is performed to provide quantitative uncertainties in estimated CH{sub 4} emissions. Three inverse model estimates of CH{sub 4} emissions are reported. First, linear regressions of modeled and measured CH{sub 4} mixing ratios obtain slopes of 0.73 {+-} 0.11 and 1.09 {+-} 0.14 using California specific and Edgar 3.2 emission maps respectively, suggesting that actual CH{sub 4} emissions were about 37 {+-} 21% higher than California specific inventory estimates. Second, a Bayesian 'source' analysis suggests that livestock emissions are 63 {+-} 22% higher than the a priori estimates. Third, a Bayesian 'region' analysis is carried out for CH{sub 4} emissions from 13 sub-regions, which shows that inventory CH{sub 4} emissions from the Central Valley are underestimated and uncertainties in CH{sub 4} emissions are reduced for sub-regions near the tower site, yielding best estimates of flux from those regions consistent with 'source' analysis results. The uncertainty reductions for regions near the tower indicate that a regional network of measurements will be necessary to provide accurate estimates of surface CH{sub 4} emissions for multiple regions.

  19. Improved Meteorological Input for Atmospheric Release Decision support Systems and an Integrated LES Modeling System for Atmospheric Dispersion of Toxic Agents: Homeland Security Applications

    SciTech Connect (OSTI)

    Arnold, E; Simpson, M; Larsen, S; Gash, J; Aluzzi, F; Lundquist, J; Sugiyama, G

    2010-04-26

    When hazardous material is accidently or intentionally released into the atmosphere, emergency response organizations look to decision support systems (DSSs) to translate contaminant information provided by atmospheric models into effective decisions to protect the public and emergency responders and to mitigate subsequent consequences. The Department of Homeland Security (DHS)-led Interagency Modeling and Atmospheric Assessment Center (IMAAC) is one of the primary DSSs utilized by emergency management organizations. IMAAC is responsible for providing 'a single piont for the coordination and dissemination of Federal dispersion modeling and hazard prediction products that represent the Federal position' during actual or potential incidents under the National Response Plan. The Department of Energy's (DOE) National Atmospheric Release Advisory Center (NARAC), locatec at the Lawrence Livermore National Laboratory (LLNL), serves as the primary operations center of the IMAAC. A key component of atmospheric release decision support systems is meteorological information - models and data of winds, turbulence, and other atmospheric boundary-layer parameters. The accuracy of contaminant predictions is strongly dependent on the quality of this information. Therefore, the effectiveness of DSSs can be enhanced by improving the meteorological options available to drive atmospheric transport and fate models. The overall goal of this project was to develop and evaluate new meteorological modeling capabilities for DSSs based on the use of NASA Earth-science data sets in order to enhance the atmospheric-hazard information provided to emergency managers and responders. The final report describes the LLNL contributions to this multi-institutional effort. LLNL developed an approach to utilize NCAR meteorological predictions using NASA MODIS data for the New York City (NYC) region and demonstrated the potential impact of the use of different data sources and data parameterizations on IMAAC/NARAC fate and transport predictions. A case study involving coastal sea breeze circulation patterns in the NYC region was used to investigate the sensitivity of atmospheric dispersion results on the source of three-dimensional wind field data.

  20. Radon Measurements of Atmospheric Mixing (RAMIX) 2006-2014 Final Campaign

    Office of Scientific and Technical Information (OSTI)

    Summary (Program Document) | SciTech Connect Radon Measurements of Atmospheric Mixing (RAMIX) 2006-2014 Final Campaign Summary Citation Details In-Document Search Title: Radon Measurements of Atmospheric Mixing (RAMIX) 2006-2014 Final Campaign Summary Uncertainty in vertical mixing between the surface layer, boundary layer, and free troposphere leads to large uncertainty in "top-down" estimates of regional land-atmosphere carbon exchange (i.e., estimates based on measurements of

  1. Radon Measurements of Atmospheric Mixing (RAMIX) 2006-2014 Final Campaign

    Office of Scientific and Technical Information (OSTI)

    Summary (Program Document) | SciTech Connect Radon Measurements of Atmospheric Mixing (RAMIX) 2006-2014 Final Campaign Summary Citation Details In-Document Search Title: Radon Measurements of Atmospheric Mixing (RAMIX) 2006-2014 Final Campaign Summary Uncertainty in vertical mixing between the surface layer, boundary layer, and free troposphere leads to large uncertainty in "top-down" estimates of regional land-atmosphere carbon exchange (i.e., estimates based on measurements of

  2. NSRD-2015-TD01, Technical Report for Calculations of Atmospheric Dispersion

    Office of Environmental Management (EM)

    at Onsite Locations for DOE Nuclear Facilities | Department of Energy NSRD-2015-TD01, Technical Report for Calculations of Atmospheric Dispersion at Onsite Locations for DOE Nuclear Facilities NSRD-2015-TD01, Technical Report for Calculations of Atmospheric Dispersion at Onsite Locations for DOE Nuclear Facilities The Department of Energy (DOE) has performed an evaluation of the technical bases for the default value for the atmospheric dispersion parameter χ/Q. This parameter appears in the

  3. Atmospheric Radiation Measurement (ARM) Data from Niamey, Niger for the Radiative Atmospheric Divergence using AMF, GERB and AMMA Stations (RADAGAST)

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    The Atmospheric Radiation Measurement (ARM) Program is the largest global change research program supported by the U.S. Department of Energy. The primary goal of the ARM Program is to improve the treatment of cloud and radiation physics in global climate models in order to improve the climate simulation capabilities of these models. To achieve this goal, ARM scientists and researchers around the world use continuous data obtained through the ARM Climate Research Facility. The ARM Mobile Facility (AMF) operates at non-permanent sites selected by the ARM Program. Sometimes these sites can become permanent ARM sites, as was the case with Graciosa Island in the Azores. It is now known as the Eastern North Atlantic permanent site. In January 2006 the AMF deployed to Niamey, Niger, West Africa, at the Niger Meteorological Office at Niamey International Airport. This deployment was timed to coincide with the field phases and Special Observing Periods of the African Monsoon Multidisciplinary Analysis (AMMA). The ARM Program participated in this international effort as a field campaign called "Radiative Divergence using AMF, GERB and AMMA Stations (RADAGAST).The primary purpose of the Niger deployment was to combine an extended series of measurements from the AMF with those from the Geostationary Earth Radiation Budget (GERB) Instrument on the Meteosat operational geostationary satellite in order to provide the first well-sampled, direct estimates of the divergence of solar and thermal radiation across the atmosphere. A large collection of data plots based on data streams from specific instruments used at Niamey are available via a link from ARM's Niamey, Niger site information page. Other data can be found at the related websites mentioned above and in the ARM Archive. Users will be requested to create a password, but the plots and data files are free for viewing and downloading. The ARM Archive physically resides at the Oak Ridge National Laboratory.

  4. Multi-scale Atmospheric Modeling of Green House Gas Dispersion in Complex Terrain. Controlled Release Study

    SciTech Connect (OSTI)

    Costigan, Keeley Rochelle; Sauer, Jeremy A.; Dubey, Manvendra Krishna

    2015-07-10

    This report discusses the ghgas IC project which when applied, allows for an evaluation of LANL's HIGRAD model which can be used to create atmospheric simulations.

  5. Clouds and Chemistry in the Atmosphere of Extrasolar Planet HR8799b...

    Office of Scientific and Technical Information (OSTI)

    taken across the H and K bands. These data are combined with previously published photometry for an analysis of the planet's atmospheric properties. Thick photospheric dust...

  6. Latitudinal survey of middle atmospheric water vapor revealed by shipboard microwave spectroscopy. Master's thesis

    SciTech Connect (OSTI)

    Schrader, M.L.

    1994-05-01

    Water vapor is one of the most important greenhouse gases and is an important tracer of atmospheric motions in the middle atmosphere. It also plays an important role in the chemistry of the middle atmosphere and through its photodissociation by solar radiation, it is the major source of hydrogen escaping to space. Ground-based microwave measurements conducted in the 1980s have provided a fair understanding of the seasonal variation of mesospheric water vapor in the northern hemisphere mid-latitudes, but the global distribution of water vapor in the middle atmosphere is only beginning to be revealed by space-based measurements.

  7. Atmospheric circulation of eccentric hot Jupiter HAT-P-2B

    SciTech Connect (OSTI)

    Lewis, Nikole K.; Showman, Adam P.; Fortney, Jonathan J.; Knutson, Heather A.; Marley, Mark S.

    2014-11-10

    The hot Jupiter HAT-P-2b has become a prime target for Spitzer Space Telescope observations aimed at understanding the atmospheric response of exoplanets on highly eccentric orbits. Here we present a suite of three-dimensional atmospheric circulation models for HAT-P-2b that investigate the effects of assumed atmospheric composition and rotation rate on global scale winds and thermal patterns. We compare and contrast atmospheric models for HAT-P-2b, which assume one and five times solar metallicity, both with and without TiO/VO as atmospheric constituents. Additionally we compare models that assume a rotation period of half, one, and two times the nominal pseudo-synchronous rotation period. We find that changes in assumed atmospheric metallicity and rotation rate do not significantly affect model predictions of the planetary flux as a function of orbital phase. However, models in which TiO/VO are present in the atmosphere develop a transient temperature inversion between the transit and secondary eclipse events that results in significant variations in the timing and magnitude of the peak of the planetary flux compared with models in which TiO/VO are omitted from the opacity tables. We find that no one single atmospheric model can reproduce the recently observed full orbit phase curves at 3.6, 4.5 and 8.0 ?m, which is likely due to a chemical process not captured by our current atmospheric models for HAT-P-2b. Further modeling and observational efforts focused on understanding the chemistry of HAT-P-2b's atmosphere are needed and could provide key insights into the interplay between radiative, dynamical, and chemical processes in a wide range of exoplanet atmospheres.

  8. Energy considerations in the Community Atmosphere Model (CAM)

    SciTech Connect (OSTI)

    Williamson, David L.; Olson, Jerry G.; Hannay, Cécile; Toniazzo, Thomas; Yudin, Valery; Taylor, Mark

    2015-06-30

    An error in the energy formulation in the Community Atmosphere Model (CAM) is identified and corrected. Ten year AMIP simulations are compared using the correct and incorrect energy formulations. Statistics of selected primary variables all indicate physically insignificant differences between the simulations, comparable to differences with simulations initialized with rounding sized perturbations. The two simulations are so similar mainly because of an inconsistency in the application of the incorrect energy formulation in the original CAM. CAM used the erroneous energy form to determine the states passed between the parameterizations, but used a form related to the correct formulation for the state passed from the parameterizations to the dynamical core. If the incorrect form is also used to determine the state passed to the dynamical core the simulations are significantly different. In addition, CAM uses the incorrect form for the global energy fixer, but that seems to be less important. The difference of the magnitude of the fixers using the correct and incorrect energy definitions is very small.

  9. Energy considerations in the Community Atmosphere Model (CAM)

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Williamson, David L.; Olson, Jerry G.; Hannay, Cécile; Toniazzo, Thomas; Yudin, Valery; Taylor, Mark

    2015-06-30

    An error in the energy formulation in the Community Atmosphere Model (CAM) is identified and corrected. Ten year AMIP simulations are compared using the correct and incorrect energy formulations. Statistics of selected primary variables all indicate physically insignificant differences between the simulations, comparable to differences with simulations initialized with rounding sized perturbations. The two simulations are so similar mainly because of an inconsistency in the application of the incorrect energy formulation in the original CAM. CAM used the erroneous energy form to determine the states passed between the parameterizations, but used a form related to the correct formulation for themore » state passed from the parameterizations to the dynamical core. If the incorrect form is also used to determine the state passed to the dynamical core the simulations are significantly different. In addition, CAM uses the incorrect form for the global energy fixer, but that seems to be less important. The difference of the magnitude of the fixers using the correct and incorrect energy definitions is very small.« less

  10. The charge ratio of the atmospheric muons at low energy

    SciTech Connect (OSTI)

    Bahmanabadi, M.; Samimi, J.; Sheidaei, F.; Ghomi, M. Khakian

    2006-10-15

    From the nature of the muon production processes, it can be seen that the ratio of positive to negative cosmic muons has important information in both 'the atmospheric neutrino problem', and 'the hadronic interactions'. We have carried out an experiment for the measurement of the muon charge ratio in the cosmic ray flux in momentum range 0.112-0.178 GeV/c. The muon charge ratio is found to be 1.21{+-}0.01 with a mean zenith angle of 32 deg. {+-}5 deg. . From the measurements it has been obtained a zenithal angle distribution of muons as I({theta})=I(0)cos{sup n}{theta} with n=1.95{+-}0.13. An asymmetry has been observed in East-West directions because of the geomagnetic field. Meanwhile, in about the same momentum range, positive and negative muons have been studied on the basis of Monte Carlo simulations of the extensive air shower developement (Cosmic Ray Simulations for Kascade), using the Quark Gluon String model with JETs model as generator.

  11. Atmospheric escape by magnetically driven wind from gaseous planets

    SciTech Connect (OSTI)

    Tanaka, Yuki A.; Suzuki, Takeru K.; Inutsuka, Shu-ichiro

    2014-09-01

    We calculate the mass loss driven by magnetohydrodynamic (MHD) waves from hot Jupiters by using MHD simulations in one-dimensional flux tubes. If a gaseous planet has a magnetic field, MHD waves are excited by turbulence at the surface, dissipate in the upper atmosphere, and drive gas outflows. Our calculation shows that mass-loss rates are comparable to the observed mass-loss rates of hot Jupiters; therefore, it is suggested that gas flow driven by MHD waves can play an important role in the mass loss from gaseous planets. The mass-loss rate varies dramatically with the radius and mass of a planet: a gaseous planet with a small mass but an inflated radius produces a very large mass-loss rate. We also derive an analytical expression for the dependence of mass-loss rate on planet radius and mass that is in good agreement with the numerical calculation. The mass-loss rate also depends on the amplitude of the velocity dispersion at the surface of a planet. Thus, we expect to infer the condition of the surface and the internal structure of a gaseous planet from future observations of mass-loss rate from various exoplanets.

  12. Atmospheric radiation measurement unmanned aerospace vehicle (ARM-UAV) program

    SciTech Connect (OSTI)

    Bolton, W.R.

    1996-11-01

    ARM-UAV is part of the multi-agency U.S. Global Change Research Program and is addressing the largest source of uncertainty in predicting climatic response: the interaction of clouds and the sun`s energy in the Earth`s atmosphere. An important aspect of the program is the use of unmanned aerospace vehicles (UAVs) as the primary airborne platform. The ARM-UAV Program has completed two major flight series: The first series conducted in April, 1994, using an existing UAV (the General Atomics Gnat 750) consisted of eight highly successful flights at the DOE climate site in Oklahoma. The second series conducted in September/October, 1995, using two piloted aircraft (Egrett and Twin Otter), featured simultaneous measurements above and below clouds and in clear sky. Additional flight series are planned to continue study of the cloudy and clear sky energy budget in the Spring and Fall of 1996 over the DOE climate site in Oklahoma. 3 refs., 4 figs., 1 tab.

  13. Atmospheric Radiation Measurement Climate Research Facility (ACRF) Annual Report 2007

    SciTech Connect (OSTI)

    LR Roeder

    2007-12-01

    This annual report describes the purpose and structure of the program, and presents key accomplishments in 2007. Notable achievements include: Successful review of the ACRF as a user facility by the DOE Biological and Environmental Research Advisory Committee. The subcommittee reinforced the importance of the scientific impacts of this facility, and its value for the international research community. Leadership of the Cloud Land Surface Interaction Campaign. This multi-agency, interdisciplinary field campaign involved enhanced surface instrumentation at the ACRF Southern Great Plains site and, in concert with the Cumulus Humilis Aerosol Processing Study sponsored by the DOE Atmospheric Science Program, coordination of nine aircraft through the ARM Aerial Vehicles Program. Successful deployment of the ARM Mobile Facility in Germany, including hosting nearly a dozen guest instruments and drawing almost 5000 visitors to the site. Key advancements in the representation of radiative transfer in weather forecast models from the European Centre for Medium-Range Weather Forecasts. Development of several new enhanced data sets, ranging from best estimate surface radiation measurements from multiple sensors at all ACRF sites to the extension of time-height cloud occurrence profiles to Niamey, Niger, Africa. Publication of three research papers in a single issue (February 2007) of the Bulletin of the American Meteorological Society.

  14. Atmospheric Radiation Measurement (ARM) Data from the ARM Aerial Facility

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    The Atmospheric Radiation Measurement (ARM) Program is the largest global change research program supported by the U.S. Department of Energy. The primary goal of the ARM Program is to improve the treatment of cloud and radiation physics in global climate models in order to improve the climate simulation capabilities of these models. ARM data is collected both through permanent monitoring stations and field campaigns around the world. Airborne measurements required to answer science questions from researchers or to validate ground data are also collected. To find data from all categories of aerial operations, follow the links from the AAF information page at http://www.arm.gov/sites/aaf. Tables of information will provide start dates, duration, lead scientist, and the research site for each of the named campaigns. The title of a campaign leads, in turn, to a project description, contact information, and links to the data. Users will be requested to create a password, but the data files are free for viewing and downloading. The ARM Archive physically resides at the Oak Ridge National Laboratory.

  15. ENERGY CONTENT AND PROPAGATION IN TRANSVERSE SOLAR ATMOSPHERIC WAVES

    SciTech Connect (OSTI)

    Goossens, M.; Van Doorsselaere, T.; Soler, R.; Verth, G.

    2013-05-10

    Recently, a significant amount of transverse wave energy has been estimated propagating along solar atmospheric magnetic fields. However, these estimates have been made with the classic bulk Alfven wave model which assumes a homogeneous plasma. In this paper, the kinetic, magnetic, and total energy densities and the flux of energy are computed for transverse MHD waves in one-dimensional cylindrical flux tube models with a piecewise constant or continuous radial density profile. There are fundamental deviations from the properties for classic bulk Alfven waves. (1) There is no local equipartition between kinetic and magnetic energy. (2) The flux of energy and the velocity of energy transfer have, in addition to a component parallel to the magnetic field, components in the planes normal to the magnetic field. (3) The energy densities and the flux of energy vary spatially, contrary to the case of classic bulk Alfven waves. This last property has the important consequence that the energy flux computed with the well known expression for bulk Alfven waves could overestimate the real flux by a factor in the range 10-50, depending on the flux tube equilibrium properties.

  16. Atmospheric System Research (ASR) Program | U.S. DOE Office of Science (SC)

    Office of Science (SC) Website

    Atmospheric System Research (ASR) Program Biological and Environmental Research (BER) BER Home About Research Biological Systems Science Division (BSSD) Climate and Environmental Sciences Division (CESD) ARM Climate Research Facility Atmospheric System Research (ASR) Program Data Management Earth System Modeling (ESM) Program William R. Wiley Environmental Molecular Sciences Laboratory (EMSL) Integrated Assessment of Global Climate Change Regional & Global Climate Modeling (RGCM) Program

  17. Atmospheric-Pressure Chemical Vapor Deposition of Iron Pyrite...

    Office of Scientific and Technical Information (OSTI)

    FeSsub 2) is a promising candidate absorber material for earth-abundant thin-film solar cells. In this report, single-phase, large-grain, and uniform polycrystalline pyrite...

