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Summary: Time-resolved CARS studies of vibrational
coherences in the condensed phase:
I2 in solid krypton
Michael Karavitis1
, Ilya Goldschleger1
, V. Ara Apkarian1
, and Takayuki Kumada2
1
Department of Chemistry, University of California, Irvine, CA 92697-2025, USA
E-mail: aapkaria@uci.edu
2
Advanced Science Research Center, Japan Atomic Energy Research Institute, Tokai,
Ibaraki 319-1195, Japan
E-mail: kumada@popsvr.tokai.jaeri.go.jp
Abstract. Vibrational dephasing in the prototypical system of I2 isolated in solid Kr is
studied using TRCARS. Decay |0>
temperature (T = 6 45 K), are extracted and analyzed.
1. Introduction
Time-resolved, electronically resonant, parametric four-wave mixing processes
allow detailed preparation, manipulation, and interrogation of molecular ro-
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