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Title: Recent palladium membrane reactor development at the tritium systems test assembly

Conference ·
OSTI ID:97343

The palladium membrane reactor (PMR) is proving to be a simple and effective means for recovering hydrogen isotopes from fusion fuel impurities such as methane and water. This device directly combines two techniques which have long been utilized for hydrogen processing, namely catalytic shift reactions and palladium/silver permeators. A proof-of-principle (PMR) has been constructed and tested at the Tritium Systems Test Assembly of Los Alamos National Laboratory. The first tests with this device showed that is was effective for the proposed purpose. Initial work concluded that a nickel catalyst was an appropriate choice for use in a PMR. More detailed testing of the PMR with such a catalyst was performed and reported in other works. It was shown that a nickel catalyst-packed PMR did, indeed, recover hydrogen from water and methane with efficiencies approaching 100% in a single processing pass. These experiments were conducted over an extended period of time and no failure or need for regeneration was encountered. These positive results have prompted further PMR development. Topics addressed include alternate PMR geometries and initial testing of the PMR with tritium. These are the subjects of this paper.

Research Organization:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Organization:
USDOE, Washington, DC (United States)
DOE Contract Number:
W-7405-ENG-36
OSTI ID:
97343
Report Number(s):
LA-UR-95-1472; CONF-950506-15; ON: DE95014009; TRN: 95:019212
Resource Relation:
Conference: 5. topical meeting on tritium technology in fission, fusion and isotopic applications, Ispra (Italy), 28 May - 3 Jun 1995; Other Information: PBD: [1995]
Country of Publication:
United States
Language:
English