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We encourage you to perform a real-time search of NLEBeta
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1

Atmospheric Concentrations of CO2 from Mauna Loa, Hawaii  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Atmospheric Concentrations of CO2 from Mauna Loa, Hawaii Atmospheric Concentrations of CO2 from Mauna Loa, Hawaii The graphs on this page are generated from data taken from "Trends in Carbon Dioxide" page on the Department of Commerce/National Oceanic and Atmospheric Administration (NOAA) website. The NOAA website presents monthly and weekly atmospheric CO2 concentrations measured at the Mauna Loa Observatory in Hawaii. It offers weekly and monthly data, additional graphs, analysis, descriptions of how the data are collected, and an animation of historical changes in atmospheric CO2. Mauna Loa constitutes the longest record of direct measurements of CO2 in the atmosphere. The measurents were started by C. David Keeling of the Scripps Institution of Oceanography in March of 1958. Recent Monthly Average CO2

2

If Anthropogenic CO2 Emissions Cease, Will Atmospheric CO2 Concentration Continue to Increase?  

Science Journals Connector (OSTI)

If anthropogenic CO2 emissions were to suddenly cease, the evolution of the atmospheric CO2 concentration would depend on the magnitude and sign of natural carbon sources and sinks. Experiments using Earth system models indicate that the overall ...

Andrew H. MacDougall; Michael Eby; Andrew J. Weaver

2013-12-01T23:59:59.000Z

3

Leaf isoprene emission rate as a function of atmospheric CO2 concentration  

E-Print Network [OSTI]

Leaf isoprene emission rate as a function of atmospheric CO2 concentration M I C H A E L J . W I L not show an increase in isoprene emission at the lowest CO2 concentration. However, isoprene emission rates exhibited a 30­40% reduction in isoprene emission rate when grown at 800 ppmv CO2, compared with 400 ppmv CO

Jackson, Robert B.

4

THE INCREASING CONCENTRATION OF ATMOSPHERIC CO2: HOW MUCH, WHEN, AND WHY?  

E-Print Network [OSTI]

consequence of the varying ratio of H to C is that different fuels have different rates of CO2 emissions per emissions when fuel consumption is expressed in energy units. Table 1: CO2 Emission Rates for Fossil community has achieved a broad consensus that: 1.) the atmospheric concentration of carbon dioxide (CO2

5

Atmospheric CO2 Concentrations from Aircraft for 1972-1981, CSIRO  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Atmospheric Trace Gases » CO2 » Concentrations from Aircraft for Atmospheric Trace Gases » CO2 » Concentrations from Aircraft for 1972-1981 Atmospheric CO2 Concentrations from Aircraft for 1972-1981, CSIRO Monitoring Program DOI: 10.3334/CDIAC/atg.ndp007 data Data (NDP-007) PDF PDF Investigators D. J. Beardsmore and G. I. Pearman Methods From 1972 through 1981, air samples were collected in glass flasks from aircraft at a variety of latitudes and altitudes over Australia, New Zealand, and Antarctica. The samples were analyzed for CO2 concentrations with nondispersive infrared gas analysis. The resulting data contain the sampling dates, type of aircraft, flight number, flask identification number, sampling time, geographic sector, distance in kilometers from the listed distance measuring equipment (DME) station, station number of the

6

Technical Report: Influence of an enhanced use of biomass for energy on the CO2 concentration in the atmosphere  

Science Journals Connector (OSTI)

In this study, the influence of different strategies of 'biomass for energy' was modelled by means of a global carbon cycle model in order to compute the annual atmospheric CO2 concentration until the year 2100. A 'Combined Energy and Biosphere Model' was developed on the basis of the Osnabrck Biosphere Model (OBM).

Gilbert Ahamer

1994-01-01T23:59:59.000Z

7

Airborne CO2 DIAL measurement of atmospheric tracer gas concentration distributions  

Science Journals Connector (OSTI)

An airborne differential absorption lidar system employing high-energy line-tunable CO2 lasers has been used to map cross-plume vertical distributions resulting from a...

Uthe, Edward E

1986-01-01T23:59:59.000Z

8

The response of soil CO2 ux to changes in atmospheric CO2, nitrogen supply and plant diversity  

E-Print Network [OSTI]

three major anthropogenic global changes: atmos- pheric carbon dioxide (CO2) concentration, nitrogen (N atmospheric carbon dioxide (CO2) concentra- tions, increasing rates of nitrogen (N) deposition, and decliningThe response of soil CO2 ¯ux to changes in atmospheric CO2, nitrogen supply and plant diversity J O

Minnesota, University of

9

RESPONSES OF PRIMARY PRODUCTION AND TOTAL CARBON STORAGE TO CHANGES IN CLIMATE AND ATMOSPHERIC CO2 CONCENTRATION  

E-Print Network [OSTI]

Model (TEM, version 4.0) to estimate global responses of annual net primary production (NPP) and total. For contemporary climate with 315 ppmv CO2, TEM estimated that global NPP is 47.9 PgC/yr and global total carbon-q climate and +20.6% (9.9 PgC/yr) for the GISS climate. The responses of global total carbon storage are +17

10

Observations and simulations of synoptic, regional, and local variations in atmospheric CO2  

E-Print Network [OSTI]

Observations and simulations of synoptic, regional, and local variations in atmospheric CO2 Jih] Synoptic events may play an important role in determining the CO2 spatial distribution and temporal 2001, which had the most significant CO2 concentration variation in our case pool. The CO2

Collett Jr., Jeffrey L.

11

A 40-million-year history of atmospheric CO2  

Science Journals Connector (OSTI)

...40-million-year history of atmospheric CO2 Yi Ge Zhang 1 Mark Pagani 1 Zhonghui Liu...Pleistocene epochs). The present long-term CO2 record is a composite of data from multiple...growth conditions that potentially bias CO2 results. In this study, we present a pCO2...

2013-01-01T23:59:59.000Z

12

Falsification Of The Atmospheric CO2 Greenhouse Effects  

E-Print Network [OSTI]

Falsification Of The Atmospheric CO2 Greenhouse Effects Within The Frame Of Physics Version 4 Gerlich and Ralf D. Tscheuschner Abstract The atmospheric greenhouse effect, an idea that many authors Of The Atmospheric CO2 Greenhouse Effects . . . 3 Contents Abstract 2 1 Introduction 6 1.1 Problem background

Learned, John

13

Monitoring and interpreting the ocean uptake of atmospheric CO2  

Science Journals Connector (OSTI)

...interpreting the ocean uptake of atmospheric CO2 Andrew J. Watson 1 * Nicolas Metzl 2 Ute...important sink for anthropogenically produced CO2, and on time scales longer than a century they will be the main repository for the CO2 that humans are emitting. Our knowledge...

2011-01-01T23:59:59.000Z

14

Photosynthetic Traits in Wheat Grown under Decreased and Increased CO2 Concentration, and after Transfer to Natural CO2 concentration  

Science Journals Connector (OSTI)

Wheat plants were grown from sowing to day 18 in 26-dm3 chambers at three different CO2 concentrations: 150 (-CO2), 350 (C, control), 800 (+CO2) ?mol mol-1. Afterwards, plants of the three variants were grown at ...

P. Ulman; J. ?atsk; J. Pospilov

2000-08-01T23:59:59.000Z

15

Atmospheric CO2 From Flask Air Samples at 10 Sites in the SIO Air Sampling  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Flask Air Samples, SIO Network Flask Air Samples, SIO Network Atmospheric CO2 From Flask Air Samples at 10 Sites in the SIO Air Sampling Network Scripps Institution of Oceanography Monitoring Sites Scripps Institution of Oceanography Monitoring Sites Mauna Loa, Hawaii Mauna Loa weekly average CO2 concentrations derived from continuous air samples Barrow, Alaska American Samoa South Pole Daily average CO2 concentrations derived from continuous air samples Alert, NWT, Canada Cape Kumukahi Christmas Island Baring Head Kermadec Island La Jolla Pier La Jolla Pier weekly average CO2 concentrations derived from continuous air samples PDF Documentation available as Atmospheric Carbon Dioxide Concentrations at 10 Locations Spanning Latitudes 82°N to 90°S, (NDP-001a) For information on calibration and some additional literature, go to

16

Modern Records of Atmospheric Carbon Dioxide (CO2) and a 2000-year Ice-core  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Carbon Dioxide (CO2) » Ice Cores Carbon Dioxide (CO2) » Ice Cores Modern Records of Atmospheric Carbon Dioxide (CO2) and a 2000-year Ice-core Record from Law Dome, Antarctica Introduction This page provides an introduction and links to records of atmospheric carbon dioxide (CO2) concentrations over the last 2000 years, emphasizing large data bases each representing many currently active stations. Records since about 1960 (depending on location) have been obtained from samples of ambient-air at remote stations, which represent changing global atmospheric concentrations rather than influences of local sources. The longer (2000-year) record is from the Law Dome ice core in Antarctica. The ice-core record has been merged with modern annual data from Cape Grim, Tasmania to provide a 2000-year record ending with the most recent data. A

17

CO2 sorption and reaction kinetic performance of K2CO3/AC in low temperature and CO2 concentration  

Science Journals Connector (OSTI)

Abstract Reducing or removing CO2 is critical to the confined spaces such as submarines, space-crafts or aircrafts while using solid sorbents has been regarded as a promising method. In this work, K2CO3 loaded on activated carbon (K2CO3/AC) was developed as a new and regenerable sorbent for CO2 removing in confined spaces. CO2 sorption performances of K2CO3/AC were investigated under different conditions by varying the K2CO3 loadings, CO2 concentrations, H2O concentrations, CO2 sorption temperatures and water pretreatment durations as well as the purge gas flow rates. The CO2 sorption capacity and carbonation conversion of K2CO3/AC decrease with increasing temperature and increase with increasing mole ratio of H2O concentration over CO2 concentration. Sufficient water vapor pretreatment is found to be beneficial to the sorption-enhanced performance. Increasing flow rate will weaken the CO2 sorption performance. The carbonation kinetics was also investigated with the correlation between the shrinking core model and experimental data. Additionally, the sorbent is proved to be regenerable and stable during 20-cycle CO2 sorptiondesorption experiments. K2CO3/AC presents high carbonation conversion efficiency, high thermal stability, and low dependency on CO2 partial pressure. Therefore, it can be considered as a new option for CO2 removal in confined spaces.

Yafei Guo; Chuanwen Zhao; Changhai Li; Ye Wu

2015-01-01T23:59:59.000Z

18

Decarbonization and the time-delay between peak CO2 emissions and concentrations  

E-Print Network [OSTI]

Carbon-dioxide (CO2) is the main contributor to anthropogenic global warming, and the timing of its peak concentration in the atmosphere is likely to govern the timing of maximum radiative forcing. While dynamics of atmospheric CO2 is governed by multiple time-constants, we idealize this by a single time-constant to consider some of the factors describing the time-delay between peaks in CO2 emissions and concentrations. This time-delay can be understood as the time required to bring CO2 emissions down from its peak to a small value, and is governed by the rate of decarbonizaton of economic activity. This decarbonization rate affects how rapidly emissions decline after having achieved their peak, and a rapid decline in emissions is essential for limiting peak radiative forcing. Long-term mitigation goals for CO2 should therefore consider not only the timing of peak emissions, but also the rate of decarbonization. We discuss implications for mitigation of the fact that the emissions peak corresponds to small bu...

Seshadri, Ashwin K

2015-01-01T23:59:59.000Z

19

E-Print Network 3.0 - atmospheric co2 emissions Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

University Collection: Environmental Sciences and Ecology 16 EARTH'S CLIMATE, THE GREENHOUSE EFFECT, AND ENERGY Summary: al. Mauna Loa - Keeling 12;ATMOSPHERIC CO2 EMISSIONS Time...

20

Climate sensitivity constrained by CO2 concentrations over the past 420 million years  

E-Print Network [OSTI]

CO2 level on the rate of CO2 uptake by weathering of calcium and magnesium silicate minerals. A rise atmospheric CO2 consump- tion, forming a negative feedback loop. Here, using the logarithmic relation between for the weathering of calcium and magnesium silicates13 , and held this and all other parameters in GEOCARBSULF fixed

Royer, Dana

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


21

Carbonation of alkaline paper mill waste to reduce CO2 greenhouse gas1 emissions into the atmosphere2  

E-Print Network [OSTI]

ppm in the pre-industrial revolution to 37942 ppm in 2005, rising faster in the last 10 years (average atmospheric CO2 concentration doubles the pre-industrial revolution concentration (IPCC,49 2007a 36 insu-00351929,version1-12Jan2009 #12;1. Introduction37 38 Coal caused the first industrial

Boyer, Edmond

22

Abstract Atmospheric CO2 partial pressure (pCO2) was as low as 18 Pa during the Pleistocene and is projected to  

E-Print Network [OSTI]

Abstract Atmospheric CO2 partial pressure (pCO2) was as low as 18 Pa during the Pleistocene and is projected to increase from 36 to 70 Pa CO2 before the end of the 21st century. High pCO2 often increases the growth and repro- duction of C3 annuals, whereas low pCO2 decreases growth and may reduce or prevent

Antonovics, Janis

23

Effect of Elevated CO2 Concentration on Leaf Structure of Brassica Juncea under Water Stress  

Science Journals Connector (OSTI)

Study on the effect of elevated CO2 concentration on leaf structure of Brassica juncea L. cv. Bio-141 (95) under moisture stress revealed, that CO2 elevated to 600 ?mol mol?1 increased the length of epidermal cel...

D.C. Uprety; N. Dwivedi; R. Mohan; G. Paswan

2001-01-01T23:59:59.000Z

24

Stomatal limitation of photosynthesis as affected by water stress and CO2 concentration  

Science Journals Connector (OSTI)

A water stress effect on photosynthesis and transpiration of wheat seedlings at 50-500 mol(CO2) mol-1 was measured in an open ... -1 MPa, and it decreased with increasing CO2 concentration.

J. Jan?ek

1998-01-01T23:59:59.000Z

25

Pulse shaping of transversely excited atmospheric CO2 laser using a simple plasma shutter  

E-Print Network [OSTI]

Pulse shaping of transversely excited atmospheric CO2 laser using a simple plasma shutter Noah excited atmospheric CO2 laser consists of a sharp spike followed by a long, drawn out tail region spanning applications because it decreases the average power of the laser pulse. We employ a pinhole plasma shutter

Harilal, S. S.

26

Modelling of CO2 content in the atmosphere until 2300: influence of energy intensity of gross domestic product and carbon intensity of energy  

Science Journals Connector (OSTI)

The study provides a model of CO2 content in the atmosphere based on the global carbon cycle and the Kaya identity. The influences of: 1) energy intensity of GDP; 2) carbon intensity of energy on CO2 trajectories are given under four scenarios. The results from the most optimistic and technologically challenging scenario show that the atmospheric CO2 concentration can stabilise at 610 ppmv. It is also shown that the annual growth rates of atmospheric CO2 peak for all the scenarios before 2100 due to the expected world population peak in 2075 and the large share of fossil fuel energy.

Wojciech M. Budzianowski

2013-01-01T23:59:59.000Z

27

Effects of elevated CO2 concentration on growth and water usage of tomato seedlings under different ammonium/nitrate ratios  

Science Journals Connector (OSTI)

Increasing atmospheric CO2 concentration is generally expected to enhance photosynthesis and growth of agricultural C3 vegetable crops, and therefore results in an increase in crop yield. However, little is known about the combined effect of elevated CO2 and N species on plant growth and development. Two growth-chamber experiments were conducted to determine the effects of NH4+/NO3? ratio and elevated CO2 concentration on the physiological development and water use of tomato seedlings. Tomato was grown for 45 d in containers with nutrient solutions varying in NH4+/NO3? ratios and CO2 concentrations in growth chambers. Results showed that plant height, stem thickness, total dry weight, dry weight of the leaves, stems and roots, G value (total plant dry weight/seedling days), chlorophyll content, photosynthetic rate, leaf-level and whole plant-level water use efficiency and cumulative water consumption of tomato seedlings were increased with increasing proportion of NO3? in nutrient solutions in the elevated CO2 treatment. Plant biomass, plant height, stem thickness and photosynthetic rate were 67%, 22%, 24% and 55% higher at elevated CO2 concentration than at ambient CO2 concentration, depending on the values of NH4+/NO3? ratio. These results indicated that elevating CO2 concentration did not mitigate the adverse effects of 100% NH4+-N (in nutrient solution) on the tomato seedlings. At both CO2 levels, NH4+/NO3? ratios of nutrient solutions strongly influenced almost every measure of plant performance, and nitrate-fed plants attained a greater biomass production, as compared to ammonium-fed plants. These phenomena seem to be related to the coordinated regulation of photosynthetic rate and cumulative water consumption of tomato seedlings.

Juan LI; Jian-min ZHOU; Zeng-qiang DUAN

2007-01-01T23:59:59.000Z

28

Simple model to estimate the contribution of atmospheric CO2 to the Earths greenhouse effect  

Science Journals Connector (OSTI)

We show how the CO2 contribution to the Earths greenhouse effect can be estimated from relatively simple physical considerations and readily available spectroscopic data. In particular we present a calculation of the climate sensitivity (that is the increase in temperature caused by a doubling of the concentration of CO2) in the absence of feedbacks. Our treatment highlights the important role played by the frequency dependence of the CO2absorptionspectrum. For pedagogical purposes we provide two simple models to visualize different ways in which the atmosphere might return infrared radiation back to the Earth. The more physically realistic model based on the Schwarzschild radiative transfer equations uses as input an approximate form of the atmospheres temperature profile and thus includes implicitly the effect of heat transfer mechanisms other than radiation.

Derrek J. Wilson; Julio Gea-Banacloche

2012-01-01T23:59:59.000Z

29

A 40-million-year history of atmospheric CO2  

Science Journals Connector (OSTI)

...ecosystems. Proc. Natl Acad. Sci. USA 105, 449-453. ( doi:10...2011 Convergent Cenozoic CO2 history. Nat. Geosci. 4, 418-420...Yellowlees, W Leggat, and GD Price. 1998 The diversity and coevolution...Washington, DC: US Department of Energy. 96 Pagani, M . In press Biomarker-based...

2013-01-01T23:59:59.000Z

30

Regional Impacts of Climate Change and Atmospheric CO2 on Future Ocean Carbon Uptake: A Multimodel Linear Feedback Analysis  

Science Journals Connector (OSTI)

The increase in atmospheric CO2 over this century depends on the evolution of the oceanic airsea CO2 uptake, which will be driven by the combined response to rising atmospheric CO2 itself and climate change. Here, the future oceanic CO2 uptake is ...

Tilla Roy; Laurent Bopp; Marion Gehlen; Birgit Schneider; Patricia Cadule; Thomas L. Frlicher; Joachim Segschneider; Jerry Tjiputra; Christoph Heinze; Fortunat Joos

2011-05-01T23:59:59.000Z

31

In situ Carbon 13 and Oxygen 18 Ratios of Atmospheric CO2 from Cape Grim,  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Oxygen Isotopes and Ratios » 13C and 18O Oxygen Isotopes and Ratios » 13C and 18O Ratios, Atmospheric CO2, Cape Grim In situ Carbon 13 and Oxygen 18 Ratios of Atmospheric CO2 from Cape Grim, Tasmania, Australia: 1982-1993 DOI: 10.3334/CDIAC/atg.db1014 data Data Investigators Francey R. J. and C. E. Allison Description Since 1982, a continuous program of sampling atmospheric CO2 to determine stable isotope ratios has been maintained at the Australian Baseline Air Pollution Station, Cape Grim, Tasmania (40°, 40'56"S, 144°, 41'18"E). The process of in situ extraction of CO2 from air, the preponderance of samples collected in conditions of strong wind from the marine boundary layer of the Southern Ocean, and the determination of all isotope ratios relative to a common high purity CO2 reference gas with isotopic δ13C close to

32

Developing Model Constraints on Northern Extra-Tropical Carbon Cycling Based on measurements of the Abundance and Isotopic Composition of Atmospheric CO2  

SciTech Connect (OSTI)

The objective of this project was to perform CO2 data syntheses and modeling activities to address two central questions: 1) how much has the seasonal cycle in atmospheric CO2 at northern high latitudes changed since the 1960s, and 2) how well do prognostic biospheric models represent these changes. This project also supported the continuation of the Scripps time series of CO2 isotopes and concentration at ten baseline stations distributed globally.

Keeling, Ralph [UCSD-SIO

2014-12-12T23:59:59.000Z

33

Stomatal proxy record of CO2 concentrations from the last termination suggests an important role for CO2 at climate change transitions  

E-Print Network [OSTI]

Stomatal proxy record of CO2 concentrations from the last termination suggests an important role for CO2 at climate change transitions Margret Steinthorsdottir a,*, Barbara Wohlfarth a , Malin E2 reconstruction Betula nana Sweden a b s t r a c t A new stomatal proxy-based record of CO2

Wohlfarth, Barbara

34

arbon dioxide (CO2 atmosphere has increased by  

E-Print Network [OSTI]

on how plants and ecosystems may respond to this change in atmospheric composition, giving us confidence surface and scale up to affect the landscape water balance. Thus, through its impacts on plant water use and water to produce organic compounds. Since photosynthesis is an unsaturated biochemical reaction

35

An estimate of monthly global emissions of anthropogenic CO2: Impact on the seasonal cycle of atmospheric CO2  

E-Print Network [OSTI]

An estimate of monthly global emissions of anthropogenic CO2: Impact on the seasonal cycle of anthropogenic CO2 are presented. Approximating the seasonal CO2 emission cycle using a 2-harmonic Fourier series with regions of strong anthropogenic CO2 emissions. Citation: Erickson, D. J., III, R. T. Mills, J. Gregg, T. J

Hoffman, Forrest M.

36

WELL KNOWN . . . TO A FEW PEOPLE: ATTRIBUTION OF EXCESS ATMOSPHERIC CO2 AND RESULTING GLOBAL TEMPERATURE CHANGE TO  

E-Print Network [OSTI]

century the major source of incremental atmospheric CO2 was not FF emissions but emissions from so to deforestation. LUC CO2 emissions have been a substantial fraction of anthropogenic CO2 emissions throughout the industrial period and even at present are about a third as great as FF emissions. Cumulative LUC CO2

37

Diversity in neotropical wet forests during the Cenozoic is linked more to atmospheric CO2 than temperature  

Science Journals Connector (OSTI)

...the Cenozoic is linked more to atmospheric CO2 than temperature Dana L. Royer 1 2 Barry...distinguish between the effects of atmospheric CO2 and temperature, which limits their ability...hypotheses owing to their strong sensitivity to CO2, temperature and moisture. We find that...

2013-01-01T23:59:59.000Z

38

Light source and CO2 concentration affect growth and anthocyanin content of lettuce under controlled environment  

Science Journals Connector (OSTI)

The effect of light source and CO2 concentration on the growth and anthocyanin content of lettuce (Lactuca sativa L. Seonhong Jeokchukmyeon) grown in growth chambers was examined. The plant was grown under 140 ...

Yoo Gyeong Park; Ji Eun Park

2012-12-01T23:59:59.000Z

39

NETL: CO2 Emissions Control  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Post-Combustion CO2 Control Post-Combustion CO2 Control Post-combustion CO2 control systems separate CO2 from the flue gas produced by conventional coal combustion in air. The flue gas is at atmospheric pressure and has a CO2 concentration of 10-15 volume percent. Read More! Capturing CO2 under these conditions is challenging because: (1) the low pressure and dilute concentration dictate a high total volume of gas to be treated; (2) trace impurities in the flue gas tend to reduce the effectiveness of the CO2 separation processes; and (3) compressing captured CO2 from atmospheric pressure to pipeline pressure (1,200 - 2,200 pounds per square inch) represents a large parasitic energy load. Plant Picture DOE/NETL's post-combustion CO2 control technology R&D program includes

40

CO2 tracer gas concentration decay method for measuring air change rate  

Science Journals Connector (OSTI)

Abstract The measure of air change rate (ACR) in building is a difficult and usually expensive task. The tracer gas method is the reference technique but its implementation is difficult and the interpretation of results is not straightforward. In the present work, the concentration decay method by multiple CO2 transmitters is experimentally validated in the case of cross-ventilation. It is observed that in-situ CO2 transmitters lead to ACR values in good agreement with reference measurements obtained from mechanically controlled values. Whereas multiple transmitters in different sampling positions show the imperfect mixing, a sensor located at the outlet or an averaged value of all sensors can provide an accurate measure of the ACR. Moreover, the spatial variation of CO2 concentration can be used to assess the ventilation efficiency in the test chamber. Different measures and calculation methods are discussed, and the uncertainty analysis of each method is carried out.

Shuqing Cui; Michal Cohen; Pascal Stabat; Dominique Marchio

2015-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


41

A Database of Herbaceous Vegetation Responses to Elevated Atmospheric CO2  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Herbaceous Vegetation Responses to Elevated Atmospheric CO2 Herbaceous Vegetation Responses to Elevated Atmospheric CO2 (NDP-073) image Data image PDF file image Contributed by Michael H. Jones Peter S. Curtis Department of Evolution, Ecology, and Organismal Biology The Ohio State University Columbus, Ohio Prepared by Robert M. Cushman and Antoinette L. Brenkert Carbon Dioxide Information Analysis Center Environmental Sciences Division Publication No. 4909 Date Published: November 1999 Prepared for the Environmental Sciences Division Office of Biological and Environmental Research Budget Activity Number KP 12 04 01 0 Prepared by the Carbon Dioxide Information Analysis Center OAK RIDGE NATIONAL LABORATORY Oak Ridge, Tennessee 37831-6290 managed by LOCKHEED MARTIN ENERGY RESEARCH CORP. for the U.S. DEPARTMENT OF ENERGY under contract DE-AC05-96OR22464

42

Can a Convective Cloud Feedback Help to Eliminate Winter Sea Ice at High CO2 Concentrations?  

E-Print Network [OSTI]

have remote effects on global climate as well. Accurate forecasting of winter sea ice has significantCan a Convective Cloud Feedback Help to Eliminate Winter Sea Ice at High CO2 Concentrations? DORIAN) ABSTRACT Winter sea ice dramatically cools the Arctic climate during the coldest months of the year and may

Tziperman, Eli

43

GEOCARBSULF: A combined model for Phanerozoic atmospheric O2 and CO2  

Science Journals Connector (OSTI)

A model for the combined long-term cycles of carbon and sulfur has been constructed which combines all the factors modifying weathering and degassing of the GEOCARB III model [Berner R.A., Kothavala Z., 2001. GEOCARB III: a revised model of atmospheric CO2 over Phanerozoic time. Am. J. Sci. 301, 182204] for CO2 with rapid recycling and oxygen dependent carbon and sulfur isotope fractionation of an isotope mass balance model for O2 [Berner R.A., 2001. Modeling atmospheric O2 over Phanerozoic time. Geochim. Cosmochim. Acta 65, 685694]. New isotopic data for both carbon and sulfur are used and new feedbacks are created by combining the models. Sensitivity analysis is done by determining (1) the effect on weathering rates of using rapid recycling (rapid recycling treats carbon and sulfur weathering in terms of young rapidly weathering rocks and older more slowly weathering rocks); (2) the effect on O2 of using different initial starting conditions; (3) the effect on O2 of using different data for carbon isotope fractionation during photosynthesis and alternative values of oceanic ?13C for the past 200 million years; (4) the effect on sulfur isotope fractionation and on O2 of varying the size of O2 feedback during sedimentary pyrite formation; (5) the effect on O2 of varying the dependence of organic matter and pyrite weathering on tectonic uplift plus erosion, and the degree of exposure of coastal lands by sea level change; (6) the effect on CO2 of adding the variability of volcanic rock weathering over time [Berner, R.A., 2006. Inclusion of the weathering of volcanic rocks in the GEOCARBSULF model. Am. J. Sci. 306 (in press)]. Results show a similar trend of atmospheric CO2 over the Phanerozoic to the results of GEOCARB III, but with some differences during the early Paleozoic and, for variable volcanic rock weathering, lower CO2 values during the Mesozoic. Atmospheric oxygen shows a major broad late Paleozoic peak with a maximum value of about 30% O2 in the Permian, a secondary less-broad peak centered near the Silurian/Devonian boundary, variation between 15% and 20% O2 during the Cambrian and Ordovician, a very sharp drop from 30% to 15% O2 at the Permo-Triassic boundary, and a more-or less continuous rise in O2 from the late Triassic to the present.

Robert A. Berner

2006-01-01T23:59:59.000Z

44

High Accuracy 14C Measurements for Atmospheric CO2 Samples from the South  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Carbon Isotopes » CIO 14C Measurements Carbon Isotopes » CIO 14C Measurements High Accuracy 14C Measurements for Atmospheric CO2 Samples from the South Pole and Point Barrow, Alaska by Accelerator Mass Spectrometry graphics South Pole Graphics graphics Pt. Barrow Graphics data South Pole Digital Data - Trends Only data South Pole Digital Data - Complete Data data Pt. Barrow Digital Data - Trends Only data Pt. Barrow Digital Data - Complete Data Investigators H. A. J. Meijer, M. H. Pertuisot and J. van der Plicht Centrum voor Isotopen Onderzook (Center for Isotope Research, CIO) University of Groningen The Netherlands http://www.rug.nl/ees/onderzoek/cio/index Period of Record: 1984-1992 Methods Accelerator mass spectrometry (AMS) was used to obtain 14CO2 measurements from flasks collected at the South Pole and Point Barrow, Alaska, USA, at

45

Atmospheric CO2> Record from In Situ Measurements at K-Puszta, Hungary  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

K-Puszta, Hungary K-Puszta, Hungary Atmospheric CO2 Record from In Situ Measurements at K-Puszta, Hungary graphics Graphics data Data Investigator László Haszpra Hungarian Meteorological Service, Institute for Atmospheric Physics, Department for Analysis of Atmospheric Environment, H-1675, P.O. Box 39, Budapest, Hungary Period of Record 1981-1997 Location The K-puszta regional background air pollution monitoring station was established in a clearing in a mixed forest on the Hungarian Great Plain in the middle of the Carpathian Basin. K-puszta is as free from direct pollution as possible in the highly industrialized, densely populated central Europe. Because of the growing vegetation, the station was moved in September 1993 to a larger clearing, also at the same elevation,

46

Influence of reduced carbon emissions and oxidation on the distribution of atmospheric CO2: Implications for inversion analyses  

E-Print Network [OSTI]

Influence of reduced carbon emissions and oxidation on the distribution of atmospheric CO2 carbon emissions. We used TransCom3 annual mean simulations from three transport models to evaluate carbon emission and oxidation processes in deriving inversion estimates of CO2 surface fluxes. Citation

Krakauer, Nir Y.

47

Relationships between soil CO2 concentration and CO2 production, temperature, water content, and gas diffusivity: implications for field studies through sensitivity analyses  

Science Journals Connector (OSTI)

Soil CO2 levels reflect CO2 production and transport in soil and provide valuable information about soil CO2 dynamics. However, extracting information from soil CO2 profiles is often difficult because of the comp...

Shoji Hashimoto; Hikaru Komatsu

2006-02-01T23:59:59.000Z

48

The Anthropogenic Perturbation of Atmospheric CO2 and the Climate System  

E-Print Network [OSTI]

of carbon dioxide (CO2), a powerful greenhouse gas (GHG), are redistributed within the climate system

Fortunat, Joos

49

Atmospheric CO2 Record from In Situ Measurements at Amsterdam Island  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Amsterdam Island Amsterdam Island Atmospheric CO2 Record from In Situ Measurements at Amsterdam Island graphics Graphics data Data Investigators A. Gaudry, V. Kazan, and P. Monfray Centre des Faibles Radioactivités, Laboratoire de Modélisation du Climat et de l'Environnement, Centre d'Etudes de Saclay, Bâtiment 709, Orme des Merisiers, 91191-Gif-sur-Yvette Cedex, France Period of Record 1980-95 Methods Until 1993 air samples were collected continuously through an air intake located at the top of a tower, 9 m above ground and 65 m above mean sea level. Since 1994, the intake has been situated 20 m above ground and 76 m above mean sea level. The tower is located at the north-northwest end of the island on the edge of a 55 m cliff. The air is dried by means of a cryogenic water trap at -60°C. Until 1990, determinations of CO2 were made

50

Estimating the Overall Impact of A Change in Agricultural Practices on Atmospheric CO2  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

the Overall Impact of A Change the Overall Impact of A Change In Agricultural Practices on Atmospheric CO 2 T.O. West (westto@ornl.gov; 865-574-7322) G. Marland (marlandgh@ornl.gov; 865-241-4850) Environmental Sciences Division, Oak Ridge National Laboratory P.O. Box 2008 Oak Ridge, TN 37831-6335 Introduction One option for sequestering carbon in the terrestrial biosphere is to increase the carbon (C) stocks in agricultural soils. There is now an extensive literature on the amount of C that has been lost from soils as a consequence of humans disturbing natural ecosystems, and of the amount of C that might be returned to soils with improved management practices. Improvements in management practices could include efficient use of fertilizers and irrigation water, use of crop rotations, and changing from conventional tillage (CT) to conservation tillage

51

Syngas Production from Coal Gasification with CO2 Rich Gas Mixtures  

Science Journals Connector (OSTI)

Coal gasification with CO2 rich gas mixture is one of several promising new technologies associated with CO2 reduction in the atmosphere. Coal gasification with high CO2 concentration is suitable for producing la...

M. S. Alam; A. T. Wijayanta; K. Nakaso

2013-01-01T23:59:59.000Z

52

Twenty-First-Century Compatible CO2 Emissions and Airborne Fraction Simulated by CMIP5 Earth System Models under Four Representative Concentration Pathways  

Science Journals Connector (OSTI)

The carbon cycle is a crucial Earth system component affecting climate and atmospheric composition. The response of natural carbon uptake to CO2 and climate change will determine anthropogenic emissions compatible with a target CO2 pathway. For ...

Chris Jones; Eddy Robertson; Vivek Arora; Pierre Friedlingstein; Elena Shevliakova; Laurent Bopp; Victor Brovkin; Tomohiro Hajima; Etsushi Kato; Michio Kawamiya; Spencer Liddicoat; Keith Lindsay; Christian H. Reick; Caroline Roelandt; Joachim Segschneider; Jerry Tjiputra

2013-07-01T23:59:59.000Z

53

Edinburgh Research Explorer Can seasonal and interannual variation in landscape CO2 fluxes  

E-Print Network [OSTI]

Edinburgh Research Explorer Can seasonal and interannual variation in landscape CO2 fluxes be detected by atmospheric observations of CO2 concentrations made at a tall tower? Citation for published in landscape CO2 fluxes be detected by atmospheric observations of CO2 concentrations made at a tall tower

Millar, Andrew J.

54

Carbon Dynamics in Aquatic Ecosystems in Response to Elevated Atmospheric CO2 and Altered Nutrients Availability  

E-Print Network [OSTI]

. Our results show that elevated CO2 led to enhanced photosynthetic carbon uptake and dissolved organic carbon (DOC) production. DOC occupied larger percentage in total organic carbon production in high CO2 environment. N addition stimulated biomass...

Song, Chao

2011-04-26T23:59:59.000Z

55

HVAC system optimization with CO2 concentration control using genetic algorithms  

Science Journals Connector (OSTI)

This study describes the use of genetic algorithms (GAs) for operating standard HVAC systems (HVACheating, ventilation and air conditioning) in order to optimize performance, primarily with regard to power saving. Genetic algorithms were introduced as an instrument for solving optimization problems. Analytic optimization procedures are widely used in other fields of engineering, but they are difficult to operate within HVAC systems, because the range of the research is usually too broad, the problems are not linear but rather discontinuous, and they mostly have complex limitations. This is why for this type of system genetic algorithms are used, since they have the qualities of robustness and efficiency that are crucial for finding the optimal solution. A simulation is conducted in order to demonstrate how much power can be saved by using the suggested method of CO2 concentration control in a standard HVAC system. In addition to Matlab Simulink, the suggested method is verified with Energy software.

Velimir Congradac; Filip Kulic

2009-01-01T23:59:59.000Z

56

Stratospheric and mesospheric pressure-temperature profiles from rotational analysis of CO2 lines in atmospheric trace molecule spectroscopy/ATLAS 1 infrared solar occultation spectra  

SciTech Connect (OSTI)

A simple, classical, and expedient method for the retrieval of atmospheric pressure-temperature profiles has been applied to the high-resolution infrared solar absorption spectra obtained with the atmospheric trace molecule spectroscopy (ATMOS) instrument. The basis for this method is a rotational analysis of retrieved apparent abundances from CO2 rovibrational absorption lines, employing existing constituent concentration retrieval software used in the analysis of data returned by ATMOS. Pressure-temperature profiles derived from spectra acquired during the ATLAS 1 space shuttle mission of March-April 1992 are quantitatively evaluated and compared with climatological and meteorological data as a means of assessing the validity of this approach.

Stiller, G.P.; Gunson, M.R.; Lowes, L.L.; Abrams, M.C.; Raper, O.F.; Farmer, C.B.; Zander, R.; Rinsland, C.P. [Kernforschungszentrum Karlsruhe, Karlsruhe (Germany)] [Kernforschungszentrum Karlsruhe, Karlsruhe (Germany); [Jet Propulsion Lab., California Inst. of Tech., Pasadena, CA (United States); [Liege Univ., Liege (Belgium); [NASA, Langley Research Center, Hampton, VA (United States)

1995-02-01T23:59:59.000Z

57

New Technique for the Direct Analysis of Food Powders Confined in a Small Hole Using Transversely Excited Atmospheric CO2 Laser-Induced Gas Plasma  

Science Journals Connector (OSTI)

Taking advantage of the differences between the interactions of transversely excited atmospheric (TEA) CO2 lasers with metal and with organic powder, a new technique for...

Khumaeni, Ali; Ramli, Muliadi; Deguchi, Yoji; Lee, Yong Inn; Idris, Nasrullah; Kurniawan, Koo Hendrik; Lie, Tjung Jie; Kagawa, Kiichiro

2008-01-01T23:59:59.000Z

58

CO2 Sequestration short course  

SciTech Connect (OSTI)

Given the publics interest and concern over the impact of atmospheric greenhouse gases (GHGs) on global warming and related climate change patterns, the course is a timely discussion of the underlying geochemical and mineralogical processes associated with gas-water-mineral-interactions encountered during geological sequestration of CO2. The geochemical and mineralogical processes encountered in the subsurface during storage of CO2 will play an important role in facilitating the isolation of anthropogenic CO2 in the subsurface for thousands of years, thus moderating rapid increases in concentrations of atmospheric CO2 and mitigating global warming. Successful implementation of a variety of geological sequestration scenarios will be dependent on our ability to accurately predict, monitor and verify the behavior of CO2 in the subsurface. The course was proposed to and accepted by the Mineralogical Society of America (MSA) and The Geochemical Society (GS).

DePaolo, Donald J. [Lawrence Berkeley National Laboratory; Cole, David R [The Ohio State University; Navrotsky, Alexandra [University of California-Davis; Bourg, Ian C [Lawrence Berkeley National Laboratory

2014-12-08T23:59:59.000Z

59

A Portable Eddy Covariance System for the Measurement of EcosystemAtmosphere Exchange of CO2, Water Vapor, and Energy  

Science Journals Connector (OSTI)

To facilitate the study of flux heterogeneity within a region, the authors have designed and field-tested a portable eddy covariance system to measure exchange of CO2, water vapor, and energy between the land surface and the atmosphere. The ...

D. P. Billesbach; M. L. Fischer; M. S. Torn; J. A. Berry

2004-04-01T23:59:59.000Z

60

Enhanced Water Use Efficiency in Dry Loess Grassland Species Grown at Elevated Air CO2 Concentration  

Science Journals Connector (OSTI)

Net CO2 assimilation rate (PN), stomatal conductance (gs), transpiration rate (E), and water use efficiency (WUE) in four perennial C3 species...

K. Szente; Z. Nagy; Z. Tuba

1998-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


61

Evolutionary context for understanding and manipulating plant responses to past, present and future atmospheric [CO2  

Science Journals Connector (OSTI)

...across species or environments and will not be...are underway to engineer plants to: (i...elevated [CO2] environments. Moreover, crosses...inform efforts to engineer crops for improved...elevated [CO2] environments. Already, efforts are underway to engineer plants to overcome...

2012-01-01T23:59:59.000Z

62

The effect of anthropogenic emissions corrections on the seasonal cycle of atmospheric CO2  

SciTech Connect (OSTI)

A previous study (Erickson et al. 2008) approximated the monthly global emission estimates of anthropogenic CO{sub 2} by applying a 2-harmonic Fourier expansion with coefficients as a function of latitude to annual CO{sub 2} flux estimates derived from United States data (Blasing et al. 2005) that were extrapolated globally. These monthly anthropogenic CO{sub 2} flux estimates were used to model atmospheric concentrations using the NASA GEOS-4 data assimilation system. Local variability in the amplitude of the simulated CO{sub 2} seasonal cycle were found to be on the order of 2-6 ppmv. Here we used the same Fourier expansion to seasonally adjust the global annual fossil fuel CO{sub 2} emissions from the SRES A2 scenario. For a total of four simulations, both the annual and seasonalized fluxes were advected in two configurations of the NCAR Community Atmosphere Model (CAM) used in the Carbon-Land Model Intercomparison Project (C-LAMP). One configuration used the NCAR Community Land Model (CLM) coupled with the CASA (carbon only) biogeochemistry model and the other used CLM coupled with the CN (coupled carbon and nitrogen cycles) biogeochemistry model. All four simulations were forced with observed sea surface temperatures and sea ice concentrations from the Hadley Centre and a prescribed transient atmospheric CO{sub 2} concentration for the radiation and land forcing over the 20th century. The model results exhibit differences in the seasonal cycle of CO{sub 2} between the seasonally corrected and uncorrected simulations. Moreover, because of differing energy and water feedbacks between the atmosphere model and the two land biogeochemistry models, features of the CO{sub 2} seasonal cycle were different between these two model configurations. This study reinforces previous findings that suggest that regional near-surface atmospheric CO{sub 2} concentrations depend strongly on the natural sources and sinks of CO{sub 2}, but also on the strength of local anthropogenic CO{sub 2} emissions and geographic position. This work further attests to the need for remotely sensed CO{sub 2} observations from space.

Hoffman, Forrest M [ORNL] [ORNL; Erickson III, David J [ORNL] [ORNL; Blasing, T J [ORNL] [ORNL

2009-01-01T23:59:59.000Z

63

GEOPHYSICAL RESEARCH LETTERS, VOL. 27, NO. 10, PAGES 1519-1522, MAY 15, 2000 The impact of rising atmospheric CO2 on simulated sea  

E-Print Network [OSTI]

Atlantic sys- tem. The presence of sea ice also impacts the heat budget through its insulation of the ocean atmospheric CO2 on simulated sea ice induced thermohaline circulation variability Marika M. Holland1 , Aaron J atmospheric CO2 lev- els on the sea ice induced low frequency variability of the North Atlantic climate

64

E-Print Network 3.0 - atmospheric co2 content Sample Search Results  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

questions for Exam 1, section on climate change. Summary: content and CO2 emissions per unit of energy vary among coal, oil and natural gas? 2. Draw a diagram... natural carbon...

65

Influence of Nanoclay Concentration on the CO2 Diffusion and Physical Properties of PMMA Montmorillonite Microcellular Foams  

Science Journals Connector (OSTI)

Influence of Nanoclay Concentration on the CO2 Diffusion and Physical Properties of PMMA Montmorillonite Microcellular Foams ... (3, 4) Particularly, the dispersion of high aspect ratio nanoclays in polymers has been used as a possible strategy to improve some properties of the base material at relatively low filler amounts (<10 wt %). ...

Vera Realinho; Marcelo Antunes; Antonio B. Martnez; Jos I. Velasco

2011-11-08T23:59:59.000Z

66

On Leakage from Geologic Storage Reservoirs of CO2  

SciTech Connect (OSTI)

Large amounts of CO2 would need to be injected underground to achieve a significant reduction of atmospheric emissions. The large areal extent expected for CO2 plumes makes it likely that caprock imperfections will be encountered, such as fault zones or fractures, which may allow some CO2 to escape from the primary storage reservoir. Leakage of CO2 could also occur along wellbores. Concerns with escape of CO2 from a primary geologic storage reservoir include (1) acidification of groundwater resources, (2) asphyxiation hazard when leaking CO2 is discharged at the land surface, (3) increase in atmospheric concentrations of CO2, and (4) damage from a high-energy, eruptive discharge (if such discharge is physically possible). In order to gain public acceptance for geologic storage as a viable technology for reducing atmospheric emissions of CO2, it is necessary to address these issues and demonstrate that CO2 can be injected and stored safely in geologic formations.

Pruess, Karsten

2006-02-14T23:59:59.000Z

67

Engineering the Cyanobacterial Carbon Concentrating Mechanism for Enhanced CO2 Capture and Fixation  

SciTech Connect (OSTI)

In cyanobacteria CO2 fixation is localized in a special proteinaceous organelle, the carboxysome. The CO2 fixation enzymes are encapsulated by a selectively permeable protein shell. By structurally and functionally characterizing subunits of the carboxysome shell and the encapsulated proteins, we hope to understand what regulates the shape, assembly and permeability of the shell, as well as the targeting mechanism and organization of the encapsulated proteins. This knowledge will be used to enhance CO2 fixation in both cyanobacteria and plants through synthetic biology. The same strategy can also serve as a template for the production of modular synthetic bacterial organelles. Our research is conducted using a variety of techniques such as genomic sequencing and analysis, transcriptional regulation, DNA synthesis, synthetic biology, protein crystallization, Small Angle X-ray Scattering (SAXS), protein-protein interaction assays and phenotypic characterization using various types of cellular imaging, e.g. fluorescence microscopy, Transmission Electron Microscopy (TEM), and Soft X-ray Tomography (SXT).

