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Excited-state reversible geminate recombination with quenching in one dimension

Summary: Excited-state reversible geminate recombination with quenching
in one dimension
Hyojoon Kim and Kook Joe Shina)
Department of Chemistry and Center for Molecular Catalysis, Seoul National University, Seoul 151-742,
Noam Agmonb)
The Fritz Haber Research Center, Department of Physical Chemistry, The Hebrew University,
Jerusalem 91904, Israel
Received 5 April 1999; accepted 3 June 1999
We obtain the exact Green function for excited-state geminate reversible dissociation with two
different lifetimes and quenching in one dimension, in the absence of a potential of interaction. We
consider the ground-state and irreversible reactions as special limits, and investigate the long time
asymptotic behavior in comparison with that observed in three dimensions. 1999 American
Institute of Physics. S0021-9606 99 50633-8
Reversible diffusion-influenced reactions attract increas-
ing attention. Recently, an interesting transition has been dis-
covered in the approximate long time asymptotic solution for
geminate excited-state reversible recombination with two
different lifetimes,1,2


Source: Agmon, Noam - Institute of Chemistry, Hebrew University of Jerusalem


Collections: Chemistry