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110 ' ACCOUNTS OF CHEMICAL RESEARCH ' 110119 ' 2012 ' Vol. 45, No. 1 Published on the Web 11/08/2011 www.pubs.acs.org/accounts 10.1021/ar200152v & 2011 American Chemical Society
 

Summary: 110 ' ACCOUNTS OF CHEMICAL RESEARCH ' 110119 ' 2012 ' Vol. 45, No. 1 Published on the Web 11/08/2011 www.pubs.acs.org/accounts
10.1021/ar200152v & 2011 American Chemical Society
Organization of Water and Atmospherically
Relevant Ions and Solutes: Vibrational Sum
Frequency Spectroscopy at the Vapor/Liquid and
Liquid/Solid Interfaces
AARON M. JUBB, WEI HUA, AND HEATHER C. ALLEN*
Department of Chemistry, The Ohio State University, 100 West 18th Avenue,
Columbus, Ohio 43210, United States
RECEIVED ON JUNE 7, 2011
C O N S P E C T U S
T he nature of water's hydrogen-bonding network is a vital in
fluence on the chemistry that occurs at interfaces, but a
complete understanding of interfacial water has proven elusive.
Even-order nonlinear opticalspectroscopies,such asvibrational sum
frequency generation (VSFG) spectroscopy and heterodyne detected
phase-sensitive sum frequency generation (PS-SFG) spectroscopy,
are inherently surface specific. With the advent of advances in these
spectroscopic techniques, researchers can now explore many long-
standing questions about the dynamics and structures present at the

  

Source: Allen, Heather C.- Department of Chemistry, Ohio State University

 

Collections: Chemistry