Sandh, Gustaf; Cai, Fei; Shih, Patrick; Kinney, James; Axen, Seth; Salmeen, Annette; Zarzycki, Jan; Sutter, Markus; Kerfeld, Cheryl

2011-06-02T23:59:59.000Z

68

Hypothesized Link Between Glacial/Interglacial Atmospheric CO2 Cycles and Storage/Release of CO2-Rich Fluids From Deep-Sea Sediments  

E-Print Network [OSTI]

volcanic vents. Hydrothermal systems in the Pacific act as both a source and sink for carbon by changes in 14 C production alone and therefore appears to require a flux of 14 C- depleted carbon of CO2 regulation. Here we explore the possibility that hydrothermal sources of CO2 contributed

Stott, Lowell

69

Evolutionary context for understanding and manipulating plant responses to past, present and future atmospheric [CO2  

Science Journals Connector (OSTI)

...providing food, fuel and fibre for...ii) supplying energy to terrestrial...CO2] dropped, rates of A would have...nitrogen and energy. There has been...greater catalytic rate or impaired oxygenation...conductance in Florida vegetation. Proc...tree mortality rates in the Western...

2012-01-01T23:59:59.000Z

70

Forest Sensitivity to Elevated Atmospheric CO2 and its Relevance to Carbon Management Richard J. Norby  

E-Print Network [OSTI]

to these questions. In a closed-canopy deciduous forest in Oak Ridge3 (a sweetgum plantation), photosynthesis by the ecosystem (Figure 1). In the first #12;year of CO2 enrichment, aboveground stem biomass increased 33%, but in subsequent years the response of wood increment has been smaller and not significant. Instead, the extra C

71

Faster Decomposition Under Increased Atmospheric CO2 Limits Soil Carbon Storage  

Science Journals Connector (OSTI)

...atmosphere is a major focus of Earth system models, because the C cycle is sensitive...cycle affect our climate. Earth system models project that rising atmospheric...through microbial decomposition. Earth system models typically treat decomposition...

Kees Jan van Groenigen; Xuan Qi; Craig W. Osenberg; Yiqi Luo; Bruce A. Hungate

2014-05-02T23:59:59.000Z

72

A Regional Atmospheric Continuous CO2 Network in the Rocky Mountains (Rocky RACCOON) Panel 2. Storm Peak Laboratory (SPL), near Steamboat Springs, Colorado  

E-Print Network [OSTI]

A Regional Atmospheric Continuous CO2 Network in the Rocky Mountains (Rocky RACCOON) Panel 2. Storm in the Rocky Mountains to improve our understanding of regional carbon fluxes and to fill key gaps in the North Sep. 16, 2005. Large increases and a relatively flat profile at night indicate pooling of CO2 respired

Stephens, Britton B.

73

The Potential for Increased Atmospheric CO2 Emissions and Accelerated Consumption of Deep Geologic CO2 Storage Resources Resulting from the Large-Scale Deployment of a CCS-Enabled Unconventional Fossil Fuels Industry in the U.S.  

SciTech Connect (OSTI)

Desires to enhance the energy security of the United States have spurred significant interest in the development of abundant domestic heavy hydrocarbon resources including oil shale and coal to produce unconventional liquid fuels to supplement conventional oil supplies. However, the production processes for these unconventional fossil fuels create large quantities of carbon dioxide (CO2) and this remains one of the key arguments against such development. Carbon dioxide capture and storage (CCS) technologies could reduce these emissions and preliminary analysis of regional CO2 storage capacity in locations where such facilities might be sited within the U.S. indicates that there appears to be sufficient storage capacity, primarily in deep saline formations, to accommodate the CO2 from these industries. Nevertheless, even assuming wide-scale availability of cost-effective CO2 capture and geologic storage resources, the emergence of a domestic U.S. oil shale or coal-to-liquids (CTL) industry would be responsible for significant increases in CO2 emissions to the atmosphere. The authors present modeling results of two future hypothetical climate policy scenarios that indicate that the oil shale production facilities required to produce 3MMB/d from the Eocene Green River Formation of the western U.S. using an in situ retorting process would result in net emissions to the atmosphere of between 3000-7000 MtCO2, in addition to storing potentially 900-5000 MtCO2 in regional deep geologic formations via CCS in the period up to 2050. A similarly sized, but geographically more dispersed domestic CTL industry could result in 4000-5000 MtCO2 emitted to the atmosphere in addition to potentially 21,000-22,000 MtCO2 stored in regional deep geologic formations over the same period. While this analysis shows that there is likely adequate CO2 storage capacity in the regions where these technologies are likely to deploy, the reliance by these industries on large-scale CCS could result in an accelerated rate of utilization of the nations CO2 storage resource, leaving less high-quality storage capacity for other carbon-producing industries including electric power generation.

Dooley, James J.; Dahowski, Robert T.; Davidson, Casie L.

2009-11-02T23:59:59.000Z

74

Elevated atmospheric CO2 and humidity delay leaf fall in Betula pendula, but not in Alnus glutinosa or Populus tremula??tremuloides  

Science Journals Connector (OSTI)

Anthropogenic activity has increased the level of atmospheric CO2, which is driving an increase of global temperatures and associated changes in precipitation patterns. At Northern latitudes, one of the likely co...

Douglas Godbold; Arvo Tullus; Priit Kupper; Jaak Sber

2014-12-01T23:59:59.000Z

75

ARM - Datastreams - 30co2flx60m  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

flx60m flx60m Documentation Data Quality Plots Citation DOI: 10.5439/1025038 [ What is this? ] Generate Citation ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Datastream : 30CO2FLX60M Eddy Correlation CO2 Flux Data: 60 m samples, 30-min avg Active Dates 2001.01.01 - 2013.01.27 Measurement Categories Atmospheric Carbon, Atmospheric State, Surface Properties Originating Instrument Carbon Dioxide Flux Measurement Systems (CO2FLX) Measurements The measurements below provided by this product are those considered scientifically relevant. Measurement Variable Atmospheric turbulence Lmoni CO2 flux fc_corr CO2 flux fc_wpl_h CO2 flux fc_wpl_le Sensible heat flux h Latent heat flux le CO2 concentration mean_c Atmospheric moisture

76

Falsification Of The Atmospheric CO2 Greenhouse Effects Within The Frame Of Physics  

E-Print Network [OSTI]

The atmospheric greenhouse effect, an idea that authors trace back to the traditional works of Fourier 1824, Tyndall 1861 and Arrhenius 1896 and is still supported in global climatology essentially describes a fictitious mechanism in which a planetary atmosphere acts as a heat pump driven by an environment that is radiatively interacting with but radiatively equilibrated to the atmospheric system. According to the second law of thermodynamics such a planetary machine can never exist. Nevertheless, in almost all texts of global climatology and in a widespread secondary literature it is taken for granted that such mechanism is real and stands on a firm scientific foundation. In this paper the popular conjecture is analyzed and the underlying physical principles are clarified. By showing that (a) there are no common physical laws between the warming phenomenon in glass houses and the fictitious atmospheric greenhouse effects, (b) there are no calculations to determine an average surface temperature of a planet, ...

Gerlich, Gerhard

2007-01-01T23:59:59.000Z

77

CO2.indd  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

STORAGE & ENHANCED OIL RECOVERY STORAGE & ENHANCED OIL RECOVERY Objective R MOTC can play a signifi cant role in carbon dioxide (CO 2 ) storage and enhanced oil recovery technology development and fi eld demonstra- tions. RMOTC completed a scoping engineering study on Naval Petroleum Reserve No. 3's (NPR-3) CO 2 enhanced oil recovery potential. More recent character- ization studies indicate geologic carbon storage would also be an excellent use of NPR-3 resources beyond their economic life in conventional production. Geologic Storage Fossil fuels will remain the mainstay of energy production well into the 21st century. Availability of these fuels to provide clean, affordable energy is es- sential for the prosperity and security of the United States. However, increased atmospheric concentrations

78

Visible-light photoconductivity of Zn1-xCoxO and its dependence on Co2+ concentration  

Science Journals Connector (OSTI)

Many metal oxides investigated for solar photocatalysis or photoelectrochemistry have band gaps that are too wide to absorb a sufficient portion of the solar spectrum. Doping with impurity ions has been extensively explored as a strategy to sensitize such oxides to visible light, but the electronic structures of the resulting materials are frequently complex and poorly understood. Here, we report a detailed photoconductivity investigation of the wide-gap II-VI semiconductor ZnO doped with Co2+ (Zn1-xCoxO), which responds to visible light in photoelectrochemical and photoconductivity experiments and thus represents a well-defined model system for understanding dopant-sensitized oxides. Variable-temperature scanning photoconductivity measurements have been performed on Zn1-xCoxO epitaxial films to examine the relationship between dopant concentration (x) and visible-light photoconductivity, with particular focus on mid-gap intra-d-shell (d-d) photoactivity. Excitation into the intense 4T1(P) d-d band at ?2.0 eV (620 nm) leads to Co2+/3+ ionization with a quantum efficiency that increases with decreasing cobalt concentration and increasing sample temperature. Both spontaneous and thermally assisted ionization from the Co2+ d-d excited state are found to become less effective as x is increased, attributed to an increasing conduction-band-edge potential. These trends counter the increasing light absorption with increasing x, explaining the experimental maximum in external photon-to-current conversion efficiencies at values well below the solid solubility of Co2+ in ZnO.

Claire A. Johnson; Alicia Cohn; Tiffany Kaspar; Scott A. Chambers; G. Mackay Salley; Daniel R. Gamelin

2011-09-06T23:59:59.000Z

79

The impact of soil microorganisms on the global budget of ?18O in atmospheric CO2  

Science Journals Connector (OSTI)

...Environmental Sciences and Energy Research, Weizmann...for predicting the rate of change in atmospheric...than the uncatalyzed rate, consistent with...associated with fossil fuel burning (7.1 GtC y...forest Tallahassee Florida, USA Closed 0...temperature, C Flow rate, l min 1 Cin, ppm...

Lisa Wingate; Jrme Oge; Matthias Cuntz; Bernard Genty; Ilja Reiter; Ulli Seibt; Dan Yakir; Kadmiel Maseyk; Elise G. Pendall; Margaret M. Barbour; Behzad Mortazavi; Rgis Burlett; Philippe Peylin; John Miller; Maurizio Mencuccini; Jee H. Shim; John Hunt; John Grace

2009-01-01T23:59:59.000Z

80

The future of the carbon cycle: review, calcification response, ballast and feedback on atmospheric CO2  

Science Journals Connector (OSTI)

...inorganic carbon ( C O2) in seawater is in the form HCO- 3 , the...inorganic carbon species in seawater is such that, for a given...effective buffering capacity of seawater is analogous to the Revelle...larger capacity for carbon storage in the oceans than in the atmosphere...

2003-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


81

Response of the middle atmosphere to CO2 doubling: results from the Canadian  

E-Print Network [OSTI]

, Ontario, Canada Department of Atmospheric and Oceanic Sciences, McGill University, Montréal, Québec, Canada #Department of Physics, University of Toronto, Toronto, Ontario, Canada (Manuscript received 2 an increase in solar heating and a decrease in infrared cooling, with the latter accounting for up to 15

Wirosoetisno, Djoko

82

Reversible Ionic Liquids as Double-action Solvents for Efficient CO2 Capture  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Reversible Ionic Liquids as Double-action Reversible Ionic Liquids as Double-action Solvents for Efficient CO 2 Capture Background Post-combustion carbon dioxide (CO 2 ) capture presents technical challenges because the flue gas is at atmospheric pressure and the CO 2 concentration is 10 to 15 volume percent, resulting in a low CO 2 partial pressure and a large volume of gas that needs to be treated. In spite of this difficulty, post-combustion CO 2 capture offers the

83

Renewable Energy and CO2: Current Status and Costs  

Science Journals Connector (OSTI)

In this chapter, it is exposed a brief description of the current use and theoretical potential of renewable and conventional energies, the evolution of the CO2 emissions and atmospheric concentration and their i...

Ricardo Guerrero-Lemus; Jos Manuel Martnez-Duart

2013-01-01T23:59:59.000Z

84

NETL: CO2 Compression  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

CO2 Compression CO2 Compression The CO2 captured from a power plant will need to be compressed from near atmospheric pressure to a pressure between 1,500 and 2,200 psi in order to be transported via pipeline and then injected into an underground sequestration site. Read More! CO2 Compression The compression of CO2 represents a potentially large auxiliary power load on the overall power plant system. For example, in an August 2007 study conducted for DOE/NETL, CO2 compression was accomplished using a six-stage centrifugal compressor with interstage cooling that required an auxiliary load of approximately 7.5 percent of the gross power output of a subcritical pressure, coal-fired power plant. As a result, DOE/NETL is sponsoring R&D to develop novel methods that can significantly decrease the

85

Clouds in the atmospheres of extrasolar planets. IV. On the scattering greenhouse effect of CO2 ice particles: Numerical radiative transfer studies  

E-Print Network [OSTI]

Owing to their wavelengths dependent absorption and scattering properties, clouds have a strong impact on the climate of planetary atmospheres. Especially, the potential greenhouse effect of CO2 ice clouds in the atmospheres of terrestrial extrasolar planets is of particular interest because it might influence the position and thus the extension of the outer boundary of the classic habitable zone around main sequence stars. We study the radiative effects of CO2 ice particles obtained by different numerical treatments to solve the radiative transfer equation. The comparison between the results of a high-order discrete ordinate method and simpler two-stream approaches reveals large deviations in terms of a potential scattering efficiency of the greenhouse effect. The two-stream methods overestimate the transmitted and reflected radiation, thereby yielding a higher scattering greenhouse effect. For the particular case of a cool M-type dwarf the CO2 ice particles show no strong effective scattering greenhouse eff...

Kitzmann, D; Rauer, H

2013-01-01T23:59:59.000Z

86

Novel integration options of concentrating solar thermal technology with fossil-fuelled and CO2 capture processes  

Science Journals Connector (OSTI)

Concentrating solar thermal (CST) technology has been commercially proven in utility-scale power plants that have been in operation since the 1980s. CST uses reflecting surfaces to focus solar energy onto collectors, generating extreme heat than can be used for a variety of purposes. The current focus of CST is large-scale electrical power generation. However, new applications, such as solar fuels, are quickly gaining momentum. One key shortcoming of CST technology is its sensitivity to disruptions in sunlight availability over time. CST systems require either thermal energy storage or backup systems to operate during heavy cloud periods or at night. On the other hand, fossil-based energy systems have high availability and reliability, but they generate substantial CO2 emissions compared to equivalent CST processes. A novel solution would combine the benefits of CST technology and of fossil-fueled energy systems. Such a solar-fossil hybrid system would guarantee energy availability in the absence of sunlight or stored solar energy. The addition of carbon capture to these systems could reduce their carbon intensity to almost zero. This paper introduces three important solar-fossil hybrid energy systems: (1) Integrated Solar Combined Cycle (ISCC), (2) Solar-assisted post-combustion capture (SAPCAP), and (3) Solar gasification with CO2 capture. These novel concepts have great potential to overcome the inherent limitations of their component technologies and to achieve superior greenhouse gas mitigation techno-economic performance in large-scale applications. The paper describes the features of the three solar-fossil hybrid systems described earlier, discusses its advantages and disadvantages, and provides examples of applications. The goal of this manuscript is to introduce experts in the CCS and CST fields to the opportunities of integration between these technologies and their potential benefits.

Guillermo Ordorica-Garcia; and Alfonso Vidal Delgado; Aranzazu Fernandez Garcia

2011-01-01T23:59:59.000Z

87

Reaction Mechanism of Coal Chemical Looping Process for Syngas Production with CaSO4 Oxygen Carrier in the CO2 Atmosphere  

Science Journals Connector (OSTI)

Reaction Mechanism of Coal Chemical Looping Process for Syngas Production with CaSO4 Oxygen Carrier in the CO2 Atmosphere ... (5) One is to carry out first coal gasification and subsequently to introduce the syngas produced in the CLC system,(6) while the other is to feed the solid fuel directly to the fuel reactor in a CLC process. ... When oxygen supported by oxygen carrier is enough for converting the coal into CO2 and H2O, a considerable amount of heat will produce for electricity generation. ...

Yongzhuo Liu; Qingjie Guo; Yu Cheng; Ho-Jung Ryu

2012-07-13T23:59:59.000Z

88

Radon-222 Daughter Concentrations in Uranium Mine Atmospheres  

Science Journals Connector (OSTI)

... undertaken to measure the concentrations of 210Pb and 210Po in uranium mine atmospheres at various radon daughter concentration levels, and to determine the amount of 210Pb in the mine atmosphere ... atmosphere relative to that which would be produced from the decay of the short-lived radon daughters deposited in the lungs. Radium-226 was also measured in air so as ...

RICHARD L. BLANCHARD

1969-07-19T23:59:59.000Z

89

INVESTIGATIONS ON THE IMPACTS OF LAND-COVER CHANGES AND/OR INCREASED CO2 CONCENTRATIONS ON FOUR REGIONAL WATER CYCLES  

E-Print Network [OSTI]

REGIONAL WATER CYCLES AND THEIR INTERACTIONS WITH THE GLOBAL WATER CYCLE By Zhao Li RECOMMENDED-COVER CHANGES AND/OR INCREASED CO2 CONCENTRATIONS ON FOUR REGIONAL WATER CYCLES AND THEIR INTERACTIONS WITH THE GLOBAL WATER CYCLE A THESIS Presented to the Faculty of the University of Alaska Fairbanks In Partial

Moelders, Nicole

90

Whitings as a Potential Mechanism for Controlling Atmospheric Carbon Dioxide Concentrations Final Project Report  

SciTech Connect (OSTI)

Species of cyanobacteria in the genera Synechococcus and Synechocystis are known to be the catalysts of a phenomenon called "whitings", which is the formation and precipitation of fine-grained CaCO3 particles. Whitings occur when the cyanobacteria fix atmospheric CO2 through the formation of CaCO3 on their cell surfaces which leads to precipitation to the ocean floor and subsequent entombment in mud. Whitings represent one potential mechanism for CO2 sequestration. Research was performed to determine the ability of various strains of Synechocystis and Synechococcus to calcify when grown in microcosms amended with 2.5 mM HCO3- and 3.4 mM Ca2+. Results indicated that while all strains tested have the ability to calcify, only two, Synechococcus species, strains PCC 8806 and PCC 8807, were able to calcify to the extent that CaCO3 was precipitated. Enumeration of the cyanobacterial cultures during testing indicated that cell density did not appear to have an effect on calcification. Factors that had the greatest effect on calcification were CO2 removal and subsequent generation of alkaline pH. As CO2 was removed, growth medium pH increased and soluble Ca2+ was removed from solution. The largest increases in growth medium pH occurred when CO2 levels dropped below 400 ppmv. Precipitation of CaCO3 catalyzed by the growth and physiology of cyanobacteria in the Genus Synechococcus represents a potential mechanism for sequestration of atmospheric CO2 produced during the burning of coal for power generation. Synechococcus sp. strain PCC 8806 and Synechococcus sp. strain PCC 8807 were tested in microcosm experiments for their ability to calcify when exposed to a fixed calcium concentration of 3.4 mM and dissolved inorganic carbon concentrations of 0.5, 1.25 and 2.5 mM. Synechococcus sp. strain PCC 8806 removed calcium continuously over the duration of the experiment producing approximately 18.6 mg of solid-phase calcium. Calcium removal occurred over a two-day time period when Synechococcus sp. strain PCC 8807 was tested and only 8.9 mg of solid phase calcium was produced. The ability of the cyanobacteria to create an alkaline growth environment appeared to be the primary factor responsible for CaCO3 precipitation in these experiments. These research results demonstrate the potential of using cyanobacterial catalyzed whitings as a method to sequester CO2 from the atmosphere.

Brady D. Lee; William A. Apel; Michelle R. Walton

2006-03-01T23:59:59.000Z

91

The feasibility of low CO2 concentration targets and the role of bio-energy with carbon capture and storage (BECCS)  

Science Journals Connector (OSTI)

The United Nations Framework Convention on Climate Change (UNFCCC 1992) calls for stabilization of atmospheric greenhouse gas (GHG) concentrations at a level that would prevent dangerous anthropogenic interferenc...

Christian Azar; Kristian Lindgren; Michael Obersteiner; Keywan Riahi

2010-05-01T23:59:59.000Z

92

Hydrogeology of Stromboli volcano, Aeolian Islands (Italy) from the interpretation of resistivity tomograms, self-potential, soil temperature and soil CO2 concentration measurements  

Science Journals Connector (OSTI)

......France 9 Earth and Atmospheric Sciences Department...can occur when water encounters a...measurements with a generator and a voltmeter...two-phase (liquid water and steam) flow...concentration below atmospheric level (350 ppm...The evidence of atmospheric levels of soil...infiltration of meteoric water can flow on the......

A. Revil; A. Finizola; T. Ricci; E. Delcher; A. Peltier; S. Barde-Cabusson; G. Avard; T. Bailly; L. Bennati; S. Byrdina; J. Colonge; F. Di Gangi; G. Douillet; M. Lupi; J. Letort; E. Tsang Hin Sun

2011-09-01T23:59:59.000Z

93

The economic feasibility of enhanced coalbed methane recovery using CO2 sequestration in the San Juan Basin  

E-Print Network [OSTI]

Carbon dioxide emissions are considered a major source of increased atmospheric CO2 levels leading towards global warming. CO2 sequestration in coal bed reservoirs is one technique that can reduce the concentration of CO2 in the air. In addition...

Agrawal, Angeni

2007-09-17T23:59:59.000Z

94

Concentration of Atmospheric Radon and Wind Direction  

Science Journals Connector (OSTI)

... in Lisbon, near the sea, is therefore excellent to test any probable relationship between radon concentration and wind directions since only half the possible wind directions are continental ones, ... since only half the possible wind directions are continental ones, therefore corresponding probably to higher radon concentrations. In order to study any correlation, the concentration of ...

F. BARREIRA

1961-06-17T23:59:59.000Z

95

ARM - Instrument - co2flx  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

govInstrumentsco2flx govInstrumentsco2flx Documentation CO2FLX : Handbook CO2FLX : Instrument Mentor Monthly Summary (IMMS) reports CO2FLX : Data Quality Assessment (DQA) reports ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Instrument : Carbon Dioxide Flux Measurement Systems (CO2FLX) Instrument Categories Atmospheric Carbon General Overview The Southern Great Plains (SGP) carbon dioxide flux (CO2 flux) measurement systems provide half-hour average fluxes of CO2, H2O (latent heat), and sensible heat. The fluxes are obtained by the eddy covariance technique, which computes the flux as the mean product of the vertical wind component with CO2 and H2O densities, or estimated virtual temperature. A three-dimensional sonic anemometer is used to obtain the orthogonal wind

96

A Multiscale and Multidisciplinary Investigation Of EcosystemAtmosphere CO2 Exchange Over the Rocky Mountains of Colorado  

Science Journals Connector (OSTI)

A significant fraction of Earth consists of mountainous terrain. However, the question of how to monitor the surfaceatmosphere carbon exchange over complex terrain has not been fully explored. This article reports on studies by a team of ...

Jielun Sun; Steven P. Oncley; Sean P. Burns; Britton B. Stephens; Donald H. Lenschow; Teresa Campos; Andrew S. Watt; Russell K. Monson; David J. P. Moore; Jia Hu; Mark Tschudi; David S. Schimel; Steven Aulenbach; William J. Sacks; Stephan F. J. De Wekker; Chun-Ta Lai; Brian Lamb; Eugene Allwine; Teresa Coons; Dennis Ojima; Patrick Z. Ellsworth; Leonel S. L. Sternberg; Sharon Zhong; Craig Clements; Dean E. Anderson

2010-02-01T23:59:59.000Z

97

Transient Responses of a Coupled OceanAtmosphere Model to Gradual Changes of Atmospheric CO2. Part I. Annual Mean Response  

Science Journals Connector (OSTI)

This study investigates the response of a climate model to a gradual increase or decrease of atmospheric carbon dioxide. The model is a general circulation model of the coupled atmosphere-ocean-land surface system with global geography and ...

S. Manabe; R. J. Stouffer; M. J. Spelman; K. Bryan

1991-08-01T23:59:59.000Z

98

IMPACTS OF INTERACTING ELEVATED ATMOSPHERIC CO2 AND O3 ON THE STRUCTURE AND FUNCTIONING OF A NORTHERN FOREST ECOSYSTEM: OPERATING AND DECOMMISSIONING THE ASPEN FACE PROJECT  

SciTech Connect (OSTI)

Two of the most important and pervasive greenhouse gases driving global change and impacting forests in the U.S. and around the world are atmospheric CO2 and tropospheric O3. As the only free air, large-scale manipulative experiment studying the interaction of elevated CO2 and O3 on forests, the Aspen FACE experiment was uniquely designed to address the long-term ecosystem level impacts of these two greenhouse gases on aspen-birch-maple forests, which dominate the richly forested Lake States region. The project was established in 1997 to address the overarching scientific question: What are the effects of elevated [CO2] and [O3], alone and in combination, on the structure and functioning of northern hardwood forest ecosystems? From 1998 through the middle of the 2009 growing season, we examined the interacting effects of elevated CO2 and O3 on ecosystem processes in an aggrading northern forest ecosystem to compare the responses of early-successional, rapid-growing shade intolerant trembling aspen and paper birch to those of a late successional, slower growing shade tolerant sugar maple. Fumigations with elevated CO2 (560 ppm during daylight hours) and O3 (approximately 1.5 x ambient) were conducted during the growing season from 1998 to 2008, and in 2009 through harvest date. Response variables quantified during the experiment included growth, competitive interactions and stand dynamics, physiological processes, plant nutrient status and uptake, tissue biochemistry, litter quality and decomposition rates, hydrology, soil respiration, microbial community composition and respiration, VOC production, treatment-pest interactions, and treatment-phenology interactions. In 2009, we conducted a detailed harvest of the site. The harvest included detailed sampling of a subset of trees by component (leaves and buds, fine branches, coarse branches and stem, coarse roots, fine roots) and excavation of soil to a depth of 1 m. Throughout the experiment, aspen and birch photosynthesis increased with elevated CO2 and tended to decrease with elevated O3, compared to the control. In contrast to aspen and birch, maple photosynthesis was not enhanced by elevated CO2. Elevated O3 did not cause significant reductions in maximum photosynthesis in birch or maple. In addition, photosynthesis in ozone sensitive clones was affected to a much greater degree than that in ozone tolerant aspen clones. Treatment effects on photosynthesis contributed to CO2 stimulation of aboveground and belowground growth that was species and genotype dependent, with birch and aspen being most responsive and maple being least responsive. The positive effects of elevated CO2 on net primary productivity NPP were sustained through the end of the experiment, but negative effects of elevated O3 on NPP had dissipated during the final three years of treatments. The declining response to O3 over time resulted from the compensatory growth of O3-tolerant genotypes and species as the growth of O3-sensitive individuals declined over time. Cumulative NPP over the entire experiment was 39% greater under elevated CO2 and 10% lower under elevated O3. Enhanced NPP under elevated CO2 was sustained by greater root exploration of soil for growth-limiting N, as well as more rapid rates of litter decomposition and microbial N release during decay. Results from Aspen FACE clearly indicate that plants growing under elevated carbon dioxide, regardless of community type or ozone level, obtained significantly greater amounts of soil N. These results indicate that greater plant growth under elevated carbon dioxide has not led to progressive N limitation. If similar forests growing throughout northeastern North America respond in the same manner, then enhanced forest NPP under elevated CO2 may be sustained for a longer duration than previously thought, and the negative effect of elevated O3 may be diminished by compensatory growth of O3-tolerant plants as they begin to dominate forest communities. By the end of the experiment, elevated CO2 increased ecosystem C content by 11%, whereas

Burton, Andrew J. [Michigan Technological University; Zak, Donald R. [University of Michigan; Kubiske, Mark E. [USDA Forest Service; Pregitzer, Kurt S. [University of Idaho

2014-06-30T23:59:59.000Z

99

Responses of primary production and total carbon storage to changes in climate and atmospheric CO? concentration  

E-Print Network [OSTI]

The authors used the terrestrial ecosystem model (TEM, version 4.0) to estimate global responses of annual net primary production (NPP) and total carbon storage to changes in climate and atmospheric CO2, driven by the ...

Xiao, Xiangming.; Kicklighter, David W.; Melillo, Jerry M.; McGuire, A. David.; Stone, Peter H.; Sokolov, Andrei P.

100

Modeling of CO2 storage in aquifers  

E-Print Network [OSTI]

Feb 6, 2011 ... atmosphere, increasing its temperature (greenhouse effect). To minimize climate change impacts, geological sequestration of CO2 is an...

santos,,,

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
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they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
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101

Globally Averaged Atmospheric CFC-11 Concentrations: Monthly and Annual  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Chlorofluorocarbons » Chlorofluorocarbons » Atmospheric CFC-11 Concentrations Globally Averaged Atmospheric CFC-11 Concentrations: Monthly and Annual Data for the Period 1975-1992 DOI: 10.3334/CDIAC/atg.db1010 data Data (DB1010) Investigator M. A. K. Khalil and R. A. Rasmussen Description This data set presents globally averaged atmospheric concentrations of chlorofluorocarbon 11, known also as CFC-11 or F-11 (chemical name: trichlorofluoromethane; formula: CCl3F). The monthly global average data are derived from flask air samples collected at eight sites in six locations over the period August 1980-July 1992. The sites are Barrow (Alaska), Cape Meares (Oregon), Cape Kumukahi and Mauna Loa (Hawaii), Cape Matatula (American Samoa), Cape Grim (Tasmania), Palmer Station, and the

102

Acclimation response of spring wheat in a free-air CO2 enrichment (FACE) atmosphere with variable soil nitrogen regimes. 3. Canopy architecture and gas exchange  

Science Journals Connector (OSTI)

The response of whole-canopy net CO2 exchange rate (CER) and canopy architecture to CO2 enrichment and N stress during 1996 and 1997 for open-field-grown wheat ecosystem (Triticum aestivum L. cv. Yecora Rojo) are...

Talbot J. Brooks; Gerard W. Wall; Paul J. Pinter Jr.

103

The influence of clouds and diffuse radiation on ecosystem-atmosphere CO2 and CO18O exhanges  

SciTech Connect (OSTI)

This study evaluates the potential impact of clouds on ecosystem CO{sub 2} and CO{sub 2} isotope fluxes ('isofluxes') in two contrasting ecosystems (a broadleaf deciduous forest and a C{sub 4} grassland), in a region for which cloud cover, meteorological, and isotope data are available for driving the isotope-enabled land surface model, ISOLSM. Our model results indicate a large impact of clouds on ecosystem CO{sub 2} fluxes and isofluxes. Despite lower irradiance on partly cloudy and cloudy days, predicted forest canopy photosynthesis was substantially higher than on clear, sunny days, and the highest carbon uptake was achieved on the cloudiest day. This effect was driven by a large increase in light-limited shade leaf photosynthesis following an increase in the diffuse fraction of irradiance. Photosynthetic isofluxes, by contrast, were largest on partly cloudy days, as leaf water isotopic composition was only slightly depleted and photosynthesis was enhanced, as compared to adjacent clear sky days. On the cloudiest day, the forest exhibited intermediate isofluxes: although photosynthesis was highest on this day, leaf-to-atmosphere isofluxes were reduced from a feedback of transpiration on canopy relative humidity and leaf water. Photosynthesis and isofluxes were both reduced in the C{sub 4} grass canopy with increasing cloud cover and diffuse fraction as a result of near-constant light limitation of photosynthesis. These results suggest that some of the unexplained variation in global mean {delta}{sup 18}O of CO{sub 2} may be driven by large-scale changes in clouds and aerosols and their impacts on diffuse radiation, photosynthesis, and relative humidity.

Still, C.J.; Riley, W.J.; Biraud, S.C.; Noone, D.C.; Buenning, N.H.; Randerson, J.T.; Torn, M.S.; Welker, J.; White, J.W.C.; Vachon, R.; Farquhar, G.D.; Berry, J.A.

2009-05-01T23:59:59.000Z

104

Final Technical Report: Response of Mediterranean-Type Ecosystems to Elevated Atmospheric CO2 and Associated Climate Change  

SciTech Connect (OSTI)

This research incorporated an integrated hierarchical approach in space, time, and levels of biological/ecological organization to help understand and predict ecosystem response to elevated CO{sub 2} and concomitant environmental change. The research utilized a number of different approaches, and collaboration of both PER and non-PER investigators to arrive at a comprehensive, integrative understanding. Central to the work were the CO{sub 2}-controlled, ambient Lit, Temperature controlled (CO{sub 2}LT) null-balance chambers originally developed in the arctic tundra, which were re-engineered for the chaparral with treatment CO{sub 2} concentrations of from 250 to 750 ppm CO{sub 2} in 100 ppm increments, replicated twice to allow for a regression analysis. Each chamber was 2 meters on a side and 2 meters tall, which were installed over an individual shrub reprouting after a fire. This manipulation allowed study of the response of native chaparral to varying levels of CO{sub 2}, while regenerating from an experimental burn. Results from these highly-controlled manipulations were compared against Free Air CO{sub 2} Enrichment (FACE) manipulations, in an area adjacent to the CO{sub 2}LT null balance greenhouses. These relatively short-term results (5-7 years) were compared to long-term results from Mediterranean-type ecosystems (MTEs) surrounding natural CO{sub 2} springs in northern Italy, near Laiatico, Italy. The springs lack the controlled experimental rigor of our CO{sub 2}LT and FACE manipulation, but provide invaluable validation of our long-term predictions.

Oechel, Walter C

2002-08-15T23:59:59.000Z

105

CO2 sequestration | EMSL  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

CO2 sequestration CO2 sequestration Leads No leads are available at this time. Low-Temperature Carbon Monoxide Oxidation Catalysed by Regenerable Atomically Dispersed Palladium on...

106

Sustainable Carbon Sequestration: Increasing CO2-Storage Efficiency through a CO2-Brine Displacement Approach  

E-Print Network [OSTI]

CO2 sequestration is one of the proposed methods for reducing anthropogenic CO2 emissions to the atmosphere and therefore mitigating global climate change. Few studies on storing CO2 in an aquifer have been conducted on a regional scale. This study...

Akinnikawe, Oyewande

2012-10-19T23:59:59.000Z

107

Locating Nearby Sources of Air Pollution by Nonparametric Regression of Atmospheric Concentrations on Wind Direction  

E-Print Network [OSTI]

Locating Nearby Sources of Air Pollution by Nonparametric Regression of Atmospheric Concentrations. #12;1 Locating Nearby Sources of Air Pollution by Nonparametric Regression of Atmospheric. * Corresponding author. Submitted to Atmospheric Environment July, 2001. Abstract The relationship

Washington at Seattle, University of

108

Feedbacks in Emission-Driven and Concentration-Driven Global Carbon Budgets  

Science Journals Connector (OSTI)

Emissions of CO2 into the atmosphere affect the carbon budgets of the land and ocean as biogeochemical processes react to increased CO2 concentrations. Biogeochemical processes also react to changes in temperature and other climate parameters. ...

G. J. Boer; V. K. Arora

2013-05-01T23:59:59.000Z

109

NETL: Carbon Storage - CO2 Utilization Focus Area  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

CO2 Utilization CO2 Utilization Carbon Storage CO2 Utilization Focus Area Carbon dioxide (CO2) utilization efforts focus on pathways and novel approaches for reducing CO2 emissions by developing beneficial uses for the CO2 that will mitigate CO2 emissions in areas where geologic storage may not be an optimal solution. CO2 can be used in applications that could generate significant benefits. It is possible to develop alternatives that can use captured CO2 or convert it to useful products such chemicals, cements, or plastics. Revenue generated from the utilized CO2 could also offset a portion of the CO2 capture cost. Processes or concepts must take into account the life cycle of the process to ensure that additional CO2 is not produced beyond what is already being removed from or going into the atmosphere. Furthermore, while the utilization of CO2 has some potential to reduce greenhouse gas emissions to the atmosphere, CO2 has certain disadvantages as a chemical reactant. Carbon dioxide is rather inert and non-reactive. This inertness is the reason why CO2 has broad industrial and technical applications. Each potential use of CO2 has an energy requirement that needs to be determined; and the CO2 produced to create the energy for the specific utilization process must not exceed the CO2 utilized.

110

Atmospheric Mercury Concentrations Near Salmon Falls Creek Reservoir - Phase 1  

SciTech Connect (OSTI)

Elemental and reactive gaseous mercury (EGM/RGM) were measured in ambient air concentrations over a two-week period in July/August 2005 near Salmon Falls Creek Reservoir, a popular fishery located 50 km southwest of Twin Falls, Idaho. A fish consumption advisory for mercury was posted at the reservoir in 2002 by the Idaho Department of Health and Welfare. The air measurements were part of a multi-media (water, sediment, precipitation, air) study initiated by the Idaho Department of Environmental Quality and the U.S. Environmental Protection Agency (EPA) Region 10 to identify potential sources of mercury contamination to the reservoir. The sampling site is located about 150 km northeast of large gold mining operations in Nevada, which are known to emit large amounts of mercury to the atmosphere (est. 2,200 kg/y from EPA 2003 Toxic Release Inventory). The work was co-funded by the Idaho National Laboratorys Community Assistance Program and has a secondary objective to better understand mercury inputs to the environment near the INL, which lies approximately 230 km to the northeast. Sampling results showed that both EGM and RGM concentrations were significantly elevated (~ 30 70%, P<0.05) compared to known regional background concentrations. Elevated short-term RGM concentrations (the primary form that deposits) were likely due to atmospheric oxidation of high EGM concentrations, which suggests that EGM loading from upwind sources could increase Hg deposition in the area. Back-trajectory analyses indicated that elevated EGM and RGM occurred when air parcels came out of north-central and northeastern Nevada. One EGM peak occurred when the air parcels came out of northwestern Utah. Background concentrations occurred when the air was from upwind locations in Idaho (both northwest and northeast). Based on 2003 EPA Toxic Release Inventory data, it is likely that most of the observed peaks were from Nevada gold mine sources. Emissions from known large natural mercury sources in that area cannot account for the observed EGM peaks due to their diffuse source geometry and the large (170 km) transport distance involved. The EGM peak originating from northwestern Utah air may be from three known mercury sources west of Salt Lake City (Kennecott, US Magnesium, Clean Harbors Aragonite) and/or the 1600 MW coal-fired Intermountain Power plant near Delta. However, the relative importance of these short-term peaks for long-term watershed mercury loading (critical factor affecting fish concentrations) is not known, and there is a need to better quantify the annual frequency and magnitude of these different inputs over a longer period of time.

M. L. Abbott

2005-10-01T23:59:59.000Z

111

A Vehicular Wireless Sensor Network for CO2 Monitoring  

E-Print Network [OSTI]

the concentration of carbon dioxide (CO2) gas in areas of interest. The reported data are sent to a server, which the concentration of carbon dioxide (CO2) gas in areas of interest. CO2 gas is a critical index of air qualityA Vehicular Wireless Sensor Network for CO2 Monitoring Shu-Chiung Hu1, You-Chiun Wang1, Chiuan

Tseng, Yu-Chee

112

Formation Damage due to CO2 Sequestration in Saline Aquifers  

E-Print Network [OSTI]

Carbon dioxide (CO2) sequestration is defined as the removal of gas that would be emitted into the atmosphere and its subsequent storage in a safe, sound place. CO2 sequestration in underground formations is currently being considered to reduce...

Mohamed, Ibrahim Mohamed 1984-

2012-10-25T23:59:59.000Z

113

E-Print Network 3.0 - atmospheric carbon isotope Sample Search...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

of terrestrial ecosystems to rising Summary: to rising concentrations of atmospheric carbon dioxide (CO2 ), and the resulting global changes,are still... from the...

114

A shallow subsurface controlled release facility in Bozeman, Montana, USA, for testing near surface CO2 detection techniques and transport models  

SciTech Connect (OSTI)

A facility has been constructed to perform controlled shallow releases of CO2 at flow rates that challenge near surface detection techniques and can be scalable to desired retention rates of large scale CO2 storage projects. Preinjection measurements were made to determine background conditions and characterize natural variability at the site. Modeling of CO2 transport and concentration in saturated soil and the vadose zone was also performed to inform decisions about CO2 release rates and sampling strategies. Four releases of CO2 were carried out over the summer field seasons of 2007 and 2008. Transport of CO2 through soil, water, plants, and air was studied using near surface detection techniques. Soil CO2 flux, soil gas concentration, total carbon in soil, water chemistry, plant health, net CO2 flux, atmospheric CO2 concentration, movement of tracers, and stable isotope ratios were among the quantities measured. Even at relatively low fluxes, most techniques were able to detect elevated levels of CO2 in the soil, atmosphere, or water. Plant stress induced by CO2 was detectable above natural seasonal variations.

Spangler, Lee H.; Dobeck, Laura M.; Repasky, Kevin S.; Nehrir, Amin R.; Humphries, Seth D.; Barr, Jamie L.; Keith, Charlie J.; Shaw, Joseph A.; Rouse, Joshua H.; Cunningham, Alfred B.; Benson, Sally M.; Oldenburg, Curtis M.; Lewicki, Jennifer L.; Wells, Arthur W.; Diehl, J. R.; Strazisar, Brian; Fessenden, Julianna; Rahn, Thom A.; Amonette, James E.; Barr, Jonathan L.; Pickles, William L.; Jacobson, James D.; Silver, Eli A.; Male, Erin J.; Rauch, Henry W.; Gullickson, Kadie; Trautz, Robert; Kharaka, Yousif; Birkholzer, Jens; Wielopolski, Lucien

2010-03-01T23:59:59.000Z

115

Transcriptome-Wide Changes in Chlamydomonas reinhardtii Gene Expression Regulated by Carbon Dioxide and the CO2-Concentrating Mechanism Regulator CIA5/CCM1  

Science Journals Connector (OSTI)

...microalgae because of the poor solubility and diffusion rate of CO2 in water and the critical importance...to 152 ppm). Selection of gas flow lines and position on...Nar1 gene family by carbon and nitrogen. Protist 157 : 421-433...

Wei Fang; Yaqing Si; Stephen Douglass; David Casero; Sabeeha S. Merchant; Matteo Pellegrini; Istvan Ladunga; Peng Liu; Martin H. Spalding

2012-05-25T23:59:59.000Z

116

A Novel CO2 Separation System  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Novel CO Novel CO 2 Separation System Robert J. Copeland (copeland@tda.com 303-940-2323) Gokhan Alptekin (galtpekin@tda.com 303 940-2349) Mike Cesario (czar@tda.com 303-940-2336) Yevgenia Gershanovich (ygershan@tda.com 303-940-2346) TDA Research, Inc. 12345 West 52 nd Avenue Wheat Ridge, Colorado 80033-1917 Project Summary NEED Concern over global climate change has led to a need to reduce CO 2 emissions from power plants. Unfortunately, current CO 2 capture processes reduce the efficiency with which fuel can be converted to electricity by 9-37%, and CO 2 capture costs can exceed $70 per tonne 1 of CO 2 (Herzog, Drake, and Adams 1997). OBJECTIVE To generate electricity with little reduction in conversion efficiency while emitting little or no CO 2 to the atmosphere, TDA Research, Inc. (TDA) is developing a Novel CO

117

CO2 Sequestration in Basalt Formations  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

CO CO 2 SequeStratiOn in BaSalt FOrmatiOnS Background There is growing concern that buildup of greenhouse gases, especially carbon dioxide (CO 2 ), in the atmosphere is contributing to global climate change. One option for mitigating this effect is to sequester CO 2 in geologic formations. Numerous site assessments for geologic sequestration of CO 2 have been conducted in virtually every region of the United States. For the most part, these studies have involved storing CO 2 in saline formation, deep coal seams, and depleted oil and gas reservoirs. Another option, however, is basalt formations. Basalt is a dark-colored, silica-rich, volcanic rock that contains cations-such as calcium, magnesium, and iron-that can combine with CO 2 to form carbonate minerals. Basalt formations have not received much

118

Assessing methane oxidation under landfill covers and its contribution to the above atmospheric CO2 levels: The added value of the isotope  

E-Print Network [OSTI]

biogas fluxes, which was expected in clay covers presenting fissures, through which CH4 is rapidly transported. At shallow depth, more immobile biogas pockets show a higher level of CH4 oxidation., 1998). The main com- ponents of biogas are CH4 (50­60%) and carbon dioxide (CO2; 40­50%). A major

119

What CO2 well gases tell us about the origin of noble gases in the mantle and their relationship to the atmosphere  

Science Journals Connector (OSTI)

...mantle-rich CO2 well gases, with samples lying on the air-solar mixing line. The most solar-rich gas, from Bravo Dome in New Mexico, had a 10 per cent excess above air value. Since solar and Q-Xe are so similar in composition, it is not possible...

2008-01-01T23:59:59.000Z

120

The CO2 Reforming of Natural Gas in a Pulsed Corona Discharge Reactor  

Science Journals Connector (OSTI)

The conversion of CO 2 and (CH 4+CO 2 ) mixtures to CO, at room temperature and atmospheric pressure conditions, in...

