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Exact solution for the geminate ABCD reaction Alexander V. Popova)
 

Summary: Exact solution for the geminate ABCD reaction
Alexander V. Popova)
and Noam Agmonb)
Department of Physical Chemistry and the Fritz Haber Research Center, The Hebrew University,
Jerusalem 91904, Israel
Received 13 May 2002; accepted 25 June 2002
We obtain exact analytic solution for the Green functions and survival probabilities of the reversible,
geminate diffusion-influenced reaction A BC D in Laplace space, and in the time domain for
various spatial dimensionalities. The asymptotic behavior in one and three dimensions goes as
t 1/2
, like in the irreversible case, but approach to this limit may occur from either above or below.
The implications of these results are demonstrated and discussed. й 2002 American Institute of
Physics. DOI: 10.1063/1.1501127
I. INTRODUCTION
Recently there has been intensive activity regarding the
many-particle effect on the transfer reactions,1н12
A B
k2
k1
C D,

  

Source: Agmon, Noam - Institute of Chemistry, Hebrew University of Jerusalem

 

Collections: Chemistry