  18. A comparison between characteristics of atmospheric-pressure...

    Office of Scientific and Technical Information (OSTI)

    Authors: Zhang, Cheng ; Shao, Tao, E-mail: st@mail.iee.ac.cn ; Wang, Ruixue ; Yan, Ping 1 ; Key Laboratory of Power Electronics and Electric Drive, Chinese Academy of Sciences, ...

  19. Characterization of an atmospheric double arc argon-nitrogen plasma source

    SciTech Connect (OSTI)

    Tu, X.; Cheron, B. G.; Yan, J. H.; Yu, L.; Cen, K. F.

    2008-05-15

    In the framework of studies devoted to hazardous waste destruction, an original dc double anode plasma torch has been designed and tested, which produces an elongated, weak fluctuation and reproducible plasma jet at atmospheric pressure. The arc instabilities and dynamic behavior of the double arc argon-nitrogen plasma jet are investigated through the oscillations of electrical signals by combined means of fast Fourier transform and Wigner distribution. In our experiment, the restrike mode is identified as the typical fluctuation behavior in an argon-nitrogen plasma jet. The Fourier spectra and Wigner distributions exhibit two characteristic frequencies of 150 Hz and 4.1 kHz, which reveals that the nature of fluctuations in the double arc argon-nitrogen plasma can be ascribed to the undulation of the power supply and both arc roots motion on the anode channels. In addition, the microscopic properties of the plasma jet inside and outside the arc chamber are investigated by means of optical emission spectroscopy, which yields excitation, electronic, rotational, and vibrational temperatures, as well as the electron number density. The results allow us to examine the validity criteria of a local thermodynamic equilibrium (LTE) state in the plasma arc. The measured electron densities are in good agreement with those calculated from the LTE model, which indicates that the atmospheric double arc argon-nitrogen plasma in the core region is close to the LTE state under our experimental conditions.

  20. Implications of 'peak oil' for atmospheric CO{sub 2} and climate - article no. GB3012

    SciTech Connect (OSTI)

    Kharecha, P.A.; Hansen, J.E.

    2008-08-15

    Unconstrained CO{sub 2} emission from fossil fuel burning has been the dominant cause of observed anthropogenic global warming. The amounts of 'proven' and potential fossil fuel reserves are uncertain and debated. Regardless of the true values, society has flexibility in the degree to which it chooses to exploit these reserves, especially unconventional fossil fuels and those located in extreme or pristine environments. If conventional oil production peaks within the next few decades, it may have a large effect on future atmospheric CO{sub 2} and climate change, depending upon subsequent energy choices. Assuming that proven oil and gas reserves do not greatly exceed estimates of the Energy Information Administration, and recent trends are toward lower estimates, we show that it is feasible to keep atmospheric CO{sub 2} from exceeding about 450 ppm by 2100, provided that emissions from coal, unconventional fossil fuels, and land use are constrained. Coal-fired power plants without sequestration must be phased out before midcentury to achieve this CO{sub 2} limit. It is also important to 'stretch' conventional oil reserves via energy conservation and efficiency, thus averting strong pressures to extract liquid fuels from coal or unconventional fossil fuels while clean technologies are being developed for the era 'beyond fossil fuels'. We argue that a rising price on carbon emissions is needed to discourage conversion of the vast fossil resources into usable reserves, and to keep CO{sub 2} beneath the 450 ppm ceiling.

  1. Atmospheric Neutrino Induced Muons in the MINOS Far Detector

    SciTech Connect (OSTI)

    Rahman, Dipu; /Minnesota U.

    2007-02-01

    The Main Injector Neutrino Oscillation Search (MINOS) is a long baseline neutrino oscillation experiment. The MINOS Far Detector, located in the Soudan Underground Laboratory in Soudan MN, has been collecting data since August 2003. The scope of this dissertation involves identifying the atmospheric neutrino induced muons that are created by the neutrinos interacting with the rock surrounding the detector cavern, performing a neutrino oscillation search by measuring the oscillation parameter values of {Delta}m{sub 23}{sup 2} and sin{sup 2} 2{theta}{sub 23}, and searching for CPT violation by measuring the charge ratio for the atmospheric neutrino induced muons. A series of selection cuts are applied to the data set in order to extract the neutrino induced muons. As a result, a total of 148 candidate events are selected. The oscillation search is performed by measuring the low to high muon momentum ratio in the data sample and comparing it to the same ratio in the Monte Carlo simulation in the absence of neutrino oscillation. The measured double ratios for the ''all events'' (A) and high resolution (HR) samples are R{sub A} = R{sub low/high}{sup data}/R{sub low/high}{sup MC} = 0.60{sub -0.10}{sup +0.11}(stat) {+-} 0.08(syst) and R{sub HR} = R{sub low/high}{sup data}/R{sub low/high}{sup MC} = 0.58{sub -0.11}{sup +0.14}(stat) {+-} 0.05(syst), respectively. Both event samples show a significant deviation from unity giving a strong indication of neutrino oscillation. A combined momentum and zenith angle oscillation fit is performed using the method of maximum log-likelihood with a grid search in the parameter space of {Delta}m{sup 2} and sin{sup 2} 2{theta}. The best fit point for both event samples occurs at {Delta}m{sub 23}{sup 2} = 1.3 x 10{sup -3} eV{sup 2}, and sin{sup 2} 2{theta}{sub 23} = 1. This result is compatible with previous measurements from the Super Kamiokande experiment and Soudan 2 experiments. The MINOS Far Detector is the first underground neutrino detector to be able to distinguish the charge of the muons. The measured charge is used to test the rate of the neutrino to the anti-neutrino oscillations by measuring the neutrino induced muon charge ratio. Using the high resolution sample, the {mu}{sup +} to {mu}{sup -} double charge ratio has been determined to be R{sub CPT} = R{sub {mu}{sup -}/{mu}{sup +}}{sup data}/R{sub {mu}{sup -}/{mu}{sup +}}{sup MC} = 0.90{sub -0.18}{sup +0.24}(stat) {+-} 0.09(syst). With the uncertainties added in quadrature, the CPT double ratio is consistent with unity showing no indication for CPT violation.

  2. Long Range Weather Prediction III: Miniaturized Distributed Sensors for Global Atmospheric Measurements

    SciTech Connect (OSTI)

    Teller, E; Leith, C; Canavan, G; Wood, L

    2001-11-13

    We continue consideration of ways-and-means for creating, in an evolutionary, ever-more-powerful manner, a continually-updated data-base of salient atmospheric properties sufficient for finite differenced integration-based, high-fidelity weather prediction over intervals of 2-3 weeks, leveraging the 10{sup 14} FLOPS digital computing systems now coming into existence. A constellation comprised of 10{sup 6}-10{sup 9} small atmospheric sampling systems--high-tech superpressure balloons carrying early 21st century semiconductor devices, drifting with the local winds over the meteorological spectrum of pressure-altitudes--that assays all portions of the troposphere and lower stratosphere remains the central feature of the proposed system. We suggest that these devices should be active-signaling, rather than passive-transponding, as we had previously proposed only for the ground- and aquatic-situated sensors of this system. Instead of periodic interrogation of the intra-atmospheric transponder population by a constellation of sophisticated small satellites in low Earth orbit, we now propose to retrieve information from the instrumented balloon constellation by existing satellite telephony systems, acting as cellular tower-nodes in a global cellular telephony system whose ''user-set'' is the atmospheric-sampling and surface-level monitoring constellations. We thereby leverage the huge investment in cellular (satellite) telephony and GPS technologies, with large technical and economic gains. This proposal minimizes sponsor forward commitment along its entire programmatic trajectory, and moreover may return data of weather-predictive value soon after field activities commence. We emphasize its high near-term value for making better mesoscale, relatively short-term weather predictions with computing-intensive means, and its great long-term utility in enhancing the meteorological basis for global change predictive studies. We again note that adverse impacts of weather involve continuing costs of the order of 1% of GDP, a large fraction of which could be retrieved if high-fidelity predictions of two weeks forward applicability were available. These {approx}$10{sup 2} B annual savings dwarf the <$1 B costs of operating a rational, long-range weather prediction system of the type proposed.

  3. Long Range Weather Prediction III: Miniaturized Distributed Sensors for Global Atmospheric Measurements

    DOE R&D Accomplishments [OSTI]

    Teller, E.; Leith, C.; Canavan, G.; Wood, L.

    2001-11-13

    We continue consideration of ways-and-means for creating, in an evolutionary, ever-more-powerful manner, a continually-updated data-base of salient atmospheric properties sufficient for finite differenced integration-based, high-fidelity weather prediction over intervals of 2-3 weeks, leveraging the 10{sup 14} FLOPS digital computing systems now coming into existence. A constellation comprised of 10{sup 6}-10{sup 9} small atmospheric sampling systems--high-tech superpressure balloons carrying early 21st century semiconductor devices, drifting with the local winds over the meteorological spectrum of pressure-altitudes--that assays all portions of the troposphere and lower stratosphere remains the central feature of the proposed system. We suggest that these devices should be active-signaling, rather than passive-transponding, as we had previously proposed only for the ground- and aquatic-situated sensors of this system. Instead of periodic interrogation of the intra-atmospheric transponder population by a constellation of sophisticated small satellites in low Earth orbit, we now propose to retrieve information from the instrumented balloon constellation by existing satellite telephony systems, acting as cellular tower-nodes in a global cellular telephony system whose ''user-set'' is the atmospheric-sampling and surface-level monitoring constellations. We thereby leverage the huge investment in cellular (satellite) telephony and GPS technologies, with large technical and economic gains. This proposal minimizes sponsor forward commitment along its entire programmatic trajectory, and moreover may return data of weather-predictive value soon after field activities commence. We emphasize its high near-term value for making better mesoscale, relatively short-term weather predictions with computing-intensive means, and its great long-term utility in enhancing the meteorological basis for global change predictive studies. We again note that adverse impacts of weather involve continuing costs of the order of 1% of GDP, a large fraction of which could be retrieved if high-fidelity predictions of two weeks forward applicability were available. These{approx}$10{sup 2} B annual savings dwarf the<$1 B costs of operating a rational, long-range weather prediction system of the type proposed.

  4. PHOTOCHEMISTRY IN TERRESTRIAL EXOPLANET ATMOSPHERES. I. PHOTOCHEMISTRY MODEL AND BENCHMARK CASES

    SciTech Connect (OSTI)

    Hu Renyu; Seager, Sara; Bains, William

    2012-12-20

    We present a comprehensive photochemistry model for exploration of the chemical composition of terrestrial exoplanet atmospheres. The photochemistry model is designed from the ground up to have the capacity to treat all types of terrestrial planet atmospheres, ranging from oxidizing through reducing, which makes the code suitable for applications for the wide range of anticipated terrestrial exoplanet compositions. The one-dimensional chemical transport model treats up to 800 chemical reactions, photochemical processes, dry and wet deposition, surface emission, and thermal escape of O, H, C, N, and S bearing species, as well as formation and deposition of elemental sulfur and sulfuric acid aerosols. We validate the model by computing the atmospheric composition of current Earth and Mars and find agreement with observations of major trace gases in Earth's and Mars' atmospheres. We simulate several plausible atmospheric scenarios of terrestrial exoplanets and choose three benchmark cases for atmospheres from reducing to oxidizing. The most interesting finding is that atomic hydrogen is always a more abundant reactive radical than the hydroxyl radical in anoxic atmospheres. Whether atomic hydrogen is the most important removal path for a molecule of interest also depends on the relevant reaction rates. We also find that volcanic carbon compounds (i.e., CH{sub 4} and CO{sub 2}) are chemically long-lived and tend to be well mixed in both reducing and oxidizing atmospheres, and their dry deposition velocities to the surface control the atmospheric oxidation states. Furthermore, we revisit whether photochemically produced oxygen can cause false positives for detecting oxygenic photosynthesis, and find that in 1 bar CO{sub 2}-rich atmospheres oxygen and ozone may build up to levels that have conventionally been accepted as signatures of life, if there is no surface emission of reducing gases. The atmospheric scenarios presented in this paper can serve as the benchmark atmospheres for quickly assessing the lifetime of trace gases in reducing, weakly oxidizing, and highly oxidizing atmospheres on terrestrial exoplanets for the exploration of possible biosignature gases.

  5. Precision laser surveying instrument using atmospheric turbulence compensation by determining the absolute displacement between two laser beam components

    DOE Patents [OSTI]

    Veligdan, James T. (Manorville, NY)

    1993-01-01

    Atmospheric effects on sighting measurements are compensated for by adjusting any sighting measurements using a correction factor that does not depend on atmospheric state conditions such as temperature, pressure, density or turbulence. The correction factor is accurately determined using a precisely measured physical separation between two color components of a light beam (or beams) that has been generated using either a two-color laser or two lasers that project different colored beams. The physical separation is precisely measured by fixing the position of a short beam pulse and measuring the physical separation between the two fixed-in-position components of the beam. This precisely measured physical separation is then used in a relationship that includes the indexes of refraction for each of the two colors of the laser beam in the atmosphere through which the beam is projected, thereby to determine the absolute displacement of one wavelength component of the laser beam from a straight line of sight for that projected component of the beam. This absolute displacement is useful to correct optical measurements, such as those developed in surveying measurements that are made in a test area that includes the same dispersion effects of the atmosphere on the optical measurements. The means and method of the invention are suitable for use with either single-ended systems or a double-ended systems.

  6. Computational studies for plasma filamentation by magnetic field in atmospheric microwave discharge

    SciTech Connect (OSTI)

    Takahashi, Masayuki; Ohnishi, Naofumi

    2014-12-01

    Plasma filamentation is induced by an external magnetic field in an atmospheric discharge using intense microwaves. A discrete structure is obtained at low ambient pressure if a strong magnetic field of more than 1 T is applied, due to the suppression of electron diffusion, whereas a diffusive pattern is generated with no external field. Applying a magnetic field can slow the discharge front propagation due to magnetic confinement of the electron transport. If the resonance conditions are satisfied for electron cyclotron resonance and its higher harmonics, the propagation speed increases because the heated electrons easily ionize neutral particles. The streamer velocity and the pattern of the microwave plasma are positively controlled by adjusting two parameters—the electron diffusion coefficient and the ionization frequency—through the resonance process and magnetic confinement, and hot, dense filamentary plasma can be concentrated in a compact volume to reduce energy loss in a plasma device like a microwave rocket.

  7. A comprehensive study of different gases in inductively coupled plasma torch operating at one atmosphere

    SciTech Connect (OSTI)

    Punjabi, Sangeeta B.; Joshi, N. K.; Mangalvedekar, H. A.; Lande, B. K.; Das, A. K.; Kothari, D. C.

    2012-01-15

    A numerical study is done to understand the possible operating regimes of RF-ICP torch (3 MHz, 50 kW) using different gases for plasma formation at atmospheric pressure. A two dimensional numerical simulation of RF-ICP torch using argon, nitrogen, oxygen, and air as plasma gas has been investigated using computational fluid dynamic (CFD) software fluent{sup (c)}. The operating parameters varied here are central gas flow, sheath gas flow, RF-power dissipated in plasma, and plasma gas. The temperature contours, flow field, axial, and radial velocity profiles were investigated under different operating conditions. The plasma resistance, inductance of the torch, and the heat distribution for various plasma gases have also been investigated. The plasma impedance of ICP torch varies with different operating parameters and plays an important role for RF oscillator design and power coupling. These studies will be useful to decide the design criteria for ICP torches required for different material processing applications.

  8. Microwave plasma based single step method for free standing graphene synthesis at atmospheric conditions

    SciTech Connect (OSTI)

    Tatarova, E.; Henriques, J.; Dias, A.; Ferreira, C. M.; Luhrs, C. C.; Phillips, J.; Abrashev, M. V.

    2013-09-23

    Microwave atmospheric pressure plasmas driven by surface waves were used to synthesize graphene sheets from vaporized ethanol molecules carried through argon plasma. In the plasma, ethanol decomposes creating carbon atoms that form nanostructures in the outlet plasma stream, where external cooling/heating was applied. It was found that the outlet gas stream temperature plays an important role in the nucleation processes and the structural quality of the produced nanostructures. The synthesis of few layers (from one to five) graphene has been confirmed by high-resolution transmission electron microscopy. Raman spectral studies were conducted to determine the ratio of the 2D to G peaks (>2). Disorder D-peak to G-peak intensity ratio decreases when outlet gas stream temperature decreases.

  9. Functionalization of polymers using an atmospheric plasma jet in a fluidized bed reactor and the impact on SLM-processes

    SciTech Connect (OSTI)

    Sachs, M. Schmitt, A. Schmidt, J. Peukert, W. Wirth, K-E

    2014-05-15

    In order to improve thermoplastics (e.g. Polyamide, Polypropylene and Polyethylene) for Selective Laser Beam Melting (SLM) processes a new approach to functionalize temperature sensitive polymer powders in a large scale is investigated. This is achieved by combining an atmospheric pressure plasma jet and a fluidized bed reactor. Using pressurized air as the plasma gas, radicals like OH* are created. The functionalization leads to an increase of the hydrophilicity of the treated polymer powder without changing the bulk properties. Using the polymers in a SLM process to build single layers of melted material leads to an improvement of the melted layers.

  10. NDE to Manage Atmospheric SCC in Canisters for Dry Storage of Spent Fuel: An Assessment

    SciTech Connect (OSTI)

    Meyer, Ryan M.; Pardini, Allan F.; Cuta, Judith M.; Adkins, Harold E.; Casella, Andrew M.; Qiao, Hong; Larche, Michael R.; Diaz, Aaron A.; Doctor, Steven R.

    2013-09-01

    This report documents efforts to assess representative horizontal (Transuclear NUHOMS) and vertical (Holtec HI-STORM) storage systems for the implementation of non-destructive examination (NDE) methods or techniques to manage atmospheric stress corrosion cracking (SCC) in canisters for dry storage of used nuclear fuel. The assessment is conducted by assessing accessibility and deployment, environmental compatibility, and applicability of NDE methods. A recommendation of this assessment is to focus on bulk ultrasonic and eddy current techniques for direct canister monitoring of atmospheric SCC. This assessment also highlights canister regions that may be most vulnerable to atmospheric SCC to guide the use of bulk ultrasonic and eddy current examinations. An assessment of accessibility also identifies canister regions that are easiest and more difficult to access through the ventilation paths of the concrete shielding modules. A conceivable sampling strategy for canister inspections is to sample only the easiest to access portions of vulnerable regions. There are aspects to performing an NDE inspection of dry canister storage system (DCSS) canisters for atmospheric SCC that have not been addressed in previous performance studies. These aspects provide the basis for recommendations of future efforts to determine the capability and performance of eddy current and bulk ultrasonic examinations for atmospheric SCC in DCSS canisters. Finally, other important areas of investigation are identified including the development of instrumented surveillance specimens to identify when conditions are conducive for atmospheric SCC, characterization of atmospheric SCC morphology, and an assessment of air flow patterns over canister surfaces and their influence on chloride deposition.