M. A. Malik; X. Z. Jiang

1999-12-01T23:59:59.000Z

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


121

Geologic CO2 Sequestration  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Geologic CO2 Sequestration Geologic CO2 Sequestration Geologic reservoirs offer promising option for long- term storage of captured CO 2 Accumulations of gases (including CO 2 ) in geologic reservoirs, by natural processes or through enhanced oil recovery operations, demonstrate that gas can be stored for long periods of time and provide insights to the efficacy and impacts of geological gas storage. Los Alamos scientists in the Earth and Environmental Sciences (EES) Division have been involved in geologic CO 2 storage research for over a decade. Research Highlights * Led first-ever US field test on CO 2 sequestration in depleted oil reservoirs * Participant in two Regional Carbon Sequestration Partnerships (Southwest Regional and Big Sky) * Part of the National Risk Assessment Partnership (NRAP) for CO

122

Is CO2 an Indoor Pollutant? Direct Effects of Low-to-Moderate CO2  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Is CO2 an Indoor Pollutant? Direct Effects of Low-to-Moderate CO2 Is CO2 an Indoor Pollutant? Direct Effects of Low-to-Moderate CO2 Concentrations on Human Decision-Making Performance Title Is CO2 an Indoor Pollutant? Direct Effects of Low-to-Moderate CO2 Concentrations on Human Decision-Making Performance Publication Type Journal Article Refereed Designation Refereed LBNL Report Number LBNL-6196E Year of Publication 2012 Authors Satish, Usha, Mark J. Mendell, Krishnamurthy Shekhar, Toshifumi Hotchi, Douglas P. Sullivan, Siegfried Streufert, and William J. Fisk Journal Environmental Health Perspectives Volume 120 Issue 12 Pagination 1671-1677 Date Published 09/20/2012 Keywords carbon dioxide, cognition, Decision Making, human performance, indoor environmental quality, ventilation Abstract Background - Associations of higher indoor carbon dioxide (CO2) concentrations with impaired

123

Response of a Coupled OceanAtmosphere Model to Increasing Atmospheric Carbon Dioxide: Sensitivity to the Rate of Increase  

Science Journals Connector (OSTI)

The influence of differing rates of increase of the atmospheric CO2 concentration on the climatic response is investigated using a coupled oceanatmosphere model. Five transient integrations are performed each using a different constant ...

Ronald J. Stouffer; Syukuro Manabe

1999-08-01T23:59:59.000Z

124

EMSL - CO2 sequestration  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

co2-sequestration en Low-Temperature Carbon Monoxide Oxidation Catalysed by Regenerable Atomically Dispersed Palladium on Alumina. http:www.emsl.pnl.govemslwebpublications...

125

Uncertainty in Contaminant Concentration Fields Resulting from Atmospheric Boundary Layer Depth Uncertainty  

Science Journals Connector (OSTI)

The relationship between atmospheric boundary layer (ABL) depth uncertainty and uncertainty in atmospheric transport and dispersion (ATD) simulations is investigated by examining profiles of predicted concentrations of a contaminant. Because ...

Brian P. Reen; Kerrie J. Schmehl; George S. Young; Jared A. Lee; Sue Ellen Haupt; David R. Stauffer

2014-11-01T23:59:59.000Z

126

Time dependences of atmospheric Carbon dioxide fluxes  

E-Print Network [OSTI]

Understanding the lifetime of CO2 in the atmosphere is critical for predictions regarding future climate changes. A simple mass conservation analysis presented here generates tight estimations for the atmosphere's retention time constant. The analysis uses a leaky integrator model that combines the observed deficit (only less than 40% of CO2 produced from combustion of fossil fuels is actually retained in the atmosphere, while more than 60% is continuously shed) with the exponential growth of fossil fuel burning. It reveals a maximum characteristic time of less than 23 year for the transfer of atmospheric CO2 to a segregation sink. This time constant is further constrained by the rapid disappearance of 14C after the ban of atmospheric atomic bomb tests, which provides a lower limit of 18 years for this transfer. The study also generates evaluations of other CO2 fluxes, exchange time constants and volumes exchanged. Analysis of large harmonic oscillations of atmospheric CO2 concentration, often neglected in th...

DeSalvo, Riccardo

2014-01-01T23:59:59.000Z

127

BNL | CO2 Laser  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

CO2 Laser CO2 Laser The ATF is one of the only two facilities worldwide operating picosecond, terawatt-class CO2 lasers. Our laser system consists of a picoseconds pulse-injector based on fast optical switching from the output of a conventional CO2 laser oscillator, and a chain of high-pressure laser amplifiers. It starts with a wavelength converter wherein a near-IR picosecond solid-state laser with l»1 μm produces a mid-IR 10-μm pulse. This process employs two methods; semiconductor optical switching, and the Kerr effect. First, we combine the outputs from a multi-nanosecond CO2 laser oscillator with a picosecond Nd:YAG laser on a germanium Brewster-plate to produce an ~200 ps, 10μm pulse by semiconductor optical switching. Co-propagating this pulse with a Nd:YAG's 2nd harmonic in a

128

Enhancement of CO2/N2 selectivity in a metal-organic framework by cavity modification  

E-Print Network [OSTI]

electricity is a major source of CO2 in the atmosphere, but the capture and sequestration of CO2 from flue gas two-thirds), CO2, water vapor, oxygen, and minor components such as carbon monoxide, nitrogen oxides

129

In Situ Delta-13 CO2 from Cape Grim, Tasmania, Australia: 1982-1993  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

In Situ δ13CO2 from Cape In Situ δ13CO2 from Cape Grim, Australia In Situ δ13CO2 from Cape Grim, Tasmania, Australia: 1982-1993 graphics Graphics data Data Investigators R.J. Francey and C.E. Allison CSIRO, Division of Atmospheric Research, Private Bag No. 1, Mordialloc, Victoria, Australia 3195 Period of Record 1982-1993 Methods Air samples are collected during baseline condition episodes at a frequency of around one sample per week. Baseline conditions are characterized by wind direction in the sector 190-280°, condensation nucleus concentration below 600 cm3, and steady, continuous CO2 concentrations (variation + 0.2 ppmv per hour). The Cape Grim in situ extraction line is based on 3 high-efficiency glass U-tube traps with internal cooling coils. A vacuum pump draws air from either the 10 m or 70 m intakes, and sampling

130

Steam Gasification of Coal at Low?Medium (600?800 C) Temperature with Simultaneous CO2 Capture in a Bubbling Fluidized Bed at Atmospheric Pressure. 2. Results and Recommendations for Scaling Up  

Science Journals Connector (OSTI)

Steam Gasification of Coal at Low?Medium (600?800 C) Temperature with Simultaneous CO2 Capture in a Bubbling Fluidized Bed at Atmospheric Pressure. ... Once the existence of segregation in the bed of the gasifier with the particles' sizes used for coal and for the CaO in the preliminary tests are confirmed and analyzed, the particle size of the coal was increased to 0.4?2.0 ... In general small differences in d. readily lead to segregation while quite differently sized particles are fairly easily mixed. ...

Jose Corella; Jose M. Toledo; Gregorio Molina

2008-02-15T23:59:59.000Z

131

Vegetation Response to CO2 and Climate  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Vegetation Response to CO2 and Climate Vegetation Response to CO2 and Climate Area and Carbon Content of Sphagnum Since Last Glacial Maximum (2002) TDE Model Intercomparison Project Data Archive Presentations and abstracts from the recent DOE Terrestrial Science Team Meeting (Argonne National Laboratory, October 29-31, 2001) FACE (Free-Air CO2 Enrichment) Walker Branch Throughfall Displacement Experiment Data Report: Site Characterization, System Performance, Weather, Species Composition, and Growth (2001), NDP-078A | PDF Bibliography on CO2 Effects on Vegetation and Ecosystems: 1990-1999 Literature (2000), CDIAC-129 Direct effects of atmospheric CO2 enrichment on plants and ecosystems: An updated bibliographic data base (1994), CDIAC-70 A Database of Herbaceous Vegetation Responses to Elevated

132

E-Print Network 3.0 - atmospheric krypton-85 concentrations Sample...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Geosciences Union Atmospheric Chemistry and Physics Characterization of aerosol... -shale-burning industrial areas. Ion chro- matography analysis showed that concentrations of...

133

Two-Temperature Two-Dimensional Non Chemical Equilibrium Modeling of ArCO2H2 Induction Thermal Plasmas at Atmospheric Pressure  

Science Journals Connector (OSTI)

Here the authors developed a two-dimensional two-temperature chemical non-equilibrium (2T-NCE) model of Ar...2H2 inductively coupled thermal plasmas (ICTP) around atmospheric pressure (760torr). Assuming 22 di...

Sharif Abdullah Al-Mamun; Yasunori Tanaka

2010-02-01T23:59:59.000Z

134

Atmospheric Environment 34 (2000) 2851}2863 Resolution of pollutant concentrations in the boundary layer  

E-Print Network [OSTI]

Atmospheric Environment 34 (2000) 2851}2863 Resolution of pollutant concentrations in the boundary 1999 Abstract This paper investigates the solution of a 3D atmospheric dispersion problem using a time to solve the atmospheric di!usion equation. Preliminary studies of dispersion from a single source

Utah, University of

135

ARM - Datastreams - 30co2flx4mmet  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

mmet mmet Documentation Data Quality Plots Citation DOI: 10.5439/1025037 [ What is this? ] Generate Citation ARM Data Discovery Browse Data Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Datastream : 30CO2FLX4MMET Eddy Correlation CO2 Flux Data: 4 m samples, meteorological data, 30-min stats Active Dates 2002.12.18 - 2013.01.27 Measurement Categories Atmospheric Carbon, Atmospheric State, Radiometric, Surface Properties Originating Instrument Carbon Dioxide Flux Measurement Systems (CO2FLX) Measurements The measurements below provided by this product are those considered scientifically relevant. Measurement Variable Atmospheric turbulence Lmoni Atmospheric pressure bar_pres CO2 flux fc_corr CO2 flux fc_wpl_h CO2 flux fc_wpl_le Sensible heat flux

136

Synthesis, characterization and performance of single-component CO2-binding organic liquids (CO2BOL) for post combustion CO2 capture  

SciTech Connect (OSTI)

Carbon dioxide (CO2) emission to the atmosphere will increase significantly with the shift to coal powered plants for energy generation. This increase in CO2 emission will contribute to climate change. There is need to capture and sequester large amounts of CO2 emitted from these coal power plants in order to mitigate the environmental effects. Here we report the synthesis, characterization and system performance of multiple third generation CO2 binding organic liquids (CO2BOLs) as a solvent system for post combustion gas capture. Alkanolguanidines and alkanolamidines are single component CO2BOLs that reversibly bind CO2 chemically as liquid zwitterionic amidinium / guanidinium alkylcarbonates. Three different alkanolguanidines and alkanolamidines were synthesized and studied for CO2 capacity and binding energetics. Solvent performance of these three CO2BOLs was evaluated by batch-wise CO2 uptake and release over multiple cycles. Synthesis of CO2BOLs, characterization, CO2 uptake, selectivity towards CO2 as well as solvent tolerance to water will be discussed.

Koech, Phillip K.; Heldebrant, David J.; Rainbolt, James E.; Zheng, Feng; Smurthwaite, Tricia D.

2010-03-31T23:59:59.000Z

137

CO2 maritime transportation  

Science Journals Connector (OSTI)

The objective of this study is to describe the complete transport chain of CO2 between capture and storage including a ship transport. This last one is composed by the following steps: Shore terminal including the liquefaction, temporary storage and CO2 loading. Ship with a capacity of 30,000m3. On or off shore terminal including an unloading system, temporary storage and export towards the final storage. Between all the possible thermodynamic states, the liquid one is most relevant two options are compared in the study (?50C, 7bar) and (?30C, 15bar). The ship has an autonomy of 6 days, is able to cover 1000km with a cargo of 2.5Mt/year. Several scenarios are studied varying the geographical position of the CO2 source, the number of harbours and the way the CO2 is finally stored. Depending on the option, the transport cost varies from 24 to 32/tCO2. This study confirms the conclusion of a previous study supported by ADEME, the cost transport is not negligible regarding the capture one when ships are considered. Transport by ship becomes a more economical option compared with an off shore pipeline when the distance exceeds 350km and with an onshore pipeline when it exceeds 1100km.

Sandrine Decarre; Julien Berthiaud; Nicolas Butin; Jean-Louis Guillaume-Combecave

2010-01-01T23:59:59.000Z

138

The Effects of CO2 Disposal on Marine Nitrification Processes  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Effects of CO Effects of CO 2 Disposal on Marine Nitrification Processes Michael H. Huesemann (michael.huesemann@pnl.gov, 360-681-3618) Pacific Northwest National Laboratory - Marine Sciences Laboratory 1529 West Sequim Bay Road Sequim, WA 98382 Ann D. Skillman (ann.skillman@pnl.gov, 360-681-3649) Pacific Northwest National Laboratory - Marine Sciences Laboratory 1529 West Sequim Bay Road Sequim, WA 98382 Eric A. Crecelius (eric.crecelius@pnl.gov, 360-681-3604) Pacific Northwest National Laboratory - Marine Sciences Laboratory 1529 West Sequim Bay Road Sequim, WA 98382 Abstract In an attempt to reduce the threat of global warming, it has been proposed that the rise of atmospheric carbon dioxide concentrations be reduced by the ocean disposal of CO 2 from the flue gases of fossil fuel-fired power plants. The release of large amounts of

139

Long-time evolution of sequestered CO$_2$ in porous media  

E-Print Network [OSTI]

CO$_2$ sequestration in subsurface reservoirs is important for limiting atmospheric CO$_2$ concentrations. However, a complete physical picture able to predict the structure developing within the porous medium is lacking. We investigate theoretically reactive transport in the long-time evolution of carbon in the brine-rock environment. As CO$_2$ is injected into a brine-rock environment, a carbonate-rich region is created amid brine. Within the carbonate-rich region minerals dissolve and migrate from regions of high concentration to low concentration, along with other dissolved carbonate species. This causes mineral precipitation at the interface between the two regions. We argue that precipitation in a small layer reduces diffusivity, and eventually causes mechanical trapping of the CO$_2$. Consequently, only a small fraction of the CO$_2$ is converted to solid mineral; the remainder either dissolves in water or is trapped in its original form. We also study the case of a pure CO$_2$ bubble surrounded by bri...

Cohen, Yossi

2014-01-01T23:59:59.000Z

140

A superstructure-based optimal synthesis of PSA cycles for post-combustion CO2 capture  

SciTech Connect (OSTI)

Recent developments have shown pressure/vacuum swing adsorption (PSA/VSA) to be a promising option to effectively capture CO2 from flue gas streams. In most commercial PSA cycles, the weakly adsorbed component in the mixture is the desired product, and enriching the strongly adsorbed CO2 is not a concern. On the other hand, it is necessary to concentrate CO2 to high purity to reduce CO2 sequestration costs and minimize safety and environmental risks. Thus, it is necessary to develop PSA processes specifically targeted to obtain pure strongly adsorbed component. A multitude of PSA/VSA cycles have been developed in the literature for CO2 capture from feedstocks low in CO2 concentration. However, no systematic methodology has been suggested to develop, evaluate, and optimize PSA cycles for high purity CO2 capture. This study presents a systematic optimization-based formulation to synthesize novel PSA cycles for a given application. In particular, a novel PSA superstructure is presented to design optimal PSA cycle configurations and evaluate CO2 capture strategies. The superstructure is rich enough to predict a number of different PSA operating steps. The bed connections in the superstructure are governed by time-dependent control variables, which can be varied to realize most PSA operating steps. An optimal sequence of operating steps is achieved through the formulation of an optimal control problem with the partial differential and algebraic equations of the PSA system and the cyclic steady state condition. Large-scale optimization capabilities have enabled us to adopt a complete discretization methodology to solve the optimal control problem as a largescale nonlinear program, using the nonlinear optimization solver IPOPT. The superstructure approach is demonstrated for case studies related to post-combustion CO2 capture. In particular, optimal PSA cycles were synthesized, which maximize CO2 recovery for a given purity, and minimize overall power consumption. The results show the potential of the superstructure to predict PSA cycles with up to 98% purity and recovery of CO2. Moreover, for recovery of around 85% and purity of over 90%, these cycles can recover CO2 from atmospheric flue gas with a low power consumption of 465 kWh tonne#1;1 CO2. The approach presented is, therefore, very promising and quite useful for evaluating the suitability of different adsorbents, feedstocks, and operating strategies for PSA, and assessing its usefulness for CO2 capture.

Agarwal, A.; Biegler, L.; Zitney, S.

2010-07-01T23:59:59.000Z

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


141

Enhanced transfer of terrestrially derived carbon to the atmosphere in a flooding event  

E-Print Network [OSTI]

November 2012; revised 14 October 2012; accepted 21 November 2012. [1] Rising CO2 concentration the adjacent shelf contributed to northern Gulf shelf waters changing from a net sink to a net source of CO2 in the water can be exchanged with the atmosphere with approximately ~100 Tg of CO2 degassed from U.S. streams

Grossman, Ethan L.

142

Experimental trial of a hollow-core waveguide used as an absorption cell for concentration measurement of NH3 gas with a CO2 laser  

Science Journals Connector (OSTI)

The basic idea of using a hollow-core waveguide as an absorption cell in a spectroscopic gas measurement system is proposed. Measurements of NH3 gas concentration were made...

Saito, Yasunori; Kanaya, Tatsunori; Nomura, Akio; Kano, Tetsuo

1993-01-01T23:59:59.000Z

143

NETL: CO2 Emissions Control  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Home > Technologies > Coal & Power Systems > Innovations for Existing Plants > CO2 Emissions Control Home > Technologies > Coal & Power Systems > Innovations for Existing Plants > CO2 Emissions Control Innovations for Existing Plants CO2 Emissions Control RD&D Roadmap Technology Update DOE/NETL Advanced CO2 Capture R&D Program: Technology Update DOE/NETL Advanced CO2 Capture R&D Program Accomplishments DOE/NETL Carbon Dioxide Capture and Storage RD&D Roadmap 2013 NETL CO2 Capture Technology Meeting Presentations DOE/NETL's Monthly Carbon Sequestration Newsletter Program Goals and Targets Pre-Combustion CO2 Control Post-Combustion CO2 Control Advanced Combustion CO2 Compression Other Systems Analysis Regulatory Drivers Reference Shelf Carbon capture involves the separation of CO2 from coal-based power plant flue gas or syngas. There are commercially available 1st-Generation CO2

144

Efficiency of Sequestrating CO2 in the Ocean  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Efficiency of Sequestrating CO Efficiency of Sequestrating CO 2 in the Ocean Richard Dewey (RDewey@uvic.ca ; 250-472-4009) University of Victoria, P.O. Box 3055, Victoria BC Canada V8N 3P6 Gilbert Stegen (Dr_Stegen@hotmail.com ; 425-869-7236) SAIC and GRS Associates 17257 NE 116 th St., Redmond WA USA 98052 Abstract Ocean disposal of CO 2 continues to be of great interest as a possible mitigation strategy for reducing atmospheric emissions of anthropogenic CO 2 . The ocean, and ultimately ocean sediments, naturally represents the single largest sink of CO 2 , and annually sequesters several gigatons of carbon from the atmosphere. The injection of additional CO 2 to artificially accelerate the use of the ocean as a sink for atmospheric CO 2 and avoid a short-term build-up of greenhouse gases has been investigated for

145

Reply to "Comment on 'Falsification Of The Atmospheric CO2 Greenhouse Effects Within The Frame Of Physics' by Joshua B. Halpern, Christopher M. Colose, Chris Ho-Stuart, Joel D. Shore, Arthur P. Smith, J\\"org Zimmermann"  

E-Print Network [OSTI]

It is shown that the notorious claim by Halpern et al. recently repeated in their comment that the method, logic, and conclusions of our "Falsification Of The CO2 Greenhouse Effects Within The Frame Of Physics" would be in error has no foundation. Since Halpern et al. communicate our arguments incorrectly, their comment is scientifcally vacuous. In particular, it is not true that we are "trying to apply the Clausius statement of the Second Law of Thermodynamics to only one side of a heat transfer process rather than the entire process" and that we are "systematically ignoring most non-radiative heat flows applicable to Earth's surface and atmosphere". Rather, our falsification paper discusses the violation of fundamental physical and mathematical principles in 14 examples of common pseudo-derivations of fictitious greenhouse effects that are all based on simplistic pictures of radiative transfer and their obscure relation to thermodynamics, including but not limited to those descriptions (a) that define a "Pe...

Gerlich, Gerhard; 10.1142/S0217979210055573

2010-01-01T23:59:59.000Z

146

Vehicular Sensing System for CO2 Monitoring Applications  

E-Print Network [OSTI]

--We are interested in monitoring the concentration of carbon dioxide (CO2) gas in a large field such as an urban area sensor, vehicular sensing system, wireless sensor network. I. INTRODUCTION Carbon dioxide (CO2) gas has1 Vehicular Sensing System for CO2 Monitoring Applications Shu-Chiung Hu, You-Chiun Wang, Chiuan

Tseng, Yu-Chee

147

E-Print Network 3.0 - atmospheric oxygen concentration Sample...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

< 1 2 3 4 5 > >> 1 Sulfur and oxygen isotope composition of the atmosphere in Saxony (Germany) Tichomirowa et al. Summary: Conclusions Mean SO2 concentrations in 2003 12;Sulfur...

148

Synthesis of Scrub-Oak Ecosystem Responses to Elevated CO2  

SciTech Connect (OSTI)

This report summarizes a synthesis project of a long-term global change experiment conducted at the Kennedy Space Center, Florida, investigating how increasing concentrations of atmospheric carbon dioxide (CO2) influences the functioning of a fire-dominated scrub-oak ecosystem. The experiment began in 1996 and ended in 2007. Results presented here summarize the effects of elevated CO2 on plant growth, soil processes, carbon and nutrient cycling, and other responses. Products include archived data from the experiment, as well as six publications in the peer-reviewed literature.

Hungate, Bruce

2014-11-07T23:59:59.000Z

149

Optimal synthesis of a pressure swing adsorption process for CO2 capture  

SciTech Connect (OSTI)

The emission of carbon dioxide from cement industry and power plants that burn fossil fuels is the major cause for the accumulation of CO2 in the atmosphere, which causes long-range environmental problems. One option to mitigate the emission of CO2 is to capture it from the emission sources and store it to the ocean or depleted oil field or use it for enhanced oil recovery. CO2 recovery has been achieved by gas absorption employing solutions of carbonates and alkanolamines. However, this process is energy-intensive for the regeneration of solvent and also faces problems due to corrosion. Recently, the pressure swing adsorption (PSA) process has been considered as an alternative to the absorption process. PSA processes have been widely applied for the removal of CO2 from various feed mixtures, such as CO2 in the steam reformer off gas, landfill gas and natural gas. In all these commercial PSA cycles, the weakly adsorbed component in the mixture is the desired product and enriching the strongly adsorbed CO2 is not a concern. On the other hand, for the capture of CO2 for sequestration, it is necessary to concentrate the CO2 to a high purity to reduce the compression and transportation cost. Thus, it is necessary to develop a PSA cycle by which a high-purity product for the strongly adsorbed component with a high recovery is obtained. A multitude of PSA cycles and adsorbents have been developed for producing highly pure heavy component (CO2) from feedstock with low CO2 concentration. Kikkinides et al. suggested a 4-bed 4-step process with activated carbon as the sorbent and could recover 68% of CO2 at 99.997% purity. Chue et al. compared activated carbon and zeolite 13X on a 3-bed 7-step process and concluded that the latter is better than the former for CO2 recovery. However, the CO2 recovery was low in their process due to the lack of a countercurrent step in the chosen cycle. Choi et al. reported more than 70% CO2 recovery at more than 90% purity for a modified 3-bed 7-step cycle. However, they solved a very small two variable optimization problem, thus being a specialized case. Zhang et al. have given justifications for using a specific cyclic component step in the adsorption cycle in the context of CO2 capture by using a simplistic mathematical model for the PSA process. Reynolds et al. have suggested a variety of stripping PSA cycles for CO2 recovery at high temperature using a hydrotalcite-like adsorbent. In this study, a two-bed superstructure of the PSA process has been developed to optimally synthesize an appropriate cycle for CO2 capture. The superstructure considers all the possible operating steps in a PSA cycle with two beds. An optimal control problem with a PDE-based model for PSA system has been formulated in which different steps within a cycle are realized with the help of control variables changing with time. The optimization problem has been solved for three different cases of maximizing CO2 recovery (for a given purity), maximizing feed throughput and minimizing specific power (for a given level of CO2 purity and recovery). Current results indicate the superstructure-based approach as a promising technique for deriving optimal PSA cycles. Different cases with different number of control variables indicate convergence to a particular kind of PSA cycle with over 99% purity and recovery of CO2. The results obtained from optimization problem will also be compared with the optimal PSA cycle simulated more accurately in a dynamic simulation environment.

Agarwal, A.; Biegler, L.; Zitney, S.

2008-01-01T23:59:59.000Z

150

Energy consumption analysis for CO2 separation from gas mixtures  

Science Journals Connector (OSTI)

Abstract CO2 separation is an energy intensive process, which plays an important role in both energy saving and CO2 capture and storage (CCS) implementation to deal with global warming. To quantitatively investigate the energy consumption of CO2 separation from different CO2 streams and analyze the effect of temperature, pressure and composition on energy consumption, in this work, the theoretical energy consumption of CO2 separation from flue gas, lime kiln gas, biogas and bio-syngas was calculated. The results show that the energy consumption of CO2 separation from flue gas is the highest and that from biogas is the lowest, and the concentration of CO2 is the most important factor affecting the energy consumption when the CO2 concentration is lower than 0.15 in mole fraction. Furthermore, if the CO2 captured from flue gases in CCS was replaced with that from biogases, i.e. bio-CO2, the energy saving would be equivalent to 7.31 million ton standard coal for China and 28.13 million ton standard coal globally, which corresponds to 0.30 billion US$ that can be saved for China and 1.36 billion US$ saved globally. This observation reveals the importance of trading fossil fuel-based CO2 with bio-CO2.

Yingying Zhang; Xiaoyan Ji; Xiaohua Lu

2014-01-01T23:59:59.000Z

151

Novel CO2 - Philic Absorbents  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Novel Co Novel Co 2 - PhiliC AbsorbeNts Summary The ability to separate a high pressure mixture of CO 2 and H 2 such that a high pressure stream of CO 2 for sequestration and a high pressure stream of H 2 for energy are produced remains an elusive goal. This research has identified a class of compounds that melt in the presence of high pressure CO 2 , forming a liquid phase composed of roughly 50wt% CO 2 and 50wt% of the compound. Unlike conventional solvents that require substantial depressurization during regeneration to release a low pressure CO 2 stream, these novel compounds completely release the CO 2 at many hundreds of psia as the compound solidifies. This work will reveal whether one of more of these compounds can selectively remove CO 2 from a mixture

152

Hyperspectral Geobotanical Remote Sensing For Co2 Storage Monitoring | Open  

Open Energy Info (EERE)

Hyperspectral Geobotanical Remote Sensing For Co2 Storage Monitoring Hyperspectral Geobotanical Remote Sensing For Co2 Storage Monitoring Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Book: Hyperspectral Geobotanical Remote Sensing For Co2 Storage Monitoring Details Activities (1) Areas (1) Regions (0) Abstract: This project's goal is to develop remote sensing methods for early detection and spatial mapping, over whole regions simultaneously, of any surface areas under which there are significant CO2 leaks from deep underground storage formations. If large amounts of CO2 gas percolated up from a storage formation below to within plant root depth of the surface, the CO2 soil concentrations near the surface would become elevated and would affect individual plants and their local plant ecologies. Excessive soil CO2 concentrations are observed to significantly affect local plant

153

Economic and energetic analysis of capturing CO2 from ambient air  

Science Journals Connector (OSTI)

...the CO 2 from a feed gas. After absorption...concentrated stream of CO 2 gas is produced, with the...purify CO 2 from coal-fired power plant flue gases, where the CO 2 concentration...capture using current-generation capture and compression...

Kurt Zenz House; Antonio C. Baclig; Manya Ranjan; Ernst A. van Nierop; Jennifer Wilcox; Howard J. Herzog

2011-01-01T23:59:59.000Z

154

Satellite vibration measurements with an autodyne CO2 laser radar  

Science Journals Connector (OSTI)

Vibration signatures of the Low Power Atmospheric Compensation Experiment satellite were obtained with a ground-based CO2 laser radar. The laser radar operated in a cw mode...

Schultz, K I; Kocher, D G; Daley, J A; Theriault, J R; Spinks, J; Fisher, S

1994-01-01T23:59:59.000Z

155

Electricity generation from coal with CO2 capture by means of a novel power cycle  

SciTech Connect (OSTI)

Climate modelers have estimated that anthropogenic emissions of CO2 must be reduced substantially from the present rate to stabilize atmospheric concentration. To achieve this, electricity generation from fossil fuels with CO2 capture and direct sequestration may play an important role. If so, it will be worthwhile to consider power cycles that are designed to minimize atmospheric CO2 emissions and deliver CO2 ready for pipeline transport in addition to providing other desirable attributes of environmental performance and efficiency. One such novel approach, named the Matiant cycle, employs self generated CO2 as the working fluid with both Bryton and Rankine cycle turbines. Process modeling studies are being conducted at the NETL to investigate the promise of this cycle. In the work to be reported, synthesis gas is provided to the Matiant cycle by oxygen-blown dry coal entrained gasification. Oxygen for both the gasifier and the Matiant cycle is provided by use of an Ion Transport Membrane (ITM). ITM is a revolutionary approach for producing high purity oxygen from a high temperature pressurized air stream. ASPEC Plus is used as the simulation tool to compute energy balances and system performance. Two flowsheets are analyzed, the difference being the treatment of the low oxygen content raffinate stream from the ITM. Computed thermal efficiencies of the ITM/Matiant cycle are comparable to those of conventional IGCC without carbon capture. Specific carbon emissions per net MWh are many times lower for the new cycle than for other approaches being developed for power generation with CO2 capture, however. As much as 99.5% of the carbon in synthesis gas fed to the Matiant cycle could be recovered and removed in a pipeline as a high pressure liquid. Such high capture efficiencies at large central generating stations could allow use of fossil fuels without capture at smaller installations or by mobile sources, yielding a modest overall rate of CO2 emissions.

Ruether, J.; Le, P.; White, C.

2000-07-01T23:59:59.000Z

156

Screening and Ranking of Hydrocarbon Reservoirs for CO2 Storage in the Alberta Basin, Canada  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Screening and Ranking of Hydrocarbon Reservoirs for CO Screening and Ranking of Hydrocarbon Reservoirs for CO 2 Storage in the Alberta Basin, Canada Stefan Bachu (Stefan.Bachu@gov.ab.ca; 780-427-1517) Alberta Energy and Utilities Board 4999-98 Avenue Edmonton, AB, T6B 2X3, Canada Introduction Human activity since the industrial revolution has had the effect of increasing atmospheric concentrations of gases with a greenhouse effect, such as carbon dioxide (CO 2 ) and methane (CH 4 ), leading to climate warming and weather changes (Bryant, 1997; Jepma and Munasinghe, 1998). Because of its relative abundance compared with the other greenhouse gases, CO 2 is by far the most important, being responsible for about 64% of the enhanced "greenhouse effect" (Bryant, 1997). Given their inherent advantages, such as availability, competitive cost, ease of

157

Quantitative Analysis of CO2 Mitigation in Thai Low Carbon Power Sector towards 2050  

Science Journals Connector (OSTI)

Abstract Recently, Low Carbon Society (LCS) principle has emerged as a practicable campaign for both developing and developed countries to deal with the dramatic increment of greenhouse gas concentration in the atmosphere. Various key features of LCS entail reducing energy demand and consumption while avoiding the fossil fuel utilization which is a major contributor to substantial CO2 emissions. In this study, Thailand's power sector is modeled using Asia-Pacific Integrated Model (AIM/Enduse). The objective of this study is to model the Thai power sector such that the viability of clean generating technologies for Thailand is considered and their mitigating effects are analyzed. The results demonstrate that the fossil fuel based technology would be replaced by clean technologies including, coal-fired power plant with CCS technology and renewable energies in the LCS scenario. The LCS scenario can mitigate CO2 emissions by 58,098 ktCO2 in 2050 when compared to BAU scenario.

P. Chunark; K. Promjiraprawat; P. Winyuchakrit; B. Limmeechokchai; T. Masui; T. Hanaoka; Y. Matsuoka

2014-01-01T23:59:59.000Z

158

Analysis of Hydroxide Sorbents for CO2 Capture from Warm Syngas  

Science Journals Connector (OSTI)

Analysis of Hydroxide Sorbents for CO2 Capture from Warm Syngas ... (1, 2) However, conventional coal combustion releases large amounts of the greenhouse gas CO2 into the atmosphere. ...

David J. Couling; Ujjal Das; William H. Green

2012-09-04T23:59:59.000Z

159

Adsorption separation of CO2 from simulated flue gas mixtures by novel CO2 ''molecular basket'' adsorbents  

Science Journals Connector (OSTI)

Adsorption separation of CO2 from simulated flue gas mixtures containing CO2, O2, and N2 by using a novel CO2 ''molecular basket'' adsorbent was investigated in a flow adsorption separation system. The novel CO2 ''molecular basket'' adsorbents were developed by synthesising mesoporous molecular sieve MCM-41 and modifying it with polyethylenimine (PEI). The influence of operation conditions, including feed flow rate, temperature, feed CO2 concentration, and sweep gas flow rate, on the CO2 adsorption/desorption separation performance and CO2 breakthrough were examined. The CO2 adsorption capacity was 91.0 ml (STP)/g-PEI, which was 27 times higher than that of the MCM-41 alone. Further, the adsorbent showed separation selectivity of greater than 1000 for CO2/N2 ratio and approximately 180 for CO2/O2, which are significantly higher than those of the MCM-41, zeolites, and activated carbons. Cyclic adsorption/desorption measurements showed that the CO2 ''molecular basket'' adsorbent was stable at 75°C. However, the CO2 ''molecular basket'' adsorbent was not stable when the operation temperature was higher than 100C.

Xiaochun Xu; Chunshan Song; John M. Andresen; Bruce G. Miller; Alan W. Scaroni

2004-01-01T23:59:59.000Z

160

Summary Much attention is focused today on predicting how plants will respond to anticipated changes in atmospheric  

E-Print Network [OSTI]

, such as methane, became oxidized to form an early CO2-rich atmosphere. Over time, the concentration of carbon the atmosphere. Burial and lithification of carbonates and organic matter to limestone, coal or keragen the detailed history of CO2 is not well known for the whole of earth's history, some periods are reasonably

Ehleringer, Jim

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
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We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


161

Comparison of observed and predicted short-term tracer gas concentrations in the atmosphere  

SciTech Connect (OSTI)

The Savannah River Laboratory is in the process of conducting a series of atmospheric tracer studies. The inert gas sulfurhexafluoride is released from a height of 62 m for 15 min and concentrations in air are measured on sampling arcs up to 30 km downwind of the release point. Maximum 15 min. air concentrations from 14 of these tracer tests have been compared with the ground-level, centerline air concentration predicted with a Gaussian plume atmospheric transport model using eight different sets of atmospheric dispersion parameters. Preliminary analysis of the results from these comparisons indicates that the dispersion parameters developed at Juelich, West Germany, based on tracers released from a height of 50 m, give the best overall agreement between the predicted and observed values. The median value of the ratio of predicted to observed air concentrations for this set of parameters is 1.3, and the correlation coefficient between the log of the predictions and the log of the observations is 0.72. For the commonly used Pasquill-Gifford dispersion parameters, the values of these same statistics are 4.4 and 0.68, respectively. The Gaussian plume model is widely used to predict air concentrations resulting from short-term radionuclide release to the atmosphere. The results of comparisons such as these must be considered whenever the Gaussian model is used for such purposes. 22 references, 3 tables.

Cotter, S.J.; Miller, C.W.; Lin, W.C.T.

1985-01-01T23:59:59.000Z

162

CO2 Sequestration Potential of Texas Low-Rank Coals  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Co Co 2 SequeStration Potential of texaS low-rank CoalS Background Fossil fuel combustion is the primary source of emissions of carbon dioxide (CO 2 ), a major greenhouse gas. Sequestration of CO 2 by injecting it into geologic formations, such as coal seams, may offer a viable method for reducing atmospheric CO 2 emissions. Injection into coal seams has the potential added benefit of enhanced coalbed methane recovery. The potential for CO 2 sequestration in low-rank coals, while as yet undetermined, is believed to differ significantly from that for bituminous coals. To evaluate the feasibility and the environmental, technical, and economic impacts of CO 2 sequestration in Texas low-rank coal beds, the Texas Engineering Experimental Station is conducting a four-year study

163

Energy and Climate Impacts of Producing Synthetic Hydrocarbon Fuels from CO2  

Science Journals Connector (OSTI)

These platforms make the case for (more) research on the conversion of CO2 into synthetic fuels as means to utilize CO2 and thereby mitigate its accumulation in the atmosphere. ... Stechel, E. B.; Miller, J. E.Re-energizing CO2 to fuels with the sun: Issues of efficiency, scale, and economics J. CO2 Util. ... Published analyses suggest these air capture systems may cost a few hundred dollars per ton of CO2, making it cost competitive with mainstream CO2 mitigation options like renewable energy, nuclear power, and carbon dioxide capture and storage from large CO2 emitting point sources. ...

Coen van der Giesen; Ren Kleijn; Gert Jan Kramer

2014-05-15T23:59:59.000Z

164

Evaluating impacts of CO2 gas intrusion into a confined sandstone aquifer: Experimental results  

SciTech Connect (OSTI)

Deep subsurface storage and sequestration of CO2 has been identified as a potential mitigation technique for rising atmospheric CO2 concentrations. Sequestered CO2 represents a potential risk to overlying aquifers if the CO2 leaks from the deep storage reservoir. Experimental and modeling work is required to evaluate potential risks to groundwater quality and develop a systematic understanding of how CO2 leakage may cause important changes in aquifer chemistry and mineralogy by promoting dissolution/precipitation, adsorption/desorption, and redox reactions. Sediments from the High Plains aquifer in Kansas, United States, were used in this investigation, which is part of the National Risk Assessment Partnership Program sponsored by the US Department of Energy. This aquifer was selected to be representative of consolidated sand and gravel/sandstone aquifers overlying potential CO2 sequestration repositories within the continental US. In this paper, we present results from batch experiments conducted at room temperature and atmospheric pressure with four High Plains aquifer sediments. Batch experiments simulate sudden, fast, and short-lived releases of the CO2 gas as would occur in the case of well failure during injection. Time-dependent release of major, minor, and trace elements were determined by analyzing the contacting solutions. Characterization studies demonstrated that the High Plains aquifer sediments were abundant in quartz and feldspars, and contained about 15 to 20 wt% montmorillonite and up to 5 wt% micas. Some of the High Plains aquifer sediments contained no calcite, while others had up to about 7 wt% calcite. The strong acid extraction tests confirmed that in addition to the usual elements present in most soils, rocks, and sediments, the High Plains aquifer sediments had appreciable amounts of As, Cd, Pb, Cu, and occasionally Zn, which potentially may be mobilized from the solid to the aqueous phase during or after exposure to CO2. However, the results from the batch experiments showed that the High Plains sediments mobilized only low concentrations of trace elements (potential contaminants), which were detected occasionally in the aqueous phase during these experiments. Importantly, these occurrences were more frequent in the calcite-free sediment. Results from these investigations provide useful information to support site selection, risk assessment, and public education efforts associated with geological CO2 storage and sequestration.

Qafoku, Nikolla; Lawter, Amanda R.; Shao, Hongbo; Wang, Guohui; Brown, Christopher F.

2014-12-31T23:59:59.000Z

165

Atmospheric Environment 38 (2004) 14171423 Measurements of ion concentration in gasoline and diesel  

E-Print Network [OSTI]

Atmospheric Environment 38 (2004) 1417­1423 Measurements of ion concentration in gasoline of a gasoline engine (K-car) and a diesel engine (diesel generator). Under the experimental set-up reported all of the ions smaller than 3 nm in the gasoline engine exhaust, and is above 2.7 ? 108 cm?3

Yu, Fangqun

166

Carbon project-atmosphere "BL meteorology along route  

E-Print Network [OSTI]

2 CO2 CO2 CO2 CO2 Mixing heightEddie/coherent structure mixing Atmospheric CO2 gas CO2 gas layer and why is it important in a CO2 context · What are we doing onboard · What are we looking for and why · Interesting messurements from Coast of Namibia #12;What is a boundary layer ? CO2 CO2 CO2 CO2 CO

167

CO2 interaction with geomaterials.  

SciTech Connect (OSTI)

This work compares the sorption and swelling processes associated with CO2-coal and CO2-clay interactions. We investigated the mechanisms of interaction related to CO2 adsortion in micropores, intercalation into sub-micropores, dissolution in solid matrix, the role of water, and the associated changes in reservoir permeability, for applications in CO2 sequestration and enhanced coal bed methane recovery. The structural changes caused by CO2 have been investigated. A high-pressure micro-dilatometer was equipped to investigate the effect of CO2 pressure on the thermoplastic properties of coal. Using an identical dilatometer, Rashid Khan (1985) performed experiments with CO2 that revealed a dramatic reduction in the softening temperature of coal when exposed to high-pressure CO2. A set of experiments was designed for -20+45-mesh samples of Argonne Premium Pocahontas No.3 coal, which is similar in proximate and ultimate analysis to the Lower Kittanning seam coal that Khan used in his experiments. No dramatic decrease in coal softening temperature has been observed in high-pressure CO2 that would corroborate the prior work of Khan. Thus, conventional polymer (or 'geopolymer') theories may not be directly applicable to CO2 interaction with coals. Clays are similar to coals in that they represent abundant geomaterials with well-developed microporous structure. We evaluated the CO2 sequestration potential of clays relative to coals and investigated the factors that affect the sorption capacity, rates, and permanence of CO2 trapping. For the geomaterials comparison studies, we used source clay samples from The Clay Minerals Society. Preliminary results showed that expandable clays have CO2 sorption capacities comparable to those of coal. We analyzed sorption isotherms, XRD, DRIFTS (infrared reflectance spectra at non-ambient conditions), and TGA-MS (thermal gravimetric analysis) data to compare the effects of various factors on CO2 trapping. In montmorillonite, CO2 molecules may remain trapped for several months following several hours of exposure to high pressure (supercritical conditions), high temperature (above boiling point of water) or both. Such trapping is well preserved in either inert gas or the ambient environment and appears to eventually result in carbonate formation. We performed computer simulations of CO2 interaction with free cations (normal modes of CO2 and Na+CO2 were calculated using B3LYP / aug-cc-pVDZ and MP2 / aug-cc-pVDZ methods) and with clay structures containing interlayer cations (MD simulations with Clayff potentials for clay and a modified CO2 potential). Additionally, interaction of CO2 with hydrated Na-montmorillonite was studied using density functional theory with dispersion corrections. The sorption energies and the swelling behavior were investigated. Preliminary modeling results and experimental observations indicate that the presence of water molecules in the interlayer region is necessary for intercalation of CO2. Our preliminary conclusion is that CO2 molecules may intercalate into interlayer region of swelling clay and stay there via coordination to the interlayer cations.

Guthrie, George D. (U.S. Department of Energy, Pittsburgh, PA); Al-Saidi, Wissam A. (University of Pittsburgh, Pittsburgh, PA); Jordan, Kenneth D. (University of Pittsburgh, Pittsburgh, PA); Voora, Vamsee, K. (University of Pittsburgh, Pittsburgh, PA); Romanov, Vyacheslav N. (U.S. Department of Energy, Pittsburgh, PA); Lopano, Christina L (U.S. Department of Energy, Pittsburgh, PA); Myshakin, Eugene M. (URS Corporation, Pittsburgh, PA); Hur, Tae Bong (University of Pittsburgh, Pittsburgh, PA); Warzinski, Robert P. (U.S. Department of Energy, Pittsburgh, PA); Lynn, Ronald J. (URS Corporation, Pittsburgh, PA); Howard, Bret H. (U.S. Department of Energy, Pittsburgh, PA); Cygan, Randall Timothy

2010-09-01T23:59:59.000Z

168

NETL: IEP - Post-Combustion CO2 Emissions Control - Post-Combustion CO2  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Post-Combustion CO2 Capture for Existing PC Boilers by Self-concentrating Amine Absorbent Post-Combustion CO2 Capture for Existing PC Boilers by Self-concentrating Amine Absorbent Project No.: DE-FE0004274 3H Company will evaluate the feasibility of its "Self-Concentrating Absorbent CO2 Capture Process." The process is based on amines in a non-aqueous solvent which, upon reaction with CO2, separate into two distinct phases: a CO2-rich liquid phase and a dilute lean phase. The proposed process offers several potential advantages. Preliminary experimental data show that the process has the potential of reducing the total regeneration energy by as much as 70 percent. The solvent has high working capacity, thus required solvent volume would be lower than that required in a currently available amine system. This results in lower pumping requirements, lower auxiliary power demands, and reduced equipment size. In addition, since the solvent is non-aqueous, corrosion issues would be reduced. During the three-year project, an engineering design supported by laboratory data and economic justification will be developed to construct and operate a slipstream demonstration facility at an E-ON power plant in the United States as a next stage of commercialization development.

