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Summary: An implementation of the DeutschJozsa algorithm
on molecular vibronic coherences through four-wave mixing:
a theoretical study
Zsolt Bihary a
, David R. Glenn b
, Daniel A. Lidar c,*,1
, V. Ara Apkarian a
a
Department of Chemistry, University of California, Irvine, CA 92697, USA
b
Physics Department, University of Toronto, 60 St. George Street, Toronto, Ont., Canada M5S 3H6
c
Chemical Physics Theory Group, University of Toronto, 80 St. George Street, Toronto, Ont., Canada M5S 3H6
Received 12 February 2002; in final form 2 May 2002
Abstract
Time-frequency resolved coherent anti-Stokes Raman scattering (TFRCARS) was recently proposed as a means to
implement quantum logic using the molecular ro-vibrational manifold as a quantum register [R. Zadoyan et al., Chem.
Phys. 266 (2001) 323]. We give a concrete example of how this can be accomplished through an illustrative algorithm
that solves the DeutschJozsa (DJ) problem. We use realistic molecular parameters to recognize that, as the problem
size expands, shaped pulses must be tailored to maintain fidelity of the algorithm. Ó 2002 Published by Elsevier
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