Succinic anhydrides from epoxides

Coates, Geoffrey W.; Rowley, John M.

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Title: Succinic anhydrides from epoxides

Abstract

Catalysts and methods for the double carbonylation of epoxides are disclosed. Each epoxide molecule reacts with two molecules of carbon monoxide to produce a succinic anhydride. The reaction is facilitated by catalysts combining a Lewis acidic species with a transition metal carbonyl complex. The double carbonylation is achieved in single process by using reaction conditions under which both carbonylation reactions occur without the necessity of isolating or purifying the product of the first carbonylation.

Inventors:: Coates, Geoffrey W.; Rowley, John M.

Issue Date:: Tue Jul 09 00:00:00 EDT 2013

Research Org.:: DOESC (USDOE Office of Science (SC) (United States))

Sponsoring Org.:: USDOE

OSTI Identifier:: 1087883

Patent Number(s):: 8481756

Application Number:: 12/204,411

Assignee:: Cornell Research Foundation, Inc. (Ithaca, NY)

Patent Classifications (CPCs):: C - CHEMISTRY C07 - ORGANIC CHEMISTRY C07D - HETEROCYCLIC COMPOUNDS

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C - CHEMISTRY C07 - ORGANIC CHEMISTRY C07D - HETEROCYCLIC COMPOUNDS
C07D307/60 - Two oxygen atoms, e.g. succinic anhydride

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DOE Contract Number:: FG02-05ER15687

Resource Type:: Patent

Country of Publication:: United States

Language:: English

Subject:: 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY

Citation Formats


                    Coates, Geoffrey W., and Rowley, John M. Succinic anhydrides from epoxides.  United States: N. p., 2013. 
        Web.

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                    Coates, Geoffrey W., & Rowley, John M. Succinic anhydrides from epoxides.  United States.

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                    Coates, Geoffrey W., and Rowley, John M. Tue .  
        "Succinic anhydrides from epoxides".  United States.  https://www.osti.gov/servlets/purl/1087883.

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@article{osti_1087883,

  title        = {Succinic anhydrides from epoxides},

  author       = {Coates, Geoffrey W. and Rowley, John M.},

  abstractNote = {Catalysts and methods for the double carbonylation of epoxides are disclosed. Each epoxide molecule reacts with two molecules of carbon monoxide to produce a succinic anhydride. The reaction is facilitated by catalysts combining a Lewis acidic species with a transition metal carbonyl complex. The double carbonylation is achieved in single process by using reaction conditions under which both carbonylation reactions occur without the necessity of isolating or purifying the product of the first carbonylation.},

  doi          = {},

  journal      = {},
number       = ,

  volume       = ,

  place        = {United States},

  year         = {Tue Jul 09 00:00:00 EDT 2013},

  month        = {Tue Jul 09 00:00:00 EDT 2013}

}

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Works referenced in this record:

Catalytic Carbonylation of β-Lactones to Succinic Anhydrides
journal, June 2004

Getzler, Yutan D. Y. L.; Kundnani, Vinod; Lobkovsky, Emil B.
Journal of the American Chemical Society, Vol. 126, Issue 22, p. 6842-6843
https://doi.org/10.1021/ja048946m

Low pressure carbonylation of heterocycles
patent, August 2009

Coates, Geoffrey W.; Kramer, John W.
US Patent Document 7,569,709
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7569709

Polycarbonates made using highly selective catalysts
patent-application, May 2008

Coates, Geoffrey W.; Qin, Zengquan; Cohen, Claire Tova
US Patent Application 11/976800; 20080108499
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20080108499

Catalytic carbonylation of three and four membered heterocycles
patent, February 2005

Coates, Geoffrey W.; Getzler, Yutan D. Y. L.; Wolczanski, Peter
US Patent Document 6,852,865
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6852865

Low Pressure Carbonylation of Heterocycles
patent-application, November 2009

Coates, Geoffrey W.; Kramer, John
US Patent Application 12/486158; 20090287000
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20090287000

Catalytic Double Carbonylation of Epoxides to Succinic Anhydrides: Catalyst Discovery, Reaction Scope, and Mechanism
journal, April 2007

Rowley, John M.; Lobkovsky, Emil B.; Coates, Geoffrey W.
Journal of the American Chemical Society, Vol. 129, Issue 16, p. 4948-4960
https://doi.org/10.1021/ja066901a

Low pressure carbonylation of heterocycles
patent-application, September 2007

Coates, Geoffrey W.; Kramer, John
US Patent Application 11/705528; 20070213524
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20070213524