  11. High resolution transmission spectroscopy as a diagnostic for Jovian exoplanet atmospheres: constraints from theoretical models

    SciTech Connect (OSTI)

    Kempton, Eliza M.-R.; Perna, Rosalba; Heng, Kevin

    2014-11-01

    We present high resolution transmission spectra of giant planet atmospheres from a coupled three-dimensional (3D) atmospheric dynamics and transmission spectrum model that includes Doppler shifts which arise from winds and planetary motion. We model Jovian planets covering more than two orders of magnitude in incident flux, corresponding to planets with 0.9-55 day orbital periods around solar-type stars. The results of our 3D dynamical models reveal certain aspects of high resolution transmission spectra that are not present in simple one-dimensional (1D) models. We find that the hottest planets experience strong substellar to anti-stellar (SSAS) winds, resulting in transmission spectra with net blueshifts of up to 3 km s{sup 1}, whereas less irradiated planets show almost no net Doppler shifts. We find only minor differences between transmission spectra for atmospheres with temperature inversions and those without. Compared to 1D models, peak line strengths are significantly reduced for the hottest atmospheres owing to Doppler broadening from a combination of rotation (which is faster for close-in planets under the assumption of tidal locking) and atmospheric winds. Finally, high resolution transmission spectra may be useful in studying the atmospheres of exoplanets with optically thick clouds since line cores for very strong transitions should remain optically thick to very high altitude. High resolution transmission spectra are an excellent observational test for the validity of 3D atmospheric dynamics models, because they provide a direct probe of wind structures and heat circulation. Ground-based exoplanet spectroscopy is currently on the verge of being able to verify some of our modeling predictions, most notably the dependence of SSAS winds on insolation. We caution that interpretation of high resolution transmission spectra based on 1D atmospheric models may be inadequate, as 3D atmospheric motions can produce a noticeable effect on the absorption signatures.

  12. External Merit Review for the Atmosphere to Electrons (A2e) Initiative |

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Department of Energy External Merit Review for the Atmosphere to Electrons (A2e) Initiative External Merit Review for the Atmosphere to Electrons (A2e) Initiative The Atmosphere to Electrons (A2e) Initiative within the U.S. Department of Energy's (DOE) Office of Energy Efficiency and Renewable Energy held an External Merit Review in Washington, DC, on February 4-5, 2014. The External Review Panel reviewed the current program planning and provided suggestions on the formulation of A2e

  13. A marine biogenic source of atmospheric ice-nucleating particles (Journal

    Office of Scientific and Technical Information (OSTI)

    Article) | SciTech Connect A marine biogenic source of atmospheric ice-nucleating particles Citation Details In-Document Search Title: A marine biogenic source of atmospheric ice-nucleating particles The formation of ice in clouds is facilitated by the presence of airborne ice nucleating particles1,2. Sea spray is one of the major global sources of atmospheric particles, but it is unclear to what extent these particles are capable of nucleating ice3-11. Here we show that material in the sea

  14. Submit a Public Comment on The Atmosphere to Electrons (A2e) External Merit

    Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

    Review Meeting Summary | Department of Energy Submit a Public Comment on The Atmosphere to Electrons (A2e) External Merit Review Meeting Summary Submit a Public Comment on The Atmosphere to Electrons (A2e) External Merit Review Meeting Summary March 5, 2014 - 9:01am Addthis The Atmosphere to Electrons (A2e) Initiative within the U.S. Department of Energy's (DOE) Office of Energy Efficiency and Renewable Energy is a multi-year DOE research initiative targeting significant reductions in the

  15. Radon Measurements of Atmospheric Mixing (RAMIX) 2006–2014 Final Campaign Summary

    SciTech Connect (OSTI)

    Fischer, ML; Biraud, SC; Hirsch, A

    2015-05-01

    Uncertainty in vertical mixing between the surface layer, boundary layer, and free troposphere leads to large uncertainty in “top-down” estimates of regional land-atmosphere carbon exchange (i.e., estimates based on measurements of atmospheric CO2 mixing ratios). The radioisotope radon-222 (222Rn) is a valuable tracer for measuring atmospheric mixing because it is emitted from the land surface and has a short enough half-life (3.8 days) to allow characterization of mixing processes based on vertical profile measurements.

  16. Radon Measurements of Atmospheric Mixing (RAMIX) 2006–2014 Final Campaign Summary

    SciTech Connect (OSTI)

    Fischer, ML; Biraud, SC

    2015-05-01

    Uncertainty in vertical mixing between the surface layer, boundary layer, and free troposphere leads to large uncertainty in “top-down” estimates of regional land-atmosphere carbon exchange (i.e., estimates based on measurements of atmospheric CO2 mixing ratios. Radon-222 (222Rn) is a valuable tracer for measuring atmospheric mixing because it is emitted from the land surface and has a short enough half-life (3.8 days) to allow characterization of mixing processes based on vertical profile measurements.

  17. An Evaluation of the Nonlinearity Correction Applied to Atmospheric Emitted Radiance Interferometer (AERI) Data Collected by the Atmospheric Radiation Measurement Program

    SciTech Connect (OSTI)

    Turner, DD; Revercomb, HE; Knuteson, RO; Dedecker, RG; Feltz, WF

    2004-09-01

    Mercury Cadmium Telluride (MCT) detectors provide excellent sensitivity to infrared radiation and are used in passive infrared remote sensors such as the Atmospheric Emitted Radiance Interferometer (AERI). However, MCT detectors have a nonlinear response and thus this nonlinearity must be characterized and corrected to provide accurate infrared radiance observations. This paper discusses the significance of the nonlinearity correction applied to AERI data and its impacts on the parameters retrieved from the AERI spectra. It also evaluates the accuracy of the scheme used to determine the nonlinearity of the MCT detectors used in the Atmospheric Radiation Measurement (ARM) Programs AERIs.

  18. Overview of the United States Department of Energy's ARM (Atmospheric Radiation Measurement) Program

    SciTech Connect (OSTI)

    Stokes, G.M. ); Tichler, J.L. )

    1990-06-01

    The Department of Energy (DOE) is initiating a major atmospheric research effort, the Atmospheric Radiation Measurement Program (ARM). The program is a key component of DOE's research strategy to address global climate change and is a direct continuation of DOE's decade-long effort to improve the ability of General Circulation Models (GCMs) to provide reliable simulations of regional, and long-term climate change in response to increasing greenhouse gases. The effort is multi-disciplinary and multi-agency, involving universities, private research organizations and more than a dozen government laboratories. The objective of the ARM Research is to provide an experimental testbed for the study of important atmospheric effects, particularly cloud and radiative processes, and to test parameterizations of these processes for use in atmospheric models. This effort will support the continued and rapid improvement of GCM predictive capability. 2 refs.

  19. Atmosphere to Electrons: Update on Strategic Plan for Wind Plant Reliability; NREL (National Renewable Energy Laboratory)

    SciTech Connect (OSTI)

    Keller, J.; Westergaard, C.

    2015-02-01

    An update on the Reliability focus area of the Atmosphere to Electrons (A2e) center is provided, including highlighted projects from each of the four major work packages.

  20. Boundary Layer The U.S. Department of Energy's Atmospheric Radiation

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    layer is the atmosphere between the Earth's surface and an altitude of about 1 to 2 kilometers. In a marine environment, boundary-layer clouds passively filter the sun, but also...

  1. An approach for verifying biogenic greenhouse gas emissions inventories with atmospheric CO 2 concentration data

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Ogle, Stephen; Davis, Kenneth J.; Lauvaux, Thomas; Schuh, Andrew E.; Cooley, Dan; West, Tristram O.; Heath, L.; Miles, Natasha; Richardson, S. J.; Breidt, F. Jay; et al

    2015-03-10

    Verifying national greenhouse gas (GHG) emissions inventories is a critical step to ensure that reported emissions data to the United Nations Framework Convention on Climate Change (UNFCCC) are accurate and representative of a country’s contribution to GHG concentrations in the atmosphere. Verification could include a variety of evidence, but arguably the most convincing verification would be confirmation of a change in GHG concentrations in the atmosphere that is consistent with reported emissions to the UNFCCC. We report here on a case study evaluating this option based on a prototype atmospheric CO2 measurement network deployed in the Mid-Continent Region of themore » conterminous United States. We found that the atmospheric CO2 measurement data did verify the accuracy of the emissions inventory within the confidence limits of the emissions estimates, suggesting that this technology could be further developed and deployed more widely in the future for verifying reported emissions.« less

  2. Unmanned Aerial Systems (UAS) Evaluation of Routine Atmospheric Sounding Measurements using Unmanned Systems (ERASMUS)

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    De Boer, Gijs

    2016-01-05

    Data were collected to improve understanding of the Arctic troposphere, and to provide researchers with a focused case-study period for future observational and modeling studies pertaining to Arctic atmospheric processes.

  3. Advanced Process Technology: Combi Materials Science and Atmospheric Processing (Fact Sheet)

    SciTech Connect (OSTI)

    Not Available

    2011-06-01

    Capabilities fact sheet for the National Center for Photovoltaics: Process Technology and Advanced Concepts -- High-Throughput Combi Material Science and Atmospheric Processing that includes scope, core competencies and capabilities, and contact/web information.

  4. The impact of atmospheric aerosols on trace metal chemistry in open ocean surface seawater 3. Lead

    SciTech Connect (OSTI)

    Maring, H.B.; Duce, R.A. )

    1990-04-15

    Atmospheric aerosols collected at Enewetak Atoll in the tropical North Pacific were exposed to seawater in laboratory experiments to assess the impact of atmospheric aerosols on lead chemistry in surface seawater. The net atmospheric flux of soluble lead to the ocean is between 16 and 32 pmol cm{sup {minus}2}/yr at Enewetak. The stable lead isotopic composition of soluble aerosol lead indicates that it is of anthropogenic origin. Anthropogenic aerosol lead from Central and North America appears to be less soluble and/or to dissolve less rapidly than that from Asia. Dissolved organic matter and possibly lower pH appear to increase the nonaluminosilicate aerosol lead solubility and/or dissolution rate. The isotopic composition of lead in air, seawater and dry deposition suggests that after deposition in the ocean, nonaluminosilicate particulate lead can be reinjected into the atmosphere during sea salt aerosol production.

  5. Atmospheric Radiation Measurement program climate research facility operations quarterly report.

    SciTech Connect (OSTI)

    Sisterson, D. L.; Decision and Information Sciences

    2006-09-06

    Individual raw data streams from instrumentation at the Atmospheric Radiation Measurement (ARM) Program Climate Research Facility (ACRF) fixed and mobile sites are collected and sent to the Data Management Facility (DMF) at Pacific Northwest National Laboratory (PNNL) for processing in near real time. Raw and processed data are then sent daily to the ACRF Archive, where they are made available to users. For each instrument, we calculate the ratio of the actual number of data records received daily at the Archive to the expected number of data records. The results are tabulated by (1) individual data stream, site, and month for the current year and (2) site and fiscal year dating back to 1998. The U.S. Department of Energy requires national user facilities to report time-based operating data. The requirements concern the actual hours of operation (ACTUAL); the estimated maximum operation or uptime goal (OPSMAX), which accounts for planned downtime; and the VARIANCE [1-(ACTUAL/OPSMAX)], which accounts for unplanned downtime. The OPSMAX time for the third quarter for the Southern Great Plains (SGP) site is 2,074.80 hours (0.95 x 2,184 hours this quarter). The OPSMAX for the North Slope Alaska (NSA) locale is 1,965.60 hours (0.90 x 2,184), and that for the Tropical Western Pacific (TWP) locale is 1,856.40 hours (0.85 x 2,184). The OPSMAX time for the ARM Mobile Facility (AMF) is 2,074.80 hours (0.95 x 2,184). The differences in OPSMAX performance reflect the complexity of local logistics and the frequency of extreme weather events. It is impractical to measure OPSMAX for each instrument or data stream. Data availability reported here refers to the average of the individual, continuous data streams that have been received by the Archive. Data not at the Archive are caused by downtime (scheduled or unplanned) of the individual instruments. Therefore, data availability is directly related to individual instrument uptime. Thus, the average percent of data in the Archive represents the average percent of the time (24 hours per day, 91 days for this quarter) the instruments were operating this quarter. Table 1 shows the accumulated maximum operation time (planned uptime), the actual hours of operation, and the variance (unplanned downtime) for the period April 1 through June 30, 2006, for the fixed and mobile sites. Although the AMF is currently up and running in Niamey, Niger, Africa, the AMF statistics are reported separately and not included in the aggregate average with the fixed sites. The third quarter comprises a total of 2,184 hours. For all fixed sites (especially the TWP locale) and the AMF, the actual data availability (and therefore actual hours of operation) exceeded the individual (and well as aggregate average of the fixed sites) operational goal for the third quarter of fiscal year (FY) 2006.

  6. Prediction of Ice Crystal Number in Community Atmospheric Model (CAM3.0)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Prediction of Ice Crystal Number in Community Atmospheric Model (CAM3.0) Liu, Xiaohong Pacific Northwest National Laboratory Ghan, Steven Pacific Northwest National Laboratory Wang, M University of Michigan Penner, Joyce University of Michigan Category: Modeling A prognostic equation of ice crystal number concentrations is implemented in the Community Atmospheric Model (CAM3.0) with the aim to study the aerosol effects on climate through changing the ice cloud properties. The microphysical

  7. Final Report. "Collaborative Project. Contributions of organic compounds to the growth of freshly nucleated atmospheric nanoparticles"

    SciTech Connect (OSTI)

    Smith, James N

    2015-12-23

    This is the final technical report for the portion of the project that took place at the National Center for Atmospheric Research, which covers approximately the first year of the three-year project. During this time we focused primarily on analysis and modeling of DOE-funded observations as well as preparation for laboratory studies of individual processes that contribute to atmospheric new particle formation.

  8. Modelled Black Carbon Radiative Forcing and Atmospheric Lifetime in AeroCom

    Office of Scientific and Technical Information (OSTI)

    Phase II Constrained by Aircraft Observations (Journal Article) | SciTech Connect Modelled Black Carbon Radiative Forcing and Atmospheric Lifetime in AeroCom Phase II Constrained by Aircraft Observations Citation Details In-Document Search Title: Modelled Black Carbon Radiative Forcing and Atmospheric Lifetime in AeroCom Phase II Constrained by Aircraft Observations Black carbon (BC) aerosols absorb solar radiation, and are generally held to exacerbate global warming through exerting a

  9. Multi-model Mean Nitrogen and Sulfur Deposition from the Atmospheric

    Office of Scientific and Technical Information (OSTI)

    Chemistry and Climate Model Intercomparison Project (ACCMIP): Evaluation of Historical and Projected Future Changes (Journal Article) | SciTech Connect Multi-model Mean Nitrogen and Sulfur Deposition from the Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP): Evaluation of Historical and Projected Future Changes Citation Details In-Document Search Title: Multi-model Mean Nitrogen and Sulfur Deposition from the Atmospheric Chemistry and Climate Model Intercomparison

  10. Improved atmosphere-ocean coupled modeling in the tropics for climate

    Office of Scientific and Technical Information (OSTI)

    prediction (Technical Report) | SciTech Connect Improved atmosphere-ocean coupled modeling in the tropics for climate prediction Citation Details In-Document Search Title: Improved atmosphere-ocean coupled modeling in the tropics for climate prediction We investigated the initial development of the double ITCZ in the Community Climate System Model (CCSM Version 3) in the central Pacific. Starting from a resting initial condition of the ocean in January, the model developed a warm bias of

  11. Atmospheric Rivers Coming to a Cloud Near You (Other) | SciTech Connect

    Office of Scientific and Technical Information (OSTI)

    Other: Atmospheric Rivers Coming to a Cloud Near You Citation Details In-Document Search Title: Atmospheric Rivers Coming to a Cloud Near You Learn about the ARM Cloud Aerosol Precipitation Experiment (ACAPEX) field campaign in this short video. Ruby Leung, PNNL's lead scientist on this campaign's observational strategy to monitor precipitation. Authors: Leung, Ruby Publication Date: 2014-03-29 OSTI Identifier: 1133941 Resource Type: Other Research Org: PNNL (Pacific Northwest National

  12. Determination of atmospheric carbonyl sulfide by isotope dilution gas chromatography/mass spectrometry

    SciTech Connect (OSTI)

    Lewin, E.E.; Taggart, R.L.; Lalevic, M.; Bandy, A.R.

    1987-05-01

    A gas chromatography/mass spectrometry (GB/MS) method for determining atmospheric carbonyl sulfide (OCS) with a precision better than 2% is reported. High precision and insensitivity to sample loss and changes in detector response were achieved by using isotopically labeled OCS as an internal standard. Tenax, Molecular Sieve 5A, Carbosieve B, and Carbosieve S were evaluated for collecting atmospheric OCS. Molecular Sieve 5A provided the best trapping and recovery efficiencies.

  13. Data Assimilation C. L. Martin and A.-L. Barrett National Center for Atmospheric Research

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    C. L. Martin and A.-L. Barrett National Center for Atmospheric Research Boulder, CO 80307-3000 The integrated sounding system (188) combines a suite of in situ and remote sensing systems with local computing capabilities. The resulting integrated instrument provides detailed real-time vertical profiles of the basic atmospheric parameters at a variety of time and space resolutions. One hallmark of the system is its configurability, which allows individual sensing systems to be added or removed as

  14. Data Assimilation J. S. Van Baelen(a) National Center for Atmospheric Research(b)

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    S. Van Baelen(a) National Center for Atmospheric Research(b) Boulder, CO 80307-3000 Introduction of wind profilers to provide accurate estimates of the momentum and heat fluxes might be their most important contribution yet to the field of atmospheric dynamic studies, especially when those measurements can be ingested into circulation models. In particular, flux measurements in the planetary boundary layer can provide critically needed information on the pel turbulent structures and their effect

  15. Discovery of oxygen in atmosphere could mean life for Saturn's moon Dione

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Discovery of oxygen in atmosphere could mean life for Saturn's moon Dione Discovery of oxygen in atmosphere could mean life for Saturn's moon Dione Discovery could mean ingredients for life are abundant on icy space bodies. March 5, 2012 Curiosity rover bears three LANL technologies Inside Titan: This artist's concept shows a possible scenario for the internal structure of Titan, as suggested by data from NASA's Cassini spacecraft. Scientists have been trying to determine what is under Titan's

  16. Simulated response of the atmosphere-ocean system to deforestation in the

    Office of Scientific and Technical Information (OSTI)

    Indonesian Archipelago (Journal Article) | SciTech Connect Simulated response of the atmosphere-ocean system to deforestation in the Indonesian Archipelago Citation Details In-Document Search Title: Simulated response of the atmosphere-ocean system to deforestation in the Indonesian Archipelago No abstract prepared. Authors: Delire, Christine ; Behling, Pat ; Coe, Michael T. ; Foley, Johnathan A. ; Jacob, Robert ; Kutzbach, John ; Liu, Zhengyu ; Vavrus, Stever Publication Date: 2001-05-15

  17. A technique for measuring winds in the lower atmosphere using incoherent Doppler lidar

    SciTech Connect (OSTI)

    DeSlover, D.H.; Slaughter, D.R.; Tulloch, W.M.; White, W.E.