169

Developing a Comprehensive Risk Assessment Framework for Geological Storage CO2  

SciTech Connect (OSTI)

The operational risks for CCS projects include: risks of capturing, compressing, transporting and injecting CO?; risks of well blowouts; risk that CO? will leak into shallow aquifers and contaminate potable water; and risk that sequestered CO? will leak into the atmosphere. This report examines these risks by using information on the risks associated with analogue activities such as CO2 based enhanced oil recovery (CO2-EOR), natural gas storage and acid gas disposal. We have developed a new analysis of pipeline risk based on Bayesian statistical analysis. Bayesian theory probabilities may describe states of partial knowledge, even perhaps those related to non-repeatable events. The Bayesian approach enables both utilizing existing data and at the same time having the capability to adsorb new information thus to lower uncertainty in our understanding of complex systems. Incident rates for both natural gas and CO2 pipelines have been widely used in papers and reports on risk of CO2 pipelines as proxies for the individual risk created by such pipelines. Published risk studies of CO2 pipelines suggest that the individual risk associated with CO2 pipelines is between 10-3 and 10-4, which reflects risk levels approaching those of mountain climbing, which many would find unacceptably high. This report concludes, based on a careful analysis of natural gas pipeline failures, suggests that the individual risk of CO2 pipelines is likely in the range of 10-6 to 10-7, a risk range considered in the acceptable to negligible range in most countries. If, as is commonly thought, pipelines represent the highest risk component of CCS outside of the capture plant, then this conclusion suggests that most (if not all) previous quantitative- risk assessments of components of CCS may be orders of magnitude to high. The potential lethality of unexpected CO2 releases from pipelines or wells are arguably the highest risk aspects of CO2 enhanced oil recovery (CO2-EOR), carbon capture, and storage (CCS). Assertions in the CCS literature, that CO2 levels of 10% for ten minutes, or 20 to 30% for a few minutes are lethal to humans, are not supported by the available evidence. The results of published experiments with animals exposed to CO2, from mice to monkeys, at both normal and depleted oxygen levels, suggest that lethal levels of CO2 toxicity are in the range 50 to 60%. These experiments demonstrate that CO2 does not kill by asphyxia, but rather is toxic at high concentrations. It is concluded that quantitative risk assessments of CCS have overestimated the risk of fatalities by using values of lethality a factor two to six lower than the values estimated in this paper. In many dispersion models of CO2 releases from pipelines, no fatalities would be predicted if appropriate levels of lethality for CO2 had been used in the analysis.

Duncan, Ian

2014-08-31T23:59:59.000Z

170

Carbon Dioxide Emissions and Concentrations on the Rise as Kyoto Era Fades  

Science Journals Connector (OSTI)

According to on-site measurements by the Scripps Institute of Oceanography, global atmospheric carbon dioxide (CO2) concentrations reached 391.3 parts per million (ppm) in 2011, up from 388.56 ppm in 2010 and fro...

Xing Fu-Bertaux

2013-01-01T23:59:59.000Z

171

CANMET CO2 Consortium - O2/CO2 Recycle Combustion  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

CANMET CO CANMET CO 2 Consortium - O 2 /CO 2 Recycle Combustion Background The mission of the U.S. Department of Energy/National Energy Technology Laboratory (DOE/NETL) Existing Plants, Emissions & Capture (EPEC) Research & Development (R&D) Program is to develop innovative environmental control technologies to enable full use of the nation's vast coal reserves, while at the same time allowing the current fleet of coal-fired power plants to comply with existing and emerging environmental

172

Geological Sequestration of CO2: The GEO-SEQ Project  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

GeoloGical SequeStration of co GeoloGical SequeStration of co 2 : the Geo-Seq Project Background Growing concern over the potential adverse effects of carbon dioxide (CO 2 ) buildup in the atmosphere leading to global climate change may require reductions in carbon emissions from industrial, transportation, and other sources. One promising option is the capture of CO 2 from large point sources and subsequent sequestration in geologic formations. For this approach to achieve wide acceptance, t assurances that safe, permanent, and verifiable CO 2 geologic storage is attained during sequestration operations must be made. Project results are made available to potential CO 2 storage operators and other interested stakeholders. The primary performing organizations of the GEO-SEQ project team are Lawrence

173

Industrial CO2 Removal: CO2 Capture from Ambient Air and Geological Sequestration  

SciTech Connect (OSTI)

This abstract and its accompanying presentation will provide an overview of two distinct industrial processes for removing carbon dioxide (CO2) from the atmosphere as a means of addressing anthropogenic climate change. The first of these is carbon dioxide capture and storage (CCS) coupled with large scale biomass production (hereafter referred to as bioCCS). The second is CO2 capture from ambient air via industrial systems (hereafter referred to as direct air capture (DAC)). In both systems, the captured CO2 would be injected into deep geologic formations so as to isolate it from the atmosphere. The technical literature is clear that both of these technologies are technically feasible as of today (IPCC, 2005; Keith, 2009; Lackner, 2009; Luckow et al., 2010; Ranjan and Herzog, 2011). What is uncertain is the relative cost of these industrial ambient-air CO2 removal systems when compared to other emissions mitigation measures, the ultimate timing and scale of their deployment, and the resolution of potential site specific constraints that would impact their ultimate commercial deployment.

Dooley, James J.

2011-06-08T23:59:59.000Z

174

Production of CO2 in Soil Profiles of a California Annual Grassland  

E-Print Network [OSTI]

Production of CO2 in Soil Profiles of a California Annual Grassland Noah Fierer,1 * Oliver A play a key role in the global cycling of carbon (C), storing organic C, and releasing CO2 to the atmosphere. Although a large number of studies have focused on the CO2 flux at the soil­air inter- face

Fierer, Noah

175

Elevated CO2 affects shell dissolution rate but not calcification rate in a marine snail  

Science Journals Connector (OSTI)

...Research articles 1001 60 69 70 Elevated CO2 affects shell dissolution rate but not calcification...authors contributed equally to this work. As CO2 levels increase in the atmosphere, so too...Although direct effects of moderately elevated CO2 in sea water may be of little consequence...

2010-01-01T23:59:59.000Z

176

Potential for CO2 Sequestration and Enhanced Coalbed Methane Production, Blue Creek Field, NW Black Warrior Basin, Alabama  

E-Print Network [OSTI]

Carbon dioxide (CO2) is a primary source of greenhouse gases. Injection of CO2 from power plants near coalbed reservoirs is a win-win method to reducing emissions of CO2 to the atmosphere. Limited studies have investigated CO2 sequestration...

He, Ting

2011-02-22T23:59:59.000Z

177

10 MW Supercritical CO2 Turbine Test  

SciTech Connect (OSTI)

The Supercritical CO2 Turbine Test project was to demonstrate the inherent efficiencies of a supercritical carbon dioxide (s-CO2) power turbine and associated turbomachinery under conditions and at a scale relevant to commercial concentrating solar power (CSP) projects, thereby accelerating the commercial deployment of this new power generation technology. The project involved eight partnering organizations: NREL, Sandia National Laboratories, Echogen Power Systems, Abengoa Solar, University of Wisconsin at Madison, Electric Power Research Institute, Barber-Nichols, and the CSP Program of the U.S. Department of Energy. The multi-year project planned to design, fabricate, and validate an s-CO2 power turbine of nominally 10 MWe that is capable of operation at up to 700C and operates in a dry-cooled test loop. The project plan consisted of three phases: (1) system design and modeling, (2) fabrication, and (3) testing. The major accomplishments of Phase 1 included: Design of a multistage, axial-flow, s-CO2 power turbine; Design modifications to an existing turbocompressor to provide s-CO2 flow for the test system; Updated equipment and installation costs for the turbomachinery and associated support infrastructure; Development of simulation tools for the test loop itself and for more efficient cycle designs that are of greater commercial interest; Simulation of s-CO2 power cycle integration into molten-nitrate-salt CSP systems indicating a cost benefit of up to 8% in levelized cost of energy; Identification of recuperator cost as a key economic parameter; Corrosion data for multiple alloys at temperatures up to 650C in high-pressure CO2 and recommendations for materials-of-construction; and Revised test plan and preliminary operating conditions based on the ongoing tests of related equipment. Phase 1 established that the cost of the facility needed to test the power turbine at its full power and temperature would exceed the planned funding for Phases 2 and 3. Late in Phase 1 an opportunity arose to collaborate with another turbine-development team to construct a shared s-CO2 test facility. The synergy of the combined effort would result in greater facility capabilities than either separate project could produce and would allow for testing of both turbine designs within the combined budgets of the two projects. The project team requested a no-cost extension to Phase 1 to modify the subsequent work based on this collaborative approach. DOE authorized a brief extension, but ultimately opted not to pursue the collaborative facility and terminated the project.

Turchi, Craig

2014-01-29T23:59:59.000Z

178

AZ CO2 Storage Pilot  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

CO2 Storage Pilot Regional Carbon Sequestration Partnerships Initiative Review Meeting Pittsburgh, Pennsylvania October 7, 2008 John Henry Beyer, Ph.D. WESTCARB Program Manager, Geophysicist 510-486-7954, jhbeyer@lbl.gov Lawrence Berkeley National Laboratory Earth Sciences Division, MS 90-1116 Berkeley, CA 94720 2 WESTCARB region has major CO2 point sources 3 WESTCARB region has many deep saline formations - candidates for CO2 storage WESTCARB also created GIS layers for oil/gas fields and deep coal basins Source: DOE Carbon Sequestration Atlas of the United States and Canada 4 - Aspen Environmental - Bevilacqua-Knight, Inc. Arizona Utilities CO2 Storage Pilot Contracting and Funding Flow Department of Energy National Energy Technology Laboratory Lawrence Berkeley National

179

Northern California CO2 Reduction Project  

SciTech Connect (OSTI)

C6 Resources LLC, a wholly owned subsidiary of Shell Oil Company, worked with the US Department of Energy (DOE) under a Cooperative Agreement to develop the Northern California CO2 Reduction Project. The objective of the Project is to demonstrate the viability of using Carbon Capture and Sequestration (CCS) to reduce existing greenhouse gas emissions from industrial sources on a large-scale. The Project will capture more than 700,000 metric tonnes of CO2 per year, which is currently being vented to the atmosphere from the Shell Martinez Refinery in Contra Costa County. The CO2 will be compressed and dehydrated at the refinery and then transported via pipeline to a sequestration site in a rural area in neighboring Solano County. The CO2 will be sequestered into a deep saline formation (more than two miles underground) and will be monitored to assure secure, long-term containment. The pipeline will be designed to carry as much as 1,400,000 metric tonnes of CO2 per year, so additional capacity will be available to accommodate CO2 captured from other industrial sources. The Project is expected to begin operation in 2015. The Project has two distinct phases. The overall objective of Phase 1 was to develop a fully definitive design basis for the Project. The Cooperative Agreement with the DOE provided cost sharing for Phase 1 and the opportunity to apply for additional DOE cost sharing for Phase 2, comprising the design, construction and operation of the Project. Phase 1 has been completed. DOE co-funding is provided by the American Recovery and Reinvestment Act (ARRA) of 2009. As prescribed by ARRA, the Project will stimulate the local economy by creating manufacturing, transportation, construction, operations, and management jobs while addressing the need to reduce greenhouse gas emissions at an accelerated pace. The Project, which will also assist in meeting the CO2 reduction requirements set forth in California?s Climate Change law, presents a major opportunity for both the environment as well as the region. C6 Resources is conducting the Project in collaboration with federally-funded research centers, such as Lawrence Berkeley National Lab and Lawrence Livermore National Lab. C6 Resources and Shell have identified CCS as one of the critical pathways toward a worldwide goal of providing cleaner energy. C6 Resources, in conjunction with the West Coast Regional Carbon Sequestration Partnership (WESTCARB), has conducted an extensive and ongoing public outreach and CCS education program for local, regional and state-wide stakeholders. As part of a long term relationship, C6 Resources will continue to engage directly with community leaders and residents to ensure public input and transparency. This topical report summarizes the technical work from Phase 1 of the Project in the following areas: ? Surface Facility Preliminary Engineering: summarizes the preliminary engineering work performed for CO2 capture, CO2 compression and dehydration at the refinery, and surface facilities at the sequestration site ? Pipeline Preliminary Engineering: summarizes the pipeline routing study and preliminary engineering design ? Geologic Sequestration: summarizes the work to characterize, model and evaluate the sequestration site ? Monitoring, Verification and Accounting (MVA): summarizes the MVA plan to assure long-term containment of the sequestered CO2

Hymes, Edward

2010-06-16T23:59:59.000Z

180

CO2 Utilization | Department of Energy  

Broader source: Energy.gov (indexed) [DOE]

CO2 CO2 Utilization CO2 Utilization Carbon dioxide (CO2) use and reuse efforts focus on the conversion of CO2 to useable products and fuels that will reduce CO2 emissions in areas where geologic storage may not be an optimal solution. These include: Enhanced Oil/Gas Recovery - Injecting CO2 into depleting oil or gas bearing fields to maximize the amount of CO2 that could be stored as well as maximize hydrocarbon production. CO2 as Feedstock - Use CO2 as a feedstock to produce chemicals (including fuels and polymers) and find applications for the end products. Non-Geologic Storage of CO2 - Use CO2 from an effluent stream to immobilize the CO2 permanently by producing stable solid material that are either useful products with economic value or a low cost produced material.

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


181

Economic and energetic analysis of capturing CO2 from ambient air  

Science Journals Connector (OSTI)

...capture from atmospheric airThermodynamic...thermal energy recovery from the...Not reported. Recovery cycle only...ion-exchange resin. Condensation of water and heat from...compression of CO2 to atmospheric pressure included...

Kurt Zenz House; Antonio C. Baclig; Manya Ranjan; Ernst A. van Nierop; Jennifer Wilcox; Howard J. Herzog

2011-01-01T23:59:59.000Z

182

Multi-Channel Auto-Dilution System for Remote Continuous Monitoring of High Soil-CO2 Fluxes  

SciTech Connect (OSTI)

Geological sequestration has the potential capacity and longevity to significantly decrease the amount of anthropogenic CO2 introduced into the atmosphere by combustion of fossil fuels such as coal. Effective sequestration, however, requires the ability to verify the integrity of the reservoir and ensure that potential leakage rates are kept to a minimum. Moreover, understanding the pathways by which CO2 migrates to the surface is critical to assessing the risks and developing remediation approaches. Field experiments, such as those conducted at the Zero Emissions Research and Technology (ZERT) project test site in Bozeman, Montana, require a flexible CO2 monitoring system that can accurately and continuously measure soil-surface CO2 fluxes for multiple sampling points at concentrations ranging from background levels to several tens of percent. To meet this need, PNNL is developing a multi-port battery-operated system capable of both spatial and temporal monitoring of CO2 at concentrations from ambient to at least 150,000 ppmv. This report describes the system components (sampling chambers, measurement and control system, and power supply) and the results of a field test at the ZERT site during the late summer and fall of 2008. While the system performed well overall during the field test, several improvements to the system are suggested for implementation in FY2009.

Amonette, James E.; Barr, Jonathan L.

2009-04-23T23:59:59.000Z

183

CO2 | OpenEI  

Open Energy Info (EERE)

CO2 CO2 Dataset Summary Description Emissions from energy use in buildings are usually estimated on an annual basis using annual average multipliers. Using annual numbers provides a reasonable estimation of emissions, but it provides no indication of the temporal nature of the emissions. Therefore, there is no way of understanding the impact on emissions from load shifting and peak shaving technologies such as thermal energy storage, on-site renewable energy, and demand control. Source NREL Date Released April 11th, 2011 (3 years ago) Date Updated April 11th, 2011 (3 years ago) Keywords buildings carbon dioxide emissions carbon footprinting CO2 commercial buildings electricity emission factors ERCOT hourly emission factors interconnect nitrogen oxides NOx SO2 sulfur dioxide emissions

184

Update on CO2 emissions  

SciTech Connect (OSTI)

Emissions of CO2 are the main contributor to anthropogenic climate change. Here we present updated information on their present and near-future estimates. We calculate that global CO2 emissions from fossil fuel burning decreased by 1.3% in 2009 owing to the global financial and economic crisis that started in 2008; this is half the decrease anticipated a year ago1. If economic growth proceeds as expected2, emissions are projected to increase by more than 3% in 2010, approaching the high emissions growth rates that were observed from 2000 to 20081, 3, 4. We estimate that recent CO2 emissions from deforestation and other land-use changes (LUCs) have declined compared with the 1990s, primarily because of reduced rates of deforestation in the tropics5 and a smaller contribution owing to forest regrowth elsewhere.

Friedingstein, P. [University of Exeter, Devon, England; Houghton, R.A. [Woods Hole Research Center, Woods Hole, MA; Marland, Gregg [ORNL; Hackler, J. [Woods Hole Research Center, Woods Hole, MA; Boden, Thomas A [ORNL; Conway, T.J. [NOAA, Boulder, CO; Canadell, J.G. [CSIRO Marine and Atmospheric Research; Raupach, Mike [GCP, Canberra, Australia; Ciais, Philippe [Laboratoire des Sciences du Climat et de l'Environement, France; Le Quere, Corrine [University of East Anglia, Norwich, United Kingdom

2010-12-01T23:59:59.000Z

185

Materials, methods and devices to detect and quantify water vapor concentrations in an atmosphere  

DOE Patents [OSTI]

We have demonstrated that a surface acoustic wave (SAW) sensor coated with a nanoporous framework material (NFM) film can perform ultrasensitive water vapor detection at concentrations in air from 0.05 to 12,000 ppmv at 1 atmosphere pressure. The method is extendable to other MEMS-based sensors, such as microcantilevers, or to quartz crystal microbalance sensors. We identify a specific NFM that provides high sensitivity and selectivity to water vapor. However, our approach is generalizable to detection of other species using NFM to provide sensitivity and selectivity.

Allendorf, Mark D; Robinson, Alex L

2014-12-09T23:59:59.000Z

186

Capture and Sequestration of CO2 From Stationary Combustion Systems by Photosynthesis of Microalgae  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Capture and Sequestration of CO Capture and Sequestration of CO 2 From Stationary Combustion Systems by Photosynthesis of Microalgae Takashi Nakamura (nakamura@psicorp.com; 925-743-1110) Constance Senior (senior@psicorp.com; 978-689-0003) Physical Sciences Inc Andover, MA 01810 Miguel Olaizola (molaizola@aquasearch.com; 808-326-9301 Michael Cushman (mcushman@aquasearch.com; 808-326-9301) Aquasearch Inc. Kailua-Kona, HI 96740 Stephen Masutani (masutan@wiliki.eng.hawaii.edu; 808-956-7388) University of Hawaii Honolulu, HI 96822 Introduction Emissions of carbon dioxide are predicted to increase this century 1 leading to increases in the concentrations of carbon dioxide in the atmosphere. While there is still much debate on the effects of increased CO 2 levels on global climate, many scientists agree that the projected increases could have a

187

CO2 Mineral Sequestration Studies  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Sequestration Studies Sequestration Studies Introduction, Issues and Plans Philip Goldberg National Energy Technology Laboratory Workshop on CO 2 Sequestration with Minerals August 8, 2001 Mineral Sequestration Program Research effort seeks to refine and validate a promising CO 2 sequestration technology option, mineral sequestration also known as mineral carbonation Goals: * Understand the fundamental mechanisms involved in mineral carbonation * Generate data to support process development * Operate continuous, integrated small-scale process unit to support design Current Partnerships In order to effectively develop Mineral Sequestration, a multi-laboratory Working Group was formed in the Summer of 1998, participants include: * Albany Research Center * Arizona State University * Los Alamos National Laboratory

188

Estimation of CO2 effluxes from suburban forest floor and grass using a process-based model  

Science Journals Connector (OSTI)

Abstract Carbon dioxide is an important greenhouse gas, and its atmospheric concentration has been predicted to increase in the future. The objective of this study was to quantify the soil CO2 efflux in a suburban area including mixed deciduous forest and grass by numerically modeling the CO2 transport through the soil profile. Three stations per land-cover (forest and grass) were selected at the Cub Hill site (MD, USA), where the US Forest Service operates an urban flux tower. Six VAISALA CO2 sensors (Vaisala Inc., Finland) per monitoring station were horizontally installed at 6 different depths (soil surface, 0.02, 0.05, 0.10, 0.20, and 0.30m from the soil surface) in the mid of May, 2011. Temperature and volumetric soil moisture measurements were taken using thermistors and EC-5 sensors (Decagon devices, Pullman, WA, USA) that were installed at the same depths as the CO2 sensors except for the soil surface. These data were recorded every 10min. To evaluate the numerical model (SOILCO2), CO2 efflux using the standard chamber method was measured once a week. The CO2 effluxes from the standard chamber method ranged from 3.32נ10?9 to 7.28נ10?8m3m?2s?1 and 6.79נ10?9 to 1.45נ10?7m3m?2s?1 for forest and grass, respectively. The CO2 effluxes from bare soil at the grass site varied with the range of 3.63נ10?8 to 9.37נ10?8m3m?2s?1. The pulse effect (a rapid increase of CO2 concentrations right after rainfall events) in grass, where changes in soil moisture were larger than in the forest, was more apparent than in the forest. Diurnal patterns similar to those of temperature were observed from CO2 profiles in soils. The SOILCO2 model estimated the soil CO2 effluxes with coefficients of correlation of 0.64 and 0.76 at forest and grass, respectively, and root mean square error (RMSE) of 1.58נ10?8 and 2.06נ10?8m3m?2s?1 for forest and grass, respectively. This study suggests that the SOILCO2 model can provide a better understanding of the contribution of the soil ecosystem to the carbon cycle in suburban environments including mixed deciduous forest and grass.

J.A. Chun; K. Szlavecz; M. Bernard; D. Ferrer; J. Hom; N. Saliendra

2014-01-01T23:59:59.000Z

189

8, 73737389, 2008 Scientists' CO2  

E-Print Network [OSTI]

ACPD 8, 7373­7389, 2008 Scientists' CO2 emissions A. Stohl Title Page Abstract Introduction substantial emissions of carbon dioxide (CO2). In this pa- per, the CO2 emissions of the employees working, the total annual per capita CO2 emissions are 4.5 t worldwide, 1.2 t for India, 3.8 t for China, 5

Paris-Sud XI, Université de

190

E-Print Network 3.0 - atmospheric pollutant concentrations Sample...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

sunlight, and natural atmospheric gases. Primary and secondary pollutants 12;Air Pollutants 12... , an atmospheric inversion occurs that can restrict circulation in...

191

Modeling the CO2 Footprint of the U.S. Coal Mining Industry and the Potential Economic Costs of CO2 Legislation.  

E-Print Network [OSTI]

??The U.S. government is expected to develop a federal mandate which will aim tocurb CO2 emissions into the atmosphere. This legislation will most likely be (more)

Aziz, AbdulMajeed

2010-01-01T23:59:59.000Z

192

Short communication Satellite-derived surface water pCO2 and airsea CO2 fluxes  

E-Print Network [OSTI]

Short communication Satellite-derived surface water pCO2 and air­sea CO2 fluxes in the northern for the estimation of the partial pressure of carbon dioxide (pCO2) and air­sea CO2 fluxes in the northern South), respectively, the monthly pCO2 fields were computed. The derived pCO2 was compared with the shipboard pCO2

193

Development of experimental methods for intermediate scale testing of deep geologic CO2 sequestration trapping processes at ambient laboratory conditions.  

E-Print Network [OSTI]

??Carbon Capture and Storage (CCS) is a potential strategy to reduce CO2 emissions into the atmosphere. Deep geological formations provide a viable storage site for (more)

Vargas-Johnson, Javier

2014-01-01T23:59:59.000Z

194

Low Cost Open-Path Instrument for Monitoring Atmospheric Carbon Dioxide at Sequestration Sites  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Low Cost open-path Instrument for Low Cost open-path Instrument for monItorIng atmospherIC Carbon DIoxIDe at sequestratIon sItes Background Growing concern over the effect on global climate of the buildup of greenhouse gases (GHG), particularly carbon dioxide (CO 2 ), in the atmosphere may lead to the curtailment of CO 2 emissions. One potential course of action by industry to reduce GHG emissions is the subsurface disposal of CO 2 . An important requirement of such disposal is verification that the injected gases remain in place and do not leak to the surface. Perhaps the most direct evidence of a successful sequestration project is the lack of a detectable CO 2 concentration above the background level in the air near the ground. Although measurement of CO 2 concentration can be performed, it is

195

NETL: Alstom's Chemical Looping Combustion Technology with CO2 Capture  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Oxy-Combustion CO2 Emissions Control Oxy-Combustion CO2 Emissions Control Commercialization of the Iron Based Coal Direct Chemical Looping Process for Power Production with in situ CO2 Capture Project No.: DE-FE0009761 CDLC Process Concept CDLC Process Concept (click to enlarge) Babcock & Wilcox Power Generation Group (B&W) is developing the coal direct chemical looping (CDCL) process. The CDCL process consists of a unique moving bed reactor - the reducer - where pulverized coal is fully converted using iron-based oxygen carriers. The oxygen carrier is reduced from Fe2O3 to FeO/Fe and the flue gas is a concentrated stream of CO2 that is available for storage or beneficial use. The reduced FeO/Fe is oxidized to Fe2O3 using air in the combustor, liberating heat to produce steam for a

196

Direct Solar Energy Conversion by the Reduction of CO2  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Direct Solar Energy Conversion by the Reduction of CO2 Direct Solar Energy Conversion by the Reduction of CO2 Speaker(s): Reed Jensen Date: August 25, 2005 - 12:00pm Location: Bldg. 90 Reed Jensen has successfully demonstrated the direct solar reduction of CO2 to CO and O2 using a solar concentrator dish and ceramic converter that grew out of his work at Los Alamos National Laboratory. He will discuss the thermochemical, kinetic and spectral properties of the CO2 /CO/ O2 system that enable this process and how the CO is subsequently converted to useful fuels by a range of catalytic processes. He will also discuss the technical difficulties associated with the design, construction and operation of a multi-component optical system that must operate at high temperatures. Results from a prototype system will be discussed defining the efficiencies

197

Adsorption and Reaction of CO2 and SO2 at a Water Surface Teresa L. Tarbuck and Geraldine L. Richmond*  

E-Print Network [OSTI]

of SO2 and CO2 gas are examined using vibrational sum-frequency spectroscopy (VSFS) to gain insight of SO2 and CO2 in atmospheric aerosols depends on factors including gas-phase diffusion, solubility reactions: Dissolved in water, SO2 and CO2 are in clathrate (gas hydrate) and loosely hydrated structures

Richmond, Geraldine L.

198

Characterization and performance of Cu/ZnO/Al2O3 catalysts prepared via decomposition of M(Cu, Zn)-ammonia complexes under sub-atmospheric pressure for methanol synthesis from H2 and CO2  

Science Journals Connector (OSTI)

Methanol synthesis from hydrognation of CO2 is investigated over Cu/ZnO/Al2O3 catalysts prepared by decomposition of M(Cu, Zn)-ammonia complexes (DMAC) at various temperatures. The catalysts were characterized in detail, including X-ray diffraction, N2 adsorption-desorption, N2O chemisorption, temperature-programmed reduction and evolved gas analyses. The influences of DMAC temperature, reaction temperature and specific Cu surface area on catalytic performance are investigated. It is considered that the aurichalcite phase in the precursor plays a key role in improving the physiochemical properties and activities of the final catalysts. The catalyst from rich-aurichalcite precursor exhibits large specific Cu surface area and high space time yield of methanol (212 g/(Lcat h); T = 513 K, p = 3 MPa, SV = 12000 h?1).

Danjun Wang; Jun Zhao; Huanling Song; Lingjun Chou

2011-01-01T23:59:59.000Z

199

CO2 http://andrew.ucsd.edu/co2qc/ University of California, San Diego  

E-Print Network [OSTI]

cooled by liquid nitrogen. The water and CO2 are separated from one another by sublimation and the CO2 for oceanic CO2 analysis: A method for the certification of total alkalinity. Marine Chemistry 80, 185

200

NETL: CO2 Emissions Control  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Systems Analysis Systems Analysis DOE/NETL possesses strong systems analysis and policy-support capabilities. Systems analysis in support of the Innovations for Existing Plants Program consists of conducting various energy analyses that provide input to decisions on issues such as national plans and programs, resource use, environmental and energy security policies, technology options for research and development programs, and paths to deployment of energy technology. This work includes technology, benefits, and current situation and trends analyses related to CO2 emissions control. Systems analyses and economic modeling of potential new processes are crucial to providing sound guidance to R&D efforts. Since the majority of new CO2 capture technologies are still at a bench scale level of development, a conceptual design is first generated with emphasis on mass and energy balances. Based on available data and/or engineering estimates, these systems are optimized, and "what-if" scenarios are evaluated to identify barriers to deployment and help the process developers establish system performance targets. Reports that have been generated describing systems analyses in support of carbon capture efforts are shown in the table below.

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
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We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


201

CO2-Emissionszertifikate - Preismodellierung und Derivatebewertung.  

E-Print Network [OSTI]

??EU-Unternehmen mssen seit 2005 entsprechend ihrem CO2-Aussto gengend Emissionszertifikate einreichen. Da die Zertifikate frei handelbar sind, stellt sich ihnen CO2 als ein zustzlicher Produktionsfaktor mit (more)

Wagner, Michael W.

2007-01-01T23:59:59.000Z

202

Engineered yeast for enhanced CO2 mineralization  

E-Print Network [OSTI]

In this work, a biologically catalysed CO2 mineralization process for the capture of CO2 from point sources was designed, constructed at a laboratory scale, and, using standard chemical process scale-up protocols, was ...

Barbero, Roberto Juan

2013-01-01T23:59:59.000Z

203

QGESS: CO2 Impurity Design Parameters  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

10. Shah, Minish. Capturing CO2 from Oxy-Fuel Combustion Flue Gas. Cottbus, Germany : Praxair Inc., 2005. 11. Spitznogle, Gary O. CO2 Impurity Specification at AEP Mountaineer....

204

Legal Implications of CO2 Ocean Storage  

E-Print Network [OSTI]

, ocean currents may prevent stagnation or accumulatioLegal Implications of CO2 Ocean Storage Jason Heinrich Working Paper Laboratory for Energy #12;Introduction Ocean sequestration of CO2, a potentially significant technique to be used

205

CO2 please | ornl.gov  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

CO2 please CO2 please ORNL researchers look to carbon dioxide as a more environmentally friendly refrigerant gas In an indoor research area, Brian Fricke preps display cases for...

206

Advanced Research Power Program--CO2 Mineral Sequestration  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Sequestration Sequestration Robert Romanosky National Energy Technology Laboratory Mineral Carbonation Workshop August 8, 2001 Advanced Research Power Program Descriptor - include initials, /org#/date Mineral Sequestration Research Research effort seeks to refine and validate a promising CO 2 sequestration technology option, mineral sequestration also known as mineral carbonation Descriptor - include initials, /org#/date What is Mineral Carbonation * Reaction of CO 2 with Mg or Ca containing minerals to form carbonates * Lowest energy state of carbon is a carbonate and not CO 2 * Occurs naturally in nature as weathering of rock * Already proven on large scale - Carbonate formation linked to formation of the early atmosphere Descriptor - include initials, /org#/date Advantages of Mineral Carbonation

207

Distributed Optical Sensor for CO2 Leak Detection  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Optical Sensor for CO Optical Sensor for CO 2 Leak Detection Opportunity Research is active on the technology "Distributed Optical Sensor for CO 2 Leak Detection," for which a Patent Application has been filed. This technology is available for licensing and/or further collaborative research from the U.S. Department of Energy's National Energy Technology Laboratory (NETL). Overview The availability of fossil fuels to provide clean, affordable energy is essential for domestic and global prosperity and security well into the 21st century. However, there are concerns over the impacts of greenhouse gases (GHGs) in the atmosphere-particularly carbon dioxide (CO 2 ). Carbon capture and storage in geologic formations is a promising technology to reduce the impact of CO

208

An inversion technique for the retrieval of single-point emissions from atmospheric concentration measurements  

Science Journals Connector (OSTI)

...retrieval of single-point emissions from atmospheric...Atmospheric Sciences, Indian Institute of Technology...for the retrieval of point sources of atmospheric...the seven runs of the Indian Institute of Technology...of identification of point sources has raised much...

2009-01-01T23:59:59.000Z

209

Effects of diurnally oscillating pCO2 on the calcification and survival of coral recruits  

Science Journals Connector (OSTI)

...pCO2-mediated, night-time storage of dissolved inorganic...atmospheric CO2 in seawater is thought to be...with surrounding seawater after approximately...indicating active DIC storage is possible. Short-term...store DIC is through storage in the cytosol...transports DIC from seawater into coral tissues...

2012-01-01T23:59:59.000Z

210

Effects of long-term elevated atmospheric CO{sub 2} concentrations on Pinus ponderosa  

SciTech Connect (OSTI)

This report details the results from an experiment of the effects of long-term elevated atmospheric CO{sub 2} concentrations on ponderosa pine (Pinus ponderosa Laws.) saplings and seedlings. The study began in 1983 as a pilot study designed to explore the feasibility of using open-top chambers for continuous multi-year exposures on sapling-sized trees and to examine possible CO{sub 2} responses so that future research could be adequately designed. however, following the first year of exposure, preliminary results from the study indicated that measurements of CO{sub 2} responses should be intensified. Open-top chambers proved suitable for use in multiyear exposures of mature trees. With respect to the preliminary examination of CO{sub 2} responses, many interesting observations were made. The nature of the preliminary results suggests that future long-term field CO{sub 2} exposures on perennial species may be critical to the understanding and preparation for future environments. Other research reported here attempted to adapt an existing western coniferous forest growth and succession model for use in elevated CO{sub 2} scenarios using differential species responses, and assessed the usefulness of the model in that regard. Seven papers have been processed separately for inclusion in the appropriate data bases.

Surano, K.A.; Kercher, J.R. [eds.

1993-10-01T23:59:59.000Z

211

Physisorption of CO2 on non-ice materials relevant to icy satellites  

SciTech Connect (OSTI)

CO2 is known to adsorb onto clay and other minerals when a significant atmospheric pressure is present. We have found that CO2 can also adsorb onto some clays when the CO2 partial pressure is effectively zero under ultra-high vacuum (UHV) if cooled to the surface temperatures of the icy satellites of Jupiter and Saturn. The strength of adsorption and the spectral characteristics of the adsorbed CO2 infrared (IR) ?3 absorption band near 4.25 ?m depend on the composition and temperature of the adsorbent. CO2 remains adsorbed onto the clay mineral montmorillonite for >10 s of min when exposed to a vacuum of ?110?8 Torr at ?125 K. CO2 does not adsorb onto serpentine, goethite, or palagonite under these conditions. A small amount may adsorb onto kaolinite. When heated above 150 K under vacuum, the CO2 desorbs from the montmorillonite within a few minutes. The ?3 absorption band of CO2 adsorbed onto montmorillonite at 125 K is similar to that of the CO2 detected on the saturnian and Galilean satellites and is markedly different from CO2 adsorbed onto montmorillonite at room temperature. We infer the adsorption process is physisorption and postulate that this mechanism may explain the presence and spectral characteristics of the CO2 detected in the surfaces of these outer satellites.

Hibbitts, Charles A.; Szanyi, Janos

2007-11-01T23:59:59.000Z

212

CO2 laser frequency multiplication  

SciTech Connect (OSTI)

The duration of the mode-locked CO(2) laser pulses was measured to be 0.9 + or - nsec by the technique of (second harmonic) autocorrelation. Knowing the pulse duration, the spot size, and the harmonic conversion efficiency, a detailed fit of experiment to theory gave an estimate of the nonlinear coefficient of AgGaSe(2). d36 = 31 + or - V(1), in agreement with the most accurate literature values. A number of experiments were made with longer pulse trains in which the highest harmonic energy conversion reached 78%. The damage threshold was measured and it turned out to be related much more strongly to fluence than intensity. The shorter pulse trains had peak intensities of close to 300 MW 1/cm squared whereas the longer trains (3 usec) had intensities up to 40 MW 1/cm squared.

Not Available

1992-03-01T23:59:59.000Z

213

Semi-analytical Solution for Multiphase Fluid Flow Applied to CO 2 Sequestration in Geologic Porous Media  

E-Print Network [OSTI]

The increasing concentration of CO_(2) has been linked to global warming and changes in climate. Geologic sequestration of CO_(2) in deep saline aquifers is a proposed greenhouse gas mitigation technology with potential to significantly reduce...

Mohamed, Ahmed Mohamed Anwar Sayed

2013-08-01T23:59:59.000Z

214

Optimal electrochemical performances of CO2 activated carbon aerogels for supercapacitors  

Science Journals Connector (OSTI)

Activated carbon aerogels(ACAs) derived from sol-gel polycondensation of resorcinol (R) and formaldehyde (F) were pyrolyzed under Ar flow and activated in CO2 atmosphere. The morphology of ACAs was characterized ...

Lijuan Chang ???; Zhibing Fu; Miao Liu

2014-04-01T23:59:59.000Z

215

Long-term effects of anthropogenic CO2 emissions simulated with a complex earth system model  

E-Print Network [OSTI]

Long-term effects of anthropogenic CO2 emissions simulated with a complex earth system model Uwe earth system model con- sisting of an atmospheric general circulation model, an ocean general

Winguth, Arne

216

Simulation assessment of CO2 sequestration potential and enhanced methane recovery in low-rank coalbeds of the Wilcox Group, east-central Texas  

E-Print Network [OSTI]

Carbon dioxide (CO2) from energy consumption is a primary source of greenhouse gases. Injection of CO2 from power plants in coalbed reservoirs is a plausible method for reducing atmospheric emissions, and it can have the additional benefit...

Hernandez Arciniegas, Gonzalo

2006-10-30T23:59:59.000Z

217

Assessment of CO2 capture options from various points in steam methane reforming for hydrogen production  

Science Journals Connector (OSTI)

Abstract Steam methane reforming (SMR) is currently the main hydrogen production process in industry, but it has high emissions of CO2, at almost 7kg CO2/kg H2 on average, and is responsible for about 3% of global industrial sector CO2 emissions. Here, the results are reported of an investigation of the effect of steam-to-carbon ratio (S/C) on CO2 capture criteria from various locations in the process, i.e. synthesis gas stream (location 1), pressure swing adsorber (PSA) tail gas (location 2), and furnace flue gases (location 3). The CO2 capture criteria considered in this study are CO2 partial pressure, CO2 concentration, and CO2 mass ratio compared to the final exhaust stream, which is furnace flue gases. The CO2 capture number (Ncc) is proposed as measure of capture favourability, defined as the product of the three above capture criteria. A weighting of unity is used for each criterion. The best S/C ratio, in terms of providing better capture option, is determined. CO2 removal from synthesis gas after the shift unit is found to be the best location for CO2 capture due to its high partial pressure of CO2. However, furnace flue gases, containing almost 50% of the CO2 in produced in the process, are of great significance environmentally. Consequently, the effects of oxygen enrichment of the furnace feed are investigated, and it is found that this measure improves the CO2 capture conditions for lower S/C ratios. Consequently, for an S/C ratio of 2.5, CO2 capture from a flue gas stream is competitive with two other locations provided higher weighting factors are considered for the full presence of CO2 in the flue gases stream. Considering carbon removal from flue gases, the ratio of hydrogen production rate and Ncc increases with rising reformer temperature.

R. Soltani; M.A. Rosen; I. Dincer

2014-01-01T23:59:59.000Z

218

E-Print Network 3.0 - atmospheric elemental concentration Sample...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

- Department of Geography, University of North Texas Collection: Geosciences 4 Project EARTH-11-TM1: Volcanoes and the global atmospheric phosphorus cycle Summary: volcanic...

219

MAC-Kaust Project P1 CO2 Sequestration Modeling of CO2 sequestration including parameter  

E-Print Network [OSTI]

MAC-Kaust Project P1 ­ CO2 Sequestration Modeling of CO2 sequestration including parameter identification and numerical simulation M. Brokate, O. A. PykhteevHysteresis aspects of CO2 sequestration modeling K-H. Hoffmann, N. D. Botkin Objectives and methods of CO2 sequestration There is a popular belief

Turova, Varvara

220

Experimental Determination of Ca-Silicate Dissolution Rates: A Source of Calcium for Geologic CO2 Sequestration  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Experimental Determination of Ca-Silicate Dissolution Rates: Experimental Determination of Ca-Silicate Dissolution Rates: A Source of Calcium for Geologic CO 2 Sequestration Susan A. Carroll (carroll6@llnl.gov; 925-423-5694) Energy and Environment Directorate Lawrence Livermore National Laboratory L-219 Livermore, CA 94550 Kevin G. Knauss (knauss@llnl.gov; 925-422-1372) Energy and Environment Directorate Lawrence Livermore National Laboratory L-219 Livermore, CA 94550 2 Introduction The international scientific community recognizes that greenhouse gases have the potential to influence climate, and that potential changes in sea level and weather patterns would be largely deleterious. Because CO 2 is emitted in such large quantities and its atmospheric concentration has been consistently rising throughout the recent past, it is only prudent to focus attention on reducing

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


221

Opportunities for Using Anthropogenic CO2 for Enhanced Oil Recovery and CO2 Storage  

Science Journals Connector (OSTI)

Colorado and Wyoming ... At the end of a CO2 flood, essentially all of the CO2 that is originally purchased is stored in the reservoir when the operator closes the field at pressure. ... Under special conditions, such as gravity-stable CO2 flooding, the CO2-EOR process can store considerably more CO2 than the carbon content of the oil (Figure 7). ...

Michael L. Godec; Vello A. Kuuskraa; Phil Dipietro

2013-02-07T23:59:59.000Z

222

Reversible zwitterionic liquids, the reaction of alkanol guanidines, alkanol amidines, and diamines with CO2  

SciTech Connect (OSTI)

Carbon dioxide chemistry is increasingly relevant to real-world issues, thanks to global warming. Key chemistry issues currently being studied are the capture, storage, and utilization of CO2. While the relevance of capture and storage are obvious, the relevance of CO2 utilization is less clear. Although CO2 utilization is unlikely to consume significant quantities of CO2, it can be an significant strategy for the development of sustainable processes. As part of our research efforts towards CO2 utilization, some of us invented switchable solvents, meaning solvents that can switch reversibly from one version to another.1Our original version was a mixture of an amidine and an alcohol (equation 1, where B is a liquid amidine), but since then we and others have developed others such as guanidine/alcohol mixtures (equation 1, where B is a liquid guanidine),2 amidine/primary amine mixtures,3 and secondary amines (equation 2).4Switchable solvents of these types all convert from a low-polarity to a high-polarity ionic liquid form upon exposure to an atmosphere of CO2 and revert back to the low polarity form when the CO2 is removed by heat or flushing with inert gas. We also demonstrated that these switchable solvents can be used as reversible CO2-binding organic liquids (CO2BOLs) for CO2 capture, and are more energy-efficient in that role than aqueous solutions of ethanolamine.

Heldebrant, David J.; Koech, Phillip K.; Ang, Trisha; Liang, Chen; Rainbolt, James E.; Yonker, Clement R.; Jessop, Philip G.

2010-04-01T23:59:59.000Z

223

Surface Condensation of CO2 onto Kaolinite. | EMSL  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Condensation of CO2 onto Kaolinite. Surface Condensation of CO2 onto Kaolinite. Abstract: The fundamental adsorption behavior of gaseous and supercritical carbon dioxide (CO2) onto...

224

Biomimetric Membrane for CO2 Capture from Flue Gas  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Biomimetic memBrane for co Biomimetic memBrane for co 2 capture from flue Gas Background Carbon Capture and Sequestration (CCS) is a three-step process including capture, pipeline transport and geologic storage of which the capture of carbon dioxide (CO 2 ) is the most costly and technically challenging. Current available methods impose significant energy burdens that severely impact their overall effectiveness as a significant deployment option. Of the available capture technologies for post combustion applications - absorption, adsorption, reaction and membranes chemically facilitated absorption promises to be the most cost-effective membrane solution for post combustion application. The Carbozyme technology extracts CO 2 from low concentration, low pressure sources by means of chemical facilitation of a polymer membrane. The chemical

225

Spatially Distributed CO2, Sensible, and Latent Heat Fluxes Over the  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Spatially Distributed CO2, Sensible, and Latent Heat Fluxes Over the Spatially Distributed CO2, Sensible, and Latent Heat Fluxes Over the Southern Great Plains Berry, Joseph Carnegie Inst.of Washington Riley, William Lawrence Berkeley National Laboratory Biraud, Sebastien Lawrence Berkeley National Laboratory Torn, Margaret Lawrence Berkeley National Laboratory Fischer, Marc Lawrence Berkeley National Laboratory Category: Atmospheric State and Surface Vegetation strongly influences the spatial distribution of surface sensible and latent heat fluxes, and also impacts the ecosystem to atmosphere CO2 exchanges. We describe here a methodology to estimate surface energy fluxes and Net Ecosystem Exchange (NEE) of CO2 continuously over the Southern Great Plains, using (1) data from the Atmospheric Radiation Measurement (ARM) program in Oklahoma and Kansas; (2) meteorological forcing data from

226

CO2 Heat Pump Water Heater  

Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

CO 2 Heat Pump Water Heater 2014 Building Technologies Office Peer Review Evaporator Kyle Gluesenkamp, gluesenkampk@ornl.gov Oak Ridge National Laboratory Project Summary Timeline:...