Polycarbonates made using high activity catalysts
patent, October 2000

Coates, Geoffrey W.; Cheng, Ming
US Patent Document 6,133,402
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6133402

Polycarbonates made using highly selective catalysts
patent-application, November 2007

Coates, Geoffrey W.; Qin, Zengquan; Cohen, Claire Tova
US Patent Application 11/812106; 20070255039
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20070255039

Catalytic carbonylation of three and four membered heterocycles
patent-application, August 2003

Coates, Geoffrey W.; Getzler, Yutan D. Y. L.; Wolczanski, Peter
US Patent Application 10/307520; 20030162961
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20030162961

Polycarbonates made using highly selective catalysts
patent-application, April 2006

Coates, Geoffrey; Qin, Zengquan; Cohen, Claire
US Patent Application 11/244231; 20060089252
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20060089252

Polycarbonates made using highly selective catalysts
patent, December 2007

Coates, Geoffrey W.; Qin, Zengquan; Cohen, Claire
US Patent Document 7,304,172
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7304172

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Succinic anhydrides from epoxides

Patent Coates, Geoffrey W.; Rowley, John M.

Catalysts and methods for the double carbonylation of epoxides are disclosed. Each epoxide molecule reacts with two molecules of carbon monoxide to produce a succinic anhydride. The reaction is facilitated by catalysts combining a Lewis acidic species with a transition metal carbonyl complex. The double carbonylation is achieved in single process by using reaction conditions under which both carbonylation reactions occur without the necessity of isolating or purifying the product of the first carbonylation.
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Succinic anhydrides from epoxides

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Catalysts and methods for the double carbonylation of epoxides are disclosed. Each epoxide molecule reacts with two molecules of carbon monoxide to produce a succinic anhydride. The reaction is facilitated by catalysts combining a Lewis acidic species with a transition metal carbonyl complex. The double carbonylation is achieved in single process by using reaction conditions under which both carbonylation reactions occur without the necessity of isolating or purifying the product of the first carbonylation.
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Method to produce succinic acid from raw hydrolysates

Patent Donnelly, Mark I.; Sanville-Millard, Cynthia Y.; Nghiem, Nhuan Phu

A method for producing succinic acid from industrial-grade hydrolysates is provided, comprising supplying an organism that contains mutations for the genes ptsG, pflB, and ldhA, allowing said organism to accumulate biomass, and allowing said organism to metabolize the hydrolysate. Also provided is a bacteria mutant characterized in that it produces succinic acid from substrate contained in industrial-grade hydrolysate in a ratio of between 0.6:1 and 1.3:1 succinic acid to substrate.
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Similar Records

Title: Succinic anhydrides from epoxides

Abstract

Citation Formats

Catalytic Carbonylation of β-Lactones to Succinic Anhydrides journal, June 2004

Low pressure carbonylation of heterocycles patent, August 2009

Polycarbonates made using highly selective catalysts patent-application, May 2008

Catalytic carbonylation of three and four membered heterocycles patent, February 2005

Low Pressure Carbonylation of Heterocycles patent-application, November 2009

Catalytic Double Carbonylation of Epoxides to Succinic Anhydrides: Catalyst Discovery, Reaction Scope, and Mechanism journal, April 2007

Low pressure carbonylation of heterocycles patent-application, September 2007

Polycarbonates made using high activity catalysts patent, October 2000

Polycarbonates made using highly selective catalysts patent-application, November 2007

Catalytic carbonylation of three and four membered heterocycles patent-application, August 2003

Polycarbonates made using highly selective catalysts patent-application, April 2006

Polycarbonates made using highly selective catalysts patent, December 2007

Catalytic Carbonylation of β-Lactones to Succinic Anhydrides
journal, June 2004

Low pressure carbonylation of heterocycles
patent, August 2009

Polycarbonates made using highly selective catalysts
patent-application, May 2008

Catalytic carbonylation of three and four membered heterocycles
patent, February 2005

Low Pressure Carbonylation of Heterocycles
patent-application, November 2009

Catalytic Double Carbonylation of Epoxides to Succinic Anhydrides: Catalyst Discovery, Reaction Scope, and Mechanism
journal, April 2007

Low pressure carbonylation of heterocycles
patent-application, September 2007

Polycarbonates made using high activity catalysts
patent, October 2000

Polycarbonates made using highly selective catalysts
patent-application, November 2007

Catalytic carbonylation of three and four membered heterocycles
patent-application, August 2003

Polycarbonates made using highly selective catalysts
patent-application, April 2006

Polycarbonates made using highly selective catalysts
patent, December 2007