    1993-04-14

    Wind speed is useful from a meteorological standpoint, in atmospheric modeling, and assessment of trace gas dispersal. A continuing effort is involved in improving the sensitivity of such measurements, and is exemplified by the literature. The Mobile Atmospheric Research Laboratory (MARL) at Lawrence Livermore National Laboratory (LLNL) is currently developing a method to improve the sensitivity of wind sounding in the lower through middle atmosphere using a pair of Fabry- Perot interferometers in parallel. This technique, first described by Chanin, et al., for the middle atmosphere using Doppler Rayleigh lidar, can be applied to the lower atmosphere where Mie (aerosol) backscatter is strong. Elastic events, inherent in both Rayleigh and Mie backscatter, dominate the return signal throughout the atmosphere. Both are susceptible to local wind vectors; which will Doppler shift the laser frequency proportional to the wind velocity. A pair of Fabry-Perot interferometers, tuned to either side of the laser frequency, will provide necessary data to determine the shift in frequency of the backscattered signal. Spectral drift and jitter of the laser and a lack of data points to determine the wind vector place limits on the sensitivity of the system. A method to minimize each of these is presented.

  18. A technique for measuring winds in the lower atmosphere using incoherent Doppler lidar

    SciTech Connect (OSTI)

    DeSlover, D.H.; Slaughter, D.R.; Tulloch, W.M.; White, W.E.

    1993-04-14

    Wind speed is useful from a meteorological standpoint, in atmospheric modeling, and assessment of trace gas dispersal. A continuing effort is involved in improving the sensitivity of such measurements, and is exemplified by the literature. The Mobile Atmospheric Research Laboratory (MARL) at Lawrence Livermore National Laboratory (LLNL) is currently developing a method to improve the sensitivity of wind sounding in the lower through middle atmosphere using a pair of Fabry-Perot interferometers in parallel. This technique, first described by Chanin, et al., for the middle atmosphere using Doppler Rayleigh lidar, can be applied to the lower atmosphere where Mie (aerosol) backscatter is strong. Elastic events, inherent in both Rayleigh and Mie backscatter, dominate the return signal throughout the atmosphere. Both are susceptible to local wind vectors; which will Doppler shift the laser frequency proportional to the wind velocity. A pair of Fabry-Perot interferometers, tuned to either side of the laser frequency, will provide necessary data to determine the shift in frequency of the backscattered signal. Spectral drift and jitter of the laser and a lack of data points to determine the wind vector place limits on the sensitivity of the system. A method to minimize each of these is presented.

  19. Impact of California Phase 2 reformulated gasoline on atmospheric reactivity of exhaust and evaporative emissions

    SciTech Connect (OSTI)

    Kirchstetter, T.W.; Singer, B.C.; Harley, R.A.; Kendall, G.R.; Traverse, M.

    1997-12-31

    Phase 2 of California`s reformulated gasoline (RFG) program took effect statewide in the first half of 1996. Changes to gasoline composition required by Phase 2 specifications included: lower vapor pressure; lower olefin, aromatic, benzene, and sulfur content; lower T50 and T90; and a minimum oxygen content. In this paper, impacts of Phase 2 RFG on the atmospheric reactivity of motor vehicle exhaust and evaporative emissions are described. Volatile organic compounds in motor vehicle exhaust were measured at the Caldecott tunnel in summer 1995 and 1996. Aggregate emissions of greater than 8000 vehicles were measured each day. Regular and premium grade gasoline samples were collected from service stations in Berkeley concurrently with tunnel measurements both summers. Liquid gasoline samples and their headspace vapors were analyzed to determine detailed chemical composition. Normalized reactivity was calculated for exhaust and evaporative emissions by applying maximum incremental reactivity values to the detailed speciation profiles. Results indicate that the composition of gasoline in 1996 differed markedly from that of 1995. Changes in liquid gasoline composition led to corresponding changes in the speciation of vehicle exhaust and of gasoline headspace vapors. Benzene concentration in liquid gasoline decreased from 2.0 to 0.6 wt%, which contributed to a 70 and 37% reduction in benzene weight fraction in headspace vapors and vehicle exhaust, respectively. Addition of MTBE and reduction of olefins and aromatics in gasoline led to significant reductions in the atmospheric reactivity of unburned gasoline and gasoline headspace vapors. The normalized reactivity of liquid gasoline and headspace vapors decreased by 23 and 19%, respectively, between 1995 and 1996. The normalized reactivity of non-methane organic compounds in vehicle exhaust decreased by about 8%, but the uncertainty in this change was large.

  20. OH radicals distribution in an Ar-H{sub 2}O atmospheric plasma jet

    SciTech Connect (OSTI)

    Li, L.; Leys, C.; Nikiforov, A.; Institute of Solution Chemistry of the Russian Academy of Sciences, Academicheskaya St., 1, Ivanono, 153045 ; Xiong, Q.; College of Electrical and Electronic Engineering, HuaZhong University of Science and Technology, WuHan, Hubei 430074 ; Britun, N.; Snyders, R.; Materia Nova Research Centre, Parc Initialis, B-7000 Mons ; Lu, X.

    2013-09-15

    Recently, plasma jet systems found numerous applications in the field of biomedicine and treatment of temperature-sensitive materials. OH radicals are one of the main active species produced by these plasmas. Present study deals with the investigation of RF atmospheric pressure plasma jet in terms of OH radicals production by admixture of H{sub 2}O into argon used as a feed gas. Generation of OH radicals is studied by laser-induced fluorescence spectroscopy. The excitation dynamics of OH radicals induced by the laser photons is studied by time-resolved spectroscopy. It is shown that vibrational and rotational energy transfer processes, which are sensitive to the surrounding species, can lead to the complication in the OH radicals diagnostics at high pressure and have to be considered during experiments. The axial and radial 2D maps of absolute densities of hydroxyl radicals at different water contents are obtained. The highest density of 1.15 10{sup 20} m{sup ?3} is measured in the plasma core for the case of 0.3% H{sub 2}O. In the xy-plane, the OH density steeply decreases within a range of 2 mm from its maximum value down to 10{sup 18} m{sup ?3}. The effect of H{sub 2}O addition on the generation of OH radicals is investigated and discussed.

  1. Development and field testing of a rapid and ultra-stable atmospheric carbon dioxide spectrometer

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Xiang, B.; Nelson, D. D.; McManus, J. B.; Zahniser, M. S.; Wehr, R. A.; Wofsy, S. C.

    2014-12-15

    We present field test results for a new spectroscopic instrument to measure atmospheric carbon dioxide (CO2) with high precision (0.02 μmol mol-1, or ppm at 1 Hz) and demonstrate high stability (within 0.1 ppm over more than 8 months), without the need for hourly, daily, or even monthly calibration against high-pressure gas cylinders. The technical novelty of this instrument (ABsolute Carbon dioxide, ABC) is the spectral null method using an internal quartz reference cell with known CO2 column density. Compared to a previously described prototype, the field instrument has better stability and benefits from more precise thermal control of themore » optics and more accurate pressure measurements in the sample cell (at the mTorr level). The instrument has been deployed at a long-term ecological research site (the Harvard Forest, USA), where it has measured for 8 months without on-site calibration and with minimal maintenance, showing drift bounds of less than 0.1 ppm. Field measurements agree well with those of a commercially available cavity ring-down CO2 instrument (Picarro G2301) run with a standard calibration protocol. This field test demonstrates that ABC is capable of performing high-accuracy, unattended, continuous field measurements with minimal use of reference gas cylinders.« less

  2. Development and field testing of a rapid and ultra-stable atmospheric carbon dioxide spectrometer

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Xiang, B.; Nelson, D. D.; McManus, J. B.; Zahniser, M. S.; Wehr, R.; Wofsy, S. C.

    2014-08-05

    We present field test results for a new spectroscopic instrument to measure atmospheric carbon dioxide (CO2) with high precision (0.02 ppm at 1 Hz) and demonstrate high stability (within 0.1 ppm over more than 8 months), without the need for hourly, daily, or even monthly calibration against high-pressure gas cylinders. The technical novelty of this instrument (ABsolute Carbon dioxide, ABC) is the spectral null method using an internal quartz reference cell with known CO2 column density. Compared to a previously described prototype, the field instrument has better stability and benefits from more precise thermal control of the optics and moremore » accurate pressure measurements in the sample cell (at the mTorr level). The instrument has been deployed at a long-term ecological research site (the Harvard Forest, USA), where it has measured for eight months without on-site calibration and with minimal maintenance, showing drift bounds of less than 0.1 ppm. Field measurements agree well with those of another commercially available cavity ring-down CO2 instrument (Picarro G2301) run with a standard calibration protocol. This field test demonstrates that ABC is capable of performing high-accuracy, unattended, continuous field measurements with minimal use of calibration cylinders.« less

  3. Technical Sessions D. A. Randall K. Xu Department of Atmospheric...

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    andor destabilizing and moistening rates, as well as large-scale pre:ssure gradient forces) and underlying surface conditions. The horizontal domain is 512 km wide with a...

  4. Pacific Northwest Laboratory annual report for 1985 to the DOE Office of Energy Research. Part 3. Atmospheric sciences

    SciTech Connect (OSTI)

    Elderkin, C.E.

    1986-02-01

    The goals of atmospheric research at Pacific Northwest Laboratory (PNL) are to describe and predict the nature and fate of atmospheric contaminants and to develop an understanding of the atmospheric processes contributing to their distribution on local, regional, and continental scales. In 1985, this research has examined the transport and diffusion of atmospheric contaminants in areas of complex terrain, summarized the field studies and analyses of dry deposition and resuspension conducted in past years, and begun participation in a large, multilaboratory program to assess the precipitation scavenging processes important to the transformation and wet deposition of chemicals composing ''acid rain.'' The description of atmospheric research at PNL is organized in terms of the following study areas: Atmospheric Studies in Complex Terrain; Dispersion, Deposition, and Resuspension of Atmospheric Contaminants; and Processing of Emissions by Clouds and Precipitation (PRECP).

  5. DIRECT IMAGING DETECTION OF METHANE IN THE ATMOSPHERE OF GJ 504 b

    SciTech Connect (OSTI)

    Janson, Markus; Brandt, Timothy D.; Kuzuhara, Masayuki; Spiegel, David S.; Thalmann, Christian; Currie, Thayne; Bonnefoy, Mickal; Zimmerman, Neil; Schlieder, Joshua; Brandner, Wolfgang; Feldt, Markus; Sorahana, Satoko; Kotani, Takayuki; Hashimoto, Jun; Kusakabe, Nobuhiko; Kudo, Tomoyuki; Egner, Sebastian; Abe, Lyu; Carson, Joseph C.; Goto, Miwa; and others

    2013-11-20

    Most exoplanets detected by direct imaging thus far have been characterized by relatively hot (?1000K) and cloudy atmospheres. A surprising feature in some of their atmospheres has been a distinct lack of methane, possibly implying non-equilibrium chemistry. Recently, we reported the discovery of a planetary companion to the Sun-like star GJ 504 using Subaru/HiCIAO within the Strategic Exploration of Exoplanets and Disks with Subaru survey. The planet is substantially colder (<600K) than previously imaged planets, and has indications of fewer clouds, which implies that it represents a new class of planetary atmospheres with expected similarities to late T-type brown dwarfs in the same temperature range. If so, one might also expect the presence of significant methane absorption, which is characteristic of such objects. Here, we report the detection of deep methane absorption in the atmosphere of GJ 504 b, using the Spectral Differential Imaging mode of HiCIAO to distinguish the absorption features around 1.6 ?m. We also report updated JHK photometry based on new K {sub s}-band data and a re-analysis of the existing data. The results support the notion that GJ 504 b has atmospheric properties distinct from other imaged exoplanets, and will become a useful reference object for future planets in the same temperature range.

  6. Mass spectrometers for studying the ionic and neutral composition of the upper layers of the atmosphere

    SciTech Connect (OSTI)

    Shutov, M.D.

    1984-04-01

    The investigation of the ionic and neutral composition of the upper layers of the atmosphere and outer space which is of interest for solving theoretical and applied problems of astrophysics, geophysics, space biology, and other closely-tied areas of science is discussed. The upper layers of the atmosphere are of practical significance for launching rockets and artificial satellites, for which the nature of movement depends on the structure and composition of the atmosphere. The study of the chemical composition of the ionosphere, the degree of ionization of the upper layers of the atmosphere at different latitudes and different times of day, and the dependence of ionization on the action of ultraviolet and corpuscular radiation is necessary to study the processes of the propagation of radio waves, and to explain the chemical and photochemical reaction which cause the ionosphere to exist. The most modern methods of study the composition of the mass spectral method which is a direct method and is especially valuable at great altitudes to study the composition of the upper atmosphere is considered. The mass spectrometric method is the only one to analyze the composition of ionizing gases.

  7. A TRANSMISSION SPECTRUM OF TITAN'S NORTH POLAR ATMOSPHERE FROM A SPECULAR REFLECTION OF THE SUN

    SciTech Connect (OSTI)

    Barnes, Jason W.; Clark, Roger N.; Sotin, Christophe; Buratti, Bonnie J.; dmkovics, Mt; Appr, Thomas; Rodriguez, Sebastien; Brown, Robert H.; Baines, Kevin H.; Le Moulic, Stphane; Nicholson, Philip D.

    2013-11-10

    Cassini/VIMS T85 observations of a solar specular reflection off of Kivu Lacus (87.4N 241.1E) provide an empirical transmission spectrum of Titan's atmosphere. Because this observation was acquired from short range (33,000 km), its intensity makes it visible within the 2.0, 2.7, and 2.8 ?m atmospheric windows in addition to the 5 ?m window where all previous specular reflections have been seen. The resulting measurement of the total one-way normal atmospheric optical depth (corresponding to haze scattering plus haze and gas absorption) provides strong empirical constraints on radiative transfer models. Using those models, we find that the total haze column abundance in our observation is 20% higher than the Huygens equatorial value. Ours is the first measurement in the 2-5 ?m wavelength range that probes all the way to the surface in Titan's arctic, where the vast majority of surface liquids are located. The specular technique complements other probes of atmospheric properties such as solar occultations and the direct measurements from Huygens. In breaking the degeneracy between surface and atmospheric absorptions, our measured optical depths will help to drive future calculations of deconvolved surface albedo spectra.

  8. Atmospheric Carbon Dioxide and the Global Carbon Cycle: The Key Uncertainties

    DOE R&D Accomplishments [OSTI]

    Peng, T. H.; Post, W. M.; DeAngelis, D. L.; Dale, V. H.; Farrell, M. P.

    1987-12-01

    The biogeochemical cycling of carbon between its sources and sinks determines the rate of increase in atmospheric CO{sub 2} concentrations. The observed increase in atmospheric CO{sub 2} content is less than the estimated release from fossil fuel consumption and deforestation. This discrepancy can be explained by interactions between the atmosphere and other global carbon reservoirs such as the oceans, and the terrestrial biosphere including soils. Undoubtedly, the oceans have been the most important sinks for CO{sub 2} produced by man. But, the physical, chemical, and biological processes of oceans are complex and, therefore, credible estimates of CO{sub 2} uptake can probably only come from mathematical models. Unfortunately, one- and two-dimensional ocean models do not allow for enough CO{sub 2} uptake to accurately account for known releases. Thus, they produce higher concentrations of atmospheric CO{sub 2} than was historically the case. More complex three-dimensional models, while currently being developed, may make better use of existing tracer data than do one- and two-dimensional models and will also incorporate climate feedback effects to provide a more realistic view of ocean dynamics and CO{sub 2} fluxes. The instability of current models to estimate accurately oceanic uptake of CO{sub 2} creates one of the key uncertainties in predictions of atmospheric CO{sub 2} increases and climate responses over the next 100 to 200 years.

  9. Coupled land-ocean-atmosphere processes and South Asian monsoon variability

    SciTech Connect (OSTI)

    Meehl, G.A.

    1994-10-14

    Results from a global coupled ocean-atmosphere climate model and a model with specified tropical convective heating anomalies show that the South Asian monsoon was an active part of the tropical biennial oscillation (TBO). Convective heating anomalies over Africa and the western Pacific Ocean associated with the TBO altered the simulated pattern of atmospheric circulation for the Northern Hemisphere winter mid-latitude over Asia. This alteration in the mid-latitude circulation maintained temperature anomalies over South Asia through winter and helped set up the land-sea temperature contrast for subsequent monsoon development. South Asian snow cover contributed to monsoon strength but was symptomatic of the larger scale alteration in the mid-latitude atmospheric circulation pattern. 36 refs., 5 figs.

  10. Acoustic waves in the atmosphere and ground generated by volcanic activity

    SciTech Connect (OSTI)

    Ichihara, Mie; Lyons, John; Oikawa, Jun; Takeo, Minoru

    2012-09-04

    This paper reports an interesting sequence of harmonic tremor observed in the 2011 eruption of Shinmoe-dake volcano, southern Japan. The main eruptive activity started with ashcloud forming explosive eruptions, followed by lava effusion. Harmonic tremor was transmitted into the ground and observed as seismic waves at the last stage of the effusive eruption. The tremor observed at this stage had unclear and fluctuating harmonic modes. In the atmosphere, on the other hand, many impulsive acoustic waves indicating small surface explosions were observed. When the effusion stopped and the erupted lava began explosive degassing, harmonic tremor started to be transmitted also to the atmosphere and observed as acoustic waves. Then the harmonic modes became clearer and more stable. This sequence of harmonic tremor is interpreted as a process in which volcanic degassing generates an open connection between the volcanic conduit and the atmosphere. In order to test this hypothesis, a laboratory experiment was performed and the essential features were successfully reproduced.

  11. Improved determination of the atmospheric parameters of the pulsating sdB star Feige 48

    SciTech Connect (OSTI)

    Latour, M.; Fontaine, G.; Brassard, P.; Green, E. M.; Chayer, P.

    2014-06-10

    As part of a multifaceted effort to better exploit the asteroseismological potential of the pulsating sdB star Feige 48, we present an improved spectroscopic analysis of that star based on new grids of NLTE, fully line-blanketed model atmospheres. To that end, we gathered four high signal-to-noise ratio time-averaged optical spectra of varying spectral resolutions from 1.0 to 8.7 , and we made use of the results of four independent studies to fix the abundances of the most important metals in the atmosphere of Feige 48. The mean atmospheric parameters we obtained from our four spectra of Feige 48 are: T {sub eff} = 29,850 60 K, log g = 5.46 0.01, and log N(He)/N(H) = 2.88 0.02. We also modeled, for the first time, the He II line at 1640 from the STIS archive spectrum of the star, and with this line we found an effective temperature and a surface gravity that match well with the values obtained with the optical data. With some fine tuning of the abundances of the metals visible in the optical domain, we were able to achieve a very good agreement between our best available spectrum and our best-fitting synthetic one. Our derived atmospheric parameters for Feige 48 are in rather good agreement with previous estimates based on less sophisticated models. This underlines the relatively small effects of the NLTE approach combined with line blanketing in the atmosphere of this particular star, implying that the current estimates of the atmospheric parameters of Feige 48 are reliable and secure.