227

Risk Assessment and Monitoring of Stored CO2 in Organic Rocks Under Non-Equilibrium Conditions  

SciTech Connect (OSTI)

The USA is embarking upon tackling the serious environmental challenges posed to the world by greenhouse gases, especially carbon dioxide (CO2). The dimension of the problem is daunting. In fact, according to the Energy Information Agency, nearly 6 billion metric tons of CO2 were produced in the USA in 2007 with coal-burning power plants contributing about 2 billion metric tons. To mitigate the concerns associated with CO2 emission, geological sequestration holds promise. Among the potential geological storage sites, unmineable coal seams and shale formations in particular show promise because of the probability of methane recovery while sequestering the CO2. However. the success of large-scale sequestration of CO2 in coal and shale would hinge on a thorough understanding of CO2's interactions with host reservoirs. An important parameter for successful storage of CO2 reservoirs would be whether the pressurized CO2 would remain invariant in coal and shale formations under reasonable internal and/or external perturbations. Recent research has brought to the fore the potential of induced seismicity, which may result in caprock compromise. Therefore, to evaluate the potential risks involved in sequestering CO2 in Illinois bituminous coal seams and shale, we studied: (i) the mechanical behavior of Murphysboro (Illinois) and Houchin Creek (Illinois) coals, (ii) thermodynamic behavior of Illinois bituminous coal at - 100oC ? T ? 300oC, (iii) how high pressure CO2 (up to 20.7 MPa) modifies the viscosity of the host, (iv) the rate of emission of CO2 from Illinois bituminous coal and shale cores if the cores, which were pressurized with high pressure (? 20.7 MPa) CO2, were exposed to an atmospheric pressure, simulating the development of leakage pathways, (v) whether there are any fractions of CO2 stored in these hosts which are resistance to emission by simply exposing the cores to atmospheric pressure, and (vi) how compressive shockwaves applied to the coal and shale cores, which were pressurized with high pressure CO2, determine the fate of sequestered CO2 in these cores. Our results suggested that Illinois bituminous coal in its unperturbed state, i.e., when not pressurized with CO2, showed large variations in the mechanical properties. Modulus varied from 0.7 GPa to 3.4 GPa even though samples were extracted from a single large chunk of coal. We did not observe any glass transition for Illinois bituminous coal at - 100oC ? T ? 300oC, however, when the coal was pressurized with CO2 at ambient ? P ? 20.7 MPa, the viscosity of the coal decreased and inversely scaled with the CO2 pressure. The decrease in viscosity as a function of pressure could pose CO2 injection problems for coal as lower viscosity would allow the solid coal to flow to plug the fractures, fissures, and cleats. Our experiments also showed a very small fraction of CO2 was absorbed in coal; and when CO2 pressurized coals were exposed to atmospheric conditions, the loss of CO2 from coals was massive. Half of the sequestered gas from the coal cores was lost in less than 20 minutes. Our shockwave experiments on Illinois bituminous coal, New Albany shale (Illinois), Devonian shale (Ohio), and Utica shale (Ohio) presented clear evidence that the significant emission of the sequestered CO2 from these formations cannot be discounted during seismic activity, especially if caprock is compromised. It is argued that additional shockwave studies, both compressive and transverse, would be required for successfully mapping the risks associated with sequestering high pressure CO2 in coal and shale formations.

Malhotra, Vivak

2014-06-30T23:59:59.000Z

228

Atmospheric Carbon Dioxide Record from Mauna Loa  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

SIO Air Sampling Network » Mauna Loa SIO Air Sampling Network » Mauna Loa Atmospheric Carbon Dioxide Record from Mauna Loa DOI: 10.3334/CDIAC/atg.035 graphics Graphics data Data Investigators R.F. Keeling, S.C. Piper, A.F. Bollenbacher and J.S. Walker Carbon Dioxide Research Group Scripps Institution of Oceanography University of California La Jolla, California 92093-0444, U.S.A. Period of Record 1958-2008 Methods Air samples at Mauna Loa are collected continuously from air intakes at the top of four 7-m towers and one 27-m tower. Four air samples are collected each hour for the purpose of determining the CO2 concentration. Determinations of CO2 are made by using a Siemens Ultramat 3 nondispersive infrared gas analyzer with a water vapor freeze trap. This analyzer registers the concentration of CO2 in a stream of air flowing at ~0.5

229

Uncertainty of ConcentrationTerrestrial Carbon Feedback in Earth System Models  

Science Journals Connector (OSTI)

Carbon uptake by land and ocean as a biogeochemical response to increasing atmospheric CO2 concentration is called concentrationcarbon feedback and is one of the carbon cycle feedbacks of the global climate. This feedback can have a major impact ...

Tomohiro Hajima; Kaoru Tachiiri; Akihiko Ito; Michio Kawamiya

2014-05-01T23:59:59.000Z

230

The supply chain of CO2 emissions  

Science Journals Connector (OSTI)

...secondary fuels (e.g., diesel, gasoline, electricity, etc.), which...Warming and Energy Policy , Free-market approaches to controlling...ofnatural gas (MtCO2) GDP[B$, Market Exchange Rate(MER...ofnatural gas (MtCO2) GDP[B$, Market Exchange Rate(MER...

Steven J. Davis; Glen P. Peters; Ken Caldeira

2011-01-01T23:59:59.000Z

231

Interactions of Supercritical CO2 with Coal  

Science Journals Connector (OSTI)

Carbon dioxide (CO2) mainly emitted from fossil fuel combustion causes global warming. ... (23) CO2 and methane might penetrate the coal matrix and cause coals to expand to some extent. ... Four coals ranging in carbon content from 77 to 84% C were warmed in the weak swelling solvent chlorobenzene at 132C for 2 wk, and samples were withdrawn at intervals. ...

Dengfeng Zhang; Lili Gu; Songgeng Li; Peichao Lian; Jun Tao

2012-12-15T23:59:59.000Z

232

Sequestration of CO2 by Concrete Carbonation  

Science Journals Connector (OSTI)

Sequestration of CO2 by Concrete Carbonation ... Carbonation of reinforced concrete is one of the causes of corrosion, but it is also a way to sequester CO2. ... This work attempts to advance the knowledge of the carbon footprint of cement. ...

Isabel Galan; Carmen Andrade; Pedro Mora; Miguel A. Sanjuan

2010-03-12T23:59:59.000Z

233

Absorption of 9.6-?m CO2 laser radiation by CO2 at elevated temperatures  

Science Journals Connector (OSTI)

Absorption of 9.6-?m CO2 laser radiation by CO2 at temperatures between 296 and 625 K has been measured at a pressure of 200 Torr. Experimental results for the...

Robinson, A M

1983-01-01T23:59:59.000Z

234

Study of CO 2 Mobility Control in Heterogeneous Media Using CO 2 Thickening Agents  

E-Print Network [OSTI]

CO 2 injection is an effective method for performing enhanced oil recovery (EOR). There are several factors that make CO 2 useful for EOR, including promoting swelling, reducing oil viscosity, decreasing oil density, and vaporizing and extracting...

Al Yousef, Zuhair

2012-10-19T23:59:59.000Z

235

Interactions between reducing CO2 emissions, CO2 removal and solar radiation management  

Science Journals Connector (OSTI)

...World Energy Council. 41 World Energy Council.2009 Survey of energy resources interim update 2009. London, UK: World Energy Council. 42 Haszeldine, R. S...CO2 emissions, CO2 removal and solar radiation management. | We use...

2012-01-01T23:59:59.000Z

236

NETL: IEP – Oxy-Combustion CO2 Emissions Control - CANMET CO2  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

– Oxy-Combustion CO2 Emissions Control – Oxy-Combustion CO2 Emissions Control CANMET CO2 Consortium-O2/CO2 Recycle Combustion Project No.: IEA-CANMET-CO2 (International Agreement) Photograph of CANMET's Vertical Combustor Research Facility. Photograph of CANMET’s Vertical Combustor Research Facility. The CANMET carbon dioxide (CO2) consortium will conduct research to further the development of oxy-combustion for retrofit to coal-fired power plants. Research activities include: (1) modeling of an advanced, supercritical pressure oxy-coal plant, including an analysis of the impact of oxygen (O2) purity and O2 partial enrichment, overall process performance, and cost; (2) testing of pilot-scale CO2 capture and compression; (3) investigating CO2 phase change at liquid and supercritical states in gas mixtures

237

NETL: NATCARB - CO2 Storage Formations  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Storage Formations Storage Formations NATCARB CO2 Storage Formations CO2 Storage Resource Methodology NATCARB Viewer The NATCARB Viewer is available at: http://www.natcarbviewer.com. 2012 Atlas IV DOE's Regional Carbon Sequestration Partnerships (RCSPs) were charged with providing a high-level, quantitative estimate of carbon dioxide (CO2) storage resource available in subsurface environments of their regions. Environments considered for CO2 storage were categorized into five major geologic systems: oil and gas reservoirs, unmineable coal areas, saline formations, shale, and basalt formations. Where possible, CO2 storage resource estimates have been quantified for oil and gas reservoirs, saline formations, and unmineable coal in the fourth edition of the United States Carbon Utilization and Storage Atlas (Atlas IV). Shale and basalt

238

Impact of mesophyll diffusion on estimated global land CO2 fertilization  

Science Journals Connector (OSTI)

...historical atmospheric CO2 by Earth system models. Without this correction...limitation. Our results imply that Earth system models (ESMs) will overpredict the long-term...atmospheric carbon dioxide biases in Earth System Models . J Geophys Res Biogeosci 119 ( 2 ): 141...

Ying Sun; Lianhong Gu; Robert E. Dickinson; Richard J. Norby; Stephen G. Pallardy; Forrest M. Hoffman

2014-01-01T23:59:59.000Z

239

meters in CO2 euthanasia chambers. All CO2 euthanasia chambers in both  

E-Print Network [OSTI]

meters in CO2 euthanasia chambers. All CO2 euthanasia chambers in both the facilities and laboratories will need flow meters. ULAR is currently in the process of identifying a cost-effective, accurate, and durable flow meter to install in all of the CO2 chambers in all of the vivaria. When a specific model

Bushman, Frederic

240

Trace gases, CO2, climate, and the greenhouse effect  

Science Journals Connector (OSTI)

Weather is driven by the suns energy input and the difference between insolation per unit area of the poles and the equator. The energy flux of the Earth is in long?term balanceas much is radiated away by the Earth as is absorbed or the mean temperature would have to increase or decrease steadily (and of course this is not observed). CO2 and other trace gases can cause the Earths mean temperature to rise through the Greenhouse Effect. The mean temperature in the Little Ice Age was only 1?C cooler but large effects were felt especially toward the poles. The CO2 which stays in the atmosphere will raise Earths mean temperature with effects which are relatively certain: a lot of warming at the poles and a very small amount of warming at the equator.

Gordon J. Aubrecht II

1988-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


241

Effects of CO2-Induced Seawater Acidification on Microbial Processes Involving Dissolved Organic Matter  

Science Journals Connector (OSTI)

Abstract We used laboratory experiments covering a wide range of carbon dioxide (CO2) induced seawater acidification to simulate ocean CO2 storage and assess the potential effects on heterotrophic microbial processes associated with labile dissolved organic matter (DOM). There was no noticeable effect of increased CO2 concentration on short-term decomposition of labile DOM or nutrient uptake. However, microbial activities producing new DOM were apparently enhanced under treatments with 2000 or 5000ppm CO2. Under these conditions, production of aggregates was inhibited in early stage. Both of acute and chronic effects should be included for assessment of biogeochemical cycle related to microbe process.

Namiha Yamada; Nobuo Tsurushima; Masahiro Suzumura

2013-01-01T23:59:59.000Z

242

Impact of Solar Resource and Atmospheric Constituents on Energy Yield Models for Concentrated Photovoltaic Systems .  

E-Print Network [OSTI]

??Global economic trends suggest that there is a need to generate sustainable renewable energy to meet growing global energy demands. Solar energy harnessed by concentrated (more)

Mohammed, Jafaru

2013-01-01T23:59:59.000Z

243

E-Print Network 3.0 - atmospheric radon-222 concentration Sample...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

1. Radon-222... concentrations in air include ... Source: Baskaran, Mark - Department of Geology, Wayne State University Collection: Geosciences ; Chemistry 30 1.0 MAJOR STUDIES...

244

Estimates of Radioxenon Released from Southern Hemisphere Medical isotope Production Facilities Using Measured Air Concentrations and Atmospheric Transport Modeling  

SciTech Connect (OSTI)

Abstract The International Monitoring System (IMS) of the Comprehensive-Nuclear-Test-Ban-Treaty monitors the atmosphere for radioactive xenon leaking from underground nuclear explosions. Emissions from medical isotope production represent a challenging background signal when determining whether measured radioxenon in the atmosphere is associated with a nuclear explosion prohibited by the treaty. The Australian Nuclear Science and Technology Organisation (ANSTO) operates a reactor and medical isotope production facility in Lucas Heights, Australia. This study uses two years of release data from the ANSTO medical isotope production facility and Xe-133 data from three IMS sampling locations to estimate the annual releases of Xe-133 from medical isotope production facilities in Argentina, South Africa, and Indonesia. Atmospheric dilution factors derived from a global atmospheric transport model were used in an optimization scheme to estimate annual release values by facility. The annual releases of about 6.81014 Bq from the ANSTO medical isotope production facility are in good agreement with the sampled concentrations at these three IMS sampling locations. Annual release estimates for the facility in South Africa vary from 1.21016 to 2.51016 Bq and estimates for the facility in Indonesia vary from 6.11013 to 3.61014 Bq. Although some releases from the facility in Argentina may reach these IMS sampling locations, the solution to the objective function is insensitive to the magnitude of those releases.

Eslinger, Paul W.; Friese, Judah I.; Lowrey, Justin D.; McIntyre, Justin I.; Miley, Harry S.; Schrom, Brian T.

2014-04-06T23:59:59.000Z

245

Ancient Lava Flows Trap CO2 for Long-Term Storage in Big Sky Injection |  

Broader source: Energy.gov (indexed) [DOE]

Ancient Lava Flows Trap CO2 for Long-Term Storage in Big Sky Ancient Lava Flows Trap CO2 for Long-Term Storage in Big Sky Injection Ancient Lava Flows Trap CO2 for Long-Term Storage in Big Sky Injection August 13, 2013 - 1:59pm Addthis Photo by J.D. Griggs, courtesy of U.S.Geological Survey Photo by J.D. Griggs, courtesy of U.S.Geological Survey For Additional Information To learn more about the carbon storage projects in which NETL is involved, please visit the NETL Carbon Storage website How can a prehistoric volcanic eruption help us reduce the amount of CO2 released into the atmosphere today? The answer is found in the basalt formations created by the lava - formations that can be used as sites for injecting carbon dioxide (CO2) captured from industrial sources in a process called carbon capture and storage (CCS).

246

Ancient Lava Flows Trap CO2 for Long-Term Storage in Big Sky Injection |  

Broader source: Energy.gov (indexed) [DOE]

Ancient Lava Flows Trap CO2 for Long-Term Storage in Big Sky Ancient Lava Flows Trap CO2 for Long-Term Storage in Big Sky Injection Ancient Lava Flows Trap CO2 for Long-Term Storage in Big Sky Injection August 13, 2013 - 1:59pm Addthis Photo by J.D. Griggs, courtesy of U.S.Geological Survey Photo by J.D. Griggs, courtesy of U.S.Geological Survey For Additional Information To learn more about the carbon storage projects in which NETL is involved, please visit the NETL Carbon Storage website How can a prehistoric volcanic eruption help us reduce the amount of CO2 released into the atmosphere today? The answer is found in the basalt formations created by the lava - formations that can be used as sites for injecting carbon dioxide (CO2) captured from industrial sources in a process called carbon capture and storage (CCS).

247

CO2 Emissions from Fuel Combustion | Open Energy Information  

Open Energy Info (EERE)

CO2 Emissions from Fuel Combustion CO2 Emissions from Fuel Combustion Jump to: navigation, search Tool Summary Name: CO2 Emissions from Fuel Combustion Agency/Company /Organization: International Energy Agency Sector: Energy Topics: Baseline projection, GHG inventory Resource Type: Dataset, Publications Website: www.iea.org/co2highlights/co2highlights.pdf CO2 Emissions from Fuel Combustion Screenshot References: CO2 Emissions from Fuel Combustion[1] Overview "This annual publication contains: estimates of CO2 emissions by country from 1971 to 2008 selected indicators such as CO2/GDP, CO2/capita, CO2/TPES and CO2/kWh CO2 emissions from international marine and aviation bunkers, and other relevant information" Excel Spreadsheet References ↑ "CO2 Emissions from Fuel Combustion"

248

Particle Phase Concentrations of Polycyclic Aromatic Hydrocarbons in the Atmospheric Environment of Jinmar, Gran Canaria  

Science Journals Connector (OSTI)

Airborne concentrations of 8 polycyclic aromatic hydrocarbons (PAHs): fluoranthene, Flt, Pyrene, Pyr, benzo(a)anthracene, BaA, chrysene, Chr, benzo(b)fluoranthene + benzo(k)fluoranthene,B(b + k)F, benzo(a)pyrene,...

Jos A. Lpez Cancio; Antonio Vera Castellano

2002-05-01T23:59:59.000Z

249

Microsoft Word - CO2 Supplement.doc  

Gasoline and Diesel Fuel Update (EIA)

Understanding the Decline in Carbon Dioxide Understanding the Decline in Carbon Dioxide Emissions in 2009 1 EIA projects carbon dioxide (CO2) emissions from fossil fuels in 2009 to be 5.9 percent below the 2008 level in the Short-Term Energy Outlook, October 2009 (STEO) (Table 1). Projected coal CO2 emissions fall by 10.1 percent in 2009, primarily because of lower consumption for electricity generation. Coal accounts for 63 percent of the total decline in CO2 emissions from fossil fuels this year. Forecast lower natural gas and petroleum emissions this year make up 7 percent and 30 percent of the projected total decline in CO2 emissions from fossil fuels, respectively. Table 1. Short-Term Energy Outlook CO

250

Increasing CO2 Storage in Oil Recovery  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Increasing CO Increasing CO 2 Storage in Oil Recovery Kristian Jessen (krisj@pangea.stanford.edu, 650-723-6348) Linda C. Sam-Olibale (chizoba@pangea.stanford.edu, 650-725-0831) Anthony R. Kovscek (kovscek@pangea.stanford.edu, 650-723-1218) Franklin M. Orr, Jr. (fmorr@pangea.stanford.edu, 650-723-2750) Department of Petroleum Engineering, Stanford University 65 Green Earth Sciences Building 367 Panama Street Stanford, CA 94305-2220 Introduction Carbon dioxide (CO 2 ) injection has been used as a commercial process for enhanced oil recovery (EOR) since the 1970's. Because the cost of oil recovered is closely linked to the purchase cost of the CO 2 injected, considerable reservoir engineering design effort has gone into reducing the total amount of CO 2 required to recover each barrel of oil. If,

251

Microsoft Word - TURBO EXPO CO2 draft  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

MAN TURBO MAN TURBO CO2 Compression Challenges presented on May 15, 2007 at the ASME Turbo Expo, Montreal, CO2 Compression Panel By Pierre L. Bovon, MAN TURBO Calgary (pierre.bovon@ca.manturbo.com, tel. +403 233 7151) And Dr. Rolf Habel, MAN TURBO Berlin (rolf.habel@de.manturbo.com, tel. +49 304 301 2224) CO2 has been used for a very long time, for instance in the food industry, and most applications have required it to be compressed. For Sequestration or Enhanced Oil Recovery, the traditional approach to CO2 compression has been to use high-speed reciprocating compressors. The main reasons are: - Flexibility with regards to pressure ratio, and capacity (if equipped with variable speed drive or valve unloaders). - Short delivery times, since many recip. packagers dispose of a selection of frames

252

India Fossil-Fuel CO2 Emissions  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

India India India Fossil-Fuel CO2 Emissions Graph graphic Graphics Data graphic Data Trends India's 2008 total fossil-fuel CO2 emissions rose 8.1% over the 2007 level to 475 million metric tons of carbon. From 1950 to 2008, India experienced dramatic growth in fossil-fuel CO2 emissions averaging 5.7% per year and becoming the world's third largest fossil-fuel CO2-emitting country. Indian total emissions from fossil-fuel consumption and cement production have more than doubled since 1994. Fossil-fuel emissions in India continue to result largely from coal burning with India being the world's third largest producer of coal. Coal contributed 87% of the emissions in 1950 and 71% in 2008; at the same time, the oil fraction increased from 11% to 20%. Indian emissions data reveal little impact from the oil price increases that

253

081001 CA CO2 Storage Pilot  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

California California CO2 Storage Pilot Regional Carbon Sequestration Partnerships Initiative Review Meeting Pittsburgh, Pennsylvania October 7, 2008 John Henry Beyer, Ph.D. WESTCARB Program Manager, Geophysicist 510-486-7954, jhbeyer@lbl.gov Lawrence Berkeley National Laboratory Earth Sciences Division, MS 90-1116 Berkeley, CA 94720 2 Industry Partner: Shell Oil Company Committed to reducing global CO2 emissions Extensive technical expertise in: - Geologic evaluation - Well log analysis - Porosity and permeability evaluation - Geophysics - Deep well drilling - CO2 injection A welcome industry partner 3 - Bevilacqua-Knight, Inc. (DOE/PIER) - Lawrence Berkeley National Lab (PIER) - Sandia Technologies, LLC (DOE/PIER) - Terralog (DOE) Northern California CO2 Storage Pilot Contracting and Funding Flow

254

CO2 Europipe | Open Energy Information  

Open Energy Info (EERE)

Page Page Edit with form History Facebook icon Twitter icon » CO2 Europipe Jump to: navigation, search Tool Summary LAUNCH TOOL Name: CO2 Europipe Focus Area: Clean Fossil Energy Topics: Potentials & Scenarios Website: www.co2europipe.eu/ Equivalent URI: cleanenergysolutions.org/content/co2-europipe Language: English Policies: "Deployment Programs,Regulations,Financial Incentives" is not in the list of possible values (Deployment Programs, Financial Incentives, Regulations) for this property. DeploymentPrograms: Project Development Regulations: "Emissions Mitigation Scheme,Emissions Standards,Enabling Legislation" is not in the list of possible values (Agriculture Efficiency Requirements, Appliance & Equipment Standards and Required Labeling, Audit Requirements, Building Certification, Building Codes, Cost Recovery/Allocation, Emissions Mitigation Scheme, Emissions Standards, Enabling Legislation, Energy Standards, Feebates, Feed-in Tariffs, Fuel Efficiency Standards, Incandescent Phase-Out, Mandates/Targets, Net Metering & Interconnection, Resource Integration Planning, Safety Standards, Upgrade Requirements, Utility/Electricity Service Costs) for this property.

255

NETL: NATCARB - CO2 Stationary Sources  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Stationary Sources Stationary Sources NATCARB CO2 Stationary Sources CO2 Stationary Source Emission Estimation Methodology NATCARB Viewer The NATCARB Viewer is available at: http://www.natcarbviewer.com. 2012 Atlas IV DOE's Regional Carbon Sequestration Partnerships (RCSPs) employed carbon dioxide (CO2) emissions estimate methodologies that are based on the most readily available representative data for that particular industry type within the respective partnership area. Carbon dioxide emissions data provided by databases (for example, eGRID, IEA GHG, or NATCARB) were the first choice for all of the RCSPs, both for identifying major CO2 stationary sources and for providing reliable emission estimations. Databases are considered to contain reliable and accurate data obtained

256

co2-transport | netl.doe.gov  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Tools and Data Baseline Studies Quality Guidelines (QGESS) About Energy Analysis FENETL CO2 Transport Cost Model About the model: This model was developed to estimate the cost of...

257

Enhanced CO2 Gas Storage in Coal  

Science Journals Connector (OSTI)

Greenhouse gas (GHG) such as carbon dioxide (CO2) is largely believed to be a primary contributor to global warming. ... Four coals of various rank exploited from four main coal seams in China were tested. ...

Shu-Qing Hao; Sungho Kim; Yong Qin; Xue-Hai Fu

2013-12-05T23:59:59.000Z

258

Adsorption Behavior of CO2 in Coal and Coal Char  

Science Journals Connector (OSTI)

Coals of diverse characteristics have been chosen to provide a better understanding on the influence of various coal properties, such as maceral, volatile matter, and ash contents. ... In addition, char samples from two of these coals (a non-coking coal A and a coking coal B) were prepared by pyrolysis at 800 and 1000 C in a nitrogen atmosphere and were tested for CO2 adsorption capacity. ... As stated earlier, virgin coal samples considered for the adsorption measurements include coals A, C, and D, which are of low-, high-, and medium-volatile sub-bituminous rank, respectively. ...

Shanmuganathan Ramasamy; Pavan Pramod Sripada; Md Moniruzzaman Khan; Su Tian; Japan Trivedi; Rajender Gupta

2014-07-01T23:59:59.000Z

259

Research on CO2 Emission Control  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

of Clean Energy Utilization of Clean Energy Utilization Zhejing University 29 th May, 2008 Status of CCS in China 2 nd U.S.-China Symposium on CO 2 Emission Control Science & Technology, Hangzhou China 28 th -30 th , May, 2008 Prof. Zhongyang Luo Global CO 2 Emissions Country CO 2 Emissions (Million Tons Carbon) 1990 1997 2001 2010 USA 1345 1480 1559 1800 China 620 822 832 1109 Former USSR 1034 646 654 825 Japan 274 297 316 334 World 5836 6175 6522 8512 Source: Energy Information Administration/International Energy Outlook 2001 Global CO 2 Emissions from Fossil Fuel Use in 2006 11.72 3,330 EU-15 5.75 1,620 Russia 4.3 1,210 Japan 20.17 5,680 China 20.42 5,750 USA 100 28,160 Total Percentage (%) CO 2 Emissions (1 million metric tons CO 2 ) Country BP Statistical Review of World Energy, June 2007 (http://www.bp.com/sectiongenericarticle.do?categoryId=6914&contentI

260

Co-Location of Air Capture, Subseafloor CO2 Sequestration, and Energy Production on the Kerguelen Plateau  

Science Journals Connector (OSTI)

Reducing atmospheric CO2 using a combination of air capture and offshore geological storage can address technical and policy concerns with climate mitigation. ... Our analysis suggests that Kerguelen offers a remote and environmentally secure location for CO2 sequestration using renewable energy. ...

David S. Goldberg; Klaus S. Lackner; Patrick Han; Angela L. Slagle; Tao Wang

2013-06-07T23:59:59.000Z

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


261

Thermal Imaging of Vegetation to Detect CO2 Gas Leaking From Underground  

Science Journals Connector (OSTI)

Thermal imaging of vegetation has been used to detect CO2 gas leaking from an underground gas reservoir. Plant stress caused by increased soil gas concentration results in warmer...

Shaw, Joseph A; Johnson, Jennifer E; Lawrence, Rick; Nugent, Paul W

262

Radiocarbon Measurements of Atmospheric Volatile Organic Compounds:? Quantifying the Biogenic Contribution  

Science Journals Connector (OSTI)

The ability to obtain quality (interpretable) [14C]VOC measurements however relies on additional factors:? (1) transferring individual VOCs to the measurement system in a manner that preserves their original relative concentrations in the atmosphere (recovery), (2) quantifying limitations in the VOC isolation process (bias), and 3) quantifying chemical and isotopic contamination (blanks). ... The fM results for the VOC fractions from calibration mixtures and ambient samples are corrected for CO2 contamination using eq 2, where ?BLK in this case is defined as in which mCO2 is the carbon mass of residual atmospheric CO2 following LiOH treatment plus the carbon mass of CO2 contamination from the O2 used for VOC oxidation, and mREC is the total recovered carbon (Table 3). ... During pressurized sampling of humid air, water will be condensed in the canisters. ...

George A. Klouda; Charles W. Lewis; Reinhold A. Rasmussen; George C. Rhoderick; Robert L. Sams; Robert K. Stevens; Lloyd A. Currie; Douglas J. Donahue; A. J. Timothy Jull; Robert L. Seila

1996-03-26T23:59:59.000Z

263

Biomass combustion with in situ CO2 capture by CaO in a 300kWth circulating fluidized bed facility  

Science Journals Connector (OSTI)

Abstract This paper reports experimental results from a new 300kWth calcium looping pilot plant designed to capture CO2 in situ during the combustion of biomass in a fluidized bed. This novel concept relies on the high reactivity of biomass as a fuel, which allows for effective combustion around 700C in air at atmospheric pressure. In these conditions, CaO particles fed into the fluidized bed combustor react with the CO2 generated during biomass combustion, allowing for an effective CO2 capture. A subsequent step of regeneration of CaCO3 in an oxy-fired calciner is also needed to release a concentrated stream of CO2. This regeneration step is assumed to be integrated in a large scale oxyfired power plant and/or a larger scale post-combustion calcium looping system. The combustor-carbonator is the key reactor in this novel concept, and this work presents experimental results from a 300kWth pilot to test such a reactor. The pilot involves two 12m height interconnected circulating fluidized bed reactors. Several series of experiments to investigate the combustor-carbonator reactor have been carried out achieving combustion efficiencies close to 100% and CO2 capture efficiencies between 70 and 95% in dynamic and stationary state conditions, using wood pellets as a fuel. Different superficial gas velocities, excess air ratios above stoichiometric requirements, and solid circulating rates between combustor-carbonator and combustor-calciner have been tested during the experiments. Closure of the carbon and oxygen balances during the combustion and carbonation trials has been successful. A simple reactor model for combustion and CO2 capture in the combustor-carbonator has been applied to aid in the interpretation of results, which should facilitate the future scaling up of this process concept.

M. Alonso; M.E. Diego; C. Prez; J.R. Chamberlain; J.C. Abanades

2014-01-01T23:59:59.000Z

264

Development of Novel CO2 Adsorbents for Capture of CO2 from Flue...  

Office of Scientific and Technical Information (OSTI)

Bloomfield Avenue, University of Hartford, West Hartford, Connecticut 06117-1599 ABSTRACT Carbon Sequestration, the capturing and storing of carbon dioxide (CO 2 ) emissions...

265

ANEMOS: A computer code to estimate air concentrations and ground deposition rates for atmospheric nuclides emitted from multiple operating sources  

SciTech Connect (OSTI)

This code estimates concentrations in air and ground deposition rates for Atmospheric Nuclides Emitted from Multiple Operating Sources. ANEMOS is one component of an integrated Computerized Radiological Risk Investigation System (CRRIS) developed for the US Environmental Protection Agency (EPA) for use in performing radiological assessments and in developing radiation standards. The concentrations and deposition rates calculated by ANEMOS are used in subsequent portions of the CRRIS for estimating doses and risks to man. The calculations made in ANEMOS are based on the use of a straight-line Gaussian plume atmospheric dispersion model with both dry and wet deposition parameter options. The code will accommodate a ground-level or elevated point and area source or windblown source. Adjustments may be made during the calculations for surface roughness, building wake effects, terrain height, wind speed at the height of release, the variation in plume rise as a function of downwind distance, and the in-growth and decay of daughter products in the plume as it travels downwind. ANEMOS can also accommodate multiple particle sizes and clearance classes, and it may be used to calculate the dose from a finite plume of gamma-ray-emitting radionuclides passing overhead. The output of this code is presented for 16 sectors of a circular grid. ANEMOS can calculate both the sector-average concentrations and deposition rates at a given set of downwind distances in each sector and the average of these quantities over an area within each sector bounded by two successive downwind distances. ANEMOS is designed to be used primarily for continuous, long-term radionuclide releases. This report describes the models used in the code, their computer implementation, the uncertainty associated with their use, and the use of ANEMOS in conjunction with other codes in the CRRIS. A listing of the code is included in Appendix C.

Miller, C.W.; Sjoreen, A.L.; Begovich, C.L.; Hermann, O.W.

1986-11-01T23:59:59.000Z

266

CO2 Heat Pump Water Heater | Department of Energy  

Office of Energy Efficiency and Renewable Energy (EERE) Indexed Site

Heater CO2 Heat Pump Water Heater CO2 Heat Pump Water Heater Prototype
Credit: Oak Ridge National Lab CO2 Heat Pump Water Heater Prototype Credit: Oak Ridge National Lab...

267

Poland Fossil-Fuel CO2 Emissions  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Europe Europe » Poland Poland Fossil-Fuel CO2 Emissions Graph graphic Graphics Data graphic Data Trends Carbon dioxide emissions from Poland's use of fossil-fuels and cement production climbed at a remarkably steady rate of 3.9% per year from 1800 until 1980, when they dropped abruptly (11.7%). Fossil-fuel CO2 emissions crept back up throughout the 1980s peaking in 1987 at 127 million metric tons of carbon. Since the 1987 high, CO2 emissions have plummeted 32% to early 1970s levels while per capita emissions have dropped to late 1960s levels. Poland is the world's ninth largest producer of coal and emissions are predominantly from coal burning: 97% in 1950 and 68% in 2008. The drop following 1980 is apparent in rates of liquid fuel burning but releases from consumption of petroleum products have returned and surpassed 1980s

268

Japan Fossil-Fuel CO2 Emissions  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Oceania » Japan Oceania » Japan Japan Fossil-Fuel CO2 Emissions Graph graphic Graphics Data graphic Data Trends The history of fossil-fuel CO2 emissions from Japan is remarkable for the abrupt change that occurred in 1973. With postwar growth at 9.8% per year from 1950 to 1973, total emissions were virtually constant from 1974-1987. From 1987-96, emissions grew 25.3% reaching 329 million metric tons of carbon. Growth during this period was characterized by a return to mid-1970s consumption levels for liquid petroleum products and increased contributions from coal and natural gas use. Since 1996, Japan's fossil-fuel CO2 emissions have vacilated and now total 329 million metric tons of carbon in 2008. Based on United Nations energy trade data for 2008, Japan is the world's largest importer of coal (184 million metric tons) and

269

NETL: IEP – Oxy-Combustion CO2 Emissions Control - Oxygen-Based PC Boiler  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

– Oxy-Combustion CO2 Emissions Control – Oxy-Combustion CO2 Emissions Control Oxygen-Based PC Boiler Project No.: FC26-04NT42207 & FC26-03NT41736 Spatial Comparison of an Air-Fired Furnace versus an Oxygen-Fired Furnace. Spatial Comparison of an Air-Fired Furnace versus an Oxygen-Fired Furnace. Foster Wheeler North America Corporation will conduct to two projects to improve carbon dioxide (CO2) capture technology by developing a conceptual pulverized coal-fired boiler system design using oxygen as the combustion medium. Using oxygen instead of air produces a flue gas with a high CO2 concentration, which will facilitate CO2 capture for subsequent sequestration. The first project will develop modeling simulations that will lead to a conceptual design that addresses costs, performance, and emissions, and

270

Geologic CO2 sequestration inhibits microbial growth | EMSL  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

community and could improve overall efficiency of CO2 sequestration. The Science Carbon dioxide (CO2) sequestration in deep subsurface environments has received...

271

Cryogenic CO2 Formation on Oxidized Gold Clusters Synthesized...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Cryogenic CO2 Formation on Oxidized Gold Clusters Synthesized via Reactive Layer Assisted Deposition. Cryogenic CO2 Formation on Oxidized Gold Clusters Synthesized via Reactive...

272

Exsolution Enhanced Oil Recovery with Concurrent CO2 Sequestration...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Exsolution Enhanced Oil Recovery with Concurrent CO2 Sequestration. Exsolution Enhanced Oil Recovery with Concurrent CO2 Sequestration. Abstract: A novel EOR method using...

273

Reaction of Water-Saturated Supercritical CO2 with Forsterite...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Water-Saturated Supercritical CO2 with Forsterite: Evidence for Magnesite Formation at Low Temperatures. Reaction of Water-Saturated Supercritical CO2 with Forsterite: Evidence for...

274

numerical methodology to model and monitor co2 sequestration  

E-Print Network [OSTI]

CO2 sequestration is a means of mitigating the greenhouse effect [1]. Geologic sequestration involves injecting CO2 into a target geologic formation at depths...

santos,,,

275

Numerical Simulation of CO2 Sequestration in Natural CO2 Reservoirs on the Colorado Plateau  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Simulation of CO Simulation of CO 2 Sequestration in Natural CO 2 Reservoirs on the Colorado Plateau Stephen P. White (S.White@irl.cri.nz, (64) 4 5690000) Graham J. Weir (G.Weir@irl.cri.nz, (64) 4 5690000) Warwick M. Kissling (W.Kissling@irl.cri.nz, (64) 4 5690000) Industrial Research Ltd. P.O. Box 31310 Lower Hutt, New Zealand Abstract This paper outlines the proposed research and summarizes pre-project work that forms a basis for a new research program on CO 2 sequestration in saline aquifers. The pre-project work considers storage and disposal of CO 2 several kilometers beneath the surface in generic aquifers and demonstrates the use of reactive chemical transport modeling to simulate mineral sequestration of CO 2. The current research project applies these techniques to particular saline

276

Field Demonstration of CO2 Leakage Detection in Potable Aquifers with a Pulselike CO2-Release Test  

Science Journals Connector (OSTI)

Field Demonstration of CO2 Leakage Detection in Potable Aquifers with a Pulselike CO2-Release Test ... This study presents two field pulselike CO2-release tests to demonstrate CO2 leakage detection in a shallow aquifer by monitoring groundwater pH, alkalinity, and dissolved inorganic carbon (DIC) using the periodic groundwater sampling method and a fiber-optic CO2 sensor for real-time in situ monitoring of dissolved CO2 in groundwater. ...

Changbing Yang; Susan D. Hovorka; Jesus Delgado-Alonso; Patrick J. Mickler; Ramn H. Trevio; Straun Phillips

2014-11-10T23:59:59.000Z

277

Measurement of Atmospheric Sea Salt Concentration in the Dry Storage Facility of the Spent Nuclear Fuel  

SciTech Connect (OSTI)

Spent nuclear fuel coming from a Japanese nuclear power plant is stored in the interim storage facility before reprocessing. There are two types of the storage methods which are wet and dry type. In Japan, it is anticipated that the dry storage facility will increase compared with the wet type facility. The dry interim storage facility using the metal cask has been operated in Japan. In another dry storage technology, there is a concrete overpack. Especially in USA, a lot of concrete overpacks are used for the dry interim storage. In Japan, for the concrete cask, the codes of the Japan Society of Mechanical Engineers and the governmental technical guidelines are prepared for the realization of the interim storage as well as the code for the metal cask. But the interim storage using the concrete overpack has not been in progress because the evaluation on the stress corrosion cracking (SCC) of the canister is not sufficient. Japanese interim storage facilities would be constructed near the seashore. The metal casks and concrete overpacks are stored in the storage building in Japan. On the other hand, in USA they are stored outside. It is necessary to remove the decay heat of the spent nuclear fuel in the cask from the storage building. Generally, the heat is removed by natural cooling in the dry storage facility. Air including the sea salt particles goes into the dry storage facility. Concerning the concrete overpack, air goes into the cask body and cools the canister. Air goes along the canister surface and is in contact with the surface directly. In this case, the sea salt in the air attaches to the surface and then there is the concern about the occurrence of the SCC. For the concrete overpack, the canister including the spent fuel is sealed by the welding. The loss of sealability caused by the SCC has to be avoided. To evaluate the SCC for the canister, it is necessary to make clear the amount of the sea salt particles coming into the storage building and the concentration on the canister. In present, the evaluation on that point is not sufficient. In this study, the concentration of the sea salt particles in the air and on the surface of the storage facility are measured inside and outside of the building. For the measurement, two sites of the dry storage facility using the metal cask are chosen. This data is applicable for the evaluation on the SCC of the canister to realize the interim storage using the concrete overpack. (authors)

Masumi Wataru; Hisashi Kato; Satoshi Kudo; Naoko Oshima; Koji Wada [Central Research Institute of Electric Power Industry - CRIEPI (Japan); Hirofumi Narutaki [Electric Power Engineering Systems Co. Ltd. (Japan)

2006-07-01T23:59:59.000Z

278

Commitment accounting of CO2 emissions  

Science Journals Connector (OSTI)

The world not only continues to build new coal-fired power plants, but built more new coal plants in the past decade than in any previous decade. Worldwide, an average of 89 gigawatts per year (GW yr1) of new coal generating capacity was added between 2010 and 2012, 23 GW yr1 more than in the 20002009 time period and 56 GW yr1 more than in the 19901999 time period. Natural gas plants show a similar pattern. Assuming these plants operate for 40 years, the fossil-fuel burning plants built in 2012 will emit approximately 19 billion tons of CO2 (Gt CO2) over their lifetimes, versus 14 Gt CO2 actually emitted by all operating fossil fuel power plants in 2012. We find that total committed emissions related to the power sector are growing at a rate of about 4% per year, and reached 307 (with an estimated uncertainty of 192439) Gt CO2 in 2012. These facts are not well known in the energy policy community, where annual emissions receive far more attention than future emissions related to new capital investments. This paper demonstrates the potential for 'commitment accounting' to inform public policy by quantifying future emissions implied by current investments.

Steven J Davis; Robert H Socolow

2014-01-01T23:59:59.000Z

279

Amine Scrubbing for CO2 Capture  

Science Journals Connector (OSTI)

...distillation columns in the air separation unit...excess and leakage air along with the CO...will not provide solutions as energy-efficient...tf9363201291 2 National Air Pollution Control Administration...CO 2 Removal from Fossil-FuelFired Power Plants (IE-7365...

Gary T. Rochelle

2009-09-25T23:59:59.000Z

280

Aquifer Management for CO2 Sequestration  

E-Print Network [OSTI]

Storage of carbon dioxide is being actively considered for the reduction of green house gases. To make an impact on the environment CO2 should be put away on the scale of gigatonnes per annum. The storage capacity of deep saline aquifers...

Anchliya, Abhishek

2010-07-14T23:59:59.000Z

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


281

Techno-economic assessment of CO2 capture at steam methane reforming facilities using commercially available technology  

Science Journals Connector (OSTI)

This study aimed to identify the optimal techno-economic configuration of CO2 capture at steam methane reforming facilities using currently available technologies by means of process simulations. Results indicate that the optimal system is CO2 capture with ADIP-X located between the watergas shift and pressure swing adsorption units. Process simulations of this system configuration showed a CO2 emission reduction of 60% at 41/t CO2 avoidance. This is at the lower end of the range reported in open literature for CO2 capture at refineries (2682/t CO2) and below the avoidance costs for CO2 capture at natural gas-fired power plants (4493/t CO2). CO2 avoidance costs are dominated by the natural gas consumption, responsible for up to 66% of total costs. Using imported steam and electricity can reduce CO2 avoidance costs by 45%. Addition of small amounts of piperazine to aqueous MDEA solutions results in up to 70% smaller absorbers or 10% lower reboiler heat duty. Optimising the whole capture process instead of individual units resulted in lower piperazine concentrations than the common industrial practice (3mass% vs. 5mass%). Finally, keeping the solvent rate constant when operating the capture unit below its design load resulted in a lower specific energy for CO2 capture than when the solvent rate was downscaled with the syngas flow.

J.C. Meerman; E.S. Hamborg; T. van Keulen; A. Ramrez; W.C. Turkenburg; A.P.C. Faaij

2012-01-01T23:59:59.000Z

282

Modeling the Direct Solar Conversion of CO2 to CO and O2  

Science Journals Connector (OSTI)

Ralph J. Price , David A. Morse , Steven L. Hardy , and Thomas H. Fletcher * ... If the path length, temperature, and concentration of CO2 are high enough, the photolysis reaction of sunlight with CO2 can also form CO and O.1 From an inlet stream of pure CO2, a product stream with 4?6 mol % CO was produced in a prototype unit using reflected sunlight as the heat source.2 This CO can then be separated and (a) used as a fuel or (b) converted to H2 through the water?gas shift reaction. ... Energy Fuels 1993, 7, 874. ...

Ralph J. Price; David A. Morse; Steven L. Hardy; Thomas H. Fletcher; Scott C. Hill; Reed J. Jensen

2004-04-20T23:59:59.000Z

283

Diurnal tracking of anthropogenic CO2 emissions in the Los Angeles basin  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Diurnal tracking of anthropogenic CO2 emissions in the Los Angeles basin Diurnal tracking of anthropogenic CO2 emissions in the Los Angeles basin megacity during spring 2010 Title Diurnal tracking of anthropogenic CO2 emissions in the Los Angeles basin megacity during spring 2010 Publication Type Journal Article Year of Publication 2012 Authors Newman, Sally, Seongeun Jeong, Marc L. Fischer, Xiaomei Xu, Christine L. Haman, Barry Lefer, Sergio Alvarez, Bernhard Rappenglueck, Eric A. Kort, Arlyn E. Andrews, Jeffrey Peischl, Kevin R. Gurney, Charles E. Miller, and Yuk L. Yung Journal Atmospheric Chemistry and Physics Volume 13 Pagination 4359-4372 Abstract Attributing observed CO2 variations to human or natural cause is critical to deducing and tracking emissions from observations. We have used in situ CO2, CO, and planetary boundary layer height (PBLH) measurements recorded during the CalNex-LA (CARB et al., 2008) ground campaign of 15 May-15 June 2010, in Pasadena, CA, to deduce the diurnally varying anthropogenic component of observed CO2 in the megacity of Los Angeles (LA). This affordable and simple technique, validated by carbon isotope observations and WRF-STILT (Weather Research and Forecasting model - Stochastic Time-Inverted Lagrangian Transport model) predictions, is shown to robustly attribute observed CO2 variation to anthropogenic or biogenic origin over the entire diurnal cycle. During CalNex-LA, local fossil fuel combustion contributed up to ~50% of the observed CO2 enhancement overnight, and ~100% of the enhancement near midday. This suggests that sufficiently accurate total column CO2 observations recorded near midday, such as those from the GOSAT or OCO-2 satellites, can potentially be used to track anthropogenic emissions from the LA megacity.

284

Cost Assessment of CO2 Sequestration by Mineral Carbonation  

E-Print Network [OSTI]

Cost Assessment of CO2 Sequestration by Mineral Carbonation Frank E. Yeboah Tuncel M. Yegulalp Harmohindar Singh Research Associate Professor Professor Center for Energy Research... them carbon dioxide (CO 2 ). This paper assesses the cost of sequestering CO 2 produced by a ZEC power plant using solid sequestration process. INTRODUCTION CO 2 is produced when electrical energy is generated using conventional fossil...

Yeboah, F. E.; Yegulalp, T. M.; Singh, H.

2006-01-01T23:59:59.000Z

285

Study of Lean Premixed Methane Combustion with CO2 Dilution under Gas Turbine Conditions  

Science Journals Connector (OSTI)

In gas turbines, high air dilution is used in order to keep the turbine inlet temperature (TIT)(7) below the metallurgical temperature limit of the first turbine stages. ... It was shown that CO2 dilution could be an efficient method for increasing CO2 concentration in exhaust gas, thus making its capture easier. ... Efforts were focused on the impacts on cycle efficiency, combustion, gas turbine components, and cost. ...

Stphanie de Persis; Gilles Cabot; Laure Pillier; Iskender Gkalp; Abdelakrim Mourad Boukhalfa

2012-12-29T23:59:59.000Z

286

Measurements of NH3 and CO2 with distributed-feedback diode lasers near 2.0 m in bioreactor vent gases  

E-Print Network [OSTI]

absorption transition at 5016.977 cm 1 was selected for trace gas monitoring. For CO2, an isolated transition of a diode-laser sensor used to record gas-phase NH3 and CO2 mole fractions, ex- plain the motivation for NH3 and 40 ppm for CO2, which is suitable for the expected vent gas concentrations. 2. Theory

287

CO2 http://andrew.ucsd.edu/co2qc/ University of California, San Diego  

E-Print Network [OSTI]

by sublimation and the CO2 is transferred into an electronic constant-volume manometer [ECM]. There its pressure of total alkalinity. Marine Chemistry 80, 185­197). Nutrients Nutrient levels were determined using

288

Novel Solvent System for CO2 Capture  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Solvent System for CO Solvent System for CO 2 Capture Background The mission of the U.S. Department of Energy/National Energy Technology Laboratory (DOE/NETL) Existing Plants, Emissions & Capture (EPEC) Research & Development (R&D) Program is to develop innovative environmental control technologies to enable full use of the nation's vast coal reserves, while at the same time allowing the current fleet of coal-fired power plants to comply with existing and emerging environmental

289

CO2 Laser CVD of Disilane  

Science Journals Connector (OSTI)

Amorphous silicon films were deposited by a CO2 laser CVD (chemical vapor deposition) method using disilane gas. With this gas, the films were deposited reasonably fast at relatively low substrate temperatures of 350C or above. Unlike monosilane, photo-induced effects in the gas phase following light absorption were negligible in deposition processes, and only the pyrolytic process taking place at the laser-heated substrate was important. Some of the physical properties of deposited films were described.

Takehiko Iwanaga; Mitsugu Hanabusa

1984-01-01T23:59:59.000Z

290

Continuous CO2 extractor and methods  

SciTech Connect (OSTI)

The purpose of this CRADA was to assist in technology transfer from Russia to the US and assist in development of the technology improvements and applications for use in the U.S. and worldwide. Over the period of this work, ORNL has facilitated design, development and demonstration of a low-pressure liquid extractor and development of initial design for high-pressure supercritical CO2 fluid extractor.

None listed

2010-06-15T23:59:59.000Z

291

IMPLEMENTING A NOVEL CYCLIC CO2 FLOOD IN PALEOZOIC REEFS  

SciTech Connect (OSTI)

Recycled CO2 will be used in this demonstration project to produce bypassed oil from the Silurian Charlton 6 pinnacle reef (Otsego County) in the Michigan Basin. Contract negotiations by our industry partner to gain access to this CO2 that would otherwise be vented to the atmosphere are near completion. A new method of subsurface characterization, log curve amplitude slicing, is being used to map facies distributions and reservoir properties in two reefs, the Belle River Mills and Chester 18 Fields. The Belle River Mills and Chester18 fields are being used as typefields because they have excellent log-curve and core data coverage. Amplitude slicing of the normalized gamma ray curves is showing trends that may indicate significant heterogeneity and compartmentalization in these reservoirs. Digital and hard copy data continues to be compiled for the Niagaran reefs in the Michigan Basin. Technology transfer took place through technical presentations regarding the log curve amplitude slicing technique and a booth at the Midwest PTTC meeting.

James R. Wood; W. Quinlan; A. Wylie

2003-07-01T23:59:59.000Z

292

Study of CO2 Mobility Control Using Cross-linked Gel Conformance Control and CO2 Viscosifiers in Heterogeneous Media  

E-Print Network [OSTI]

result, early gas breakthrough has been a very common problem in CO2-related projects, reducing the overall sweep efficiency of CO2 flooding. This research aims at improving the CO2 flood efficiency using cross-linked gel conformance control and CO2...

Cai, Shuzong

2011-10-21T23:59:59.000Z

293

Uncertainty analyses of CO2 plume expansion subsequent to wellbore CO2 leakage into aquifers  

SciTech Connect (OSTI)

In this study, we apply an uncertainty quantification (UQ) framework to CO2 sequestration problems. In one scenario, we look at the risk of wellbore leakage of CO2 into a shallow unconfined aquifer in an urban area; in another scenario, we study the effects of reservoir heterogeneity on CO2 migration. We combine various sampling approaches (quasi-Monte Carlo, probabilistic collocation, and adaptive sampling) in order to reduce the number of forward calculations while trying to fully explore the input parameter space and quantify the input uncertainty. The CO2 migration is simulated using the PNNL-developed simulator STOMP-CO2e (the water-salt-CO2 module). For computationally demanding simulations with 3D heterogeneity fields, we combined the framework with a scalable version module, eSTOMP, as the forward modeling simulator. We built response curves and response surfaces of model outputs with respect to input parameters, to look at the individual and combined effects, and identify and rank the significance of the input parameters.

Hou, Zhangshuan; Bacon, Diana H.; Engel, David W.; Lin, Guang; Fang, Yilin; Ren, Huiying; Fang, Zhufeng

2014-08-01T23:59:59.000Z

294

Gulf of Mexico Miocene CO2 Site Characterization Mega Transect  

SciTech Connect (OSTI)

This project characterized the Miocene-age sub-seafloor stratigraphy in the near-offshore portion of the Gulf of Mexico adjacent to the Texas coast. The large number of industrial sources of carbon dioxide (CO2) in coastal counties and the high density of onshore urbanization and environmentally sensitive areas make this offshore region extremely attractive for long-term storage of carbon dioxide emissions from industrial sources (CCS). The study leverages dense existing geologic data from decades of hydrocarbon exploration in and around the study area to characterize the regional geology for suitability and storage capacity. Primary products of the study include: regional static storage capacity estimates, sequestration leads and prospects with associated dynamic capacity estimates, experimental studies of CO2-brine-rock interaction, best practices for site characterization, a large-format Atlas of sequestration for the study area, and characterization of potential fluid migration pathways for reducing storage risks utilizing novel high-resolution 3D (HR3D) seismic surveys. In addition, three subcontracted studies address source-to-sink matching optimization, offshore well bore management and environmental aspects. The various geologic data and interpretations are integrated and summarized in a series of cross-sections and maps, which represent a primary resource for any near-term commercial deployment of CCS in the area. The regional study characterized and mapped important geologic features (e.g., Clemente-Tomas fault zone, the regionally extensive Marginulina A and Amphistegina B confining systems, etc.) that provided an important context for regional static capacity estimates and specific sequestration prospects of the study. A static capacity estimate of the majority of the Study area (14,467 mi2) was estimated at 86 metric Gigatonnes. While local capacity estimates are likely to be lower due to reservoir-scale characteristics, the offshore Miocene interval is a storage resource of National interest for providing CO2 storage as an atmospheric emissions abatement strategy. The natural petroleum system was used as an analog to infer seal quality and predict possible migration pathways of fluids in an engineered system of anthropogenic CO2 injection and storage. The regional structural features (e.g., Clemente-Tomas fault zone) that exert primary control on the trapping and distribution of Miocene hydrocarbons are expected to perform similarly for CCS. Industrial?scale CCS will require storage capacity utilizing well?documented Miocene hydrocarbon (dominantly depleted gas) fields and their larger structural closures, as well as barren (unproductive, brine?filled) closures. No assessment was made of potential for CO2 utilization for enhanced oil and gas recovery. The use of 3D numerical fluid flow simulations have been used in the study to greatly assist in characterizing the potential storage capacity of a specific reservoir. Due to the complexity of geologic systems (stratigraphic heterogeneity) and inherent limitations on producing a 3D geologic model, these simulations are typically simplified scenarios that explore the influence of model property variability (sensitivity study). A specific site offshore San Luis Pass (southern Galveston Island) was undertaken successfully, indicating stacked storage potential. Downscaling regional capacity estimates to the local scale (and the inverse) has proven challenging, and remains an outstanding gap in capacity assessments. In order to characterize regional seal performance and identify potential brine and CO2 leakage pathways, results from three high-resolution 3D (HR3D) seismic datasets acquired by the study using novel HR3D (P-Cable) acquisition system showed steady and significant improvements in data quality because of improved acquisition and processing technique. Finely detailed faults and stratigraphy in the shallowest 1000 milliseconds (~800 m) of data allowed for the identification and mapping of unconformable surfaces including what is probably

Meckel, Timothy; Trevino, Ramon

2014-09-30T23:59:59.000Z

295

Simulation of Coupled Processes of Flow, Transport, and Storage of CO2 in Saline Aquifers  

SciTech Connect (OSTI)

This report is the final scientific one for the award DE- FE0000988 entitled Simulation of Coupled Processes of Flow, Transport, and Storage of CO2 in Saline Aquifers. The work has been divided into six tasks. In task, Development of a Three-Phase Non-Isothermal CO2 Flow Module, we developed a fluid property module for brine-CO2 mixtures designed to handle all possible phase combinations of aqueous phase, sub-critical liquid and gaseous CO2, supercritical CO2, and solid salt. The thermodynamic and thermophysical properties of brine-CO2 mixtures (density, viscosity, and specific enthalpy of fluid phases; partitioning of mass components among the different phases) use the same correlations as an earlier fluid property module that does not distinguish between gaseous and liquid CO2-rich phases. We verified the fluid property module using two leakage scenarios, one that involves CO2 migration up a blind fault and subsequent accumulation in a secondary parasitic reservoir at shallower depth, and another investigating leakage of CO2 from a deep storage reservoir along a vertical fault zone. In task, Development of a Rock Mechanical Module, we developed a massively parallel reservoir simulator for modeling THM processes in porous media brine aquifers. We derived, from the fundamental equations describing deformation of porous elastic media, a momentum conservation equation relating mean stress, pressure, and temperature, and incorporated it alongside the mass and energy conservation equations from the TOUGH2 formulation, the starting point for the simulator. In addition, rock properties, namely permeability and porosity, are functions of effective stress and other variables that are obtained from the literature. We verified the simulator formulation and numerical implementation using analytical solutions and example problems from the literature. For the former, we matched a one-dimensional consolidation problem and a two-dimensional simulation of the Mandel-Cryer effect. For the latter, we obtained a good match of temperature and gas saturation profiles, and surface uplift, after injection of hot fluid into a model of a caldera structure. In task, Incorporation of Geochemical Reactions of Selected Important Species, we developed a novel mathematical model of THMC processes in porous and fractured saline aquifers, simulating geo-chemical reactions associated with CO2 sequestration in saline aquifers. Two computational frameworks, sequentially coupled and fully coupled, were used to simulate the reactions and transport. We verified capabilities of the THMC model to treat complex THMC processes during CO2 sequestration by analytical solutions and we constructed reactive transport models to analyze the THMC process quantitatively. Three of these are 1D reactive transport under chemical equilibrium, a batch reaction model with equilibrium chemical reactions, and a THMC model with CO2 dissolution. In task Study of Instability in CO2 Dissolution-Diffusion-Convection Processes, We reviewed literature related to the study of density driven convective flows and on the instability of CO2 dissolution-diffusion-convection processes. We ran simulations that model the density-driven flow instability that would occur during CO2 sequestration. CO2 diffused through the top of the system and dissolved in the aqueous phase there, increasing its density. Density fingers formed along the top boundary, and coalesced into a few prominent ones, causing convective flow that forced the fluid to the system bottom. These simulations were in two and three dimensions. We ran additional simulations of convective mixing with density contrast caused by variable dissolved CO2 concentration in saline water, modeled after laboratory experiments in which supercritical CO2 was circulated in the headspace above a brine saturated packed sand in a pressure vessel. As CO2 dissolved into the upper part of the saturated sand, liquid phase density increases causing instability and setting off convective mixing. We obtained good agreement

Wu, Yu-Shu; Chen, Zizhong; Kazemi, Hossein; Yin, Xiaolong; Pruess, Karsten; Oldenburg, Curt; Winterfeld, Philip; Zhang, Ronglei

2014-09-30T23:59:59.000Z

296

CO2 Gasification Kinetics of Biomass Char Derived from High-Temperature Rapid Pyrolysis  

Science Journals Connector (OSTI)

CO2 Gasification Kinetics of Biomass Char Derived from High-Temperature Rapid Pyrolysis ... The rapid pyrolysis char produced was isothermally gasified in a thermogravimetric analyzer (TGA) under a CO2 atmosphere. ... In the study by Zhang and co-workers, where as much as 14 biomass chars were gasified, gasification rates of all of the wooden biomass chars present a similar feature as Figure 7a (PS char), but this feature has not been found from gasification rates of the herbaceous biomass char. ...

Shuai Yuan; Xue-li Chen; Jun Li; Fu-chen Wang

2011-03-30T23:59:59.000Z

297

NETL: IEP – Post-Combustion CO2 Emissions Control - Dry Regenerable  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Dry Regenerable Sorbents Dry Regenerable Sorbents Project No.: FC26-07NT43089 CLICK ON IMAGE TO ENLARGE Schematic of RTI’s Dry Carbonate Process Research Triangle Institute (RTI) International completed two projects, NT43089 and NT40923, to investigate the use of sodium carbonate (Na2CO3 or soda ash) as an inexpensive, dry, and regenerable sorbent for carbon dioxide (CO2) capture in the Dry Carbonate Process. In this process, Na2CO3 reacts with CO2 and water to form sodium bicarbonate at the temperature of the flue gas exhaust; the sorbent is then regenerated at modest temperatures (~120°C) to yield a concentrated stream of CO2 for sequestration or other use. The regenerated sorbent is recycled to the absorption step for subsequent CO2 capture. See schematic of RTI's Dry Carbonate Process.

298

Growth and Chemical Responses to CO2 Enrichment Virginia Pine (Pinus  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Growth and Chemical Responses to CO2 Enrichment Virginia Pine (Pinus Growth and Chemical Responses to CO2 Enrichment Virginia Pine (Pinus Virginiana Mill.) (1985) (NDP-009) image Data Investigators R. J. Luxmoore, R. J. Norby, E. G. O'Neill, D. G. Weller, J. M. Ells, and H. H. Rogers From June 28 to October 29 in 1982, Virginia pine seedlings were exposed to elevated CO2 levels in open-top growth chambers at one of four concentrations (75, 150, 300, and 600 ppm above ambient). Plant dry weight; height; stem diameter; and chemical contents of leaf, stem, and root tissues were measured before and after exposure. Soil variables were also characterized. These data illustrate the short-term physical and chemical response of Virginia pine seedlings to elevated levels of CO2. The data are in seven files: initial dry weights before exposure (844 kB), dry weights after

299

Critical Material and Process Issues for CO2 Separation from Coal-Powered Plants  

SciTech Connect (OSTI)

Concentrating CO2 from the dilute coal combustion or gasification gas stream to a level suitable for sequestration purposes represents a major cost factor to curtail CO2 emissions by capture and sequestration schemes. This paper provides a short review of CO2 capture incentives, current separation processes, and research progress of various new technologies. Technically, CO2 can be separated out of a gas mixture by all the methods discussed in this work, such as distillation, absorption, adsorption, gas/solid reaction, membrane, electrochemical pump, hydrate formation, etc. The challenge lies in determining which approach is the most practical or feasible, and ultimately the most cost-efficient. Important material issues and their impacts on the process viability will be discussed.

Liu, Wei; King, David L.; Liu, Jun; Johnson , Brad R.; Wang, Yong; Yang, Zhenguo

2009-04-30T23:59:59.000Z

300

A CO2 sensor based upon a continuous-wave thermoelectrically-cooled quantum cascade laser  

Science Journals Connector (OSTI)

A CO2 sensor based upon a continuous-wave thermoelectrically-cooled distributed feedback quantum cascade laser operating between 2305 and 2310cm?1 and a 54.2cm long optical cell has been developed. Two approaches for direct absorption spectroscopy have been evaluated and applied for monitoring of the CO2 concentration in gas lines and ambient laboratory air. In the first approach optical transmittance was derived from the single channel laser intensity, whilst in the second approach a ratio of signal and reference laser intensities (balanced detection) was used. The optimum residual absorption standard deviation was estimated to be 1.9נ10?4 for 100 averages of 1ms duration and 0.1cm?1 scans over the P(46) CO2 absorption line of the ?3 vibrational band at 2306.926cm?1. A CO2 detection limit (1 standard deviation) of 36ppb was estimated for 0.1s average and balanced detection.

Vasili L. Kasyutich; Philip A. Martin

2011-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


301

PLAINS CO2 REDUCTION (PCOR) PARTNERSHIP  

SciTech Connect (OSTI)

During the period of October 1, 2003, through September 30, 2005, the Plains CO2 Reduction (PCOR) Partnership, identified geologic and terrestrial candidates for near-term practical and environmentally sound carbon dioxide (CO2) sequestration demonstrations in the heartland of North America. The PCOR Partnership region covered nine states and three Canadian provinces. The validation test candidates were further vetted to ensure that they represented projects with (1) commercial potential and (2) a mix that would support future projects both dependent and independent of CO2 monetization. This report uses the findings contained in the PCOR Partnership's two dozen topical reports and half-dozen fact sheets as well as the capabilities of its geographic information system-based Decision Support System to provide a concise picture of the sequestration potential for both terrestrial and geologic sequestration in the PCOR Partnership region based on assessments of sources, sinks, regulations, deployment issues, transportation, and capture and separation. The report also includes concise action plans for deployment and public education and outreach as well as a brief overview of the structure, development, and capabilities of the PCOR Partnership. The PCOR Partnership is one of seven regional partnerships under Phase I of the U.S. Department of Energy National Energy Technology Laboratory's Regional Carbon Sequestration Partnership program. The PCOR Partnership, comprising 49 public and private sector members, is led by the Energy & Environmental Research Center at the University of North Dakota. The international PCOR Partnership region includes the Canadian provinces of Alberta, Saskatchewan, and Manitoba and the states of Montana (part), Wyoming (part), North Dakota, South Dakota, Nebraska, Missouri, Iowa, Minnesota, and Wisconsin.

Edward N. Steadman; Daniel J. Daly; Lynette L. de Silva; John A. Harju; Melanie D. Jensen; Erin M. O'Leary; Wesley D. Peck; Steven A. Smith; James A. Sorensen

2006-01-01T23:59:59.000Z

302

Ambient-atmosphere glow discharge for determination of elemental concentration in solutions in a high-throughput or transient fashion  

DOE Patents [OSTI]

An ambient atmosphere glow discharge spectrometer is disclosed having a capillary, two electrodes and a means for recording the atomic emissions.

Webb, Michael R. (Somerville, MA); Hieftje, Gary M. (Bloomington, IN); Andrade, Francisco (Leeds, GB)

2011-04-19T23:59:59.000Z

303

Natural CO2 Reservoirs on the Colorado Plateau … Candidates for CO2 Sequestration  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

CO CO 2 Reservoirs on the Colorado Plateau and Southern Rocky Mountains: Candidates for CO 2 Sequestration. R. Allis (nrugs.rallis@state.ut.us; 801-537-3301) T. Chidsey (nrugs.tchidsey@state.ut.us; 801-537-3364) W. Gwynn (nrugs.wgwynn@state.ut.us; 801-537-3366) C. Morgan (nrugs.cmorgan@state.ut.us; 801-537-3370) Utah Geological Survey P.O. Box 146100 Salt Lake City, UT 84114 S. White (s.white@irl.cri.nz; 64-4-569-0000) Industrial Research Ltd. P.O. Box 31-310 Lower Hutt, New Zealand M. Adams (madams@egi.utah.edu; 801-585-7784) J. Moore (jmoore@egi.utah.edu; 801-585-6931) Energy and Geoscience Institute, 427 Wakara Way, Suite 300 Salt Lake City, UT84107 Abstract Numerous natural accumulations of CO 2 -dominant gases have been discovered as a result of

304

NETL: IEP – Post-Combustion CO2 Emissions Control - CO2 Capture from Flue  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

from Flue Gas by Phase Transitional Absorption from Flue Gas by Phase Transitional Absorption Project No.: FG26-05NT42488 Basic Illustration of the Phase Transitional Absorption Process. Basic Illustration of the Phase Transitional Absorption Process. Hampton University researched a novel carbon dioxide (CO2) absorption concept, phase transitional absorption, that utilizes a two-part proprietary absorbent consisting of an activated agent dissolved in a solvent. Phase separation of the activated agent from the chemical solvent occurs during CO2 absorption and physical separation of the two phases exiting the absorber reduces the volume of process liquid requiring thermal regeneration. This unique aspect of phase transitional absorption also decreases the amount of energy (i.e., steam) required to liberate the CO2. If the proper liquid

305

Hybrid Solvent-Membrane CO2 Capture: A Solvent/Membrane Hybrid Post-combustion CO2 Capture Process for Existing Coal-Fired Power Plants  

SciTech Connect (OSTI)

IMPACCT Project: The University of Kentucky is developing a hybrid approach to capturing CO2 from the exhaust gas of coal-fired power plants. In the first, CO2 is removed as flue gas is passed through an aqueous ammonium-based solvent. In the second, carbon-rich solution from the CO2 absorber is passed through a membrane that is designed to selectively transport the bound carbon, enhancing its concentration on the permeate side. The teams approach would combine the best of both membrane- and solventbased carbon capture technologies. Under the ARPA-E award, the team is enabling the membrane operation to be a drop-in solution.

None

2010-07-01T23:59:59.000Z

306

A multiresolution spatial parametrization for the estimation of fossil-fuel carbon dioxide emissions via atmospheric inversions.  

SciTech Connect (OSTI)

The estimation of fossil-fuel CO2 emissions (ffCO2) from limited ground-based and satellite measurements of CO2 concentrations will form a key component of the monitoring of treaties aimed at the abatement of greenhouse gas emissions. To that end, we construct a multiresolution spatial parametrization for fossil-fuel CO2 emissions (ffCO2), to be used in atmospheric inversions. Such a parametrization does not currently exist. The parametrization uses wavelets to accurately capture the multiscale, nonstationary nature of ffCO2 emissions and employs proxies of human habitation, e.g., images of lights at night and maps of built-up areas to reduce the dimensionality of the multiresolution parametrization. The parametrization is used in a synthetic data inversion to test its suitability for use in atmospheric inverse problem. This linear inverse problem is predicated on observations of ffCO2 concentrations collected at measurement towers. We adapt a convex optimization technique, commonly used in the reconstruction of compressively sensed images, to perform sparse reconstruction of the time-variant ffCO2 emission field. We also borrow concepts from compressive sensing to impose boundary conditions i.e., to limit ffCO2 emissions within an irregularly shaped region (the United States, in our case). We find that the optimization algorithm performs a data-driven sparsification of the spatial parametrization and retains only of those wavelets whose weights could be estimated from the observations. Further, our method for the imposition of boundary conditions leads to a 10computational saving over conventional means of doing so. We conclude with a discussion of the accuracy of the estimated emissions and the suitability of the spatial parametrization for use in inverse problems with a significant degree of regularization.

Ray, Jaideep; Lee, Jina; Lefantzi, Sophia; Yadav, Vineet [Carnegie Institution for Science, Stanford, CA; Michalak, Anna M. [Carnegie Institution for Science, Stanford, CA; van Bloemen Waanders, Bart Gustaaf [Sandia National Laboratories, Albuquerque, NM; McKenna, Sean Andrew [IBM Research, Mulhuddart, Dublin 15, Ireland

2013-04-01T23:59:59.000Z

307

Plains CO2 Reduction Partnership PCOR | Open Energy Information  

Open Energy Info (EERE)

CO2 Reduction Partnership PCOR CO2 Reduction Partnership PCOR Jump to: navigation, search Name Plains CO2 Reduction Partnership (PCOR) Place Grand Forks, North Dakota Zip 58202-9018 Product North Dakota-based consortium researching CO2 storage options. PCOR is busy with the ECBM in the Unminable Lignite Research Project. References Plains CO2 Reduction Partnership (PCOR)[1] LinkedIn Connections CrunchBase Profile No CrunchBase profile. Create one now! This article is a stub. You can help OpenEI by expanding it. Plains CO2 Reduction Partnership (PCOR) is a company located in Grand Forks, North Dakota . References ↑ "Plains CO2 Reduction Partnership (PCOR)" Retrieved from "http://en.openei.org/w/index.php?title=Plains_CO2_Reduction_Partnership_PCOR&oldid=349772"

308

NETL: 2013 Conference Proceedings - 2013 NETL CO2 Capture Technology  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

2013 NETL CO2 Capture Technology Meeting 2013 NETL CO2 Capture Technology Meeting July 8-11, 2013 Previous Proceedings 2012: NETL CO2 Capture Technology Meeting 2011: NETL CO2 Capture Technology Meeting 2010: NETL CO2 Capture Technology Meeting 2009: Annual NETL CO2 Capture Technology for Existing Plants R&D Meeting Proceedings of the 2013 NETL CO2 Capture Technology Meeting Table of Contents Presentations Monday, July 8 Opening/Overview Post-Combustion Sorbent-Based Capture Tuesday, July 9 Post-Combustion Solvent-Based Capture CO2 Compression Wednesday, July 10 Post-Combustion Membrane-Based Capture Pre-Combustion Capture Projects Thursday, July 11 ARPA-E Capture Projects System Studies and Modeling Oxy-Combustion and Chemical Looping Posters PRESENTATIONS Monday, July 8, 2013 Opening/Overview Introduction [PDF-MB]

309

CO2 Capture by Absorption with Potassium Carbonate  

E-Print Network [OSTI]

CO2 Capture by Absorption with Potassium Carbonate Fourth Quarterly Report 2005 Quarterly Progress. #12;3 Abstract The objective of this work is to improve the process for CO2 capture by alkanolamine

Rochelle, Gary T.

310

CO2 Capture by Absorption with Potassium Carbonate  

E-Print Network [OSTI]

CO2 Capture by Absorption with Potassium Carbonate Third Quarterly Report 2005 Quarterly Progress. #12;3 Abstract The objective of this work is to improve the process for CO2 capture by alkanolamine

Rochelle, Gary T.

311

CO2 Capture by Absorption with Potassium Carbonate  

E-Print Network [OSTI]

CO2 Capture by Absorption with Potassium Carbonate First Quarterly Report 2006 Quarterly Progress the process for CO2 capture by alkanolamine absorption/stripping by developing an alternative solvent, aqueous

Rochelle, Gary T.

312

CO2-laser gas discharges in narrow gaps  

Science Journals Connector (OSTI)

We have studied RF discharges as excitation mechanisms for distributed feedback (DFB) CO2 lasers. For CO2 laser plasmas the reduced electric fieldE/N has to be in a well-defined range. The reduced electric fields

W. Leuthard; F. K. Kneubhl; H. J. Schtzau

1989-01-01T23:59:59.000Z

313

Summary Report on CO2 Geologic Sequestration & Water Resources Workshop  

E-Print Network [OSTI]

2 exposure in both CO 2 -EOR and natural CO 2 reservoirs (as enhanced oil recovery (EOR) and enhanced gas recovery (2 field injections for CCS-EOR, where the water quality of

Varadharajan, C.

2013-01-01T23:59:59.000Z

314

Integrated Assessment of Energy-Options for CO2 Reduction  

Science Journals Connector (OSTI)

Energy technology options for CO2 reduction are evaluated in a process-oriented dynamic national costs minimizing LP-model of the Dutch energy system. To identify cost-effective CO2 reduction strategies two scena...

T. Kram; P. A. Okken

1989-01-01T23:59:59.000Z

315

Chemical Impact of Elevated CO2on Geothermal Energy Production...  

Broader source: Energy.gov (indexed) [DOE]

Chemical Impact of Elevated CO2on Geothermal Energy Production Chemical Impact of Elevated CO2on Geothermal Energy Production This is a two phase project to assess the geochemical...

316

Enhanced Geothermal Systems (EGS) with CO2as Heat Transmission...  

Broader source: Energy.gov (indexed) [DOE]

study heat extraction from hot porous systems by injection of cold CO 2 . * Reactive chemistry experiments for CO 2 -brine-rock are being assembled (INL). 6 | US DOE Geothermal...

317

natural gas+ condensing flue gas heat recovery+ water creation+ CO2  

Open Energy Info (EERE)

natural gas+ condensing flue gas heat recovery+ water creation+ CO2 natural gas+ condensing flue gas heat recovery+ water creation+ CO2 reduction+ cool exhaust gases+ Energy efficiency+ commercial building energy efficiency+ industrial energy efficiency+ power plant energy efficiency+ Home Increase Natural Gas Energy Efficiency Description: Increased natural gas energy efficiency = Reduced utility bills = Profit In 2011 the EIA reports that commercial buildings, industry and the power plants consumed approx. 17.5 Trillion cu.ft. of natural gas. How much of that energy was wasted, blown up chimneys across the country as HOT exhaust into the atmosphere? 40% ~ 60% ? At what temperature? Links: The technology of Condensing Flue Gas Heat Recovery natural gas+ condensing flue gas heat recovery+ water creation+ CO2 reduction+ cool exhaust gases+ Energy efficiency+ commercial building

318

Scientific Considerations Related to Regulation Development for CO2 Sequestration in Brine Formations  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

SCIENTIFIC CONSIDERATIONS RELATED TO REGULATION SCIENTIFIC CONSIDERATIONS RELATED TO REGULATION DEVELOPMENT FOR CO 2 SEQUESTRATION IN BRINE FORMATIONS Chin-Fu Tsang (cftsang@lbl.gov; (510) 486-5782) Sally M. Benson (smbenson@lbl.gov; (510) 486-7071) Earth Sciences Division, Ernest Orlando Lawrence Berkeley National Laboratory One Cyclotron Road, MS 90-1116, Berkeley, CA 94720 Bruce Kobelski (kobelski.bruce@epa.gov) Robert Smith (smith.robert-eu@epamail.epa.gov) U.S. Environmental Protection Agency Office of Drinking Water and Ground Water, Washington D.C. Introduction Reduction of atmospheric emissions of CO 2 (DOE, 1999a) through injection of CO 2 into in deep brine formations is being actively studied both in the U.S. and internationally. If this technology is to be employed broadly enough to make a significant impact on global

319

CO2 Capture Membrane Process for Power Plant Flue Gas  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

CO CO 2 Capture Membrane Process for Power Plant Flue Gas Background The U.S. Department of Energy's (DOE) Existing Plants, Emissions & Capture (EPEC) Program is performing research to develop advanced technologies focusing on carbon dioxide (CO 2 ) emissions control for existing pulverized coal-fired plants. This new focus on post-combustion and oxy-combustion CO 2 emissions control technology, CO 2 compression, and beneficial reuse is in response to the priority for advanced

320

CHARACTERIZATION OF MIXED CO2-TBPB HYDRATE FOR REFRIGERATION APPLICATIONS  

E-Print Network [OSTI]

in a dynamic loop and an Ostwald-de Waele model was obtained. Keywords: CO2, TBPB, mixed hydrates, solubility

Paris-Sud XI, Université de

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


321

A field study combined with modeling investigation demonstrates that the organization of transport by mountain terrain strongly affects the regional CO2  

E-Print Network [OSTI]

,b), and Moore et al. (2008) showed that 1) an aggrading Rocky Mountain subalpine forest is a net annual CO2 sink- A MULTISCALE AND MULTIDISCIPLINARY INVESTIGATION OF ECOSYSTEM­ATMOSPHERE CO2 EXCHANGE OVER THE ROCKY MOUNTAINS/sinks associated with plant distributions over heterogeneous surfaces, regardless of whether the surface is flat

322

A thermochemical study of ceria: exploiting an old material for new modes of energy conversion and CO2 mitigation  

Science Journals Connector (OSTI)

...partial molar free energy of lattice oxygen...solar-to-fuel conversion efficiency, which...the mobilities on carrier concentrations...J. Hydrogen Energy 31 5561( doi...for new modes of energy conversion and CO2 mitigation...

2010-01-01T23:59:59.000Z

323

CO2 Capture by Absorption with Potassium Carbonate  

E-Print Network [OSTI]

CO2 Capture by Absorption with Potassium Carbonate Second Quarterly Report 2006 Quarterly Progress of this work is to improve the process for CO2 capture by alkanolamine absorption/stripping by developing for simultaneous removal of CO2 and SO2. Corrosion of carbon steel in uninhibited MEA solution is increased

Rochelle, Gary T.

324

Central serotonin neurons are required for arousal to CO2  

E-Print Network [OSTI]

Central serotonin neurons are required for arousal to CO2 Gordon F. Buchanana,b,1 and George B neurons are stimulated by CO2, and sero- tonin activates thalamocortical networks, we hypothesized any arousal response to inhalation of 10% CO2 (with 21% O2 in balance N2) but had normal arousal

325

On the scatteringgreenhouse effect of CO 2 ice clouds  

E-Print Network [OSTI]

that young Mars was warm enough to support flowing water present a continuing enigma (Squyres and Kasting 1994). Kasting (1991) showed that, owing to the effects of CO 2 condensation on temperature lapse rate the optical effects of CO 2 ­ice clouds, but remarked that because CO 2 ­ice (unlike water­ice) has very low

Pierrehumbert, Raymond

326

In situ carbonation of peridotite for CO2 storage  

Science Journals Connector (OSTI)

...reaction in 1 region can be pumped into an adjacent area to...dissolved CO 2 in convecting seawateronly ?10 4 tons of CO 2 per km 3...convection, near-surface seawater would descend one hole...dissolved CO 2 from evolving seawater along the flow path...

Peter B. Kelemen; Jrg Matter

2008-01-01T23:59:59.000Z

327

Aqueous Carbonation of Natural Brucite: Relevance to CO2 Sequestration  

Science Journals Connector (OSTI)

Aqueous Carbonation of Natural Brucite: Relevance to CO2 Sequestration ... Products and reaction kinetics of natural brucite carbonation are studied at room temperature and moderate pCO2. ... Carbonation of natural brucite in H2O and diluted HCl is investigated at room temperature and moderate pCO2 to explore the products mineralogy and reaction kinetics. ...

Liang Zhao; Liqin Sang; Jun Chen; Junfeng Ji; H. Henry Teng

2009-11-30T23:59:59.000Z

328

CO2 Hydrate Composite for Ocean Carbon Sequestration  

Science Journals Connector (OSTI)

CO2 Hydrate Composite for Ocean Carbon Sequestration ... Further studies are needed to address hydrate conversion efficiency, scale-up criteria, sequestration longevity, and impact on the ocean biota before in-situ production of sinking CO2 hydrate composite can be applied to oceanic CO2 storage and sequestration. ...

Sangyong Lee; Liyuan Liang; David Riestenberg; Olivia R. West; Costas Tsouris; Eric Adams

2003-07-18T23:59:59.000Z

329

B.2 Subproject Brokate Simulating CO2 Sequestration  

E-Print Network [OSTI]

79 B.2 Subproject Brokate Simulating CO2 Sequestration Hysteretic Aspects of CO2 Sequestration and implement models describing the hysteresis in the context of the CO2 sequestration process. The hysteresis's law but in contrast to most Darcy's law based models it assumes the phases to be weakly compressible

Turova, Varvara

330

Mesoporous Organosilica with Amidoxime Groups for CO2 Sorption  

Science Journals Connector (OSTI)

Mesoporous Organosilica with Amidoxime Groups for CO2 Sorption ... This work reports a successful use of the aforementioned strategy for the development of ordered mesoporous organosilica (OMO) with amidoxime groups for CO2 sorption. ... The resulting series of amidoxime-containing OMO was prepared and used for CO2 sorption at low (25 C) and elevated (60, 120 C) temperatures. ...

Chamila Gunathilake; Mietek Jaroniec

2014-07-03T23:59:59.000Z

331

Enhanced CO2 Storage and Sequestration in Deep Saline Aquifers by Nanoparticles: Commingled Disposal of Depleted Uranium and CO2  

Science Journals Connector (OSTI)

Geological storage of anthropogenic CO2 emissions in deep saline aquifers has recently received tremendous attention in the scientific literature. Injected buoyant CO2 accumulates at the top part of the aquifer u...

Farzam Javadpour; Jean-Philippe Nicot

2011-09-01T23:59:59.000Z

332

CO2 Flux Estimated from Air-Sea Difference in CO2 Partial Pressure  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

CO2 Flux Estimated from Air-Sea Difference in CO2 Partial Pressure (Revised October 2009) CO2 Flux Estimated from Air-Sea Difference in CO2 Partial Pressure (Revised October 2009) The files in this site contain a revised (October 2009) version of the climatological mean values in 4° Latitude X 5° Longitude box areas and the distribution maps. These were originally published in: Takahashi, et al. (2009), DSR II, 56, 554-577. The data file containing annual flux data for each 4° X 5° box is located here. The data file from which this map was created, including all 12 months of data is here. This data file, in ASCII form, also contains the flux data and the intermediate values used to calculate that flux for each month. In December 2010 our colleague, R. Wanninkhof pointed out a problem with the flux data for the month of December. The file of ice coverage for December was corrupted and showed zero ice for the entire month, worldwide. This has been corrected with the estimated percent of ice and the flux recalculated. Version "c" of the data files contain this correction.

333

Interactions between reducing CO2 emissions, CO2 removal and solar radiation management  

Science Journals Connector (OSTI)

...the geological storage capacity for CO2. For the SRM...reduction in incoming solar radiation that fully...3. Results (a) Solar radiation management...scale set by the heat capacity in the model. For s2030srm2015...reduction in incoming solar radiation in the first...

2012-01-01T23:59:59.000Z

334

CO2 Mineral Sequestration Studies in US  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Mineral Sequestration Studies in US Mineral Sequestration Studies in US Philip Goldberg 1 , Zhong-Ying Chen 2 , William O'Connor 3 , Richard Walters 3 , and Hans Ziock 4 1 National Energy Technology Laboratory, P.O. Box 10940, Pittsburgh, PA 15236, goldberg@netl.doe.gov, (412)386-5806 2 Science Applications International Corporation, 1710 Goodridge Dr. McLean, VA, zhong- ying.chen@saic.com, (703)676-7328 3 Albany Research Center, Albany, OR oconner@arc.doe.gov, walters@alrc.doe, (541)967-5834 4 Los Alamos National Laboratory, Los Alamos, NM, ksl@lanl.gov, ziock@lanl.gov, (505)667- 7265 Abstract Carbon sequestration by reacting naturally occurring Mg and Ca containing minerals with CO 2 to form carbonates has many unique advantages. Most notably is the fact that carbonates have a lower energy state than CO

335

Experimental Investigation into a Pilot-Scale Entrained-Flow Gasification of Pulverized Coal Using CO2 As Carrier Gas  

Science Journals Connector (OSTI)

Regarding syngas composition in dry basis, there was a desired drop in inert gas (N2) concentration from about 6% to less than 2%, while the CO2 concentration increased by about 4%age points in optimal operation conditions when CO2 carrier substituted for N2. ... This technology has been validated and proven in many commercially operating units including 32 GE,(1) 15 Shell,(2) and 17 OMB (opposed multi burner) licenses. ...

Xiaolei Guo; Wenxue Lu; Zhenghua Dai; Haifeng Liu; Xin Gong; Lei Li; Honglin Zhang; Baogui Guo

2011-12-27T23:59:59.000Z

336

CINETIQUES DE SORPTION DU CO2 DANS LE CADRE DU STOCKAGE GEOLOGIQUE DU CO2 DANS LE CHARBON  

E-Print Network [OSTI]

CINETIQUES DE SORPTION DU CO2 DANS LE CADRE DU STOCKAGE GEOLOGIQUE DU CO2 DANS LE CHARBON KINETIC PROCESSES OF CO2 SORPTION FOR CO2 STORAGE IN COAL SEAMS Delphine CHARRIERE1, 2 , Zbigniew POKRYSZKA1 récupération assistée du méthane requiert des informations sur les mécanismes de sorption de gaz. Dans ce

Boyer, Edmond

337

Aminosilane-Grafted Polymer/Silica Hollow Fiber Adsorbents for CO2 Capture from Flue Gas  

Science Journals Connector (OSTI)

In this approach, polymeric hollow fibers similar to those already prepared on commercial scales for membrane gas separations are prepared and loaded with large volumes of solid CO2 adsorbing materials. ... In this regard, the hollow fiber RTSA process is ideally suited for application of typical silica amine adsorbents, as it (i) allows for effective heat integration,(11) (ii) gives fast cycle times (expected to be on the order of 24 min),(8) and (iii) minimizes contact of aminosilica-adsorbents with high-temperature steam, which can degrade the adsorbent. ... The moles of CO2 adsorbed were calculated by integration of the area bounded by the CO2 breakthrough front and the He breakthrough front from the initial concentration to the final equilibration concentration. ...

Fateme Rezaei; Ryan P. Lively; Ying Labreche; Grace Chen; Yanfang Fan; William J. Koros; Christopher W. Jones

2013-03-29T23:59:59.000Z

338

Selection of coals of different maturities for CO2 Storage by modelling of CH4 and CO2 adsorption isotherms  

E-Print Network [OSTI]

of this study is to compare and model pure gas sorption isotherms (CO2 and CH4) for well-characterised coals of different maturities to determine the most suitable coal for CO2 storage. Carbon dioxide and methane; Coals; Methane and carbon dioxide adsorption; Modelling isotherms 1. Introduction CO2 is a greenhouse

Paris-Sud XI, Université de

339

TOUGH+CO2: A multiphase fluid-flow simulator for CO2 geologic sequestration in saline aquifers  

Science Journals Connector (OSTI)

TOUGH+CO"2 is a new simulator for modeling of CO"2 geologic sequestration in saline aquifers. It is a member of TOUGH+, the successor to the TOUGH2 family of codes for multicomponent, multiphase fluid and heat flow simulation. The code accounts for heat ... Keywords: CO2 geologic sequestration, Modeling, Multiphase flow, Parallel computing, Saline aquifer, TOUGH+, TOUGH2

Keni Zhang; George Moridis; Karsten Pruess

2011-06-01T23:59:59.000Z

340

Nanoclay-Based Solid Sorbents for CO2 Capture  

Science Journals Connector (OSTI)

Nanoclay-Based Solid Sorbents for CO2 Capture ... As seen from the figure, the untreated nanoclay shows very little CO2 capture, while amine-treated nanoclays show considerably higher CO2 capture capacities, demonstrating the effectiveness of the amine treatment. ... The CO2 sorption capacity increases as the temperature is increased from 50 to 85 C, and it reaches as high as 7.5% at 85 C for the nanoclay treated with both APTMS and PEI, although the nanoclays treated with either APTMS or PEI show about 6% CO2 capture capacity. ...

Elliot A. Roth; Sushant Agarwal; Rakesh K. Gupta

2013-03-19T23:59:59.000Z

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


341

Net primary production of terrestrial ecosystems in China and its equilibrium response to changes in climate and atmospheric CO? concentration  

E-Print Network [OSTI]

The Terrestrial Ecosystem Model (TEM, version 4.0) was used to estimate net primary production (NPP) in China for contemporary climate and NPP responses to elevated CO? and climate changes projected by three atmospheric ...

Xiao, Xiangming.; Melillo, Jerry M.; Kicklighter, David W.; Pan, Yude.; McGuire, A. David.; Helfrich III, J.V.K.

342

Impact of Closing Canadas Largest Point-Source of Mercury Emissions on Local Atmospheric Mercury Concentrations  

Science Journals Connector (OSTI)

(29) Solar radiation measurements at the airport were initiated in August 2010. ... Steffen, A.; Schroeder, W. Standard Operating Procedures for Total Gaseous Mercury MeasurementsCanadian Atmospheric Mercury Measurement Network (CAMNet); Environment Canada: Toronto, Canada, 1999. ...