  12. North America's net terrestrial carbon exchange with the atmosphere 1990-2009

    SciTech Connect (OSTI)

    King, Anthony W.; Andres, Robert; Davis, Kenneth J.; Hafer, M.; Hayes, Daniel J.; Huntzinger, Deborah N.; de Jong, Bernardus; Kurz, Werner; McGuire, A. David; Vargas, Rodrigo; Wei, Yaxing; West, Tristram O.; Woodall, Chris W.

    2015-01-01

    Scientific understanding of the global carbon cycle is required for developing national and international policy to mitigate fossil-fuel CO2 emissions by managing terrestrial carbon uptake. Toward that understanding and as a contribution to the REgional Carbon Cycle Assessment and Processes (RECCAP) project, this paper provides a synthesis of net land-atmosphere CO2 exchange for North America over the period (1990-2009). This synthesis is based on results from three different methods: atmospheric inversion, inventory-based methods and terrestrial biosphere modeling. All methods indicate that the North America land surface was a sink for atmospheric CO2, with a net transfer from atmosphere to land. Estimates ranged from -890 to -280 Tg C yr-1, where the atmospheric inversion estimate forms the lower bound of that range (a larger land-sink) and the inventory-based estimate the upper (a smaller land sink). Integrating across estimates, a best estimates (i.e., measures of central tendency) are -472 281 Tg C yr-1 based on the mean and standard deviation of the distribution and -360 Tg C yr-1 (with an interquartile range of -496 to -337) based on the median. Considering both the fossil-fuel emissions source and the land sink, our analysis shows that North America was, however, a net contributor to the growth of CO2 in the atmosphere in the late 20th and early 21st century. The continents CO2 source to sink ratio for this time period was likely in the range of 4:1 to 3:1.

  13. LABLE: A multi-institutional, student-led, atmospheric boundary layer experiment

    SciTech Connect (OSTI)

    Klein, P.; Bonin, T. A.; Newman, J. F.; Turner, D. D.; Chilson, P. B.; Wainwright, C. E.; Blumberg, W. G.; Mishra, S.; Carney, M.; Jacobsen, E. P.; Wharton, Sonia; Newsom, Rob K.

    2015-10-23

    This paper presents an overview of the Lower Atmospheric Boundary Layer Experiment (LABLE), which included two measurement campaigns conducted at the Atmospheric Radiation Measurement (ARM) Southern Great Plains site in Oklahoma during 2012 and 2013. LABLE was conducted as a collaborative effort between the University of Oklahoma (OU), the National Severe Storms Laboratory, Lawrence Livermore National Laboratory (LLNL), and the ARM program. LABLE can be considered unique in that it was designed as a multi-phase, low-cost, multi-agency collaboration. Graduate students served as principal investigators and took the lead in designing and conducting experiments aimed at examining boundary-layer processes. The main objective of LABLE was to study turbulent phenomena in the lowest 2 km of the atmosphere over heterogeneous terrain using a variety of novel atmospheric profiling techniques. Several instruments from OU and LLNL were deployed to augment the suite of in-situ and remote sensing instruments at the ARM site. The complementary nature of the deployed instruments with respect to resolution and height coverage provides a near-complete picture of the dynamic and thermodynamic structure of the atmospheric boundary layer. This paper provides an overview of the experiment including i) instruments deployed, ii) sampling strategies, iii) parameters observed, and iv) student involvement. To illustrate these components, the presented results focus on one particular aspect of LABLE, namely the study of the nocturnal boundary layer and the formation and structure of nocturnal low-level jets. During LABLE, low-level jets were frequently observed and they often interacted with mesoscale atmospheric disturbances such as frontal passages.

  14. HGSYSTEMUF6. Model for Simulating Dispersion due to Atmospheric Release of UF6

    SciTech Connect (OSTI)

    Hanna, G; Chang, J.C.; Zhang, J.X.; Bloom, S.G.; Goode, W.D. Jr; Lombardi, D.A.; Yambert, M.W.

    1998-08-01

    HGSYSTEMUF6 is a suite of models designed for use in estimating consequences associated with accidental, atmospheric release of Uranium Hexafluoride (UF6) and its reaction products, namely Hydrogen Fluoride (HF), and other non-reactive contaminants which are either negatively, neutrally, or positively buoyant. It is based on HGSYSTEM Version 3.0 of Shell Research LTD., and contains specific algorithms for the treatment of UF6 chemistry and thermodynamics. HGSYSTEMUF6 contains algorithms for the treatment of dense gases, dry and wet deposition, effects due to the presence of buildings (canyon and wake), plume lift-off, and the effects of complex terrain. The models components of the suite include (1) AEROPLUME/RK, used to model near-field dispersion from pressurized two-phase jet releases of UF6 and its reaction products, (2) HEGADAS/UF6 for simulating dense, ground based release of UF6, (3) PGPLUME for simulation of passive, neutrally buoyant plumes (4) UF6Mixer for modeling warm, potentially reactive, ground-level releases of UF6 from buildings, and (5) WAKE, used to model elevated and ground-level releases into building wake cavities of non-reactive plumes that are either neutrally or positively buoyant.

  15. Synthesis of YBa2CU3O7 using sub-atmospheric processing

    DOE Patents [OSTI]

    Wiesmann, Harold; Solovyov, Vyacheslav

    2004-09-21

    The present invention is a method of forming thick films of crystalline YBa.sub.2 Cu.sub.3 O.sub.7 that includes forming a precursor film comprising barium fluoride (BaF.sub.2), yttrium (Y) and copper (Cu). The precursor film is heat-treated at a temperature above 500.degree. C. in the presence of oxygen, nitrogen and water vapor at sub-atmospheric pressure to form a crystalline structure. The crystalline structure is then annealed at about 500.degree. C. in the presence of oxygen to form the crystalline YBa.sub.2 Cu.sub.3 O.sub.7 film. The YBa.sub.2 Cu.sub.3 O.sub.7 film formed by this method has a resistivity of from about 100 to about 600 .mu.Ohm-cm at room temperature and a critical current density measured at 77 K in a magnetic field of 1 Tesla of about 1.0.times.10.sup.5 Ampere per square centimeter (0.1 MA/cm.sup.2) or greater.

  16. Model for Simulating Dispersion due to Atmospheric Release of UF6

    Energy Science and Technology Software Center (OSTI)

    1997-01-01

    HGSYSTEMUF6 is a suite of models designed for use in estimating consequences associated with accidental, atmospheric release of Uranium Hexafluoride (UF6) and its reaction products, namely Hydrogen Fluoride (HF), and other non-reactive contaminants which are either negatively, neutrally, or positively buoyant. It is based on HGSYSTEM Version 3.0 of Shell Research LTD., and contains specific algorithms for the treatment of UF6 chemistry and thermodynamics. HGSYSTEMUF6 contains algorithms for the treatment of dense gases, dry andmore » wet deposition, effects due to the presence of buildings (canyon and wake), plume lift-off, and the effects of complex terrain. The models components of the suite include (1) AEROPLUME/RK, used to model near-field dispersion from pressurized two-phase jet releases of UF6 and its reaction products, (2) HEGADAS/UF6 for simulating dense, ground based release of UF6, (3) PGPLUME for simulation of passive, neutrally buoyant plumes (4) UF6Mixer for modeling warm, potentially reactive, ground-level releases of UF6 from buildings, and (5) WAKE, used to model elevated and ground-level releases into building wake cavities of non-reactive plumes that are either neutrally or positively buoyant.« less

  17. A first-look atmospheric modeling study of the young directly imaged

    Office of Scientific and Technical Information (OSTI)

    planet-mass companion, ROXS 42Bb (Journal Article) | SciTech Connect A first-look atmospheric modeling study of the young directly imaged planet-mass companion, ROXS 42Bb Citation Details In-Document Search Title: A first-look atmospheric modeling study of the young directly imaged planet-mass companion, ROXS 42Bb We present and analyze JK{sub s}L' photometry and our previously published H-band photometry and K-band spectroscopy for ROXs 42Bb, an object Currie et al. first reported as a

  18. Atmospheric and soil-gas monitoring for surface leakage at the San Juan

    Office of Scientific and Technical Information (OSTI)

    Basin CO{sub 2} pilot test site at Pump Canyon New Mexico, using perfluorocarbon tracers, CO{sub 2} soil-gas flux and soil-gas hydrocarbons (Journal Article) | SciTech Connect Atmospheric and soil-gas monitoring for surface leakage at the San Juan Basin CO{sub 2} pilot test site at Pump Canyon New Mexico, using perfluorocarbon tracers, CO{sub 2} soil-gas flux and soil-gas hydrocarbons Citation Details In-Document Search Title: Atmospheric and soil-gas monitoring for surface leakage at the

  19. Developing El Niño The National Oceanic and Atmospheric Administration

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    2 Developing El Niño The National Oceanic and Atmospheric Administration (NOAA) recently announced the development of El Niño conditions in the tropical Pacific Ocean near the South American coastline. Scientists detected a 4ºF increase in the sea-surface temperatures during February. Conrad C. Lautenbacher, NOAA administrator and Under Secretary of Commerce for Oceans and Atmosphere, indicated that this warming is a sign that the Pacific Ocean is heading toward an El Niño condition.

  20. COLLOQUIUM: The Alfvénic Motions of the Sun's Outer Atmosphere | Princeton

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Plasma Physics Lab 8, 2013, 4:15pm to 5:30pm Colloquia MBG Auditorium COLLOQUIUM: The Alfvénic Motions of the Sun's Outer Atmosphere Scott McIntosh National Center for Atmospheric Research (NCAR) Presentation: PDF icon WC08MAY2013_SWMcIntosh.pdf In 2005 a novel imaging spectro-polarimeter, the Coronal Multi-channel Polarimeter (CoMP), was deployed to the Evans Facility in Sunspot, NM to measure the solar corona's magnetic field. The design of the instrument permitted it to capture something

  1. Continuous Water Vapor Profiles for the Fixed Atmospheric Radiation Measurement Sites

    SciTech Connect (OSTI)

    Jensen, M; Troyan, D

    2006-01-09

    The Atmospheric Radiation Measurement (ARM) Program defined a specific metric for the first quarter of Fiscal Year 2006 to complete a continuous time series of the vertical profile of water vapor for selected 30-day periods from each of the fixed ARM sites. In order to accomplish this metric, a new technique devised to incorporate radiosonde data, microwave radiometer data and analysis information from numerical weather forecast models has been developed. The product of this analysis, referred to as the merged sounding value-added product, includes vertical profiles of atmospheric water vapor concentration and several other important thermodynamic state variables at 1-minute time intervals and 266 vertical levels.

  2. Asymmetry in the Diurnal Cycle of Atmospheric Downwelling Radiation at the ARM SGP CF Site Over 1995-2001 Period

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Asymmetry in the Diurnal Cycle of Atmospheric Downwelling Radiation at the ARM SGP CF Site Over 1995-2001 Period A. P. Trishchenko Canada Centre for Remote Sensing Ottawa, Ontario, Canada Introduction The shape of the diurnal cycle of atmospheric downwelling radiation is an important climatic feature of cloud-radiation interactions and atmospheric properties. Adequate characterization of this diurnal cycle is critical for accurate determination of monthly and seasonal radiation budgets from a

  3. Remote Raman - laser induced breakdown spectroscopy (LIBS) geochemical investigation under Venus atmospheric conditions

    SciTech Connect (OSTI)

    Clegg, Sanuel M; Barefield, James E; Humphries, Seth D; Wiens, Roger C; Vaniman, D. T.; Sharma, S. K.; Misra, A. K.; Dyar, M. D.; Smrekar, S. E.

    2010-12-13

    The extreme Venus surface temperatures ({approx}740 K) and atmospheric pressures ({approx}93 atm) create a challenging environment for surface missions. Scientific investigations capable of Venus geochemical observations must be completed within hours of landing before the lander will be overcome by the harsh atmosphere. A combined remote Raman - LIBS (Laser Induced Breakdown Spectroscopy) instrument is capable of accomplishing the geochemical science goals without the risks associated with collecting samples and bringing them into the lander. Wiens et al. and Sharma et al. demonstrated that both analytical techniques can be integrated into a single instrument capable of planetary missions. The focus of this paper is to explore the capability to probe geologic samples with Raman - LIBS and demonstrate quantitative analysis under Venus surface conditions. Raman and LIBS are highly complementary analytical techniques capable of detecting both the mineralogical and geochemical composition of Venus surface materials. These techniques have the potential to profoundly increase our knowledge of the Venus surface composition, which is currently limited to geochemical data from Soviet Venera and VEGA landers that collectively suggest a surface composition that is primarily tholeiitic basaltic with some potentially more evolved compositions and, in some locations, K-rich trachyandesite. These landers were not equipped to probe the surface mineralogy as can be accomplished with Raman spectroscopy. Based on the observed compositional differences and recognizing the imprecise nature of the existing data, 15 samples were chosen to constitute a Venus-analog suite for this study, including five basalts, two each of andesites, dacites, and sulfates, and single samples of a foidite, trachyandesite, rhyolite, and basaltic trachyandesite under Venus conditions. LIBS data reduction involved generating a partial least squares (PLS) model with a subset of the rock powder standards to quantitatively determine the major elemental abundance of the remaining samples. PLS analysis suggests that the major element compositions can be determined with root mean square errors ca. 5% (absolute) for SiO{sub 2}, Al{sub 2}O{sub 3}, Fe{sub 2}O{sub 3}(total), MgO, and CaO, and ca. 2% or less for TiO{sub 2}, Cr{sub 2}O{sub 3}, MnO, K{sub 2}O, and Na{sub 2}O. Finally, the Raman experiments have been conducted under supercritical CO{sub 2} involving single-mineral and mixed-mineral samples containing talc, olivine, pyroxenes, feldspars, anhydrite, barite, and siderite. The Raman data have shown that the individual minerals can easily be identified individually or in mixtures.

  4. Ambient-atmosphere glow discharge for determination of elemental concentration in solutions in a high-throughput or transient fashion

    DOE Patents [OSTI]

    Webb, Michael R. (Somerville, MA); Hieftje, Gary M. (Bloomington, IN); Andrade, Francisco (Leeds, GB)

    2011-04-19

    An ambient atmosphere glow discharge spectrometer is disclosed having a capillary, two electrodes and a means for recording the atomic emissions.

  5. Closure Report for Corrective Action Unit 104: Area 7 Yucca Flat Atmospheric Test Sites, Nevada National Security Site, Nevada

    SciTech Connect (OSTI)

    2013-06-27

    This Closure Report (CR) presents information supporting closure of Corrective Action Unit (CAU) 104, Area 7 Yucca Flat Atmospheric Test Sites, and provides documentation supporting the completed corrective actions and confirmation that closure objectives for CAU 104 were met. This CR complies with the requirements of the Federal Facility Agreement and Consent Order (FFACO) that was agreed to by the State of Nevada; the U.S. Department of Energy (DOE), Environmental Management; the U.S. Department of Defense; and DOE, Legacy Management. CAU 104 consists of the following 15 Corrective Action Sites (CASs), located in Area 7 of the Nevada National Security Site: CAS 07-23-03, Atmospheric Test Site T-7C CAS 07-23-04, Atmospheric Test Site T7-1 CAS 07-23-05, Atmospheric Test Site CAS 07-23-06, Atmospheric Test Site T7-5a CAS 07-23-07, Atmospheric Test Site - Dog (T-S) CAS 07-23-08, Atmospheric Test Site - Baker (T-S) CAS 07-23-09, Atmospheric Test Site - Charlie (T-S) CAS 07-23-10, Atmospheric Test Site - Dixie CAS 07-23-11, Atmospheric Test Site - Dixie CAS 07-23-12, Atmospheric Test Site - Charlie (Bus) CAS 07-23-13, Atmospheric Test Site - Baker (Buster) CAS 07-23-14, Atmospheric Test Site - Ruth CAS 07-23-15, Atmospheric Test Site T7-4 CAS 07-23-16, Atmospheric Test Site B7-b CAS 07-23-17, Atmospheric Test Site - Climax Closure activities began in October 2012 and were completed in April 2013. Activities were conducted according to the Corrective Action Decision Document/Corrective Action Plan for CAU 104. The corrective actions included No Further Action and Clean Closure. Closure activities generated sanitary waste, mixed waste, and recyclable material. Some wastes exceeded land disposal limits and required treatment prior to disposal. Other wastes met land disposal restrictions and were disposed in appropriate onsite landfills. The U.S. Department of Energy, National Nuclear Security Administration Nevada Field Office (NNSA/NFO) requests the following: A Notice of Completion from the Nevada Division of Environmental Protection to NNSA/NFO for closure of CAU 104 The transfer of CAU 104 from Appendix III to Appendix IV, Closed Corrective Action Units, of the FFACO

  6. Element- and charge-state-resolved ion energies in the cathodic arc plasma from composite AlCr cathodes in argon, nitrogen and oxygen atmospheres

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Franz, Robert; Polcik, Peter; Anders, André

    2015-06-01

    The energy distribution functions of ions in the cathodic arc plasma using composite AlCr cathodes were measured as a function of the background gas pressure in the range 0.5 to 3.5 Pa for different cathode compositions and gas atmospheres. The most abundant aluminium ions were Al+ regardless of the background gas species, whereas Cr2+ ions were dominating in Ar and N2 and Cr+ in O2 atmospheres. The energy distributions of the aluminium and chromium ions typically consisted of a high-energy fraction due to acceleration in the expanding plasma plume from the cathode spot and thermalised ions that were subjected tomore » collisions in the plasma cloud. The fraction of the latter increased with increasing background gas pressure. Atomic nitrogen and oxygen ions showed similar energy distributions as the aluminium and chromium ions, whereas the argon and molecular nitrogen and oxygen ions were formed at greater distance from the cathode spot and thus less subject to accelerating gradients. In addition to the positively charged metal and gas ions, negatively charged oxygen and oxygen-containing ions were observed in O2 atmosphere. The obtained results are intended to provide a comprehensive overview of the ion energies and charge states in the arc plasma of AlCr composite cathodes in different gas atmospheres as such plasmas are frequently used to deposit thin films and coatings.« less

  7. Element- and charge-state-resolved ion energies in the cathodic arc plasma from composite AlCr cathodes in argon, nitrogen and oxygen atmospheres

    SciTech Connect (OSTI)

    Franz, Robert; Polcik, Peter; Anders, Andr

    2015-06-01

    The energy distribution functions of ions in the cathodic arc plasma using composite AlCr cathodes were measured as a function of the background gas pressure in the range 0.5 to 3.5 Pa for different cathode compositions and gas atmospheres. The most abundant aluminium ions were Al+ regardless of the background gas species, whereas Cr2+ ions were dominating in Ar and N2 and Cr+ in O2 atmospheres. The energy distributions of the aluminium and chromium ions typically consisted of a high-energy fraction due to acceleration in the expanding plasma plume from the cathode spot and thermalised ions that were subjected to collisions in the plasma cloud. The fraction of the latter increased with increasing background gas pressure. Atomic nitrogen and oxygen ions showed similar energy distributions as the aluminium and chromium ions, whereas the argon and molecular nitrogen and oxygen ions were formed at greater distance from the cathode spot and thus less subject to accelerating gradients. In addition to the positively charged metal and gas ions, negatively charged oxygen and oxygen-containing ions were observed in O2 atmosphere. The obtained results are intended to provide a comprehensive overview of the ion energies and charge states in the arc plasma of AlCr composite cathodes in different gas atmospheres as such plasmas are frequently used to deposit thin films and coatings.