Chris S. Eckley; Matthew T. Parsons; Rachel Mintz; Monique Lapalme; Maxwell Mazur; Robert Tordon; Robert Elleman; Jennifer A. Graydon; Pierrette Blanchard; Vincent St Louis

2013-08-26T23:59:59.000Z

343

Dual-phase membrane for High temperature CO2 separation  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Jerry Y.S. Lin Jerry Y.S. Lin Chemical Engineering Arizona State University Tempe, AZ 85287 Jerry.lin@asu.edu Pre-Combustion Carbon Dioxide Capture by a New Dual-Phase Ceramic-Carbonate Membrane Reactor 2 Background 3 CO 2 Capture Methods and Efficiency Improvement Coal, Natural gas, Biomass CO 2 separation Power plant CO 2 compression, conditioning for sequestration Gasification Reforming Shift CO 2 Separation Power plant Power plant Air separation N 2 /O 2 CO 2 Post- combustion H 2 /CO H 2 /CO H 2 CO 2 H 2 O/N 2 /O 2 CO 2 H 2 Pre- combustion Air N 2 O 2 or O 2 /CO 2 CO 2 Oxyfuel Combustion Air separation Air Air separation Air Air separation Air Air Air Air Air separation Air Air separation Air N 2 Air separation Air O 2 or O 2 /CO 2 N 2 Air separation Air N 2 Air O 2 or O 2 /CO 2 N 2 Air Air separation N 2 Air 4 Water-Gas-Shift Reaction and Membrane Reactor Reforming

344

NETL - World CO2 Emissions - Projected Trends Tool | Open Energy  

Open Energy Info (EERE)

NETL - World CO2 Emissions - Projected Trends Tool NETL - World CO2 Emissions - Projected Trends Tool Jump to: navigation, search Tool Summary LAUNCH TOOL Name: NETL - World CO2 Emissions - Projected Trends Tool Agency/Company /Organization: National Energy Technology Laboratory Sector: Energy Topics: GHG inventory Resource Type: Software/modeling tools Website: www.netl.doe.gov/energy-analyses/refshelf/results.asp?ptype=Models/Too References: NETL - World CO2 Emissions - Projected Trends Tool [1] NETL - World CO2 Emissions - Projected Trends Tool This interactive tool enables the user to look at both total and power sector CO2 emissions from the use of coal, oil, or natural gas, over the period 1990 to 2030. One can use the tool to compare five of the larger CO2 emitters to each other or to overall world emissions. The data are from the

345

Site Characterization of Promising Geologic Formations for CO2 Storage |  

Broader source: Energy.gov (indexed) [DOE]

Site Characterization of Promising Geologic Formations for CO2 Site Characterization of Promising Geologic Formations for CO2 Storage Site Characterization of Promising Geologic Formations for CO2 Storage In September 2009, the U.S. Department of Energy announced the award of 11 projects with a total project value of $75.5 million* to conduct site characterization of promising geologic formations for CO2 storage. These Recovery Act projects will increase our understanding of the potential for these formations to safely and permanently store CO2. The information gained from these projects (detailed below) will further DOE's efforts to develop a national assessment of CO2 storage capacity in deep geologic formations. Site Characterization of Promising Geologic Formations for CO2 Storage * Subsequently, the Board of Public Works project in Holland, MI has been

346

Alternations of Structure and Functional Activity of Below Ground Microbial Communities at Elevated Atmospheric Carbon Dioxide  

SciTech Connect (OSTI)

The global atmospheric concentration of CO2 has increased by more than 30percent since the industrial revolution. Although the stimulating effects of elevated CO2 (eCO2) on plant growth and primary productivity have been well studied, its influences on belowground microbial communities are poorly understood and controversial. In this study, we showed a significant change in the structure and functional potential of soil microbial communities at eCO2 in a grassland ecosystem, the BioCON (Biodiversity, CO2 and Nitrogen) experimental site (http://www.biocon.umn.edu/) using a comprehensive functional gene array, GeoChip 3.0, which contains about 28,0000 probes and covers approximately 57,000 gene variants from 292 functional gene families involved in carbon, nitrogen, phosphorus and sulfur cycles as well as other functional processes. GeoChip data indicated that the functional structure of microbial communities was markedly different between ambient CO2 (aCO2) and eCO2 by detrended correspondence analysis (DCA) of all 5001 detected functional gene probes although no significant differences were detected in the overall microbial diversity. A further analysis of 1503 detected functional genes involved in C, N, P, and S cycles showed that a considerable portion (39percent) of them were only detected under either aCO2 (14percent) or eCO2 (25percent), indicating that the functional characteristics of the microbial community were significantly altered by eCO2. Also, for those shared genes (61percent) detected, some significantly (p<0.05) changed their abundance at eCO2. Especially, genes involved in labile C degradation, such as amyA, egl, and ara for starch, cellulose, and hemicelluloses, respectively, C fixation (e.g., rbcL, pcc/acc), N fixation (nifH), and phosphorus utilization (ppx) were significantly increased under eCO2, while those involved in decomposing recalcitrant C, such as glx, lip, and mnp for lignin degradation remained unchanged. This study provides insights into our understanding of belowground microbial communities and their feedbacks to terrestrial ecosystems at eCO2.

He, Zhili; Xu, Meiying; Deng, Ye; Kang, Sanghoon; Wu, Liyou; Van Nostrand, Joy D.; Hobbie, Sarah E.; Reich, Peter B.; Zhou, Jizhong

2010-05-17T23:59:59.000Z

347

Assessment of Methanol Synthesis Utilizing Exhaust CO2 for Chemical Storage of Electrical Energy  

Science Journals Connector (OSTI)

(1, 2) Sequestration is principally an available and technologically feasible way to reduce the CO2 emission into the atmosphere, although there are still obvious ecological, environmental, and safety aspects to clarify before it can be implemented in large scale. ... Furthermore, these chemicals could be used also as traffic fuel, where they are applicable easily with minor modifications with the existing infrastructure and vehicle fleet. ... The product H is considered a fuel for fuel cell vehicles and a substitute for gasoline. ...

Liisa K. Rihko-Struckmann; Andreas Peschel; Richard Hanke-Rauschenbach; Kai Sundmacher

2010-09-17T23:59:59.000Z

348

Fossil Fuels Without CO2 Emissions  

Science Journals Connector (OSTI)

...from the atmosphere (1). Recent work in carbon...capacity ?200 to 500 GtC), deep coal beds...molar ratio of ?2:1, allowing...sequestrationa tax rebate or creation...global capacity ~200 to 500 GtC), deep coal...molar ratio of ~2:1, allowing...

E. A. Parson; D. W. Keith

1998-11-06T23:59:59.000Z

349

The Climate Impact of Past Changes in Halocarbons and CO2 in the Tropical UTLS Region  

Science Journals Connector (OSTI)

A chemistryclimate model coupled to an ocean model is used to compare the climate impact of past (19602010) changes in concentrations of halocarbons with those of CO2 in the tropical upper troposphere and lower stratosphere (UTLS). The ...

Charles McLandress; Theodore G. Shepherd; M. Catherine Reader; David A. Plummer; Keith P. Shine

2014-12-01T23:59:59.000Z

350

Fuels from Water, CO2, and Solar Energy Prof. Aldo Steinfeld  

E-Print Network [OSTI]

Fuels from Water, CO2, and Solar Energy Prof. Aldo Steinfeld Department of Mechanical and Process fuels make use of concentrated solar radiation as the energy source of high-temperature process heat Engineering, ETH Zurich, Switzerland and Solar Technology Laboratory, Paul Scherrer Institute, Switzerland

Ponce, V. Miguel

351

NETL: IEP - Post-Combustion CO2 Emissions Control - CO2 Capture Membrane  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

CO2 Capture Membrane Process for Power Plant Flue Gas CO2 Capture Membrane Process for Power Plant Flue Gas Project No.: DE-NT0005313 CLICK ON IMAGE TO ENLARGE Research Triangle Institute (RTI) International is researching fluorinated polymer membranes for carbon dioxide capture. RTI's research effort includes membrane materials development, module design, and process design. RTI is pursuing the development of two hollow-fiber membrane materials. First, RTI is working with Generon to develop a membrane material constructed of polycarbonate-based polymers. Lab-scale membrane modules are being studied with simulated flue-gas mixtures with and without flue gas emission contaminants. Two larger-scale polycarbonate membrane module prototypes are being tested with a slipstream of actual flue gas from the U.S. Environmental Protection Agency's (EPA) Multipollutant

352

Supersonic Technology for CO2 Capture: A High Efficiency Inertial CO2 Extraction System  

SciTech Connect (OSTI)

IMPACCT Project: Researchers at ATK and ACENT Laboratories are developing a device that relies on aerospace wind-tunnel technologies to turn CO2 into a condensed solid for collection and capture. ATKs design incorporates a special nozzle that converges and diverges to expand flue gas, thereby cooling it off and turning the CO2 into solid particles which are removed from the system by a cyclonic separator. This technology is mechanically simple, contains no moving parts and generates no chemical waste, making it inexpensive to construct and operate, readily scalable, and easily integrated into existing facilities. The increase in the cost to coal-fired power plants associated with introduction of this system would be 50% less than current technologies.

None

2010-07-01T23:59:59.000Z

353

System-level modeling for geological storage of CO2  

SciTech Connect (OSTI)

One way to reduce the effects of anthropogenic greenhousegases on climate is to inject carbon dioxide (CO2) from industrialsources into deep geological formations such as brine formations ordepleted oil or gas reservoirs. Research has and is being conducted toimprove understanding of factors affecting particular aspects ofgeological CO2 storage, such as performance, capacity, and health, safetyand environmental (HSE) issues, as well as to lower the cost of CO2capture and related processes. However, there has been less emphasis todate on system-level analyses of geological CO2 storage that considergeological, economic, and environmental issues by linking detailedrepresentations of engineering components and associated economic models.The objective of this study is to develop a system-level model forgeological CO2 storage, including CO2 capture and separation,compression, pipeline transportation to the storage site, and CO2injection. Within our system model we are incorporating detailedreservoir simulations of CO2 injection and potential leakage withassociated HSE effects. The platform of the system-level modelingisGoldSim [GoldSim, 2006]. The application of the system model is focusedon evaluating the feasibility of carbon sequestration with enhanced gasrecovery (CSEGR) in the Rio Vista region of California. The reservoirsimulations are performed using a special module of the TOUGH2 simulator,EOS7C, for multicomponent gas mixtures of methane and CO2 or methane andnitrogen. Using this approach, the economic benefits of enhanced gasrecovery can be directly weighed against the costs, risks, and benefitsof CO2 injection.

Zhang, Yingqi; Oldenburg, Curtis M.; Finsterle, Stefan; Bodvarsson, Gudmundur S.

2006-04-24T23:59:59.000Z

354

QGESS: CO2 Impurity Design Parameters  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Q Q U U A A L L I I T T Y Y G G U U I I D D E E L L I I N N E E S S F F O O R R E E N N E E R R G G Y Y S S Y Y S S T T E E M M S S T T U U D D I I E E S S C C O O 2 2 I I m m p p u u r r i i t t y y D D e e s s i i g g n n P P a a r r a a m m e e t t e e r r s s DOE/NETL-2010/???? DOE/NETL-341/011212 August 2013 CO 2 Impurity Design Parameters Quality Guidelines for Energy System Studies Disclaimer This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights.

355

Oxygen supply for oxyfuel CO2 capture  

Science Journals Connector (OSTI)

This paper presents the results of a study to develop Air Products air separation unit (ASU) offerings for oxyfuel coal CO2 capture projects. A scalable reference plant concept is described to match particular sizes of power generation equipment, taking into account factors such as safety, reliability, operating flexibility, efficiency, and low capital cost. We describe the selection of a process cycle to exploit the low purity requirements, as well as the options for compression machinery and drivers as the scale of the plant increases and the sizes of referenced equipment limit the possibilities. We also explore integration with other elements of the system, such as preheating condensate or heating and expanding pressurised nitrogen. In addition, we consider how the ASU affects the flexibility of the oxyfuel system and discuss how its power consumption can be reduced during periods of high power demand. Finally, the advantages and disadvantages of different execution strategies for air separation unit projects are discussed, as well as alternative commercial models for the supply of oxygen.

Paul Higginbotham; Vince White; Kevin Fogash; Galip Guvelioglu

2011-01-01T23:59:59.000Z

356

Conversion of the greenhouse gas CO2 to the fuel gas CO via the Boudouard reaction: A review  

Science Journals Connector (OSTI)

Abstract The remediation of carbon dioxide emitted into the atmosphere has become the topic of the day due to the enormous contribution of CO2 to the devastating global warming. The Boudouard reaction, in which solid carbon (char) reacts with CO2 to produce carbon monoxide (CO2 (g)+C(s)?CO (g)), is a straightforward route for the CO2 emission mitigation. Through this reaction, the CO2 coming from variety of combustion plants, including exhaust/flue gas and synthesis gas, can be upgraded to the fuel gas, CO. This work presents a review on the CO2 gasification of char, from coal, biomass, municipal solid wastes, sewage sludge or any co-utilized blend of them, to produce CO through the Boudouard reaction. An outline of the most effective parameters on the char gasification rate is presented. The parameters which affect the char reactivity are reviewed as those related to the char and its structural features (surface area and porosity, active sites, mineral content, structural evolution of char during gasification, pyrolysis condition and carbon source) and operation parameters (use of catalyst, gasification temperature, gasification pressure and CO2 partial pressure, char particle size and gasification heat source). The kinetics of the char gasification reaction is studied and several theoretical or semi-empirical kinetic models used to interpret the reaction rate data and calculation of kinetic parameters, specifically activation energy, are reviewed and discussed.

Pooya Lahijani; Zainal Alimuddin Zainal; Maedeh Mohammadi; Abdul Rahman Mohamed

2015-01-01T23:59:59.000Z

357

Hybrid heat exchange for the compression capture of CO2 from recirculated flue gas  

SciTech Connect (OSTI)

An approach proposed for removal of CO2 from flue gas cools and compresses a portion of a recirculated flue-gas stream, condensing its volatile materials for capture. Recirculating the flue gas concentrates SOx, H2O and CO2 while dramatically reducing N2 and NOx, enabling this approach, which uses readily available industrial components. A hybrid system of indirect and direct-contact heat exchange performs heat and mass transfer for pollutant removal and energy recovery. Computer modeling and experimentation combine to investigate the thermodynamics, heat and mass transfer, chemistry and engineering design of this integrated pollutant removal (IPR) system.

Oryshchyn, Danylo B.; Ochs, Thomas L.; Summers, Cathy A.

2004-01-01T23:59:59.000Z

358

Plants, Weathering, and the Evolution of Atmospheric Carbon Dioxide and Oxygen  

SciTech Connect (OSTI)

Over the past six years we have published 24 papers that can be divided into three sections: (1) Study of plants and weathering, (2) modeling the evolution of atmospheric CO2 over Phanerozoic time (past 550 million years). (3) Modeling of atmospheric O2 over Phanerozoic time. References to papers published acknowledging this grant can be found at the end of this report and almost all are supplied in pdf form. (1) In the temperate forests of the Cascade Mountains, USA, calcium and magnesium meet vastly different fates beneath angiosperms vs gymnosperms. Calcium is leached beneath both groves of trees, but leached 20-40% more beneath the angiosperms. Magnesium is retained in the forest system beneath the angiosperms and leached from beneath the gymnosperms. (2) We have shown that climate and CO2, based on both carbon cycle modeling and hundreds of independent proxies for paleo-CO2, correlate very well over the past 550 million year. In a recent paper we use this correlation to deduce the sensitivity of global mean temperature to a doubling of atmospheric CO2, and results are in excellent agreement with the results of climatologists based on the historical record and on theoretical climate models (GCMs).(3) We have shown that concentrations of atmospheric oxygen, calculated by a combined carbon-sulfur cycle model, over the past 550 million years have varied with and influenced biological evolution.

Berner, Robert A

2008-02-05T23:59:59.000Z

359

Spatial Relationships of Sector-Specific Fossil-fuel CO2 Emissions in the United States  

SciTech Connect (OSTI)

Quantification of the spatial distribution of sector-specific fossil fuel CO2 emissions provides strategic information to public and private decision-makers on climate change mitigation options and can provide critical constraints to carbon budget studies being performed at the national to urban scales. This study analyzes the spatial distribution and spatial drivers of total and sectoral fossil fuel CO2 emissions at the state and county levels in the United States. The spatial patterns of absolute versus per capita fossil fuel CO2 emissions differ substantially and these differences are sector-specific. Area-based sources such as those in the residential and commercial sectors are driven by a combination of population and surface temperature with per capita emissions largest in the northern latitudes and continental interior. Emission sources associated with large individual manufacturing or electricity producing facilities are heterogeneously distributed in both absolute and per capita metrics. The relationship between surface temperature and sectoral emissions suggests that the increased electricity consumption due to space cooling requirements under a warmer climate may outweigh the savings generated by lessened space heating. Spatial cluster analysis of fossil fuel CO2 emissions confirms that counties with high (low) CO2 emissions tend to be clustered close to other counties with high (low) CO2 emissions and some of the spatial clustering extends to multi-state spatial domains. This is particularly true for the residential and transportation sectors, suggesting that emissions mitigation policy might best be approached from the regional or multi-state perspective. Our findings underscore the potential for geographically focused, sector-specific emissions mitigation strategies and the importance of accurate spatial distribution of emitting sources when combined with atmospheric monitoring via aircraft, satellite and in situ measurements. Keywords: Fossil-fuel; Carbon dioxide emissions; Sectoral; Spatial cluster; Emissions mitigation policy

Zhou, Yuyu; Gurney, Kevin R.

2011-07-01T23:59:59.000Z

360

Section 6. Deep Time: Modelling of Atmospheric CO2 and the Marine CO2-Carbonic Acid-Carbonate System  

Science Journals Connector (OSTI)

...original MAGic model (Arvidson et al., 2006) as revised in Arvidson et al. (2011). There are a number of Earth system models in the literature (e.g., Berner and Canfield 1989; Hansen and Wallmann, 2003; Berner 2004; Bergman et al...

Fred T. Mackenzie; Andreas J. Andersson

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


361

NETL: 2011 Conference Proceedings - 2011 NETL CO2 Capture Technology  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

2011 NETL CO2 Capture Technology Meeting 2011 NETL CO2 Capture Technology Meeting August 22 - 26, 2011 Previous Proceedings 2009: Annual NETL CO2 Capture Technology for Existing Plants R&D Meeting 2010: 2010 NETL CO2 Capture Technology Meeting Proceedings of the 2011 NETL CO2 Capture Technology Meeting Table of Contents Presentations Monday, August 22 Opening/Overview Post-combustion Sorbent-Based Capture Post-combustion Membrane-Based Capture Tuesday, August 23 Post-combustion Solvent-Based Capture ARPA-E Capture Projects Wednesday, August 24 Oxy-Combustion and Oxygen Production Chemical Looping Process CO2 Compression Thursday, August 25 FutureGen 2.0, CCPI and ICCS Demonstration Projects System Studies and Modeling Pre-Combustion Capture Projects Friday, August 26 Pre-combustion Capture Projects Posters

362

High Co2 Emissions Through Porous Media- Transport Mechanisms And  

Open Energy Info (EERE)

Co2 Emissions Through Porous Media- Transport Mechanisms And Co2 Emissions Through Porous Media- Transport Mechanisms And Implications For Flux Measurement And Fractionation Jump to: navigation, search GEOTHERMAL ENERGYGeothermal Home Journal Article: High Co2 Emissions Through Porous Media- Transport Mechanisms And Implications For Flux Measurement And Fractionation Details Activities (1) Areas (1) Regions (0) Abstract: Diffuse emissions of CO2 are known to be large around some volcanoes and hydrothermal areas. Accumulation-chamber measurements of CO2 flux are increasingly used to estimate the total magmatic or metamorphic CO2 released from such areas. To assess the performance of accumulation chamber systems at fluxes one to three orders of magnitude higher than normally encountered in soil respiration studies, a test system was

363

People's Republic of China Fossil-Fuel CO2 Emissions  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Asia Asia » People's Republic of China People's Republic of China Fossil-Fuel CO2 Emissions Graph graphic Graphics Data graphic Data Trends According to reported energy statistics, coal production and use in China has increased ten-fold since the 1960s. As a result, Chinese fossil-fuel CO2 emissions have more than doubled 2000 alone. At 1.92 billion metric tons of carbon in 2008, the People's Republic of China is the world's largest emitter of CO2 due to fossil-fuel use and cement production. Even with the reported decline in Chinese emissions from 1997 to 1999, China's industrial emissions of CO2 have grown phenomenally since 1950, when China stood tenth among nations based on annual fossil-fuel CO2 emissions. From 1970 to 1997, China's fossil-fuel CO2 emissions grew at an annual rate of

364

Uncertainty quantification for CO2 sequestration and enhanced oil recovery  

E-Print Network [OSTI]

This study develops a statistical method to perform uncertainty quantification for understanding CO2 storage potential within an enhanced oil recovery (EOR) environment at the Farnsworth Unit of the Anadarko Basin in northern Texas. A set of geostatistical-based Monte Carlo simulations of CO2-oil-water flow and reactive transport in the Morrow formation are conducted for global sensitivity and statistical analysis of the major uncertainty metrics: net CO2 injection, cumulative oil production, cumulative gas (CH4) production, and net water injection. A global sensitivity and response surface analysis indicates that reservoir permeability, porosity, and thickness are the major intrinsic reservoir parameters that control net CO2 injection/storage and oil/gas recovery rates. The well spacing and the initial water saturation also have large impact on the oil/gas recovery rates. Further, this study has revealed key insights into the potential behavior and the operational parameters of CO2 sequestration at CO2-EOR s...

Dai, Zhenxue; Fessenden-Rahn, Julianna; Middleton, Richard; Pan, Feng; Jia, Wei; Lee, Si-Yong; McPherson, Brian; Ampomah, William; Grigg, Reid

2014-01-01T23:59:59.000Z

365

Reaction of Cp*(CO)2ReRe(CO)2Cp* with Alkynes Produces Dimetallacyclopentenones Cp*(CO)2Re(?-?1,?3-CRCRCO)Re(CO)Cp* Which React with Acid To Form Cationic Bridging Vinyl Complexes  

Science Journals Connector (OSTI)

Reaction of Cp*(CO)2ReRe(CO)2Cp* with Alkynes Produces Dimetallacyclopentenones Cp*(CO)2Re(?-?1,?3-CRCRCO)Re(CO)Cp* Which React with Acid To Form Cationic Bridging Vinyl Complexes ... Cp*(CO)2ReRe(CO)2Cp* reacted with terminal alkynes HC?CR to produce dimetallacyclopentenones Cp*(CO)2Re(?-?1,?3-CHCRCO)Re(CO)Cp*. ... Protonation of the dimetallacyclopentenones with CF3CO2H produced (?-vinyl)dirhenium cations [Cp*(CO)2Re(?-?1,?2-CHCHR)Re(CO)2Cp*]+. ...

Charles P. Casey; Ronald S. Cario; Hiroyuki Sakaba

1997-02-04T23:59:59.000Z

366

Aquatic primary production in a high-CO2 world  

E-Print Network [OSTI]

Aquatic primary production in a high-CO2 world Etienne Low-De´carie, Gregor F. Fussmann, and Graham-Penfield, Montreal, QC, H3A 1B1, Canada Here, we provide a review of the direct effect of increas- ing CO2 on aquatic: the assessment of theories about limitation of productivity and the integration of CO2 into the co

Fussman, Gregor

367

NETL: IEP - Post-Combustion CO2 Emissions Control - Low Cost Sorbent for  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Low Cost Sorbent for Capturing CO2 Emissions Generated by Existing Coal-Fired Power Plants Low Cost Sorbent for Capturing CO2 Emissions Generated by Existing Coal-Fired Power Plants Project No.: DE-NT0005497 TDA sorbent test equipment TDA sorbent test equipment. TDA Research Inc. will produce and evaluate a low-cost solid sorbent developed in prior laboratory testing. The process uses an alkalized alumina adsorbent to capture carbon dioxide (CO2) at intermediate temperature and near ambient pressure. The physical adsorbent is regenerated with low-pressure steam. Although the regeneration is primarily by concentration swing, the adsorption of steam on the sorbent during regeneration also provides approximately 8°C to 10°C of temperature swing, further enhancing the regeneration rate. The sorbent is transferred between two moving bed reactors. Cycling results in gas

368

Superstructure Optimization: Reaction Yield Dependent CO2 Removal from OCM Product Gas  

Science Journals Connector (OSTI)

Abstract The oxidative coupling of methane presents an alternative for the production of ethene as opposed to the standard steam cracking of crude oil. A drawback of the reaction is the byproduct creation of CO2. Due to economic reasons, CO2 needs to be removed from the product gas efficiently, while keeping the ethene loss below 5%. Therefore, an overall assessment of the reaction and gas purification section of an OCM process is required. In the past, experiments have shown that a combination of various gas separation membranes with an absorption-desorption process leads to efficient hybrid separation processes. In this contribution, superstructure optimization of the separation section is performed combining various gas separation membranes (in type and number) with an absorption-desorption process and using different input values of CO2 and ethene concentrations leading to a significant energy reduction compared to standard absorption processes.

Christian Bock; Erik Esche; David Mller; Gnter Wozny

2014-01-01T23:59:59.000Z

369

Grangemouth Advanced CO2 Capture Project GRACE | Open Energy...  

Open Energy Info (EERE)

GRACE is a project consortium that aims to develop cost improving technologies for carbon capture and separation. References: Grangemouth Advanced CO2 Capture Project...

370

Synthesis and CO2 Adsorption Properties of Molecularly Imprinted Adsorbents  

Science Journals Connector (OSTI)

Synthesis and CO2 Adsorption Properties of Molecularly Imprinted Adsorbents ... Adsorption Separation of Carbon Dioxide from Flue Gas by a Molecularly Imprinted Adsorbent ...

Yi Zhao; Yanmei Shen; Lu Bai; Rongjie Hao; Liyan Dong

2012-01-12T23:59:59.000Z

371

Characterization New CO2 Laser Universidad del Valle Cali Colombia  

Science Journals Connector (OSTI)

The new CO2 laser constructed in Cali Colombia was characterized. Include power vs. pressure, for a constant voltage and constant pressure, spectrum visible for mixture, stability of...

Bedoya, Alvaro Casas; Goyes, Clara E; Garcia, Hans; Rodrguez, Efrain Solarte

372

Validation of CO2 line parameters used in temperature retrievals  

Science Journals Connector (OSTI)

A simultaneous retrieval procedure is utilized to investigate CO2 spectroscopic line parameters in order to reduce systematic errors in temperature retrievals. Provided are initial...

Shephard, Mark W; Clough, Shepard A; Delamere, Jennifer; Tobin, David C; Turner, David D; Revercomb, Hank E; Knuteson, Robert; Beer, Reinhard

373

CO2-SELECTIVE MEMBRANE FOR FUEL CELL APPLICATIONS.  

E-Print Network [OSTI]

??We have developed CO2-selective membranes to purified hydrogen and nitrogenfor fuel cell processes. Hydrogen purification impacts other industries such as ammoniaproduction and flue gas purification (more)

El-Azzami, Louei Abdel Raouf

2006-01-01T23:59:59.000Z

374

Novel Processes for Power Plant with CO2 Capture.  

E-Print Network [OSTI]

?? The purpose of this thesis was to examine different technologies, which enhances the CO2 partial pressure in the flue gas from the natural gas (more)

Ekre, Kjetil Vinjerui

2012-01-01T23:59:59.000Z

375

Technological Options for Reducing Non-CO2 GHG Emissions  

Science Journals Connector (OSTI)

A project titled Clearinghouse of Technological Options for Reducing Anthropogenic Non-CO 2 GHG Emissions from All Sectors was recently conducted. The o...

Prof. Dr. Jeff Kuo Ph.D.; P.E.

2012-01-01T23:59:59.000Z

376

Supercontinuum generation versus optical breakdown in CO2 gas  

Science Journals Connector (OSTI)

Threshold powers for optical breakdown (OB) and supercontinuum (SC) generation in high-pressure CO2 gas have been measured at different focusing conditions. It has been...

Ilkov, F A; Ilkova, L Sh; Chin, S L

1993-01-01T23:59:59.000Z

377

Gravity monitoring of CO2 movement during sequestration: Model studies  

E-Print Network [OSTI]

CO 2 enhanced oil recovery (EOR) and sequestration in afor a coalbed methane formation. EOR/sequestration petroleumbut shallow compared to either EOR or brine formations. The

Gasperikova, E.

2008-01-01T23:59:59.000Z

378

CO2ReMoVe - Progress Report  

E-Print Network [OSTI]

Seismic characterization of thin beds containing patchy carbon dioxide-brine .... different fluids involved in the CO2 sequestration procedure at variable formation

Danilo R. Velis

379

Enhanced Geothermal Systems (EGS) with CO2as Heat Transmission...  

Broader source: Energy.gov (indexed) [DOE]

precipitation with spatial and temporal flow variations in CO2brinerock systems Tracer Methods for Characterizing Fracture Stimulation in Engineered Geothermal Systems (EGS)...

380

International Symposium on Site Characterization for CO2 Geological Storage  

E-Print Network [OSTI]

EOR) and enhanced coalbed methane recovery (ECBMR) becauseand potential for coalbed methane. The Mannville coals areCO 2 injectivity and coalbed methane producibility. Thus,

Tsang, Chin-Fu

2006-01-01T23:59:59.000Z

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


381

Chemical Impact of Elevated CO2on Geothermal Energy Production  

Broader source: Energy.gov (indexed) [DOE]

Chemical Impact of Elevated CO 2 on Geothermal Energy Production Principal Investigator Susan Carroll Lawrence Livermore National Lab Track Name May 18-20, 2010 This presentation...

382

Influence of capillary pressure on CO2 storage and monitoring  

E-Print Network [OSTI]

solutions to mitigate the greenhouse effect. We are interested in analyzing the influence of capillary pressure on CO2 in- jection, storage and monitoring in saline...

gabriela

383

Geothermal: Sponsored by OSTI -- Integrated, Geothermal-CO2 Storage...  

Office of Scientific and Technical Information (OSTI)

Integrated, Geothermal-CO2 Storage Reservoirs: Adaptable, Multi-Stage, Sustainable, Energy-Recovery Strategies that Reduce Carbon Intensity and Environmental Risk...

384

Source Term Estimation of Radioxenon Released from the Fukushima Dai-ichi Nuclear Reactors Using Measured Air Concentrations and Atmospheric Transport Modeling  

SciTech Connect (OSTI)

Systems designed to monitor airborne radionuclides released from underground nuclear explosions detected radioactive fallout from the Fukushima Daiichi nuclear accident in March 2011. Atmospheric transport modeling (ATM) of plumes of noble gases and particulates were performed soon after the accident to determine plausible detection locations of any radioactive releases to the atmosphere. We combine sampling data from multiple International Modeling System (IMS) locations in a new way to estimate the magnitude and time sequence of the releases. Dilution factors from the modeled plume at five different detection locations were combined with 57 atmospheric concentration measurements of 133-Xe taken from March 18 to March 23 to estimate the source term. This approach estimates that 59% of the 1.241019 Bq of 133-Xe present in the reactors at the time of the earthquake was released to the atmosphere over a three day period. Source term estimates from combinations of detection sites have lower spread than estimates based on measurements at single detection sites. Sensitivity cases based on data from four or more detection locations bound the source term between 35% and 255% of available xenon inventory.

Eslinger, Paul W. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Biegalski, S. [Univ. of Texas at Austin, TX (United States); Bowyer, Ted W. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Cooper, Matthew W. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Haas, Derek A. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Hayes, James C. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Hoffman, Ian [Radiation Protection Bureau, Health Canada, Ottawa, ON (Canada); Korpach, E. [Radiation Protection Bureau, Health Canada, Ottawa, ON (Canada); Yi, Jing [Radiation Protection Bureau, Health Canada, Ottawa, ON (Canada); Miley, Harry S. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Rishel, Jeremy P. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States); Ungar, R. Kurt [Radiation Protection Bureau, Health Canada, Ottawa, ON (Canada); White, Brian [Radiation Protection Bureau, Health Canada, Ottawa, ON (Canada); Woods, Vincent T. [Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

2014-01-01T23:59:59.000Z

385

D-optimal design for Rapid Assessment Model of CO2 flooding in high water cut oil reservoirs  

Science Journals Connector (OSTI)

Abstract Most of major oilfields in China have reached high water cut stage, but still, they contribute to more than 70% of domestic oil production. How to extract more oil from mature oilfields has become a hot topic in petroleum engineering. Carbon dioxide flooding is a winwin strategy because it can enhance oil recovery and simultaneously reduce CO2 emissions into the atmosphere. In order to evaluate the potentials of CO2 flooding in high water cut oil reservoirs, various 3-D heterogeneous geological models were built based on Guan 104 fault block in Dagang Oilfield to perform reservoir simulations. The D-optimal design was applied to build and verify the Rapid Assessment Model of CO2 flooding in high water cut oil reservoirs. Five quantitative variables were considered, including average horizontal permeability, permeability variation coefficient, ratio of vertical to horizontal permeability, net thickness of formation and percentage of recoverable reserves by water flooding. The process of weighting emphasized the contributions of linear terms, quadratic terms and first-order interactions of five quantitative parameters to improved recovery factor and Net Present Value of CO2 flooding. Using the Rapid Assessment Model of CO2 flooding in high water cut oil reservoirs, significant first-order interactions were sorted out and type curves were established and analyzed for the evaluation of technical and economic efficiency of CO2 flooding in high water cut oil reservoirs. Aimed at oil reservoirs with the similar geological conditions and fluid properties as Guan 104 fault block, the Rapid Assessment Model and type curves of CO2 flooding in high water cut oil reservoirs can be applied to predict improved recovery factor and Net Present Value of water-alternating-CO2 flooding at different conditions of reservoir parameters and development parameter. The approach could serve as a guide for the application and spread of CO2-EOR projects.

Zhaojie Song; Zhiping Li; Chunsheng Yu; Jirui Hou; Mingzhen Wei; Baojun Bai; Yunpeng Hu

2014-01-01T23:59:59.000Z

386

Impact of porous medium desiccation during anhydrous CO2 injection in deep saline aquifers: up scaling from experimental  

E-Print Network [OSTI]

into the atmosphere. CO2 is captured from exhaust gas in power plants or industrial units and then stored of the saturation profile evolution with two phase flow model integrating thermal effects. An up scaling on recent experiments and numerical simulations, the near-well injection zone is identified

Boyer, Edmond

387

Optimale Energisystemer for LNG-anlegg med CO2-fangst; Optimal Energy Systems for LNG Plants with CO2 Capture.  

E-Print Network [OSTI]

?? Produksjon av LNG er en energikrevende prosess, spesielt p grunn av hyt kraftbehov for gjre naturgassen flytende. Utfordringer knyttet til utslipp av CO2 (more)

Bratseth, Arne

2008-01-01T23:59:59.000Z

388

Using of the tunable CO2-laser without frequency stabilization for diagnostics of CO2 gas mixture at barometric pressure  

Science Journals Connector (OSTI)

It is presented a technique for determining temperature and pressure of CO2 in gas mixture using absorption factor spectral distribution. Errors calculated for tunable frequency...

Arshinov, K

389

A Theoretical Study of CO2 Anions on Anatase (101) Surface. ...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

CO2 Anions on Anatase (101) Surface. A Theoretical Study of CO2 Anions on Anatase (101) Surface. Abstract: Binding configurations of CO2 and CO2 - on perfect and oxygen-deficient...

390

Highlights of the 2009 SEG summer research workshop on "CO2 Sequestration Geophysics"  

E-Print Network [OSTI]

CO 2 saturation at the Weyburn CO 2 EOR injection project inMonitoring CO 2 storage during EOR at the Weyburn-Midalean excellent example of a CO 2 EOR (enhanced oil recovery)

Lumley, D.

2010-01-01T23:59:59.000Z

391

Single photon ionization of van der Waals clusters with a soft x-ray laser: ,,CO2...n and ,,CO2...n,,H2O...m  

E-Print Network [OSTI]

Single photon ionization of van der Waals clusters with a soft x-ray laser: ,,CO2...n and ,,CO2...n 2006; published online 20 October 2006 Pure neutral CO2 n clusters and mixed CO2 n H2O m clustersV. The distribution of pure CO2 n clusters decreases roughly exponentially with increasing cluster size. During

Rocca, Jorge J.

392

CO2 Capture by Absorption with Potassium Carbonate  

E-Print Network [OSTI]

CO2 Capture by Absorption with Potassium Carbonate Fourth Quarterly Report 2006 Quarterly Progress of this work is to improve the process for CO2 capture by alkanolamine absorption/stripping by developing% in the order: thiosulfatecarbonate is ineffective in the absence of oxygen

Rochelle, Gary T.

393

CO2 Capture by Absorption with Potassium Carbonate  

E-Print Network [OSTI]

CO2 Capture by Absorption with Potassium Carbonate First Quarterly Report 2007 Quarterly Progress of this work is to improve the process for CO2 capture by alkanolamine absorption/stripping by developing% to 160% in the order: thiosulfatecarbonate is ineffective

Rochelle, Gary T.

394

CO2 Capture by Absorption with Potassium Carbonate  

E-Print Network [OSTI]

CO2 Capture by Absorption with Potassium Carbonate Third Quarterly Report 2006 Quarterly Progress of this work is to improve the process for CO2 capture by alkanolamine absorption/stripping by developing by Jou and Mather. Corrosion of carbon steel without inhibitors increases from 19 to 181 mpy in lean

Rochelle, Gary T.

395

Oxidation in Environments with Elevated CO2 Levels  

SciTech Connect (OSTI)

Efforts to reduce greenhouse gas emissions from fossil energy power productions focus primarily on either pre- or post-combustion removal of CO2. The research presented here examines corrosion and oxidation issues associated with two types of post-combustion CO2 removal processesoxyfuel combustion in refit boilers and oxyfuel turbines.

Gordon H. Holcomb

2009-05-01T23:59:59.000Z

396

Chemical Impact of Elevated CO2on Geothermal Energy Production  

Broader source: Energy.gov [DOE]

This is a two phase project to assess the geochemical impact of CO2on geothermal energy production by: analyzing the geochemistry of existing geothermal fields with elevated natural CO2; measuring realistic rock-water rates for geothermal systems using laboratory and field-based experiments to simulate production scale impacts.

397

Implementation of the El Mar (Delaware) Unit CO2 flood  

SciTech Connect (OSTI)

Union Royalty, Inc., Amoco Production Company, and Enron Liquids Pipeline Company recently announced that they have commenced operations of an innovative enhanced oil recovery project at the El Mar (Delaware) Unit in Loving County, Texas, about 100 miles west of Midland, Texas. The project will convert the unit`s existing oil recovery system from a secondary (waterflood) system to a tertiary (CO2 flood) system designed to use carbon dioxide and water to increase crude oil production from the unit. What makes this EOR project unique is the creative deal structured by the partners involved. Amoco, Union Royalty, and Enron have worked out an unprecedented arrangement whereby Amoco essentially trades CO2 for an interest in Union Royalty`s future oil production from the unit. By pioneering this innovative deal new production life has been restored to a field that otherwise might dry up. Enron is participating in the project by transporting CO2 to the unit via a 40-mile expansion of its Central Basin Pipeline system from the Dollarhide oil field in Andrews county, Texas. The project will be implemented in four phases. The first phase in operation today comprises seven CO2 injection wells which have begun to process the reservoir with CO2. Plans now call for more CO2 injectors to be installed during the next three to five years until a total of 65 CO2 injectors and an on-site CO2 compression facility serve the unit`s 70 production wells.

McKnight, T.N. Jr. [Union Royalty, Inc., Midland, TX (United States); Merchant, D.L.

1995-12-31T23:59:59.000Z

398

Energy Resonances between Molecular Species in CO2 Gas Lasers  

Science Journals Connector (OSTI)

... to a, number of other close energy resonances which exist, between laser levels of CO2, and the diatomic and triatomic; species expected to be present in various discharges in ... the diatomic and triatomic; species expected to be present in various discharges in. which CO2 laser action has been achieved. ...

R. W. NICHOLLS

1970-04-25T23:59:59.000Z

399

THERMOCATALYTIC CO2-FREE PRODUCTION OF HYDROGEN FROM HYDROCARBON FUELS  

E-Print Network [OSTI]

THERMOCATALYTIC CO2- FREE PRODUCTION OF HYDROGEN FROM HYDROCARBON FUELS N. Muradov Florida Solar Energy Center 1679 Clearlake Road, Cocoa, Florida 32922 tel. 321-638-1448, fax. 321-638-1010, muradov (except for the start-up operation). This results in the following advantages: (1) no CO/CO2 byproducts

400

Energy solutions for CO2 emission peak and subsequent decline  

E-Print Network [OSTI]

Energy solutions for CO2 emission peak and subsequent decline Edited by Leif Sønderberg Petersen and Hans Larsen Risø-R-1712(EN) September 2009 Proceedings Risø International Energy Conference 2009 #12;Editors: Leif Sønderberg Petersen and Hans Larsen Title: Energy solutions for CO2 emission peak

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


401

Distribution of anthropogenic CO2 in the Pacific Ocean  

E-Print Network [OSTI]

Distribution of anthropogenic CO2 in the Pacific Ocean C. L. Sabine,1 R. A. Feely,2 R. M. Key,3 J] This work presents an estimate of anthropogenic CO2 in the Pacific Ocean based on measurements from the WOCE tracers; 9355 Information Related to Geographic Region: Pacific Ocean; KEYWORDS: Pacific Ocean

402

Numerical investigation on photocatalytic CO2 reduction by solar energy in double-skin sheet reactor  

Science Journals Connector (OSTI)

Abstract Double-skin sheet reactor (DSSR) attracts attention in recent years due to the simple design and high mass transfer, but its application to photocatalytic CO2 reduction with immobilized catalyst is still a new trial. In this paper, the three-dimensional models describing the photocatalytic CO2 reduction in DSSR by means of solar energy were developed and numerically simulated, on the basis of the transient and continuous solar light distributions. A performance evaluation approach was proposed to guide the structural optimization of DSSR in photocatalytic CO2 reduction. The effects of operation parameters and reactor structures on CH3OH concentration were analyzed and discussed. The results show that the outlet CH3OH concentration of 2.68נ10?4molm?3 in DSSR is much greater than that of 1.77נ10?5molm?3 in optical fiber monolith reactor under the same conditions. It increases as both the inlet water vapor concentration ratio and day-average light flux increase, but decreases with increasing the inlet velocity, all of which are beneficial to the CH3OH productivity. The CH3OH concentration will decrease with the increase of the number of parallel-flow channels, but increase thanks to the rise in the widthheight ratio and inserting flow guiding pieces, which are recommended for higher CH3OH concentration in the design of DSSR.

Tianchen Wang; Lijun Yang; Kai Yuan; Xiaoze Du; Yongping Yang

2014-01-01T23:59:59.000Z

403

Global Fossil-Fuel CO2 Emissions  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Data (ASCII, Fixed Format) Data graphic Data (ASCII, Fixed Format) Data graphic Data (ASCII, Comma-delimited) Trends Since 1751 approximately 337 billion metric tonnes of carbon have been released to the atmosphere from the consumption of fossil fuels and cement production. Half of these emissions have occurred since the mid 1970s. The 2007 global fossil-fuel carbon emission estimate, 8365 million metric tons of carbon, represents an all-time high and a 1.7% increase from 2006. Globally, liquid and solid fuels accounted for 76.3% of the emissions from fossil-fuel burning and cement production in 2007. Combustion of gas fuels (e.g., natural gas) accounted for 18.5% (1551 million metric tons of carbon) of the total emissions from fossil fuels in 2007 and reflects a gradually increasing global utilization of natural gas. Emissions from

404

Quantifying Regional Economic Impacts of CO2 Intensity Targets in China  

E-Print Network [OSTI]

To address rising energy use and CO2 emissions, Chinas leadership has enacted energy and CO2 intensity

Zhang, Da

2012-09-01T23:59:59.000Z

405

DOE Regional Partnership Successfully Demonstrates Terrestrial CO2 Storage  

Broader source: Energy.gov (indexed) [DOE]

Successfully Demonstrates Terrestrial CO2 Successfully Demonstrates Terrestrial CO2 Storage Practices in Great Plains Region of U.S. and Canada DOE Regional Partnership Successfully Demonstrates Terrestrial CO2 Storage Practices in Great Plains Region of U.S. and Canada August 19, 2010 - 1:00pm Addthis Washington, DC - A field test demonstrating the best approaches for terrestrial carbon dioxide (CO2) storage in the heartland of North America has been successfully completed by one of the U.S. Department of Energy's (DOE) seven Regional Carbon Sequestration Partnerships (RCSPs). The Plains CO2 Reduction (PCOR) Partnership , a collaboration of over 80 U.S. and Canadian stakeholders, conducted the field test at sites in the Prairie Pothole Region, extending from central Iowa into Northern Alberta,

406

North Korea Fossil-Fuel CO2 Emissions  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Far East » North Korea Far East » North Korea North Korea Fossil-Fuel CO2 Emissions Graph graphic Graphics Data graphic Data Trends The total fossil-fuel CO2 emissions for North Korea, or the Democratic People's Republic of Korea, averaged 11.2% growth from 1950-93, reaching 71 million metric tons of carbon. Since 1993 according to published UN energy statistics, fossil-fuel CO2 emissions have declined 70% to 21.4 million metric tons of carbon. As the world's 14th largest producer of coal, it is no surprise North Korea's fossil-fuel CO2 emissions record is dominated by emissions from coal burning. Coal consumption accounted for 93% of the 2008 CO2 emission total. With no natural gas usage, another 3.4% currently comes from liquid petroleum consumption, and the remainder is from cement

407

Super Building Insulation by CO2 Foaming Process Research Project |  

Broader source: Energy.gov (indexed) [DOE]

Emerging Technologies » Super Building Insulation by CO2 Foaming Emerging Technologies » Super Building Insulation by CO2 Foaming Process Research Project Super Building Insulation by CO2 Foaming Process Research Project The Department of Energy is currently researching the development of building superinsulation through a carbon dioxide (CO2) foaming process. Project Description This project seeks to develop building super insulation through a carbon dioxide foaming process that does not use hydrofluorocarbons (HFCs), and which produces insulation with a high R-value. Project Partners Research is being undertaken between the Department of Energy and The Industrial Science & Technology Network. Project Goals The goal of this project is to develop advanced insulation without HFC, and to achieve a competitive processing cost for CO2 foaming technology.