  8. Symposium on intermediate-range atmospheric-transport processes and technology assessment. [Lead Abstract

    SciTech Connect (OSTI)

    Not Available

    1981-10-01

    Separate abstracts were prepared for the 47 papers in this proceedings. The purpose of this meeting was to assess the state of the art of modeling atmospheric transport processes 10 to 100 km downwind of point and area sources of pollution. (KRM)

  9. National Oceanic and Atmospheric Administration's Honolulu Laboratory Renewal Project, Honolulu, Hawaii

    SciTech Connect (OSTI)

    Not Available

    2002-08-01

    This brochure provides an overview of The National Oceanic and Atmospheric Administration's Honolulu Laboratory Renewal Project, a project designed to adhere to the U.S. Green Building Council's Leadership in Energy and Environmental Design (LEED) rating system. Diagrams of the HVAC system and the rainwater collection system are included.

  10. Proceedings of the third Atmospheric Radiation Measurement (ARM) science team meeting

    SciTech Connect (OSTI)

    Not Available

    1994-03-01

    This document contains the summaries of papers presented at the 1993 Atmospheric Radiation Measurement (ARM) Science Team meeting held in Morman, Oklahoma. To put these papers in context, it is useful to consider the history and status of the ARM Program at the time of the meeting. Individual papers have been cataloged separately.

  11. Preliminary analysis of results of a mountain area atmospheric diffusion test

    SciTech Connect (OSTI)

    Not Available

    1983-12-01

    The results of diffusion test of artificial smoke clouds and neutron activated smoke were used to calculate the atmospheric diffusion parameters especially focusing on the differences of the diffusion diluting capabilities of the pollutants and comparing them with related foreign results where upon useful results were obtained.

  12. Compact 180-kV Marx generator triggered in atmospheric air by femtosecond laser filaments

    SciTech Connect (OSTI)

    Arantchouk, L. Larour, J.; Point, G.; Brelet, Y.; Carbonnel, J.; Andr, Y.-B.; Mysyrowicz, A.; Houard, A.

    2014-03-10

    We developed a compact Marx generator triggered in atmospheric air by a single femtosecond laser beam undergoing filamentation. Voltage pulses of 180?kV could be generated with a subnanosecond jitter. The same laser beam was also used to initiate simultaneously guided discharges up to 21?cm long at the output of the generator.

  13. Environmental assessment for the satellite power system concept development and evaluation program: atmospheric effects

    SciTech Connect (OSTI)

    Rote, D.M.; Brubaker, K.L.; Lee, J.L.

    1980-11-01

    The US Department of Energy (DOE) has undertaken a preliminary, three-year program to investigate the impacts of the construction and operation of a satellite power system, of unprecedented scale. The Department of Energy's program, titled The Concept Development and Evaluation Program, focused its investigations on a Reference System description that calls for the use of either silicon (Si) or gallium aluminum-arsenide (GaAlAs) photovoltaic cells on 60 satellites to be constructed in GEO over a 30-yr period. Rectennas would be constructed on the ground to receive microwave energy from the satellites. Each satellite-rectenna pair is designed to produce 5 GW of power on an essentially continuous basis for use as a baseload power source for an electric power distribution system. The environmental assessment part of the program was divided into five interdependent task areas. The present document constitutes the final technical report on one of the five task areas, the Assessment of the Atmospheric Effects, and as such presents an in-depth summary of work performed during the assessment program. The issues associated with SPS activities in the troposphere are examined. These include tropospheric weather modification related to rectenna operations and rocket launches, and air quality impacts related to rocketlaunch ground clouds. Then progressing upward through the various levels of the atmosphere, the principal middle and upper atmospheric effects associated with rocket effluents are analyzed. Finally, all of the potential SPS atmospheric effects are summarized.

  14. Influence of the atmosphere on remotely sensed reflection from vegetation surfaces

    SciTech Connect (OSTI)

    Simmer, C.; Gerstl, S.A.W.

    1985-01-01

    Multiple scattering of solar radiation in a vegetation canopy is modelled equivalent to absorbing and scattering in a turbid medium with direction-dependent cross sections. Perturbations of plant reflection patterns due to atmospheric effects are computed at different altitudes and compared to the angular reflection characteristics caused by Lambertian surfaces of varying albedoes.

  15. Ellerman bombsevidence for magnetic reconnection in the lower solar atmosphere

    SciTech Connect (OSTI)

    Nelson, C. J.; Doyle, J. G.; Madjarska, M. S. [Armagh Observatory, College Hill, Armagh BT61 9DG (United Kingdom); Shelyag, S. [Monash Centre for Astrophysics, School of Mathematical Sciences, Monash University, Clayton, VIC 3800 (Australia); Mathioudakis, M. [Astrophysical Research Centre, School of Mathematics and Physics, Queen's University, Belfast BT7 1NN (United Kingdom); Uitenbroek, H. [National Solar Observatory, Sacramento Peak, P.O. Box 62, Sunpsot, NM 88349 (United States); Erdlyi, R. [Solar Physics and Space Plasma Research Centre, University of Sheffield, Hicks Building, Hounsfield Road, Sheffield S3 7RH (United Kingdom)

    2013-12-20

    The presence of photospheric magnetic reconnection has long been thought to give rise to short and impulsive events, such as Ellerman bombs (EBs) and Type II spicules. In this article, we combine high-resolution, high-cadence observations from the Interferometric BIdimensional Spectrometer and Rapid Oscillations in the Solar Atmosphere instruments at the Dunn Solar Telescope, National Solar Observatory, New Mexico, with co-aligned Solar Dynamics Observatory Atmospheric Imaging Assembly and Hinode Solar Optical Telescope (SOT) data to observe small-scale events situated within an active region. These data are then compared with state-of-the-art numerical simulations of the lower atmosphere made using the MURaM code. It is found that brightenings, in both the observations and the simulations, of the wings of the H? line profile, interpreted as EBs, are often spatially correlated with increases in the intensity of the Fe I ?6302.5 line core. Bipolar regions inferred from Hinode/SOT magnetic field data show evidence of flux cancellation associated, co-spatially, with these EBs, suggesting that magnetic reconnection could be a driver of these high-energy events. Through the analysis of similar events in the simulated lower atmosphere, we are able to infer that line profiles analogous to the observations occur co-spatially with regions of strong opposite-polarity magnetic flux. These observed events and their simulated counterparts are interpreted as evidence of photospheric magnetic reconnection at scales observable using current observational instrumentation.

  16. Atmospheric Radiation Measurement Climate Research Facility (ACRF Instrumentation Status: New, Current, and Future)

    SciTech Connect (OSTI)

    JW Voyles

    2008-01-30

    The purpose of this report is to provide a concise but comprehensive overview of Atmospheric Radiation Measurement Climate Research Facility instrumentation status. The report is divided into the following four sections: (1) new instrumentation in the process of being acquired and deployed, (2) existing instrumentation and progress on improvements or upgrades, (3) proposed future instrumentation, and (4) Small Business Innovation Research instrument development.

  17. Long-Term Operation Of Ground-Based Atmospheric Sensing Systems In The Tropical Western Pacific

    SciTech Connect (OSTI)

    Ivey, Mark; Jones, Larry J.; Porch, W. M.; Apple, Monty L.; Widener, Kevin B.

    2004-10-14

    Three semi-autonomous atmospheric sensing systems were installed in the tropical western Pacific region. The first of these Atmospheric Radiation and Cloud Stations (ARCS) began operation in 1996. Each ARCS is configured as a system-of-systems since it comprises an ensemble of independent instrument systems. The ARCS collect, process, and transmit large volumes of cloud, solar and thermal radiation, and meteorological data to support climate studies and climate-modeling improvements as part of the U.S Department of Energys Atmospheric and Radiation Measurement (ARM) Program. Data from these tropical ARCS stations have been used for satellite ground-truth data comparisons and validations, including comparisons for MTI and AQUA satellite data. Our experiences with these systems in the tropics led to modifications in their design. An ongoing international logistics effort is required to keep gigabytes per day of quality-assured data flowing to the ARM programs archives. Design criteria, performance, communications methods, and the day-to-day logistics required to support long-term operations of ground-based remote atmospheric sensing systems are discussed. End-to-end data flow from the ARCS systems to the ARM Program archives is discussed.

  18. Fungi in the future: Interannual variation and effects of atmospheric change on arbuscular mycorrhizal fungal communities

    SciTech Connect (OSTI)

    Cotton, T. E. Anne; Fitter, Alastair H.; Miller, R. Michael; Dumbrell, Alex J.; Helgason, Thorunn

    2015-01-05

    Understanding the natural dynamics of arbuscular mycorrhizal (AM) fungi and their response to global environmental change is essential for the prediction of future plant growth and ecosystem functions. We investigated the long-term temporal dynamics and effect of elevated atmospheric carbon dioxide (CO2) and ozone (O3) concentrations on AM fungal communities. Molecular methods were used to characterize the AM fungal communities of soybean (Glycine max) grown under elevated and ambient atmospheric concentrations of both CO2 and O3 within a free air concentration enrichment experiment in three growing seasons over 5 yr. Elevated CO2 altered the community composition of AM fungi, increasing the ratio of Glomeraceae to Gigasporaceae. By contrast, no effect of elevated O3 on AM fungal communities was detected. However, the greatest compositional differences detected were between years, suggesting that, at least in the short term, large-scale interannual temporal dynamics are stronger mediators than atmospheric CO2 concentrations of AM fungal communities. We conclude that, although atmospheric change may significantly alter AM fungal communities, this effect may be masked by the influences of natural changes and successional patterns through time. We suggest that changes in carbon availability are important determinants of the community dynamics of AM fungi.

  19. ATMOSPHERIC DISPERSION COEFFICIENTS AND RADIOLOGICAL AND TOXICOLOGICAL EXPOSURE METHODOLOGY FOR USE IN TANK FARMS

    SciTech Connect (OSTI)

    GRIGSBY KM

    2011-04-07

    This report presents the atmospheric dispersion coefficients used in Tank Farms safety analysis. The basis equations for calculating radiological and toxicological exposures are also included. In this revision, the time averaging for toxicological consequence evaluations is clarified based on a review of DOE complex guidance and a review of tank farm chemicals.

  20. Fungi in the future: Interannual variation and effects of atmospheric change on arbuscular mycorrhizal fungal communities

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Cotton, T. E. Anne; Fitter, Alastair H.; Miller, R. Michael; Dumbrell, Alex J.; Helgason, Thorunn

    2015-01-05

    Understanding the natural dynamics of arbuscular mycorrhizal (AM) fungi and their response to global environmental change is essential for the prediction of future plant growth and ecosystem functions. We investigated the long-term temporal dynamics and effect of elevated atmospheric carbon dioxide (CO2) and ozone (O3) concentrations on AM fungal communities. Molecular methods were used to characterize the AM fungal communities of soybean (Glycine max) grown under elevated and ambient atmospheric concentrations of both CO2 and O3 within a free air concentration enrichment experiment in three growing seasons over 5 yr. Elevated CO2 altered the community composition of AM fungi, increasingmore » the ratio of Glomeraceae to Gigasporaceae. By contrast, no effect of elevated O3 on AM fungal communities was detected. However, the greatest compositional differences detected were between years, suggesting that, at least in the short term, large-scale interannual temporal dynamics are stronger mediators than atmospheric CO2 concentrations of AM fungal communities. We conclude that, although atmospheric change may significantly alter AM fungal communities, this effect may be masked by the influences of natural changes and successional patterns through time. We suggest that changes in carbon availability are important determinants of the community dynamics of AM fungi.« less

  1. Method of enhanced lithiation of doped silicon carbide via high temperature annealing in an inert atmosphere

    SciTech Connect (OSTI)

    Hersam, Mark C.; Lipson, Albert L.; Bandyopadhyay, Sudeshna; Karmel, Hunter J; Bedzyk, Michael J

    2014-05-27

    A method for enhancing the lithium-ion capacity of a doped silicon carbide is disclosed. The method utilizes heat treating the silicon carbide in an inert atmosphere. Also disclosed are anodes for lithium-ion batteries prepared by the method.

  2. Causes and Implications of Persistent Atmospheric Carbon Dioxide Biases in Earth System Models

    SciTech Connect (OSTI)

    Hoffman, Forrest M [ORNL] [ORNL; Randerson, James T. [University of California, Irvine] [University of California, Irvine; Arora, Vivek K. [Canadian Centre for Climate Modelling and Analysis, Meteorological Service of Canada] [Canadian Centre for Climate Modelling and Analysis, Meteorological Service of Canada; Bao, Qing [State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics] [State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics; Cadule, Patricia [Institut Pierre Simon Laplace, Laboratoire des Sciences du Climat et de l'Environment] [Institut Pierre Simon Laplace, Laboratoire des Sciences du Climat et de l'Environment; Ji, Duoying [State Key Laboratory of Earth Surface Processes and Resource Ecology, Beijing] [State Key Laboratory of Earth Surface Processes and Resource Ecology, Beijing; Jones, Chris D. [Hadley Centre, U.K. Met Office] [Hadley Centre, U.K. Met Office; Kawamiya, Michio [Japan Agency for Marine-Earth Science and Technology (JAMSTEC)] [Japan Agency for Marine-Earth Science and Technology (JAMSTEC); Khatiwala, Samar [Lamont-Doherty Earth Observatory, Columbia University, Palisades, NY] [Lamont-Doherty Earth Observatory, Columbia University, Palisades, NY; Lindsay, Keith [National Center for Atmospheric Research (NCAR)] [National Center for Atmospheric Research (NCAR); Obata, Atsushi [Meteorological Research Institute, Japan] [Meteorological Research Institute, Japan; Shevliakova, Elena [Princeton University] [Princeton University; Six, Katharina D. [Max Planck Institute for Meteorology, Hamburg, Germany] [Max Planck Institute for Meteorology, Hamburg, Germany; Tjiputra, Jerry F. [Uni Climate, Uni Research] [Uni Climate, Uni Research; Volodin, Evgeny M. [Institute of Numerical Mathematics, Russian Academy of Science, Moscow] [Institute of Numerical Mathematics, Russian Academy of Science, Moscow; Wu, Tongwen [China Meteorological Administration (CMA), Beijing] [China Meteorological Administration (CMA), Beijing

    2014-01-01

    The strength of feedbacks between a changing climate and future CO2 concentrations are uncertain and difficult to predict using Earth System Models (ESMs). We analyzed emission-driven simulations--in which atmospheric CO2 levels were computed prognostically--for historical (1850-2005) and future periods (RCP 8.5 for 2006-2100) produced by 15 ESMs for the Fifth Phase of the Coupled Model Intercomparison Project (CMIP5). Comparison of ESM prognostic atmospheric CO2 over the historical period with observations indicated that ESMs, on average, had a small positive bias in predictions of contemporary atmospheric CO2. Weak ocean carbon uptake in many ESMs contributed to this bias, based on comparisons with observations of ocean and atmospheric anthropogenic carbon inventories. We found a significant linear relationship between contemporary atmospheric CO2 biases and future CO2 levels for the multi-model ensemble. We used this relationship to create a contemporary CO2 tuned model (CCTM) estimate of the atmospheric CO2 trajectory for the 21st century. The CCTM yielded CO2 estimates of 600 {plus minus} 14 ppm at 2060 and 947 {plus minus} 35 ppm at 2100, which were 21 ppm and 32 ppm below the multi-model mean during these two time periods. Using this emergent constraint approach, the likely ranges of future atmospheric CO2, CO2-induced radiative forcing, and CO2-induced temperature increases for the RCP 8.5 scenario were considerably narrowed compared to estimates from the full ESM ensemble. Our analysis provided evidence that much of the model-to-model variation in projected CO2 during the 21st century was tied to biases that existed during the observational era, and that model differences in the representation of concentration-carbon feedbacks and other slowly changing carbon cycle processes appear to be the primary driver of this variability. By improving models to more closely match the long-term time series of CO2 from Mauna Loa, our analysis suggests uncertainties in future climate projections can be reduced.

  3. Prospects for Simulating Macromolecular Surfactant Chemistry at the Ocean-Atmosphere Boundary

    SciTech Connect (OSTI)

    Elliott, S.; Burrows, Susannah M.; Deal, C.; Liu, Xiaohong; Long, M.; Ogunro, O.; Russell, Lynn M.; Wingenter, O.

    2014-05-01

    Biogenic lipids and polymers are surveyed for their ability to adsorb at the water-air interfaces associated with bubbles, marine microlayers and particles in the overlying boundary layer. Representative ocean biogeochemical regimes are defined in order to estimate local concentrations for the major macromolecular classes. Surfactant equilibria and maximum excess are then derived based on a network of model compounds. Relative local coverage and upward mass transport follow directly, and specific chemical structures can be placed into regional rank order. Lipids and denatured protein-like polymers dominate at the selected locations. The assigned monolayer phase states are variable, whether assessed along bubbles or at the atmospheric spray droplet perimeter. Since oceanic film compositions prove to be irregular, effects on gas and organic transfer are expected to exhibit geographic dependence as well. Moreover, the core arguments extend across the sea-air interface into aerosol-cloud systems. Fundamental nascent chemical properties including mass to carbon ratio and density depend strongly on the geochemical state of source waters. High surface pressures may suppress the Kelvin effect, and marine organic hygroscopicities are almost entirely unconstrained. While bubble adsorption provides a well-known means for transporting lipidic or proteinaceous material into sea spray, the same cannot be said of polysaccharides. Carbohydrates tend to be strongly hydrophilic so that their excess carbon mass is low despite stacked polymeric geometries. Since sugars are abundant in the marine aerosol, gel-based mechanisms may be required to achieve uplift. Uncertainties in the surfactant logic distill to a global scale dearth of information regarding two dimensional kinetics and equilibria. Nonetheless simulations are recommended, to initiate the process of systems level quantification.

  4. Atmosphere Model

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    energy balance due to aerosol-radiation interactions, but the effect depends on the dust optical properties assumed in the simulations without mineralogy. More importantly, the...

  5. Pacific Northwest Laboratory: Annual report for 1986 to the DOE Office of Energy Research: Part 3, Atmospheric sciences

    SciTech Connect (OSTI)

    Elderkin, C.E.

    1987-06-01

    The goals of atmospheric research at Pacific Northwest Laboratory (PNL) are to describe and predict the nature and fate of atmospheric contaminants and to develop an understanding of the atmospheric processes contributing to their distribution on local, regional, and continental scales. In 1986, atmospheric research examined the transport and diffusion of atmospheric contaminants in areas of complex terrain and participated in a large, multilaboratory program to assess the precipitation scavenging processes important to the transformation and wet deposition of chemicals composing ''acid rain.'' In addition, during 1986, a special opportunity for measuring the transport and removal of radioactivity occurred after the Chernobyl reactor accident in April 1986. Separate abstracts were prepared for individual projects.

  6. Accurate atmospheric parameters at moderate resolution using spectral indices: Preliminary application to the marvels survey

    SciTech Connect (OSTI)

    Ghezzi, Luan; Da Costa, Luiz N.; Maia, Marcio A. G.; Ogando, Ricardo L. C.; Dutra-Ferreira, Letcia; Lorenzo-Oliveira, Diego; Porto de Mello, Gustavo F.; Santiago, Baslio X.; De Lee, Nathan; Lee, Brian L.; Ge, Jian; Wisniewski, John P.; Gonzlez Hernndez, Jonay I.; Stassun, Keivan G.; Cargile, Phillip; Pepper, Joshua; Fleming, Scott W.; Schneider, Donald P.; Mahadevan, Suvrath; Wang, Ji; and others

    2014-12-01

    Studies of Galactic chemical, and dynamical evolution in the solar neighborhood depend on the availability of precise atmospheric parameters (effective temperature T {sub eff}, metallicity [Fe/H], and surface gravity log g) for solar-type stars. Many large-scale spectroscopic surveys operate at low to moderate spectral resolution for efficiency in observing large samples, which makes the stellar characterization difficult due to the high degree of blending of spectral features. Therefore, most surveys employ spectral synthesis, which is a powerful technique, but relies heavily on the completeness and accuracy of atomic line databases and can yield possibly correlated atmospheric parameters. In this work, we use an alternative method based on spectral indices to determine the atmospheric parameters of a sample of nearby FGK dwarfs and subgiants observed by the MARVELS survey at moderate resolving power (R ? 12,000). To avoid a time-consuming manual analysis, we have developed three codes to automatically normalize the observed spectra, measure the equivalent widths of the indices, and, through a comparison of those with values calculated with predetermined calibrations, estimate the atmospheric parameters of the stars. The calibrations were derived using a sample of 309 stars with precise stellar parameters obtained from the analysis of high-resolution FEROS spectra, permitting the low-resolution equivalent widths to be directly related to the stellar parameters. A validation test of the method was conducted with a sample of 30 MARVELS targets that also have reliable atmospheric parameters derived from the high-resolution spectra and spectroscopic analysis based on the excitation and ionization equilibria method. Our approach was able to recover the parameters within 80 K for T {sub eff}, 0.05 dex for [Fe/H], and 0.15 dex for log g, values that are lower than or equal to the typical external uncertainties found between different high-resolution analyses. An additional test was performed with a subsample of 138 stars from the ELODIE stellar library, and the literature atmospheric parameters were recovered within 125 K for T {sub eff}, 0.10 dex for [Fe/H], and 0.29 dex for log g. These precisions are consistent with or better than those provided by the pipelines of surveys operating with similar resolutions. These results show that the spectral indices are a competitive tool to characterize stars with intermediate resolution spectra.

  7. North America's net terrestrial CO2 exchange with the atmosphere 19902009

    SciTech Connect (OSTI)

    King, Anthony W.; Andres, Robert; Davis, Kenneth J.; Hafer, M.; Hayes, Daniel J.; Huntzinger, Deborah N.; de Jong, Bernardus; Kurz, Werner; McGuire, A. David; Vargas, Rodrigo; Wei, Yaxing; West, Tristram O.; Woodall, Chris W.

    2015-01-21

    Scientific understanding of the global carbon cycle is required for developing national and international policy to mitigate fossil fuel CO2 emissions by managing terrestrial carbon uptake. Toward that understanding and as a contribution to the REgional Carbon Cycle Assessment and Processes (RECCAP) project, this paper provides a synthesis of net landatmosphere CO2 exchange for North America (Canada, United States, and Mexico) over the period 19902009. Only CO2 is considered, not methane or other greenhouse gases. This synthesis is based on results from three different methods: atmospheric inversion, inventory-based methods and terrestrial biosphere modeling. All methods indicate that the North American land surface was a sink for atmospheric CO2, with a net transfer from atmosphere to land. Estimates ranged from -890 to -280 Tg C yr-1, where the mean of atmospheric inversion estimates forms the lower bound of that range (a larger land sink) and the inventory-based estimate using the production approach the upper (a smaller land sink). This relatively large range is due in part to differences in how the approaches represent trade, fire and other disturbances and which ecosystems they include. Integrating across estimates, \\"best\\" estimates (i.e., measures of central tendency) are -472 281 Tg C yr-1 based on the mean and standard deviation of the distribution and -360 Tg C yr-1 (with an interquartile range of -496 to -337) based on the median. Considering both the fossil fuel emissions source and the land sink, our analysis shows that North America was, however, a net contributor to the growth of CO2 in the atmosphere in the late 20th and early 21st century. With North America's mean annual fossil fuel CO2 emissions for the period 19902009 equal to 1720 Tg C yr-1 and assuming the estimate of -472 Tg C yr-1 as an approximation of the true terrestrial CO2 sink, the continent's source : sink ratio for this time period was 1720:472, or nearly 4:1.

  8. Nuclear Emergency and the Atmospheric Dispersion of Nuclear Aerosols: Discussion of the Shared Nuclear Future - 13163

    SciTech Connect (OSTI)

    Rana, Mukhtar A.; Ali, Nawab; Akhter, Parveen; Khan, E.U.; Mathieson, John

    2013-07-01

    This paper has a twofold objective. One is to analyze the current status of high-level nuclear waste disposal along with presentation of practical perspectives about the environmental issues involved. Present disposal designs and concepts are analyzed on a scientific basis and modifications to existing designs are proposed from the perspective of environmental safety. Other is to understand the aerosol formation in the atmosphere for the case of the leakage from the nuclear waste containers or a nuclear accident. Radio-nuclides released from the waste will attach themselves to the existing aerosols in the atmosphere along with formation of new aerosols. Anticipating the nuclear accident when a variety of radioactive aerosols will form and exist in the atmosphere, as a simple example, measurement of naturally existing radioactive aerosols are made in the atmosphere of Islamabad and Murree. A comparison with similar measurements in 3 cities of France is provided. Measurement of radionuclides in the atmosphere, their attachment to aerosols and follow up transport mechanisms are key issues in the nuclear safety. It is studied here how {sup 7}Be concentration in the atmospheric air varies in the capital city of Islamabad and a Himalaya foothill city of Murree (Pakistan). Present results are compared with recent related published results to produce a {sup 7}Be concentration versus altitude plot up to an altitude of 4000 m (a.s.l.). Origin and variance of {sup 7}Be concentration at different altitudes is discussed in detail. The relevance of results presented here with the evaluation of implications of Chernobyl and Fukushima nuclear disasters has been discussed in a conclusive manner. It is the first international report of a joint collaboration/project. The project is being generalized to investigate and formulate a smooth waste storage and disposal policy. The project will address the fission and fusion waste reduction, its storage, its recycling, air, water and soil quality monitoring, and the final disposal with the major foci of dealing with related chemical, biogical, physical, geophysical, engineering, management and administration aspects. (authors)

  9. North America's net terrestrial CO2 exchange with the atmosphere 1990–2009

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    King, Anthony W.; Andres, Robert; Davis, Kenneth J.; Hafer, M.; Hayes, Daniel J.; Huntzinger, Deborah N.; de Jong, Bernardus; Kurz, Werner; McGuire, A. David; Vargas, Rodrigo; et al

    2015-01-21

    Scientific understanding of the global carbon cycle is required for developing national and international policy to mitigate fossil fuel CO2 emissions by managing terrestrial carbon uptake. Toward that understanding and as a contribution to the REgional Carbon Cycle Assessment and Processes (RECCAP) project, this paper provides a synthesis of net land–atmosphere CO2 exchange for North America (Canada, United States, and Mexico) over the period 1990–2009. Only CO2 is considered, not methane or other greenhouse gases. This synthesis is based on results from three different methods: atmospheric inversion, inventory-based methods and terrestrial biosphere modeling. All methods indicate that the North Americanmore » land surface was a sink for atmospheric CO2, with a net transfer from atmosphere to land. Estimates ranged from -890 to -280 Tg C yr-1, where the mean of atmospheric inversion estimates forms the lower bound of that range (a larger land sink) and the inventory-based estimate using the production approach the upper (a smaller land sink). This relatively large range is due in part to differences in how the approaches represent trade, fire and other disturbances and which ecosystems they include. Integrating across estimates, \\"best\\" estimates (i.e., measures of central tendency) are -472 ± 281 Tg C yr-1 based on the mean and standard deviation of the distribution and -360 Tg C yr-1 (with an interquartile range of -496 to -337) based on the median. Considering both the fossil fuel emissions source and the land sink, our analysis shows that North America was, however, a net contributor to the growth of CO2 in the atmosphere in the late 20th and early 21st century. With North America's mean annual fossil fuel CO2 emissions for the period 1990–2009 equal to 1720 Tg C yr-1 and assuming the estimate of -472 Tg C yr-1 as an approximation of the true terrestrial CO2 sink, the continent's source : sink ratio for this time period was 1720:472, or nearly 4:1.« less

  10. Development of the Variable Atmosphere Testing Facility for Blow-Down Analysis of the Mars Hopper Prototype

    SciTech Connect (OSTI)

    Nathan D. Jerred; Robert C. O'Brien; Steven D. Howe; James E. O'Brien

    2013-02-01

    Recent developments at the Center for Space Nuclear Research (CSNR) on a Martian exploration probe have lead to the assembly of a multi-functional variable atmosphere testing facility (VATF). The VATF has been assembled to perform transient blow-down analysis of a radioisotope thermal rocket (RTR) concept that has been proposed for the Mars Hopper; a long-lived, long-ranged mobile platform for the Martian surface. This study discusses the current state of the VATF as well as recent blow-down testing performed on a laboratory-scale prototype of the Mars Hopper. The VATF allows for the simulation of Mars ambient conditions within the pressure vessel as well as to safely perform blow-down tests through the prototype using CO2 gas; the proposed propellant for the Mars Hopper. Empirical data gathered will lead to a better understanding of CO2 behavior and will provide validation of simulation models. Additionally, the potential of the VATF to test varying propulsion system designs has been recognized. In addition to being able to simulate varying atmospheres and blow-down gases for the RTR, it can be fitted to perform high temperature hydrogen testing of fuel elements for nuclear thermal propulsion.

  11. Design, fabrication, and testing of a getter-based atmosphere purification and waste treatment system for a nitrogen-hydrogen-helium glovebox

    SciTech Connect (OSTI)

    Bibeault, M. L.; Paglieri, S. N.; Tuggle, D. G.; Wermer, J. R.; Nobile Jr, A.

    2008-07-15

    A system containing a combination of getters (Zr-Mn-Fe, SAES St909; and Zr{sub 2}Fe, SAES St198) was used to process the nitrogen-hydrogen-helium atmosphere in a glovebox used for handling metal tritide samples. During routine operations, the glovebox atmosphere is recirculated and hydrogenous impurities (i.e. CQ{sub 4}, Q{sub 2}O, and NQ{sub 3}, where Q =H, D, T) are decomposed (cracked) and removed by Zr-Mn-Fe without absorbing elemental hydrogen isotopes. If the tritium content of the glovebox atmosphere becomes unacceptably high, the getter system can rapidly strip the glovebox atmosphere of all hydrogen isotopes by absorption on the Zr{sub 2}Fe, thus lessening the burden on the facility waste gas treatment system. The getter system was designed for high flowrate ( > 100 1/min), which is achieved by using a honeycomb support for the getter pellets and 1.27-cm diameter tubing throughout the system for reduced pressure drop. The novel getter bed design also includes an integral preheater and copper liner to accommodate swelling of the getter pellets, which occurs during loading with oxygen and carbon impurities. Non-tritium functional tests were conducted to determine the gettering efficiencies at different getter bed temperatures and flowrates by recirculating gas through the system from, a 6-m{sup 3} glovebox containing known concentrations of impurities. (authors)

  12. Dynamical and thermodynamical modulations of future changes in landfalling atmospheric rivers over North America

    SciTech Connect (OSTI)

    Gao, Yang; Lu, Jian; Leung, Lai-Yung R.; Yang, Qing; Hagos, Samson M.; Qian, Yun

    2015-09-12

    This study examines the changes of landfalling atmospheric rivers (ARs) over the west coast of North America in response to future warming using model outputs from the Coupled Model Intercomparison Project phase 5 (CMIP5). The result reveals a strikingly large magnitude of increase of AR days by the end of the 21st century in the RCP8.5 climate change scenario, with fractional increases ranging between ~50% and 600%, depending on the seasons and the landfall locations. These increases are predominantly controlled by the super-Clausius-Clapeyron rate of increase of atmospheric water vapor with warming, while changes of winds that transport moisture in the ARs, or dynamical effect, mostly counter the thermodynamical effect of increasing water vapor, limiting the increase of AR events in the future. The consistent negative effect of wind changes on AR days during spring and fall can be further linked to the robust poleward shift of the subtropical jet in the North Pacific basin.

  13. DETECTING INDUSTRIAL POLLUTION IN THE ATMOSPHERES OF EARTH-LIKE EXOPLANETS

    SciTech Connect (OSTI)

    Lin, Henry W.; Abad, Gonzalo Gonzalez; Loeb, Abraham E-mail: ggonzalezabad@cfa.harvard.edu

    2014-09-01

    Detecting biosignatures, such as molecular oxygen in combination with a reducing gas, in the atmospheres of transiting exoplanets has been a major focus in the search for alien life. We point out that in addition to these generic indicators, anthropogenic pollution could be used as a novel biosignature for intelligent life. To this end, we identify pollutants in the Earth's atmosphere that have significant absorption features in the spectral range covered by the James Webb Space Telescope. We focus on tetrafluoromethane (CF{sub 4}) and trichlorofluoromethane (CCl{sub 3}F), which are the easiest to detect chlorofluorocarbons (CFCs) produced by anthropogenic activity. We estimate that ?1.2 days (?1.7 days) of total integration time will be sufficient to detect or constrain the concentration of CCl{sub 3}F (CF{sub 4}) to ?10 times the current terrestrial level.

  14. The purification of inert glove box atmospheres using hot reactive metals

    SciTech Connect (OSTI)

    Johnson, R.E.; Gravelle, F.B.; Shultz, C.M.

    1988-09-01

    Current practice for the handling of pure tritium gas involves the use of inert atmosphere glove boxes. The purity of the inert gas is maintained by recirculation through a purification system. Due to the high toxicity of tritium in the form of water it is desirable to avoid oxidation of the elemental tritium and to remove tritium by forming stable metal tritides. This paper describes the use of SAES ST707 Alloy for the removal of hydrogen from a glove box atmosphere and briefly relates largely unsuccessful attempts at hydrogen removal using a variety of metals and alloys. The details of a proposed purification system for the control of chronic tritium releases and for the collection and recovery of a large tritium release are presented.

  15. Plant Response and Environmental Data from the Oldfield Community Climate and Atmospheric Manipulation (OCCAM) Project

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    The Oldfield Community Climate and Atmospheric Manipulation (OCCAM) project is a joint effort of ORNL and the University of Tennessee to investigate community and ecosystem response to global change, specifically looking at the interactive effects of atmospheric carbon dioxide, surface temperatures, and soil moisture. The plants studied for their response to warming temperatures, elevated carbon dioxide, and altered water availability include C3 and C4 grasses, forbs, and legumes. These plants are typical of an old-field ecosystem that establishes itself on unused agricultural land. The results of the research focus on species abundance, production, phenology, and what is going on chemically below ground. Data are currently available from 2003 through July, 2008.

  16. Production of extremely low volatile organic compounds from biogenic emissions: Measured yields and atmospheric implications

    SciTech Connect (OSTI)

    Jokinen, Tuija; Berndt, Torsten; Makkonen, Risto; Kerminen, Veli-Matti; Junninen, Heikki; Paasonen, Pauli; Stratmann, Frank; Herrmann, Hartmut; Guenther, Alex B.; Worsnop, Douglas R.; Kulmala, M.; Ehn, Mikael K.; Sipila, Mikko

    2015-06-09

    Extremely low volatility organic compounds (ELVOC) are suggested to promote aerosol particle formation and cloud condensation nuclei (CCN) production in the atmosphere. We show that the capability of biogenic VOC (BVOC) to produce ELVOC depends strongly on their chemical structure and relative oxidant levels. BVOC with an endocyclic double bond, representative emissions from, e.g., boreal forests, efficiently produce ELVOC from ozonolysis. Compounds with exocyclic double bonds or acyclic compounds including isoprene, emission representative of the tropics, produce minor quantities of ELVOC, and the role of OH radical oxidation is relatively larger. Implementing these findings into a global modeling framework shows that detailed assessment of ELVOC production pathways is crucial for understanding biogenic secondary organic aerosol and atmospheric CCN formation.

  17. Spectrometer for Sky-Scanning Sun-Tracking Atmospheric Research (4STAR): Instrument Technology

    SciTech Connect (OSTI)

    Dunagan, Stephen; Johnson, Roy; Zavaleta, Jhony; Russell, P. B.; Schmid, Beat; Flynn, Connor J.; Redemann, Jens; Shinozuka, Yohei; Livingston, J.; Segal Rozenhaimer, Michal

    2013-08-06

    The Spectrometer for Sky-Scanning, Sun-Tracking Atmospheric Research (4STAR) combines airborne sun tracking and sky scanning with diffraction spectroscopy, to improve knowledge of atmospheric constituents and their links to air-pollution/climate. Direct beam hyper-spectral measurement of optical depth improves retrievals of gas constituents and determination of aerosol properties. Sky scanning enhances retrievals of aerosol type and size distribution. 4STAR measurements will tighten the closure between satellite and ground-based measurements. 4STAR incorporates a modular sun-tracking/ sky-scanning optical head with fiber optic signal transmission to rack mounted spectrometers, permitting miniaturization of the external optical head, and future detector evolution. Technical challenges include compact optical collector design, radiometric dynamic range and stability, and broad spectral coverage. Test results establishing the performance of the instrument against the full range of operational requirements are presented, along with calibration, engineering flight test, and scientific field campaign data and results.

  18. ANALYTICAL SOLUTION FOR WAVES IN PLANETS WITH ATMOSPHERIC SUPERROTATION. I. ACOUSTIC AND INERTIA-GRAVITY WAVES

    SciTech Connect (OSTI)

    Peralta, J.; Lpez-Valverde, M. A.; Imamura, T.; Read, P. L.; Luz, D.; Piccialli, A.

    2014-07-01

    This paper is the first of a two-part study devoted to developing tools for a systematic classification of the wide variety of atmospheric waves expected on slowly rotating planets with atmospheric superrotation. Starting with the primitive equations for a cyclostrophic regime, we have deduced the analytical solution for the possible waves, simultaneously including the effect of the metric terms for the centrifugal force and the meridional shear of the background wind. In those cases when the conditions for the method of the multiple scales in height are met, these wave solutions are also valid when vertical shear of the background wind is present. A total of six types of waves have been found and their properties were characterized in terms of the corresponding dispersion relations and wave structures. In this first part, only waves that are direct solutions of the generic dispersion relation are studiedacoustic and inertia-gravity waves. Concerning inertia-gravity waves, we found that in the cases of short horizontal wavelengths, null background wind, or propagation in the equatorial region, only pure gravity waves are possible, while for the limit of large horizontal wavelengths and/or null static stability, the waves are inertial. The correspondence between classical atmospheric approximations and wave filtering has been examined too, and we carried out a classification of the mesoscale waves found in the clouds of Venus at different vertical levels of its atmosphere. Finally, the classification of waves in exoplanets is discussed and we provide a list of possible candidates with cyclostrophic regimes.