408

South Korea Fossil-Fuel CO2 Emissions  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Far East » South Korea Far East » South Korea South Korea Fossil-Fuel CO2 Emissions Graph graphic Graphics Data graphic Data Trends South Korea, or the Republic of Korea, is the world's tenth largest emitter of CO2 based on 2008 fossil-fuel consumption and cement production with 139 million metric tons of carbon. From 1946-1997 South Korea experienced phenomenal growth in fossil-fuel CO2 emissions with a growth rate that averaged 11.5%. Initial growth in emissions was due to coal consumption, which still accounts for 46.9% of South Korea's fossil-fuel CO2 emissions. Since the late 1960s oil consumption has been a major source of emissions. South Korea is the world's fifth largest importer of crude oil. Natural gas became a significant source of CO2 for the first time in 1987, as South

409

CO2 Injection in Kansas Oilfield Could Greatly Increase Production,  

Broader source: Energy.gov (indexed) [DOE]

CO2 Injection in Kansas Oilfield Could Greatly Increase Production, CO2 Injection in Kansas Oilfield Could Greatly Increase Production, Permanently Store Carbon Dioxide, DOE Study Says CO2 Injection in Kansas Oilfield Could Greatly Increase Production, Permanently Store Carbon Dioxide, DOE Study Says August 31, 2011 - 1:00pm Addthis Washington, DC - The feasibility of using carbon dioxide (CO2) injection for recovering between 250 million and 500 million additional barrels of oil from Kansas oilfields has been established in a study funded by the U.S. Department of Energy (DOE). The University of Kansas Center for Research studied the possibility of near-miscible CO2 flooding for extending the life of mature oilfields in the Arbuckle Formation while simultaneously providing permanent geologic storage of carbon dioxide, a major greenhouse gas.

410

NETL: Low-Pressure Membrane Contactors for CO2 Capture  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Low-Pressure Membrane Contactors for CO2 Capture Low-Pressure Membrane Contactors for CO2 Capture Project No.: DE-FE0007553 Membrane Technology and Research, Inc. (MTR) is developing a new type of membrane contactor (or mega-module) to separate carbon dioxide (CO2) from power plant flue gas. This module's membrane area is 500 square meters, 20 to 25 times larger than that of current modules used for CO2 capture. A 500-MWe coal power plant requires 0.5 to 1 million square meters of membrane to achieve 90 percent CO2 capture. The new mega-modules can drastically reduce the cost, complexity, and footprint of commercial-scale membrane module integration. Energy savings due to low-pressure drops for gases circulated through the modules, as well as improved countercurrent flow, are additional benefits. The feasibility of using mega-modules in several different hybrid process designs is being evaluated for future development potential.

411

NETL: 2010 Conference Proceedings - 2010 NETL CO2 Capture Technology  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

2010 NETL CO2 Capture Technology Meeting 2010 NETL CO2 Capture Technology Meeting September 13-17, 2010 Table of Contents Presentations Monday, September 13 Opening/Overview Post-combustion Sorbent Based Capture Post-combustion Solvent Based Capture Tuesday, September 14 Post-combustion Membrane Based Capture Pulverized Coal Oxy-combustion ARPA-E Projects Wednesday, September 15 National Carbon Capture Center Chemical Looping Processes Systems Studies and Modeling Efforts CO2 Compression New CO2 Capture Projects Thursday, September 16 New CO2 Capture Projects - Cont'd CCPI and ICCS Demonstration Projects Pre-combustion Capture Projects Friday, September 17 Pre-combustion Capture Projects - Cont'd Posters Advanced Research Projects Agency - Energy (ARPA-E) NETL Office of Research and Development Research Projects

412

CO2 Geologic Storage (Kentucky) | Department of Energy  

Broader source: Energy.gov (indexed) [DOE]

CO2 Geologic Storage (Kentucky) CO2 Geologic Storage (Kentucky) CO2 Geologic Storage (Kentucky) < Back Eligibility Industrial Program Info State Kentucky Program Type Industry Recruitment/Support Provider Consultant, Division of Carbon Management Division staff, in partnership with the Kentucky Geological Survey (KGS), continued to support projects to investigate and demonstrate the technical feasibility of geologic storage of carbon dioxide (CO2) in Kentucky. In 2012, KGS conducted a test of carbon dioxide enhanced natural gas recovery in the Devonian Ohio Shale, Johnson County, east Kentucky. During the test, 87 tons of CO2 were injected through perforations in a cased, shut-in shale gas well. Industry partners for this research included Crossrock Drilling, Advanced Resources International, Schlumberger, Ferus Industries, and

413

Definition: Reduced Co2 Emissions | Open Energy Information  

Open Energy Info (EERE)

Co2 Emissions Co2 Emissions Jump to: navigation, search Dictionary.png Reduced Co2 Emissions Functions that provide this benefit can lead to avoided vehicle miles, decrease the amount of central generation needed to their serve load (through reduced electricity consumption, reduced electricity losses, more optimal generation dispatch), and or reduce peak generation. These impacts translate into a reduction in CO2 emissions produced by fossil-based electricity generators and vehicles.[1] Related Terms electricity generation, reduced electricity losses, smart grid References ↑ SmartGrid.gov 'Description of Benefits' An in LikeLike UnlikeLike You like this.Sign Up to see what your friends like. line Glossary Definition Retrieved from "http://en.openei.org/w/index.php?title=Definition:Reduced_Co2_Emissions&oldid=502618

414

Efficient CO2 Fixation Pathways: Energy Plant: High Efficiency Photosynthetic Organisms  

SciTech Connect (OSTI)

PETRO Project: UCLA is redesigning the carbon fixation pathways of plants to make them more efficient at capturing the energy in sunlight. Carbon fixation is the key process that plants use to convert carbon dioxide (CO2) from the atmosphere into higher energy molecules (such as sugars) using energy from the sun. UCLA is addressing the inefficiency of the process through an alternative biochemical pathway that uses 50% less energy than the pathway used by all land plants. In addition, instead of producing sugars, UCLAs designer pathway will produce pyruvate, the precursor of choice for a wide variety of liquid fuels. Theoretically, the new biochemical pathway will allow a plant to capture 200% as much CO2 using the same amount of light. The pathways will first be tested on model photosynthetic organisms and later incorporated into other plants, thus dramatically improving the productivity of both food and fuel crops.

None

2012-01-01T23:59:59.000Z

415

Atmospheric tritium  

SciTech Connect (OSTI)

Research progress for the year 1979 to 1980 are reported. Concentrations of tritiated water vapor, tritium gas and tritiated hydrocarbons in the atmosphere at selected sampling points are presented. (ACR)

Oestlund, H.G.; Mason, A.S.

1980-01-01T23:59:59.000Z

416

Temporal and Spatial Deployment of Carbon Dioxide Capture and Storage Technologies across the Representative Concentration Pathways  

SciTech Connect (OSTI)

The Intergovernmental Panel on Climate Changes (IPCC) Fifth Assessment (to be published in 2013-2014) will to a significant degree be built around four Representative Concentration Pathways (RCPs) that are intended to represent four scenarios of future development of greenhouse gas emissions, land use, and concentrations that span the widest range of potential future atmospheric radiative forcing. Under the very stringent climate policy implied by the 2.6 W/m2 overshoot scenario, all electricity is eventually generated from low carbon sources. However, carbon dioxide capture and storage (CCS) technologies never comprise more than 50% of total electricity generation in that very stringent scenario or in any of the other cases examined here. There are significant differences among the cases studied here in terms of how CCS technologies are used, with the most prominent being is the significant expansion of biomass+CCS as the stringency of the implied climate policy increases. Cumulative CO2 storage across the three cases that imply binding greenhouse gas constraints ranges by nearly an order of magnitude from 170GtCO2 (radiative forcing of 6.0W/m2 in 2100) to 1600GtCO2 (2.6W/m2 in 2100) over the course of this century. This potential demand for deep geologic CO2 storage is well within published estimates of total global CO2 storage capacity.

Dooley, James J.; Calvin, Katherine V.

2011-04-18T23:59:59.000Z

417

Dynamics of Planetary Atmospheres  

E-Print Network [OSTI]

pressure (bars) N2 82%; Ar 12%; CH4 6%CO2 96.5%; N2 3.5%Atmospheric composition 26177Orbital inclination (1992) orbiter ­ Winds from cloud-tracking and probe drifts ­ IR temperatures, solar-fixed tides, polar-Huygens mission (from 2005) ­ Doppler wind descent profile ­ IR temperature and composition maps ­ Visible, IR

Read, Peter L.

418

NETL: IEP - Post-Combustion CO2 Emissions Control - Hybrid  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Hybrid Membrane/Absorption Process for Post-Combustion CO2 Capture Hybrid Membrane/Absorption Process for Post-Combustion CO2 Capture Project No.: DE-FE0004787 Gas Technology Institute is partnering with PoroGen Corporation and Aker Process Systems in a three-year effort to develop a hybrid technology for CO2 capture from flue gases based on a combination of solvent absorption and hollow fiber membrane technologies. The technology could also apply to removal of numerous other gas pollutants such as NOx and SOx, separation of CO2 from hydrogen in refinery streams, and separation of CO2 from natural gas (natural gas sweetening). The technology increases interfacial gas/liquid area by a factor of ten over conventional packed or tray columns, thus increasing mass transfer. The selectivity is controlled by the chemical affinity of CO2 with a hindered amine. The process results in lower steam regeneration energy, and the CO2 is generated at pressure, reducing compression costs. The project includes bench-scale testing on a 25 kWe-equivalent slipstream at Midwest Generation's Joliet Power Station.

419

Combustion-Assisted CO2 Capture Using MECC Membranes  

SciTech Connect (OSTI)

Mixed Electron and Carbonate ion Conductor (MECC) membranes have been proposed as a means to separate CO2 from power plant flue gas. Here a modified MECC CO2 capture process is analyzed that supplements retentate pressurization and permeate evacuation as a means to create a CO2 driving force with a process assisted by the catalytic combustion of syngas on the permeate side of the membrane. The combustion reactions consume transported oxygen, making it unavailable for the backwards transport reaction. With this change, the MECC capture system becomes exothermic, and steam for electricity production may be generated from the waste heat. Greater than 90% of the CO2 in the flue gas may be captured, and a compressed CO2 product stream is produced. A fossil-fueled power plant using this process would consume 14% more fuel per unit electricity produced than a power plant with no CO2 capture system, and has the potential to meet U.S. DOE s goal that deployment of a CO2 capture system at a fossil-fueled power plant should not increase the cost of electricity from the combined facility by more than 30%.

Sherman, Steven R [ORNL; Gray, Dr. Joshua R. [Savannah River National Laboratory (SRNL), Aiken, S.C.; Brinkman, Dr. Kyle S. [Savannah River National Laboratory (SRNL), Aiken, S.C.; Huang, Dr. Kevin [University of South Carolina, Columbia

2012-01-01T23:59:59.000Z

420

Integrated Energy System with Beneficial Carbon Dioxide (CO2) Use  

SciTech Connect (OSTI)

To address the public concerns regarding the consequences of climate change from anthropogenic carbon dioxide (CO2) emissions, the U.S. Department of Energy National Energy Technology Laboratory (DOE-NETL) is actively funding a CO2 management program to develop technologies capable of reducing the CO2 emissions from fossil fuel power plants and other industrial facilities. Over the past decade, this program has focused on reducing the costs of carbon capture and storage technologies. Recently, DOE-NETL launched an alternative CO2 mitigation program focusing on beneficial CO2 reuse and supporting the development of technologies that mitigate emissions by converting CO2 to solid mineral form that can be utilized for enhanced oil recovery, in the manufacturing of concrete or as a benign landfill, in the production of valuable chemicals and/or fuels. This project was selected as a CO2 reuse activity which would conduct research and development (R&D) at the pilot scale via a cost-shared Cooperative Agreement number DE-FE0001099 with DOE-NETL and would utilize funds setaside by the American Recovery and Reinvestment Act (ARRA) of 2009 for Industrial Carbon Capture and Sequestration R&D,

Sun, Xiaolei; Rink, Nancy

2011-04-30T23:59:59.000Z

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


421

CO2 CH4 flux Air temperature Soil temperature and Soil moisture, Barrow, Alaska 2013 ver. 1  

DOE Data Explorer [Office of Scientific and Technical Information (OSTI)]

This dataset consists of field measurements of CO2 and CH4 flux, as well as soil properties made during 2013 in Areas A-D of Intensive Site 1 at the Next-Generation Ecosystem Experiments (NGEE) Arctic site near Barrow, Alaska. Included are i) measurements of CO2 and CH4 flux made from June to September (ii) Calculation of corresponding Gross Primary Productivity (GPP) and CH4 exchange (transparent minus opaque) between atmosphere and the ecosystem (ii) Measurements of Los Gatos Research (LGR) chamber air temperature made from June to September (ii) measurements of surface layer depth, type of surface layer, soil temperature and soil moisture from June to September.

Margaret Torn

422

Discussion of the Influence of CO and CH4 in CO2 Transport, Injection, and Storage for CCS Technology  

Science Journals Connector (OSTI)

The goal of CCS is to avoid the release to the atmosphere of anthropogenic CO2 generated by industrial and energy-related sources. ... (26, 28) The experiments were performed at T and P relevant to those in CO2 pipelines and in geologic storage sites (geothermic gradient = 25 K/km; hydrostatic pressure gradient = 10 MPa/km). ... assessment, which showed an energetic improvement of 0.7?-points for the CASPER model solvent system in comparison to the baseline 30wt? MEA case. ...

Sofa T. Blanco; Clara Rivas; Ramn Bravo; Javier Fernndez; Manuela Artal; Inmaculada Velasco

2014-08-20T23:59:59.000Z

423

HARNESSING THE CHEMISTRY OF CO2  

SciTech Connect (OSTI)

Our research program is broadly focused on activating CO{sub 2} through the use of organic and organometallic based catalysts. Some of our methods have centered on annulation reactions of unsaturated hydrocarbons (and carbonyl substrates) to provide a diverse array of carbocycles and heterocycles. We use a combination of catalyst discovery and optimization in conjunction with classical physical organic chemistry to elucidate the key mechanistic features of the cycloaddition reactions such that the next big advances in catalyst development can be made. Key to all of our cycloaddition reactions is the use of a sterically hindered, electron donating N heterocyclic carbene (NHC) ligand, namely IPr (or SIPr), in conjunction with a low valent nickel pre-catalyst. The efficacy of this ligand is two-fold: (1) the high {delta}-donating ability of the NHC increases the nucleophilicity of the metal center which thereby facilitates interaction with the electrophilic carbonyl and (2) the steric hindrance prevents an otherwise competitive side reaction involving only the alkyne substrate. Such a system has allowed for the facile cycloaddition to prepare highly functionalized pyrones, pyridones, pyrans, as well as novel carbocycles. Importantly, all reactions proceed under extremely mild conditions (room temperature, atmospheric pressures, and short reaction times), require only catalytic amounts of Ni/NHC and readily available starting materials, and afford annulated products in excellent yields. Our current focus revolves around understanding the fundamental processes that govern these cycloadditions such that the next big advance in the cyclization chemistry of CO{sub 2} can be made. Concurrent to our annulation chemistry is our investigation of the potential for imidazolylidenes to function as thermally-actuated CO{sub 2} sequestering and delivery agents.

Louie, Janis

2010-05-11T23:59:59.000Z

424

Argonne Coal Structure Rearrangement Caused by Sorption of CO2  

Science Journals Connector (OSTI)

Argonne Coal Structure Rearrangement Caused by Sorption of CO2 ... The sorption of CO2 on seven Argonne premium coals was measured by using attenuated total reflectance-Fourier transform infrared (ATR-FTIR) spectroscopy as a function of time at constant CO2 pressure (0.62 MPa) and temperature (55 C). ... The following seven Argonne premium coals were investigated:? Upper Freeport (medium volatile bituminous), Pittsburgh No. 8 (high volatile bituminous), Lewiston?Stockton (high volatile bituminous), Blind Canyon (high volatile bituminous), Illinois No. 6 (high volatile bituminous), Wyodak (sub-bituminous), and Beulah Zap (lignite). ...

A. L. Goodman; R. N. Favors; John W. Larsen

2006-10-05T23:59:59.000Z

425

ADVANCED CO2 CYCLE POWER GENERATION  

SciTech Connect (OSTI)

Research is being conducted under United States Department of Energy (DOE) Contract DE-FC26-02NT41621 to develop a conceptual design and determine the performance characteristics of a new IGCC plant configuration that facilitates CO{sub 2} removal for sequestration. This new configuration will be designed to achieve CO{sub 2} sequestration without the need for water gas shifting and CO{sub 2} separation, and may eliminate the need for a separate sequestration compressor. This research introduces a novel concept of using CO{sub 2} as a working fluid for an advanced coal gasification based power generation system, where it generates power with high system efficiency while concentrating CO{sub 2} for sequestration. This project supports the DOE research objective of development of concepts for the capture and storage of CO{sub 2}.

A. Nehrozoglu

2004-01-01T23:59:59.000Z

426

ADVANCED CO2 CYCLE POWER GENERATION  

SciTech Connect (OSTI)

Research is being conducted under United States Department of Energy (DOE) Contract DE-FC26-02NT41621 to develop a conceptual design and determine the performance characteristics of a new IGCC plant configuration that facilitates CO{sub 2} removal for sequestration. This new configuration will be designed to achieve CO{sub 2} sequestration without the need for water gas shifting and CO{sub 2} separation, and may eliminate the need for a separate sequestration compressor. This research introduces a novel concept of using CO{sub 2} as a working fluid for an advanced coal gasification based power generation system, where it generates power with high system efficiency while concentrating CO{sub 2} for sequestration. This project supports the DOE research objective of development of concepts for the capture and storage of CO{sub 2}.

A. Nehrozoglu

2003-10-01T23:59:59.000Z

427

Atmospheric Measurements of Climate-Relevant Species  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Atmospheric Measurements of Climate-Relevant Species Atmospheric Measurements of Climate-Relevant Species CDIAC's data collection includes measurements of the following climate-relevant chemical species. A summary of recent greenhouse gas concentrations is also available. To determine how compounds are named, see the CDIAC "Name that compound" page. Butane (C4H10) Carbon Dioxide (CO2) Carbon Isotopes Carbon Monoxide (CO) Carbon Tetrachloride (CCl4) Chlorofluorocarbons Chloroform (CHCl3) Deuterium (2H) Ethane (C2H6) Ethyl Nitrate (C2H5ONO2) Ethyne (C2H2) Fluoroform (CHF3) Halogenated Compounds (modern records) Halons (fluorocarbons) Hydrogen (H2) Hydrochlorofluorocarbons (HCFCs) Hydrofluorocarbons (HFCs) i-Propyl Nitrate (C3H7ONO2) Methane (CH4) Methyl Bromide (CH3Br) Methyl Chloride (CH3Cl) Methyl Chloroform (CH3CCl3)

428

PASSIVE WIRELESS SURFACE ACOUSTIC WAVE SENSORS FOR MONITORING SEQUESTRATION SITES CO2 EMISSION  

SciTech Connect (OSTI)

University of Pittsburghs Transducer lab has teamed with the U.S. Department of Energys National Energy Technology Laboratory (DOE NETL) to conduct a comprehensive study to develop/evaluate low-cost, efficient CO2 measuring technologies for geological sequestration sites leakage monitoring. A passive wireless CO2 sensing system based on surface acoustic wave technology and carbon nanotube nanocomposite was developed. Surface acoustic wave device was studied to determine the optimum parameters. Delay line structure was adopted as basic sensor structure. CNT polymer nanocomposite was fabricated and tested under different temperature and strain condition for natural environment impact evaluation. Nanocomposite resistance increased for 5 times under pure strain, while the temperature dependence of resistance for CNT solely was -1375ppm/?. The overall effect of temperature on nanocomposite resistance was -1000ppm/?. The gas response of the nanocomposite was about 10% resistance increase under pure CO2. The sensor frequency change was around 300ppm for pure CO2. With paralyne packaging, the sensor frequency change from relative humidity of 0% to 100% at room temperature decreased from over 1000ppm to less than 100ppm. The lowest detection limit of the sensor is 1% gas concentration, with 36ppm frequency change. Wireless module was tested and showed over one foot transmission distance at preferred parallel orientation.

Wang, Yizhong; Chyu, Minking; Wang, Qing-Ming

2012-11-30T23:59:59.000Z

429

CO2 Geologic Storage (Kentucky) | Open Energy Information  

Open Energy Info (EERE)

CO2 Geologic Storage (Kentucky) CO2 Geologic Storage (Kentucky) No revision has been approved for this page. It is currently under review by our subject matter experts. Jump to: navigation, search Last modified on February 12, 2013. EZFeed Policy Place Kentucky Name CO2 Geologic Storage (Kentucky) Policy Category Other Policy Policy Type Industry Recruitment/Support , Technical Feasibility Projects Affected Technologies Coal with CCS Active Policy Yes Implementing Sector State/Province Program Administrator Brandon Nutall, Division of Carbon Management Primary Website http://energy.ky.gov/carbon/Pages/default.aspx Summary Division staff, in partnership with the Kentucky Geological Survey (KGS), continued to support projects to investigate and demonstrate the technical feasibility of geologic storage of carbon dioxide (CO2) in Kentucky. In

430

CO2 Separation from Low-Temperature Flue Gases  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

partners interested in implementing United States Patent Number 7,842,126 entitled "Co 2 Separation from Low-Temperature Flue Gases." Disclosed in this patent are novel methods for processing carbon dioxide (CO 2 ) from combustion gas streams. Researchers at NETL are focused on the development of novel sorbent systems that can effectively remove CO 2 and other gases in an economically feasible manner with limited impact on energy production cost. The current invention will help in reducing greenhouse gas emissions by using an improved, regenerable aqueous amine and soluble potassium carbonate sorbent system. This novel solvent system may be capable of achieving CO 2 capture from larger emission streams at lower overall cost. Overview Sequestration of CO

431

CO2 Injection Begins in Illinois | Department of Energy  

Broader source: Energy.gov (indexed) [DOE]

Begins in Illinois Begins in Illinois CO2 Injection Begins in Illinois November 17, 2011 - 12:00pm Addthis Washington, DC - The Midwest Geological Sequestration Consortium (MGSC), one of seven regional partnerships created by the U.S. Department of Energy (DOE) to advance carbon storage technologies nationwide, has begun injecting carbon dioxide (CO2) for their large-scale CO2 injection test in Decatur, Illinois. The test is part of the development phase of the Regional Carbon Sequestration Partnerships program, an Office of Fossil Energy initiative launched in 2003 to determine the best approaches for capturing and permanently storing gases that can contribute to global climate change. "Establishing long-term, environmentally safe and secure underground CO2 storage is a critical component in achieving successful commercial

432

CO2 Storage and Sink Enhancements: Developing Comparable Economics  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Storage and Sink Enhancements: Storage and Sink Enhancements: Developing Comparable Economics Richard G. Rhudy (rrhudy@epri.com; 650-855-2421) Electric Power Research Institute P.O. Box 10412 Palo Alto, CA 94303-0813 Bert R. Bock (brbock@tva.gov; 256-386-3095) David E. Nichols (denichols@tva.gov; 256-386-2489) Tennessee Valley Authority P.O. Box 1010 Muscle Shoals, AL 35662-1010 Abstract One of the major difficulties in evaluating CO 2 sequestration technologies and practices, both geologic storage of captured CO 2 and storage in biological sinks, is obtaining consistent, transparent, accurate, and comparable economics. This paper reports on a project that compares the economics of major technologies and practices under development for CO 2 sequestration, including captured CO 2 storage options, such as active oil reservoirs, depleted oil and gas

433

Italy (including San Marino) Fossil-Fuel CO2 Emissions  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Western Europe » Italy Western Europe » Italy (including San Marino) Italy (including San Marino) Fossil-Fuel CO2 Emissions Graph graphic Graphics Data graphic Data Trends As occurred in many industrialized nations, CO2 emissions from Italy rose steeply since the late 1940's until the growth was abruptly terminated in 1974. Since 1974, emissions from liquid fuels have vacillated, dropping from 76% to 46% of a static but varying total. Significant increases in natural gas consumption have compensated for the drop in oil consumption. In 2008, 35.8% of Italy's fossil-fuel CO2 emissions were due to natural gas consumption. Coal usage grew steadily until 1985 when CO2 emissions from coal consumption reached 16 million metric tons of carbon. Not until 2004 did coal usage exceed 1985 levels and now accounts for 13.9% of Italy's

434

Kyoto-Related Fossil-Fuel CO2 Emission Totals  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Kyoto-Related Emissions Kyoto-Related Emissions Kyoto-Related Fossil-Fuel CO2 Emission Totals DOI: 10.3334/CDIAC/ffe.007_V2012 world map Kyoto-Related Fossil-Fuel CO2 Emission Totals Year Annex B Countries Non Annex B Countries Fossil-Fuel CO2 Emissions (million metric tonnes C) Bunkers (million metric tonnes C) Fossil-Fuel CO2 Emissions (million metric tonnes C) Bunkers (million metric tonnes C) 1990 3894 90 2111 46 1991 3801 94 2299 38 1992 3750 109 2263 44 1993 3685 107 2339 48 1994 3656 107 2469 54 1995 3681 110 2570 59 1996 3704 111 2657 72 1997 3727 114 2737 74 1998 3746 118 2698 82 1999 3678 124 2718 90 2000 3725 130 2821 90 2001 3781 120 2936 92 2002 3764 128 3013 94 2003 3853 123 3347 98 2004 3888 135 3683 107 2005 3933 142 3926 106

435

ARM - Field Campaign - Boundary Layer CO2 Using CW Lidar  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

govCampaignsBoundary Layer CO2 Using CW Lidar govCampaignsBoundary Layer CO2 Using CW Lidar Comments? We would love to hear from you! Send us a note below or call us at 1-888-ARM-DATA. Send Campaign : Boundary Layer CO2 Using CW Lidar 2005.05.21 - 2005.05.24 Lead Scientist : Michael Dobbs Description Overflights Underway at ACRF Southern Great Plains Site (M.Dobbs/J.Liljegren) Science collaborators at ITT Industries and the National Aeronautics and Space Administration (NASA) Langley Research Center (LaRC) conducted flights over the Central Facility at ACRF's Southern Great Plains (SGP) site as part of the Climate Sources and Sink (CO2) Intensive Operational Period (IOP), using a CW lidar. The objective of the flights was to validate, by demonstration and comparison with SGP ground observations, the performance of the ITT system when used in conjunction with retrieval

436

Coal-CO2 Slurry Feeding System for Pressurized Gasifiers  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Feed Systems Feed Systems Coal-CO2 Slurry Feeding System for Pressurized Gasifiers Massachusetts Institute of Technology Project Number: FE0012500 Project Description This project will develop and assess a slurry feeding system based on a suspension of coal in liquid CO2 that can be pumped into a high-pressure gasifier. The advantages of this solution are that CO2 has a low heat capacity, a low heat of vaporization and low viscosity. Thus, the liquid CO2 imposes a much smaller thermal load on the gasifier relative to a water slurry, and has the potential to improve the efficiency and economics of integrated gasification combined cycle (IGCC) power plants with carbon capture and dramatically reduce greenhouse gas emissions from coal fired power plants. Project Details

437

The Role of CO2 Reduction Catalysis in Carbon Capture  

Science Journals Connector (OSTI)

In addition to the algae-mediated process discussed in Chap.7, to generate hydrocarbon-based fuels and useful chemicals from CO2, it is also possible to use electrochemical and photocatalytic processes to carry ...

Prof. Jennifer Wilcox

2012-01-01T23:59:59.000Z

438

Carbon Capture and a Commercial Market for CO2  

Science Journals Connector (OSTI)

With increasing evidence that the earth is warming at a faster rate than previously expected, there is pressure to reduce carbon dioxide (CO2) emissions on a large scale. Because carbon capture helps to internali...

Thomas R. Sadler

2013-05-01T23:59:59.000Z

439

electroseismic monitoring of co2 sequestration: a finite element ...  

E-Print Network [OSTI]

The injection of large amounts of man-produced CO2 in depleted oil wells below ..... [7] SANTOS, J. E., Global and domain-decomposed mixed methods for the...

Fabio Zyserman

440

co2-use-reuse | netl.doe.gov  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

under certain conditions that do not necessarily require intensive energy input. Using CO2 as a feedstock for a variety of products is a promising research area, particularly in...

Note: This page contains sample records for the topic "atmospheric co2 concentrations" from the National Library of EnergyBeta (NLEBeta).
While these samples are representative of the content of NLEBeta,
they are not comprehensive nor are they the most current set.
We encourage you to perform a real-time search of NLEBeta
to obtain the most current and comprehensive results.


441

Split system CO2 heat pump water heaters  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Split-system-CO2-heat-pump-water-heaters- Sign In About | Careers | Contact | Investors | bpa.gov Search Policy & Reporting Expand Policy & Reporting EE Sectors Expand EE...

442

Novel CO2-Thickeners for Improved Mobility Control  

SciTech Connect (OSTI)

The objective of this contract was to design, synthesize, and characterize thickening agents for dense carbon dioxide and to evaluate their solubility and viscosity-enhancing potential in CO2.

Enick, Dr. Robert M.; Beckman, Dr. Eric J.; Hamilton, Dr. Andrew

2002-01-15T23:59:59.000Z

443

Hierarchically Porous Aminosilica Monolith as a CO2 Adsorbent  

Science Journals Connector (OSTI)

Danon, A.; Stair, P. C.; Weitz, E.FTIR Study of CO2 Adsorption on Amine-Grafted SBA-15: Elucidation of Adsorbed Species J. Phys. ... Danon, Alon; Stair, Peter C.; Weitz, Eric ...

Young Gun Ko; Hyun Jeong Lee; Jae Yong Kim; Ung Su Choi

2014-07-07T23:59:59.000Z

444

From CO2 to Methanol via Novel Nanocatalysts  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

have found novel nanocatalysts that lower the barrier to converting carbon dioxide (CO2)-an abundant greenhouse gas-into methanol (CH3OH)-a key commodity used to produce...

445

Magnetic behaviour of synthetic Co2SiO4  

Science Journals Connector (OSTI)

The magnetic structure of the synthetic cobalt olivine, Co2SiO4, is determined by means of non-polarized and polarized neutron diffraction on single-crystal and powder samples.

Sazonov, A.

2009-11-16T23:59:59.000Z

446

Synthetic fuel concept to steal CO2 from air  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

to steal CO2 from air Lab has developed a low-risk, transformational concept, called Green Freedom(tm), for large-scale production of carbon-neutral, sulfur-free fuels and...

447

LED-based CO2 Sensor for Balloon Deployment  

Science Journals Connector (OSTI)

We are developing a sensor for monitoring ambient CO2 from unmanned aircraft and balloons. The sensor consists of a mid-IR LED coupled with a high dynamic range gated integrator. The...

Sonnenfroh, David; Parameswaran, Krishnan

448

Electron drift velocity in CO2 laser mixtures  

Science Journals Connector (OSTI)

A modified Bradbury-Nielsen grid system has been used to measure...W in two gas mixtures of special interest when modelling h.p. CO2 lasers. The results are compared with the theoretical values obtained with the ...

G. L. Braglia; L. Roman; W. Roznerski

449

Improving CO2 Efficiency for Recovering Oil in Heterogeneous Reservoirs  

SciTech Connect (OSTI)

The work strived to improve industry understanding of CO2 flooding mechanisms with the ultimate goal of economically recovering more of the U.S. oil reserves. The principle interests are in the related fields of mobility control and injectivity.

Grigg, Reid B.; Svec, Robert K.

2003-03-10T23:59:59.000Z

450

International Symposium on Site Characterization for CO2 Geological Storage  

E-Print Network [OSTI]

FEASIBILITY: TEAPOT DOME EOR PILOT L. Chiaramonte, M.TO IDENTIFY OPTIMAL CO 2 EOR STORAGE SITES V. Nez Lopez,from a carbon dioxide EOR/sequestration project. Energy

Tsang, Chin-Fu

2006-01-01T23:59:59.000Z

451

Near Miscible CO2 Application to Improve Oil Recovery  

E-Print Network [OSTI]

...................................................................................................................... XIV 1 INTRODUCTION AND LITERATURE REVIEW ....................................................................... 1 1.1 THE BASICS OF CO2 EOR... ....................................................................................................................................... 104 APPENDICES ....................................................................................................................................... 107 vii LIST OF FIGURES FIGURE 1-1 GAS INJECTION EOR IN U.S [1...

Bui, Ly H.

2010-07-26T23:59:59.000Z

452

Carbon Dioxide Flux Measurement Systems (CO2Flux) Handbook  

SciTech Connect (OSTI)

The Southern Great Plains (SGP) carbon dioxide flux (CO2 flux) measurement systems provide half-hour average fluxes of CO2, H2O (latent heat), and sensible heat. The fluxes are obtained by the eddy covariance technique, which computes the flux as the mean product of the vertical wind component with CO2 and H2O densities, or estimated virtual temperature. A three-dimensional sonic anemometer is used to obtain the orthogonal wind components and the virtual (sonic) temperature. An infrared gas analyzer is used to obtain the CO2 and H2O densities. A separate sub-system also collects half-hour average measures of meteorological and soil variables from separate 4-m towers.

Fischer, M

2005-01-01T23:59:59.000Z

453

Biominetic Membrane for Co2 Capture from Flue Gas  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Biomimetic Membrane for CO Biomimetic Membrane for CO 2 Capture from Flue Gas Background Carbon Capture and Sequestration (CCS) is a three-step process including capture, pipeline transport, and geologic storage of which the capture of carbon dioxide (CO 2 ) is the most costly and technically challenging. Current available methods impose significant energy burdens that severely impact their overall effectiveness as a significant deployment option. Of the available capture technologies for post

454

Dehydrated Prussian Blues for CO2 Storage and Separation Applications  

SciTech Connect (OSTI)

Adsorption isotherms of pure gases present in flue and natural gas including CO2, N2, CH4 and water were studied using prussian blues of chemical formula M3[Co(CN)6]2 (M = Cu, Ni, Mn). These materials adsorbed 8-12 wt % of CO2 at room temperature and 1 bar of pressure with heats of adsorption ranging from 6 to 16 kcal/mol.

Motkuri, Radha K.; Thallapally, Praveen K.; McGrail, B. Peter; Ghorishi, Behrooz S.

2010-08-13T23:59:59.000Z

455

Developing a Mechanistic Understanding of Lamellar Hydroxide Mineral Carbonation Reaction Processes to Reduce CO2 Mineral Sequestration Process Cost  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Mechanistic Understanding of Lamellar Hydroxide Mechanistic Understanding of Lamellar Hydroxide Mineral Carbonation Reaction Processes to Reduce CO 2 Mineral Sequestration Process Cost Michael J. McKelvy (mckelvy@asu.edu; 480-965-4535), Andrew V. G. Chizmeshya (chizmesh@asu.edu; 480-965-6072), Hamdallah Bearat (Hamdallah.Bearat@asu.edu; 480-965-2624), Renu Sharma (Renu.Sharma@asu.edu; 480-965-4541), and Ray W. Carpenter (carpenter@asu.edu; 480-965-4549) Center for Solid State Science and Science and Engineering of Materials PhD Program, P.O. Box 871704, Arizona State University, Tempe, Arizona 85287 USA ABSTRACT The potential environmental effects of increasing atmospheric CO 2 levels are of major worldwide concern. One alternative for managing CO 2 emissions is carbon sequestration: the capture and secure confinement of CO

456

Tropical forest responses to increasing [CO2]: current knowledge and opportunities for future research  

SciTech Connect (OSTI)

Elevated atmospheric [CO2] (ca) will undoubtedly affect the metabolism of tropical forests worldwide; however, critical aspects of how tropical forests will respond remain largely unknown. Here we review the current state of knowledge about physiological and ecological responses, with the aim of providing a framework that can help to guide future experimental research. Modelling studies have indicated that elevated ca can potentially stimulate photosynthesis more in the tropics than at higher latitudes, because suppression of photorespiration by elevated ca increases with temperature. However, canopy leaves in tropical forests could also potentially reach a high temperature threshold under elevated ca that will moderate the rise in photosynthesis. Belowground responses, including fine root production, nutrient foraging, and soil organic matter processing, will be especially important to the integrated ecosystem response to elevated CO2. Water-use efficiency will increase as ca rises, potentially impacting upon soil moisture status and nutrient availability. Recruitment may be differentially altered for some functional groups, potentially decreasing ecosystem carbon storage. Whole-forest CO2 enrichment experiments are urgently needed to test predictions of tropical forest functioning under elevated ca. Smaller scale experiments in the understory and in gaps would also be informative, and could provide stepping stones toward stand-scale manipulations.

Cernusak, Lucas [Australian National University, Canberra, Australia; Winter, Klaus [Smithsonian Tropical Research Institute; Dalling, James [University of Illinois, Urbana-Champaign; Holtum, Joseph [James Cook University; Jaramillo, Carlos [Smithsonian Tropical Research Institute; Korner, Christian [University of Basel; Leakey, Andrew D.B. [University of Illinois; Norby, Richard J [ORNL; Poulter, Benjamin [Laboratoire des Sciences du Climat et de l'Environement, France; Turner, Benjamin [Smithsonian Tropical Research Institute; Wright, S. Joseph [Smithsonian Tropical Research Institute

2013-01-01T23:59:59.000Z

457

Generation of a Doubly Bridging CO2 Ligand and Deoxygenation of CO2 by an (NHC)Ni(0) Complex  

E-Print Network [OSTI]

for CO2, µ-2,2-CO2, at a dinickel core. The reaction of [(IPr)Ni(µ-Cl)]2 18 (IPr ) 1,3-bis(2,6-diisopro, (IPr)- Ni(6-C6D6). We note that this symmetric pattern for the backbone protons is observed in reacted isolation of the product as a solid. Reaction of [(IPr)Ni(µ-Cl)]2 with Li(HBEt3) or with NaOt-Bu followed

Müller, Peter

458

ENHANCED PRACTICAL PHOTOSYNTHETIC CO2 MITIGATION  

SciTech Connect (OSTI)

This report documents significant achievements in the Enhanced Practical Photosynthetic CO{sub 2} Mitigation project during the period from 10/2/2001 through 10/01/2002. This report marks the end of year 2 of a three-year project as well as the milestone date for completion of Phase I activities. This report includes our current status and defines the steps being taken to ensure that we meet the project goals by the end of year 3. As indicated in the list of accomplishments below our current efforts are focused on evaluating candidate organisms and growth surfaces, preparing to conduct long-term tests in the bench-scale bioreactor test systems, and scaling-up the test facilities from bench scale to pilot scale. Specific results and accomplishments for the third quarter of 2002 include: Organisms and Growth Surfaces: (1) Test results continue to indicate that thermophilic cyanobacteria have significant advantages as agents for practical photosynthetic CO{sub 2} mitigation before mesophilic forms. (2) Additional thermal features with developed cyanobacterial mats, which might be calcium resistant, were found in YNP. (3) Back to back tests show that there is no detectable difference in the growth of isolate 1.2 s.c. (2) in standard and Ca-modified BG-11 medium. The doubling time for both cases was about 12 hours. (4) The cultivation of cyanobacteria in Ca-BG medium should proceed in the pH range between 7 and 7.4, but this suggestion requires additional experiments. (5) Cyanobacteria can be grown in media where sodium is present at trace levels. (6) Ca{sup 2+} enriched medium can be used as a sink for CO{sub 2} under alkaline conditions. (7) Cyanobacteria are able to generate cones of filaments on travertine surfaces. [Travertine is a mixture of CaCO{sub 3} and CaSO{sub 4}]. We hypothesize that SO{sub 4}{sup 2-} stimulates the generation of such cones, because they are not almost generated on CaCO3 surface. On the other hand, we know that plant gas contains elevated concentrations of SO{sub 4}{sup 2-}. We may speculate that the introduction of 11.2 isolate in CRF might significantly increase the productivity of such facility. It is possible that a higher colonization potential for the screens may allow a higher surface productivity than some of the other isolates. (8) The colonization of Omnisil surface is an auto-inducible and time-requiring process. (9) Omnisil coupons should be treated under pH control, preferably using KOH. Bioreactor support systems and test facilities: (1) The pilot-scale bioreactor construction and debugging is continuing on schedule. Tests of the ''natural'' lighting system have shown acceptable levels of illumination for the bioreactor screens using only collected sunlight. (2) Flow control inserts have been designed for the CRF-2 screens, which require header pipes for flow distribution and control. A staggered drilled-hole design and a thick shim design have both shown acceptable performance results (little to no clogging, uniform flow, ability to load algae on to the screen). They will both be tested in the CRF-2 to see which performs the best over long durations, and the best performing design will be used for the pilot scale bioreactor screens.

Dr. Gregory Kremer; Dr. David J. Bayless; Dr. Morgan Vis; Dr. Michael Prudich; Dr. Keith Cooksey; Dr. Jeff Muhs

2002-10-15T23:59:59.000Z

459

NETL: Bench-Scale Development of a Hybrid Membrane-Absorption CO2 Capture  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Bench-Scale Development of a Hybrid Membrane-Absorption CO2 Capture Process Bench-Scale Development of a Hybrid Membrane-Absorption CO2 Capture Process Project No.: DE-FE0013118 Membrane Technology and Research (MTR) is developing and evaluating a hybrid membrane-absorption CO2 capture system. This work builds on prior DOE-funded work and combines MTR's Polaris(tm) membrane, in a low-pressure-drop, large area, plate-and-frame module, with UT Austin's piperazine (PZ) solvent and advanced, high-temperature and pressure regeneration technology. Preliminary estimates indicate that this hybrid system could lower the regeneration energy by 30 percent compared to that required with 30 weight percent monoethanolamine (MEA). MTR is evaluating two variations of the hybrid design consisting of the cross-flow Polaris membrane, which enriches flue gas to approximately 20 percent CO2, and an advanced 5 molal PZ advanced flash stripper with cold-rich bypass. The flash stripper will be optimized to take advantage of the higher CO2 concentration. In the first variation, the two systems are operated in series; in the second, the flue gas flow is split and treated by each system in parallel. The first phase of this project will include an examination of both hybrid configurations, using an integrated process model and a preliminary techno-economic assessment. In the second phase, MTR will manufacture and test a low pressure drop, large-area membrane module and UT Austin will modify their 0.1 MWe pilot plant and operate it under simulated series and parallel configurations. Based on the model and test results, the most promising configuration will be identified. In the final stage of the project, the membrane module will be integrated into the pilot plant where the fully integrated hybrid system, in its most promising cost optimized configuration, will be tested on simulated flue gas.

460

Microsoft Word - SECARB Phase III CO2 sequestration Final EA...  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

Greenhouse gases (GHG) are components of the atmosphere that contribute to the greenhouse effect and climate change. Some greenhouse gases occur naturally in the atmosphere,...

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461

A Comparative Economical Analysis of Technologies for CO2 Removal from Offshore Natural Gas  

Science Journals Connector (OSTI)

Abstract In the scenario of the Brazilian Pre-Salt fields, where associated Natural Gas (NG) shows high concentration of CO2, gas conditioning comes out as one of the main challenges. Among the possible capture technologies available, three alternatives stand out for CO2 sequestration: (A) gas permeation through membranes, (B) absorption columns using aqueous blends of ethanolamines and (C) application of hybrid - membrane modules in series with amine absorption and regeneration columns. The main objective of this work is to investigate the technical and economical feasibility of applying these three separation processes on offshore platforms, given the stringent constraints on footprint and equipment weight, and for minimizing NG production and transportation costs. The methodology involves: (i) development of cases based on the Brazilian Pre-Salt gas composition. NG streams with CO2 molar concentrations ranging from 8 to 18% are applied; (ii) Simulations of three process flowsheets, corresponding to each one of chosen technologies - A, B and C; (iii) Equipment sizing; and (iv) Analysis of economic performance through calculation of capital (CAPEX) and operational (OPEX) costs.

Tatiana S. Gadelha; Aline R.S. Guimares; Andressa Nakao; Oflia de Q.F. Arajo; Jos Luiz de Medeiros

2012-01-01T23:59:59.000Z

462

Annual Fossil-Fuel CO2 Emissions: Global Stable Carbon Isotopic Signature  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

2 2 data Data image Documentation Contributors R.J. Andres, T.A. Boden, and G. Marland The 2012 revision of this database contains estimates of the annual, global mean value of δ 13C of CO2 emissions from fossil-fuel consumption and cement manufacture for 1751-2009. These estimates of the carbon isotopic signature account for the changing mix of coal, petroleum, and natural gas being consumed and for the changing mix of petroleum from various producing areas with characteristic isotopic signatures. This time series of global fossil-fuel del 13C signature provides an additional constraint for balancing the sources and sinks of the global carbon cycle and complements the atmospheric δ 13C measurements that are used to partition the uptake of fossil carbon emissions among the ocean, atmosphere, and terrestrial

463

Annual Fossil-Fuel CO2 Emissions: Global Stable Carbon Isotopic Signature  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

3 3 data Data image Documentation Contributors R.J. Andres, T.A. Boden, and G. Marland The 2013 revision of this database contains estimates of the annual, global mean value of δ 13C of CO2 emissions from fossil-fuel consumption and cement manufacture for 1751-2010. These estimates of the carbon isotopic signature account for the changing mix of coal, petroleum, and natural gas being consumed and for the changing mix of petroleum from various producing areas with characteristic isotopic signatures. This time series of global fossil-fuel del 13C signature provides an additional constraint for balancing the sources and sinks of the global carbon cycle and complements the atmospheric δ 13C measurements that are used to partition the uptake of fossil carbon emissions among the ocean, atmosphere, and terrestrial

464

Annual Fossil-Fuel CO2 Emissions: Global Stable Carbon Isotopic Signature  

Broader source: All U.S. Department of Energy (DOE) Office Webpages (Extended Search)

1 1 data Data image Documentation Contributors R.J. Andres, T.A. Boden, and G. Marland The 2011 revision of this database contains estimates of the annual, global mean value of del 13C of CO2 emissions from fossil-fuel consumption and cement manufacture for 1751-2008. These estimates of the carbon isotopic signature account for the changing mix of coal, petroleum, and natural gas being consumed and for the changing mix of petroleum from various producing areas with characteristic isotopic signatures. This time series of global fossil-fuel del 13C signature provides an additional constraint for balancing the sources and sinks of the global carbon cycle and complements the atmospheric del 13C measurements that are used to partition the uptake of fossil carbon emissions among the ocean