  19. Proposed ground-based incoherent Doppler lidar with iodine filter discriminator for atmospheric wind profiling

    SciTech Connect (OSTI)

    Liu, Z.S.; Chen, W.B.; Hair, J.W.; She, C.Y.

    1996-12-31

    A new incoherent lidar for measuring atmospheric wind using iodine molecular filter is proposed. A unique feature of the proposed lidar lies in its capability for simultaneous measurement of aerosol mixing ratio, with which the radial wind can be determined uniquely from lidar return. A preliminary laboratory experiment using a dye laser at 589 nm and a rotating wheel has been performed demonstrating the feasibility of the proposed wind measurement.

  20. National Oceanic and Atmospheric Administration Provides Forecasting Support for CLASIC and CHAPS 2007

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    NOAA Provides Forecasting Support for CLASIC and CHAPS 2007 Forecasting Challenge While weather experiments in the heart of Tornado Alley typically focus on severe weather, the CLASIC and CHAPS programs will have different emphases. Forecasters from the National Oceanic and Atmospheric Administration in Norman, Okla. will provide weather forecasting support to these two Department of Energy experiments based in the state. Forecasting support for meteorological research field programs usually

  1. Gulf Stream Locale R. J. Alliss and S. Raman Department of Marine, Earth and Atmospheric Sciences

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    R. J. Alliss and S. Raman Department of Marine, Earth and Atmospheric Sciences North Carolina State University Raleigh, NC 27695-8208 Introduction Clouds have long been recognized as having a major impact on the radiation budget in the earth's climate system. One of the preferred areas for the production of clouds is off the east coast of the United States. The formation of clouds in this region, particularly during the winter months, is caused predominately by the presence of the Gulf Stream,

  2. A moist aquaplanet variant of the HeldSuarez test for atmospheric model dynamical cores

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Thatcher, D. R.; Jablonowski, C.

    2015-09-29

    A moist idealized test case (MITC) for atmospheric model dynamical cores is presented. The MITC is based on the HeldSuarez (HS) test that was developed for dry simulations on a flat Earth and replaces the full physical parameterization package with a Newtonian temperature relaxation and Rayleigh damping of the low-level winds. This new variant of the HS test includes moisture and thereby sheds light on the non-linear dynamics-physics moisture feedbacks without the complexity of full physics parameterization packages. In particular, it adds simplified moist processes to the HS forcing to model large-scale condensation, boundary layer mixing, and the exchange ofmorelatent and sensible heat between the atmospheric surface and an ocean-covered planet. Using a variety of dynamical cores of NCAR's Community Atmosphere Model (CAM), this paper demonstrates that the inclusion of the moist idealized physics package leads to climatic states that closely resemble aquaplanet simulations with complex physical parameterizations. This establishes that the MITC approach generates reasonable atmospheric circulations and can be used for a broad range of scientific investigations. This paper provides examples of two application areas. First, the test case reveals the characteristics of the physics-dynamics coupling technique and reproduces coupling issues seen in full-physics simulations. In particular, it is shown that sudden adjustments of the prognostic fields due to moist physics tendencies can trigger undesirable large-scale gravity waves, which can be remedied by a more gradual application of the physical forcing. Second, the moist idealized test case can be used to intercompare dynamical cores. These examples demonstrate the versatility of the MITC approach and suggestions are made for further application areas. The new moist variant of the HS test can be considered a test case of intermediate complexity.less

  3. Rice straw burning in Southeast Asia as a source of CO and COS to the atmosphere

    SciTech Connect (OSTI)

    Nguyen, B.C.; Mihalopoulos, N.; Putaud, J.P. [Centre des Faibles Radioactivites, Gif-sur-Yvette (France)

    1994-08-20

    This paper discusses the results of aerosol monitoring field tests conducted in four locations in Viet Nam during 1992 and 1993. Atmospheric samples were collected during the dry and wet seasons during the time when rice straw burning was taking place in the agricultural rangelands. The samples were analyzed for carbon monoxide, carbon dioxide, and carbonyl sulfide. Experimental methods and implications of the analytical results are described. 21 refs., 2 figs., 3 tabs.

  4. Reactivity of liquid and semisolid secondary organic carbon with chloride and nitrate in atmospheric aerosols

    SciTech Connect (OSTI)

    Wang, Bingbing; O'Brien, Rachel E.; Kelly, Stephen T.; Shilling, John E.; Moffet, Ryan C.; Gilles, Mary K.; Laskin, Alexander

    2015-05-14

    Constituents of secondary organic carbon (SOC) in atmospheric aerosols are often mixed with inorganic components and compose a significant mass fraction of fine particulate matter in the atmosphere. Interactions between SOC and other condensed-phase species are not well understood. Here, we investigate the reactions of liquid-like and semi-solid SOC from ozonolysis of limonene (LSOC) and ?-pinene (PSOC) with NaCl using a set of complementary micro-spectroscopic analyses. These reactions result in chloride depletion in the condensed phase, release of gaseous HCl, and formation of organic salts. The reactions attributed to acid displacement by SOC acidic components are driven by the high volatility of HCl. Similar reactions can take place in SOC/NaNO? particles. The results show that an increase in SOC mass fraction in the internally mixed SOC/NaCl particles leads to higher chloride depletion. Glass transition temperatures and viscosity of PSOC were estimated for atmospherically relevant conditions. Data show that the reaction extent depends on SOC composition, particle phase state and viscosity, mixing state, temperature, relative humidity (RH), and reaction time. LSOC shows slightly higher potential to deplete chloride than PSOC. Higher particle viscosity at low temperatures and RH can hinder these acid displacement reactions. Formation of organic salts from these overlooked reactions can alter particle physiochemical properties and may affect their reactivity and ability to act as cloud condensation and ice nuclei. The release and potential recycling of HCl and HNO? from reacted aerosol particles may have important implications for atmospheric chemistry.

  5. DOE/SC-ARM-14-034 Lower Atmospheric Boundary Layer Experiment

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    4 Lower Atmospheric Boundary Layer Experiment (LABLE) Final Campaign Report P Klein WG Blumberg TA Bonin S Mishra JF Newman M Carney DD Turner EP Jacobsen PB Chilson S Wharton CE Wainwright RK Newsom November 2014 DISCLAIMER This report was prepared as an account of work sponsored by the U.S. Government. Neither the United States nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy,

  6. DOE/SC-ARM-15-027 Radon Measurements of Atmospheric Mixing

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    7 Radon Measurements of Atmospheric Mixing (RAMIX) 2006-2014 Final Campaign Summary ML Fischer SC Biraud A Hirsch May 2015 DISCLAIMER This report was prepared as an account of work sponsored by the U.S. Government. Neither the United States nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or

  7. Evaluation of Routine Atmospheric Sounding Measurements using Unmanned Systems (ERASMUS) Science Plan

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    8 Evaluation of Routine Atmospheric Sounding Measurements using Unmanned Systems (ERASMUS) Science Plan G de Boer B Argrow G Bland J Elston D Lawrence J Maslanik S Palo M Tschudi December 2015 DISCLAIMER This report was prepared as an account of work sponsored by the U.S. Government. Neither the United States nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of

  8. Four-Dimensional Data Assimilation J.-F. Louis Atmospheric and Environmental Research, Inc.

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    J.-F. Louis Atmospheric and Environmental Research, Inc. Cambridge, MA 02139 The main purpose of the ARM program is to provide the necessary data to develop, test and validate the parameterization of clouds and of their interactions with the radiation field, and the computation of radiative transfer in climate models. For the most part, however, the ARM observations will be imperfect, incomplete, redundant, indirect, and unrepresentative. This is unavoidable, despite the best efforts at

  9. Chlorinated dibenzofurans and dioxins in atmospheric samples from cities in New York

    SciTech Connect (OSTI)

    Smith, R.M.; O'Keefe, P.W.; Aldous, K.M.; Valente, H.; Connor, S.P.; Donnelly, R.J. )

    1990-10-01

    Chlorinated dibenzofurans and chlorinated dibenzo-p-dioxins were detected in air samples from Albany, Binghamton, Utica, and Niagara Falls, NY, in concentrations ranging up to 8.8 pg/m{sup 3}. The air results showed a variety of homologue distributions including a previously unreported one dominated by lower chlorinated CDFs, which may result following particulate fallout. Other results were more typical of urban and suburban air that is subject to the processes of atmospheric aging as reported in the literature.

  10. Interpretation of AIRS Data in Thin Cirrus Atmospheres Based on a Fast

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Radiative Transfer Model and ARM Data Interpretation of AIRS Data in Thin Cirrus Atmospheres Based on a Fast Radiative Transfer Model and ARM Data Yue, Qing Dept. of Atomspheric & Oceanic Sciences, UCLA Liou, Kuo-Nan UCLA Ou, Szu-cheng University of California, Los Angeles Kahn, Brian Jet Propulsion Laboratory Yang, Ping Texas A&M Mace, Gerald University of Utah Category: Radiation A thin cirrus cloud thermal infrared radiative transfer model has been developed to interpret AIRS

  11. Method of Enhancing the Signal at the Atmosphere Produced by an Electron

    Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

    Beam Injected from an Earth Orbiting Spacecraft | Princeton Plasma Physics Lab of Enhancing the Signal at the Atmosphere Produced by an Electron Beam Injected from an Earth Orbiting Spacecraft One of the most important problems in space research, whose solution is also of high value to today's society which relies more and more on the reliability of the communication satellites, is mapping of the magnetic field lines in the Earth's magnetosphere. Obtaining such mapping is however technically

  12. Continuous Profiles of Cloud Microphysical Properties for the Fixed Atmospheric Radiation Measurement Sites

    SciTech Connect (OSTI)

    Jensen, M; Jensen, K

    2006-06-01

    The Atmospheric Radiation Measurement (ARM) Program defined a specific metric for the third quarter of Fiscal Year 2006 to produce and refine a one-year continuous time series of cloud microphysical properties based on cloud radar measurements for each of the fixed ARM sites. To accomplish this metric, we used a combination of recently developed algorithms that interpret radar reflectivity profiles, lidar backscatter profiles, and microwave brightness temperatures into the context of the underlying cloud microphysical structure.

  13. Evaluation of Routine Atmospheric Sounding Measurements using Unmanned Systems (ERASMUS) Science Plan

    SciTech Connect (OSTI)

    de Boer, G; Bland, G; Elston, J; Lawrence, D; Maslanik, J; Palo, S; Tschudi, M

    2015-12-01

    The use of unmanned aerial systems (UAS) is becoming increasingly popular for a variety of applications. One way in which these systems can provide revolutionary scientific information is through routine measurement of atmospheric conditions, particularly properties related to clouds, aerosols, and radiation. Improved understanding of these topics at high latitudes, in particular, has become very relevant because of observed decreases in ice and snow in polar regions.

  14. Staggered-grid finite-difference acoustic modeling with the Time-Domain Atmospheric Acoustic Propagation Suite (TDAAPS).

    SciTech Connect (OSTI)

    Aldridge, David Franklin; Collier, Sandra L.; Marlin, David H.; Ostashev, Vladimir E.; Symons, Neill Phillip; Wilson, D. Keith

    2005-05-01

    This document is intended to serve as a users guide for the time-domain atmospheric acoustic propagation suite (TDAAPS) program developed as part of the Department of Defense High-Performance Modernization Office (HPCMP) Common High-Performance Computing Scalable Software Initiative (CHSSI). TDAAPS performs staggered-grid finite-difference modeling of the acoustic velocity-pressure system with the incorporation of spatially inhomogeneous winds. Wherever practical the control structure of the codes are written in C++ using an object oriented design. Sections of code where a large number of calculations are required are written in C or F77 in order to enable better compiler optimization of these sections. The TDAAPS program conforms to a UNIX style calling interface. Most of the actions of the codes are controlled by adding flags to the invoking command line. This document presents a large number of examples and provides new users with the necessary background to perform acoustic modeling with TDAAPS.

  15. Aqueous Processing of Atmospheric Organic Particles in Cloud Water Collected via Aircraft Sampling

    SciTech Connect (OSTI)

    Boone, Eric J.; Laskin, Alexander; Laskin, Julia; Wirth, Christopher; Shepson, Paul B.; Stirm, Brian H.; Pratt, Kerri A.

    2015-07-21

    Cloud water and below-cloud atmospheric particle samples were collected onboard a research aircraft during the Southern Oxidant and Aerosol Study (SOAS) over a forested region of Alabama in June 2013. The organic molecular composition of the samples was studied to gain insights into the aqueous-phase processing of organic compounds within cloud droplets. High resolution mass spectrometry with nanospray desorption electrospray ionization and direct infusion electrospray ionization were utilized to compare the organic composition of the particle and cloud water samples, respectively. Isoprene and monoterpene-derived organosulfates and oligomers were identified in both the particles and cloud water, showing the significant influence of biogenic volatile organic compound oxidation above the forested region. While the average O:C ratios of the organic compounds were similar between the atmospheric particle and cloud water samples, the chemical composition of these samples was quite different. Specifically, hydrolysis of organosulfates and formation of nitrogen-containing compounds were observed for the cloud water when compared to the atmospheric particle samples, demonstrating that cloud processing changes the composition of organic aerosol.

  16. Development of NEXRAD Wind Retrievals as Input to Atmospheric Dispersion Models

    SciTech Connect (OSTI)

    Fast, Jerome D.; Newsom, Rob K.; Allwine, K Jerry; Xu, Qin; Zhang, Pengfei; Copeland, Jeffrey H.; Sun, Jenny

    2007-03-06

    The objective of this study is to determine the feasibility that routinely collected data from the Doppler radars can appropriately be used in Atmospheric Dispersion Models (ADMs) for emergency response. We have evaluated the computational efficiency and accuracy of two variational mathematical techniques that derive the u- and v-components of the wind from radial velocities obtained from Doppler radars. A review of the scientific literature indicated that the techniques employ significantly different approaches in applying the variational techniques: 2-D Variational (2DVar), developed by NOAAs (National Oceanic and Atmospheric Administration's) National Severe Storms Laboratory (NSSL) and Variational Doppler Radar Analysis System (VDRAS), developed by the National Center for Atmospheric Research (NCAR). We designed a series of numerical experiments in which both models employed the same horizontal domain and resolution encompassing Oklahoma City for a two-week period during the summer of 2003 so that the computed wind retrievals could be fairly compared. Both models ran faster than real-time on a typical single dual-processor computer, indicating that they could be used to generate wind retrievals in near real-time. 2DVar executed ~2.5 times faster than VDRAS because of its simpler approach.

  17. Forcing, feedbacks and climate sensitivity in CMIP5 coupled atmosphere-ocean climate models

    DOE Public Access Gateway for Energy & Science Beta (PAGES Beta)

    Andrews, Timothy; Gregory, Jonathan M.; Webb, Mark J.; Taylor, Karl E.

    2012-05-15

    We quantify forcing and feedbacks across available CMIP5 coupled atmosphere-ocean general circulation models (AOGCMs) by analysing simulations forced by an abrupt quadrupling of atmospheric carbon dioxide concentration. This is the first application of the linear forcing-feedback regression analysis of Gregory et al. (2004) to an ensemble of AOGCMs. The range of equilibrium climate sensitivity is 2.1–4.7 K. Differences in cloud feedbacks continue to be important contributors to this range. Some models show small deviations from a linear dependence of top-of-atmosphere radiative fluxes on global surface temperature change. We show that this phenomenon largely arises from shortwave cloud radiative effects overmore » the ocean and is consistent with independent estimates of forcing using fixed sea-surface temperature methods. Moreover, we suggest that future research should focus more on understanding transient climate change, including any time-scale dependence of the forcing and/or feedback, rather than on the equilibrium response to large instantaneous forcing.« less

  18. Coal Fly Ash as a Source of Iron in Atmospheric Dust

    SciTech Connect (OSTI)

    Chen, Haihan; Laskin, Alexander; Baltrusaitis, Jonas; Gorski, Christopher A.; Scherer, Michelle; Grassian, Vicki H.

    2012-01-18

    Anthropogenic coal fly ash aerosols may represent a significant source of bioavailable iron in the open ocean. Few measurements have been made to compare the solubility of atmospheric iron from anthropogenic aerosols and other sources. We report an investigation of the iron dissolution of three fly ash samples in acidic aqueous solutions and compare the solubilities with that of Arizona test dust, a reference material of mineral dust. The effects of pH, cloud processing, and solar irradiation on Fe solubility were explored. Similar to previously reported results on mineral dust, iron in aluminosilicate phases provide predominant dissolved iron compared with iron in oxides. Iron solubility of fly ash is higher than Arizona test dust, especially at the higher pH conditions investigated. Simulated atmospheric processing elevates iron solubility due to significant changes in the morphology aluminosilicate glass, a dominantly material in fly ash particle. Iron continuously releases into the aqueous solution as fly ash particles break up into smaller fragments. The assessment of dissolved atmospheric iron deposition fluxes, and their effect on the biogeochemistry at ocean surface should be constrained by taking into account the source, environment pH, Fe speciation, and solar radiation.

  19. Atmospheric Radiation Measurement (ARM) Data from Specific Instruments Used in the ARM Program

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    ARM is known for its comprehensive set of world-class, and in some cases, unique, instruments available for use by the global scientific community. In addition to the ARM instruments, the ARM Climate Research Facility identifies and acquires a wide variety of data including model, satellite, and surface data, from "external instruments," to augment the data being generated within the program. External instruments belong to organizations that are outside of the ARM Program. Field campaign instruments are another source of data used to augment routine observations. The huge archive of ARM data can be organized by instrument categories into twelve "collections:" Aerosols, Airborne Observations, Atmospheric Carbon, Atmospheric Profiling, Cloud Properties, Derived Quantities and Models, Ocean Observations, Radiometric, Satellite Observations, Surface Meteorology, Surface/Subsurface Properties, and Other. Clicking on one of the instrument categories leads to a page that breaks that category down into sub-categories. For example, "Atmospheric Profiling" is broken down into ARM instruments (with 11 subsets), External Instruments (with 6 subsets), and Field Campaign Instruments (with 42 subsets). Each of the subset links, in turn, leads to detailed information pages and links to specific data streams. Users will be requested to create a password, but the data files are free for viewing and downloading.

  20. Atmospheric Radiation Measurement (ARM) Data from the ARM Specific Measurement Categories

    DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

    The ARM Program gathers a wide variety of measurements from many different sources. Each day, the Data Archive stores and distributes large quantities of data collected from these sources. Scientists then use these data to research atmospheric radiation balance and cloud feedback processes, which are critical elements of global climate change. The huge archive of ARM data can be organized by measurement categories into six "collections:" Aerosols, Atmospheric Carbon, Atmospheric State, Cloud Properties, Radiometric, and Surface Properties. Clicking on one of the measurement categories leads to a page that breaks that category down into sub-categories. For example, "Aerosols" is broken down into Microphysical and Chemical Properties (with 9 subsets) and Optical and Radiative Properties (with 7 subsets). Each of the subset links, in turn, leads to detailed information pages and links to specific data streams. Users will be requested to create a password, but the data files are free for viewing and downloading. The ARM Archive physically resides at the Oak Ridge National Laboratory.